FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Datye, A Li, L Zhang, W Wei, YJ Gao, YF Pharr, GM AF Datye, Amit Li, Lin Zhang, Wei Wei, Yujie Gao, Yanfei Pharr, George M. TI Extraction of Anisotropic Mechanical Properties From Nanoindentation of SiC-6H Single Crystals SO JOURNAL OF APPLIED MECHANICS-TRANSACTIONS OF THE ASME LA English DT Article DE nanoindentation; elastic and plastic anisotropy; basal slip ID SMALL STRESSED VOLUMES; SILICON-CARBIDE; INDENTATION; DEFORMATION; ORIENTATION; SLIP; PLASTICITY; MAGNESIUM; MG; BEHAVIOR AB Because brittle solids fail catastrophically during normal tension and compression testing, nanoindentation is often a useful alternative technique for measuring their mechanical properties and assessing their deformation characteristics. One practical question to be addressed in such studies is the relationship between the anisotropy in the uniaxial mechanical behavior to that in the indentation response. To this end, a systematic study of the mechanical behavior the 6H polytype of a hexagonal silicon carbide single crystal (SiC-6H) was performed using standard nanoindentation methods. The indentation elastic modulus and hardness measured using a Berkovich indenter at a peak load of 500 mN varied over a wide range of crystal orientation by only a few percent. The variation in modulus is shown to be consistent with an anisotropic elastic contact analysis based on the known single crystal elastic constants of the material. The variation in hardness is examined using a single crystal plasticity model that considers the anisotropy of slip in hexagonal crystals. When compared to experimental measurements, the analysis confirms that plasticity in SiC-6H is dominated by basal slip. An anisotropic elastic contact analysis provides insights into the relationship between the pop-in load, which characterizes the transition from elasticity to plasticity during nanoindentation testing, and the theoretical strength of the material. The observations and analyses lay the foundations for further examination of the deformation and failure mechanisms in anisotropic materials by nanoindentation techniques. C1 [Datye, Amit; Li, Lin; Zhang, Wei; Gao, Yanfei; Pharr, George M.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Wei, Yujie] Chinese Acad Sci, Inst Mech, LNM, Beijing 100190, Peoples R China. [Gao, Yanfei; Pharr, George M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Gao, YF; Pharr, GM (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.; Gao, YF; Pharr, GM (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM pharr@utk.edu RI Gao, Yanfei/F-9034-2010; Wei, Yujie/A-3770-2009 OI Gao, Yanfei/0000-0003-2082-857X; Wei, Yujie/0000-0002-3213-7891 FU U.S. National Science Foundation [CMMI 0926798, DMR 1427812]; Natural Science Foundation of China [11425211] FX This research was supported by the U.S. National Science Foundation CMMI 0926798 (AD, LL, YFG) and DMR 1427812 (GMP), and the Natural Science Foundation of China 11425211 (YJW). Y.F.G. and G.M.P. are grateful to Dr. A.A. Wereszczak for his critical review of the manuscript. NR 32 TC 1 Z9 1 U1 10 U2 15 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0021-8936 EI 1528-9036 J9 J APPL MECH-T ASME JI J. Appl. Mech.-Trans. ASME PD SEP PY 2016 VL 83 IS 9 AR 091003 DI 10.1115/1.4033790 PG 7 WC Mechanics SC Mechanics GA DV2KS UT WOS:000382750000003 ER PT J AU DuPont, B Azam, R Proper, S Cotilla-Sanchez, E Hoyle, C Piacenza, J Oryshchyn, D Zitney, SE Bossart, S AF DuPont, Bryony Azam, Ridwan Proper, Scott Cotilla-Sanchez, Eduardo Hoyle, Christopher Piacenza, Joseph Oryshchyn, Danylo Zitney, Stephen E. Bossart, Stephen TI An Optimization Framework for Decision Making in Large, Collaborative Energy Supply Systems SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID POWER-SYSTEMS AB As demand for electricity in the U.S. continues to increase, it is necessary to explore the means through which the modern power supply system can accommodate both increasing affluence (which is accompanied by increased per-capita consumption) and the continually growing global population. Though there has been a great deal of research into the theoretical optimization of large-scale power systems, research into the use of an existing power system as a foundation for this growth has yet to be fully explored. Current successful and robust power generation systems that have significant renewable energy penetration-despite not having been optimized a priori-can be used to inform the advancement of modern power systems to accommodate the increasing demand for electricity. This work explores how an accurate and state-of-the-art computational model of a large, regional energy system can be employed as part of an overarching power systems optimization scheme that looks to inform the decision making process for next generation power supply systems. Research scenarios that explore an introductory multi-objective power flow analysis for a case study involving a regional portion of a large grid will be explored, along with a discussion of future research directions. C1 [DuPont, Bryony; Proper, Scott; Hoyle, Christopher] Oregon State Univ, Sch Mech Ind & Mfg Engn, Corvallis, OR 97331 USA. [Azam, Ridwan; Cotilla-Sanchez, Eduardo] Oregon State Univ, Sch Elect Engn & Comp Sci, Corvallis, OR 97331 USA. [Piacenza, Joseph] Calif State Univ Fullerton, Mech Engn, Fullerton, CA 92834 USA. [Oryshchyn, Danylo; Zitney, Stephen E.; Bossart, Stephen] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP DuPont, B (reprint author), Oregon State Univ, Sch Mech Ind & Mfg Engn, Corvallis, OR 97331 USA. FU National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL under RES [1100426] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES Contract No. 1100426. NR 19 TC 0 Z9 0 U1 1 U2 1 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2016 VL 138 IS 5 AR 051601 DI 10.1115/1.4032521 PG 8 WC Energy & Fuels SC Energy & Fuels GA DV2MJ UT WOS:000382754400001 ER PT J AU Kodavasal, J Harms, K Srivastava, P Som, S Quan, S Richards, K Garcia, M AF Kodavasal, Janardhan Harms, Kevin Srivastava, Priyesh Som, Sibendu Quan, Shaoping Richards, Keith Garcia, Marta TI Development of a Stiffness-Based Chemistry Load Balancing Scheme, and Optimization of Input/Output and Communication, to Enable Massively Parallel High-Fidelity Internal Combustion Engine Simulations SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID COMPRESSION IGNITION COMBUSTION; MODEL; DURATION AB A closed-cycle gasoline compression ignition (GCI) engine simulation near top dead center (TDC) was used to profile the performance of a parallel commercial engine computational fluid dynamics (CFD) code, as it was scaled on up to 4096 cores of an IBM Blue Gene/Q (BG/Q) supercomputer. The test case has 9 x 10(6) cells near TDC, with a fixed mesh size of 0.15 mm, and was run on configurations ranging from 128 to 4096 cores. Profiling was done for a small duration of 0.11 crank angle degrees near TDC during ignition. Optimization of input/output (I/O) performance resulted in a significant speedup in reading restart files, and in an over 100-times speedup in writing restart files and files for postprocessing. Improvements to communication resulted in a 1400-times speedup in the mesh load balancing operation during initialization, on 4096 cores. An improved, "stiffness-based" algorithm for load balancing chemical kinetics calculations was developed, which results in an over three-times faster runtime near ignition on 4096 cores relative to the original load balancing scheme. With this improvement to load balancing, the code achieves over 78% scaling efficiency on 2048 cores, and over 65% scaling efficiency on 4096 cores, relative to 256 cores. C1 [Kodavasal, Janardhan; Som, Sibendu] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Harms, Kevin; Garcia, Marta] Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. [Srivastava, Priyesh; Quan, Shaoping; Richards, Keith] Convergent Sci Inc, 6400 Enterprise Lane, Madison, WI 53719 USA. RP Kodavasal, J (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jkodavasal@anl.gov; harms@alcf.anl.gov; priyesh.srivastava@convergecfd.com; ssom@anl.gov; shaoping.quan@convergecfd.com; krichards@convergecfd.com; mgarcia@alcf.anl.gov FU U.S. Department of Energy (DOE) Office of Science Laboratory [DE-AC02-06CH11357]; DOE's Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357]; DOE Office of Science User Facility [DE-AC02-06CH11357] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne). Argonne, a U.S. Department of Energy (DOE) Office of Science Laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. This research was funded by DOE's Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy under Contract No. DE-AC02-06CH11357. The authors wish to thank Gurpreet Singh, program manager at DOE, for his support. We gratefully acknowledge the computing resources provided on Fusion, an HPC cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC02-06CH11357. The authors would like to thank Joseph Insley of the ALCF for help with visualization, and Dr. Joshua Strodtbeck of Convergent Science, Inc. for useful discussions. NR 38 TC 1 Z9 1 U1 1 U2 1 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2016 VL 138 IS 5 AR 052203 DI 10.1115/1.4032623 PG 11 WC Energy & Fuels SC Energy & Fuels GA DV2MJ UT WOS:000382754400015 ER PT J AU Saha, K Som, S Battistoni, M Li, YH Quan, SP Senecal, PK AF Saha, Kaushik Som, Sibendu Battistoni, Michele Li, Yanheng Quan, Shaoping Senecal, Peter Kelly TI Modeling of Internal and Near-Nozzle Flow for a Gasoline Direct Injection Fuel Injector SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID RELAXATION MODEL; ATOMIZATION; SPRAYS AB A numerical study of two-phase flow inside the nozzle holes and the issuing spray jets for a multihole direct injection gasoline injector has been presented in this work. The injector geometry is representative of the Spray G nozzle, an eight-hole counterbore injector, from the engine combustion network (ECN). Simulations have been carried out for a fixed needle lift. The effects of turbulence, compressibility, and noncondensable gases have been considered in this work. Standard k-epsilon turbulence model has been used to model the turbulence. Homogeneous relaxation model (HRM) coupled with volume of fluid (VOF) approach has been utilized to capture the phase-change phenomena inside and outside the injector nozzle. Three different boundary conditions for the outlet domain have been imposed to examine nonflashing and evaporative, nonflashing and nonevaporative, and flashing conditions. Noticeable hole-to-hole variations have been observed in terms of mass flow rates for all the holes under all the operating conditions considered in this study. Inside the nozzle holes mild cavitationlike and in the near-nozzle region flash-boiling phenomena have been predicted when liquid fuel is subjected to superheated ambiance. Under favorable conditions, considerable flashing has been observed in the near-nozzle regions. An enormous volume is occupied by the gasoline vapor, formed by the flash boiling of superheated liquid fuel. Large outlet domain connecting the exits of the holes and the pressure outlet boundary appeared to be necessary leading to substantial computational cost. Volume-averaging instead of mass-averaging is observed to be more effective, especially for finer mesh resolutions. C1 [Saha, Kaushik; Som, Sibendu] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Battistoni, Michele] Univ Perugia, Dept Engn, I-106123 Perugia, Italy. [Li, Yanheng; Quan, Shaoping; Senecal, Peter Kelly] Convergent Sci Inc, Madison, WI 53719 USA. RP Saha, K (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ksaha@anl.gov; ssom@anl.gov; michele.battistoni@unipg.it; yanheng.li@convergecfd.com; shaoping.quan@convergecfd.com; senecal@convergecfd.com RI Battistoni, Michele/M-9194-2014 OI Battistoni, Michele/0000-0001-6807-9657 FU U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357]; DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy [DE-AC02-06CH11357] FX UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"), a U.S. Department of Energy Office of Science Laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. This research was partially funded by DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy under Contract No. DE-AC02-06CH11357. The authors wish to thank Gurpreet Singh and Leo Breton, program manager at DOE, for his support. NR 28 TC 0 Z9 0 U1 7 U2 7 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2016 VL 138 IS 5 AR 052208 DI 10.1115/1.4032979 PG 11 WC Energy & Fuels SC Energy & Fuels GA DV2MJ UT WOS:000382754400020 ER PT J AU Salvi, AA Hoard, J Styles, D Assanis, D AF Salvi, Ashwin A. Hoard, John Styles, Dan Assanis, Dennis TI In Situ Thermophysical Properties of an Evolving Carbon Nanoparticle Based Deposit Layer Utilizing a Novel Infrared and Optical Methodology SO JOURNAL OF ENERGY RESOURCES TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID GAS RECIRCULATION COOLERS; PARTICULATE DEPOSITION; FLOWS AB The use of exhaust gas recirculation (EGR) in internal combustion engines has significant impacts on engine combustion and emissions. EGR can be used to reduce in-cylinder NOx production, reduce fuel consumption, and enable advanced forms of combustion. To maximize the benefits of EGR, the exhaust gases are often cooled with liquid to gas heat exchangers. However, the build up of a fouling deposit layer from exhaust particulates and volatiles results in the decrease of heat exchanger efficiency, increasing the outlet temperature of the exhaust gases and decreasing the advantages of EGR. This paper presents an experimental data from a novel in situ measurement technique in a visualization rig during the development of a 378 mu m thick deposit layer. Measurements were performed every 6 hrs for up to 24 hrs. The results show a nonlinear increase in deposit thickness with an increase in layer surface area as deposition continued. Deposit surface temperature and temperature difference across the thickness of the layer was shown to increase with deposit thickness while heat transfer decreased. The provided measurements combine to produce deposit thermal conductivity. A thorough uncertainty analysis of the in situ technique is presented and suggests higher measurement accuracy at thicker deposit layers and with larger temperature differences across the layer. The interface and wall temperature measurements are identified as the strongest contributors to the measurement uncertainty. Due to instrument uncertainty, the influence of deposit thickness and temperature could not be determined. At an average deposit thickness of 378 mu m and at a temperature of 100 degrees C, the deposit thermal conductivity was determined to be 0.044 +/- 60.0062 W/m K at a 90% confidence interval based on instrument accuracy. C1 [Salvi, Ashwin A.] US DOE, ARPA E, 1000 Independence Ave SW, Washington, DC 20585 USA. [Hoard, John] Univ Michigan, Walter E Lay Automot Lab 1012, 1231 Beal Ave, Ann Arbor, MI 48109 USA. [Styles, Dan] Ford Motor Co, 2101 Village Rd, Dearborn, MI 48121 USA. [Assanis, Dennis] SUNY Stony Brook, 407 Adm Bldg, Stony Brook, NY 11794 USA. RP Salvi, AA (reprint author), US DOE, ARPA E, 1000 Independence Ave SW, Washington, DC 20585 USA. EM asalvi@umich.edu; hoardjw@umich.edu; dstyles@ford.com; dennis.assanis@stonybrook.edu FU Ford Motor Company FX The authors would like to thank Ford Motor Company for their financial and intellectual support. NR 31 TC 0 Z9 0 U1 3 U2 3 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0195-0738 J9 J ENERG RESOUR-ASME JI J. Energy Resour. Technol.-Trans. ASME PD SEP PY 2016 VL 138 IS 5 AR 052207 DI 10.1115/1.4032942 PG 7 WC Energy & Fuels SC Energy & Fuels GA DV2MJ UT WOS:000382754400019 ER PT J AU Kambhampati, A Shioda, K Gould, LH Sharp, D Brown, LG Parashar, UD Hall, AJ AF Kambhampati, Anita Shioda, Kayoko Gould, L. Hannah Sharp, Donald Brown, Laura G. Parashar, Umesh D. Hall, Aron J. TI A State-by-State Assessment of Food Service Regulations for Prevention of Norovirus Outbreaks SO JOURNAL OF FOOD PROTECTION LA English DT Article DE Food service; Norovirus; Prevention; Regulation; Retail food code ID UNITED-STATES; ACUTE GASTROENTERITIS; NORWALK VIRUS; HANDLER; CONTAMINATION; TRANSMISSION AB Noroviruses are the leading cause of foodborne disease in the United States. Foodborne transmission of norovirus is often associated with contamination of food during preparation by an infected food worker. The U.S. Food and Drug Administration's Food Code provides model food safety regulations for preventing transmission of foodborne disease in restaurants; however, adoption of specific provisions is at the discretion of state and local governments. We analyzed the food service regulations of all 50 states and the District of Columbia (i.e., 51 states) to describe differences in adoption of norovirus-related Food Code provisions into state food service regulations. We then assessed potential correlations between adoption of these regulations and characteristics of foodborne norovirus outbreaks reported to the National Outbreak Reporting System from 2009 through 2014. Of the 51 states assessed, all (100%) required food workers to wash their hands, and 39 (76%) prohibited bare-hand contact with ready-to-eat food. Thirty states (59%) required exclusion of staff with vomiting and diarrhea until 24 h after cessation of symptoms. Provisions requiring a certified food protection manager (CFPM) and a response plan for contamination events (i.e., vomiting) were least commonly adopted; 26 states (51%) required a CFPM, and 8 (16%) required a response plan. Although not statistically significant, states that adopted the provisions prohibiting bare-hand contact (0.45 versus 0.74, P = 0.07), requiring a CFPM (0.38 versus 0.75, P = 0.09), and excluding ill staff for >= 24 h after symptom resolution (0.44 versus 0.73, P = 0.24) each reported fewer foodborne norovirus outbreaks per million person-years than did those states without these provisions. Adoption and compliance with federal recommended food service regulations may decrease the incidence of foodborne norovirus outbreaks. C1 [Kambhampati, Anita; Shioda, Kayoko; Parashar, Umesh D.; Hall, Aron J.] Ctr Dis Control & Prevent, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA. [Gould, L. Hannah; Sharp, Donald] Ctr Dis Control & Prevent, Natl Ctr Emerging & Zoonot Infect Dis, Atlanta, GA 30333 USA. [Brown, Laura G.] Ctr Dis Control & Prevent, Natl Ctr Environm Hlth, Atlanta, GA 30333 USA. [Kambhampati, Anita; Shioda, Kayoko] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA. RP Kambhampati, A (reprint author), Ctr Dis Control & Prevent, Natl Ctr Immunizat & Resp Dis, Atlanta, GA 30333 USA.; Kambhampati, A (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA. EM wyc4@cdc.gov FU U.S. Department of Energy; CDC; Agriculture and Food Research Initiative Competitive Grant from U.S. Department of Agriculture, National Institute of Food and Agriculture [2011-68003-30395] FX This research was supported in part by appointments to the Research Participation Program at the Centers for Disease Control and Prevention (A.K. and K.S.) administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and the CDC. This work was also supported in part by Agriculture and Food Research Initiative Competitive Grant 2011-68003-30395 from the U.S. Department of Agriculture, National Institute of Food and Agriculture. The findings and conclusions in this report are those of the authors and do not necessarily represent the official position of the CDC. NR 31 TC 0 Z9 0 U1 5 U2 5 PU INT ASSOC FOOD PROTECTION PI DES MOINES PA 6200 AURORA AVE SUITE 200W, DES MOINES, IA 50322-2863 USA SN 0362-028X EI 1944-9097 J9 J FOOD PROTECT JI J. Food Prot. PD SEP PY 2016 VL 79 IS 9 BP 1527 EP 1536 DI 10.4315/0362-028X.JFP-16-088 PG 10 WC Biotechnology & Applied Microbiology; Food Science & Technology SC Biotechnology & Applied Microbiology; Food Science & Technology GA DV3DP UT WOS:000382801500008 PM 28221948 ER PT J AU Mani, A Tsai, FTC Kao, SC Naz, BS Ashfaq, M Rastogi, D AF Mani, Amir Tsai, Frank T. -C. Kao, Shih-Chieh Naz, Bibi S. Ashfaq, Moetasim Rastogi, Deeksha TI Conjunctive management of surface and groundwater resources under projected future climate change scenarios SO JOURNAL OF HYDROLOGY LA English DT Article DE Conjunctive use; Multi-reservoir system; Groundwater; Climate change; Uncertainty; Fractional programming ID FRACTIONAL-PROGRAMMING APPROACH; CHANGE IMPACT ASSESSMENT; WATER-RESOURCES; UNITED-STATES; QUANTIFYING UNCERTAINTY; GENETIC ALGORITHMS; BIAS CORRECTION; VIC-2L MODEL; LARGE-SCALE; OPTIMIZATION AB This study introduces a mixed integer linear fractional programming (MILFP) method to optimize conjunctive use of future surface water and groundwater resources under projected climate change scenarios. The conjunctive management model maximizes the ratio of groundwater usage to reservoir water usage. Future inflows to the reservoirs were estimated from the future runoffs projected through hydro climate modeling considering the Variable Infiltration Capacity model, and 11 sets of downscaled Coupled Model Intercomparison Project phase 5 global climate model projections. Bayesian model averaging was adopted to quantify uncertainty in future runoff projections and reservoir inflow projections due to uncertain future climate projections. Optimized conjunctive management solutions were investigated for a water supply network in northern Louisiana which includes the Sparta aquifer. Runoff projections under climate change scenarios indicate that runoff will likely decrease in winter and increase in other seasons. Results from the developed conjunctive management model with MILFP indicate that the future reservoir water, even at 2.5% low inflow cumulative probability level, could counterbalance groundwater pumping reduction to satisfy demands while improving the Sparta aquifer through conditional groundwater head constraints. (C) 2016 Elsevier B.V. All rights reserved. C1 [Mani, Amir; Tsai, Frank T. -C.] Louisiana State Univ, Dept Civil & Environm Engn, 3526G Patrick F Taylor Hall, Baton Rouge, LA 70803 USA. [Kao, Shih-Chieh; Naz, Bibi S.; Ashfaq, Moetasim; Rastogi, Deeksha] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Kao, Shih-Chieh; Naz, Bibi S.] Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37831 USA. [Ashfaq, Moetasim; Rastogi, Deeksha] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Tsai, FTC (reprint author), Louisiana State Univ, Dept Civil & Environm Engn, 3526G Patrick F Taylor Hall, Baton Rouge, LA 70803 USA. EM amani1@lsu.edu; ftsai@lsu.edu; kaos@ornl.gov; naz.bibi2007@gmail.com; mashfaq@ornl.gov; rastogid@ornl.gov RI Kao, Shih-Chieh/B-9428-2012; OI Kao, Shih-Chieh/0000-0002-3207-5328; Naz, Bibi/0000-0001-9888-1384 FU Louisiana Board of Regents [LEQSF(2012-15)-RD-A-03]; U.S. Geological Survey under (LWRRI) [G11AP20082]; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported in part by the Louisiana Board of Regents under award number LEQSF(2012-15)-RD-A-03 and by the U.S. Geological Survey under Grant/Cooperative Agreement No. G11AP20082 (through LWRRI). The authors acknowledge Brian Clark of USGS for providing the Sparta groundwater model, Pierre Sargent of USGS for providing water use data for northern Louisiana, and the Louisiana Sparta Ground Water Commission for providing technical reports. The LSU Center for Computation & Technology (CCT) and the High Performance Computing (HPC) are acknowledged for providing computing resources and technical assistance. This paper was coauthored by employees of the Oak Ridge National Laboratory, managed by UT Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. Accordingly, the publisher, by accepting the article for publication, acknowledges that the United States government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States government purposes. NR 69 TC 1 Z9 1 U1 12 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD SEP PY 2016 VL 540 BP 397 EP 411 DI 10.1016/j.jhydrol.2016.06.021 PG 15 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA DU5RR UT WOS:000382269500032 ER PT J AU Malama, B Kuhlman, KL Brauchler, R Bayer, P AF Malama, Bwalya Kuhlman, Kristopher L. Brauchler, Ralf Bayer, Peter TI Modeling cross-hole slug tests in an unconfined aquifer SO JOURNAL OF HYDROLOGY LA English DT Article DE Cross-hole slug tests; Multi-level; Unconfined aquifer; Hydraulic conductivity; Specific storage; Specific yield ID PARTIALLY PENETRATING WELLS; UNSATURATED FRACTURED TUFF; HYDRAULIC CHARACTERIZATION; NUMERICAL INVERSION; INTERFERENCE TESTS; WATER; FLOW; ROCK; APPLICABILITY; CONDUCTIVITY AB A modified version of a published slug test model for unconfined aquifers is applied to cross-hole slug test data collected in field tests conducted at the Widen site in Switzerland. The model accounts for water-table effects using the linearized kinematic condition. The model also accounts for inertial effects in source and observation wells. The primary objective of this work is to demonstrate applicability of this semi-analytical model to multi-well and multi-level pneumatic slug tests. The pneumatic perturbation was applied at discrete intervals in a source well and monitored at discrete vertical intervals in observation wells. The source and observation well pairs were separated by distances of up to 4 m. The analysis yielded vertical profiles of hydraulic conductivity, specific storage, and specific yield at observation well locations. The hydraulic parameter estimates are compared to results from prior pumping and single-well slug tests conducted at the site, as well as to estimates from particle size analyses of sediment collected from boreholes during well installation. The results are in general agreement with results from prior tests and are indicative of a sand and gravel aquifer. Sensitivity analysis show that model identification of specific yield is strongest at late-time. However, the usefulness of late-time data is limited due to the low signal-to-noise ratios. (C) 2016 Elsevier B.V. All rights reserved. C1 [Malama, Bwalya] Calif Polytech State Univ San Luis Obispo, Nat Resources Management & Environm Sci Dept, San Luis Obispo, CA 93407 USA. [Kuhlman, Kristopher L.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Brauchler, Ralf] AF Consult Switzerland Ltd, Baden, Switzerland. [Bayer, Peter] ETH, Zurich, Switzerland. RP Malama, B (reprint author), Calif Polytech State Univ San Luis Obispo, Nat Resources Management & Environm Sci Dept, San Luis Obispo, CA 93407 USA. EM bmalama@scalpoly.edu RI Bayer, Peter/J-8245-2013; OI Bayer, Peter/0000-0003-4884-5873; Kuhlman, Kristopher/0000-0003-3397-3653 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 51 TC 0 Z9 0 U1 5 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-1694 EI 1879-2707 J9 J HYDROL JI J. Hydrol. PD SEP PY 2016 VL 540 BP 784 EP 796 DI 10.1016/j.jhydrol.2016.06.060 PG 13 WC Engineering, Civil; Geosciences, Multidisciplinary; Water Resources SC Engineering; Geology; Water Resources GA DU5RR UT WOS:000382269500061 ER PT J AU Es-Said, OS Alcisto, J Guerra, J Jones, E Dominguez, A Hahn, M Ula, N Zeng, L Ramsey, B Mulazimoglu, H Li, YJ Miller, M Alrashid, J Papakyriakou, M Kalnaus, S Lee, EW Frazier, WE AF Es-Said, O. S. Alcisto, J. Guerra, J. Jones, E. Dominguez, A. Hahn, M. Ula, N. Zeng, L. Ramsey, B. Mulazimoglu, H. Li, Yong-Jun Miller, M. Alrashid, J. Papakyriakou, M. Kalnaus, S. Lee, E. W. Frazier, W. E. TI Effect of Cadmium Plating Thickness on the Charpy Impact Energy of Hydrogen-Charged 4340 Steel SO JOURNAL OF MATERIALS ENGINEERING AND PERFORMANCE LA English DT Article DE 4340 steel; cadmium plating; Charpy impact test; hydrogen charging ID MECHANICAL-PROPERTIES; INDUCED CRACKING; EMBRITTLEMENT; TRANSPORT; BEHAVIOR; FRACTURE; MICROSTRUCTURE; DEFORMATION AB Hydrogen was intentionally introduced into ultra-high strength steel by cadmium plating. The purpose was to examine the effect of cadmium plate thickness and hence hydrogen on the impact energy of the steel. The AISI 4340 steel was austenitized at 1000 A degrees C for 1 h, water quenched, and tempered at temperatures between 257 and 593 A degrees C in order to achieve a range of targeted strength levels. The specimens were cadmium plated with 0.00508 mm (0.2 mils), 0.00762 mm (0.3 mils), and 0.0127 mm (0.5 mils). Results demonstrated that the uncharged specimens exhibited higher impact energy values when compared to the plated specimens at all tempering temperatures. The cadmium-plated specimens had very low Charpy impact values irrespective of their ultimate tensile strength values. The model of hydrogen transport by mobile dislocations to the fracture site appears to provide the most suitable explanation of the results. C1 [Es-Said, O. S.; Alcisto, J.; Guerra, J.; Jones, E.; Dominguez, A.; Miller, M.; Alrashid, J.; Papakyriakou, M.] Loyola Marymount Univ, Dept Mech Engn, Los Angeles, CA 90045 USA. [Hahn, M.] Northrop Grumman, Mat & Proc F35, Redondo Beach, CA 90278 USA. [Ula, N.] Loyola Marymount Univ, Dept Elect Engn, Los Angeles, CA 90045 USA. [Zeng, L.; Ramsey, B.] Sargent Aerosp & Def, Torrance, CA 90502 USA. [Mulazimoglu, H.] ALCOA Fastening Syst & Rings, Torrance, CA 90502 USA. [Li, Yong-Jun] Loyola Marymount Univ, Coll Sci & Engn, MANE Labs, Los Angeles, CA 90045 USA. [Kalnaus, S.] Oak Ridge Natl Lab, Computat Engn & Energy Sci Grp, Oak Ridge, TN USA. [Lee, E. W.; Frazier, W. E.] Naval Air Syst Command, Patuxent River, MD 20670 USA. RP Es-Said, OS (reprint author), Loyola Marymount Univ, Dept Mech Engn, Los Angeles, CA 90045 USA. EM oessaid@lmu.edu NR 44 TC 0 Z9 0 U1 5 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1059-9495 EI 1544-1024 J9 J MATER ENG PERFORM JI J. Mater. Eng. Perform. PD SEP PY 2016 VL 25 IS 9 BP 3606 EP 3614 DI 10.1007/s11665-016-2246-6 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA DV2JT UT WOS:000382747400008 ER PT J AU Chen, GQ Feng, ZL Zhu, YC Shi, QY AF Chen, Gaoqiang Feng, Zhili Zhu, Yucan Shi, Qingyu TI An Alternative Frictional Boundary Condition for Computational Fluid Dynamics Simulation of Friction Stir Welding SO JOURNAL OF MATERIALS ENGINEERING AND PERFORMANCE LA English DT Article DE frictional boundary condition; friction stir welding; heat generation; material flow; thermal-mechanical processing condition ID MATERIAL FLOW; ALUMINUM-ALLOY; HEAT-GENERATION; TOOL; MODEL; STEEL; VISUALIZATION AB For better application of numerical simulation in optimization and design of friction stir welding (FSW), this paper presents a new frictional boundary condition at the tool/workpiece interface for computational fluid dynamics (CFD) modeling of FSW. The proposed boundary condition is based on an implementation of the Coulomb friction model. Using the new boundary condition, the CFD simulation yields non-uniform distribution of contact state over the tool/workpiece interface, as validated by the experimental weld macrostructure. It is found that interfacial sticking state is present over large area at the tool-workpiece interface, while significant interfacial sliding occurs at the shoulder periphery, the lower part of pin side, and the periphery of pin bottom. Due to the interfacial sticking, a rotating flow zone is found under the shoulder, in which fast circular motion occurs. The diameter of the rotating flow zone is smaller than the shoulder diameter, which is attributed to the presence of the interfacial sliding at the shoulder periphery. For the simulated welding condition, the heat generation due to friction and plastic deformation makes up 54.4 and 45.6% of the total heat generation rate, respectively. The simulated temperature field is validated by the good agreement to the experimental measurements. C1 [Chen, Gaoqiang; Zhu, Yucan; Shi, Qingyu] Tsinghua Univ, State Key Lab Tribol, 1 Tsinghua Yuan Pk, Beijing 100084, Peoples R China. [Chen, Gaoqiang; Zhu, Yucan; Shi, Qingyu] Tsinghua Univ, Dept Mech Engn, Key Lab Adv Mat Proc Technol, 1 Tsinghua Yuan Pk, Beijing 100084, Peoples R China. [Chen, Gaoqiang; Feng, Zhili] Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Chen, GQ; Shi, QY (reprint author), Tsinghua Univ, State Key Lab Tribol, 1 Tsinghua Yuan Pk, Beijing 100084, Peoples R China.; Chen, GQ; Shi, QY (reprint author), Tsinghua Univ, Dept Mech Engn, Key Lab Adv Mat Proc Technol, 1 Tsinghua Yuan Pk, Beijing 100084, Peoples R China.; Chen, GQ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM Gaoqiang.chen@hotmail.com; shqy@tsinghua.edu.cn FU National Natural Science Foundation of China [51375259]; National Science and Technology Major Project of the Ministry of Science and Technology of China [2012ZX04012-011]; China Scholarship Council [20130620105] FX The research was supported by the National Natural Science Foundation of China (Grant No. 51375259) and the National Science and Technology Major Project of the Ministry of Science and Technology of China (No. 2012ZX04012-011). Besides, Gaoqiang Chen was supported by the China Scholarship Council (File No. 20130620105) for 2-year study at Oak Ridge National Laboratory. NR 37 TC 1 Z9 1 U1 17 U2 17 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1059-9495 EI 1544-1024 J9 J MATER ENG PERFORM JI J. Mater. Eng. Perform. PD SEP PY 2016 VL 25 IS 9 BP 4016 EP 4023 DI 10.1007/s11665-016-2219-9 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA DV2JT UT WOS:000382747400051 ER PT J AU Martin, WE Srijanto, BR Collier, CP Vosch, T Richards, CI AF Martin, W. Elliott Srijanto, Bernadeta R. Collier, C. Patrick Vosch, Tom Richards, Christopher I. TI A Comparison of Single-Molecule Emission in Aluminum and Gold Zero-Mode Waveguides SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ENHANCED RAMAN-SCATTERING; FLUORESCENCE CORRELATION SPECTROSCOPY; NEAR-INFRARED FLUORESCENCE; PLASMON-COUPLED EMISSION; POLYELECTROLYTE MULTILAYERS; BOWTIE NANOANTENNAS; MICROSCOPY; NANORODS; NANOPARTICLES; EXCITATION AB The effect of gold and aluminum zero-mode waveguides (ZMWs) on the brightness of immobilized Single emitters was characterized by probing fluorophores that absorb in the green. and red regions of the visible spectrum. Aluminum ZMWs enhance the emission of Atto565 fluorophores upon green excitation, but they do not enhance the emission of Atto647N fluorophores upon red excitation. Gold ZMWs increase emission of both fluorophores with Atto647N showing enhancement that is threefold higher than that observed for Atto565. This work indicates that 200 nm gold ZMWs are better suited for Single Molecule fluorescence studies the red region of:the visible spectrum, while aluminum appears more-suited for the green region of the visible spectrum. C1 [Martin, W. Elliott; Richards, Christopher I.] Univ Kentucky, Dept Chem, 505 Rose St, Lexington, KY 40506 USA. [Srijanto, Bernadeta R.; Collier, C. Patrick] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Vosch, Tom] Univ Copenhagen, Dept Chem, Nanosci Ctr, Univ Pk 5, DK-2100 Copenhagen, Denmark. RP Richards, CI (reprint author), Univ Kentucky, Dept Chem, 505 Rose St, Lexington, KY 40506 USA. EM chris.richards@uky.edu RI Srijanto, Bernadeta/D-4213-2016; Vosch, Tom/B-4234-2015 OI Srijanto, Bernadeta/0000-0002-1188-1267; Vosch, Tom/0000-0001-5435-2181 FU HFSP [RGY0081/2014]; "Center for Synthetic Biology" at Copenhagen Univ. by the UNIK research initiative of the Danish Ministry of Science, Technology and Innovation [09-065274]; bioSYNergy, Univ. of Copenhagen's Excellence Programme for Interdisciplinary Research FX C.I.R. and T.V. acknowledge support from HFSP (RGY0081/2014). T.V. gratefully acknowledges financial support from the "Center for Synthetic Biology" at Copenhagen Univ. funded by the UNIK research initiative of the Danish Ministry of Science, Technology and Innovation (Grant No. 09-065274) and bioSYNergy, Univ. of Copenhagen's Excellence Programme for Interdisciplinary Research. Fabrication of 200 nm gold ZMWs was conducted at the Center for Nanophase Materials Sciences, which is a Department of Energy Office of Science User Facility. NR 72 TC 0 Z9 0 U1 7 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD SEP 1 PY 2016 VL 120 IS 34 BP 6719 EP 6727 DI 10.1021/acs.jpca.6b03309 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DV0GU UT WOS:000382596800006 PM 27499174 ER PT J AU Lee, L Wilson, K AF Lee, Lance Wilson, Kevin TI The Reactive-Diffusive Length of OH and Ozone in Model Organic Aerosols SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID HETEROGENEOUS OXIDATION; OLEIC-ACID; SUBMICRON SQUALANE; TRACER DIFFUSION; GAS-PHASE; RADICALS; CHEMISTRY; PRODUCTS; KINETICS; EMISSIONS AB A key step in the heterogeneous oxidation of atmospheric aerosols is the reaction of ozone (O-3) and hydroxyl radicals (OH) at the gas-particle interface. The formation of reaction products and free radical intermediates and their spatial distribution inside the particle is a sensitive function of the length over which these oxidants diffuse prior to reaction. The reactive-diffusive length of OH and ozone at organic aerosol interfaces is determined by observing the change in the effective uptake coefficient for size-selected model aerosols comprising a reactive core and a thin nanometer-sized (0-12 nm) organic shell. The core and shell materials are selected so that they are immiscible and adopt an assumed core-shell configuration. The results indicate a reactive-diffusive length of 1.4 run for hydroxyl (OH) radicals in squalane and 1.0 nm for ozone in squalene. Measurements for a purely diffusive system allow for an estimate for diffusion constant (1.6 x 10(-6) cm(2)/s) of ozone in squalane to be determined. The reactive-diffusive length offers a simple first order estimate of how shielding of aerosols by immiscible layers can alter estimates of oxidative lifetimes of aerosols in the atmosphere. C1 [Lee, Lance; Wilson, Kevin] Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. RP Wilson, K (reprint author), Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. EM krwilson@lbl.gov FU Department of Energy's Office of Science Early Career Research Program; Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work is supported by the Department of Energy's Office of Science Early Career Research Program and by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 57 TC 1 Z9 1 U1 11 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD SEP 1 PY 2016 VL 120 IS 34 BP 6800 EP 6812 DI 10.1021/acs.jpca.6b05285 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DV0GU UT WOS:000382596800016 PM 27509443 ER PT J AU Cai, QX Wang, JG Wang, Y Mei, DH AF Cai, Qiuxia Wang, Jian-guo Wang, Yong Mei, Donghai TI First-Principles Thermodynamics Study of Spinel MgAl2O4 Surface Stability SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; ATOMISTIC SIMULATION; IR CATALYSTS; BASIS-SET; OXIDATION; NANOPARTICLES; EFFICIENT; ETHANOL AB The surface stability of all possible terminations for three low-index (100, 110, 111) structures of spinel MgAl2O4 was studied using a first-principles-based thermodynamic approach. The surface Gibbs free energy results indicate that the 100_AlO2 termination is the most stable surface structure under ultrahigh vacuum at T = 1100 K regardless of an Al-poor or Al-rich condition. With increasing oxygen pressure, the 111_O-2(Al) termination becomes the most stable surface in the Al-rich condition. The oxygen vacancy formation is thermodynamically favorable over the 100_AlO2, 111_O-2(Al), and (111) structures with Mg/O connected terminations. On the basis of the surface Gibbs free energies for both perfect and defective surface terminations, 100_AlO2. and 111_O-2(Al) are the most dominant surfaces in Al-rich conditions tinder atmospheric conditions. This is, also consistent with our previously reported experimental observation. C1 [Cai, Qiuxia; Wang, Jian-guo] Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310014, Zhejiang, Peoples R China. [Cai, Qiuxia; Wang, Yong; Mei, Donghai] Pacific Northwest Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Wang, Yong] Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. RP Wang, JG (reprint author), Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310014, Zhejiang, Peoples R China.; Wang, Y; Mei, DH (reprint author), Pacific Northwest Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.; Wang, Y (reprint author), Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. EM jgw@zjut.edu.cn; yong.wang@pnnl.gov; donghai.mei@pnnl.gov RI Mei, Donghai/A-2115-2012; Mei, Donghai/D-3251-2011 OI Mei, Donghai/0000-0002-0286-4182; FU National Energy Research Scientific Computing Center (NERSC); William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) FX The research described in this paper is part of the MS3 Initiative at the Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program (LDRD) at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy (DOE). The computing time was granted by the National Energy Research Scientific Computing Center (NERSC). Part of the computing time was also granted by a scientific theme user proposal in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), which is a U.S. Department of Energy national scientific user facility located at PNNL in Richland, Washington. NR 39 TC 0 Z9 0 U1 24 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD SEP 1 PY 2016 VL 120 IS 34 BP 19087 EP 19096 DI 10.1021/acs.jpcc.6b02998 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DV0GV UT WOS:000382596900017 ER PT J AU Carpenter, TS Parkin, J Khalid, S AF Carpenter, Timothy S. Parkin, Jamie Khalid, Syma TI The Free Energy of Small Solute Permeation through the Escherichia coli Outer Membrane Has a Distinctly Asymmetric Profile SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; LIPID-BILAYER; COMPUTER-SIMULATIONS; FORCE-FIELD; EQUILIBRIUM AB Permeation of small molecules across cell membranes is a ubiquitous process in biology and is dependent on the principles of physical chemistry at the molecular level. Here we use atomistic molecular dynamics simulations to calculate the free energy of permeation of a range of small molecules through a model of the outer membrane of Escherichia coli, an archetypical Gram-negative bacterium. The model membrane contains lipopolysaccharide (LPS) molecules in the outer leaflet and phospholipids in the inner leaflet. Our results show that the energetic barriers to permeation through the two leaflets of the membrane are distinctly asymmetric; the LPS headgroups provide a less energetically favorable environment for organic compounds than do phospholipids. In summary, we provide the first reported estimates of the relative free energies associated with the different chemical environments experienced by solutes as they attempt to cross the outer membrane of a Gram-negative bacterium. These results provide key insights for the development of novel antibiotics that target these bacteria. C1 [Carpenter, Timothy S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Parkin, Jamie; Khalid, Syma] Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England. RP Khalid, S (reprint author), Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England. EM S.Khalid@soton.ac.uk RI Khalid, Syma/B-8108-2009 OI Khalid, Syma/0000-0002-3694-5044 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-685118] FX We acknowledge use of the Iridis III and IV supercomputers at the University of Southampton. We also thank Livermore Computing for the computing time. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, LLNL-JRNL-685118. NR 17 TC 1 Z9 1 U1 8 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD SEP 1 PY 2016 VL 7 IS 17 BP 3446 EP 3451 DI 10.1021/acs.jpclett.6b01399 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DV0JH UT WOS:000382603300026 PM 27518381 ER PT J AU Buck, C Yeh, MF AF Buck, Christian Yeh, Minfang TI Metal-loaded organic scintillators for neutrino physics SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Review DE liquid scintillators; neutrinos; large scale detectors ID DOUBLE-BETA DECAY; LIQUID SCINTILLATOR; SOLAR NEUTRINOS; ENERGY-TRANSFER; LIGHT YIELD; DETECTOR; BOREXINO; TIME; SPECTROSCOPY; SYSTEM AB Organic liquid scintillators are used in many neutrino physics experiments of the past and present. In particular for low energy neutrinos when realtime and energy information are required, liquid scintillators have several advantages compared to other technologies. In many cases the organic liquid needs to be loaded with metal to enhance the neutrino signal over background events. Several metal loaded scintillators of the past suffered from chemical and optical instabilities, limiting the performance of these neutrino detectors. Different ways of metal loading are described in the article with a focus on recent techniques providing metal loaded scintillators that can be used under stable conditions for many years even in ton scale experiments. Applications of metal loaded scintillators in neutrino experiments are reviewed and the performance as well as the prospects of different scintillator types are compared. C1 [Buck, Christian] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Yeh, Minfang] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Buck, C (reprint author), Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. EM Christian.Buck@mpi-hd.mpg.de NR 112 TC 1 Z9 1 U1 4 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 EI 1361-6471 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD SEP PY 2016 VL 43 IS 9 AR 093001 DI 10.1088/0954-3899/43/9/093001 PG 40 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU6CB UT WOS:000382299600001 ER PT J AU Allu, S Kalnaus, S Simunovic, S Nanda, J Turner, JA Pannala, S AF Allu, S. Kalnaus, S. Simunovic, S. Nanda, J. Turner, J. A. Pannala, S. TI A three-dimensional meso-macroscopic model for Li-Ion intercalation batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Li-ion; Modeling and simulation ID LITHIUM DEPOSITION; POROUS-ELECTRODES; MICROBATTERIES; ARCHITECTURES; CELLS; SIMULATIONS; TRANSPORT; CAPACITY AB In this paper we present a three-dimensional computational formulation for electrode-electrolyte electrode system of Li-Ion batteries. The physical consistency between electrical, thermal and chemical equations is enforced at each time increment by driving the residual of the resulting coupled system of nonlinear equations to zero. The formulation utilizes a rigorous volume averaging approach typical of multiphase formulations used in other fields and recently extended to modeling of supercapacitors [1]. Unlike existing battery modeling methods which use segregated solution of conservation equations and idealized geometries, our unified approach can model arbitrary battery and electrode configurations. The consistency of multi-physics solution also allows for consideration of a wide array of initial conditions and load cases. The formulation accounts for spatio-temporal variations of material and state properties such as electrode/void volume fractions and anisotropic conductivities. The governing differential equations are discretized using the finite element method and solved using a nonlinearly consistent approach that provides robust stability and convergence. The new formulation was validated for standard Li-ion cells and compared against experiments. Its scope and ability to capture spatio-temporal variations of potential and lithium distribution is demonstrated on a prototypical three-dimensional electrode problem. (C) 2016 Elsevier B.V. All rights reserved. C1 [Allu, S.; Kalnaus, S.; Simunovic, S.; Nanda, J.; Turner, J. A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Pannala, S.] SABIC, Houston, TX USA. RP Allu, S (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM allus@ornl.gov OI Turner, John/0000-0003-2521-4091; allu, srikanth/0000-0003-2841-4398 FU U.S. Department of Energy [DE-AC05-00OR22725]; Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy FX This research at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725, was sponsored by the Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy. NR 38 TC 2 Z9 2 U1 10 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2016 VL 325 BP 42 EP 50 DI 10.1016/j.jpowsour.2016.06.001 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DT0HX UT WOS:000381165600006 ER PT J AU Song, BH Li, WD Yan, PF Oh, SM Wang, CM Manthiram, A AF Song, Bohang Li, Wangda Yan, Pengfei Oh, Seung-Min Wang, Chong-Min Manthiram, Arumugam TI A facile cathode design combining Ni-rich layered oxides with Li-rich layered oxides for lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Nickel-rich layered oxide; Lithium-rich layered oxide; Surface chemical stability; Pouch-type full cell ID ELECTROCHEMICAL PROPERTIES; CAPACITY; ELECTRODES; MN; CHEMISTRY; EVOLUTION; PHASE; FADE AB A facile synthesis method has been developed to prepare xLi(2)MnO(3)center dot(1-x)LiNi0.7Co0.5Mn0.15O2 (x = 0, 0.03, 0.07, 0.10, 0.20, and 0.30) cathode materials, combining the advantages of the high specific capacity of the Ni-rich layered phase and the surface chemical stability of the Li-rich layered phase. X-ray diffraction (XRD), transmission electron microscopy (TEM), and electrochemical charge/discharge measurements confirm the formation of a Li-rich layered phase with C2/m symmetry. The high-angle annular dark-field (HAADF) scanning transmission electron microscopy (STEM) reveals a spatial relationship that the Li-rich nano-domain islands are integrated into the conventional Ni-rich layered matrix (R (3) over barm). Most importantly, this is the first time that Li-rich phase has been directly observed inside a particle at the nano-scale, when the overall composition of the layered oxide Li1+delta Ni1-y-z-delta MnyMzO2 (M = metal) is Ni-rich (>0.5) rather than Mn-rich (>0.5). Remarkably, the xLi(2)MnO(3)center dot(1-x)LiNi0.7Co0.15Mn0.15O2 cathodes with optimized x value shows superior electrochemical performance at C/3 rate: an initial capacity of 190 mA h g(-1) with 90% capacity retention after 400 cycles in a half cell and 73.5% capacity retention after 900 cycles in a pouch-type full cell. (C) 2016 Elsevier B.V. All rights reserved. C1 [Song, Bohang; Li, Wangda; Oh, Seung-Min; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Song, Bohang; Li, Wangda; Oh, Seung-Min; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Yan, Pengfei; Wang, Chong-Min] Pacific Northwest Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA.; Manthiram, A (reprint author), Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI yan, pengfei/E-4784-2016; Song, Bohang/F-8239-2016 OI yan, pengfei/0000-0001-6387-7502; Song, Bohang/0000-0002-6477-609X FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-EE0006447]; Welch Foundation [F-1254]; DOE's Office of Biological and Environmental Research; Department of Energy [DE-AC05-76RLO1830] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract no. DE-EE0006447 and Welch Foundation grant F-1254. The STEM work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the Department of Energy under Contract DE-AC05-76RLO1830. The authors acknowledge the assistance and valuable discussion with Dr. Pilgun Oh and Dr. Jin-Yun Liao. NR 36 TC 3 Z9 3 U1 40 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2016 VL 325 BP 620 EP 629 DI 10.1016/j.jpowsour.2016.06.056 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DT0HX UT WOS:000381165600071 ER PT J AU Lipson, AL Han, SD Kim, S Pan, BF Sa, NY Liao, C Fister, TT Burrell, AK Vaughey, JT Ingram, BJ AF Lipson, Albert L. Han, Sang-Don Kim, Soojeong Pan, Baofei Sa, Niya Liao, Chen Fister, Timothy T. Burrell, Anthony K. Vaughey, John T. Ingram, Brian J. TI Nickel hexacyanoferrate, a versatile intercalation host for divalent ions from nonaqueous electrolytes SO JOURNAL OF POWER SOURCES LA English DT Article DE Nickel hexacyanoferrate; Magnesium battery; Calcium battery; XANES; Nonaqueous ID PRUSSIAN BLUE; COPPER HEXACYANOFERRATE; RECHARGEABLE BATTERIES; IRON HEXACYANOFERRATE; MAGNESIUM BATTERIES; CATHODE MATERIALS; OPEN FRAMEWORK; INSERTION; LITHIUM; 1ST-PRINCIPLES AB New energy storage chemistries based on Mg ions or Ca ions can theoretically improve both the energy density and reduce the costs of batteries. To date there has been limited progress in implementing these systems due to the challenge of finding a high voltage high capacity cathode that is compatible with an electrolyte that can plate and strip the elemental metal. In order to accelerate the discovery of such a system, model systems are needed that alleviate some of the issues of incompatibility. This report demonstrates the ability of nickel hexacyanoferrate to electrochemically intercalate Mg, Ca and Zn ions from a nonaqueous electrolyte. This material has a relatively high insertion potential and low over potential in the electrolytes used in this study. Furthermore, since it is not an oxide based cathode it should be able to resist attack by corrosive electrolytes such as the chloride containing electrolytes that are often used to plate and strip magnesium. This makes it an excellent cathode for use in developing and understanding the complex electrochemistry of multivalent ion batteries. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lipson, Albert L.; Han, Sang-Don; Kim, Soojeong; Pan, Baofei; Sa, Niya; Liao, Chen; Fister, Timothy T.; Burrell, Anthony K.; Vaughey, John T.; Ingram, Brian J.] Argonne Natl Lab, Joint Ctr Energy Storage Res, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. RP Ingram, BJ (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM ingram@anl.gov RI BM, MRCAT/G-7576-2011; SA, NIYA/E-8521-2017 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. We would also like to acknowledge the use of the Center for Nanoscale Materials, supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT (APS sector 10BM) operations are supported by the Department of Energy and the MRCAT member institutions. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 29 TC 3 Z9 3 U1 46 U2 51 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2016 VL 325 BP 646 EP 652 DI 10.1016/j.jpowsour.2016.06.019 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DT0HX UT WOS:000381165600075 ER PT J AU Shinozaki, K Morimoto, Y Pivovar, BS Kocha, SS AF Shinozaki, Kazuma Morimoto, Yu Pivovar, Bryan S. Kocha, Shyam S. TI Suppression of oxygen reduction reaction activity on Pt-based electrocatalysts from ionomer incorporation SO JOURNAL OF POWER SOURCES LA English DT Article DE Oxygen reduction reaction; Platinum; Platinum alloy; Neon ionomer; Rotating disk electrode method; Ionomer coverage ID ROTATING-DISK ELECTRODE; FUEL-CELL ELECTRODES; CATALYST LAYERS; ACID-SOLUTION; 111 SURFACE; THIN-FILM; PLATINUM; TRANSPORT; PEMFC; ADSORPTION AB The impact of Nafion on the oxygen reduction reaction (ORR) activity is studied for Pt/C and Pt-alloy/C catalysts using thin-film rotating disk electrode (TF-RDE) methods in 0.1 M HClO4. Ultrathin uniform catalyst layers and standardized activity measurement protocols are employed to obtain accurate and reproducible ORR activity. Nafion lowers the ORR activity which plateaus with increasing loading on Pt catalysts. Pt particle size is found not to have significant influence on the extent of the SA decrease upon Nafion incorporation. Catalysts using high surface area carbon (HSC) support exhibit attenuated activity loss resulting from lower ionomer coverage on catalyst particles located within the deep pores. The impact of metallic composition on the activity loss due to Nafion incorporation is also discussed. (C) 2016 Elsevier B.V. All rights reserved. C1 [Shinozaki, Kazuma; Pivovar, Bryan S.; Kocha, Shyam S.] Natl Renewable Energy Lab, Electrochem Characterizat Labs, Golden, CO 80401 USA. [Shinozaki, Kazuma] Colorado Sch Mines, Dept Chem, Golden, CO 80401 USA. [Shinozaki, Kazuma; Morimoto, Yu] Toyota Cent Res & Dev Labs Inc, Nagakute, Aichi 4801192, Japan. RP Shinozaki, K (reprint author), Toyota Cent Res & Dev Labs Inc, Nagakute, Aichi 4801192, Japan. EM Shinozaki@mosk.tytlabs.co.jp FU U.S. Department of Energy, Fuel Cells Technologies Program [DE-AC36-08-GO28308]; Toyota Central RD Labs., Inc. FX Shyam S. Kocha gratefully acknowledges funding from the U.S. Department of Energy, Fuel Cells Technologies Program under Contract No. DE-AC36-08-GO28308 to the National Renewable Energy Laboratory. Kazuma Shinozaki's stay at NREL and CSM was funded by Toyota Central R&D Labs., Inc. We would like to acknowledge Umicore for providing their catalysts. NR 41 TC 1 Z9 1 U1 34 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD SEP 1 PY 2016 VL 325 BP 745 EP 751 DI 10.1016/j.jpowsour.2016.06.062 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DT0HX UT WOS:000381165600088 ER PT J AU Gupta, S Feng, J Chan, LJG Petzold, CJ Ralston, CY AF Gupta, Sayan Feng, Jun Chan, Leanne Jade G. Petzold, Christopher J. Ralston, Corie Y. TI Synchrotron X-ray footprinting as a method to visualize water in proteins SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE bound water; hydroxyl radical labeling; mass spectrometry; protein conformation; protein modification ID STRUCTURAL MASS-SPECTROMETRY; MOLECULAR-DYNAMICS SIMULATIONS; ZINC TRANSPORTER YIIP; HEART CYTOCHROME-C; NEUTRON-SCATTERING; CRYSTAL-STRUCTURE; RADICAL PROBE; ELECTROSPRAY-IONIZATION; 3-DIMENSIONAL STRUCTURE; HYDRATION DYNAMICS AB The vast majority of biomolecular processes are controlled or facilitated by water interactions. In enzymes, regulatory proteins, membrane-bound receptors and ion-channels, water bound to functionally important residues creates hydrogen-bonding networks that underlie the mechanism of action of the macromolecule. High-resolution X-ray structures are often difficult to obtain with many of these classes of proteins because sample conditions, such as the necessity of detergents, often impede crystallization. Other biophysical techniques such as neutron scattering, nuclear magnetic resonance and Fourier transform infrared spectroscopy are useful for studying internal water, though each has its own advantages and drawbacks, and often a hybrid approach is required to address important biological problems associated with proteinwater interactions. One major area requiring more investigation is the study of bound water molecules which reside in cavities and channels and which are often involved in both the structural and functional aspects of receptor, transporter and ion channel proteins. In recent years, significant progress has been made in synchrotron-based radiolytic labeling and mass spectroscopy techniques for both the identification of bound waters and for characterizing the role of water in protein conformational changes at a high degree of spatial and temporal resolution. Here the latest developments and future capabilities of this method for investigating water-protein interactions and its synergy with other synchrotron-based methods are discussed. C1 [Gupta, Sayan; Ralston, Corie Y.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. [Feng, Jun] Lawrence Berkeley Natl Lab, Expt Syst, Adv Light Source, Berkeley, CA 94720 USA. [Chan, Leanne Jade G.; Petzold, Christopher J.] Lawrence Berkeley Natl Lab, Biol Syst & Engn, Berkeley, CA 94720 USA. RP Ralston, CY (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. EM cyralston@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; NIBIB [P30-EB0966]; Welcome Trust; NIH; DOE; Office of Science, Office of Biological and Environmental Research, US DOE [DE-AC02-05CH11231] FX We thank Rich Celestre for help with the studies performed at the Advanced Light Source. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. The National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The Center for Synchrotron Biosciences at the National Synchrotron Light Sources is supported by NIBIB under P30-EB0966. Studies on potassium channel work are supported by the Welcome Trust. Studies on YiiP are supported by NIH and DOE. Study on OCP is supported by NIH and DOE. This research used resources of the Joint BioEnergy Institute supported by the Office of Science, Office of Biological and Environmental Research, US DOE under contract DE-AC02-05CH11231. NR 102 TC 0 Z9 0 U1 9 U2 9 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1056 EP 1069 DI 10.1107/S1600577516009024 PN 5 PG 14 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500001 PM 27577756 ER PT J AU Dufresne, EM Dunford, RW Kanter, EP Gao, Y Moon, S Walko, DA Zhang, XS AF Dufresne, Eric M. Dunford, Robert W. Kanter, Elliot P. Gao, Yuan Moon, Seoksu Walko, Donald A. Zhang, Xusheng TI Pink-beam focusing with a one-dimensional compound refractive lens SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE compound refractive lenses; pink beam; chromatic aberration ID RESOLVED SYNCHROTRON EXPERIMENTS AB The performance of a cooled Be compound refractive lens (CRL) has been tested at the Advanced Photon Source (APS) to enable vertical focusing of the pink beam and permit the X-ray beam to spatially overlap with an 80 mu m-high low-density plasma that simulates astrophysical environments. Focusing the fundamental harmonics of an insertion device white beam increases the APS power density; here, a power density as high as 500 W mm(-2) was calculated. A CRL is chromatic so it does not efficiently focus X-rays whose energies are above the fundamental. Only the fundamental of the undulator focuses at the experiment. A two-chopper system reduces the power density on the imaging system and lens by four orders of magnitude, enabling imaging of the focal plane without any X-ray filter. A method to measure such high power density as well as the performance of the lens in focusing the pink beam is reported. C1 [Dufresne, Eric M.; Dunford, Robert W.; Kanter, Elliot P.; Gao, Yuan; Moon, Seoksu; Walko, Donald A.; Zhang, Xusheng] Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA. RP Dufresne, EM (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA. EM dufresne@anl.gov OI Dufresne, Eric/0000-0002-2077-4754 FU US DOE [DE-AC02-06CH11357] FX The authors wish to thank Harold Gibson for technical support. This work was performed on the APS 7-ID beamline. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under contract No. DE-AC02-06CH11357. NR 12 TC 0 Z9 0 U1 5 U2 5 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1082 EP 1086 DI 10.1107/S1600577516009310 PN 5 PG 5 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500004 PM 27577759 ER PT J AU Zhou, L Huang, L Bouet, N Kaznatcheev, K Vescovi, M Dai, YF Li, SY Idir, M AF Zhou, Lin Huang, Lei Bouet, Nathalie Kaznatcheev, Konstantine Vescovi, Matthew Dai, Yifan Li, Shengyi Idir, Mourad TI New figuring model based on surface slope profile for grazing-incidence reflective optics SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE ion beam figuring; synchrotron optics; one-dimensional; surface slope ID MEASURING MACHINE; MIRRORS AB Surface slope profile is widely used in the metrology of grazing-incidence reflective optics instead of surface height profile. Nevertheless, the theoretical and experimental model currently used in deterministic optical figuring processes is based on surface height, not on surface slope. This means that the raw slope profile data from metrology need to be converted to height profile to perform the current height-based figuring processes. The inevitable measurement noise in the raw slope data will introduce significant cumulative error in the resultant height profiles. As a consequence, this conversion will degrade the determinism of the figuring processes, and will have an impact on the ultimate surface figuring results. To overcome this problem, an innovative figuring model is proposed, which directly uses the raw slope profile data instead of the usual height data as input for the deterministic process. In this paper, first the influence of the measurement noise on the resultant height profile is analyzed, and then a new model is presented; finally a demonstration experiment is carried out using a one-dimensional ion beam figuring process to demonstrate the validity of our approach. C1 [Zhou, Lin; Dai, Yifan; Li, Shengyi] Natl Univ Def Technol, Coll Mechatron Engn & Automat, 109 Deya Rd, Changsha 410073, Hunan, Peoples R China. [Zhou, Lin; Huang, Lei; Bouet, Nathalie; Kaznatcheev, Konstantine; Vescovi, Matthew; Idir, Mourad] Brookhaven Natl Lab, NSLS 2, POB 5000, Upton, NY 11973 USA. [Zhou, Lin; Dai, Yifan; Li, Shengyi] Hunan Key Lab Ultraprecis Machining Technol, 47 Yanzheng St, Changsha 410073, Hunan, Peoples R China. RP Idir, M (reprint author), Brookhaven Natl Lab, NSLS 2, POB 5000, Upton, NY 11973 USA. EM midir@bnl.gov FU US Department of Energy, Office of Science, Office of Basic Energy sciences [DE-AC-02-98CH10886]; National Natural Science Foundation of China [91323302]; Program for New Century Excellent Talents in University [NCET-13-0165] FX This work was supported by the US Department of Energy, Office of Science, Office of Basic Energy sciences, under contract No. DE-AC-02-98CH10886. LZ was supported by the National Natural Science Foundation of China (No. 91323302) and the Program for New Century Excellent Talents in University (No. NCET-13-0165). The authors acknowledge Ray Conley for his support during the beginning of this project. NR 18 TC 0 Z9 0 U1 5 U2 5 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1087 EP 1090 DI 10.1107/S1600577516010882 PN 5 PG 4 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500005 ER PT J AU Stoupin, S Antipov, S Butler, JE Kolyadin, AV Katrusha, A AF Stoupin, Stanislav Antipov, Sergey Butler, James E. Kolyadin, Alexander V. Katrusha, Andrey TI Large-surface-area diamond (111) crystal plates for applications in high-heat-load wavefront-preserving X-ray crystal optics SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE X-ray monochromator; high heat load; diamond crystal; wavefront preservation ID MONOCHROMATOR; RESOLUTION; BEAMLINE AB Fabrication and results of high-resolution X-ray topography characterization of diamond single-crystal plates with large surface area (10 mm x 10 mm) and (111) crystal surface orientation for applications in high-heat-load X-ray crystal optics are reported. The plates were fabricated by laser-cutting of the (111) facets of diamond crystals grown using high-pressure high-temperature methods. The intrinsic crystal quality of a selected 3 mm x 7 mm crystal region of one of the studied samples was found to be suitable for applications in wavefront-preserving high-heat-load crystal optics. Wavefront characterization was performed using sequential X-ray diffraction topography in the pseudo plane wave configuration and data analysis using rocking-curve topography. The variations of the rocking-curve width and peak position measured with a spatial resolution of 13 mu m x 13 mu m over the selected region were found to be less than 1 mu rad. C1 [Stoupin, Stanislav] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Antipov, Sergey; Butler, James E.] Euclid Techlabs LLC, Solon, OH USA. [Kolyadin, Alexander V.; Katrusha, Andrey] New Diamond Technol LLC, St Petersburg, Russia. RP Stoupin, S (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM sstoupin@aps.anl.gov RI Butler, James/B-7965-2008 OI Butler, James/0000-0002-4794-7176 FU US Department of Energy, Office of Science [DE-AC02-06CH11357] FX K. Lang, R. Woods and J. Kirchman are acknowledged for technical support of the X-ray topography experiments. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 22 TC 0 Z9 0 U1 6 U2 6 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1118 EP 1123 DI 10.1107/S1600577516011796 PN 5 PG 6 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500010 PM 27577765 ER PT J AU Jones, MWM Phillips, NW van Riessen, GA Abbey, B Vine, DJ Nashed, YSG Mudie, ST Afshar, N Kirkham, R Chen, B Balaur, E de Jonge, MD AF Jones, Michael W. M. Phillips, Nicholas W. van Riessen, Grant A. Abbey, Brian Vine, David J. Nashed, Youssef S. G. Mudie, Stephen T. Afshar, Nader Kirkham, Robin Chen, Bo Balaur, Eugeniu de Jonge, Martin D. TI Simultaneous X-ray fluorescence and scanning X-ray diffraction microscopy at the Australian Synchrotron XFM beamline SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE X-ray fluorescence; scanning X-ray diffraction microscopy; ptychography ID PTYCHOGRAPHY; RESOLUTION; METALS AB Owing to its extreme sensitivity, quantitative mapping of elemental distributions via X-ray fluorescence microscopy (XFM) has become a key microanalytical technique. The recent realisation of scanning X-ray diffraction microscopy (SXDM) meanwhile provides an avenue for quantitative super-resolved ultra-structural visualization. The similarity of their experimental geometries indicates excellent prospects for simultaneous acquisition. Here, in both stepand fly-scanning modes, robust, simultaneous XFM-SXDM is demonstrated. C1 [Jones, Michael W. M.; Mudie, Stephen T.; Afshar, Nader; de Jonge, Martin D.] Australian Synchrotron, 800 Blackburn Rd, Clayton, Vic 3168, Australia. [Jones, Michael W. M.; Phillips, Nicholas W.; Abbey, Brian; Chen, Bo; Balaur, Eugeniu] La Trobe Univ, La Trobe Inst Mol Sci, ARC Ctr Excellence Adv Mol Imaging, Bundoora, Vic 3086, Australia. [Phillips, Nicholas W.] CSIRO Mfg, Parkville, Vic 3052, Australia. [van Riessen, Grant A.] La Trobe Univ, Dept Chem & Phys, La Trobe Inst Mol Sci, Bundoora, Vic 3086, Australia. [Vine, David J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Nashed, Youssef S. G.] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA. [Kirkham, Robin] CSIRO Mfg, Clayton, Vic 3168, Australia. [Jones, Michael W. M.] Queensland Univ Technol, Fac Hlth, Brisbane, Qld 4000, Australia. [Jones, Michael W. M.] Queensland Univ Technol, Inst Hlth & Biomed Innovat, Brisbane, Qld 4000, Australia. RP Jones, MWM; de Jonge, MD (reprint author), Australian Synchrotron, 800 Blackburn Rd, Clayton, Vic 3168, Australia.; Jones, MWM (reprint author), La Trobe Univ, La Trobe Inst Mol Sci, ARC Ctr Excellence Adv Mol Imaging, Bundoora, Vic 3086, Australia.; Jones, MWM (reprint author), Queensland Univ Technol, Fac Hlth, Brisbane, Qld 4000, Australia.; Jones, MWM (reprint author), Queensland Univ Technol, Inst Hlth & Biomed Innovat, Brisbane, Qld 4000, Australia. EM mw.jones@qut.edu.au; martin.dejonge@synchrotron.org.au RI van Riessen, Grant/H-3840-2011 OI van Riessen, Grant/0000-0002-6240-7143 FU Multi-modal Australian ScienceS Imaging and Visualization Environment (MASSIVE); Australian Research Council (ARC) Centre of Excellence for Advanced Molecular Imaging FX We thank Dectris Ltd, Baden, Switzerland, for loan of the EIGER X 1M detector. This research was undertaken on the XFM beamline at the Australian Synchrotron, Victoria, Australia, and supported by the Multi-modal Australian ScienceS Imaging and Visualization Environment (MASSIVE) (http://www.massive.org.au). The authors acknowledge the support of the Australian Research Council (ARC) Centre of Excellence for Advanced Molecular Imaging. This work was performed in part at the Melbourne Centre for Nanofabrication (MCN) in the Victorian Node of the Australian National Fabrication Facility (ANFF). NR 30 TC 0 Z9 0 U1 1 U2 1 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1151 EP 1157 DI 10.1107/S1600577516011917 PN 5 PG 7 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500015 PM 27577770 ER PT J AU Chen, YY Sanchez, C Yue, Y Gonzalez, JM Parkinson, DY Liang, H AF Chen, Yunyun Sanchez, Carlos Yue, Yuan Gonzalez, Jorge M. Parkinson, Dilworth Y. Liang, Hong TI Observation of two-dimensional yttrium oxide nanoparticles in mealworm beetles (Tenebrio molitor) SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE synchrotron X-ray micro-tomography; K-edge subtraction; yttrium oxide nanoparticles; mealworms; particle distribution ID TROPHIC TRANSFER; TOMOGRAPHY AB Nanomaterials are being used in medicine, manufacturing and consumer products, but their effects on organisms and the environment are not well understood because of the difficulty in detecting them. Here dual-energy X-ray K-edge subtraction was used to track two-dimensional yttrium oxide nanoparticles (which can be found in such household objects as color televisions) in adult mealworms (Tenebrio molitor). The insects ingested nanoparticle-infused feed for different time periods, up to 24 h, and the nanoparticles could then be identified at several locations in the insects' head, thorax and abdomen, mostly within the digestive tract. In time, all particles were excreted. C1 [Chen, Yunyun; Yue, Yuan; Liang, Hong] Texas A&M Univ, Mat Sci & Engn, MS 3123, College Stn, TX 77843 USA. [Sanchez, Carlos; Liang, Hong] Texas A&M Univ, Mech Engn, MS 3123, College Stn, TX 77843 USA. [Gonzalez, Jorge M.] Calif State Univ Fresno, Dept Plant Sci, Fresno, CA 93740 USA. [Parkinson, Dilworth Y.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Liang, H (reprint author), Texas A&M Univ, Mat Sci & Engn, MS 3123, College Stn, TX 77843 USA.; Liang, H (reprint author), Texas A&M Univ, Mech Engn, MS 3123, College Stn, TX 77843 USA. EM hliang@tamu.edu RI Yue, Yuan/F-2177-2017 FU ALS fellowship; Provost's Assigned Time for Research; California State University Fresno; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX YYC was partially sponsored by an ALS fellowship. JMG was supported by the Provost's Assigned Time for Research (Summer 2015) and California State University Fresno, Research, Scholarship and Creative proposal Awarded (2014-2015). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. YYC, CS, YY and JMG conducted the experiments; YYC and JMG analyzed the data; DYP and HL designed the experiments; YYC, JMG, DYP and HL wrote the paper. All authors reviewed the manuscript. Authors state no competing financial interests. NR 24 TC 1 Z9 1 U1 7 U2 7 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1197 EP 1201 DI 10.1107/S1600577516009942 PN 5 PG 5 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500020 PM 27577775 ER PT J AU Logan, J Harder, R Li, LX Haskel, D Chen, P Winarski, R Fuesz, P Schlagel, D Vine, D Benson, C McNulty, I AF Logan, Jonathan Harder, Ross Li, Luxi Haskel, Daniel Chen, Pice Winarski, Robert Fuesz, Peter Schlagel, Deborah Vine, David Benson, Christa McNulty, Ian TI Hard X-ray polarizer to enable simultaneous three-dimensional nanoscale imaging of magnetic structure and lattice strain SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE Bragg coherent diffractive imaging; XMCD; nanomagnetism; strain ID CRYSTALS AB Recent progress in the development of dichroic Bragg coherent diffractive imaging, a new technique for simultaneous three-dimensional imaging of strain and magnetization at the nanoscale, is reported. This progress includes the installation of a diamond X-ray phase retarder at beamline 34-ID-C of the Advanced Photon Source. The performance of the phase retarder for tuning X-ray polarization is demonstrated with temperature-dependent X-ray magnetic circular dichroism measurements on a gadolinium foil in transmission and on a Gd5Si2Ge2 crystal in diffraction geometry with a partially coherent, focused X-ray beam. Feasibility tests for dichroic Bragg coherent diffractive imaging are presented. These tests include (1) using conventional Bragg coherent diffractive imaging to determine whether the phase retarder introduces aberrations using a nonmagnetic gold nanocrystal as a control sample, and (2) collecting coherent diffraction patterns of a magnetic Gd5Si2Ge2 nanocrystal with left- and right-circularly polarized X-rays. Future applications of dichroic Bragg coherent diffractive imaging for the correlation of strain and lattice defects with magnetic ordering and inhomogeneities are considered. C1 [Logan, Jonathan; Winarski, Robert; McNulty, Ian] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60439 USA. [Harder, Ross; Li, Luxi; Haskel, Daniel; Fuesz, Peter; Benson, Christa] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. [Chen, Pice] Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. [Schlagel, Deborah] Ames Lab, Div Mat Sci & Engn, 2405 Kooser Dr, Ames, IA 50011 USA. [Vine, David] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Logan, J (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60439 USA. EM jmlogan@anl.gov OI Chen, Pice/0000-0003-4401-5637; Logan, Jonathan/0000-0003-2554-9457 FU Center for Nanoscale Materials, a US Department of Energy Office of Science User Facility [DE-AC02-06CH11357]; US Department of Energy Office of Science User Facility [DE-AC02-06CH11357]; [DE-AC02-07CH11358] FX Gd5Si2Ge2 single-crystal preparation was performed at the Ames Laboratory. Ames Laboratory is operated by Iowa State University under contract No DE-AC02-07CH11358. We would like to thank Vitalij Pecharsky for reading the manuscript and offering useful suggestions. We would also like to thank Carlos Giles, Zahirul Islam and Jonathan Lang for helpful discussions, and Dan Legnini and Huyue Zhao for engineering support. This work was performed, in part, at the Center for Nanoscale Materials, a US Department of Energy Office of Science User Facility under contract No. DE-AC02-06CH11357. This research used resources of the Advanced Photon Source, a US Department of Energy Office of Science User Facility operated by Argonne National Laboratory under contract No. DE-AC02-06CH11357. NR 18 TC 0 Z9 0 U1 4 U2 5 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1210 EP 1215 DI 10.1107/S1600577516009632 PN 5 PG 6 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500022 PM 27577777 ER PT J AU Cha, W Liu, WJ Harder, R Xu, RQ Fuoss, PH Hruszkewycz, SO AF Cha, Wonsuk Liu, Wenjun Harder, Ross Xu, Ruqing Fuoss, Paul H. Hruszkewycz, Stephan O. TI Utilizing broadband X-rays in a Bragg coherent X-ray diffraction imaging experiment SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE coherent X-ray diffraction imaging; polychromatic X-ray diffraction; materials characterization ID MICRODIFFRACTION AB A method is presented to simplify Bragg coherent X-ray diffraction imaging studies of complex heterogeneous crystalline materials with a two-stage screening/imaging process that utilizes polychromatic and monochromatic coherent X-rays and is compatible with in situ sample environments. Coherent white-beam diffraction is used to identify an individual crystal particle or grain that displays desired properties within a larger population. A three-dimensional reciprocal-space map suitable for diffraction imaging is then measured for the Bragg peak of interest using a monochromatic beam energy scan that requires no sample motion, thus simplifying in situ chamber design. This approach was demonstrated with Au nanoparticles and will enable, for example, individual grains in a polycrystalline material of specific orientation to be selected, then imaged in three dimensions while under load. C1 [Cha, Wonsuk; Fuoss, Paul H.; Hruszkewycz, Stephan O.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. [Liu, Wenjun; Harder, Ross; Xu, Ruqing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Hruszkewycz, SO (reprint author), Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. EM shrus@anl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work, including use of the Advanced Photon Source, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. PHF and SOH were supported by US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 9 TC 1 Z9 1 U1 7 U2 7 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD SEP PY 2016 VL 23 BP 1241 EP 1244 DI 10.1107/S1600577516010523 PN 5 PG 4 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DU6CA UT WOS:000382299500027 ER PT J AU Knapik, JJ Trone, DW Austin, KG Steelman, RA Farina, EK Lieberman, HR AF Knapik, Joseph J. Trone, Daniel W. Austin, Krista G. Steelman, Ryan A. Farina, Emily K. Lieberman, Harris R. TI Prevalence, Adverse Events, and Factors Associated with Dietary Supplement and Nutritional Supplement Use by US Navy and Marine Corps Personnel SO JOURNAL OF THE ACADEMY OF NUTRITION AND DIETETICS LA English DT Article DE Vitamin; Mineral; Prohormone; Sport drinks; Sport bars/gels ID ACUTE LIVER-INJURY; WEIGHT-LOSS; UNITED-STATES; GENDER-DIFFERENCES; NATIONAL-HEALTH; NO-XPLODE; CARE UTILIZATION; ACUTE HEPATITIS; OXYELITE PRO; HYDROXYCUT AB Background About 50% of Americans and 60% to 70% of US military personnel use dietary supplements, some of which have been associated with adverse events (AEs). Nutritional supplements like sport drinks and sport bars/gels are also commonly used by athletes and service members. Previous dietary supplement and nutritional supplement surveys were conducted on Army, Air Force, and Coast Guard personnel. Objective The aim of this cross-sectional study was to investigate dietary and nutritional supplement use in Navy and Marine Corps personnel, including the prevalence, types, factors associated with use, and AEs. Design A random sample of 10,000 Navy and Marine Corps personnel were contacted. Service members were asked to complete a detailed questionnaire describing their personal characteristics, supplement use, and AEs experienced. Results In total, 1,708 service members completed the questionnaire during August through December 2014, with 1,683 used for analysis. Overall, 73% reported using dietary supplements one or more times per week. The most commonly used dietary supplements (used one or more times per week) were multivitamins/multiminerals (48%), protein/amino acids (34%), combination products (33%), and individual vitamins and minerals (29%). About 31% of service members reported using five or more dietary supplements. Sport drinks and sport bars/gels were used by 45% and 23% of service members, respectively. Monthly expenditures on dietary supplements averaged $39; 31% of service members spent >=$50/mo. Multivariate logistic regression modeling indicated that female sex (women/men; odds ratio [OR]=1.76, 95% CI 1.32 to 2.36), higher educational level (college degree/no college degree; OR=2.23, 95% CI 1.62 to 3.30), higher body mass index (calculated as kg/m(2)) (>= 30/<25; OR=1.67, 95% CI 1.06 to 2.63), and a greater amount of resistance training (>= 271/0 to 45 min/week; OR=2.85, 95% CI 1.94 to 4.17) were associated with dietary supplement use. Twenty-two percent of dietary supplement users and 6% of nutritional supplement users reported one or more AEs. For combination products alone, 29% of users reported one or more AEs. Conclusions The prevalence of dietary supplement use in Navy and Marine Corps personnel was considerably higher than reported in civilian investigations for almost all types of dietary supplements, although similar to most other military services. Factors associated with dietary supplement use were similar to those reported in previous military and civilian investigations. Prevalence of self-reported AEs was very high, especially for combination products. C1 [Knapik, Joseph J.; Austin, Krista G.; Farina, Emily K.; Lieberman, Harris R.] US Army Res Inst Environm Med, Mil Nutr Div, 10 Gen Greene Ave, Natick, MA 01760 USA. [Knapik, Joseph J.; Steelman, Ryan A.] US Army Publ Hlth Ctr, Aberdeen Proving Ground, MD USA. [Knapik, Joseph J.; Austin, Krista G.; Farina, Emily K.] Oak Ridge Inst Sci & Educ, Belcamp, MD USA. [Trone, Daniel W.] Naval Hlth Res Ctr, San Diego, CA USA. RP Knapik, JJ (reprint author), US Army Res Inst Environm Med, Mil Nutr Div, 10 Gen Greene Ave, Natick, MA 01760 USA. EM joseph.j.knapik.ctr@mail.mil FU Knowledge Preservation Program at the US Army Research Institute of Environmental Medicine (USARIEM); Army Institute of Public Health (AIPH); Center Alliance for Nutrition and Dietary Supplement Research FX This research was supported in part by an appointment to the Knowledge Preservation Program at the US Army Research Institute of Environmental Medicine (USARIEM) and the Army Institute of Public Health (AIPH) administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the US Department of Energy and USARIEM. Funding was also provided by the Center Alliance for Nutrition and Dietary Supplement Research. NR 81 TC 2 Z9 2 U1 9 U2 9 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 2212-2672 EI 2212-2680 J9 J ACAD NUTR DIET JI J. Acad. Nutr. Diet. PD SEP PY 2016 VL 116 IS 9 BP 1423 EP 1442 DI 10.1016/j.jand.2016.02.015 PG 20 WC Nutrition & Dietetics SC Nutrition & Dietetics GA DU8QH UT WOS:000382478300009 PM 27083989 ER PT J AU Aubry, S Rhee, M Hommes, G Bulatov, VV Arsenlis, A AF Aubry, S. Rhee, M. Hommes, G. Bulatov, V. V. Arsenlis, A. TI Dislocation dynamics in hexagonal close-packed crystals SO JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS LA English DT Article DE Dislocation dynamics; Hexagonal close-packed; Composites dislocations ID HCP METALS; SLIP SYSTEMS; SIMULATIONS; MAGNESIUM; ALLOYS; DEFORMATION; JUNCTIONS; STRENGTH AB Extensions of the dislocation dynamics methodology necessary to enable accurate simulations of crystal plasticity in hexagonal close-packed (HCP) metals are presented. They concern the introduction of dislocation motion in HCP crystals through linear and nonlinear mobility laws, as well as the treatment of composite dislocation physics. Formation, stability and dissociation of < c + a > and other dislocations with large Burgers vectors defined as composite dislocations are examined and a new topological operation is proposed to enable their dissociation. The results of our simulations suggest that composite dislocations are omnipresent and may play important roles both in specific dislocation mechanisms and in bulk crystal plasticity in HCP materials. While fully microscopic, our bulk DD simulations provide wealth of data that can be used to develop and parameterize constitutive models of crystal plasticity at the mesoscale. Published by Elsevier Ltd. C1 [Aubry, S.; Rhee, M.; Hommes, G.; Bulatov, V. V.; Arsenlis, A.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RP Aubry, S (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Army Research Laboratory [W911NF-12-2-0022] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Also, research was sponsored by the Army Research Laboratory and was accomplished under cooperative agreement number W911NF-12-2-0022. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing the official policies, either expressed or implied, of the Army Research Laboratory or the U.S. Government. The U.S. Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. NR 33 TC 0 Z9 0 U1 11 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-5096 EI 1873-4782 J9 J MECH PHYS SOLIDS JI J. Mech. Phys. Solids PD SEP PY 2016 VL 94 BP 105 EP 126 DI 10.1016/j.jmps.2016.04.019 PG 22 WC Materials Science, Multidisciplinary; Mechanics; Physics, Condensed Matter SC Materials Science; Mechanics; Physics GA DU6RM UT WOS:000382342300007 ER PT J AU Runnels, B Beyerlein, IJ Conti, S Ortiz, M AF Runnels, Brandon Beyerlein, Irene J. Conti, Sergio Ortiz, Michael TI A relaxation method for the energy and morphology of grain boundaries and interfaces SO JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS LA English DT Article ID FCC METALS; BCC METALS; PLASTIC-DEFORMATION; CRYSTAL-SURFACES; 100 PLANES; COPPER; GROWTH AB The energy density of crystal interfaces exhibits a characteristic "cusp" structure that renders it non-convex. Furthermore, crystal interfaces are often observed to be faceted, i.e., to be composed of flat facets in alternating directions. In this work, we forge a connection between these two observations by positing that the faceted morphology of crystal interfaces results from energy minimization. Specifically, we posit that the lack of convexity of the interfacial energy density drives the development of finely faceted microstructures and accounts for their geometry and morphology. We formulate the problem as a generalized minimal surface problem couched in a geometric measure-theoretical framework. We then show that the effective, or relaxed, interfacial energy density, with all possible interfacial morphologies accounted for, corresponds to the convexification of the bare or unrelaxed interfacial energy density, and that the requisite convexification can be attained by means of a faceting construction. We validate the approach by means of comparisons with experiment and atomistic simulations including symmetric and asymmetric tilt boundaries in face-centered cubic (FCC) and body-centered cubic (BCC) crystals. By comparison with simulated and experimental data, we show that this simple model of interfacial energy combined with a general microstructure construction based on convexification is able to replicate complex interfacial morphologies, including thermally induced morphological transitions. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Runnels, Brandon; Ortiz, Michael] CALTECH, Div Engn & Appl Sci, 1200 E Calif Blvd, Pasadena, CA 91125 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. [Conti, Sergio] Univ Bonn, Inst Angew Math, D-53115 Bonn, Germany. RP Ortiz, M (reprint author), CALTECH, Div Engn & Appl Sci, 1200 E Calif Blvd, Pasadena, CA 91125 USA. OI Runnels, Brandon/0000-0003-3043-5227; Conti, Sergio/0000-0001-7987-9174 FU NNSA's High Energy Density Laboratory Plasmas program [DE-NA0001805]; Los Alamos National Laboratory Seaborg Institute; Laboratory Directed Research and Development program [20140348ER]; DFG [SFB 1060] FX Brandon Runnels and Michael Ortiz would like to thank the NNSA's High Energy Density Laboratory Plasmas program under award #DE-NA0001805. Brandon Runnels additionally thanks the Los Alamos National Laboratory Seaborg Institute for support during Summer 2014. Irene Beyerlein would like to acknowledge support by a Laboratory Directed Research and Development program award number 20140348ER. Sergio Conti would like to acknowledge support of the DFG under SFB 1060. NR 46 TC 1 Z9 1 U1 7 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-5096 EI 1873-4782 J9 J MECH PHYS SOLIDS JI J. Mech. Phys. Solids PD SEP PY 2016 VL 94 BP 388 EP 408 DI 10.1016/j.jmps.2015.11.007 PG 21 WC Materials Science, Multidisciplinary; Mechanics; Physics, Condensed Matter SC Materials Science; Mechanics; Physics GA DU6RM UT WOS:000382342300022 ER PT J AU Finnell, J AF Finnell, Joshua TI Nutshell SO LIBRARY JOURNAL LA English DT Book Review C1 [Finnell, Joshua] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Finnell, J (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. NR 1 TC 0 Z9 0 U1 0 U2 0 PU REED BUSINESS INFORMATION PI NEW YORK PA 360 PARK AVENUE SOUTH, NEW YORK, NY 10010 USA SN 0363-0277 J9 LIBR J JI Libr. J. PD SEP 1 PY 2016 VL 141 IS 14 BP 100 EP 100 PG 1 WC Information Science & Library Science SC Information Science & Library Science GA DV0IX UT WOS:000382602300141 ER PT J AU O'Bryhim, JR Parsons, ECM Gilmore, MP Lance, SL AF O'Bryhim, Jason R. Parsons, E. C. M. Gilmore, Michael P. Lance, Stacey L. TI Evaluating support for shark conservation among artisanal fishing communities in Costa Rica SO MARINE POLICY LA English DT Article DE Artisanal fishermen; Conservation; Sharks; Potential behaviors; Social surveys ID TRADITIONAL ECOLOGICAL KNOWLEDGE; FISHERIES; MANAGEMENT; SCIENCE; MARINE; TRADE AB Many shark populations have experienced severe declines in the past few decades due to increased demand for their products. As fisheries managers, conservation biologists, and other invested groups move to develop new conservation measures to better protect sharks it will be important to understand the potential reactions (behaviors) local fishermen will have to new regulations. To determine the potential behaviors local artisanal fishermen in Costa Rica would have toward new conservation measures for sharks a structured survey (n=72) was distributed to several fishing communities along Costa Rica's Pacific coast. Overall, 89% of fishermen felt that protecting sharks was important with 97% stating a willingness to support shark conservation. However, support dropped to 67% if they would have to change some of their fishing practices. Almost all fishermen surveyed (93%) were in support of the formation of marine protected areas (MPAs). Although, if MPAs restricted their current fishing practices support dropped to between 6% and 65% depending on the restrictiveness of regulations implemented in the MPA. The majority (86%) of the fishermen surveyed also indicated they would be more likely to support new legislative measures to protect sharks if they were included in the decision making process. The results suggest that artisanal fishermen in Costa Rica are willing to protect sharks, but only if their current fishing practices are minimally impacted. It is therefore important that mangers work with these communities to develop management plans that will provide the best protection possible for sharks while also garnering local support to ensure continued compliance. (C) 2016 Elsevier Ltd. All rights reserved. C1 [O'Bryhim, Jason R.; Parsons, E. C. M.] George Mason Univ, Dept Environm Sci & Policy, Fairfax, VA 22030 USA. [O'Bryhim, Jason R.; Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Gilmore, Michael P.] George Mason Univ, Sch Integrat Studies, Fairfax, VA 22030 USA. RP O'Bryhim, JR (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM jobryhim@gmail.com FU Rufford Foundation, United Kingdom [13921-1]; George Mason University, United States; Explorers Club Washington Group Exploration and Field Research Grant Program; Department of Energy, United States [DE-FC09-07SR22506]; George Mason University Human Subjects Review Board [8665] FX We would like to thank everyone in Costa Rica who helped make this research possible including: Dr. Ted Bradley, Randall Arauz, Maike Heidemeyer, Andy Bystrom, Taylor Clarke, Dr. Ingo Wehrtmann, PRETOMA, the University of Costa Rica, and the fishermen who were willing to participate in this research. We also would like to thank Chelsie Romulo for producing the map for this paper. Finally, we would like to thank the Rufford Foundation, United Kingdom (ref. number 13921-1) for being the main funding agency of this research as well as George Mason University, United States and the Explorers Club Washington Group Exploration and Field Research Grant Program for financial assistance. This research was also partially supported by the Department of Energy, United States under Award number DE-FC09-07SR22506 to the University of Georgia Research Foundation. Permission to conduct this research was granted by the George Mason University Human Subjects Review Board (Protocol #8665). NR 39 TC 0 Z9 0 U1 15 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0308-597X EI 1872-9460 J9 MAR POLICY JI Mar. Pol. PD SEP PY 2016 VL 71 BP 1 EP 9 DI 10.1016/j.marpol.2016.05.005 PG 9 WC Environmental Studies; International Relations SC Environmental Sciences & Ecology; International Relations GA DT6KT UT WOS:000381593800001 ER PT J AU Panova, O Chen, XC Bustillo, KC Ophus, C Bhatt, MP Balsara, N Minor, AM AF Panova, Ouliana Chen, X. Chelsea Bustillo, Karen C. Ophus, Colin Bhatt, Mahesh P. Balsara, Nitash Minor, Andrew M. TI Orientation mapping of semicrystalline polymers using scanning electron nanobeam diffraction SO MICRON LA English DT Article DE TEM; STEM; Spatially resolved; Diffraction; Crystal orientation; P3HT; Polymers; Locally resolved structure ID STRUCTURAL FEATURES; CRYSTAL-STRUCTURE; RADIATION-DAMAGE; MOLECULAR-WEIGHT; THIN-FILMS; POLY(3-HEXYLTHIOPHENE); MICROSCOPY; P3HT; POLY(3-ALKYLTHIOPHENES); MICROSTRUCTURE AB We demonstrate a scanning electron nanobeam diffraction technique that can be used for mapping the size and distribution of nanoscale crystalline regions in a polymer blend. In addition, it can map the relative orientation of crystallites and the degree of crystallinity of the material. The model polymer blend is a 50:50 w/w mixture of semicrystalline poly(3-hexylthiophene-2,5-diyl) (P3HT) and amorphous polystyrene (PS). The technique uses a scanning electron beam to raster across the sample and acquires a diffraction image at each probe position. Through image alignment and filtering, the diffraction image dataset enables mapping of the crystalline regions within the scanned area and construction of an orientation map. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Panova, Ouliana; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Panova, Ouliana; Bustillo, Karen C.; Ophus, Colin; Minor, Andrew M.] Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA USA. [Chen, X. Chelsea; Balsara, Nitash] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Chen, X. Chelsea; Bhatt, Mahesh P.; Balsara, Nitash] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA. [Bhatt, Mahesh P.; Balsara, Nitash] Lawrence Berkeley Natl Lab, Joint Ctr Energy Storage Res, Berkeley, CA USA. RP Minor, AM (reprint author), Univ Calif Berkeley, One Cyclotron Rd,MS 72, Berkeley, CA 94720 USA. EM aminor@lbl.gov FU Electron Microscopy of Soft Matter Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC02-05CH11231] FX Primary funding for the work was provided by the Electron Microscopy of Soft Matter Program from the Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The electron microscopy was performed as a user project at the Molecular Foundry at Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy under Contract # DE-AC02-05CH11231. We wish to thank Christoph Gammer for writing the custom scripts to drive the diffraction mapping acquisition. NR 45 TC 0 Z9 0 U1 13 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0968-4328 J9 MICRON JI Micron PD SEP PY 2016 VL 88 BP 30 EP 36 DI 10.1016/j.micron.2016.05.008 PG 7 WC Microscopy SC Microscopy GA DT5NZ UT WOS:000381531200005 PM 27323282 ER PT J AU Johnson, RH Tutu, H AF Johnson, Raymond H. Tutu, Hlanganani TI Predictive Reactive Transport Modeling at a Proposed Uranium In Situ Recovery Site with a General Data Collection Guide SO MINE WATER AND THE ENVIRONMENT LA English DT Article DE Geochemical modeling; PHREEQC; Batch sorption ID GROUND-WATER AB Restoration of uranium in situ recovery (ISR) sites to predevelopment conditions is often very difficult. Future downgradient groundwater geochemistry can be evaluated using reactive transport modeling coupled with appropriate data collection. U.S. regulatory requirements specify that the geochemistry at the aquifer exemption boundary should never be affected, but compliance with this regulation has not been monitored at previous ISR sites. At the Dewey Burdock site near Edgemont, SD, USA, a change in groundwater flow direction created a scenario in which the oxidized side of a U roll-front deposit is downgradient of the ore zone. This increases the potential for future U transport, since conventional understanding of U geochemistry is that the reduced side provides more natural attenuation. Reactive transport modeling using U sorption parameters from batch sorption tests provides a predictive tool for future U transport. Prediction variations were tested using two different samples, considering different reaction assumptions and possible pH measurement errors. The results indicate a large range in U transport predictions, with high sensitivity to sorption parameters due to sample heterogeneity, pH, and the presence or absence of calcite. While the sample data set for these initial predictions was limited, the results highlight the need for additional calibration points and a thorough understanding of rock/water interactions in the downgradient zone. We provide a general data collection guide for steps in evaluating downgradient transport at future U ISR sites. These steps include core sampling in the downgradient and restored zones, along with batch sorption and column testing with restored and background groundwater in contact with the restored zone solid phase. Final reactive transport modeling will rely on high-quality calibration data from batch and column testing (plus any available field testing), but thorough site evaluation will also require appropriate long-term monitoring. C1 [Johnson, Raymond H.] US DOE, Navarro Res & Engn, Off Legacy Management, 2597 Legacy Way, Grand Junction, CO 81503 USA. [Tutu, Hlanganani] Univ Witwatersrand WITS, Inst Mol Sci, Sch Chem, P Bag X3, ZA-2050 Johannesburg, South Africa. RP Johnson, RH (reprint author), US DOE, Navarro Res & Engn, Off Legacy Management, 2597 Legacy Way, Grand Junction, CO 81503 USA. EM ray.johnson@lm.doe.gov; hlanganani.tutu@wits.ac.za FU U.S. Department of Energy Office of Legacy Management; University of Witwatersrand, South Africa FX Funding for this work was provided by the U.S. Department of Energy Office of Legacy Management. Additional funding was provided by the University of Witwatersrand, South Africa. We also thank Dr. James Stone (South Dakota School of Mines and Technology), the journal editors and two anonymous journal reviewers for additional comments that helped improve this manuscript. NR 22 TC 0 Z9 0 U1 8 U2 8 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1025-9112 EI 1616-1068 J9 MINE WATER ENVIRON JI Mine Water Environ. PD SEP PY 2016 VL 35 IS 3 BP 369 EP 380 DI 10.1007/s10230-015-0376-y PG 12 WC Water Resources SC Water Resources GA DU4PB UT WOS:000382193900011 ER PT J AU Hochstrasser, ML Taylor, DW Kornfeld, JE Nogales, E Doudna, JA AF Hochstrasser, Megan L. Taylor, David W. Kornfeld, Jack E. Nogales, Eva Doudna, Jennifer A. TI DNA Targeting by a Minimal CRISPR RNA-Guided Cascade SO MOLECULAR CELL LA English DT Article ID IN-VITRO RECONSTITUTION; PROCESSES PRE-CRRNA; R-LOOP FORMATION; CAS SYSTEMS; SURVEILLANCE COMPLEX; ESCHERICHIA-COLI; IMMUNE-SYSTEM; CRYSTAL-STRUCTURE; FUNCTIONAL-CHARACTERIZATION; EFFECTOR COMPLEXES AB Bacteria employ surveillance complexes guided by CRISPR (clustered, regularly interspaced, short palindromic repeats) RNAs (crRNAs) to target foreign nucleic acids for destruction. Although most type I and type III CRISPR systems require four or more distinct proteins to form multi-subunit surveillance complexes, the type I-C systems use just three proteins to achieve crRNA maturation and double-stranded DNA target recognition. We show that each protein plays multiple functional and structural roles: Cas5c cleaves pre-crRNAs and recruits Cas7 to position the RNA guide for DNA binding and unwinding by Cas8c. Cryoelectron microscopy reconstructions of free and DNA-bound forms of the Cascade/I-C surveillance complex reveal conformational changes that enable R-loop formation with distinct positioning of each DNA strand. This streamlined type I-C system explains how CRISPR pathways can evolve compact structures that retain full functionality as RNA-guided DNA capture platforms. C1 [Hochstrasser, Megan L.; Taylor, David W.; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Taylor, David W.; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Kornfeld, Jack E.; Nogales, Eva; Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Nogales, Eva; Doudna, Jennifer A.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Taylor, David W.] Univ Texas Austin, Dept Mol Biosci, Austin, TX 78712 USA. RP Taylor, DW; Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Taylor, DW; Doudna, JA (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Taylor, DW (reprint author), Univ Texas Austin, Dept Mol Biosci, Austin, TX 78712 USA. EM dtaylor@utexas.edu; doudna@berkeley.edu FU Damon Runyon Cancer Research Foundation [DRG-2218-15] FX We thank R. Louder, A. Patel, E. Kellogg, P. Grob, T. Houweling, Z. Yu and C. Hong for expert electron microscopy assistance and S. Floor, P. Kranzusch, T. Liu, J. Nunez, S. Sternberg, S. Strutt, and R. Wilson for helpful discussions and critical reading of the manuscript. D.W.T. is a Damon Runyon Fellow supported by the Damon Runyon Cancer Research Foundation (DRG-2218-15). J.A.D and E.N. are Howard Hughes Medical Institute Investigators. J.A.D. is a co-founder of Editas Medicine, Intellia Therapeutics, and Caribou Biosciences and a scientific advisor to Caribou, Intellia, eFFECTOR Therapeutics, and Driver. NR 50 TC 1 Z9 1 U1 20 U2 27 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD SEP 1 PY 2016 VL 63 IS 5 BP 840 EP 851 DI 10.1016/j.molcel.2016.07.027 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DU9MO UT WOS:000382542000012 PM 27588603 ER PT J AU Voiry, D Fullon, R Yang, JE Silva, CDCE Kappera, R Bozkurt, I Kaplan, D Lagos, MJ Batson, PE Gupta, G Mohite, AD Dong, L Er, DQ Shenoy, VB Asefa, T Chhowalla, M AF Voiry, Damien Fullon, Raymond Yang, Jieun Castro e Silva, Cecilia de Carvalho Kappera, Rajesh Bozkurt, Ibrahim Kaplan, Daniel Lagos, Maureen J. Batson, Philip E. Gupta, Gautam Mohite, Aditya D. Dong, Liang Er, Dequan Shenoy, Vivek B. Asefa, Tewodros Chhowalla, Manish TI The role of electronic coupling between substrate and 2D MoS2 nanosheets in electrocatalytic production of hydrogen SO NATURE MATERIALS LA English DT Article ID AMORPHOUS MOLYBDENUM SULFIDE; ACTIVE EDGE SITES; EVOLUTION REACTION; 2-DIMENSIONAL SEMICONDUCTORS; CATALYTIC-ACTIVITY; DISULFIDE; TRANSISTORS; GRAPHENE; CONTACTS; DEFECTS AB The excellent catalytic activity of metallic MoS2 edges for the hydrogen evolution reaction (HER) has led to substantial efforts towards increasing the edge concentration. The 2H basal plane is less active for the HER because it is less conducting and therefore possesses less efficient charge transfer kinetics. Here we show that the activity of the 2H basal planes of monolayer MoS2 nanosheets can be made comparable to state-of-the-art catalytic properties of metallic edges and the 1T phase by improving the electrical coupling between the substrate and the catalyst so that electron injection from the electrode and transport to the catalyst active site is facilitated. Phase-engineered low-resistance contacts on monolayer 2H-phase MoS2 basal plane lead to higher efficiency of charge injection in the nanosheets so that its intrinsic activity towards the HER can be measured. We demonstrate that onset potentials and Tafel slopes of similar to-0.1 V and similar to 50 mV per decade can be achieved from 2H-phase catalysts where only the basal plane is exposed. We show that efficient charge injection and the presence of naturally occurring sulfur vacancies are responsible for the observed increase in catalytic activity of the 2H basal plane. Our results provide new insights into the role of contact resistance and charge transport on the performance of two-dimensional MoS2 nanosheet catalysts for the HER. C1 [Voiry, Damien; Fullon, Raymond; Yang, Jieun; Castro e Silva, Cecilia de Carvalho; Kappera, Rajesh; Bozkurt, Ibrahim; Lagos, Maureen J.; Batson, Philip E.; Chhowalla, Manish] Rutgers State Univ, Mat Sci & Engn, 607 Taylor Rd, Piscataway, NJ 08854 USA. [Kaplan, Daniel] US Army RDECOM ARDEC, Acoust & Networked Sensors Div, Picatinny Arsenal, NJ 07806 USA. [Lagos, Maureen J.; Batson, Philip E.] Rutgers State Univ, Dept Phys, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. [Lagos, Maureen J.; Batson, Philip E.] Rutgers State Univ, Inst Adv Mat Devices & Nanotechnol, 607 Taylor Rd, Piscataway, NJ 08854 USA. [Gupta, Gautam; Mohite, Aditya D.] Los Alamos Natl Lab, MPA Mat Synth & Integrated Devices 11, Los Alamos, NM 87545 USA. [Dong, Liang; Er, Dequan; Shenoy, Vivek B.] Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. [Asefa, Tewodros] Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. [Asefa, Tewodros] Rutgers State Univ, Dept Chem & Biochem Engn, 98 Brett Rd, Piscataway, NJ 08854 USA. RP Chhowalla, M (reprint author), Rutgers State Univ, Mat Sci & Engn, 607 Taylor Rd, Piscataway, NJ 08854 USA. EM manish1@rci.rutgers.edu RI Voiry, Damien/G-3541-2016; OI Voiry, Damien/0000-0002-1664-2839; Kappera, Rajesh/0000-0003-1792-4405 FU NSF [DGE 0903661, ECCS 1128335, CAREER CHE-1004218, DMR-0968937, NanoEHS-1134289, 0959905]; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-Brazil; Rutgers Energy Institute; LDRD program at LANL; US DOE, Office of Science, BES Award [DE-SC0005132]; US National Science Foundation [EFMA-542879, CMMI-1363203, CBET-1235870] FX M.C. and D.V. acknowledge financial support from NSF DGE 0903661 and ECCS 1128335. T.A. acknowledges financial assistance from NSF (CAREER CHE-1004218, DMR-0968937, NanoEHS-1134289, NSF-ACIF, and Special Creativity Grant).; C.d.C.C.e.S. acknowledges the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-Brazil, for a fellowship. J.Y. and M.C. acknowledge financial support from Rutgers Energy Institute. A.M. acknowledges LDRD program at LANL for funding this work. M.J.L. and P.E.B. acknowledge support from the US DOE, Office of Science, BES Award No. DE-SC0005132 and NSF No. 0959905. L.B., D.E., and V.B.S. acknowledge EFMA-542879, CMMI-1363203 and CBET-1235870 from the US National Science Foundation. NR 48 TC 18 Z9 18 U1 144 U2 170 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD SEP PY 2016 VL 15 IS 9 BP 1003 EP 1009 DI 10.1038/NMAT4660 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DU7YG UT WOS:000382429900019 PM 27295098 ER PT J AU Tsvetkov, N Lu, QY Sun, LX Crumlin, EJ Yildiz, B AF Tsvetkov, Nikolai Lu, Qiyang Sun, Lixin Crumlin, Ethan J. Yildiz, Bilge TI Improved chemical and electrochemical stability of perovskite oxides with less reducible cations at the surface SO NATURE MATERIALS LA English DT Article ID SENSITIZED SOLAR-CELLS; ELECTRONIC-STRUCTURE; FUEL-CELLS; EXCHANGE KINETICS; SPIN-STATE; THIN-FILMS; OXYGEN; CATHODE; SEGREGATION; PERFORMANCE AB Segregation and phase separation of aliovalent dopants on perovskite oxide (ABO(3)) surfaces are detrimental to the performance of energy conversion systems such as solid oxide fuel/electrolysis cells and catalysts for thermochemical H2O and CO2 splitting. One key reason behind the instability of perovskite oxide surfaces is the electrostatic attraction of the negatively charged A-site dopants (for example, Sr'(La)) by the positively charged oxygen vacancies (V-o(center dot center dot)) enriched at the surface. Here we show that reducing the surface V-o(center dot center dot) concentration improves the oxygen surface exchange kinetics and stability significantly, albeit contrary to the well-established understanding that surface oxygen vacancies facilitate reactions with O-2 molecules. We take La0.8Sr0.2CoO3 (LSC) as a model perovskite oxide, and modify its surface with additive cations that are more and less reducible than Co on the B-site of LSC. By using ambient-pressure X-ray absorption and photoelectron spectroscopy, we proved that the dominant role of the less reducible cations is to suppress the enrichment and phase separation of Sr while reducing the concentration of V-o(center dot center dot) and making the LSC more oxidized at its surface. Consequently, we found that these less reducible cations significantly improve stability, with up to 30 times faster oxygen exchange kinetics after 54 h in air at 530 degrees C achieved by Hf addition onto LSC. Finally, the results revealed a 'volcano' relation between the oxygen exchange kinetics and the oxygen vacancy formation enthalpy of the binary oxides of the additive cations. This volcano relation highlights the existence of an optimum surface oxygen vacancy concentration that balances the gain in oxygen exchange kinetics and the chemical stability loss. C1 [Tsvetkov, Nikolai; Lu, Qiyang; Sun, Lixin; Yildiz, Bilge] MIT, Lab Electrochem Interfaces, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Tsvetkov, Nikolai; Sun, Lixin; Yildiz, Bilge] MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Lu, Qiyang; Yildiz, Bilge] MIT, Dept Mat Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Crumlin, Ethan J.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Yildiz, B (reprint author), MIT, Lab Electrochem Interfaces, 77 Massachusetts Ave, Cambridge, MA 02139 USA.; Yildiz, B (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA.; Yildiz, B (reprint author), MIT, Dept Mat Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM byildiz@mit.edu FU NSF CAREER Award of the National Science Foundation, Division of Materials Research, Ceramics Program [1055583]; National Aeronautics and Space Administration (NASA); NSF [DMR-1419807]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The authors are grateful for funding support from the NSF CAREER Award of the National Science Foundation, Division of Materials Research, Ceramics Program, Grant No. 1055583, and from the National Aeronautics and Space Administration (NASA) in support of the Mars Oxygen ISRU Experiment (MOXIE), an instrument on the Mars 2020 rover mission. We thank M. Youssef for useful discussions on the defects in LSC and Q. Liu for experiment assistance at Advanced Light Source Beamline 9.3.2. The authors also acknowledge the use of the Center for Materials Science and Engineering, an MRSEC Shared Experimental Facility of the NSF at MIT, supported by the NSF under award number DMR-1419807. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 7 Z9 7 U1 84 U2 122 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD SEP PY 2016 VL 15 IS 9 BP 1010 EP 1016 DI 10.1038/NMAT4659 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DU7YG UT WOS:000382429900020 PM 27295099 ER PT J AU Jiang, YW Carvalho-de-Souza, JL Wong, RCS Luo, ZQ Isheim, D Zuo, XB Nicholls, AW Jung, IW Yue, JP Liu, DJ Wang, YC De Andrade, V Xiao, XH Navrazhnykh, L Weiss, DE Wu, XY Seidman, DN Bezanilla, F Tian, BZ AF Jiang, Yuanwen Carvalho-de-Souza, Joao L. Wong, Raymond C. S. Luo, Zhiqiang Isheim, Dieter Zuo, Xiaobing Nicholls, Alan W. Jung, Il Woong Yue, Jiping Liu, Di-Jia Wang, Yucai De Andrade, Vincent Xiao, Xianghui Navrazhnykh, Luizetta Weiss, Dara E. Wu, Xiaoyang Seidman, David N. Bezanilla, Francisco Tian, Bozhi TI Heterogeneous silicon rnesostructures for lipid-supported bioelectric interfaces SO NATURE MATERIALS LA English DT Article ID POROUS SILICON; MESOPOROUS SILICON; THIN-FILMS; ELECTRONICS; NANOPARTICLES; CELLS; REDUCTION; NANOWIRES; DYNAMICS; TISSUES AB Silicon-based materials have widespread application as biophysical tools and biomedical devices. Here we introduce a biocompatible and degradable mesostructured form of silicon with multi-scale structural and chemical heterogeneities. The material was synthesized using mesoporous silica as a template through a chemical vapour deposition process. It has an amorphous atomic structure, an ordered nanowire-based framework and random submicrometre voids, and shows an average Young's modulus that is 2-3 orders of magnitude smaller than that of single-crystalline silicon. In addition, we used the heterogeneous silicon mesostructures to design a lipid-bilayer-supported bioelectric interface that is remotely controlled and temporally transient, and that permits non-genetic and subcellular optical modulation of the electrophysiology dynamics in single dorsal root ganglia neurons. Our findings suggest that the biomimetic expansion of silicon into heterogeneous and deformable forms can open up opportunities in extracellular biomaterial or bioelectric systems. C1 [Jiang, Yuanwen; Luo, Zhiqiang; Wang, Yucai; Navrazhnykh, Luizetta; Weiss, Dara E.; Tian, Bozhi] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Jiang, Yuanwen; Wong, Raymond C. S.; Luo, Zhiqiang; Wang, Yucai; Tian, Bozhi] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Carvalho-de-Souza, Joao L.; Wong, Raymond C. S.; Bezanilla, Francisco] Univ Chicago, Dept Biochem & Mol Biol, Chicago, IL 60637 USA. [Isheim, Dieter; Seidman, David N.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Isheim, Dieter; Seidman, David N.] Northwestern Univ, NUCAPT, Evanston, IL 60208 USA. [Zuo, Xiaobing; De Andrade, Vincent; Xiao, Xianghui] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Nicholls, Alan W.] Univ Illinois, Res Resources Ctr, Chicago, IL 60607 USA. [Jung, Il Woong] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Wu, Xiaoyang] Univ Chicago, Ben May Dept Canc Res, Chicago, IL 60637 USA. [Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Bezanilla, Francisco; Tian, Bozhi] Univ Chicago, Inst Biophys Dynam, Chicago, IL 60637 USA. RP Tian, BZ (reprint author), Univ Chicago, Dept Chem, Chicago, IL 60637 USA.; Tian, BZ (reprint author), Univ Chicago, James Franck Inst, Chicago, IL 60637 USA.; Bezanilla, F (reprint author), Univ Chicago, Dept Biochem & Mol Biol, Chicago, IL 60637 USA.; Bezanilla, F; Tian, BZ (reprint author), Univ Chicago, Inst Biophys Dynam, Chicago, IL 60637 USA. EM fbezanilla@uchicago.edu; btian@uchicago.edu RI Seidman, David/B-6697-2009; Wang, Yucai/A-1098-2017 OI Wang, Yucai/0000-0001-6046-2934 FU Air Force Office of Scientific Research [AFOSR FA9550-14-1-0175, FA9550-15-1-0285]; National Science Foundation (NSF CAREER) [DMR-1254637]; National Science Foundation (NSF MRSEC) [DMR 1420709]; Searle Scholars Foundation; National Institutes of Health [NIH GM030376]; University of Chicago Start-up Fund; NSF-MRI grant [DMR-0420532]; ONR-DURIP grant [N00014-0400798, N00014-0610539, N00014-0910781]; National Science Foundation's MRSEC programme [DMR-1121262]; MRI-R2 grant from the National Science Foundation [DMR-0959470]; Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [E-AC02-06CH11357]; DOE Office of Science [DE-AC02-06CH11357] FX This work is supported by the Air Force Office of Scientific Research (AFOSR FA9550-14-1-0175, FA9550-15-1-0285), the National Science Foundation (NSF CAREER, DMR-1254637; NSF MRSEC, DMR 1420709), the Searle Scholars Foundation, the National Institutes of Health (NIH GM030376), and the University of Chicago Start-up Fund. Atom-probe tomography was performed at the Northwestern University Center for Atom-Probe Tomography (NUCAPT), whose APT was purchased and upgraded with funding from NSF-MRI (DMR-0420532) and ONR-DURIP (N00014-0400798, N00014-0610539, N00014-0910781) grants. NUCAPT is a Research Facility at the Materials Research Center of Northwestern University, supported by the National Science Foundation's MRSEC programme (grant number DMR-1121262). Instrumentation at NUCAPT was further upgraded by the Initiative for Sustainability and Energy at Northwestern (ISEN). This work made use of the JEOL JEM-ARM200CF and JEOL JEM-3010 TEM in the Electron Microscopy Service (Research Resources Center, UIC). The acquisition of the UIC JEOL JEM-ARM200CF was supported by an MRI-R2 grant from the National Science Foundation (DMR-0959470). A portion of this work was performed at the Center for Nanoscale Materials, a US Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. This research used the resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors thank D. Talapin, V. Srivastava, Y. Chen, J. Treger, T. Sun, Q. Guo, J. Jureller and R. N. S. Divan for providing technical support and stimulating discussions. NR 50 TC 2 Z9 2 U1 52 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD SEP PY 2016 VL 15 IS 9 BP 1023 EP 1030 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DU7YG UT WOS:000382429900022 PM 27348576 ER PT J AU Gurdal, G Mccutchan, EA AF Gurdal, G. Mccutchan, E. A. TI Nuclear Data Sheets for A=70 SO NUCLEAR DATA SHEETS LA English DT Article ID LOW-LYING STATES; HIGH-SPIN STATES; EVEN ZN ISOTOPES; DECAY HALF-LIVES; ALPHA' INELASTIC-SCATTERING; DRIFTED GERMANIUM DETECTOR; THERMAL-NEUTRON CAPTURE; DOUBLE-BETA DECAY; 64ZN 66ZN 68ZN; 50 MEV PROTONS AB Spectroscopic data for all nuclei with mass number A=70 have been evaluated, and the corresponding level schemes from radioactive decay and reaction studies are presented. Since the previous evaluation, the half-life of Mn-70 has been measured and excited states in Fe-70 observed for the first time. Excited states in Ni-70 have been more extensively studied while Coulomb excitation and collinear laser spectroscopy measurements in Cu-70 have allowed for firm J pi assignments. Despite new measurements, there remain some discrepancies in half-lives of low lying states in Zn-70. New measurements have extended the knowledge of high-spin band structures in Ge-70 and As-70. This evaluation supersedes the prior A=70 evaluation of 2004Tu09. C1 [Gurdal, G.] Millsaps Coll, Dept Phys, Jackson, MS 39210 USA. [Mccutchan, E. A.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Gurdal, G (reprint author), Millsaps Coll, Dept Phys, Jackson, MS 39210 USA. FU Office of Nuclear Physics, Office of Science, US Department of Energy [DE-AC02-98CH10946] FX Research sponsored by Office of Nuclear Physics, Office of Science, US Department of Energy, under contract DE-AC02-98CH10946. NR 288 TC 0 Z9 0 U1 5 U2 5 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 EI 1095-9904 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD SEP-OCT PY 2016 VL 136 BP 1 EP 162 DI 10.1016/j.nds.2016.08.001 PG 162 WC Physics, Nuclear SC Physics GA DV0HG UT WOS:000382598000001 ER PT J AU Joye, SB Kleindienst, S Gilbert, JA Handley, KM Weisenhorn, P Overholt, WA Kostka, JE AF Joye, Samantha B. Kleindienst, Sara Gilbert, Jack A. Handley, Kim M. Weisenhorn, Pam Overholt, Will A. Kostka, Joel E. TI Responses of Microbial Communities to Hydrocarbon Exposures SO OCEANOGRAPHY LA English DT Article ID DEEP-WATER-HORIZON; GULF-OF-MEXICO; POLYCYCLIC AROMATIC-HYDROCARBONS; OIL-WELL BLOWOUT; DEGRADING BACTERIA; ALKANE DEGRADATION; ANAEROBIC BIODEGRADATION; MACONDO OIL; SPILL; DISPERSANTS AB The responses of microbial communities to hydrocarbon exposures are complex and variable, driven to a large extent by the nature of hydrocarbon infusion, local environmental conditions, and factors that regulate microbial physiology (e.g., substrate and nutrient availability). Although present at low abundance in the ocean, hydrocarbon-degrading seed populations are widely distributed, and they respond rapidly to hydrocarbon inputs at natural and anthropogenic sources. Microbiomes from environments impacted by hydrocarbon discharge may appear similar at a higher taxonomic rank (e.g., genus level) but diverge at increasing phylogenetic resolution (e.g., sub-OTU [operational taxonomic unit] levels). Such subtle changes are detectable by computational methods such as oligotyping or by genome reconstruction from metagenomic sequence data. The ability to reconstruct these genomes, and to characterize their transcriptional activities in different environmental contexts through metatranscriptomic mapping, is revolutionizing our ability to understand the diverse and adaptable microbial communities in marine ecosystems. Our knowledge of the environmental factors that regulate microbial hydrocarbon degradation and the efficiency with which marine hydrocarbon-degrading microbial communities bioremediate hydrocarbon contamination is incomplete. Moreover, detailed baseline descriptions of naturally occurring hydrocarbon-degrading microbial communities and a more robust understanding of the factors that regulate their activity are needed. C1 [Joye, Samantha B.] Univ Georgia, Dept Marine Sci, Arts & Sci, Athens, GA 30602 USA. [Kleindienst, Sara] Univ Tubingen, Microbial Ecol Grp, Ctr Appl Geosci, Tubingen, Germany. [Gilbert, Jack A.] Univ Chicago, Dept Surg, Chicago, IL 60637 USA. [Handley, Kim M.] Univ Auckland, Sch Biol Sci, Auckland, New Zealand. [Weisenhorn, Pam] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Overholt, Will A.] Georgia Inst Technol, Sch Biol, Atlanta, GA 30332 USA. [Kostka, Joel E.] Georgia Inst Technol, Atlanta, GA 30332 USA. RP Joye, SB (reprint author), Univ Georgia, Dept Marine Sci, Arts & Sci, Athens, GA 30602 USA. EM mjoye@uga.edu RI Kleindienst, Sara/O-9908-2016 OI Kleindienst, Sara/0000-0001-8304-9149 FU GoMRI "Ecosystem Impacts of Oil and Gas Inputs to the Gulf2" (ECOGIG-2) consortia; GoMRI "Center for Integrated Modeling and Analysis of the Gulf Ecosystem-2" (C-IMAGE-2) consortia; RFP-II program "Creating a predictive model of microbially mediated carbon remediation in the Gulf of Mexico (JAG)" FX We thank L. Nigro for assistance with the literature review and our colleagues in the Gulf of Mexico Research Initiative's (GoMRI) program for invigorating discussions on this topic. Funding for the preparation of this manuscript was provided by GoMRI's "Ecosystem Impacts of Oil and Gas Inputs to the Gulf2" (ECOGIG-2; SBJ) and the "Center for Integrated Modeling and Analysis of the Gulf Ecosystem-2" (C-IMAGE-2; JEC) consortia and RFP-II program "Creating a predictive model of microbially mediated carbon remediation in the Gulf of Mexico (JAG)." This is ECOGIG contribution no. 430. NR 69 TC 1 Z9 1 U1 26 U2 26 PU OCEANOGRAPHY SOC PI ROCKVILLE PA P.O. BOX 1931, ROCKVILLE, MD USA SN 1042-8275 J9 OCEANOGRAPHY JI Oceanography PD SEP PY 2016 VL 29 IS 3 SI SI BP 136 EP 149 DI 10.5670/oceanog.2016.78 PG 14 WC Oceanography SC Oceanography GA DU6OM UT WOS:000382334500020 ER PT J AU Koohbor, B Kidane, A Lu, WY AF Koohbor, Behrad Kidane, Addis Lu, Wei-Yang TI Characterizing the constitutive response and energy absorption of rigid polymeric foams subjected to intermediate-velocity impact SO POLYMER TESTING LA English DT Article DE Polymeric foam; Direct impact; Digital image correlation; Inertia; Energy absorption ID REPRESENTATIVE VOLUME ELEMENT; COMPRESSIVE RESPONSE; BEHAVIOR; MICROSTRUCTURES; BAR AB As an optimum energy-absorbing material system, polymeric foams are needed to dissipate the kinetic energy of an impact, while maintaining the impact force transferred to the protected object at a low level. Therefore, it is crucial to accurately characterize the load bearing and energy dissipation performance of foams at high strain rate loading conditions. There are certain challenges faced in the accurate measurement of the deformation response of foams due to their low mechanical impedance. In the present work, a non-parametric method is successfully implemented to enable the accurate assessment of the compressive constitutive response of rigid polymeric foams subjected to impact loading conditions. The method is based on stereovision high speed photography in conjunction with 3D digital image correlation, and allows for accurate evaluation of inertia stresses developed within the specimen during deformation time. Full-field distributions of stress, strain and strain rate are used to extract the local constitutive response of the material at any given location along the specimen axis. In addition, the effective energy absorbed by the material is calculated. Finally, results obtained from the proposed non parametric analysis are compared with data obtained from conventional test procedures. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Koohbor, Behrad; Kidane, Addis] Univ South Carolina, Dept Mech Engn, 300 Main St,Room A132, Columbia, SC 29208 USA. [Lu, Wei-Yang] Sandia Natl Labs, Livermore, CA 94551 USA. RP Kidane, A (reprint author), Univ South Carolina, Dept Mech Engn, 300 Main St,Room A132, Columbia, SC 29208 USA. EM kidanea@cec.sc.edu RI Koohbor, Behrad/F-9771-2015; OI Koohbor, Behrad/0000-0002-5787-4644; , Addis/0000-0003-0830-0158 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 24 TC 0 Z9 0 U1 7 U2 7 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0142-9418 EI 1873-2348 J9 POLYM TEST JI Polym. Test PD SEP PY 2016 VL 54 BP 48 EP 58 DI 10.1016/j.polymertesting.2016.06.023 PG 11 WC Materials Science, Characterization & Testing; Polymer Science SC Materials Science; Polymer Science GA DV3CJ UT WOS:000382798300007 ER PT J AU Linville, JL Shen, YW Schoene, RP Nguyen, M Urgun-Demirtas, M Snyder, SW AF Linville, Jessica L. Shen, Yanwen Schoene, Robin P. Nguyen, Maximilian Urgun-Demirtas, Meltem Snyder, Seth W. TI Impact of trace element additives on anaerobic digestion of sewage sludge with in-situ carbon dioxide sequestration SO PROCESS BIOCHEMISTRY LA English DT Article DE Anaerobic digestion; Trace elements; Carbon dioxide sequestration; Olivine; Renewable methane production ID MICROBIAL COMMUNITY; METHANE PRODUCTION; BIOGAS PRODUCTION; WASTE-WATER; KINETICS; OPTIMIZATION; MODEL AB Anaerobic digestion (AD) of sludge at wastewater treatment plants can benefit from addition of essential trace metals such as iron, nickel and cobalt to increase biogas production for utilization in combined heat and power systems, fed into natural gas pipelines or as a vehicle fuel. This study evaluated the impact and benefits of Ni/Co and olivine addition to the digester at mesophilic temperatures. These additions supplement previously reported research in which iron-rich olivine (MgSiO4) was added to sequester CO2 in-situ during batch AD of sludge. Trace element addition has been shown to stimulate and stabilize biogas production and have a synergistic effect on the mineral carbonation process. AD with 5% w/v olivine and 1.5 mg/L Ni/Co addition had a 17.3% increase in methane volume, a 6% increase in initial exponential methane production rate and a 56% increase in methane yield (mL CH4/g CODdegraded) compared to the control due to synergistic trace element and olivine addition while maintaining 17.7% CO2 sequestration from olivine addition. Both first-order kinetic modeling and response surface methodology modeling confirmed the combined benefit of the trace elements and olivine addition. These results were significantly higher than previously reported results with olivine addition alone [1] (Linville et al., 2016). (C) 2016 Elsevier Ltd. All rights reserved. C1 [Linville, Jessica L.; Shen, Yanwen; Schoene, Robin P.; Nguyen, Maximilian; Urgun-Demirtas, Meltem; Snyder, Seth W.] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Lemont, IL 60439 USA. RP Urgun-Demirtas, M (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Lemont, IL 60439 USA. EM demirtasmu@anl.gov FU California Energy Commission of California Government [ARV-10-003-01 SMUD]; [DE-AC02-06CH11357] FX This work was sponsored by via Sacramento Municipal Utilities by the California Energy Commission of California Government (ARV-10-003-01 SMUD). The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"), Argonne, a US Department of Energy Office of Science laboratory, is operated under contract no. DE-AC02-06CH11357. The US Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. The funding source for the work reported here did not have a role in study design, data collection, analysis, data interpretation, writing, or in the decision to publish. NR 46 TC 0 Z9 0 U1 16 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1359-5113 EI 1873-3298 J9 PROCESS BIOCHEM JI Process Biochem. PD SEP PY 2016 VL 51 IS 9 BP 1283 EP 1289 DI 10.1016/j.procbio.2016.06.003 PG 7 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Engineering, Chemical SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Engineering GA DU6UG UT WOS:000382349500020 ER PT J AU Gao, YF Bei, HB AF Gao, Yanfei Bei, Hongbin TI Strength statistics of single crystals and metallic glasses under small stressed volumes SO PROGRESS IN MATERIALS SCIENCE LA English DT Review DE Strength statistics; Intrinsic thermal-activation mechanism; Extrinsic stochastic mechanism; Universal relationship between strength and sample size ID ANISOTROPIC HALF-SPACES; SUBMICRON LENGTH SCALES; MO-ALLOY MICROPILLARS; ON-SUBSTRATE SYSTEMS; POP-IN BEHAVIOR; DISLOCATION NUCLEATION; INCIPIENT PLASTICITY; SIZE DEPENDENCE; YIELD STRENGTH; DEFORMATION MECHANISMS AB It has been well documented that plastic deformation of crystalline and amorphous metals/alloys shows a general trend of "smaller is stronger". The majority of the experimental and modeling studies along this line have been focused on finding and reasoning the scaling slope or exponent in the logarithmic plot of strength versus size. In contrast to this view, here we show that the universal picture should be the thermally activated nucleation mechanisms in small stressed volume, the stochastic behavior as to find the weakest links in intermediate sizes of the stressed volume, and the convolution of these two mechanisms with respect to variables such as indenter radius in nanoindentation pop-in, crystallographic orientation, pre-strain level, sample length as in uniaxial tests, and others. Experiments that cover the entire spectrum of length scales and a unified model that treats both thermal activation and spatial stochasticity have discovered new perspectives in understanding and correlating the strength statistics in a vast of observations in nanoindentation, micro-pillar compression, and fiber/whisker tension tests of single crystals and metallic glasses. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Gao, Yanfei; Bei, Hongbin] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Gao, Yanfei] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Gao, YF; Bei, HB (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM ygao7@utk.edu; beih@ornl.gov RI Gao, Yanfei/F-9034-2010; OI Gao, Yanfei/0000-0003-2082-857X; Bei, Hongbin/0000-0003-0283-7990 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was sponsored by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 169 TC 2 Z9 2 U1 33 U2 39 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0079-6425 J9 PROG MATER SCI JI Prog. Mater. Sci. PD SEP PY 2016 VL 82 BP 118 EP 150 DI 10.1016/j.pmatsci.2016.05.002 PG 33 WC Materials Science, Multidisciplinary SC Materials Science GA DV0ER UT WOS:000382591300004 ER PT J AU Deur, A Brodsky, SJ de Teramond, GF AF Deur, Alexandre Brodsky, Stanley J. de Teramond, Guy F. TI The QCD running coupling SO PROGRESS IN PARTICLE AND NUCLEAR PHYSICS LA English DT Review DE QCD; Coupling constant; Non-perturbative; Renormalization; Infrared properties; Hadron physics ID SPIN STRUCTURE-FUNCTION; ABELIAN GAUGE-THEORIES; DEEP-INELASTIC-SCATTERING; YANG-MILLS THEORY; ANALYTIC PERTURBATION-THEORY; DEPENDENT STRUCTURE-FUNCTION; DYSON-SCHWINGER EQUATIONS; TO-LEADING ORDER; CHIRAL-SYMMETRY BREAKING; EFFECTIVE GLUON MASS AB We review the present theoretical and empirical knowledge for alpha(s), the fundamental coupling underlying the interactions of quarks and gluons in Quantum Chromodynamics (QCD). The dependence of us alpha(s)(Q(2)) on momentum transfer Q encodes the underlying dynamics of hadron physics-from color confinement in the infrared domain to asymptotic freedom at short distances. We review constraints on alpha(s)(Q(2)) at high Q(2), as predicted by perturbative QCD, and its analytic behavior at small Q(2), based on models of nonperturbative dynamics. In the introductory part of this review, we explain the phenomenological meaning of the coupling, the reason for its running, and the challenges facing a complete understanding of its analytic behavior in the infrared domain. In the second, more technical, part of the review, we discuss the behavior of as alpha(s)(Q(2)) in the high momentum transfer domain of QCD. We review how alpha(s) is defined, including its renormalization scheme dependence, the definition of its renormalization scale, the utility of effective charges, as well as "Commensurate Scale Relations" which connect the various definitions of the QCD coupling without renormalization-scale ambiguity. We also report recent significant measurements and advanced theoretical analyses which have led to precise QCD predictions at high energy. As an example of an important optimization procedure, we discuss the "Principle of Maximum Conformality", which enhances QCD's predictive power by removing the dependence of the predictions for physical observables on the choice of theoretical conventions such as the renormalization scheme. In the last part of the review, we discuss the challenge of understanding the analytic behavior as alpha(s)(Q2) in the low momentum transfer domain. We survey various theoretical models for the nonperturbative strongly coupled regime, such as the light-front holographic approach to QCD. This new framework predicts the form of the quark-confinement potential underlying hadron spectroscopy and dynamics, and it gives a remarkable connection between the perturbative QCD scale A and hadron masses. One can also identify a specific scale Q(0) which demarcates the division between perturbative and nonperturbative QCD. We also review other important methods for computing the QCD coupling, including lattice QCD, the Schwinger-Dyson equations and the Gribov-Zwanziger analysis. After describing these approaches and enumerating their conflicting predictions, we discuss the origin of these discrepancies and how to remedy them. Our aim is not only to review the advances in this difficult area, but also to suggest what could be an optimal definition of as alpha(s)(Q(2)) in order to bring better unity to the subject. (C) 2016 Elsevier B.V. All rights reserved. C1 [Deur, Alexandre] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Brodsky, Stanley J.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [de Teramond, Guy F.] Univ Costa Rica, San Jose, Costa Rica. RP Deur, A (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM deurpam@jlab.org; sjbth@slac.stanford.edu; gdt@asterix.crnet.cr FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177, DE-AC02-76SF00515] FX We thank Hans Guenter Dosch, David d'Enterria, John A. Gracey, Andrei L. Kataev, Cedric Lorce, Matin Mojaza, Christian Weiss, Xing-Gang Wu and Ma Yang for instructive discussions on as and related topics. We are grateful to A. Faessler for his invitation to write this review. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract DE-AC05-06OR23177 and DE-AC02-76SF00515. SLAC-PUB-16448. NR 731 TC 7 Z9 7 U1 5 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0146-6410 EI 1873-2224 J9 PROG PART NUCL PHYS JI Prog. Part. Nucl. Phys. PD SEP PY 2016 VL 90 BP 1 EP 74 DI 10.1016/j.ppnp.2016.04.003 PG 74 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU6RP UT WOS:000382342600001 ER PT J AU Cronauer, SL Briner, JP Kelley, SE Zimmerman, SRH Morlighem, M AF Cronauer, Sandra L. Briner, Jason P. Kelley, Samuel E. Zimmerman, Susan R. H. Morlighem, Mathieu TI Be-10 dating reveals early-middle Holocene age of the Drygalski Moraines in central West Greenland SO QUATERNARY SCIENCE REVIEWS LA English DT Article; Proceedings Paper CT 2nd International Conference of the Palaeo-Arctic-Spatial-and-Temporal-Gateways-Network (PAST Gateways) CY 2014 CL Trieste, ITALY SP Palaeo Arctic Spatial & Temporal Gateways Network DE Cosmogenic nuclide exposure dating; Greenland Ice Sheet; Proglacial-threshold lake; Holocene ID ICE STREAM SYSTEM; JAKOBSHAVN ISBRAE; THERMAL MAXIMUM; LAST RECESSION; SHEET; RETREAT; TEMPERATURE; HISTORY; CLIMATE; REGION AB We reconstruct the history of the Greenland Ice Sheet margin on the Nuussuaq Peninsula in central West Greenland through the Holocene using lake sediment analysis and cosmogenic Be-10 exposure dating of the prominent Drygalski Moraines. Erratics perched on bedrock outboard of the Drygalski Moraines constrain local deglaciation to similar to 9.9 +/- 0.6 ka (n = 2). Three Drygalski Moraine crests yield mean Be-10 ages of 8.6 +/- 0.4 ka (n = 2), 8.5 +/- 0.2 ka (n = 3), and 7.6 +/- 0.1 ka (n = 2) from outer to inner. Perched erratics between the inner two moraines average 7.8 +/- 0.1 ka (n = 2) and are consistent with the moraine ages. Sediments from a proglacial lake with a catchment area extending an estimated 2 km beneath (inland of) the present ice sheet terminus constrain an ice sheet minimum extent from 5.4 ka to 0.6 ka. The moraine chronology paired with the lake sediment stratigraphy reveals that the ice margin likely remained within similar to 2 km of its present position from similar to 9.9 to 5.4 ka. This unexpected early Holocene stability, preceded by rapid ice retreat and followed by minimum ice extent between similar to 5.4 and 0.6 ka, contrasts with many records of early Holocene warmth and the Northern Hemisphere summer insolation maximum. We suggest ice margin stability may instead be tied to adjacent ocean temperatures, which reached an optimum in the middle Holocene. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Cronauer, Sandra L.; Briner, Jason P.; Kelley, Samuel E.] Univ Buffalo, Dept Geol, 411 Cooke Hall, Buffalo, NY 14260 USA. [Zimmerman, Susan R. H.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, 7000 East Ave, Livermore, CA 94550 USA. [Morlighem, Mathieu] Univ Calif Irvine, Dept Earth Syst Sci, Croul Hall, Irvine, CA 92697 USA. [Kelley, Samuel E.] Univ Waterloo, Dept Earth & Environm Sci, 200 Univ Ave W, Waterloo, ON N2L 3G1, Canada. RP Briner, JP (reprint author), Univ Buffalo, Dept Geol, 411 Cooke Hall, Buffalo, NY 14260 USA. NR 53 TC 5 Z9 5 U1 4 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-3791 J9 QUATERNARY SCI REV JI Quat. Sci. Rev. PD SEP 1 PY 2016 VL 147 SI SI BP 59 EP 68 DI 10.1016/j.quascirev.2015.08.034 PG 10 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA DU7QK UT WOS:000382409500005 ER PT J AU Leung, MCK Hutson, MS Seifert, AW Spencer, RM Knudsen, TB AF Leung, Maxwell C. K. Hutson, M. Shane Seifert, Ashley W. Spencer, Richard M. Knudsen, Thomas B. TI Computational modeling and simulation of genital tubercle development SO REPRODUCTIVE TOXICOLOGY LA English DT Article; Proceedings Paper CT 44th Annual Conference of the European-Teratology-Society CY SEP 11-14, 2016 CL Dublin, IRELAND SP European Teratol Soc DE Agent-based model; Genital tubercle; Hypospadias; Computational toxicology ID TISSUE-SPECIFIC ROLES; EPITHELIAL-MESENCHYMAL TRANSFORMATION; REPRODUCTIVE-TRACT DEVELOPMENT; MATE GENITOURINARY SYSTEM; EXTERNAL GENITALIA; SONIC-HEDGEHOG; ANDROGEN RECEPTOR; ENDOCRINE DISRUPTION; URETHRAL DEVELOPMENT; DIVERSE MECHANISMS AB Hypospadias is a developmental defect of urethral tube closure that has a complex etiology involving genetic and environmental factors, including anti-androgenic and estrogenic disrupting chemicals; however, little is known about the morphoregulatory consequences of androgen/estrogen balance during genital tubercle (GT) development. Computer models that predictively model sexual dimorphism of the GT may provide a useful resource to translate chemical-target bipartite networks and their developmental consequences across the human-relevant chemical universe. Here, we describe a multicellular agent-based model of genital tubercle (GT) development that simulates urethrogenesis from the sexually-indifferent urethral plate stage to urethral tube closure. The prototype model, constructed in CompuCell3D, recapitulates key aspects of GT morphogenesis controlled by SHH, FGF10, and androgen pathways through modulation of stochastic cell behaviors, including differential adhesion, motility, proliferation, and apoptosis. Proper urethral tube closure in the model was shown to depend quantitatively on SHH- and FGF10-induced effects on mesenchymal proliferation and epithelial apoptosis-both ultimately linked to androgen signaling. In the absence of androgen, GT development was feminized and with partial androgen deficiency, the model resolved with incomplete urethral tube closure, thereby providing an in silico platform for probabilistic prediction of hypospadias risk across combinations of minor perturbations to the GT system at various stages of embryonic development. (C) 2016 Elsevier Inc. All rights reserved. C1 [Leung, Maxwell C. K.; Knudsen, Thomas B.] US EPA, Natl Ctr Computat Toxicol, Res Triangle Pk, NC 27711 USA. [Leung, Maxwell C. K.; Hutson, M. Shane] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Hutson, M. Shane] Vanderbilt Univ, Vanderbilt Inst Integrat Biosyst Res & Educ, Dept Phys & Astron, Nashville, TN 37235 USA. [Seifert, Ashley W.] Univ Kentucky, Dept Biol, Lexington, KY 40506 USA. [Spencer, Richard M.] Lockheed Martin, Res Triangle Pk, NC 27709 USA. RP Leung, MCK; Knudsen, TB (reprint author), US EPA, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. EM leung.maxwell@epa.gov; knudsen.thomas@epa.gov OI Leung, Maxwell/0000-0003-1530-3306 NR 79 TC 0 Z9 0 U1 3 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0890-6238 J9 REPROD TOXICOL JI Reprod. Toxicol. PD SEP PY 2016 VL 64 SI SI BP 151 EP 161 DI 10.1016/j.reprotox.2016.05.005 PG 11 WC Reproductive Biology; Toxicology SC Reproductive Biology; Toxicology GA DU1GR UT WOS:000381956700013 PM 27180093 ER PT J AU Bakhti, S Tishchenko, AV Zambrana-Puyalto, X Bonod, N Dhuey, SD Schuck, PJ Cabrini, S Alayoglu, S Destouches, N AF Bakhti, Said Tishchenko, Alexandre V. Zambrana-Puyalto, Xavier Bonod, Nicolas Dhuey, Scott D. Schuck, P. James Cabrini, Stefano Alayoglu, Selim Destouches, Nathalie TI Fano-like resonance emerging from magnetic and electric plasmon mode coupling in small arrays of gold particles SO SCIENTIFIC REPORTS LA English DT Article ID NEGATIVE REFRACTIVE-INDEX; METAL NANOPARTICLES; SURFACE-PLASMONS; NANOSTRUCTURES; SCATTERING; METAMATERIALS; NANOCLUSTERS; PERMEABILITY; FREQUENCIES; RESONATORS AB In this work we theoretically and experimentally analyze the resonant behavior of individual 3 x 3 gold particle oligomers illuminated under normal and oblique incidence. While this structure hosts both dipolar and quadrupolar electric and magnetic delocalized modes, only dipolar electric and quadrupolar magnetic modes remain at normal incidence. These modes couple into a strongly asymmetric spectral response typical of a Fano-like resonance. In the basis of the coupled mode theory, an analytical representation of the optical extinction in terms of singular functions is used to identify the hybrid modes emerging from the electric and magnetic mode coupling and to interpret the asymmetric line profiles. Especially, we demonstrate that the characteristic Fano line shape results from the spectral interference of a broad hybrid mode with a sharp one. This structure presents a special feature in which the electric field intensity is confined on different lines of the oligomer depending on the illumination wavelength relative to the Fano dip. This Fano-type resonance is experimentally observed performing extinction cross section measurements on arrays of gold nano-disks. The vanishing of the Fano dip when increasing the incidence angle is also experimentally observed in accordance with numerical simulations. C1 [Bakhti, Said; Tishchenko, Alexandre V.; Destouches, Nathalie] Univ Lyon, UJM St Etienne, CNRS, Inst Opt Grad Sch,Lab Hubert Curien UMR 5516, F-42023 St Etienne, France. [Zambrana-Puyalto, Xavier; Bonod, Nicolas] Aix Marseille Univ, Cent Marseille, Inst Fresnel, CNRS, Marseille, France. [Dhuey, Scott D.; Schuck, P. James; Cabrini, Stefano] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA USA. [Alayoglu, Selim] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA USA. RP Destouches, N (reprint author), Univ Lyon, UJM St Etienne, CNRS, Inst Opt Grad Sch,Lab Hubert Curien UMR 5516, F-42023 St Etienne, France. EM nathalie.destouches@univ-st-etienne.fr RI Bonod, Nicolas/F-3344-2014 FU LABEX MANUTECH-SISE of Universite de Lyon, within the program "Investissements d'Avenir" [ANR-10-LABX-0075, ANR-11-IDEX-0007]; ANR [12-NANO-0006]; A*MIDEX project - Investissements d'Avenir French Government program [ANR-11-IDEX-0001-02]; Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231] FX N.D. is grateful to Ali Belkacem, from the Chemical Sciences Division (CSD), Berkeley, for fruitful discussions and his support to initiate this joint work. This work was supported by the LABEX MANUTECH-SISE (ANR-10-LABX-0075) of Universite de Lyon, within the program "Investissements d'Avenir" (ANR-11-IDEX-0007) operated by the French National Research Agency (ANR). The authors thank ANR for its financial support in the framework of project PHOTOFLEX no. 12-NANO-0006. Work at Institut Fresnel has been carried out thanks to the support of the A*MIDEX project (no. ANR-11-IDEX-0001-02) funded by the Investissements d'Avenir French Government program managed by the French National Research Agency (ANR). Work at the Molecular Foundry was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 53 TC 0 Z9 0 U1 22 U2 22 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD SEP 1 PY 2016 VL 6 AR 32061 DI 10.1038/srep32061 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU7AL UT WOS:000382365600001 PM 27580515 ER PT J AU Hu, ZQ Wang, XJ Nan, TX Zhou, ZY Ma, BH Chen, XQ Jones, JG Howe, BM Brown, GJ Gao, Y Lin, H Wang, ZG Guo, RD Chen, SY Shi, XL Shi, W Sun, HZ Budil, D Liu, M Sun, NX AF Hu, Zhongqiang Wang, Xinjun Nan, Tianxiang Zhou, Ziyao Ma, Beihai Chen, Xiaoqin Jones, John G. Howe, Brandon M. Brown, Gail J. Gao, Yuan Lin, Hwaider Wang, Zhiguang Guo, Rongdi Chen, Shuiyuan Shi, Xiaoling Shi, Wei Sun, Hongzhi Budil, David Liu, Ming Sun, Nian X. TI Non-Volatile Ferroelectric Switching of Ferromagnetic Resonance in NiFe/PLZT Multiferroic Thin Film Heterostructures SO SCIENTIFIC REPORTS LA English DT Article ID ELECTRIC-FIELD CONTROL; ROOM-TEMPERATURE; OXIDE HETEROSTRUCTURES; MAGNETIC-ANISOTROPY; SPIN POLARIZATION; TUNNEL-JUNCTIONS; ATOMIC LAYERS; VOLTAGE; MEMORY; CHARGE AB Magnetoelectric effect, arising from the interfacial coupling between magnetic and electrical order parameters, has recently emerged as a robust means to electrically manipulate the magnetic properties in multiferroic heterostructures. Challenge remains as finding an energy efficient way to modify the distinct magnetic states in a reliable, reversible, and non-volatile manner. Here we report ferroelectric switching of ferromagnetic resonance in multiferroic bilayers consisting of ultrathin ferromagnetic NiFe and ferroelectric Pb0.92La0.08Zr0.52Ti0.48O3 (PLZT) films, where the magnetic anisotropy of NiFe can be electrically modified by low voltages. Ferromagnetic resonance measurements confirm that the interfacial charge-mediated magnetoelectric effect is dominant in NiFe/PLZT heterostructures. Nonvolatile modification of ferromagnetic resonance field is demonstrated by applying voltage pulses. The ferroelectric switching of magnetic anisotropy exhibits extensive applications in energy-efficient electronic devices such as magnetoelectric random access memories, magnetic field sensors, and tunable radio frequency (RF)/microwave devices. C1 [Hu, Zhongqiang; Wang, Xinjun; Nan, Tianxiang; Chen, Xiaoqin; Gao, Yuan; Lin, Hwaider; Wang, Zhiguang; Guo, Rongdi; Chen, Shuiyuan; Shi, Xiaoling; Shi, Wei; Sun, Hongzhi; Sun, Nian X.] Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. [Hu, Zhongqiang; Jones, John G.; Howe, Brandon M.; Brown, Gail J.] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. [Zhou, Ziyao; Liu, Ming] Xi An Jiao Tong Univ, Elect Mat Res Lab, Key Lab, Minist Educ, Xian 710049, Peoples R China. [Zhou, Ziyao; Liu, Ming] Xi An Jiao Tong Univ, Int Ctr Dielect Res, Xian 710049, Peoples R China. [Ma, Beihai] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Budil, David] Northeastern Univ, Dept Chem, Boston, MA 02115 USA. RP Sun, NX (reprint author), Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA.; Liu, M (reprint author), Xi An Jiao Tong Univ, Elect Mat Res Lab, Key Lab, Minist Educ, Xian 710049, Peoples R China.; Liu, M (reprint author), Xi An Jiao Tong Univ, Int Ctr Dielect Res, Xian 710049, Peoples R China. EM mingliu@mail.xjtu.edu.cn; n.sun@neu.edu RI Gao, Yuan/E-4277-2016; Liu, Ming/B-4143-2009 OI Gao, Yuan/0000-0002-2444-1180; Liu, Ming/0000-0002-6310-948X FU National Science Foundation [1160504]; NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems TANMS; W.M. Keck Foundation; Air Force Research Laboratory [FA8650-14-C-5706]; U.S. Department of Energy, Vehicle Technologies Program [DE-AC02-06CH11357]; Air Force Office of Scientific Research (AFOSR) FX This work was supported by the National Science Foundation Award 1160504, NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems TANMS, the W.M. Keck Foundation, and the Air Force Research Laboratory through Contract No. FA8650-14-C-5706. Work at Argonne was funded by the U.S. Department of Energy, Vehicle Technologies Program, under Contract No. DE-AC02-06CH11357. B.H. and G.B. gratefully acknowledge the financial support from the Air Force Office of Scientific Research (AFOSR). NR 54 TC 0 Z9 0 U1 34 U2 42 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD SEP 1 PY 2016 VL 6 AR 32408 DI 10.1038/srep32408 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU6MS UT WOS:000382329800001 PM 27581071 ER PT J AU Alazizi, A Smith, D Erdemir, A Kim, SH AF Alazizi, Ala Smith, David Erdemir, Ali Kim, Seong H. TI Silane Treatment of Diamond-Like Carbon: Improvement of Hydrophobicity, Oleophobicity, and Humidity Tolerance of Friction SO TRIBOLOGY LETTERS LA English DT Article DE Diamond-like carbon; DLC; Humidity tolerance; Silane treatment ID TRIBOLOGICAL MOISTURE SENSITIVITY; CHEMICAL-VAPOR-DEPOSITION; RUN-IN BEHAVIOR; WATER-ADSORPTION; INTERNAL-STRESS; FILMS; WEAR; LUBRICATION; SI; SURFACES AB Hydrophobicity and humidity tolerance of the low friction behavior of hydrogenated diamond-like carbon (H-DLC) were improved via surface modification using vapor-phase chemical reactions with organic silanes at 250-280 degrees C. Water and hexadecane contact angles increased after silane treatments. Unlike pristine H-DLC which loses ultra-low friction behavior as soon as relative humidity (RH) increases to a few percent, silane-treated H-DLC films maintained a low friction behavior (with a coefficient less than 0.08) up to 30 % RH. Elemental analysis of the transfer films accumulated on the balls after friction tests indicated that the silane molecules not only decorated the topmost surface of the H-DLC, but also penetrated into and reacted with the subsurface. Surface roughness, water adsorption behavior, and hardness measurements also showed that silane treatment affected the surface morphology and subsurface porosity of the H-DLC film. C1 [Alazizi, Ala; Kim, Seong H.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Alazizi, Ala; Kim, Seong H.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Smith, David] SilcoTek Corp, Bellefonte, PA 16823 USA. [Erdemir, Ali] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Kim, SH (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA.; Kim, SH (reprint author), Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. EM shkim@engr.psu.edu FU National Science Foundation [CMMI-1131128]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation (Grant No. CMMI-1131128). Additional support was provided by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office under Contract DE-AC02-06CH11357. The authors acknowledged Dr. Osman Eryilmaz for preparing H-DLC samples on silicon substrates for this study. NR 50 TC 0 Z9 0 U1 13 U2 13 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1023-8883 EI 1573-2711 J9 TRIBOL LETT JI Tribol. Lett. PD SEP PY 2016 VL 63 IS 3 AR 43 DI 10.1007/s11249-016-0733-4 PG 11 WC Engineering, Chemical; Engineering, Mechanical SC Engineering GA DU7KD UT WOS:000382392200014 ER PT J AU Dwivedi, D Mohanty, BP Lesikar, BJ AF Dwivedi, Dipankar Mohanty, Binayak P. Lesikar, Bruce J. TI Impact of the Linked Surface Water-Soil Water-Groundwater System on Transport of E. coli in the Subsurface SO WATER AIR AND SOIL POLLUTION LA English DT Article DE E. coli transport; Seasonal variability; Septic tanks; Surface water and groundwater interaction ID SATURATED POROUS-MEDIA; ALLUVIAL GRAVEL AQUIFER; ESCHERICHIA-COLI; SAND COLUMNS; CRYPTOSPORIDIUM OOCYSTS; HYDRAULIC CONDUCTIVITY; BACTERIAL TRANSPORT; VIRUS TRANSPORT; MODEL; FILTRATION AB Escherichia coli (E. coli) contamination of groundwater (GW) and surface water (SW) occurs significantly through the subsurface from onsite wastewater treatment systems (OWTSs). However, E. coli transport in the subsurface remains inadequately characterized at the field scale, especially within the vadose zone. Therefore, the aim of this research is to investigate the impact of groundwater fluctuations (e.g., recharging, discharging conditions) and variable conditions in the vadose zone (e.g., pulses of E. coli flux) by characterizing E. coli fate and transport in a linked surface watersoil water-groundwater system (SW-SoW-GW). In particular, this study characterizes the impact of flow regimes on E. coli transport in the subsurface and evaluates the sensitivity of parameters that control the transport of E. coli in the SW-SoW-GW system. This study was conducted in Lake Granbury, which is an important water supply in north-central Texas providing water for over 250,000 people. Results showed that there was less removal of E. coli during groundwater recharge events as compared to GW discharge events. Also, groundwater and surface water systems largely control E. coli transport in the subsurface; however, temporal variability of E. coli can be explained by linking the SW-SoW-GW system. Moreover, sensitivity analysis revealed that saturated water content of the soil, total retention rate coefficient, and hydraulic conductivity are important parameters for E. coli transport in the subsurface. C1 [Dwivedi, Dipankar] Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. [Dwivedi, Dipankar; Mohanty, Binayak P.; Lesikar, Bruce J.] Texas A&M Univ, Dept Biol & Agr Engn, College Stn, TX 77843 USA. [Lesikar, Bruce J.] Kaselco LLC Texas, Shiner, TX 77984 USA. RP Dwivedi, D (reprint author), Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. EM DDwivedi@lbl.gov FU EPA 319(h) grant; National Institute of Environmental Health Sciences [5R01ES015634]; Texas Water Resources Institute; Texas AM [02-130003] FX This research was supported by EPA 319(h) grant for TMDL in Texas streams and partly supported by the National Institute of Environmental Health Sciences (grant 5R01ES015634), Texas Water Resources Institute, and Texas A&M support a/c 02-130003. The content is solely the responsibility of the authors and does not necessarily represent the official views of the funding agencies. NR 73 TC 0 Z9 0 U1 17 U2 17 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0049-6979 EI 1573-2932 J9 WATER AIR SOIL POLL JI Water Air Soil Pollut. PD SEP PY 2016 VL 227 IS 9 AR 351 DI 10.1007/s11270-016-3053-2 PG 16 WC Environmental Sciences; Meteorology & Atmospheric Sciences; Water Resources SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences; Water Resources GA DV2OY UT WOS:000382761400059 ER PT J AU Cardenas, AJP O'Hagan, M AF Cardenas, Allan Jay P. O'Hagan, Molly TI Crystal structure of dimethylformamidium bis(trifluoromethanesulfonyl)amide: an ionic liquid SO ACTA CRYSTALLOGRAPHICA SECTION E-CRYSTALLOGRAPHIC COMMUNICATIONS LA English DT Article DE crystal structure; ionic liquid; electrolyte; hydrogen bond AB At 100 K, the title molecular salt, C3H8NO+center dot C2F6NO4S2-, has orthorhombic (P2(1)2(1)2(1)) symmetry; the amino H atom of bis(trifluoromethanesulfonyl) amine (HNTf2) was transferred to the basic O atom of dimethylformamide (DMF) when the ionic liquid components were mixed. The structure displays an O-H center dot center dot center dot N hydrogen bond, which links the cation to the anion, which is reinforced by a non-conventional C-H center dot center dot center dot O interaction, generating an R-2(2) (7) loop. A further very weak C-H center dot center dot center dot O interaction generates an [001] chain. C1 [Cardenas, Allan Jay P.; O'Hagan, Molly] Pacific Northwest Natl Lab, POB 999 MSIN K2-57, Richland, WA 99352 USA. RP O'Hagan, M (reprint author), Pacific Northwest Natl Lab, POB 999 MSIN K2-57, Richland, WA 99352 USA. EM Molly.OHagan@pnnl.gov NR 9 TC 0 Z9 0 U1 0 U2 0 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2056-9890 J9 ACTA CRYSTALLOGR E JI Acta Crystallogr. Sect. E.-Crystallogr. Commun. PD SEP PY 2016 VL 72 BP 1290 EP + DI 10.1107/S2056989016012251 PN 9 PG 7 WC Crystallography SC Crystallography GA DU6CL UT WOS:000382301000016 PM 27920919 ER PT J AU Hong, YC Hensley, A McEwen, JS Wang, Y AF Hong, Yongchun Hensley, Alyssa McEwen, Jean-Sabin Wang, Yong TI Perspective on Catalytic Hydrodeoxygenation of Biomass Pyrolysis Oils: Essential Roles of Fe-Based Catalysts SO CATALYSIS LETTERS LA English DT Article DE Biofuel; Hydrodeoxygenation Lignin; Fe catalyst; Bimetallic catalyst; Pyrolysis oil ID GAS-PHASE HYDRODEOXYGENATION; H-2 DISSOCIATIVE ADSORPTION; FISCHER-TROPSCH SYNTHESIS; 1ST PRINCIPLES; BIO-OIL; M-CRESOL; GUAIACOL HYDRODEOXYGENATION; HYDROPROCESSING CATALYSTS; HYDROTREATING CATALYSTS; BIODIESEL PRODUCTION AB Catalytic fast pyrolysis is the most promising approach for biofuel production due to its simple process and versatility to handle lignocellulosic biomass feedstocks with varying and complex compositions. Compared with in situ catalytic fast pyrolysis, ex situ catalytic pyrolysis has the flexibility of optimizing the pyrolysis step and catalytic process individually to improve the quality of pyrolysis oil (stability, oxygen content, acid number, etc.) and to maximize the carbon efficiency in the conversion of biomass to pyrolysis oil. Hydrodeoxygenation is one of the key catalytic functions in ex situ catalytic fast pyrolysis. Recently, Fe-based catalysts have been reported to exhibit superior catalytic properties in the hydrodeoxygenation of model compounds in pyrolysis oil, which potentially makes the ex situ pyrolysis of biomass commercially viable due to the abundance and low cost of Fe. Here, we briefly summarize the recent progress on Fe-based catalysts for the hydrodeoxygenation of biomass, and provide perspectives on how to further improve Fe-based catalysts (activity and stability) for their potential applications in the emerging area of biomass conversion. C1 [Hong, Yongchun; Hensley, Alyssa; McEwen, Jean-Sabin; Wang, Yong] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Hong, Yongchun; Wang, Yong] Pacific Northwest Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [McEwen, Jean-Sabin] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [McEwen, Jean-Sabin] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. RP Wang, Y (reprint author), Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA.; Wang, Y (reprint author), Pacific Northwest Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. EM yong.wang@pnnl.gov FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-05ER15712, DE-SC0014560]; Department of Energy's Office of Biological and Environmental Research FX Y. W. and Y. H. acknowledge the financial support from the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under award numbers DE-FG02-05ER15712. J.-S. M. and A. H. acknowledge the financial support from the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under award number DE-SC0014560. A portion of the research was performed at Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). NR 129 TC 1 Z9 1 U1 39 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1011-372X EI 1572-879X J9 CATAL LETT JI Catal. Lett. PD SEP PY 2016 VL 146 IS 9 BP 1621 EP 1633 DI 10.1007/s10562-016-1770-1 PG 13 WC Chemistry, Physical SC Chemistry GA DU2AD UT WOS:000382011600001 ER PT J AU Magee, JW Palomino, RM White, MG AF Magee, Joseph W. Palomino, Robert M. White, Michael G. TI Infrared Spectroscopy Investigation of Fe-Promoted Rh Catalysts Supported on Titania and Ceria for CO Hydrogenation SO CATALYSIS LETTERS LA English DT Article DE Heterogeneous catalysis; Infrared spectroscopy; CO Hydrogenation; FeRh alloy; Ethanol ID WATER-GAS-SHIFT; CARBON-MONOXIDE; HIGH-PRESSURE; RHODIUM CATALYSTS; SIO2-SUPPORTED RH; ETHANOL SYNTHESIS; IRON CATALYSTS; FT-IR; SYNGAS; ADSORPTION AB The nature of the promotional effect of Fe addition to Rh/TiO2 and Rh/CeO2 catalysts for CO hydrogenation was investigated using FT-IR spectroscopy in an ultrahigh vacuum compatible transmission IR cell. CO adsorption experiments on Rh and FeRh showed vibrational signatures characteristic of linear and bridge bound CO on Rh-0 as well as geminal-dicarbonyl species associated with Rh+. Compared to TiO2, the CeO2-supported catalysts show increased dispersion, reflected by decreased particle size, and a lower signal for linear versus geminal-dicarbonyl bonded CO. The absorption frequencies for CO on Rh/CeO2 are also redshifted relative to Rh/TiO2, which results from a weaker Rh-CO interaction, likely due to the increased reducibility of the CeO2 support. Upon addition of Fe, a new spectral feature is observed and attributed to CO bound to Rh in close contact with Fe, likely as a surface alloy. CO hydrogenation on (Fe)Rh catalysts on both supports was also studied. Compared to bare Rh, Fe containing catalysts promote formate and methoxy species on the surface at lower temperature (180 A degrees C), which suggests an enhancement in methanol selectivity by Fe addition. At higher temperatures (220 A degrees C), the spectral features appear similar, further confirming the role of Fe as a disrupter of large Rh-0 crystallites and regulator of CO dissociation and CH4 formation. C1 [Magee, Joseph W.; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Palomino, Robert M.; White, Michael G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP White, MG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; White, MG (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM jmagee@bnl.gov; rpalomino@bnl.gov; mgwhite@bnl.gov OI Palomino, Robert/0000-0003-4476-3512 FU Brookhaven National Laboratory [DE-SC0012704]; Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences FX The work was carried out at Brookhaven National Laboratory under Contract No. DE-SC0012704 with the U.S Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences. The authors gratefully acknowledge Dr. Jordi Llorca of the Technical University of Catalonia (Barcelona, Spain) for performing electron microscopy characterization of the catalysts used in these experiments. NR 47 TC 0 Z9 0 U1 17 U2 25 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1011-372X EI 1572-879X J9 CATAL LETT JI Catal. Lett. PD SEP PY 2016 VL 146 IS 9 BP 1771 EP 1779 DI 10.1007/s10562-016-1801-y PG 9 WC Chemistry, Physical SC Chemistry GA DU2AD UT WOS:000382011600014 ER PT J AU Dane, M Gonis, A AF Dane, Markus Gonis, Antonios TI On the v-Representabilty Problem in Density Functional Theory: Application to Non-Interacting Systems SO COMPUTATION LA English DT Article DE density functional theory; v-representability; constrained search ID SELF-INTERACTION PROBLEM; UPSILON-REPRESENTABILITY; ELECTRON-DENSITIES; CONSTRUCTION; ORBITALS AB Based on a computational procedure for determining the functional derivative with respect to the density of any antisymmetric N- particle wave function for a non-interacting system that leads to the density, we devise a test as to whether or not a wave function known to lead to a given density corresponds to a solution of a Schrdinger equation for some potential. We examine explicitly the case of non-interacting systems described by Slater determinants. Numerical examples for the cases of a one-dimensional square-well potential with infinite walls and the harmonic oscillator potential illustrate the formalism. C1 [Dane, Markus; Gonis, Antonios] Lawrence Livermore Natl Lab, POB 808,L-372, Livermore, CA 94551 USA. RP Dane, M (reprint author), Lawrence Livermore Natl Lab, POB 808,L-372, Livermore, CA 94551 USA. EM daene1@llnl.gov; gonis1@llnl.gov RI Dane, Markus/H-6731-2013 OI Dane, Markus/0000-0001-9301-8469 NR 22 TC 1 Z9 1 U1 3 U2 3 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 2079-3197 J9 COMPUTATION JI Computation PD SEP PY 2016 VL 4 IS 3 AR 24 DI 10.3390/computation4030024 PG 13 WC Mathematics, Interdisciplinary Applications SC Mathematics GA DU8RB UT WOS:000382480300002 ER PT J AU Houde, S Spurlock, CA AF Houde, Sebastien Spurlock, C. Anna TI Minimum Energy Efficiency Standards for Appliances: Old and New Economic Rationales SO ECONOMICS OF ENERGY & ENVIRONMENTAL POLICY LA English DT Article DE Appliances; Minimum Energy Efficiency Standards; Energy Efficiency Policy ID FUEL-ECONOMY; QUALITY STANDARDS; DISCOUNT RATES; GASOLINE PRICES; COMPETITION; COSTS; CONSUMPTION; INNOVATION; PURCHASE; POLICIES AB We revisit Hausman and Joskow (1982)'s economic rationales for appliance minimum energy efficiency standards. In addition to the four market failures they argued could justify appliance standards energy prices below marginal social cost, consumers underestimating energy prices, consumer discount rates above social discount rates, and principal-agent problems we discuss two additional market failures that are relevant and potentially economically important in this context: market power and innovation market failures. We highlight puzzles uncovered by recent empirical results, and suggest directions future research should take to better understand the normative implications of appliance standards. C1 [Houde, Sebastien] Univ Maryland, Dept Agr & Resource Econ, College Pk, MD 20742 USA. [Spurlock, C. Anna] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Houde, S (reprint author), Univ Maryland, Dept Agr & Resource Econ, College Pk, MD 20742 USA. EM shoude@umd.edu; caspurlock@lbl.gov FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Thank you to Catherine Wolfram, Paul Joskow, Louis-Gaetan Giraudet, Larry Dale, and Louis-Benoit Desroches for comments and suggestions. NR 68 TC 0 Z9 0 U1 4 U2 4 PU INT ASSOC ENERGY ECONOMICS PI CLEVELAND PA 28790 CHAGRIN BLVD, STE 210, CLEVELAND, OH 44122 USA SN 2160-5882 EI 2160-5890 J9 ECON ENERGY ENV POL JI Econ. Energy Environ. Policy PD SEP PY 2016 VL 5 IS 2 BP 65 EP 83 DI 10.5547/2160-5890.5.2.shou PG 19 WC Economics; Environmental Studies SC Business & Economics; Environmental Sciences & Ecology GA DU3HL UT WOS:000382101300005 ER PT J AU Fleck, SC Churchwell, MI Doerge, DR Teeguarden, JG AF Fleck, Stefanie C. Churchwell, Mona I. Doerge, Daniel R. Teeguarden, Justin G. TI Urine and serum biomonitoring of exposure to environmental estrogens II: Soy isoflavones and zearalenone in pregnant women SO FOOD AND CHEMICAL TOXICOLOGY LA English DT Article DE Soy isoflavones; Zearalenone; Exposure; Pregnancy; Biomonitoring; Endocrine disruptors ID SPRAGUE-DAWLEY RATS; BREAST-CANCER RISK; PHYSIOLOGICAL CONCENTRATIONS; MYCOTOXIN EXPOSURE; PLACENTAL-TRANSFER; RECEPTOR-ALPHA; GENISTEIN; DIETARY; GROWTH; PHARMACOKINETICS AB Urine and serum biomonitoring was used to measure internal exposure to selected dietary estrogens in a cohort of 30 pregnant women. Exposure was measured over a period comprising one-half day in the field (6 h) and one day in a clinic (24 h). Biomonitoring of the dietary phytoestrogens genistein (GEN), daidzein (DDZ) and equol (EQ), as well as the mycoestrogen, zearalenone (ZEN) and its congeners, was conducted using UPLC-MS/MS. Biomonitoring revealed evidence of internal exposure to naturally occurring dietary estrogens during pregnancy. Urinary concentrations of total GEN, DDZ and EQ were similar to levels reported for general adult U.S. population. Measurable concentrations of total (parent and metabolites) GEN, DDZ and EQ were present in 240, 207 and 2 of 270 serum samples, respectively. Six out of 30 subjects had measurable concentrations of unconjugated GEN and/or DDZ in serum between 0.6 and 7.1 nM. Urine to serum total isoflavone ratios for GEN, DDZ and EQ were 13, 47, and 180, respectively. ZEN and its reductive metabolite, alpha-zearalenol (alpha-ZEL), were present in pregnant women (11 out of 30 subjects) as conjugates at levels near the limit of quantification. The average total urinary concentration was 0.10 mu g/L for ZEN and 0.11 mu g/L for alpha-ZEL. (C) 2016 Published by Elsevier Ltd. C1 [Fleck, Stefanie C.; Churchwell, Mona I.; Doerge, Daniel R.] US FDA, Div Biochem Toxicol, Natl Ctr Toxicol Res, Jefferson, AR 72079 USA. [Teeguarden, Justin G.] Pacific Northwest Natl Lab, Hlth Effects & Exposure Sci, Richland, WA 99352 USA. [Teeguarden, Justin G.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97331 USA. RP Teeguarden, JG (reprint author), 902 Battelle Blvd, Richland, WA 99352 USA. EM stefanie.fleck@fda.hhs.gov; mona.churchwell@fda.hhs.gov; daniel.doerge@fda.hhs.gov; jt@pnnl.gov NR 46 TC 1 Z9 1 U1 13 U2 15 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0278-6915 EI 1873-6351 J9 FOOD CHEM TOXICOL JI Food Chem. Toxicol. PD SEP PY 2016 VL 95 BP 19 EP 27 DI 10.1016/j.fct.2016.05.021 PG 9 WC Food Science & Technology; Toxicology SC Food Science & Technology; Toxicology GA DT9PX UT WOS:000381835900003 PM 27255803 ER PT J AU Bowman, WM Bowman, JD AF Bowman, Warigia M. Bowman, J. David TI Censorship or self-control? Hate speech, the state and the voter in the Kenyan election of 2013 SO JOURNAL OF MODERN AFRICAN STUDIES LA English DT Article ID SOCIAL MEDIA; POLITICAL-CHANGE; INTERNET; MOBILIZATION; VIOLENCE; DEMOCRATIZATION; AFRICA AB In 2013, the Kenyan government adopted a hybrid censorship strategy that relied on regulation, the presence of a strong security state, and the willingness of Kenyans to self-censor. The goal of this censorship strategy was to ensure a peaceful election. This study examines two issues. First, it investigates steps taken by the Kenyan government to minimise hate speech. Second, it explores how efforts to minimise hate speech affected citizen communications over SMS during the 2013 election. An initial round of qualitative data was gathered (n = 101) through a structured exit interview administered election week. A statistically significant, representative sample of quantitative data was gathered by a reputable Kenyan polling firm (n 2000). Both sets of empirical data indicate that Kenyan citizens cooperated in large part with efforts to limit political speech. Yet speech was not always completely peaceful'. Rather, voters used electronic media to insult, offend, and express contentious political views as well as express peace speech. This study argues that the empirical evidence suggests hate speech over text messages during the Kenyan election declined between 2008 and 2013. C1 [Bowman, Warigia M.] Univ Arkansas, Clinton Sch Publ Serv, 1200 President Clinton Ave, Little Rock, AR 72201 USA. [Bowman, J. David] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Bowman, WM (reprint author), Univ Arkansas, Clinton Sch Publ Serv, 1200 President Clinton Ave, Little Rock, AR 72201 USA. EM wbowman@clintonschool.uasys.edu; bowmanjd@ornl.gov FU University of Arkansas Clinton School of Public Service FX We wish to express our deepest gratitude for the work of our colleagues on the Kenya Information Communications Technology List ('Kictanet'). Specifically, we would like to thank our colleagues Michael Kipsang Bullut, Grace Githaiga, Wambui Ngugi, Brian Munyao Longwe, Mwendwa Kivuva, Abraham Mulwo, Muchiri Nyaggah, and Norbert Wildermuth for helping to collect the data that form the foundation of this paper. Thank you also to the University of Arkansas Clinton School of Public Service for funding part of the research upon which this paper is based. We would also like to thank participants of the Kenya Elections Workshop held in June 2013 for their comments, which helped improve this paper. We are particularly grateful to Tom Wolf of IPSOS Synovate. We would also like to thank Dorina Bekoe, Fodei Batty, Paola Cavallari and Florence Muema as well as two anonymous reviewers from JMAS for their valuable insights. Finally, my thanks go to Kimani Njogu of Twaweza Publishing, for his elegant Kiswahili translations. NR 53 TC 0 Z9 0 U1 7 U2 7 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0022-278X EI 1469-7777 J9 J MOD AFR STUD JI J. Mod. Afr. Stud. PD SEP PY 2016 VL 54 IS 3 BP 495 EP 531 DI 10.1017/S0022278X16000380 PG 37 WC Area Studies SC Area Studies GA DU7FR UT WOS:000382379300006 ER PT J AU Duenas, ME Carlucci, L Lee, YJ AF Duenas, Maria Emilia Carlucci, Laura Lee, Young Jin TI Matrix Recrystallization for MALDI-MS Imaging of Maize Lipids at High-Spatial Resolution SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE Mass spectrometry imaging; MALDI; Matrix; Recrystallization; Maize; Lipids; High spatial resolution ID MASS-SPECTROMETRY; LATENT FINGERMARKS; TOF MS; TISSUE; SUBLIMATION; METABOLITES; EFFICIENCY AB Matrix recrystallization is optimized and applied to improve lipid ion signals in maize embryos and leaves. A systematic study was performed varying solvent and incubation time. During this study, unexpected side reactions were found when methanol was used as a recrystallization solvent, resulting in the formation of a methyl ester of phosphatidic acid. Using an optimum recrystallization condition with isopropanol, there is no apparent delocalization demonstrated with a transmission electron microscopy (TEM) pattern and maize leaf images obtained at 10 mu m spatial resolution. C1 [Duenas, Maria Emilia; Carlucci, Laura; Lee, Young Jin] US DOE, Ames Lab, Ames, IA 50011 USA. [Duenas, Maria Emilia; Lee, Young Jin] Iowa State Univ Sci & Technol, Dept Chem, Ames, IA 50011 USA. RP Lee, YJ (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.; Lee, YJ (reprint author), Iowa State Univ Sci & Technol, Dept Chem, Ames, IA 50011 USA. EM yjlee@iastate.edu FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE [DE-AC02-07CH11358] FX The authors acknowledge support for this work by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The Ames Laboratory is operated by Iowa State University under DOE Contract DE-AC02-07CH11358. NR 13 TC 0 Z9 0 U1 11 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 EI 1879-1123 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD SEP PY 2016 VL 27 IS 9 BP 1575 EP 1578 DI 10.1007/s13361-016-1422-0 PG 4 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA DT1YR UT WOS:000381278500016 PM 27349253 ER PT J AU Bannister, ME Meyer, FW Hijazi, H Unocic, KA Garrison, LM Parish, CM AF Bannister, M. E. Meyer, F. W. Hijazi, H. Unocic, K. A. Garrison, L. M. Parish, C. M. TI Surface morphologies of He-implanted tungsten SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 21st International Workshop on Inelastic Ion-Surface Collisions (IISC) CY OCT 18-23, 2015 CL Donostia San Sebastian, SPAIN DE He nanofuzz formation; Tungsten surface modification; Plasma wall interactions ID THERMAL-DESORPTION; HELIUM AB Surface morphologies of tungsten surfaces, both polycrystalline and single-crystal [1 1 0], were investigated using SEM and FIB/SEM techniques after implantations at elevated surfaces temperatures (1200-1300 K) using well-characterized, mono-energetic He ion beams with a wide range of ion energies (218 eV-250 keV). Nanofuzz was observed on polycrystalline tungsten (PCW) following implantation of 100-keV He ions at a flux threshold of 0.9 x 10(16) cm(-2) s(-1), but not following 200-keV implantations with similar fluxes. No nanofuzz formation was observed on single-crystal [1 1 0] tungsten (SCW), despite fluxes exceeding those demonstrated previously to produce nanofuzz on polycrystalline tungsten. Pre-damaging the single-crystal tungsten with implanted C impurity interstitials did not significantly affect the, surface morphologies resulting from the high-flux He ion implantations. The main factor leading to the different observed surface structures for the pristine and C-implanted single-crystal W samples appeared to be the peak He ion flux characterizing the different exposures. It was speculated that nano fuzz formation was not observed for any SCW target exposures because of increased incubation fluences required for such targets. (C) 2016 Published by Elsevier B.V. C1 [Bannister, M. E.; Meyer, F. W.; Hijazi, H.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Unocic, K. A.; Garrison, L. M.; Parish, C. M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. [Hijazi, H.] Aix Marseille Univ, CNRS, PIIM UMR 7345, F-13397 Marseille, France. RP Bannister, ME (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. EM bannisterme@ornl.gov RI Parish, Chad/J-8381-2013; Garrison, Lauren/S-2526-2016; OI Garrison, Lauren/0000-0002-5673-8333; Bannister, Mark E./0000-0002-9572-8154 NR 30 TC 0 Z9 0 U1 6 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD SEP 1 PY 2016 VL 382 BP 76 EP 81 DI 10.1016/j.nimb.2016.05.003 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DU7RY UT WOS:000382413500015 ER PT J AU Dong, T Van Wychen, S Nagle, N Pienkos, PT Laurens, LML AF Dong, T. Van Wychen, S. Nagle, N. Pienkos, P. T. Laurens, L. M. L. TI Impact of biochemical composition on susceptibility of algal biomass to acid-catalyzed pretreatment for sugar and lipid recovery SO ALGAL RESEARCH-BIOMASS BIOFUELS AND BIOPRODUCTS LA English DT Article DE Algae; Biorefinery; Biomass composition; Lipids; Carbohydrates; Bioethanol; Renewable diesel; Process economics ID HIGH-PRESSURE HOMOGENIZATION; CELL DISRUPTION; ASSISTED EXTRACTION; BIOFUELS PRODUCTION; CHLORELLA-VULGARIS; MICROALGAE; OIL; HYDROLYSIS; PARAMETERS; ULTRASOUND AB One of the major challenges associated with algal biofuels production in a biorefinery-type setting is improving biomass utilization in its entirety, increasing the process energetic yields and providing economically viable and scalable co-product concepts. We focus on the impact of compositional characteristics of biomass on the susceptibility to pretreatment in order to maximize the valorization of algal biomass conversion for biofuels and bioproducts. The release of monomeric carbohydrates in the aqueous phase and extractability of the lipid fraction was measured based a response surface methodology to find significant explanatory variables and interaction terms. We studied the effect of harvest timing on the conversion yields, using three algal strains; Chlorella vulgaris and Scenedesmus acutus and Nannochloropsis granulata representing three different nutritionalmetabolic phases. Four cultivation conditions of high (>= 90 gallon gasoline equivalent/ton biomass) value for a combined sugar- and lipid-based biofuels process were identified. These four conditions represent eithermid or late stage harvest cultivation regimes. The results indicate that acid pretreatment has potential to be applicable for a vast range of biomass samples to obtain high energy yields, but that the exact conditions and optima are dependent on the strain and likely the starting composition of the biomass. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Dong, T.; Van Wychen, S.; Nagle, N.; Pienkos, P. T.; Laurens, L. M. L.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Laurens, LML (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Lieve.Laurens@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy as part of the BioEnergy Technology Office (BETO) [1.3.4.300, 1.3.1.200, 1.3.4.201]; National Renewable Energy, Sustainable Algal Biofuels Consortium project - DOE [DE-EE0003372] FX We thank Drs. JohnMcGowen and Thomas Dempster (AzCATI, ASU, Mesa, AZ) for providing the biomass used for this work. We acknowledge technical assistance from Nicholas Sweeney and Deborah Hyman for the help with microscopy and HPLC analysis of carbohydrates, respectively, for this work. The work presented here was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy as part of the BioEnergy Technology Office (BETO) task #1.3.4.300, 1.3.1.200 and 1.3.4.201, and as part of the Sustainable Algal Biofuels Consortium project, funded under DOE Award # DE-EE0003372. NR 29 TC 0 Z9 0 U1 16 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-9264 J9 ALGAL RES JI Algal Res. PD SEP PY 2016 VL 18 BP 69 EP 77 DI 10.1016/j.algal.2016.06.004 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DT8NV UT WOS:000381748800009 ER PT J AU Novoveska, L Zapata, AKM Zabolotney, JB Atwood, MC Sundstrom, ER AF Novoveska, Lucie Zapata, Anastasia K. M. Zabolotney, Jeffrey B. Atwood, Matthew C. Sundstrom, Eric R. TI Optimizing microalgae cultivation and wastewater treatment in large-scale offshore photobioreactors SO ALGAL RESEARCH-BIOMASS BIOFUELS AND BIOPRODUCTS LA English DT Article DE Microalgae cultivation; Polyculture; Wastewater treatment; Offshore photobioreactors; Biofuel ID ALGAL BIOFUEL PRODUCTION; PHYTOPLANKTON COMMUNITIES; DIVERSITY; COMPETITION; STABILITY; BIODIESEL; DEMAND; BATCH AB Algae Systems LLC has designed and implemented a novel approach to wastewater treatment in which municipal wastewater is used to cultivate microalgae in modular, offshore photobioreactors (PBRs). At the Algae Systems plant in Daphne AL, this process was used to treat up to 50,000 gal/day of incoming raw wastewater. A combination of algae nutrient uptake, aeration by photosynthetically produced oxygen, and dewatering via suspended air flotation removed 75% of total nitrogen, 93% of total phosphorus and 92% BOD from influent wastewater. Offshore PBRs contained evolving polycultures of microalgae and associated heterotrophs, with community composition shifting based on the dynamic external and internal environment. During one year of operation, microalgae composition shifted from dominance of Scenedesmus dimorphus to a diverse polyculture dominated by genus Chlorella, Cryptomonas and Scenedesmus. "The more, the merrier" approach to species richness produced resilient communities, enabling efficient nutrient uptake due to niche complementarity and eliminating process downtime due to biological disruptions. The resulting biomass was suitable for fuel conversion via hydrothermal liquefaction due to consistent lipid content, low ash content, and consistent elemental composition. Biomass production rates ranged from 3.5 to 22.7 g/m(2)/day during continuous operation, with productivity predominantly driven by temperature and frequency of harvest. (C) 2016 Elsevier B.V. All rights reserved. C1 [Novoveska, Lucie; Zapata, Anastasia K. M.; Zabolotney, Jeffrey B.; Atwood, Matthew C.; Sundstrom, Eric R.] Algae Syst LLC, 6321 Jordan Rd, Daphne, AL 36526 USA. [Zabolotney, Jeffrey B.] Univ S Alabama, Dept Biol, Mobile, AL 36688 USA. [Novoveska, Lucie] Dauphin Isl Sea Lab, 101 Bienville Blvd, Dauphin Isl, AL 36528 USA. [Zapata, Anastasia K. M.] Algae Energy, 2460 Ind Pk Blvd, Cumming, GA 30041 USA. [Sundstrom, Eric R.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Novoveska, L (reprint author), Algae Syst LLC, 6321 Jordan Rd, Daphne, AL 36526 USA.; Novoveska, L (reprint author), Dauphin Isl Sea Lab, 101 Bienville Blvd, Dauphin Isl, AL 36528 USA. FU Algae Systems LLC FX Funding was provided by Algae Systems LLC. We would like to thank our talented offshore crew and the operation team. Tom Dempster (AzCATI) and Eric Brunden provided valuable insight. We thank Daphne Utilities for their continuous support. We also thank two anonymous reviewers for their critical contributions to the manuscript. NR 52 TC 4 Z9 4 U1 29 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-9264 J9 ALGAL RES JI Algal Res. PD SEP PY 2016 VL 18 BP 86 EP 94 DI 10.1016/j.algal.2016.05.033 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DT8NV UT WOS:000381748800011 ER PT J AU Pegallapati, AK Frank, ED AF Pegallapati, Ambica K. Frank, Edward D. TI Energy use and greenhouse gas emissions from an algae fractionation process for producing renewable diesel SO ALGAL RESEARCH-BIOMASS BIOFUELS AND BIOPRODUCTS LA English DT Article DE Algae; Life-cycle analysis; Greenhouse gas emissions; Biofuels; Renewable energy ID BIOFUELS AB In one approach to algal biofuel production, lipids are extracted and converted to renewable diesel and non-lipid remnants are converted to biogas, which is used for renewable heat and power to support the process. Since biofuel economics benefit from increased fuel yield, the National Renewable Energy Laboratory analyzed an alternative pathway that extracts lipids and also makes ethanol from carbohydrates in the biomass. In this paper, we examine the environmental sustainability of this "fractionation pathway" through life-cycle analysis (LCA) of greenhouse gas emissions and energy use. When the feedstock productivity was 30 (18) g/m(2)/d, this pathway emitted 31 (36) gCO(2)e/MJ of total fuel, which is less than the emissions associated with conventional low sulfur petroleum diesel (96 gCO(2)e/MJ). The fractionation pathway performed well in this model despite the diversion of carbon to the ethanol fuel. (C) 2016 Elsevier B.V. All rights reserved. C1 [Pegallapati, Ambica K.; Frank, Edward D.] Argonne Natl Lab, Ctr Transportat Res, 9700 South Cass Ave, Argonne, IL 60439 USA. RP Frank, ED (reprint author), Argonne Natl Lab, Ctr Transportat Res, 9700 South Cass Ave, Argonne, IL 60439 USA. EM apegallapati@anl.gov; efrank@anl.gov FU Bioenergy Technologies Office in the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy; Argonne, a US Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX We would like to thank Ryan Davis and Jennifer Markham from the National Renewable Energy Laboratory for data and for helpful comments. This work was sponsored by the Bioenergy Technologies Office in the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a US Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The US Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 12 TC 0 Z9 0 U1 15 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-9264 J9 ALGAL RES JI Algal Res. PD SEP PY 2016 VL 18 BP 235 EP 240 DI 10.1016/j.algal.2016.06.019 PG 6 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DT8NV UT WOS:000381748800026 ER PT J AU Qiu, DR Xie, M Dai, JC An, WX Wei, HH Tian, CY Kempher, ML Zhou, AF He, ZL Gu, BH Zhou, JZ AF Qiu, Dongru Xie, Ming Dai, Jingcheng An, Weixing Wei, Hehong Tian, Chunyuan Kempher, Megan L. Zhou, Aifen He, Zhili Gu, Baohua Zhou, Jizhong TI Differential Regulation of the Two Ferrochelatase Paralogues in Shewanella loihica PV-4 in Response to Environmental Stresses SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID HEME-BIOSYNTHESIS PATHWAY; LIGHT-SENSITIVE MUTANTS; PROTOPORPHYRIN-IX; ESCHERICHIA-COLI; ONEIDENSIS MR-1; SYSTEMS BIOLOGY; SIGMA-FACTORS; GENES; GENUS; IDENTIFICATION AB Determining the function and regulation of paralogues is important in understanding microbial functional genomics and environmental adaptation. Heme homeostasis is crucial for the survival of environmental microorganisms. Most Shewanella species encode two paralogues of ferrochelatase, the terminal enzyme in the heme biosynthesis pathway. The function and transcriptional regulation of two ferrochelatase genes, hemH1 and hemH2, were investigated in Shewanella loihica PV-4. The disruption of hemH1 but not hemH2 resulted in a significant accumulation of extracellular protoporphyrin IX (PPIX), the precursor to heme, and decreased intracellular heme levels. hemH1 was constitutively expressed, and the expression of hemH2 increased when hemH1 was disrupted. The transcription of hemH1 was regulated by the housekeeping sigma factor RpoD and potentially regulated by OxyR, while hemH2 appeared to be regulated by the oxidative stress-associated sigma factor RpoE2. When an oxidative stress condition was mimicked by adding H2O2 to the medium or exposing the culture to light, PPIX accumulation was suppressed in the Delta hemH1 mutant. Consistently, transcriptome analysis indicated enhanced iron uptake and suppressed heme synthesis in the Delta hemH1 mutant. These data indicate that the two paralogues are functional in the heme synthesis pathway but regulated by environmental conditions, providing insights into the understanding of bacterial response to environmental stresses and a great potential to commercially produce porphyrin compounds. IMPORTANCE Shewanella is capable of utilizing a variety of electron acceptors for anaerobic respiration because of the existence of multiple c-type cytochromes in which heme is an essential component. The cytochrome-mediated electron transfer across cellular membranes could potentially be used for biotechnological purposes, such as electricity generation in microbial fuel cells and dye decolorization. However, the mechanism underlying the regulation of biosynthesis of heme and cytochromes is poorly understood. Our study has demonstrated that two ferrochelatase genes involved in heme biosynthesis are differentially regulated in response to environmental stresses, including light and reactive oxygen species. This is an excellent example showing how bacteria have evolved to maintain cellular heme homeostasis. More interestingly, the high yields of extracellular protoporphyrin IX by the Shewanella loihica PV-4 mutants could be utilized for commercial production of this valuable chemical via bacterial fermentation. C1 [Qiu, Dongru; Dai, Jingcheng; An, Weixing; Wei, Hehong] Chinese Acad Sci, Inst Hydrobiol, Wuhan, Peoples R China. [Qiu, Dongru; Dai, Jingcheng; An, Weixing; Wei, Hehong] Univ Chinese Acad Sci, Beijing, Peoples R China. [Qiu, Dongru; Xie, Ming; Kempher, Megan L.; Zhou, Aifen; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Gen, Norman, OK 73019 USA. [Tian, Chunyuan] Hubei Engn Univ, Sch Life Sci & Technol, Xiaogan, Peoples R China. [Gu, Baohua] Oak Ridge Natl Lab, Div Earth Sci, Oak Ridge, TN 37831 USA. [Zhou, Jizhong] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China. RP Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Gen, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.; Zhou, JZ (reprint author), Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China. EM jzhou@ou.edu FU DOE [DE-FG02-07ER64383]; Chinese Academy of Sciences [Y15103-1-401]; One-Hundred Scholar Award; [WO2014144329 A2] FX This work was supported by DOE grant DE-FG02-07ER64383 to J.Z. and the Chinese Academy of Sciences grant Y15103-1-401 and One-Hundred Scholar Award to D.Q.; J.Z., D.Q., Z.H., and M.X. have a potential financial conflict of interest resulting from a published patent application (no. WO2014144329 A2) regarding the Shewanella-based production of protoporphyrin IX. NR 39 TC 0 Z9 0 U1 17 U2 17 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD SEP PY 2016 VL 82 IS 17 BP 5077 EP 5088 DI 10.1128/AEM.00203-16 PG 12 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA DT5DI UT WOS:000381500700003 PM 27287322 ER PT J AU Chen, J Garcia, HE AF Chen, Jun Garcia, Humberto E. TI Economic optimization of operations for hybrid energy systems under variable markets SO APPLIED ENERGY LA English DT Article DE Hybrid energy systems; Renewable; Operations optimization; Economic analysis; Power market ID ELECTRICITY MARKET; COMBINED HEAT; MICRO-GRIDS; STORAGE; GENERATION; MANAGEMENT; DESIGN AB Hybrid energy systems (HES) have been proposed to be an important element to enable increasing penetration of clean energy. This paper proposes a methodology for operations optimization to maximize their economic value based on predicted renewable generation and market information. A multi environment computational platform for performing such operations optimization is also developed. To compensate for prediction error, a control strategy is accordingly designed to operate a standby energy storage element (ESE) to avoid energy imbalance within HES. The proposed operations optimizer allows systematic control of energy conversion for maximal economic value. Simulation results of two specific HES configurations illustrate the proposed methodology and computational capability. Economic advantages of such operations optimizer and associated flexible operations are demonstrated by comparing the economic performance of flexible operations with that of constant operations. Sensitivity analysis with respect to market variability and prediction error are also performed. Published by Elsevier Ltd. C1 [Chen, Jun; Garcia, Humberto E.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Garcia, HE (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM humberto.garcia@inl.gov OI Chen, Jun/0000-0002-0934-8519 FU Energy Security Initiative (ESI); Nuclear-Renewable Energy Systems Program at Idaho National Laboratory (INL) under the U.S. Department of Energy [DE-AC-07-05ID14517] FX This research is supported by the Energy Security Initiative (ESI) and the Nuclear-Renewable Energy Systems Program at Idaho National Laboratory (INL) under the U.S. Department of Energy contract DE-AC-07-05ID14517. The authors would like to acknowledge the assistance of Mr. Wesley R. Deason and Dr. Michael G. McKellar in providing part of cost parameters, and the leadership of Dr. Richard D. Boardman and Dr. Shannon M. Bragg-Sitton in the Nuclear-Renewable Energy Systems Program at INL. NR 63 TC 9 Z9 9 U1 4 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2016 VL 177 BP 11 EP 24 DI 10.1016/j.apenergy.2016.05.056 PG 14 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2OR UT WOS:000380623900002 ER PT J AU Yin, RX Kara, EC Li, YP DeForest, N Wang, K Yong, TY Stadler, M AF Yin, Rongxin Kara, Emre C. Li, Yaping DeForest, Nicholas Wang, Ke Yong, Taiyou Stadler, Michael TI Quantifying flexibility of commercial and residential loads for demand response using setpoint changes SO APPLIED ENERGY LA English DT Article DE Demand response; Thermostatically controlled loads; Regression models; Two-state model; Simplified DR potential estimation ID BUILDING ENERGY PERFORMANCE; ANCILLARY SERVICE; SMART APPLIANCES; HVAC SYSTEMS; OPTIMIZATION; MODEL; PILOT; IDENTIFICATION; CONSUMPTION; INTEGRATION AB This paper presents a novel demand response estimation framework for residential and commercial buildings using a combination of EnergyPlus and two-state models for thermostatically controlled loads. Specifically, EnergyPlus models for commercial and multi-dwelling residential units are applied to construct exhaustive datasets (i.e., with more than 300M data points) that capture the detailed load response and complex thermodynamics of several building types. Subsequently, regression models are fit to each dataset to predict DR potential based on key inputs, including hour of day, set point change and outside air temperature. For single residential units, and residential thermostatically controlled loads (i.e. water heaters and refrigerators) a two-state model from the literature is applied. For commercial office building and Multiple Dwelling Units (MDUs) building, the fitted regression model can predict DR potential with 80-90% accuracy for more than 90% of data points. The coefficients of, determination (i.e. R-2 value) range between 0.54 and 0.78 for the office buildings and 0.39-0.81 for MDUs, respectively. The proposed framework is then validated for commercial buildings through a comparison with a dataset composed of 11 buildings during 12 demand response events. In addition, the use of the proposed simplified DR estimation framework is presented in terms of two cases (1) peak load shed prediction in an individual building and (2) aggregated DR up/down capacity from a large-scale group of different buildings. Published by Elsevier Ltd. C1 [Yin, Rongxin; Kara, Emre C.; DeForest, Nicholas; Stadler, Michael] Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA USA. [Li, Yaping; Wang, Ke; Yong, Taiyou] China Elect Power Res Inst, Beijing, Peoples R China. [Kara, Emre C.] SLAC Natl Accelerator Lab, Grid Integrat Syst & Mobil Grp, Menlo Pk, CA USA. RP Yin, RX (reprint author), Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA USA. EM ryin@lbl.gov FU State Grid Corporation of China Project (Study on Key Technologies for Power and Frequency Control of System with Source-Grid-Load Interactions) [DZN17201300197] FX The work described in this study was coordinated by the Grid Integration Group of Lawrence Berkeley National Laboratory and was supported by the State Grid Corporation of China Project (DZN17201300197, Study on Key Technologies for Power and Frequency Control of System with Source-Grid-Load Interactions). NR 54 TC 3 Z9 3 U1 16 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2016 VL 177 BP 149 EP 164 DI 10.1016/j.apenergy.2016.05.090 PG 16 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2OR UT WOS:000380623900014 ER PT J AU Zhang, CY Wang, Q Wang, JH Korpas, M Pinson, P Ostergaard, J Khodayar, ME AF Zhang, Chunyu Wang, Qi Wang, Jianhui Korpas, Magnus Pinson, Pierre Ostergaard, Jacob Khodayar, Mohammad E. TI Trading strategies for distribution company with stochastic distributed energy resources SO APPLIED ENERGY LA English DT Article DE Distributed energy resources (DERs); Proactive distribution company (PDISCO); Electricity markets; Bilevel game-theoretic model; Multi-period AC power flow; Mathematical program with equilibrium constraints (MPEC); Mathematical program with primal and dual constraints (MPPDC) ID DISTRIBUTION-SYSTEM; DEMAND RESPONSE; GENERATION; OPERATION; MARKET; LOAD; MICROGRIDS; DEVICES; MODEL; WIND AB This paper proposes a methodology to address the trading strategies of a proactive distribution company (PDISCO) engaged in the transmission-level (TL) markets. A one-leader multi-follower bilevel model is presented to formulate the gaming framework between the PDISCO and markets. The lower-level (LL) problems include the TL day-ahead market and scenario-based real-time markets, respectively with the objectives of maximizing social welfare and minimizing operation cost. The upper-level (UL) problem is to maximize the PDISCO's profit across these markets. The PDISCO's strategic offers/bids interactively influence the outcomes of each market. Since the LL problems are linear and convex, while the UL problem is non-linear and non-convex, an equivalent primal-dual approach is used to reformulate this bilevel model to a solvable mathematical program with equilibrium constraints (MPEC). The effectiveness of the proposed model is verified by case studies. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Zhang, Chunyu; Korpas, Magnus] Norwegian Univ Sci & Technol, Dept Elect Power Engn, Trondheim, Norway. [Wang, Qi; Pinson, Pierre; Ostergaard, Jacob] Tech Univ Denmark, Ctr Elect Power & Energy, Lyngby, Denmark. [Wang, Jianhui] Argonne Natl Lab, Energy Syst Div, Argonne, IL USA. [Khodayar, Mohammad E.] So Methodist Univ, Dept Elect Engn, Dallas, TX USA. RP Wang, JH (reprint author), Argonne Natl Lab, Energy Syst Div, Argonne, IL USA. EM chunyu.zhang@ntnu.no; qiwa@elektro.dtu.dk; jianhui.wang@anl.gov; magnus.korpas@ntnu.no; ppin@elektro.dtu.dk; joe@elektro.dtu.dk; mkhodayar@smu.edu FU Research Council of Norway [255209]; Danish iPower Platform Project [10-095378]; U.S. Department of Energy (DOE)'s Office of Electricity Delivery and Energy Reliability FX The authors would like to acknowledge the support from the Research Council of Norway under Grant 255209, the Danish iPower Platform Project under Grant 10-095378, and the U.S. Department of Energy (DOE)'s Office of Electricity Delivery and Energy Reliability. NR 24 TC 2 Z9 2 U1 2 U2 2 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2016 VL 177 BP 625 EP 635 DI 10.1016/j.apenergy.2016.05.143 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2OR UT WOS:000380623900052 ER PT J AU Mo, JK Kang, ZY Yang, GQ Retterer, ST Cullen, DA Toops, TJ Green, JB Zhang, FY AF Mo, Jingke Kang, Zhenye Yang, Gaoqiang Retterer, Scott T. Cullen, David A. Toops, Todd J. Green, Johney B., Jr. Zhang, Feng-Yuan TI Thin liquid/gas diffusion layers for high-efficiency hydrogen production from water splitting SO APPLIED ENERGY LA English DT Article DE Proton exchange membrane fuel; cells/electrolyzer cells; Liquid/gas diffusion layers; Hydrogen production; Water splitting; Performance and efficiency ID ELECTROLYTE FUEL-CELL; MICROPOROUS LAYER; BIPOLAR PLATES; PERFORMANCE; MEMBRANE; ENERGY; TRANSPORT; OPTIMIZATION; MEDIA; DURABILITY AB In this study, a novel titanium thin LGDL with well-tunable pore morphologies was developed by employing nano-manufacturing and was applied in a standard PEMEC. The LGDL tests show significant performance improvements. The operating voltages required at a current density of 2.0 A/cm(2) were as low as 1.69 V, and its efficiency reached a report high of up to 88%. The new thin and flat LGDL with well-tunable straight pores has been demonstrated to remarkably reduce the ohmic, interfacial and transport losses. In addition, well-tunable features, including pore size, pore shape, pore distribution, and thus porosity and permeability, will be very valuable for developing PEMEC models and for validation of its simulations with optimal and repeatable performance. The LGDL thickness reduction from greater than 350 mu m of conventional LGDLs to 25 mu m will greatly decrease the weight and volume of PEMEC stacks, and represents a new direction for future developments of low-cost PEMECs with high performance. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Mo, Jingke; Kang, Zhenye; Yang, Gaoqiang; Zhang, Feng-Yuan] Univ Tennessee, UT Space Inst, Dept Mech Aerosp & Biomed Engn, Nanodynam & High Efficiency Lab Prop & Power Nano, Knoxville, TN 37388 USA. [Retterer, Scott T.; Cullen, David A.; Toops, Todd J.; Green, Johney B., Jr.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhang, FY (reprint author), Univ Tennessee, UT Space Inst, Dept Mech Aerosp & Biomed Engn, Nanodynam & High Efficiency Lab Prop & Power Nano, Knoxville, TN 37388 USA. EM fzhang@utk.edu RI Green, Johney/B-3391-2017; OI Green, Johney/0000-0003-2383-7260; Cullen, David/0000-0002-2593-7866; Zhang, Feng-Yuan/0000-0003-2535-0966 FU U.S. Department of Energy's National Energy Technology Laboratory [DE-FE0011585]; DOE Office of Basic Energy Sciences FX The authors greatly appreciate the support from U.S. Department of Energy's National Energy Technology Laboratory under Award DE-FE0011585. The research was partially performed at ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by DOE Office of Basic Energy Sciences. The authors also wish to express their appreciations to Dr. Bo Han, Stuart Steen, William C. Barnhill, Alexander Terekhov, Douglas Warnberg, Kate Lansford, Andrew Mays, and Rong Chen for their help. NR 51 TC 6 Z9 6 U1 7 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2016 VL 177 BP 817 EP 822 DI 10.1016/j.apenergy.2016.05.154 PG 6 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2OR UT WOS:000380623900068 ER PT J AU Dong, T Knoshaug, EP Pienkos, PT Laurens, LML AF Dong, Tao Knoshaug, Eric P. Pienkos, Philip T. Laurens, Lieve M. L. TI Lipid recovery from wet oleaginous microbial biomass for biofuel production: A critical review SO APPLIED ENERGY LA English DT Article DE Oleaginous microorganism; Lipid; Wet extraction; Mass transfer; Cell disruption; Biofuel ID PULSED-ELECTRIC-FIELD; HIGH-PRESSURE HOMOGENIZATION; YEAST RHODOSPORIDIUM-TORULOIDES; ENZYME-ASSISTED EXTRACTION; CELL-WALL DEGRADATION; FED-BATCH CULTURE; BIODIESEL PRODUCTION; CHLORELLA-VULGARIS; SOLVENT-EXTRACTION; MICROALGAL BIOMASS AB Biological lipids derived from oleaginous microorganisms are promising precursors for renewable biofuel productions. Direct lipid extraction from wet cell-biomass is favored because it eliminates the need for costly dehydration. However, the development of a practical and scalable process for extracting lipids from wet cell-biomass is far from ready to be commercialized, instead, requiring intensive research and development to understand the lipid accessibility, mechanisms in mass transfer and establish robust lipid extraction approaches that are practical for industrial applications. This paper aims to present a critical review on lipid recovery in the context of biofuel productions with special attention to cell disruption and lipid mass transfer to support extraction from wet biomass. (C) 2016 The Author(s). Published by Elsevier Ltd. C1 [Dong, Tao; Knoshaug, Eric P.; Pienkos, Philip T.; Laurens, Lieve M. L.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80228 USA. RP Laurens, LML (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80228 USA. EM Lieve.Laurens@nrel.gov FU DOE Bioenergy Technology Office (BETO) [DE-AC36-08GO28308] FX This work was supported by the DOE Bioenergy Technology Office (BETO) under Contract no. DE-AC36-08GO28308. Special thanks to Nick Sweeney for photomicrographs, and Jacob Kruger for conducting HPH on algae biomass. NR 190 TC 1 Z9 1 U1 22 U2 32 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD SEP 1 PY 2016 VL 177 BP 879 EP 895 DI 10.1016/j.apenergy.2016.06.002 PG 17 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2OR UT WOS:000380623900073 ER PT J AU Marquardt, D Kucerka, N Wassall, SR Harroun, TA Katsaras, J AF Marquardt, Drew Kucerka, Norbert Wassall, Stephen R. Harroun, Thad A. Katsaras, John TI Cholesterol's location in lipid bilayers SO CHEMISTRY AND PHYSICS OF LIPIDS LA English DT Article DE Cholesterol; Sterol; Membrane dynamics; Membrane structure; Lipid domains ID MOLECULAR-DYNAMICS SIMULATIONS; NUCLEAR-MAGNETIC-RESONANCE; ACYL-CHAIN UNSATURATION; FLIP-FLOP; NEUTRON-DIFFRACTION; PHASE-DIAGRAM; DEUTERIUM NMR; MODEL SYSTEMS; PHOSPHATIDYLCHOLINE BILAYERS; PHOSPHOLIPID-BILAYERS AB It is well known that cholesterol modifies the physical properties of lipid bilayers. For example, the much studied liquid-ordered L-0 phase contains rapidly diffusing lipids with their acyl chains in the all trans configuration, similar to gel phase bilayers. Moreover, the L-0 phase is commonly associated with cholesterol-enriched lipid rafts, which are thought to serve as platforms for signaling proteins in the plasma membrane. Cholesterol's location in lipid bilayers has been studied extensively, and it has been shown - at least in some bilayers - to align differently from its canonical upright orientation, where its hydroxyl group is in the vicinity of the lipid-water interface. In this article we review recent works describing cholesterol's location in different model membrane systems with emphasis on results obtained from scattering, spectroscopic and molecular dynamics studies. (C) 2016 Elsevier Ireland Ltd. All rights reserved. C1 [Marquardt, Drew] Graz Univ, Inst Mol Biosci, Div Biophys, NAWI Graz, Humboldtstr 50-3, A-8010 Graz, Austria. [Marquardt, Drew] BioTechMed Graz, Graz, Austria. [Kucerka, Norbert] Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna 141980, Moscow Region, Russia. [Kucerka, Norbert] Comenius Univ, Dept Phys Chem Drugs, Fac Pharm, Bratislava 83232, Slovakia. [Wassall, Stephen R.] Indiana Univ Purdue Univ, Dept Phys, Indianapolis, IN 46202 USA. [Harroun, Thad A.; Katsaras, John] Brock Univ, Dept Phys, St Catharines, ON L2S 3A1, Canada. [Katsaras, John] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Katsaras, John] Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Katsaras, John] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. RP Marquardt, D (reprint author), Graz Univ, Inst Mol Biosci, Div Biophys, NAWI Graz, Humboldtstr 50-3, A-8010 Graz, Austria.; Marquardt, D (reprint author), BioTechMed Graz, Graz, Austria.; Katsaras, J (reprint author), Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. EM drew.marquardt@uni-graz.at; katsarasj@ornl.gov OI Katsaras, John/0000-0002-8937-4177 FU VEGA grant [1/0916/16]; collaborative SR-JINR program [04-4-1121-2015/2017]; Scientific User Facilities Division of the DOE Office of Basic Energy Sciences under US DOE [DE-AC05-00OR22725] FX DM thanks Georg Pabst for his support. NK is supported through the VEGA grant 1/0916/16 and collaborative SR-JINR program under theme 04-4-1121-2015/2017, JK is supported through the Scientific User Facilities Division of the DOE Office of Basic Energy Sciences under US DOE Contract No. DE-AC05-00OR22725. NR 114 TC 1 Z9 1 U1 17 U2 32 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0009-3084 EI 1873-2941 J9 CHEM PHYS LIPIDS JI Chem. Phys. Lipids PD SEP PY 2016 VL 199 SI SI BP 17 EP 25 DI 10.1016/j.chemphyslip.2016.04.001 PG 9 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA DT9PC UT WOS:000381833800004 PM 27056099 ER PT J AU Haaskjold, YL Bolkan, HA Krogh, KO Jongopi, J Lundeby, KM Mellesmo, S Garces, PSJ Josendal, O Opstad, A Svensen, E Fuentes, LMZ Kamara, AS Riera, M Arranz, J Roberts, DP Stamper, PD Austin, P Moosa, AJ Marke, D Hassan, S Eide, GE Berg, A Blomberg, B AF Haaskjold, Yngvar Lunde Bolkan, Hakon Angell Krogh, Kurt Osthuus Jongopi, James Lundeby, Karen Marie Mellesmo, Sindre Jose Garces, Pedro San Josendal, Ola Opstad, Asmund Svensen, Erling Zabala Fuentes, Luis Matias Kamara, Alfred Sandy Riera, Melchor Arranz, Javier Roberts, David P. Stamper, Paul D. Austin, Paula Moosa, Alfredo J. Marke, Dennis Hassan, Shoaib Eide, Geir Egil Berg, Ase Blomberg, Bjorn TI Clinical Features of and Risk Factors for Fatal Ebola Virus Disease, Moyamba District, Sierra Leone, December 2014 February 2015 SO EMERGING INFECTIOUS DISEASES LA English DT Article ID HEMORRHAGIC-FEVER; WEST-AFRICA; HOLDING UNITS; OUTBREAK; EPIDEMIC; OUTCOMES; TRANSMISSION; MANAGEMENT; FREETOWN; ORIGIN AB The 2013-2016 outbreak of Ebola virus disease (EVD) in West Africa infected >28,000 people, including >11,000 who died, and disrupted social life in the region. We retrospectively studied clinical signs and symptoms and risk factors for fatal outcome among 31 Ebola virus positive patients admitted to the Ebola Treatment Center in Moyamba District, Sierra Leone. We found a higher rate of bleeding manifestations than reported elsewhere during the outbreak. Significant predictors for death were shorter time from symptom onset to admission, male sex, high viral load on initial laboratory testing, severe pain, diarrhea, bloody feces, and development of other bleeding manifestations during hospitalization. These risk factors for death could be used to identify patients in need of more intensive medical support. The lack of fever in as many as one third of EVD cases may have implications for temperature-screening practices and case definitions. C1 [Haaskjold, Yngvar Lunde; Josendal, Ola; Svensen, Erling; Eide, Geir Egil; Blomberg, Bjorn] Haukeland Hosp, Bergen, Norway. [Bolkan, Hakon Angell; Krogh, Kurt Osthuus; Mellesmo, Sindre] St Olav Hosp, Trondheim, Norway. [Jongopi, James; Kamara, Alfred Sandy; Moosa, Alfredo J.; Marke, Dennis] Moyamba Dist Hosp, Moyamba, Sierra Leone. [Lundeby, Karen Marie] Oslo Univ Hosp, Oslo, Norway. [Jose Garces, Pedro San; Zabala Fuentes, Luis Matias; Arranz, Javier] Med Mundo, Madrid, Spain. [Opstad, Asmund] Haraldsplass Diaconal Hosp, Bergen, Norway. [Svensen, Erling; Eide, Geir Egil; Blomberg, Bjorn] Univ Bergen, Bergen, Norway. [Riera, Melchor] Hosp Son Espases, Palma De Mallorca, Spain. [Arranz, Javier] Inst Invest Palma IDISPA, Madrid, Spain. [Roberts, David P.; Stamper, Paul D.] MRIGlobal, Rockville, MD USA. [Austin, Paula] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Hassan, Shoaib] FELTP Publ Hlth, Islamabad, Pakistan. [Berg, Ase] Stavanger Univ Hosp, Stavanger, Norway. RP Blomberg, B (reprint author), Haukeland Hosp, Dept Med, Post Box 1400, N-5021 Bergen, Norway. EM bjorn.blomberg@uib.no OI Arranz, Javier/0000-0003-0728-9751 NR 38 TC 0 Z9 0 U1 14 U2 14 PU CENTERS DISEASE CONTROL PI ATLANTA PA 1600 CLIFTON RD, ATLANTA, GA 30333 USA SN 1080-6040 EI 1080-6059 J9 EMERG INFECT DIS JI Emerg. Infect. Dis PD SEP PY 2016 VL 22 IS 9 BP 1537 EP 1544 DI 10.3201/eid2209.151621 PG 8 WC Immunology; Infectious Diseases SC Immunology; Infectious Diseases GA DU1GJ UT WOS:000381955900002 PM 27268303 ER PT J AU Bubbosh, P AF Bubbosh, Paul TI FROM LAB TO MARKET SO FOREIGN AFFAIRS LA English DT Letter C1 [Bubbosh, Paul] US DOE, Energy Secur Div, Washington, DC 20585 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU COUNCIL FOREIGN RELAT IONS INC PI NEW YORK PA HAROLD PRATT HOUSE, 58 E 68TH ST, NEW YORK, NY 10065 USA SN 0015-7120 J9 FOREIGN AFF JI Foreign Aff. PD SEP-OCT PY 2016 VL 95 IS 5 BP 192 EP 192 PG 1 WC International Relations SC International Relations GA DT1KG UT WOS:000381240500077 ER PT J AU Beckingham, LE Mitnick, EH Steefel, CI Zhang, S Voltolini, M Swift, AM Yang, L Cole, DR Sheets, JM Ajo-Franklin, JB DePaolo, DJ Mito, S Xue, ZQ AF Beckingham, Lauren E. Mitnick, Elizabeth H. Steefel, Carl I. Zhang, Shuo Voltolini, Marco Swift, Alexander M. Yang, Li Cole, David R. Sheets, Julia M. Ajo-Franklin, Jonathan B. DePaolo, Donald J. Mito, Saeko Xue, Ziqiu TI Evaluation of mineral reactive surface area estimates for prediction of reactivity of a multi-mineral sediment SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Reactive surface area; CO2 sequestration; Mineral reaction rates ID BASALTIC GLASS DISSOLUTION; SOLUTION SATURATION STATE; KAOLINITE DISSOLUTION; DEGREES-C; NUMERICAL-SIMULATION; DIOPSIDE DISSOLUTION; FELDSPAR DISSOLUTION; QUARTZ DISSOLUTION; AQUEOUS-SOLUTIONS; CONTINUUM SCALE AB Our limited understanding of mineral reactive surface area contributes to significant uncertainties in quantitative simulations of reactive chemical transport in subsurface processes. Continuum formulations for reactive transport typically use a number of different approximations for reactive surface area, including geometric, specific, and effective surface area. In this study, reactive surface area estimates are developed and evaluated for their ability to predict dissolution rates in a well-stirred flow-through reactor experiment using disaggregated samples from the Nagaoka pilot CO2 injection site (Japan). The disaggregated samples are reacted with CO2 acidified synthetic brine under conditions approximating the field conditions and the evolution of solute concentrations in the reactor effluent is tracked over time. The experiments, carried out in fluid-dominated conditions at a pH of 3.2 for 650 h, resulted in substantial dissolution of the sample and release of a disproportionately large fraction of the divalent cations. Traditional reactive surface area estimation methods, including an adjusted geometric surface area and a BET-based surface area, are compared to a newly developed image-based method. Continuum reactive transport modeling is used to determine which of the reactive surface area models provides the best match with the effluent chemistry from the well-stirred reactor. The modeling incorporates laboratory derived mineral dissolution rates reported in the literature and the initial modal mineralogy of the Nagaoka sediment was determined from scanning electron microscopy (SEM) characterization. The closest match with the observed steady-state effluent concentrations was obtained using specific surface area estimates from the image-based approach supplemented by literature-derived BET measurements. To capture the evolving effluent chemistry, particularly over the first 300 h of the experiment, it was also necessary to account for the grain size distribution in the sediment and the presence of a highly reactive volcanic glass phase that shows preferential cation leaching. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Beckingham, Lauren E.; Steefel, Carl I.; Voltolini, Marco; Yang, Li; Ajo-Franklin, Jonathan B.; DePaolo, Donald J.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Mitnick, Elizabeth H.; Zhang, Shuo; DePaolo, Donald J.] Univ Calif Berkeley, Earth & Planetary Sci, Berkeley, CA 94720 USA. [Swift, Alexander M.; Cole, David R.; Sheets, Julia M.] Ohio State Univ, Mendenhall Lab 275, 125 South Oval Mall, Columbus, OH 43210 USA. [Mito, Saeko; Xue, Ziqiu] Res Inst Innovat Technol Earth RITE, 9-2 Kizugawadai, Kizugawa, Kyoto 6190292, Japan. [Beckingham, Lauren E.] Auburn Univ, Harbert Engn Ctr 211, Auburn, AL 36830 USA. RP Beckingham, LE (reprint author), Auburn Univ, Dept Civil Engn, Auburn, AL 36830 USA. EM leb@auburn.edu RI Ajo-Franklin, Jonathan/G-7169-2015; Steefel, Carl/B-7758-2010; Voltolini, Marco/G-2781-2015; OI Mito, Saeko/0000-0001-7647-8674; Zhang, Shuo/0000-0002-2170-4299 FU Center for Nanoscale Control of Geologic CO2 (NCGC), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-05CH11231]; Ministry of Economy, Trade and Industry (METI) FX This work was supported as part of the Center for Nanoscale Control of Geologic CO2 (NCGC), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award # DE-AC02-05CH11231. Rock sample collection at the Nagaoka pilot CO2 injection site was financed by Ministry of Economy, Trade and Industry (METI) under the contract of "Research and Development of Underground Storage for Carbon Dioxide". NR 96 TC 0 Z9 0 U1 24 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD SEP 1 PY 2016 VL 188 BP 310 EP 329 DI 10.1016/j.gca.2016.05.040 PG 20 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS4LN UT WOS:000380752700018 ER PT J AU Wang, YG Gelabert, A Michel, FM Choi, Y Gescher, J Ona-Nguema, G Eng, PJ Bargar, JR Farges, F Spormann, AM Brown, GE AF Wang, Yingge Gelabert, Alexandre Michel, F. Marc Choi, Yongseong Gescher, Johannes Ona-Nguema, Georges Eng, Peter J. Bargar, John R. Farges, Francois Spormann, Alfred M. Brown, Gordon E., Jr. TI Effect of biofilm coatings at metal-oxide/water interfaces I: Pb(II) and Zn(II) partitioning and speciation at Shewanella oneidensis/metal-oxide/water interfaces SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Shewanella oneidensis; Biofilms; Metal-oxide surface; Sorption; Pb; Zn; Hematite; Alumina; X-ray standing wave; LP-XSW-FY; Metal partitioning; Diffusion; Kinetics ID BURKHOLDERIA-CEPACIA BIOFILMS; BOND-VALENCE DETERMINATION; OXIDE-WATER INTERFACES; RAY STANDING-WAVE; BACTERIAL SURFACES; MICROBIAL BIOFILMS; ZINC SORPTION; HEMATITE 0001; INFRARED-SPECTROSCOPY; COMPETITIVE-BINDING AB Microbial biofilms are often present as coatings on metal-oxide surfaces in natural and industrial environments and may induce significant changes in the partitioning behavior and speciation of aqueous metal ions, which in turn can impact their transport and fate. In this study, long-period X-ray standing wave-fluorescence yield (LP-XSW-FY) spectroscopy was used to measure under in situ conditions the partitioning of aqueous Pb(II) and Zn(II) between multilayer Shewanella oneidensis MR-1 biofilms and highly polished, oriented single-crystal surfaces of alpha-Al2O3 and alpha-Fe2O3 as a function of metal-ion concentration and time at pH 6.0. We show that after 3-h exposure time, Pb(II) binds preferentially to the alpha-Al2O3 (1-102) and alpha-Fe2O3 (0001) surfaces at low Pb concentration ([Pb] = 10(-7) M) and then increasingly partitions into the biofilm coatings at higher concentrations (10(-6) to 10(-4) M). In contrast, Zn(II) partitions preferentially into the biofilm coating for both surfaces at all Zn concentrations studied (10(-7) to 10(-4) M). In comparison, the alpha-Al2O3 (0001) surface has a low affinity for both Pb(II) and Zn(II), and the biofilm coatings are the dominant sink for both ions. These findings suggest that in the presence of S. oneidensis biofilm coatings, alpha-Al2O3 (0001) is the least reactive surface for Pb(II) and Zn(II) compared to alpha-Al2O3 (1-102) and alpha-Fe2O3 (0001). They also show that Zn(II) has a lower affinity than Pb(II) for reactive sites on alpha-Al2O3 (1-102) and alpha-Fe2O3 (0001) at [Me(II)] of 10(-7) M; at 10(-5) M, the bulk of the metal ions partition into the biofilm coatings. At longer exposure times (20-24 h), both Pb(II) and Zn(II) increasingly partition to the metal-oxide surfaces at [Me(II)] = 10(-5) M and pH 6.0, indicating possible reaction/diffusion-controlled sorption processes. Pb L-III-edge and Zn K-edge grazing-incidence extended X-ray absorption fine structure (GI-EXAFS) measurements suggest that both Pb(II) and Zn(II) ions may be complexed by carboxyl groups in S. oneidensis biofilms after 3-h exposure at pH 6.0 and [Me(II)] = 10(-5) M. In contrast with Burkholderia cepacia, which was used in our previous studies of monolayer biofilm-coated metal-oxide surfaces (Templeton et al., 2001), S. oneidensis MR-1 forms relatively thick biofilm coatings (6-20 mu m) that are rich in reactive functional groups and are expected to dominate metal-ion adsorption. Our results show that even thick and highly reactive biofilms like S. oneidensis do not cause much change in the intrinsic chemical reactivities of the underlying metal-oxide surfaces with respect to aqueous Pb(II) and Zn(II) and don't block reactive sites on the metal-oxide surfaces; instead they reduce the rate of Pb(II) and Zn(II) sorption onto these surfaces. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Wang, Yingge; Gelabert, Alexandre; Michel, F. Marc; Farges, Francois; Brown, Gordon E., Jr.] Stanford Univ, Sch Earth Energy & Environm Sci, Dept Geol Sci, Surface & Aqueous Geochem Grp, Stanford, CA 94305 USA. [Gelabert, Alexandre] Univ Paris Diderot, Aqueous Geochem Grp, Sorbonne Paris Cite, Inst Phys Globe Paris,UMR 7154,CNRS, F-75013 Paris, France. [Michel, F. Marc; Bargar, John R.; Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, MS 69,2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Choi, Yongseong] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. [Gescher, Johannes] Karlsruhe Inst Technol, Inst Appl Biosci, Fritz Haber Weg 2, D-76131 Karlsruhe, Germany. [Gescher, Johannes; Spormann, Alfred M.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. [Ona-Nguema, Georges] Univ Paris 06, IMPMC, UMR 7590, F-75015 Paris, France. [Eng, Peter J.] Univ Chicago, Consortium Adv Radiat Sources, Chicago, IL 60637 USA. [Farges, Francois] Museum Natl Hist Nat, USM 201, Paris, France. [Farges, Francois] Museum Natl Hist Nat, CNRS, UMR 7160, Paris, France. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Dept Photon Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Brown, GE (reprint author), Stanford Univ, Sch Earth Energy & Environm Sci, Dept Geol Sci, Surface & Aqueous Geochem Grp, Stanford, CA 94305 USA.; Brown, GE (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, MS 69,2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Brown, GE (reprint author), SLAC Natl Accelerator Lab, Dept Photon Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM gordon.brown@stanford.edu FU U.S. National Science Foundation [CHE-0431425]; DOE-Office of Biological and Environmental Research through the Science Focus Area at the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory; U.S. DOE Office of Basic Energy Sciences; GeoSoilEnviroCARS Sector 13 at the Advanced Photon Source, Argonne National Laboratory; U.S. National Science Foundation - Earth Sciences [EAR-0622171]; U.S. Department of Energy - Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This study was supported by U.S. National Science Foundation Grant CHE-0431425 (Stanford Environmental Molecular Science Institute) and by the DOE-Office of Biological and Environmental Research through the Science Focus Area at the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory. The XSW and EXAFS data reported in this paper were collected at the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, which is supported by the U.S. DOE Office of Basic Energy Sciences, and at the GeoSoilEnviroCARS Sector 13 at the Advanced Photon Source, Argonne National Laboratory. GeoSoilEnviroCARS is supported by the U.S. National Science Foundation - Earth Sciences (EAR-0622171) and the U.S. Department of Energy - Geosciences (DE-FG02-94ER14466). The Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank Carmen Cordova for help with the biofilm growth and Sanjit Ghose for help with XSW data collection at the APS. We also wish to thank three anonymous reviewers for suggestions that clarified the manuscript as well as GCA Editor Marc Norman and former GCA Associate Editor Roy Wogelius for their patience during the revision process. NR 94 TC 3 Z9 3 U1 22 U2 25 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD SEP 1 PY 2016 VL 188 BP 368 EP 392 DI 10.1016/j.gca.2016.04.052 PG 25 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS4LN UT WOS:000380752700021 ER PT J AU Wang, YG Gelabert, A Michel, FM Choi, Y Eng, PJ Spormann, AM Brown, GE AF Wang, Yingge Gelabert, Alexandre Michel, F. Marc Choi, Yongseong Eng, Peter J. Spormann, Alfred M. Brown, Gordon E., Jr. TI Effect of biofilm coatings at metal-oxide/water interfaces II: Competitive sorption between Pb(II) and Zn(II) at Shewanella oneidensis/metal-oxide/water interfaces SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Shewanella oneidensis; Biofilm; Metal-oxide surface; Competitive sorption; Pb; Zn; Hematite; Alumina; X-ray standing wave; LP-XSW-FY; Metal partitioning ID RAY STANDING WAVES; AMORPHOUS IRON OXYHYDROXIDE; CHEMICAL-EQUILIBRIUM MODEL; BOND-VALENCE DETERMINATION; OXIDE-WATER INTERFACES; ELECTROCHEMICAL INTERFACES; SURFACE COMPLEXATION; POLY(ACRYLIC ACID); AQUEOUS-SOLUTIONS; HEAVY-METALS AB Competitive sorption of Pb(II) and Zn(II) on Shewanella oneidensis MR-1 biofilm-coated single-crystal alpha-Al2O3 (1-102) and alpha-Fe2O3 (0001) surfaces was investigated using long-period X-ray standing wave-florescence yield (LP-XSW-FY) spectroscopy. In situ partitioning of aqueous Pb(II) and Zn(II) between the biofilms and underlying metal-oxide substrates was probed following exposure of these complex interfaces to equi-molar Pb and Zn solutions (0.01 M NaNO3 as background electrolyte, pH = 6.0, and 3-h equilibration time). At higher Pb and Zn concentrations (>= 10(-5) M), more than 99% of these ions partitioned into the biofilms at S. oneidensis/alpha-Al2O3 (1-102)/water interfaces, which is consistent with the partitioning behavior of both Pb(II) or Zn(II) in single-metal-ion experiments. Thus, no apparent competitive effects were found in this system at these relatively high metal-ion concentrations. However, at lower equi-molar concentrations (<= 10(-6) M), Pb(II) and Zn(II) partitioning in the same system changed significantly compared to the single-metal-ion systems. The presence of Zn(II) decreased Pb(II) partitioning onto alpha-Al2O3 (1-10 2) substantially (similar to 52% to similar to 13% at 10(-7) M, and similar to 23% to similar to 5% at 10(-6) M), whereas the presence of Pb(II) caused more Zn(II) to partition onto alpha-Al2O3 (1-102) surfaces (similar to 15% to similar to 28% at 10(-7) M, and similar to 1% to similar to 7% at 10(-6) M). The higher observed partitioning of Zn(II) (similar to 28%) at the alpha-Al2O3 (1-102) surfaces compared to Pb(II) (similar to 13%) in the mixed-metal-ion systems at the lowest concentration (10(-7) M) suggests that Zn(II) is slightly favored over Pb(II) for sorption sites on alpha-Al2O3 (1-102) surfaces under our experimental conditions. Competitive sorption of Pb(II) and Zn(II) at S. oneidensis/alpha-Fe2O3 (0001)/water interfaces at equi-molar metal-ion concentrations of <= 10(-6) M showed that the presence of Pb(II) ions decreased Zn(II) partitioning onto alpha-Fe2O3 (0001) significantly (similar to 45% to <1% at 10(-7) M, and similar to 41% to 3% at 10(-6) M), whereas adding Zn(II) caused only small changes in Pb(II) partitioning (similar to 59% to similar to 47% at 10(-7) M, and similar to 26% to similar to 23% at 10(-6) M), suggesting that Pb(II) strongly outcompetes Zn(II) for sorption sites on S. oneidensis-coated alpha-Fe2O3 (0001) surfaces. Our study implies that caution should be taken when applying results obtained from partitioning studies of single-metal-ion systems to mixed-metal-ion systems at complex biofilm/mineral interfaces. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Wang, Yingge; Gelabert, Alexandre; Michel, F. Marc; Brown, Gordon E., Jr.] Stanford Univ, Sch Earth Energy & Environm Sci, Dept Geol Sci, Surface & Aqueous Geochem Grp, Stanford, CA 94305 USA. [Gelabert, Alexandre] Univ Paris 07, Dept Earth Sci, IMPMC, IPGP,CNRS,UMR 7590, F-75015 Paris, France. [Michel, F. Marc] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, MS 69,2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Choi, Yongseong] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. [Eng, Peter J.] Univ Chicago, Consortium Adv Radiat Sources, Chicago, IL 60637 USA. [Spormann, Alfred M.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Dept Photon Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Michel, F. Marc] Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. RP Wang, YG (reprint author), Stanford Univ, Sch Earth Energy & Environm Sci, Dept Geol Sci, Surface & Aqueous Geochem Grp, Stanford, CA 94305 USA. EM wang.yingge@gmail.com FU U.S. National Science Foundation [CHE-0431425]; National Science Foundation Earth Sciences [EAR-1128799]; U.S. Department of Energy - Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This study was supported by U.S. National Science Foundation Grant CHE-0431425 (Stanford Environmental Molecular Science Institute). The LP-XSW-FY data reported here were obtained at GeoSoilEnviroCARS (Advanced Photon Source Sector 13) at the Advanced Photon Source, Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation Earth Sciences (EAR-1128799) and the U.S. Department of Energy - Geosciences (DE-FG02-94ER14466). The Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We also wish to thank two anonymous reviewers for helpful comments and thank GCA Editor Dr. Marc Norman and former GCA Associate Editor Dr. Roy Wogelius for their patience during the revision process. NR 57 TC 1 Z9 1 U1 12 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD SEP 1 PY 2016 VL 188 BP 393 EP 406 DI 10.1016/j.gca.2016.04.054 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS4LN UT WOS:000380752700022 ER PT J AU Wang, YG Michel, FM Choi, Y Eng, PJ Levard, C Siebner, H Gu, BH Bargar, JR Brown, GE AF Wang, Yingge Michel, F. Marc Choi, Yongseong Eng, Peter J. Levard, Clement Siebner, Hagar Gu, Baohua Bargar, John R. Brown, Gordon E., Jr. TI Pb, Cu, and Zn distributions at humic acid-coated metal-oxide surfaces SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Humic acid; Pb; Cu; Zn; Ca; Metal-oxide surfaces; Single crystal; X-ray standing wave; LP-XSW-FY; Metal partitioning; Hematite; Alumina; pH effect ID RAY STANDING WAVES; NATURAL ORGANIC-MATTER; ION-BINDING; X-RAYS; COMPETITIVE ADSORPTION; MINERAL SURFACES; HEMATITE 0001; IRON-OXIDE; ELECTROCHEMICAL INTERFACES; DYNAMICAL DIFFRACTION AB Mineral surfaces are often coated by natural organic matter (NOM), which has a major influence on metal-ion sorption and sequestration because of the abundance of binding sites in such coatings and the changes they cause in local nanoscale environments. The effects of NOM coatings on mineral surfaces are, however, still poorly understood at the molecular level due to the complexity of these systems. In this study, we have applied long-period X-ray standing wave-fluorescence yield (LP-XSW-FY) spectroscopy to measure the partitioning of naturally present Cu(II) (0.0226%), Zn(II) (0.009%), and Pb(II) (similar to 0.0004%) between Elliott Soil Humic Acid (ESHA) coatings and three model single-crystal metal-oxide substrates: alpha-Al2O3 (00 01), alpha-Al2O3 (1-102), and alpha-Fe2O3 (0001). The competitive sorption effects among these metal ions for binding sites in the ESHA coatings and on the metal-oxide surfaces were investigated as a function of reaction time, calcium content, and solution pH. Pb(II) ions present in the ESHA coatings were found to redistribute to reactive alpha-Al2O3 (1-102) and alpha-Fe2O3 (0001) surfaces after 3 h of reaction (pH = 6.0, [Ca(II)] = 2 mM). Pb(II) partitioning onto these reactive metal-oxide surfaces increased with increasing reaction time (up to 7 d). In addition, the partitioning of Cu(II) and Zn(II) from the ESHA coating to the alpha-Fe2O3 (0001) substrate increased slightly with reaction time (2.4% and 3.7% for Cu(II) and Zn(II), respectively, after 3 h and 6.4% and 7.7% for Cu(II) and Zn(II), respectively, after 72 h of reaction time). However, no changes in the partitioning of Cu(II) and Zn(II) onto the alpha-Al2O3 (1-102) surface were observed with increasing reaction time, suggesting that these ions strongly complex with functional groups in the ESHA coatings. Similar results were obtained for Cu(II) and Zn(II) on the ESHA-coated alpha-Al2O3 (1-102) surfaces in samples without the addition of calcium. However, the amounts of Pb(II) mobilized from the ESHA coatings onto the alpha-Al2O3 (1-102) surfaces increased from 40% (no added Ca) to 58% (with 2 mM Ca) after 72 h of reaction time, possibly due to displacement of Pb(II) by Ca(II) from binding sites in the ESHA coatings. In contrast, Pb(II), Cu(II), and Zn(II) present in the ESHA coatings were found to be unreactive with the alpha-Al2O3 (0001) surface. The observed reactivities of the three ESHA-coated metal-oxide surfaces with respect to metal-ion sorption are consistent with the trend observed for the uncoated metal-oxide surfaces: alpha-Fe2O3 (0001) > alpha-Al2O3 (1-102) > alpha-Al2O3 (0001). In addition, Pb(II) partitioning onto alpha-Al2O3 (1-102) surfaces increased with increasing pH from 4.0 to 9.0 as a result of the increasingly negative surface charge. These results show that intrinsic properties (nature of binding sites, binding affinities, and surface charge) of the ESHA coatings and metal-oxide surfaces, as well as external parameters such as pH and competing ions, are key factors governing the distribution and speciation of metal ions at complex NOM/mineral interfaces. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Wang, Yingge; Michel, F. Marc; Levard, Clement; Siebner, Hagar; Brown, Gordon E., Jr.] Stanford Univ, Dept Geol Sci, Surface & Aqueous Geochem Grp, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA. [Michel, F. Marc; Bargar, John R.; Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, MS 69,2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Choi, Yongseong] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. [Eng, Peter J.] Univ Chicago, Consortium Adv Radiat Sources, Chicago, IL 60637 USA. [Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Dept Photon Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Brown, GE (reprint author), Stanford Univ, Dept Geol Sci, Surface & Aqueous Geochem Grp, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA.; Brown, GE (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, MS 69,2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Brown, GE (reprint author), SLAC Natl Accelerator Lab, Dept Photon Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM gordon.brown@stanford.edu FU U.S. National Science Foundation [CHE-0431425]; U.S. National Science Foundation-Center for Environmental Implications for Nanotechnology (based at Duke University) (U.S. National Science Foundation) [EF-0830093]; U.S. National Science Foundation - Earth Sciences [EAR-1128799]; U.S. Department of Energy - Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This study was supported by U.S. National Science Foundation Grant CHE-0431425 (Stanford Environmental Molecular Science Institute) and by the U.S. National Science Foundation-Center for Environmental Implications for Nanotechnology (based at Duke University) (U.S. National Science Foundation Cooperative Agreement EF-0830093). The LP-XSW-FY data reported in this paper were collected at GeoSoilEnviroCARS (Advanced Photon Source Sector 13) at the Advanced Photon Source, Argonne National Laboratory. GeoSoilEnviroCARS is supported by the U.S. National Science Foundation - Earth Sciences (EAR-1128799) and the U.S. Department of Energy - Geosciences (DE-FG02-94ER14466). The Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We wish to thank Guangchao Li (Stanford University) for ICP-AES analysis and Prof. Zhenan Bao (Chemical Engineering, Stanford University) for allowing us to use her spin coater. We also wish to thank three reviewers for their valuable suggestions. The STXM data reported in this paper were collected at the Advanced Light Source, Lawrence Berkeley National Laboratory. The Advanced Light Source is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 75 TC 0 Z9 0 U1 26 U2 33 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD SEP 1 PY 2016 VL 188 BP 407 EP 423 DI 10.1016/j.gca.2016.05.009 PG 17 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS4LN UT WOS:000380752700023 ER PT J AU Wesnousky, SG Briggs, RW Caffee, MW Ryerson, FJ Finkel, RC Owen, LA AF Wesnousky, Steven G. Briggs, Richard W. Caffee, Marc W. Ryerson, F. J. Finkel, Robert C. Owen, Lewis A. TI Terrestrial cosmogenic surface exposure dating of glacial and associated landforms in the Ruby Mountains-East Humboldt Range of central Nevada and along the northeastern flank of the Sierra Nevada SO GEOMORPHOLOGY LA English DT Article DE Geomorphology; Moraines; Cosmogenic dating; Sierra Nevada; Ruby Mountains-East Humboldt Range ID HIMALAYAN-TIBETAN OROGEN; DENUDATION RATES; PLEISTOCENE GLACIATION; QUATERNARY GLACIATION; CENTRAL KARAKORAM; GREAT-BASIN; ICE AGES; BE-10; MORAINES; AL-26 AB Deposits near Lamoille in the Ruby Mountains-East Humboldt Range of central Nevada and at Woodfords on the eastern edge of the Sierra Nevada each record two distinct glacial advances. We compare independent assessments of terrestrial cosmogenic nuclide (TCN) surface exposure ages for glacial deposits that we have determined to those obtained by others at the two sites. At each site, TCN ages of boulders on moraines of the younger advance are between 15 and 30 ka and may be associated with marine oxygen isotope stage (MIS) 2. At Woodfords, TCN ages of boulders on the moraine of the older advance are younger than similar to 60 ka and possibly formed during MIS 4, whereas boulders on the correlative outwash surface show ages approaching 140 ka (similar to MIS 6). The TCN ages of boulders on older glacial moraine at Woodfords thus appear to severely underestimate the true age of the glacial advance responsible for the deposit. The same is possibly true at Lamoille where clasts sampled from the moraine of the oldest advance have ages ranging between 20 and 40 ka with a single outlier age of similar to 80 ka The underestimations are attributed to the degradation and denudation of older moraine crests. Noting that boulder ages on the older advances at each site overlap significantly with MIS 2. We speculate that erosion of the older moraines has been episodic, with a pulse of denudation accompanying the inception of MIS 2 glaciation. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wesnousky, Steven G.] Univ Nevada, Ctr Neotecton Studies, 1664 North Virginia St, Reno, NV 89557 USA. [Briggs, Richard W.] US Geol Survey, 1711 Illinois St, Golden, CO 80401 USA. [Caffee, Marc W.] Dept Phys, 525 Northwestern Ave, W Lafayette, IN 47907 USA. [Ryerson, F. J.; Finkel, Robert C.] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, L-202,7000 East Ave, Livermore, CA 94550 USA. [Owen, Lewis A.] Univ Cincinnati, POB 210013, Cincinnati, OH 45221 USA. RP Wesnousky, SG (reprint author), Univ Nevada, Ctr Neotecton Studies, 1664 North Virginia St, Reno, NV 89557 USA. EM wesnousky@unr.edu; rbriggs@usgs.gov; mcaffee@purdue.edu; ryerson1@llnl.gov; owenls@ucmail.uc.edu OI Ryerson, Frederick/0000-0002-6235-4408; Briggs, Richard/0000-0001-8108-0046 FU USGS Grants [G15AP00088, G14AP00048] FX The manuscript has benefited from the critical and constructive comments of Jaako Pukonen, Ben Laabs and two anonymous reviewers. We give particular thanks to Editor Richard Marston for his time and careful comments that improved the manuscript. Anne-Sophie Meriaux assisted with sample preparation. This research was supported in part by USGS Grants G15AP00088 and G14AP00048. Center for Neotectonics Contribution No. 68. NR 51 TC 0 Z9 0 U1 3 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-555X EI 1872-695X J9 GEOMORPHOLOGY JI Geomorphology PD SEP 1 PY 2016 VL 268 BP 72 EP 81 DI 10.1016/j.geomorph.2016.04.027 PG 10 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA DT0JA UT WOS:000381168600008 ER PT J AU Daley, TM Miller, DE Dodds, K Cook, P Freifeld, BM AF Daley, T. M. Miller, D. E. Dodds, K. Cook, P. Freifeld, B. M. TI Field testing of modular borehole monitoring with simultaneous distributed acoustic sensing and geophone vertical seismic profiles at Citronelle, Alabama SO GEOPHYSICAL PROSPECTING LA English DT Article DE Acquisition; Borehole Geophysics; Seismics; Fibre-optic DAS AB A modular borehole monitoring concept has been implemented to provide a suite of well-based monitoring tools that can be deployed cost effectively in a flexible and robust package. The initial modular borehole monitoring system was deployed as part of a CO2 injection test operated by the Southeast Regional Carbon Sequestration Partnership near Citronelle, Alabama. The Citronelle modular monitoring system transmits electrical power and signals, fibre-optic light pulses, and fluids between the surface and a reservoir. Additionally, a separate multi-conductor tubing-encapsulated line was used for borehole geophones, including a specialized clamp for casing clamping with tubing deployment. The deployment of geophones and fibre-optic cables allowed comparison testing of distributed acoustic sensing. We designed a large source effort (>64 sweeps per source point) to test fibre-optic vertical seismic profile and acquired data in 2013. The native measurement in the specific distributed acoustic sensing unit used (an iDAS from Silixa Ltd) is described as a localized strain rate. Following a processing flow of adaptive noise reduction and rebalancing the signal to dimensionless strain, improvement from repeated stacking of the source was observed. Conversion of the rebalanced strain signal to equivalent velocity units, via a scaling by local apparent velocity, allows quantitative comparison of distributed acoustic sensing and geophone data in units of velocity. We see a very good match of uncorrelated time series in both amplitude and phase, demonstrating that velocity-converted distributed acoustic sensing data can be analyzed equivalent to vertical geophones. We show that distributed acoustic sensing data, when averaged over an interval comparable to typical geophone spacing, can obtain signal-to-noise ratios of 18 dB to 24 dB below clamped geophones, a result that is variable with noise spectral amplitude because the noise characteristics are not identical. With vertical seismic profile processing, we demonstrate the effectiveness of downgoing deconvolution from the large spatial sampling of distributed acoustic sensing data, along with improved upgoing reflection quality. We conclude that the extra source effort currently needed for tubing-deployed distributed acoustic sensing vertical seismic profile, as part of a modular monitoring system, is well compensated by the extra spatial sampling and lower deployment cost as compared with conventional borehole geophones. C1 [Daley, T. M.; Cook, P.; Freifeld, B. M.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Miller, D. E.] Silixa Ltd, Elstree, England. RP Daley, TM (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM tmdaley@lbl.gov RI Daley, Thomas/G-3274-2015; Freifeld, Barry/F-3173-2010; Cook, Paul/I-4788-2016 OI Daley, Thomas/0000-0001-9445-0843; FU CO2 Capture Project; Lawrence Berkeley Laboratory [DE-AC02-05CH11231] FX We would like to thank the CO2 Capture Project for support of the modular borehole monitoring (MBM) concept, development, and deployment. We thank the SECARB team, including Jerry Hill of SSEB, Rob Trautz of EPRI, George Koperna and Dave Riestenberg of ARI, and Gary Dittmar of Denbury. Acquisition of seismic data (geophone and DAS) was assisted by Dale Adessi of SR2020 and Michelle Robertson of LBNL. We would like to thank Bjorn Paulsson and John Thornburg of Paulsson, Inc. for the fabrication and deployment support of MBM geophones. This paper was greatly improved by the efforts of the anonymous reviewers and the editor. This work was supported by the CO2 Capture Project, and performed by Lawrence Berkeley Laboratory under Contract No. DE-AC02-05CH11231. NR 20 TC 1 Z9 1 U1 7 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0016-8025 EI 1365-2478 J9 GEOPHYS PROSPECT JI Geophys. Prospect. PD SEP PY 2016 VL 64 IS 5 BP 1318 EP 1334 DI 10.1111/1365-2478.12324 PG 17 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS6UI UT WOS:000380917900008 ER PT J AU Rosenberg, G Haghnegahdar, P Goddard, P Carr, P Wu, KS de Prado, ML AF Rosenberg, Gili Haghnegahdar, Poya Goddard, Phil Carr, Peter Wu, Kesheng de Prado, Marcos Lopez TI Solving the Optimal Trading Trajectory Problem Using a Quantum Annealer SO IEEE JOURNAL OF SELECTED TOPICS IN SIGNAL PROCESSING LA English DT Article DE Optimal trading trajectory; portfolio optimization; quantum annealing ID PORTFOLIO SELECTION PROBLEM; MINIMUM TRANSACTION LOTS; ALGORITHM; COSTS AB We solve a multi-period portfolio optimization problem using D-Wave Systems' quantum annealer. We derive a formulation of the problem, discuss several possible integer encoding schemes, and present numerical examples that show high success rates. The formulation incorporates transaction costs (including permanent and temporary market impact), and, significantly, the solution does not require the inversion of a covariance matrix. The discrete multi-period portfolio optimization problem we solve is significantly harder than the continuous variable problem. We present insight into how results may be improved using suitable software enhancements and why current quantum annealing technology limits the size of problem that can be successfully solved today. The formulation presented is specifically designed to be scalable, with the expectation that as quantum annealing technology improves, larger problems will be solvable using the same techniques. C1 [Rosenberg, Gili; Goddard, Phil] 1QBit, Vancouver, BC V6C 2B5, Canada. [Haghnegahdar, Poya] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Carr, Peter] NYU, Courant Inst Math Sci, 251 Mercer St, New York, NY 10012 USA. [Wu, Kesheng] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [de Prado, Marcos Lopez] Guggenheim Partners LLC, New York, NY 10017 USA. [de Prado, Marcos Lopez] Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Rosenberg, G (reprint author), 1QBit, Vancouver, BC V6C 2B5, Canada. EM gili.rosenberg@1qbit.com; phagh-neg@phas.ubc.ca; phil.goddard@1qbit.com; Peter.P.Carr@morganstanley.com; kwu@lbl.gov; Marcos.LopezDePrado@guggenheimpartners.com FU 1QB Information Technologies (1QBit); Mitacs FX This work was supported by 1QB Information Technologies (1QBit) and Mitacs. The guest editor coordinating the review of this manuscript was Daniel. P. Palomar. NR 48 TC 1 Z9 1 U1 3 U2 4 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1932-4553 EI 1941-0484 J9 IEEE J-STSP JI IEEE J. Sel. Top. Signal Process. PD SEP PY 2016 VL 10 IS 6 BP 1053 EP 1060 DI 10.1109/JSTSP.2016.2574703 PG 8 WC Engineering, Electrical & Electronic SC Engineering GA DT4XA UT WOS:000381483500008 ER PT J AU Kou, F Yang, SL Zhang, LH Teat, SJ Tian, GX AF Kou, Fei Yang, Suliang Zhang, Lihua Teat, Simon J. Tian, Guoxin TI Complexation of Ho(III) with tetraalkyl-diglycolamide in aqueous solutions and a solid state compared in organic solutions of solvent extraction SO INORGANIC CHEMISTRY COMMUNICATIONS LA English DT Article DE Ho(III); Diglycolamide; Solvent extraction; Crystallography; Spectrophotometry ID MUTUAL SEPARATION; TODGA; LANTHANIDES; ACTINIDES; AM(III); SYSTEM; IONS; N,N'-DIMETHYL-N,N'-DIHEXYL-3-OXAPENTANEDIAMIDE; N,N,N',N'-TETRAETHYLDIGLYCOLAMIDE; COMBINATION AB The complexation of Ho(III) with tetramethyl-diglycolamide (TMDGA) and N,N'-dimethyl-N,N'-dioctyldiglycolamide (DMDODGA) were investigated with spectrophotometry and X-ray crystallography. Single crystals of a solid compound HoL3(ClO4)(3) (L = TMDGA) were grown from aqueous solutions by slow evaporation. The crystal structure of HoL3(ClO4)(3) shows that in the solid compound Ho(III) is coordinated by nine oxygen atoms from three tridentate TMDGA molecules in a distorted tricapped trigonal prism (TCTP) geometry. In aqueous solution, three successive complex species, HoL3+, HoL23+, and HoL33+ (L = TMDGA) were identified and their stability constants were determined to be 2.20 +/- 0.09, 4.48 +/- 0.18, 5.88 +/- 0.18, respectively, with spectral titration method at 25 degrees C and 1 M ionic strength (1 M NaNO3). The UV-Vis absorption/reflection spectra of the 1:3 species HoL33+ (L = TMDGA) in aqueous solution/solid state HoL3(ClO4)(3) compound were very well comparable to the absorption spectra of the extracted samples of Ho(III) with DMDODGA in various organic solvents in solvent extraction. The similarity in the spectra suggest that Ho(III) in the extracted samples is also coordinated by three tridentate DMDODGA with similar coordination geometry as that in HoL33+ (L = TMDGA) in aqueous solution/solid HoL3(ClO4)(3) compound. In the organic phase of solvent extraction with DMDODGA as extractant, the nitrate anions do not directly bond to Ho(III) in the extracted complex but just act as far away counter -ion to neutralize the positive charge of HoL33+ (L = DMDODGA), and the diluents do not have much influence on the formation of the extracted Ho(III)-DMDODGA complex. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kou, Fei; Yang, Suliang; Zhang, Lihua; Tian, Guoxin] China Inst Atom Chem, Radiochem Dept, Beijing 102413, Peoples R China. [Teat, Simon J.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Tian, Guoxin] Harbin Engn Univ, Coll Nucl Sci & Technol, Harbin 150001, Heilongjiang, Peoples R China. RP Yang, SL; Tian, GX (reprint author), China Inst Atom Chem, Radiochem Dept, Beijing 102413, Peoples R China. EM gtian@ciae.ac.cn FU National Natural Science Foundation of China [91426302]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Natural Science Foundation of China (91426302). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 29 TC 1 Z9 1 U1 8 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-7003 EI 1879-0259 J9 INORG CHEM COMMUN JI Inorg. Chem. Commun. PD SEP PY 2016 VL 71 BP 41 EP 44 DI 10.1016/j.inoche.2016.06.035 PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DT9PV UT WOS:000381835700010 ER PT J AU Rasmusson, K Rasmusson, M Tsang, Y Niemi, A AF Rasmusson, K. Rasmusson, M. Tsang, Y. Niemi, A. TI A simulation study of the effect of trapping model, geological heterogeneity and injection strategies on CO2 trapping SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE CCS; Capillary trapping; Hysteresis; Injection strategies; Residual trapping; Solubility trapping ID GOVERNING MULTIPHASE FLOW; CARBON-DIOXIDE; RELATIVE PERMEABILITY; SALINE AQUIFERS; RESERVOIR CONDITIONS; CAPILLARY FORCES; DISSOLUTION; STORAGE; SEQUESTRATION; HELETZ AB Industrial CO2 emissions to the atmosphere can be reduced through geological storage, where the gas is injected into the subsurface and trapped by several mechanisms. Residual and solubility trapping are two important processes providing trapping, and their effectiveness ultimately determines the feasibility of geological storage. By means of numerical modeling, a systematic analysis was made concerning the factors potentially affecting trapping, to guide the planned injection experiments at the Heletz test injection site. The effect of enhanced-trapping injection strategies along with the role of geological heterogeneity and the choice of trapping model (TM) were evaluated. The results showed that adding chase-fluid stages to a conventional CO2 injection enhanced the trapping. Taking into account the geological heterogeneity decreased trapping, as this retarded the buoyant migration, resulting in less imbibition and residual trapping. The choice of TM was significant, with the simplified Land TM producing the highest trapping, and the Aissaoui TM the lowest. The results stress the importance of using an appropriate TM as well as heterogeneity model for the site in question for any predictive modeling of CO2 sequestration, as different assumptions may lead to significant discrepancies in the predicted trapping. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Rasmusson, K.; Rasmusson, M.; Tsang, Y.; Niemi, A.] Uppsala Univ, Dept Earth Sci, Villavagen 16, S-75236 Uppsala, Sweden. [Tsang, Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Geosci Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Rasmusson, K (reprint author), Uppsala Univ, Dept Earth Sci, Villavagen 16, S-75236 Uppsala, Sweden. EM kristina.rasmusson@geo.uu.se; maria.rasmusson@geo.uu.se; yttsang@lbl.gov; auli.niemi@geo.uu.se FU European Community's 7th Framework Programme (project MUSTANG) [227286]; EU FP7 R&D program (project TRUST) [309067] FX lThe research leading to these results is supported by funding from the European Community's 7th Framework Programme FP7/2007-2013 under grant agreement no. 227286 (project MUSTANG) and the EU FP7 R&D program under grant agreement no. 309067 (project TRUST), which is gratefully acknowledged. We would like to thank S.M. Benson at Stanford University for providing us with experimental data for the characteristic functions. We would also like to thank two anonymous reviewers for their review and constructive comments for improvement of the manuscript. NR 58 TC 1 Z9 1 U1 8 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD SEP PY 2016 VL 52 BP 52 EP 72 DI 10.1016/j.ijggc.2016.06.020 PG 21 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DT8GQ UT WOS:000381728300006 ER PT J AU Serno, S Johnson, G LaForce, TC Ennis-King, J Haese, RR Boreham, CJ Paterson, L Freifeld, BM Cook, PJ Kirste, D Haszeldine, RS Gilfillan, SMV AF Serno, Sascha Johnson, Gareth LaForce, Tara C. Ennis-King, Jonathan Haese, Ralf R. Boreham, Christopher J. Paterson, Lincoln Freifeld, Barry M. Cook, Paul J. Kirste, Dirk Haszeldine, R. Stuart Gilfillan, Stuart M. V. TI Using oxygen isotopes to quantitatively assess residual CO2 saturation during the CO2CRC Otway Stage 2B Extension residual saturation test SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Residual saturation; Oxygen isotopes; Otway; Geochemical tracer; CO2 storage ID CARBON-DIOXIDE STORAGE; THERMOMINERAL WATERS; DISSOLUTION TEST; FRACTIONATION; INJECTION; DISPOSAL; EXCHANGE; AQUIFERS; SITE; H2O AB Residual CO2 trapping is a key mechanism of secure CO2 storage, an essential component of the Carbon Capture and Storage technology. Estimating the amount of CO2 that will be residually trapped in a saline aquifer formation remains a significant challenge. Here, we present the first oxygen isotope ratio (delta O-18) measurements from a single-well experiment, the CO2CRC Otway 2B Extension, used to estimate levels of residual trapping of CO2. Following the initiation of the drive to residual saturation in the reservoir, reservoir water delta O-18 decreased, as predicted from the baseline isotope ratios of water and CO2, over a time span of only a few days. The isotope shift in the near-wellbore reservoir water is the result of isotope equilibrium exchange between residual CO2 and water. For the region further away from the well, the isotopic shift in the reservoir water can also be explained by isotopic exchange with mobile CO2 from ahead of the region driven to residual, or continuous isotopic exchange between water and residual CO2 during its back-production, complicating the interpretation of the change in reservoir water delta O-18 in terms of residual saturation. A small isotopic distinction of the baseline water and CO2 delta O-18, together with issues encountered during the field experiment procedure, further prevents the estimation of residual CO2 saturation levels from oxygen isotope changes without significant uncertainty. The similarity of oxygen isotope-based near-wellbore saturation levels and independent estimates based on pulsed neutron logging indicates the potential of using oxygen isotope as an effective inherent tracer for determining residual saturation on a field scale within a few days. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Serno, Sascha; Johnson, Gareth; Haszeldine, R. Stuart; Gilfillan, Stuart M. V.] Univ Edinburgh, Sch Geosci, Grant Inst, Kings Bldg,James Hutton Rd, Edinburgh EH9 3FE, Midlothian, Scotland. [LaForce, Tara C.; Ennis-King, Jonathan; Haese, Ralf R.; Boreham, Christopher J.; Paterson, Lincoln; Kirste, Dirk] Univ Melbourne, Ltd CO2CRC, Carlton, Vic 3010, Australia. [LaForce, Tara C.; Ennis-King, Jonathan; Paterson, Lincoln] CSIRO Energy, Private Bag 10, Clayton, Vic 3169, Australia. [Haese, Ralf R.] Univ Melbourne, Sch Earth Sci, Carlton, Vic 3010, Australia. [Boreham, Christopher J.] Geosci Australia, GPO Box 378, Canberra, ACT 2601, Australia. [Freifeld, Barry M.; Cook, Paul J.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kirste, Dirk] Simon Fraser Univ, Dept Earth Sci, Burnaby, BC V5A 1S6, Canada. RP Serno, S (reprint author), Univ Edinburgh, Sch Geosci, Grant Inst, Kings Bldg,James Hutton Rd, Edinburgh EH9 3FE, Midlothian, Scotland. EM Sascha.Serno@ed.ac.uk RI Freifeld, Barry/F-3173-2010; Cook, Paul/I-4788-2016 FU UK CCS Research Centre (UKCCSRC) through Call 2 grant; ECR International Travel Exchange Fund; EPSRC as part of the RCUK Energy Programme; CO2CRC; AGOS; COSPL; Australian government through CRC programme; Carbon Storage Program, U.S. DOE, Assistant Secretary for Fossil Energy, Office of Clean Coal and Carbon Management through the NETL FX This work was supported by funding from the UK CCS Research Centre (UKCCSRC) through the Call 2 grant to S.M.V.G., GJ. and R.S.S., and the ECR International Travel Exchange Fund to S.S. The UKCCSRC is funded by the EPSRC as part of the RCUK Energy Programme. Funding for the Otway 2B Extension comes through CO2CRC, AGOS and COSPL. The authors acknowledge the funding provided by the Australian government through its CRC programme to support this CO2CRC research project. C.J.B. publishes with the permission of the CEO, Geoscience Australia. Funding for the group from the Lawrence Berkeley National Laboratory was provided by the Carbon Storage Program, U.S. DOE, Assistant Secretary for Fossil Energy, Office of Clean Coal and Carbon Management through the NETL. We would like to thank Sue Golding and Kim Baublys for conducting stable isotope measurements at the Stable Isotope Geochemistry Laboratory of the School of Earth Sciences, University of Queensland, Australia. We appreciate the help in sample collection from Jay Black, Hong Phuc Vu and the field operating team under the supervision of Rajindar Singh. The paper was improved by constructive comments from two anonymous reviewers. NR 53 TC 0 Z9 0 U1 10 U2 10 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD SEP PY 2016 VL 52 BP 73 EP 83 DI 10.1016/j.ijggc.2016.06.019 PG 11 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DT8GQ UT WOS:000381728300007 ER PT J AU Pawar, RJ Bromhal, GS Chu, SP Dilmore, RM Oldenburg, CM Stauffer, PH Zhang, YQ Guthrie, GD AF Pawar, Rajesh J. Bromhal, Grant S. Chu, Shaoping Dilmore, Robert M. Oldenburg, Curtis M. Stauffer, Philip H. Zhang, Yingqi Guthrie, George D. TI The National Risk Assessment Partnership's integrated assessment model for carbon storage: A tool to support decision making amidst uncertainty SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Risk assessment; Risk quantification; CO2 sequestration; Risk profiles; Integrated assessment model; Reduced order models; NRAP ID REDUCED-ORDER MODELS; DEEP SALINE AQUIFERS; CO2 STORAGE; GEOLOGICAL SEQUESTRATION; INDUCED SEISMICITY; BRINE LEAKAGE; SYSTEM MODEL; DIOXIDE; SENSITIVITY; MANAGEMENT AB The US DOE-funded National Risk Assessment Partnership (NRAP) has developed an integrated assessment model (NRAP-IAM-CS) that can be used to simulate carbon dioxide (CO2) injection, migration, and associated impacts at a geologic carbon storage site. The model, NRAP-IAM-CS, incorporates a system modeling-based approach while taking into account the full subsurface system from the storage reservoir to groundwater aquifers and the atmosphere. The approach utilizes reduced order models (ROMs) that allow fast computations of entire system performance even for periods of hundreds to thousands of years. The ROMs are run in Monte Carlo mode allowing estimation of uncertainties of the entire system without requiring long computational times. The NRAP-IAM-CS incorporates ROMs that realistically represent several key processes and properties of storage reservoirs, wells, seals, and groundwater aquifers. Results from the NRAP-IAM-CS model are used to quantify risk profiles for selected parameter distributions of reservoir properties, seal properties, numbers of wells, well properties, thief zones, and groundwater aquifer properties. A series of examples is used to illustrate how the risk under different storage conditions evolves over time, both during injection, in the near-term post injection period, and over the long term. It is also shown how results from NRAP-IAM-CS can be used to investigate the importance of different parameters on risk of leakage and risk of groundwater contamination under different storage conditions. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Pawar, Rajesh J.; Chu, Shaoping; Stauffer, Philip H.; Guthrie, George D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Bromhal, Grant S.; Dilmore, Robert M.] Natl Energy Technol Lab, South Pk Township, PA USA. [Oldenburg, Curtis M.; Zhang, Yingqi] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Pawar, RJ (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div EES 16, Los Alamos, NM 87545 USA. EM rajesh@lanl.gov RI Oldenburg, Curtis/L-6219-2013; OI Oldenburg, Curtis/0000-0002-0132-6016; Stauffer, Philip/0000-0002-6976-221X FU U.S. Department of Energy's (DOE) Office of Fossil Energy's Crosscutting Research program FX This work was completed as part of the National Risk Assessment Partnership (NRAP) project. Support for this project came from the U.S. Department of Energy's (DOE) Office of Fossil Energy's Crosscutting Research program. The authors wish to acknowledge Traci Rodosta and M. Kylee Rice (NETL Strategic Center for Coal) and Mark Ackiewicz (DOE Office of Fossil Energy) for programmatic guidance, direction, and support. The authors also wish to acknowledge contributions from researchers across the NRAP technical teams, who developed ROMs that are implemented in the NRAP-IAM-CS model. NR 44 TC 5 Z9 5 U1 5 U2 7 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD SEP PY 2016 VL 52 BP 175 EP 189 DI 10.1016/j.ijggc.2016.06.015 PG 15 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DT8GQ UT WOS:000381728300015 ER PT J AU Trainor-Guitton, W Mansoor, K Sun, YW Carroll, S AF Trainor-Guitton, Whitney Mansoor, Kayyum Sun, Yunwei Carroll, Susan TI Merits of pressure and geochemical data as indicators of CO2/brine leakage into a heterogeneous, sedimentary aquifer SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE CO2 storage; CO2 and brine leakage; Monitoring Reactive transport; Detectability ID SHALLOW GROUNDWATER SYSTEM; CO2 LEAKAGE; CARBON SEQUESTRATION; UNCERTAINTY QUANTIFICATION; ELECTRICAL-RESISTIVITY; SITE; STORAGE; PERFORMANCE; MIGRATION; IMPACTS AB This study assesses the merits of pressure data and geochemical data as indicators of a combined CO2/brine leakage into a heterogeneous, sedimentary aquifer. We simulate the changes in three aquifer responses (pressure, total dissolved solids (TDS), and pH) due to CO2/brine leakage at an abandoned well with an uncertain location and hypothesize that these changes can only be observed from a single shallow monitoring well, mimicking the low density of observation wells for the considered aquifer. Specifically, detection likelihoods are calculated to describe how frequently pressure, TDS, and pH signals will coincide with a leak for observations made at different distances and times from the initiation of the CO2/brine leakage rate. The pressure signal gives a more spatially extensive signal than either TDS or pH, and pressure detection probabilities increase upstream of flow barriers (pressurizing-affect). The pH and TDS rebound down-stream of the flow barriers. When only considering the samples that experience the highest leakage volumes, there is a 50% likelihood of detecting a pressure change 400 m away at times >= 30 years. However, the TDS and pH detection likelihoods are <20% at 100 m distance for times >= 30 years. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Trainor-Guitton, Whitney] Colorado Sch Mines, Dept Geophys, 1500 Illinois St, Golden, CO 80401 USA. [Trainor-Guitton, Whitney; Mansoor, Kayyum; Sun, Yunwei; Carroll, Susan] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Trainor-Guitton, W (reprint author), Colorado Sch Mines, Dept Geophys, 1500 Illinois St, Golden, CO 80401 USA. EM wtrainor@mines.edu FU U.S. Department of Energy's (DOE's) Office of Fossil Energy's Cross-cutting Research program FX This work is part of the National Risk Assessment Partnership (NRAP) which is supported by the U.S. Department of Energy's (DOE's) Office of Fossil Energy's Cross-cutting Research program. NR 30 TC 0 Z9 0 U1 3 U2 3 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD SEP PY 2016 VL 52 BP 237 EP 249 DI 10.1016/j.ijggc.2016.07.002 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DT8GQ UT WOS:000381728300020 ER PT J AU Keating, E Bacon, D Carroll, S Mansoor, K Sun, YW Zheng, LE Harp, D Dai, ZX AF Keating, Elizabeth Bacon, Diana Carroll, Susan Mansoor, Kayyum Sun, Yunwei Zheng, Liange Harp, Dylan Dai, Zhenxue TI Applicability of aquifer impact models to support decisions at CO2 sequestration sites SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Carbon sequestration; Groundwater impacts; Risk assessment; Reduced-order modeling ID DISSOLUTION KINETICS; GEOCHEMICAL IMPACTS; EVALUATING IMPACTS; POTABLE AQUIFERS; CARBON-DIOXIDE; SHALLOW; LEAKAGE; GROUNDWATER; ADSORPTION; FIELD AB The National Risk Assessment Partnership has developed a suite of tools to assess and manage risk at CO2 sequestration sites. This capability includes polynomial or look-up table based reduced-order models (ROMs) that predict the impact of CO2 and brine leaks on overlying aquifers. The development of these computationally-efficient models and the underlying reactive transport simulations they emulate has been documented elsewhere (Carroll et al, 2014a,b; Dal et al., 2014: Keating et al., 2016). In this paper, we seek to demonstrate applicability of ROM-based analysis by considering what types of decisions and aquifer types would benefit from the ROM analysis. We present four hypothetical examples where applying ROMs, in ensemble mode, could support decisions during a geologic CO2 sequestration project. These decisions pertain to site selection, site characterization, monitoring network evaluation, and health impacts. In all cases, we consider potential brine/CO2 leak rates at the base of the aquifer to be uncertain. We show that derived probabilities provide information relevant to the decision at hand. Although the ROMs were developed using site-specific data from two aquifers (High Plains and Edwards), the models accept aquifer characteristics as variable inputs and so they may have more broad applicability. We conclude that pH and TDS predictions are the most transferable to other aquifers based on the analysis of the nine water quality metrics (pH, TDS, 4 trace metals, 3 organic compounds). Guidelines are presented for determining the aquifer types for which the ROMs should be applicable. (C) Published by Elsevier Ltd. C1 [Keating, Elizabeth; Harp, Dylan; Dai, Zhenxue] Los Alamos Natl Lab, Earth & Environm Sci Div, MS T003, Los Alamos, NM 87545 USA. [Bacon, Diana] Pacific Northwest Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. [Carroll, Susan; Mansoor, Kayyum; Sun, Yunwei] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Zheng, Liange] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Keating, E (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, MS T003, Los Alamos, NM 87545 USA. EM ekeating@lanl.gov; Diana.Bacon@pnnl.gov; carroll6@llnl.gov; mansoor1@llnl.gov; sun4@llnl.gov; lzheng@lbl.gov; dharp@lanl.gov; daiz@lanl.gov RI zheng, liange/B-9748-2011; OI zheng, liange/0000-0002-9376-2535; Dai, Zhenxue/0000-0002-0805-7621 FU DOE Office of Fossil Energy's Crosscutting Research program FX This work was completed as part of National Risk Assessment Partnership (NRAP) project. Support for this project came from the DOE Office of Fossil Energy's Crosscutting Research program. The authors wish to acknowledge Robert Romanosky (NETL Strategic Center for Coal) and Regis Conrad (DOE Office of Fossil Energy) for programmatic guidance, direction, and support. Additionally, this work benefited greatly from thoughtful comments from three anonymous reviewers. NR 51 TC 0 Z9 0 U1 6 U2 7 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD SEP PY 2016 VL 52 BP 319 EP 330 DI 10.1016/j.ijggc.2016.07.001 PG 12 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DT8GQ UT WOS:000381728300025 ER PT J AU Rhiger, DR Smith, EP Kolasa, BP Kim, JK Klem, JF Hawkins, SD AF Rhiger, David R. Smith, Edward P. Kolasa, Borys P. Kim, Jin K. Klem, John F. Hawkins, Samuel D. TI Analysis of III-V Superlattice nBn Device Characteristics SO JOURNAL OF ELECTRONIC MATERIALS LA English DT Article DE Infrared; nBn; III-V material; superlattice; InAs/InAsSb; capacitance measurements AB Mid-wavelength infrared nBn detectors built with III-V superlattice materials have been tested by means of both capacitance and direct-current methods. By combining the results, it is possible to achieve clear separation of the two components of dark current, namely the generation-recombination (GR) current due to the Shockley-Read-Hall mechanism in the depletion region, and the diffusion current from the neutral region. The GR current component is unambiguously identified by two characteristics: (a) it is a linear function of the depletion width, and (b) its activation energy is approximately one-half the bandgap. The remaining current is shown to be due to diffusion because of its activation energy equaling the full bandgap. In addition, the activation energy of the total measured dark current in each local region of the temperature-bias parameter space is evaluated. We show the benefits of capacitance analysis applied to the nBn device and review some of the requirements for correct measurements. The carrier concentration of the unintentionally doped absorber region is found to be 1.2 x 10(14) cm(-3) n-type. It is shown that the depletion region resides almost entirely within the absorber. Also, the doping in the nBn barrier is found to be 4 x 10(15) cm(-3) p-type. Minority-carrier lifetimes estimated from the dark current components are on the order of 10 mu s. C1 [Rhiger, David R.; Smith, Edward P.; Kolasa, Borys P.] Raytheon Vis Syst, 75 Coromar Dr, Goleta, CA 93117 USA. [Kim, Jin K.; Klem, John F.; Hawkins, Samuel D.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Rhiger, DR (reprint author), Raytheon Vis Syst, 75 Coromar Dr, Goleta, CA 93117 USA. EM drhiger@raytheon.com NR 19 TC 2 Z9 2 U1 10 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0361-5235 EI 1543-186X J9 J ELECTRON MATER JI J. Electron. Mater. PD SEP PY 2016 VL 45 IS 9 BP 4646 EP 4653 DI 10.1007/s11664-016-4545-y PG 8 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Physics, Applied SC Engineering; Materials Science; Physics GA DS9CM UT WOS:000381080000022 ER PT J AU Yoo, W Sim, A AF Yoo, Wucherl Sim, Alex TI Time-Series Forecast Modeling on High-Bandwidth Network Measurements SO JOURNAL OF GRID COMPUTING LA English DT Article DE Data modeling; Time series; Prediction model; Network measurements; Network traffic ID AVAILABLE BANDWIDTH; TCP THROUGHPUT AB With the increasing number of geographically distributed scientific collaborations and the growing sizes of scientific data, it has become challenging for users to achieve the best possible network performance on a shared network. We have developed a model to forecast expected bandwidth utilization on high-bandwidth wide area networks. The forecast model can improve the efficiency of the resource utilization and scheduling of data movements on high-bandwidth networks to accommodate ever increasing data volume for large-scale scientific data applications. A univariate time-series forecast model is developed with the Seasonal decomposition of Time series by Loess (STL) and the AutoRegressive Integrated Moving Average (ARIMA) on Simple Network Management Protocol (SNMP) path utilization measurement data. Compared with the traditional approach such as Box-Jenkins methodology to train the ARIMA model, our forecast model reduces computation time up to 92.6 %. It also shows resilience against abrupt network usage changes. Our forecast model conducts the large number of multi-step forecast, and the forecast errors are within the mean absolute deviation (MAD) of the monitored measurements. C1 [Yoo, Wucherl; Sim, Alex] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Yoo, W (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wyoo@lbl.gov FU Office of Advanced Scientific Computing Research, Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Office of Advanced Scientific Computing Research, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors would like to thank Chris Tracy, Jon Dugan, Brian Tierney, Inder Monga, and Gregory Bell at ESnet; Arie Shoshani, K. John Wu, Joy Bonaguro, and Jay Krous at LBNL; Richard Carlson at Dept. of Energy. NR 38 TC 0 Z9 0 U1 5 U2 5 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1570-7873 EI 1572-9184 J9 J GRID COMPUT JI J. Comput. PD SEP PY 2016 VL 14 IS 3 BP 463 EP 476 DI 10.1007/s10723-016-9368-9 PG 14 WC Computer Science, Information Systems; Computer Science, Theory & Methods SC Computer Science GA DT0FP UT WOS:000381158800005 ER PT J AU Glosser, D Kutchko, B Benge, G Crandall, D Ley, MT AF Glosser, D. Kutchko, B. Benge, G. Crandall, D. Ley, M. T. TI Relationship between operational variables, fundamental physics and foamed cement properties in lab and field generated foamed cement slurries SO JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING LA English DT Article DE Energy; Foamed cement; Wellbores; Engineering ID PASTE AB Foamed cement is a critical component for wellbore stability. The mechanical performance of a foamed cement depends on its microstructure, which in turn depends on the preparation method and attendant operational variables. Determination of cement stability for field use is based on laboratory testing protocols governed by API Recommended Practice 10B-4 (API RP 10B-4, 2015). However, laboratory and field operational variables contrast considerably in terms of scale, as well as slurry mixing and foaming processes. Here, laboratory and field operational processes are characterized within a physics-based framework. It is shown that the "atomization energy" imparted by the high pressure injection of nitrogen gas into the field mixed foamed cement slurry is - by a significant margin - the highest energy process, and has a major impact on the void system in the cement slurry. There is no analog for this high energy exchange in current laboratory cement preparation and testing protocols. Quantifying the energy exchanges across the laboratory and field processes provides a basis for understanding relative impacts of these variables on cement structure, and can ultimately lead to the development of practices to improve cement testing and performance. Published by Elsevier B.V. C1 [Glosser, D.; Kutchko, B.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Glosser, D.] Oak Ridge Inst Sci Educ, Oak Ridge, TN USA. [Crandall, D.] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Benge, G.] Benge Consulting, The Woodlands, TX USA. [Ley, M. T.] Oklahoma State Univ, Sch Civil & Environm Engn, Stillwater, OK 74078 USA. RP Kutchko, B (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM Barbara.Kutchko@netl.doe.gov FU U.S. Department of Energy FX This work was completed as part of National Energy Technology Laboratory (NETL) research for the Department of Energy's Complementary Research Program under Section 999 of the Energy Policy Act of 2005. This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. The authors wish to acknowledge Roy Long (NETL Strategic Center for Natural Gas and Oil) and Elena Melchert (DOE Office of Fossil Energy) for programmatic guidance, direction, and support. The authors would like to thank Bryan Tennant, Karl Jarvis and Roger Lapeer for making the CT scanner lab functional. Thanks to Rick Spaulding and Jim Fazio for superior laboratory assistance. The authors extend a special thanks to Erick Cunningham and Woody Lawrence, and to Kelly Rose and Jen Bauer. DBG would also like to thank S. Miaskeiwicz, E. Anish, the Millers, Russell Schwartz, and the Arnolds. NR 27 TC 0 Z9 1 U1 6 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-4105 EI 1873-4715 J9 J PETROL SCI ENG JI J. Pet. Sci. Eng. PD SEP PY 2016 VL 145 BP 66 EP 76 DI 10.1016/j.petrol.2016.03.014 PG 11 WC Energy & Fuels; Engineering, Petroleum SC Energy & Fuels; Engineering GA DT9PU UT WOS:000381835600006 ER PT J AU Dhuwe, A Klara, A Sullivan, J Lee, J Cummings, S Beckman, E Enick, R Perry, R AF Dhuwe, Aman Klara, Alex Sullivan, James Lee, Jason Cummings, Stephen Beckman, Eric Enick, Robert Perry, Robert TI Assessment of solubility and viscosity of ultra-high molecular weight polymeric thickeners in ethane, propane and butane for miscible EOR SO JOURNAL OF PETROLEUM SCIENCE AND ENGINEERING LA English DT Article DE Ethane; Propane; Butane; Thickener; Ultrahigh molecular weight polymer; Poly-alpha-olefin ID THERMODYNAMIC PROPERTY MODEL; PRESSURE PHASE-BEHAVIOR; CARBON-DIOXIDE; POLY(ETHYLENE-CO-METHYL ACRYLATE); N-BUTANE; SYSTEMS; EQUILIBRIA; COPOLYMER; OIL; CO2 AB Natural gas liquid (NGL), a mixture consisting primarily of ethane, propane, and butane, is an excellent enhanced oil recovery (EOR) solvent. However, NGL is typically about ten times less viscous than the crude oil within the carbonate or sandstone porous media, which causes the NGL to finger through the rock toward production wells resulting in low volumetricsweep efficiency in five-spot patterns or during a linear drive displacement. The viscosity of candidate polymeric NGL thickeners is measured with a windowed, close-clearance falling ball viscometer, and an expression for the average shear rate associated with this type of viscometer is derived. High molecular weight polydimethyl siloxane (PDMS, MW 9.8 10(5)) can thicken ethane, propane and butane, but the viscosity enhancement is very modest (e.g. a doubling of butane viscosity with 2% PDMS at 7 MPa and 25 degrees C), making field application of PDMS unlikely. A dilute concentration of a drag-reducing agent (DRA) poly-alpha-olefin that has an average molecular weight greater than 2.0 10(7) is more promising as a potential thickener for liquid butane, liquid propane and liquid or supercritical ethane. The DRA polymer, which is introduced as an extremely viscous 1% or 2% solution in hexane, is soluble in butane and propane at 25-60 degrees C and concentrations up to at least 0.5 wt% at pressures slightly above the vapor pressure of butane or propane. The DRA polymer is much more difficult to dissolve in ethane, however, requiring pressures of more than 20 MPa. The DRA polymer is especially effective for thickening butane (e.g. a 4.8-fold viscosity increase at 25 degrees C, 55.16 MPa and 0.2 wt% DRA). The DRA is less effective for increasing propane viscosity (e.g. a 2.3-fold viscosity increase at the same conditions), and even less effective for thickening ethane. In general, viscosity enhancement increases with decreasing temperature, increasing pressure, and an increase in the carbon number of the light alkane, which are reflective of increased NGL solvent strength at low temperature and high pressure. Practical application of DRA during EOR may be hindered, however, by the relatively high concentration (similar to 5000 ppm) of DRA polymer required for order-of-magnitude viscosity increases, very high pressure requirements for DRA dissolution if the ethane content of the NGL is high, and the large amount of hexane that would have to be introduced if the DRA polymer if it is introduced as a solution in hexane. (C) 2016 Elsevier B.V. All rights reserved. C1 [Dhuwe, Aman; Sullivan, James; Lee, Jason; Cummings, Stephen; Beckman, Eric; Enick, Robert] Univ Pittsburgh, Swanson Sch Engn, Dept Chem & Petr Engn, 940 Benedum Engn Hall,3700 OHara St, Pittsburgh, PA 15261 USA. [Klara, Alex] Penn State Univ, Sch Elect Engn & Comp Sci, University Pk, PA 16802 USA. [Enick, Robert] US DOE, Natl Energy Technol Lab, Off Res & Dev, Pittsburgh, PA 15236 USA. [Perry, Robert] GE Global Res, Res Circle, Niskayuna, NY 12309 USA. RP Enick, R (reprint author), Univ Pittsburgh, Swanson Sch Engn, Dept Chem & Petr Engn, 940 Benedum Engn Hall,3700 OHara St, Pittsburgh, PA 15261 USA. EM rme@pitt.edu FU U.S. Department of Energy Advanced Research Project Agency-Energy (ARPA-E) [DE-AR0000292] FX This work was supported by the U.S. Department of Energy Advanced Research Project Agency-Energy (ARPA-E) (Contract No. DE-AR0000292). The authors are grateful to them for their support. We would also like to express our appreciation to Lubrizol for their enthusiastic support of the newly formed Lubrizol Innovation Collaboration in the Department of Chemical and Petroleum Engineering at the Swanson School of Engineering at the University of Pittsburgh. NR 48 TC 2 Z9 2 U1 9 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-4105 EI 1873-4715 J9 J PETROL SCI ENG JI J. Pet. Sci. Eng. PD SEP PY 2016 VL 145 BP 266 EP 278 DI 10.1016/j.petrol.2016.05.018 PG 13 WC Energy & Fuels; Engineering, Petroleum SC Energy & Fuels; Engineering GA DT9PU UT WOS:000381835600024 ER PT J AU Yu, HJ Takeuchi, H Takeuchi, M Liu, Q Kantharia, J Haltiwanger, RS Li, HL AF Yu, Hongjun Takeuchi, Hideyuki Takeuchi, Megumi Liu, Qun Kantharia, Joshua Haltiwanger, Robert S. Li, Huilin TI Structural analysis of Notch-regulating Rumi reveals basis for pathogenic mutations SO NATURE CHEMICAL BIOLOGY LA English DT Article ID O-GLCNAC TRANSFERASE; SQUAMOUS-CELL CARCINOMA; CANCER; GLUCOSYLTRANSFERASE; MECHANISM; DIFFRACTION; PATHWAY; GLYCOSYLTRANSFERASES; XYLOSYLTRANSFERASE; GLYCOSYLATION AB Rumi O-glucosylates the EGF repeats of a growing list of proteins essential in metazoan development, including Notch. Rumi is essential for Notch signaling, and Rumi dysregulation is linked to several human diseases. Despite Rumi's critical roles, it is unknown how Rumi glucosylates a serine of many but not all EGF repeats. Here we report crystal structures of Drosophila Rumi as binary and ternary complexes with a folded EGF repeat and/or donor substrates. These structures provide insights into the catalytic mechanism and show that Rumi recognizes structural signatures of the EGF motif, the U-shaped consensus sequence,C-X-S-X-(P/A)-C and a conserved hydrophobic region. We found that five Rumi mutations identified in cancers and Dowling-Degos disease are clustered around the enzyme active site and adversely affect its activity. Our study suggests that loss of Rumi activity may underlie these diseases, and the mechanistic insights may facilitate the development of modulators of Notch signaling. C1 [Yu, Hongjun; Liu, Qun; Li, Huilin] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Takeuchi, Hideyuki; Takeuchi, Megumi; Haltiwanger, Robert S.] Univ Georgia, Complex Carbohydrate Res Ctr, 220 Riverbend Rd, Athens, GA 30602 USA. [Kantharia, Joshua; Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. RP Li, HL (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.; Haltiwanger, RS (reprint author), Univ Georgia, Complex Carbohydrate Res Ctr, 220 Riverbend Rd, Athens, GA 30602 USA.; Li, HL (reprint author), SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. EM rhalti@uga.edu; hli@bnl.gov FU NIH [GM061126, AG029979]; SBU-BNL; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-AC02-06CH11357] FX We thank members of the Li and Haltiwanger labs for critical comments on this work, as well as S. Singh Johar for technical assistance. The work was supported by the NIH (grants GM061126 (to R.S.H.) and AG029979 (to H.L.)) and SBU-BNL (seed grant to R.S.H. and H.L.). We acknowledge access to beamlines X25, X29 and X4A at NSLS, Brookhaven National Laboratory and LRL-CAT at APS, Argonne National Laboratory, and we thank the staff at these beamlines. NSLS and APS were supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract nos. DE-AC02-98CH10886 and DE-AC02-06CH11357, respectively. Use of the Lilly Research Laboratories Collaborative Access Team (LRL-CAT) beamline at Sector 31 of the Advanced Photon Source was provided by Eli Lilly Company, which operates the facility. The results published here are in part based on data generated by the TCGA Research Network (http://cancergenome.nih.gov/). H.L. dedicates this work to the loving memory of his son Paul J. Li. NR 52 TC 0 Z9 0 U1 7 U2 7 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1552-4450 EI 1552-4469 J9 NAT CHEM BIOL JI Nat. Chem. Biol. PD SEP PY 2016 VL 12 IS 9 BP 735 EP + DI 10.1038/nchembio.2135 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DU5MF UT WOS:000382255100016 PM 27428513 ER PT J AU Souhan, B Chen, CP Lu, M Stein, A Bakhru, H Grote, RR Bergman, K Green, WMJ Osgood, RM AF Souhan, Brian Chen, Christine P. Lu, Ming Stein, Aaron Bakhru, Hassaram Grote, Richard R. Bergman, Keren Green, William M. J. Osgood, Richard M., Jr. TI Ar+-Implanted Si-Waveguide Photodiodes for Mid-Infrared Detection SO PHOTONICS LA English DT Article DE silicon; photodetectors; integrated optics devices ID ERROR-FREE OPERATION; MU-M; INFRARED PHOTODIODES; AVALANCHE PHOTODIODE; SILICON; PHOTODETECTORS; MODULATION; BANDWIDTH; MODE; BAND AB Complementary metal-oxide-semiconductor (CMOS)-compatible Ar+-implanted Si-waveguide p-i-n photodetectors operating in the mid-infrared (2.2 to 2.3 mu m wavelengths) are demonstrated at room temperature. Responsivities exceeding 21 mA/ W are measured at a 5 V reverse bias with an estimated internal quantum efficiency of 3.1%-3.7%. The dark current is found to vary from a few nanoamps down to less than 11 pA after post-implantation annealing at 350 degrees C. Linearity is demonstrated over four orders of magnitude, confirming a single-photon absorption process. The devices demonstrate a higher thermal processing budget than similar Si+-implanted devices and achieve higher responsivity after annealing up to 350 degrees C. C1 [Souhan, Brian] US Mil Acad, Photon Res Ctr, West Point, NY 10996 USA. [Chen, Christine P.; Bergman, Keren] Columbia Univ, Dept Elect Engn, 500 W 120th St, New York, NY 10027 USA. [Lu, Ming; Stein, Aaron] Brookhaven Natl Lab, Ctr Funct Nanomat, POB 5000, Upton, NY 11973 USA. [Bakhru, Hassaram] SUNYPOLY, Coll Nanoscale Sci & Engn, Albany, NY 12203 USA. [Grote, Richard R.] Univ Penn, Dept Elect & Syst Engn, 200 S 33rd St, Philadelphia, PA 19104 USA. [Green, William M. J.] IBM TJ Watson Res Ctr, 1101 Kitchawan Rd, Yorktown Hts, NY 10598 USA. [Osgood, Richard M., Jr.] Columbia Univ, Microelect Sci Labs, 500 W 120th St, New York, NY 10027 USA. RP Souhan, B (reprint author), US Mil Acad, Photon Res Ctr, West Point, NY 10996 USA. EM brian.souhan@gmail.com; cpc2143@columbia.edu; mlu@bnl.gov; stein@bnl.gov; hbakhru@sunypoly.edu; rgrote@seas.upenn.edu; bergman@ee.columbia.edu; wgreen@us.ibm.com; osgood@columbia.edu NR 27 TC 0 Z9 0 U1 6 U2 8 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 2304-6732 J9 PHOTONICS JI Photonics PD SEP PY 2016 VL 3 IS 3 AR 46 DI 10.3390/photonics3030046 PG 8 WC Optics SC Optics GA DT9ZG UT WOS:000381860400006 ER PT J AU Hommel, R Siegwolf, R Zavadlav, S Arend, M Schaub, M Galiano, L Haeni, M Kayler, ZE Gessler, A AF Hommel, R. Siegwolf, R. Zavadlav, S. Arend, M. Schaub, M. Galiano, L. Haeni, M. Kayler, Z. E. Gessler, A. TI Impact of interspecific competition and drought on the allocation of new assimilates in trees SO PLANT BIOLOGY LA English DT Article DE Carbon isotope labelling; mean residence time; osmotic adjustment; phloem transport; respiration ID BEECH FAGUS-SYLVATICA; CARBON-ISOTOPE COMPOSITION; RECENTLY FIXED CARBON; EUROPEAN BEECH; ACER-PLATANOIDES; CLIMATE-CHANGE; NORWAY SPRUCE; NITROGEN-COMPOUNDS; RESIDENCE TIME; FOREST AB In trees, the interplay between reduced carbon assimilation and the inability to transport carbohydrates to the sites of demand under drought might be one of the mechanisms leading to carbon starvation. However, we largely lack knowledge on how drought effects on new assimilate allocation differ between species with different drought sensitivities and how these effects are modified by interspecific competition. We assessed the fate of C-13 labelled assimilates in above- and belowground plant organs and in root/rhizosphere respired CO2 in saplings of drought-tolerant Norway maple (Acer platanoides) and drought-sensitive European beech (Fagus sylvatica) exposed to moderate drought, either in mono- or mixed culture. While drought reduced stomatal conductance and photosynthesis rates in both species, both maintained assimilate transport belowground. Beech even allocated more new assimilate to the roots under moderate drought compared to non-limited water supply conditions, and this pattern was even more pronounced under interspecific competition. Even though maple was a superior competitor compared to beech under non-limited soil water conditions, as indicated by the changes in above- and belowground biomass of both species in the interspecific competition treatments, we can state that beech was still able to efficiently allocate new assimilate belowground under combined drought and interspecific competition. This might be seen as a strategy to maintain root osmotic potential and to prioritise root functioning. Our results thus show that beech tolerates moderate drought stress plus competition without losing its ability to supply belowground tissues. It remains to be explored in future work if this strategy is also valid during long-term drought exposure. C1 [Hommel, R.; Kayler, Z. E.; Gessler, A.] Inst Landscape Biogeochem, Leibniz Ctr Agr Landscape Res ZALF, Muncheberg, Germany. [Siegwolf, R.] Paul Scherrer Inst, Lab Atmospher Chem Stable Isotopes & Ecosyst Flux, Villigen, Switzerland. [Zavadlav, S.] Dept Forest Physiol & Genet, Ljubljana, Slovenia. [Arend, M.; Schaub, M.; Galiano, L.; Haeni, M.; Gessler, A.] Swiss Fed Inst Forest Snow & Landscape Res WSL, CH-8903 Birmensdorf, Switzerland. [Galiano, L.] Univ Freiburg, Inst Hydrol, Freiburg, Germany. [Gessler, A.] Berlin Brandenburg Inst Adv Biodivers Res BBIB, Berlin, Germany. [Kayler, Z. E.] US Forest Serv, USDA, Northern Res Stn, Lawrence Livermore Natl Lab, Livermore, CA USA. RP Gessler, A (reprint author), Swiss Fed Inst Forest Snow & Landscape Res WSL, CH-8903 Birmensdorf, Switzerland. EM arthur.gessler@wsl.ch RI Gessler, Arthur/C-7121-2008; Arend, Matthias/L-7795-2013; Galiano, Lucia/P-1818-2016; Haeni, Matthias/A-3446-2013; Schaub, Marcus/E-4874-2012 OI Gessler, Arthur/0000-0002-1910-9589; Galiano, Lucia/0000-0003-0123-1882; Haeni, Matthias/0000-0003-3977-2166; Schaub, Marcus/0000-0002-0158-8892 FU Deutsche Forschungsgemeinschaft [GE 1090/8-1, GE 1090/9-1] FX The authors are grateful to Eva Hilbig for continuous support during all labelling experiments, and Johannes Bruckhoff for preparing the custom chambers. Special thanks to Katja Felsmann, Ruth Lamparter, Kirstin Jansen, Lucia Atanet, Susanne Remus, Florian Reverey, Richard Hommel, Rainer Hentschel and Martin Hentschel for huge help during the harvests and analyses. We thank Stephan Wirth for the supply of the Picarro. The project was funded by the Deutsche Forschungsgemeinschaft (Grant numbers: GE 1090/8-1 and 9-1). NR 69 TC 3 Z9 3 U1 31 U2 52 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1435-8603 EI 1438-8677 J9 PLANT BIOLOGY JI Plant Biol. PD SEP PY 2016 VL 18 IS 5 BP 785 EP 796 DI 10.1111/plb.12461 PG 12 WC Plant Sciences SC Plant Sciences GA DS8IT UT WOS:000381027400006 PM 27061772 ER PT J AU Jones-Albertus, R Feldman, D Fu, R Horowitz, K Woodhouse, M AF Jones-Albertus, Rebecca Feldman, David Fu, Ran Horowitz, Kelsey Woodhouse, Michael TI Technology advances needed for photovoltaics to achieve widespread grid price parity SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE economics; LCOE; photovoltaics AB To quantify the potential value of technological advances to the photovoltaics (PV) sector, this paper examines the impact of changes to key PV module and system parameters on the levelized cost of energy (LCOE). The parameters selected include module manufacturing cost, efficiency, degradation rate, and service lifetime. NREL's System Advisor Model (SAM) is used to calculate the lifecycle cost per kilowatt-hour (kWh) for residential, commercial, and utility scale PV systems within the contiguous United States, with a focus on utility scale. Different technological pathways are illustrated that may achieve the Department of Energy's SunShot goal of PV electricity that is at grid price parity with conventional electricity sources. In addition, the impacts on the 2015 baseline LCOE due to changes to each parameter are shown. These results may be used to identify research directions with the greatest potential to impact the cost of PV electricity. Copyright (c) 2016 John Wiley & Sons, Ltd. C1 [Jones-Albertus, Rebecca] US DOE, Off Energy Efficiency & Renewable Energy, Solar Energy Technol Off, Washington, DC 20585 USA. [Feldman, David; Fu, Ran; Horowitz, Kelsey; Woodhouse, Michael] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO USA. RP Jones-Albertus, R (reprint author), US DOE, Off Energy Efficiency & Renewable Energy, Solar Energy Technol Off, Washington, DC 20585 USA.; Woodhouse, M (reprint author), Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO USA.; Woodhouse, M (reprint author), Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Washington, DC USA. EM rebecca.jones-albertus@ee.doe.gov; michael.woodhouse@nrel.gov NR 14 TC 3 Z9 3 U1 13 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD SEP PY 2016 VL 24 IS 9 BP 1272 EP 1283 DI 10.1002/pip.2755 PG 12 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DS7LJ UT WOS:000380964700010 ER PT J AU Ward, JS Remo, T Horowitz, K Woodhouse, M Sopori, B VanSant, K Basore, P AF Ward, J. Scott Remo, Timothy Horowitz, Kelsey Woodhouse, Michael Sopori, Bhushan VanSant, Kaitlyn Basore, Paul TI Techno-economic analysis of three different substrate removal and reuse strategies for III-V solar cells SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE photovoltaics; III-V; substrate; reuse ID EPITAXIAL LIFT-OFF; HIGH-EFFICIENCY; SI; TECHNOLOGY; CRACKING; FILMS AB The high cost of wafers suitable for epitaxial deposition of III-V solar cells has been a primary barrier to widespread use of these cells in low-concentration and one-sun terrestrial solar applications. A possible solution is to reuse the substrate many times, thus spreading its cost across many cells. We performed a bottom-up techno-economic analysis of three different strategies for substrate reuse in high-volume manufacturing: epitaxial lift-off, spalling, and the use of a porous germanium release layer. The analysis shows that the potential cost reduction resulting from substrate reuse is limited in all three strategies--not by the number of reuse cycles achievable, but by the costs that are incurred in each cycle to prepare the substrate for another epitaxial deposition. The dominant substrate-preparation cost component is different for each of the three strategies, and the cost-ranking of these strategies is subject to change if future developments substantially reduce the cost of epitaxial deposition. Copyright (c) 2016 John Wiley & Sons, Ltd. C1 [Ward, J. Scott; Remo, Timothy; Horowitz, Kelsey; Woodhouse, Michael; Sopori, Bhushan; VanSant, Kaitlyn; Basore, Paul] Natl Renewable Energy Lab, Golden, CO USA. RP Ward, JS (reprint author), Natl Renewable Energy Lab, Golden, CO USA. EM scott.ward@nrel.gov FU US Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; DOE Solar Energy Technologies Office [DE-EE00025784] FX This work was supported by the US Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding provided by the DOE Solar Energy Technologies Office under agreement DE-EE00025784 for "PV Partnering & Business Development." The US Government and the publisher, by accepting the article for publication, acknowledge that the US Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for US Government purposes. NR 27 TC 1 Z9 1 U1 8 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD SEP PY 2016 VL 24 IS 9 BP 1284 EP 1292 DI 10.1002/pip.2776 PG 9 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DS7LJ UT WOS:000380964700011 ER PT J AU Ginley, D Granqvist, CG Kiriakidis, G Klein, A Kamiya, T Hosono, H AF Ginley, David Granqvist, Claes-G. Kiriakidis, George Klein, Andreas Kamiya, Toshio Hosono, Hideo TI 9th International Symposium on Transparent Oxide and Related Materials for Electronics and Optics (TOEO9) Preface SO THIN SOLID FILMS LA English DT Editorial Material C1 [Ginley, David] NREL, Golden, CO 80401 USA. [Granqvist, Claes-G.] Uppsala Univ, Uppsala, Sweden. [Kiriakidis, George] Univ Crete, Rethimnon, Greece. [Klein, Andreas] Tech Univ Darmstadt, Darmstadt, Germany. [Kamiya, Toshio; Hosono, Hideo] Tokyo Tech, Tokyo, Japan. RP Ginley, D (reprint author), NREL, Golden, CO 80401 USA. RI Kamiya, Toshio/E-8615-2014; Kiriakidis, George/G-9685-2011 OI Kamiya, Toshio/0000-0002-8358-240X; NR 0 TC 0 Z9 0 U1 3 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD SEP 1 PY 2016 VL 614 BP 43 EP 43 DI 10.1016/j.tsf.2016.07.054 PN B PG 1 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DS8KW UT WOS:000381033200001 ER PT J AU de Souza, MM Oostrom, M White, MD da Silva, GC Barbosa, MC AF de Souza, Michelle Matos Oostrom, Mart White, Mark D. da Silva, Gerson Cardoso, Jr. Barbosa, Maria Claudia TI Simulation of Subsurface Multiphase Contaminant Extraction Using a Bioslurping Well Model SO TRANSPORT IN POROUS MEDIA LA English DT Article DE Well model; Bioslurping; STOMP; Multiphase extraction; LNAPL recovery ID NUMERICAL RESERVOIR SIMULATION; NONAQUEOUS PHASE LIQUIDS; POROUS-MEDIA; UNCONFINED AQUIFERS; FLOW; HYDROCARBON; PERMEABILITY; REMEDIATION; MIGRATION; RECOVERY AB Subsurface simulation of multiphase extraction from wells is notoriously difficult. Explicit representation of well geometry requires small grid resolution, potentially leading to large computational demands. To reduce the problem dimensionality, multiphase extraction is mostly modeled using vertically averaged approaches. In this paper, a multiphase well model approach is presented as an alternative to simplify the application. The well model, a multiphase extension of the classic Peaceman model, has been implemented in the STOMP simulator. The numerical solution approach accounts for local conditions and gradients in the exchange of fluids between the well and the aquifer. Advantages of this well model implementation include the option to simulate the effects of well characteristics and operation. Simulations were conducted investigating the effects of extraction location, applied vacuum pressure, and a number of hydraulic properties. The obtained results were all consistent and logical. A major outcome of the test simulations is that, in contrast to common recommendations to extract from either the gas-NAPL or the NAPL-aqueous phase interface, the optimum extraction location should be in between these two levels. The new model implementation was also used to simulate extraction at a field site in Brazil. The simulation shows a good match with the field data, suggesting that the new STOMP well module may correctly represent oil removal. The field simulations depend on the quality of the site conceptual model, including the porous media and contaminant properties and the boundary and extraction conditions adopted. The new module may potentially be used to design field applications and analyze extraction data. C1 [de Souza, Michelle Matos; Barbosa, Maria Claudia] Univ Fed Rio de Janeiro, COPPE UFRJ, Civil Engn Program, Pedro Calmon Ave,POB 68506, Rio De Janeiro, RJ, Brazil. [Oostrom, Mart; White, Mark D.] Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [da Silva, Gerson Cardoso, Jr.] Univ Fed Rio de Janeiro, Dept Geol, CCMN, Athos da Silveira Ramos Ave 274, Rio De Janeiro, RJ, Brazil. RP de Souza, MM (reprint author), Univ Fed Rio de Janeiro, COPPE UFRJ, Civil Engn Program, Pedro Calmon Ave,POB 68506, Rio De Janeiro, RJ, Brazil. EM mmsouza79@gmail.com; mart.oostrom@pnnl.gov; mark.white@pnnl.gov; gerson@acd.ufrj.br; mclaudia@coc.ufrj.br RI da Silva Jr., Gerson/C-5767-2013 OI da Silva Jr., Gerson/0000-0002-7160-0893 FU Department of Energy (DOE) [DE-AC06-76RLO 1830]; National Counsel of Technological and Scientific Development (CNPq); Science without Borders Program (CAPES-Ciencia sem fronteiras) FX Pacific Northwest National Laboratory (PNNL) is operated by the Battelle Memorial Institute for the Department of Energy (DOE) under Contract DE-AC06-76RLO 1830. Part of the work was completed by the senior author as a visiting scholar at the Environmental Molecular Sciences Laboratory (EMSL), a scientific user facility of the United States Department of Energy's Office of Biological and Environmental Research operated by the Pacific Northwest National Laboratory (PNNL). The senior author is grateful to the Brazilian agencies-National Counsel of Technological and Scientific Development (CNPq) and the Science without Borders Program (CAPES-Ciencia sem fronteiras)-for a research scholarship under which this work was carried out. NR 49 TC 0 Z9 0 U1 5 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0169-3913 EI 1573-1634 J9 TRANSPORT POROUS MED JI Transp. Porous Media PD SEP PY 2016 VL 114 IS 3 BP 649 EP 673 DI 10.1007/s11242-016-0738-3 PG 25 WC Engineering, Chemical SC Engineering GA DU3EZ UT WOS:000382094900002 ER PT J AU Vine, EL Jones, CM AF Vine, Edward L. Jones, Christopher M. TI Competition, carbon, and conservation: Assessing the energy savings potential of energy efficiency competitions SO ENERGY RESEARCH & SOCIAL SCIENCE LA English DT Article DE Energy efficiency; Competition; Persistence; Behavior; Comparative feedback; Social norms ID CONSUMPTION; RISK AB Competition has become an increasingly popular strategy to engage individuals in energy and resource conservation; however, there has not been an objective, independent review of existing competition programs focusing on the reduction of energy use. This paper attempts to address this shortcoming. This paper reviews a representative selection of completed and ongoing energy reduction competitions in the United States and uses the lessons learned to provide best practice guidance on the design, implementation, and evaluation of future programs. Four key research questions are addressed in this study: How effective have competitions been at changing behavior and reducing energy? How long do energy savings persist after the end of competitions? Under what circumstances are competitions more or less effective? What are common best practices for the design, implementation and evaluation of energy and resource conservation competitions? The primary target audiences for this paper are electric and natural gas utilities seeking to broaden their portfolio of behavior-based interventions, as well as potential designers, implementers and evaluators of energy reduction competitions. Our intention is to improve the effectiveness of competitions and to suggest when competition may or may not be an effective strategy to save energy over the long term. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Vine, Edward L.] Calif Inst Energy & Environm, Berkeley, CA USA. [Jones, Christopher M.] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Vine, EL (reprint author), Lawrence Berkeley Natl Lab, CIEE, Bldg 90-2128, Berkeley, CA 94720 USA. EM elvine@lbl.gov NR 49 TC 0 Z9 0 U1 4 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2214-6296 EI 2214-6326 J9 ENERGY RES SOC SCI JI Energy Res. Soc. Sci. PD SEP PY 2016 VL 19 BP 158 EP 176 DI 10.1016/j.erss.2016.06.013 PG 19 WC Environmental Studies SC Environmental Sciences & Ecology GA DT7BJ UT WOS:000381640400017 ER PT J AU McManamay, R Brewer, S Jager, H Troia, M AF McManamay, Ryan A. Brewer, Shannon K. Jager, Henriette I. Troia, Matthew J. TI Organizing Environmental Flow Frameworks to Meet Hydropower Mitigation Needs SO ENVIRONMENTAL MANAGEMENT LA English DT Article DE Dams; Rivers; Regulation; Policy; Environmental flow; Hydrology ID MODIFYING DAM OPERATIONS; HYDROLOGIC ALTERATION; ECOLOGICAL RESPONSES; RESERVOIR OPERATION; RIVER ECOSYSTEMS; FISH ASSEMBLAGE; STREAM; WATER; HABITAT; REGIME AB The global recognition of the importance of natural flow regimes to sustain the ecological integrity of river systems has led to increased societal pressure on the hydropower industry to change plant operations to improve downstream aquatic ecosystems. However, a complete reinstatement of natural flow regimes is often unrealistic when balancing water needs for ecosystems, energy production, and other human uses. Thus, stakeholders must identify a prioritized subset of flow prescriptions that meet ecological objectives in light of realistic constraints. Yet, isolating aspects of flow regimes to restore downstream of hydropower facilities is among the greatest challenges of environmental flow science due, in part, to the sheer volume of available environmental flow tools in conjunction with complex negotiation-based regulatory procedures. Herein, we propose an organizational framework that structures information and existing flow paradigms into a staged process that assists stakeholders in implementing environmental flows for hydropower facilities. The framework identifies areas where regulations fall short of the needed scientific process, and provide suggestions for stakeholders to ameliorate those situations through advanced preparation. We highlight the strengths of existing flow paradigms in their application to hydropower settings and suggest when and where tools are most applicable. Our suggested framework increases the effectiveness and efficiency of the e-flow implementation process by rapidly establishing a knowledge base and decreasing uncertainty so more time can be devoted to filling knowledge gaps. Lastly, the framework provides the structure for a coordinated research agenda to further the science of environmental flows related to hydropower environments. C1 [McManamay, Ryan A.; Jager, Henriette I.; Troia, Matthew J.] Oak Ridge Natl Lab, Div Environm Sci, 1 Bethel Valley Rd,MS-6351,POB 2008, Oak Ridge, TN 37831 USA. [Brewer, Shannon K.] Oklahoma State Univ, US Geol Survey, Oklahoma Cooperat Fish & Wildlife Res Unit, Stillwater, OK 74078 USA. RP McManamay, R (reprint author), Oak Ridge Natl Lab, Div Environm Sci, 1 Bethel Valley Rd,MS-6351,POB 2008, Oak Ridge, TN 37831 USA. EM mcmanamayra@ornl.gov FU US Department of Energy [AC05-00OR22725]; Department of Energy FX This manuscript has been authored by employees of UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doepublic-access-plan). NR 88 TC 0 Z9 0 U1 12 U2 12 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0364-152X EI 1432-1009 J9 ENVIRON MANAGE JI Environ. Manage. PD SEP PY 2016 VL 58 IS 3 BP 365 EP 385 DI 10.1007/s00267-016-0726-y PG 21 WC Environmental Sciences SC Environmental Sciences & Ecology GA DS3IM UT WOS:000380676300001 PM 27344163 ER PT J AU Gao, J Zhang, AP Lam, SK Zhang, XS Thomson, AM Lin, E Jiang, KJ Clarke, LE Edmonds, JA Kyle, PG Yu, S Zhou, YY Zhou, S AF Gao, Ji Zhang, Aiping Lam, Shu Kee Zhang, Xuesong Thomson, Allison M. Lin, Erda Jiang, Kejun Clarke, Leon E. Edmonds, James A. Kyle, Page G. Yu, Sha Zhou, Yuyu Zhou, Sheng TI An integrated assessment of the potential of agricultural and forestry residues for energy production in China SO GLOBAL CHANGE BIOLOGY BIOENERGY LA English DT Article DE bioenergy; carbon tax; carbon capture and storage; climate policy; integrated assessment; residue biomass ID ORGANIC-CARBON STOCKS; CO2 CONCENTRATIONS; PROJECTED CHANGES; RURAL CHINA; LAND-USE; BIOMASS; MITIGATION; BIOENERGY; SYSTEMS; STORAGE AB Biomass has been widely recognized as an important energy source with high potential to reduce greenhouse gas emissions while minimizing environmental pollution. In this study, we employ the Global Change Assessment Model to estimate the potential of agricultural and forestry residue biomass for energy production in China. Potential availability of residue biomass as an energy source was analyzed for the 21st century under different climate policy scenarios. Currently, the amount of total annual residue biomass, averaged over 2003-2007, is around 15519PJ in China, consisting of 10818PJ from agriculture residues (70%) and 4701PJ forestry residues (30%). We estimate that 12693PJ of the total biomass is available for energy production, with 66% derived from agricultural residue and 34% from forestry residue. Most of the available residue is from south central China (3347PJ), east China (2862PJ) and south-west China (2229PJ), which combined exceeds 66% of the total national biomass. Under the reference scenario without carbon tax, the potential availability of residue biomass for energy production is projected to be 3380PJ by 2050 and 4108PJ by 2095, respectively. When carbon tax is imposed, biomass availability increases substantially. For the CCS 450ppm scenario, availability of biomass increases to 9002PJ (2050) and 11524PJ (2095), respectively. For the 450ppm scenario without CCS, 9183 (2050) and 11150PJ (2095) residue biomass, respectively, is projected to be available. Moreover, the implementation of CCS will have a little impact on the supply of residue biomass after 2035. Our results suggest that residue biomass has the potential to be an important component in China's sustainable energy production portfolio. As a low carbon emission energy source, climate change policies that involve carbon tariff and CCS technology promote the use of residue biomass for energy production in a low carbon-constrained world. C1 [Gao, Ji; Zhang, Aiping; Lin, Erda] Chinese Acad Agr Sci, Inst Environm & Sustainable Dev Agr, Beijing 100081, Peoples R China. [Lam, Shu Kee] Univ Melbourne, Crop & Soil Sci Sect, Fac Vet & Agr Sci, Melbourne, Vic 3010, Australia. [Zhang, Xuesong; Clarke, Leon E.; Edmonds, James A.; Kyle, Page G.; Yu, Sha] Pacific Northwest Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Zhang, Xuesong; Clarke, Leon E.; Edmonds, James A.; Kyle, Page G.; Yu, Sha] Univ Maryland, College Pk, MD 20740 USA. [Zhang, Xuesong] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Thomson, Allison M.] Alliance Sustainable Agr, Field Market, 777 N Capitol St NE,Suite 803, Washington, DC 20002 USA. [Jiang, Kejun] ERI, Beijing 100038, Peoples R China. [Zhou, Yuyu] Iowa State Univ, Dept Geol & Atmospher Sci, Ames, IA 50011 USA. [Zhou, Sheng] Tsinghua Univ, Inst Energy Environm & Econ, Beijing 100084, Peoples R China. RP Lin, E (reprint author), Chinese Acad Agr Sci, Inst Environm & Sustainable Dev Agr, Beijing 100081, Peoples R China.; Jiang, KJ (reprint author), ERI, Beijing 100038, Peoples R China. EM lined@ami.ac.cn; kjiang@eri.org.cn OI Lam, Shu Kee/0000-0001-7943-5004 FU Ministry of Science and Technology of the People's Republic of China [2013BAD11B03, 2012CB955801]; National Natural Science Foundation of China [71373142] FX This work was supported by the Ministry of Science and Technology of the People's Republic of China (2013BAD11B03 and 2012CB955801) and the National Natural Science Foundation of China (71373142). NR 60 TC 0 Z9 0 U1 12 U2 21 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1757-1693 EI 1757-1707 J9 GCB BIOENERGY JI GCB Bioenergy PD SEP PY 2016 VL 8 IS 5 BP 880 EP 893 DI 10.1111/gcbb.12305 PG 14 WC Agronomy; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA DS6SR UT WOS:000380913500004 ER PT J AU Morris, GP Hu, ZB Grabowski, PP Borevitz, JO de Graaff, MA Miller, RM Jastrow, JD AF Morris, Geoffrey P. Hu, Zhenbin Grabowski, Paul P. Borevitz, Justin O. de Graaff, Marie-Anne Miller, R. Michael Jastrow, Julie D. TI Genotypic diversity effects on biomass production in native perennial bioenergy cropping systems SO GLOBAL CHANGE BIOLOGY BIOENERGY LA English DT Article DE big bluestem; biomass feedstock; cultivars; ecotype; fertilization; low-input high-diversity; polymorphism; switchgrass; tallgrass prairie; yield ID SWITCHGRASS PANICUM-VIRGATUM; BIG BLUESTEM; CELLULOSIC ETHANOL; PLANT COMMUNITY; US MIDWEST; REGISTRATION; GRASSLAND; FEEDSTOCK; MONOCULTURES; MANAGEMENT AB The perennial grass species that are being developed as biomass feedstock crops harbor extensive genotypic diversity, but the effects of this diversity on biomass production are not well understood. We investigated the effects of genotypic diversity in switchgrass (Panicum virgatum) and big bluestem (Andropogon gerardii) on perennial biomass cropping systems in two experiments conducted over 2008-2014 at a 5.4-ha fertile field site in northeastern Illinois, USA. We varied levels of switchgrass and big bluestem genotypic diversity using various local and nonlocal cultivars - under low or high species diversity, with or without nitrogen inputs - and quantified establishment, biomass yield, and biomass composition. In one experiment (agronomic trial'), we compared three switchgrass cultivars in monoculture to a switchgrass cultivar mixture and three different species mixtures, with or without N fertilization. In another experiment (diversity gradient'), we varied diversity levels in switchgrass and big bluestem (1, 2, 4, or 6 cultivars per plot), with one or two species per plot. In both experiments, cultivar mixtures produced yields equivalent to or greater than the best cultivars. In the agronomic trial, the three switchgrass mixture showed the highest production overall, though not significantly different than best cultivar monoculture. In the diversity gradient, genotypic mixtures had one-third higher biomass production than the average monoculture, and none of the monocultures were significantly higher yielding than the average mixture. Year-to-year variation in yields was lowest in the three-cultivar switchgrass mixtures and Cave-In-Rock (the southern Illinois cultivar) and also reduced in the mixture of switchgrass and big bluestem relative to the species monocultures. The effects of genotypic diversity on biomass composition were modest relative to the differences among species and genotypes. Our findings suggest that local genotypes can be included in biomass cropping systems without compromising yields and that genotypic mixtures could help provide high, stable yields of high-quality biomass feedstocks. C1 [Morris, Geoffrey P.; Hu, Zhenbin] Kansas State Univ, Dept Agron, Manhattan, KS 66506 USA. [Grabowski, Paul P.] USDA ARS Dairy Forage Res Ctr, Madison, WI 53706 USA. [Borevitz, Justin O.] Australian Natl Univ, Res Sch Biol, Acton, ACT 2601, Australia. [de Graaff, Marie-Anne] Boise State Univ, Dept Biol Sci, Boise, ID 83725 USA. [Miller, R. Michael; Jastrow, Julie D.] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Morris, GP (reprint author), Kansas State Univ, Dept Agron, Manhattan, KS 66506 USA. EM gpmorris@ksu.edu OI Morris, Geoffrey/0000-0002-3067-3359 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-06CH11357]; Argonne/UChicago Energy Initiative; USDA-NIFA [2010-03894]; USDA-AFRI [2012-67010-20069]; National Institutes of Health Training Grant [T32 GM007197] FX Funding for this research was provided by the US Department of Energy, Office of Science, Office of Biological and Environmental Research under contract DE-AC02-06CH11357 to Argonne National Laboratory (RMM and JDJ). Additional support was provided by the Argonne/UChicago Energy Initiative to RMM and JOB, USDA-NIFA grant 2010-03894 to RMM, and a USDA-AFRI grant 2012-67010-20069 to M-AG, JDJ, and GPM. PPG was partially supported by National Institutes of Health Training Grant T32 GM007197. We thank Timothy Vugteveen, Whitney Panneton, Nina Noah, Jeremy Lederhouse, Scott Hofmann, Susan Kirt Alterio, Kelly Moran Sturner, and Cheryl Martin for technical assistance, and two anonymous reviewers for helpful comments and suggestions. NR 77 TC 0 Z9 0 U1 11 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1757-1693 EI 1757-1707 J9 GCB BIOENERGY JI GCB Bioenergy PD SEP PY 2016 VL 8 IS 5 BP 1000 EP 1014 DI 10.1111/gcbb.12309 PG 15 WC Agronomy; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA DS6SR UT WOS:000380913500012 PM 27668013 ER PT J AU Ma, TH Li, CJ Lu, ZM AF Ma, Tuhua Li, Changjiang Lu, Zhiming TI Geographical environment determinism for discovery of mineral deposits SO JOURNAL OF GEOCHEMICAL EXPLORATION LA English DT Article DE Mineral resources; Spatial distribution; Geographic environments; Undiscovered deposit number; Exploration level; Power-law (fractal) model ID LAW; DISTRIBUTIONS AB The spatial distribution of metallic mineral deposits discovered in China during 1901 to 2007 shows that nearly 85% of the total 2906 metallic mineral deposits with the magnitude greater than medium-size are located on the southeastern side of the famous Heihe-Tengchong "geo-demographic demarcation line". This spatial pattern is consistent with the population distribution of China, indicating that the spatial distribution of discovered mineral deposits may be related to exploration level that is strongly restricted by the geographic environments. We found that the number of discovered deposits per unit area in explored regions increases with the exploration level, following a power-law model. From this model, if the geological, geochemical and geophysical exploration in the NW region of the geo-demographic demarcation line reaches the same level as that in the SE region of the line, about 2000 metallic mineral deposits with magnitudes greater than medium-size remain to be discovered in the NW region of China. (C) 2016 Elsevier B.V. All rights reserved. C1 [Ma, Tuhua; Li, Changjiang] Zhejiang Informat Ctr Land & Resources, Hangzhou 310007, Zhejiang, Peoples R China. [Lu, Zhiming] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87545 USA. RP Li, CJ (reprint author), Zhejiang Informat Ctr Land & Resources, Hangzhou 310007, Zhejiang, Peoples R China. EM zjigmr@mail.hz.zj.cn FU Special Fund from Zhejiang Provincial Government, China [98] FX This study was partially funded by the Special Fund from Zhejiang Provincial Government, China (zjcx. 2011 No. 98). We would like to thank the editor and two anonymous reviewers for their valuable comments and suggestions, which have improved the paper. NR 24 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-6742 EI 1879-1689 J9 J GEOCHEM EXPLOR JI J. Geochem. Explor. PD SEP PY 2016 VL 168 BP 163 EP 168 DI 10.1016/j.gexplo.2016.07.001 PG 6 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DT7DV UT WOS:000381648200013 ER PT J AU Tan, L Snead, LL Katoh, Y AF Tan, L. Snead, L. L. Katoh, Y. TI Development of new generation reduced activation ferritic-martensitic steels for advanced fusion reactors SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Precipitates; Strengthening; Toughness; ODS ferritic steel; Reduced activation ferritic-martensitic steels ID LOW-CYCLE FATIGUE; MECHANICAL-PROPERTIES; RAFM STEEL; PRECIPITATION BEHAVIOR; CREEP DEFORMATION; LAVES PHASE; MICROSTRUCTURE; STRENGTH; TUNGSTEN; IMPACT AB International development of reduced activation ferritic-martensitic (RAFM) steels has focused on 9 wt percentage Cr, which primarily contain M23C6 (M = Cr-rich) and small amounts of MX (M = Ta/V, X = C/N) precipitates, not adequate to maintain strength and creep resistance above similar to 500 degrees C. To enable applications at higher temperatures for better thermal efficiency of fusion reactors, computational alloy thermodynamics coupled with strength modeling have been employed to explore a new generation RAFM steels. The new alloys are designed to significantly increase the amount of MX nanoprecipitates, which are manufacturable through standard and scalable industrial steelmaking methods. Preliminary experimental results of the developed new alloys demonstrated noticeably increased amount of MX, favoring significantly improved strength, creep resistance, and Charpy impact toughness as compared to current RAFM steels. The strength and creep resistance were comparable or approaching to the lower bound of, but impact toughness was noticeably superior to 9-20Cr oxide dispersion-strengthened ferritic alloys. (C) 2016 Elsevier B.V. All rights reserved. C1 [Tan, L.; Katoh, Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Snead, L. L.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Tan, L (reprint author), One Bethel Valley Rd,POB 2008,MS-6136, Oak Ridge, TN 37831 USA. EM tanl@ornl.gov RI Tan, Lizhen/A-7886-2009 OI Tan, Lizhen/0000-0002-3418-2450 FU U.S. Department of Energy, Office of Science, Fusion Energy Sciences; U.S. Department of Energy, Office of Nuclear Energy, Nuclear Energy Enabling Technology FY Award; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was supported by the U.S. Department of Energy, Office of Science, Fusion Energy Sciences and Office of Nuclear Energy, Nuclear Energy Enabling Technology FY 2012 Award. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 49 TC 3 Z9 3 U1 11 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 42 EP 49 DI 10.1016/j.jnucmat.2016.05.037 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500006 ER PT J AU Koyanagi, T Katoh, Y Ozawa, K Shimoda, K Hinoki, T Snead, LL AF Koyanagi, Takaaki Katoh, Yutai Ozawa, Kazumi Shimoda, Kazuya Hinoki, Tatsuya Snead, Lance L. TI Neutron-irradiation creep of silicon carbide materials beyond the initial transient SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SIC/SIC COMPOSITES; SIC FIBERS; ELEVATED-TEMPERATURES; BEHAVIOR; GROWTH; STEELS; DPA AB Irradiation creep beyond the transient regime was investigated for various silicon carbide (SiC) materials. The materials examined included polycrystalline or monocrystalline high-purity SiC, nanopowder sintered SiC, highly crystalline and near-stoichiometric SiC fibers (including Hi-Nicalon Type S, Tyranno SA3, isotopically-controlled Sylramic and Sylramic-iBN fibers), and a Tyranno SA3 fiber-reinforced SiC matrix composite fabricated through a nano-infiltration transient eutectic phase process. Neutron irradiation experiments for bend stress relaxation tests were conducted at irradiation temperatures ranging from 430 to 1180 degrees C up to 30 dpa with initial bend stresses of up to similar to 1 GPa for the fibers and similar to 300 MPa for the other materials. Initial bend stress in the specimens continued to decrease from 1 to 30 dpa. Analysis revealed that (1) the stress exponent of irradiation creep above 1 dpa is approximately unity, (2) the stress normalized creep rate is similar to 1 x 10(-7) [dpa(-1) MPa-1] at 430-750 degrees C for the range of 1-30 dpa for most polycrystalline SiC materials, and (3) the effects on irradiation creep of initial micro-structures-such as grain boundary, crystal orientation, and secondary phases-increase with increasing irradiation temperature. (C) 2016 Elsevier B.V. All rights reserved. C1 [Koyanagi, Takaaki; Katoh, Yutai] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Ozawa, Kazumi] Japan Atom Energy Agcy, Aomori 0393212, Japan. [Shimoda, Kazuya; Hinoki, Tatsuya] Kyoto Univ, Inst Adv Energy, Kyoto 6110011, Japan. [Snead, Lance L.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Koyanagi, T (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, 1 Bethel Valley Rd,A-154 Bldg 4500S, Oak Ridge, TN 37831 USA. EM koyanagit@ornl.gov RI Koyanagi, Takaaki/D-9841-2017 OI Koyanagi, Takaaki/0000-0001-7272-4049 FU Office of Fusion Energy Sciences, U.S. Department of Energy [DE-C05-00OR22725]; UT-Battelle, LLC; US-Japan TITAN Collaboration on Fusion Blanket Technology and Materials; High Flux Isotope Reactor - Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the Office of Fusion Energy Sciences, U.S. Department of Energy, under contract DE-C05-00OR22725 with UT-Battelle, LLC, and the US-Japan TITAN Collaboration on Fusion Blanket Technology and Materials. Research was supported in part by the High Flux Isotope Reactor, which is sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy. The authors would like to gratefully acknowledge contributions to pre- and post-irradiation experiments from F. C. Montgomery, C. M. Silva, A. M. Williams, P. S. Tedder, C. Shih and M. R. McAlister at Oak Ridge National Laboratory, and M. Fukuda at Tohoku University. NR 34 TC 0 Z9 0 U1 6 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 97 EP 111 DI 10.1016/j.jnucmat.2016.06.006 PG 15 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500013 ER PT J AU Guo, XF Wu, D Xu, HW Burns, PC Navrotsky, A AF Guo, Xiaofeng Wu, Di Xu, Hongwu Burns, Peter C. Navrotsky, Alexandra TI Thermodynamic studies of studtite thermal decomposition pathways via amorphous intermediates UO3, U2O7, and UO4 SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE UO2; Studtite; Calorimetry; Enthalpy of formation; Nuclear fuel alteration ID HIGH-TEMPERATURE CALORIMETRY; NUCLEAR-FUEL; URANIUM PEROXIDE; URANYL PEROXIDE; METASTUDTITE; STABILITY; DISSOLUTION; DIRECTIONS; CORROSION; PROGRESS AB The thermal decomposition of studtite (UO2)O-2(H2O)(2)center dot 2H(2)O results in a series of intermediate X-ray amorphous materials with general composition UO3+x (x = 0, 0.5, 1). As an extension of a structural study on U2O7., this work provides detailed calorimetric data on these amorphous oxygen-rich materials since their energetics and thermal stability are unknown. These were characterized in situ by thermogravimetry, and mass spectrometry. Ex situ X-ray diffraction and infrared spectroscopy characterized their chemical bonding and local structures. This detailed characterization formed the basis for obtaining formation enthalpies by high temperature oxide melt solution calorimetry. The thermodynamic data demonstrate the metastability of the amorphous UO3+x materials, and explain their irreversible and spontaneous reactions to generate oxygen and form metaschoepite. Thus, formation of studtite in the nuclear fuel cycle, followed by heat treatment, can produce metastable amorphous UO3+x materials that pose the risk of significant O2 gas. Quantitative knowledge of the energy landscape of amorphous UO3+x was provided for stability analysis and assessment of conditions for decomposition. (C) 2016 Elsevier B.V. All rights reserved. C1 [Guo, Xiaofeng; Xu, Hongwu] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Wu, Di; Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Wu, Di; Navrotsky, Alexandra] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. [Wu, Di] Washington State Univ, Gene & Lina Voiland Sch Chem Engn & Bioengn, Pullman, WA 99163 USA. [Burns, Peter C.] Univ Notre Dame, Dept Civil & Environm Engn & Earth Sci, Notre Dame, IN 46556 USA. [Burns, Peter C.] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. RP Navrotsky, A (reprint author), Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA.; Navrotsky, A (reprint author), Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. EM anavrotsky@ucdavis.edu RI Wu, Di/A-3039-2014; OI Wu, Di/0000-0001-6879-321X; Xu, Hongwu/0000-0002-0793-6923 FU Materials Science of Actinides, an Energy Frontier Research Center - the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001089]; Seaborg postdoctoral fellowship from the Laboratory Directed Research and Development (LDRD) program, through the G. T. Seaborg Institute, of Los Alamos National Laboratory (LANL); DOE [DE-AC52-06NA25396] FX Calorimetric studies at UC Davis and data analysis were supported by the Materials Science of Actinides, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DESC0001089. X. G was supported by a Seaborg postdoctoral fellowship from the Laboratory Directed Research and Development (LDRD) program, through the G. T. Seaborg Institute, of Los Alamos National Laboratory (LANL), which is operated by Los Alamos National Security LLC, under DOE Contract DE-AC52-06NA25396. We thank Sabrina Labs and Dirk Bosbach for providing the initial studtite sample. NR 31 TC 3 Z9 3 U1 16 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 158 EP 163 DI 10.1016/j.jnucmat.2016.06.014 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500020 ER PT J AU Miao, YB Mo, K Yao, TK Lian, J Fortner, J Jamison, L Xu, RQ Yacout, AM AF Miao, Yinbin Mo, Kun Yao, Tiankai Lian, Jie Fortner, Jeffrey Jamison, Laura Xu, Ruqing Yacout, Abdellatif M. TI Correlation between crystallographic orientation and surface faceting in UO2 SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Uranium dioxide; Surface faceting; Morphology; Synchrotron diffraction; Scanning electron microscopy ID F/M ODS STEEL; VICINAL SURFACES; GAS-RELEASE; FUEL; SYNCHROTRON; ENERGY; NANOPARTICLES; LEED; FERRITE/MARTENSITE; MICROSTRUCTURE AB Here coordinated experimental efforts to quantitatively correlate crystallographic orientation and surface faceting features in UO2 are reported upon. A sintered polycrystalline UO2 sample was thermally etched to induce the formation of surface faceting features. Synchrotron Laue microdiffraction was used to obtain a precise crystallographic orientation map for the UO2 surface grains. Scanning electron microscopy (SEM) was utilized to collect the detailed information on the surface morphology of the sample. The surface faceting features were found to be highly dependent on the crystallographic orientation. In most cases, Triple-plane structures containing one {100} plane and two {111} planes were found to dominate the surface of UO2. The orientation-faceting relationship established in this study revealed a practical and efficient method of determining crystallographic orientation based on the surface features captured by SEM images. (C) 2016 Published by Elsevier B.V. C1 [Miao, Yinbin; Mo, Kun; Fortner, Jeffrey; Jamison, Laura; Xu, Ruqing; Yacout, Abdellatif M.] Argonne Natl Lab, Lemont, IL 60439 USA. [Yao, Tiankai; Lian, Jie] Rensselaer Polytech Inst, Troy, NY 12180 USA. RP Mo, K (reprint author), Argonne Natl Lab, Lemont, IL 60439 USA.; Lian, J (reprint author), Rensselaer Polytech Inst, Troy, NY 12180 USA. EM kunmo@anl.gov; lianj@rpi.edu OI Jamison, Laura/0000-0003-2759-6310; Miao, Yinbin/0000-0002-3128-4275 FU U.S. Department of Energy (DOE)'s Nuclear Energy Advanced Modeling and Simulation (NEAMS) program; U.S. DOE's Nuclear Energy University Program (NEUP) [DE-NE0008440]; DOE Office of Science by Argonne National Laboratory [DE-AC-02-06CH11357] FX This work was funded by the U.S. Department of Energy (DOE)'s Nuclear Energy Advanced Modeling and Simulation (NEAMS) program and the U.S. DOE's Nuclear Energy University Program (NEUP) DE-NE0008440. This research used resources of the Advanced Photon Source, a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC-02-06CH11357 between UChicago Argonne, LLC and the U.S. Department of Energy. NR 36 TC 1 Z9 1 U1 6 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 176 EP 184 DI 10.1016/j.jnucmat.2016.05.044 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500023 ER PT J AU Martinez, E Soisson, F Caro, A Uberuaga, BP AF Martinez, Enrique Soisson, Frederic Caro, Alfredo Uberuaga, Blas P. TI Atomistic modeling of the reordering process of gamma ' disordered particles in Ni-Al alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Segregation; Diffusion; Irradiation ID MONTE-CARLO-SIMULATION; MATERIAL INCONEL X-750; ION IRRADIATION; INTERMETALLIC COMPOUNDS; MOLECULAR-DYNAMICS; BEAM WINDOW; KINETICS; TEMPERATURE; DISSOLUTION; EVOLUTION AB Ni-based alloys are used in nuclear applications, including as a window material at isotope production facilities, withstanding high fluxes of different energetic particles like protons. Irradiation disorders the gamma' precipitates that in large extent confer the mechanical properties characterizing these materials. Upon disordering, the gamma' phase transforms into oversaturated gamma, degrading the materials properties. Experimentally it is observed that disordering might take place at fairly low irradiation doses. Once the particles are disordered, a competition between dissolution, due to strong concentration gradients in an oversaturated solid solution, and reordering appears. Here, we examine this competition in a model Ni-Al alloy under thermal conditions for different precipitates sizes and temperatures. We observe Al interdiffusion from the supersaturated particle to the matrix. Also, stochasticity appears as an important factor in to where precipitates locate. Stress relaxation seems to modify the precipitation process, with a stronger interface effect compared to rigid lattice simulations. (C) 2016 Elsevier B.V. All rights reserved. C1 [Martinez, Enrique; Caro, Alfredo; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, MST-8, Los Alamos, NM 87545 USA. [Soisson, Frederic] Univ Paris Saclay, CEA, DEN Serv Rech Met Phys, F-91191 Gif Sur Yvette, France. RP Martinez, E (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST-8, Los Alamos, NM 87545 USA. EM enriquem@lanl.gov OI Martinez Saez, Enrique/0000-0002-2690-2622 FU US Department of Energy (DOE) through the LANL/LDRD Program; U.S. DOE [DE-AC52-06NA25396] FX The authors gratefully acknowledge the support of the US Department of Energy (DOE) through the LANL/LDRD Program for this work. This research used resources provided by the LANL Institutional Computing Program. LANL, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. NR 33 TC 0 Z9 0 U1 6 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 207 EP 214 DI 10.1016/j.jnucmat.2016.06.019 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500026 ER PT J AU Fadzil, SM Hrma, P Schweiger, MJ Riley, BJ AF Fadzil, Syazwani Mohd Hrma, Pavel Schweiger, Michael J. Riley, Brian J. TI Component effects on crystallization of RE-containing aluminoborosilicate glass SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Lanthanide borosilicate glass; Pyroprocessing; Liquidus temperature; Crystalline phases ID LEVEL WASTE GLASS; LIQUIDUS TEMPERATURE; PYROCHEMICAL PROCESS AB Lanthanide-aluminoborosilicate (LABS) glass is one option for immobilizing rare earth (RE) oxide fission products generated during reprocessing of pyroprocessed fuel. This glass system can accommodate a high loading of RE oxides and has excellent chemical durability. The present study describes efforts to model equilibrium crystallinity as a function of glass composition and temperature as well as liquidus temperature (T-L) as a function of glass composition. The experimental method for determining T-L was ASTM C1720-11. Typically, three crystalline phases were formed in each glass: Ce-borosilicate (Ce3B-Si2O10), mullite (Al10Si2O19), and corundum (Al2O3). Cerianite (CeO2) was a common minor crystalline phase and Nd-silicate (Nd2Si2O7) occurred in some of the glasses. In the composition region studied, T-L decreased as SiO2 and B2O3 fractions increased and strongly increased with increasing fractions of RE oxides; Al2O3 had a moderate effect on the T-L but, as expected, it strongly affected the precipitation of Al-containing crystals. (C) 2016 Elsevier B.V. All rights reserved. C1 [Fadzil, Syazwani Mohd; Hrma, Pavel] Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang 790784, South Korea. [Fadzil, Syazwani Mohd] Natl Univ Malaysia, Fac Sci & Technol, Sch Appl Phys, Bandar Baru Bangi 43650, Selangor, Malaysia. [Hrma, Pavel; Schweiger, Michael J.; Riley, Brian J.] Pacific Northwest Natl Lab, POB 999, Richland, WA USA. RP Fadzil, SM (reprint author), Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang 790784, South Korea. EM syazwanimf@ukm.edu.my OI Riley, Brian/0000-0002-7745-6730 FU Department of Energy's Waste Treatment and Immobilization Plant Federal Project Office; U.S. Department of Energy [DE-AC05-76RL01830]; BK21 + program through National Research Foundation of Korea - Ministry of Education, Science and Technology FX The authors greatly appreciate B.R. Johnson and other staff members of Pacific Northwest National Laboratory (PNNL) with the financial support of the Department of Energy's Waste Treatment and Immobilization Plant Federal Project Office under the direction of A. A. Kruger. PNNL is operated by Battelle for the U.S. Department of Energy under Contract Number DE-AC05-76RL01830. This work was also supported by the BK21 + program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology. NR 28 TC 0 Z9 0 U1 4 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 261 EP 267 DI 10.1016/j.jnucmat.2016.06.018 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500033 ER PT J AU Kim, YS Jeong, GY Sohn, DS Jamison, LM AF Kim, Yeon Soo Jeong, G. Y. Sohn, D. -S. Jamison, L. M. TI Pore growth in U-Mo/Al dispersion fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE U-Mo/Al dispersion fuel; Pore growth; Porosity; In-pile data; Modeling ID IRRADIATION BEHAVIOR; PARTICLE DISPERSION; ENHANCED DIFFUSION; AL MATRIX; MO FUEL; PRODUCT; ENERGIES; TENSION; SURFACE; ALLOY AB U-Mo/Al dispersion fuel is currently under development in the DOE's Material Management and Minimization program to convert HEU-fueled research reactors to LEU-fueled reactors. In some demanding conditions in high-power and high-performance reactors, large pores form in the interaction layers between the U-Mo fuel particles and the Al matrix, which pose a potential to cause fuel failure. In this study, comprehension of the formation and growth of these pores was explored. As a product, a model to predict pore growth and porosity increase was developed. The model includes three major topics: fission gas release from the U-Mo and the IL to the pores, stress evolution in the fuel meat, and the effect of amorphous IL growth. Well-characterized in-pile data from reduced-size plates were used to fit the model parameters. A data set from full-sized plates, independent and distinctively different from those used to fit the model parameters, was used to examine the accuracy of the model. The model showed fair agreement with the measured data. The model suggested that the growth of the IL has a critical effect on pore growth, as both its material properties and energetics are favorable to pore formation. Therefore, one area of the current effort, focused on suppressing IL growth, appears to be on the right track to improve the performance of this fuel. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kim, Yeon Soo; Jamison, L. M.] Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA. [Jeong, G. Y.; Sohn, D. -S.] Ulsan Natl Inst Sci & Technol, 50 UNIST Gil, Ulsan 689798, South Korea. RP Kim, YS (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Argonne, IL 60439 USA. EM yskim@anl.gov OI Jeong, Gwan Yoon/0000-0002-3326-3718; Jamison, Laura/0000-0003-2759-6310 FU U.S. Department of Energy, National Nuclear Security Administration (NNSA), Office of Material Management and Minimization (NA-23) Reactor Conversion Program [DE-AC-02-06CH11357]; National Research Foundation of Korea (NRF) grant - Korean government (Ministry of Education, Science and Technology) [2011-0031771] FX This study used information gathered from three reduced-size plates from RERTR-4, -5, and -9 tests and two full-size plates from AFIP-1 test irradiated at the ATR. For the former three reduced-size plates, the authors acknowledge Drs. S. Hayes, D. Wachs and M. Meyer from INL and G. Hofman from ANL for the irradiation test designs, T. Wiencek from ANL and C. Clark from INL for the test plate fabrication, and late R. Strain from ANL and A. Robinson from INL for PIEs. For the latter full-size plates, Mr. A. Robinson and Dr. D. Wachs are recognized. The operations staff at the ATR is also acknowledged for these irradiation tests. The physics data available by Dr. G. Chang and Ms. M. Lillo are also appreciated. The authors wish to thank Drs. A. Leenaers and P. Lemoine for the FUTURE test PIE images available in the literature that were used to obtain data in Table 4. This work was supported by the U.S. Department of Energy, National Nuclear Security Administration (NNSA), Office of Material Management and Minimization (NA-23) Reactor Conversion Program under Contract No. DE-AC-02-06CH11357 between UChicago Argonne, LLC and the US Department of Energy, and in part by the National Research Foundation of Korea (NRF) grant funded by the Korean government (Ministry of Education, Science and Technology) under contract number 2011-0031771. NR 48 TC 0 Z9 0 U1 5 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 275 EP 286 DI 10.1016/j.jnucmat.2016.06.029 PG 12 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500035 ER PT J AU Imada, K Ishimaru, M Xue, HZ Zhang, YW Shannon, SC Weber, WJ AF Imada, Kenta Ishimaru, Manabu Xue, Haizhou Zhang, Yanwen Shannon, Steven C. Weber, William J. TI Amorphization resistance of nano-engineered SiC under heavy ion irradiation SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Nanostructured materials; Carbides; Amorphization; Scanning/transmission electron microscopy (STEM) ID NANOCRYSTALLINE SILICON-CARBIDE; RADIATION TOLERANCE; SICF/SIC COMPOSITES; NUCLEAR-WASTE; IMMOBILIZATION; SPECTROSCOPY; IMPLANTATION; TEMPERATURE; PLUTONIUM; DENSITY AB Silicon carbide (SiC) with a high-density of planar defects (hereafter, 'nano-engineered SiC') and epitaxially-grown single-crystalline 3C-SiC were simultaneously irradiated with Au ions at room temperature, in order to compare their relative resistance to radiation-induced amorphization. It was found that the local threshold dose for amorphization is comparable for both samples under 2 MeV Au ion irradiation; whereas, nano-engineered SiC exhibits slightly greater radiation tolerance than single crystalline SiC under 10 MeV Au irradiation. Under 10 MeV Au ion irradiation, the dose for amorphization increased by about a factor of two in both nano-engineered and single crystal SiC due to the local increase in electronic energy loss that enhanced dynamic recovery. (C) 2016 Elsevier B.V. All rights reserved. C1 [Imada, Kenta; Ishimaru, Manabu] Kyushu Inst Technol, Dept Mat Sci & Engn, Kitakyushu, Fukuoka 8048550, Japan. [Xue, Haizhou; Zhang, Yanwen; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Shannon, Steven C.] North Carolina State Univ, Dept Nucl Engn, Raleigh, NC 27695 USA. RP Ishimaru, M (reprint author), Kyushu Inst Technol, Dept Mat Sci & Engn, Kitakyushu, Fukuoka 8048550, Japan. EM ishimaru@post.matsc.kyutech.ac.jp RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU Kazuchika Okura Memorial Foundation; Ministry of Education, Sports, Science, and Technology, Japan [16H04518]; U.S. Department of Energy, Office of Sciences, Basic Energy Sciences, Materials Sciences and Engineering Division; Nuclear Energy University Programs FX This work was supported in part by the Kazuchika Okura Memorial Foundation, Grant-in-Aid for Scientific Research (B) (Grant No. 16H04518) from the Ministry of Education, Sports, Science, and Technology, Japan (MI), by the U.S. Department of Energy, Office of Sciences, Basic Energy Sciences, Materials Sciences and Engineering Division (YZ and WJW), and Nuclear Energy University Programs (HX and SS). MI appreciates Mr. Shinsuke Inoue (Kyushu Institute of Technology) for supporting SRIM calculations. NR 31 TC 0 Z9 0 U1 9 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 310 EP 314 DI 10.1016/j.jnucmat.2016.06.031 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500039 ER PT J AU Pizzocri, D Rabiti, C Luzzi, L Barani, T Van Uffelen, P Pastore, G AF Pizzocri, D. Rabiti, C. Luzzi, L. Barani, T. Van Uffelen, P. Pastore, G. TI PolyPole-1: An accurate numerical algorithm for intra-granular fission gas release SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Diffusion; Nuclear fuel modelling; Intra-granular fission gas release; Numerical algorithms; Modal methods; FORMAS; URGAS; PolyPole ID UO2 FUEL; SPHERICAL GRAINS; DIFFUSIVE FLOW; XE DIFFUSION; IRRADIATION; BEHAVIOR; PRECIPITATION; MIGRATION; BOUNDARY; BUBBLES AB The transport of fission gas from within the fuel grains to the grain boundaries (intra-granular fission gas release) is a fundamental controlling mechanism of fission gas release and gaseous swelling in nuclear fuel. Hence, accurate numerical solution of the corresponding mathematical problem needs to be included in fission gas behaviour models used in fuel performance codes. Under the assumption of equilibrium between trapping and resolution, the process can be described mathematically by a single diffusion equation for the gas atom concentration in a grain. In this paper, we propose a new numerical algorithm (PolyPole-1) to efficiently solve the fission gas diffusion equation in time-varying conditions. The PolyPole-1 algorithm is based on the analytic modal solution of the diffusion equation for constant conditions, combined with polynomial corrective terms that embody the information on the deviation from constant conditions. The new algorithm is verified by comparing the results to a finite difference solution over a large number of randomly generated operation histories. Furthermore, comparison to state-of-the-art algorithms used in fuel performance codes demonstrates that the accuracy of PolyPole-1 is superior to other algorithms, with similar computational effort. Finally, the concept of PolyPole-1 may be extended to the solution of the general problem of intra-granular fission gas diffusion during non-equilibrium trapping and resolution, which will be the subject of future work. Published by Elsevier B.V. C1 [Pizzocri, D.; Luzzi, L.; Barani, T.] Politecn Milan, Dept Energy, Nucl Engn Div, Via Masa 34, I-20156 Milan, Italy. [Rabiti, C.; Pastore, G.] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. [Van Uffelen, P.] European Commiss, Inst Transuranium Elements, Joint Res Ctr, POB 2340, D-76125 Karlsruhe, Germany. RP Pastore, G (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM giovanni.pastore@inl.gov OI Barani, Tommaso/0000-0002-6771-9461; Pastore, Giovanni/0000-0003-2812-506X; Luzzi, Lelio/0000-0002-9754-4535 FU DOE Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program at Idaho National Laboratory (INL, USA); GENTLE Project at Institute for Transuranium Elements (JRC- ITU, Germany) [198236]; Doctoral Program in "Energy and Nuclear Science and Technology" at Politecnico di Milano (POLIMI, Italy); U.S. Government [DE-AC07-05ID14517] FX This work was funded by the DOE Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program at Idaho National Laboratory (INL, USA), the GENTLE Project 198236 at Institute for Transuranium Elements (JRC- ITU, Germany), and the Doctoral Program in "Energy and Nuclear Science and Technology" at Politecnico di Milano (POLIMI, Italy).; The submitted manuscript has been authored by a contractor of the U.S. Government under Contract DE-AC07-05ID14517. Accordingly, the U.S. Government retains a non-exclusive, royalty free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 37 TC 0 Z9 0 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 333 EP 342 DI 10.1016/j.jnucmat.2016.06.028 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500042 ER PT J AU Burkes, DE Casella, AJ Casella, AM AF Burkes, Douglas E. Casella, Amanda J. Casella, Andrew M. TI Measurement of fission gas release from irradiated U-Mo dispersion fuel samples SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NUCLEAR-FUEL; PRODUCTS; ALLOYS AB The uranium-molybdenum (U-Mo) alloy dispersed in an Al-Si matrix has been proposed as one fuel design capable of converting some of the world's highest power research reactors from the use of high enriched uranium (HEU) to low enriched uranium (LEU). One aspect of the fuel development and qualification process is to demonstrate appropriate understanding of the extent of fission product release from the fuel under anticipated service environments. In this paper, two irradiated samples containing 53.9 vol% U-7wt% Mo fuel particles dispersed in an Al-2wt% Si matrix were subjected to specified thermal profiles under a controlled atmosphere using a thermogravimetric/ differential thermal analyzer coupled with a mass spectrometer inside a hot cell. Measurements revealed three distinct fission gas release events for the samples from 400 to 700 degrees C, as well as a number of minor fission gas releases below and above this temperature range. The mechanisms responsible for these events are discussed, and the results have been compared with available information in the literature with exceptional agreement. (C) 2016 Elsevier B.V. All rights reserved. C1 [Burkes, Douglas E.; Casella, Amanda J.; Casella, Andrew M.] Pacific Northwest Natl Lab, Nucl Engn & Anal Grp, POB 999,MSIN K8-34, Richland, WA 99352 USA. RP Burkes, DE (reprint author), Pacific Northwest Natl Lab, Nucl Engn & Anal Grp, POB 999,MSIN K8-34, Richland, WA 99352 USA. EM Douglas.Burkes@pnnl.gov FU National Nuclear Security Administration's Office of Material Management and Minimization Reactor Conversion Program [DE-AC05-76RL01830]; United States Government FX The authors would like to acknowledge Dr. Bruce McNamara for his review of the manuscript and helpful discussion. The authors would like to acknowledge Mr. Jason Schulthess, Mr. Adam Robinson, Dr. Barry Rabin, and Mrs. Susan Case from Idaho National Laboratory for the preparation and delivery of the irradiated fuel segment. Installation of equipment into hot cells and the operations conducted in hot cells is a large undertaking. The authors would like to acknowledge those at Pacific Northwest National Laboratory who were involved in the preparation of samples and performance of measurements, specifically Ms. Nicole Green, Mr. Jake Bohlke, Mr. Dustin Blundon, Dr. Edgar Buck, Mr. Eric Hanson, Mr. Kevin Heaton, Mr. Paul MacFarlan, Mr. Robert Orton, Mr. Bruce Slonecker, Ms. Franciska Steen, Mr. Randy Thornhill, and Mr. Patrick Valdez. Finally, the authors would like to acknowledge the sponsor, the National Nuclear Security Administration's Office of Material Management and Minimization Reactor Conversion Program, for the opportunity to conduct this work under contract DE-AC05-76RL01830.; This paper was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor Battelle Memorial Institute, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof, or Battelle Memorial Institute. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 29 TC 1 Z9 1 U1 3 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 365 EP 374 DI 10.1016/j.jnucmat.2016.05.039 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500044 ER PT J AU Piro, MHA Banfield, J Clarno, K Simunovic, S Besmann, TM Lewis, BJ Thompson, WT AF Piro, M. H. A. Banfield, J. Clarno, K. Simunovic, S. Besmann, T. M. Lewis, B. J. Thompson, W. T. TI Coupled thermochemical, isotopic evolution and heat transfer simulations in highly irradiated UO2 nuclear fuel (vol 441, pg 240, 2013) SO JOURNAL OF NUCLEAR MATERIALS LA English DT Correction C1 [Piro, M. H. A.; Besmann, T. M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. [Banfield, J.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Clarno, K.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN USA. [Simunovic, S.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN USA. [Lewis, B. J.; Thompson, W. T.] Royal Mil Coll Canada, Dept Chem & Chem Engn, Kingston, ON, Canada. [Piro, M. H. A.] Canadian Nucl Labs, Chalk River, ON, Canada. [Banfield, J.] Gen Elect Hitachi Nucl Energy, Wilmington, NC USA. [Besmann, T. M.] Univ South Carolina, Columbia, SC USA. RP Piro, MHA (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA.; Piro, MHA (reprint author), Canadian Nucl Labs, Chalk River, ON, Canada. EM markus.piro@cnl.ca NR 4 TC 0 Z9 0 U1 4 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD SEP PY 2016 VL 478 BP 375 EP 377 DI 10.1016/j.jnucmat.2016.06.030 PG 3 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DT7CM UT WOS:000381644500045 ER PT J AU Sanjeewa, LD McGuire, MA Pellizzeri, TMS McMillen, CD Garlea, VO Willett, D Chumanov, G Kolis, JW AF Sanjeewa, Liurukara D. McGuire, Michael A. Pellizzeri, Tiffany M. Smith McMillen, Colin D. Garlea, V. Ovidiu Willett, Daniel Chumanov, George Kolis, Joseph W. TI Synthesis and characterization of new fluoride-containing manganese vanadates A(2)Mn(2)V(2)O(7)F(2) (A=Rb, Cs) and Mn2VO4F SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article DE Hydrothermal; Vanadate; Manganese(II); Antiferromagnetism ID HYDROTHERMAL SYNTHESIS; CRYSTAL-STRUCTURE; MAGNETIC-PROPERTIES; METAL OXYFLUORIDE; BUILDING UNITS; GROUP MINERALS; FLUOROPHOSPHATE; CHEMISTRY; POLAR; LATTICES AB Large single crystals of A(2)Mn(2)V(2)O(7)F(2) (A =Rb, Cs) and Mn2VO4F were grown using a high-temperature (similar to 600 degrees C) hydrothermal technique. Single crystal X-ray diffraction and powder X-ray diffraction were utilized to characterize the structures, which both possess MnO4F2 building blocks. The A(2)Mn(2)V(2)O(7)F2 series crystallizes as a new structure type in space group Pbcn (No. 60), Z=4 (Rb(2)Mn(2)V(2)O(7)F2: a=7.4389 (17) angstrom, b=11.574(3) angstrom, c=10.914(2) angstrom; Cs2Mn2V2O7F2: a=7.5615(15) angstrom, b= 11.745(2) angstrom, c= 11.127(2) angstrom). The structure is composed of zigzag chains of edge-sharing MnO4F2 units running along the a-axis, and interconnected through V2O7 pyrovanadate groups. Temperature dependent magnetic susceptibility measurements on this interesting one-dimensional structural feature based on Mn2+ indicated that Cs2Mn2V2O7F2 is antiferromagnetic with a Neel temperature, T-N= similar to 3 K and a Weiss constant, theta, of -11.7 (1) K. Raman and infrared spectra were also analyzed to identify the fundamental V-O vibrational modes in Cs2Mn2V2O7F2. Mn-2(VO4)F crystalizes in the monoclinic space group of C2/c (no. 15), Z=8 with unit cell parameters of a=13.559(2) angstrom, b=6.8036(7) angstrom, c=10.1408(13) A and beta=116.16(3)degrees. The structure is associated with those of triplite and wagnerite. Dynamic fluorine disorder gives rise to complex alternating chains of five-and six-coordinate Mn2+. These interpenetrating chains are additionally connected through isolated VO4 tetrahedra to form the condensed structure. (C) 2016 Elsevier Inc. All rights reserved. C1 [Sanjeewa, Liurukara D.; Pellizzeri, Tiffany M. Smith; McMillen, Colin D.; Willett, Daniel; Chumanov, George; Kolis, Joseph W.] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Sanjeewa, Liurukara D.; Pellizzeri, Tiffany M. Smith; McMillen, Colin D.; Willett, Daniel; Chumanov, George; Kolis, Joseph W.] Clemson Univ, COMSET, Clemson, SC 29634 USA. [McGuire, Michael A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Garlea, V. Ovidiu] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Kolis, JW (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA.; Kolis, JW (reprint author), Clemson Univ, COMSET, Clemson, SC 29634 USA. EM kjoseph@clemson.edu RI McGuire, Michael/B-5453-2009 OI McGuire, Michael/0000-0003-1762-9406 FU National Science Foundation [DMR-1410727] FX The authors thank the National Science Foundation Grants #DMR-1410727 for financial support. NR 49 TC 1 Z9 1 U1 13 U2 19 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD SEP PY 2016 VL 241 BP 30 EP 37 DI 10.1016/j.jssc.2016.05.008 PG 8 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA DS4EJ UT WOS:000380733900005 ER PT J AU Heffernan, KM Ross, NL Spencer, EC Boatner, LA AF Heffernan, Karina M. Ross, Nancy L. Spencer, Elinor C. Boatner, Lynn A. TI The structural response of gadolinium phosphate to pressure SO JOURNAL OF SOLID STATE CHEMISTRY LA English DT Article ID MONAZITE; SPECTRA AB Accurate elastic constants for gadolinium phosphate (GdPO4) have been measured by single-crystal high-pressure diffraction methods. The bulk modulus of GdPO4 determined under hydrostatic conditions, 128.1(8) GPa (K'=5.8(2)), is markedly different from that obtained with GdPO4 under non-hydrostatic conditions (160(2) GPa), which indicates the importance of shear stresses on the elastic response of this phosphate. High pressure Raman and diffraction analysis indicate that the PO4 tetrahedra behave as rigid units in response to pressure and that contraction of the GdPO4 structure is facilitated by bending/ twisting of the Gd-O-P links that result in increased distortion in the GdO9 polyhedra. (C) 2016 Elsevier Inc. All rights reserved. C1 [Heffernan, Karina M.; Ross, Nancy L.; Spencer, Elinor C.] Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. [Boatner, Lynn A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Ross, NL (reprint author), Virginia Tech, Dept Geosci, Blacksburg, VA 24061 USA. EM nross@vt.edu FU National Science Foundation [EAR-1118691]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX N.L. R., K.M. H., and E.C. S. gratefully acknowledge support from the National Science Foundation (Grant No. EAR-1118691). K.M. H. and E.C. S. would also like to thank Drs. Carla Slebonick and Jing Zhou for their help and valuable insight on this project. Research at the Oak Ridge National Laboratory for one author (LAB) was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 19 TC 2 Z9 2 U1 7 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-4596 EI 1095-726X J9 J SOLID STATE CHEM JI J. Solid State Chem. PD SEP PY 2016 VL 241 BP 180 EP 186 DI 10.1016/j.jssc.2016.06.009 PG 7 WC Chemistry, Inorganic & Nuclear; Chemistry, Physical SC Chemistry GA DS4EJ UT WOS:000380733900025 ER PT J AU Tabackman, AA Frankson, R Marsan, ES Perry, K Cole, KE AF Tabackman, Alexa A. Frankson, Rochelle Marsan, Eric S. Perry, Kay Cole, Kathryn E. TI Structure of 'linkerless' hydroxamic acid inhibitor-HDAC8 complex confirms the formation of an isoform-specific subpocket SO JOURNAL OF STRUCTURAL BIOLOGY LA English DT Article DE Histone deacetylase 8; Histone deacetylase inhibitors (HDACi); Hydroxamic acids; AutoDock Vina ID HISTONE DEACETYLASE INHIBITORS; T-CELL LYMPHOMA; CRYSTAL-STRUCTURE; HUMAN HDAC8; DOCKING; CANCER; SUBSTRATE; SOFTWARE; BINDING; ROLES AB Histone deacetylases (HDACs) catalyze the hydrolysis of acetylated lysine side chains in histone and nonhistone proteins, and play a critical role in the regulation of many biological processes, including cell differentiation, proliferation, senescence, and apoptosis. Aberrant HDAC activity is associated with cancer, making these enzymes important targets for drug design. In general, HDAC inhibitors (HDACi) block the proliferation of tumor cells by inducing cell differentiation, cell cycle arrest, and/or apoptosis, and comprise some of the leading therapies in cancer treatments. To date, four HDACi have been FDA approved for the treatment of cancers: suberoylanilide hydroxamic acid (SAHA, Vorinostat, Zolinza(R)), romidepsin (FK228, Istodax(R)), belinostat (Beleodaq(R)), and panobinostat (Farydak(R)). Most current inhibitors are pan-HDACi, and non-selectively target a number of HDAC isoforms. Six previously reported HDACi were rationally designed, however, to target a unique sub-pocket found only in HDAC8. While these inhibitors were indeed potent against HDAC8, and even demonstrated specificity for HDAC8 over HDACs 1 and 6, there were no structural data to confirm the mode of binding. Here we report the X-ray crystal structure of Compound 6 complexed with HDAC8 to 1.98 angstrom resolution. We also describe the use of molecular docking studies to explore the binding interactions of the other 5 related HDACi. Our studies confirm that the HDACi induce the formation of and bind in the HDAC8-specific subpocket, offering insights into isoform-specific inhibition. (C) 2016 Elsevier Inc. All rights reserved. C1 [Tabackman, Alexa A.; Marsan, Eric S.; Cole, Kathryn E.] Christopher Newport Univ, Dept Mol Biol & Chem, 1 Ave Arts, Newport News, VA 23606 USA. [Frankson, Rochelle] Ithaca Coll, Dept Chem, 950 Danby Rd, Ithaca, NY 14850 USA. [Perry, Kay] Cornell Univ, Northeastern Collaborat Access Team NE CAT, Argonne Natl Lab, Bldg 436E,9700 South Cass Ave, Argonne, IL 60439 USA. [Perry, Kay] Cornell Univ, Dept Chem & Chem Biol, Argonne Natl Lab, Bldg 436E,9700 South Cass Ave, Argonne, IL 60439 USA. RP Cole, KE (reprint author), Christopher Newport Univ, Dept Mol Biol & Chem, 1 Ave Arts, Newport News, VA 23606 USA. EM kathryn.cole@cnu.edu FU National Institute of General Medical Sciences of the National Institutes of Health [P41 GM103403]; NIH-ORIP HEI grant [S10 RR029205]; US DOE [DE-AC02-06CH11357]; Ithaca College; Christopher Newport University FX This work is based upon research conducted at the Advanced Photon Source on the Northeastern Collaborative Access Team beamlines, which are supported by a grant from the National Institute of General Medical Sciences (P41 GM103403) of the National Institutes of Health. The Pilatus 6M detector on 24-ID-C beam line is funded by a NIH-ORIP HEI grant (S10 RR029205). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. KEC would like to thank Ithaca College and Christopher Newport University for funding. Undergraduate summer research was supported by the Dana Award (RF, Ithaca College) and the Summer Scholars Program (AT, Christopher Newport University). We would also like to thank Dr. Scott Ulrich for providing the inhibitors, and Dr. Daniel Dowling for helpful conversations. NR 31 TC 1 Z9 1 U1 8 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1047-8477 EI 1095-8657 J9 J STRUCT BIOL JI J. Struct. Biol. PD SEP PY 2016 VL 195 IS 3 BP 373 EP 378 DI 10.1016/j.jsb.2016.06.023 PG 6 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA DT8WZ UT WOS:000381777700012 PM 27374062 ER PT J AU DebRoy, S Hiraga, N Imamura, M Hayes, CN Akamatsu, S Canini, L Perelson, AS Pohl, RT Persiani, S Uprichard, SL Tateno, C Dahari, H Chayama, K AF DebRoy, S. Hiraga, N. Imamura, M. Hayes, C. N. Akamatsu, S. Canini, L. Perelson, A. S. Pohl, R. T. Persiani, S. Uprichard, S. L. Tateno, C. Dahari, H. Chayama, K. TI Hepatitis C virus dynamics and cellular gene expression in uPA-SCID chimeric mice with humanized livers during intravenous silibinin monotherapy SO JOURNAL OF VIRAL HEPATITIS LA English DT Article DE anti-inflammatory; chimeric mice with humanized livers; gene expression; uPA-SCID; viral kinetic modelling ID TRANSFERRIN RECEPTOR 1; SERUM AMYLOID-A; ANTIVIRAL ACTIVITY; PROTEASE-INHIBITOR; HCV KINETICS; IN-VITRO; INFECTION; SILYMARIN; THERAPY; SOFOSBUVIR AB Legalon SIL (SIL) is a chemically hydrophilized version of silibinin, an extract of milk thistle (Silybum marianum) seeds that has exhibited hepatoprotective and antiviral effectiveness against hepatitis C virus (HCV) in patients leading to viral clearance in combination with ribavirin. To elucidate the incompletely understood mode of action of SIL against HCV, mathematical modelling of HCV kinetics and human hepatocyte gene expression studies were performed in uPA-SCID-chimeric mice with humanized livers. Chronically HCV-infected mice (n = 15) were treated for 14 days with daily intravenous SIL at 469, 265 or 61.5 mg/kg. Serum HCV and human albumin (hAlb) were measured frequently, and liver HCV RNA was analysed at days 3 and 14. Microarray analysis of human hepatocyte gene expression was performed at days 0, 3 and 14 of treatment. While hAlb remained constant, a biphasic viral decline in serum was observed consisting of a rapid 1st phase followed by a second slower phase (or plateau with the two lower SIL dosings). SIL effectiveness in blocking viral production was similar among dosing groups (median epsilon = 77%). However, the rate of HCV-infected hepatocyte decline, , was dose-dependent. Intracellular HCV RNA levels correlated (r = 0.66, P = 0.01) with serum HCV RNA. Pathway analysis revealed increased anti-inflammatory and antiproliferative gene expression in human hepatocytes in SIL-treated mice. The results suggest that SIL could lead to a continuous second-phase viral decline, that is potentially viral clearance, in the absence of adaptive immune response along with increased anti-inflammatory and antiproliferative gene expression in human hepatocytes. C1 [DebRoy, S.; Canini, L.; Uprichard, S. L.; Dahari, H.] Loyola Univ, Med Ctr, Dept Med, Program Expt & Theoret Modeling,Div Hepatol, Maywood, IL 60153 USA. [DebRoy, S.] Univ South Carolina Beaufort, Dept Math & Computat Sci, Bluffton, SC USA. [Hiraga, N.; Imamura, M.; Hayes, C. N.; Akamatsu, S.; Chayama, K.] Hiroshima Univ, Inst Biomed & Hlth Sci, Dept Gastroenterol & Metab, Appl Life Sci, Hiroshima, Japan. [Canini, L.] Univ Edinburgh, Ctr Immun Infect & Evolut, Edinburgh, Midlothian, Scotland. [Perelson, A. S.] Los Alamos Natl Lab, Theoret Biol & Biophys, Los Alamos, NM USA. [Pohl, R. T.] German Assoc Phytotherapy, Speyer, Germany. [Persiani, S.] Rottapharm Biotech SRL, Monza, MB, Italy. [Tateno, C.] PhoenixBio Co Ltd, Higashihiroshima, Japan. RP Chayama, K (reprint author), Hiroshima Univ, Inst Biomed & Hlth Sci, Dept Gastroenterol & Metab, Minami Ku, 1-2-3 Kasumi, Hiroshima, Hiroshima 7348551, Japan. EM chayama@hiroshima-u.ac.jp FU PhoenixBio Co. Ltd.; NIH [P20-GM103452, R01-AI028433, R01-AI011095, R01-AI078881]; U.S. Department of Energy [DE-AC52-06NA25396]; USCB research grant award; UK Biotechnology and Biological Sciences Research Council [1698: BB/L001330/1]; Research Program on Hepatitis from the Japan Agency for Medical Research and Development, AMED [15fk0210001h0002] FX Portions of this work were supported by PhoenixBio Co. Ltd., NIH grants P20-GM103452, R01-AI028433, R01-AI011095 and R01-AI078881 and performed under the auspices of the U.S. Department of Energy under contract DE-AC52-06NA25396, USCB research grant award, and the UK Biotechnology and Biological Sciences Research Council - grant reference 1698: BB/L001330/1. SIL was provided by Rottapharm vertical bar Madaus Ltd. This research is partially supported by research funding from the Research Program on Hepatitis from the Japan Agency for Medical Research and Development, AMED (grant number: 15fk0210001h0002). NR 47 TC 0 Z9 0 U1 0 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1352-0504 EI 1365-2893 J9 J VIRAL HEPATITIS JI J. Viral Hepatitis PD SEP PY 2016 VL 23 IS 9 BP 708 EP 717 DI 10.1111/jvh.12551 PG 10 WC Gastroenterology & Hepatology; Infectious Diseases; Virology SC Gastroenterology & Hepatology; Infectious Diseases; Virology GA DS6NF UT WOS:000380898000006 PM 27272497 ER PT J AU Mondo, SJ Salvioli, A Bonfante, P Morton, JB Pawlowska, TE AF Mondo, Stephen J. Salvioli, Alessandra Bonfante, Paola Morton, Joseph B. Pawlowska, Teresa E. TI Nondegenerative Evolution in Ancient Heritable Bacterial Endosymbionts of Fungi SO MOLECULAR BIOLOGY AND EVOLUTION LA English DT Article DE diversifying selection; effective population size; evolution rate; genetic drift; Glomeribacter gigasporarum; mutation rate; purifying selection; vertical transmission ID NONSYNONYMOUS NUCLEOTIDE SUBSTITUTIONS; CANDIDATUS GLOMERIBACTER GIGASPORARUM; BAYESIAN PHYLOGENETIC INFERENCE; DELETERIOUS MUTATIONS; POPULATION-SIZE; MOLECULAR EVOLUTION; DNA POLYMORPHISM; DELETIONAL BIAS; GENETIC DRIFT; SELECTION AB Bacterial endosymbionts are critical to the existence of many eukaryotes. Among them, vertically transmitted endobacteria are uniquely typified by reduced genomes and molecular evolution rate acceleration relative to free-living taxa. These patterns are attributable to genetic drift-dominated degenerative processes associated with reproductive dependence on the host. The degenerative evolution scenario is well supported in endobacteria with strict vertical transmission, such as essential mutualists of insects. In contrast, heritable endosymbionts that are nonessential to their hosts and engage occasionally in horizontal transmission are expected to display deviations from the degenerative evolution model. To explore evolution patterns in such nonessential endobacteria, we focused on Candidatus Glomeribacter gigasporarum ancient heritable mutualists of fungi. Using a collection of genomes, we estimated in Glomeribacter mutation rate at 2.03 X 10(-9) substitutions per site per year and effective population size at 1.44 X 10(8). Both fall within the range of values observed in free-living bacteria. To assess the ability of Glomeribacter to purge slightly deleterious mutations, we examined genome-wide d(N)/ d(S) values and distribution patterns. We found that these dN/ dS profiles cluster Glomeribacter with free-living bacteria as well as with other nonessential endosymbionts, while distinguishing it from essential heritable mutualists of insects. Finally, our evolutionary simulations revealed that the molecular evolution rate acceleration in Glomeribacter is caused by limited recombination in a largely clonal population rather than by increased fixation of slightly deleterious mutations. Based on these patterns, we propose that genome evolution in Glomeribacter is nondegenerative and exemplifies a departure from the model of degenerative evolution in heritable endosymbionts. C1 [Mondo, Stephen J.; Pawlowska, Teresa E.] Cornell Univ, Sch Integrat Plant Sci Plant Pathol & Plant Micro, Ithaca, NY 14853 USA. [Salvioli, Alessandra; Bonfante, Paola] Univ Turin, Dept Life Sci & Syst Biol, Turin, Italy. [Morton, Joseph B.] West Virginia Univ, Div Plant & Soil Sci, Morgantown, WV 26506 USA. [Mondo, Stephen J.] US DOE Joint Genome Inst, Walnut Creek, CA USA. RP Pawlowska, TE (reprint author), Cornell Univ, Sch Integrat Plant Sci Plant Pathol & Plant Micro, Ithaca, NY 14853 USA. EM tep8@cornell.edu FU National Science Foundation [DEB-0918880, CSBR-1349308]; University of Torino FX We thank R. Hernandez for advice on SDF_CODE, E. Angert, O. Lastovetsky, J. Russell, G. Turgeon and two anonymous reviewers for helpful comments. This study was supported by the National Science Foundation grant DEB-0918880 to T.E.P. and CSBR-1349308 to J.B.M. as well as the 60% project from the University of Torino to P.B. NR 103 TC 0 Z9 0 U1 9 U2 14 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0737-4038 EI 1537-1719 J9 MOL BIOL EVOL JI Mol. Biol. Evol. PD SEP PY 2016 VL 33 IS 9 BP 2216 EP 2231 DI 10.1093/molbev/msw086 PG 16 WC Biochemistry & Molecular Biology; Evolutionary Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Evolutionary Biology; Genetics & Heredity GA DT7XU UT WOS:000381702500005 PM 27189571 ER PT J AU Adams, CJ Yu, JS Mao, JH Jen, KY Costes, SV Wade, M Shoemake, J Aina, OH Del Rosario, R Menchavez, PT Cardiff, RD Wahl, GM Balmain, A AF Adams, Cassandra J. Yu, Jennifer S. Mao, Jian-Hua Jen, Kuang-Yu Costes, Sylvain V. Wade, Mark Shoemake, Jocelyn Aina, Olulanu H. Del Rosario, Reyno Menchavez, Phuong Thuy Cardiff, Robert D. Wahl, Geoffrey M. Balmain, Allan TI The Trp53 delta proline (Trp53 Delta P) mouse exhibits increased genome instability and susceptibility to radiation-induced, but not spontaneous, tumor development SO MOLECULAR CARCINOGENESIS LA English DT Article DE Trp53; cancer radiation; genomic instability ID P53-DEFICIENT MICE; RICH REGION; DNA-DAMAGE; P53; SUPPRESSION; TUMORIGENESIS; APOPTOSIS; CANCER; DOMAIN; LYMPHOMAS AB The tumor suppressor TP53 can initiate a plethora of anti-proliferative effects to maintain genomic integrity under conditions of genotoxic stress. The N-terminal proline-rich domain (PRD) of TP53 is important in the regulation of TP53 activity and stability. A common polymorphism at codon 72 in this region has been associated with altered cancer risk in humans. The Trp53P mouse, which carries a germline homozygous deletion of a region of the PRD, does not develop spontaneous tumors in a mixed 129/Sv and C57BL/6 genetic background, but is highly susceptible to a broad range of tumor types following total body exposure to 4 Gy gamma () radiation. This contrasts with the tumor spectrum in Trp53 null (-/-) mice, which mainly develop thymic lymphomas and osteosarcomas. Analysis of genomic instability in tissues and cells from Trp53P mice demonstrated elevated basal levels of aneuploidy, but this is not sufficient to drive spontaneous tumorigenesis, which requires an additional DNA damage stimulus. Levels of genomic instability did not increase significantly in Trp53P mice following irradiation exposure, suggesting that other radiation effects including tissue inflammation, altered metabolism or autophagy, may play an important role. The Trp53P mouse is a novel model to dissect the mechanisms of tumor development induced by radiation exposure. (c) 2015 Wiley Periodicals, Inc. C1 [Adams, Cassandra J.; Del Rosario, Reyno; Menchavez, Phuong Thuy; Balmain, Allan] Univ Calif San Francisco, Helen Diller Family Comprehens Canc Ctr, 1450 3rd St, San Francisco, CA 94158 USA. [Yu, Jennifer S.; Shoemake, Jocelyn] Cleveland Clin, Dept Radiat Oncol, Dept Stem Cell Biol, Main Campus, Cleveland, OH 44106 USA. [Mao, Jian-Hua; Costes, Sylvain V.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA USA. [Jen, Kuang-Yu] Univ Calif San Francisco, Dept Pathol, San Francisco, CA 94140 USA. [Wade, Mark] Fdn Ist Italiano Tecnol IIT, Ctr Genom Sci IIT SEMM, Milan, Italy. [Aina, Olulanu H.; Cardiff, Robert D.] Univ Calif Davis, Dept Pathol & Lab Med, Primate Dr, CA USA. [Wahl, Geoffrey M.] Salk Inst Biol Studies, Gene Express Lab, 10010 N Torrey Pines Rd, La Jolla, CA 92037 USA. RP Balmain, A (reprint author), Univ Calif San Francisco, Helen Diller Family Comprehens Canc Ctr, 1450 3rd St, San Francisco, CA 94158 USA. FU NASA Specialized Center for Research in Radiation Health Effects [NNX09AM52G, UO1 CA84244, CA141455]; Department of Energy Low Dose Radiation Research Program [DESC0003679]; Leukemia and Lymphoma Society [5409-13] FX Grant sponsor: NASA Specialized Center for Research in Radiation Health Effects; Grant numbers: NNX09AM52G; UO1 CA84244; CA141455; Grant sponsor: The Department of Energy Low Dose Radiation Research Program; Grant number: DESC0003679; Grant sponsor: The Leukemia and Lymphoma Society Fellowship; Grant number: 5409-13 NR 35 TC 0 Z9 0 U1 3 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0899-1987 EI 1098-2744 J9 MOL CARCINOGEN JI Mol. Carcinog. PD SEP PY 2016 VL 55 IS 9 BP 1387 EP 1396 DI 10.1002/mc.22377 PG 10 WC Biochemistry & Molecular Biology; Oncology SC Biochemistry & Molecular Biology; Oncology GA DS6LU UT WOS:000380894100009 PM 26310697 ER PT J AU Li, H Yang, XR Weng, BS Su, JQ Nie, SA Gilbert, JA Zhu, YG AF Li, Hu Yang, Xiaoru Weng, Bosen Su, Jianqiang Nie, San'an Gilbert, Jack A. Zhu, Yong-Guan TI The phenological stage of rice growth determines anaerobic ammonium oxidation activity in rhizosphere soil SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE N loss; Anammox; Rhizosphere; Rice growth period; Root exudates; N-15-tracing ID METHANE-OXIDIZING BACTERIA; CANDIDATUS BROCADIA FULGIDA; CHINESE PADDY SOILS; ORYZA-SATIVA L.; ANAMMOX BACTERIA; ACTIVATED-SLUDGE; NITROGEN LOSS; DENITRIFICATION; DIVERSITY; COMMUNITY AB Anaerobic oxidation of ammonium (anammox) plays an important role in nitrogen (N) loss from agricultural systems. Recently, the rice rhizosphere was demonstrated to be a hotspot for anammox, yet the dynamics of anammox activity and the distribution of anammox bacteria in rhizosphere soil at different phenological stages of rice growth are still unknown. In this study, the activity, diversity and abundance of anammox bacteria in both rhizosphere and bulk soils were investigated over the entire rice growth season. From tillering to ripening stage, significantly higher anammox bacterial abundance was detected in rhizosphere soils compared to bulk soils. The rhizosphere soils also had significantly higher anammox rates at tillering and booting stages (0.71 and 0.32 nmol N g(-1) dry soil h(-1), respectively) compared to bulk soils. The anammox rate in rhizosphere soil was positively correlated to the concentrations of NOx- (total of nitrate and nitrite) and acetate. The abundance of anammox bacteria was significantly correlated with the concentration of succinate in rhizosphere soils. A total of five anammox genera of Brocadia, Kuenenia, Anammoxoglobus, Jettenia and Scalindua were detected, with Brocadia predominating in all examined samples. The distribution of anammox bacteria in rhizosphere and bulk soils varied with phenological stages. Statistical analysis indicated that C/N ratio, formate, citrate and ammonium were key factors influencing the composition of anammox bacteria. Variations in activity, abundance and distribution of anammox bacteria in rhizosphere were observed over the phenological progression, demonstrating that the root exudates might be influential for the anammox process. This study implies that future efforts in estimating the rate of anammox should consider the temporal variation during plant life cycles. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Li, Hu; Yang, Xiaoru; Weng, Bosen; Su, Jianqiang; Nie, San'an; Zhu, Yong-Guan] Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, Xiamen 361021, Peoples R China. [Zhu, Yong-Guan] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Urban & Reg Ecol, Beijing 100085, Peoples R China. [Gilbert, Jack A.] Univ Chicago, Dept Surg, Chicago, IL 60637 USA. [Gilbert, Jack A.] Argonne Natl Lab, Biosci Div, Lemont, IL 60439 USA. [Gilbert, Jack A.] Marine Biol Lab, Woods Hole, MA 02543 USA. RP Zhu, YG (reprint author), Chinese Acad Sci, Inst Urban Environm, Key Lab Urban Environm & Hlth, Xiamen 361021, Peoples R China. EM ygzhu@iue.ac.cn RI SPRP, XDB150200/N-7373-2016; Su, Jian Qiang/C-2388-2009; CAS, KLUEH/G-8978-2016; Zhu, Yong-Guan/A-1412-2009 OI Su, Jian Qiang/0000-0003-1875-249X; Zhu, Yong-Guan/0000-0003-3861-8482 FU Strategic Priority Research Program of Chinese Academy of Sciences [XDB15020302, XDB15020402]; Natural Science Foundation of China [41430858]; International Science & Technology Cooperation Program of China [2011DFB91710]; U.S. Dept. of Energy [DE-AC02-06CH11357] FX This study was financially supported by the Strategic Priority Research Program of Chinese Academy of Sciences (XDB15020302, XDB15020402), the Natural Science Foundation of China (41430858), and the International Science & Technology Cooperation Program of China (2011DFB91710). We thank Dr. Juan Wang for her help in rice cultivation and Dr. Han Zhang for assistance in the equipment of Isotope Ratio Mass Spectrometer. This work was supported in part by the U.S. Dept. of Energy under Contract DE-AC02-06CH11357. NR 49 TC 0 Z9 0 U1 34 U2 41 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD SEP PY 2016 VL 100 BP 59 EP 65 DI 10.1016/j.soilbio.2016.05.015 PG 7 WC Soil Science SC Agriculture GA DS2LD UT WOS:000380600100007 ER PT J AU Huh, U Cho, W Joy, DC AF Huh, U. Cho, W. Joy, D. C. TI Monte Carlo modeling of ion beam induced secondary electrons SO ULTRAMICROSCOPY LA English DT Article DE Monte Carlo; Secondary electron; Yield; Ion beam; Stopping power; Ion microscope ID MICROSCOPE; METROLOGY; EMISSION AB Ion induced secondary electrons (iSE) can produce high-resolution images ranging from a few eV to 100 keV over a wide range of materials. The interpretation of such images requires knowledge of the secondary electron yields (iSE 6) for each of the elements and materials present and as a function of the incident beam energy. Experimental data for helium ions are currently limited to 40 elements and six compounds while other ions are not well represented. To overcome this limitation, we propose a simple procedure based on the comprehensive work of Berger et al. Here we show that between the energy range of 10-100 keV the Berger et al. data for elements and compounds can be accurately represented by a single universal curve. The agreement between the limited experimental data that is available and the predictive model is good, and has been found to provide reliable yield data for a wide range of elements and compounds. (C) 2016 Elsevier B.V. All rights reserved. C1 [Huh, U.; Joy, D. C.] Univ Tennessee, Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Cho, W.] Univ Tennessee, Elect & Comp Engn, Knoxville, TN 37996 USA. [Joy, D. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Huh, U (reprint author), Univ Tennessee, Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. EM uhuh@vols.utk.edu FU DS [R011082032]; Center of Excellence [R011310039] FX This work was partially supported by DS Account number R011082032 and Center of Excellence Account number R011310039 for the Center for Materials Processing at the University of Tennessee, Knoxville. NR 32 TC 0 Z9 0 U1 2 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD SEP PY 2016 VL 168 BP 28 EP 33 DI 10.1016/j.ultramic.2016.05.010 PG 6 WC Microscopy SC Microscopy GA DS4MB UT WOS:000380754100004 PM 27337603 ER PT J AU Poudel, S Tokmina-Lukaszewska, M Colman, DR Refai, M Schut, GJ King, PW Maness, PC Adams, MWW Peters, JW Bothner, B Boyd, ES AF Poudel, Saroj Tokmina-Lukaszewska, Monika Colman, Daniel R. Refai, Mohammed Schut, Gerrit J. King, Paul W. Maness, Pin-Ching Adams, Michael W. W. Peters, John W. Bothner, Brian Boyd, Eric S. TI Unification of [FeFe]-hydrogenases into three structural and functional groups SO BIOCHIMICA ET BIOPHYSICA ACTA-GENERAL SUBJECTS LA English DT Article DE [FeFe]-hydrogenase; Hydrogen; Electron bifurcation; Post-translational modification; Regulation; Bioinformatics ID ALGA CHLAMYDOMONAS-REINHARDTII; SULFATE-REDUCING BACTERIA; THERMOTOGA-MARITIMA; MASS-SPECTROMETRY; IRON-HYDROGENASE; HISTIDINE-KINASE; ACTIVE-SITE; BIOCHEMICAL-CHARACTERIZATION; CLOSTRIDIUM-PASTEURIANUM; PROTEIN-PHOSPHORYLATION AB Background: [FeFe]-hydrogenases (Hyd) are structurally diverse enzymes that catalyze the reversible oxidation of hydrogen (H-2). Recent biochemical data demonstrate new functional roles for these enzymes, including those that function in electron bifurcation where an exergonic reaction is coupled with an endergonic reaction to drive the reversible oxidation/production of H-2. Methods: To identify the structural determinants that underpin differences in enzyme functionality, a total of 714 homologous sequences of the catalytic subunit, HydA, were compiled. Bioinformatics approaches informed by biochemical data were then used to characterize differences in inferred quaternary structure, HydA active site protein environment, accessory iron-sulfur clusters in HydA, and regulatory proteins encoded in HydA gene neighborhoods. Results: HydA homologs were clustered into one of three classification groups, Group 1 (G1), Group 2 (G2), and Group 3 (G3). G1 enzymes were predicted to be monomeric while those in G2 and G3 were predicted to be multimeric and include HydB, HydC (G2/G3) and HydD (G3) subunits. Variation in the HydA active site and accessory iron-sulfur clusters did not vary by group type. Group-specific regulatory genes were identified in the gene neighborhoods of both G2 and G3 Hyd. Analyses of purified G2 and G3 enzymes by mass spectrometry strongly suggest that they are post-translationally modified by phosphorylation. Conclusions: These results suggest that bifurcation capability is dictated primarily by the presence of both HydB and HydC in Hyd complexes, rather than by variation in HydA. General significance: This classification scheme provides a framework for future biochemical and mutagenesis studies to elucidate the functional role of Hyd enzymes. (C) 2016 Elsevier B.V. All rights reserved. C1 [Poudel, Saroj; Colman, Daniel R.; Boyd, Eric S.] Montana State Univ, Dept Microbiol & Immunol, POB 173520, Bozeman, MT 59717 USA. [Tokmina-Lukaszewska, Monika; Refai, Mohammed; Peters, John W.; Bothner, Brian] Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA. [Schut, Gerrit J.; Adams, Michael W. W.] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. [King, Paul W.; Maness, Pin-Ching] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. RP Boyd, ES (reprint author), Montana State Univ, Dept Microbiol & Immunol, POB 173520, Bozeman, MT 59717 USA. EM saroz189@gmail.com; tokminalukas@gmail.com; daniel.colman@montana.edu; refai1982@gmail.com; gerti@uga.edu; Paul.King@nrel.gov; PinChing.Maness@nrel.gov; adams@bmb.uga.edu; john.peters@chemistry.montana.edu; bbothner@montana.edu; eboyd@montana.edu RI King, Paul/D-9979-2011; OI King, Paul/0000-0001-5039-654X; Peters, John/0000-0001-9117-9568 FU Biological Electron Transfer and Catalysis Energy Frontier Research Center - U.S. Department of Energy, Office of Science, and Basic Energy Sciences [DE-SC0012518]; Murdock Charitable Trust; National Institute of Health of the Centers of Biomedical Research Excellence program [5P20RR02437] FX This work was supported as part of the Biological Electron Transfer and Catalysis Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Basic Energy Sciences under Award # DE-SC0012518. The mass spectrometry facility at Montana State University receives funding from the Murdock Charitable Trust and National Institute of Health 5P20RR02437 of the Centers of Biomedical Research Excellence program. NR 88 TC 2 Z9 2 U1 11 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-4165 EI 1872-8006 J9 BBA-GEN SUBJECTS JI Biochim. Biophys. Acta-Gen. Subj. PD SEP PY 2016 VL 1860 IS 9 BP 1910 EP 1921 DI 10.1016/j.bbagen.2016.05.034 PG 12 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA DS2LQ UT WOS:000380601400010 PM 27241847 ER PT J AU Fraga, MB Delplanque, JP Yang, N Lavernia, EJ Monson, TC AF Fraga, Martin B. Delplanque, Jean-Pierre Yang, Nancy Lavernia, Enrique J. Monson, Todd C. TI High pressure FAST of nanocrystalline barium titanate SO CERAMICS INTERNATIONAL LA English DT Article DE Barium titanate; Sintering; Grain size; Spark plasma sintering ID ABNORMAL GRAIN-GROWTH; DIELECTRIC-PROPERTIES; BATIO3 CERAMICS; COMPUTER-SIMULATION; SIZE; FERROELECTRICS; DENSIFICATION; BEHAVIOR; CONSOLIDATION; ATMOSPHERE AB This work studies the microstructural evolution of nanocrystalline (< 1 mu m) barium titanate (BaTiO3), and presents high pressure in field-assisted sintering (FAST) as a robust methodology to obtain > 100 nm BaTiO3 compacts. Using FAST, two commercial similar to 50 nm powders were consolidated into compacts of varying densities and grain sizes. Microstructural inhomogeneities were investigated for each case, and an interpretation is developed using a modified Monte Carlo Potts (MCP) simulation. Two recurrent microstructural inhomogeneities are highlighted, heterogeneous grain growth and low-density regions, both ubiqutously present in all samples to varying degrees. In the worst cases, HGG presents an area coverage of 52%. Because HGG is sporadic but homogenous throughout a sample, the catalyst (e.g., the local segregation of species) must be, correspondingly, distributed in a homogenous manner. MCP demonstrates that in such a case, a large distance between nucleating abnormal grains is required otherwise abnormal grains prematurely impinge on each other, and their size is not distinguishable from that of normal grains. Compacts sintered with a pressure of 300 MPa and temperatures of 900 degrees C, were 99.5% dense and had a grain size of 90 +/- 24 nm. These are unprecedented results for commercial BaTiO3 powders or any starting powder of 50 nm particle size other authors have used 16 nm lab-produced powder to obtain similar results. (C) 2016 Elsevier Ltd and Techna Group S.r.l. All rights reserved. C1 [Fraga, Martin B.; Delplanque, Jean-Pierre] Univ Calif Davis, Davis, CA 95616 USA. [Yang, Nancy] Sandia Natl Labs, Livermore, CA USA. [Lavernia, Enrique J.] Univ Calif Irvine, Irvine, CA USA. [Monson, Todd C.] Sandia Natl Labs, Albuquerque, NM USA. RP Fraga, MB (reprint author), Univ Calif Davis, Davis, CA 95616 USA. EM mbfraga@ucdavis.edu OI Monson, Todd/0000-0002-9782-7084; Delplanque, Jean-Pierre/0000-0003-1774-1641 FU Air Force Research Laboratory/High Power Microwave Electromagnetic Microwave Division; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge the support of Sandia National Laboratories. The authors also wish to thank Dr. Susan Heidger of the Air Force Research Laboratory/High Power Microwave Electromagnetic Microwave Division for additional support of this work. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of the Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract no. DE-AC04-94AL85000. NR 50 TC 1 Z9 1 U1 17 U2 27 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0272-8842 EI 1873-3956 J9 CERAM INT JI Ceram. Int. PD SEP PY 2016 VL 42 IS 12 BP 13868 EP 13875 DI 10.1016/j.ceramint.2016.05.193 PG 8 WC Materials Science, Ceramics SC Materials Science GA DR7LT UT WOS:000380081900068 ER PT J AU Lin, F Leyffer, S Munson, T AF Lin, Fu Leyffer, Sven Munson, Todd TI A two-level approach to large mixed-integer programs with application to cogeneration in energy-efficient buildings SO COMPUTATIONAL OPTIMIZATION AND APPLICATIONS LA English DT Article DE Coarsened models; Distributed generation; Large-scale problems; Two-level approach; Multi-period planning; Resource and cost allocation; Two-stage mixed-integer programs ID DISTRIBUTED GENERATION SYSTEMS; NONLINEAR OPTIMIZATION; LAGRANGIAN-RELAXATION; SIMULATION PROGRAM; COLUMN GENERATION; LINEAR-PROGRAMS; OPTIMAL-DESIGN; BILEVEL; AGGREGATION; BOUNDS AB We study a two-stage mixed-integer linear program (MILP) with more than 1 million binary variables in the second stage. We develop a two-level approach by constructing a semi-coarse model that coarsens with respect to variables and a coarse model that coarsens with respect to both variables and constraints. We coarsen binary variables by selecting a small number of prespecified on/off profiles. We aggregate constraints by partitioning them into groups and taking convex combination over each group. With an appropriate choice of coarsened profiles, the semi-coarse model is guaranteed to find a feasible solution of the original problem and hence provides an upper bound on the optimal solution. We show that solving a sequence of coarse models converges to the same upper bound with proven finite steps. This is achieved by adding violated constraints to coarse models until all constraints in the semi-coarse model are satisfied. We demonstrate the effectiveness of our approach in cogeneration for buildings. The coarsened models allow us to obtain good approximate solutions at a fraction of the time required by solving the original problem. Extensive numerical experiments show that the two-level approach scales to large problems that are beyond the capacity of state-of-the-art commercial MILP solvers. C1 [Lin, Fu; Leyffer, Sven; Munson, Todd] Argonne Natl Lab, Math & Comp Sci Div, 9700 South Cass Ave, Lemont, IL 60439 USA. RP Lin, F (reprint author), Argonne Natl Lab, Math & Comp Sci Div, 9700 South Cass Ave, Lemont, IL 60439 USA. EM fulin@mcs.anl.gov; leyffer@mcs.anl.gov; tmunson@mcs.anl.gov FU U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program under contract number DE-AC02-06CH11357. We thank the reviewers for their helpful comments. Fu Lin thanks Dr. Ralph Muehleisen for useful discussions on EnergyPlus. NR 40 TC 0 Z9 0 U1 9 U2 9 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0926-6003 EI 1573-2894 J9 COMPUT OPTIM APPL JI Comput. Optim. Appl. PD SEP PY 2016 VL 65 IS 1 BP 1 EP 46 DI 10.1007/s10589-016-9842-0 PG 46 WC Operations Research & Management Science; Mathematics, Applied SC Operations Research & Management Science; Mathematics GA DS0CF UT WOS:000380262200001 ER PT J AU Zhang, N Hu, ZG Springer, C Li, YN Shen, B AF Zhang, Ning Hu, Zhaoguang Springer, Cecilia Li, Yanning Shen, Bo TI A bi-level integrated generation-transmission planning model incorporating the impacts of demand response by operation simulation SO ENERGY CONVERSION AND MANAGEMENT LA English DT Article DE Unit commitment; Generation-transmission expansion planning; Bi-level planning model; Demand response; Peak load reduction ID POWER-GENERATION; ELECTRICITY MARKETS; UNIT COMMITMENT; SYSTEMS; COORDINATION; RESOURCE; OPTIMIZATION AB If all the resources in power supply side, transmission part, and power demand side are considered together, the optimal expansion scheme from the perspective of the whole system can be achieved. In this paper, generation expansion planning and transmission expansion planning are combined into one model. Moreover, the effects of demand response in reducing peak load are taken into account in the planning model, which can cut back the generation expansion capacity and transmission expansion capacity. Existing approaches to considering demand response for planning tend to overestimate the impacts of demand response on peak load reduction. These approaches usually focus on power reduction at the moment of peak load without considering the situations in which load demand at another moment may unexpectedly become the new peak load due to demand response. These situations are analyzed in this paper. Accordingly, a novel approach to incorporating demand response in a planning model is proposed. A modified unit commitment model with demand response is utilized. The planning model is thereby a bi-level model with interactions between generation-transmission expansion planning and operation simulation to reflect the actual effects of demand response and find the reasonably optimal planning result. (C) 2016 Elsevier Ltd. All rights, reserved. C1 [Zhang, Ning] Beijing Jiaotong Univ, Sch Elect Engn, Beijing 100044, Peoples R China. [Zhang, Ning; Hu, Zhaoguang] State Grid Corp China, State Grid Energy Res Inst, Beijing 102200, Peoples R China. [Springer, Cecilia; Shen, Bo] Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, Berkeley, CA 94720 USA. [Springer, Cecilia] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Li, Yanning] Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China. RP Zhang, N (reprint author), Beijing Jiaotong Univ, Sch Elect Engn, Beijing 100044, Peoples R China. EM 12121580@bjtu.edu.cn NR 44 TC 1 Z9 1 U1 5 U2 5 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0196-8904 EI 1879-2227 J9 ENERG CONVERS MANAGE JI Energy Conv. Manag. PD SEP 1 PY 2016 VL 123 BP 84 EP 94 DI 10.1016/j.enconman.2016.06.020 PG 11 WC Thermodynamics; Energy & Fuels; Mechanics SC Thermodynamics; Energy & Fuels; Mechanics GA DS2LP UT WOS:000380601300008 ER PT J AU Jay, DA Borde, AB Diefenderfer, HL AF Jay, David A. Borde, Amy B. Diefenderfer, Heida L. TI Tidal-Fluvial and Estuarine Processes in the Lower Columbia River: II. Water Level Models, Floodplain Wetland Inundation, and System Zones SO ESTUARIES AND COASTS LA English DT Article DE Environmental flows; Estuarine processes; Hydropower impacts; Non-stationary tides; Sum exceedance value; Tidal freshwater; Tidal river zonation; Tides; Wetlands; Water levels ID PLANT-SPECIES RICHNESS; HARMONIC-ANALYSIS; CLIMATE INFLUENCES; SALMONID HABITAT; LAWRENCE-RIVER; SALT MARSHES; FRESH-WATER; FLOW; VEGETATION; GRADIENTS AB Spatially varying water-level regimes are a factor controlling estuarine and tidal-fluvial wetland vegetation patterns. As described in Part I, water levels in the Lower Columbia River and estuary (LCRE) are influenced by tides, river flow, hydropower operations, and coastal processes. In Part II, regression models based on tidal theory are used to quantify the role of these processes in determining water levels in the mainstem river and floodplain wetlands, and to provide 21-year inundation hindcasts. Analyses are conducted at 19 LCRE mainstem channel stations and 23 tidally exposed floodplain wetland stations. Sum exceedance values (SEVs) are used to compare wetland hydrologic regimes at different locations on the river floodplain. A new predictive tool is introduced and validated, the potential SEV (pSEV), which can reduce the need for extensive new data collection in wetland restoration planning. Models of water levels and inundation frequency distinguish four zones encompassing eight reaches. The system zones are the wave- and current-dominated Entrance to river kilometer (rkm) 5; the Estuary (rkm-5 to 87), comprised of a lower reach with salinity, the energy minimum (where the turbidity maximum normally occurs), and an upper estuary reach without salinity; the Tidal River (rkm-87 to 229), with lower, middle, and upper reaches in which river flow becomes increasingly dominant over tides in determining water levels; and the steep and weakly tidal Cascade (rkm-229 to 234) immediately downstream from Bonneville Dam. The same zonation is seen in the water levels of floodplain stations, with considerable modification of tidal properties. The system zones and reaches defined here reflect geological features and their boundaries are congruent with five wetland vegetation zones. C1 [Jay, David A.] Portland State Univ, Dept Civil & Environm Engn, POB 751, Portland, OR 97207 USA. [Borde, Amy B.; Diefenderfer, Heida L.] Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. RP Jay, DA (reprint author), Portland State Univ, Dept Civil & Environm Engn, POB 751, Portland, OR 97207 USA. EM djay@cecs.pdx.edu; amy.borde@pnnl.gov; heida.diefenderfer@pnnl.gov FU US Army Corps of Engineers Columbia River Fish Mitigation Program; PNNL by the Bonneville Power Administration; Lower Columbia Estuary Partnership; National Science Foundation [OCE-0929055] FX This work was supported by the US Army Corps of Engineers Columbia River Fish Mitigation Program. Funding for flood-plain water-level data collection by PNNL was also provided in part by the Bonneville Power Administration and Lower Columbia Estuary Partnership. Partial support for D. A. Jay was provided by the National Science Foundation, grant OCE-0929055. We thank V. Cullinan, R. Kaufmann, K. Leffler, C. McNeil, and S. Zimmerman for technical assistance. NR 80 TC 2 Z9 2 U1 12 U2 19 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1559-2723 EI 1559-2731 J9 ESTUAR COAST JI Estuaries Coasts PD SEP PY 2016 VL 39 IS 5 BP 1299 EP 1324 DI 10.1007/s12237-016-0082-4 PG 26 WC Environmental Sciences; Marine & Freshwater Biology SC Environmental Sciences & Ecology; Marine & Freshwater Biology GA DS0EO UT WOS:000380268400001 ER PT J AU Nyhan, M Sobolevsky, S Kang, CG Robinson, P Corti, A Szell, M Streets, D Lu, ZF Britter, R Barrett, SRH Ratti, C AF Nyhan, Marguerite Sobolevsky, Stanislav Kang, Chaogui Robinson, Prudence Corti, Andrea Szell, Michael Streets, David Lu, Zifeng Britter, Rex Barrett, Steven R. H. Ratti, Carlo TI Predicting vehicular emissions in high spatial resolution using pervasively measured transportation data and microscopic emission's model SO ATMOSPHERIC ENVIRONMENT LA English DT Article DE Air quality; Transportation; Emissions; Microscopic emissions model; Microscopic vehicle movement ID AIR-POLLUTION; LOS-ANGELES; VEHICLE; MORTALITY; CITIES; VARIABILITY; REDUCTION; EVOLUTION; NETWORKS; QUALITY AB Air pollution related to traffic emissions pose an especially significant problem in cities; this is due to its adverse impact on human health and well-being. Previous studies which have aimed to quantify emissions from the transportation sector have been limited by either simulated or coarsely resolved traffic volume data. Emissions inventories form the basis of urban pollution models, therefore in this study, Global Positioning System (GPS) trajectory data from a taxi fleet of over 15,000 vehicles were analyzed with the aim of predicting air pollution emissions for Singapore. This novel approach enabled the quantification of instantaneous drive cycle parameters in high spatio-temporal resolution, which provided the basis for a microscopic emissions model. Carbon dioxide (CO2), nitrogen oxides (NOx), volatile organic compounds (VOCs) and particulate matter (PM) emissions were thus estimated. Highly localized areas of elevated emissions levels were identified, with a spatio-temporal precision not possible with previously used methods for estimating emissions. Relatively higher emissions areas were mainly concentrated in a few districts that were the Singapore Downtown Core area, to the north of the central urban region and to the east of it. Daily emissions quantified for the total motor vehicle population of Singapore were found to be comparable to another emissions dataset Results demonstrated that high resolution spatio-temporal vehicle traces detected using GPS in large taxi fleets could be used to infer highly localized areas of elevated acceleration and air pollution emissions in cities, and may become a complement to traditional emission estimates, especially in emerging cities and countries where reliable fine-grained urban air quality data is not easily available. This is the first study of its kind to investigate measured microscopic vehicle movement in tandem with microscopic emissions modeling for a substantial study domain. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Nyhan, Marguerite; Robinson, Prudence; Britter, Rex; Ratti, Carlo] MIT, SENSEable City Lab, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Sobolevsky, Stanislav] NYU, Ctr Urban Sci & Progress, New York, NY USA. [Kang, Chaogui] Wuhan Univ, Wuhan, Hubei, Peoples R China. [Corti, Andrea] Politecn Milan, 32 Piazza Leonardo da Vinci, Milan, Italy. [Szell, Michael] Northeastern Univ, Dept Phys, Ctr Complex Network Res, Boston, MA 02115 USA. [Streets, David; Lu, Zifeng] NASA, Argonne Natl Lab, Lemont, IL USA. [Barrett, Steven R. H.] MIT, Dept Aeronaut & Astronaut, Cambridge, MA 02139 USA. RP Nyhan, M (reprint author), MIT, SENSEable City Lab, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM mnyhan@mit.edu OI Kang, Chaogui/0000-0002-0122-9419 FU MIT SENSEable City Lab Consortium; Singapore-MIT Alliance for Research & Technology program FX All the authors wish to thank the MIT SENSEable City Lab Consortium and the Singapore-MIT Alliance for Research & Technology program for supporting the research. M. Nyhan would like to thank Fulbright and the Irish Environmental Protection Agency. The authors would also like to acknowledge Dr. Luc Int. Panis for providing advice on some modeling aspects of the study. NR 68 TC 1 Z9 1 U1 30 U2 43 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1352-2310 EI 1873-2844 J9 ATMOS ENVIRON JI Atmos. Environ. PD SEP PY 2016 VL 140 BP 352 EP 363 DI 10.1016/j.atmosenv.2016.06.018 PG 12 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DR7MG UT WOS:000380083200031 ER PT J AU Kupwade-Patil, K Diallo, SO Hossain, DZ Islam, MR Allouche, EN AF Kupwade-Patil, Kunal Diallo, Souleymane O. Hossain, Dewan Zayid Islam, Md Rashedul Allouche, Erez N. TI Investigation of activation kinetics in geopolymer paste using quasielastic neutron scattering SO CONSTRUCTION AND BUILDING MATERIALS LA English DT Article DE Fly ash; Quasielastic neutron scattering (QENS); Geopolymer; Characterization; Gelation; Dissolution ID CALCIUM SILICATE HYDRATE; PORTLAND-CEMENT PASTES; TRICALCIUM SILICATE; FLY-ASH; TRANSLATIONAL DYNAMICS; GEL FORMATION; WATER; MICROSTRUCTURE; EVOLUTION; STATE AB Quasielastic neutron scattering (QENS) has been used to investigate the binding process of water molecules in pastes of calcium geopolymer prepared with low and high calcium fly ash contents, and at two different NaOH molarities, 10 and 14 M. The in situ measurements were carried at ambient and elevated curing temperatures (60 degrees C). By carefully monitoring the time evolution of the elastic peak intensity, we infer a gelation process, followed by polymerization and a hardening in the high calcium geopolymer paste at 60 degrees C, in agreement with previously proposed geopolymerization model. This behavior was neither observed at ambient temperature in both low and high calcium geopolymer cement paste, within the precision of the neutron instrument. Our study clearly shows that a minimal amount of heat is necessary to form gelation and polymerization during the activation process. The activation of geopolymer paste with high NaOH molarity involves more chemically bound water molecules than that at lower activator concentration. This work shows that the QENS technique can be effectively used to characterize the alkali-activation kinetics in certain geopolymer pastes, and that temperature and molarity of the activator play a vital role in controlling the gel mechanism. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Kupwade-Patil, Kunal; Hossain, Dewan Zayid; Islam, Md Rashedul; Allouche, Erez N.] Louisiana Tech Univ, Dept Civil Engn, ACBL, Ruston, LA 71272 USA. [Diallo, Souleymane O.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN USA. RP Kupwade-Patil, K (reprint author), MIT, Dept Civil & Environm Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM kunalk@mit.edu FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; DOE-EPSCoR Grant [DE-FG02-08ER46528] FX This research at ORNL's Spallation Neutron Source (SNS) was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Travel to Oak Ridge National Laboratory to carry out this work was supported by a Travel Fellowship, from, the DOE-EPSCoR Grant to the University of Tennessee, DE-FG02-08ER46528. This study was conducted when the first author of the paper was at Louisiana Tech University. We would like to thank Dr. Eugene Mamontov from Oak Ridge National Laboratory for fruitful discussions during the course of these experiments. The authors are also thankful to Dr. Claire White from Princeton University for reviewing the initial version of this manuscript and for her feedback. NR 44 TC 1 Z9 1 U1 3 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0950-0618 EI 1879-0526 J9 CONSTR BUILD MATER JI Constr. Build. Mater. PD SEP 1 PY 2016 VL 120 BP 181 EP 188 DI 10.1016/j.conbuildmat.2016.05.104 PG 8 WC Construction & Building Technology; Engineering, Civil; Materials Science, Multidisciplinary SC Construction & Building Technology; Engineering; Materials Science GA DR7MP UT WOS:000380084100020 ER PT J AU Ramezani, H Wang, Y Yablonovitch, E Zhang, X AF Ramezani, Hamidreza Wang, Yuan Yablonovitch, Eli Zhang, Xiang TI Unidirectional Perfect Absorber SO IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS LA English DT Article DE critical coupling; exceptional point; metrology; Parity time symmetry; perfect absorber; spectral singularity; unidirectional perfect absorber ID PARITY-TIME SYMMETRY; EXCEPTIONAL POINT; ABSORPTION; LASER AB We show an interplay between Fano resonances and a judicious absorption mechanism leads to a unidirectional perfect absorber, which can be controlled in both direction and frequency. Critical coupling phenomenon created by interference, separates the left-and right-side of the system. At the same time, Fano resonance causes a divergence in the delay time of photons traveling through the loss part of the system, which results in full absorption of the photons from one side. Moreover, we depict that coincidence of the two unidirectional perfect absorber modes from opposite directions results in a perfect absorber mode, which is distinct from the CPA modes. Furthermore, we show that the unidirectional perfect absorber mode is at the same time a spectral singularity and an exceptional point, which makes this point ultrasensitive to any changes in the system. Our results open a direction for designing new type of absorbers, sensors, and switches. C1 [Ramezani, Hamidreza; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, Natl Sci Fdn, Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA. [Yablonovitch, Eli] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Yablonovitch, Eli] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhang, X (reprint author), Univ Calif Berkeley, Natl Sci Fdn, Nanoscale Sci & Engn Ctr, Berkeley, CA 94720 USA.; Zhang, X (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM ramezani@berkeley.edu; yuanwang@berkeley.edu; eliy@eecs.berkeley.edu; xiang@berkeley.edu RI Wang, Yuan/F-7211-2011 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05-CH11231]; U.S. Air Force Office of Scientific Research (AFOSR) MURI program [FA9550-12-1-0024] FX This work was primarily funded by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231. Calculation of the mode sensitivity was supported by U.S. Air Force Office of Scientific Research (AFOSR) MURI program (No. FA9550-12-1-0024). (Corresponding author: Xiang Zhang.) NR 43 TC 0 Z9 0 U1 15 U2 29 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1077-260X EI 1558-4542 J9 IEEE J SEL TOP QUANT JI IEEE J. Sel. Top. Quantum Electron. PD SEP-OCT PY 2016 VL 22 IS 5 DI 10.1109/JSTQE.2016.2545644 PG 6 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA DR5DW UT WOS:000379924200001 ER PT J AU Li, WT Ren, XT Huang, YW Yu, ZH Mi, ZY Tamura, N Li, XD Peng, F Wang, L AF Li, Wentao Ren, Xiangting Huang, Yanwei Yu, Zhenhai Mi, Zhongying Tamura, Nobumichi Li, Xiaodong Peng, Fang Wang, Lin TI Phase transformation and fluorescent enhancement of ErF3 at high pressure SO SOLID STATE COMMUNICATIONS LA English DT Article DE Rare-earth trifluorides; Structure and fluorescence; Phase transitions and enhancement of fluorescence; High pressure ID LAF3; TRANSITION; STRAIN; NANOPARTICLES; CRYSTALS; LASER; IONS AB Pressure-induced phase transformation and fluorescent properties of ErF3 were investigated here using in-situ synchrotron X-ray diffraction and photoluminescence up to 32.1 GPa at room temperature. Results showed that ErF3 underwent a reversible pressure-induced phase transition from the beta-YF3-type to the fluocerite LaF3-type at 9.8 GPa. The bulk moduli B-0 for low- and high-pressure phases were determined to be 130 and 208 GPa, respectively. Photoluminescencent studies showed that new emission lines belonging to the transition of H-2(11/2) -> I-4(15/2), S-4(3/2) -> I-4(15/2), and F-4(9/2) -> I-4(15/2) appeared during phase transition, suggesting pressure-induced electronic band splitting. Remarkably, significant pressure-induced enhancement of photoluminescence was observed, which was attributed to lattice distortion of the material under high pressure. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Li, Wentao; Peng, Fang] Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China. [Li, Wentao; Ren, Xiangting; Huang, Yanwei; Yu, Zhenhai; Mi, Zhongying; Wang, Lin] Ctr High Pressure Sci & Technol Adv Res HPSTAR, Shanghai 201203, Peoples R China. [Tamura, Nobumichi] Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. [Li, Xiaodong] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Wang, Lin] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Wang, Lin] Carnegie Inst Sci, High Pressure Synerget Consortium, Geophys Lab, Argonne, IL 60439 USA. RP Peng, F (reprint author), Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China.; Wang, L (reprint author), Ctr High Pressure Sci & Technol Adv Res HPSTAR, Shanghai 201203, Peoples R China. EM pengfang@scu.edu.cn; wanglin@hpstar.ac.cn FU National Natural Science Foundation of China, China Chinese Academy of Sciences Fund [U1332104]; NSAF [U1530402]; Chinese Academy of Sciences [KJCX2-SW-N03, KJCX2-SW-N20] FX This work was supported by the joint fund of the National Natural Science Foundation of China, China Chinese Academy of Sciences Fund (Grant no. U1332104) and NSAF (Grant no. U1530402). The high pressure XRD experiments were carried out at beamline 4W2 of the Beijing Synchrotron Radiation Facility (BSRF), which is supported by the Chinese Academy of Sciences (Grant no. KJCX2-SW-N03, KJCX2-SW-N20). NR 32 TC 0 Z9 0 U1 6 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 EI 1879-2766 J9 SOLID STATE COMMUN JI Solid State Commun. PD SEP PY 2016 VL 242 BP 30 EP 35 DI 10.1016/j.ssc.2016.05.014 PG 6 WC Physics, Condensed Matter SC Physics GA DR1UI UT WOS:000379690000007 ER PT J AU Brown, CS Zhang, HB AF Brown, C. S. Zhang, Hongbin TI Uncertainty quantification and sensitivity analysis with CASL Core Simulator VERA-CS SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE CASL; VERA-CS; Uncertainty quantification; Sensitivity analysis AB VERA-CS (Virtual Environment for Reactor Applications, Core Simulator) is a coupled neutron transport and thermal-hydraulics code under development by the Conscirtium for Advanced Simulation of Light Water Reactors (CASL). An approach to uncertainty quantification and sensitivity analysis with VERA-CS was developed and a new toolkit was created to perform uncertainty quantification and sensitivity analysis. A 2 x 2 fuel assembly model was developed and Simulated by VERA-CS, and uncertainty quantification and Sensitivity analysis were performed with fourteen uncertain. input parameters. The minimum departure from nucleate boiling ratio (MDNBR), maximum fuel center-line temperature, and maximum outer clad surface temperature were chosen as the selected figures of merit. Pearson, Spearman, and partial correlation coefficients were considered for all of the figures of merit in sensitivity analysis and coolant inlet temperature was consistently the most influential parameter. Parameters used as inputs to the critical heat flux calculation with the W-3 correlation were shown to be the most influential on the MDNBR, maximum fuel center-line temperature, and maximum outer clad surface temperature. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Brown, C. S.] North Carolina State Univ, Dept Nucl Engn, 2500 Stinson Dr, Raleigh, NC 27695 USA. [Zhang, Hongbin] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. RP Zhang, HB (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM csbrown3@ncsu.edu; Hongbin.Zhang@inl.gov FU Office of Nuclear Energy of the U.S. Department of Energy [DE-AC07-05ID14517]; U.S. Department of Energy [DE-AC07-05ID14517] FX This research made use of the resources of the High Performance Computing Center at Idaho National Laboratory, which is supported by the Office of Nuclear Energy of the U.S. Department of Energy under Contract No. DE-AC07-05ID14517. The authors would like to thank Andrew Godfrey and Mark Baird at ORNL as well as Vefa Kucukboyaci and Yixing Sung at Westinghouse for their assistance with VERA-CS. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 18 TC 1 Z9 1 U1 2 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD SEP PY 2016 VL 95 BP 188 EP 201 DI 10.1016/j.anucene.2016.05.016 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DQ7EG UT WOS:000379369100021 ER PT J AU Bhagia, S Nunez, A Wyman, CE Kumar, R AF Bhagia, Samarthya Nunez, Angelica Wyman, Charles E. Kumar, Rajeev TI Robustness of two-step acid hydrolysis procedure for composition analysis of poplar SO BIORESOURCE TECHNOLOGY LA English DT Article DE Compositional analysis; Lignocellulosic biomass; Poplar; Sulfuric acid hydrolysis; Lignin-carbohydrate complex AB The NREL standard procedure for lignocellulosic biomass composition has two steps: primary hydrolysis in 72% wt sulfuric acid at 30 degrees C for 1 h followed by secondary hydrolysis of the slurry in 4 wt% acid at 121 degrees C for 1 h. Although pointed out in the NREL procedure, the impact of particle size on composition has never been shown. In addition, the effects of primary hydrolysis time and separation of solids prior to secondary hydrolysis on composition have never been shown. Using poplar, it was found that particle sizes less than 0.250 mm significantly lowered the glucan content and increased the Klason lignin but did not affect xylan, acetate, or acid soluble lignin contents. Composition was unaffected for primary hydrolysis time between 30 and 90 min. Moreover, separating solids prior to secondary hydrolysis had negligible effect on composition suggesting that lignin and polysaccharides are completely separated in the primary hydrolysis stage. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Bhagia, Samarthya; Nunez, Angelica; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, 900 Univ Ave, Riverside, CA 92521 USA. [Bhagia, Samarthya; Nunez, Angelica; Wyman, Charles E.; Kumar, Rajeev] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol, 1084 Columbia Ave, Riverside, CA 92507 USA. [Bhagia, Samarthya; Wyman, Charles E.; Kumar, Rajeev] Oak Ridge Natl Lab, BESC, POB 2008 MS6341, Oak Ridge, TN 37831 USA. RP Wyman, CE (reprint author), Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol, 1084 Columbia Ave, Riverside, CA 92507 USA.; Wyman, CE (reprint author), Univ Calif Riverside, Dept Chem & Environm Engn, Bourns Coll Engn, 1084 Columbia Ave, Riverside, CA 92507 USA. EM cewyman@engr.ucr.edu FU Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BioEnergy Science Center (BESC) at Oak Ridge National Laboratory [DE-PS02-06ER64304]; UCR Hispanic Serving Institutions (HSI) Undergraduate Research Program through the U. S. Department of Education; Ford Motor Company FX This work was supported by the Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BioEnergy Science Center (BESC) at Oak Ridge National Laboratory (Contract DE-PS02-06ER64304). Stipend for undergraduate research was awarded by UCR Hispanic Serving Institutions (HSI) Undergraduate Research Program through the U. S. Department of Education. We thank Daniel Lee, Department of Chemical and Environmental Engineering at UCR for assistance in milling of poplar used in this study. We also acknowledge the Center for Environmental Research and Technology (CE-CERT) of the Bourns College of Engineering for providing the facilities and the Ford Motor Company for funding the Chair in Environmental Engineering that facilitates projects such as this one. NR 8 TC 2 Z9 2 U1 10 U2 21 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD SEP PY 2016 VL 216 BP 1077 EP 1082 DI 10.1016/j.biortech.2016.04.138 PG 6 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA DQ9UX UT WOS:000379555900133 PM 27282557 ER PT J AU Elrick-Barr, CE Smith, TF Preston, BL Thomsen, DC Baum, S AF Elrick-Barr, Carmen E. Smith, Timothy F. Preston, Benjamin L. Thomsen, Dana C. Baum, Scott TI How are coastal households responding to climate change? SO ENVIRONMENTAL SCIENCE & POLICY LA English DT Article DE Vulnerability; Resilience; Risk; Decision-making; Environmental hazards ID BUILDING ADAPTIVE CAPACITY; CHANGE ADAPTATION; RISK; RESPONSIBILITIES; AUSTRALIA; BEHAVIOR; VULNERABILITY; PERCEPTIONS; RESILIENCE; GOVERNANCE AB In Australia, shared responsibility is a concept advocated to promote collective climate change adaptation by multiple actors and institutions. However, a shared response is often promoted in the absence of information regarding actions currently taken; in particular, there is limited knowledge regarding action occurring at the household scale. To address this gap, we examine household actions taken to address climate change and associated hazards in two Australian coastal communities. Mixed methods research is conducted to answer three questions: (1) what actions are currently taken (mitigation, actions to lobby for change or adaptation to climate impacts)? (2) why are these actions taken (e.g. are they consistent with capacity, experience, perceptions of risk); and (3) what are the implications for adaptation? We find that households are predominantly mitigating greenhouse gas emissions and that impact orientated adaptive actions are limited. Coping strategies are considered sufficient to mange climate risks, proving a disincentive for additional adaptive action. Influencing factors differ, but generally, risk perception and climate change belief are associated with action. However, the likelihood of more action is a function of homeownership and a tendency to plan ahead. Addressing factors that support or constrain household adaptive decision-making and action, from the physical (e.g. homeownership) to.the social (e.g. skills in planning and a culture of adapting to change) will be critical in increasing household participation in adaptation. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Elrick-Barr, Carmen E.; Smith, Timothy F.; Thomsen, Dana C.] Univ Sunshine Coast, Sustainabil Res Ctr, 90 Sippy Downs Dr, Sippy Downs, Qld 4556, Australia. [Preston, Benjamin L.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Baum, Scott] Griffith Univ, Griffith Sch Environm, Nathan Campus,170 Kessels Rd, Nathan, Qld 4111, Australia. RP Elrick-Barr, CE (reprint author), Univ Sunshine Coast, Sustainabil Res Ctr, 90 Sippy Downs Dr, Sippy Downs, Qld 4556, Australia. EM celrick@usc.edu.au; tsmith5@usc.edu.au; prestonbl@ornl.gov; dthomsen@usc.edu.au; s.baum@griffith.edu.au OI Preston, Benjamin/0000-0002-7966-2386 FU Australian Research Council (ARC) through the project Community Vulnerability and Extreme Events: Development of a Typology of Coastal Settlement Vulnerability to Aid Adaptation Strategies' [DP1093583]; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was supported by the Australian Research Council (ARC) through the project Community Vulnerability and Extreme Events: Development of a Typology of Coastal Settlement Vulnerability to Aid Adaptation Strategies' (DP1093583). This manuscript has been authored in part by UTBattelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 78 TC 0 Z9 0 U1 13 U2 27 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1462-9011 EI 1873-6416 J9 ENVIRON SCI POLICY JI Environ. Sci. Policy PD SEP PY 2016 VL 63 BP 177 EP 186 DI 10.1016/j.envsci.2016.05.013 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA DR0ZJ UT WOS:000379635300019 ER PT J AU Blankenship, D Dobson, P Garg, S Ghassemi, A Kohl, T AF Blankenship, Douglas Dobson, Patrick Garg, Sabodh Ghassemi, Ahmad Kohl, Thomas TI SPECIAL ISSUE: Enhanced Geothermal Systems: State of the Art Preface SO GEOTHERMICS LA English DT Editorial Material C1 [Blankenship, Douglas] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Dobson, Patrick] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Garg, Sabodh] Leidos Inc, San Diego, CA 92121 USA. [Ghassemi, Ahmad] Univ Oklahoma, Norman, OK 73019 USA. [Kohl, Thomas] Karlsruhe Inst Technol, D-76021 Karlsruhe, Germany. RP Garg, S (reprint author), Leidos Inc, San Diego, CA 92121 USA. EM gargs@leidos.com RI Dobson, Patrick/D-8771-2015; Kohl, Thomas/M-5704-2013 OI Dobson, Patrick/0000-0001-5031-8592; NR 0 TC 0 Z9 0 U1 15 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD SEP PY 2016 VL 63 SI SI BP 1 EP 1 DI 10.1016/j.geothermics.2016.04.001 PG 1 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR0XT UT WOS:000379630900001 ER PT J AU Kelkar, S WoldeGabriel, G Rehfeldt, K AF Kelkar, Sharad WoldeGabriel, Giday Rehfeldt, Kenneth TI Lessons learned from the pioneering hot dry rock project at Fenton Hill, USA SO GEOTHERMICS LA English DT Article DE EGS; HDR; Fenton Hill; Stimulation; Field test ID HYDRAULIC FRACTURING EXPERIMENTS; GEOTHERMAL-ENERGY; NEW-MEXICO; CRYSTALLINE ROCK; VALLES CALDERA; STRESS; RESERVOIRS; EXTRACTION; SYSTEMS; FLOW AB Interest in geothermal energy production has grown rapidly in recentyears due to the increasing demand for clean, renewable, domestic energy. Recent publications have suggested that geothermal energy from Enhanced Geothermal Systems could satisfy a large portion of the energy needs in the U.S. if the technology were implemented on a large scale. Pertinent to this goal are many of the lessons learned from the pioneering Hot Dry Rock project aimed at producing usable energy form the heat of the earth, conducted from 1970 to 1995 at Fenton Hill, New Mexico, USA. During this project, the Los Alamos National Laboratory created and tested two reservoirs at depths in the range of 2.8-3.5 km in crystalline rock formations underlying the Fenton Hill site. Thermal energies in the range of 3-10 MWt were produced demonstrating the technical feasibility of the concept. Many important lessons were learned regarding the creation, engineering and operation of such subsurface systems these lessons will prove valuable as the geothermal community moves towards the goal of realizing the immense potential of this ubiquitous renewable energy resource. The purpose of this paper is to provide a brief, easy to read overview of this pioneering project. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Kelkar, Sharad; WoldeGabriel, Giday] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Rehfeldt, Kenneth] Navarro Res & Engn, Oak Ridge, TN USA. [Rehfeldt, Kenneth] Los Alamos Natl Lab, Los Alamos, NM USA. RP Kelkar, S (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. EM Kelkar@lanl.gov FU U.S. Department of Energy- Geothermal Technologies Program Office [DE-AC52-06NA25396] FX This work was supported in part by the U.S. Department of Energy- Geothermal Technologies Program Office under contract No.DE-AC52-06NA25396. The authors gratefully acknowledge many useful and knowledgeable discussions with Don Brown and Dave Duchane, who are retired members of the HDR staff. We acknowledge Don Brown further for a critical review of the manuscript. NR 73 TC 2 Z9 2 U1 7 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD SEP PY 2016 VL 63 SI SI BP 5 EP 14 DI 10.1016/j.geothermics.2015.08.008 PG 10 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR0XT UT WOS:000379630900003 ER PT J AU Garcia, J Hartline, C Walters, M Wright, M Rutqvist, J Dobson, PF Jeanne, P AF Garcia, Julio Hartline, Craig Walters, Mark Wright, Melinda Rutqvist, Jonny Dobson, Patrick F. Jeanne, Pierre TI The Northwest Geysers EGS Demonstration Project, California Part 1: Characterization and reservoir response to injection SO GEOTHERMICS LA English DT Article DE Enhanced Geothermal Systems; The Geysers; Induced seismicity; Reservoir stimulation; Shear zones ID MAGMATIC-HYDROTHERMAL SYSTEM; GEOTHERMAL-RESERVOIRS; FLUID INCLUSION; FIELD AB An Enhanced Geothermal System (EGS) Demonstration Project is currently underway in the Northwest Geysers. The project goal is to demonstrate the feasibility of stimulating a deep high-temperature reservoir (HTR) (up to 400 degrees C, 750 degrees F). Two previously abandoned wells, Prati State 31 (PS-31) and Prati 32 (P-32), were reopened and deepened to be used as an injection and production doublet to stimulate the HTR. The deepened portions of both wells have conductive temperature gradients of 10 degrees F/100 ft (182 degrees C/km), produce connate native fluids and magmatic gas, and the rocks were isotopically unexchanged by meteoric water. The ambient temperature meteoric water injected into these hot dry rocks has evidently created a permeability volume of several cubic kilometers as determined by seismic monitoring. Preliminary isotopic analyses of the injected and produced water indicate that 50-75% of the steam from the created EGS reservoir is injection-derived. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Garcia, Julio; Hartline, Craig; Walters, Mark; Wright, Melinda] Calpine Corp, Middletown, CA 95461 USA. [Rutqvist, Jonny; Dobson, Patrick F.; Jeanne, Pierre] LBNL, Berkeley, CA 94720 USA. RP Garcia, J (reprint author), Calpine Corp, Middletown, CA 95461 USA. EM julio.garcia@calpine.com RI Rutqvist, Jonny/F-4957-2015; Dobson, Patrick/D-8771-2015; OI Rutqvist, Jonny/0000-0002-7949-9785; Dobson, Patrick/0000-0001-5031-8592; Garcia, Julio/0000-0001-6917-4998; Walters, Mark/0000-0001-8458-4813 FU Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department of Energy under the U.S. Department of Energy [DE-FC36-08G018201, DE-AC02-05CH11231]; Calpine Corporation FX This work was conducted with funding by the Assistant Secretary for Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department of Energy under the U.S. Department of Energy Contract No. DE-FC36-08G018201 and No. DE-AC02-05CH11231, and by Calpine Corporation. NR 40 TC 2 Z9 2 U1 8 U2 16 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD SEP PY 2016 VL 63 SI SI BP 97 EP 119 DI 10.1016/j.geothermics.2015.08.003 PG 23 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR0XT UT WOS:000379630900009 ER PT J AU Rutqvist, J Jeanne, P Dobson, PF Garcia, J Hartline, C Hutchings, L Singh, A Vasco, DW Walters, M AF Rutqvist, Jonny Jeanne, Pierre Dobson, Patrick F. Garcia, Julio Hartline, Craig Hutchings, Lawrence Singh, Ankit Vasco, Donald W. Walters, Mark TI The Northwest Geysers EGS Demonstration Project, California - Part 2: Modeling and interpretation SO GEOTHERMICS LA English DT Article DE The Geysers; EGS; Stimulation; Coupled THM Modeling; Seismicity; Seismic tomography; Ground surface deformations ID ENHANCED GEOTHERMAL SYSTEM; INDUCED EARTHQUAKES; FLUID-FLOW; RESERVOIR; FIELD; ROCK; PERMEABILITY AB In this paper, we summarize the results of coupled thermal, hydraulic, and mechanical (THM) modeling in support of the Northwest Geysers EGS Demonstration Project, which aims at enhancing production from a known High Temperature Reservoir (HTR) (280-400 degrees C) located under the conventional (240 degrees C) geothermal steam reservoir. The THM modeling was conducted to investigate geomechanical effects of cold-water injection during the stimulation of the EGS, first to predict the extent of the stimulation zone for a given injection schedule, and then to conduct interpretive analyses of the actual stimulation. By using a calibrated THM model based on historic injection and microseismic data at a nearby well, we could reasonably predict the extent of the stimulation zone around the injection well, at least for the first few months of injection. However, observed microseismic evolution and pressure responses over the one-year stimulation-injection revealed more heterogeneous behavior as a result of more complex geology, including a network of shear zones. Therefore, for an interpretive analysis of the one-year stimulation campaign, we included two sets of vertical shear zones within the model; a set of more permeable NW striking shear zones and a set of less permeable NE-striking shear zones. Our modeling indicates that the microseismic events in this system are related to shear reactivation of pre-existing fractures, triggered by the combined effects of injection-induced cooling around the injection well and rapid (but small) changes in steam pressure as far as a kilometer from the injection well. Overall, the integrated monitoring and modeling of microseismicity, ground surface deformations, reservoir pressure, fluid chemical composition, and seismic tomography depict an EGS system hydraulically bounded by some of the NE-striking low permeability shear zones, with the more permeable NW-striking shear zone providing liquid flow paths for stimulation deep (several kilometers) down into the HTR. The modeling indicates that a significant mechanical degradation (damage) inferred from seismic tomography, and potential changes in fracture porosity inferred from cross-well pressure responses, are related to shear rupture in the stimulation zone driven by both pressure and cooling effects. (C) 2015 The Authors. Published by Elsevier Ltd. C1 [Rutqvist, Jonny; Jeanne, Pierre; Dobson, Patrick F.; Hutchings, Lawrence; Singh, Ankit; Vasco, Donald W.] LBNL, Berkeley, CA 94720 USA. [Garcia, Julio; Hartline, Craig; Walters, Mark] Calpine Corp, Middletown, CA 95461 USA. RP Rutqvist, J (reprint author), LBNL, Berkeley, CA 94720 USA. EM Jrutqvist@lbl.gov RI Rutqvist, Jonny/F-4957-2015; Dobson, Patrick/D-8771-2015; Vasco, Donald/G-3696-2015 OI Rutqvist, Jonny/0000-0002-7949-9785; Dobson, Patrick/0000-0001-5031-8592; Vasco, Donald/0000-0003-1210-8628 FU Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department of Energy under the U.S. Department of Energy [DE-AC02-05CH11231, DE-FC36-08GO18201]; Calpine Corporation FX This work was conducted with funding by the Assistant Secretary for Energy Efficiency and Renewable Energy, Geothermal Technologies Program, of the U.S. Department of Energy under the U.S. Department of Energy Contract No. DE-AC02-05CH11231 and No. DE-FC36-08GO18201, and by Calpine Corporation. NR 44 TC 2 Z9 2 U1 14 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD SEP PY 2016 VL 63 SI SI BP 120 EP 138 DI 10.1016/j.geothermics.2015.08.002 PG 19 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR0XT UT WOS:000379630900010 ER PT J AU Benato, S Hickman, S Davatzes, NC Taron, J Spielman, P Elsworth, D Majer, EL Boyle, K AF Benato, Stefano Hickman, Stephen Davatzes, Nicholas C. Taron, Joshua Spielman, Paul Elsworth, Derek Majer, Ernest L. Boyle, Katie TI Conceptual model and numerical analysis of the Desert Peak EGS project: Reservoir response to the shallow medium flow-rate hydraulic stimulation phase SO GEOTHERMICS LA English DT Article DE Desert Peak; Enhanced geothermal systems; Reservoir stimulation modeling; Induced seismicity ID ENHANCED GEOTHERMAL SYSTEM; CALIFORNIA; GEYSERS; MICROSEISMICITY; PERMEABILITY; SEISMICITY; INJECTIONS; ROCKS AB A series of stimulation treatments were performed as part of the Engineered Geothermal System (EGS) experiment in the shallow open-hole section of Desert Peak well 27-15 (September 2010-November 2012). These injections at variable wellhead pressures, both below and above the magnitude of the least horizontal principal stress (S-hmin), produced injectivity gains consistent with hydraulically induced mechanical shear and tensile failure in the surrounding rock. A conceptual framework for the overall Desert Peak EGS experiment is developed and tested based on a synthesis of available structural and geological data. These data include down-hole fracture attributes, in situ stress conditions, pressure interference tests, geochemical tracer studies, and observed induced seismicity. Induced seismicity plays a key role in identifying the geometry of large-scale geological structures that could potentially serve as preferential flow paths during some of the stimulation phases. The numerical code FLAC3D is implemented to simulate the reservoir response to hydraulic stimulation and to investigate in situ conditions conducive to both tensile and shear failure. Results from the numerical analysis show that conditions for shear failure could have occurred along fractures associated with a large northeast-trending normal fault structure located similar to 400 m below the injection interval which coincides with the locations of most of the observed micro-seismicity. This structure may also provide a hydrologic connection between EGS well 27-15 and injection/production wells further to the south-southwest. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Benato, Stefano] Desert Res Inst, Div Hydrol Sci, Reno, NV 89512 USA. [Hickman, Stephen; Taron, Joshua] US Geol Survey, 345 Middlefield Rd, Menlo Pk, CA 94025 USA. [Davatzes, Nicholas C.] Temple Univ, Philadelphia, PA 19122 USA. [Spielman, Paul] Ormat Nevada Inc, Reno, NV 89511 USA. [Elsworth, Derek] Penn State Univ, University Pk, PA 16802 USA. [Boyle, Katie] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Benato, S (reprint author), Desert Res Inst, Div Hydrol Sci, Reno, NV 89512 USA. EM stefano.benato@gmail.com FU Desert Research Institute through a DHS fund; Great Basin Center for Geothermal Energy under a Geothermal Technology Program (GTP) Faculty Seed Grant; Ormat Technologies, Inc.; Itasca Education Partnership program FX This work was supported by the Desert Research Institute through a DHS fund, by the Great Basin Center for Geothermal Energy under a Geothermal Technology Program (GTP) Faculty Seed Grant, by Ormat Technologies, Inc., and by the Itasca Education Partnership program. The first author wishes to acknowledge Prof. Jim Faulds, Prof. Greg Pohll and Dr. Jonny Rutqvist for their comments/feedback while reviewing the document. NR 54 TC 0 Z9 0 U1 16 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0375-6505 EI 1879-3576 J9 GEOTHERMICS JI Geothermics PD SEP PY 2016 VL 63 SI SI BP 139 EP 156 DI 10.1016/j.geothermics.2015.06.008 PG 18 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR0XT UT WOS:000379630900011 ER PT J AU Yoo, J Estrada-Perez, CE Hassan, YA AF Yoo, Junsoo Estrada-Perez, Carlos E. Hassan, Yassin A. TI Experimental study on bubble dynamics and wall heat transfer arising from a single nucleation site at subcooled flow boiling conditions - Part 2: Data analysis on sliding bubble characteristics and associated wall heat transfer SO INTERNATIONAL JOURNAL OF MULTIPHASE FLOW LA English DT Article DE Subcooled flow boiling; Single nucleation site; Bubble sliding; Bubble coalescence; Sliding bubble velocity; Bubble size distribution; Boiling heat transfer ID DEPARTURE FREQUENCY; VERTICAL UPFLOW; NARROW CHANNEL; LOW-PRESSURES; SYSTEM; FLUX; VISUALIZATION; DIAMETER; VELOCITY; BEHAVIOR AB This second of two companion papers presents an analysis of sliding bubble and wall heat transfer parameters measured during subcooled boiling in a square, vertical, upward flow channel. Bubbles were generated only from a single nucleation site for better observation of both the sliding bubble characteristics and their impact on wall heat transfer through optical measurement techniques. Specific interests include: (i) bubbles departure and subsequent growth while sliding, (ii) bubbles release frequency, (iii) coalescence of sliding bubbles, (iv) sliding bubbles velocity, (v) bubbles size distribution and (vi) wall heat transfer influenced by sliding bubbles. The results showed that sliding bubbles involve two distinct growth behaviors: (i) at low mass fluxes, sliding bubbles grew fast near the nucleation site, subsequently shrank, and then grew again, (ii) as mass flux increased, however, sliding bubbles grew more steadily. The bubbles originating from the single nucleation site coalesced frequently while sliding, which showed close relation with bubbles release frequency. The sliding bubble velocity near the nucleation site consistently decreased by increasing mass flux, while the observation often became reversed as the bubbles slid downstream due to the effect of interfacial drag. The sliding bubbles moved faster than the local liquid (i.e., u(r) < 0) at low mass flux conditions, but it became reversed as the mass flux increased. The size distribution of sliding bubbles followed Gaussian distribution well both near and far from the nucleation site. The standard deviation of bubble size varied insignificantly through sliding compared to the changes in mean bubble size. Lastly, the sliding bubbles enhanced the wall heat transfer and the effect became more noticeable as inlet subcooling/mass flux decreased or wall heat flux increased. In particular, the sliding bubble characteristics such as bubble growth behavior observed near the nucleation site played a dominant role in determining the ultimate level of wall heat transfer enhancement within the test channel. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Yoo, Junsoo] Idaho Natl Lab, 2525 North Fremont Ave,POB 3860, Idaho Falls, ID 83415 USA. [Estrada-Perez, Carlos E.; Hassan, Yassin A.] Texas A&M Univ, Dept Mech Engn, 100 MEOB, College Stn, TX 77843 USA. [Hassan, Yassin A.] Texas A&M Univ, Dept Nucl Engn, 253 Bizzell West, College Stn, TX 77843 USA. RP Yoo, J (reprint author), Idaho Natl Lab, 2525 North Fremont Ave,POB 3860, Idaho Falls, ID 83415 USA. EM kaks2000@gmail.com FU CASL (Consortium for Advanced Simulation of Light Water Reactors), an Energy Innovation Hub under U.S. Department of Energy [DE-AC05-00OR22725] FX This research was supported by CASL (Consortium for Advanced Simulation of Light Water Reactors), an Energy Innovation Hub under U.S. Department of Energy Contract No. DE-AC05-00OR22725. The support is gratefully acknowledged. NR 43 TC 0 Z9 0 U1 13 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0301-9322 EI 1879-3533 J9 INT J MULTIPHAS FLOW JI Int. J. Multiph. Flow PD SEP PY 2016 VL 84 BP 292 EP 314 DI 10.1016/j.ijmultiphaseflow.2016.04.019 PG 23 WC Mechanics SC Mechanics GA DQ9XM UT WOS:000379562600024 ER PT J AU Mamontov, E AF Mamontov, Eugene TI A novel approach to neutron scattering instrumentation for probing multiscale dynamics in soft and biological matter SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE neutron scattering; dynamics; bio/soft matter ID WATER AB We present a concept and ray-tracing simulation of a mechanical device that will enable inelastic neutron scattering measurements where the data at energy transfers from a few mu eV to several hundred meV can be collected in a single, gapless spectrum. Besides covering 5 orders of magnitude on the energy (time) scale, the device provides data over 2 orders of magnitude on the scattering momentum (length) scale in a single measurement. Such capabilities are geared primarily toward soft and biological matter, where the broad dynamical features of relaxation origin largely overlap with vibration features, thus necessitating gapless spectral coverage over several orders of magnitude in time and space. Furthermore, neutron scattering experiments with such a device are performed with a fixed neutron final energy, which enables measurements, with neutron energy loss in the sample, at arbitrarily low temperatures over the same broad spectral range. This capability is also invaluable in biological and soft matter research, as the variable temperature dependence of different relaxation components allows their separation in the scattering spectra as a function of temperature. C1 [Mamontov, Eugene] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Mamontov, E (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM mamontove@ornl.gov RI Mamontov, Eugene/Q-1003-2015 OI Mamontov, Eugene/0000-0002-5684-2675 FU Laboratory Directed Research and Development Program [32112563]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE; U.S. DOE [DE-AC05-00OR22725] FX This research was conducted with support from the Laboratory Directed Research and Development Program (project 32112563) and the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE. Oak Ridge National Laboratory is managed by UTBattelle, LLC, for the U.S. DOE under Contract No. DE-AC05-00OR22725. NR 18 TC 0 Z9 0 U1 1 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD SEP 1 PY 2016 VL 28 IS 34 AR 345201 DI 10.1088/0953-8984/28/34/345201 PG 5 WC Physics, Condensed Matter SC Physics GA DQ9UU UT WOS:000379555600010 PM 27355223 ER PT J AU Caldwell, A Adli, E Amorim, L Apsimon, R Argyropoulos, T Assmann, R Bachmann, AM Batsch, E Bauche, J Olsen, VKB Bernardini, M Bingham, R Biskup, B Bohl, T Bracco, C Burrows, PN Burt, G Buttenschon, B Butterworth, A Cascella, M Chattopadhyay, S Chevallay, E Cipiccia, S Damerau, H Deacon, L Dirksen, R Doebert, S Dorda, U Eisen, E Farmer, J Fartoukh, S Fedosseev, V Feldbaumer, E Fiorito, R Fonseca, R Friebel, F Geschonke, G Goddard, B Gorn, AA Grulke, O Gschwendtner, E Hansen, J Hessler, C Hillenbrand, S Hofle, W Holloway, J Huang, C Huther, M Jaroszynski, D Jensen, L Jolly, S Joulaei, A Kasim, M Keeble, F Kersevan, R Kumar, N Li, Y Liu, S Lopes, N Lotov, KV Lu, W Machacek, J Mandry, S Martin, I Martorelli, R Martyanov, M Mazzoni, S Meddahi, M Merminga, L Mete, O Minakov, VA Mitchell, J Moody, J Muller, AS Najmudin, Z Noakes, TCQ Norreys, P Osterhoff, J Oz, E Pardons, A Pepitone, K Petrenko, A Plyushchev, G Pozimski, J Pukhov, A Reimann, O Rieger, K Roesler, S Ruhl, H Rusnak, T Salveter, E Savard, N Schmidt, J von der Schmitt, H Seryi, A Shaposhnikova, E Sheng, ZM Sherwood, R Silva, L Simon, F Soby, L Sosedkin, AP Spitsyn, RI Tajima, T Tarkeshian, R Timko, H Trines, R Tuckmantel, T Tuev, PV Turner, M Velotti, E Verzilov, V Vieira, J Vincke, H Wei, Y Welsch, CP Wing, M Xia, G Yakimenko, V Zhang, H Zimmermann, F AF Caldwell, A. Adli, E. Amorim, L. Apsimon, R. Argyropoulos, T. Assmann, R. Bachmann, A. -M. Batsch, E. Bauche, J. Olsen, V. K. Berglyd Bernardini, M. Bingham, R. Biskup, B. Bohl, T. Bracco, C. Burrows, P. N. Burt, G. Buttenschoen, B. Butterworth, A. Cascella, M. Chattopadhyay, S. Chevallay, E. Cipiccia, S. Damerau, H. Deacon, L. Dirksen, R. Doebert, S. Dorda, U. Eisen, E. Farmer, J. Fartoukh, S. Fedosseev, V. Feldbaumer, E. Fiorito, R. Fonseca, R. Friebel, F. Geschonke, G. Goddard, B. Gorn, A. A. Grulke, O. Gschwendtner, E. Hansen, J. Hessler, C. Hillenbrand, S. Hofle, W. Holloway, J. Huang, C. Huether, M. Jaroszynski, D. Jensen, L. Jolly, S. Joulaei, A. Kasim, M. Keeble, F. Kersevan, R. Kumar, N. Li, Y. Liu, S. Lopes, N. Lotov, K. V. Lu, W. Machacek, J. Mandry, S. Martin, I. Martorelli, R. Martyanov, M. Mazzoni, S. Meddahi, M. Merminga, L. Mete, O. Minakov, V. A. Mitchell, J. Moody, J. Mueller, A. -S. Najmudin, Z. Noakes, T. C. Q. Norreys, P. Osterhoff, J. Oez, E. Pardons, A. Pepitone, K. Petrenko, A. Plyushchev, G. Pozimski, J. Pukhov, A. Reimann, O. Rieger, K. Roesler, S. Ruhl, H. Rusnak, T. Salveter, E. Savard, N. Schmidt, J. von der Schmitt, H. Seryi, A. Shaposhnikova, E. Sheng, Z. M. Sherwood, R. Silva, L. Simon, F. Soby, L. Sosedkin, A. P. Spitsyn, R. I. Tajima, T. Tarkeshian, R. Timko, H. Trines, R. Tueckmantel, T. Tuev, P. V. Turner, M. Velotti, E. Verzilov, V. Vieira, J. Vincke, H. Wei, Y. Welsch, C. P. Wing, M. Xia, G. Yakimenko, V. Zhang, H. Zimmermann, F. TI Path to AWAKE: Evolution of the concept SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Plasma wakefield acceleration; Proton driver; Self-modulation instability ID PLASMA-WAKEFIELD ACCELERATION; WAKE-FIELD ACCELERATOR; IN-CELL CODE; ULTRARELATIVISTIC BEAM DYNAMICS; ELECTRON-BEAM; SIMULATION; BUNCHES; PHYSICS; PULSE; CERN AB This paper describes the conceptual steps in reaching the design of the AWAKE experiment currently under construction at CERN. We start with an introduction to plasma wakefield acceleration and the motivation for using proton drivers. We then describe the self-modulation instability - a key to an early realization of the concept. This is then followed by the historical development of the experimental design, where the critical issues that arose and their solutions are described. We conclude with the design of the experiment as it is being realized at CERN and some words on the future outlook. A summary of the AWAKE design and construction status as presented in this conference is given in Gschwendtner et al. [1]. (C) 2016 Published by Elsevier B.V. C1 [Noakes, T. C. Q.] STFC Daresbury Lab, ASTeC, Accelerator Sci & Technol Ctr, Warrington WA4 4AD, Cheshire, England. [Martin, I.] Aix Marseille Univ, IUSTI, CNRS, UMR 7343, Polytech Marseille, France. [Fiorito, R.; Gorn, A. A.; Lotov, K. V.; Minakov, V. A.; Sosedkin, A. P.; Spitsyn, R. I.; Tuev, P. V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Argyropoulos, T.; Bauche, J.; Bernardini, M.; Biskup, B.; Bohl, T.; Bracco, C.; Butterworth, A.; Chevallay, E.; Cipiccia, S.; Damerau, H.; Doebert, S.; Fartoukh, S.; Fedosseev, V.; Feldbaumer, E.; Friebel, F.; Geschonke, G.; Goddard, B.; Gschwendtner, E.; Hessler, C.; Hillenbrand, S.; Hofle, W.; Jensen, L.; Kersevan, R.; Mazzoni, S.; Meddahi, M.; Pardons, A.; Pepitone, K.; Petrenko, A.; Plyushchev, G.; Roesler, S.; Salveter, E.; von der Schmitt, H.; Shaposhnikova, E.; Soby, L.; Timko, H.; Turner, M.; Velotti, E.; Vincke, H.; Zhang, H.; Zimmermann, F.] CERN, Geneva, Switzerland. [Apsimon, R.; Burt, G.; Li, Y.; Mete, O.; Mitchell, J.; Wei, Y.; Welsch, C. P.; Xia, G.; Zhang, H.] Cockcroft Inst, Warrington WA4 4AD, Cheshire, England. [Biskup, B.] Czech Tech Univ, Zikova 1903-4, Prague 16636 6, Czech Republic. [Assmann, R.; Dorda, U.; Eisen, E.; Osterhoff, J.; Wing, M.] DESY, Notkestr 85, D-22607 Hamburg, Germany. [Chattopadhyay, S.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Farmer, J.; Martorelli, R.; Pukhov, A.] Univ Dusseldorf, Moorenstr 5, D-40225 Dusseldorf, Germany. [Amorim, L.; Fonseca, R.; Lopes, N.; Silva, L.; Vieira, J.] Univ Lisbon, Inst Super Tecn, GoLP Inst Plasmas & Fusao Nucl, Lisbon, Portugal. [Lopes, N.; Najmudin, Z.; Pozimski, J.] Imperial Coll London, Blackett Lab, London SW7 2BW, England. [Burrows, P. N.; Kasim, M.; Seryi, A.; Tueckmantel, T.] John Adams Inst Accelerator Sci, Oxford, England. [Caldwell, A.; Butterworth, A.; Joulaei, A.; Mueller, A. -S.; Pardons, A.; Petrenko, A.; Pukhov, A.; Reimann, O.] Karlsruhe Inst Technol, D-76021 Karlsruhe, Germany. [Apsimon, R.; Burt, G.; Mitchell, J.] Univ Lancaster, Lancaster LA1 4YR, England. [Huang, C.] Los Alamos Natl Lab, Los Alamos, NM USA. [Ruhl, H.; Tajima, T.] Univ Munich, D-80539 Munich, Germany. [Kumar, N.] Max Planck Inst Nucl Phys, Saupfercheckweg 1, D-69117 Heidelberg, Germany. [Caldwell, A.; Bachmann, A. -M.; Batsch, E.; Huether, M.; Joulaei, A.; Machacek, J.; Martyanov, M.; Moody, J.; Oez, E.; Reimann, O.; Rieger, K.; Rusnak, T.; Savard, N.; von der Schmitt, H.; Simon, F.] Max Planck Inst Phys & Astrophys, Fohringer Ring 6, D-80805 Munich, Germany. [Buttenschoen, B.; Grulke, O.] Max Planck Inst Plasma Phys, Wendelsteinstr 1, D-17491 Greifswald, Germany. [Chattopadhyay, S.] Northern Illinois Univ, 1425 W Lincoln Hwy, De Kalb, IL 60115 USA. [Gorn, A. A.; Lotov, K. V.; Minakov, V. A.; Sosedkin, A. P.; Spitsyn, R. I.; Tuev, P. V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Tarkeshian, R.] PSI, CH-5232 Villigen, Switzerland. [Sheng, Z. M.] Shanghai Jiao Tong Univ, Shanghai 200240, Peoples R China. [Yakimenko, V.] SLAC Natl Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Sheng, Z. M.] STFC Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Plyushchev, G.] Ecole Polytech Fed Lausanne, Swiss Plasma Ctr, CH-1015 Lausanne, Switzerland. [Huether, M.; Rieger, K.] Tech Univ Munich, Arcisstr 21, D-80333 Munich, Germany. [Dirksen, R.; Liu, S.; Savard, N.; Verzilov, V.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Fiorito, R.; Lu, W.] Tsinghua Univ, Beijing 100084, Peoples R China. [Cascella, M.; Deacon, L.; Jolly, S.; Keeble, F.; Mandry, S.; Sherwood, R.; Wing, M.] UCL, Gower St, London WC1E 6BT, England. [Wei, Y.; Welsch, C. P.; Zhang, H.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Li, Y.; Mete, O.; Xia, G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Adli, E.; Olsen, V. K. Berglyd] Univ Oslo, N-0316 Oslo, Norway. [Burrows, P. N.; Holloway, J.; Kasim, M.; Norreys, P.; Seryi, A.] Univ Oxford, Oxford OX1 2JD, England. [Cipiccia, S.; Jaroszynski, D.; Sheng, Z. M.] Univ Strathclyde, 16 Richmond St, Glasgow G1 1XQ, Lanark, Scotland. [Savard, N.] Univ Victoria, 3800 Finnerty Rd, Victoria, BC, Canada. RP Caldwell, A (reprint author), Max Planck Inst Phys & Astrophys, Fohringer Ring 6, D-80805 Munich, Germany. RI Sheng, Zheng-Ming/H-5371-2012; Assmann, Ralph/L-8457-2016; Lopes, Nelson/C-6540-2009; Fonseca, Ricardo/B-7680-2009; pukhov, alexander/C-8082-2016; Petrenko, Alexey/R-6313-2016; Lotov, Konstantin/H-6217-2016; Fedosseev, Valentin/A-6240-2010; Cascella, Michele/B-6156-2013; Tuev, Petr/R-7929-2016; OI Huang, Chengkun/0000-0002-3176-8042; Amorim, Ligia/0000-0002-1445-0032; Lopes, Nelson/0000-0001-8355-4727; Fonseca, Ricardo/0000-0001-6342-6226; Petrenko, Alexey/0000-0002-7772-8206; Fedosseev, Valentin/0000-0001-8767-1445; Cascella, Michele/0000-0003-2091-2501; Biskup, Bartolomej/0000-0003-0833-3267; Farmer, John/0000-0002-6758-2127 NR 111 TC 5 Z9 5 U1 11 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 3 EP 16 DI 10.1016/j.nima.2015.12.050 PG 14 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100002 ER PT J AU Lishilin, O Gross, M Brinkmann, R Engel, J Gruner, F Kos, G Krasilnikov, M de la Ossa, AM Mehrling, T Osterhoff, J Pathak, G Philipp, S Renier, Y Richter, D Schroeder, C Schutze, R Stephan, E AF Lishilin, O. Gross, M. Brinkmann, R. Engel, J. Gruener, F. Koss, G. Krasilnikov, M. de la Ossa, A. Martinez Mehrling, T. Osterhoff, J. Pathak, G. Philipp, S. Renier, Y. Richter, D. Schroeder, C. Schuetze, R. Stephan, E. TI First results of the plasma wakefield acceleration experiment at PITZ SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE PWFA; Self-modulation instability; Heat pipe oven; Electron beam scattering AB The self-modulation instability of long particle beams was proposed as a new mechanism to produce driver beams for proton driven plasma wakefield acceleration (PWFA). The PWFA experiment at the Photo Injector Test facility at DESY, Zeuthen site (PITZ) was launched to experimentally demonstrate and study the self modulation of long electron beams in plasma. Key aspects for the experiment are the very flexible photocathode laser system, a plasma cell and well-developed beam diagnostics. In this contribution we report about the plasma cell design, preparatory experiments and the results of the first PWFA experiment at PITZ. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lishilin, O.; Gross, M.; Engel, J.; Koss, G.; Krasilnikov, M.; Pathak, G.; Philipp, S.; Renier, Y.; Schuetze, R.; Stephan, E.] DESY, Deutsch Elektronen Synchrotron, Zeuthen, Germany. [Brinkmann, R.; de la Ossa, A. Martinez; Mehrling, T.; Osterhoff, J.] DESY, Deutsch Elektronen Synchrotron, Hamburg, Germany. [Gruener, F.] Univ Hamburg, UHH, Hamburg, Germany. [Gruener, F.] Ctr Free Electron Laser Sci, CFEL, Hamburg, Germany. [Richter, D.] Helmholtz Zentrum Berlin, Berlin, Germany. [Schroeder, C.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Lishilin, O (reprint author), DESY, Deutsch Elektronen Synchrotron, Zeuthen, Germany. EM osip.lishilin@desy.de RI Gruner, Florian/M-1212-2016; OI Gruner, Florian/0000-0001-8382-9225; Schroeder, Carl/0000-0002-9610-0166; Mehrling, Timon J./0000-0002-1280-4642 NR 21 TC 0 Z9 0 U1 6 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 37 EP 42 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100007 ER PT J AU Schroeder, CB Benedetti, C Esarey, E Leemans, WP AF Schroeder, C. B. Benedetti, C. Esarey, E. Leemans, W. P. TI Laser-plasma-based linear collider using hollow plasma channels SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Laser-plasma accelerator; Linear collider ID ELECTRON-ACCELERATORS AB A linear electron-positron collider based on laser-plasma accelerators using hollow plasma channels is considered. Laser propagation and energy depletion in the hollow channel is discussed, as well as the overall efficiency of the laser-plasma accelerator. Example parameters are presented for a 1-TeV and 3-TeV center-of-mass collider based on laser-plasma accelerators. (C) 2016 Elsevier B.V. All rights reserved. C1 [Schroeder, C. B.; Benedetti, C.; Esarey, E.; Leemans, W. P.] Lawrence Berkeley Natl Lab, BELLA Ctr, Berkeley, CA 94720 USA. RP Schroeder, CB (reprint author), Lawrence Berkeley Natl Lab, BELLA Ctr, Berkeley, CA 94720 USA. EM CBSchroeder@lbl.gov OI Schroeder, Carl/0000-0002-9610-0166 NR 21 TC 0 Z9 0 U1 9 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 113 EP 116 DI 10.1016/j.nima.2016.03.001 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100022 ER PT J AU Zholents, A Gai, W Doran, S Lindberg, R Power, JG Strelnikov, N Sun, Y Trakhtenberg, E Vasserman, I Jing, C Kanareykin, A Li, Y Gao, Q Shchegolkov, DY Simakov, EI AF Zholents, A. Gai, W. Doran, S. Lindberg, R. Power, J. G. Strelnikov, N. Sun, Y. Trakhtenberg, E. Vasserman, I. Jing, C. Kanareykin, A. Li, Y. Gao, Q. Shchegolkov, D. Y. Simakov, E. I. TI A preliminary design of the collinear dielectric wakefield accelerator SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Wakefield; Dielectric; Beam breakup; BNS damping; Free-electron laser; Quadrupole wiggler AB A preliminary design of the multi-meter long collinear dielectric wakefield accelerator that achieves a highly efficient transfer of the drive bunch energy to the wakefields and to the witness bunch is considered. It is made from similar to 0.5 m long accelerator modules containing a vacuum chamber with dielectric lined walls, a quadrupole wiggler, an rf coupler, and BPM assembly. The single bunch breakup instability is a major limiting factor for accelerator efficiency, and the BNS damping is applied to obtain the stable multi-meter long propagation of a drive bunch. Numerical simulations using a 6D particle tracking computer code are performed and tolerances to various errors are defined. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zholents, A.; Gai, W.; Doran, S.; Lindberg, R.; Power, J. G.; Strelnikov, N.; Sun, Y.; Trakhtenberg, E.; Vasserman, I.] ANL, Argonne, IL 60439 USA. [Jing, C.; Kanareykin, A.; Li, Y.] Euclid Techlabs LLC, Solon, OH 44139 USA. [Gao, Q.] Tsinghua Univ, Beijing, Peoples R China. [Shchegolkov, D. Y.; Simakov, E. I.] LANL, Los Alamos, NM 87545 USA. RP Zholents, A (reprint author), ANL, Argonne, IL 60439 USA. OI Shchegolkov, Dmitry/0000-0002-0721-3397; Simakov, Evgenya/0000-0002-7483-1152 NR 13 TC 2 Z9 2 U1 3 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 190 EP 193 DI 10.1016/j.nima.2016.02.003 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100040 ER PT J AU Teryaev, VE Kazakov, SY Hirshfield, JL AF Teryaev, Vladimir E. Kazakov, Sergey Yu. Hirshfield, Jay L. TI Multi-beam linear accelerator EVT SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Linear accelerator; Two-beam accelerator; Electron gun; Drive beam; Accelerated beam; RF buncher AB A novel electron multi-beam accelerator is presented. The accelerator, short-named EVT (Electron Voltage Transformer) belongs to the class of two-beam accelerators. It combines an RF generator and essentially an accelerator within the same vacuum envelope. Drive beam-lets and an accelerated beam are modulated in RF modulators and then bunches pass into an accelerating structure, comprising uncoupled with each other and inductive tuned cavities, where the energy transfer from the drive beams to the accelerated beam occurs. A phasing of bunches is solved by choice correspond distances between gaps of the adjacent cavities. Preliminary results of numerical simulations and the initial specification of EVT operating in S-band, with a 60 kV gun and generating a 2.7 A, 1.1 MV beam at its output is presented. A relatively high efficiency of 67% and high design average power suggest that EVT can find its use in industrial applications. Published by Elsevier B.V. C1 [Teryaev, Vladimir E.; Hirshfield, Jay L.] Omega P Inc, New Haven, CT 06510 USA. [Kazakov, Sergey Yu.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Hirshfield, Jay L.] Yale Univ, New Haven, CT 06511 USA. RP Teryaev, VE (reprint author), Omega P Inc, New Haven, CT 06510 USA. EM viadimir_teryaev@mail.ru NR 4 TC 0 Z9 0 U1 4 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 221 EP 223 DI 10.1016/j.nima.2016.03.066 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100045 ER PT J AU Lotov, KV Vay, JL AF Lotov, K. V. Vay, J. -L. TI Summary of working group 6: Theory and simulations SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Theory and numerical simulations; Plasma based accelerators; Laser wakefield accelerator AB The paper briefly summarizes the contributions presented during the working group 6 sessions on theory and simulations. (C) 2016 Published by Elsevier B.V. C1 [Lotov, K. V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Lotov, K. V.] RAS, SB, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Vay, J. -L.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA USA. RP Lotov, KV (reprint author), Novosibirsk State Univ, Novosibirsk 630090, Russia.; Lotov, KV (reprint author), RAS, SB, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. EM K.V.Lotov@inp.nsk.su RI Lotov, Konstantin/H-6217-2016 NR 18 TC 0 Z9 0 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 348 EP 349 DI 10.1016/j.nima.2015.12.014 PG 2 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100071 ER PT J AU Vay, JL Lehe, R Vincenti, H Godfrey, BB Haber, I Lee, P AF Vay, J. -L. Lehe, R. Vincenti, H. Godfrey, B. B. Haber, I. Lee, P. TI Recent advances in high-performance modeling of plasma-based acceleration using the full PIC method SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE Particle-in-cell; Particle accelerators; Plasma based accelerators; Laser wakefield accelerator; Plasma simulations; Relativistic plasmas ID NUMERICAL STABILITY; PARTICLE CODES; SIMULATIONS; ALGORITHM; INSTABILITIES AB Numerical simulations have been critical in the recent rapid developments of plasma-based acceleration concepts. Among the various available numerical techniques, the particle-in-cell (PIC) approach is the method of choice for self-consistent simulations from first principles. The fundamentals of the PIC method were established decades ago, but improvements or variations are continuously being proposed. We report on several recent advances in PIC-related algorithms that are of interest for application to plasma-based accelerators, including (a) detailed analysis of the numerical Cherenkov instability and its remediation for the modeling of plasma accelerators in laboratory and Lorentz boosted frames, (b) analytic pseudo-spectral electromagnetic solvers in Cartesian and cylindrical (with azimuthal modes decomposition) geometries, and (c) novel analysis of Maxwell's solvers' stencil variation and truncation, in application to domain decomposition strategies and implementation of perfectly matched layers in high-order and pseudo-spectral solvers. (C) 2016 Published by Elsevier B.V. C1 [Vay, J. -L.; Lehe, R.; Godfrey, B. B.] LBNL, Berkeley, CA 94720 USA. [Vincenti, H.] CEA, Saclay, France. [Godfrey, B. B.; Haber, I.] Univ Maryland, College Pk, MD 20742 USA. [Lee, P.] Univ Paris Saclay, CNRS, LPGP, F-91405 Orsay, France. RP Vay, JL (reprint author), LBNL, Berkeley, CA 94720 USA. EM jlvay@lbl.gov OI Godfrey, Brendan/0000-0003-2311-7060 NR 36 TC 1 Z9 1 U1 7 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 353 EP 357 DI 10.1016/j.nima.2015.12.033 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100073 ER PT J AU Lee, P Audet, TL Lehe, R Vay, JL Maynard, G Cros, B AF Lee, P. Audet, T. L. Lehe, R. Vay, J. -L. Maynard, G. Cros, B. TI Modeling laser-driven electron acceleration using WARP with Fourier decomposition SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE LPA; PIC; WARP; Ionization-induced injection AB WARP is used with the recent implementation of the Fourier decomposition algorithm to model laser driven electron acceleration in plasmas. Simulations were carried out to analyze the experimental results obtained on ionization-induced injection in a gas cell. The simulated results are in good agreement with the experimental ones, confirming the ability of the code to take into account the physics of electron injection and reduce calculation time. We present a detailed analysis of the laser propagation, the plasma wave generation and the electron beam dynamics. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lee, P.; Audet, T. L.; Maynard, G.; Cros, B.] Univ Paris Saclay, Univ Paris 11, CNRS, LPGP, F-91405 Orsay, France. [Lehe, R.; Vay, J. -L.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lee, P (reprint author), Univ Paris Saclay, Univ Paris 11, CNRS, LPGP, F-91405 Orsay, France. EM patrick.lee@u-psud.fr OI Lee, Patrick/0000-0003-4931-1021 NR 7 TC 1 Z9 1 U1 5 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 358 EP 362 DI 10.1016/j.nima.2015.12.036 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100074 ER PT J AU Pogorelsky, IV Babzien, M Ben-Zvi, I Skaritka, J Polyanskiy, MN AF Pogorelsky, Igor V. Babzien, Markus Ben-Zvi, Ilan Skaritka, John Polyanskiy, Mikhail N. TI BESTIA - The next generation ultra-fast CO2 laser for advanced accelerator research SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article; Proceedings Paper CT 2nd Workshop on European Advanced Accelerator Concepts (EAAC) CY 2015 CL INFN, ITALY SP Amplitude, Ocem, RadiaBeam, EuroNNAc2 Network, EuCARD 2 Project, DESY, CERN HO INFN DE CO2 laser; Pulse compression; Strong field phenomena; Ion acceleration; Laser wake field ID PULSE AMPLIFICATION AB Over the last two decades, BNL's ATF has pioneered the use of high-peak power CO2 lasers for research in advanced accelerators and radiation sources. Our recent developments in ion acceleration, Compton scattering, and IFELs have further underscored the benefits from expanding the landscape of strong-field laser interactions deeper into the mid-infrared (MIR) range of wavelengths. This extension validates our ongoing efforts in advancing CO2 laser technology, which we report here. Our next-generation, multiterawatt, femtosecond CO2 laser will open new opportunities for studying ultra-relativistic laser interactions with plasma in the MIR spectral domain, including new regimes in the particle acceleration of ions and electrons. (C) 2015 Elsevier B.V. All rights reserved. C1 [Pogorelsky, Igor V.; Babzien, Markus; Ben-Zvi, Ilan; Skaritka, John; Polyanskiy, Mikhail N.] Brookhaven Natl Lab, Accelerator Tests Facil, Upton, NY 11973 USA. RP Pogorelsky, IV (reprint author), Brookhaven Natl Lab, Accelerator Tests Facil, Upton, NY 11973 USA. EM igar@bni.gov NR 7 TC 3 Z9 3 U1 5 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD SEP 1 PY 2016 VL 829 BP 432 EP 437 DI 10.1016/j.nima.2015.11.126 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DQ4AB UT WOS:000379144100090 ER PT J AU Rainwater, BH Velisavljevic, N Park, C Sun, HB Waller, GH Tsoi, GM Vohra, YK Liu, ML AF Rainwater, Ben H. Velisavljevic, Nenad Park, Changyong Sun, Haibin Waller, Gordon H. Tsoi, Georgiy M. Vohra, Yogesh K. Liu, Meilin TI High pressure structural study of samarium doped CeO2 oxygen vacancy conductor - Insight into the dopant concentration relationship to the strain effect in thin film ionic conductors SO SOLID STATE IONICS LA English DT Article DE Solid state ionics; Nanoionics; Solid oxide fuel cells; Strain effect; Doped-ceria; Isothermal bulk modulus ID X-RAY-DIFFRACTION; SOLID ELECTROLYTES; ACTIVATION-ENERGY; TRANSPORT; SUPERLATTICES; TEMPERATURE; SIMULATION; MODULUS; OXIDES; MODEL AB The bulk modulus of nanocrystalline, fluorite-structured samarium doped ceria, Sm0.2Ce0.8O1.9, has been investigated using synchrotron-based high-pressure X-ray diffraction technique. Experiments were carried out under both quasi-hydrostatic condition with silicon oil pressure transmitting medium (PTM) and nonhydrostatic conditions without PTM. The high pressure structural results indicate that the highly defected ionic conductor is stable up to 20 GPa and has a lower bulk modulus than what has been reported for undoped-CeO2. The isothermal bulk modulus of Sm0.2Ce0.8O1.9 is similar to 150-190 GPa compared to similar to 210-220 GPa for CeO2. The collected data experimentally verifies the effect of Sm3+ dopant and oxygen vacancy defect formation on bulk modulus in doped CeO2. The effect of modulus on misfit dislocation formation and dopant ion segregation is discussed in relation to a fundamental understanding of the strain effect in this important family of fast ionic conductors, with potential application as oxygen vacancy conducting solid state electrolytes. (C) 2016 Elsevier B.V. All rights reserved. C1 [Rainwater, Ben H.; Sun, Haibin; Waller, Gordon H.; Liu, Meilin] Georgia Inst Technol, Sch Mat Sci & Engn, Ctr for Innovat Fuel Cell & Battery Technol, Atlanta, GA 30332 USA. [Velisavljevic, Nenad] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Park, Changyong] Carnegie Inst Sci, Geophys Lab, High Pressure Collaborat Access Team, Argonne, IL 60439 USA. [Tsoi, Georgiy M.; Vohra, Yogesh K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RP Rainwater, BH (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Ctr for Innovat Fuel Cell & Battery Technol, Atlanta, GA 30332 USA. RI Liu, Meilin/E-5782-2010; Park, Changyong/A-8544-2008 OI Liu, Meilin/0000-0002-6188-2372; Park, Changyong/0000-0002-3363-5788 FU National Science Foundation [DGE-1148903, DMR-1410320]; Department of Energy ARPA-E REBELS Program [DE-AR0000502]; Los Alamos National Laboratory (LANL) [DE-AC52-06NA25396]; DOE-NNSA [DE-NA0001974, DE-NA0002014]; DOE-BES [DE-FG02-99ER45775]; NSF; US DOE [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation under Grant Nos. DGE-1148903 and DMR-1410320, Department of Energy ARPA-E REBELS Program under award number DE-AR0000502, and Los Alamos National Laboratory (LANL) operated by LANS, LLC for the DOE-NNSA under Contract No. DE-AC52-06NA25396. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. YKV would like to acknowledge support from the DOE-NNSA under Award No. DE-NA0002014. NR 36 TC 0 Z9 0 U1 17 U2 40 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD SEP PY 2016 VL 292 BP 59 EP 65 DI 10.1016/j.ssi.2016.05.010 PG 7 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA DR0YP UT WOS:000379633100010 ER PT J AU Mao, J Ma, MZ Liu, PP Hu, JH Shao, GS Battaglia, V Dai, KH Liu, G AF Mao, Jing Ma, Mengze Liu, Panpan Hu, Junhua Shao, Guosheng Battaglia, Vince Dai, Kehua Liu, Gao TI The effect of cobalt doping on the morphology and electrochemical performance of high-voltage spinel LiNi0.5Mn1.5O4 cathode material SO SOLID STATE IONICS LA English DT Article DE High-voltage spinel; Lithium nickel manganese oxide; Lithium chemical diffusion coefficient; Cycling performance; Rate performance ID LITHIUM-ION BATTERIES; 55 DEGREES-C; RATE CAPABILITY; LICR0.2NI0.4MN1.4O4 SPINEL; PARTICLE-SIZE; LIMN1.5NI0.5O4; TEMPERATURE; FE; ELECTRODE; PROGRESS AB To reveal the effects of Co-doping on the electrochemical performance of micro-sized LiNi0.5Mn1.5O4 (LNMO), undoped LNMO and Co-doped LiCo0.1Ni0.45Mn1.45O4 (LCoNMO) are synthesized via a PVP-combustion method and calcined at 1000 degrees C for 6 h. SEM and XRD analyses suggest that Co-doping decreases the particle size and the Li2Ni1-zO2 impurity at the calcination temperature of 1000 degrees C. LCoNMO has much better rate capability while its specific capacity at C/5 is 10% lower than that of LNMO. At 15 C rate, their specific capacities are closed, and the LCoNMO delivers 86.2% capacity relative to C/5, and this value for LNMO is only 77.0%. The D-Li + values determined by potential intermittent titration technique (PITT) test of LCoNMO are 1-2 times higher than that of LNMO in most SOC region. The LCoNMO shows very excellent cycling performance, which is the best value compared with literatures. After 1000 cycles, the LCoNMO still delivers 94.1% capacity. Moreover, its coulombic efficiency and energy efficiency keep at 99.84% and over 973% during 1 C. cycling, respectively. (C) 2015 Published by Elsevier B.V. C1 [Mao, Jing; Ma, Mengze; Liu, Panpan; Hu, Junhua; Shao, Guosheng] Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450002, Peoples R China. [Mao, Jing; Ma, Mengze; Liu, Panpan; Hu, Junhua; Shao, Guosheng] Zhengzhou Univ, Int Joint Res Lab Low Carbon Environm Mat Henan P, Zhengzhou 450002, Peoples R China. [Mao, Jing; Battaglia, Vince; Dai, Kehua; Liu, Gao] Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resource Div, Energy Technol Area, Berkeley, CA 94720 USA. [Dai, Kehua] Northeastern Univ, Sch Met & Mat, Shenyang 110004, Peoples R China. RP Liu, G (reprint author), Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resource Div, Energy Technol Area, Berkeley, CA 94720 USA.; Dai, KH (reprint author), Northeastern Univ, Sch Met & Mat, Shenyang 110004, Peoples R China. EM daikh@smm.neu.edu.cn; gliu@lbl.gov RI Shao, Guosheng/C-2143-2016 OI Shao, Guosheng/0000-0003-1498-7929 FU National Natural Science Foundation of China [51204038, U1504521]; Fundamental Research Funds for the Central. Universities of China [N110802002, L1502004]; Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Natural Science Foundation of China (51204038, U1504521) and the Fundamental Research Funds for the Central. Universities of China (N110802002, L1502004). This work was also supported by the Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy, under the Advanced Battery Materials Research (BMR) Program and Applied Battery Research (ABR) Program under contract No. DE-AC02-05CH11231. NR 45 TC 1 Z9 1 U1 28 U2 55 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2738 EI 1872-7689 J9 SOLID STATE IONICS JI Solid State Ion. PD SEP PY 2016 VL 292 BP 70 EP 74 DI 10.1016/j.ssi.2016.05.008 PG 5 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA DR0YP UT WOS:000379633100012 ER PT J AU Sati, M Lindstrom, P Rossignac, J AF Sati, Mukul Lindstrom, Peter Rossignac, Jarek TI eBits: Compact stream of mesh refinements for remote visualization SO COMPUTER-AIDED DESIGN LA English DT Article; Proceedings Paper CT Symposium on Solid and Physical Modelling (SPM) CY JUN 20-24, 2016 CL Berlin, GERMANY DE Triangle mesh compression; Remote visualization; Level of detail; Selective transmission; Local refinement; Triangle collapse ID TRIANGLE MESHES; POLYGONAL MODELS; COMPRESSION; EDGEBREAKER AB We focus on applications where a remote client needs to visualize or process a complex, manifold triangle mesh, M, but only in a relatively small, user controlled, Region of Interest (RoI) at a time. The client first downloads a coarse base mesh, pre-computed on the server via a series of simplification passes on M, one per Level of Detail (LoD), each pass identifying an independent set of triangles, collapsing them, and, for each collapse, storing, in a Vertex Expansion Record (VER), the information needed to reverse the collapse. On each client initiated RoI modification request, the server pushes to the client a selected subset of these VERs, which, when decoded and applied to refine the mesh locally, ensure that the portion in the RoI is always at full resolution. The eBits approach proposed here offers state of the art compression ratios (using less than 2.5 bits per new full resolution RoI triangle when the RoI has more than 2000 vertices to transmit the connectivity for the selective refinements) and fine-grain control (allowing the user to adjust the RoI by small increments). The effectiveness of eBits results from several novel ideas and novel variations of previous solutions. We represent the VERs using persistent labels so that they can be applied in different orders within a given LoD. The server maintains a shadow copy of the client's mesh. To avoid sending IDs identifying which vertices should be expanded, we either transmit, for each new vertex, a compact encoding of its death tag the LoD at which it will be expanded if it lies in the RoI or transmit vertex masks for the RoI and its neighboring vertices. We also propose a three-step simplification that reduces the overall transmission cost by increasing both the simplification effectiveness and the regularity of the valences in the resulting meshes. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Sati, Mukul; Rossignac, Jarek] Georgia Inst Technol, Sch Interact Comp, Atlanta, GA 30332 USA. [Lindstrom, Peter] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Sati, M (reprint author), Georgia Inst Technol, Sch Interact Comp, Atlanta, GA 30332 USA. EM mukul@gatech.edu; pl@llnl.gov; jarek@cc.gatech.edu OI Lindstrom, Peter/0000-0003-3817-4199 NR 31 TC 0 Z9 0 U1 3 U2 4 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0010-4485 EI 1879-2685 J9 COMPUT AIDED DESIGN JI Comput.-Aided Des. PD SEP PY 2016 VL 78 SI SI BP 168 EP 178 DI 10.1016/j.cad.2016.05.016 PG 11 WC Computer Science, Software Engineering SC Computer Science GA DQ3JN UT WOS:000379098700017 ER PT J AU Chatterjee, K Venkataraman, A Garbaciak, T Rotella, J Sangid, MD Beaudoin, AJ Kenesei, P Park, JS Pilchak, AL AF Chatterjee, K. Venkataraman, A. Garbaciak, T. Rotella, J. Sangid, M. D. Beaudoin, A. J. Kenesei, P. Park, J-S. Pilchak, A. L. TI Study of grain-level deformation and residual stresses in Ti-7Al under combined bending and tension using high energy diffraction microscopy (HEDM) SO INTERNATIONAL JOURNAL OF SOLIDS AND STRUCTURES LA English DT Article DE High energy diffraction microscopy; Ti-7Al alloy; Stress gradient; Stress triaxiality; Slip tendency ID X-RAY-DIFFRACTION; TI-6AL-4V TITANIUM-ALLOY; TI-AL ALLOYS; ELASTIC-CONSTANTS; CRYSTAL PLASTICITY; INDIVIDUAL GRAINS; FRACTURE LOCUS; STRAIN TENSOR; SINGLE-GRAIN; CREEP AB In-situ high energy diffraction microscopy (HEDM) experiments are carried out to analyze the state of combined bending and tension in a Ti-7Al alloy under room temperature creep. Grain-level elastic strain tensors are evaluated from HEDM data. Atomistic calculations are used to predict elastic constants of Ti-7Al, to be used in determination of stress from strain. The stress gradient and residual stresses are successfully determined, which allows the demarcation between macroqmicro-level residual stresses. A cluster of three neighboring grains are identified that highlight the variation of mean and effective stress between grains. Crystallographic orientations and slip characteristics are analyzed for the selected grains. It is inferred that the interfaces between loaded grains with markedly different stress triaxiality and slip tendency are potential spots for material damage. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Chatterjee, K.; Garbaciak, T.; Beaudoin, A. J.] Univ Illinois, Dept Mech Sci & Engn, 1206 W Green St, Urbana, IL 61801 USA. [Venkataraman, A.; Rotella, J.; Sangid, M. D.] Purdue Univ, Sch Aeronaut & Astronaut Engn, 701 W Stadium Ave, W Lafayette, IN 47907 USA. [Kenesei, P.; Park, J-S.] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Lemont, IL 60439 USA. [Pilchak, A. L.] US Air Force, Res Lab, Mat & Mfg Directorate AFRL RXCM, Wright Patterson AFB, OH 45433 USA. RP Beaudoin, AJ (reprint author), Univ Illinois, Dept Mech Sci & Engn, 1206 W Green St, Urbana, IL 61801 USA. EM abeaudoi@illinois.edu FU Air Force Office of Scientific Research [FA9550-14-1-0369, FA9550-14-1-0284]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A. Beaudoin and K. Chatterjee are supported by the Air Force Office of Scientific Research under Contract No. FA9550-14-1-0369. M. D. Sangid, A. Venkataraman, and J. Rotella acknowledge support from the Air Force Office of Scientific Research under Contract No. FA9550-14-1-0284. The use of Advance Photon Source is granted by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. We thank Drs. Paul A. Shade, Todd J. Turner, Michael Mills, and David Rugg for interesting conversations. NR 80 TC 1 Z9 1 U1 16 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0020-7683 EI 1879-2146 J9 INT J SOLIDS STRUCT JI Int. J. Solids Struct. PD SEP PY 2016 VL 94-95 BP 35 EP 49 DI 10.1016/j.ijsolstr.2016.05.010 PG 15 WC Mechanics SC Mechanics GA DQ5VE UT WOS:000379272500003 ER PT J AU Muransky, O Hamelin, CJ Hosseinzadeh, F Prime, MB AF Muransky, O. Hamelin, C. J. Hosseinzadeh, F. Prime, M. B. TI Mitigating cutting-induced plasticity in the contour method. Part 2: Numerical analysis SO INTERNATIONAL JOURNAL OF SOLIDS AND STRUCTURES LA English DT Article DE Residual stress; Contour method; Finite element modelling ID RESIDUAL-STRESS MEASUREMENT; FIELDS AB Cutting-induced plasticity can have a significant effect on the measurement accuracy of the contour method. The present study examines the benefit of a double-embedded cutting configuration that relies on self-restraint of the specimen, relative to conventional edge-crack cutting configurations. A series of finite element analyses are used to simulate the planar sectioning performed during double-embedded and conventional edge-crack contour cutting configurations. The results of numerical analyses are first compared to measured results to validate the cutting simulations. The simulations are then used to compare the efficacy of different cutting configurations by predicting the deviation of the residual stress profile from an original (pre-cutting) reference stress field, and the extent of cutting-induced plasticity. Comparisons reveal that while the double-embedded cutting configuration produces the most accurate residual stress measurements, the highest levels of plastic flow are generated in this process. This cutting-induced plastic deformation is, however, largely confined to small ligaments formed as a consequence of the sample sectioning process, and as such it does not significantly affect the back-calculated residual stress field. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Muransky, O.; Hamelin, C. J.] ANSTO, Inst Mat Engn, Lucas Heights, NSW, Australia. [Hosseinzadeh, F.] Open Univ, Mat Engn, Milton Keynes MK7 7AA, Bucks, England. [Prime, M. B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Muransky, O (reprint author), ANSTO, Inst Mat Engn, Lucas Heights, NSW, Australia. EM ondrej.muransky@ansto.gov.au OI Prime, Michael/0000-0002-4098-5620 FU NeT programme FX Residual stress measurements and weld simulations produced under the auspices of the NeT programme via Task Group 4 have significantly advanced best-practice guidelines for treatment of WRS and post-weld plastic strain, adding considerable value to the present work. The authors are also grateful for insightful discussions regarding computational weld mechanics with Prof. M.C. Smith (University of Manchester) and Dr. P.J. Bendeich (ANSTO). NR 26 TC 2 Z9 2 U1 2 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0020-7683 EI 1879-2146 J9 INT J SOLIDS STRUCT JI Int. J. Solids Struct. PD SEP PY 2016 VL 94-95 BP 254 EP 262 DI 10.1016/j.ijsolstr.2015.12.033 PG 9 WC Mechanics SC Mechanics GA DQ5VE UT WOS:000379272500020 ER PT J AU Chen, YC Manna, S Narayanan, B Wang, ZW Reimanis, IE Ciobanu, CV AF Chen, Yachao Manna, Sukriti Narayanan, Badri Wang, Zhongwu Reimanis, Ivar E. Ciobanu, Cristian V. TI Pressure-induced phase transformation in beta-eucryptite: An X-ray diffraction and density functional theory study SO SCRIPTA MATERIALIA LA English DT Article DE Density functional theory; XRD; Eucryptite; Ceramics ID TOTAL-ENERGY CALCULATIONS; EARTHS LOWER MANTLE; WAVE BASIS-SET; THERMAL-EXPANSION; IONIC-CONDUCTIVITY; CATHODE MATERIALS; LI-DIFFUSION; HIGH-QUARTZ; LIALSIO4; RUBY AB Certain alumino-silicates display exotic properties enabled by their framework structure made of corner-sharing tetrahedral rigid units. Using in situ diamond-anvil cell x-ray diffraction (XRD), we study the pressure-induced transformation of beta eucryptite, a prototypical alumino-silicate that undergoes a phase transformation at moderate pressures. The atomic structure and symmetry group of the new pressure-stabilized phase has not yet been reported. Based on density functional theory studies and Rietveld analysis of XRD patterns, we find that the new phase belongs to the Pna2(1) space group and report its atomic structure. Furthermore, we discover two other possible pressure-stabilized polymorphs, P1c1 and Pca2(1). (C) 2016 Elsevier Ltd. All rights reserved. C1 [Chen, Yachao; Narayanan, Badri; Reimanis, Ivar E.] Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. [Manna, Sukriti; Ciobanu, Cristian V.] Colorado Sch Mines, Dept Mech Engn, Golden, CO 80401 USA. [Wang, Zhongwu] Cornell Univ, Cornell High Energy Synchrotron Source, Ithaca, NY 14853 USA. [Narayanan, Badri] Argonne Natl Lab, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Reimanis, IE (reprint author), Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA.; Ciobanu, CV (reprint author), Colorado Sch Mines, Dept Mech Engn, Golden, CO 80401 USA. EM reimanis@mines.edu; cciobanu@mines.edu RI Ciobanu, Cristian/B-3580-2009 FU U.S. Department of Energy's Office of Basic Energy Sciences [DE-FG02-07ER46397]; NSF; NIH/NIGMS via NSF [DMR-1332208] FX We gratefully acknowledge the support of U.S. Department of Energy's Office of Basic Energy Sciences through grant no. DE-FG02-07ER46397. CHESS is supported by the NSF and NIH/NIGMS via NSF award DMR-1332208. NR 42 TC 0 Z9 0 U1 6 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD SEP PY 2016 VL 122 BP 64 EP 67 DI 10.1016/j.scriptamat.2016.05.005 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DQ1KG UT WOS:000378959300015 ER PT J AU McBriarty, ME Ellis, DE AF McBriarty, Martin E. Ellis, Donald E. TI Cation synergies affect ammonia adsorption over VOX and (V,W)O-X dispersed on alpha-Al2O3 (0001) and alpha-Fe2O3 (0001) SO SURFACE SCIENCE LA English DT Article DE Nitric oxide reduction; Vanadium oxide; Oxide support; Ammonia adsorption; Electronic structure; Density functional theory ID SELECTIVE CATALYTIC-REDUCTION; VANADIUM-OXIDE CATALYSTS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; BOND-VALENCE PARAMETERS; ATOMIC-SCALE VIEW; WAVE BASIS-SET; NITRIC-OXIDE; SCR REACTION; MECHANISTIC ASPECTS AB The catalytic behavior of oxide-supported metal oxide species depends on the nature of the support and the presence of co-catalysts. We use density functional theory (DFT) to explore the relationship between the structure and chemical behavior of vanadium oxide in light of its industrial use for the selective catalytic reduction of nitric oxide with ammonia (NO-SCR). The relative stabilities of dispersed VOX monomers, dimers, and long-chain oligomers on two model oxide support surfaces with similar structure but drastically different chemical behavior, alpha-Al2O3 (0001) and alpha-Fe2O3 (0001), are determined. The effect of added tungsten, known to promote NO-SCR, is also investigated on the relatively inert alpha-Al2O3 (0001) support. We find that the adsorption behavior of NH3, representing the first step of the NO-SCR reaction, depends strongly on the VOX local structure. Protonation of NH3 to NH4+ over surface hydroxyls is energetically favorable over VOX-WOX dimers and VOX oligomers, which are stabilized by the reducible alpha-Fe2O3 (0001) support. (C) 2016 Elsevier B.V. All rights reserved. C1 [McBriarty, Martin E.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ellis, Donald E.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Ellis, Donald E.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP McBriarty, ME (reprint author), Pacific Northwest Natl Lab, Richland, WA 99354 USA. EM mcbriarty@u.northwestern.edu OI McBriarty, Martin/0000-0002-7802-3267 FU National Science Foundation [DGE-0824162]; Institute for Catalysis in Energy Processes (U.S. Department of Energy (DOE)) [DE-FG02-03ER15457] FX M.E.M. was supported by a National Science Foundation Graduate Research Fellowship under Grant DGE-0824162. M.E.M. and D.E.E. were supported in part by the Institute for Catalysis in Energy Processes (U.S. Department of Energy (DOE) under Contract DE-FG02-03ER15457). Computational equipment support was provided by the Initiative for Sustainability and Energy at Northwestern University. Atomic structure and charge density plots were made using VESTA software [73]. NR 73 TC 0 Z9 0 U1 20 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD SEP PY 2016 VL 651 BP 41 EP 50 DI 10.1016/j.susc.2016.03.015 PG 10 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA DQ3MD UT WOS:000379105500007 ER PT J AU Eren, B Zherebetskyy, D Hao, YB Patera, LL Wang, LW Somorjai, GA Salmeron, M AF Eren, Baran Zherebetskyy, Danylo Hao, Yibo Patera, Laerte L. Wang, Lin-Wang Somorjai, Gabor A. Salmeron, Miquel TI One-dimensional nanoclustering of the Cu(100) surface under CO gas in the mbar pressure range SO SURFACE SCIENCE LA English DT Article DE Cu(100); Carbon monoxide; Nanoclustering; HPSTM; DFT ID SCANNING TUNNELING MICROSCOPE; RAY PHOTOELECTRON-SPECTROSCOPY; METHANOL SYNTHESIS; COPPER SURFACES; ADSORPTION; CATALYST; CHEMISTRY; OXIDATION; COVERAGE; CU(110) AB The bulk terminated Cu(100) surface becomes unstable in the presence of CO at room temperature when the pressure reaches the mbar range. Scanning tunneling microscopy images show that above 0.25 mbar the surface forms nanoclusters with CO attached to peripheral Cu atoms. At 20 mbar and above 3-atom wide one-dimensional nanoclusters parallel to < 001 > directions cover the surface, with CO on every Cu atom, increasing in density up to 115 mbar. Density functional theory explains the findings as a result of the detachment of Cu atoms from step edges caused by the stronger binding of CO relative to that on flat terraces. (C) 2016 Elsevier B.V. All rights reserved. C1 [Eren, Baran; Zherebetskyy, Danylo; Hao, Yibo; Patera, Laerte L.; Wang, Lin-Wang; Somorjai, Gabor A.; Salmeron, Miquel] Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Zherebetskyy, Danylo] Nanosys Inc, Milpitas, CA 95035 USA. [Patera, Laerte L.] CNR IOM, Lab TASC, Str Statale 14,Km 163-5, I-34149 Trieste, Italy. [Patera, Laerte L.] Univ Trieste, Dept Phys, Via A Valerio 2, I-34127 Trieste, Italy. [Patera, Laerte L.] Univ Trieste, CENMAT, Via A Valerio 2, I-34127 Trieste, Italy. [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Salmeron, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov RI Eren, Baran/A-9644-2013; OI Patera, Laerte/0000-0002-6214-5681 FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) through the Chemical and Mechanical Properties of Surfaces, Interfaces [DE-AC02-05CH11231, FWP KC3101]; "Organic/Inorganic Nanocomposite Materials" program; Office of Science of the U.S. DOE; Innovative and Novel Computational Impact on Theory and Experiment (INCITE) project FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) under contract no. DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces (FWP KC3101). The calculations by D.Z. and L.-W.W. were supported by the "Organic/Inorganic Nanocomposite Materials" program. It used resources of the National Energy Research Scientific Computing Center which is supported by the Office of Science of the U.S. DOE. The computation also used the resources of Oak Ridge Leadership Computing Facility (OLCF) with the computational time allocated by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) project. NR 33 TC 3 Z9 3 U1 15 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD SEP PY 2016 VL 651 BP 210 EP 214 DI 10.1016/j.susc.2016.04.016 PG 5 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA DQ3MD UT WOS:000379105500029 ER PT J AU Cho, H AF Cho, Herman TI Dependence of nuclear quadrupole resonance transitions on the electric field gradient asymmetry parameter for nuclides with half-integer spins SO ATOMIC DATA AND NUCLEAR DATA TABLES LA English DT Article DE NQR spectroscopy; Nuclear quadrupole moments; Electric field gradient; Electronic structure ID MAGNETIC-RESONANCE; SPECTRA; SOLIDS; CHEMISTRY; MOMENTS; ORBIT; NMR AB Allowed transition energies and eigenstate expansions have been calculated and tabulated in numerical form as functions of the electric field gradient asymmetry parameter for the zero field Hamiltonian of quadrupolar nuclides with I = 3/2, 5/2, 7/2, and 9/2. These results are essential to interpret nuclear quadrupole resonance (NQR) spectra and extract accurate values of the electric field gradient tensors. Applications of NQR methods to studies of electronic structure in heavy element systems are proposed. (C) 2016 Elsevier Inc. All rights reserved. C1 [Cho, Herman] Pacific NW Natl Lab, Phys & Computat Sci Directorate, POB 999, Richland, WA 99352 USA. RP Cho, H (reprint author), Pacific NW Natl Lab, Phys & Computat Sci Directorate, POB 999, Richland, WA 99352 USA. EM hm.cho@pnnl.gov FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Heavy Element Chemistry program FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences, Heavy Element Chemistry program. NR 27 TC 0 Z9 0 U1 8 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0092-640X EI 1090-2090 J9 ATOM DATA NUCL DATA JI Atom. Data Nucl. Data Tables PD SEP-NOV PY 2016 VL 111 BP 29 EP 40 DI 10.1016/j.adt.2016.02.003 PG 12 WC Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA DP7DQ UT WOS:000378659800002 ER PT J AU Chen, HL Meng, LY Chen, SH Jiao, Y Liu, YM AF Chen, Hailong Meng, Lingyi Chen, Shaohua Jiao, Yang Liu, Yongming TI Numerical investigation of microstructure effect on mechanical properties of bi-continuous and particulate reinforced composite materials SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Voxel-based analysis; Microstructure; Homogenization; Fracture; Composites ID PORE-SPACE RECONSTRUCTION; MULTIPLE-POINT STATISTICS; METAL-MATRIX COMPOSITES; HETEROGENEOUS MATERIALS; FRACTURE SIMULATION; 2D; ALGORITHM; MODELS; MEDIA AB In this paper, numerical simulations are proposed to investigate mechanical properties of bi-continuous and particulate reinforced composite materials using a non-local voxel-based discrete computational model. Special focus of this article is the effect of 3D microstructure and its heterogeneity on elastic deformation and fracture behaviors. First, a review on model formulation is presented. Model parameters are derived in terms of material constants using the concept of energy equivalency. Interface representation and numerical homogenization scheme are discussed. Following this, numerical investigations on the effects of interface properties and inclusion characteristics, i.e. the volume fraction and material constants, on homogenized elastic constants and fracture behaviors of statistically isotropic bi-phase composites are performed. The effective elastic constants predicted by the proposed model agree well with analytical results. Fracture simulation demonstrates good capability of the proposed model for the microstructure-sensitive failure analysis. Conclusions and future work are drawn based on the proposed study. (C) 2016 Elsevier B.V. All rights reserved. C1 [Chen, Hailong; Chen, Shaohua; Jiao, Yang; Liu, Yongming] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. [Meng, Lingyi] S China Univ Technol, Sch Civil Engn & Transportat, Guangzhou 510641, Guangdong, Peoples R China. [Chen, Hailong] Idaho Natl Lab, Fuels Modeling & Simulat, Idaho Falls, ID 83402 USA. RP Liu, YM (reprint author), Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. EM Yongming.Liu@asu.edu RI Chen, Hailong/C-7197-2017 OI Chen, Hailong/0000-0002-6564-7230 FU DARPA [N66001-14-1-4036] FX This work is partially supported by DARPA under Grant No. N66001-14-1-4036. NR 39 TC 1 Z9 1 U1 7 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD SEP PY 2016 VL 122 BP 288 EP 294 DI 10.1016/j.commatsci.2016.05.037 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA DP5DT UT WOS:000378516900031 ER PT J AU Ren, BY Zhong, DK Sun, YG Zhao, XH Zhang, QJ Liu, Y Jurow, M Sun, ML Zhang, ZS Zhao, Y AF Ren, Bao-Yi Zhong, Dao-Kun Sun, Ya-Guang Zhao, Xiang-Hua Zhang, Qi-Jian Liu, Yi Jurow, Matthew Sun, Ming-Li Zhang, Zhen-Song Zhao, Yi TI Quinolyl functionalized spiro[fluorene-9,9 '-xanthene] host materials with bipolar characteristics for green and red phosphorescent organic light-emitting diodes SO ORGANIC ELECTRONICS LA English DT Article DE PhOLEDs; Host materials; Spiro[fluorene-9,9 '-xanthene]; Quinoline; Substitution effect ID ACTIVATED DELAYED FLUORESCENCE; RIGID-ROD POLYQUINOLINES; HOLE-TRANSPORT MATERIAL; PEROVSKITE SOLAR-CELLS; HIGHLY EFFICIENT RED; INTERMOLECULAR PI-PI; ELECTROLUMINESCENT DEVICES; PHOSPHINE OXIDE; ELECTROPHOSPHORESCENT DEVICES; UNIVERSAL HOST AB Spiro[fluorene-9,9'-xanthene] (SFX) bipolar hosts bearing one, two and three quinolyl substituents, namely SFX-bPy, SFX-DbPy and SFX-TbPy, were designed and synthesized for phosphorescent organic light emitting diodes (PhOLEDs). The successive substitution of quinoline at 20, 2 and 70 positions of SFX results in reduced LUMO energy levels while leaving the HOMO energy levels nearly intact. The impact of quinoline substitution in these SFX-based hosts on PhOLED performance was investigated in detail through green and red model devices. For the green emitting devices, the device based on SFX-bPy host showed better performance (23.6 cd A(-1), 23.4 lm W-1, 6.3%) due to high triplet energy level (T-1) and balanced carriers-transporting ability. In contrast, for the red PhOLED devices, the device hosted by SFX-DbPy displayed higher performance (15.8 cd A(-1), 16.0 lm W-1, 9.1%), attributable to the well matched T-1 and separated frontier molecular orbitals. This work thus sheds light on the rational design of SFX-based bipolar hosts for more efficient PhOLEDs. (C) 2016 Elsevier B.V. All rights reserved. C1 [Ren, Bao-Yi; Zhong, Dao-Kun; Sun, Ya-Guang] Shenyang Univ Chem Technol, Coll Appl Chem, Key Lab Inorgan Mol Based Chem Liaoning Prov, Shenyang 110142, Peoples R China. [Zhao, Xiang-Hua] Xinyang Normal Univ, Coll Chem & Chem Engn, Xinyang 464000, Peoples R China. [Zhang, Qi-Jian; Liu, Yi; Jurow, Matthew] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. [Sun, Ming-Li] Northeast Forestry Univ, Coll Sci, Dept Chem, Harbin 150040, Peoples R China. [Zhang, Zhen-Song; Zhao, Yi] Jilin Univ, Coll Elect Sci & Engn, State Key Lab Integrated Optoelect, Changchun 130012, Peoples R China. RP Zhao, XH (reprint author), Xinyang Normal Univ, Coll Chem & Chem Engn, Xinyang 464000, Peoples R China.; Liu, Y (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA.; Sun, ML (reprint author), Northeast Forestry Univ, Coll Sci, Dept Chem, Harbin 150040, Peoples R China. EM 4773zxh@163.com; yliu@lbl.gov; sml98@163.com RI Liu, yi/A-3384-2008; OI Liu, yi/0000-0002-3954-6102; Sun, Yaguang/0000-0001-5850-0938 FU National Natural Scince Foundation of China [61405170]; Molecular Foundry, through Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Students Sustentation Fund of Xinyang Normal University [2014-DXS-136] FX We express our sincere gratitude to the Doctoral Research Foundation of Liaoning Province (20131091), National Natural Scince Foundation of China (grant no. 61405170) and Students Sustentation Fund of Xinyang Normal University (No. 2014-DXS-136). Y. L. acknowledges the support from the Molecular Foundry, a user facility supported through the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 57 TC 0 Z9 0 U1 30 U2 71 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1566-1199 EI 1878-5530 J9 ORG ELECTRON JI Org. Electron. PD SEP PY 2016 VL 36 BP 140 EP 147 DI 10.1016/j.orgel.2016.06.006 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DP5NO UT WOS:000378544500019 ER PT J AU Horowitz, KAW Fu, R Woodhouse, M AF Horowitz, Kelsey A. W. Fu, Ran Woodhouse, Michael TI An analysis of glass-glass CIGS manufacturing costs SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article DE CIGS; Photovoltaic; Co-evaporation; Selenization; Manufacturing cost analysis; LCOE ID CU(IN,GA)SE-2 SOLAR-CELLS; THICKNESS AB This article examines current cost drivers and potential avenues to reduced cost for monolithic, glass glass Cu(In,Ga)(Se,S)(2) (CIGS) modules by constructing a comprehensive bottom-up cost model. For a reference case where sputtering plus batch sulfurization after selenization (SAS) is employed, we compute a manufacturing cost of $69/m(2) if the modules are made in the United States at a 1 GW/year production volume. At 14% module efficiency, this corresponds to a manufacturing cost of $0.49/W-DC and a minimum sustainable price (MSP) of $0.67/W-DC. We estimate that MSP could vary within 20% of this value given the range of quoted input prices, and existing variations in module design, manufacturing processes, and manufacturing location. Potential for reduction in manufacturing costs to below $0.40/W-DC may be possible if average production module efficiencies can be increased above 17% without increasing $/m(2) costs; even lower costs could be achieved if $/m(2) costs could be reduced, particularly via innovations in the CIGS deposition process or balance-of-module elements. We present the impact on cost of regional factors, CIGS deposition method, device design, and price fluctuations. One metric of competitiveness-levelized cost of energy (LCOE) - is also assessed for several U.S. locations and compared to that of standard multi-crystalline silicon (m(c-Si)) and cadmium telluride (CdTe). (C) 2016 Elsevier B.V. All rights reserved. C1 [Horowitz, Kelsey A. W.; Fu, Ran; Woodhouse, Michael] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Horowitz, KAW (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Kelsey.Horowitz@nrel.gov FU Solar Energy Technologies Office of the U.S. Department of Energy [DE-AC36-08GO28308] FX The authors thank the Solar Energy Technologies Office of the U.S. Department of Energy for funding this work through Contract no. DE-AC36-08GO28308. We thank Lorelle Mansfield, Kannan Ramanathan, Miguel Contreras, Karlynn Cory, and Donald Chung for insightful discussion. Finally, we would like to acknowledge the significant contribution from all our industry collaborators, who provided data and feedback that made this study possible. NR 29 TC 1 Z9 1 U1 21 U2 40 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD SEP PY 2016 VL 154 BP 1 EP 10 DI 10.1016/j.solmat.2016.04.029 PG 10 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DP5WT UT WOS:000378569600001 ER PT J AU O'Brien, TA Kashinath, K Cavanaugh, NR Collins, WD O'Brien, JP AF O'Brien, Travis A. Kashinath, Karthik Cavanaugh, Nicholas R. Collins, William D. O'Brien, John P. TI A fast and objective multidimensional kernel density estimation method: fastKDE SO COMPUTATIONAL STATISTICS & DATA ANALYSIS LA English DT Article DE Empirical characteristic function; ECF; Kernel density estimation; Histogram; Nonuniform FFT; NuFFT; Multidimensional; KDE AB Numerous facets of scientific research implicitly or explicitly call for the estimation of probability densities. Histograms and kernel density estimates (KDEs) are two commonly used techniques for estimating such information, with the KDE generally providing a higher fidelity representation of the probability density function (PDF). Both methods require specification of either a bin width or a kernel bandwidth. While techniques exist for choosing the kernel bandwidth optimally and objectively, they are computationally intensive, since they require repeated calculation of the ROE. A solution for objectively and optimally choosing both the kernel shape and width has recently been developed by Bernacchia and Pigolotti (2011). While this solution theoretically applies to multidimensional KDEs, it has not been clear how to practically do so. A method for practically extending the Bernacchia-Pigolotti KDE to multidimensions is introduced. This multidimensional extension is combined with a recently-developed computational improvement to their method that makes it computationally efficient: a 2D KDE on 10(5) samples only takes 1 s on a modern workstation. This fast and objective KDE method, called the fastKDE method, retains the excellent statistical convergence properties that have been demonstrated for univariate samples. The fastKDE method exhibits statistical accuracy that is comparable to state-of-the-science KDE methods publicly available in R, and it produces kernel density estimates several orders of magnitude faster. The fastKDE method does an excellent job of encoding covariance information for bivariate samples. This property allows for direct calculation of conditional PDFs with fastKDE. It is demonstrated how this capability might be leveraged for detecting non-trivial relationships between quantities in physical systems, such as transitional behavior. (C) 2016 The Authors and Lawrence Berkeley National Laboratory. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [O'Brien, Travis A.; Kashinath, Karthik; Cavanaugh, Nicholas R.; Collins, William D.; O'Brien, John P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [O'Brien, Travis A.] Univ Calif Davis, Davis, CA 95616 USA. [Collins, William D.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [O'Brien, John P.] Univ Calif Santa Cruz, Santa Cruz, CA 95064 USA. RP O'Brien, TA (reprint author), 1 Cyclotron Rd,MS74R-316C, Berkeley, CA USA. EM TAOBrien@lbl.gov RI Collins, William/J-3147-2014; O'Brien, Travis/M-5250-2013; Kashinath, Karthik/B-2265-2015; OI Collins, William/0000-0002-4463-9848; O'Brien, Travis/0000-0002-6643-1175; Kashinath, Karthik/0000-0002-9311-5215; Cavanaugh, Nicholas/0000-0002-7638-4501 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy Regional and Global Climate Modeling Program (RGCM) [ESD13052]; National Energy Research Scientific Computing Center (NERSC) [m1949, m1517]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank two anonymous reviewers whose comments greatly helped improve the quality of the manuscript. The authors would also like to thank Dr. Chris Paciorek of UCB for helpful comments in the framing of the manuscript. This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy Regional and Global Climate Modeling Program (RGCM) (ESD13052) and used resources of the National Energy Research Scientific Computing Center (NERSC) (m1949 and m1517), also supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 23 TC 1 Z9 1 U1 3 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-9473 EI 1872-7352 J9 COMPUT STAT DATA AN JI Comput. Stat. Data Anal. PD SEP PY 2016 VL 101 BP 148 EP 160 DI 10.1016/j.csda.2016.02.014 PG 13 WC Computer Science, Interdisciplinary Applications; Statistics & Probability SC Computer Science; Mathematics GA DP4CY UT WOS:000378444200012 ER PT J AU Linley, TJ Krogstad, EJ Nims, MK Langshaw, RB AF Linley, Timothy J. Krogstad, Eirik J. Nims, Megan K. Langshaw, Russell B. TI Geochemical signatures in fin rays provide a nonlethal method to distinguish the natal rearing streams of endangered juvenile Chinook Salmon Oncorhynchus tshawytscha in the Wenatchee River, Washington SO FISHERIES RESEARCH LA English DT Article DE Fin ray geochemistry ID INDUCTIVELY-COUPLED PLASMA; SPOT LEIOSTOMUS-XANTHURUS; WESTSLOPE CUTTHROAT TROUT; STABLE-ISOTOPE ANALYSIS; UPPER COLUMBIA-RIVER; OTOLITH CHEMISTRY; LIFE-HISTORY; WATER CHEMISTRY; FRESH-WATER; RAINBOW-TROUT AB Rebuilding fish populations that have undergone a major decline is a challenging task that can be made more complicated when estimates of abundance obtained from physical tags are biased or imprecise. Abundance estimates based on natural tags where each fish in the population is marked can help address these problems, but generally requires that the samples be obtained in a nonlethal manner. We evaluated the potential of using geochemical signatures in fin rays as a nonlethal method to determine the natal tributaries of endangered juvenile spring Chinook Salmon in the Wenatchee River, Washington. Archived samples of anal fin clips collected from yearling smolt in 2009, 2010 and 2011 were analyzed for Ba/Ca, Mn/Ba, Mg/Ca, Sr/Ca, Zn/Ca and Sr-87/Sr-86 by inductively coupled plasma mass spectrometry. Water samples collected from these same streams in 2012 were also quantified for geochemical composition. Fin ray and water Ba/Ca, Sr/Ca, and Sr-87/Sr-86 were highly correlated despite the samples having been collected in different years. Fin ray Ba/Ca, Mg/Ca, Sr/Ca, Zn/Ca and Sr-87/Sr-86 ratios differed significantly among the natal streams, but also among years within streams. A linear discriminant model that included Ba/Ca, Mg/Ca, Sr/Ca, and Sr-87/Sr-86 correctly classified 95% of the salmon to their natal stream. Our results suggest that fin ray geochemistry may provide an effective, nonlethal method to identify mixtures of Wenatchee River spring Chinook Salmon for recovery efforts when these involve the capture of juvenile fish to estimate population abundance. (C) 2016 Elsevier B.V. All rights reserved. C1 [Linley, Timothy J.; Krogstad, Eirik J.; Nims, Megan K.] Pacific NW Natl Lab, Earth Syst Sci Div, Richland, WA USA. [Langshaw, Russell B.] Publ Util Dist Grant Cty 2, Washington, DC USA. [Langshaw, Russell B.] Ecosyst Insights, Mesa, AZ USA. RP Linley, TJ (reprint author), Pacific NW Natl Lab, Earth Syst Sci Div, Richland, WA USA. EM Timothy.Linley@pnnl.gov; Russell@ecoinsights.us FU Priest Rapids Coordinating Committee (PRCC) No-Net Impact Fund FX We thank Liz Alexander and Matt Newburn of the Environmental and Molecular Sciences Laboratory (EMSL) for their support and assistance with the ICP-MS analyses, Valerie Cullinan (PNNL) for statistical help, and the Washington Department of Fish and Wildlife (Andrew Murdoch, Mike Hughes) and the NOAA Northwest Fisheries Science Center (Mike Ford, Sharon Howard) for providing the fin-ray samples. Additional thanks to Jill Janak and Kathleen Carter from PNNL for their help in preparing the manuscript, and for the constructive comments from two anonymous reviewers. Funding for this study was provided by the Priest Rapids Coordinating Committee (PRCC) No-Net Impact Fund. The PRCC includes representatives NOAA Fisheries, U.S. Fish & Wildlife Service, Washington Department of Fish & Wildlife, Colville Confederated Tribes, Yakama Nation, Confederated Tribes of the Umatilla Reservation and Grant County Public Utility District. NR 99 TC 0 Z9 0 U1 5 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0165-7836 EI 1872-6763 J9 FISH RES JI Fish Res. PD SEP PY 2016 VL 181 BP 234 EP 246 DI 10.1016/j.fishres.2016.04.004 PG 13 WC Fisheries SC Fisheries GA DP0LS UT WOS:000378181900023 ER PT J AU Guo, XY Hu, B Wei, CD Sun, JG Jung, YG Li, L Knapp, J Zhang, J AF Guo, Xingye Hu, Bin Wei, Changdong Sun, Jiangang Jung, Yeon-Gil Li, Li Knapp, James Zhang, Jing TI Image-based multi-scale simulation and experimental validation of thermal conductivity of lanthanum zirconate SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Article DE Lanthanum zirconate; Thermal conductivity; Molecular dynamics; Finite element; Microstructure; Imaging; Flash laser technique; Pulsed thermal imaging-multilayer analysis ID NONEQUILIBRIUM MOLECULAR-DYNAMICS; BARRIER COATINGS; PORES AB Lanthanum zirconate (La2Zr2O7) is a promising candidate material for thermal barrier coating (TBC) applications due to its low thermal conductivity and high-temperature phase stability. In this work, a novel image-based multi-scale simulation framework combining molecular dynamics (MD) and finite element (FE) calculations is proposed to study the thermal conductivity of La2Zr2O7 coatings. Since there is no experimental data of single crystal La2Zr2O7 thermal conductivity, a reverse non-equilibrium molecular dynamics (reverse NEMD) approach is first employed to compute the temperature-dependent thermal conductivity of single crystal La2Zr2O7. The single crystal data is then passed to a FE model which takes into account of realistic thermal barrier coating microstructures. The predicted thermal conductivities from the FE model are in good agreement with experimental validations using both flash laser technique and pulsed thermal imaging-multilayer analysis. The framework proposed in this work provides a powerful tool for future design of advanced coating systems. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Guo, Xingye; Zhang, Jing] Indiana Univ Purdue Univ, Dept Mech Engn, Indianapolis, IN 46202 USA. [Hu, Bin] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. [Wei, Changdong] Ohio State Univ, Dept Mat Sci & Engn, 116 W 19Th Ave, Columbus, OH 43210 USA. [Sun, Jiangang] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Jung, Yeon-Gil] Changwon Natl Univ, Sch Nano & Adv Mat Engn, Chang Won 641773, Gyeongnam, South Korea. [Li, Li; Knapp, James] Praxair Surface Technol, Indianapolis, IN 46222 USA. RP Zhang, J (reprint author), Indiana Univ Purdue Univ, Dept Mech Engn, Indianapolis, IN 46202 USA. EM jz29@iupui.edu OI Zhang, Jing/0000-0002-8200-5117 FU U.S. Department of Energy [DE-FE0008868]; Indiana University Research Support Funds Grant (RSFG); International Research Development Fund (IRDF); National Research Foundation of Korea (NRF) grant - Korean Government (MEST) [2011-0030058]; Changwon National University; U.S. Department of Energy, Office of Fossil Energy, Crosscutting Research Program; Novel Functionally Graded Thermal Barrier Coatings in Coal-fired Power Plant Turbines FX J.Z. acknowledges the financial support provided by the U.S. Department of Energy (Award Number: DE-FE0008868; Project Title: Novel Functionally Graded Thermal Barrier Coatings in Coal-fired Power Plant Turbines; Program Manager: Richard Dunst) and Indiana University Research Support Funds Grant (RSFG) and International Research Development Fund (IRDF). Y.J. acknowledges the financial support provided by a National Research Foundation of Korea (NRF) grant funded by the Korean Government (MEST) (2011-0030058), and by Changwon National University in 2015-2016. J.S. acknowledges the support provided by the U.S. Department of Energy, Office of Fossil Energy, Crosscutting Research Program. NR 31 TC 1 Z9 1 U1 9 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD SEP PY 2016 VL 100 BP 34 EP 38 DI 10.1016/j.ijheatmasstransfer.2016.04.067 PG 5 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA DP2ZI UT WOS:000378361700004 ER PT J AU Forsberg, U Rudolph, D Andersson, LL Di Nitto, A Dullmann, CE Fahlander, C Gates, JM Golubev, P Gregorich, KE Gross, CJ Herzberg, RD Hessberger, FP Khuyagbaatar, J Kratz, JV Rykaczewski, K Sarmiento, LG Schadel, M Yakushev, A Aberg, S Ackermann, D Block, M Brand, H Carlsson, BG Cox, D Derkx, X Dobaczewski, J Eberhardt, K Even, J Gerl, J Jager, E Kindler, B Krier, J Kojouharov, I Kurz, N Lommel, B Mistry, A Mokry, C Nazarewicz, W Nitsche, H Omtvedt, JP Papadakis, P Ragnarsson, I Runke, J Schaffner, H Schausten, B Shi, Y Thorle-Pospiech, P Torres, T Traut, T Trautmann, N Tuerler, A Ward, A Ward, DE Wiehl, N AF Forsberg, U. Rudolph, D. Andersson, L. -L. Di Nitto, A. Duellmann, Ch. E. Fahlander, C. Gates, J. M. Golubev, P. Gregorich, K. E. Gross, C. J. Herzberg, R. -D. Hessberger, F. P. Khuyagbaatar, J. Kratz, J. V. Rykaczewski, K. Sarmiento, L. G. Schaedel, M. Yakushev, A. Aberg, S. Ackermann, D. Block, M. Brand, H. Carlsson, B. G. Cox, D. Derkx, X. Dobaczewski, J. Eberhardt, K. Even, J. Gerl, J. Jaeger, E. Kindler, B. Krier, J. Kojouharov, I. Kurz, N. Lommel, B. Mistry, A. Mokry, C. Nazarewicz, W. Nitsche, H. Omtvedt, J. P. Papadakis, P. Ragnarsson, I. Runke, J. Schaffner, H. Schausten, B. Shi, Yue Thoerle-Pospiech, P. Torres, T. Traut, T. Trautmann, N. Tuerler, A. Ward, A. Ward, D. E. Wiehl, N. TI Recoil-alpha-fission and recoil-alpha-alpha-fission events observed in the reaction Ca-48+Am-243 SO NUCLEAR PHYSICS A LA English DT Article DE Superheavy elements; Element 115; Uup; alpha decay; Spontaneous fission ID 115 DECAY CHAINS; SUPERHEAVY ELEMENTS; HEAVIEST ELEMENTS; NUCLEI; TASCA; HEAVY; SPECTROSCOPY; SIMULATION; SEPARATOR; CHEMISTRY AB Products of the fusion-evaporation reaction Ca-48 + Am-243 were studied with the TASISpec set-up at the gas-filled separator TASCA at the GSI Helmholtzzentrum fur Schwerionenforschung, Darmstadt, Germany. Amongst the detected thirty correlated alpha-decay chains associated With the production of element Z = 115, two recoil-alpha-fission and five recoil-alpha-alpha-fission events were observed. The latter five chains are similar to four such events reported from experiments performed at the Dubna gas-filled separator, and three such events reported from an experiment at the Berkeley gas-filled separator. The four chains observed at the Dubna gas-filled separator were assigned to start from the 2n-evaporation channel (289)115 due to the fact that these recoil-alpha-alpha-fission events were observed only at low excitation energies. Contrary to this interpretation, we suggest that some of these recoil-alpha-alpha-fission decay chains, as well as some of the recoil-alpha-alpha-fission and recoil-alpha-fission decay chains reported from Berkeley and in this article, start from the 3n-evaporation channel (288)115. (C) 2016 Elsevier B.V. All rights reserved. C1 [Forsberg, U.; Rudolph, D.; Fahlander, C.; Golubev, P.; Sarmiento, L. G.; Aberg, S.; Carlsson, B. G.; Ragnarsson, I.; Ward, D. E.] Lund Univ, S-22100 Lund, Sweden. [Andersson, L. -L.; Duellmann, Ch. E.; Hessberger, F. P.; Khuyagbaatar, J.; Block, M.; Derkx, X.; Eberhardt, K.; Even, J.; Mistry, A.; Mokry, C.; Thoerle-Pospiech, P.; Wiehl, N.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Di Nitto, A.; Duellmann, Ch. E.; Kratz, J. V.; Block, M.; Derkx, X.; Eberhardt, K.; Mokry, C.; Thoerle-Pospiech, P.; Traut, T.; Trautmann, N.; Wiehl, N.] Johannes Gutenberg Univ Mainz, D-55099 Mainz, Germany. [Duellmann, Ch. E.; Hessberger, F. P.; Schaedel, M.; Yakushev, A.; Ackermann, D.; Block, M.; Brand, H.; Gerl, J.; Jaeger, E.; Kindler, B.; Krier, J.; Kojouharov, I.; Kurz, N.; Lommel, B.; Runke, J.; Schaffner, H.; Schausten, B.; Torres, T.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Gates, J. M.; Gregorich, K. E.; Nitsche, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gross, C. J.; Rykaczewski, K.; Nazarewicz, W.; Shi, Yue] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Herzberg, R. -D.; Cox, D.; Mistry, A.; Papadakis, P.; Ward, A.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Schaedel, M.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Dobaczewski, J.; Nazarewicz, W.] Univ Warsaw, PL-00681 Warsaw, Poland. [Dobaczewski, J.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Nazarewicz, W.; Shi, Yue] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Nazarewicz, W.; Shi, Yue] Michigan State Univ, NSCL FRIB Lab, E Lansing, MI 48824 USA. [Omtvedt, J. P.] Univ Oslo, N-0315 Oslo, Norway. [Tuerler, A.] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Tuerler, A.] Univ Bern, CH-5232 Villigen, Switzerland. [Even, J.] Univ Groningen, KVI Ctr Adv Radiat Technol, NL-9747 AA Groningen, Netherlands. [Papadakis, P.] Univ Jyvaskyla, Dept Phys, FIN-40014 Jyvaskyla, Finland. RP Forsberg, U (reprint author), Lund Univ, S-22100 Lund, Sweden. EM ulrika.forsberg@nuclear.lu.se RI Block, Michael/I-2782-2015; Even, Julia/K-1186-2016; Rudolph, Dirk/D-4259-2009; Turler, Andreas/D-3913-2014 OI Block, Michael/0000-0001-9282-8347; Even, Julia/0000-0002-6314-9094; Rudolph, Dirk/0000-0003-1199-3055; Turler, Andreas/0000-0002-4274-1056 FU European Community FP7 - Capacities ENSAR [262010]; Royal Physiographic Society in Lund; Euroball Owners Committee; Swedish Research Council; German BMBF; U.S. Department of Energy, Office of Science (Stewardship Science Academic Alliances program) [DOE-DE-NA0002574]; UK Science and Technology Facilities Council; U.S. Department of Energy, Office of Science (NUCLEI SciDAC-3 Collaboration) [DE-SC0008511] FX The authors would like to thank the ion-source and the accelerator staff at GSI. This work is supported by the European Community FP7 - Capacities ENSAR No. 262010, the Royal Physiographic Society in Lund, the Euroball Owners Committee, the Swedish Research Council, the German BMBF, the U.S. Department of Energy, Office of Science, under Award Numbers DOE-DE-NA0002574 (the Stewardship Science Academic Alliances program) and DE-SC0008511 (NUCLEI SciDAC-3 Collaboration), and the UK Science and Technology Facilities Council. NR 56 TC 10 Z9 10 U1 9 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD SEP PY 2016 VL 953 BP 117 EP 138 DI 10.1016/j.nuclphysa.2016.04.025 PG 22 WC Physics, Nuclear SC Physics GA DP4IX UT WOS:000378460700007 ER PT J AU Zhao, L Shaffer, F Robinson, B King, T D'Ambrose, C Pan, Z Gao, F Miller, RS Conmy, RN Boufadel, MC AF Zhao, Lin Shaffer, Franklin Robinson, Brian King, Thomas D'Ambrose, Christopher Pan, Zhong Gao, Feng Miller, Richard S. Conmy, Robyn N. Boufadel, Michel C. TI Underwater oil jet: Hydrodynamics and droplet size distribution SO CHEMICAL ENGINEERING JOURNAL LA English DT Article DE Subsurface oil release; Oil spill; Large scale experiment; Plume trajectory; Droplet size distribution; Ohmsett wave tank ID WATER-HORIZON OIL; GAS BLOWOUTS; BUOYANT JETS; SUBSEA OIL; CRUDE-OIL; FLOW-RATE; MODEL; BREAKUP; SIMULATION; ATOMIZATION AB We conducted a large scale experiment of underwater oil release of 6.3 L/s through a 25.4 mm (one inch) horizontal pipe. Detailed measurements of plume trajectory, velocity, oil droplet size distribution, and oil holdup were obtained. The obtained experimental data were used for the validation of the models JETLAG and VDROP-J. Key findings include: (1) formation of two plumes, one due to momentum and subsequently plume buoyancy, and another due mostly to the buoyancy of individual oil droplets that separate upward from the first plume; (2) modeling results indicated that the traditional miscible plume models matched the momentum and buoyancy plume, but were not able to simulate the upward motion plume induced by individual oil droplets; (3) high resolution images in the jet primary breakup region showed the formation of ligaments and drops in a process known as "primary breakup". These threads re-entered the plume to re-break in a process known as "secondary breakup"; (4) the plume velocity was highly heterogeneous with regions of high velocity surrounded by stagnant regions for various durations. The results from this study revealed that the primary breakup is a key factor for quantifying the droplet size distribution which plays a crucial role in determining the ultimate fate and transport of the released oil in the marine environment. The observed spatial heterogeneity in the oil plume implies that the effectiveness of applied dispersants may vary greatly when applying directly in the discharged oil flow. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zhao, Lin; D'Ambrose, Christopher; Pan, Zhong; Gao, Feng; Boufadel, Michel C.] New Jersey Inst Technol, Dept Civil & Environm Engn, Ctr Nat Resources Dev & Protect, Newark, NJ 07102 USA. [Shaffer, Franklin] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Robinson, Brian; King, Thomas] Bedford Inst Oceanog, Dept Fisheries & Oceans, Dartmouth, NS, Canada. [Miller, Richard S.] Clemson Univ, Dept Mech Engn, Clemson, SC 29634 USA. [Conmy, Robyn N.] US EPA, Natl Risk Management Res Lab, Off Res & Dev, Cincinnati, OH 45268 USA. RP Boufadel, MC (reprint author), New Jersey Inst Technol, Dept Civil & Environm Engn, Ctr Nat Resources Dev & Protect, Newark, NJ 07102 USA. EM boufadel@gmail.com FU Bureau of Safety and Environmental Enforcement [1027]; Department of Fisheries and Ocean Canada (DFO) [F5211-130060]; Gulf of Mexico Research Initiative through the Consortium DROPPS II FX This research was made possible through funding from the Bureau of Safety and Environmental Enforcement, Project # 1027 (2014); the Department of Fisheries and Ocean Canada (DFO), Contract No. F5211-130060; and the Gulf of Mexico Research Initiative through the Consortium DROPPS II. Data are publicly available through the Gulf of Mexico Research Initiative Information & Data Cooperative (GRIIDC) at https://data.gulfresearchinitiative.org (doi:10.7266/N7D798DN). However, no endorsement of these sponsors is implied. NR 35 TC 1 Z9 1 U1 14 U2 58 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 1385-8947 EI 1873-3212 J9 CHEM ENG J JI Chem. Eng. J. PD SEP 1 PY 2016 VL 299 BP 292 EP 303 DI 10.1016/j.cej.2016.04.061 PG 12 WC Engineering, Environmental; Engineering, Chemical SC Engineering GA DO5ON UT WOS:000377832500035 ER PT J AU Movshovitz, N Nimmo, F Korycansky, DG Asphaug, E Owen, JM AF Movshovitz, N. Nimmo, F. Korycansky, D. G. Asphaug, E. Owen, J. M. TI Impact disruption of gravity-dominated bodies: New simulation data and scaling SO ICARUS LA English DT Article DE Collisional physics; Planetesimals; Planetary formation ID LATE HEAVY BOMBARDMENT; OUTER SOLAR-SYSTEM; CATASTROPHIC DISRUPTION; NUMERICAL SIMULATIONS; CRATERING RATES; POSSIBLE ORIGIN; GIANT PLANETS; LATE-STAGE; COLLISIONS; SATELLITES AB We present results from a suite of 169 hydrocode simulations of collisions between planetary bodies with radii from 100 to 1000 km. The simulation data are used to derive a simple scaling law for the threshold for catastrophic disruption, defined as a collision that leads to half the total colliding mass escaping the system post impact For a target radius 100 <= R-T <= 1000km and a mass M-T and a projectile radius r(p) <= R-T and mass m(p) we find that a head-on impact with velocity magnitude v is catastrophic if the kinetic energy of the system in the center of mass frame, K = 0.5M(T)m(p)v(2)/(M-T + m(p)), exceeds a threshold value K* that is a few times U = (3/5)GM(T)(2)/R-T (3/5)Gm(p)(2)/r(p) GM(T)m(p)(R-T r(p)), the gravitational binding energy of the system at the moment of impact; G is the gravitational constant. In all head-on collision runs we find K* = (5.5 +/- 2.9)U. Oblique impacts are catastrophic when the fraction of kinetic energy contained in the volume of the projectile intersecting the target during impact exceeds similar to 2K* for 30 degrees impacts and similar to 3.5K* for 45 degrees impacts. We compare predictions made with this scaling to those made with existing scaling laws in the literature extrapolated from numerical studies on smaller targets. We find significant divergence between predictions where in general our results suggest a lower threshold for disruption except for highly oblique impacts with r(p) << R-T. This has implications for the efficiency of collisional grinding in the asteroid belt (Morbidelli et al., [2009] Icarus, 204, 558-573), Kuiper belt (Greenstreet et al., [2015] Icarus, 258, 267-288), and early Solar System accretion (Chambers [2013], Icarus, 224, 43-56). (C) 2016 Elsevier Inc. All rights reserved. C1 [Movshovitz, N.; Nimmo, F.; Korycansky, D. G.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. [Asphaug, E.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA. [Owen, J. M.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Movshovitz, N (reprint author), Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95064 USA. EM nmovshov@ucsc.edu OI Movshovitz, Naor/0000-0001-5583-0042 FU NASA PGG grant [NNX13AR66G]; NASA Origins grant [NNX11AK60G-002] FX We wish to thank our funding sources for this project. Research by N.M., D.G.K., and E.A. was supported by NASA PG&G grant NNX13AR66G. Research by F.N. was supported by NASA Origins grant NNX11AK60G-002. NR 41 TC 1 Z9 1 U1 2 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD SEP 1 PY 2016 VL 275 BP 85 EP 96 DI 10.1016/j.icarus.2016.04.018 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DO8FB UT WOS:000378016900006 ER PT J AU Nettelmann, N Wang, K Fortney, JJ Hamel, S Yellamilli, S Bethkenhagen, M Redmer, R AF Nettelmann, N. Wang, K. Fortney, J. J. Hamel, S. Yellamilli, S. Bethkenhagen, M. Redmer, R. TI Uranus evolution models with simple thermal boundary layers SO ICARUS LA English DT Article DE Uranus; Neptune; Planetary Evolution ID GIANT PLANETS; INTERIOR MODELS; ENERGY-BALANCE; NEPTUNE; JUPITER; ATMOSPHERES; CONVECTION; SATURN; WATER; MASS AB The strikingly low luminosity of Uranus (T-eff similar or equal to T-eq) constitutes a long-standing challenge to our understanding of Ice Giant planets. Here we present the first Uranus structure and evolution models that are constructed to agree with both the observed low luminosity and the gravity field data. Our models make use of modern ab initio equations of state at high pressures for the icy components water, methane, and ammonia. Proceeding step by step, we confirm that adiabatic models yield cooling times that are too long, even when uncertainties in the ice:rock ratio (I:R) are taken into account. We then argue that the transition between the ice/rock-rich interior and the HA-le-rich outer envelope should be stably stratified. Therefore, we introduce a simple thermal boundary and adjust it to reproduce the low luminosity. Due to this thermal boundary, the deep interior of the Uranus models are up to 2-3 warmer than adiabatic models, necessitating the presence of rocks in the deep interior with a possible I:R of 1 x solar. Finally, we allow for an equilibrium evolution (T-eff similar or equal to T-eq) that begun prior to the present day, which would therefore no longer require the current era to be a "special time" in Uranus' evolution. In this scenario, the thermal boundary leads to more rapid cooling of the outer envelope. When T-eff similar or equal to T-eq is reached, a shallow, subadiabatic zone in the atmosphere begins to develop. Its depth is adjusted to meet the luminosity constraint. This work provides a simple foundation for future Ice Giant structure and evolution models, that can be improved by properly treating the heat and particle fluxes in the diffusive zones. (C) 2016 Elsevier Inc. All rights reserved. C1 [Nettelmann, N.; Fortney, J. J.] Univ Rostock, Inst Phys, Albert Einstein Str 23, D-18051 Rostock, Germany. [Hamel, S.; Bethkenhagen, M.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Nettelmann, N.; Bethkenhagen, M.; Redmer, R.] Univ Calif Santa Cruz, Dept Astron & Astrophys, 1156 High St, Santa Cruz, CA 95064 USA. [Wang, K.] Castilleja High Sch, Palo Alto, CA USA. [Yellamilli, S.] Saratoga High Sch, Saratoga, CA USA. [Yellamilli, S.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Wang, K.; Yellamilli, S.] UCSC 2014, Sci Internship Program, Santa Cruz, CA USA. RP Nettelmann, N (reprint author), Univ Rostock, Inst Phys, Albert Einstein Str 23, D-18051 Rostock, Germany. EM nadine.nettelmann@uni-rostock.de OI Yellamilli, Shivaram/0000-0001-9209-4830 FU NASA [NNH12AU441, NNX11AJ40G-001]; German Science Foundation (DFG) [SFB 652]; NSF [AST-1010017] FX We thank the two anonymous referees for constructive comments. NN thanks R. Helled and M. Podolak for interesting conversations, and participants of the Workshop on Ice Giant Planets 2014 in Laurel, MD, for fruitful discussions. We gratefully acknowledge the funding support from NASA under Contract No. NNH12AU441. MB and RR acknowledge support from the German Science Foundation (DFG) via SFB 652 and the computation time provided by the North-German Supercomputing Alliance (HLRN) and the ITMZ of the University of Rostock. JJF acknowledges support from NSF grant AST-1010017 and NASA grant NNX11AJ40G-001. NR 60 TC 0 Z9 0 U1 6 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD SEP 1 PY 2016 VL 275 BP 107 EP 116 DI 10.1016/j.icarus.2016.04.008 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DO8FB UT WOS:000378016900008 ER PT J AU Makarova, OV Adams, DL Divan, R Rosenmann, D Zhu, PX Li, SH Amstutz, P Tang, CM AF Makarova, Olga V. Adams, Daniel L. Divan, Ralu Rosenmann, Daniel Zhu, Peixuan Li, Shuhong Amstutz, Platte Tang, Cha-Mei TI Polymer microfilters with nanostructured surfaces for the culture of circulating cancer cells SO MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS LA English DT Article DE Tumor cell culture; Structured culture; RIE treated polymer; Nanostructure; Surface topography ID TUMOR-CELLS; ALUMINUM-OXIDE; PRECISION MICROFILTERS; EFFICIENT CAPTURE; ANODIC ALUMINA; FABRICATION; CARCINOMA; ARRAYS; DEVICE; MICRO AB There is a critical need to improve the accuracy of drug screening and testing through the development of in vitro culture systems that more effectively mimic the in vivo environment. Surface topographical features on the nano scale level, in short nanotopography, effect the cell growth patterns, and hence affect cell function in culture. We report the preliminary results on the fabrication, and subsequent cellular growth, of nanoscale surface topography on polymer microfilters using cell lines as a precursor to circulating tumor cells (CTCs). To create various nanoscale features on the microfilter surface, we used reactive ion etching (RIE) with and without an etching mask. An anodized aluminum oxide (AAO) membrane fabricated directly on the polymer surface served as an etching mask. Polymer filters with a variety of modified surfaces were used to compare the effects on the culture of cancer cell lines in blank culture wells, with untreated microfilters or with RIE-treated microfilters. We then report the differences of cell shape, phenotype and growth patterns of bladder and glioblastoma cancer cell lines after isolation on the various types of material modifications. Our data suggest that RIE modified polymer filters can isolate model cell lines while retaining ell viability, and that the RIE filter modification allows T24 monolayering cells to proliferate as a structured cluster. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Makarova, Olga V.] Creatv MicroTech Inc, 2242 West Harrison St, Chicago, IL 60612 USA. [Adams, Daniel L.] Create MicroTech Inc, 1 Deer Pk Dr, Monmouth Jct, NJ 08852 USA. [Divan, Ralu; Rosenmann, Daniel] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhu, Peixuan; Li, Shuhong; Amstutz, Platte; Tang, Cha-Mei] Create MicroTech Inc, 11609 Lake Potomac Dr, Potomac, MD 20854 USA. RP Adams, DL (reprint author), Create MicroTech Inc, 1 Deer Pk Dr, Monmouth Jct, NJ 08852 USA. EM dan@creatvmicrotech.com FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Maryland TEDCO under MTTCF Phase I award FX Use of the Center for Nanoscale Materials, an Office of Science user Facility, Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This research was funded in part by Maryland TEDCO under MTTCF Phase I award. NR 35 TC 1 Z9 1 U1 15 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0928-4931 EI 1873-0191 J9 MAT SCI ENG C-MATER JI Mater. Sci. Eng. C-Mater. Biol. Appl. PD SEP 1 PY 2016 VL 66 BP 193 EP 198 DI 10.1016/j.msec.2016.04.075 PG 6 WC Materials Science, Biomaterials SC Materials Science GA DO4FK UT WOS:000377737000023 PM 27207054 ER PT J AU Knox, AS Paller, MH Milliken, CE Redder, TM Wolfe, JR Seaman, J AF Knox, Anna Sophia Paller, Michael H. Milliken, Charles E. Redder, Todd M. Wolfe, John R. Seaman, John TI Environmental impact of ongoing sources of metal contamination on remediated sediments SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Metals; Passive caps; Active caps; Remediated sediment; Bioavailability; Re-contamination ID SEQUESTERING AGENTS; AQUEOUS-SOLUTION; BIOAVAILABILITY AB A challenge to all remedial approaches for contaminated sediments is the continued influx of contaminants from uncontrolled sources following remediation. We investigated the effects of ongoing contamination in mesocosms employing sediments remediated by different types of active and passive caps and in-situ treatment. Our hypothesis was that the sequestering agents used in active caps and in situ treatment will bind elements (arsenic, chromium, cadmium, cobalt, copper, nickel, lead, selenium, and zinc) from ongoing sources thereby reducing their bioavailability and protecting underlying remediated sediments from recontamination. Most element concentrations in surface water remained significantly lower in mesocosms with apatite and mixed amendment caps than in mesocosms with passive caps (sand), uncapped sediment, and spike solution throughout the 2520 h experiment. Element concentrations were significantly higher in Lumbriculus variegatus from untreated sediment than in Lumbriculus from most active caps. Pearson correlations between element concentrations in Lumbriculus and metal concentrations in the top 2.5 cm of sediment or cap measured by diffusive gradient in thin films (DGT) sediment probes were generally strong (as high as 0.98) and significant (p < 0.05) for almost all tested elements. Metal concentrations in both Lumbriculus and sediment/cap were lowest in apatite, mixed amendment, and activated carbon treatments. These findings show that some active caps can protect remediated sediments by reducing the bioavailable pool of metals/metalloids in ongoing sources of contamination. (c) 2016 Elsevier B.V. All rights reserved. C1 [Knox, Anna Sophia; Paller, Michael H.; Milliken, Charles E.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Redder, Todd M.; Wolfe, John R.] LimnoTech, Ann Arbor, MI 48108 USA. [Seaman, John] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. RP Knox, AS (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA. EM anna.knox@srn.doe.gov; michael.paller@srnl.doe.gov; charles.milliken@srnl.doe.gov; tredder@limno.com; jwolfe@limno.com; seaman@srel.uga.edu FU DoD Strategic Environmental Research and Development Program (SERDP) [ER 2427]; U.S. Department of Energy [DE-AC09-798861048] FX This work was sponsored by the DoD Strategic Environmental Research and Development Program (SERDP) under project ER 2427. The SRNL is operated by Savannah River Nuclear Solutions, LLC for the U.S. Department of Energy under Contract DE-AC09-798861048. NR 33 TC 2 Z9 2 U1 16 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD SEP 1 PY 2016 VL 563 BP 108 EP 117 DI 10.1016/j.scitotenv.2016.04.050 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA DO4ZG UT WOS:000377792800012 PM 27135572 ER PT J AU Kenwell, A Navarre-Sitchler, A Prugue, R Spear, JR Hering, AS Maxwell, RM Carroll, RH Williams, KH AF Kenwell, Amy Navarre-Sitchler, Alexis Prugue, Rodrigo Spear, John R. Hering, Amanda S. Maxwell, Reed M. Carroll, RosemaryW. H. Williams, Kenneth H. TI Using geochemical indicators to distinguish high biogeochemical activity in floodplain soils and sediments SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Microbial DNA; Extractable metals; Floodplain geochemistry ID LARGE RIVER FLOODPLAIN; REACTIVE TRANSPORT; DENITRIFYING BACTERIA; ORGANIC-CARBON; RIPARIAN ZONE; FIELD-SCALE; DENITRIFICATION; PCR; HETEROGENEITY; TRANSFORMATIONS AB A better understanding of how microbial communities interact with their surroundings in physically and chemically heterogeneous subsurface environments will lead to improved quantification of biogeochemical reactions and associated nutrient cycling. This study develops a methodology to predict potential elevated rates of biogeochemical activity (microbial "hotspots") in subsurface environments by correlating microbial DNA and aspects of the community structure with the spatial distribution of geochemical indicators in subsurface sediments. Multiple linear regression models of simulated precipitation leachate, HCl and hydroxylamine extractable iron and manganese, total organic carbon (TOC), and microbial community structure were used to identify sample characteristics indicative of biogeochemical hotspots within fluvially-derived aquifer sediments and overlying soils. The method has been applied to (a) alluvial materials collected at a former uranium mill site near Rifle, Colorado and (b) relatively undisturbed floodplain deposits (soils and sediments) collected along the East River near Crested Butte, Colorado. At Rifle, 16 alluvial samples were taken from 8 sediment cores, and at the East River, 46 soil/sediment samples were collected across and perpendicular to 3 active meanders and an oxbow meander. Regression models using TOC and TOC combined with extractable iron and manganese results were determined to be the best fitting statistical models of microbial DNA (via 16S rRNA gene analysis). Fitting these models to observations in both contaminated and natural floodplain deposits, and their associated alluvial aquifers, demonstrates the broad applicability of the geochemical indicator based approach. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kenwell, Amy; Navarre-Sitchler, Alexis; Prugue, Rodrigo; Maxwell, Reed M.] Colorado Sch Mines, Hydrol Sci & Engn Program, 1500 Illinois St, Golden, CO 80401 USA. [Spear, John R.] Colorado Sch Mines, Dept Civil & Environm Engn, 1500 Illinois St, Golden, CO 80401 USA. [Hering, Amanda S.] Colorado Sch Mines, Dept Appl Math & Stat, 1500 Illinois St, Golden, CO 80401 USA. [Carroll, RosemaryW. H.] Desert Res Inst, Div Hydrol Sci, 2215 Raggio Pkwy, Reno, NV 89512 USA. [Williams, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Navarre-Sitchler, A (reprint author), Colorado Sch Mines, Hydrol Sci & Engn Program, 1500 Illinois St, Golden, CO 80401 USA. EM asitchle@mines.edu RI Navarre-Sitchler, Alexis/J-3389-2014; Williams, Kenneth/O-5181-2014 OI Williams, Kenneth/0000-0002-3568-1155 FU Subsurface Science Scientific Focus Area at Lawrence Berkeley National Laboratory - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-737 AC02-05CH11231]; Natural Sciences and Engineering Research Council of Canada (NSERC); Marathon Oil Corporation FX This material is based upon work supported as part of the Subsurface Science Scientific Focus Area at Lawrence Berkeley National Laboratory funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under Award Number DE-737 AC02-05CH11231. A. Kenwell was supported by the Natural Sciences and Engineering Research Council of Canada (NSERC) and R. Prugue was supported by the Marathon Oil Corporation through student fellowships. We thank four anonymous reviewers whose comments greatly improved the manuscript. NR 38 TC 0 Z9 0 U1 17 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD SEP 1 PY 2016 VL 563 BP 386 EP 395 DI 10.1016/j.scitotenv.2016.04.014 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA DO4ZG UT WOS:000377792800041 PM 27145490 ER PT J AU Shin, Y Liu, W Schwenzer, B Manandhar, S Chase-Woods, D Engelhard, MH Devanathan, R Fifield, LS Bennett, WD Ginovska, B Gotthold, DW AF Shin, Yongsoon Liu, Wei Schwenzer, Birgit Manandhar, Sandeep Chase-Woods, Dylan Engelhard, Mark H. Devanathan, Ram Fifield, Leonard S. Bennett, Wendy D. Ginovska, Bojana Gotthold, David W. TI Graphene oxide membranes with high permeability and selectivity for dehumidification of air SO CARBON LA English DT Article ID POLY(BUTYLENE TEREPHTHALATE); BLOCK-COPOLYMERS; GAS SEPARATION; WATER-VAPOR; ENERGY; PERMEATION; BEHAVIOR; SYSTEM; SHEETS AB Hierarchically stacked 2D graphene oxide (GO) membranes are a fascinating and promising new class of materials with the potential for radically improved water vapor/gas separation with excellent selectivity and high permeability. This paper details dehumidification results from flowing gas mixtures through free-standing GO membrane samples prepared by a casting method. The first demonstrated use of freestanding GO membranes for water vapor separation reveals outstanding water vapor permeability and H2O/N-2 selectivity. Free-standing GO membranes exhibit extremely high water vapor permeability of 1.82 x 10(5) Barrer and a water vapor permeance of 1.01 x 10(-5) mol/m(2)sPa, while the nitrogen permeability was below the system's detection limit, yielding a selectivity >10(4) in 80% relative humidity (RH) air at 30.8 degrees C. The results show great potential for a range of energy conversion and environmental applications. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Shin, Yongsoon; Schwenzer, Birgit; Ginovska, Bojana] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Liu, Wei; Chase-Woods, Dylan; Devanathan, Ram; Fifield, Leonard S.; Bennett, Wendy D.; Gotthold, David W.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Manandhar, Sandeep; Engelhard, Mark H.] Pacific NW Natl Lab, WR Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. [Manandhar, Sandeep] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Chase-Woods, Dylan] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Gotthold, DW (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM david.gotthold@pnnl.gov OI Devanathan, Ram/0000-0001-8125-4237; Manandhar, Sandeep/0000-0001-8613-5317 FU DOE's Office of Biological and Environmental Research (BER) at PNNL FX The research described in this paper is part of the Materials Synthesis, Simulation, and across the Scale (MS3) Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi-program national laboratory operated by Battelle for the U.S. Department of Energy. A portion of the research was performed using the Environmental Molecular Sciences Laboratory (EMSL) (http://www.emsl.pnl.gov; user proposal #48749), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research (BER) and located at PNNL. NR 30 TC 2 Z9 2 U1 18 U2 61 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD SEP PY 2016 VL 106 BP 164 EP 170 DI 10.1016/j.carbon.2016.05.023 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DO1NI UT WOS:000377544900020 ER PT J AU Melaet, G Ralston, WT Liu, WC Somorjai, GA AF Melaet, Gerome Ralston, Walter T. Liu, Wen-Chi Somorjai, Gabor A. TI Product distribution change in the early stages of carbon monoxide hydrogenation over cobalt magnesium Fischer-Tropsch catalyst SO CATALYSIS TODAY LA English DT Article; Proceedings Paper CT 249th ACS National Meeting and Exposition CY MAR 22-26, 2015 CL Denver, CO DE Fischer-Tropsch synthesis; CO hydrogenation; Cobalt; Transient experiments; Time-resolved; Temporal analysis of products ID PARTICLE-SIZE; TRANSIENT KINETICS; CO HYDROGENATION; SYNTHESIS GAS AB The catalytic hydrogenation of carbon monoxide, known as the Fischer-Tropsch process, is a technologically important, complex multipath reaction which produces long chain hydrocarbons. In order to access the initial kinetics and the mechanism, we developed a reactor that provides information under non-steady state conditions. We tested a CoMgO catalyst and monitored the initial product formation within 2 s of exposure to CO as well as the time dependence of high molecular weight products (in a 60 s window) and found drastic changes in the product selectivity. The probability for forming branched isomers (C-4 and C-5) peaks in the first 25 s, and within that time frame no unsaturated products were detected. The subsequent decline (at 35 to 40 s) of branched isomers coincides with the detection of olefins (from C-2 to C-5) and the change in carbon coverage at the surface of the catalyst. This indicates a change in the reaction pathway. (C) 2016 Elsevier B.V. All rights reserved. C1 [Melaet, Gerome; Ralston, Walter T.; Liu, Wen-Chi; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ralston, Walter T.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Melaet, Gerome; Liu, Wen-Chi; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM Somorjai@berkeley.edu OI Liu, Wen-Chi/0000-0002-0810-9014 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division [DE-AC02-05CH11231] FX The present paper was submitted in honor of Dr. Jens Rostrup-Nielsen. The authors want to thank the Molecular Foundry of the Lawrence National Laboratory for the help in the SEM and EDS (Proposal #3806). This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division under Contract DE-AC02-05CH11231 NR 18 TC 0 Z9 0 U1 13 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD SEP 1 PY 2016 VL 272 BP 69 EP 73 DI 10.1016/j.cattod.2016.03.027 PG 5 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DN9GA UT WOS:000377386300011 ER PT J AU Dorier, M Yildiz, O Ibrahim, S Orgerie, AC Antoniu, G AF Dorier, Matthieu Yildiz, Orcun Ibrahim, Shadi Orgerie, Anne-Cecile Antoniu, Gabriel TI On the energy footprint of I/O management in Exascale HPC systems SO FUTURE GENERATION COMPUTER SYSTEMS-THE INTERNATIONAL JOURNAL OF ESCIENCE LA English DT Article DE Exascale computing; Energy; I/O; Dedicated cores; Dedicated nodes; Damaris AB The advent of unprecedentedly scalable yet energy hungry Exascale supercomputers poses a major challenge in sustaining a high performance-per-watt ratio. With I/O management acquiring a crucial role in supporting scientific simulations, various I/O management approaches have been proposed to achieve high performance and scalability. However, the details of how these approaches affect energy consumption have not been studied yet. Therefore, this paper aims to explore how much energy a supercomputer consumes while running scientific simulations when adopting various I/O management approaches. In particular, we closely examine three radically different I/O schemes including time partitioning, dedicated cores, and dedicated nodes. To do so, we implement the three approaches within the Damaris I/O middleware and perform extensive experiments with one of the target HPC applications of the Blue Waters sustained-petaflop supercomputer project: the CM1 atmospheric model. Our experimental results obtained on the French Grid'5000 platform highlight the differences among these three approaches and illustrate in which way various configurations of the application and of the system can impact performance and energy consumption. Moreover, we propose and validate a mathematical model that estimates the energy consumption of a HPC simulation under different I/O approaches. Our proposed model gives hints to pre-select the most energy-efficient I/O approach for a particular simulation on a particular HPC system and therefore provides a step towards energy-efficient HPC simulations in Exascale systems. To the best of our knowledge, our work provides the first in-depth look into the energy-performance tradeoffs of I/O management approaches. (C) 2016 Elsevier B.V. All rights reserved. C1 [Dorier, Matthieu] ENS Rennes, IRISA, Rennes, France. [Dorier, Matthieu] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Yildiz, Orcun; Ibrahim, Shadi; Antoniu, Gabriel] Inria Rennes Bretagne Atlantique, Rennes, France. [Orgerie, Anne-Cecile] CNRS, IRISA, Rennes, France. RP Ibrahim, S (reprint author), Inria Rennes Bretagne Atlantique, Rennes, France. EM shadi.ibrahim@inria.fr OI Dorier, Matthieu/0000-0001-9293-2021 NR 36 TC 0 Z9 0 U1 9 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-739X EI 1872-7115 J9 FUTURE GENER COMP SY JI Futur. Gener. Comp. Syst. PD SEP PY 2016 VL 62 BP 17 EP 28 DI 10.1016/j.future.2016.03.002 PG 12 WC Computer Science, Theory & Methods SC Computer Science GA DN8FZ UT WOS:000377315900002 ER PT J AU Margolin, LG AF Margolin, L. G. TI A strain space framework for numerical hyperplasticity SO MATHEMATICS AND COMPUTERS IN SIMULATION LA English DT Article DE Numerical plasticity; Hyperplasticity; Wilkins' method ID EULERIAN COMPUTING METHOD; PLASTICITY THEORY; HYPO-ELASTICITY; FLOW SPEEDS; ENERGY AB Numerical simulations of high strain rate plastic flow have historically been built in a hypoelastic framework and use radial return (Wilkins' method) as the solution algorithm. We show how each of these choices can lead to inaccurate and possibly nonconvergent results. We describe an alternative solution procedure based on a simple multiple time scale perturbation theory that is stable, accurate, computationally efficient and simple to implement. Further extension of these results then leads to a strain space formulation that has additional computational advantages. We illustrate our development with numerical experiments. This paper is dedicated to my friend and colleague Christo Christov on the occasion of his 60th birthday, in recognition of his many important and creative contributions to the formulation of continuum mechanics. (C) 2012 IMACS. Published by Elsevier B.V. All rights reserved. C1 [Margolin, L. G.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Margolin, LG (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM len@lanl.gov NR 23 TC 0 Z9 0 U1 3 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-4754 EI 1872-7166 J9 MATH COMPUT SIMULAT JI Math. Comput. Simul. PD SEP PY 2016 VL 127 SI SI BP 178 EP 188 DI 10.1016/j.matcom.2012.06.016 PG 11 WC Computer Science, Interdisciplinary Applications; Computer Science, Software Engineering; Mathematics, Applied SC Computer Science; Mathematics GA DM7BT UT WOS:000376508600013 ER PT J AU Chong, XY Kim, KJ Li, EW Zhang, YJ Ohodnicki, PR Chang, CH Wang, AX AF Chong, Xinyuan Kim, Ki-Joong Li, Erwen Zhang, Yujing Ohodnicki, Paul R. Chang, Chih-Hung Wang, Alan X. TI Near-infrared absorption gas sensing with metal-organic framework on optical fibers SO SENSORS AND ACTUATORS B-CHEMICAL LA English DT Article DE Infrared absorption; Fiber-optic sensors; Metal-organic; Framework; Gas sensors ID DRUG-DELIVERY; HYDROGEN STORAGE; WATER-VAPOR; CO2; ADSORPTION; SEPARATION; SUBSTRATE; CATALYSIS; MIXTURES; REMOVAL AB Despite significant advantages in terms of portability and cost, near-infrared (NIR) gas sensing still remains a great challenge due to its relatively weak overtone absorption from the fundamental vibrational bond absorption at the mid-IR frequency. In this paper, we demonstrated ultra-sensitive NIR gas sensing for carbon dioxide (CO2) at 1.57 mu m wavelength through nanoporous Cu-BTC (BTC = benzene-1,3,5-tricarboxylate) metal-organic framework (MOF) coated single-mode optical fiber. For the first time, we obtained high-resolution NIR spectroscopy of CO2 sorbed in MOF without seeing any rotational side band, indicating that the tightly confined gas molecules in the MOF pores do not have any freedom of rotation. Real-time measurement of the mixed gas flow of CO2 and Ar showed different response time depending on the concentration of CO2, which is attributed to the complex sorption mechanism of CO2 in Cu-BTC MOF. Most importantly, we realized ultra-low detection limit of CO2 (<20 ppm) with only 5 cm long Cu-BTC MOF thin film coated on single-mode optical fibers. (C) 2016 Elsevier B.V. All rights reserved. C1 [Chong, Xinyuan; Li, Erwen; Wang, Alan X.] Oregon State Univ, Sch Elect Engn & Comp Sci, Corvallis, OR 97331 USA. [Kim, Ki-Joong; Zhang, Yujing; Chang, Chih-Hung] Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. [Ohodnicki, Paul R.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Ohodnicki, Paul R.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Wang, AX (reprint author), Oregon State Univ, Sch Elect Engn & Comp Sci, Corvallis, OR 97331 USA. EM wang@eecs.oregonstate.edu FU National Energy Technology Laboratory's (NETL) [DE-FE0004000]; National Science Foundation [1449383]; Graduate Student Fellowship from NETL FX This technical effort was performed in support of the National Energy Technology Laboratory's (NETL) research under the RES contract DE-FE0004000 and the National Science Foundation under grant No. 1449383. Xinyuan Chong and Yujing Zhang are sponsored by the Graduate Student Fellowship from NETL. NR 50 TC 1 Z9 1 U1 57 U2 158 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-4005 J9 SENSOR ACTUAT B-CHEM JI Sens. Actuator B-Chem. PD SEP PY 2016 VL 232 BP 43 EP 51 DI 10.1016/j.snb.2016.03.135 PG 9 WC Chemistry, Analytical; Electrochemistry; Instruments & Instrumentation SC Chemistry; Electrochemistry; Instruments & Instrumentation GA DL2RO UT WOS:000375483000006 ER PT J AU Wang, PB Lu, XN Yang, X Wang, W Xu, DG AF Wang, Panbao Lu, Xiaonan Yang, Xu Wang, Wei Xu, Dianguo TI An Improved Distributed Secondary Control Method for DC Microgrids With Enhanced Dynamic Current Sharing Performance SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Current sharing; dc microgrid (MG); droop control; low-bandwidth communication (LBC); secondary control ID ADAPTIVE DROOP CONTROL; HIERARCHICAL CONTROL; CONTROL STRATEGY; DECENTRALIZED CONTROL; VOLTAGE; MANAGEMENT; SYSTEMS; COMMUNICATION; CONVERTERS; DESIGN AB This paper proposes an improved distributed secondary control scheme for dc microgrids (MGs), aiming at overcoming the drawbacks of conventional droop control method. The proposed secondary control scheme can remove the dc voltage deviation and improve the current sharing accuracy by using voltage-shifting and slope-adjusting approaches simultaneously. Meanwhile, the average value of droop coefficients is calculated, and then it is controlled by an additional controller included in the distributed secondary control layer to ensure that each droop coefficient converges at a reasonable value. Hence, by adjusting the droop coefficient, each participating converter has equal output impedance, and the accurate proportional load current sharing can be achieved with different line resistances. Furthermore, the current sharing performance in steady and transient states can be enhanced by using the proposed method. The effectiveness of the proposed method is verified by detailed experimental tests based on a 3 x 1 kW prototype with three interface converters. C1 [Wang, Panbao; Yang, Xu; Wang, Wei; Xu, Dianguo] Harbin Inst Technol, Dept Elect Engn, Harbin 150001, Peoples R China. [Lu, Xiaonan] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Wang, PB; Yang, X; Wang, W; Xu, DG (reprint author), Harbin Inst Technol, Dept Elect Engn, Harbin 150001, Peoples R China.; Lu, XN (reprint author), Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. EM wangpanbao@hit.edu.cn; primerxu@aol.com; xiaonan.lu@anl.gov; wangwei602@hit.edu.cn; xudiang@hit.edu.cn FU National Nature Science Foundation of China [51477033] FX This work was supported by the National Nature Science Foundation of China ( 51477033). Recommended for publication by Associate Editor S. Mazumder. NR 39 TC 3 Z9 4 U1 8 U2 40 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 EI 1941-0107 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD SEP PY 2016 VL 31 IS 9 BP 6658 EP 6673 DI 10.1109/TPEL.2015.2499310 PG 16 WC Engineering, Electrical & Electronic SC Engineering GA DH9FM UT WOS:000373101800056 ER PT J AU Cuevas-Maraver, J Kevrekidis, PG Saxena, A Cooper, F Khare, A Comech, A Bender, CM AF Cuevas-Maraver, Jesus Kevrekidis, Panayotis G. Saxena, Avadh Cooper, Fred Khare, Avinash Comech, Andrew Bender, Carl M. TI Solitary Waves of a PT-Symmetric Nonlinear Dirac Equation SO IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS LA English DT Article DE Nonlinear dynamical systems; nonlinear differential equations; bifurcation ID FIELD-THEORIES; LINEAR INSTABILITY; STABILITY; ENERGY AB In this study we consider we consider a prototypical example of a PT-symmetric Dirac model. We discuss the underlying linear limit of the model and identify the threshold of the PT-phase transition in an analytical form. We then focus on the examination of the nonlinear model. We consider the continuation in the PT-symmetric model of the solutions of the corresponding Hamiltonianmodel and find that the solutions can be continued robustly as stable ones all the way up to thePT-transition threshold. In the latter, they degenerate into linearwaves. We also examine the dynamics of the model. Given the stability of the waveforms in the PT-exact phase, we consider them as initial conditions for parameters outside of that phase. We find that both oscillatory dynamics and exponential growth may arise, depending on the size of the corresponding " quench". The former can be characterized by an interesting form of bifrequency solutions that have been predicted on the basis of the SU(1, 1) symmetry. Finally, we explore some special, analytically tractable, but not PT-symmetric solutions in the massless limit of the model. C1 [Cuevas-Maraver, Jesus] Univ Seville, Dept Fis Aplicada 1, Nonlinear Phys Grp, Escuela Politecn Super, Seville 41011, Spain. [Cuevas-Maraver, Jesus] Univ Seville, Inst Matemat, IMUS, E-41012 Seville, Spain. [Kevrekidis, Panayotis G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Kevrekidis, Panayotis G.; Saxena, Avadh; Cooper, Fred] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Kevrekidis, Panayotis G.; Saxena, Avadh; Cooper, Fred] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Cooper, Fred] Santa Fe Inst, Santa Fe, NM 87501 USA. [Khare, Avinash] Savitribai Phule Pune Univ, Dept Phys, Pune 411007, Maharashtra, India. [Comech, Andrew] Texas A&M Univ, Dept Math, College Stn, TX 77843 USA. [Comech, Andrew] Inst Informat Transmiss Problems, Moscow 127994, Russia. [Bender, Carl M.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. RP Cuevas-Maraver, J (reprint author), Univ Seville, Dept Fis Aplicada 1, Nonlinear Phys Grp, Escuela Politecn Super, Seville 41011, Spain. EM jcuevas@us.es; kevrekid@math.umass.edu; avadh@lanl.gov; fredcath@earthlink.net; khare@physics.unipune.ac.in; comech@math.tamu.edu; cmb@wuphys.wustl.edu RI Cuevas-Maraver, Jesus/A-1255-2008 OI Cuevas-Maraver, Jesus/0000-0002-7162-5759 FU Indian National Science Academy (INSA); Center for Non Linear Studies; Los Alamos National Laboratory FX A. Khare wishes to thank Indian National Science Academy (INSA) for the award of INSA Senior Scientist Position. P.G. Kevrekidis gratefully acknowledges the hospitality and support of the Center for Non Linear Studies and the Los Alamos National Laboratory. NR 47 TC 1 Z9 1 U1 2 U2 64 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1077-260X EI 1558-4542 J9 IEEE J SEL TOP QUANT JI IEEE J. Sel. Top. Quantum Electron. PD SEP-OCT PY 2016 VL 22 IS 5 AR 5000109 DI 10.1109/JSTQE.2015.2485607 PG 9 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA CY8OE UT WOS:000366667400001 ER PT J AU Favaro, M Jeong, B Ross, PN Yano, J Hussain, Z Liu, Z Crumlin, EJ AF Favaro, Marco Jeong, Beomgyun Ross, Philip N. Yano, Junko Hussain, Zahid Liu, Zhi Crumlin, Ethan J. TI Unravelling the electrochemical double layer by direct probing of the solid/liquid interface SO NATURE COMMUNICATIONS LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; ELECTRICAL DOUBLE-LAYER; WATER-MOLECULES; ABSORPTION SPECTROSCOPY; OXYGEN REDUCTION; LIQUID INTERFACE; SURFACE SCIENCE; STERN LAYER; ELECTRODES; ELECTROCATALYSIS AB The electrochemical double layer plays a critical role in electrochemical processes. Whilst there have been many theoretical models predicting structural and electrical organization of the electrochemical double layer, the experimental verification of these models has been challenging due to the limitations of available experimental techniques. The induced potential drop in the electrolyte has never been directly observed and verified experimentally, to the best of our knowledge. In this study, we report the direct probing of the potential drop as well as the potential of zero charge by means of ambient pressure X-ray photoelectron spectroscopy performed under polarization conditions. By analyzing the spectra of the solvent (water) and a spectator neutral molecule with numerical simulations of the electric field, we discern the shape of the electrochemical double layer profile. In addition, we determine how the electrochemical double layer changes as a function of both the electrolyte concentration and applied potential. C1 [Favaro, Marco; Jeong, Beomgyun; Hussain, Zahid; Liu, Zhi; Crumlin, Ethan J.] Lawrence Berkeley Natl Lab, Adv Light Source, One Cyclotron Rd, Berkeley, CA 94720 USA. [Favaro, Marco; Yano, Junko] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynthesis, One Cyclotron Rd, Berkeley, CA 94720 USA. [Favaro, Marco] Lawrence Berkeley Natl Lab, Div Chem Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. [Jeong, Beomgyun] Gwangju Inst Sci & Technol, Sch Environm Sci & Engn, Ertl Ctr Electrochem & Catalysis, Gwangju 500712, South Korea. [Jeong, Beomgyun] Gwangju Inst Sci & Technol, Ctr Adv Xray Sci, Gwangju 500712, South Korea. [Ross, Philip N.] Lawrence Berkeley Natl Lab, Div Mat Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. [Yano, Junko] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, One Cyclotron Rd, Berkeley, CA 94720 USA. [Liu, Zhi] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China. [Liu, Zhi] ShanghaiTech Univ, Sch Phys Sci & Technol, Div Photon Sci & Condensed Matter Phys, Shanghai 200031, Peoples R China. [Crumlin, Ethan J.] Lawrence Berkeley Natl Lab, Joint Ctr Energy Storage Res, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Liu, Z; Crumlin, EJ (reprint author), Lawrence Berkeley Natl Lab, Adv Light Source, One Cyclotron Rd, Berkeley, CA 94720 USA.; Liu, Z (reprint author), Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China.; Liu, Z (reprint author), ShanghaiTech Univ, Sch Phys Sci & Technol, Div Photon Sci & Condensed Matter Phys, Shanghai 200031, Peoples R China.; Crumlin, EJ (reprint author), Lawrence Berkeley Natl Lab, Joint Ctr Energy Storage Res, One Cyclotron Rd, Berkeley, CA 94720 USA. EM zliu2@mail.sim.ac.cn; ejcrumlin@lbl.gov RI Liu, Zhi/B-3642-2009; OI Liu, Zhi/0000-0002-8973-6561; Favaro, Marco/0000-0002-3502-8332 FU Office of Science, Office of Basic Energy Science (BES), of the U.S. Department of Energy (DOE) [DE-SC0004993]; Joint Center for Energy Storage Research (JCESR), DOE Energy Innovation Hubs; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [11227902]; CAS-Shanghai Science Research Center [CAS-SSRC-YH-2015-01] FX This work was supported through the Office of Science, Office of Basic Energy Science (BES), of the U.S. Department of Energy (DOE) under award no. DE-SC0004993 to the Joint Center for Artificial Photosynthesis (JCAP) and as part of the Joint Center for Energy Storage Research (JCESR), DOE Energy Innovation Hubs.; The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.; Z.L. thanks the support from National Natural Science Foundation of China under Contract No. 11227902. This work was also partially supported by CAS-Shanghai Science Research Center, Grant No.: CAS-SSRC-YH-2015-01. NR 55 TC 3 Z9 3 U1 22 U2 22 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD AUG 31 PY 2016 VL 7 AR 12695 DI 10.1038/ncomms12695 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH6KI UT WOS:000391881500001 PM 27576762 ER PT J AU Stone, G Ophus, C Birol, T Ciston, J Lee, CH Wang, K Fennie, CJ Schlom, DG Alem, N Gopalan, V AF Stone, Greg Ophus, Colin Birol, Turan Ciston, Jim Lee, Che-Hui Wang, Ke Fennie, Craig J. Schlom, Darrell G. Alem, Nasim Gopalan, Venkatraman TI Atomic scale imaging of competing polar states in a Ruddlesden-Popper layered oxide SO NATURE COMMUNICATIONS LA English DT Article ID BILBAO CRYSTALLOGRAPHIC SERVER; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; GIANT MAGNETORESISTANCE; COMPLEX OXIDES; BASIS-SET; PEROVSKITES; INTERFACES; CHEMISTRY; HETEROSTRUCTURES AB Layered complex oxides offer an unusually rich materials platform for emergent phenomena through many built-in design knobs such as varied topologies, chemical ordering schemes and geometric tuning of the structure. A multitude of polar phases are predicted to compete in Ruddlesden-Popper (RP), A(n+1)BnO(3n+1), thin films by tuning layer dimension (n) and strain; however, direct atomic-scale evidence for such competing states is currently absent. Using aberration-corrected scanning transmission electron microscopy with sub-Angstrom resolution in Srn+1TinO3n+1 thin films, we demonstrate the coexistence of antiferroelectric, ferroelectric and new ordered and low-symmetry phases. We also directly image the atomic rumpling of the rock salt layer, a critical feature in RP structures that is responsible for the competing phases; exceptional quantitative agreement between electron microscopy and density functional theory is demonstrated. The study shows that layered topologies can enable multifunctionality through highly competitive phases exhibiting diverse phenomena in a single structure. C1 [Stone, Greg; Lee, Che-Hui; Alem, Nasim; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Stone, Greg; Lee, Che-Hui; Alem, Nasim; Gopalan, Venkatraman] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Ophus, Colin; Ciston, Jim] Lawrence Berkeley Natl Lab, Natl Ctr Elect Microscopy Mol Foundry, Berkeley, CA 94720 USA. [Birol, Turan] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Lee, Che-Hui; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Wang, Ke] Penn State Univ, Mat Res Inst, Mat Characterizat Lab, University Pk, PA 16802 USA. [Fennie, Craig J.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Gopalan, V (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA.; Gopalan, V (reprint author), Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. EM vgopalan@psu.edu RI Birol, Turan/D-1948-2012 OI Birol, Turan/0000-0001-5174-3320 FU Center for Nanoscale Science, a National Science Foundation center [DMR-1420620]; NSF [DMR-1210588, DMR-1056441]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Rutgers Center for Materials Theory FX G.S., C.-H.L., D.G.S., V.G. and N.A. were primarily supported by the Center for Nanoscale Science, a National Science Foundation center through Grant number DMR-1420620. G.S. and V.G. also received partial support from NSF Grant number DMR-1210588. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. T.B. was supported by the Rutgers Center for Materials Theory. C.J.F. acknowledges support from the NSF Grant number DMR-1056441. We would like to thank Marissa Libbee for her helpful guidance preparing TEM samples. We would also like to thank Roman Engel-Herbert for useful discussions and Haiying Wang with sample prep. NR 47 TC 0 Z9 0 U1 14 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD AUG 31 PY 2016 VL 7 AR 12572 DI 10.1038/ncomms12572 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH6GD UT WOS:000391870000001 PM 27578622 ER PT J AU Yang, Y Yang, MJ Zhu, K Johnson, JC Berry, JJ van de Lagemaat, J Beard, MC AF Yang, Ye Yang, Mengjin Zhu, Kai Johnson, Justin C. Berry, Joseph J. van de lagemaat, Jao Beard, Matthew C. TI Large polarization-dependent exciton optical Stark effect in lead iodide perovskites SO NATURE COMMUNICATIONS LA English DT Article ID SEMICONDUCTOR-LASER; QUANTUM-DOT; SPIN AB A strong interaction of a semiconductor with a below-bandgap laser pulse causes a blue-shift of the bandgap transition energy, known as the optical Stark effect. The energy shift persists only during the pulse duration with an instantaneous response time. The optical Stark effect has practical relevance for applications, including quantum information processing and communication, and passively mode-locked femtosecond lasers. Here we demonstrate that solution-processable lead-halide perovskites exhibit a large optical Stark effect that is easily resolved at room temperature resulting from the sharp excitonic feature near the bandedge. We also demonstrate that a polarized pump pulse selectively shifts one spin state producing a spin splitting of the degenerate excitonic states. Such selective spin manipulation is an important prerequisite for spintronic applications. Our result implies that such hybrid semiconductors may have great potential for optoelectronic applications beyond photovoltaics. C1 [Yang, Ye; Yang, Mengjin; Zhu, Kai; Johnson, Justin C.; Berry, Joseph J.; van de lagemaat, Jao; Beard, Matthew C.] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. RP Yang, Y; Beard, MC (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM ye.yang@nrel.gov; matt.beard@nrel.gov OI BEARD, MATTHEW/0000-0002-2711-1355; Yang, Mengjin/0000-0003-2019-4298 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy through the Solar Photochemistry programme [DE-AC36-08GO28308]; US Department of Energy, Office of Energy Efficiency and Renewable Energy, Solar Energy Technologies Office FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy through the Solar Photochemistry programme under contract DE-AC36-08GO28308 to the National Renewable Energy Laboratory, Golden, Colorado. Perovskite films were supplied from the Hybrid Perovskite Solar Cell program of the National Center for Photovoltaics funded by the US Department of Energy, Office of Energy Efficiency and Renewable Energy, Solar Energy Technologies Office. NR 33 TC 1 Z9 1 U1 4 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD AUG 31 PY 2016 VL 7 AR 12613 DI 10.1038/ncomms12613 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH6GW UT WOS:000391872000001 PM 27577007 ER PT J AU Zhang, WG Mao, JH Zhu, W Jain, AK Liu, K Brown, JB Karpen, GH AF Zhang, Weiguo Mao, Jian-Hua Zhu, Wei Jain, Anshu K. Liu, Ke Brown, James B. Karpen, Gary H. TI Centromere and kinetochore gene misexpression predicts cancer patient survival and response to radiotherapy and chemotherapy SO NATURE COMMUNICATIONS LA English DT Article ID CELL LUNG-CANCER; CENP-A; BREAST-CANCER; CHROMOSOMAL INSTABILITY; ADJUVANT CHEMOTHERAPY; GENOMIC INSTABILITY; MITOTIC CHECKPOINT; DRUG-SENSITIVITY; DNA-DAMAGE; ANEUPLOIDY AB Chromosomal instability (CIN) is a hallmark of cancer that contributes to tumour heterogeneity and other malignant properties. Aberrant centromere and kinetochore function causes CIN through chromosome missegregation, leading to aneuploidy, rearrangements and micronucleus formation. Here we develop a Centromere and kinetochore gene Expression Score (CES) signature that quantifies the centromere and kinetochore gene misexpression in cancers. High CES values correlate with increased levels of genomic instability and several specific adverse tumour properties, and prognosticate poor patient survival for breast and lung cancers, especially early-stage tumours. They also signify high levels of genomic instability that sensitize cancer cells to additional genotoxicity. Thus, the CES signature forecasts patient response to adjuvant chemotherapy or radiotherapy. Our results demonstrate the prognostic and predictive power of the CES, suggest a role for centromere misregulation in cancer progression, and support the idea that tumours with extremely high CIN are less tolerant to specific genotoxic therapies. C1 [Zhang, Weiguo; Mao, Jian-Hua; Karpen, Gary H.] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, One Cyclotron Rd,Mailstop 977, Berkeley, CA 94720 USA. [Zhang, Weiguo; Karpen, Gary H.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Zhu, Wei] Cellular Biomed Grp Inc, Dept Translat Bioinformat, Level 5,Bldg 1,333 Guiping Rd, Shanghai 200233, Peoples R China. [Jain, Anshu K.] Yale Univ, Dept Therapeut Radiol, Yale Sch Med, New Haven, CT 06510 USA. [Jain, Anshu K.] Ashland Bellefonte Canc Ctr, 122 St Christopher Dr, Ashland, KY 41101 USA. [Liu, Ke; Brown, James B.] Lawrence Berkeley Natl Lab, Environm Genom & Syst Biol Div, One Cyclotron Rd,Mailstop 977, Berkeley, CA 94720 USA. [Liu, Ke; Brown, James B.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Brown, James B.] Univ Birmingham, Dept Environm Bioinformat, Birmingham B15 2TT, W Midlands, England. RP Karpen, GH (reprint author), Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, One Cyclotron Rd,Mailstop 977, Berkeley, CA 94720 USA.; Karpen, GH (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.; Zhu, W (reprint author), Cellular Biomed Grp Inc, Dept Translat Bioinformat, Level 5,Bldg 1,333 Guiping Rd, Shanghai 200233, Peoples R China. EM wzhang2@lbl.gov; ghkarpen@lbl.gov FU NIH [R01 GM066272, GM119011, CA116481] FX We are grateful to members of the Karpen lab and Dr Hao Tang for critical reading of the manuscript, Ms Hannah K. Connolly from the UCSF breast cancer SPORE for her enthusiastic support and Mr Kevin Peet for editorial assistance. We thank Dr Joe Gray for the breast cancer data set with radiotherapy information, Drs Hao Tang and Yang Xie for normalized GSE42127 data set, Dr K.J. Gao for neo-therapy data associated with GSE20685, and Dr Balazs Gyorffy for technical assistance on K-M Plotter database. We thank TCGA, Broad Institute, Cancer Genome Project at Sanger Institute and K-M Plotter for maintaining critical public databases and services. We apologize to numerous colleagues in the centromere and kinetochore field for being unable to cite many important papers due to space limitations. This work was supported by NIH grants R01 GM066272 and GM119011 (G.H.K.) and CA116481 (J.-H.M.). NR 80 TC 0 Z9 0 U1 0 U2 0 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD AUG 31 PY 2016 VL 7 AR 12619 DI 10.1038/ncomms12619 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH6GY UT WOS:000391872200001 PM 27577169 ER PT J AU Gallis, MA Koehler, TP Torczynski, JR Plimpton, SJ AF Gallis, M. A. Koehler, T. P. Torczynski, J. R. Plimpton, S. J. TI Direct simulation Monte Carlo investigation of the Rayleigh-Taylor instability SO PHYSICAL REVIEW FLUIDS LA English DT Article ID GAS-FLOWS; FLUIDS; TRANSITION; TURBULENCE; FUSION; GAIN AB The Rayleigh-Taylor instability (RTI) is investigated using the direct simulation Monte Carlo (DSMC) method of molecular gas dynamics. Here, fully resolved two-dimensional DSMC RTI simulations are performed to quantify the growth of flat and single-mode perturbed interfaces between two atmospheric-pressure monatomic gases as a function of the Atwood number and the gravitational acceleration. The DSMC simulations reproduce many qualitative features of the growth of the mixing layer and are in reasonable quantitative agreement with theoretical and empirical models in the linear, nonlinear, and self-similar regimes. In some of the simulations at late times, the instability enters the self-similar regime, in agreement with experimental observations. For the conditions simulated, diffusion can influence the initial instability growth significantly. C1 [Gallis, M. A.; Koehler, T. P.; Torczynski, J. R.] Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. [Plimpton, S. J.] Sandia Natl Labs, Ctr Res Comp, POB 5800, Albuquerque, NM 87185 USA. RP Gallis, MA (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM magalli@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors would like to thank Dr. D. J. Rader and Dr. S. N. Kempka of Sandia National Laboratories and Professor D. I. Pullin of the California Institute of Technology for many useful discussions and suggestions. SPARTA is an open-source DSMC code available from Ref. [44]. NR 50 TC 2 Z9 2 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-990X J9 PHYS REV FLUIDS JI Phys. Rev. Fluids PD AUG 31 PY 2016 VL 1 IS 4 AR 043403 DI 10.1103/PhysRevFluids.1.043403 PG 20 WC Physics, Fluids & Plasmas SC Physics GA EF3IL UT WOS:000390217900001 ER PT J AU Aaboud, M Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Ali, B Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, 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Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zwalinski, L. CA ATLAS Collaboration TI Measurement of exclusive gamma gamma -> W+W- production and search for exclusive Higgs boson production in pp collisions at root s=8 TeV using the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID 2-PHOTON PROCESSES; LHC; PHYSICS AB Searches for exclusively produced W boson pairs in the process pp(gamma gamma) -> pW(+) W- p and an exclusively produced Higgs boson in the process pp(gg) -> pHp have been performed using e(+/-) mu(-/+) final states. These measurements use 20.2 fb(-1) of pp collisions collected by the ATLAS experiment at a center-of-mass energy root s = 8 TeV at the LHC. Exclusive production of W+ W- consistent with the Standard Model prediction is found with 3.0 sigma significance. The exclusive W+ W- production cross section is determined to be sigma(gamma gamma -> W+ W- -> e(+/-) mu(-/+) X) = 6.9 +/- 2.2(stat) +/- 1.4(sys) fb, in agreement with the Standard Model prediction. Limits on anomalous quartic gauge couplings are set at 95% confidence level as -1.7 x 10(-6) < a(0)(W) / Lambda(2) < 1.7 x 10(-6) GeV-2 and -6.4 x 10(-6) < a(C)(W) / Lambda(2) < 6.3 x 10(-6) GeV-2. A 95% confidence-level upper limit on the total production cross section for an exclusive Higgs boson is set to 1.2 pb. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. 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V.; Kroseberg, J.; Kruger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; Von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Phy Inst, Bonn, Germany. [Ahlen, S. P.; Aloisio, A.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Dhaliwal, S.; Goblirsch-Kolb, M.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes; Peralva, B. S.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Elmsheuser, J.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Stucci, S. A.; Takai, H.; Tricoli, A.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Aloisio, A.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. [Gravila, P. M.] West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Marceca, G.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ruiz-Martinez, A.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backhaus, M.; Barak, L.; Barisits, M-S; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Bortfeldt, J.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Cortes-Gonzalez, A.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Di Nardo, R.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Faltova, J.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hanisch, S.; Hawkings, R. J.; Helary, L.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Manousos, A.; Mapelli, L.; Marzin, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nessi, M.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Starz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Unal, G.; Van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Aloisio, A.; Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Liang, Z.; Merino, J. Llorente; Lou, X.; Mansour, J. D.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Aloisio, A.; Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Li, C.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Wang, W.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Aloisio, A.; Du, Y.; Feng, C.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Hu, S.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, PKU CHEP, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Aloisio, A.; Boumediene, D.; Busato, E.; Calvet, D.; Chomont, A. R.; Donini, J.; Gris, Ph.; Pallin, D.; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Callea, G.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Palazzo, S.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Cairo, V. M.; Callea, G.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Palazzo, S.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Aloisio, A.; Alonso, A.; Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Aloisio, A.; Cao, T.; Firan, A.; Gupta, R.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX USA. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Gasnikova, K.; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Gasnikova, K.; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Cinca, D.; Dette, K.; Erdmann, J.; Esch, H.; Gossling, C.; Homann, M.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Aloisio, A.; Alonso, A.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mijovic, L.; Mills, C.; Pino, S. A. Olivares; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Glatzer, J.; Gonella, G.; Herten, G.; Hirose, M.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Nagel, M.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Albert Ludwigs Univ, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Iacobucci, G.; Katre, A.; Khoo, T. J.; Lanfermann, M. C.; Lionti, A. E.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, High Energy Phys Inst, Tbilisi, Rep of Georgia. [Duren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Justus Liebig Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Bisanz, T.; Blumenschein, U.; Brandt, G.; De Maria, A.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Quadt, A.; Rieger, J.; Rosien, N. -A.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Georg August Univ, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Aloisio, A.; Berlendis, S.; Bethani, A.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [Aloisio, A.; Alonso, A.; Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Antel, C.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Zu Theenhausen, H. Meyer; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; de Lima, D. E. Ferreira; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.; Tu, Y.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Clear Water Bay, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Guenther, J.; Jansky, R.; Kneringer, E.; Lukas, W.; Milic, A.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Werner, M. D.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Turchikhin, S.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Aloisio, A.; Alonso, A.; Amako, K.; Amorim, A.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Aloisio, A.; Alonso, A.; Amorim, A.; Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Reale, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Reale, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lewis, D.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Aloisio, A.; Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Kilby, C. R.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Grout, Z. J.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Lopez, S. Calvente; Cueto, A.; De la Torre, H.; Del Peso, J.; Glasman, C.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Cuth, J.; Dudder, A. Chr.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Geisen, M.; Groh, S.; Heck, T.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Schulte, A.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Yildirim, E.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schweiger, H.; Shaw, S. M.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Lefebvre, B.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Goldfarb, S.; Jennens, D.; Kubota, T.; Le, B.; McDonald, E. F.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Citterio, M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Camplani, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Billoud, T. R. V.; Dallaire, F.; Ducu, O. A.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Mochizuki, K.; Manh, T. Nguyen; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Aloisio, A.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Aloisio, A.; Bender, M.; Biebel, O.; Bock, C.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Hartmann, N. M.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Losel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Schachtner, B. M.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Ludwig Maximilians Univ Munchen, Fak Phys, Munich, Germany. [Aloisio, A.; Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Koehler, N. M.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; McCarthy, T. G.; Menke, S.; Mueller, F.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Savic, N.; Schacht, P.; Schmidt-Sommerfeld, K. R.; Spettel, F.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aloisio, A.; Horii, Y.; Kentaro, K.; Nakahama, Y.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kentaro, K.; Nakahama, Y.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Bruni, L. S.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van denWollenberg, W.; Van der Deijl, P. C.; van der Graaf, H.; Van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.; Wolf, T. M. H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Bruni, L. S.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van denWollenberg, W.; Van der Deijl, P. C.; van der Graaf, H.; Van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.; Wolf, T. M. H.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Brost, E.; Burghgrave, B.; Chakraborty, D.; Klimek, P.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. 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[Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris Saclay, Univ Paris Sud, CNRS IN2P3, LAL, Orsay, France. [Ishijima, N.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Aloisio, A.; Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Burr, J. T. P.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Radescu, V.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Dondero, P.; Farina, E. M.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Kourkoumeli-Charalampidi, A.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Dondero, P.; Farina, E. M.; Fraternali, M.; Introzzi, G.; Kourkoumeli-Charalampidi, A.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Brendlinger, K.; Haney, B.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Reichert, J.; Thomson, E.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] Kurchatov Inst, Natl Res Ctr, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Andreazza, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Pedro, R.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Ali, B.; Augsten, K.; Caforio, D.; Gallus, P.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Aloisio, A.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Staroba, P.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Vaniachine, A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.; Worm, S. D.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Tehrani, F. Safai; Vanadia, M.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cerrito, L.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cerrito, L.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.; Tayalati, Y.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Rodriguez, L. Pacheco; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schier, S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torr; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Campoverde, A.; Czirr, H.; Fleck, I.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Armbruster, A. J.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Dado, T.; Melo, M.; Plazak, L.; Smiesko, J.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Aloisio, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjlin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Aloisio, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjlin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Backes, M.; Balestri, T.; Bee, C. P.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Aloisio, A.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Lerner, G.; Miano, F.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Soffer, A.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gentsos, C.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Enari, Y.; Hanawa, K.; Ishino, M.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kishimoto, T.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Okumura, Y.; Saito, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Aloisio, A.; Alonso, A.; Amorim, A.; Andreazza, A.; Asai, S.; Chen, S.; Enari, Y.; Hanawa, K.; Ishino, M.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kishimoto, T.; Kobayashi, A.; Kobayashi, T.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Mori, T.; Morinaga, M.; Nakamura, T.; Nobe, T.; Saito, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hayakawa, D.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Tanaka, M.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Hod, N.; Jovicevic, J.; Codina, E. Perez; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Pinamonti, M.; Serkin, L.; Shaw, K.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Maddocks, H. J.; Ohman, H.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Aloisio, A.; Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Khader, M.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Outschoorn, V. I. Martinez; Neubauer, M. S.; Rybar, M.; Shang, R.; Sickles, A. M.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Aloisio, A.; Alonso, A.; Piqueras, D. Alvarez; Amorim, A.; Andreazza, A.; Angerami, A.; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Aloisio, A.; Alonso, A.; Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Ferrer, A.; Fuster, J.; Garcia, C.; Higon-Rodriguez, E.; Lacasta, C.; Mamuzic, J.; Melini, D.; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Valero, A.; Ferrer, J. A. Valls] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Aloisio, A.; Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez, D. Rodriguez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. 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[Aloisio, A.; Banerjee, Sw.; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Herget, V.; Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strhmer, R.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wrzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Ellinghaus, F.; Ernis, G.; Gilles, G.; Hirschbuehl, D.; Riegel, C. J.; Tepel, F.; Zeitnitz, C.] Berg Univ Wuppertal, Fak Math & Nat Wissensch, Fachgrp Phys, Wuppertal, Germany. [Baker, O. K.; Noccioli, E. Benhar; Cummings, J.; Ideal, E.; Leister, A. G.; Loginov, A.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Vasquez, J. G.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Lin, S. C.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC, Canada. [Banerjee, Sw.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, Barcelona, Spain. [Castro, N. F.] Univ Porto, Dept Fis & Astron, Fac Ciencias, Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Ottawa, ON, Canada. [Ducu, O. A.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Geng, C.; Guo, Y.; Li, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Govender, N.] Ctr High Performance Comp, CSIR Campus, Cape Town, South Africa. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Taipei, Taiwan. [Igonkina, O.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] Georgian Tech Univ GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pasztor, G.] Eotvos Lorand Univ, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. [Smirnova, L. N.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Song, H. Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. [Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] CNRS IN2P3, Marseille, France. RI Chekulaev, Sergey/O-1145-2015; Lazzaroni, Massimo/N-3675-2015; Prokoshin, Fedor/E-2795-2012; Warburton, Andreas/N-8028-2013; Owen, Mark/Q-8268-2016; Gladilin, Leonid/B-5226-2011; Livan, Michele/D-7531-2012; Ventura, Andrea/A-9544-2015; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; White, Ryan/E-2979-2015; Kantserov, Vadim/M-9761-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Zhukov, Konstantin/M-6027-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015 OI Lazzaroni, Massimo/0000-0002-4094-1273; Prokoshin, Fedor/0000-0001-6389-5399; Warburton, Andreas/0000-0002-2298-7315; Owen, Mark/0000-0001-6820-0488; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; Ventura, Andrea/0000-0002-3368-3413; Mashinistov, Ruslan/0000-0001-7925-4676; White, Ryan/0000-0003-3589-5900; Kantserov, Vadim/0000-0001-8255-416X; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Solodkov, Alexander/0000-0002-2737-8674; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, USA; NSF, USA; BCKDF; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; Investissement d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, USA. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN, the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), BNL (USA), the Tier-2 facilities worldwide and large non-WLCG resource providers. Major contributors of computing resources are listed in Ref. [74]. NR 73 TC 2 Z9 2 U1 26 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 31 PY 2016 VL 94 IS 3 AR 032011 DI 10.1103/PhysRevD.94.032011 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DV6LH UT WOS:000383046500001 ER PT J AU Artamonov, AV Bassalleck, B Bhuyan, B Blackmore, EW Bryman, DA Chen, S Chiang, IH Christidi, IA Cooper, PS Diwan, MV Frank, JS Fujiwara, T Hu, J Ives, J Izmaylov, AO Jaffe, DE Kabe, S Kettell, SH Khabibullin, MM Khotjantsev, AN Kitching, P Kobayashi, M Komatsubara, TK Konaka, A Kudenko, YG Landsberg, LG Lewis, B Li, KK Littenberg, LS Macdonald, JA Mildenberger, J Mineev, OV Miyajima, M Mizouchi, K Muramatsu, N Nakano, T Nomachi, M Nomura, T Numao, T Obraztsov, VF Omata, K Patalakha, DI Poutissou, R Redlinger, G Sato, T Sekiguchi, T Shaikhiev, AT Shinkawa, T Strand, RC Sugimoto, S Tamagawa, Y Tschirhart, R Tsunemi, T Vavilov, DV Viren, B Wang, Z Wei, HY Yershov, NV Yoshimura, Y Yoshioka, T AF Artamonov, A. V. Bassalleck, B. Bhuyan, B. Blackmore, E. W. Bryman, D. A. Chen, S. Chiang, I-H. Christidi, I. -A. Cooper, P. S. Diwan, M. V. Frank, J. S. Fujiwara, T. Hu, J. Ives, J. Izmaylov, A. O. Jaffe, D. E. Kabe, S. Kettell, S. H. Khabibullin, M. M. Khotjantsev, A. N. Kitching, P. Kobayashi, M. Komatsubara, T. K. Konaka, A. Kudenko, Yu. G. Landsberg, L. G. Lewis, B. Li, K. K. Littenberg, L. S. Macdonald, J. A. Mildenberger, J. Mineev, O. V. Miyajima, M. Mizouchi, K. Muramatsu, N. Nakano, T. Nomachi, M. Nomura, T. Numao, T. Obraztsov, V. F. Omata, K. Patalakha, D. I. Poutissou, R. Redlinger, G. Sato, T. Sekiguchi, T. Shaikhiev, A. T. Shinkawa, T. Strand, R. C. Sugimoto, S. Tamagawa, Y. Tschirhart, R. Tsunemi, T. Vavilov, D. V. Viren, B. Wang, Zhe Wei, Hanyu Yershov, N. V. Yoshimura, Y. Yoshioka, T. CA E949 Collaboration TI Search for the rare decay K+ -> mu(+) nu(nu)over-bar nu SO PHYSICAL REVIEW D LA English DT Article AB Evidence of the K+ -> mu(+) nu(nu) over bar nu decay was searched for using E949 ( Brookhaven National Laboratory, USA) experimental data with an exposure of 1.70 x 10(12) stopped kaons. The data sample is dominated by the background process K+ -> mu(+) nu(mu)gamma. An upper limit on the decay rate Gamma(K+ -> mu(+) nu(nu) over bar nu) < 2.4 x 10(-6)Gamma(K+ -> all) at 90% confidence level was set assuming the standard model muon spectrum. The data are presented in such a way as to allow calculation of rates for any assumed mu(+) spectrum. C1 [Artamonov, A. V.; Landsberg, L. G.; Obraztsov, V. F.; Patalakha, D. I.; Vavilov, D. V.] Inst High Energy Phys, Protvino 142280, Moscow Region, Russia. [Bassalleck, B.; Lewis, B.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Bhuyan, B.; Chiang, I-H.; Diwan, M. V.; Frank, J. S.; Jaffe, D. E.; Kettell, S. H.; Li, K. K.; Littenberg, L. S.; Redlinger, G.; Strand, R. C.; Viren, B.; Wang, Zhe] Brookhaven Natl Lab, Upton, NY 11973 USA. [Blackmore, E. W.; Chen, S.; Hu, J.; Konaka, A.; Macdonald, J. A.; Mildenberger, J.; Numao, T.; Poutissou, R.; Vavilov, D. V.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Bryman, D. A.; Ives, J.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Chen, S.; Wang, Zhe; Wei, Hanyu] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Christidi, I. -A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Cooper, P. S.; Tschirhart, R.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Fujiwara, T.; Mizouchi, K.; Nomura, T.; Tsunemi, T.] Kyoto Univ, Dept Phys, Sakyo Ku, Kyoto 6068502, Japan. [Izmaylov, A. O.; Khabibullin, M. M.; Khotjantsev, A. N.; Kudenko, Yu. G.; Mineev, O. V.; Shaikhiev, A. T.; Yershov, N. V.] RAS, Inst Nucl Res, 60 October Revolut Prospect 7a, Moscow 117312, Russia. [Kabe, S.; Kobayashi, M.; Komatsubara, T. K.; Nomura, T.; Omata, K.; Sato, T.; Sekiguchi, T.; Sugimoto, S.; Tsunemi, T.; Yoshimura, Y.; Yoshioka, T.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Kitching, P.] Univ Alberta, Ctr Subat Res, Edmonton, AB T6G 2N5, Canada. [Kudenko, Yu. G.] Moscow Inst Phys & Technol, Moscow 141700, Russia. [Kudenko, Yu. G.] Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Moscow 115409, Russia. [Miyajima, M.; Tamagawa, Y.] Univ Fukui, Dept Appl Phys, 3-9-1 Bunkyo, Fukui, Fukui 9108507, Japan. [Muramatsu, N.; Nakano, T.] Osaka Univ, Nucl Phys Res Ctr, 10-1 Mihogaoka, Osaka 5670047, Japan. [Nomachi, M.] Osaka Univ, Lab Nucl Studies, 1-1 Machikaneyama, Toyonaka, Osaka 5600043, Japan. [Shinkawa, T.] Natl Def Acad, Dept Appl Phys, Yokosuka, Kanagawa 2398686, Japan. [Christidi, I. -A.] Indian Inst Technol Guwahati, Dept Phys, Gauhati 781039, Assam, India. [Frank, J. S.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki 54124, Greece. [Kabe, S.; Landsberg, L. G.; Macdonald, J. A.; Sugimoto, S.] 1 Nathan Hale Dr, Setauket, NY 11733 USA. [Muramatsu, N.] Tohoku Univ, Res Ctr Electron Photon Sci, Taihaku Ku, Sendai, Miyagi 9820826, Japan. [Yoshioka, T.] Kyushu Univ, Dept Phys, Higashi Ku, Fukuoka 8128581, Japan. RP Artamonov, AV (reprint author), Inst High Energy Phys, Protvino 142280, Moscow Region, Russia. RI Wei, Hanyu/D-7291-2017 OI Wei, Hanyu/0000-0003-1973-4912 FU Russian Science Foundation [14-12-00560]; U.S. Department of Energy; Ministry of Education, Culture, Sports, Science and Technology of Japan through the Japan-U.S. Cooperative Research Program in High Energy Physics; Natural Sciences and Engineering Research Council [157985]; National Research Council of Canada; National Natural Science Foundation of China; Tsinghua University Initiative Scientific Research Program FX This research was supported in part by Grant #14-12-00560 of the Russian Science Foundation, the U.S. Department of Energy, the Ministry of Education, Culture, Sports, Science and Technology of Japan through the Japan-U.S. Cooperative Research Program in High Energy Physics and under Grant-in-Aids for Scientific Research, the Natural Sciences and Engineering Research Council (Grant no. 157985) and the National Research Council of Canada, National Natural Science Foundation of China, and the Tsinghua University Initiative Scientific Research Program. NR 9 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 31 PY 2016 VL 94 IS 3 AR 032012 DI 10.1103/PhysRevD.94.032012 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DV6LH UT WOS:000383046500002 ER PT J AU Love, CN Winzeler, ME Beasley, R Scott, DE Nunziata, SO Lance, SL AF Love, Cara N. Winzeler, Megan E. Beasley, Rochelle Scott, David E. Nunziata, Schyler O. Lance, Stacey L. TI Patterns of amphibian infection prevalence across wetlands on the Savannah River Site, South Carolina, USA SO DISEASES OF AQUATIC ORGANISMS LA English DT Article DE Batrachochytrium; Chytrid; Metals; Ranavirus; Wetland ID AMBYSTOMA-TIGRINUM VIRUS; BATRACHOCHYTRIUM-DENDROBATIDIS; POPULATION DECLINES; CHYTRID FUNGUS; WIDESPREAD OCCURRENCE; DISEASE DYNAMICS; BUFO-TERRESTRIS; RANAVIRUS; CHYTRIDIOMYCOSIS; MORTALITY AB Amphibian diseases, such as chytridiomycosis caused by Batrachochytrium dendrobatidis (Bd) and ranaviral disease caused by ranaviruses, are often linked to global amphibian population declines, yet the ecological dynamics of both pathogens are poorly understood. The goal of our study was to determine the baseline prevalence, pathogen loads, and co-infection rate of Bd and ranavirus across the Savannah River Site (SRS) in South Carolina, USA, a region with rich amphibian diversity and a history of amphibian-based research. We tested over 1000 individuals, encompassing 21 amphibian species from 11 wetlands for both Bd and ranavirus. The prevalence of Bd across individuals was 9.7%. Using wetland means, the mean (+/- SE) Bd prevalence was 7.9 +/- 2.9%. Among toad species, Anaxyrus terrestris had 95 and 380% greater odds of being infected with Bd than Scaphiopus holbrookii and Gastrophryne carolinensis, respectively. Odds of Bd infection in adult A. terrestris and Lithobates sphenocephalus were 75 to 77% greater in metal-contaminated sites. The prevalence of ranavirus infections across all individuals was 37.4%. Mean wetland ranavirus prevalence was 29.8 +/- 8.8% and was higher in post-metamorphic individuals than in aquatic larvae. Ambystoma tigrinum had 83 to 85% higher odds of ranavirus infection than A. opacum and A. talpoideum. We detected a 4.8% co-infection rate, with individuals positive for ranavirus having a 5% higher occurrence of Bd. In adult Anaxyrus terrestris, odds of Bd infection were 13% higher in ranavirus-positive animals and odds of co-infection were 23% higher in contaminated wetlands. Overall, we found the pathogen prevalence varied by wetland, species, and life stage. C1 [Love, Cara N.; Winzeler, Megan E.; Beasley, Rochelle; Scott, David E.; Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Love, Cara N.; Winzeler, Megan E.] Univ Georgia, Odum Sch Ecol, Athens, GA 30602 USA. [Nunziata, Schyler O.] Univ Kentucky, Dept Biol Sci, Lexington, KY 40506 USA. RP Lance, SL (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM lance@srel.uga.edu OI Winzeler, Megan/0000-0002-0361-1582 FU US Department of Energy [DE-FC09-07SR22506]; DOE National Nuclear Security Administration FX We thank C. Muletz and N. McInerney for providing the Bd standards, P. Johnson for providing the oligo sequence for the ranavirus standard, and J. Hoverman and S. Kimble for assistance with optimizing the ranavirus qPCR. A. L. Bryan and D. Soteropolous provided field and laboratory assistance, and R. W. Flynn, C. Rumrill, S. Weir, A. Coleman, J. O'Bryhim and 2 anonymous reviewers provided valuable comments on earlier versions of the manuscript. This research was partially supported by US Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation, and was also made possible by the status of the SRS as a National Environmental Research Park (NERP), as well as the protection of research wetlands in the SRS Set-Aside Program. Project funding was provided by the DOE National Nuclear Security Administration. Animals were collected under SCDNR permit #G-09-03 following IACUC procedures (AUP A2009 10-175-Y2-A0) from the University of Georgia. NR 70 TC 0 Z9 0 U1 13 U2 14 PU INTER-RESEARCH PI OLDENDORF LUHE PA NORDBUNTE 23, D-21385 OLDENDORF LUHE, GERMANY SN 0177-5103 EI 1616-1580 J9 DIS AQUAT ORGAN JI Dis. Aquat. Org. PD AUG 31 PY 2016 VL 121 IS 1 BP 1 EP 14 DI 10.3354/dao03039 PG 14 WC Fisheries; Veterinary Sciences SC Fisheries; Veterinary Sciences GA DX2ZV UT WOS:000384243300001 PM 27596855 ER PT J AU Tran, AP Dafflon, B Hubbard, SS Kowalsky, MB Long, P Tokunaga, TK Williams, KH AF Anh Phuong Tran Dafflon, Baptiste Hubbard, Susan S. Kowalsky, Michael B. Long, Philip Tokunaga, Tetsu K. Williams, Kenneth H. TI Quantifying shallow subsurface water and heat dynamics using coupled hydrological-thermal-geophysical inversion SO HYDROLOGY AND EARTH SYSTEM SCIENCES LA English DT Article ID ELECTRICAL-RESISTIVITY TOMOGRAPHY; DATA INCORPORATING TOPOGRAPHY; GROUND-PENETRATING RADAR; DC RESISTIVITY; SOIL-MOISTURE; TIME-LAPSE; HYDROGEOPHYSICAL INVERSION; HYDRAULIC-PROPERTIES; TEMPERATURE; CONDUCTIVITY AB Improving our ability to estimate the parameters that control water and heat fluxes in the shallow subsurface is particularly important due to their strong control on recharge, evaporation and biogeochemical processes. The objectives of this study are to develop and test a new inversion scheme to simultaneously estimate subsurface hydrological, thermal and petrophysical parameters using hydrological, thermal and electrical resistivity tomography (ERT) data. The inversion scheme - which is based on a nonisothermal, multiphase hydrological model - provides the desired subsurface property estimates in high spatiotemporal resolution. A particularly novel aspect of the inversion scheme is the explicit incorporation of the dependence of the subsurface electrical resistivity on both moisture and temperature. The scheme was applied to synthetic case studies, as well as to real datasets that were autonomously collected at a biogeochemical field study site in Rifle, Colorado. At the Rifle site, the coupled hydrological-thermal-geophysical inversion approach well predicted the matric potential, temperature and apparent resistivity with the Nash-Sutcliffe efficiency criterion greater than 0.92. Synthetic studies found that neglecting the subsurface temperature variability, and its effect on the electrical resistivity in the hydrogeophysical inversion, may lead to an incorrect estimation of the hydrological parameters. The approach is expected to be especially useful for the increasing number of studies that are taking advantage of autonomously collected ERT and soil measurements to explore complex terrestrial system dynamics. C1 [Anh Phuong Tran; Dafflon, Baptiste; Hubbard, Susan S.; Kowalsky, Michael B.; Long, Philip; Tokunaga, Tetsu K.; Williams, Kenneth H.] Lawrence Berkeley Natl Lab, Climate & Ecosyst Div, Earth & Environm Sci Area, Berkeley, CA 94720 USA. RP Tran, AP (reprint author), Lawrence Berkeley Natl Lab, Climate & Ecosyst Div, Earth & Environm Sci Area, Berkeley, CA 94720 USA. EM aptran@lbl.gov RI Hubbard, Susan/E-9508-2010; Long, Philip/F-5728-2013; Tokunaga, Tetsu/H-2790-2014; Williams, Kenneth/O-5181-2014; Dafflon, Baptiste/G-2441-2015; Tran, Anh Phuong/G-1911-2015 OI Long, Philip/0000-0003-4152-5682; Tokunaga, Tetsu/0000-0003-0861-6128; Williams, Kenneth/0000-0002-3568-1155; Tran, Anh Phuong/0000-0002-7703-6621 FU Sub-surface Science Scientific Focus Area - US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This material is based upon work supported as part of the Sub-surface Science Scientific Focus Area funded by the US Department of Energy, Office of Science, Office of Biological and Environmental Research under award number DE-AC02-05CH11231. The authors would like to thank Stefan Finsterle for providing iTOUGH2 codes and support, and Thomas Gunther for providing the BERT codes. NR 54 TC 0 Z9 0 U1 7 U2 7 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1027-5606 EI 1607-7938 J9 HYDROL EARTH SYST SC JI Hydrol. Earth Syst. Sci. PD AUG 31 PY 2016 VL 20 IS 8 BP 3477 EP 3491 DI 10.5194/hess-20-3477-2016 PG 15 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA DW8GM UT WOS:000383892900001 ER PT J AU Fu, SF Zhu, CZ Song, JH Engelhard, M Xia, HB Du, D Lin, YH AF Fu, Shaofang Zhu, Chengzhou Song, Junhua Engelhard, Mark Xia, Haibing Du, Dan Lin, Yuehe TI PdCuPt Nanocrystals with Multibranches for Enzyme-Free Glucose Detection SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE branched nanocrystals; alloys; galvanic replacement reaction; enzyme-free biosensors; glucose detection ID ELECTROCHEMICAL SYNTHESIS; ONE-STEP; GRAPHENE; SENSORS; NANOSTRUCTURES; NANOWIRES; PLATINUM; ELECTROOXIDATION; NANOCOMPOSITES; NANOPARTICLES AB By carefully controlling the synthesis condition, branched PtCu bimetallic templates were synthesized in aqueous solution. After the galvanic replacement reaction between PtCu templates and the Pt precursors, PdCuPt trimetallic nanocrystals with branched structures were obtained. Owing to the open structure and the optimized composition, the electrochemical experimental results reveal that the PdCuPt trimetallic nanocrystals possess high electrocatalytic activity, selectivity and stability for the oxidation of glucose in alkaline solution. In detail, a detection limit of 1.29 mu M and a sensitivity of 378 mu A/mM/cm(2) are achieved. The good electrocatalytic performance should be attributed to the unique branched nanostructure as well as the synergistic effect among metals. The superior catalytic properties suggest that these nanocrystals are promising for enzyme-free detection of glucose. C1 [Fu, Shaofang; Zhu, Chengzhou; Song, Junhua; Du, Dan; Lin, Yuehe] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Engelhard, Mark; Lin, Yuehe] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Xia, Haibing] Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China. RP Lin, YH (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA.; Lin, YH (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. EM yuehe.lin@wsu.edu RI Zhu, Chengzhou/M-3566-2014; Xia, Haibing/A-8711-2008; FU, SHAOFANG/D-2328-2016 OI Xia, Haibing/0000-0003-2262-7958; FU, SHAOFANG/0000-0002-7871-6573 FU Washington State University, USA FX This work was supported by a start-up funding of Washington State University, USA. NR 32 TC 1 Z9 1 U1 24 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 31 PY 2016 VL 8 IS 34 BP 22196 EP 22200 DI 10.1021/acsami.6b06158 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU9CP UT WOS:000382514100042 PM 27494365 ER PT J AU Wu, XH Xu, GL Zhong, GM Gong, ZL McDonald, MJ Zheng, SY Fu, RQ Chen, ZH Amine, K Yang, Y AF Wu, Xuehang Xu, Gui-Liang Zhong, Guiming Gong, Zhengliang McDonald, Matthew J. Zheng, Shiyao Fu, Riqiang Chen, Zonghai Amine, Khalil Yang, Yong TI Insights into the Effects of Zinc Doping on Structural Phase Transition of P2-Type Sodium Nickel Manganese Oxide Cathodes for High-Energy Sodium Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE sodium ion battery; cathode material; Zn doping sodium nickel manganese oxide; structural transition ID ELECTROCHEMICAL PROPERTIES; POSITIVE ELECTRODE; RATE PERFORMANCE; NA BATTERIES; LITHIUM; STABILITY; SUBSTITUTION; CAPACITY; STORAGE AB P2-type sodium nickel manganese oxide-based cathode materials with higher energy densities are prime candidates for :,applications in rechargeable sodium ion batteries. A systematic study combining in situ high energy X-ray diffraction (HEXRD), ex situ X-ray absorption fine spectroscopy (XAFS), transmission electron microscopy (TEM), and solid-state nuclear magnetic resonance (SS-NMR) techniques was carried out to gain a deep insight into the :structural evolution of P-2-Na0.66Ni0.33-xZnxMn0.67O2 (x = 0, 0.07) :during cycling. In situ HEXRD and ex situ TEM. measurements indicate that an irreversible phase transition occurs upon sodium insertion-extraction of Na0.66Ni0.33Mn0.67O2. Zinc doping of this system results in a high structural reversibility. XAFS measurements indicate that both materials are almost completely dependent on the Ni4+/Ni3+/Ni2+ redox couple to provide charge/discharge capacity. SS-NMR measurements indicate that both reversible and irreversible migration of transition metal ions into the sodium layer occurs in the material at the fully charged state. The irreversible migration of transition metal ions triggers a structural distortion, leading to the observed capacity and voltage fading. Our results allow a new understanding of the importance of improving the stability of transition metal layers. C1 [Wu, Xuehang; Zhong, Guiming; McDonald, Matthew J.; Zheng, Shiyao; Yang, Yong] Xiamen Univ, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Fujian, Peoples R China. [Wu, Xuehang; Zhong, Guiming; McDonald, Matthew J.; Zheng, Shiyao; Yang, Yong] Xiamen Univ, Dept Chem, Xiamen 361005, Fujian, Peoples R China. [Gong, Zhengliang; Yang, Yong] Xiamen Univ, Sch Energy Res, Xiamen 361005, Peoples R China. [Xu, Gui-Liang; Chen, Zonghai; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. [Wu, Xuehang] Guangxi Univ, Collaborat Innovat Ctr Renewable Energy Mat, Nanning 530004, Guangxi, Peoples R China. [Fu, Riqiang] Natl High Magnet Field Lab, 1800 East Paul Dirac Dr, Tallahassee, FL 32310 USA. RP Yang, Y (reprint author), Xiamen Univ, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Fujian, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Dept Chem, Xiamen 361005, Fujian, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Sch Energy Res, Xiamen 361005, Peoples R China. EM yyang@xmu.edu.cn RI Chen, Zhong/G-4601-2010; Yang, Yong/G-4650-2010; XU, GUILIANG/F-3804-2017 FU National Natural Science Foundation of China [21233004, 21473148, 21428303]; National Basic Research Program of China (973 program) [2011CB935903] FX The authors acknowledge financial support of their research from the National Natural Science Foundation of China (Grant Nos. 21233004, 21473148, and 21428303) and the National Basic Research Program of China (973 program, Grant No. 2011CB935903). We sincerely acknowledge Dr. W. Wen and other staff of the XAFS beamline of Shanghai Synchrotron Radiation Facility for their support. R.F. is also indebted to the support for being a PCOSS fellow by the State Key Lab of Physical Chemistry of Solid Surfaces, Xiamen University, China. NR 39 TC 4 Z9 4 U1 65 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 31 PY 2016 VL 8 IS 34 BP 22227 EP 22237 DI 10.1021/acsami.6b06701 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU9CP UT WOS:000382514100046 PM 27494351 ER PT J AU Steinmann, V Chakraborty, R Rekemeyer, PH Hartman, K Brandt, RE Polizzotti, A Yang, CX Moriarty, T Gradecak, S Gordon, RG Buonassisi, T AF Steinmann, Vera Chakraborty, Rupak Rekemeyer, Paul H. Hartman, Katy Brandt, Riley E. Polizzotti, Alex Yang, Chuanxi Moriarty, Tom Gradecak, Silvija Gordon, Roy G. Buonassisi, Tonio TI A Two-Step Absorber Deposition Approach To Overcome Shunt Losses in Thin-Film Solar Cells: Using Tin Sulfide as a Proof-of-Concept Material System SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE thin-films; photovoltaics; novel absorber materials; tin sulfide; device shunting; performance reliability ID DEFECT-TOLERANT SEMICONDUCTORS; ATOMIC LAYER DEPOSITION; PHOTOVOLTAIC-DEVICE; ENERGY CONVERSION AB As novel absorber materials are developed and screened for their photovoltaic (PV) properties, the challenge remains to reproducibly test promising candidates for high-performing PV devices. Many early-stage devices are prone to device shunting due to pinholes in the absorber layer, producing "false-negative" results. Here, we demonstrate a device engineering solution toward a robust device architecture, using a two-step absorber deposition approach. We use tin sulfide (SnS) as a test absorber material. The SnS bulk is processed at high temperature (400 degrees C) to stimulate grain growth, followed by a much thinner, low-temperature (200 degrees C) absorber deposition. At a lower process temperature, the thin absorber overlayer contains significantly smaller, densely packed grains, which are likely to provide a continuous coating and fill pinholes in the underlying absorber bulk. We compare this two-step approach to the more standard approach of using a semi-insulating buffer layer directly on top of the annealed absorber bulk, and we demonstrate a more than 3.5X superior shunt resistance R-sh with smaller standard error sigma(Rsh). Electron-beam-induced current (EBIC) measurements indicate a lower density of pinholes in the SnS absorber bulk when using the two-step absorber deposition approach. We correlate those findings to improvements in the device performance and device performance reproducibility. C1 [Steinmann, Vera; Chakraborty, Rupak; Hartman, Katy; Brandt, Riley E.; Polizzotti, Alex; Buonassisi, Tonio] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Rekemeyer, Paul H.; Gradecak, Silvija] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Yang, Chuanxi; Gordon, Roy G.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Moriarty, Tom] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Steinmann, V (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM vsteinma@mit.edu; buonassisi@mit.edu OI Rekemeyer, Paul/0000-0002-5901-9027 FU TOTAL SA grant; Engineering Research Center Program of the National Science Foundation; Office of Energy Efficiency and Renewable Energy of the Department of Energy under NSF [EEC-1041895]; U.S. Department of Energy through SunShot Initiative [DE-EE0005329]; Alexander von Humboldt foundation; MITei/TOTAL Energy fellowship; NSF GRFP; NSF [DMR-08-19762, ECS-0335765]; Center for Nanoscale Systems at Harvard University FX The authors thank K. Emery from the cell certification team at the National Renewable Energy Laboratory for his assistance with current density voltage measurements, M. L. Castillo for her help with substrate preparation, and J. R Poindexter and R.L.Z. Hoye for fruitful scientific discussions. This work was supported by a TOTAL SA grant, by the Engineering Research Center Program of the National Science Foundation, by the Office of Energy Efficiency and Renewable Energy of the Department of Energy under NSF Cooperative Agreement No. EEC-1041895, and by the U.S. Department of Energy through the SunShot Initiative under contract DE-EE0005329. V.S., R.C., R.E.B., and A.P. acknowledge the support of the Alexander von Humboldt foundation, a MITei/TOTAL Energy fellowship, and two NSF GRFP fellowships, respectively. This work made use of the Center for Materials Science and Engineering at MIT which is supported by the NSF under award DMR-08-19762, and the Center for Nanoscale Systems at Harvard University which is supported by NSF under award ECS-0335765. NR 29 TC 0 Z9 0 U1 9 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 31 PY 2016 VL 8 IS 34 BP 22664 EP 22670 DI 10.1021/acsami.6b07198 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU9CP UT WOS:000382514100098 PM 27494110 ER PT J AU Woods, TA Mendez, HM Ortega, S Shi, XR Marx, D Bai, JF Moxley, RA Nagaraja, TG Graves, SW Deshpande, A AF Woods, Travis A. Mendez, Heather M. Ortega, Sandy Shi, Xiaorong Marx, David Bai, Jianfa Moxley, Rodney A. Nagaraja, T. G. Graves, Steven W. Deshpande, Alina TI Development of 11-Plex MOL-PCR Assay for the Rapid Screening of Samples for Shiga Toxin-Producing Escherichia coil SO FRONTIERS IN CELLULAR AND INFECTION MICROBIOLOGY LA English DT Article DE STEC; MOL-PCR; multiplex PCR; Shiga toxin; EHEC ID MAJOR VIRULENCE FACTORS; MULTIPLEX PCR; CATTLE FECES; COLI INFECTIONS; O157 SEROGROUPS; UNITED-STATES; GENES; O145; O111; O103 AB Strains of Shiga toxin-producing Escherichia coli (STEC) are a serious threat to the health, with approximately half of the STEC related food-borne illnesses attributable to contaminated beef. We developed an assay that was able to screen samples for several important STEC associated serogroups (O26, O45, O103, O104, O111, O121, O145, O157) and three major virulence factors (eae, stx(1), stx(2)) in a rapid and multiplexed format using the Multiplex oligonucleotide ligation-PCR (MOL-PCR) assay chemistry. This assay detected unique STEC DNA signatures and is meant to be used on samples from various sources related to beef production, providing a multiplex and high-throughput complement to the multiplex PCR assays currently in use. Multiplex oligonucleotide ligation-PCR (MOL-PCR) is a nucleic acid-based assay chemistry that relies on flow cytometry/image cytometry and multiplex microsphere arrays for the detection of nucleic acid-based signatures present in target agents. The STEC MOL-PCR assay provided greater than 90% analytical specificity across all sequence markers designed when tested against panels of DNA samples that represent different STEC serogroups and toxin gene profiles. This paper describes the development of the 11-plex assay and the results of its validation. This highly multiplexed, but more importantly dynamic and adaptable screening assay allows inclusion of additional signatures as they are identified in relation to public health. As the impact of STEC associated illness on public health is explored additional information on classification will be needed on single samples; thus, this assay can serve as the backbone for a complex screening system. C1 [Woods, Travis A.; Mendez, Heather M.; Graves, Steven W.] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Mendez, Heather M.] New Mexico Consortium, Los Alamos, NM USA. [Ortega, Sandy] Univ Rochester, Translat Biomed Sci, Rochester, NY USA. [Shi, Xiaorong; Bai, Jianfa; Nagaraja, T. G.] Kansas State Univ, Coll Vet Med, Dept Diagnost Med Pathobiol, Manhattan, KS 66506 USA. [Marx, David] Univ Nebraska Lincoln, Dept Stat, Lincoln, NE USA. [Moxley, Rodney A.] Univ Nebraska Lincoln, Sch Vet Med & Biomed Sci, Lincoln, NE USA. [Deshpande, Alina] Los Alamos Natl Lab, Analyt Intelligence & Technol Div, Los Alamos, NM USA. RP Deshpande, A (reprint author), Los Alamos Natl Lab, Analyt Intelligence & Technol Div, Los Alamos, NM USA. EM deshpande_a@lanl.gov FU U.S. Department of Agriculture (USDA), National Institute of Food and Agriculture [2012-68003-30155] FX This material is based on work that is supported by the U.S. Department of Agriculture (USDA), National Institute of Food and Agriculture under award 2012-68003-30155. NR 35 TC 0 Z9 0 U1 2 U2 2 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2235-2988 J9 FRONT CELL INFECT MI JI Front. Cell. Infect. Microbiol. PD AUG 31 PY 2016 VL 6 AR 92 DI 10.3389/fcimb.2016.00092 PG 12 WC Immunology; Microbiology SC Immunology; Microbiology GA DU5VY UT WOS:000382282700001 PM 27630828 ER PT J AU Azad, A Rajwa, B Pothen, A AF Azad, Ariful Rajwa, Bartek Pothen, Alex TI Immunophenotype Discovery, Hierarchical Organization, and Template-Based Classification of Flow Cytometry Samples SO FRONTIERS IN ONCOLOGY LA English DT Article DE flow cytometry; clusters; meta-clusters; template; matching; classification ID ACUTE MYELOID-LEUKEMIA; CELL-POPULATIONS; EXPRESSION; PROGNOSIS; IDENTIFICATION; COMPENSATION; DISTANCE; DISPLAY AB We describe algorithms for discovering immunophenotypes from large collections of flow cytometry samples and using them to organize the samples into a hierarchy based on phenotypic similarity. The hierarchical organization is helpful for effective and robust cytometry data mining, including the creation of collections of cell populations characteristic of different classes of samples, robust classification, and anomaly detection. We summarize a set of samples belonging to a biological class or category with a statistically derived template for the class. Whereas individual samples are represented in terms of their cell populations (clusters), a template consists of generic meta-populations (a group of homogeneous cell populations obtained from the samples in a class) that describe key phenotypes shared among all those samples. We organize an FC data collection in a hierarchical data structure that supports the identification of immunophenotypes relevant to clinical diagnosis. A robust template-based classification scheme is also developed, but our primary focus is in the discovery of phenotypic signatures and inter-sample relationships in an FC data collection. This collective analysis approach is more efficient and robust since templates describe phenotypic signatures common to cell populations in several samples while ignoring noise and small sample-specific variations. We have applied the template-based scheme to analyze several datasets, including one representing a healthy immune system and one of acute myeloid leukemia (AML) samples. The last task is challenging due to the phenotypic heterogeneity of the several subtypes of AML. However, we identified thirteen immunophenotypes corresponding to subtypes of AML and were able to distinguish acute promyelocytic leukemia (APL) samples with the markers provided. Clinically, this is helpful since APL has a different treatment regimen from other subtypes of AML. Core algorithms used in our data analysis are available in the flowMatch package at www.bioconductor.org. It has been downloaded nearly 6,000 times since 2014. C1 [Azad, Ariful] Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA USA. [Rajwa, Bartek] Purdue Univ, Bindley Biosci Ctr, W Lafayette, IN 47907 USA. [Pothen, Alex] Purdue Univ, Dept Comp Sci, W Lafayette, IN 47907 USA. RP Pothen, A (reprint author), Purdue Univ, Dept Comp Sci, W Lafayette, IN 47907 USA. EM apothen@purdue.edu RI Rajwa, Bartek/B-3169-2009 OI Rajwa, Bartek/0000-0001-7540-8236 FU NIBIB NIH HHS [R21 EB015707] NR 60 TC 0 Z9 0 U1 1 U2 1 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2234-943X J9 FRONT ONCOL JI Front. Oncol. PD AUG 31 PY 2016 VL 6 AR 188 DI 10.3389/fonc.2016.00188 PG 20 WC Oncology SC Oncology GA DU5XI UT WOS:000382286600001 PM 27630823 ER PT J AU Park, W Park, SJ Cho, S Shin, H Jung, YS Lee, B Na, K Kim, DH AF Park, Wooram Park, Sin-Jung Cho, Soojeong Shin, Heejun Jung, Young-Seok Lee, Byeongdu Na, Kun Kim, Dong-Hyun TI Intermolecular Structural Change for Thermoswitchable Polymeric Photosensitizer SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AQUEOUS METHYLCELLULOSE SOLUTIONS; PHOTODYNAMIC THERAPY; SINGLET OXYGEN; FIBRILLAR STRUCTURE; GOLD NANORODS; CANCER; HYDROXYPROPYLCELLULOSE; WATER; NANOPARTICLES; PHEOPHORBIDE AB We developed a thermoswitchable polymeric photosensitizer (T-PPS) by conjugating PS (Pheophorbide-a, PPb-a) to a. temperature-responsive polymer backbone of biacoinpatible hydroxypropyl cellulose. Self-quenched PS molecules linked in close proximity by pi-pi stacking in T-PPS were easily transited to an active monomeric state by the temperature-induced phase transition of polymer backbones. The temperature: responsive intermolecular interaction changes of PS Molecules in T-PPS were demonstrated in synchrotron small-angle X-ray scattering and UV-vis spectrophotometer analysis. The T-PPS allowed switchable activation and synergistically enhanced cancer cell killing effect at the hyperthermia temperature (45 degrees C). Our developed T-PPS has the considerable potential not only as a new class of photomedicine in clinics but also as a biosensor based on temperature responsiveness. C1 [Park, Wooram; Cho, Soojeong; Kim, Dong-Hyun] Northwestern Univ, Dept Radiol, Feinberg Sch Med, Chicago, IL 60611 USA. [Kim, Dong-Hyun] Northwestern Univ, Robert H Lurie Comprehens Canc Ctr, Chicago, IL 60611 USA. [Park, Sin-Jung; Shin, Heejun; Jung, Young-Seok; Na, Kun] Catholic Univ Korea, Dept Biotechnol, Ctr Photomed, Bucheon Si 14662, Gyeonggi Do, South Korea. [Lee, Byeongdu] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Park, Sin-Jung] Univ Illinois, Coll Pharm, Dept Biopharmaceut Sci, Chicago, IL 60612 USA. RP Kim, DH (reprint author), Northwestern Univ, Dept Radiol, Feinberg Sch Med, Chicago, IL 60611 USA.; Kim, DH (reprint author), Northwestern Univ, Robert H Lurie Comprehens Canc Ctr, Chicago, IL 60611 USA.; Na, K (reprint author), Catholic Univ Korea, Dept Biotechnol, Ctr Photomed, Bucheon Si 14662, Gyeonggi Do, South Korea.; Lee, B (reprint author), Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM blee@aps.anl.gov; kna6997@catholic.ac.kr; dhkim@northwestern.edu OI Kim, Dong-Hyun/0000-0001-6815-3319 FU NCI [R01CA141047, R21CA173491, R21EB017986, R21CA185274]; NIBIB; Basic Research Laboratory (BRL) Program through the National Research Foundation of Korea (NRF) - Korean government (MSIP) [2015R1A4A1042350]; MICCoM as part of the Computational Materials Sciences Program - U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE Office of Science [DE-AC02-06CH11357] FX This work was supported by four grants R01CA141047, R21CA173491, R21EB017986, and R21CA185274 from the NCI and NIBIB. This research was also supported by the Basic Research Laboratory (BRL) Program (no. 2015R1A4A1042350), through the National Research Foundation of Korea (NRF) grant funded by the Korean government (MSIP). B.L. was supported by MICCoM as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. This work used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. NR 44 TC 1 Z9 1 U1 30 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10734 EP 10737 DI 10.1021/jacs.6b04875 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300005 PM 27535204 ER PT J AU Zhao, YB Lee, SY Becknell, N Yaghi, OM Angell, CA AF Zhao, Yingbo Lee, Seung-Yul Becknell, Nigel Yaghi, Omar M. Angell, C. Austen TI Nanoporous Transparent MOF Glasses with Accessible Internal Surface SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; FORMING LIQUIDS; PHASE-TRANSITION; AMORPHOUS ICE; COORDINATION; TEMPERATURE; SOLIDS; NETWORKS; CRYSTALS; STATE AB While glassy materials can be made from virtually every class of liquid (metallic, molecular, covalent, and ionic), to date, formation of glasses in which structural units impart porosity on the nanoscopic level remains Undeveloped. In view of the well-established porosity of metal organic frameworks (MOFs) and the flexibility of 'their design, we have sought to combine their formation principles with the general versatility of glassy materials. Although the preparation of glassy MOFs can be achieved by amorphization 'of crystalline frameworks, transparent glassy MOFs exhibiting permanent porosity accessible to gases are yet to be reported. Here, we present a generalizable chemical strategy for making such MOF glasses by assembly from viscous solutions of metal node and organic strut and subsequent evaporation of a plasticizer modulator solvent. This process yields glasses With 300 m(2)/g internal surface area (obtained' from N-2 adsorption isotherms) and a 2 nm pore pore separation. On a volumetric basis, this porosity (0.33 cm(3)/cm(3)) is 3 times that of the early MOFs (0.11 cm(3)/cm(3) for MOF-2) and within range of the most porous MOFs known (0.60 cm(3)/cm(3) for MOF-5). We believe the porosity originates from a 3D covalent network as evidenced by the disappearance-of the glass transition signature as the solvent is removed and the highly cross-linked nanostructure builds up. Our work represents an important step forward in translating the versatility and porosity of MOFs to glassy materials. C1 [Zhao, Yingbo; Becknell, Nigel; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Zhao, Yingbo; Becknell, Nigel; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lee, Seung-Yul; Angell, C. Austen] Arizona State Univ, Sch Mol Sci, Tempe, AZ 85287 USA. [Yaghi, Omar M.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Kavli Energy NanoSci Inst Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Angell, CA (reprint author), Arizona State Univ, Sch Mol Sci, Tempe, AZ 85287 USA.; Yaghi, OM (reprint author), King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. EM yaghi@berkeley.edu; caa@asu.edu OI Yaghi, Omar/0000-0002-5611-3325; Becknell, Nigel/0000-0001-7857-6841 FU Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02- 05CH11231]; U.S. Department of Energy [DE-AC02-05CH11231, 6920968]; BASF SE (Ludwigshafen, Germany); King Abdulaziz City for Science and Technology (Riyadh, Saudi Arabia); Suzhou Industrial Park fellowship FX This work made use of facilities at the Molecular Foundry and Advanced Light Source BL 10.3.2. The Advanced Light Source and Molecular Foundry are supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02- 05CH11231. We acknowledge Mr. N. Kornienko for help on the MOF thin film preparation, Dr. Y. Ma and Prof. O. Terasaki for discussions on TEM, Dr. J. Guo and Dr. X. Feng for help and discussion of the EXAFS study, Dr. H. Furukawa for help on the density measurement, and Mr. J. Yang for help and discussion on nitrogen isotherm measurements. S.-Y.L. and C.A.A. acknowledge support of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 6920968, under the Batteries for Advanced Transportation Technologies Program. Partial financial support for aspects of the synthesis and porosity measurements is provided to O.M.Y. by BASF SE (Ludwigshafen, Germany) and King Abdulaziz City for Science and Technology (Riyadh, Saudi Arabia). Y.Z. acknowledges support of the Suzhou Industrial Park fellowship. NR 40 TC 1 Z9 1 U1 77 U2 95 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10818 EP 10821 DI 10.1021/jacs.6b07078 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300026 PM 27539546 ER PT J AU Catarineu, NR Schoedel, A Urban, P Morla, MB Trickett, CA Yaghi, OM AF Catarineu, Noelle R. Schoedel, Alexander Urban, Philipp Morla, Maureen B. Trickett, Christopher A. Yaghi, Omar M. TI Two Principles of Reticular Chemistry Uncovered in a Metal Organic Framework of Heterotritopic Linkers and Infinite Secondary Building Units SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID FUNCTIONAL-GROUPS; POROUS CRYSTALS; COORDINATION; POLYMERS AB Structural diversity of metal organic frameworks (MOFs) has been largely limited to linkers with at most two different types of coordinating groups. MOFs constructed from linkers with three or more nonidentical coordinating groups have not been explored. Here, we report a robust and porous crystalline MOF, Zo(3)(PBSP)(2) or MOF-910, constructed from a novel linker PBSP(phenylyne-1-benzoate, 3-benzosemiquinonate, 5-oxidopyridine) bearing three distinct types of coordinative functionality. The MOF adopts a complex and previously unreported topology termed tto. Our study suggests that simple, symmetric linkers are not a necessity for formation of crystalline extended structures and that new, more complex topologies are attainable with irregular, heterotopic linkers. This work illustrates two principles of reticular chemistry: first, selectivity for helical over straight rod secondary building units (SBUs) is achievable with polyheterotopic linkers, and second, the pitch of the resulting helical SBUs may be fine-tuned based on the metrics of the polyheterotopic linker. C1 [Catarineu, Noelle R.; Schoedel, Alexander; Urban, Philipp; Morla, Maureen B.; Trickett, Christopher A.; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Div Mat Sci, Lawrence Berkeley Natl Lab,Kavli Energy NanoSci I, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Div Mat Sci, Lawrence Berkeley Natl Lab,Kavli Energy NanoSci I, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. EM yaghi@berkeley.edu RI Schoedel, Alexander/B-3971-2013; OI Schoedel, Alexander/0000-0001-6548-9300; Yaghi, Omar/0000-0002-5611-3325 FU BASF SE (Ludwigshafen, Germany); NSF; UC Berkeley Graduate Division; German Research Foundation (DFG) [PU 286/1-1, SCHO 1639/1-1]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Financial support for this work was provided by BASF SE (Ludwigshafen, Germany). N.R.C. thanks the NSF for a Graduate Research Fellowship and the UC Berkeley Graduate Division for a Chancellor's Fellowship. A.S. and P.U. acknowledge the German Research Foundation (DFG, PU 286/1-1 and SCHO 1639/1-1) for financial support. We thank Wenjia Ma and Elena Lopez-Maya for technical assistance with MOF synthesis, Drs. Adam Duong, Michael O'Keeffe, and Hans-Beat Burgi for useful discussions, Dr. Ruchira Chatterjee for assistance with EPR measurements, and Drs. Kevin J. Gagnon and Simon J. Teat for help collecting single-crystal XRD data at Beamline 11.3.1 of the Advanced Light Source at Lawrence Berkeley National Lab, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 36 TC 5 Z9 5 U1 50 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10826 EP 10829 DI 10.1021/jacs.6b07267 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300028 PM 27517606 ER PT J AU Mostofian, B Cai, CM Smith, MD Petridis, L Cheng, XL Wyman, CE Smith, JC AF Mostofian, Barmak Cai, Charles M. Smith, Micholas Dean Petridis, Loukas Cheng, Xiaolin Wyman, Charles E. Smith, Jeremy C. TI Local Phase Separation of Co-solvents Enhances Pretreatment of Biomass for Bioenergy Applications SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PARTICLE MESH EWALD; LIGNOCELLULOSIC BIOMASS; CELLULOSE MICROFIBRILS; MOLECULAR-DYNAMICS; IONIC LIQUIDS; TETRAHYDROFURAN-WATER; CRYSTALLINE CELLULOSE; SOLVATION STRUCTURES; ETHANOL-PRODUCTION; BIOGAS PRODUCTION AB Pretreatment facilitates more complete deconstruction of plant biomass to enable more economic production of lignocellulosic biofuels and byproducts. Various co-solvent pretreatments have demonstrated advantages relative to aqueous-only methods by enhancing lignin removal to allow unfettered access to cellulose. However, there is a limited mechanistic understanding of the interactions between the co-solvents and cellulose that impedes further improvement of such pretreatment methods. Recently, tetrahydrofuran (THF) has been identified as a highly effective co-solvent for the pretreatment and fractionation of biomass. To elucidate the mechanism of the THF water interactions with cellulose, we pair simulation and experimental data demonstrating that enhanced solubilization of cellulose can be achieved by the THF water co-solvent system at equivolume mixtures and moderate temperatures (<445 K). The simulations show that THF and water spontaneously phase separate on the local surface of a cellulose fiber, owing to hydrogen bonding of water molecules with the hydrophilic cellulose faces and stacking of THF molecules on the hydrophobic faces. Furthermore, a single fully solvated cellulose chain is shown to be preferentially bound by water molecules in the THF water mixture. In light of these findings, co-solvent reactions were performed on microcrystalline cellulose and maple wood to show thatTHF significantly enhanced cellulose deconstruction and lignocellulose solubilization at simulation conditions, enabling a highly versatile and efficient biomass pretreatment and fractionation method. C1 [Mostofian, Barmak; Smith, Micholas Dean; Petridis, Loukas; Cheng, Xiaolin; Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA. [Mostofian, Barmak] Oak Ridge Natl Lab, Joint Inst Biol Sci, Oak Ridge, TN 37830 USA. [Mostofian, Barmak; Cai, Charles M.; Smith, Micholas Dean; Petridis, Loukas; Cheng, Xiaolin; Wyman, Charles E.; Smith, Jeremy C.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37830 USA. [Cai, Charles M.; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol CE CERT, Riverside, CA 92507 USA. [Cai, Charles M.; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, Riverside, CA 92521 USA. [Smith, Micholas Dean; Petridis, Loukas; Cheng, Xiaolin; Smith, Jeremy C.] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. RP Smith, JC (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA.; Smith, JC (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37830 USA.; Smith, JC (reprint author), Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. EM smithjc@ornl.gov RI Petridis, Loukas/B-3457-2009; smith, jeremy/B-7287-2012; OI Petridis, Loukas/0000-0001-8569-060X; smith, jeremy/0000-0002-2978-3227; Smith, Micholas/0000-0002-0777-7539 FU BioEnergy Science Center, a U.S. Department of Energy (DOE) Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; INCITE - DOE Office of Science [DE-AC05-00OR22725]; U.S. DOE [DE-AC05-00OR22725]; Department of Energy FX The authors thank Yunqiao Pu from the Oak Ridge National Laboratory for helpful discussions regarding the CELF pretreatment method. This research was funded by the BioEnergy Science Center, a U.S. Department of Energy (DOE) Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory under an INCITE award, which is supported by the DOE Office of Science under Contract no. DE-AC05-00OR22725. This manuscript has been authored by UT Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. DOE. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.goy/downloads/doe-public-access-plan). NR 67 TC 0 Z9 0 U1 32 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10869 EP 10878 DI 10.1021/jacs.6b03285 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300036 PM 27482599 ER PT J AU Rudolf, JD Dong, LB Cao, HN Hatzos-Skintges, C Osipiuk, J Endres, M Chang, CY Ma, M Babnigg, G Joachimiak, A Phillips, GN Shen, B AF Rudolf, Jeffrey D. Dong, Liao-Bin Cao, Hongnan Hatzos-Skintges, Catherine Osipiuk, Jerzy Endres, Michael Chang, Chin-Yuan Ma, Ming Babnigg, Gyorgy Joachimiak, Andrzej Phillips, George N., Jr. Shen, Ben TI Structure of the ent-Copalyl Diphosphate Synthase PtmT2 from Streptomyces platensis CB00739, a Bacterial Type II Diterpene Synthase SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TERPENE SYNTHASES; OXIDOSQUALENE CYCLASE; FARNESYL DIPHOSPHATE; FUNCTIONAL-ANALYSIS; CRYSTAL-STRUCTURE; ABIES-GRANDIS; BIOSYNTHESIS; BIOLOGY; SQUALENE; CLONING AB Terpenoids are the largest and most structurally diverse family of natural products found in nature, yet their presence in bacteria is underappreciated. The carbon skeletons of terpenoids are generated through carbocation-dependent cyclization cascades catalyzed by terpene synthases (TSs). Type I and type II TSs initiate cyclization via diphosphate ionization and protonation, respectively, and protein structures of both types are known. Most plant diterpene synthases (DTSs) possess three alpha-helical domains (alpha beta gamma), which are thought to have arisen from the fusion of discrete, ancestral bacterial type I TSs (alpha) and type II TSs (beta gamma). Type II DTSs of bacterial origin, of which there are no structurally characterized members, are a missing piece in the structural evolution of TSs. Here, we report the first crystal structure of a type II DTS from bacteria. PtnaT2 from Streptomyces platensis CB00739 was verified as an ent-copalyl diphosphate synthase involved in the biosynthesis of platensimycin and platencin. The crystal structure of PtmT2 was solved at a resolution of 1.80 angstrom, and docking studies suggest the catalytically active conformation of geranylgeranyl diphosphate (GGPP). Site-directed mutagenesis confirmed residues involved in binding the diphosphate moiety of GGPP and identified DxxxxE as a potential Mg2+-binding motif for type II DTSs of bacterial origin. Finally, both the shape and physicochemical properties of the active sites are responsible for determining specific catalytic outcomes of TSs. The structure of PtmT2 fundamentally advances the knowledge of bacterial TSs, their mechanisms, and their role in the evolution of TSs. C1 [Rudolf, Jeffrey D.; Dong, Liao-Bin; Chang, Chin-Yuan; Ma, Ming; Shen, Ben] Scripps Res Inst, Dept Chem, Jupiter, FL 33458 USA. [Cao, Hongnan; Phillips, George N., Jr.] Rice Univ, Dept Biosci, Houston, TX 77005 USA. [Hatzos-Skintges, Catherine; Osipiuk, Jerzy; Endres, Michael; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Midwest Ctr Struct Genom, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hatzos-Skintges, Catherine; Osipiuk, Jerzy; Endres, Michael; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Shen, Ben] Scripps Res Inst, Dept Mol Therapeut, Jupiter, FL 33458 USA. [Shen, Ben] Scripps Res Inst, Nat Prod Lib Initiat, Jupiter, FL 33458 USA. RP Shen, B (reprint author), Scripps Res Inst, Dept Chem, Jupiter, FL 33458 USA.; Shen, B (reprint author), Scripps Res Inst, Dept Mol Therapeut, Jupiter, FL 33458 USA.; Shen, B (reprint author), Scripps Res Inst, Nat Prod Lib Initiat, Jupiter, FL 33458 USA. EM shenb@scripps.edu FU National Institute of General Medical Sciences Protein Structure Initiative [GM094585, GM098248]; National Institutes of Health [GM109456, GM114353]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX We thank Prof. C. Dale Poulter at the University of Utah for the generous gift of GGSPP. This work is supported in part by the National Institute of General Medical Sciences Protein Structure Initiative Grants GM094585 (AJ) and GM098248 (G.N.P.), and National Institutes of Health Grants GM109456 (G.N.P.) and GM114353 (BS). The use of Structural Biology Center beamlines at the Advanced Photon Source was supported by U.S. Department of Energy, Office of Biological and Environmental Research grant DE-AC02-06CH11357 (AJ). NR 59 TC 3 Z9 3 U1 11 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10905 EP 10915 DI 10.1021/jacs.6b04317 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300040 PM 27490479 ER PT J AU de Oteyza, DG Paz, AP Chen, YC Pedramrazi, Z Riss, A Wickenburg, S Tsai, HZ Fischer, FR Crommie, MF Rubio, A AF de Oteyza, Dimas G. Perez Paz, Alejandro Chen, Yen-Chia Pedramrazi, Zahra Riss, Alexander Wickenburg, Sebastian Tsai, Hsin-Zon Fischer, Felix R. Crommie, Michael F. Rubio, Angel TI Noncovalent Dimerization after Enediyne Cyclization on Au(111) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BERGMAN CYCLIZATION; SURFACE; POLYPHENYLENE; THERMOLYSIS; DERIVATIVES; CHEMISTRY; BENZYNE AB We investigate the thermally induced cyclization of 1,2-bis(2-phenylethynyl)benzene on Au(111) using scanning tunneling microscopy and computer simulations. Cyclization of sterically hindered enediynes is known to proceed via two competing mechanisms in solution: a classic C-1-C-6 (Bergman) or a C-1-C-5 cyclization pathway. On Au(111), we find that the C-1-C-5 cyclization is suppressed and that the C-1-C-6 cyclization yields a highly strained bicyclic olefin whose surface chemistry was hitherto unknown. The C-1-C-6 product self assembles into discrete noncovalently bound dimers on the surface. The reaction mechanism and driving forces behind noncovalent association are discussed in light of density functional theory calculations. C1 [de Oteyza, Dimas G.] Donostia Int Phys Ctr, E-20018 San Sebastian, Spain. [de Oteyza, Dimas G.] Ikerbasque, Basque Fdn Sci, E-48011 Bilbao, Spain. [Perez Paz, Alejandro; Rubio, Angel] Univ Basque Country, CFM CSIC UPV EHU MPC, Nanobio Spect Grp, San Sebastian 20018, Spain. [Perez Paz, Alejandro; Rubio, Angel] Univ Basque Country, CFM CSIC UPV EHU MPC, ETSF, San Sebastian 20018, Spain. [Chen, Yen-Chia; Pedramrazi, Zahra; Riss, Alexander; Wickenburg, Sebastian; Tsai, Hsin-Zon; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fischer, Felix R.; Crommie, Michael F.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Fischer, Felix R.; Crommie, Michael F.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Fischer, Felix R.; Crommie, Michael F.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rubio, Angel] Max Planck Inst Struct & Dynam Matter, Luruper Chaussee 149, D-22761 Hamburg, Germany. [Rubio, Angel] Ctr Free Electron Laser Sci CFEL, Luruper Chaussee 149, D-22761 Hamburg, Germany. RP de Oteyza, DG (reprint author), Donostia Int Phys Ctr, E-20018 San Sebastian, Spain.; de Oteyza, DG (reprint author), Ikerbasque, Basque Fdn Sci, E-48011 Bilbao, Spain. EM d_oteyza@ehu.eus RI de Oteyza, Dimas/H-5955-2013; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; Rubio, Angel/A-5507-2008; CSIC-UPV/EHU, CFM/F-4867-2012 OI de Oteyza, Dimas/0000-0001-8060-6819; Rubio, Angel/0000-0003-2060-3151; FU U.S. Department of Energy Office of Basic Energy Sciences Nanomachine Program [DE-AC02-05CH11231]; Office of Naval Research BRC Program; European Research Council [ERC-2010-AdG-267374-DYNamo, ERC-2014-STG-635919-SURFINK]; Grupos Consolidados UPV/EHU del Gobiemo Vasco [IT-578-13]; Ayuda para la Especializacion de Personal Investigador del Vicerrectorado de Investigation de la UPV/EHU; Spanish "Juan de la Cierva-incorporacion" program [IJCI-2014-20147]; [FIS2013-46159-C3-1-P] FX Research was supported by the U.S. Department of Energy Office of Basic Energy Sciences Nanomachine Program under Contract No. DE-AC02-05CH11231 (STM imaging), by the Office of Naval Research BRC Program (molecular synthesis), by the European Research Council Grants ERC-2010-AdG-267374-DYNamo and ERC-2014-STG-635919-SURFINK (computational resources and surface analysis, respectively), by Spanish Grant No. FIS2013-46159-C3-1-P (simulated reaction landscape), and by Grupos Consolidados UPV/EHU del Gobiemo Vasco No. IT-578-13 (simulated dimer binding energy). A.P.P. acknowledges postdoctoral fellowship support from "Ayuda para la Especializacion de Personal Investigador del Vicerrectorado de Investigation de la UPV/EHU-2013" and from the Spanish "Juan de la Cierva-incorporacion" program (IJCI-2014-20147). E. Goiri is acknowledged for help and discussion on the statistical analysis of interparticle distances. NR 25 TC 2 Z9 2 U1 22 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 10963 EP 10967 DI 10.1021/jacs.6b05203 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300046 PM 27490459 ER PT J AU Hadt, RG Hayes, D Brodsky, CN Ullmann, AM Casa, DM Upton, MH Nocera, DG Chen, LX AF Hadt, Ryan G. Hayes, Dugan Brodsky, Casey N. Ullmann, Andrew M. Casa, Diego M. Upton, Mary H. Nocera, Daniel G. Chen, Lin X. TI X-ray Spectroscopic Characterization of Co(IV) and Metal-Metal Interactions in Co4O4: Electronic Structure Contributions to the Formation of High-Valent States Relevant to the Oxygen Evolution Reaction SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID WATER OXIDATION CATALYSTS; COBALT(III)-OXO CUBANE CLUSTERS; DIFFERENTIAL ORBITAL COVALENCY; MIXED-VALENCE; ABSORPTION-SPECTROSCOPY; EVOLVING CATALYST; L-EDGE; ELECTROCHEMICAL PROPERTIES; MAGNETIC-PROPERTIES; METHANE OXIDATION AB The formation of high-valent states is a key factor in making highly active transition-metal-based catalysts of the oxygen evolution reaction (OER). These high oxidation states will be strongly influenced by the local geometric and electronic structures of the metal ion, which are difficult to study due to spectroscopically active and complex backgrounds, short lifetimes, and limited concentrations. Here, we use a wide range of complementary Xray spectroscopies coupled to DFT calculations to study Co(III)(4)O-4 cubanes and their first oxidized derivatives, which provide insight into the high-valent Co(IV) centers responsible for the activity of molecular and heterogeneous OER catalysts. The combination of X-ray absorption and 1s3p resonant inelastic X-ray scattering (K beta RIXS) allows Co(IV) to be isolated and studied against a spectroscopically active Co(III) background. Co K- and L-edge X-ray absorption data allow for a detailed characterization of the 3d-manifold of effectively localized Co(IV) centers and provide a direct handle on the tag-based redox-active molecular orbital. K beta RIXS is also shown to provide a powerful probe of Co(IV), and specific spectral features are sensitive to the degree of oxo-mediated metal metal coupling across Co4O4. Guided by the data, calculations show that electron hole delocalization can actually oppose Co(IV) formation. Computational extension of Co4O4 to CoM3O4 structures (M = redox-inactive metal) defines electronic structure contributions to Co(IV) formation. Redox activity is shown to be linearly related to covalency, and M(III) oxo inductive effects on Co(IV) oxo bonding can tune the covalency of high-valent sites over a large range and thereby tune E-0 over hundreds of millivolts. Additionally, redox-inactive metal substitution can also switch the ground state and modify metal metal and antibonding interactions across the cluster. C1 [Hadt, Ryan G.; Hayes, Dugan; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Casa, Diego M.; Upton, Mary H.] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. [Chen, Lin X.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Brodsky, Casey N.; Ullmann, Andrew M.; Nocera, Daniel G.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. RP Chen, LX (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.; Chen, LX (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Nocera, DG (reprint author), Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. EM dnocera@fas.harvard.edu; lchen@anl.gov FU Division of Chemical Sciences, Biosciences, Office of Basic Energy Science (OBES), DOE [DE-AC02-06CH11357]; U.S. DOE Office of Science [DE-SC0009758]; Joseph J. Katz Postdoctoral Fellowship at Argonne National Laboratory (ANL); National Science Foundation's Graduate Research Fellowship FX Work at ANL was supported by funding from the Division of Chemical Sciences, Biosciences, Office of Basic Energy Science (OBES), DOE through Grant DE-AC02-06CH11357. Synchrotron facilities were provided by the Advanced Photon Source (APS) and Advanced Light Source (ALS) operated by DOE BES. Work at Harvard was performed under a grant from the U.S. DOE Office of Science (DE-SC0009758). D.H. is supported by the Joseph J. Katz Postdoctoral Fellowship at Argonne National Laboratory (ANL). C.N.B. acknowledges the National Science Foundation's Graduate Research Fellowship. We acknowledge Sungsik Lee for assistance in making Co K-edge measurements and Robert Schoenlein and Amy Cordones-Hahn for assistance in making Co L-edge measurements. We acknowledge Edward Solomon, Michael Mara, Thomas Kroll, and Bryce Anderson for helpful discussions. We gratefully acknowledge the computing resources provided on Blues and Fusion, both high-performance computing clusters operated by the Laboratory Computing Resource Center at ANL. NR 112 TC 4 Z9 4 U1 76 U2 90 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 31 PY 2016 VL 138 IS 34 BP 11017 EP 11030 DI 10.1021/jacs.6b04663 PG 14 WC Chemistry, Multidisciplinary SC Chemistry GA DU9CH UT WOS:000382513300053 PM 27515121 ER PT J AU Winiarski, MJ Wiendlocha, B Golab, S Kushwaha, SK Wisniewski, P Kaczorowski, D Thompson, JD Cava, RJ Klimczuk, T AF Winiarski, M. J. Wiendlocha, B. Golab, S. Kushwaha, S. K. Wisniewski, P. Kaczorowski, D. Thompson, J. D. Cava, R. J. Klimczuk, T. TI Superconductivity in CaBi2 SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID TRANSITION-TEMPERATURE; TOPOLOGICAL INSULATORS; CRYSTAL-STRUCTURE; YBSB2; SR AB Superconductivity is observed with critical temperature T-c = 2.0 K in self-flux-grown single crystals of CaBi2. This material adopts the ZrSi2 structure type with lattice parameters a = 4.696(1) angstrom, b = 17.081(2) angstrom and c = 4.611(1) angstrom. The crystals of CaBi2 were studied by means of magnetic susceptibility, specific heat and electrical resistivity measurements. The heat capacity jump at T-c is Delta C/gamma T-c = 1.41, confirming bulk superconductivity; the Sommerfeld coefficient gamma = 4.1 mJ mol(-1) K-2 and the Debye temperature Theta(D) = 157 K. The electron-phonon coupling strength is lambda(el-ph) = 0.59, and the thermodynamic critical field H-c is low, between 111 and 124 Oe CaBi2 is a moderate coupling type-I superconductor. Results of electronic structure calculations are reported and charge densities, electronic bands, densities of states and Fermi surfaces are discussed, focusing on the effects of spin-orbit coupling and electronic property anisotropy. We find a mixed quasi-2D + 3D character in the electronic structure, which reflects the layered crystal structure of the material. C1 [Winiarski, M. J.; Klimczuk, T.] Gdansk Univ Technol, Fac Appl Phys & Math, Narutowicza 11-12, PL-80233 Gdansk, Poland. [Wiendlocha, B.; Golab, S.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Aleja Mickiewicza 30, PL-30059 Krakow, Poland. [Kushwaha, S. K.; Cava, R. J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Wisniewski, P.; Kaczorowski, D.] Polish Acad Sci, Inst Low Temp & Struct Res, PNr 1410, PL-50950 Wroclaw, Poland. [Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Winiarski, MJ; Klimczuk, T (reprint author), Gdansk Univ Technol, Fac Appl Phys & Math, Narutowicza 11-12, PL-80233 Gdansk, Poland. EM mwiniarski@mif.pg.gda.pl; tomasz.klimczuk@pg.gda.pl RI Wisniewski, Piotr/C-8952-2011; Winiarski, Michal/G-6243-2016; Wiendlocha, Bartlomiej/G-4121-2011; Kushwaha, Satya/B-8287-2017 OI Wisniewski, Piotr/0000-0002-6741-2793; Winiarski, Michal/0000-0001-9083-8066; Wiendlocha, Bartlomiej/0000-0001-9536-7216; Kushwaha, Satya/0000-0002-3169-969X FU National Science Centre (Poland) [DEC-2012/07/E/ST3/00584]; Polish Ministry of Science and Higher Education; Department of Energy Division of Basic Energy Sciences [DE-FG02-98ER45706]; Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX The research performed at the Gdansk University of Technology was supported by the National Science Centre (Poland) grant (DEC-2012/07/E/ST3/00584). B. W. was partially supported by the Polish Ministry of Science and Higher Education. The research at Princeton was supported by the Department of Energy Division of Basic Energy Sciences, Grant DE-FG02-98ER45706. Work at Los Alamos was performed under the auspices of the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 42 TC 0 Z9 0 U1 23 U2 31 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 31 PY 2016 VL 18 IS 31 BP 21737 EP 21745 DI 10.1039/c6cp02856j PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT3YV UT WOS:000381418000083 PM 27435423 ER PT J AU Kundu, J Pascal, T Prendergast, D Whitelam, S AF Kundu, Joyjit Pascal, Tod Prendergast, David Whitelam, Stephen TI Selective gas capture via kinetic trapping SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; POSTCOMBUSTION CARBON CAPTURE; MOLECULAR SIMULATION; SWING ADSORPTION; DIOXIDE CAPTURE; CO2 ADSORPTION; HIGH-CAPACITY; SEPARATION; SITES; DIFFUSION AB Conventional approaches to the capture of CO2 by metal-organic frameworks focus on equilibrium conditions, and frameworks that contain little CO2 in equilibrium are often rejected as carbon-capture materials. Here we use a statistical mechanical model, parameterized by quantum mechanical data, to suggest that metal-organic frameworks can be used to separate CO2 from a typical flue gas mixture when used under nonequilibrium conditions. The origin of this selectivity is an emergent gas-separation mechanism that results from the acquisition by different gas types of different mobilities within a crowded framework. The resulting distribution of gas types within the framework is in general spatially and dynamically heterogeneous. Our results suggest that relaxing the requirement of equilibrium can substantially increase the parameter space of conditions and materials for which selective gas capture can be effected. C1 [Kundu, Joyjit; Pascal, Tod; Prendergast, David; Whitelam, Stephen] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Kundu, J; Whitelam, S (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM jkundu@lbl.gov; swhitelam@lbl.gov FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001015]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy; Batteries for Advanced Transportation Technologies program [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Pieremanuele Canepa and Rebecca Siegelman for discussions, and Rebecca Siegelman and Jeff Martell for comments on the manuscript. JK was supported by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award number DE-SC0001015. DP and SW were partially supported by the same Center, and by the Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy. TP acknowledges support from the Batteries for Advanced Transportation Technologies program, administered by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract DE-AC02-05CH11231. This work was done as part of a User Project at the Molecular Foundry at Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The simulations were performed at the compute cluster Vulcan, managed by the High Performance Computing Services Group, at Lawrence Berkeley National Laboratory. NR 43 TC 1 Z9 1 U1 12 U2 12 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD AUG 31 PY 2016 VL 18 IS 31 BP 21760 EP 21766 DI 10.1039/c6cp03940e PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT3YV UT WOS:000381418000085 PM 27435033 ER PT J AU Dubuis, G Yacoby, Y Zhou, H He, X Bollinger, AT Pavuna, D Pindak, R Bozovic, I AF Dubuis, Guy Yacoby, Yizhak Zhou, Hua He, Xi Bollinger, Anthony T. Pavuna, Davor Pindak, Ron Bozovic, Ivan TI Oxygen Displacement in Cuprates under Ionic Liquid Field-Effect Gating SO SCIENTIFIC REPORTS LA English DT Article ID INTERFACE SUPERCONDUCTIVITY; INSULATOR-TRANSITION; SURFACE; OXIDES AB We studied structural changes in a 5 unit cell thick La1.96Sr0.04CuO4 film, epitaxially grown on a LaSrAlO4 substrate with a single unit cell buffer layer, when ultra-high electric fields were induced in the film by applying a gate voltage between the film (ground) and an ionic liquid in contact with it. Measuring the diffraction intensity along the substrate-defined Bragg rods and analyzing the results using a phase retrieval method we obtained the three-dimensional electron density in the film, buffer layer, and topmost atomic layers of the substrate under different applied gate voltages. The main structural observations were: (i) there were no structural changes when the voltage was negative, holes were injected into the film making it more metallic and screening the electric field; (ii) when the voltage was positive, the film was depleted of holes becoming more insulating, the electric field extended throughout the film, the partial surface monolayer became disordered, and equatorial oxygen atoms were displaced towards the surface; (iii) the changes in surface disorder and the oxygen displacements were both reversed when a negative voltage was applied; and (iv) the c-axis lattice constant of the film did not change in spite of the displacement of equatorial oxygen atoms. C1 [Dubuis, Guy] Victoria Univ Wellington, Robinson Res Inst, MacDiarmid Inst Adv Mat & Nanotechnol, Lower Hutt 5046, New Zealand. [Dubuis, Guy; Bollinger, Anthony T.; Bozovic, Ivan] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Dubuis, Guy; Pavuna, Davor] Ecole Polytech Fed Lausanne, LPMC, CH-1015 Lausanne, Switzerland. [Yacoby, Yizhak] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. [Zhou, Hua] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [He, Xi; Bozovic, Ivan] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. [Pindak, Ron] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Pindak, R (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM pindak@bnl.gov RI Dubuis, Guy/A-6849-2012 OI Dubuis, Guy/0000-0002-8199-4953 FU DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; Israel Science Foundation under ISF-Grant [1005/11]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4410] FX This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. H.Z. was supported by the same contract; Y.Y. by the Israel Science Foundation under ISF-Grant No. 1005/11; R.P. by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704; G.D. and D.P. by the Laboratory for Physics of Complex Matter (EPFL) and the Swiss National Science Foundation, I.B. and A.T.B. by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. X.H. by the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant GBMF4410. NR 34 TC 1 Z9 1 U1 13 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 31 PY 2016 VL 6 AR 32378 DI 10.1038/srep32378 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU5HG UT WOS:000382242200001 PM 27578237 ER PT J AU Bennett, JG AF Bennett, Joel G. TI A Representative volume model for a CNT composite material SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN ENGINEERING LA English DT Article DE solids; micromechanics; composites; damage; constitutive equations ID MICROMECHANICAL ANALYSIS; ELASTIC PROPERTIES AB The concept of a Representative Volume Model' is used in combination with Equivalent Mechanical Strain' or Aboudi's Average Strain' theorem to illustrate how a carbon nanotube reinforced composite material constitutive law for a nano-composite material can be implemented into a finite element program for modeling structural applications. Current methods of modeling each individual composite layer to build up an element composed of carbon nanotube reinforced composite material may not be the best approach for modeling structural applications of this composite. The approach presented here is based upon presentations given at the National Science Foundation-Civil and Mechanical Systems division workshop at John Hopkins University in 2004, which is referred to in this paper as the Williams-Baxter approach. This approach is also used to demonstrate that damage modeling can be included as was suggested in this workshop. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Bennett, Joel G.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM joelnjackie@gmail.com NR 16 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0029-5981 EI 1097-0207 J9 INT J NUMER METH ENG JI Int. J. Numer. Methods Eng. PD AUG 31 PY 2016 VL 107 IS 9 BP 723 EP 732 DI 10.1002/nme.5182 PG 10 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA DS6MB UT WOS:000380894800001 ER PT J AU Shen, CF Ge, MY Luo, LL Fang, X Liu, YH Zhang, AY Rong, JP Wang, CM Zhou, CW AF Shen, Chenfei Ge, Mingyuan Luo, Langli Fang, Xin Liu, Yihang Zhang, Anyi Rong, Jiepeng Wang, Chongmin Zhou, Chongwu TI In Situ and Ex Situ TEM Study of Lithiation Behaviours of Porous Silicon Nanostructures SO SCIENTIFIC REPORTS LA English DT Article ID SIZE-DEPENDENT FRACTURE; LITHIUM BATTERY ANODES; LONG CYCLE LIFE; ELECTROCHEMICAL LITHIATION; PHASE-TRANSITION; ION BATTERIES; HIGH-CAPACITY; NANOWIRES; NANOPARTICLES; ELECTRODES AB In this work, we study the lithiation behaviours of both porous silicon (Si) nanoparticles and porous Si nanowires by in situ and ex situ transmission electron microscopy (TEM) and compare them with solid Si nanoparticles and nanowires. The in situ TEM observation reveals that the critical fracture diameter of porous Si particles reaches up to 1.52 mu m, which is much larger than the previously reported 150 nm for crystalline Si nanoparticles and 870 nm for amorphous Si nanoparticles. After full lithiation, solid Si nanoparticles and nanowires transform to crystalline Li15Si4 phase while porous Si nanoparticles and nanowires transform to amorphous LixSi phase, which is due to the effect of domain size on the stability of Li15Si4 as revealed by the first-principle molecular dynamic simulation. Ex situ TEM characterization is conducted to further investigate the structural evolution of porous and solid Si nanoparticles during the cycling process, which confirms that the porous Si nanoparticles exhibit better capability to suppress pore evolution than solid Si nanoparticles. The investigation of structural evolution and phase transition of porous Si nanoparticles and nanowires during the lithiation process reveal that they are more desirable as lithium-ion battery anode materials than solid Si nanoparticles and nanowires. C1 [Shen, Chenfei; Ge, Mingyuan; Fang, Xin; Zhang, Anyi; Rong, Jiepeng; Zhou, Chongwu] Univ Southern Calif, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA. [Ge, Mingyuan] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Luo, Langli; Wang, Chongmin] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Liu, Yihang; Zhou, Chongwu] Univ Southern Calif, Ming Hsieh Dept Elect Engn, Los Angeles, CA 90089 USA. RP Zhou, CW (reprint author), Univ Southern Calif, Mork Family Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA.; Zhou, CW (reprint author), Univ Southern Calif, Ming Hsieh Dept Elect Engn, Los Angeles, CA 90089 USA. EM chongwuz@usc.edu RI Shen, Chenfei/A-2471-2016; Luo, Langli/B-5239-2013; Zhou, Chongwu/F-7483-2010; OI Shen, Chenfei/0000-0001-8635-3429; Luo, Langli/0000-0002-6311-051X FU Brookhaven National Laboratory - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under the Batteries for Advanced Battery Materials Research (BMR) [DE-AC02-05CH11231, 6951379]; DOE's Office of Biological and Environmental Research FX A portion of the TEM images used in this article were generated at the Center for Electron Microscopy and Microanalysis, University of Southern California. M.G. finished the research reported in this paper at University of Southern California, and contributed to discussions after he joined Brookhaven National Laboratory. M.G. acknowledged the support of Brookhaven National Laboratory, which was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. C.W. was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 6951379 under the Batteries for Advanced Battery Materials Research (BMR). The in situ TEM work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. NR 37 TC 0 Z9 0 U1 12 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 30 PY 2016 VL 6 AR 31334 DI 10.1038/srep31334 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH7QI UT WOS:000391967200001 PM 27571919 ER PT J AU Chen, D Liu, ZQ Fast, J Ban, JM AF Chen, Dan Liu, Zhiquan Fast, Jerome Ban, Junmei TI Simulations of sulfate-nitrate-ammonium (SNA) aerosols during the extreme haze events over northern China in October 2014 SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID HETEROGENEOUS CHEMISTRY; FORMATION MECHANISM; NITROGEN-DIOXIDE; MODELING SYSTEM; SULFUR-DIOXIDE; REGIONAL HAZE; EAST-ASIA; WRF-CHEM; NO X; EMISSIONS AB Extreme haze events have occurred frequently over China in recent years. Although many studies have investigated the formation mechanisms associated with PM2.5 for heavily polluted regions in China based on observational data, adequately predicting peak PM2.5 concentrations is still challenging for regional air quality models. In this study, we evaluate the performance of one configuration of the Weather Research and Forecasting model coupled with chemistry (WRF-Chem) and use the model to investigate the sensitivity of heterogeneous reactions on simulated peak sulfate, nitrate, and ammonium concentrations in the vicinity of Beijing during four extreme haze episodes in October 2014 over the North China Plain. The highest observed PM2.5 concentration of 469 mu g m(-3) occurred in Beijing. Comparisons with observations show that the model reproduced the temporal variability in PM2.5 with the highest PM2.5 values on polluted days (defined as days in which observed PM2.5 is greater than 75 mu g m(-3)), but predictions of sulfate, nitrate, and ammonium were too low on days with the highest observed concentrations. Observational data indicate that the sulfur/nitric oxidation rates are strongly correlated with relative humidity during periods of peak PM2.5; however, the model failed to reproduce the highest PM2.5 concentrations due to missing heterogeneous/aqueous reactions. As the parameterizations of those heterogeneous reactions are not well established yet, estimates of SO2-to-H2SO4 and NO2/NO3- to-HNO3 reaction rates that depend on relative humidity were applied, which improved the simulation of sulfate, nitrate, and ammonium enhancement on polluted days in terms of both concentrations and partitioning among those species. Sensitivity simulations showed that the extremely high heterogeneous reaction rates and also higher emission rates than those reported in the emission inventory were likely important factors contributing to those peak PM2.5 concentrations. C1 [Chen, Dan; Liu, Zhiquan; Ban, Junmei] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Fast, Jerome] Pacific Northwest Natl Lab, Richland, WA USA. RP Chen, D; Liu, ZQ (reprint author), Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. EM dchen@ucar.edu; liuz@ucar.edu RI Chen, Dan/R-4486-2016 FU IBM Research China; National Science Foundation; U.S. Department of Energy's Atmospheric System Research (ASR) program [KP17010000/57131] FX This work was partially funded by IBM Research China. NCAR is sponsored by the National Science Foundation. Jerome Fast was supported by the U.S. Department of Energy's Atmospheric System Research (ASR) program (KP17010000/57131). The authors thank Lin Zhang at Peking University for his great help on the application of aqueous reactions in the model. We also thank Daven Henze, Douglas Lowe, and Ravan Ahmadov for their helpful discussions. We are grateful to the referees for their helpful comments. NR 57 TC 0 Z9 1 U1 39 U2 39 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PD AUG 30 PY 2016 VL 16 IS 16 BP 10707 EP 10724 DI 10.5194/acp-16-10707-2016 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DW6EZ UT WOS:000383743600001 ER PT J AU Eilenberg, H Weiner, I Ben-Zvi, O Pundak, C Marmari, A Liran, O Wecker, MS Milrad, Y Yacoby, I AF Eilenberg, Haviva Weiner, Iddo Ben-Zvi, Oren Pundak, Carmel Marmari, Abigail Liran, Oded Wecker, Matt S. Milrad, Yuval Yacoby, Iftach TI The dual effect of a ferredoxin-hydrogenase fusion protein in vivo: successful divergence of the photosynthetic electron flux towards hydrogen production and elevated oxygen tolerance SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE H-2 production; Ferredoxin; Hydrogenase; Oxygen sensitivity; Fusion enzyme; Chlamydomonas reinhardtii ID ALGA CHLAMYDOMONAS-REINHARDTII; H-2 PRODUCTION; PHOTOPRODUCTION; EXPRESSION; CELLS; IDENTIFICATION; BIOSENSOR; SYSTEM; GENE; FNR AB Background: Hydrogen photo-production in green algae, catalyzed by the enzyme [FeFe]-hydrogenase (HydA), is considered a promising source of renewable clean energy. Yet, a significant increase in hydrogen production efficiency is necessary for industrial scale-up. We have previously shown that a major challenge to be resolved is the inferior competitiveness of HydA with NADPH production, catalyzed by ferredoxin-NADP7(+)-reductase (FNR). In this work, we explored the in vivo hydrogen production efficiency of Fd-HydA, where the electron donor ferredoxin (Fd) is fused to HydA and expressed in the model organism Chlamydomonas reinhardtii. Results: We show that once the Fd-HydA fusion gene is expressed in micro-algal cells of C. reinhardtii, the fusion enzyme is able to intercept photosynthetic electrons and use them for efficient hydrogen production, thus supporting the previous observations made in vitro. We found that Fd-HydA has a similar to 4.5-fold greater photosynthetic hydrogen production rate standardized for hydrogenase amount (PHPRH) than that of the native HydA in vivo. Furthermore, we provide evidence suggesting that the fusion protein is more resistant to oxygen than the native HydA. Conclusions: The in vivo photosynthetic activity of the Fd-HydA enzyme surpasses that of the native HydA and shows higher oxygen tolerance. Therefore, our results provide a solid platform for further engineering efforts towards efficient hydrogen production in microalgae through the expression of synthetic enzymes. C1 [Eilenberg, Haviva; Weiner, Iddo; Ben-Zvi, Oren; Pundak, Carmel; Marmari, Abigail; Liran, Oded; Milrad, Yuval; Yacoby, Iftach] Tel Aviv Univ, George S Wise Fac Life Sci, Dept Mol Biol & Ecol Plants, IL-69978 Tel Aviv, Israel. [Wecker, Matt S.] GeneBiologics LLC, Boulder, CO 80303 USA. [Wecker, Matt S.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yacoby, I (reprint author), Tel Aviv Univ, George S Wise Fac Life Sci, Dept Mol Biol & Ecol Plants, IL-69978 Tel Aviv, Israel. EM iftachy@tau.ac.il FU KAMIN, the Ministry of Economics State of Israel [3798] FX This research was funded by KAMIN, Contract Number: 3798, the Ministry of Economics State of Israel. NR 31 TC 0 Z9 0 U1 13 U2 13 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 30 PY 2016 VL 9 AR 182 DI 10.1186/s13068-016-0601-3 PG 10 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DV6BP UT WOS:000383016000004 PM 27582874 ER PT J AU Tang, AH Wang, G AF Tang, A. H. Wang, G. TI Procedure for measuring photon and vector meson circular polarization variation with respect to the reaction plane in relativistic heavy-ion collisions SO PHYSICAL REVIEW C LA English DT Article ID PAIR PRODUCTION AB The electromagnetic (EM) field pattern created by spectators in relativistic heavy-ion collisions plants a seed of positive (negative) magnetic helicity in the hemisphere above (below) the reaction plane. Owing to the chiral anomaly, the magnetic helicity interacts with the fermionic helicity of the collision system and causes photons emitted in upper and lower hemispheres to have different preferences in the circular polarization. Similar helicity separation for massive particles, owing to the global vorticity, is also possible. In this paper, we lay out a procedure to measure the variation of the circular polarization with respect to the reaction plane in relativistic heavy-ion collisions for massless photons, as well as similar polarization patterns for vector mesons decaying into two daughters. We propose to study the yield differentially and compare the yield between upper and lower hemispheres to identify and quantify such effects. C1 [Tang, A. H.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Wang, G.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. RP Tang, AH (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. FU U.S. Department of Energy [DE-AC02-98CH10886, DE-FG02-89ER40531, DE-FG02-88ER40424] FX We would like to thank D. Kharzeev, M. Lisa, Y. Yin, and Y. Zhang for fruitful discussions. We thank Y. Yin and Y. Zhang for reading the manuscript and providing comments. A.T. was supported by the U.S. Department of Energy under Grants No. DE-AC02-98CH10886 and No. DE-FG02-89ER40531. G.W. was supported by the U.S. Department of Energy under Grant No. DE-FG02-88ER40424. NR 21 TC 1 Z9 1 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 30 PY 2016 VL 94 IS 2 AR 024920 DI 10.1103/PhysRevC.94.024920 PG 5 WC Physics, Nuclear SC Physics GA DU4IU UT WOS:000382177100008 ER PT J AU Bonnett, C Troxel, MA Hartley, W Amara, A Leistedt, B Becker, MR Bernstein, GM Bridle, SL Bruderer, C Busha, MT Kind, MC Childress, MJ Castander, FJ Chang, C Crocce, M Davis, TM Eifler, TF Frieman, J Gangkofner, C Gaztanaga, E Glazebrook, K Gruen, D Kacprzak, T King, A Kwan, J Lahav, O Lewis, G Lidman, C Lin, H MacCrann, N Miquel, R O'Neill, CR Palmese, A Peiris, HV Refregier, A Rozo, E Rykoff, ES Sadeh, I Sanchez, C Sheldon, E Uddin, S Wechsler, RH Zuntz, J Abbott, T Abdalla, FB Allam, S Armstrong, R Banerji, M Bauer, AH Benoit-Levy, A Bertin, E Brooks, D Buckley-Geer, E Burke, DL Capozzi, D Rosell, AC Carretero, J Cunha, CE D'Andrea, CB da Costa, LN DePoy, DL Desai, S Diehl, HT Dietrich, JP Doel, P Neto, AF Fernandez, E Flaugher, B Fosalba, P Gerdes, DW Gruendl, RA Honscheid, K Jain, B James, DJ Jarvis, M Kim, AG Kuehn, K Kuropatkin, N Li, TS Lima, M Maia, MAG March, M Marshall, JL Martini, P Melchior, P Miller, CJ Neilsen, E Nichol, RC Nord, B Ogando, R Plazas, AA Reil, K Romer, AK Roodman, A Sako, M Sanchez, E Santiago, B Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Vikram, V Walker, AR AF Bonnett, C. Troxel, M. A. Hartley, W. Amara, A. Leistedt, B. Becker, M. R. Bernstein, G. M. Bridle, S. L. Bruderer, C. Busha, M. T. Kind, M. Carrasco Childress, M. J. Castander, F. J. Chang, C. Crocce, M. Davis, T. M. Eifler, T. F. Frieman, J. Gangkofner, C. Gaztanaga, E. Glazebrook, K. Gruen, D. Kacprzak, T. King, A. Kwan, J. Lahav, O. Lewis, G. Lidman, C. Lin, H. MacCrann, N. Miquel, R. O'Neill, C. R. Palmese, A. Peiris, H. V. Refregier, A. Rozo, E. Rykoff, E. S. Sadeh, I. Sanchez, C. Sheldon, E. Uddin, S. Wechsler, R. H. Zuntz, J. Abbott, T. Abdalla, F. B. Allam, S. Armstrong, R. Banerji, M. Bauer, A. H. Benoit-Levy, A. Bertin, E. Brooks, D. Buckley-Geer, E. Burke, D. L. Capozzi, D. Carnero Rosell, A. Carretero, J. Cunha, C. E. D'Andrea, C. B. da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Dietrich, J. P. Doel, P. Fausti Neto, A. Fernandez, E. Flaugher, B. Fosalba, P. Gerdes, D. W. Gruendl, R. A. Honscheid, K. Jain, B. James, D. J. Jarvis, M. Kim, A. G. Kuehn, K. Kuropatkin, N. Li, T. S. Lima, M. Maia, M. A. G. March, M. Marshall, J. L. Martini, P. Melchior, P. Miller, C. J. Neilsen, E. Nichol, R. C. Nord, B. Ogando, R. Plazas, A. A. Reil, K. Romer, A. K. Roodman, A. Sako, M. Sanchez, E. Santiago, B. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Vikram, V. Walker, A. R. CA Dark Energy Survey Collaboration TI Redshift distributions of galaxies in the Dark Energy Survey Science Verification shear catalogue and implications for weak lensing SO PHYSICAL REVIEW D LA English DT Article ID STAR-FORMING GALAXIES; LARGE-SCALE STRUCTURE; PHOTO-Z PERFORMANCE; VLT DEEP SURVEY; PHOTOMETRIC REDSHIFTS; DATA RELEASE; PRECISION COSMOLOGY; SURVEY REQUIREMENTS; SHAPE MEASUREMENT; NEURAL-NETWORKS AB We present photometric redshift estimates for galaxies used in the weak lensing analysis of the Dark Energy Survey Science Verification (DES SV) data. Four model-or machine learning-based photometric redshift methods-ANNZ2, BPZ calibrated against BCC-Ufig simulations, SKYNET, and TPZ-are analyzed. For training, calibration, and testing of these methods, we construct a catalogue of spectroscopically confirmed galaxies matched against DES SV data. The performance of the methods is evaluated against the matched spectroscopic catalogue, focusing on metrics relevant for weak lensing analyses, with additional validation against COSMOS photo-z's. From the galaxies in the DES SV shear catalogue, which have mean redshift 0.72 +/- 0.01 over the range 0.3 < z < 1.3, we construct three tomographic bins with means of z = {0.45; 0.67; 1.00}. These bins each have systematic uncertainties delta z <= 0.05 in the mean of the fiducial SKYNET photo-z (dz). We propagate the errors in the redshift distributions through to their impact on cosmological parameters estimated with cosmic shear, and find that they cause shifts in the value of sigma(8) of approximately 3%. This shift is within the one sigma statistical errors on sigma(8) for the DES SV shear catalogue. We further study the potential impact of systematic differences on the critical surface density, Sigma(crit), finding levels of bias safely less than the statistical power of DES SV data. We recommend a final Gaussian prior for the photo-z bias in the mean of n(z) of width 0.05 for each of the three tomographic bins, and show that this is a sufficient bias model for the corresponding cosmology analysis. C1 [Bonnett, C.; Miquel, R.; Sanchez, C.; Carretero, J.; Fernandez, E.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Troxel, M. A.; Bridle, S. L.; MacCrann, N.; Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Oxford Rd, Manchester M13 9PL, Lancs, England. [Hartley, W.; Amara, A.; Bruderer, C.; Chang, C.; Kacprzak, T.; Refregier, A.] ETH, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. [Leistedt, B.; Lahav, O.; Palmese, A.; Peiris, H. V.; Sadeh, I.; Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Becker, M. R.; Busha, M. T.] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. [Becker, M. R.; Rykoff, E. S.; Wechsler, R. H.; Burke, D. L.; Cunha, C. E.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Bernstein, G. M.; Eifler, T. F.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [King, A.] Univ Queensland, Sch Math & Phys, Brisbane, Qld 4072, Australia. [Kind, M. Carrasco; Gruendl, R. A.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Swanson, M. E. C.] Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [Castander, F. J.; Crocce, M.; Gaztanaga, E.; Bauer, A. H.; Carretero, J.; Fosalba, P.] IEEC CSIC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, Barcelona 08193, Spain. [Eifler, T. F.; Abdalla, F. B.; Plazas, A. A.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Frieman, J.; Lin, H.; Allam, S.; Buckley-Geer, E.; Diehl, H. T.; Flaugher, B.; Kuropatkin, N.; Neilsen, E.; Nord, B.; Soares-Santos, M.; Sobreira, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Kwan, J.; Vikram, V.] Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. [Lidman, C.; Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Rozo, E.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Rykoff, E. S.; Wechsler, R. H.; Burke, D. L.; Reil, K.; Roodman, A.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Glazebrook, K.; Uddin, S.] Swinburne Univ Technol, Ctr Astrophys & Supercomp, Hawthorn, Vic 3122, Australia. [Abbott, T.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Interamer Observ, Casilla 603, La Serena, Chile. [Armstrong, R.] Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. [Banerji, M.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Banerji, M.] Univ Cambridge, Kavli Inst Cosmol, Madingley Rd, Cambridge CB3 0HA, England. [Bertin, E.] Inst Astrophys, CNRS, UMR 7095, F-75014 Paris, France. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Capozzi, D.; D'Andrea, C. B.; Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Carnero Rosell, A.; da Costa, L. N.; Fausti Neto, A.; Lima, M.; Maia, M. A. G.; Ogando, R.; Santiago, B.; Sobreira, F.] Lab Interinst Eastron LIneA, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [DePoy, D. L.; Li, T. S.; Marshall, J. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Li, T. S.; Marshall, J. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.] Univ Munich, Dept Phys, Scheinerstr 1, D-81679 Munich, Germany. [Gangkofner, C.; Sheldon, E.; Desai, S.; Dietrich, J. P.] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Gruen, D.; Dietrich, J. P.] Univ Munich, Univ Sternwarte, Fak Phys, Scheinerstr 1, D-81679 Munich, Germany. [Gerdes, D. W.; Miller, C. J.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Gruen, D.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Honscheid, K.; Martini, P.; Melchior, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Honscheid, K.; Melchior, P.; Suchyta, E.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Kim, A. G.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Martini, P.] Ohio State Univ, Dept Astron, 174 W 18Th Ave, Columbus, OH 43210 USA. [Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Pevensey Bldg, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.] CIEMAT, Madrid, Spain. [Santiago, B.] Univ Fed Rio Grande do Sul, Inst Fis, Caixa Postal 15051, BR-91501970 Porto Alegre, RS, Brazil. [Thaler, J.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Lima, M.] Univ Sao Paulo, Inst Fis, Dept Fis Matemat, CP 66318, BR-05314970 Sao Paulo, SP, Brazil. [Lewis, G.] South East Phys Network, SEPnet, Southampton, Hants, England. [Davis, T. M.; O'Neill, C. R.] Univ Queensland, Sch Math & Phys, Brisbane, Qld 4072, Australia. [Childress, M. J.] Australian Natl Univ, Res Sch Astron & Astrophys, Canberra, ACT 2611, Australia. [Sheldon, E.] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Gangkofner, C.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. RP Bonnett, C (reprint author), Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. RI Lima, Marcos/E-8378-2010; Ogando, Ricardo/A-1747-2010; Davis, Tamara/A-4280-2008; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Davis, Tamara/0000-0002-4213-8783; Gaztanaga, Enrique/0000-0001-9632-0815; Abdalla, Filipe/0000-0003-2063-4345; Sobreira, Flavia/0000-0002-7822-0658 FU European Research Council [240672]; DFG Cluster of Excellence Origin and Structure of the Universe; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; ERDF funds from the European Union; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Edinburgh; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory, Stanford University; University of Sussex; Texas AM University; Australian Astronomical Observatory [A/2013B/012]; Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO) [CE110001020]; Swiss National Science Foundation [200021_14944, 200021_143906]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Pennsylvania State University; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University; ESO Telescopes at the La Silla Paranal Observatory [179.A-2004, 177.A-3016] FX We are grateful for the extraordinary contributions of our CTIO colleagues and the DECam Construction, Commissioning and Science Verification teams in achieving the excellent instrument and telescope conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the DES Data Management group. M. T., S. B., N. M., and J. Z. acknowledge support from the European Research Council in the form of a Starting Grant with number 240672. D. G. acknowledges the support by the DFG Cluster of Excellence Origin and Structure of the Universe. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. C. G. acknowledges the support by the DFG Cluster of Excellence Origin and Structure of the Universe. The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Edinburgh, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. Based in part on observations taken at the Australian Astronomical Observatory under program A/2013B/012. Parts of this research were conducted by the Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO), through project number CE110001020. This work was supported in part by grants 200021_14944 and 200021_143906 from the Swiss National Science Foundation. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science.; r The SDSS-III web site is http://www.sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. Based on observations made with ESO Telescopes at the La Silla Paranal Observatory under programme ID 179.A-2004. Based on observations made with ESO Telescopes at the La Silla Paranal Observatory under programme ID 177.A-3016. This paper is Fermilab publication FERMILAB-PUB-15-306 and DES publication DES2015-0060. This paper has gone through internal review by the DES Collaboration. NR 95 TC 10 Z9 10 U1 4 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 30 PY 2016 VL 94 IS 4 AR 042005 DI 10.1103/PhysRevD.94.042005 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU4IW UT WOS:000382177300001 ER PT J AU Isley, SC Stern, PC Carmichael, SP Joseph, KM Arent, DJ AF Isley, Steven C. Stern, Paul C. Carmichael, Scott P. Joseph, Karun M. Arent, Douglas J. TI Online purchasing creates opportunities to lower the life cycle carbon footprints of consumer products SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbon footprint; online experiments; carbon offset; ecolabels ID ENERGY-CONSUMPTION; EMISSIONS AB A major barrier to transitions to environmental sustainability is that consumers lack information about the full environmental footprints of their purchases. Sellers' incentives do not support reducing the footprints unless customers have such information and are willing to act on it. We explore the potential of modern information technology to lower this barrier by enabling firms to inform customers of products' environmental footprints at the point of purchase and easily offset consumers' contributions through bundled purchases of carbon offsets. Using online stated choice experiments, we evaluated the effectiveness of several inexpensive features that firms in four industries could implement with existing online user interfaces for consumers. These examples illustrate the potential for firms to lower their overall carbon footprints while improving customer satisfaction by lowering the "soft costs" to consumers of proenvironmental choices. Opportunities such as these likely exist wherever firms possess environmentally relevant data not accessible to consumers or when transaction costs make proenvironmental action difficult. C1 [Isley, Steven C.; Carmichael, Scott P.; Joseph, Karun M.; Arent, Douglas J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Stern, Paul C.] Natl Acad Sci Engn & Med, Board Environm Change & Soc, Div Behav & Social Sci & Educ, Washington, DC 20001 USA. [Stern, Paul C.] Norwegian Univ Sci & Technol, Dept Psychol, N-7491 Trondheim, Norway. RP Isley, SC (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Steven.Isley@nrel.gov NR 44 TC 0 Z9 0 U1 11 U2 11 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 30 PY 2016 VL 113 IS 35 BP 9780 EP 9785 DI 10.1073/pnas.1522211113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DV7BL UT WOS:000383090700047 PM 27528670 ER PT J AU Riley, R Haridas, S Wolfe, KH Lopes, MR Hittinger, CT Goker, M Salamov, AA Wisecaver, JH Long, TM Calvey, CH Aerts, AL Barry, KW Choi, C Clum, A Coughlan, AY Deshpande, S Douglass, AP Hanson, SJ Klenk, HP LaButti, KM Lapidus, A Lindquist, EA Lipzen, AM Meier-Kolthoff, JP Ohm, RA Otillar, RP Pangilinan, JL Peng, Y Rokas, A Rosa, CA Scheuner, C Sibirny, AA Slot, JC Stielow, JB Sun, H Kurtzman, CP Blackwell, M Grigoriev, IV Jeffries, TW AF Riley, Robert Haridas, Sajeet Wolfe, Kenneth H. Lopes, Mariana R. Hittinger, Chris Todd Goeker, Markus Salamov, Asaf A. Wisecaver, Jennifer H. Long, Tanya M. Calvey, Christopher H. Aerts, Andrea L. Barry, Kerrie W. Choi, Cindy Clum, Alicia Coughlan, Aisling Y. Deshpande, Shweta Douglass, Alexander P. Hanson, Sara J. Klenk, Hans-Peter LaButti, Kurt M. Lapidus, Alla Lindquist, Erika A. Lipzen, Anna M. Meier-Kolthoff, Jan P. Ohm, Robin A. Otillar, Robert P. Pangilinan, Jasmyn L. Peng, Yi Rokas, Antonis Rosa, Carlos A. Scheuner, Carmen Sibirny, Andriy A. Slot, Jason C. Stielow, J. Benjamin Sun, Hui Kurtzman, Cletus P. Blackwell, Meredith Grigoriev, Igor V. Jeffries, Thomas W. TI Comparative genomics of biotechnologically important yeasts SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE genomics; bioenergy; biotechnological yeasts; genetic code; microbiology ID HORIZONTAL GENE-TRANSFER; SACCHAROMYCES-CEREVISIAE; PICHIA-STIPITIS; EVOLUTION; CODE; SEQUENCE; MECHANISM; PATHWAY; COMPLEX; ORIGIN AB Ascomycete yeasts are metabolically diverse, with great potential for biotechnology. Here, we report the comparative genome analysis of 29 taxonomically and biotechnologically important yeasts, including 16 newly sequenced. We identify a genetic code change, CUG-Ala, in Pachysolen tannophilus in the clade sister to the known CUG-Ser clade. Ourwell-resolved yeast phylogeny shows that some traits, such as methylotrophy, are restricted to single clades, whereas others, such as L-rhamnose utilization, have patchy phylogenetic distributions. Gene clusters, with variable organization and distribution, encode many pathways of interest. Genomics can predict some biochemical traits precisely, but the genomic basis of others, such as xylose utilization, remains unresolved. Our data also provide insight into early evolution of ascomycetes. We document the loss of H3K9me2/3 heterochromatin, the origin of ascomycete mating-type switching, and panascomycete synteny at the MAT locus. These data and analyses will facilitate the engineering of efficient biosynthetic and degradative pathways and gateways for genomic manipulation. C1 [Riley, Robert; Haridas, Sajeet; Salamov, Asaf A.; Aerts, Andrea L.; Barry, Kerrie W.; Choi, Cindy; Clum, Alicia; Deshpande, Shweta; LaButti, Kurt M.; Lapidus, Alla; Lindquist, Erika A.; Lipzen, Anna M.; Ohm, Robin A.; Otillar, Robert P.; Pangilinan, Jasmyn L.; Peng, Yi; Sun, Hui; Grigoriev, Igor V.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Wolfe, Kenneth H.; Coughlan, Aisling Y.; Douglass, Alexander P.; Hanson, Sara J.] Univ Coll Dublin, Sch Med, Conway Inst, Dublin 4, Ireland. [Lopes, Mariana R.; Hittinger, Chris Todd] Univ Wisconsin, Genet Biotechnol Ctr, Lab Genet, Madison, WI 53706 USA. [Lopes, Mariana R.; Rosa, Carlos A.] Univ Fed Minas Gerais, Inst Ciencias Biol, Dept Microbiol, BR-31270901 Belo Horizonte, MG, Brazil. [Hittinger, Chris Todd] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Dept Energy, Madison, WI 53726 USA. [Goeker, Markus; Klenk, Hans-Peter; Meier-Kolthoff, Jan P.; Scheuner, Carmen; Stielow, J. Benjamin] Leibniz Inst, Deutsch Sammlung Mikroorganismen & Zellkulturen, D-38124 Braunschweig, Germany. [Wisecaver, Jennifer H.; Rokas, Antonis] Vanderbilt Univ, Dept Biol Sci, Nashville, TN 37235 USA. [Long, Tanya M.; Jeffries, Thomas W.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Long, Tanya M.] USDA, Forest Prod Lab, Madison, WI 53726 USA. [Calvey, Christopher H.] Xylome Corp, Madison, WI 53719 USA. [Klenk, Hans-Peter] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Sibirny, Andriy A.] Natl Acad Sci Ukraine, Inst Cell Biol, Dept Mol Genet & Biotechnol, UA-79005 Lvov, Ukraine. [Sibirny, Andriy A.] Univ Rzeszow, Dept Biotechnol & Microbiol, PL-35601 Rzeszow, Poland. [Slot, Jason C.] Ohio State Univ, Dept Plant Pathol, Columbus, OH 43210 USA. [Stielow, J. Benjamin] Royal Netherlands Acad Arts & Sci, Cent Bur Schimmelcultures Fungal Biodivers Ctr, NL-3508 AD Utrecht, Netherlands. [Kurtzman, Cletus P.] ARS, Natl Ctr Agr Utilizat Res, USDA, Peoria, IL 61604 USA. [Blackwell, Meredith] Louisiana State Univ, Dept Biol Sci, Baton Rouge, LA 70803 USA. [Blackwell, Meredith] Univ South Carolina, Dept Biol Sci, Columbia, SC 29208 USA. [Lapidus, Alla] St Petersburg State Univ, Ctr Algorithm Biotechnol, St Petersburg 199004, Russia. [Ohm, Robin A.] Univ Utrecht, Dept Biol, Microbiol, NL-3508 Utrecht, Netherlands. RP Grigoriev, IV (reprint author), Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA.; Jeffries, TW (reprint author), Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. EM IVGrigoriev@lbl.gov; twjeffri@wisc.edu RI Ohm, Robin/I-6689-2016; Lapidus, Alla/I-4348-2013; OI Lapidus, Alla/0000-0003-0427-8731; Calvey, Christopher/0000-0002-7330-4983; Meier-Kolthoff, Jan Philipp/0000-0001-9105-9814; Wolfe, Kenneth/0000-0003-4992-4979 FU Office of Science of the US DOE [DE-AC02-05CH11231]; National Science Foundation [DEB-1442148, DEB-0072741, 0417180]; DOE Great Lakes Bioenergy Research Center; DOE Office of Science Grant [BER DE-FC02-07ER64494]; US Department of Agriculture (USDA) National Institute of Food and Agriculture Hatch Project [1003258]; European Research Council Grant [268893]; Science Foundation Ireland Grant [13/IA/1910]; Wellcome Trust; Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior [7371/13-6]; Pew Charitable Trusts; Alexander von Humboldt Foundation; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-CNPq; DOE Great Lakes Bioenergy Research Center DOE Office of Science Grant [BER DE-FC02-07ER64494]; USDA, Forest Products Laboratory FX We thank Marco A. Soares for computational advice. K.H.W. thanks G. Cagney, E. Dillon, and K. Wynne (University College Dublin Conway Institute Proteomics Core Facility) for help with MS. M.B. thanks Drs. S. O. Suh, H. Urbina, and N. H. Nguyen and numerous Louisiana State University undergraduates for their assistance. The work conducted by the US Department of Energy (DOE) Joint Genome Institute, a DOE Office of Science User Facility, is supported by Office of Science of the US DOE Contract DE-AC02-05CH11231. This material is based on work supported by National Science Foundation Grant DEB-1442148 (to C.T.H. and C.P.K.) and supported in part by DOE Great Lakes Bioenergy Research Center, DOE Office of Science Grant BER DE-FC02-07ER64494, and US Department of Agriculture (USDA) National Institute of Food and Agriculture Hatch Project 1003258. K.H.W. acknowledges European Research Council Grant 268893, Science Foundation Ireland Grant 13/IA/1910, and the Wellcome Trust. M.R.L. acknowledges a fellowship from the Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior (process no. 7371/13-6). C.T.H. is a Pew Scholar in the Biomedical Sciences and an Alfred Toepfer Faculty Fellow, which are supported by the Pew Charitable Trusts and the Alexander von Humboldt Foundation, respectively. C.A.R. acknowledges support from the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico-CNPq. Funding from National Science Foundation Grants DEB-0072741 (to M.B.) and 0417180 (to M.B.) supported discovery and study of many new yeast strains that contributed to this study. T.W.J. acknowledges DOE Great Lakes Bioenergy Research Center DOE Office of Science Grant BER DE-FC02-07ER64494 and the USDA, Forest Products Laboratory for financial support. NR 47 TC 7 Z9 7 U1 13 U2 15 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 30 PY 2016 VL 113 IS 35 BP 9882 EP 9887 DI 10.1073/pnas.1603941113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DV7BL UT WOS:000383090700064 PM 27535936 ER PT J AU Hanaor, DAH Hu, L Kan, WH Proust, G Foley, M Karaman, I Radovic, M AF Hanaor, D. A. H. Hu, L. Kan, W. H. Proust, G. Foley, M. Karaman, I. Radovic, M. TI Compressive performance and crack propagation in Al alloy/Ti2AlC composites SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE MAX phase; Ti2AlC; XRM Tomography, Crack propagation ID CARBIDE-ALUMINUM COMPOSITES; MECHANICAL-PROPERTIES; MATRIX COMPOSITES; CRYSTAL-STRUCTURE; POROUS TI2ALC; STRESS-STRAIN; MAX PHASES; TEMPERATURE; BEHAVIOR; TI3SIC2 AB Composite materials comprising a porous Ti2AlC matrix and Al 6061 alloy were fabricated by a current activated pressure assisted melt infiltration process. Coarse, medium and fine meso-structures were prepared with Al alloy filled pores of differing sizes. Materials were subjected to uniaxial compressive loading up to stresses of 668 MPa, leading to the failure of specimens through crack propagation in both phases. As-fabricated and post-failure specimens were analysed by X-ray microscopy and electron microscopy. Quasi-static mechanical testing results revealed that compressive strength was the highest in the fine structured composite materials. While "the coarse structured specimens exhibited a compressive strength of 80% relative to this. Reconstructed micro-scale X-ray tomography data revealed different crack propagation mechanisms. Large planar shear cracks propagated throughout the fine structured materials while the coarser specimens exhibited networks of branching cracks propagating preferentially along Al alloy-Ti2AlC phase interfaces and through shrinkage pores in the Al alloy phase. Results suggest that control of porosity, compensation for Al alloy shrinkage and enhancement of the Al alloy-Ti2AlC phase interfaces are key considerations in the design of high performance metal/Ti2AlC phase composites. (C) 2016 Elsevier B.V. All rights reserved. C1 [Hanaor, D. A. H.; Kan, W. H.; Proust, G.] Univ Sydney, Sch Civil Engn, Sydney, NSW 2006, Australia. [Karaman, I.; Radovic, M.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Foley, M.] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia. [Hu, L.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Hanaor, DAH (reprint author), Univ Sydney, Sch Civil Engn, Sydney, NSW 2006, Australia. EM dorian.hanaor@sydney.edu.au FU U.S. Air Force Office of Scientific Research, MURI Program [FA9550-09-1-0686]; US National Science Foundation [NSF-1233792]; International Program Development Fund, at the University of Sydney; DVC Research/International Research Collaboration Award, at the University of Sydney FX We acknowledge access to XRM facilities of the Australian Microscopy & Microanalysis Research Facility at the Australian Centre for Microscopy & Microanalysis at the University of Sydney. This work was further supported by the U.S. Air Force Office of Scientific Research, MURI Program (FA9550-09-1-0686) and US National Science Foundation (NSF-1233792) to Texas A&M University. The authors would like to thank the program manager Dr. David Stargel for his support. In addition, the authors are also grateful for the support of the International Program Development Fund and DVC Research/International Research Collaboration Award, at the University of Sydney. NR 47 TC 2 Z9 2 U1 4 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD AUG 30 PY 2016 VL 672 BP 247 EP 256 DI 10.1016/j.msea.2016.06.073 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DU1EZ UT WOS:000381952300028 ER PT J AU Maezawa, Y Petreczky, P AF Maezawa, Y. Petreczky, P. TI Quark masses and strong coupling constant in 2+1 flavor QCD SO PHYSICAL REVIEW D LA English DT Article AB We present a determination of the strange, charm, and bottom quark masses as well as the strong coupling constant in 2 + 1 flavor lattice QCD simulations using highly improved staggered quark action. The ratios of the charm quark mass to the strange quark mass and the bottom quark mass to the charm quark mass are obtained from the meson masses calculated on the lattice and found to be m(c)/m(s) = 11.877(91) and m(b)/m(c) = 4.528(57) in the continuum limit. We also determine the strong coupling constant and the charm quark mass using the moments of pseudoscalar charmonium correlators: alpha(s)(mu = m(c)) = 0.3697(85) and m(c)(mu = m(c)) = 1.267(12) GeV. Our result for as corresponds to the determination of the strong coupling constant at the lowest energy scale so far and is translated to the value alpha(s)(mu = M-Z, n(f) = 5) = 0.11622(84). C1 [Maezawa, Y.] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068317, Japan. [Petreczky, P.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Maezawa, Y (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068317, Japan. FU U.S. Department of Energy [DE-SC0012704] FX This work was supported by U.S. Department of Energy under Contract No. DE-SC0012704. The calculations have been carried out on USQCD clusters in Jlab. We thank Christian Hoebling for useful discussions on the form of continuum extrapolations. NR 42 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 30 PY 2016 VL 94 IS 3 AR 034507 DI 10.1103/PhysRevD.94.034507 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU4IV UT WOS:000382177200003 ER PT J AU Mantysaari, H Schenke, B AF Mantysaari, Heikki Schenke, Bjorn TI Revealing proton shape fluctuations with incoherent diffraction at high energy SO PHYSICAL REVIEW D LA English DT Article ID LARGE MOMENTUM-TRANSFER; PB-PB COLLISIONS; VECTOR-MESONS; J/PSI MESONS; SMALL-X; EXCLUSIVE ELECTROPRODUCTION; ELASTIC ELECTROPRODUCTION; PARTON DISTRIBUTIONS; ROOT-S(NN)=2.76 TEV; QCD ANALYSIS AB The differential cross section of exclusive diffractive vector meson production in electron proton collisions carries important information on the geometric structure of the proton. More specifically, the coherent cross section as a function of the transferred transverse momentum is sensitive to the size of the proton, while the incoherent or proton dissociative cross section is sensitive to fluctuations of the gluon distribution in coordinate space. We show that at high energies the experimentally measured coherent and incoherent cross sections for the production of J/psi mesons are very well reproduced within the color glass condensate framework when strong geometric fluctuations of the gluon distribution in the proton are included. For. meson production, we also find reasonable agreement. We study in detail the dependence of our results on various model parameters, including the average proton shape, analyze the effect of saturation scale and color charge fluctuations and constrain the degree of geometric fluctuations. C1 [Mantysaari, Heikki; Schenke, Bjorn] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Mantysaari, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. FU DOE [DE-SC0012704]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank E. Aschenauer, T. Lappi, S. Schlichting, M. Strikman, T. Ullrich, and R. Venugopalan for discussions. This work was supported under DOE Contract No. DE-SC0012704. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B. P. S. acknowledges a DOE Office of Science Early Career Award. NR 112 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 30 PY 2016 VL 94 IS 3 AR 034042 DI 10.1103/PhysRevD.94.034042 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU4IV UT WOS:000382177200002 ER PT J AU Morrow, R Taylor, AE Singh, DJ Xiong, J Rodan, S Wolter, AUB Wurmehl, S Buchner, B Stone, MB Kolesnikov, AI Aczel, AA Christianson, AD Woodward, PM AF Morrow, Ryan Taylor, Alice E. Singh, D. J. Xiong, Jie Rodan, Steven Wolter, A. U. B. Wurmehl, Sabine Buechner, Bernd Stone, M. B. Kolesnikov, A. I. Aczel, Adam A. Christianson, A. D. Woodward, Patrick M. TI Spin-orbit coupling control of anisotropy, ground state and frustration in 5d(2) Sr2MgOsO6 SO SCIENTIFIC REPORTS LA English DT Article ID DOUBLE PEROVSKITES; MAGNETIC-PROPERTIES; CRYSTAL-GROWTH; TRANSITION; OSMIUM AB The influence of spin-orbit coupling (SOC) on the physical properties of the 5d(2) system Sr2MgOsO6 is probed via a combination of magnetometry, specific heat measurements, elastic and inelastic neutron scattering, and density functional theory calculations. Although a significant degree of frustration is expected, we find that Sr2MgOsO6 orders in a type I antiferromagnetic structure at the remarkably high temperature of 108 K. The measurements presented allow for the first accurate quantification of the size of the magnetic moment in a 5d(2) system of 0.60(2) mu(beta)-a significantly reduced moment from the expected value for such a system. Furthermore, significant anisotropy is identified via a spin excitation gap, and we confirm by first principles calculations that SOC not only provides the magnetocrystalline anisotropy, but also plays a crucial role in determining both the ground state magnetic order and the size of the local moment in this compound. Through comparison to Sr2ScOsO6, it is demonstrated that SOC-induced anisotropy has the ability to relieve frustration in 5d(2) systems relative to their 5d(3) counterparts, providing an explanation of the high TN found in Sr2MgOsO6. C1 [Morrow, Ryan; Xiong, Jie; Woodward, Patrick M.] Ohio State Univ, Dept Chem & Biochem, Columbus, OH 43210 USA. [Taylor, Alice E.; Stone, M. B.; Aczel, Adam A.; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Singh, D. J.] Univ Missouri, Dept Phys & Astron, Columbia, MO 65211 USA. [Rodan, Steven; Wolter, A. U. B.; Wurmehl, Sabine; Buechner, Bernd] Leibniz Inst Solid State & Mat Res Dresden IFW, D-01171 Dresden, Germany. [Wurmehl, Sabine; Buechner, Bernd] Tech Univ Dresden, Inst Solid State Phys, D-01062 Dresden, Germany. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Christianson, A. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Morrow, R (reprint author), Ohio State Univ, Dept Chem & Biochem, Columbus, OH 43210 USA. EM r.c.morrow@ifw-dresden.de RI Stone, Matthew/G-3275-2011; christianson, andrew/A-3277-2016; Wurmehl, Sabine/A-5872-2009 OI Stone, Matthew/0000-0001-7884-9715; christianson, andrew/0000-0003-3369-5884; FU Center for Emergent Materials an NSF Materials Research Science and Engineering Center [DMR-1420451]; Deutsche Forschungsgemeinschaft DFG [WU595/5-1]; National Science Foundation [DMR-1107637]; DFG [WU 595/3-3, SFB 1143]; US Department of Energy, Office of Science, Basic Energy Sciences (BES), Scientific User Facilities Division; Department of Energy S3TEC Energy Frontier Research Center [DE-SC0001299/DE-FG02-09ER46577]; U.S. Department of Energy [DE-AC05-000R22725] FX Support for this research was provided by the Center for Emergent Materials an NSF Materials Research Science and Engineering Center (DMR-1420451), and in the framework of the materials world network (Deutsche Forschungsgemeinschaft DFG project no. WU595/5-1 and National Science Foundation (DMR-1107637)). S. Wurmehl gratefully acknowledges funding by DFG in project WU 595/3-3 (Emmy Noether program) and by DFG in SFB 1143. Research using Oak Ridge National Laboratory's Spallation Neutron Source and High Flux Isotope Reactor facilities was sponsored by the US Department of Energy, Office of Science, Basic Energy Sciences (BES), Scientific User Facilities Division. Work at the University of Missouri (DJS) was funded through the Department of Energy S3TEC Energy Frontier Research Center, award DE-SC0001299/DE-FG02-09ER46577. The authors would like to acknowledge S. Calder and M. D. Lumsden for helpful discussions, and the authors also thankfully acknowledge Ashfia Huq for experimental assistance with POWGEN data collection. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-000R22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doepublic-access-plan). NR 53 TC 1 Z9 1 U1 19 U2 25 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 30 PY 2016 VL 6 AR 32462 DI 10.1038/srep32462 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU4CI UT WOS:000382159000001 PM 27571715 ER PT J AU Yuan, ZL Druzhinina, IS Labbe, J Redman, R Qin, Y Rodriguez, R Zhang, CL Tuskan, GA Lin, FC AF Yuan, Zhilin Druzhinina, Irina S. Labbe, Jessy Redman, Regina Qin, Yuan Rodriguez, Russell Zhang, Chulong Tuskan, Gerald A. Lin, Fucheng TI Specialized Microbiome of a Halophyte and its Role in Helping Non-Host Plants to Withstand Salinity SO SCIENTIFIC REPORTS LA English DT Article ID 16S RIBOSOMAL-RNA; PSEUDOMONAS-FLUORESCENS WCS365; COMPETITIVE ROOT COLONIZATION; BACTERIAL COMMUNITIES; FUNGAL ASSEMBLAGES; STRESS TOLERANCE; HIGH-THROUGHPUT; RHIZOSPHERE; DIVERSITY; EVOLUTION AB Root microbiota is a crucial determinant of plant productivity and stress tolerance. Here, we hypothesize that the superior halo-tolerance of seepweed Suaeda salsa is tightly linked to a specialized belowground microbiome. To test this hypothesis, we performed a phylogenetic trait-based framework analysis based on bacterial 16S rRNA gene and fungal nuclear rRNA internal transcribed spacer profiling. Data showed that the dominant alpha-proteobacteria and gamma-proteobacteria communities in bulk soil and root endosphere tend to be phylogenetically clustered and at the same time exhibit phylogenetic over-dispersion in rhizosphere. Likewise, the dominant fungal genera occurred at high phylogenetic redundancy. Interestingly, we found the genomes of rhizospheric and endophytic bacteria associated with S. salsa to be enriched in genes contributing to salt stress acclimatization, nutrient solubilization and competitive root colonization. A wide diversity of rhizobacteria with similarity to known halotolerant taxa further supported this interpretation. These findings suggest that an ecological patterned root-microbial interaction strategy has been adopted in S. salsa system to confront soil salinity. We also demonstrated that the potential core microbiome members improve non-host plants growth and salt tolerance. This work provides a platform to improve plant fitness with halophytes-microbial associates and novel insights into the functions of plant microbiome under salinity. C1 [Yuan, Zhilin; Qin, Yuan] Chinese Acad Forestry, Inst Subtrop Forestry, Hangzhou, Zhejiang, Peoples R China. [Druzhinina, Irina S.] TU Wien, Inst Chem Engn, Res Area Biochem Technol, Vienna, Austria. [Labbe, Jessy; Tuskan, Gerald A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Redman, Regina; Rodriguez, Russell] Adapt Symbiot Technol, Seattle, WA USA. [Rodriguez, Russell] Univ Washington, Dept Biol, Seattle, WA 98195 USA. [Zhang, Chulong; Lin, Fucheng] Zhejiang Univ, Inst Biotechnol, State Key Lab Rice Biol, Hangzhou, Zhejiang, Peoples R China. RP Yuan, ZL (reprint author), Chinese Acad Forestry, Inst Subtrop Forestry, Hangzhou, Zhejiang, Peoples R China.; Labbe, J (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM yuanzl@caf.ac.cn; labbejj@ornl.gov RI Tuskan, Gerald/A-6225-2011; Labbe, Jessy/G-9532-2011 OI Tuskan, Gerald/0000-0003-0106-1289; Labbe, Jessy/0000-0003-0368-2054 FU Non-Profit Sector Special Research Fund of the Chinese Academy of Forestry [RISF2013005]; National Natural Science Foundation of China [31370704]; Austrian Science Fund (FWF) [P 25745]; Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research; Plant-Microbe Interfaces Scientific Focus Area; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was supported financially by the Non-Profit Sector Special Research Fund of the Chinese Academy of Forestry (RISF2013005) and the National Natural Science Foundation of China (No. 31370704). ISD was supported by the Austrian Science Fund (FWF): project number P 25745. JL was supported by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research as part of the Plant-Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. We would like to extend our sincerest thanks and great appreciation to Prof. Jeff Dangl, the University of North Carolina at Chapel Hill for his useful suggestions and technical assistance. NR 79 TC 3 Z9 3 U1 15 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 30 PY 2016 VL 6 AR 32467 DI 10.1038/srep32467 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU4CL UT WOS:000382159400001 PM 27572178 ER PT J AU Su, X Lin, CK Wang, XP Maroni, VA Ren, Y Johnson, CS Lu, WQ AF Su, Xin Lin, Chikai Wang, Xiaoping Maroni, Victor A. Ren, Yang Johnson, Christopher S. Lu, Wenquan TI A new strategy to mitigate the initial capacity loss of lithium ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Hard carbon; Initial capacity loss; Li5FeO4 (LFO); Lithium source additive; Lithium ion battery ID ELECTROCHEMICAL-BEHAVIOR; SILICON MONOXIDE; ANODE CELL; NANOSTRUCTURES AB Hard carbon (non-graphitizable) and related materials, like tin, tin oxide, silicon, and silicon oxide, have a high theoretical lithium delivery capacity (>550 mAh/g depending on their structural and chemical properties) but unfortunately they also exhibit a large initial capacity loss (ICL) that overrides the true reversible capacity in a full cell. Overcoming the large ICL of hard carbon in a full-cell lithium-ion battery (LIB) necessitates a new strategy wherein a sacrificial lithium source additive, such as, Li5FeO4 (LFO), is inserted on the cathode side. Full batteries using hard carbon coupled with LFO-LiCoO2 (LCO) are currently under development at our laboratory. We find that the reversible capacity of a cathode containing LFO can be increased by 14%. Furthermore, the cycle performance of full cells with LFO additive is improved from <90% to >95%. We show that the LFO additive not only can address the irreversible capacity loss of the anode, but can also provide the additional lithium ion source required to mitigate the lithium loss caused by side reactions. In addition, we have explored the possibility to achieve higher capacity with hard carbon, whereby the energy density of full cells can be increased from ca. 300 Wh/kg to >400 Wh/kg. (C) 2016 Elsevier B.V. All rights reserved. C1 [Su, Xin; Lin, Chikai; Wang, Xiaoping; Maroni, Victor A.; Johnson, Christopher S.; Lu, Wenquan] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. RP Lu, WQ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. EM suxin81@gmail.com; chikai.moses.lin@gmail.com; xiaoping.wang@anl.gov; maroni@anl.gov; ren@aps.anl.gov; cjohnson@anl.gov; luw@anl.gov FU U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Vehicle Technologies Office; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX We gratefully acknowledge support from the U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Vehicle Technologies Office. Part of this work was performed at the Electron Microscopy Center for Materials Research, the Center for Nanoscale Materials, and the Advanced Photon Source, all of which are facilities of the Office of Science (SC) located at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357. NR 15 TC 1 Z9 1 U1 36 U2 59 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 30 PY 2016 VL 324 BP 150 EP 157 DI 10.1016/j.jpowsour.2016.05.063 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DR7JU UT WOS:000380076700019 ER PT J AU Brooks, KP Bowden, ME Karkamkar, AJ Houghton, AY Autrey, ST AF Brooks, Kriston P. Bowden, Mark E. Karkamkar, Abhijeet J. Houghton, Adrian Y. Autrey, S. Thomas TI Coupling of exothermic and endothermic hydrogen storage materials SO JOURNAL OF POWER SOURCES LA English DT Article DE Chemical hydrogen storage; Fuel cell; Reaction coupling; Kinetic modeling ID AMMONIA-BORANE; CATALYTIC HYDROLYSIS; REGENERATION; BOROHYDRIDE; RELEASE; METHANOLYSIS; GENERATION; FUEL; H-2 AB Chemical hydrogen storage (CHS) materials are a high-storage-density alternative to the gaseous compressed hydrogen currently used to provide hydrogen for fuel cell vehicles. One of the challenges of CHS materials is addressing the energy barriers required to break the chemical bonds and release the hydrogen. Coupling CHS reactions that are endothermic and exothermic during dehydrogenation can improve onboard energy efficiency and thermal control for the system, making such materials viable. Acceptable coupling between reactions requires both thermodynamic and kinetic considerations. In this work, models were developed to predict the reaction enthalpy and rate required to achieve high conversions for both reactions based on experimental measurements. Modeling results show that the coupling efficiency of exothermic and endothermic reactions is more sensitive to the ratio of the exothermic and endothermic enthalpies than to the ratio of the rates of the two steps. Modeling results also show that a slower endothermic step rate is desirable to permit sufficient heating of the reactor by the exothermic step. We look at two examples of a sequential and parallel reaction scheme and provide some of the first published insight into the required temperature range to maximize the hydrogen release from 1,2-BN cyclohexane and indoline. (C) 2016 Published by Elsevier B.V. C1 [Brooks, Kriston P.; Bowden, Mark E.; Karkamkar, Abhijeet J.; Houghton, Adrian Y.; Autrey, S. Thomas] Pacific Northwest Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Brooks, KP (reprint author), Pacific Northwest Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM Kriston.brooks@pnnl.gov; Mark.bowden@pnnl.gov; Abhi.Karhamkar@pnnl.gov; Adrian.houghton@pnnl.gov; Tom.autrey@pnnl.gov FU U.S. Department of Energy; Department of Energy [DE-AC05-76RLO1830] FX This work was done at PNNL and sponsored by the U.S. Department of Energy. Special thanks to Dr. Shih-Yuan Liu (Boston College) for providing the CBN materials and directing this project. The authors would also like to thank Ned Stetson and Grace Ordaz for their outstanding support. Battelle operates PNNL for the Department of Energy under contract DE-AC05-76RLO1830. NR 33 TC 0 Z9 0 U1 14 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 30 PY 2016 VL 324 BP 170 EP 178 DI 10.1016/j.jpowsour.2016.05.067 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DR7JU UT WOS:000380076700021 ER PT J AU Wang, ZY Lee, JZ Xin, HLL Han, LL Grillon, N Guy-Bouyssou, D Bouyssou, E Proust, M Meng, YS AF Wang, Ziying Lee, Jungwoo Z. Xin, Huolin L. Han, Lili Grillon, Nathanael Guy-Bouyssou, Delphine Bouyssou, Emilien Proust, Marina Meng, Ying Shirley TI Effects of cathode electrolyte interfacial (CEI) layer on long term cycling of all-solid-state thin-film batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Thin-film battery; Interfacial phenomena; Interface resistance; Solid electrolyte ID RECHARGEABLE LITHIUM BATTERIES; LI-ION BATTERIES; OXIDES; 1ST-PRINCIPLES; INTERCALATION; STABILITY AB All-solid-state lithium-ion batteries have the potential to not only push the current limits of energy density by utilizing Li metal, but also improve safety by avoiding flammable organic electrolyte. However, understanding the role of solid electrolyte electrode interfaces will be critical to improve performance. In this study, we conducted long term cycling on commercially available lithium cobalt oxide (LCO)/lithium phosphorus oxynitride (LiPON)/lithium (Li) cells at elevated temperature to investigate the interfacial phenomena that lead to capacity decay. STEM-EELS analysis of samples revealed a previously unreported disordered layer between the LCO cathode and LiPON electrolyte. This electrochemically inactive layer grew in thickness leading to loss of capacity and increase of interfacial resistance when cycled at 80 degrees C. The stabilization of this layer through interfacial engineering is crucial to improve the long term performance of thin-film batteries especially under thermal stress. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wang, Ziying; Lee, Jungwoo Z.; Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Xin, Huolin L.; Han, Lili] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Grillon, Nathanael; Guy-Bouyssou, Delphine; Bouyssou, Emilien; Proust, Marina] STMicroelectronics, CS 97155, F-37071 Tours 2, France. RP Meng, YS (reprint author), Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM shmeng@ucsd.edu FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0002357]; STMicroelectronics; U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX We would also like to acknowledge the funding for the characterization of all-solid-state battery by the U.S. Department of Energy, Office of Basic Energy Sciences, under award number DE-SC0002357. The authors acknowledge the partial funding support and sample fabrication from STMicroelectronics. This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 23 TC 0 Z9 0 U1 63 U2 99 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 30 PY 2016 VL 324 BP 342 EP 348 DI 10.1016/j.jpowsour.2016.05.098 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DR7JU UT WOS:000380076700041 ER PT J AU Reshetenko, T Serov, A Artyushkova, K Matanovic, I Stariha, S Atanassov, P AF Reshetenko, Tatyana Serov, Alexey Artyushkova, Kateryna Matanovic, Ivana Stariha, Sarah Atanassov, Plamen TI Tolerance of non-platinum group metals cathodes proton exchange membrane fuel cells to air contaminants SO JOURNAL OF POWER SOURCES LA English DT Article DE Non-platinum group metals catalysts; PEMFC; Airborne contaminants; Segmented cell; XPS; DFT ID OXYGEN REDUCTION REACTION; DENSITY-FUNCTIONAL THEORY; ELECTROCHEMICAL IMPEDANCE SPECTROSCOPY; BRILLOUIN-ZONE INTEGRATIONS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CARBON-MONOXIDE; PEMFC PERFORMANCE; NITROGEN-OXIDES AB The effects of major airborne contaminants (SO2, NO2 and CO) on the spatial performance of Fe/N/C cathode membrane electrode assemblies were studied using a segmented cell system. The injection of 2-10 ppm SO2 in air stream did not cause any performance decrease and redistribution of local currents due to the lack of stably adsorbed SO2 molecules on Fe-N-x sites, as confirmed by density functional theory (DFT) calculations. The introduction of 5-20 ppm of CO into the air stream also did not affect fuel cell performance. The exposure of Fe/N/C cathodes to 2 and 10 ppm NO2 resulted in performance losses of 30 and 70-75 mV, respectively. DFT results showed that the adsorption energies of NO2 and NO were greater than that of O-2, which accounted for the observed voltage decrease and slight current redistribution. The cell performance partially recovered when the NO2 injection was stopped. The long-term operation of the fuel cells resulted in cell performance degradation. XPS analyses of Fe/N/C electrodes revealed that the performance decrease was due to catalyst degradation and ionomer oxidation. The latter was accelerated in the presence of air contaminants. The details of the spatial performance and electrochemical impedance spectroscopy results are presented and discussed. (C) 2016 Elsevier B.V. All rights reserved. C1 [Reshetenko, Tatyana] Univ Hawaii, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. [Serov, Alexey; Artyushkova, Kateryna; Matanovic, Ivana; Stariha, Sarah; Atanassov, Plamen] Univ New Mexico, Dept Chem & Biol Engn, UNM Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Matanovic, Ivana] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reshetenko, T (reprint author), Univ Hawaii, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. EM tatyanar@hawaii.edu FU Office of Biological and Environmental Research of the Department of Energy located at Pacific Northwest National Laboratory [48823]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [CNMS2015-027]; DOE-EERE Fuel Cell Technology Program [FC132]; Office of Naval Research [N00014-11-1-0391] FX Computational work was performed using the computational resources of EMSL, a national scientific user facility sponsored by the Office of Biological and Environmental Research of the Department of Energy located at Pacific Northwest National Laboratory (award number 48823); NERSC, supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231; and CNMS, sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (award CNMS2015-027). This work was supported in part by the DOE-EERE Fuel Cell Technology Program FC132 (subcontract to Northeastern University, with PI Sanjeev Mukerjee). T. Reshetenko is grateful for the funding from the Office of Naval Research (N00014-11-1-0391) and the Hawaiian Electric Company for their ongoing support of the Hawaii Sustainable Energy Research Facility. This paper has been designated LA-UR-15-29303. NR 92 TC 4 Z9 4 U1 26 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 30 PY 2016 VL 324 BP 556 EP 571 DI 10.1016/j.jpowsour.2016.05.090 PG 16 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DR7JU UT WOS:000380076700064 ER PT J AU Bzdak, A Koch, V Liao, JF AF Bzdak, Adam Koch, Volker Liao, Jinfeng TI Particle correlations and the chiral magnetic effect SO EUROPEAN PHYSICAL JOURNAL A LA English DT Review ID HEAVY-ION COLLISIONS; VIOLATION; TRANSPORT AB In this contribution we will discuss current measurements of particle correlations and their implication for possible local parity violation in heavy-ion collisions. C1 [Bzdak, Adam] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Koch, Volker] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Liao, Jinfeng] Indiana Univ, Dept Phys, 2401 N Milo B Sampson Lane, Bloomington, IN 47408 USA. [Liao, Jinfeng] Indiana Univ, Ctr Explorat Energy & Matter, 2401 N Milo B Sampson Lane, Bloomington, IN 47408 USA. [Liao, Jinfeng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Bldg 510A, Upton, NY 11973 USA. RP Bzdak, A (reprint author), AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. EM bzdak@fis.agh.edu.pl; vkoch@lbl.gov; liaoji@indiana.edu FU Ministry of Science and Higher Education (MNiSW); Foundation for Polish Science; National Science Centre (Narodowe Centrum Nauki) [DEC-2014/15/B/ST2/00175]; Office of Basic Energy Sciences, Division of Nuclear Sciences, of the U.S. Department of Energy [DE-AC03-76SF00098]; DOE [DE-AC02-98CH10886]; NSF [PHY-1352368]; RIKEN BNL Research Center; [DEC-2013/09/B/ST2/00497] FX AB was supported by the Ministry of Science and Higher Education (MNiSW), by funding from the Foundation for Polish Science, and by the National Science Centre (Narodowe Centrum Nauki), Grant No. DEC-2014/15/B/ST2/00175, and in part by DEC-2013/09/B/ST2/00497. VK was supported by the Director, Office of Science, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, and by the Office of Basic Energy Sciences, Division of Nuclear Sciences, of the U.S. Department of Energy under Contract No. DE-AC03-76SF00098 and DOE Contract No. DE-AC02-98CH10886. JL was partly supported by the NSF (Grant No. PHY-1352368) and by the RIKEN BNL Research Center. NR 28 TC 0 Z9 0 U1 2 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD AUG 29 PY 2016 VL 52 IS 8 AR 265 DI 10.1140/epja/i2016-16265-0 PG 6 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DZ7FC UT WOS:000386029300001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Older, AAAF Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, N Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Amor Dos Santo, SP Amorim, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Fi, FA Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barranco Navarro, L Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Bates, RL 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Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the angular coefficients in Z-boson events using electron and muon pairs from data taken at root s=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments) ID PARTON DISTRIBUTIONS; HADRONIC COLLISIONS; MONTE-CARLO; CHARGE ASYMMETRY; INTERFERENCE; RESONANCE; DECAY; ORDER; LHC AB The angular distributions of Drell-Yan charged lepton pairs in the vicinity of the Z-boson mass peak probe the underlying QCD dynamics of Z-boson production. This paper presents a measurement of the complete set of angular coefficients Lambda(0-7) describing these distributions in the Z-boson Collins-Soper frame. The data analysed correspond to 20.3 fb(-1) of pp collisions at root s = 8TeV, collected by the ATLAS detector at the CERN LHC. The measurements are compared to the most precise fixed-order calculations currently available (O (alpha(2)(s))) and with theoretical predictions embedded in Monte Carlo generators. The measurements are precise enough to probe QCD corrections beyond the formal accuracy of these calculations and to provide discrimination between different parton-shower models. A signi fi cant deviation from the O (alpha(2)(s)) predictions is observed for A(0)-A(2). Evidence is found for non-zero A(5,6, 7), consistent with expectations. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Ernst, J.; Fischer, A.; Franchini, M.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Czodrowski, P.; Dassoulas, J.; Dehghanian, N.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. 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W.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Webster, J. S.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Jones, S.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E. St.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Andeen, T.; Ilchenko, Y.; Narayan, R.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavallaro, E.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fernandez Perez, S.; Fischer, C.; Fracchia, S.; Gerbaudo, D.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Rizzi, C.; Rodriguez Perez, A.; Sorin, V.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Barcelona Inst Sci & Technol, IFAE, Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bokan, P.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Sjursen, T. B.; Smestad, L.; Stugu, B.; Yang, Z.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heim, T.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Mergelmeyer, S.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; Zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Meloni, F.; Mullier, G. A.; Rimoldi, M.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Meloni, F.; Mullier, G. A.; Rimoldi, M.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Broughton, J. H.; Casadei, D.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Foster, A. G.; Gonella, L.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Flowerdew, M. J.; Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; D'amen, G.; De Castro, S.; Fabbri, F.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Ucchielli, G.; Valentinetti, S.; Villa, M.; Vittori, C.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; D'amen, G.; De Castro, S.; Fabbri, F.; Fabbri, L.; Gabrielli, A.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Ucchielli, G.; Valentinetti, S.; Villa, M.; Vittori, C.; Zoccoli, A.] Univ Bologna, Dipartimento Fis Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Ghneimat, M.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Physikal Inst, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.; Peralva, B. S.] Fed Univ Juiz Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Elmsheuser, J.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Tricoli, A.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dobre, M.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Marceca, G.; Otero Y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Lester, C. G.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ruiz-Martinez, A.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Fi, F. Anghinol; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Di Nardo, R.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Starz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Liang, Z.; Merino, J. Llorente; Lou, X.; Mansour, J. D.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.; Zhang, H.; Zhang, R.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Li, Q.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Li, Q.; Yang, H.] PKU CHEP, Beijing, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Cosenza, Italy. [Aloisio, A.; Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Dept Phys, Dallas, TX USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Garay Walls, F. M.; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Aloisio, A.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Nagel, M.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Khoo, T. J.; Lionti, A. E.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Camincher, C.; Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; De Maria, A.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Quadt, A.; Rieger, J.; Rosien, N. -A.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Albrand, S.; Berlendis, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Zu Theenhausen, H. Meyer; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Aloisio, A.; Anders, C. F.; Annovi, A.; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Lu, H.; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Milic, A.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Reale, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Leece, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Reale, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Older, A. A. A. Ff; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Sevan, B. P. Ker; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Sevan, B. P. Ker; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris 06, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; De la Torre, H.; Del Peso, J.; Glasman, C.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Queitsch-Maitland, M.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Yildirim, E.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Raine, J. A.; Schweiger, H.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Vachon, B.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Vachon, B.; Wang, C.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Shaw, S. M.; Stockton, M. C.; Stoebe, M.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Le, B.; McDonald, E. F.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Citterio, M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Camplani, A.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energ Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Ducu, O. A.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Mochizuki, K.; Manh, T. Nguyen; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skoebltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Hartmann, N. M.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Rauscher, F.; Ruschke, A.; Schachtner, B. M.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; De Groot, N.; Filthaut, F.; Galea, C.; Igonkina, O.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Saha, P.] Northern Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Rubbo, F.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK USA. [Cantero, J.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris Saclay, CNRS, IN2P3, Univ Paris 11,LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gon, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.; Amorim, A.; Carvalho, J.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Tavares Delgado, A.; Wolters, H.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Galhardo, B.; Veloso, F.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fisica Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC Fac Ciencias Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Rome, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Thompson, E. N.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondament Univers, DSM,IRFU, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schier, S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vichou, I.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Armbruster, A. J.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Blazek, T.; Dado, T.; Melo, M.; Plazak, L.; Smiesko, J.; Sykora, I.; Zenis, T.] Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron & Chem, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Miano, F.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bartos, P.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.; Tokar, S.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Hod, N.; Jovicevic, J.; Codina, E. Perez; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.; Yacoob, S.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Cobal, M.; Govender, N.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Giordani, M. P.; Pinamonti, M.; Ruan, X.; Soualah, R.; Truong, L.] Univ Udine, Fis & Ambiente, Dipartimento Chim, Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Viazlo, O.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. 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D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Igonkina, O.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.; Tompkins, L.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pasztor, G.] Eotvos Lorand Univ, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ South Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Warburton, Andreas/N-8028-2013; Mitsou, Vasiliki/D-1967-2009; Brooks, William/C-8636-2013; Camarri, Paolo/M-7979-2015; Prokoshin, Fedor/E-2795-2012; Mindur, Bartosz/A-2253-2017; Ventura, Andrea/A-9544-2015; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; White, Ryan/E-2979-2015; Kantserov, Vadim/M-9761-2015; Shulga, Evgeny/R-1759-2016; Lazzaroni, Massimo/N-3675-2015; Maleev, Victor/R-4140-2016; Kukla, Romain/P-9760-2016; Gladilin, Leonid/B-5226-2011; Gavrilenko, Igor/M-8260-2015; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Owen, Mark/Q-8268-2016; Livan, Michele/D-7531-2012; Doyle, Anthony/C-5889-2009; Boyko, Igor/J-3659-2013; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017 OI Kuday, Sinan/0000-0002-0116-5494; Warburton, Andreas/0000-0002-2298-7315; Mitsou, Vasiliki/0000-0002-1533-8886; Brooks, William/0000-0001-6161-3570; Camarri, Paolo/0000-0002-5732-5645; Prokoshin, Fedor/0000-0001-6389-5399; Mindur, Bartosz/0000-0002-5511-2611; Ventura, Andrea/0000-0002-3368-3413; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; White, Ryan/0000-0003-3589-5900; Kantserov, Vadim/0000-0001-8255-416X; Shulga, Evgeny/0000-0001-5099-7644; Lazzaroni, Massimo/0000-0002-4094-1273; Kukla, Romain/0000-0002-1140-2465; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Owen, Mark/0000-0001-6820-0488; Livan, Michele/0000-0002-5877-0062; Doyle, Anthony/0000-0001-6322-6195; Boyko, Igor/0000-0002-3355-4662; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI; Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020 and Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme; Thales programme; Aristeia programme; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; CFI, Canada FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. NR 64 TC 0 Z9 0 U1 43 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 29 PY 2016 IS 8 AR 159 DI 10.1007/JHEP08(2016)159 PG 101 WC Physics, Particles & Fields SC Physics GA DV5OY UT WOS:000382978700001 ER PT J AU Crowhurst, JC Armstrong, MR Gates, SD Zaug, JM Radousky, HB Teslich, NE AF Crowhurst, Jonathan C. Armstrong, Michael R. Gates, Sean D. Zaug, Joseph M. Radousky, Harry B. Teslich, Nick E. TI Yielding of tantalum at strain rates up to 10(9) s(-1) SO APPLIED PHYSICS LETTERS LA English DT Article ID SPECTRAL INTERFEROMETRY; RAMP COMPRESSION; FILMS; GPA AB We have used a 45 mu J laser pulse to accelerate the free surface of fine-grained tantalum films up to peak velocities of similar to 1.2 km s(-1). The films had thicknesses of similar to 1-2 mu m and in-plane grain widths of similar to 75-150 nm. Using ultrafast interferometry, we have measured the time history of the velocity of the surface at different spatial positions across the accelerated region. The initial part of the histories (assumed to correspond to the "elastic precursor" observed previously) exhibited measured strain rates of similar to 0.6 to similar to 3.2 x 10(9) s(-1) and stresses of similar to 4 to similar to 22GPa. Importantly, we find that elastic amplitudes exhibit little variation with strain rate for a constant peak surface velocity, even though, via covariation of the strain rate with peak surface velocity, they vary with strain rate. Furthermore, by comparison with data obtained at lower strain rates, we find that amplitudes are much better predicted by peak velocities rather than by either strain rate or sample thickness. Published by AIP Publishing. C1 [Crowhurst, Jonathan C.; Armstrong, Michael R.; Gates, Sean D.; Zaug, Joseph M.; Radousky, Harry B.; Teslich, Nick E.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Crowhurst, JC (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM crowhurst1@llnl.gov; armstrong30@llnl.gov OI Zaug, Joseph/0000-0001-8999-3800 FU U.S. Department of Energy [DE-AC52-07NA27344]; Laboratory Directed Research and Development [12ERD042] FX We are grateful to K. A. Bettencourt, P. B. Mirkarimi and J. B. Alameda for the synthesis and characterization of our samples. We acknowledge numerous enlightening conversations with R. F. Smith, R. E. Rudd, H.-S. Park, C. E. Wehrenberg, B. A. Remington, V. V. Bulatov, T. W. Barbee, J. L. Belof, R. A. Austin, J. Marian, P. V. Grivickas, E. Stavrou, and L. E. Fried. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 with Laboratory Directed Research and Development funding (12ERD042). NR 30 TC 0 Z9 0 U1 18 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 094102 DI 10.1063/1.4960796 PG 5 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900052 ER PT J AU Jiang, H Chou, KW Petrash, S Williams, G Thieme, J Nykypanchuk, D Li, L Muto, A Chen-Wiegart, YCK AF Jiang, Hua Chou, Kang Wei Petrash, Stanislas Williams, Garth Thieme, Juergen Nykypanchuk, Dmytro Li, Li Muto, Atsushi Chen-Wiegart, Yu-chen Karen TI Environmentally induced chemical and morphological heterogeneity of zinc oxide thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID DAMP-HEAT; SOLAR-CELLS; TRANSPARENT; DEGRADATION; STABILITY; BEHAVIOR AB Zinc oxide (ZnO) thin films have been reported to suffer from degradation in electrical properties, when exposed to elevated heat and humidity, often leading to failures of electronic devices containing ZnO films. This degradation appears to be linked to water and oxygen penetration into the ZnO film. However, a direct observation in the ZnO film morphological evolution detailing structural and chemical changes has been lacking. Here, we systematically investigated the chemical and morphological heterogeneities of ZnO thin films caused by elevated heat and humidity, simulating an environmental aging. X-ray fluorescence microscopy, X-ray absorption spectroscopy, grazing incidence small angle and wide angle X-ray scattering, scanning electron microscopy (SEM), ultra-high-resolution SEM, and optical microscopy were carried out to examine ZnO and Al-doped ZnO thin films on two different substrates-silicon wafers and flexible polyethylene terephthalate (PET) films. In the un-doped ZnO thin film, the simulated environmental aging is resulting in pin-holes. In the Al-doped ZnO thin films, significant morphological changes occurred after the treatment, with an appearance of platelet-shaped structures that are 100-200 nm wide by 1 mu m long. Synchrotron x-ray characterization further confirmed the heterogeneity in the aged Al-doped ZnO, showing the formation of anisotropic structures and disordering. X-ray diffraction and X-ray absorption spectroscopy indicated the formation of a zinc hydroxide in the aged Al-doped films. Utilizing advanced characterization methods, our studies provided information with an unprecedented level of details and revealed the chemical and morphologically heterogeneous nature of the degradation in ZnO thin films. Published by AIP Publishing. C1 [Jiang, Hua] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11790 USA. [Chou, Kang Wei] Henkel Iber SA, Edificio Eureka,Campus UAB, Barcelona 08193, Spain. [Petrash, Stanislas] Henkel Corp, 10 Finderne Ave, Bridgewater, NJ 08807 USA. [Williams, Garth; Thieme, Juergen; Li, Li; Chen-Wiegart, Yu-chen Karen] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, 743 Brookhaven Ave, Upton, NY 11973 USA. [Nykypanchuk, Dmytro] Brookhaven Natl Lab, Ctr Funct Nanomat, 735 Brookhaven Ave, Upton, NY 11973 USA. [Muto, Atsushi] Hitachi High Technol Amer, 22610 Gateway Ctr Dr, Clarksburg, MD 20871 USA. RP Chen-Wiegart, YCK (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, 743 Brookhaven Ave, Upton, NY 11973 USA. EM ycchen@bnl.gov FU LDRD grant - Brookhaven National Laboratory; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The development of PyXRF software was supported by LDRD grant, funded by Brookhaven National Laboratory-we acknowledge the funding support and the collaboration with Yong Chu (NSLS-II), the principal investigator of the project.; The use of the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. The Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 31 TC 0 Z9 0 U1 10 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 091909 DI 10.1063/1.4962203 PG 5 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900018 ER PT J AU Lamichhane, TN Taufour, V Masters, MW Parker, DS Kaluarachchi, US Thimmaiah, S Bud'ko, SL Canfield, PC AF Lamichhane, Tej N. Taufour, Valentin Masters, Morgan W. Parker, David S. Kaluarachchi, Udhara S. Thimmaiah, Srinivasa Bud'ko, Sergey L. Canfield, Paul C. TI Discovery of ferromagnetism with large magnetic anisotropy in ZrMnP and HfMnP SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETOCRYSTALLINE ANISOTROPY; SINGLE-CRYSTALS; TEMPERATURE; TRANSITIONS; ENERGY; MNBI AB ZrMnP and HfMnP single crystals are grown by a self-flux growth technique, and structural as well as temperature dependent magnetic and transport properties are studied. Both compounds have an orthorhombic crystal structure. ZrMnP and HfMnP are ferromagnetic with Curie temperatures around 370 K and 320 K, respectively. The spontaneous magnetizations of ZrMnP and HfMnP are determined to be 1.9 mu(B)/f.u. and 2.1 mu(B)/f.u., respectively, at 50 K. The magnetocaloric effect of ZrMnP in terms of entropy change (Delta S) is estimated to be -6.7 kJ m(-3) K-1 around 369 K. The easy axis of magnetization is [100] for both compounds, with a small anisotropy relative to the [010] axis. At 50 K, the anisotropy field along the [001] axis is similar to 4.6 T for ZrMnP and similar to 10T for HfMnP. Such large magnetic anisotropy is remarkable considering the absence of rare-earth elements in these compounds. The first principle calculation correctly predicts the magnetization and hard axis orientation for both compounds, and predicts the experimental HfMnP anisotropy field within 25%. More importantly, our calculations suggest that the large magnetic anisotropy comes primarily from the Mn atoms, suggesting that similarly large anisotropies may be found in other 3d transition metal compounds. Published by AIP Publishing. C1 [Lamichhane, Tej N.; Taufour, Valentin; Masters, Morgan W.; Kaluarachchi, Udhara S.; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Lamichhane, Tej N.; Taufour, Valentin; Kaluarachchi, Udhara S.; Thimmaiah, Srinivasa; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Parker, David S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Lamichhane, TN (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.; Lamichhane, TN (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Office of Basic Energy Sciences, Materials Sciences Division, U.S. DOE; DOE [DE-AC02-07CH11358] FX We would like to thank T. Kong, G. Drachuck, W. Meier for useful discussions. Dr. Warren Straszheim is acknowledged for doing WDS on various samples. T.N.L., V.T., D.S.P., S.L.B., and P.C.C. were supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. S.T., M.W.M., and U.S.K. were supported by the Office of Basic Energy Sciences, Materials Sciences Division, U.S. DOE. This work was performed at the Ames Laboratory, operated for DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 30 TC 0 Z9 0 U1 14 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 092402 DI 10.1063/1.4961933 PG 4 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900025 ER PT J AU Lu, TM Gamble, JK Muller, RP Nielsen, E Bethke, D Ten Eyck, GA Pluym, T Wendt, JR Dominguez, J Lilly, MP Carroll, MS Wanke, MC AF Lu, T. M. Gamble, J. K. Muller, R. P. Nielsen, E. Bethke, D. Ten Eyck, G. A. Pluym, T. Wendt, J. R. Dominguez, J. Lilly, M. P. Carroll, M. S. Wanke, M. C. TI Fabrication of quantum dots in undoped Si/Si0.8Ge0.2 heterostructures using a single metal-gate layer SO APPLIED PHYSICS LETTERS LA English DT Article AB Enhancement-mode Si/SiGe electron quantum dots have been pursued extensively by many groups for their potential in quantum computing. Most of the reported dot designs utilize multiple metal-gate layers and use Si/SiGe heterostructures with Ge concentration close to 30%. Here, we report the fabrication and low-temperature characterization of quantum dots in the Si/Si0.8Ge0.2 heterostructures using only one metal-gate layer. We find that the threshold voltage of a channel narrower than 1 mu m increases as the width decreases. The higher threshold can be attributed to the combination of quantum confinement and disorder. We also find that the lower Ge ratio used here leads to a narrower operational gate bias range. The higher threshold combined with the limited gate bias range constrains the device design of lithographic quantum dots. We incorporate such considerations in our device design and demonstrate a quantum dot that can be tuned from a single dot to a double dot. The device uses only a single metal-gate layer, greatly simplifying device design and fabrication. Published by AIP Publishing. C1 [Lu, T. M.; Gamble, J. K.; Muller, R. P.; Nielsen, E.; Bethke, D.; Ten Eyck, G. A.; Pluym, T.; Wendt, J. R.; Dominguez, J.; Lilly, M. P.; Carroll, M. S.; Wanke, M. C.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Lu, TM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tlu@sandia.gov OI Muller, Richard/0000-0002-1649-7838 FU U.S. DOE's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. DOE, Office of Basic Energy Sciences, user facility. Sandia National Laboratories is a multi program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 14 TC 1 Z9 1 U1 3 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 093102 DI 10.1063/1.4961889 PG 4 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900037 ER PT J AU Pramanick, A Stoica, AD An, K AF Pramanick, Abhijit Stoica, Alexandru D. An, Ke TI High-resolution 2-D Bragg diffraction reveal heterogeneous domain transformation behavior in a bulk relaxor ferroelectric SO APPLIED PHYSICS LETTERS LA English DT Article ID SINGLE-CRYSTALS; POLARIZATION AB In-situ measurement of fine-structure of neutron Bragg diffraction peaks from a relaxor single-crystal using a time-of-flight instrument reveals highly heterogeneous mesoscale domain transformation behavior under applied electric fields. It is observed that only similar to 25% of domains undergo reorientation or phase transition contributing to large average strains, while at least 40% remain invariant and exhibit microstrains. Such insights could be central for designing new relaxor materials with better performance and longevity. The current experimental technique can also be applied to resolve complex mesoscale phenomena in other functional materials. Published by AIP Publishing. C1 [Pramanick, Abhijit] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. [Stoica, Alexandru D.; An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Pramanick, A (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. EM apramani@cityu.edu.hk RI An, Ke/G-5226-2011; OI An, Ke/0000-0002-6093-429X; Pramanick, Abhijit/0000-0003-0687-4967 FU City University of Hong Kong; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development project at ORNL FX A.P. acknowledges the funding support from the City University of Hong Kong. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors acknowledge H. D. Skorpenske for his technical support for the neutron experiment. Some equipment for this project were procured through funding from a Laboratory Directed Research and Development project at ORNL. NR 37 TC 0 Z9 0 U1 11 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 092907 DI 10.1063/1.4962270 PG 5 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900035 ER PT J AU Zaunbrecher, KN Kuciauskas, D Swartz, CH Dippo, P Edirisooriya, M Ogedengbe, OS Sohal, S Hancock, BL LeBlanc, EG Jayathilaka, PARD Barnes, TM Myers, TH AF Zaunbrecher, Katherine N. Kuciauskas, Darius Swartz, Craig H. Dippo, Pat Edirisooriya, Madhavie Ogedengbe, Olanrewaju S. Sohal, Sandeep Hancock, Bobby L. LeBlanc, Elizabeth G. Jayathilaka, Pathiraja A. R. D. Barnes, Teresa M. Myers, Thomas H. TI Impact of extended defects on recombination in CdTe heterostructures grown by molecular beam epitaxy SO APPLIED PHYSICS LETTERS LA English DT Article ID CADMIUM TELLURIDE; SOLAR-CELLS; LIFETIME; LUMINESCENCE AB Heterostructures with CdTe and CdTe1-xSex (x similar to 0.01) absorbers between two wider-band-gap Cd1-xMgxTe barriers (x similar to 0.25-0.3) were grown by molecular beam epitaxy to study carrier generation and recombination in bulk materials with passivated interfaces. Using a combination of confocal photoluminescence (PL), time-resolved PL, and low-temperature PL emission spectroscopy, two extended defect types were identified and the impact of these defects on charge-carrier recombination was analyzed. The dominant defects identified by confocal PL were dislocations in samples grown on (211) B CdTe substrates and crystallographic twinning-related defects in samples on (100)-oriented InSb substrates. Low-temperature PL shows that twin-related defects have a zero-phonon energy of 1.460 eV and a Huang-Rhys factor of 1.50, while dislocation-dominated samples have a 1.473-eV zero-phonon energy and a Huang-Rhys factor of 1.22. The charge carrier diffusion length near both types of defects is similar to 6 mu m, suggesting that recombination is limited by diffusion dynamics. For heterostructures with a low concentration of extended defects, the bulk lifetime was determined to be 2.2 mu s with an interface recombination velocity of 160 cm/s and an estimated radiative lifetime of 91 mu s. Published by AIP Publishing. C1 [Zaunbrecher, Katherine N.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Zaunbrecher, Katherine N.; Kuciauskas, Darius; Dippo, Pat; Barnes, Teresa M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Swartz, Craig H.; Edirisooriya, Madhavie; Ogedengbe, Olanrewaju S.; Sohal, Sandeep; Hancock, Bobby L.; LeBlanc, Elizabeth G.; Jayathilaka, Pathiraja A. R. D.; Myers, Thomas H.] Texas State Univ, Mat Sci Engn & Commercializat Program, San Marcos, TX 78666 USA. RP Zaunbrecher, KN (reprint author), Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA.; Zaunbrecher, KN (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. OI LeBlanc, Elizabeth/0000-0003-0520-8268; Kuciauskas, Darius/0000-0001-8091-5718 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy [DE-AC36-08GO28308] FX The authors would like to thank Jim Sites for many useful discussions. This research was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, under Contract No. DE-AC36-08GO28308. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 42 TC 4 Z9 4 U1 9 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 29 PY 2016 VL 109 IS 9 AR 091904 DI 10.1063/1.4961989 PG 4 WC Physics, Applied SC Physics GA DX5EF UT WOS:000384401900013 ER PT J AU Zhang, YW Jin, K Xue, HZ Lu, CY Olsen, RJ Beland, LK Ullah, MW Zhao, SJ Bei, HB Aidhy, DS Samolyuk, GD Wang, LM Caro, M Caro, A Stocks, GM Larson, BC Robertson, IM Correa, AA Weber, WJ AF Zhang, Yanwen Jin, Ke Xue, Haizhou Lu, Chenyang Olsen, Raina J. Beland, Laurent K. Ullah, Mohammad W. Zhao, Shijun Bei, Hongbin Aidhy, Dilpuneet S. Samolyuk, German D. Wang, Lumin Caro, Magdalena Caro, Alfredo Stocks, G. Malcolm Larson, Ben C. Robertson, Ian M. Correa, Alfredo A. Weber, William J. TI Influence of chemical disorder on energy dissipation and defect evolution in advanced alloys SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID HIGH-ENTROPY ALLOYS; SOLID-SOLUTION ALLOYS; ACTIVATION-RELAXATION TECHNIQUE; STACKING-FAULT TETRAHEDRA; ION-IRRADIATED NI; ATOMISTIC SIMULATIONS; PHYSICAL-PROPERTIES; PHASE-STABILITY; CLUSTERS; COPPER AB Historically, alloy development with better radiation performance has been focused on traditional alloys with one or two principal element(s) and minor alloying elements, where enhanced radiation resistance depends on microstructural or nanoscale features to mitigate displacement damage. In sharp contrast to traditional alloys, recent advances of single-phase concentrated solid solution alloys (SP-CSAs) have opened up new frontiers in materials research. In these alloys, a random arrangement of multiple elemental species on a crystalline lattice results in disordered local chemical environments and unique site-to-site lattice distortions. Based on closely integrated computational and experimental studies using a novel set of SP-CSAs in a face-centered cubic structure, we have explicitly demonstrated that increasing chemical disorder can lead to a substantial reduction in electron mean free paths, as well as electrical and thermal conductivity, which results in slower heat dissipation in SP-CSAs. The chemical disorder also has a significant impact on defect evolution under ion irradiation. Considerable improvement in radiation resistance is observed with increasing chemical disorder at electronic and atomic levels. The insights into defect dynamics may provide a basis for understanding elemental effects on evolution of radiation damage in irradiated materials and may inspire new design principles of radiation-tolerant structural alloys for advanced energy systems. C1 [Zhang, Yanwen; Jin, Ke; Olsen, Raina J.; Beland, Laurent K.; Ullah, Mohammad W.; Zhao, Shijun; Bei, Hongbin; Samolyuk, German D.; Stocks, G. Malcolm; Larson, Ben C.; Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Xue, Haizhou; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Lu, Chenyang; Wang, Lumin] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Aidhy, Dilpuneet S.] Univ Wyoming, Dept Mech Engn, Laramie, WY 82071 USA. [Caro, Magdalena; Caro, Alfredo] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Robertson, Ian M.] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Correa, Alfredo A.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. RP Zhang, YW (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM zhangy1@ornl.gov RI Stocks, George Malcollm/Q-1251-2016; Weber, William/A-4177-2008; Zhao, Shijun/E-1488-2017; Ullah, Mohammad/E-1526-2017; OI Stocks, George Malcollm/0000-0002-9013-260X; Weber, William/0000-0002-9017-7365; Zhao, Shijun/0000-0003-0870-8153; Ullah, Mohammad/0000-0001-6190-591X; Bei, Hongbin/0000-0003-0283-7990 FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Office of Science, US Department of Energy [DEAC02-05CH11231]; Fonds Quebeecois de recherche Nature et Technologies; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX This work was supported as part of the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. Ion beam work was performed at the University of Tennessee-Oak Ridge National Laboratory Ion Beam Materials Laboratory (IBML) located at the campus of the University of Tennessee, Knoxville. This simulation used resources of the National Energy Research Scientific Computing Center, supported by the Office of Science, US Department of Energy, under Contract No. DEAC02-05CH11231. LKB acknowledgs additional support from a fellowship awarded by the Fonds Quebeecois de recherche Nature et Technologies. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-publicaccess-plan). NR 61 TC 2 Z9 2 U1 27 U2 30 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD AUG 29 PY 2016 VL 31 IS 16 BP 2363 EP 2375 DI 10.1557/jmr.2016.269 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA DV5MX UT WOS:000382972800001 ER PT J AU Wang, RX Yang, B Luo, ZL Sun, EW Sun, Y Xu, H Zhao, JT Zheng, LM Zhou, H Gao, C Cao, WW AF Wang, Ruixue Yang, Bin Luo, Zhenlin Sun, Enwei Sun, Yuan Xu, Han Zhao, Jiangtao Zheng, Limei Zhou, Hua Gao, Chen Cao, Wenwu TI Local twin domains and tip-voltage-induced domain switching of monoclinic M-C phase in Pb(Mg1/3Nb2/3)O-3-0.34PbTiO(3) single crystal revealed by piezoresponse force microscopy SO PHYSICAL REVIEW B LA English DT Article ID ENHANCED PIEZOELECTRIC PROPERTIES; ELECTROMECHANICAL RESPONSE; FERROELECTRIC PHASE; PBZR1-XTIXO3; TRANSITION; BOUNDARY; ORIGIN; GROWTH; STATE AB The monoclinic (M) phases in high-performance relaxor-based ferroelectric single crystals have been recognized to be a vital structural factor for the outstanding piezoelectric property. However, due to the complexity of the structure in M phases, the understanding about it is still limited. In this paper, the local twin domains and tip-voltage-induced domain switching of the M-C phase in Pb(Mg1/3Nb2/3)O-3-0.34PbTiO(3) (PMN-0.34PT) single crystal have been intensively investigated by piezoresponse force microscopy (PFM). By theoretically analyzing the experimental patterns of domain walls on the (001)(C) face, the specificM(C) twin domains in the initial annealed state of a selected area have been clarified, and the polarization orientation of the M-C phase in this sample is determined to be at an angle of 29 degrees to the < 001 >(C) directions. In addition, based on the evolution of domains and the motion of domain walls under the step-increased PFM tip dc voltage (V-dc), the switching process and features of different types of M-C domain variants are visually revealed. C1 [Wang, Ruixue; Yang, Bin; Sun, Enwei; Sun, Yuan; Zheng, Limei; Cao, Wenwu] Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Harbin 150080, Peoples R China. [Luo, Zhenlin; Xu, Han; Zhao, Jiangtao; Gao, Chen] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China. [Luo, Zhenlin; Xu, Han; Zhao, Jiangtao; Gao, Chen] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. [Zhou, Hua] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Cao, Wenwu] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Cao, Wenwu] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. RP Yang, B (reprint author), Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Harbin 150080, Peoples R China. EM binyang@hit.edu.cn; zlluo@ustc.edu.cn RI Cao, Wenwu/F-6091-2012 OI Cao, Wenwu/0000-0002-2447-1486 FU National key Basic Research Program of China [2013CB632900]; National Natural Science Foundation of China [11374010, 11434009]; Department of Energy, Basic Energy Sciences [DE-AC02-06CH11357] FX This research was supported by the National key Basic Research Program of China (No. 2013CB632900). Z. Luo acknowledges the National Natural Science Foundation of China (11374010, 11434009). The synchrotron diffraction measurements were performed on 12-ID-D beamline of Advanced Photon Source at Argonne National Laboratory, which is supported by the Department of Energy, Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 56 TC 0 Z9 0 U1 38 U2 46 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 29 PY 2016 VL 94 IS 5 AR 054115 DI 10.1103/PhysRevB.94.054115 PG 7 WC Physics, Condensed Matter SC Physics GA DU2FO UT WOS:000382026700001 ER PT J AU Loelius, C Iwasaki, H Brown, BA Honma, M Bader, VM Baugher, T Bazin, D Berryman, JS Braunroth, T Campbell, CM Dewald, A Gade, A Kobayashi, N Langer, C Lee, IY Lemasson, A Lunderberg, E Morse, C Recchia, F Smalley, D Stroberg, SR Wadsworth, R Walz, C Weisshaar, D Westerberg, A Whitmore, K Wimmer, K AF Loelius, C. Iwasaki, H. Brown, B. A. Honma, M. Bader, V. M. Baugher, T. Bazin, D. Berryman, J. S. Braunroth, T. Campbell, C. M. Dewald, A. Gade, A. Kobayashi, N. Langer, C. Lee, I. Y. Lemasson, A. Lunderberg, E. Morse, C. Recchia, F. Smalley, D. Stroberg, S. R. Wadsworth, R. Walz, C. Weisshaar, D. Westerberg, A. Whitmore, K. Wimmer, K. TI Lifetime measurement of the 4(1)(+) state of Ni-58 with the recoil distance method SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; NUCLEAR; TOOL AB The quadrupole transition rate for the 4(1)(+)-> 2(1)(+) transition of Ni-58 was determined from an application of the recoil distance method with the Gamma- Ray Energy Tracking In- beam Nuclear Array ( GRETINA). The present result of the B(E2; 4(1)(+)-> 2(1)(+) ) was found to be 50(-6)(+11) e(2) fm(4), which is about three times smaller than the literature value, indicating substantially less collectivity than previously believed. Shell model calculations performed with the GXPF1A effective interaction agree with the present data and the validity of the standard effective charges in understanding collectivity in the nickel isotopes is discussed. C1 [Loelius, C.; Iwasaki, H.; Brown, B. A.; Bader, V. M.; Baugher, T.; Bazin, D.; Berryman, J. S.; Gade, A.; Kobayashi, N.; Langer, C.; Lemasson, A.; Lunderberg, E.; Morse, C.; Recchia, F.; Smalley, D.; Stroberg, S. R.; Walz, C.; Weisshaar, D.; Whitmore, K.; Wimmer, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Loelius, C.; Iwasaki, H.; Brown, B. A.; Bader, V. M.; Baugher, T.; Gade, A.; Lunderberg, E.; Morse, C.; Stroberg, S. R.; Whitmore, K.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Honma, M.] Univ Aizu, Ctr Math Sci, Fukushima 9658580, Japan. [Braunroth, T.; Dewald, A.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Campbell, C. M.; Lee, I. Y.] Lawrence Berkeley Natl Lab, Nucl Sci Div, Berkeley, CA 94720 USA. [Langer, C.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Wadsworth, R.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Walz, C.] Tech Univ Darmstadt, Inst Kernphys, D-64289 Darmstadt, Germany. [Westerberg, A.; Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. RP Loelius, C (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA.; Loelius, C (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. RI Gade, Alexandra/A-6850-2008 OI Gade, Alexandra/0000-0001-8825-0976 FU National Science Foundation (NSF) [Phy-1102511, Phy-1404442]; Department of Energy (DOE) National Nuclear Security Administration (NNSA) [DE-NA0000979]; UK STFC [ST/F000124, ST/L005727]; Bundesministerium fur Bildung und Forschung (BMBF, Germany) [05P15PKFNA]; U.S. DOE Office of Science; NSF [Phy-1102511]; DOE [DE-AC02-05CH11231] FX The authors thank C. Bancroft, D. Barofsky, and J. Lloyd from Central Michigan University for help during the experiment. This work is supported by the National Science Foundation (NSF) under Phy-1102511 and Phy-1404442, by the Department of Energy (DOE) National Nuclear Security Administration (NNSA) under Award No. DE-NA0000979, by the UK STFC under ST/F000124 and ST/L005727, by the Bundesministerium fur Bildung und Forschung (BMBF, Germany) under Contract No. 05P15PKFNA. GRETINA was funded by the U.S. DOE Office of Science. Operation of the array at the NSCL is supported by the NSF under Cooperative Agreement PHY-1102511(NSCL) and DOE under Grant No. DE-AC02-05CH11231. NR 31 TC 0 Z9 0 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 29 PY 2016 VL 94 IS 2 AR 024340 DI 10.1103/PhysRevC.94.024340 PG 7 WC Physics, Nuclear SC Physics GA DU2IF UT WOS:000382033800001 ER PT J AU Gao, TR Fang, L Fackler, S Maruyama, S Zhang, XH Wang, LL Rana, T Manchanda, P Kashyap, A Janicka, K Wysocki, AL N'Diaye, AT Arenholz, E Borchers, JA Kirby, BJ Maranville, BB Sun, KW Kramer, MJ Antropov, VP Johnson, DD Skomski, R Cui, J Takeuchi, I AF Gao, T. R. Fang, L. Fackler, S. Maruyama, S. Zhang, X. H. Wang, L. L. Rana, T. Manchanda, P. Kashyap, A. Janicka, K. Wysocki, A. L. N'Diaye, A. T. Arenholz, E. Borchers, J. A. Kirby, B. J. Maranville, B. B. Sun, K. W. Kramer, M. J. Antropov, V. P. Johnson, D. D. Skomski, R. Cui, J. Takeuchi, I. TI Large energy product enhancement in perpendicularly coupled MnBi/CoFe magnetic bilayers SO PHYSICAL REVIEW B LA English DT Article ID NANOCOMPOSITE PERMANENT-MAGNETS; INITIO MOLECULAR-DYNAMICS; EXCHANGE; SIMULATION; MEDIA AB We demonstrate substantial enhancement in the energy product of MnBi-based magnets by forming robust ferromagnetic exchange coupling between a MnBi layer and a thin CoFe layer in a unique perpendicular coupling configuration, which provides increased resistance to magnetization reversal. The measured nominal energy product of 172 kJ/m(3) at room temperature is the largest value experimentally attained for permanent magnets free of expensive raw materials. Our finding shows that exchange-coupled MnBi/CoFe magnets are a viable option for pursuing rare-earth-free magnets with energy products approaching those containing rare-earth elements. C1 [Gao, T. R.; Fang, L.; Fackler, S.; Maruyama, S.; Zhang, X. H.; Takeuchi, I.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Wang, L. L.; Janicka, K.; Wysocki, A. L.; Sun, K. W.; Kramer, M. J.; Antropov, V. P.; Johnson, D. D.] US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. [Rana, T.; Manchanda, P.; Skomski, R.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Rana, T.; Manchanda, P.; Skomski, R.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Rana, T.; Kashyap, A.] LNM Inst Informat Technol, Dept Phys, Jaipur, Rajasthan, India. [Kashyap, A.] Indian Inst Technol, Sch Basic Sci, Mandi, Himachal Prades, India. [N'Diaye, A. T.; Arenholz, E.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Borchers, J. A.; Kirby, B. J.; Maranville, B. B.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Johnson, D. D.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Cui, J.] Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Takeuchi, I (reprint author), Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. EM takeuchi@umd.edu FU Department of Energy ARPA-E REACT [0472-1549]; U.S. DOE [DE-AC02-07CH11358] FX We acknowledge valuable discussions with P. Fischer, J. C. Zhao, D. Arnold, and S. Lofland. Funding for this project was from the Department of Energy ARPA-E REACT (Grant No. 0472-1549). Additional support (computational methods development) at Ames Laboratory was from the Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 34 TC 0 Z9 0 U1 26 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 29 PY 2016 VL 94 IS 6 AR 060411 DI 10.1103/PhysRevB.94.060411 PG 5 WC Physics, Condensed Matter SC Physics GA DU2FX UT WOS:000382027700001 ER PT J AU Lin, SZ Maiti, S Chubukov, A AF Lin, Shi-Zeng Maiti, Saurabh Chubukov, Andrey TI Distinguishing between s plus id and s plus is pairing symmetries in multiband superconductors through spontaneous magnetization pattern induced by a defect SO PHYSICAL REVIEW B LA English DT Article ID BA0.6K0.4FE2AS2; KFE2AS2 AB The symmetry of the pairing state in iron pnictide superconductor Ba-1 xKxFe2As2 is still controversial. At optimal doping (x approximate to 0.4), it is very likely s wave, but for x = 1 there are experimental and theoretical arguments for both s wave and d wave. Depending on the choice for x = 1, intermediate s + is and s + id states have been proposed for intermediate doping 0.4 < x < 1. In both states, the time-reversal symmetry is broken and a spontaneous magnetization is allowed. In this work we study a spontaneous magnetization induced by a nonmagnetic defect in the s + is and s + id states by using a perturbation theory and numerical calculations for theGinzburg-Landau free energy functional. We showthat the angular dependence of the magnetization is distinct in these two states due to the difference in symmetry properties of the order parameters. Our results indicate a possible way to distinguish between the s + is and s + id pairing symmetries in multiband superconductors. C1 [Lin, Shi-Zeng] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. [Maiti, Saurabh] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Chubukov, Andrey] Univ Minnesota, Dept Phys, Minneapolis, MN 55455 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU U.S. DOE through the LDRD program [DE-AC52-06NA25396]; Office of Basic Energy Sciences, U.S. Department of Energy [DE-SC0014402]; Center for Nonlinear Studies, LANL FX The authors are indebted to James Sauls and Filip Ronning for helpful discussions. The work by S.Z.L. was carried out under the auspices of the U.S. DOE Contract No. DE-AC52-06NA25396 through the LDRD program. The work by A.V.C. was supported by the Office of Basic Energy Sciences, U.S. Department of Energy, under award DE-SC0014402. A.V.C. acknowledges with thanks the support of the Center for Nonlinear Studies, LANL as an Ulam Scholar. NR 46 TC 1 Z9 1 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 29 PY 2016 VL 94 IS 6 AR 064519 DI 10.1103/PhysRevB.94.064519 PG 8 WC Physics, Condensed Matter SC Physics GA DU2FX UT WOS:000382027700007 ER PT J AU Singh, R Suzuki, T Autry, TM Moody, G Siemens, ME Cundiff, ST AF Singh, Rohan Suzuki, Takeshi Autry, Travis M. Moody, Galan Siemens, Mark E. Cundiff, Steven T. TI Polarization-dependent exciton linewidth in semiconductor quantum wells: A consequence of bosonic nature of excitons SO PHYSICAL REVIEW B LA English DT Article ID FOURIER-TRANSFORM SPECTROSCOPY; BLOCH EQUATIONS; RESONANCE; DISORDER; SYSTEM; BEATS AB The exciton coherent signal decay rate in GaAs quantum wells, as measured in four-wave mixing experiments, depends on the polarization of the excitation pulses. Using polarization-dependent two-dimensional coherent spectroscopy, we show that this behavior is due to the bosonic character of excitons. Interference between two different quantum mechanical pathways results in a smaller decay rate for cocircular and colinear polarization of the optical excitation pulses. This interference does not exist for cross-linearly polarized excitation pulses resulting in a larger decay rate. Our result shows that the bosonic nature of excitons must be considered when interpreting ultrafast spectroscopic studies of exciton dephasing in semiconductors. This behavior should be considered while interpreting results of ultrafast spectroscopy experiments involving bosonlike excitations. C1 [Singh, Rohan; Suzuki, Takeshi; Autry, Travis M.; Moody, Galan; Cundiff, Steven T.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Singh, Rohan; Suzuki, Takeshi; Autry, Travis M.; Moody, Galan; Cundiff, Steven T.] NIST, Boulder, CO 80309 USA. [Singh, Rohan; Autry, Travis M.; Moody, Galan; Cundiff, Steven T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Singh, Rohan; Suzuki, Takeshi; Cundiff, Steven T.] Univ Michigan, Dept Phys, Ann Arbor, MI 48105 USA. [Siemens, Mark E.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Singh, Rohan] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Moody, Galan] NIST, Boulder, CO 80305 USA. RP Cundiff, ST (reprint author), Univ Colorado, JILA, Boulder, CO 80309 USA.; Cundiff, ST (reprint author), NIST, Boulder, CO 80309 USA.; Cundiff, ST (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA.; Cundiff, ST (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48105 USA. EM cundiff@umich.edu FU Chemical Sciences, Geosciences, and Energy Biosciences Division, Office of Basic Energy Science, Office of Science, US Department of Energy [DE5 FG02-02ER15346]; NSF [1125844]; Japan Society for the Promotion of Science (JSPS) FX The authors thank Gael Nardin and Hebin Li for fruitful discussions. This work was primarily supported by the Chemical Sciences, Geosciences, and Energy Biosciences Division, Office of Basic Energy Science, Office of Science, US Department of Energy under Award No. DE5 FG02-02ER15346 and by the NSF under Grant No. 1125844. T.S. acknowledges support by Japan Society for the Promotion of Science (JSPS). NR 36 TC 0 Z9 0 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 29 PY 2016 VL 94 IS 8 AR 081304 DI 10.1103/PhysRevB.94.081304 PG 5 WC Physics, Condensed Matter SC Physics GA DU2HU UT WOS:000382032700002 ER PT J AU Teknowijoyo, S Cho, K Tanatar, MA Gonzales, J Bohmer, AE Cavani, O Mishra, V Hirschfeld, PJ Bud'ko, SL Canfield, PC Prozorov, R AF Teknowijoyo, S. Cho, K. Tanatar, M. A. Gonzales, J. Bohmer, A. E. Cavani, O. Mishra, V. Hirschfeld, P. J. Bud'ko, S. L. Canfield, P. C. Prozorov, R. TI Enhancement of superconducting transition temperature by pointlike disorder and anisotropic energy gap in FeSe single crystals SO PHYSICAL REVIEW B LA English DT Article ID PENETRATION DEPTH; IRON PNICTIDES; NEMATICITY; SYMMETRY; FIELD; CHALCOGENIDES; INSTABILITY; STATE; PHASE AB A highly anisotropic superconducting gap is found in single crystals of FeSe by studying the London penetration depth Delta lambda measured down to 50 mK in samples before and after 2.5 MeV electron irradiation. The gap minimum increases with introduced pointlike disorder, indicating the absence of symmetry-imposed nodes. Surprisingly, the superconducting transition temperature T-c increases by 0.4 K from T-c0 approximate to 8.8 K while the structural transition temperature T-s decreases by 0.9 K from T-s0 approximate to 91.2 K after electron irradiation. We discuss several explanations for the T-c enhancement and propose that local strengthening of the pair interaction by irradiation-induced Frenkel defects most likely explains the phenomenon. C1 [Teknowijoyo, S.; Cho, K.; Tanatar, M. A.; Gonzales, J.; Bohmer, A. E.; Bud'ko, S. L.; Canfield, P. C.; Prozorov, R.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Cavani, O.] Univ Paris Saclay, Lab Solides Irradis, Ecole Polytech, CNRS,CEA, F-91128 Palaiseau, France. [Mishra, V.] Univ Tennessee, Joint Inst Computat Sci, Knoxville, TN 37996 USA. [Hirschfeld, P. J.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RP Prozorov, R (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM prozorov@ameslab.gov FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358]; EMIR network [11-11-0121]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Helmholtz Association [PD-226]; [NSF-DMR-1407502] FX We thank A. Chubukov, B. Andersen, A. Golubov, R. Fernandes, M. Iavarone, S. Maiti, Y. Matsuda, I. Mazin, T. Shibauchi, and L. Taillefer for useful discussions. We are particularly grateful to S. S. Rossler for drawing our attention to the effects of twins on the resistivity and to M. Konczykowski as well as the whole SIRIUS team, B. Boizot, V. Metayer, and J. Losco, for running electron irradiation at Ecole Polytechnique. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under contract DE-AC02-07CH11358. Electron irradiation was supported by EMIR network, proposal 11-11-0121. V. M. acknowledges the support from the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. P.J.H. was partially supported by NSF-DMR-1407502. A.E.B. acknowledges support from the Helmholtz Association via PD-226. NR 74 TC 2 Z9 2 U1 14 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 29 PY 2016 VL 94 IS 6 AR 064521 DI 10.1103/PhysRevB.94.064521 PG 8 WC Physics, Condensed Matter SC Physics GA DU2FX UT WOS:000382027700009 ER PT J AU Yang, C Su, ZP Xiao, FL Zheng, HN Wang, YM Wang, S Spence, HE Reeves, GD Baker, DN Blake, JB Funsten, HO AF Yang, Chang Su, Zhenpeng Xiao, Fuliang Zheng, Huinan Wang, Yuming Wang, Shui Spence, H. E. Reeves, G. D. Baker, D. N. Blake, J. B. Funsten, H. O. TI Rapid flattening of butterfly pitch angle distributions of radiation belt electrons by whistler-mode chorus SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Radiation belt; wave; particle interactions; butterfly pitch-angle distribution; chorus waves; quasi-linear simulation; Van Allen Probes ID VAN ALLEN PROBES; ENERGY DIFFUSION-COEFFICIENTS; RELATIVISTIC ELECTRONS; INNER MAGNETOSPHERE; GEOMAGNETIC STORMS; MAGNETIC-FIELD; MAGNETOSONIC WAVES; ION-CYCLOTRON; ACCELERATION; SCATTERING AB Van Allen radiation belt electrons exhibit complex dynamics during geomagnetically active periods. Investigation of electron pitch angle distributions (PADs) can provide important information on the dominant physical mechanisms controlling radiation belt behaviors. Here we report a storm time radiation belt event where energetic electron PADs changed from butterfly distributions to normal or flattop distributions within several hours. Van Allen Probes observations showed that the flattening of butterfly PADs was closely related to the occurrence of whistler-mode chorus waves. Two-dimensional quasi-linear STEERB simulations demonstrate that the observed chorus can resonantly accelerate the near-equatorially trapped electrons and rapidly flatten the corresponding electron butterfly PADs. These results provide a new insight on how chorus waves affect the dynamic evolution of radiation belt electrons. C1 [Yang, Chang; Su, Zhenpeng; Zheng, Huinan; Wang, Yuming; Wang, Shui] Univ Sci & Technol China, Dept Geophys & Planetary Sci, Hefei, Peoples R China. [Yang, Chang; Su, Zhenpeng; Zheng, Huinan; Wang, Yuming; Wang, Shui] Univ Sci & Technol China, Collaborat Innovat Ctr Astronaut Sci & Technol, Hefei, Peoples R China. [Yang, Chang; Xiao, Fuliang] Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha, Hunan, Peoples R China. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Reeves, G. D.] New Mexico Consortium, Div Space Sci, Los Alamos, NM USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Blake, J. B.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. [Funsten, H. O.] Los Alamos Natl Lab, ISR Div, Los Alamos, NM USA. RP Su, ZP (reprint author), Univ Sci & Technol China, Dept Geophys & Planetary Sci, Hefei, Peoples R China.; Su, ZP (reprint author), Univ Sci & Technol China, Collaborat Innovat Ctr Astronaut Sci & Technol, Hefei, Peoples R China. EM szpe@mail.ustc.edu.cn RI Wang, Yuming/A-8968-2012; Xiao, Fuliang/B-9245-2011; OI Wang, Yuming/0000-0002-8887-3919; Xiao, Fuliang/0000-0003-1487-6620; Su, Zhenpeng/0000-0001-5577-4538; Reeves, Geoffrey/0000-0002-7985-8098 FU National Natural Science Foundation of China [41422405, 41274169, 41274174, 41174125, 41131065, 41421063, 41231066, 41304134]; Chinese Academy of Sciences [KZCX2-EW-QN510, KZZD-EW-01-4]; National Key Basic Research Special Foundation of China [2011CB811403]; Fundamental Research Funds for the Central Universities [WK2080000077] FX This work was supported by the National Natural Science Foundation of China grants 41422405, 41274169, 41274174, 41174125, 41131065, 41421063, 41231066, and 41304134, the Chinese Academy of Sciences grant KZCX2-EW-QN510 and KZZD-EW-01-4, the National Key Basic Research Special Foundation of China grant 2011CB811403, and the Fundamental Research Funds for the Central Universities WK2080000077. Data are available at the following websites: http://cdaweb.gsfc.nasa.gov/cdaweb/istp_public/ (geomagnetic activity indices), http://emfisis.physics.uiowa.edu/Flight/ (EMFISIS), http://www.rbsp-ect.lanl.gov/data_pub/ (ECT), and http://www.space.umn.edu/rbspefw-data/ (EFW). NR 81 TC 2 Z9 2 U1 14 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2016 VL 43 IS 16 BP 8339 EP 8347 DI 10.1002/2016GL070194 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DX5TC UT WOS:000384443800002 ER PT J AU Zhang, JS Bass, JD AF Zhang, Jin S. Bass, Jay D. TI Single-crystal elasticity of natural Fe-bearing orthoenstatite across a high-pressure phase transition SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE orthoenstatite; OEN-HPCEN2 transition; X discontinuity; high pressure; single-crystal elasticity ID X-RAY-DIFFRACTION; UPPER-MANTLE; SOUND VELOCITIES; ORTHO-PYROXENE; CLINOENSTATITE TRANSITION; GEOPHYSICAL IMPLICATIONS; MGSIO3 ORTHOENSTATITE; BRILLOUIN-SCATTERING; ROOM-TEMPERATURE; SUBDUCTING SLABS AB Sound velocities and elastic moduli have been measured on Fe-bearing orthoenstatite (OEN) single crystals up to 12GPa by Brillouin spectroscopy. The ambient adiabatic bulk modulus (K-s0) and shear modulus (G(0)) are determined to be 113(1)GPa and 75.9(7)GPa, respectively. A fourth-order finite strain fit to the data yields pressure derivatives of K-s0=8.8(1), K-s0=-0.68(6), G(0)=2.9(1), and G(0)=-0.40(2). These values are significantly higher than those for other major mantle minerals up to 10.5GPa but lower than some previous measurements on OEN. A pronounced increase of shear anisotropy was observed at a pressure of 12.06(9)GPa, coinciding with a phase transition from orthoenstatite to a recently discovered high-pressure phase with space group P2(1)/c. A high-pressure phase transition in OEN is unlikely to be the cause of the X discontinuity in the 250-325km depth range. Rather, a change in seismic anisotropy would be expected to accompany the orthoenstatite-to-P2(1)/c phase transition in the upper mantle at greater depths. C1 [Zhang, Jin S.; Bass, Jay D.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA. [Zhang, Jin S.] Univ Hawaii Manoa, Univ Hawaii, Corp Res, Honolulu, HI 96822 USA. [Zhang, Jin S.] Argonne Natl Lab, Adv Photon Source, GeoSoilEnviroCARS, COMPRES Technol Ctr, Argonne, IL 60439 USA. [Zhang, Jin S.] Univ New Mexico, Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. RP Zhang, JS (reprint author), Univ Illinois, Dept Geol, Urbana, IL 61801 USA.; Zhang, JS (reprint author), Univ Hawaii Manoa, Univ Hawaii, Corp Res, Honolulu, HI 96822 USA.; Zhang, JS (reprint author), Argonne Natl Lab, Adv Photon Source, GeoSoilEnviroCARS, COMPRES Technol Ctr, Argonne, IL 60439 USA.; Zhang, JS (reprint author), Univ New Mexico, Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. EM jinzhang@unm.edu FU National Science Foundation [EAR 16-20616, 07-38871]; COMPRES, the Consortium for Materials Properties Research in Earth Sciences, under NSF [EAR 11-57758]; National Science Foundation-Earth Sciences [EAR-0622171]; Department of Energy-Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation under grants EAR 16-20616 and 07-38871. This work was also partially supported by COMPRES, the Consortium for Materials Properties Research in Earth Sciences, under NSF Cooperative Agreement EAR 11-57758. Portions of this work were performed at GESCARS (Sector 13), APS, Argonne National Laboratory. GESCARS is supported by the National Science Foundation-Earth Sciences (EAR-0622171) and Department of Energy-Geosciences (DE-FG02-94ER14466). Use of APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. We thank Sergey Tkachev for gas loading, Ian M. Steele for EMPA analysis, and Bruno Reynard for helpful discussions. The Cij values obtained at each pressure in this study can be found in supporting information Tables S1 and S2. NR 57 TC 0 Z9 0 U1 8 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2016 VL 43 IS 16 BP 8473 EP 8481 DI 10.1002/2016GL069963 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DX5TC UT WOS:000384443800018 ER PT J AU Kahn, BH Huang, XL Stephens, GL Collins, WD Feldman, DR Su, H Wong, S Yue, Q AF Kahn, Brian H. Huang, Xianglei Stephens, Graeme L. Collins, William D. Feldman, Daniel R. Su, Hui Wong, Sun Yue, Qing TI ENSO regulation of far- and mid-infrared contributions to clear-sky OLR SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE far infrared; clear sky; tropics; ENSO; upper troposphere; water vapor ID SEA-SURFACE TEMPERATURE; TROPICAL DEEP CONVECTION; WATER-VAPOR; EL-NINO; CHANGING CLIMATE; CLOUDS; TROPOSPHERE; DEPENDENCE; SIGNATURE; RADIATION AB NASA Aqua-derived thermodynamic profiles, calculated spectral clear-sky outgoing longwave radiation (OLR), and vertical velocity fields from meteorological reanalyses are combined to determine the relative proportion of the far-infrared (FIR) and mid-infrared (MIR) spectral contributions to the total clear-sky OLR during different phases of El Nino-Southern Oscillation (ENSO). In the ascending branch of the tropical circulation, the spatial variance of upper tropospheric water vapor is shown to be larger during La Nina than El Nino and is consistent with zonal symmetry changes in the tropical waveguide and associated tropical-extratropical mixing. In the descending branch, upper tropospheric water vapor shows weaker coupling to lower layers that is evidenced by changes in the ratio of FIR to MIR in the clear-sky OLR. Diagnostics from the Geophysical Fluid Dynamics Laboratory AM3 model simulation are generally similar to satellite data, but the ratio of FIR to MIR is 5-10% larger with respect to dynamic regime. C1 [Kahn, Brian H.; Stephens, Graeme L.; Su, Hui; Wong, Sun; Yue, Qing] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. [Huang, Xianglei] Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. [Collins, William D.; Feldman, Daniel R.] Lawrence Berkeley Natl Lab, Climate & Ecosyst Div, Berkeley, CA USA. [Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Kahn, BH (reprint author), CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. EM brian.h.kahn@jpl.nasa.gov RI Collins, William/J-3147-2014; Yue, Qing/F-4619-2017 OI Collins, William/0000-0002-4463-9848; Yue, Qing/0000-0002-3559-6508 FU JPL; University of Michigan; NASA [NNX14AJ50G]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Terrestrial Ecosystem Science and Atmospheric System Research programs [DE-ACO2-05CH11231] FX A portion of this research was carried out at the Jet Propulsion Laboratory (JPL), California Institute of Technology, under a contract with the National Aeronautics and Space Administration. We thank two anonymous reviewers for very constructive feedback and insights that led to an improved manuscript. B. Kahn was supported by Strategic University Research Partnership (SURP) proposal between JPL and the University of Michigan. X. Huang was supported by NASA under grant NNX14AJ50G awarded to the University of Michigan. D. Feldman and W. Collins acknowledge support by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Terrestrial Ecosystem Science and Atmospheric System Research programs, under award DE-ACO2-05CH11231. The AIRS version 6 data sets were processed by and obtained from the Goddard Earth Services Data and Information Services Center (http://daac.gsfc.nasa.gov/). The MERRA data sets were processed by and obtained from the NASA Goddard's Global Modeling and Assimilation Office (GMAO). Copyright 2016. All rights reserved. Government sponsorship acknowledged. NR 43 TC 0 Z9 0 U1 6 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 28 PY 2016 VL 43 IS 16 BP 8751 EP 8759 DI 10.1002/2016GL070263 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DX5TC UT WOS:000384443800050 ER PT J AU Cui, ZZ Xu, H Yun, Y Guo, JH Chuang, YD Huang, HL Meng, DC Wang, JL Fu, ZP Peng, RR Knize, RJ Brown, GJ Zhai, XF Lu, YL AF Cui, Zhangzhang Xu, Hui Yun, Yu Guo, Jinghua Chuang, Yi-De Huang, Haoliang Meng, Dechao Wang, Jianlin Fu, Zhengping Peng, Ranran Knize, Randy J. Brown, Gail J. Zhai, Xiaofang Lu, Yalin TI Soft X-ray absorption spectroscopy investigations of Bi6FeCoTi3O18 and LaBi5FeCoTi3O18 epitaxial thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TEMPERATURE MULTIFERROIC PROPERTIES; ELECTRICAL-PROPERTIES; ELECTRONIC-STRUCTURE; WEAK FERROMAGNETISM; CERAMICS; CO AB High-quality single-crystalline Bi6FeCoTi3O18 and LaBi5FeCoTi3O18 thin films were prepared by pulsed laser deposition. X-ray diffraction characterizations indicate a more disordered lattice structure of the LaBi5FeCoTi3O18 film. The magnetic measurement results demonstrated significantly enhanced ferromagnetism in the LaBi5FeCoTi3O18 film. The modulation of oxidation and hybridization states caused by substituting Bi with La was studied using the soft X-ray absorption spectroscopy. The spectroscopic results revealed the reduced concentration of oxygen vacancies and the more distorted lattice structure in the LaBi5FeCoTi3O18 film, which explained the enhanced ferromagnetism. Published by AIP Publishing. C1 [Cui, Zhangzhang; Xu, Hui; Yun, Yu; Huang, Haoliang; Meng, Dechao; Wang, Jianlin; Fu, Zhengping; Peng, Ranran; Zhai, Xiaofang; Lu, Yalin] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Cui, Zhangzhang; Xu, Hui; Yun, Yu; Huang, Haoliang; Meng, Dechao; Wang, Jianlin; Fu, Zhengping; Peng, Ranran; Zhai, Xiaofang; Lu, Yalin] Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China. [Cui, Zhangzhang; Huang, Haoliang; Fu, Zhengping; Peng, Ranran; Zhai, Xiaofang; Lu, Yalin] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. [Guo, Jinghua; Chuang, Yi-De] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Wang, Jianlin; Lu, Yalin] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China. [Knize, Randy J.; Lu, Yalin] US Air Force Acad, Dept Phys, Laser Opt Res Ctr, Colorado Springs, CO 80840 USA. [Brown, Gail J.] US Air Force, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. RP Zhai, XF; Lu, YL (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.; Zhai, XF; Lu, YL (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China.; Zhai, XF; Lu, YL (reprint author), Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China.; Lu, YL (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China.; Lu, YL (reprint author), US Air Force Acad, Dept Phys, Laser Opt Res Ctr, Colorado Springs, CO 80840 USA. EM xfzhai@ustc.edu.cn; yllu@ustc.edu.cn FU National Basic Research Program of China [2012CB922000]; Natural Science Foundation of China [11574287]; External Cooperation Program of BIC [211134KYSB20130017]; Fundamental Research Funds for the Central Universities FX This work was supported by the National Basic Research Program of China (2012CB922000), the Natural Science Foundation of China (Grant No. 11574287), the External Cooperation Program of BIC (Grant No. 211134KYSB20130017), and the Fundamental Research Funds for the Central Universities. NR 32 TC 1 Z9 1 U1 16 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 084101 DI 10.1063/1.4961392 PG 5 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400018 ER PT J AU Fensin, SJ Jones, DR Walker, EK Farrow, A Imhoff, SD Clarke, K Trujillo, CP Martinez, DT Gray, GT Cerreta, EK AF Fensin, S. J. Jones, D. R. Walker, E. K. Farrow, A. Imhoff, S. D. Clarke, K. Trujillo, C. P. Martinez, D. T. Gray, G. T., III Cerreta, E. K. TI The effect of distribution of second phase on dynamic damage SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FRACTURE; SPALL; FAILURE; COPPER; ALUMINUM; BEHAVIOR; SOLIDS; METALS; STEEL AB For ductile metals, dynamic fracture occurs principally through void nucleation, growth, and coalescence at heterogeneities in the microstructure. Previous experimental research on high purity metals has shown that microstructural features, such as grain boundaries, inclusions, vacancies, and heterogeneities, can act as initial void nucleation sites. In addition, other research on two-phase materials has also highlighted the importance of the properties of a second phase itself in determining the dynamic response of the overall material. However, previous research has not investigated the effects of the distribution of a second phase on damage nucleation and evolution. To approach this problem in a systematic manner, two copper alloys with 1% lead materials, with the same Pb concentration but different Pb distributions, have been investigated. A new CuPb alloy was cast with a more homogeneous distribution of Pb as compared to a CuPb where the Pb congregated in large "stringer" type configurations. These materials were shock loaded at similar to 1.2 GPa and soft recovered. In-situ free surface velocity information, and post mortem metallography, reveals that even though the spall strength of both the materials were similar, the total extent and details of damage in the materials varied by 15%. This suggests that altering the distribution of Pb in the Cu matrix leads to the creation of more void nucleation sites and also changed the rate of void growth. Published by AIP Publishing. C1 [Fensin, S. J.; Jones, D. R.; Martinez, D. T.; Gray, G. T., III; Cerreta, E. K.] Los Alamos Natl Lab, MST 8, Los Alamos, NM 87544 USA. [Walker, E. K.; Farrow, A.] Los Alamos Natl Lab, MST 2, Los Alamos, NM 87544 USA. [Imhoff, S. D.; Clarke, K.] Los Alamos Natl Lab, MST 6, Los Alamos, NM 87544 USA. [Trujillo, C. P.] Los Alamos Natl Lab, MST 16, Los Alamos, NM 87544 USA. RP Fensin, SJ (reprint author), Los Alamos Natl Lab, MST 8, Los Alamos, NM 87544 USA. EM saryuj@lanl.gov FU U.S. Department of Energy [DE-AC52-06NA25396]; DOD/DOE Joint Munitions program FX Los Alamos National Laboratory is operated by LANS, LLC, for the NNSA and the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. Funding was provided by DOD/DOE Joint Munitions program. NR 24 TC 0 Z9 0 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 085901 DI 10.1063/1.4961041 PG 7 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400078 ER PT J AU Hihath, S Santala, MK Campbell, GH van Benthem, K AF Hihath, Sahar Santala, Melissa K. Campbell, Geoffrey H. van Benthem, Klaus TI High-speed nanoscale characterization of dewetting via dynamic transmission electron microscopy SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID THIN AU FILMS; CAPILLARY INSTABILITIES; IN-SITU; INTERFACE; DIFFUSION; NI AB The dewetting of thin films can occur in either the solid or the liquid state for which different mass transport mechanisms are expected to control morphological changes. Traditionally, dewetting dynamics have been examined on time scales between several seconds to hours, and length scales ranging between nanometers and millimeters. The determination of mass transport mechanisms on the nanoscale, however, requires nanoscale spatial resolution and much shorter time scales. This study reports the high-speed observation of dewetting phenomena for kinetically constrained Ni thin films on crystalline SrTiO3 substrates. Movie-mode Dynamic Transmission Electron Microscopy (DTEM) was used for high-speed image acquisition during thin film dewetting at different temperatures. DTEM imaging confirmed that the initial stages of film agglomeration include edge retraction, hole formation, and growth. Finite element modeling was used to simulate temperature distributions within the DTEM samples after laser irradiation with different energies. For pulsed laser irradiation at 18 mu J, experimentally observed hole growth suggests that Marangoni flow dominates hole formation in the liquid nickel film. After irradiation with 13.8 mu J, however, the observations suggest that dewetting was initiated by nucleation of voids followed by hole growth through solid-state surface diffusion. Published by AIP Publishing. C1 [Hihath, Sahar; van Benthem, Klaus] Univ Calif Davis, Dept Mat Sci & Engn, 1 Shields Ave, Davis, CA 95616 USA. [Hihath, Sahar] Univ Calif Davis, Dept Phys, 1 Shields Ave, Davis, CA 95616 USA. [Santala, Melissa K.; Campbell, Geoffrey H.] Lawrence Livermore Natl Lab, Div Mat Sci, 7000 East Ave, Livermore, CA 94550 USA. [Santala, Melissa K.] Oregon State Univ, Sch Mech Ind & Mfg Engn, 204 Rogers Hall, Corvallis, OR 97331 USA. RP van Benthem, K (reprint author), Univ Calif Davis, Dept Mat Sci & Engn, 1 Shields Ave, Davis, CA 95616 USA. EM benthem@ucdavis.edu FU University of California Laboratory Fee Grant [12-LR-238313]; U.S. National Science Foundation through a NSF Faculty Early Career Award [DMR-0955638]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC52-07NA27344] FX S.H. and K.v.B. were supported by a University of California Laboratory Fee Grant No. 12-LR-238313. K.v.B. also acknowledges the financial support from the U.S. National Science Foundation through a NSF Faculty Early Career Award No. DMR-0955638. DTEM experiments at Lawrence Livermore National Laboratory were carried out under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC52-07NA27344. NR 44 TC 0 Z9 0 U1 8 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 085301 DI 10.1063/1.4961212 PG 8 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400053 ER PT J AU Leon-Brito, N Bauer, ED Ronning, F Thompson, JD Movshovich, R AF Leon-Brito, N. Bauer, E. D. Ronning, F. Thompson, J. D. Movshovich, R. TI Magnetic microstructure and magnetic properties of uniaxial itinerant ferromagnet Fe3GeTe2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID WALL ENERGY; DOMAIN; ALLOYS; COBALT AB Magnetic force microscopy was used to observe the magnetic microstructure of Fe3GeTe2 at 4K on the (001) surface. The surface magnetic structure consists of a two-phase domain branching pattern that is characteristic for highly uniaxial magnets in the plane perpendicular to the magnetic easy axis. The average surface magnetic domain width D-s = 1.3 mu m determined from this pattern, in combination with intrinsic properties calculated from bulk magnetization data (the saturation magnetization M-s = 376 emu/cm(3) and the uniaxial magnetocrystalline anisotropy constant K-u = 1.46 x 10(7) erg/cm(3)), was used to determine the following micromagnetic parameters for Fe3GeTe2 from phenomenological models: the domain wall energy gamma(w) = 4.7 erg/cm(2), the domain wall thickness delta(w) = 2.5 nm, the exchange stiffness constant Lambda(ex) = 0.95 x 10(-7) erg/cm, the exchange length l(ex) = 2.3 nm, and the critical single domain particle diameter d(c) = 470 nm. Published by AIP Publishing. C1 [Leon-Brito, N.; Bauer, E. D.; Ronning, F.; Thompson, J. D.; Movshovich, R.] Los Alamos Natl Lab, Mat Phys & Applicat Condensed Matter & Magnet Sci, Los Alamos, NM 87545 USA. RP Movshovich, R (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Condensed Matter & Magnet Sci, Los Alamos, NM 87545 USA. EM roman@lanl.gov OI Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU U.S. DOE through the Los Alamos LDRD program [DEAC52-06NA25396] FX This work at LANL was performed under the auspices of the U.S. DOE Contract No. DEAC52-06NA25396 through the Los Alamos LDRD program. NR 30 TC 1 Z9 1 U1 19 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 083903 DI 10.1063/1.4961592 PG 5 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400012 ER PT J AU Teherani, JT Agarwal, S Chern, W Solomon, PM Yablonovitch, E Antoniadis, DA AF Teherani, James T. Agarwal, Sapan Chern, Winston Solomon, Paul M. Yablonovitch, Eli Antoniadis, Dimitri A. TI Auger generation as an intrinsic limit to tunneling field-effect transistor performance SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID QUANTUM-WELL HETEROSTRUCTURE; RECOMBINATION; SEMICONDUCTORS; HGCDTE; ENERGY; GAAS; INP AB Many in the microelectronics field view tunneling field-effect transistors (TFETs) as society's best hope for achieving a > 10 x power reduction for electronic devices; however, despite a decade of considerable worldwide research, experimental TFET results have significantly underperformed simulations and conventional MOSFETs. To explain the discrepancy between TFET experiments and simulations, we investigate the parasitic leakage current due to Auger generation, an intrinsic mechanism that cannot be mitigated with improved material quality or better device processing. We expose the intrinsic link between the Auger and band-to-band tunneling rates, highlighting the difficulty of increasing one without the other. From this link, we show that Auger generation imposes a fundamental limit on ultimate TFET performance. Published by AIP Publishing. C1 [Teherani, James T.] Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. [Agarwal, Sapan] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Chern, Winston; Antoniadis, Dimitri A.] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Solomon, Paul M.] IBM TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Yablonovitch, Eli] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Teherani, JT (reprint author), Columbia Univ, Dept Elect Engn, New York, NY 10027 USA. EM j.teherani@columbia.edu OI Teherani, James/0000-0002-7778-8073; Agarwal, Sapan/0000-0002-3676-6986 FU Center for Energy Efficient Electronics Science (NSF) [0939514] FX This work was supported in part by the Center for Energy Efficient Electronics Science (NSF Award No. 0939514). The authors thank Mathieu Luisier, Roger Lake, and Rebecca Murray for their technical comments regarding the manuscript. NR 33 TC 0 Z9 0 U1 3 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 084507 DI 10.1063/1.4960571 PG 15 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400036 ER PT J AU Turley, WD Stevens, GD Hixson, RS Cerreta, EK Daykin, EP Graeve, OA La Lone, BM Novitskaya, E Perez, C Rigg, PA Veeser, LR AF Turley, W. D. Stevens, G. D. Hixson, R. S. Cerreta, E. K. Daykin, E. P. Graeve, O. A. La Lone, B. M. Novitskaya, E. Perez, C. Rigg, P. A. Veeser, L. R. TI Explosive-induced shock damage in copper and recompression of the damaged region SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID 316L STAINLESS-STEEL; SPALLATION RESPONSE; DYNAMIC FRACTURE; TAYLOR-WAVE; STRAIN AB We have studied the dynamic spall process for copper samples in contact with detonating low-performance explosives. When a triangular shaped shock wave from detonation moves through a sample and reflects from the free surface, tension develops immediately, one or more damaged layers can form, and a spall scab can separate from the sample and move ahead of the remaining target material. For dynamic experiments, we used time-resolved velocimetry and x-ray radiography. Soft-recovered samples were analyzed using optical imaging and microscopy. Computer simulations were used to guide experiment design. We observe that for some target thicknesses the spall scab continues to run ahead of the rest of the sample, but for thinner samples, the detonation product gases accelerate the sample enough for it to impact the spall scab several microseconds or more after the initial damage formation. Our data also show signatures in the form of a late-time reshock in the time-resolved data, which support this computational prediction. A primary goal of this research was to study the wave interactions and damage processes for explosives-loaded copper and to look for evidence of this postulated recompression event. We found both experimentally and computationally that we could tailor the magnitude of the initial and recompression shocks by varying the explosive drive and the copper sample thickness; thin samples had a large recompression after spall, whereas thick samples did not recompress at all. Samples that did not recompress had spall scabs that completely separated from the sample, whereas samples with recompression remained intact. This suggests that the hypothesized recompression process closes voids in the damage layer or otherwise halts the spall formation process. This is a somewhat surprising and, in some ways controversial, result, and the one that warrants further research in the shock compression community. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license C1 [Turley, W. D.; Stevens, G. D.; La Lone, B. M.; Veeser, L. R.] Natl Secur Technol LLC, Special Technol Lab, Santa Barbara, CA 93111 USA. [Hixson, R. S.] Natl Secur Technol LLC, New Mexico Operat, Los Alamos, NM 87544 USA. [Hixson, R. S.; Cerreta, E. K.; Veeser, L. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Daykin, E. P.; Perez, C.] Natl Secur Technol LLC, North Las Vegas Operat, North Las Vegas, NV 89030 USA. [Graeve, O. A.; Novitskaya, E.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Rigg, P. A.] Washington State Univ, Pullman, WA 99164 USA. RP Turley, WD (reprint author), Natl Secur Technol LLC, Special Technol Lab, Santa Barbara, CA 93111 USA. EM turleywd@nv.doe.gov FU National Security Technologies, LLC [DE-AC52-06NA25946]; Site-Directed Research and Development Program FX This manuscript has been authored by National Security Technologies, LLC, under Contract No. DE-AC52-06NA25946 with the U.S. Department of Energy and supported by the Site-Directed Research and Development Program. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published forms of the manuscript, or allow others to do so, for United States Government purposes. The U.S. Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan): DOE/NV/25946-2814. We wish to acknowledge Mike Grover of Special Technologies Laboratory for his significant part in this research and J. D. Montalvo and J. C. Foley, both of Los Alamos National Laboratory, who provided the optical imagery. We are very grateful to G. T. Gray, D. Koller, and V. Livescu for many helpful discussions and for supplying us with high-purity, annealed OFHC copper for these experiments. NR 21 TC 0 Z9 0 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 28 PY 2016 VL 120 IS 8 AR 085904 DI 10.1063/1.4962013 PG 11 WC Physics, Applied SC Physics GA DW8NS UT WOS:000383913400081 ER PT J AU Goncharov, VV Hall, GE AF Goncharov, Vasily V. Hall, Gregory E. TI Supercontinuum Fourier transform spectrometry with balanced detection on a single photodiode SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DUAL-BEAM; SPECTROSCOPY; NOISE; FILMS AB We demonstrate a method of combining a supercontinuum light source with a commercial Fourier transform spectrometer, using a novel approach to dual-beam balanced detection, implemented with phase-sensitive detection on a single light detector. A 40 dB reduction in the relative intensity noise is achieved for broadband light, analogous to conventional balanced detection methods using two matched photodetectors. Unlike conventional balanced detection, however, this method exploits the time structure of the broadband source to interleave signal and reference pulse trains in the time domain, recording the broadband differential signal at the fundamental pulse repetition frequency of the supercontinuum. The method is capable of real-time correction for instability in the supercontinuum spectral structure over a broad range of wavelengths and is compatible with commercially designed spectrometers. A proof-of-principle experimental setup is demonstrated for weak absorption in the 1500-1600 nm region. Published by AIP Publishing. C1 [Goncharov, Vasily V.; Hall, Gregory E.] Brookhaven Natl Lab, Dept Energy & Photon Sci, Div Chem, Upton, NY 11973 USA. [Goncharov, Vasily V.] Janelia Farm Res Campus, Howard Hughes Med Inst, Ashburn, VA 20147 USA. RP Hall, GE (reprint author), Brookhaven Natl Lab, Dept Energy & Photon Sci, Div Chem, Upton, NY 11973 USA. EM gehall@bnl.gov OI Hall, Gregory/0000-0002-8534-9783 FU U.S. Department of Energy [DE-AC02-98CH10886, DE-SC0012704]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences; Goldhaber Distinguished Fellowship Program at BNL FX This work was performed at Brookhaven National Laboratory under Contract Nos. DE-AC02-98CH10886 and DE-SC0012704 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences. Additional support from the Goldhaber Distinguished Fellowship Program at BNL is gratefully acknowledged. We are grateful to I. Coddington for early assistance with the design and construction of mode-locked fiber lasers. C. P. McRaven and T. J. Sears are acknowledged for helpful discussions, and we thank M. G. White for shared access to the Bruker Vertex 80V used in this work. NR 26 TC 0 Z9 0 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 084201 DI 10.1063/1.4961655 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500021 PM 27586915 ER PT J AU Miller, WH Cotton, SJ AF Miller, William H. Cotton, Stephen J. TI Communication: Wigner functions in action-angle variables, Bohr-Sommerfeld quantization, the Heisenberg correspondence principle, and a symmetrical quasi-classical approach to the full electronic density matrix SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article AB It is pointed out that the classical phase space distribution in action-angle (a-a) variables obtained from a Wigner function depends on how the calculation is carried out: if one computes the standard Wigner function in Cartesian variables (p, x), and then replaces p and x by their expressions in terms of a-a variables, one obtains a different result than if the Wigner function is computed directly in terms of the a-a variables. Furthermore, the latter procedure gives a result more consistent with classical and semiclassical theory-e.g., by incorporating the Bohr-Sommerfeld quantization condition (quantum states defined by integer values of the action variable) as well as the Heisenberg correspondence principle for matrix elements of an operator between such states-and has also been shown to be more accurate when applied to electronically non-adiabatic applications as implemented within the recently developed symmetrical quasi-classical (SQC) Meyer-Miller (MM) approach. Moreover, use of the Wigner function (obtained directly) in a-a variables shows how our standard SQC/MM approach can be used to obtain off-diagonal elements of the electronic density matrix by processing in a different way the same set of trajectories already used (in the SQC/MM methodology) to obtain the diagonal elements. Published by AIP Publishing. C1 [Miller, William H.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Miller, WH (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM millerwh@berkeley.edu; StephenJCotton47@gmail.com FU National Science Foundation [CHE-1148645]; Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation under Grant No. CHE-1148645 and by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy under Contract No. DE-AC02-05CH11231.; In addition, this research utilized computation resources provided by the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 11 TC 4 Z9 4 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 081102 DI 10.1063/1.4961551 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500002 PM 27586896 ER PT J AU Neuscamman, E AF Neuscamman, Eric TI Communication: Variation after response in quantum Monte Carlo SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; EXCITED-STATES; WAVE-FUNCTIONS; BUTADIENE; MOLECULES; EXCHANGE; SPACE AB We present a new method for modeling electronically excited states that overcomes a key failing of linear response theory by allowing the underlying ground state ansatz to relax in the presence of an excitation. The method is variational, has a cost similar to ground state variational Monte Carlo, and admits both open and periodic boundary conditions. We present preliminary numerical results showing that, when paired with the Jastrow antisymmetric geminal power ansatz, the variation-after-response formalism delivers accuracies for valence and charge transfer single excitations on par with equation of motion coupled cluster, while surpassing coupled cluster's accuracy for excitations with significant doubly excited character. Published by AIP Publishing. C1 [Neuscamman, Eric] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neuscamman, Eric] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neuscamman, E (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Neuscamman, E (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM eneuscamman@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge funding from the Office of Science, Office of Basic Energy Sciences, the U.S. Department of Energy, Contract No. DE-AC02-05CH11231. Calculations were performed on the Berkeley Research Computing Savio cluster. NR 31 TC 0 Z9 0 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 081103 DI 10.1063/1.4961686 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500003 PM 27586897 ER PT J AU Schlesinger, D Wikfeldt, KT Skinner, LB Benmore, CJ Nilsson, A Pettersson, LGM AF Schlesinger, Daniel Wikfeldt, K. Thor Skinner, Lawrie B. Benmore, Chris J. Nilsson, Anders Pettersson, Lars G. M. TI The temperature dependence of intermediate range oxygen-oxygen correlations in liquid water SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS METHOD; PHASE-TRANSITION; AMBIENT WATER; ISOTHERMAL COMPRESSIBILITY; SUPERCOOLED WATER; 2-STATE PICTURE; GLASSY WATER; ANOMALIES; MODEL; SIMULATIONS AB We analyze the recent temperature dependent oxygen-oxygen pair-distribution functions from experimental high-precision x-ray diffraction data of bulk water by Skinner et al. [J. Chem. Phys. 141, 214507 (2014)] with particular focus on the intermediate range where small, but significant, correlations are found out to 17 angstrom. The second peak in the pair-distribution function at 4.5 angstrom is connected to tetrahedral coordination and was shown by Skinner et al. to change behavior with temperature below the temperature of minimum isothermal compressibility. Here we show that this is associated also with a peak growing at 11 angstrom which strongly indicates a collective character of fluctuations leading to the enhanced compressibility at lower temperatures. We note that the peak at similar to 13.2 angstrom exhibits a temperature dependence similar to that of the density with a maximum close to 277 K or 4 degrees C. We analyze simulations of the TIP4P/2005 water model in the same manner and find excellent agreement between simulations and experiment albeit with a temperature shift of similar to 20 K. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). C1 [Schlesinger, Daniel; Wikfeldt, K. Thor; Nilsson, Anders; Pettersson, Lars G. M.] Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden. [Wikfeldt, K. Thor] Univ Iceland, Sci Inst, VR 3, IS-107 Reykjavik, Iceland. [Skinner, Lawrie B.; Benmore, Chris J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Nilsson, Anders] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Skinner, Lawrie B.] Stanford Univ, Dept Radiat Oncol, Stanford, CA 94305 USA. RP Pettersson, LGM (reprint author), Stockholm Univ, AlbaNova Univ Ctr, Dept Phys, SE-10691 Stockholm, Sweden. EM Lars.Pettersson@fysik.su.se OI Pettersson, Lars G.M./0000-0003-1133-9934; Skinner, Lawrie/0000-0001-7317-1642; Benmore, Chris/0000-0001-7007-7749 FU European Research Council (ERC) [667205]; Swedish National Research Council (VR) [2013-8823]; DOE Office of Science [DE-AC02-06CH11357] FX We acknowledge financial support from the European Research Council (ERC) Advanced Grant under Project No. 667205 and the Swedish National Research Council (VR) under Grant No. 2013-8823. Part of this work has been performed at the Advanced Photon Source which is operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 62 TC 2 Z9 2 U1 9 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 084503 DI 10.1063/1.4961404 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500037 PM 27586931 ER PT J AU Tasios, N Edison, JR van Roij, R Evans, R Dijkstra, M AF Tasios, Nikos Edison, John R. van Roij, Rene Evans, Robert Dijkstra, Marjolein TI Critical Casimir interactions and colloidal self-assembly in near-critical solvents SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MONTE-CARLO-SIMULATION; BINARY-LIQUID MIXTURES; PHASE-EQUILIBRIA; CAPILLARY CONDENSATION; ADSORPTION PHENOMENA; SPHERICAL-PARTICLES; CRITICAL FILMS; FLUIDS; TRANSITIONS; BEHAVIOR AB A binary solvent mixture close to critical demixing experiences fluctuations whose correlation length, xi, diverges as the critical point is approached. The solvent-mediated (SM) interaction that arises between a pair of colloids immersed in such a near-critical solvent can be long-ranged and this so-called critical Casimir interaction is well-studied. How a (dense) suspension of colloids will self-assemble under these conditions is poorly understood. Using a two-dimensional lattice model for the solvent and hard disks to represent the colloids, we perform extensive Monte Carlo simulations to investigate the phase behaviour of this model colloidal suspension as a function of colloid size and wettability under conditions where the solvent reservoir is supercritical. Unlike most other approaches, where the solvent is modelled as an implicit background, our model employs an explicit solvent and treats the suspension as a ternary mixture. This enables us to capture important features, including the pronounced fractionation of the solvent in the coexisting colloidal phases, of this complex system. We also present results for the partial structure factors; these shed light on the critical behaviour in the ternary mixture. The degree to which an effective two-body pair potential description can describe the phase behaviour and structure of the colloidal suspension is discussed briefly. Published by AIP Publishing. C1 [Tasios, Nikos; Dijkstra, Marjolein] Univ Utrecht, Debye Inst Nanomat Sci, Soft Condensed Matter, Princetonpl 1, NL-3584 CC Utrecht, Netherlands. [Edison, John R.] Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [van Roij, Rene] Univ Utrecht, Inst Theoret Phys, Princetonpl 5, NL-3584 CC Utrecht, Netherlands. [Evans, Robert] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. RP Dijkstra, M (reprint author), Univ Utrecht, Debye Inst Nanomat Sci, Soft Condensed Matter, Princetonpl 1, NL-3584 CC Utrecht, Netherlands. EM m.dijkstra@uu.nl RI Dijkstra, Marjolein/B-6656-2009; OI Tasios, Nikos/0000-0002-6995-5767 FU NWO-ECHO; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO) VICI grant; NWO-EW; Leverhulme Trust [EM-2016-031]; Dutch Ministry of Education, Culture and Science (OCW) FX We thank N. Wilding, D. Ashton, and A. Maciolek for stimulating discussions. N.T. and M.D. acknowledge financial support from an NWO-ECHO grant. J.R.E. and M.D. acknowledge financial support from a Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO) VICI grant. N.T., J.R.E., M.D. acknowledge a NWO-EW grant for computing time on the Dutch supercomputer Cartesius. R. Evans is grateful for the hospitality of the members of the Debye Institute, Utrecht on his frequent visits and to the Leverhulme Trust for the award of an Emeritus Fellowship No. EM-2016-031. This work is part of the D-ITP consortium, a program of the Netherlands Organisation for Scientific Research (NWO) funded by the Dutch Ministry of Education, Culture and Science (OCW). NR 73 TC 1 Z9 1 U1 9 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 084902 DI 10.1063/1.4961437 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500047 PM 27586941 ER PT J AU Yu, HG AF Yu, Hua-Gen TI An exact variational method to calculate rovibrational spectra of polyatomic molecules with large amplitude motion SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DISCRETE VARIABLE REPRESENTATION; VIBRATIONAL-ENERGY LEVELS; DIMENSIONAL MODEL REPRESENTATIONS; QUANTUM DYNAMICS; POTENTIAL-ENERGY; AB-INITIO; ITERATIVE DIAGONALIZATION; VECTOR PARAMETRIZATION; TETRAATOMIC MOLECULES; MECHANICS AB We report a new full-dimensional variational algorithm to calculate rovibrational spectra of polyatomic molecules using an exact quantum mechanical Hamiltonian. The rovibrational Hamiltonian of system is derived in a set of orthogonal polyspherical coordinates in the body-fixed frame. It is expressed in an explicitly Hermitian form. The Hamiltonian has a universal formulation regardless of the choice of orthogonal polyspherical coordinates and the number of atoms in molecule, which is suitable for developing a general program to study the spectra of many polyatomic systems. An efficient coupled-state approach is also proposed to solve the eigenvalue problem of the Hamiltonian using a multi-layer Lanczos iterative diagonalization approach via a set of direct product basis set in three coordinate groups: radial coordinates, angular variables, and overall rotational angles. A simple set of symmetric top rotational functions is used for the overall rotation whereas a potential-optimized discrete variable representation method is employed in radial coordinates. A set of contracted vibrationally diabatic basis functions is adopted in internal angular variables. Those diabatic functions are first computed using a neural network iterative diagonalization method based on a reduced-dimension Hamiltonian but only once. The final rovibrational energies are computed using a modified Lanczos method for a given total angular momentum J, which is usually fast. Two numerical applications to CH4 and H2CO are given, together with a comparison with previous results. Published by AIP Publishing. C1 [Yu, Hua-Gen] Brookhaven Natl Lab, Dept Energy & Photon Sci, Div Chem, Upton, NY 11973 USA. RP Yu, HG (reprint author), Brookhaven Natl Lab, Dept Energy & Photon Sci, Div Chem, Upton, NY 11973 USA. EM hgy@bnl.gov RI Yu, Hua-Gen/N-7339-2015 FU U.S. Department of Energy, Office of Science [DE-SC0012704]; Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences; National Energy Research Scientific Computing Center (NERSC) [DE-AC02-05CH11231] FX This work was performed at Brookhaven National Laboratory under Contract No. DE-SC0012704 with the U.S. Department of Energy, Office of Science and supported by its Division of Chemical Sciences, Geosciences, and Biosciences within the Office of Basic Energy Sciences. It also used the resource at the National Energy Research Scientific Computing Center (NERSC) under Contract No. DE-AC02-05CH11231. NR 89 TC 1 Z9 1 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 28 PY 2016 VL 145 IS 8 AR 084109 DI 10.1063/1.4961642 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8AL UT WOS:000383875500012 PM 27586906 ER PT J AU Zanonato, PL Di Bernardo, P Zhang, Z Gong, Y Tian, G Gibson, JK Rao, L AF Zanonato, P. L. Di Bernardo, P. Zhang, Z. Gong, Y. Tian, G. Gibson, J. K. Rao, L. TI Hydrolysis of thorium(IV) at variable temperatures SO DALTON TRANSACTIONS LA English DT Article ID AQUEOUS-SOLUTION; MOLECULAR CLUSTERS; STABILITY RANGE; DEGREES-C; COMPLEXATION; URANIUM(VI); EQUILIBRIA; CONSTANTS; CORE; THERMODYNAMICS AB Hydrolysis of Th(IV) was studied in tetraethylammonium perchlorate (0.10 mol kg(-1)) at variable temperatures (283-358 K) by potentiometry and microcalorimetry. Three hydrolysis reactions, mTh(4+) + nH(2)O = Th-m(OH)(n)((4m-n)+) + nH(+), in which (n,m) = (2,2), (8,4), and (15,6), were invoked to describe the potentiometric and calorimetric data for solutions with the [hydroxide]/[Th(IV)] ratio <= 2. At higher ratios, the formation of (16,5) cannot be excluded. The hydrolysis constants, (star)beta(2,2), (star)beta(8,4), and (star)beta(15,6), increased by 3, 7, and 11 orders of magnitude, respectively, as the temperature was increased from 283 to 358 K. The enhancement is mainly due to the significant increase of the degree of ionization of water as the temperature rises. All three hydrolysis reactions are endothermic at 298 K, with enthalpies of (118 +/- 4) kJ mol(-1), (236 +/- 7) kJ mol(-1), and (554 +/- 4) kJ mol(-1) for Delta H-2,H-2, Delta H-8,H-4, and Delta H-15,H-6 respectively. The hydrolysis constants at infinite dilution have been obtained with the specific ion interaction approach. The applicability of three approaches for estimating the equilibrium constants at different temperatures, including the constant enthalpy approach, the constant heat capacity approach and the DQUANT equation was evaluated with the data from this work. C1 [Zanonato, P. L.; Di Bernardo, P.] Univ Padua, Dipartimento Sci Chim, Via Marzolo 1, I-35131 Padua, Italy. [Zhang, Z.; Gong, Y.; Tian, G.; Gibson, J. K.; Rao, L.] Lawrence Berkeley Natl Lab, Glenn T Seaborg Ctr, Berkeley, CA 94720 USA. RP Zanonato, PL (reprint author), Univ Padua, Dipartimento Sci Chim, Via Marzolo 1, I-35131 Padua, Italy.; Rao, L (reprint author), Lawrence Berkeley Natl Lab, Glenn T Seaborg Ctr, Berkeley, CA 94720 USA. EM pierluigi.zanonato@unipd.it; LRao@lbl.gov FU Office of Science, the Office of Basic Energy Science of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; LBNL [7118594] FX The calorimetric experiments at all temperatures except for that at 283 K and the ESI-MS experiments were conducted at the Lawrence Berkeley National Laboratory (LBNL) and supported by the Director, the Office of Science, the Office of Basic Energy Science of the U.S. Department of Energy (DOE), under Contract No. DE-AC02-05CH11231 at LBNL. The potentiometric experiments at all temperatures and the calorimetric experiments at 283 K were conducted at the University of Padova and supported by a subcontract (#7118594) from LBNL. NR 50 TC 1 Z9 1 U1 9 U2 12 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PD AUG 28 PY 2016 VL 45 IS 32 BP 12763 EP 12771 DI 10.1039/c6dt01868h PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DT4VE UT WOS:000381478500022 PM 27460458 ER PT J AU Terai, CR Klein, SA Zelinka, MD AF Terai, C. R. Klein, S. A. Zelinka, M. D. TI Constraining the low-cloud optical depth feedback at middle and high latitudes using satellite observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID GLOBAL CLIMATE MODEL; SOUTHERN-OCEAN; TEMPERATURE-DEPENDENCE; PHASE; THICKNESS; ISCCP; SIMULATIONS; SENSITIVITY; MECHANISMS; RADIATION AB The increase in cloud optical depth with warming at middle and high latitudes is a robust cloud feedback response found across all climate models. This study builds on results that suggest the optical depth response to temperature is timescale invariant for low-level clouds. The timescale invariance allows one to use satellite observations to constrain the models' optical depth feedbacks. Three passive-sensor satellite retrievals are compared against simulations from eight models from the Atmosphere Model Intercomparison Project (AMIP) of the 5th Coupled Model Intercomparison Project (CMIP5). This study confirms that the low-cloud optical depth response is timescale invariant in the AMIP simulations, generally at latitudes higher than 40 degrees. Compared to satellite estimates, most models overestimate the increase in optical depth with warming at the monthly and interannual timescales. Many models also do not capture the increase in optical depth with estimated inversion strength that is found in all three satellite observations and in previous studies. The discrepancy between models and satellites exists in both hemispheres and in most months of the year. A simple replacement of the models' optical depth sensitivities with the satellites' sensitivities reduces the negative shortwave cloud feedback by at least 50% in the 40 degrees-70 degrees S latitude band and by at least 65% in the 40 degrees-70 degrees N latitude band. Based on this analysis of satellite observations, we conclude that the low-cloud optical depth feedback at middle and high latitudes is likely too negative in climate models. C1 [Terai, C. R.; Klein, S. A.; Zelinka, M. D.] Lawrence Livermore Natl Lab, Cloud Proc Res Grp, Livermore, CA 94550 USA. RP Terai, CR (reprint author), Lawrence Livermore Natl Lab, Cloud Proc Res Grp, Livermore, CA 94550 USA. EM crterai@gmail.com RI Klein, Stephen/H-4337-2016; OI Klein, Stephen/0000-0002-5476-858X; Terai, Christopher/0000-0002-2433-0472 FU United States Department of Energy's Office of Science; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank the climate modeling groups for producing and making available their model output. For CMIP, the U.S. Department of Energy's (DOE) Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. The model output can be obtained from the Earth System Grid Federation. The satellite observations were obtained from CFMIP-OBS, hosted at http://climserv.ipsl.polytechnique.fr/cfmip-obs/. The ECMWF Interim Reanalysis fields are publicly available from http://www.ecmwf.int/. The data used to generate the figures and tables in this study can be obtained by contacting the corresponding author. We thank Steve Ghan, Jonathan Jiang, and two anonymous reviewers for providing comments and feedback that have helped to improve the manuscript. The efforts of the authors are supported by the Regional and Global Climate Modeling Program of the United States Department of Energy's Office of Science. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. IM-Release: LLNL-JRNL-688437. NR 49 TC 2 Z9 2 U1 7 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 27 PY 2016 VL 121 IS 16 BP 9696 EP 9716 DI 10.1002/2016JD025233 PG 21 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DZ9OQ UT WOS:000386207200025 ER PT J AU Fast, JD Berg, LK Zhang, K Easter, RC Ferrare, RA Hair, JW Hostetler, CA Liu, Y Ortega, I Sedlacek, A Shilling, JE Shrivastava, M Springston, SR Tomlinson, JM Volkamer, R Wilson, J Zaveri, RA Zelenyuk, A AF Fast, Jerome D. Berg, Larry K. Zhang, Kai Easter, Richard C. Ferrare, Richard A. Hair, Johnathan W. Hostetler, Chris A. Liu, Ying Ortega, Ivan Sedlacek, Arthur, III Shilling, John E. Shrivastava, Manish Springston, Stephen R. Tomlinson, Jason M. Volkamer, Rainer Wilson, Jacqueline Zaveri, Rahul A. Zelenyuk, Alla TI Model representations of aerosol layers transported from North America over the Atlantic Ocean during the Two-Column Aerosol Project SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; PHASE FRAGMENTATION REACTIONS; CLOUD MICROPHYSICS SCHEME; SPECTRAL-RESOLUTION LIDAR; CARBON VERTICAL PROFILES; GLOBAL CLIMATE MODEL; LONG-RANGE TRANSPORT; LOW-VOLATILITY SOA; BASIS-SET APPROACH; ORGANIC AEROSOL AB The ability of the Weather Research and Forecasting model with chemistry (WRF-Chem) version 3.7 and the Community Atmosphere Model version 5.3 (CAM5) in simulating profiles of aerosol properties is quantified using extensive in situ and remote sensing measurements from the Two-Column Aerosol Project (TCAP) conducted during July of 2012. TCAP was supported by the U.S. Department of Energy's Atmospheric Radiation Measurement program and was designed to obtain observations within two atmospheric columns; one fixed over Cape Cod, Massachusetts, and the other several hundred kilometers over the ocean. The performance is quantified using most of the available aircraft and surface measurements during July, and 2 days are examined in more detail to identify the processes responsible for the observed aerosol layers. The higher-resolution WRF-Chem model produced more aerosol mass in the free troposphere than the coarser-resolution CAM5 model so that the fraction of aerosol optical thicknessabove the residual layer from WRF-Chem was more consistent with lidar measurements. We found that the free troposphere layers are likely due to mean vertical motions associated with synoptic-scale convergence that lifts aerosols from the boundary layer. The vertical displacement and the time period associated with upward transport in the troposphere depend on the strength of the synoptic system and whether relatively high boundary layer aerosol concentrations are present where convergence occurs. While a parameterization of subgrid scale convective clouds applied in WRF-Chem modulated the concentrations of aerosols aloft, it did not significantly change the overall altitude and depth of the layers. C1 [Fast, Jerome D.; Berg, Larry K.; Zhang, Kai; Easter, Richard C.; Liu, Ying; Shilling, John E.; Shrivastava, Manish; Tomlinson, Jason M.; Wilson, Jacqueline; Zaveri, Rahul A.; Zelenyuk, Alla] Pacific Northwest Natl Lab, Richland, WA 99352 USA. [Ferrare, Richard A.; Hair, Johnathan W.; Hostetler, Chris A.] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Ortega, Ivan; Volkamer, Rainer] Univ Colorado, Dept Chem, Boulder, CO 80309 USA. [Sedlacek, Arthur, III; Springston, Stephen R.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fast, JD (reprint author), Pacific Northwest Natl Lab, Richland, WA 99352 USA. EM jerome.fast@pnl.gov RI Zhang, Kai/F-8415-2010; Volkamer, Rainer/B-8925-2016 OI Zhang, Kai/0000-0003-0457-6368; Volkamer, Rainer/0000-0002-0899-1369 FU Office of Science of the U.S. Department of Energy; DOE ARM [DE-SC0006730]; National Science Foundation; [DE-A06-76RLO976 1830] FX This research was supported by the Office of Science of the U.S. Department of Energy as part of the Atmospheric Radiation Measurement (ARM) and Atmospheric System Research (ASR) programs. The Pacific Northwest National Laboratory (PNNL) is operated by DOE by the Battelle Memorial Institute under contract DE-A06-76RLO976 1830. We thank the contributions of numerous individuals, including the G-1 flight crew (M. Hubbell, W. Svancara, J. Hone, and E. Dukes), King Air flight crew (R. Yasky, L. Kagey, M. Wusk, D. Bowser, S. Sims, D. Riddick, and G. Slover), staff from the Cape Cod National Seashore (Superintendent G. Price, L. McKean, C. Skowron, and B. Dougan), Cape Cod National Seashore Atlantic Research and Learning Center, and the radiosonde launch team from the Provincetown Center for Coastal Studies (M. Dunn, S. Greene, C. Hudak, L. Ludwig, J. Melander, D. Minsky, K. Shorr, S. Sollog, D. Towler, E. Larson, D. Dionne, C. Skowron). Support for the HSRL-2 flight operations during TCAP was provided by the DOE ARM program, Interagency Agreement DE-SC0006730, while support for the development of HSRL-2 was provided by the NASA Science Mission Directorate, ESTO, AITT, and Radiation Science Programs. The NOAA-MFRSR measurements were supported by NOAA GOES-R Cal/Val Activities within NOAA's National Environmental Satellite, Data, and Information Service. We thank Joseph Michalsky (NOAA) for providing the AOD measurements from the MFRSR instrument, Louisa Emmons (NCAR) for providing the MOZART global chemistry model output, Christine Wiedinmyer (NCAR) for providing the fire emissions inventory, Stuart McKeen (NOAA) for processing the 2011 NEI, Michael Sprenger and Heini Wernli (ETH) for providing the Lagrangian Analysis Tool LAGRANTO for the CAM5 back trajectory calculations, and Po-Lun Ma (PNNL) for assisting with the set up of CAM5. The Environmental Molecular Science Laboratory (EMSL), a DOE Office of Science User Facility located at PNNL, provided computational resources for the WRF-Chem simulations. For the CAM5 simulations, we would like to acknowledge the computing support from Yellowstone (ark:/85065/d7wd3xhc) provided by NCAR's Computational and Information Systems Laboratory (sponsored by the National Science Foundation) and from the PNNL Institutional Computing (PIC). Data used in this manuscript are available from the ARM data archive (www.archive.arm.gov) or from the corresponding author (jerome.fast@pnnl.gov). NR 108 TC 1 Z9 1 U1 8 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 27 PY 2016 VL 121 IS 16 BP 9814 EP 9848 DI 10.1002/2016JD025248 PG 35 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DZ9OQ UT WOS:000386207200031 ER PT J AU Mishra, V Scalapino, DJ Maier, TA AF Mishra, Vivek Scalapino, Douglas J. Maier, Thomas A. TI s(+/-) pairing near a Lifshitz transition SO SCIENTIFIC REPORTS LA English DT Article ID LAYER FESE FILMS; SUPERCONDUCTIVITY; CS AB Observations of robust superconductivity in some of the iron based superconductors in the vicinity of a Lifshitz point where a spin density wave instability is suppressed as the hole band drops below the Fermi energy raise questions for spin-fluctuation theories. Here we discuss spin-fluctuation pairing for a bilayer Hubbard model, which goes through such a Lifshitz transition. We find s(+/-) pairing with a transition temperature that peaks beyond the Lifshitz point and a gap function that has essentially the same magnitude but opposite sign on the incipient hole band as it does on the electron band that has a Fermi surface. C1 [Mishra, Vivek] Univ Tennessee, Joint Inst Computat Sci, Knoxville, TN 37996 USA. [Scalapino, Douglas J.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Maier, Thomas A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Maier, Thomas A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Mishra, V (reprint author), Univ Tennessee, Joint Inst Computat Sci, Knoxville, TN 37996 USA. EM mishrav@ornl.gov FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Center for Nanophase Materials Sciences, a US DOE Office of Science User Facility FX Research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U. S. Department of Energy. DJS and TAM acknowledge the support of the Center for Nanophase Materials Sciences, a US DOE Office of Science User Facility. We acknowledge the Valinor cluster for computational resources. We thank A. Linscheid, S. Maiti, P. Hirschfeld for useful discussion. NR 20 TC 0 Z9 0 U1 1 U2 1 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 26 PY 2016 VL 6 AR 32078 DI 10.1038/srep32078 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH9YH UT WOS:000392127500001 PM 27561327 ER PT J AU Patil, RS Banerjee, D Simon, CM Atwood, JL Thallapally, PK AF Patil, Rahul S. Banerjee, Debasis Simon, Cory M. Atwood, Jerry L. Thallapally, Praveen K. TI Noria: A Highly Xe-Selective Nanoporous Organic Solid SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE adsorption; organic macrocyclic compounds; selective gas separation; xenon ID ADSORBED SOLUTION THEORY; NOBLE-GAS ADSORPTION; MONTE-CARLO SIMULATIONS; SOLUTION THEORY IAST; RARE-GASES; FRAMEWORKS; XENON; SEPARATION; CONDENSATION; KRYPTON AB Separation of xenon and krypton is of industrial and environmental concern; the existing technologies use cryogenic distillation. Thus, a cost-effective, alternative technology for the separation of Xe and Kr and their capture from air is of significant importance. Herein, we report the selective Xe uptake in a crystalline porous organic oligomeric molecule, noria, and its structural analogue, PgC-noria, under ambient conditions. The selectivity of noria towards Xe arises from its tailored pore size and small cavities, which allows a directed non-bonding interaction of Xe atoms with a large number of carbon atoms of the noria molecular wheel in a confined space. C1 [Patil, Rahul S.; Atwood, Jerry L.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Patil, Rahul S.; Banerjee, Debasis; Thallapally, Praveen K.] Pacific Northwest Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Simon, Cory M.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Thallapally, PK (reprint author), Pacific Northwest Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM Praveen.Thallapally@pnnl.gov OI Thallapally, Praveen Kumar/0000-0001-7814-4467; Simon, Cory/0000-0002-8181-9178 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; US Department of Energy [DEAC05-76L01830] FX We thank the US Department of Energy (DOE), Office of Nuclear Energy, and in particular, Jim Bresee and Kimberly Gray, for their support (DOE - HQ). Terry Todd (Idaho National Laboratory), John Vienna (PNNL), Denis Strachan (PNNL) and Bob Jubin (Oak Ridge National Laboratory) provided programmatic support and guidance. C.M.S. is supported through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001015. We thank Prof. Berend Smith and Dr. Maciej Haranczyk for helpful discussions. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for the US Department of Energy by Battelle Memorial Institute under Contract DEAC05-76L01830. NR 45 TC 1 Z9 1 U1 17 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD AUG 26 PY 2016 VL 22 IS 36 BP 12618 EP 12623 DI 10.1002/chem.201602131 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DW6JX UT WOS:000383758200006 PM 27377260 ER PT J AU Ding, J Strelcov, E Kalinin, SV Bassiri-Gharb, N AF Ding, J. Strelcov, E. Kalinin, S. V. Bassiri-Gharb, N. TI Electrochemical reactivity and proton transport mechanisms in nanostructured ceria SO NANOTECHNOLOGY LA English DT Article DE nanostructured ceria; tr-KPFM; proton conduction; humidity; energy discovery platforms ID GAS SHIFT REACTION; OXIDE FUEL-CELLS; PHOTOELECTRON-SPECTROSCOPY; THIN-FILMS; WATER; CATALYSTS; SURFACES; CONDUCTIVITY; ADSORPTION; STABILITY AB Electrochemical reactivity and ionic transport at the nanoscale are essential in many energy applications. In this study, time-resolved Kelvin probe force microscopy (tr-KPFM) is utilized for surface potential mapping of nanostructured ceria, in both space and time domains. The fundamental mechanisms of proton injection and transport are studied as a function of environmental conditions and the presence or absence of triple phase boundaries. Finite element modeling is used to extract physical parameters from the experimental data, allowing not only quantification of the observed processes, but also decoupling of their contributions to the measured signal. The constructed phase diagrams of the parameters demonstrate a thermally activated proton injection reaction at the triple phase boundary, and two transport processes that are responsible for the low-temperature proton conductivity of nanostructured ceria. C1 [Ding, J.; Bassiri-Gharb, N.] Georgia Inst Technol, Dept Mat Sci & Engn, Atlanta, GA 30332 USA. [Kalinin, S. V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Bassiri-Gharb, N.] Georgia Inst Technol, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Strelcov, E.] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. RP Ding, J (reprint author), Georgia Inst Technol, Dept Mat Sci & Engn, Atlanta, GA 30332 USA.; Strelcov, E (reprint author), NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. EM jding35@gatech.edu; nazanin.bassiri@gatech.edu FU National Science Foundation [DMR-1255379] FX This research was supported by the National Science Foundation under grant DMR-1255379. The tr-KPFM portion of this research was conducted at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility, under user proposal CNMS2013-123. NR 43 TC 0 Z9 0 U1 13 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 26 PY 2016 VL 27 IS 34 AR 345401 DI 10.1088/0957-4484/27/34/345401 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DW9GB UT WOS:000383963300009 PM 27407076 ER PT J AU Zhu, WS Gao, X Li, Q Li, HP Chao, YH Li, MJ Mahurin, SM Li, HM Zhu, HY Dai, S AF Zhu, Wenshuai Gao, Xiang Li, Qian Li, Hongping Chao, Yanhong Li, Meijun Mahurin, Shannon M. Li, Huaming Zhu, Huiyuan Dai, Sheng TI Controlled Gas Exfoliation of Boron Nitride into Few-Layered Nanosheets SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE boron nitride; exfoliation; liquid nitrogen; nanosheets; thermal expansion ID LIQUID-PHASE EXFOLIATION; ONE-STEP EXFOLIATION; 2-DIMENSIONAL NANOMATERIALS; FUNCTIONALIZATION AB The controlled exfoliation of hexagonal boron nitride (h-BN) into single- or few-layered nanosheets remains a grand challenge and becomes the bottleneck to essential studies and applications of h-BN. Here, we present an efficient strategy for the scalable synthesis of few-layered h-BN nanosheets (BNNS) using a novel gas exfoliation of bulk h-BN in liquid N-2 (L-N-2). The essence of this strategy lies in the combination of a high temperature triggered expansion of bulk h-BN and the cryogenic L-N-2 gasification to exfoliate the h-BN. The produced BNNS after ten cycles (BNNS-10) consisted primarily of fewer than five atomic layers with a high mass yield of 16-20%. N-2 sorption and desorption isotherms show that the BNNS-10 exhibited a much higher specific surface area of 278m(2)g(-1) than that of bulk BN (10m(2)g(-1)). Through the investigation of the exfoliated intermediates combined with a theoretical calculation, we found that the huge temperature variation initiates the expansion and curling of the bulk h-BN. Subseqently, the L-N-2 penetrates into the interlayers of h-BN along the curling edge, followed by an immediate drastic gasification of L-N-2, further peeling off h-BN. This novel gas exfoliation of high surface area BNNS not only opens up potential opportunities for wide applications, but also can be extended to produce other layered materials in high yields. C1 [Zhu, Wenshuai; Li, Hongping; Chao, Yanhong; Li, Huaming] Jiangsu Univ, Inst Energy Res, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China. [Zhu, Wenshuai; Mahurin, Shannon M.; Zhu, Huiyuan; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Gao, Xiang] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Li, Qian] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Li, Meijun; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Zhu, WS (reprint author), Jiangsu Univ, Inst Energy Res, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.; Zhu, WS; Zhu, HY; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM zhuws@ujs.edu.cn; zhuh@ornl.gov; dais@ornl.gov FU National Natural Science Foundation of China [21376111, 21576122, 21506083]; Six Big Talent Peak in Jiangsu province [JNHB-004]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; Liane B. Russell Fellowship - Laboratory Directed Research and Development Program at the Oak Ridge National Laboratory FX W.S.Z., H.Y.Z., and S.D. conceived the idea. W.S.Z. exfoliated and characterized BN. X.G. carried out STEM and EELS. Q.L. performed AFM. H.P.L., Y.H.C. and H.M.L. provided theoretical calculation and discussion. M.J.L. and S.M. performed TEM and Raman. W.S.Z. and H.Y.Z. wrote the paper. Y.H.C., H.M.L. and S.D. discussed the results and participated in the preparation of the paper. W.S.Z. and Y.H.C. appreciates the financial support from the National Natural Science Foundation of China (grant numbers 21376111, 21576122, and 21506083) and Six Big Talent Peak in Jiangsu province (JNHB-004). S.D. and S.M. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. H.Z. was supported by Liane B. Russell Fellowship sponsored by the Laboratory Directed Research and Development Program at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the US Department of Energy. We are grateful to Dr. Chenghao Wu for his help on XANES and XPS characterizations, and Dr. Yunchao Li for his help on SEM characterization. NR 42 TC 1 Z9 1 U1 105 U2 106 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 26 PY 2016 VL 55 IS 36 BP 10766 EP 10770 DI 10.1002/anie.201605515 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DW2LJ UT WOS:000383473600043 PM 27444210 ER PT J AU Pozzi, N Bystranowska, D Zuo, XB Di Cera, E AF Pozzi, Nicola Bystranowska, Dominika Zuo, Xiaobing Di Cera, Enrico TI Structural Architecture of Prothrombin in Solution Revealed by Single Molecule Spectroscopy SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE enzyme kinetics; prothrombin; single-molecule biophysics; structure-function; thrombin ID ALTERNATING-LASER EXCITATION; TRYPSIN-LIKE PROTEASES; RAY CRYSTAL-STRUCTURE; BLOOD-COAGULATION; CONFORMATIONAL SELECTION; SOLUTION SCATTERING; FRET; ACTIVATION; EVOLUTION; THROMBIN AB The coagulation factor prothrombin has a complex spatial organization of its modular assembly that comprises the N-terminal Gla domain, kringle-1, kringle-2, and the C-terminal protease domain connected by three intervening linkers. Here we use single molecule Forster resonance energy transfer to access the conformational landscape of prothrombin in solution and uncover structural features of functional significance that extend recent x-ray crystallographic analysis. Prothrombin exists in equilibrium between two alternative conformations, open and closed. The closed conformation predominates (70%) and features an unanticipated intramolecular collapse of Tyr(93) in kringle-1 onto Trp(547) in the protease domain that obliterates access to the active site and protects the zymogen from autoproteolytic conversion to thrombin. The open conformation (30%) is more susceptible to chymotrypsin digestion and autoactivation, and features a shape consistent with recent x-ray crystal structures. Small angle x-ray scattering measurements of prothrombin wild type stabilized 70% in the closed conformation and of the mutant Y93A stabilized 80% in the open conformation directly document two envelopes that differ 50 in length. These findings reveal important new details on the conformational plasticity of prothrombin in solution and the drastic structural difference between its alternative conformations. Prothrombin uses the intramolecular collapse of kringle-1 onto the active site in the closed form to prevent autoactivation. The open-closed equilibrium also defines a new structural framework for the mechanism of activation of prothrombin by prothrombinase. C1 [Pozzi, Nicola; Bystranowska, Dominika; Di Cera, Enrico] St Louis Univ, Sch Med, Edward A Doisy Dept Biochem & Mol Biol, St Louis, MO 63104 USA. [Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Bystranowska, Dominika] Wroclaw Univ Technol, Dept Biochem, PL-50370 Wroclaw, Poland. RP Di Cera, E (reprint author), St Louis Univ, Sch Med, Edward A Doisy Dept Biochem & Mol Biol, St Louis, MO 63104 USA. EM enrico@slu.edu OI Zuo, Xiaobing/0000-0002-0134-4804; Pozzi, Nicola/0000-0003-2309-7100 FU DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX We gratefully acknowledge Dr. David Gohara and Zhiwei Chen for their assistance with the model of the closed conformation of prothrombin, Daniel Shropshire and Leslie Pelc for expression and labeling of several constructs for smFRET measurements, and Dr. Tomasz Heyduk and Rachel Hickey for providing double-stranded DNA constructs used for calibration of the Micro-Time instrument and control experiments. This research used resources of the Advanced Photon Source, a U. S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. NR 49 TC 0 Z9 0 U1 4 U2 4 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD AUG 26 PY 2016 VL 291 IS 35 BP 18107 EP 18116 DI 10.1074/jbc.M116.738310 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DV9EC UT WOS:000383241800005 PM 27435675 ER PT J AU Narayanan, V Nogue, VSI van Niel, EWJ Gorwa-Grauslund, MF AF Narayanan, Venkatachalam Sanchez i Nogue, Violeta van Niel, Ed W. J. Gorwa-Grauslund, Marie F. TI Adaptation to low pH and lignocellulosic inhibitors resulting in ethanolic fermentation and growth of Saccharomyces cerevisiae SO AMB EXPRESS LA English DT Article DE Saccharomyces cerevisiae; Low pH; Lignocellulosic inhibitors; Phenotypic robustness; Adaptation; Ethanol yield ID ACETIC-ACID TOLERANCE; SHORT-TERM ADAPTATION; BACTERIAL-CONTAMINATION; CONTINUOUS-CULTURE; YEAST STRAINS; DNA; HETEROGENEITY; HYDROLYSATE; PERFORMANCE; BIOMASS AB Lignocellulosic bioethanol from renewable feedstocks using Saccharomyces cerevisiae is a promising alternative to fossil fuels owing to environmental challenges. S. cerevisiae is frequently challenged by bacterial contamination and a combination of lignocellulosic inhibitors formed during the pre-treatment, in terms of growth, ethanol yield and productivity. We investigated the phenotypic robustness of a brewing yeast strain TMB3500 and its ability to adapt to low pH thereby preventing bacterial contamination along with lignocellulosic inhibitors by short-term adaptation and adaptive lab evolution (ALE). The short-term adaptation strategy was used to investigate the inherent ability of strain TMB3500 to activate a robust phenotype involving pre-culturing yeast cells in defined medium with lignocellulosic inhibitors at pH 5.0 until late exponential phase prior to inoculating them in defined media with the same inhibitor cocktail at pH 3.7. Adapted cells were able to grow aerobically, ferment anaerobically (glucose exhaustion by 19 +/- 5 h to yield 0.45 +/- 0.01 g ethanol g glucose(-1)) and portray significant detoxification of inhibitors at pH 3.7, when compared to non-adapted cells. ALE was performed to investigate whether a stable strain could be developed to grow and ferment at low pH with lignocellulosic inhibitors in a continuous suspension culture. Though a robust population was obtained after 3600 h with an ability to grow and ferment at pH 3.7 with inhibitors, inhibitor robustness was not stable as indicated by the characterisation of the evolved culture possibly due to phenotypic plasticity. With further research, this short-term adaptation and low pH strategy could be successfully applied in lignocellulosic ethanol plants to prevent bacterial contamination. C1 [Narayanan, Venkatachalam; van Niel, Ed W. J.; Gorwa-Grauslund, Marie F.] Lund Univ, Dept Chem, Div Appl Microbiol, POB 124, S-22100 Lund, Sweden. [Sanchez i Nogue, Violeta] Natl Bioenergy Ctr, Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP van Niel, EWJ (reprint author), Lund Univ, Dept Chem, Div Appl Microbiol, POB 124, S-22100 Lund, Sweden. EM ed.van_niel@tmb.lth.se FU Swedish National Energy Agency [P35350-1] FX This research was funded by Swedish National Energy Agency (www.ener-gimyndigheten.se, Project No. P35350-1). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 66 TC 1 Z9 1 U1 11 U2 11 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2191-0855 J9 AMB EXPRESS JI AMB Express PD AUG 26 PY 2016 VL 6 AR 59 DI 10.1186/s13568-016-0234-8 PG 13 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DU6WG UT WOS:000382354700002 PM 27566648 ER PT J AU Gardas, B Deffner, S Saxena, A AF Gardas, Bartlomiej Deffner, Sebastian Saxena, Avadh TI Repeatability of measurements: Non-Hermitian observables and quantum Coriolis force SO PHYSICAL REVIEW A LA English DT Article ID CANONICAL-TRANSFORMATIONS; MECHANICS; SYMMETRY AB A noncommuting measurement transfers, via the apparatus, information encoded in a system's state to the external "observer." Classical measurements determine properties of physical objects. In the quantum realm, the very same notion restricts the recording process to orthogonal states as only those are distinguishable by measurements. Therefore, even a possibility to describe physical reality by means of non-Hermitian operators should volens nolens be excluded as their eigenstates are not orthogonal. Here, we show that non-Hermitian operators with real spectra can be treated within the standard framework of quantum mechanics. Furthermore, we propose a quantum canonical transformation that maps Hermitian systems onto non-Hermitian ones. Similar to classical inertial forces this map is accompanied by an energetic cost, pinning the system on the unitary path. C1 [Gardas, Bartlomiej; Deffner, Sebastian; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Gardas, Bartlomiej] Univ Silesia, Inst Phys, PL-40007 Katowice, Poland. [Deffner, Sebastian; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Gardas, B (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Gardas, B (reprint author), Univ Silesia, Inst Phys, PL-40007 Katowice, Poland. EM bartek.gardas@gmail.com RI Deffner, Sebastian/C-5170-2008 OI Deffner, Sebastian/0000-0003-0504-6932 FU Polish Ministry of Science and Higher Education [1060/MOB/2013/0]; U.S. Department of Energy through a LANL FX It is our pleasure to thank Wojciech H. Zurek and Rolando Somma for stimulating discussions. This work was supported by the Polish Ministry of Science and Higher Education under project Mobility Plus 1060/MOB/2013/0 (B.G.); S.D. acknowledges financial support from the U.S. Department of Energy through a LANL Director's Funded Fellowship. NR 46 TC 1 Z9 1 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD AUG 26 PY 2016 VL 94 IS 2 AR 022121 DI 10.1103/PhysRevA.94.022121 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DU1VJ UT WOS:000381997900001 ER PT J AU Huang, SC Kubo, T Geng, RL AF Huang, Shichun Kubo, Takayuki Geng, R. L. TI Dependence of trapped-flux-induced surface resistance of a large-grain Nb superconducting radio-frequency cavity on spatial temperature gradient during cooldown through T-c SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID NIOBIUM AB Recent studies by Romanenko et al. revealed that cooling down a superconducting cavity under a large spatial temperature gradient decreases the amount of trapped flux and leads to reduction of the residual surface resistance. In the present paper, the flux expulsion ratio and the trapped-flux-induced surface resistance of a large-grain cavity cooled down under a spatial temperature gradient up to 80 K/m are studied under various applied magnetic fields from 5 to 20 mu T. We show the flux expulsion ratio improves as the spatial temperature gradient increases, independent of the applied magnetic field: our results support and enforce the previous studies. We then analyze all rf measurement results obtained under different applied magnetic fields together by plotting the trapped-flux-induced surface resistance normalized by the applied magnetic field as a function of the spatial temperature gradient. All the data can be fitted by a single curve, which defines an empirical formula for the trapped-flux-induced surface resistance as a function of the spatial temperature gradient and applied magnetic field. The formula can fit not only the present results but also those obtained by Romanenko et al. previously. The sensitivity r(fl) of surface resistance from trapped magnetic flux of fine-grain and large-grain niobium cavities and the origin of dT/ds dependence of R-fl/B-a are also discussed. C1 [Huang, Shichun] Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China. [Huang, Shichun] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Huang, Shichun; Geng, R. L.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Kubo, Takayuki] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki 3050801, Japan. [Kubo, Takayuki] SOKENDAI Grad Univ Adv Studies, Hayama, Kanagawa 2400015, Japan. RP Geng, RL (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM geng@jlab.org FU U.S. DOE [DE-AC05-06OR23177]; U.S.-Japan cooperation fund; JSPS [26800157, 26600142]; Ministry of Education, Culture, Sports, Science and Technology, Japan FX This work is authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. Supplemental support is from U.S.-Japan cooperation fund. The work of T. K. is supported by JSPS Grant-in-Aid for Young Scientists (B) 26800157, JSPS Grant-in-Aid for Challenging Exploratory Research 26600142, and Photon and Quantum Basic Research Coordinated Development Program from the Ministry of Education, Culture, Sports, Science and Technology, Japan. NR 29 TC 2 Z9 2 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD AUG 26 PY 2016 VL 19 IS 8 AR 082001 DI 10.1103/PhysRevAccelBeams.19.082001 PG 9 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU1ZU UT WOS:000382010700001 ER PT J AU Tsvelik, AM Zaliznyak, IA AF Tsvelik, A. M. Zaliznyak, I. A. TI Heisenberg necklace model in a magnetic field SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM IMPURITY; 2 DIMENSIONS; SIGMA-MODEL; SPIN; ANTIFERROMAGNETS; CHAIN; DYNAMICS; GAP AB We study the low-energy sector of the Heisenberg necklace model. Using the field-theorymethods, we estimate how the coupling of the electronic spins with the paramagnetic Kondo spins affects the overall spin dynamics and evaluate its dependence on a magnetic field. We are motivated by the experimental realizations of the spin-1/2 Heisenberg chains in SrCuO2 and Sr2CuO3 cuprates, which remain one-dimensional Luttinger liquids down to temperatures much lower than the in-chain exchange coupling J. We consider the perturbation of the energy spectrum caused by the interaction. with nuclear spins (I = 3/2) present on the same sites. We find that the resulting necklace model has a characteristic energy scale, Lambda similar to J(1/3)(gamma I)(2/3), at which the coupling between (nuclear) spins of the necklace and the spins of the Heisenberg chain becomes strong. This energy scale is insensitive to a magnetic field B. For mu B-B > Lambda we find two gapless bosonic modes that have different velocities, whose ratio at strong fields approaches a universal number, root 2 + 1. C1 [Tsvelik, A. M.; Zaliznyak, I. A.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA. RP Tsvelik, AM (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA. FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE) [DE-AC02-98CH10886] FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE), under Contract No. DE-AC02-98CH10886. NR 31 TC 1 Z9 1 U1 9 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 26 PY 2016 VL 94 IS 7 AR 075152 DI 10.1103/PhysRevB.94.075152 PG 5 WC Physics, Condensed Matter SC Physics GA DU1VX UT WOS:000381999400001 ER PT J AU Gal, A Hungerford, EV Millener, DJ AF Gal, A. Hungerford, E. V. Millener, D. J. TI Strangeness in nuclear physics SO REVIEWS OF MODERN PHYSICS LA English DT Article ID P-SHELL HYPERNUCLEI; LAMBDA-LAMBDA-HYPERNUCLEI; NONMESONIC WEAK DECAY; BARYON-BARYON INTERACTIONS; EFFECTIVE-FIELD THEORY; GAMMA-RAY SPECTROSCOPY; BINDING-ENERGY VALUES; HYPERON-HYPERON INTERACTIONS; EXCHANGE-POTENTIAL APPROACH; SINGLE-PARTICLE POTENTIALS AB Extensions of nuclear physics to the strange sector are reviewed, covering data and models of. and other hypernuclei, multistrange matter, and antikaon bound states and condensation. Past achievements are highlighted, present unresolved problems are discussed, and future directions are outlined. C1 [Gal, A.] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. [Hungerford, E. V.] Univ Houston, Houston, TX 77204 USA. [Millener, D. J.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Gal, A (reprint author), Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. EM avragal@vms.huji.ac.il; hunger@uh.edu; millener@bnl.gov FU U.S. DOE [DE-SC0012704, DE-SC0011598] FX This work was supported by the U.S. DOE under Contracts No. DE-SC0012704 (D. J. M.) and No. DE-SC0011598 (E. V. H.). NR 515 TC 9 Z9 9 U1 6 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0034-6861 EI 1539-0756 J9 REV MOD PHYS JI Rev. Mod. Phys. PD AUG 26 PY 2016 VL 88 IS 3 AR 035004 DI 10.1103/RevModPhys.88.035004 PG 58 WC Physics, Multidisciplinary SC Physics GA DU2AX UT WOS:000382013900001 ER PT J AU Kagan, CR Lifshitz, E Sargent, EH Talapin, DV AF Kagan, Cherie R. Lifshitz, Efrat Sargent, Edward H. Talapin, Dmitri V. TI Building devices from colloidal quantum dots SO SCIENCE LA English DT Review ID FIELD-EFFECT TRANSISTORS; LIGHT-EMITTING-DIODES; MULTIPLE EXCITON GENERATION; ATOMIC LAYER DEPOSITION; NANOCRYSTAL SOLIDS; SEMICONDUCTOR NANOCRYSTALS; SURFACE-CHEMISTRY; SOLAR-CELLS; LOW-VOLTAGE; CDSE NANOCRYSTALS AB The continued growth of mobile and interactive computing requires devices manufactured with low-cost processes, compatible with large-area and flexible form factors, and with additional functionality. We review recent advances in the design of electronic and optoelectronic devices that use colloidal semiconductor quantum dots (QDs). The properties of materials assembled of QDs may be tailored not only by the atomic composition but also by the size, shape, and surface functionalization of the individual QDs and by the communication among these QDs. The chemical and physical properties of QD surfaces and the interfaces in QD devices are of particular importance, and these enable the solution-based fabrication of low-cost, large-area, flexible, and functional devices. We discuss challenges that must be addressed in the move to solution-processed functional optoelectronic nanomaterials. C1 [Kagan, Cherie R.] Univ Penn, Dept Elect & Syst Engn, Dept Mat Sci & Engn, 200 South 33rd St, Philadelphia, PA 19104 USA. [Kagan, Cherie R.] Univ Penn, Dept Chem, 200 South 33rd St, Philadelphia, PA 19104 USA. [Lifshitz, Efrat] Technion, Schulich Fac Chem, Inst Solid State, IL-32000 Haifa, Israel. [Lifshitz, Efrat] Technion, Russell Berrie Nanotechnol Inst, IL-32000 Haifa, Israel. [Sargent, Edward H.] Dept Elect & Comp Engn, 10 Kings Coll Rd, Toronto, ON M5S 3G4, Canada. [Talapin, Dmitri V.] Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. [Talapin, Dmitri V.] Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Talapin, Dmitri V.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Kagan, CR (reprint author), Univ Penn, Dept Elect & Syst Engn, Dept Mat Sci & Engn, 200 South 33rd St, Philadelphia, PA 19104 USA.; Kagan, CR (reprint author), Univ Penn, Dept Chem, 200 South 33rd St, Philadelphia, PA 19104 USA.; Lifshitz, E (reprint author), Technion, Schulich Fac Chem, Inst Solid State, IL-32000 Haifa, Israel.; Lifshitz, E (reprint author), Technion, Russell Berrie Nanotechnol Inst, IL-32000 Haifa, Israel.; Sargent, EH (reprint author), Dept Elect & Comp Engn, 10 Kings Coll Rd, Toronto, ON M5S 3G4, Canada.; Talapin, DV (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA.; Talapin, DV (reprint author), Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Talapin, DV (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM kagan@seas.upenn.edu; ssefrat@technion.ac.il; ted.sargent@utoronto.ca; dvtalapin@uchicago.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-SC0002158]; Israel Council for High Education-Focal Area Technology [872967]; Volkswagen Stiftung [88116, ZN2916]; Israel Science Foundation [914/15, 1508/14]; Horizon2020 PHONSI project; King Abdullah University of Science and Technology (KAUST) [KUS-11-009-21]; U.S. Department of Defense (DOD) Office of Naval Research [N00014-13-1-0490] FX C.R.K. gratefully acknowledges the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under award DE-SC0002158 for support. E.L. thanks the Israel Council for High Education-Focal Area Technology (grant 872967), the Volkswagen Stiftung (grants 88116 and ZN2916), the Israel Science Foundation (grants 914/15 and 1508/14), and the Horizon2020 PHONSI project for their support. E.H.S. acknowledges award (KUS-11-009-21) from the King Abdullah University of Science and Technology (KAUST). D.V.T. acknowledges support by the U.S. Department of Defense (DOD) Office of Naval Research grant N00014-13-1-0490. C.R.K., E.H.S., and D.V.T. hold and have applied for several patents related to QD assemblies in devices. E.H.S. has a financial interest in and serves as Chief Technology Officer and director of InVisage Technologies. NR 116 TC 14 Z9 14 U1 165 U2 243 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 26 PY 2016 VL 353 IS 6302 AR aac5523 DI 10.1126/science.aac5523 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU0CA UT WOS:000381867700027 ER PT J AU Silver, MA Cary, SK Johnson, JA Baumbach, RE Arico, AA Luckey, M Urban, M Wang, JC Polinski, MJ Chemey, A Liu, G Chen, KW Van Cleve, SM Marsh, ML Eaton, TM de Burgt, LJV Gray, AL Hobart, DE Hanson, K Maron, L Gendron, F Autschbach, J Speldrich, M Kogerler, P Yang, P Braley, J Albrecht-Schmitt, TE AF Silver, Mark A. Cary, Samantha K. Johnson, Jason A. Baumbach, Ryan E. Arico, Alexandra A. Luckey, Morgan Urban, Matthew Wang, Jamie C. Polinski, Matthew J. Chemey, Alexander Liu, Guokui Chen, Kuan-Wen Van Cleve, Shelley M. Marsh, Matthew L. Eaton, Teresa M. de Burgt, Lambertus J. van Gray, Ashley L. Hobart, David E. Hanson, Kenneth Maron, Laurent Gendron, Frederic Autschbach, Jochen Speldrich, Manfred Koegerler, Paul Yang, Ping Braley, Jenifer Albrecht-Schmitt, Thomas E. TI Characterization of berkelium(III) dipicolinate and borate compounds in solution and the solid state SO SCIENCE LA English DT Article ID MOLECULAR-ORBITAL METHODS; VALENCE BASIS-SETS; TRIVALENT ACTINIDE; CORRELATION-ENERGY; CRYSTAL-STRUCTURES; CALIFORNIUM; COMPLEXES; ELEMENT; PSEUDOPOTENTIALS; COVALENCY AB Berkelium is positioned at a crucial location in the actinide series between the inherently stable half-filled 5f(7) configuration of curium and the abrupt transition in chemical behavior created by the onset of a metastable divalent state that starts at californium. However, the mere 320-day half-life of berkelium's only available isotope, Bk-249, has hindered in-depth studies of the element's coordination chemistry. Herein, we report the synthesis and detailed solid-state and solution-phase characterization of a berkelium coordination complex, Bk(III)tris(dipicolinate), as well as a chemically distinct Bk(III) borate material for comparison. We demonstrate that berkelium's complexation is analogous to that of californium. However, from a range of spectroscopic techniques and quantum mechanical calculations, it is clear that spin-orbit coupling contributes significantly to berkelium's multiconfigurational ground state. C1 [Silver, Mark A.; Cary, Samantha K.; Arico, Alexandra A.; Wang, Jamie C.; Chemey, Alexander; Marsh, Matthew L.; Eaton, Teresa M.; de Burgt, Lambertus J. van; Hobart, David E.; Hanson, Kenneth; Albrecht-Schmitt, Thomas E.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Johnson, Jason A.; Gray, Ashley L.] Florida State Univ, Environm Hlth & Safety, Tallahassee, FL 32306 USA. [Baumbach, Ryan E.; Chen, Kuan-Wen] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Luckey, Morgan; Urban, Matthew; Braley, Jenifer] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Luckey, Morgan; Urban, Matthew; Braley, Jenifer] Colorado Sch Mines, Dept Nucl Engn, Golden, CO 80401 USA. [Polinski, Matthew J.] Bloomsburg Univ Penn, Dept Chem & Biochem, Bloomsburg, PA 17815 USA. [Liu, Guokui] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Van Cleve, Shelley M.] Oak Ridge Natl Lab, Nucl Mat Proc Grp, One Bethel Valley Rd, Oak Ridge, TN 37830 USA. [Maron, Laurent] Inst Natl Sci Appl, Lab Phys & Chim Nanoobjets, F-31077 Toulouse 4, France. [Gendron, Frederic; Autschbach, Jochen] SUNY Buffalo, Univ Buffalo, Dept Chem, Buffalo, NY 14260 USA. [Speldrich, Manfred; Koegerler, Paul] Univ Aachen, Inst Anorgan Chem, Rheinisch Westfal Tech Hsch, D-52074 Aachen, Germany. [Yang, Ping] Los Alamos Natl Lab, Div Theory, Los Alamos, NM 87545 USA. RP Albrecht-Schmitt, TE (reprint author), Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA.; Braley, J (reprint author), Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA.; Braley, J (reprint author), Colorado Sch Mines, Dept Nucl Engn, Golden, CO 80401 USA. EM jbraley@mines.edu; albrecht-schmitt@chem.fsu.edu RI Speldrich, Manfred/P-3615-2016; Autschbach, Jochen/S-5472-2016; Kogerler, Paul/H-5866-2013; OI Speldrich, Manfred/0000-0002-8626-6410; Autschbach, Jochen/0000-0001-9392-877X; Kogerler, Paul/0000-0001-7831-3953; Yang, Ping/0000-0003-4726-2860; Luckey, Morgan/0000-0001-9264-6316 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program [DE-FG02-13ER16414, DE-SC0012039, DE-SC0001136]; European Research Council [StG 308051 MOLSPINTRON]; National Science Foundation [DMR-1157490, DGE-1449440]; State of Florida; U.S. Department of Energy FX This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program under Award Number DE-FG02-13ER16414 (Florida State University) and DE-SC0012039 (Colorado School of Mines), and DE-SC0001136 (formerly DE-FG02-09ER16066) (F.G. and J.A.). M.S. and P.K. were supported by European Research Council StG 308051 MOLSPINTRON. The isotopes used in this research were supplied by the U.S. Department of Energy, Office of Science, by the Isotope Program in the Office of Nuclear Physics. The 249Bk was provided to Florida State University and the Colorado School of Mines via the Isotope Development and Production for Research and Applications Program through the Radiochemical Engineering and Development Center at Oak Ridge National Laboratory. We are especially grateful for assistance and supervision by the Office of Environmental Health and Safety at Florida State University/Colorado School of Mines and the Office of Radiation Safety for their facilitation of these studies. Magnetization measurements using the vibrating sample magnetometer SQUID magnetic properties measurement system were performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement no. DMR-1157490, the State of Florida, and the U.S. Department of Energy. We are indebted to the Office of Safety at the National High Magnetic Field Laboratory for helping to facilitate these studies as well. J.C.W. is supported by the National Science Foundation Graduate Research Fellowship under grant no. DGE-1449440. This research was support in part by an appointment to the CBFO Fellowship Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. Metrical parameters for the structures of Bk(HDPA)3center dot nH2O and Bk[B6O8(OH)5] are available free of charge from the Cambridge Crystallographic Data Centre under accession numbers CCDC-1451021 and 1490887, respectively. NR 49 TC 1 Z9 1 U1 28 U2 43 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 26 PY 2016 VL 353 IS 6302 AR aaf3762 DI 10.1126/science.aaf3762 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU0CA UT WOS:000381867700030 ER PT J AU Jones, CD Arora, V Friedlingstein, P Bopp, L Brovkin, V Dunne, J Graven, H Hoffman, F Ilyina, T John, JG Jung, M Kawamiya, M Koven, C Pongratz, J Raddatz, T Randerson, JT Zaehle, S AF Jones, Chris D. Arora, Vivek Friedlingstein, Pierre Bopp, Laurent Brovkin, Victor Dunne, John Graven, Heather Hoffman, Forrest Ilyina, Tatiana John, Jasmin G. Jung, Martin Kawamiya, Michio Koven, Charlie Pongratz, Julia Raddatz, Thomas Randerson, James T. Zaehle, Soenke TI C4MIP-The Coupled Climate-Carbon Cycle Model Intercomparison Project: experimental protocol for CMIP6 SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID EARTH SYSTEM MODELS; SOIL ORGANIC-MATTER; LAND-COVER CHANGE; ATMOSPHERIC CO2; NITROGEN INTERACTIONS; ANTHROPOGENIC CARBON; POSITIVE FEEDBACK; SOUTHERN-OCEAN; C DYNAMICS; SPIN-UP AB Coordinated experimental design and implementation has become a cornerstone of global climate modelling. Model Intercomparison Projects (MIPs) enable systematic and robust analysis of results across many models, by reducing the influence of ad hoc differences in model set-up or experimental boundary conditions. As it enters its 6th phase, the Coupled Model Intercomparison Project (CMIP6) has grown significantly in scope with the design and documentation of individual simulations delegated to individual climate science communities. The Coupled Climate-Carbon Cycle Model Intercomparison Project (C4MIP) takes responsibility for design, documentation, and analysis of carbon cycle feedbacks and interactions in climate simulations. These feedbacks are potentially large and play a leading-order contribution in determining the atmospheric composition in response to human emissions of CO2 and in the setting of emissions targets to stabilize climate or avoid dangerous climate change. For over a decade, C4MIP has coordinated coupled climate-carbon cycle simulations, and in this paper we describe the C4MIP simulations that will be formally part of CMIP6. While the climate-carbon cycle community has created this experimental design, the simulations also fit within the wider CMIP activity, conform to some common standards including documentation and diagnostic requests, and are designed to complement the CMIP core experiments known as the Diagnostic, Evaluation and Characterization of Klima (DECK). C4MIP has three key strands of scientific motivation and the requested simulations are designed to satisfy their needs: (1) pre-industrial and historical simulations (formally part of the common set of CMIP6 experiments) to enable model evaluation, (2) idealized coupled and partially coupled simulations with 1% per year increases in CO2 to enable diagnosis of feedback strength and its components, (3) future scenario simulations to project how the Earth system will respond to anthropogenic activity over the 21st century and beyond. This paper documents in detail these simulations, explains their rationale and planned analysis, and describes how to set up and run the simulations. Particular attention is paid to boundary conditions, input data, and requested output diagnostics. It is important that modelling groups participating in C4MIP adhere as closely as possible to this experimental design. C1 [Jones, Chris D.] Met Off Hadley Ctr, Exeter EX1 3PB, Devon, England. [Arora, Vivek] Canadian Ctr Climate Modelling & Anal, Div Climate Res, Environm & Climate Change, Victoria, BC, Canada. [Friedlingstein, Pierre] Univ Exeter, Coll Engn Math & Phys Sci, Exeter EX4 4QE, Devon, England. [Bopp, Laurent] Univ Paris Saclay, LSCE, IPSL, CEA,CNRS,UVSQ, F-91191 Gif Sur Yvette, France. [Brovkin, Victor; Ilyina, Tatiana; Pongratz, Julia; Raddatz, Thomas] Max Planck Inst Meteorol, Hamburg, Germany. [Dunne, John; John, Jasmin G.] NOAA, GFDL, Princeton, NJ USA. [Graven, Heather] Imperial Coll London, Dept Phys, London, England. [Graven, Heather] Imperial Coll London, Grantham Inst, London, England. [Hoffman, Forrest] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Jung, Martin; Zaehle, Soenke] Max Planck Inst Biogeochem, Biogeochem Integrat Dept, D-07745 Jena, Germany. [Kawamiya, Michio] Japan Agcy Marine Earth Sci & Technol, Yokosuka, Kanagawa, Japan. [Koven, Charlie] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Randerson, James T.] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA USA. RP Jones, CD (reprint author), Met Off Hadley Ctr, Exeter EX1 3PB, Devon, England. EM chris.d.jones@metoffice.gov.uk RI Brovkin, Victor/C-2803-2016; Hoffman, Forrest/B-8667-2012; Jones, Chris/I-2983-2014; Koven, Charles/N-8888-2014; Zaehle, Sonke/C-9528-2017 OI Brovkin, Victor/0000-0001-6420-3198; Hoffman, Forrest/0000-0001-5802-4134; Koven, Charles/0000-0002-3367-0065; Zaehle, Sonke/0000-0001-5602-7956 FU European Union [641816]; Joint UK BEIS/Defra Met Office Hadley Centre Climate Programme [GA01101]; European Commission; German Research Foundation [PO 1751/1-1] FX CRESCENDO project members (CDJ, PF, LB, VB, TI, SZ) acknowledge funding received from the Horizon 2020 European Union's Framework Programme for Research and Innovation under grant agreement no. 641816. CDJ was supported by the Joint UK BEIS/Defra Met Office Hadley Centre Climate Programme (GA01101). HDG was supported by a Marie Curie Career Integration Grant from the European Commission. JP is supported by the German Research Foundation's Emmy Noether Program (PO 1751/1-1). NR 104 TC 3 Z9 3 U1 13 U2 14 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X EI 1991-9603 J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PD AUG 25 PY 2016 VL 9 IS 8 BP 2853 EP 2880 DI 10.5194/gmd-9-2853-2016 PG 28 WC Geosciences, Multidisciplinary SC Geology GA DW7PX UT WOS:000383844500002 ER PT J AU Jacobitz, AW Naziga, EB Yi, SW McConnell, SA Peterson, R Jung, ME Clubb, RT Wereszczynski, J AF Jacobitz, Alex W. Naziga, Emmanuel B. Yi, Sung Wook McConnell, Scott A. Peterson, Robert Jung, Michael E. Clubb, Robert T. Wereszczynski, Jeff TI The "Lid" in the Streptococcus pneumoniae SrtC1 Sortase Adopts a Rigid Structure that Regulates Substrate Access to the Active Site SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID GRAM-POSITIVE BACTERIA; STAPHYLOCOCCUS-AUREUS SORTASE; MOLECULAR-DYNAMICS SIMULATIONS; PARTICLE MESH EWALD; BIOFILM DEVELOPMENT; CORYNEBACTERIUM-DIPHTHERIAE; ACTINOMYCES-ORIS; PROTEIN DYNAMICS; SORTING SIGNAL; PILI AB Many species of Grain-positive bacteria use sortase enzymes to assemble long, proteinaceous pili structures that project from the cell surface to mediate microbial adhesion. Sortases construct highly stable structures by catalyzing a transpeptidation reaction that covalently links pilin subunits together via isopeptide bonds. Most Gram-positive pili are assembled by class C sortases that contain a "lid", a structurally unique N-terminal extension that occludes the active site. It has been hypothesized that the "lid" in many sortases is mobile and thus capable of readily being displaced from the enzyme to facilitate substrate binding. Here, we show using NMR dynamics measurements, in vitro assays, and molecular dynamics simulations that the lid in the class C sortase from Streptococcus pneumoniae (SrtC1) adopts a rigid conformation in solution that is devoid of large magnitude conformational excursions that occur on mechanistically relevant time scales. Additionally, we show that point mutations in the lid induce dynamic behavior that correlates with increased hydrolytic activity and sorting signal substrate access to the active site cysteine residue. These results suggest that the lid of the S. pneumoniae SrtC1 enzyme has a negative regulatory function and imply that a significant energetic barrier must be surmounted by currently unidentified factors to dislodge it from the active site to initiate pilus biogenesis. C1 [Jacobitz, Alex W.; Yi, Sung Wook; McConnell, Scott A.; Peterson, Robert; Jung, Michael E.; Clubb, Robert T.] Univ Calif Los Angeles, Dept Chem & Biochem, 611 Charles E Young Dr East, Los Angeles, CA 90095 USA. [Jacobitz, Alex W.; Yi, Sung Wook; McConnell, Scott A.; Peterson, Robert; Jung, Michael E.; Clubb, Robert T.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, 611 Charles E Young Dr East, Los Angeles, CA 90095 USA. [Naziga, Emmanuel B.; Wereszczynski, Jeff] Illinois Inst Technol, Dept Phys, 3440 South Dearborn St, Chicago, IL 60616 USA. [Naziga, Emmanuel B.; Wereszczynski, Jeff] Illinois Inst Technol, Ctr Mol Study Condensed Soft Matter, 3440 South Dearborn St, Chicago, IL 60616 USA. RP Clubb, RT (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 611 Charles E Young Dr East, Los Angeles, CA 90095 USA.; Clubb, RT (reprint author), Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, 611 Charles E Young Dr East, Los Angeles, CA 90095 USA.; Wereszczynski, J (reprint author), Illinois Inst Technol, Dept Phys, 3440 South Dearborn St, Chicago, IL 60616 USA.; Wereszczynski, J (reprint author), Illinois Inst Technol, Ctr Mol Study Condensed Soft Matter, 3440 South Dearborn St, Chicago, IL 60616 USA. EM rclubb@mbi.ucla.edu; jwereszc@iit.edu FU National Institutes of Health Grants [K22AI104799, AI52217]; U.S. Department of Energy Office of Science, Office of Biological and Environmental Research program [DE-FC02-02ER63421]; National Science Foundation Grant [ACI-1053575] FX This work was supported, in whole or in part, by National Institutes of Health Grants K22AI104799 (to J.W.) and AI52217 (to R.T.C.) as well as funding from the U.S. Department of Energy Office of Science, Office of Biological and Environmental Research program under Award Number DE-FC02-02ER63421. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant ACI-1053575. NR 57 TC 0 Z9 0 U1 4 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8302 EP 8312 DI 10.1021/acs.jpcb.6b01930 PG 11 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200024 PM 27109553 ER PT J AU Clark, AK Wilder, JH Grayson, AW Johnson, QR Lindsay, RJ Nellas, RB Fernandez, EJ Shen, TY AF Clark, Alexander K. Wilder, J. Heath Grayson, Aaron W. Johnson, Quentin R. Lindsay, Richard J. Nellas, Ricky B. Fernandez, Elias J. Shen, Tongye TI The Promiscuity of Allosteric Regulation of Nuclear Receptors by Retinoid X Receptor SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID LIGAND-BINDING DOMAIN; STRUCTURAL DETERMINANTS; NEGATIVE COOPERATIVITY; COMMUNICATION; HETERODIMERS; RECOGNITION; SUPERFAMILY; HEMOGLOBIN; ACTIVATION; MECHANISM AB The promiscuous protein retinoid X receptor (RXR) displays essential allosteric regulation of several members in the nuclear hormone receptor superfamily via heterodimerization and (anti)cooperative binding of cognate ligands. Here, the structural basis of the positive allostery of RXR and constitutive androstane receptor (CAR) is revealed. In contrast, a similar computational approach had previously revealed the mechanism for negative allostery in the complex of RXR and thyroid receptor (TR). By comparing the positive and negative allostery of RXR complexed with CAR and TR respectively, we reported the promiscuous allosteric control involving RXR. We characterize the allosteric mechanism by expressing the correlated dynamics of selected residue residue contacts which was extracted from atomistic molecular dynamics simulation and statistical analysis. While the same set of residues in the binding pocket of RXR may initiate the residue residue interaction network, RXR. uses largely different sets of contacts (only about one-third identical) and allosteric modes to regulate TR and CAR The promiscuity of RXR control may originate from multiple factors, including (1) the frustrated fit of cognate ligand 9c to the RXR binding pocket and (2) the different ligand-binding features of TR (loose) versus CAR (tight) to their corresponding cognate ligands. C1 [Clark, Alexander K.; Wilder, J. Heath; Grayson, Aaron W.; Lindsay, Richard J.; Fernandez, Elias J.; Shen, Tongye] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. [Johnson, Quentin R.] Univ Tennessee, Natl Inst Math & Biol Synth, Knoxville, TN 37996 USA. [Johnson, Quentin R.; Lindsay, Richard J.; Shen, Tongye] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA. [Nellas, Ricky B.] Univ Philippines Diliman, Inst Chem, Quezon City, Philippines. RP Shen, TY (reprint author), Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA.; Shen, TY (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA. EM tshen@utk.edu FU JDRD program of Science Alliance at UT-ORNL; NIH [DK097337-01] FX Computational support was provided in part by NICS and by the ORNL-UT Center for Molecular Biophysics and by allocations of advanced computing resources (TG-MCB120011) on STAMPEDE at the National Institute for Computational Sciences. Support from JDRD program of Science Alliance at UT-ORNL is acknowledged. E.J.F. is supported by NIH (No. DK097337-01). NR 40 TC 0 Z9 0 U1 3 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8338 EP 8345 DI 10.1021/acs.jpcb.6b02057 PG 8 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200027 PM 27110634 ER PT J AU Purvine, E Monson, K Jurrus, E Star, K Baker, NA AF Purvine, Emilie Monson, Kyle Jurrus, Elizabeth Star, Keith Baker, Nathan A. TI Energy Minimization of Discrete Protein Titration State Models Using Graph Theory SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MONTE-CARLO-MINIMIZATION; DEAD-END ELIMINATION; MOLECULAR-DYNAMICS; SIDE-CHAIN; FOLDING PROBLEM; PROTONATION; DESIGN; ELECTROSTATICS; PK(A)S; CUTS AB There are several applications in computational biophysics that require the optimization of discrete interacting states, for example, amino acid titration states, ligand oxidation states, or discrete rotamer angles. Such optimization can be very time-consuming as it scales exponentially in the number of sites to be optimized. In this paper, we describe a new polynomial time algorithm for optimization of discrete states in macromolecular systems. This algorithm was adapted from image processing and uses techniques from discrete mathematics and graph theory to restate the optimization problem in terms of "maximum flow-minimum cut" graph analysis. The interaction energy graph, a graph in which vertices (amino acids) and edges (interactions) are weighted with their respective energies, is transformed into a flow network in which the value of the minimum cut in the network equals the minimum free energy of the protein and the cut itself encodes the state that achieves the minimum free energy. Because of its deterministic nature and polynomial time performance, this algorithm has the potential to allow for the ionization state of larger proteins to be discovered. C1 [Purvine, Emilie; Monson, Kyle; Jurrus, Elizabeth; Star, Keith] Pacific Northwest Natl Lab, Computat & Stat Analyt Div, Richland, WA 99354 USA. [Baker, Nathan A.] Pacific Northwest Natl Lab, Adv Comp Math & Data Div, Richland, WA 99354 USA. [Baker, Nathan A.] Brown Univ, Div Appl Math, Providence, RI 02912 USA. RP Purvine, E; Monson, K; Jurrus, E; Star, K (reprint author), Pacific Northwest Natl Lab, Computat & Stat Analyt Div, Richland, WA 99354 USA.; Baker, NA (reprint author), Pacific Northwest Natl Lab, Adv Comp Math & Data Div, Richland, WA 99354 USA.; Baker, NA (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA. EM emilie.purvine@pnnl.gov; kyle.monson@pnnl.gov; elizabeth.jurrus@pnnl.gov; keith@pnnl.gov; nathan.baker@pnnl.gov FU NIH [GM069702]; National Biomedical Computation Resource (NIH) [RR008605] FX We gratefully acknowledge NIH Grant GM069702 for support of this research, Dr. Jens Nielsen for his work on PDB2PKA, and the National Biomedical Computation Resource (NIH Grant RR008605) for computational support. NR 56 TC 0 Z9 0 U1 3 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8354 EP 8360 DI 10.1021/acs.jpcb.6b02059 PG 7 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200029 PM 27089174 ER PT J AU Tian, JH Nickels, J Katsaras, J Cheng, XL AF Tian, Jianhui Nickels, Jonathan Katsaras, John Cheng, Xiaolin TI Behavior of Bilayer Leaflets in Asymmetric Model Membranes: Atomistic Simulation Studies SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; RED-BLOOD-CELLS; LIPID RAFTS; BIOLOGICAL-MEMBRANES; PLASMA-MEMBRANES; FORCE-FIELD; SPHINGOMYELIN BILAYERS; LATERAL DIFFUSION; MODULATED PHASES; APOPTOTIC CELLS AB Spatial organization within lipid bilayers is an important feature for a range of biological processes. Leaflet compositional asymmetry and lateral lipid organization are just two of the ways in which membrane structure appears to be more complex than initially postulated by the fluid mosaic model. This raises the question of how the phase behavior in one bilayer leaflet may affect the apposing leaflet and how one begins to construct asymmetric model systems to investigate these interleaflet interactions. Here we report on all-atom molecular dynamics simulations (a total of 4.1 mu s) of symmetric and asymmetric bilayer systems composed of liquid-ordered (Lo) or liquid-disordered (Ld) leaflets, based on the nanodomain-forming POPC/DSPC/cholesterol system. We begin by analyzing an asymmetric bilayer with leaflets derived from simulations of symmetric Lo and Ld bilayers. In this system, we observe that the properties of the Lo and Ld leaflets corresponding symmetric systems. However, it is not obvious that mixing the equilibrium structures of their symmetric counterparts is the most appropriate way to construct asymmetric bilayers nor that these structures will manifest interleaflet couplings that lead to domain registry/antiregistry. We therefore constructed and simulated four additional asymmetric bilayer systems by systematically adding or removing lipids in the Ld leaflet to mimic potential density fluctuations. We find that the number of lipids in the Ld leaflet affects its own properties, as well as those of the apposing Lo leaflet. Collectively, the simulations reveal the presence of weak acyl chain interdigitation across bilayer leaflets, suggesting that interdigitation alone does not contribute significantly to the interleaflet coupling in nonphase-separated bilayers of this chemical composition. However, the properties of both leaflets appear to be sensitive to changes in in-plane lipid packing, possibly providing a mechanism for interleaflet coupling by modulating local density and/or curvature fluctuations. C1 [Tian, Jianhui; Cheng, Xiaolin] Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. [Nickels, Jonathan; Katsaras, John] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Nickels, Jonathan; Katsaras, John] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Katsaras, John] Bredesen Ctr Interdisciplinary Res & Grad Educ, 444 Greve Hall,821 Volunteer Blvd, Knoxville, TN 37996 USA. RP Cheng, XL (reprint author), Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37831 USA. EM chengx@ornl.gov RI Nickels, Jonathan/I-1913-2012 OI Nickels, Jonathan/0000-0001-8351-7846 FU Laboratory Directed R&D (LDRD) Fund at the Oak Ridge National Laboratory; Scientific User Facilities Division of the DOE Office of Basic Energy Sciences (BES) [DE-AC05 00OR2275]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX J.T. and X.C. are partially supported by the Laboratory Directed R&D (LDRD) Fund at the Oak Ridge National Laboratory. J.K. is supported through the Scientific User Facilities Division of the DOE Office of Basic Energy Sciences (BES), under Contract No. DE-AC05 00OR2275. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 78 TC 1 Z9 1 U1 38 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8438 EP 8448 DI 10.1021/acs.jpcb.6b02148 PG 11 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200037 PM 27121138 ER PT J AU Goliaei, A Lau, EY Adhikari, U Schwegler, E Berkowitz, ML AF Goliaei, Ardeshir Lau, Edmond Y. Adhikari, Upendra Schwegler, Eric Berkowitz, Max L. TI Behavior of P85 and P188 Poloxamer Molecules: Computer Simulations Using United-Atom Force-Field SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID PEO TRIBLOCK COPOLYMERS; PARTICLE MESH EWALD; BLOCK-COPOLYMERS; DYNAMICS SIMULATIONS; SOFT MATTER; MEMBRANES; SYSTEMS; SURFACTANTS; PEROXIDATION; INTERFACES AB To study the interaction between poloxamer molecules and lipid bilayers using molecular dynamics simulation technique with the united-atom resolution, we augmented the GROMOS force-field to include poloxamers. We validated the force-field by calculating the radii of gyration of two poloxamers,P85 and P188, solvated in water and by considering the poloxamer density distributions at the air/water interface. The emphasis of our simulations was on the study of the interaction between poloxamers and lipid bilayer. At the water/lipid bilayer interface, we observed that both poloxamers studied, P85 and P188, behaved like surfactants: the hydrophilic blocks of poloxamers became adsorbed at the polar interface, while their hydrophobic block penetrated the interface into the aliphatic tail region of the lipid bilayer. We also observed that when P85 and P188 poloxamers interacted with damaged membranes that contained pores, the hydrophobic blocks of copolymers penetrated into the membrane in the vicinity of the pore and compressed the membrane. Due to this compression, water molecules were evacuated from the pore. C1 [Adhikari, Upendra; Berkowitz, Max L.] Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA. [Goliaei, Ardeshir] Univ N Carolina, Dept Biochem & Biophys, Chapel Hill, NC 27599 USA. [Goliaei, Ardeshir] Univ N Carolina, Program Mol & Cellular Biophys, Chapel Hill, NC 27599 USA. [Lau, Edmond Y.; Schwegler, Eric] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Berkowitz, ML (reprint author), Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA. EM maxb@unc.edu FU Office of Naval Research [N00014-14-1-0241]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The support by Grant N00014-14-1-0241 from the Office of Naval Research is gratefully acknowledged. Work at the Lawrence Livermore National Laboratory (LLNL) was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Computing support for this work at LLNL came from the LLNL Institutional Computing Grand Challenge program. The authors (A.G., U.A., M.L.B.) would like to thank Professor Kabanov for useful discussions. NR 63 TC 0 Z9 0 U1 5 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8631 EP 8641 DI 10.1021/acs.jpcb.6b03030 PG 11 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200054 PM 27232763 ER PT J AU Bascom, GD Sanbonmatsu, KY Schlick, T AF Bascom, Gavin D. Sanbonmatsu, Karissa Y. Schlick, Tamar TI Mesoscale Modeling Reveals Hierarchical Looping of Chromatin Fibers Near Gene Regulatory Elements SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MESOSCOPIC OLIGONUCLEOSOME MODEL; LONG-RANGE INTERACTIONS; HIGHER-ORDER STRUCTURES; BETA-GLOBIN LOCUS; HISTONE TAILS; GENOME-WIDE; NUCLEOSOME POSITIONS; DNA; TRANSCRIPTION; EXPRESSION AB While it is well-recognized that chromatin loops play an important role in gene regulation, structural details regarding higher order chromatin loops are only emerging. Here we present a systematic study of restrained chromatin loops ranging from 25 to 427 nucleosomes (fibers of 580 Kb DNA in length), mimicking gene elements studied by 3C contact data. We find that hierarchical looping represents a stable configuration that can effectively bring distant regions of the GATA-4 gene together, satisfying connections reported by 3C experiments. Additionally, we find that restrained chromatin fibers larger than 100 nucleosomes (similar to 20Kb) form closed plectonemes, whereas fibers shorter than 100 nucleosomes form simple hairpin loops. By studying the dependence of loop structures on internal parameters, we show that loop features are sensitive to linker histone concentration, loop length, divalent ions, and DNA linker length. Specifically, increasing loop length, linker histone concentration, and divalent ion concentration are associated with increased persistence length (or decreased bending), while varying DNA linker length in a manner similar to experimentally observed "nucleosome free regions" (found near transcription start sites) disrupts intertwining and leads to loop opening and increased persistence length in linker histone depleted (-LH) fibers. Chromatin fiber structure sensitivity to these parameters, all of which vary throughout the cell cycle, tissue type, and species, suggests that caution is warranted when using uniform polymer models to fit chromatin conformation capture genome-wide data. Furthermore, the folding geometry we observe near the transcription initiation site of the GATA-4 gene suggests that hierarchical looping provides a structural mechanism for gene inhibition, and offers tunable parameters for design of gene regulation elements. C1 [Bascom, Gavin D.; Schlick, Tamar] NYU, Dept Chem, 100 Washington Sq East, New York, NY 10003 USA. [Sanbonmatsu, Karissa Y.] Los Alamos Natl Lab, Div Theoret, Theoret Biol & Biophys Grp, Bikini Atoll Rd,SM 30, Los Alamos, NM 87545 USA. [Schlick, Tamar] NYU, Courant Inst Math Sci, 251 Mercer St, New York, NY 10012 USA. RP Schlick, T (reprint author), NYU, Dept Chem, 100 Washington Sq East, New York, NY 10003 USA.; Schlick, T (reprint author), NYU, Courant Inst Math Sci, 251 Mercer St, New York, NY 10012 USA. EM schlick@nyu.edu FU National Institutes of Health [R01-055164]; Phillip-Morris USA; Phillip-Morris International; LANL LDRD FX This work was supported by the National Institutes of Health Grant R01-055164 to T.S., and Phillip-Morris USA and Phillip-Morris International to T.S. K.Y.S. was supported by LANL LDRD. We also thank Dr. Sergei Grigoryev for his invaluable comments and discussion regarding this paper. Computing was performed on the New York University HPC cluster Mercer and Los Alamos National Lab Institutional Computing resources. We also thank LANL staff for valuable direction regarding parallel resources. NR 73 TC 4 Z9 4 U1 3 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8642 EP 8653 DI 10.1021/acs.jpcb.6b03197 PG 12 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200055 PM 27218881 ER PT J AU Li, A Voronin, A Fenley, AT Gilson, MK AF Li, Amanda Voronin, Alexey Fenley, Andrew T. Gilson, Michael K. TI Evaluation of Representations and Response Models for Polarizable Force Fields SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; CLASSICAL DRUDE OSCILLATOR; ATOMIC CHARGES; FREE-ENERGIES; DIPOLE INTERACTION; NUCLEIC-ACIDS; LIQUID WATER; BASIS-SETS; SOLVATION; MECHANICS AB For classical simulations of condensed-phase systems, such as organic liquids and biomolecules, to achieve high accuracy, they will probably need to incorporate an accurate, efficient model of conformation-dependent electronic polarization. Thus, it is of interest to understand what determines the accuracy of a polarizable electrostatics model. This study approaches this problem by breaking polarization models down into two main components: the representation of electronic polarization and the response model used for mapping from an inducing field to the polarization within the chosen representation. Among the most common polarization representations are redistribution of atom-centered charges, such as those used in the fluctuating charge model, and atom-centered point dipoles, such as those used in a number of different polarization models. Each of these representations has been combined with one or more response models. The response model of fluctuating charge, for example, is based on the idea of electronegativity equalization in the context of changing electrostatic potentials (ESPs), whereas point-dipole representations typically use a response model based on point polarizabilities whose induced dipoles are computed based on interaction with other charges and dipoles. Here, we decouple polarization representations from their typical response models to analyze the strengths and weaknesses of various polarization approximations. First, we compare the maximal possible accuracies achievable by the charge redistribution and point-dipole model representations, by testing their ability to replicate quantum mechanical (QM) ESPs around small molecules polarized by external inducing charges. Perhaps not surprisingly, the atom-centered dipole model can yield higher accuracy. Next, we test two of the most commonly used response functions used for the point-dipole representations, self consistent and direct (or first-order) inducible point polarizabilities, where the polarizabilities are optimized to best fit the full set of polarized QM potentials for each molecule studied. Strikingly, the induced-dipole response model markedly degrades accuracy relative to that obtainable with optimal point dipoles. In fact, the maximal accuracy achievable with this response model is even lower than that afforded by an optimal charge-redistribution representation. This means that, if coupled with a sufficiently accurate response function, the point-charge representation could outperform the standard induced-dipole model. Furthermore, although a key advantage of the point-dipole representation, relative to charge redistribution, is its ability to capture out-of-plane polarization, the inducible dipole response model causes it to be less accurate than optimal charge redistribution for out-of-plane induction of the planar nitrobenzene molecule. Thus, the widely used inducible dipole response function falls short of the full potential accuracy achievable with the point-dipole representation it employs. Additional results reported here bear on the relative accuracy of self-consistent inducible dipoles versus that of the first-order, or direct, approximation and on methods for assigning partial atomic charges for use in conjunction with inducible dipole models. In sum, these results point to the improvement of polarization response models as an important direction for future research aimed at improving the accuracy of molecular simulations. C1 [Li, Amanda] Univ Calif San Diego, Dept Bioengn, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Voronin, Alexey; Fenley, Andrew T.; Gilson, Michael K.] Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Voronin, Alexey] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Gilson, MK (reprint author), Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM mgilson@ucsd.edu FU National Institutes of Health (NIH) [GM061300] FX We thank Prof. Jan Jensen and an anonymous reviewer for valuable questions and comments that led to improvements in the present analysis. We also thank the National Institutes of Health (NIH) for grant GM061300. The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of the NIH. Computational support was provided through the Triton Shared Computing Cluster, a research computing system operated by the San Diego Supercomputer Center for UC San Diego researchers and affiliates. NR 53 TC 1 Z9 1 U1 5 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8668 EP 8684 DI 10.1021/acs.jpcb.6b03392 PG 17 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200057 PM 27248842 ER PT J AU Jo, S Suh, D He, ZW Chipot, C Roux, B AF Jo, Sunhwan Suh, Donghyuk He, Ziwei Chipot, Christophe Roux, Benoit TI Leveraging the Information from Markov State Models To Improve the Convergence of Umbrella Sampling Simulations SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID HISTOGRAM ANALYSIS METHOD; FREE-ENERGY CALCULATIONS; ADAPTIVE BIASING FORCE; MOLECULAR-DYNAMICS; AVERAGE FORCE; LANDSCAPE; ERROR; NAMD AB Umbrella sampling (US) simulation is a highly effective method for sampling the conformations of a complex system within a small subspace of predefined coordinates. In a typical US stratification strategy, biasing "window" potentials spanning the subspace of interest are introduced to narrow down the range of accessible conformations and accelerate the sampling. The speed of convergence in each biased window simulation may, however, differ. For example, windows that coincide with a large energetic barrier along a coordinate that is orthogonal to the predefined subspace are often plagued by slow relaxation timescales. Here, we design a method that can quantitatively detect this type of issue and gain further insight into the origin of the slow relaxation timescale. Once the problematic windows affected by slow convergence are identified, additional simulations limited to only these windows can be carried out, thereby reducing the overall computational effort. Several possible approaches aimed at performing US simulations adaptively are discussed, and their respective performance is illustrated using a simple model system. Last, simulations of an atomic deca-alanine system are used to demonstrate the efficacy of analyzing US simulation trajectories using the proposed method. C1 [Jo, Sunhwan] Argonne Natl Lab, Leadership Comp Facil, 9700 Cass Ave,Bldg 240, Argonne, IL 60439 USA. [Suh, Donghyuk; He, Ziwei] Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. [Chipot, Christophe] CNRS, Lab Int Associe, BP 70239, F-54506 Vandoeuvre Les Nancy, France. [Chipot, Christophe] Univ Lorraine, Univ Illinois Urbana Champaign, UMR 7565, BP 70239, F-54506 Vandoeuvre Les Nancy, France. [Chipot, Christophe] Univ Illinois, Dept Phys, 1110 West Green St,405 North Mathews, Urbana, IL 61801 USA. [Chipot, Christophe] Univ Illinois, Beckman Inst Adv Res & Technol, 1110 West Green St,405 North Mathews, Urbana, IL 61801 USA. [Roux, Benoit] Univ Chicago, Gordon Ctr Integrat Sci, Dept Biochem & Mol Biol, Chicago, IL 60637 USA. [Roux, Benoit] Argonne Natl Lab, Ctr Nanomat, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Roux, B (reprint author), Univ Chicago, Gordon Ctr Integrat Sci, Dept Biochem & Mol Biol, Chicago, IL 60637 USA.; Roux, B (reprint author), Argonne Natl Lab, Ctr Nanomat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM roux@uchicago.edu FU DOE Oce of Science User Facility [DE-AC02-06CH11357]; Computational Post- doctoral Fellowship from ALCF; National Science Foundation [MCB-1517221]; France and Chicago Collaborating in the Sciences (FACCTS) Center of the University of Chicago FX The authors would like to acknowledge Frank Noe and Christoph Wehmeyer at Freie Universitaet Berlin for helpful discussions and comments. We also thank Wonpil Im and Soohyung Park at the University of Kansas for helpful comments. This research used resources of the Argonne Leadership Computing Facility (ALCF), which is a DOE Oce of Science User Facility supported under Contract DE-AC02-06CH11357, an award of computer time provided by the INCITE program. We also gratefully acknowledge the computing resources provided by Argonne's Laboratory Computing Resource Center (LCRC). S.J. is supported by a Computational Post- doctoral Fellowship from ALCF. This work is supported by grant MCB-1517221 from the National Science Foundation and by the France and Chicago Collaborating in the Sciences (FACCTS) Center of the University of Chicago. NR 40 TC 0 Z9 0 U1 6 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD AUG 25 PY 2016 VL 120 IS 33 BP 8733 EP 8742 DI 10.1021/acs.jpcb.6b05125 PG 10 WC Chemistry, Physical SC Chemistry GA DU4JZ UT WOS:000382180200062 PM 27409349 ER PT J AU Paez-Espino, D Eloe-Fadrosh, EA Pavlopoulos, GA Thomas, AD Huntemann, M Mikhailova, N Rubin, E Ivanova, NN Kyrpides, NC AF Paez-Espino, David Eloe-Fadrosh, Emiley A. Pavlopoulos, Georgios A. Thomas, Alex D. Huntemann, Marcel Mikhailova, Natalia Rubin, Edward Ivanova, Natalia N. Kyrpides, Nikos C. TI Uncovering Earth's virome SO NATURE LA English DT Article ID NUCLEOTIDE-SEQUENCES; PROTEIN FAMILIES; MARINE VIRUSES; PHAGE; BACTERIOPHAGE; SYSTEM; BLAST; GENE; TOOL; CLASSIFICATION AB Viruses are the most abundant biological entities on Earth, but challenges in detecting, isolating, and classifying unknown viruses have prevented exhaustive surveys of the global virome. Here we analysed over 5 Tb of metagenomic sequence data from 3,042 geographically diverse samples to assess the global distribution, phylogenetic diversity, and host specificity of viruses. We discovered over 125,000 partial DNA viral genomes, including the largest phage yet identified, and increased the number of known viral genes by 16-fold. Half of the predicted partial viral genomes were clustered into genetically distinct groups, most of which included genes unrelated to those in known viruses. Using CRISPR spacers and transfer RNA matches to link viral groups to microbial host(s), we doubled the number of microbial phyla known to be infected by viruses, and identified viruses that can infect organisms from different phyla. Analysis of viral distribution across diverse ecosystems revealed strong habitat-type specificity for the vast majority of viruses, but also identified some cosmopolitan groups. Our results highlight an extensive global viral diversity and provide detailed insight into viral habitat distribution and host-virus interactions. C1 [Paez-Espino, David; Eloe-Fadrosh, Emiley A.; Pavlopoulos, Georgios A.; Thomas, Alex D.; Huntemann, Marcel; Mikhailova, Natalia; Rubin, Edward; Ivanova, Natalia N.; Kyrpides, Nikos C.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Rubin, Edward] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rubin, Edward] Metabiota Inc, San Francisco, CA 94104 USA. RP Kyrpides, NC (reprint author), Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. EM nckyrpides@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231]; Office of Science of US Department of Energy FX We thank A. Visel and H. Maughan for critical reading and feedback, A. Pati for help in earlier versions, and the IMG and GOLD teams for their support. This work was conducted by the US Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, under contract number DE-AC02-05CH11231 and used resources of the National Energy Research Scientific Computing Center, supported by the Office of Science of the US Department of Energy. NR 65 TC 14 Z9 14 U1 24 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 25 PY 2016 VL 536 IS 7617 BP 425 EP + DI 10.1038/nature19094 PG 21 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DV0YL UT WOS:000382646600035 PM 27533034 ER PT J AU Chen, CC Muechler, L Car, R Neupert, T Maciejko, J AF Chen, Cheng-Chien Muechler, Lukas Car, Roberto Neupert, Titus Maciejko, Joseph TI Fermionic Symmetry-Protected Topological Phase in a Two-Dimensional Hubbard Model SO PHYSICAL REVIEW LETTERS LA English DT Article ID INSULATORS; SYSTEMS AB We study the two-dimensional (2D) Hubbard model using exact diagonalization for spin-1/2 fermions on the triangular and honeycomb lattices decorated with a single hexagon per site. In certain parameter ranges, the Hubbard model maps to a quantum compass model on those lattices. On the triangular lattice, the compass model exhibits collinear stripe antiferromagnetism, implying d-density wave charge order in the original Hubbard model. On the honeycomb lattice, the compass model has a unique, quantum disordered ground state that transforms nontrivially under lattice reflection. The ground state of the Hubbard model on the decorated honeycomb lattice is thus a 2D fermionic symmetry-protected topological phase. This state-protected by time-reversal and reflection symmetries-cannot be connected adiabatically to a free-fermion topological phase. C1 [Chen, Cheng-Chien] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Chen, Cheng-Chien] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Muechler, Lukas; Car, Roberto] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Neupert, Titus] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA. [Maciejko, Joseph] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Maciejko, Joseph] Univ Alberta, Inst Theoret Phys, Edmonton, AB T6G 2E1, Canada. [Maciejko, Joseph] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. RP Chen, CC (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.; Chen, CC (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RI Neupert, Titus/K-8733-2012 OI Neupert, Titus/0000-0003-0604-041X FU Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory; U.S. DOE [DE-FG02-05ER46201, DE-AC02-05CH11231]; NSERC [RGPIN-2014-4608]; Canada Research Chair Program (CRC); Canadian Institute for Advanced Research (CIFAR); University of Alberta; [DE-AC02-06CH11357] FX The authors acknowledge discussions with B. Bauer, K. Penc, H.-C. Jiang, and T. F. Seman. C.-C. C. was supported by the Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory, operated by the U.S. Department of Energy (DOE) under Contract No. DE-AC02-06CH11357. L. M. and R. C. were supported by U.S. DOE Contract No. DE-FG02-05ER46201. J. M. was supported by NSERC Grant No. RGPIN-2014-4608, the Canada Research Chair Program (CRC), the Canadian Institute for Advanced Research (CIFAR), and the University of Alberta. This research used resources of the National Energy Research Scientific Computing Center, supported by U.S. DOE Contract No. DE-AC02-05CH11231. NR 38 TC 0 Z9 0 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 25 PY 2016 VL 117 IS 9 AR 096405 DI 10.1103/PhysRevLett.117.096405 PG 5 WC Physics, Multidisciplinary SC Physics GA DU1ZA UT WOS:000382008400008 PM 27610869 ER PT J AU Jara-Almonte, J Ji, HT Yamada, M Yoo, J Fox, W AF Jara-Almonte, Jonathan Ji, Hantao Yamada, Masaaki Yoo, Jongsoo Fox, William TI Laboratory Observation of Resistive Electron Tearing in a Two-Fluid Reconnecting Current Sheet SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETIC RECONNECTION; MODE-INSTABILITY; CHALLENGE AB The spontaneous formation of plasmoids via the resistive electron tearing of a reconnecting current sheet is observed in the laboratory. These experiments are performed during driven, antiparallel reconnection in the two-fluid regime within the Magnetic Reconnection Experiment. It is found that plasmoids are present even at a very low Lundquist number, and the number of plasmoids scales with both the current sheet aspect ratio and the Lundquist number. The reconnection electric field increases when plasmoids are formed, leading to an enhanced reconnection rate. C1 [Jara-Almonte, Jonathan; Ji, Hantao; Yamada, Masaaki; Yoo, Jongsoo; Fox, William] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Jara-Almonte, J (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. EM jjaraalm@pppl.gov FU NASA [NNH15AB29I, NNH14AX631]; DOE [DE-AC0209CH11466] FX This work is supported by NASA under Agreements No. NNH15AB29I and No. NNH14AX631, as well as by the DOE under Contract No. DE-AC0209CH11466. The authors thank W. Daughton for helpful discussions regarding the structure of Hall-MHD current sheets, as well as R. Cutler for technical support. NR 36 TC 4 Z9 4 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 25 PY 2016 VL 117 IS 9 AR 095001 DI 10.1103/PhysRevLett.117.095001 PG 5 WC Physics, Multidisciplinary SC Physics GA DU1ZA UT WOS:000382008400007 PM 27610861 ER PT J AU Huang, PX Nedelcu, D Watanabe, M Jao, C Kim, Y Liu, J Salic, A AF Huang, Pengxiang Nedelcu, Daniel Watanabe, Miyako Jao, Cindy Kim, Youngchang Liu, Jing Salic, Adrian TI Cellular Cholesterol Directly Activates Smoothened in Hedgehog Signaling SO CELL LA English DT Article ID PRIMARY CILIUM; PROTEIN; CELLS; RECEPTOR; PATHWAY; BINDING; OXYSTEROLS; MODULATION; MECHANISM; COMPLEX AB In vertebrates, sterols are necessary for Hedgehog signaling, a pathway critical in embryogenesis and cancer. Sterols activate the membrane protein Smoothened by binding its extracellular, cysteine-rich domain (CRD). Major unanswered questions concern the nature of the endogenous, activating sterol and the mechanism by which it regulates Smoothened. We report crystal structures of CRD complexed with sterols and alone, revealing that sterols induce a dramatic conformational change of the binding site, which is sufficient for Smoothened activation and is unique among CRD-containing receptors. We demonstrate that Hedgehog signaling requires sterol binding to Smoothened and define key residues for sterol recognition and activity. We also show that cholesterol itself binds and activates Smoothened. Furthermore, the effect of oxysterols is abolished in Smoothened mutants that retain activation by cholesterol and Hedgehog. We propose that the endogenous Smoothened activator is cholesterol, not oxysterols, and that vertebrate Hedgehog signaling controls Smoothened by regulating its access to cholesterol. C1 [Huang, Pengxiang; Nedelcu, Daniel; Watanabe, Miyako; Jao, Cindy; Liu, Jing; Salic, Adrian] Harvard Med Sch, Dept Cell Biol, 240 Longwood Ave, Boston, MA 02115 USA. [Kim, Youngchang] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. RP Salic, A (reprint author), Harvard Med Sch, Dept Cell Biol, 240 Longwood Ave, Boston, MA 02115 USA. EM asalic@hms.harvard.edu OI liu, jing/0000-0001-9513-3591 FU NIH [RO1 GM092924, GM110041] FX This work was supported by NIH grants RO1 GM092924 and GM110041 to A.S. We thank members of the Salic lab for helpful discussions and members of the Structural Biology Center at Argonne National Laboratory for help with data collection at the 19-ID beam line. NR 44 TC 7 Z9 7 U1 7 U2 11 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD AUG 25 PY 2016 VL 166 IS 5 BP 1176 EP + DI 10.1016/j.cell.2016.08.003 PG 26 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DU5NW UT WOS:000382259500015 PM 27545348 ER PT J AU Engelmann, C Naughton, T AF Engelmann, Christian Naughton, Thomas TI A new deadlock resolution protocol and message matching algorithm for the extreme-scale simulator SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE performance prediction; message passing interface; parallel discrete event simulation; high-performance computing ID TRACES; MODEL AB Investigating the performance of parallel applications at scale on future high-performance computing (HPC) architectures and the performance impact of different HPC architecture choices is an important component of HPC hardware/software co-design. The Extreme-scale Simulator (xSim) is a simulation toolkit for investigating the performance of parallel applications at scale. xSim scales to millions of simulated Message Passing Interface (MPI) processes. The xSim toolkit strives to limit simulation overheads in order to maintain performance and productivity criteria. This paper documents two improvements to xSim: (1) a new deadlock resolution protocol to reduce the parallel discrete event simulation overhead and (2) a new simulated MPI message matching algorithm to reduce the oversubscription management cost. These enhancements resulted in significant performance improvements. The simulation overhead for running the NASA Advanced Super-computing Parallel Benchmark suite dropped from 1,020% to 238% for the conjugate gradient benchmark and 102% to 0% for the embarrassingly parallel benchmark. Additionally, the improvements were beneficial for reducing overheads in the highly accurate simulation mode of xSim, which is useful for resilience investigation studies for tracking intentional MPI process failures. In the highly accurate mode, the simulation overhead was reduced from 37,511% to 13,808% for conjugate gradient and from 3,332% to 204% for embarrassingly parallel. Copyright (C) 2016 John Wiley & Sons, Ltd. C1 [Engelmann, Christian; Naughton, Thomas] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Engelmann, C (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM engelmannc@computer.org FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); US Department of Energy [De-AC05-00OR22725]; UT-Battelle, LLC [De-AC05-00OR22725] FX This research is sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC for the US Department of Energy under contract no. De-AC05-00OR22725.; This manuscript has been authored by UT-Battelle, LLC under contract no. DE-AC05-00OR22725 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 32 TC 1 Z9 1 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD AUG 25 PY 2016 VL 28 IS 12 SI SI BP 3369 EP 3389 DI 10.1002/cpe.3805 PG 21 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA DV1CV UT WOS:000382658400007 ER PT J AU Abdelfattah, A Ltaief, H Keyes, D Dongarra, J AF Abdelfattah, Ahmad Ltaief, Hatem Keyes, David Dongarra, Jack TI Performance optimization of Sparse Matrix-Vector Multiplication for multi-component PDE-based applications using GPUs SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE sparse matrix-vector multiplication; GPU optimizations; block sparse matrices AB Simulations of many multi-component PDE-based applications, such as petroleum reservoirs or reacting flows, are dominated by the solution, on each time step and within each Newton step, of large sparse linear systems. The standard solver is a preconditioned Krylov method. Along with application of the preconditioner, memory-bound Sparse Matrix-Vector Multiplication (SpMV) is the most time-consuming operation in such solvers. Multi-species models produce Jacobians with a dense block structure, where the block size can be as large as a few dozen. Failing to exploit this dense block structure vastly underutilizes hardware capable of delivering high performance on dense BLAS operations. This paper presents a GPU-accelerated SpMV kernel for block-sparse matrices. Dense matrix-vector multiplications within the sparse-block structure leverage optimization techniques from the KBLAS library, a high performance library for dense BLAS kernels. The design ideas of KBLAS can be applied to block-sparse matrices. Furthermore, a technique is proposed to balance the workload among thread blocks when there are large variations in the lengths of nonzero rows. Multi-GPU performance is highlighted. The proposed SpMV kernel outperforms existing state-of-the-art implementations using matrices with real structures from different applications. Copyright (C) 2016 John Wiley & Sons, Ltd. C1 [Abdelfattah, Ahmad; Dongarra, Jack] Univ Tennessee, Innovat Comp Lab, Knoxville, TN 37996 USA. [Ltaief, Hatem; Keyes, David] King Abdullah Univ Sci & Technol, Extreme Comp Res Ctr, Thuwal, Saudi Arabia. [Dongarra, Jack] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Dongarra, Jack] Univ Manchester, Manchester M13 9PL, Lancs, England. RP Abdelfattah, A (reprint author), Univ Tennessee, Innovat Comp Lab, Knoxville, TN 37996 USA. EM ahmad@icl.utk.edu FU Saudi Aramco [RGC/3/1438]; NVIDIA FX This work is partly supported by Saudi Aramco, through research project RGC/3/1438. The authors would like also to thank NVIDIA for their support and generous hardware donations as well as Pascal Henon from TOTAL S.A. for fruitful technical discussions. NR 23 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD AUG 25 PY 2016 VL 28 IS 12 SI SI BP 3447 EP 3465 DI 10.1002/cpe.3874 PG 19 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA DV1CV UT WOS:000382658400012 ER PT J AU Mudgil, Y Karve, A Teixeira, PJPL Jiang, K Tunc-Ozdemir, M Jones, AM AF Mudgil, Yashwanti Karve, Abhijit Teixeira, Paulo J. P. L. Jiang, Kun Tunc-Ozdemir, Meral Jones, Alan M. TI Photosynthate Regulation of the Root System Architecture Mediated by the Heterotrimeric G Protein Complex in Arabidopsis SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE photosynthetic partitioning; positron electron tomography imaging; AGB1; lateral root density; glucose; gene expression; PIN2-GFP ID DEPENDENT AUXIN GRADIENTS; RXLR EFFECTOR AVR3A; PLASMA-MEMBRANE; CELL-DIVISION; DEVELOPMENTAL WINDOW; THALIANA SEEDLINGS; CARBON-DIOXIDE; ELEVATED CO2; BETA-SUBUNIT; TRANSPORT AB Assimilate partitioning to the root system is a desirable developmental trait to control but little is known of the signaling pathway underlying partitioning. A null mutation in the gene encoding the G beta) subunit of the heterotrimeric G protein complex, a nexus for a variety of signaling pathways, confers altered sugar partitioning in roots. While fixed carbon rapidly reached the roots of wild type and agb1-2 mutant seedlings, agb1 roots had more of this fixed carbon in the form of glucose, fructose, and sucrose which manifested as a higher lateral root density. Upon glucose treatment, the agb1-2 mutant had abnormal gene expression in the root tip validated by transcriptome analysis. In addition, PIN2 membrane localization was altered in the agb1-2 mutant. The heterotrimeric G protein complex integrates photosynthesis-derived sugar signaling incorporating both membrane-and transcriptional-based mechanisms. The time constants for these signaling mechanisms are in the same range as photosynthate delivery to the root, raising the possibility that root cells are able to use changes in carbon fixation in real time to adjust growth behavior. C1 [Mudgil, Yashwanti] Univ Delhi, Dept Bot, Delhi, India. [Mudgil, Yashwanti; Teixeira, Paulo J. P. L.; Jiang, Kun; Tunc-Ozdemir, Meral; Jones, Alan M.] Univ N Carolina, Dept Biol, Chapel Hill, NC USA. [Karve, Abhijit] Brookhaven Natl Lab, Upton, NY 11973 USA. [Jones, Alan M.] Univ N Carolina, Dept Pharmacol, Chapel Hill, NC USA. [Jiang, Kun] Zhejiang Univ, Coll Life Sci, Hangzhou, Zhejiang, Peoples R China. [Karve, Abhijit] Purdue Res Fdn, W Lafayette, IN USA. RP Mudgil, Y (reprint author), Univ Delhi, Dept Bot, Delhi, India.; Mudgil, Y (reprint author), Univ N Carolina, Dept Biol, Chapel Hill, NC USA. EM ymudgil@gmail.com FU NIGMS [R01GM065989]; DOE [DE-FG02-05er15671]; NSF [MCB-0723515, MCB-1158054, MCB-0718202]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy; DBT CREST award from the Government of INDIA; Delhi University RD; DU-DST PURSE grant; Pew Latin American Fellows Program in the Biomedical Sciences FX Work in the Jones Lab is supported by grants from the NIGMS (R01GM065989), DOE (DE-FG02-05er15671), and NSF (MCB-0723515, MCB-1158054, and MCB-0718202). The Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the US Department of Energy funded the majority of the work in this study. YM was supported by DBT CREST award (2011-2012) from the Government of INDIA and Delhi University R&D and DU-DST PURSE grant. PT is supported by The Pew Latin American Fellows Program in the Biomedical Sciences. NR 86 TC 0 Z9 0 U1 10 U2 10 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD AUG 25 PY 2016 VL 7 AR 1255 DI 10.3389/fpls.2016.01255 PG 13 WC Plant Sciences SC Plant Sciences GA DT9XC UT WOS:000381854600001 PM 27610112 ER PT J AU Harigaya, K Ibe, M Kaneta, K Nakano, W Suzuki, M AF Harigaya, Keisuke Ibe, Masahiro Kaneta, Kunio Nakano, Wakutaka Suzuki, Motoo TI Thermal relic dark matter beyond the unitarity limit SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM ID STABLE PARTICLES; CP CONSERVATION; EARLY UNIVERSE; AXION; SUPERSYMMETRY; CONSTRAINTS; ABUNDANCES; CANDIDATES; ICECUBE; MASSES AB We discuss a simple model of thermal relic dark matter whose mass can be much larger than the so-called unitarity limit on the mass of point-like particle dark matter. The model consists of new strong dynamics with one flavor of fermions in the fundamental representation which is much heavier than the dynamical scale of the new strong dynamics. Dark matter is identified with the lightest baryonic hadron of the new dynamics. The baryonic hadrons annihilate into the mesonic hadrons of the new strong dynamics when they have large radii. Resultantly, thermal relic dark matter with a mass in the PeV range is possible. C1 [Harigaya, Keisuke] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Harigaya, Keisuke] Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Ibe, Masahiro; Nakano, Wakutaka; Suzuki, Motoo] Univ Tokyo, UTIAS, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. [Ibe, Masahiro; Nakano, Wakutaka; Suzuki, Motoo] Univ Tokyo, ICRR, Kashiwa, Chiba 2778583, Japan. [Kaneta, Kunio] Inst for Basic Sci Korea, Ctr Theoret Phys Universe, Daejeon 34051, South Korea. RP Harigaya, K (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA.; Harigaya, K (reprint author), Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. EM keisukeharigaya@berkeley.edu; ibe@icrr.u-tokyo.ac.jp; kaneta@ibs.re.kr; m156077@icrr.u-tokyo.ac.jp; m0t@icrr.u-tokyo.ac.jp FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT), Japan [25105011, 15H05889]; Japan Society for the Promotion of Science (JSPS) [26287039]; World Premier International Research Center Initiative (WPI), MEXT, Japan; Department of Energy, Office of Science, Office of High Energy Physics [DE-AC02-05CH11231]; National Science Foundation [PHY-1316783, PHY-1521446]; IBS [IBS-R018-D1] FX This work is supported in part by Grants-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT), Japan, No. 25105011 and No. 15H05889 (M. I.); Grant-in-Aid No. 26287039 (M. I.) from the Japan Society for the Promotion of Science (JSPS); and by the World Premier International Research Center Initiative (WPI), MEXT, Japan (M. I.). This work is also supported in part by the Department of Energy, Office of Science, Office of High Energy Physics, under contract No. DE-AC02-05CH11231 (K.H.), by the National Science Foundation under grants PHY-1316783 and PHY-1521446 (K. H.). This work is also supported by IBS under the project code, IBS-R018-D1. NR 59 TC 1 Z9 1 U1 1 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 25 PY 2016 IS 8 AR 151 DI 10.1007/JHEP08(2016)151 PG 22 WC Physics, Particles & Fields SC Physics GA DU5XJ UT WOS:000382286700001 ER PT J AU Antonov, IO Zador, J Rotavera, B Papajak, E Osborn, DL Taatjes, CA Sheps, L AF Antonov, Ivan O. Zador, Judit Rotavera, Brandon Papajak, Ewa Osborn, David L. Taatjes, Craig A. Sheps, Leonid TI Pressure-Dependent Competition among Reaction Pathways from First- and Second-O-2 Additions in the Low-Temperature Oxidation of Tetrahydrofuran SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID PHOTOIONIZATION CROSS-SECTIONS; CYCLIC ETHERS; AUTOIGNITION CHEMISTRY; HYDROCARBON AUTOIGNITION; MULTISCALE INFORMATICS; THERMAL-DECOMPOSITION; COMBUSTION CHEMISTRY; MASS-SPECTROMETRY; REFLECTED SHOCKS; RADICAL REACTION AB We report a combined experimental and quantum chemistry study of the initial reactions in low-temperature oxidation of tetrahydrofuran (THF). Using synchrotron-based time-resolved VUV photoionization mass spectrometry, we probe numerous transient intermediates and products at P = 10-2000 Torr and T = 400-700 K. A key reaction sequence, revealed by our experiments, is the conversion of THF-yl peroxy to hydroperoxy-THF-yl radicals (QOOH), followed by a second 02 addition and subsequent decomposition to dihydrofuranyl hydroperoxide + HO2 or to gamma-butyrolactone hydroperoxide + OH. The competition between these two pathways affects the degree of radical chain-branching and is likely of central importance in modeling the autoignition of THF. We interpret our data with the aid of quantum chemical calculations of the THF-yl + O-2 and QOOH + O-2 potential energy surfaces. On the basis of our results, we propose a simplified THF oxidation mechanism below 700 K, which involves the competition among unimolecular decomposition and oxidation pathways of QOOH. C1 [Antonov, Ivan O.; Zador, Judit; Rotavera, Brandon; Papajak, Ewa; Osborn, David L.; Taatjes, Craig A.; Sheps, Leonid] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Sheps, L (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM lsheps@sandia.gov RI Zador, Judit/A-7613-2008 OI Zador, Judit/0000-0002-9123-8238 FU Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy; Argonne Sandia Consortium on High-Pressure Combustion Chemistry; National Nuclear Security Administration [DE-AC04-94AL85000] FX We thank Mr. Kendrew Au (Sandia) and the staff at the Chemical Dynamics Beamline at the ALS for excellent technical support of these experiments. This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy. L.S. and I.O.A. are supported through the Argonne Sandia Consortium on High-Pressure Combustion Chemistry. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration, under contract DE-AC04-94AL85000. This research used resources of the Advanced Light Source, which is a DOE Office of Science User Facility. NR 58 TC 1 Z9 1 U1 25 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD AUG 25 PY 2016 VL 120 IS 33 BP 6582 EP 6595 DI 10.1021/acs.jpca.6b05411 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DU4JQ UT WOS:000382179300009 PM 27441526 ER PT J AU Blaschke, DN Cirigliano, V AF Blaschke, Daniel N. Cirigliano, Vincenzo TI Neutrino quantum kinetic equations: The collision term SO PHYSICAL REVIEW D LA English DT Article ID EARLY UNIVERSE; CORE-COLLAPSE; NONEQUILIBRIUM CORRECTIONS; MASSLESS NEUTRINOS; BOLTZMANN-EQUATION; OSCILLATIONS; SPECTRA; TRANSPORT; MECHANISM; MATTER AB We derive the collision term relevant for neutrino quantum kinetic equations in the early universe and compact astrophysical objects, displaying its full matrix structure in both flavor and spin degrees of freedom. We include in our analysis neutrino-neutrino processes, scattering and annihilation with electrons and positrons, and neutrino scattering off nucleons (the latter in the low-density limit). After presenting the general structure of the collision terms, we take two instructive limiting cases. The one-flavor limit highlights the structure in helicity space and allows for a straightforward interpretation of the off-diagonal entries in terms of the product of scattering amplitudes of the two helicity states. The isotropic limit is relevant for studies of the early universe: in this case the terms involving spin coherence vanish and the collision term can be expressed in terms of two-dimensional integrals, suitable for computational implementation. C1 [Blaschke, Daniel N.; Cirigliano, Vincenzo] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Blaschke, DN (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM dblaschke@lanl.gov; cirigliano@lanl.gov OI Cirigliano, Vincenzo/0000-0002-9056-754X FU LDRD program at Los Alamos National Laboratory FX We thank T. Bhattacharya, J. Carlson, C. Lee, G. Fuller, E. Grohs, L. Johns, M. Paris, S. Reddy, S. Tulin and A. Vlasenko for insightful discussions. Special thanks go to E. Grohs for carefully reading the manuscript. We acknowledge support by the LDRD program at Los Alamos National Laboratory. NR 50 TC 4 Z9 4 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 25 PY 2016 VL 94 IS 3 AR 033009 DI 10.1103/PhysRevD.94.033009 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KV UT WOS:000381893800002 ER PT J AU Elder, B Khoury, J Haslinger, P Jaffe, M Muller, H Hamilton, P AF Elder, Benjamin Khoury, Justin Haslinger, Philipp Jaffe, Matt Muller, Holger Hamilton, Paul TI Chameleon dark energy and atom interferometry SO PHYSICAL REVIEW D LA English DT Article ID MODIFIED GRAVITY; CONSTRAINTS; TESTS AB Atom interferometry experiments are searching for evidence of chameleon scalar fields with ever-increasing precision. As experiments become more precise, so too must theoretical predictions. Previous work has made numerous approximations to simplify the calculation, which in general requires solving a three-dimensional nonlinear partial differential equation. This paper calculates the chameleonic force using a numerical relaxation scheme on a uniform grid. This technique is more general than previous work, which assumed spherical symmetry to reduce the partial differential equation to a one-dimensional ordinary differential equation. We examine the effects of approximations made in previous efforts on this subject and calculate the chameleonic force in a setup that closely mimics the recent experiment of Hamilton et al. Specifically, we simulate the vacuum chamber as a cylinder with dimensions matching those of the experiment, taking into account the backreaction of the source mass, its offset from the center, and the effects of the chamber walls. Remarkably, the acceleration on a test atomic particle is found to differ by only 20% from the approximate analytical treatment. These results allow us to place rigorous constraints on the parameter space of chameleon field theories, although ultimately the constraint we find is the same as the one we reported in Hamilton et al. because we had slightly underestimated the size of the vacuum chamber. This computational technique will continue to be useful as experiments become even more precise and will also be a valuable tool in optimizing future searches for chameleon fields and related theories. C1 [Elder, Benjamin; Khoury, Justin] Univ Penn, Dept Phys & Astron, Ctr Particle Cosmol, Philadelphia, PA 19104 USA. [Hamilton, Paul] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Haslinger, Philipp; Jaffe, Matt; Muller, Holger] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Muller, Holger] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Elder, B (reprint author), Univ Penn, Dept Phys & Astron, Ctr Particle Cosmol, Philadelphia, PA 19104 USA. FU NSF CAREER [PHY-1145525]; NASA ATP [NNX11AI95G]; New Initiative Research Grant from the Charles E. Kaufman fund of The Pittsburgh Foundation; David and Lucile Packard Foundation; DARPA Young Faculty Grant [N66001-12-1-4232]; NSF [PHY-1404566]; NASA [NNH13ZTT002N, NNH11ZTT001N] FX We are grateful for helpful discussions with Lasha Berezhiani, Sebastien Clesse, Rehan Deen, Andrei Ivanov, Sandrine Schlogel, Amol Upadhye, and Nan Yu. B. E. and J. K. are supported in part by NSF CAREER Grant No. PHY-1145525, NASA ATP Grant No. NNX11AI95G, and a New Initiative Research Grant from the Charles E. Kaufman fund of The Pittsburgh Foundation. H. W. is supported by the David and Lucile Packard Foundation; the DARPA Young Faculty Grant No. N66001-12-1-4232; NSF Grant No. PHY-1404566; and NASA Grants No. NNH13ZTT002N, No. NNH13ZTT002N, and No. NNH11ZTT001N. P. H. thanks the Austrian Science Fund: J3680. NR 63 TC 5 Z9 5 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 25 PY 2016 VL 94 IS 4 AR 044051 DI 10.1103/PhysRevD.94.044051 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0LG UT WOS:000381895400006 ER PT J AU Lucas, FWD Welch, AW Baranowski, LL Dippo, PC Hempel, H Unold, T Eichberger, R Blank, B Rau, U Mascaro, LH Zakutayev, A AF de Souza Lucas, Francisco Willian Welch, Adam W. Baranowski, Lauryn L. Dippo, Patricia C. Hempel, Hannes Unold, Thomas Eichberger, Rainer Blank, Beatrix Rau, Uwe Mascaro, Lucia H. Zakutayev, Andriy TI Effects of Thermochemical Treatment on CuSbS2 Photovoltaic Absorber Quality and Solar Cell Reproducibility SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID COPPER-ANTIMONY-SULFIDE; THIN-FILMS; SEMICONDUCTORS; RECOMBINATION; DEPOSITION; CHALLENGES; TRANSPORT; SB2SE3 AB CuSbS2 is a promising nontoxic and earth-abundant photovoltaic absorber that is chemically simpler than the widely studied Cu2ZnSnS4. However, CuSbS2 photovoltaic (PV) devices currently have relatively low efficiency and poor reproducibility, often due to suboptimal material quality and insufficient optoelectronic properties. To address these issues, here we develop a thermochemical treatment (TT) for CuSbS2 thin films, which consists of annealing in Sb2S3 vapor followed by a selective KOH surface chemical etch. The annealed CuSbS2 films show improved structural quality and optoelectronic properties, such as stronger band-edge photoluminescence and longer photoexcited carrier lifetime. These improvements also lead to mote reproducible CuSbS2 PV devices, with performance currently limited by a large cliff-type interface band offset with CdS contact. Overall, these results point to the potential avenues to further increase the performance Of CuSbS2 thin film solar cell, and the findings can be transferred to other thin film photovoltaic technologies. C1 [de Souza Lucas, Francisco Willian; Welch, Adam W.; Baranowski, Lauryn L.; Dippo, Patricia C.; Zakutayev, Andriy] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [de Souza Lucas, Francisco Willian; Mascaro, Lucia H.] Univ Fed Sao Carlos, Rd Washington Luiz,Km 235, BR-13565905 Sao Carlos, SP, Brazil. [Welch, Adam W.; Baranowski, Lauryn L.] Colorado Sch Mines, 1500 Illinois St, Golden, CO 80401 USA. [Hempel, Hannes; Unold, Thomas; Eichberger, Rainer] Helmholtz Zentrum Berlin Mat & Energie GmbH, Hahn Meitner Pl 1, D-14109 Berlin, Germany. [Blank, Beatrix; Rau, Uwe] Forschungszentrum Juelich, IEK5 Photovolta, Wilhelm Johnen Str, D-52428 Julich, Germany. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov RI Lucas, Francisco/E-8106-2016; Rau, Uwe/G-2256-2011; FAPESP, CDMF/J-3591-2015; FAPESP-GSK, CERSusChem/H-8785-2016 OI Lucas, Francisco/0000-0002-4637-8469; Rau, Uwe/0000-0003-3526-3081; FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the SunShot initiative [DE-AC36-08GO28308]; Sao Paulo Research Foundation (FAPESP) [2014/12166-3]; Helmholtz Association Initiative and Network Fund (HNSEI) [SO-075]; Hans L. Merkle Foundation FX The "Rapid Development of Earth-abundant Thin Film Solar Cells" project is supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the SunShot initiative, under Contract No. DE-AC36-08GO28308 to the NREL. For execution of this work, F.W.d.S.L was funded by the Sao Paulo Research Foundation (FAPESP), Grant 2014/12166-3. The optical pump terahertz probe absorber measurements and temperature-dependent device performance characterization were supported by the Helmholtz Association Initiative and Network Fund (HNSEI project SO-075). B.B. acknowledges support from the Hans L. Merkle Foundation via a Ph.D. scholarship. NR 56 TC 1 Z9 1 U1 27 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18377 EP 18385 DI 10.1021/acs.jpcc.6b04206 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000003 ER PT J AU Wujcik, KH Wang, DR Raghunathan, A Drake, M Pascal, TA Prendergast, D Balsara, NP AF Wujcik, Kevin H. Wang, Dunyang Rita Raghunathan, Aditya Drake, Melanie Pascal, Tod A. Prendergast, David Balsara, Nitash P. TI Lithium Polysulfide Radical Anions in Ether-Based Solvents SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; LI-S BATTERIES; SULFUR BATTERIES; ELECTROCHEMICAL REDUCTION; ALKALI POLYSULFIDES; MAGNETIC-RESONANCE; APROTIC-SOLVENTS; BLUE SOLUTIONS; DIMETHYLFORMAMIDE; IDENTIFICATION AB Lithium sulfur batteries have a theoretical specific energy 5 times greater than current lithium ion battery standards, but suffer from the issue of lithium polysulfide dissolution. The reaction mechanisms that underlie the formation of lithium polysulfide reaction intermediates have been studied for over four decades, yet still elude researchers. Polysulfide radical anions formed during the redox processes have become a focal point of fundamental Li-S battery research. The formation of radical species has even been shown to be advantageous to the electrochemical pathways. However, whether polysulfide radical anions can form and be stabilized in common Li-S battery electrolytes that are ether-based is a point of contention in Li-S battery research. The goal of this work was to examine the presence of radical polysulfide species in ether-based solvents. Lithium polysulfide solutions in tetraethylene glycol dimethyl ether and poly(ethylene oxide) are probed using a combination of ultraviolet visible (UV-vis) and electron paramagnetic resonance (EPR) spectroscopy. EPR results confirm the presence of radical species in ether-based electrolytes. Comparison of the UV vis spectra to EPR spectra establishes that the UV vis absorbance signature for radical species in ether-based solvents occurs at a wavelength of 617 nm, which is consistent with what is observed for high electron pair donor solvents such as dimethylformamide and dimethyl sulfoxide. C1 [Wujcik, Kevin H.; Raghunathan, Aditya; Drake, Melanie; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Wang, Dunyang Rita] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wujcik, Kevin H.; Wang, Dunyang Rita; Raghunathan, Aditya; Balsara, Nitash P.] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Pascal, Tod A.; Prendergast, David] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under the Battery Materials Research program [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract DE-AC02-05CH11231 under the Battery Materials Research program. UV vis spectroscopy was performed under a User Project at The Molecular Foundry. We thank Professor Jeffrey Reimer for enabling the EPR experiments and Eric Scott for his support and useful discussions regarding EPR NR 46 TC 0 Z9 0 U1 16 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18403 EP 18410 DI 10.1021/acs.jpcc.6b04264 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000006 ER PT J AU Shkrob, IA Pupek, KZ Abraham, DP AF Shkrob, Ilya A. Pupek, Krzysztof Z. Abraham, Daniel P. TI Allotropic Control: How Certain Fluorinated Carbonate Electrolytes Protect Aluminum Current Collectors by Promoting the Formation of Insoluble Coordination Polymers SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LITHIUM-ION BATTERIES; LIQUID ELECTROLYTES; ANODIC BEHAVIOR; CORROSION; CHEMISTRY; SALTS; SUPPRESSION; DISSOLUTION; ELECTRODES; STABILITY AB Presently, there is a Strong incentive for increasing the operation voltage of Li-ion cells above 4.5 V in order to increase the density of stored energy. Aluminum is an inexpensive, lightweight metal that is commonly used as a positive electrode current collector in these cells. Imide LAX salts, such as lithium bis(trifluoromethylsulfonypimide (X = TFSI), and lithium bis(fluorosulfonyl)imide (X = FSI), are chemically stable on the energized lithiated transition metal oxide electrodes, but their presence in the electrolyte causes rapid anodic dissolution and pitting of Al current collectors at potentials exceeding 4.0 V versus Li/Li+. For LiBF4 and LiPF6, the release of HF near the energized surfaces passivates the exposed Al metal, inhibiting this pitting corrosion, but it also causes the gradual degradation of the cathode active material, negating this important advantage. Here we report that in certain electrolytes containing fluorinated carbonate solvents and LiX salts, the threshold voltage for safe operation of Al current collectors can be increased to 5.5 V versus Li/Li+. Interestingly, the most efficient solvent also facilitates the formation of an insoluble gel when AlX3 is introduced into this solvent. We suggest that this solvent promotes the aggregation of coordination polymers of AlX3 at the exposed Al surface that isolate this surface from the electrolyte, thereby preventing further Al dissolution and corrosion. Other examples of Al collector protection may also involve this mechanism. Our study suggests that such "allotropic control" could be a way of widening the operation window of Li-ion cells without electrode deterioration, Al current collector corrosion, and electrolyte breakdown. C1 [Shkrob, Ilya A.; Abraham, Daniel P.] Argonne Natl Lab, Mat Engn Res Facil, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Pupek, Krzysztof Z.] Argonne Natl Lab, Mat Engn Res Facil, Energy Syst Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Shkrob, IA; Abraham, DP (reprint author), Argonne Natl Lab, Mat Engn Res Facil, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM shkrob@anl.gov; abraham@anl.gov FU Applied Battery Research (ABR) for Transportation Program; U.S. DOE Office of Vehicle Technologies; U.S. DOE Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX I.A.S. thanks M. Ferrandon for her help with X-ray studies. K.Z.P. thanks Solvay for providing the FEC used in this study. The BFEC and FEMC solvents were synthesized at Argonne's Materials Engineering Research Facility (MERF), which is supported within the core funding of the Applied Battery Research (ABR) for Transportation Program. K.Z.P. and D.P.A. are grateful for support from U.S. DOE Office of Vehicle Technologies and also for help from team members including J. Gilbert, T. Dzwiniel, and G. Krumdick. This work was supported by the U.S. DOE Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences under Contract No. DE-AC02-06CH11357 to Argonne. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory. NR 40 TC 1 Z9 1 U1 18 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18435 EP 18444 DI 10.1021/acs.jpcc.6b05241 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000010 ER PT J AU Vogiatzis, KD Haldoupis, E Xiao, DJ Long, JR Siepmann, JI Gagliardi, L AF Vogiatzis, Konstantinos D. Haldoupis, Emmanuel Xiao, Dianne J. Long, Jeffrey R. Siepmann, J. Ilja Gagliardi, Laura TI Accelerated Computational Analysis of Metal-Organic Frameworks for Oxidation Catalysis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN STORAGE; 2-STATE REACTIVITY; IRON-OXO; COMPLEXES; CHEMISTRY; DEFECTS; SITES; HYDROXYLATION; MECHANISM; ETHANOL AB High-spin iron(IV)-oxo compounds are known to activate strong C-H bonds. Stabilizing the high-spin S = 2 electronic configuration is difficult in molecular species for homogeneous catalysis, but recent experimental and computational results suggest this can be achieved in the metal-organic framework Fe-2(dobdc) (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate) and its magnesium-diluted analogues. With a novel computational screening approach, we have identified three additional frameworks that are predicted to form high-spin iron(IV)-oxo species upon dissociative adsorption of nitrous oxide. The computational work is supported by follow-up experiments which show that, among these three materials, Fe-BTT (BTT3- = 1,3,5-benzenetristetrazolate) selectively oxidizes ethane to ethanol at 120 degrees C. Subsequent spectroscopic and cycling studies suggest that framework defects, rather than the bulk framework or extraframework sites, are likely responsible for the observed reactivity. This work shows how computational methods can be used to rapidly identify promising candidate frameworks, and highlights the need for new methods that allow defect sites in metal-organic frameworks to be better understood and exploited for catalysis. C1 [Vogiatzis, Konstantinos D.; Haldoupis, Emmanuel; Siepmann, J. Ilja; Gagliardi, Laura] Univ Minnesota, Dept Chem, Minnesota Supercomp Inst, 207 Pleasant St Southeast, Minneapolis, MN 55455 USA. [Vogiatzis, Konstantinos D.; Haldoupis, Emmanuel; Siepmann, J. Ilja; Gagliardi, Laura] Univ Minnesota, Chem Theory Ctr, 207 Pleasant St Southeast, Minneapolis, MN 55455 USA. [Xiao, Dianne J.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Siepmann, J. Ilja] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. [Vogiatzis, Konstantinos D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Siepmann, JI; Gagliardi, L (reprint author), Univ Minnesota, Dept Chem, Minnesota Supercomp Inst, 207 Pleasant St Southeast, Minneapolis, MN 55455 USA.; Siepmann, JI; Gagliardi, L (reprint author), Univ Minnesota, Chem Theory Ctr, 207 Pleasant St Southeast, Minneapolis, MN 55455 USA.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Long, JR (reprint author), Lawrence Berkeley Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Siepmann, JI (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. EM jrlong@berkeley.edu; siepmann@umn.edu; gagliard@umn.edu FU Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-12ER16362]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This research was carried out within the Nanoporous Materials Genome Center, which is supported by the Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Award DE-FG02-12ER16362. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors acknowledge the Minnesota Supercomputing Institute at the University of Minnesota for providing resources that contributed to the research results reported within this paper. We thank Prachi Sharma (UMN) for useful discussion. NR 41 TC 0 Z9 0 U1 13 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18707 EP 18712 DI 10.1021/acs.jpcc.6b07115 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000039 ER PT J AU Dimitrievska, M Ivetic, TB Litvinchuk, AP Fairbrother, A Miljevic, BB Strbac, GR Rodriguez, AP Lukic-Petrovic, SR AF Dimitrievska, Mirjana Ivetic, Tamara B. Litvinchuk, Alexander P. Fairbrother, Andrew Miljevic, Bojan B. Strbac, Goran R. Perez Rodriguez, Alejandro Lukic-Petrovic, Svetlana R. TI Eu3+-Doped Wide Band Gap Zn2SnO4 Semiconductor Nanoparticles: Structure and Luminescence SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID BILBAO CRYSTALLOGRAPHIC SERVER; RAMAN-SCATTERING; NANOCRYSTALS; CRYSTAL; EU3+; PHOTOLUMINESCENCE; PHOSPHORS; OXIDES; STATES; BULK AB Nanocrystalline Zn2SnO4 powders doped with Eu3+ ions were synthesized via a mechanochemical Solid-state reaction method followed by postannealing in air at 1200 degrees C. X-ray diffraction (XRD), energy-dispersive X-ray (EDX), and Raman and photoluminescence (PL) spectroscopies provide convincing evidence for the incorporation of Eu3+ ions into the host matrix on noncentrosymmetric sites of the cubic inverse spinel lattice. Microstnictural analysis shows that the crystalline grain size decreases with the addition of Eu3+. Formation of a nanocrystalline Eu2Sn2O7 secondary phase, is also observed. Luminescence spectra of Eu3+-doped samples show several emissions, including narrow-band magnetic dipole emission at 595 nm and electric dipole emission at 615 nm of the Eu3+ ions. Excitation spectra and lifetime measurements suggest that Eu3+ ions are incorporated at only one symmetry site. According to the crystal field' theory, it is assumed that Eu3+ ions participate at octahedral sites of Zn2+ or Sn4+ under a weak crystal field, rather than at the tetrahedral sites of Zn2+, because of the high octahedral stabilization energy for Eu3+. Activation of symmetry forbidden (IR-active and silent) Modes is observed in the Raman scattering spectra of both pure and doped samples, indicating a disorder of the cation Stiblattice of Zn2SnO4 nanocrystallites. These results were further supported by the first principle lattice dynamics calculations. The spinel-type Zn2SnO4 shows effectiveness in hosting Eu3+ ions, which could, be used as a prospective green/red emitter. This work also illustrates how sustainable and simple preparation methods could be used for effective engineering of material properties. C1 [Dimitrievska, Mirjana] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Dimitrievska, Mirjana] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Dimitrievska, Mirjana; Fairbrother, Andrew; Perez Rodriguez, Alejandro] Catalonia Inst Energy Res IREC, Jardins Dones Negre 1, Barcelona 08930, Spain. [Ivetic, Tamara B.; Miljevic, Bojan B.; Strbac, Goran R.; Lukic-Petrovic, Svetlana R.] Univ Novi Sad, Dept Phys, Fac Sci, Trg Dositeja Obradovica 4, Novi Sad 21000, Serbia. [Litvinchuk, Alexander P.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Litvinchuk, Alexander P.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Miljevic, Bojan B.] Univ Novi Sad, Fac Technol, Dept Mat Engn, Bul Cara Lazara 1, Novi Sad 21000, Serbia. [Perez Rodriguez, Alejandro] Univ Barcelona, IN2UB, C Marti Franques 1, E-08028 Barcelona, Spain. RP Dimitrievska, M (reprint author), NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA.; Dimitrievska, M (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.; Dimitrievska, M (reprint author), Catalonia Inst Energy Res IREC, Jardins Dones Negre 1, Barcelona 08930, Spain. EM mira.dimitrievska@gmail.com RI Litvinchuk, Alexander/K-6991-2012; OI Litvinchuk, Alexander/0000-0002-5128-5232; Miljevic, Bojan/0000-0002-0773-7115 FU APV Provincial Secretariat for Higher Education and Scientific Research; Ministry of Education, Science, and Technological Development of the Republic of Serbia [ON 171022, III 45020]; European Union [316488]; State of Texas though the TcSUH at the University of Houston; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office [DE-AC36-08GO28308] FX This work was supported by APV Provincial Secretariat for Higher Education and Scientific Research, and we acknowledge the support of the Ministry of Education, Science, and Technological Development of the Republic of Serbia (Project numbers: ON 171022 and III 45020) and the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme FP7/2007-2013/under REA grant agreement no316488 (KESTCELLS). A. P. L. acknowledges the support from the State of Texas though the TcSUH at the University of Houston. M. D. gratefully acknowledges research support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office, under Contract No. DE-AC36-08GO28308. The authors would like to thank Dr. Miroslav Dramicanin (Vinca Institute of Nuclear Sciences, Belgrade, Serbia) for the luminescence measurements and productive discussions. NR 39 TC 1 Z9 1 U1 15 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18887 EP 18894 DI 10.1021/acs.jpcc.6b05335 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000060 ER PT J AU Suri, PK Yan, JQ Mandrus, DG Flannigan, DJ AF Suri, Pranav K. Yan, Jiaqiang Mandrus, David G. Flannigan, David J. TI Dynamical Scattering and Electron Channeling in Orthorhombic and Tetragonal LaFeAsO SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; INPLANE RESISTIVITY ANISOTROPY; IRON ARSENIDE SUPERCONDUCTOR; PHASE-DIAGRAM; ATOMIC-SCALE; MICROSCOPY; RESOLUTION; LAO1-XFXFEAS; TRANSITION; DIFFRACTION AB In the study of LaFeAsO and doped compounds thereof, high-resolution transmission electron microscopy (TEM) has been used to characterize the structural and morphological properties, while cryo-TEM has been used to purportedly observe the structural phase transition occurring at 160 K. Often, the appearance and disappearance of Bragg spots in diffraction patterns, as well as changes in diffraction contrast in bright-field images, have been pointed to as indicators of the phase transition. Here we show that effects not related to the transition can produce signatures reminiscent of those typically associated with the symmetry change. In particular, we demonstrate the effects of electron channeling and multiple scattering on intensity modulation of atomic columns and Bragg spots in high-angle annular dark-field scanning TEM (HAADF-STEM) images and parallel-beam electron diffraction (PBED) patterns, respectively, from both tetragonal and orthorhombic LaFeAsO. From electron-transparent lamellae, we quantify the spatially varying thickness and, via atomic-resolution HAADF-STEM imaging, demonstrate the thickness-dependent modulation of intensities within the (Fe,O) and (La, As) columns at 300 K. From PBED patterns and Fourier-filtered high-resolution bright field images acquired both above and below the structural phase-transition temperature, we show how intensities of forbidden reflections are modulated by moving to regions of differing thickness, independent of a symmetry change (i.e., at a fixed temperature). The experimental results are supported with multislice simulations of thickness-dependent atomic-column contrast and Bragg-spot intensities. C1 [Suri, Pranav K.; Flannigan, David J.] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. [Yan, Jiaqiang; Mandrus, David G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yan, Jiaqiang; Mandrus, David G.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Flannigan, DJ (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. EM flan0076@umn.edu FU Arnold and Mabel Beckman Foundation; 3M Nontenured Faculty Award [13673369]; Donors of the American Chemical Society Petroleum Research Fund [53116-DNI7]; NSF through the UMN MRSEC program [DMR-0819885, DMR-1420013]; NSF through the NNIN program; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division FX The work at the University of Minnesota was supported primarily by the Arnold and Mabel Beckman Foundation in the form of a Beckman Young Investigator Award and in part by a 3M Nontenured Faculty Award under Award Number 13673369. In addition, acknowledgment is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this work under Award Number 53116-DNI7. Part of this work was carried out in the College of Science and Engineering Characterization Facility, University of Minnesota, which has received capital equipment funding from the NSF through the UMN MRSEC program under Award Numbers DMR-0819885 and DMR-1420013. Part of this work was carried out in the College of Science and Engineering Minnesota Nano Center, University of Minnesota, which receives partial support from NSF through the NNIN program. Work at ORNL was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. We thank Rafael Fernandes for comments and suggestions and for reading the manuscript. We thank Jason Myers, Kevin Roberts, and Wei Zhang for assistance within the University of Minnesota shared facilities. NR 60 TC 0 Z9 0 U1 6 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18931 EP 18938 DI 10.1021/acs.jpcc.6b06339 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000066 ER PT J AU Saha, A Chattopadhyay, S Shibata, T Viswanatha, R AF Saha, Avijit Chattopadhyay, Soma Shibata, Tomohiro Viswanatha, Ranjani TI Core-Shell to Doped Quantum Dots: Evolution of the Local Environment Using XAFS SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOPING SEMICONDUCTOR NANOCRYSTALS; MAGNETIC SEMICONDUCTOR; NANOPARTICLES; PERFORMANCE; DEPENDENCE; EMITTERS; IFEFFIT AB Internal structure study at an atomic level is a challenging task with far reaching consequences to its material properties, specifically in the field of transition metal doping in quantum dots. Diffusion of transition metal ions in and out of quantum dots forming magnetic clusters has been a major bottleneck in this class of materials. Diffusion of the magnetic ions from the core into the nonmagnetic shell in a core/shell heterostructure architecture to attain uniform doping has been recently introduced and yet to be understood. In this work, we have studied the local structure variation of Fe as a function of CdS matrix thickness and annealing time during the overcoating of Fe3O4 core with CdS using X-ray absorption spectroscopy. The data reveals that Fe3O4 core initially forms a core/shell structure with CdS followed by alloying at the interface eventually completely diffusing all the way through the CdS matrix to form homogeneously Fe-doped CdS QDs with excellent control over size and size distribution. Study of Fe K-edge shows a complete change of Fe local environment from Fe-O to FeS. C1 [Saha, Avijit; Viswanatha, Ranjani] Jawaharlal Nehru Ctr Adv Sci Res, New Chem Unit, Bangalore 560064, Karnataka, India. [Viswanatha, Ranjani] Jawaharlal Nehru Ctr Adv Sci Res, Int Ctr Mat Sci, Bangalore 560064, Karnataka, India. [Chattopadhyay, Soma; Shibata, Tomohiro] CSRRI IIT, Adv Photon Source, Sect ID 10, 9700 South Cass Ave, Lemont, IL 60439 USA. [Chattopadhyay, Soma] Elgin Community Coll, Dept Phys Sci, 1700 Spartan Dr, Elgin, IL 60123 USA. [Shibata, Tomohiro] Kennametal Inc, Mat Sci, 1600 Technol Way, Latrobe, PA 15650 USA. RP Viswanatha, R (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, New Chem Unit, Bangalore 560064, Karnataka, India.; Viswanatha, R (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, Int Ctr Mat Sci, Bangalore 560064, Karnataka, India. EM rv@jncasr.ac.in RI ID, MRCAT/G-7586-2011 FU JNCASR, Sheikh Saqr Laboratory; Department of Science and Technology, Government of India; CSIR; MRCAT host institutions; U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A.S. and R.V. thank JNCASR, Sheikh Saqr Laboratory and Department of Science and Technology, Government of India for financial support. A.S. thanks CSIR for a research fellowship. RV. is grateful for the Sheikh Saqr Career Award Fellowship. Authors (S.C. and T.S.) would like to thank Dr. Vladislav Zyryanov for his help with experimental setup during XAFS measurement. MRCAT is funded by MRCAT host institutions. APS is funded by U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 34 TC 2 Z9 2 U1 12 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD AUG 25 PY 2016 VL 120 IS 33 BP 18945 EP 18951 DI 10.1021/acs.jpcc.6b06803 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DU4JX UT WOS:000382180000068 ER PT J AU Soh, DBS Hamerly, R Mabuchi, H AF Soh, Daniel B. S. Hamerly, Ryan Mabuchi, Hideo TI Comprehensive analysis of the optical Kerr coefficient of graphene SO PHYSICAL REVIEW A LA English DT Article ID OPTOELECTRONICS; GENERATION; DISPERSION; PHOTONICS AB We present a comprehensive analysis of the nonlinear optical Kerr effect in graphene. We directly solve the S-matrix element to calculate the absorption rate, utilizing the Volkov-Keldysh-type crystal wave functions. We then convert to the nonlinear refractive index coefficients through the Kramers-Kronig relation. In this formalism, the source of Kerr nonlinearity is the interplay of optical fields that cooperatively drive the transition from valence to conduction band. This formalism makes it possible to identify and compute the rates of distinct nonlinear processes that contribute to the Kerr nonlinear refractive index coefficient. The four identified mechanisms are two-photon absorption, Raman transition, self-coupling, and quadratic ac Stark effect. We also present a comparison of our theory with recent experimental and theoretical results. C1 [Soh, Daniel B. S.; Hamerly, Ryan; Mabuchi, Hideo] Stanford Univ, Edward L Ginzton Lab, Stanford, CA 94305 USA. [Soh, Daniel B. S.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Soh, DBS (reprint author), Stanford Univ, Edward L Ginzton Lab, Stanford, CA 94305 USA.; Soh, DBS (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. FU Precourt Institute for Energy at Stanford; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX R.H. is supported by a seed grant from the Precourt Institute for Energy at Stanford. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 27 TC 2 Z9 2 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD AUG 25 PY 2016 VL 94 IS 2 AR 023845 DI 10.1103/PhysRevA.94.023845 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DU0HT UT WOS:000381884300006 ER PT J AU Lane, JMD Foiles, SM Lim, H Brown, JL AF Lane, J. Matthew D. Foiles, Stephen M. Lim, Hojun Brown, Justin L. TI Strain-rate dependence of ramp-wave evolution and strength in tantalum SO PHYSICAL REVIEW B LA English DT Article ID HALL-PETCH RELATIONSHIP; EMBEDDED-ATOM-METHOD; PLASTIC-DEFORMATION; MOLECULAR-DYNAMICS; NANOCRYSTALLINE TANTALUM; METALS; COMPRESSION AB We have conducted molecular dynamics (MD) simulations of quasi-isentropic ramp-wave compression to very high pressures over a range of strain rates from 1011 down to 108 1/s. Using scaling methods, we collapse wave profiles from various strain rates to a master profile curve, which shows deviations when material response is strain-rate dependent. Thus, we can show with precision where, and how, strain-rate dependence affects the ramp wave. We find that strain rate affects the stress-strain material response most dramatically at strains below 20%, and that above 30% strain the material response is largely independent of strain rate. We show good overall agreement with experimental stress-strain curves up to approximately 30% strain, above which simulated response is somewhat too stiff. We postulate that this could be due to our interatomic potential or to differences in grain structure and/or size between simulation and experiment. Strength is directly measured from per-atom stress tensor and shows significantly enhanced elastic response at the highest strain rates. This enhanced elastic response is less pronounced at higher pressures and at lower strain rates. C1 [Lane, J. Matthew D.; Foiles, Stephen M.; Lim, Hojun; Brown, Justin L.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Lane, JMD (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 31 TC 0 Z9 0 U1 6 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 25 PY 2016 VL 94 IS 6 AR 064301 DI 10.1103/PhysRevB.94.064301 PG 6 WC Physics, Condensed Matter SC Physics GA DU0JI UT WOS:000381888700002 ER PT J AU Huang, JH Pan, BF Duan, WT Wei, XL Assary, RS Su, L Brushett, FR Cheng, L Liao, C Ferrandon, MS Wang, W Zhang, ZC Burrell, AK Curtiss, LA Shkrob, IA Moore, JS Zhang, L AF Huang, Jinhua Pan, Baofei Duan, Wentao Wei, Xiaoliang Assary, Rajeev S. Su, Liang Brushett, Fikile R. Cheng, Lei Liao, Chen Ferrandon, Magali S. Wang, Wei Zhang, Zhengcheng Burrell, Anthony K. Curtiss, Larry A. Shkrob, Ilya A. Moore, Jeffrey S. Zhang, Lu TI The lightest organic radical cation for charge storage in redox flow batteries SO SCIENTIFIC REPORTS LA English DT Article ID RESEARCH-AND-DEVELOPMENT; LITHIUM-ION BATTERIES; OVERCHARGE PROTECTION; METHOXYLATED BENZENES; AQUEOUS-SOLUTION; ENERGY-STORAGE; ELECTROLYTES; PROGRESS; SHUTTLE; DESIGN AB In advanced electrical grids of the future, electrochemically rechargeable fluids of high energy density will capture the power generated from intermittent sources like solar and wind. To meet this outstanding technological demand there is a need to understand the fundamental limits and interplay of electrochemical potential, stability, and solubility in low-weight redox-active molecules. By generating a combinatorial set of 1,4-dimethoxybenzene derivatives with different arrangements of substituents, we discovered a minimalistic structure that combines exceptional long-term stability in its oxidized form and a record-breaking intrinsic capacity of 161 mAh/g. The nonaqueous redox flow battery has been demonstrated that uses this molecule as a catholyte material and operated stably for 100 charge/discharge cycles. The observed stability trends are rationalized by mechanistic considerations of the reaction pathways. C1 [Huang, Jinhua; Pan, Baofei; Duan, Wentao; Wei, Xiaoliang; Assary, Rajeev S.; Su, Liang; Brushett, Fikile R.; Cheng, Lei; Liao, Chen; Ferrandon, Magali S.; Wang, Wei; Zhang, Zhengcheng; Burrell, Anthony K.; Curtiss, Larry A.; Shkrob, Ilya A.; Moore, Jeffrey S.; Zhang, Lu] Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA. [Huang, Jinhua; Pan, Baofei; Liao, Chen; Ferrandon, Magali S.; Zhang, Zhengcheng; Burrell, Anthony K.; Shkrob, Ilya A.; Zhang, Lu] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Duan, Wentao; Wei, Xiaoliang; Wang, Wei] Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Assary, Rajeev S.; Cheng, Lei; Curtiss, Larry A.] Argonne Natl Lab, Mat Sci Div, Argonne, IL 60439 USA. [Su, Liang; Brushett, Fikile R.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. [Moore, Jeffrey S.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Moore, Jeffrey S.] Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. RP Shkrob, IA; Moore, JS; Zhang, L (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA.; Shkrob, IA; Zhang, L (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.; Moore, JS (reprint author), Univ Illinois, Dept Chem, Urbana, IL 61801 USA.; Moore, JS (reprint author), Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. EM shkrob@anl.gov; moore@scs.illinois.edu; luzhang@anl.gov RI Wang, Wei/F-4196-2010; Duan, Wentao/E-5742-2011 OI Wang, Wei/0000-0002-5453-4695; Duan, Wentao/0000-0002-8269-6413 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-06CH11357]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences under contract No. DE-AC02-06CH11357; it was also supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 31 TC 1 Z9 1 U1 33 U2 48 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 25 PY 2016 VL 6 AR 32102 DI 10.1038/srep32102 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU0AS UT WOS:000381864300001 PM 27558638 ER PT J AU Xu, ZX Bassett, SW Hu, B Dyer, SB AF Xu, Zexuan Bassett, Seth Willis Hu, Bill Dyer, Scott Barrett TI Long distance seawater intrusion through a karst conduit network in the Woodville Karst Plain, Florida SO SCIENTIFIC REPORTS LA English DT Article ID GROUNDWATER-FLOW; SALINE GROUNDWATER; YUCATAN PENINSULA; AQUIFER; WATER; SPRINGS; MEXICO; SYSTEM AB Five periods of increased electrical conductivity have been found in the karst conduits supplying one of the largest first magnitude springs in Florida with water. Numerous well-developed conduit networks are distributed in the Woodville Karst Plain (WKP), Florida and connected to the Gulf of Mexico. A composite analysis of precipitation and electrical conductivity data provides strong evidence that the increases in conductivity are directly tied to seawater intrusion moving inland and traveling 11 miles against the prevailing regional hydraulic gradient from from Spring Creek Spring Complex (SCSC), a group of submarine springs at the Gulf Coast. A geochemical analysis of samples from the spring vent rules out anthropogenic contamination and upwelling regional recharge from the deep aquifer as sources of the rising conductivity. The interpretation is supported by the conceptual model established by prior researchers working to characterize the study area. This paper documents the first and longest case of seawater intrusion in the WKP, and also indicates significant possibility of seawater contamination through subsurface conduit networks in a coastal karst aquifer. C1 [Xu, Zexuan; Hu, Bill] Florida State Univ, Dept Earth Ocean & Atmosphere Sci, Tallahassee, FL 32306 USA. [Bassett, Seth Willis; Dyer, Scott Barrett] Florida Geol Survey, Tallahassee, FL 32303 USA. [Hu, Bill] Jinan Univ, Dept Ecol, Guangzhou, Guangdong, Peoples R China. [Xu, Zexuan] Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. RP Hu, B (reprint author), Florida State Univ, Dept Earth Ocean & Atmosphere Sci, Tallahassee, FL 32306 USA.; Bassett, SW (reprint author), Florida Geol Survey, Tallahassee, FL 32303 USA.; Hu, B (reprint author), Jinan Univ, Dept Ecol, Guangzhou, Guangdong, Peoples R China. EM Seth.Bassett@dep.state.fl.us; bill.x.hu@gmail.com FU Woodville Karst Plain Project (WKPP) FX The authors would like to thank Kristopher Barrios and Edward Chelette for providing the NWFWMD datasets used in this article. We would also like to thank the divers of the Woodville Karst Plain Project (WKPP) for their fearless efforts and dedication to science. Without their efforts installing and maintaining the 2D-ACM sensors, this study would not have been possible. Finally, thank you to Alan Baker, Rick Green, Frank Rupert, and Dr. Jon Arthur at the Florida Geological Survey for reviewing and editing this document prior to its submission for publication. NR 40 TC 0 Z9 0 U1 7 U2 9 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 25 PY 2016 VL 6 AR 32235 DI 10.1038/srep32235 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DU0BS UT WOS:000381866900001 PM 27557803 ER PT J AU Weerawarna, PM Kim, Y Kankanamalage, ACG Damalanka, VC Lushington, GH Alliston, KR Mehzabeen, N Battaile, KP Lovell, S Chang, KO Groutas, WC AF Weerawarna, Pathum M. Kim, Yunjeong Kankanamalage, Anushka C. Galasiti Damalanka, Vishnu C. Lushington, Gerald H. Alliston, Kevin R. Mehzabeen, Nurjahan Battaile, Kevin P. Lovell, Scott Chang, Kyeong-Ok Groutas, William C. TI Structure-based design and synthesis of triazole-based macrocyclic inhibitors of norovirus protease: Structural, biochemical, spectroscopic, and antiviral studies SO EUROPEAN JOURNAL OF MEDICINAL CHEMISTRY LA English DT Article DE Norovirus; Macrocyclic inhibitors; beta-strand conformation; 3CL protease ID NORWALK VIRUS; POTENT INHIBITION; 3C-LIKE PROTEASES; DATA QUALITY; MACROMOLECULAR CRYSTALLOGRAPHY; SUBSTRATE-SPECIFICITY; 3CL PROTEASE; GASTROENTERITIS; DERIVATIVES; CYSTEINE AB Outbreaks of acute gastroenteritis caused by noroviruses constitute a public health concern worldwide. To date, there are no approved drugs or vaccines for the management and prophylaxis of norovirus infections. A potentially effective strategy for the development of norovirus therapeutics entails the discovery of inhibitors of norovirus 3CL protease, an enzyme essential for noroviral replication. We describe herein the structure-based design of the first class of permeable, triazole-based macrocyclic inhibitors of norovirus 3C-like protease, as well as pertinent X-ray crystallographic, biochemical, spectroscopic, and antiviral studies. Published by Elsevier Masson SAS. C1 [Weerawarna, Pathum M.; Kankanamalage, Anushka C. Galasiti; Damalanka, Vishnu C.; Alliston, Kevin R.; Groutas, William C.] Wichita State Univ, Dept Chem, Wichita, KS 67260 USA. [Kim, Yunjeong; Chang, Kyeong-Ok] Kansas State Univ, Coll Vet Med, Dept Diagnost Med & Pathobiol, Manhattan, KS 66506 USA. [Lushington, Gerald H.] LiS Consulting, Lawrence, KS 66046 USA. [Mehzabeen, Nurjahan; Lovell, Scott] Univ Kansas, Prot Struct Lab, Lawrence, KS 66047 USA. [Battaile, Kevin P.] APS Argonne Natl Lab, Hauptman Woodward Med Res Inst, IMCA CAT, Argonne, IL 60439 USA. RP Groutas, WC (reprint author), Wichita State Univ, Dept Chem, Wichita, KS 67260 USA.; Chang, KO (reprint author), Kansas State Univ, Coll Vet Med, Dept Diagnost Med & Pathobiol, Manhattan, KS 66506 USA. EM kchang@vet.ksu.edu; bill.groutas@wichita.edu RI Damalanka, Vishnu/S-3147-2016; OI Damalanka, Vishnu/0000-0002-1946-1320; Battaile, Kevin/0000-0003-0833-3259 FU National Institutes of Health [R01AI109039]; National Institute of General Medical Sciences of the National Institutes of Health [P30GM110761]; Industrial Macromolecular Crystallography Association; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The generous financial support of this work by the National Institutes of Health (R01AI109039) is gratefully acknowledged. Use of the University of Kansas Protein Structure Laboratory was supported by a grant from the National Institute of General Medical Sciences (P30GM110761) of the National Institutes of Health. Use of the IMCA-CAT beamline 17-ID at the Advanced Photon Source as supported by the companies of the Industrial Macromolecular Crystallography Association through a contract with Hauptman Woodward Medical Research Institute. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 56 TC 4 Z9 4 U1 6 U2 18 PU ELSEVIER FRANCE-EDITIONS SCIENTIFIQUES MEDICALES ELSEVIER PI PARIS PA 23 RUE LINOIS, 75724 PARIS, FRANCE SN 0223-5234 EI 1768-3254 J9 EUR J MED CHEM JI Eur. J. Med. Chem. PD AUG 25 PY 2016 VL 119 BP 300 EP 318 DI 10.1016/j.ejmech.2016.04.013 PG 19 WC Chemistry, Medicinal SC Pharmacology & Pharmacy GA DP3YZ UT WOS:000378433600020 PM 27235842 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buescher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L 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Wiik-Fuchs, L. A. M. Wildauer, A. Wilkens, H. G. Williams, H. H. Williams, S. Willis, C. Willocq, S. Wilson, A. Wilson, J. A. Wingerter-Seez, I. Winklmeier, F. Winter, B. T. Wittgen, M. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamada, M. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yao, W-M. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yurkewicz, A. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhan, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the CP-violating phase phi(s) and the B-s(0) meson decay width difference with B-s(0) -> J/psi phi decays in ATLAS SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE B physics; CP violation; Flavor physics; Hadron-Hadron scattering (experiments) AB A measurement of the B-s(0) decay parameters in the B-s(0) -> J/psi/phi channel using an integrated luminosity of 14.3 fb(-1) collected by the ATLAS detector from 8TeV pp collisions at the LHC is presented. The measured parameters include the CP-violating phase phi(s), the decay width Gamma(s) and the width di ff erence between the mass eigenstates Delta Gamma(s). The values measured for the physical parameters are statistically combined with those from 4.9 fb-1 of 7TeV data, leading to the following: phi(s) = -0.090 +/- 0.078 (stat.) +/- 0.041 (syst.) rad Delta Gamma s = 0.085 +/- 0.011 (stat.) +/- 0.007 (syst.) ps(-1) Gamma(s) = 0.675 +/- 0.003 (stat.) +/- 0.003 (syst:) ps(-1). In the analysis the parameter Delta Gamma(s) is constrained to be positive. Results for phi(s) and Delta Gamma(s) are also presented as 68% and 95% likelihood contours in the phi(s)-Delta Gamma(s) plane. Also measured in this decay channel are the transversity amplitudes and corresponding strong phases. All measurements are in agreement with the Standard Model predictions. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand 2, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, K.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Diglio, S.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Risti, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocm, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subat & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Saraiva, J. G.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Mandi, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandi, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, C.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giuliani, C.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] Northern Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Reichert, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Experimental Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dept Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, C.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Henkelmann, S.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Victoria, BC, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] Inst Catalana Rec & Estud Avancats, ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellenic Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Scuola Int Super Studi Avanzati, SISSA, Trieste, Italy. [Purohit, M.] Univ South Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RI Camarri, Paolo/M-7979-2015; Prokoshin, Fedor/E-2795-2012; Guo, Jun/O-5202-2015; Solodkov, Alexander/B-8623-2017; Yang, Haijun/O-1055-2015; Gladilin, Leonid/B-5226-2011; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Warburton, Andreas/N-8028-2013; Tikhomirov, Vladimir/M-6194-2015; Livan, Michele/D-7531-2012; Kuday, Sinan/C-8528-2014; Mitsou, Vasiliki/D-1967-2009; Garcia, Jose /H-6339-2015 OI Camarri, Paolo/0000-0002-5732-5645; Prokoshin, Fedor/0000-0001-6389-5399; Guo, Jun/0000-0001-8125-9433; Solodkov, Alexander/0000-0002-2737-8674; Gladilin, Leonid/0000-0001-9422-8636; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Warburton, Andreas/0000-0002-2298-7315; Tikhomirov, Vladimir/0000-0002-9634-0581; Livan, Michele/0000-0002-5877-0062; Kuday, Sinan/0000-0002-0116-5494; Mitsou, Vasiliki/0000-0002-1533-8886; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos, Thales; Aristeia programmes; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. NR 35 TC 1 Z9 1 U1 22 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 24 PY 2016 IS 8 AR 147 DI 10.1007/JHEP08(2016)147 PG 45 WC Physics, Particles & Fields SC Physics GA EH5AG UT WOS:000391784400001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Gay, APR Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MCM Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJ Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vu-Tova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M El-Khateeb, E Elkafrawy, T Mohamed, A Radi, A Salama, E Calpas, B 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Schnet-zer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Montalvo, R. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Azimuthal decorrelation of jets widely separated in rapidity in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments); proton-proton scattering; Forward physics; Jets; Particle correlations and fluctuations ID INELASTIC EP SCATTERING; CARLO GENERATOR CASCADE; PERTURBATION-THEORY; POMERON; QCD; MODEL; CCFM AB The decorrelation in the azimuthal angle between the most forward and the most backward jets (Mueller-Navelet jets) is measured in data collected in pp collisions with the CMS detector at the LHC at root s = 7 TeV. The measurement is presented in the form of distributions of azimuthal-angle differences, Delta phi, between the Mueller-Navelet jets, the average cosines of (pi - Delta phi), 2(pi - Delta phi), and 3(pi - Delta phi), and ratios of these cosines. The jets are required to have transverse momenta, p(T), in excess of 35 GeV and rapidities, |y|, of less than 4.7. The results are presented as a function of the rapidity separation, Delta y, between the Mueller-Navelet jets, reaching Delta y up to 9.4 for the first time. The results are compared to predictions of various Monte Carlo event generators and to analytical predictions based on the DGLAP and BFKL parton evolution schemes. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Abdulsalam, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Inst Rudjer Boskov, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [El-Khateeb, E.; Elkafrawy, T.; Mohamed, A.; Radi, A.; Salama, E.] Arab Republ Egypt, Acad Sci Res & Technol, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wend-Land, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] CNRS, Ecole Polytech, Lab Leprince Ringuet, IN2P3, Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Strasbourg, Univ Haute Alsace Mulhouse, CNRS, IN2P3,Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouze-vitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.; Xiao, H.] Univ Lyon, Univ Lyon 1, CNRS, IN2P3,Inst Phys Nucl Lyon, Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Tsamalaidze, Z.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst I, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A III, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B III, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Gallo, E.; Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Gan-guly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] Indian Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN, Sez Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] INFN, Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Firenze, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] INFN, Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] INFN, Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN, Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Napoli Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Maron, G.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN, Sez Pavia, Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] INFN, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Mazza, G.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] INFN, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Mis-iura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Ershov, A.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Lukina, O.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Pa-lencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Campderros, J. Duarte; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gok-bulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Cerci, D. Sunar; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Gold-stein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabe-dian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Con-way, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Calif State Univ Los Angeles, Los Angeles, CA 90032 USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chle-bana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khris-tenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksi-movic, P.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska Lincoln, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastren Univ, Boston, MA USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestren Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. 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A.; Polese, G.; Ross, I.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin Madison, Madison, WI USA. [Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, Vienna, Austria. [Rabady, D.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Ulmer, K. A.] CERN, European Org Nucl Res, Geneva, Switzerland. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Plestina, R.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, Palaiseau, France. [El-Khateeb, E.; Elkafrawy, T.; Radi, A.; Salama, E.] Ain Shams Univ, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Radi, A.; Salama, E.] British Univ Egypt, Cairo, Egypt. Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. Islam Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Maron, G.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Siena, Italy. [Ali, M. A. B. Md] Int Islam Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Konecki, Marcin/G-4164-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Goh, Junghwan/Q-3720-2016 OI Della Ricca, Giuseppe/0000-0003-2831-6982; Konecki, Marcin/0000-0001-9482-4841; TUVE', Cristina/0000-0003-0739-3153; Goh, Junghwan/0000-0002-1129-2083 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariata l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); Ministry of Science and Technology; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union; Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; Thalis and Aristeia programmes; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariata l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 57 TC 0 Z9 0 U1 16 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 24 PY 2016 IS 8 AR 139 DI 10.1007/JHEP08(2016)139 PG 41 WC Physics, Particles & Fields SC Physics GA EH5AE UT WOS:000391784200002 ER PT J AU Valdez, CA Leif, RN Alcaraz, A AF Valdez, Carlos A. Leif, Roald N. Alcaraz, Armando TI Effective methylation of phosphonic acids related to chemical warfare agents mediated by trimethyloxonium tetrafluoroborate for their qualitative detection and identification by gas chromatography-mass spectrometry SO ANALYTICA CHIMICA ACTA LA English DT Article DE Methylation; Trimethyloxonium; Phosphonic acid; Nerve agent; Derivatization; Aminoethylsulfonic acids ID DEGRADATION-PRODUCTS; NERVE AGENTS; DERIVATIZATION; DECONTAMINATION; RESIDUES; ATTACK AB The effective methylation of phosphonic acids related to chemical warfare agents (CWAs) employing trimethyloxonium tetrafluoroborate (TMO center dot BF4) for their qualitative detection and identification by gas chromatography-mass spectrometry (GC-MS) is presented. The methylation occurs in rapid fashion (1 h) and can be conveniently carried out at ambient temperature, thus providing a safer alternative to the universally employed diazomethane-based methylation protocols. Optimization of the methylation parameters led us to conclude that methylene chloride was the ideal solvent to carry out the derivatization, and that even though methylated products can be observed surfacing after only 1 h, additional time was not found to be detrimental but beneficial to the process particularly when dealing with analytes at low concentrations (similar to 10 mgmL(-1)). Due to its insolubility in methylene chloride, TMO center dot BF4 conveniently settles to the bottom during the reaction and does not produce additional interfering by-products that may further complicate the GC-MS analysis. The method was demonstrated to successfully methylate a variety of Schedule 2 phosphonic acids, including their half esters, resulting in derivatives that were readily detected and identified using the instrument's spectral library. Most importantly, the method was shown to simultaneously methylate a mixture of the organophosphorus-based nerve agent hydrolysis products: pinacolyl methylphosphonate (PMPA), cyclohexyl methylphosphonate (CyMPA) and ethyl methylphosphonate (EMPA) (aat a 10 mg mL(-1) concentration each) in a fatty acid ester-rich organic matrix (OPCW-PT-O3) featured in the 38th Organisation for the Prohibition of Chemical Weapons (OPCW) Proficiency Test. In addition, the protocol was found to effectively methylate N, N-diethylamino ethanesulfonic acid and N, N-diisopropylamino ethanesulfonic acid that are products arising from the oxidative degradation of the V-series agents VR and VX respectively. The work described herein represents the first report on the use of TMO center dot BF4 as a viable, stable and safe agent for the methylation of phosphonic acids and their half esters and within the context of an OPCW Proficiency Test sample analysis. (C) 2016 Elsevier B.V. All rights reserved. C1 [Valdez, Carlos A.; Leif, Roald N.; Alcaraz, Armando] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Valdez, Carlos A.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94550 USA. [Valdez, Carlos A.; Leif, Roald N.; Alcaraz, Armando] Lawrence Livermore Natl Lab, Forens Sci Ctr, Livermore, CA 94550 USA. RP Valdez, CA (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Nucl & Chem Sci & Forens Sci Ctr, L-091, Livermore, CA 94550 USA. EM valdez11@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 37 TC 0 Z9 0 U1 7 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0003-2670 EI 1873-4324 J9 ANAL CHIM ACTA JI Anal. Chim. Acta PD AUG 24 PY 2016 VL 933 BP 134 EP 143 DI 10.1016/j.aca.2016.05.034 PG 10 WC Chemistry, Analytical SC Chemistry GA DS5UX UT WOS:000380849400015 PM 27497006 ER PT J AU van den Hurk, B Kim, HJ Krinner, G Seneviratne, SI Derksen, C Oki, T Douville, H Colin, J Ducharne, A Cheruy, F Viovy, N Puma, MJ Wada, Y Li, WP Jia, BH Alessandri, A Lawrence, DM Weedon, GP Ellis, R Hagemann, S Mao, JF Flanner, MG Zampieri, M Materia, S Law, RM Sheffield, J AF van den Hurk, Bart Kim, Hyungjun Krinner, Gerhard Seneviratne, Sonia I. Derksen, Chris Oki, Taikan Douville, Herve Colin, Jeanne Ducharne, Agnes Cheruy, Frederique Viovy, Nicholas Puma, Michael J. Wada, Yoshihide Li, Weiping Jia, Binghao Alessandri, Andrea Lawrence, Dave M. Weedon, Graham P. Ellis, Richard Hagemann, Stefan Mao, Jiafu Flanner, Mark G. Zampieri, Matteo Materia, Stefano Law, Rachel M. Sheffield, Justin TI LS3MIP (v1.0) contribution to CMIP6: the Land Surface, Snow and Soil moisture Model Intercomparison Project - aims, setup and expected outcome SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID EARTH SYSTEM MODELS; CLIMATE-CHANGE; CARBON-DIOXIDE; INTERANNUAL VARIABILITY; ALBEDO FEEDBACK; BIASES; WATER; PREDICTABILITY; CRYOSPHERE; TRENDS AB The Land Surface, Snow and Soil Moisture Model Intercomparison Project (LS3MIP) is designed to provide a comprehensive assessment of land surface, snow and soil moisture feedbacks on climate variability and climate change, and to diagnose systematic biases in the land modules of current Earth system models (ESMs). The solid and liquid water stored at the land surface has a large influence on the regional climate, its variability and predictability, including effects on the energy, water and carbon cycles. Notably, snow and soil moisture affect surface radiation and flux partitioning properties, moisture storage and land surface memory. They both strongly affect atmospheric conditions, in particular surface air temperature and precipitation, but also large-scale circulation patterns. However, models show divergent responses and representations of these feedbacks as well as systematic biases in the underlying processes. LS3MIP will provide the means to quantify the associated uncertainties and better constrain climate change projections, which is of particular interest for highly vulnerable regions (densely populated areas, agricultural regions, the Arctic, semi-arid and other sensitive terrestrial ecosystems). The experiments are subdivided in two components, the first addressing systematic land biases in offline mode ("LMIP", building upon the 3rd phase of Global Soil Wetness Project; GSWP3) and the second addressing land feedbacks attributed to soil moisture and snow in an integrated framework ("LFMIP", building upon the GLACE-CMIP blueprint). C1 [van den Hurk, Bart] KNMI, De Bilt, Netherlands. [Kim, Hyungjun; Oki, Taikan] Univ Tokyo, Inst Ind Sci, Tokyo, Japan. [Krinner, Gerhard] CNRS, LGGE, Grenoble, France. [Seneviratne, Sonia I.] Swiss Fed Inst Technol, Inst Atmospher & Climate Sci, Zurich, Switzerland. [Derksen, Chris] Environm & Climate Change, Div Climate Res, Toronto, ON, Canada. [Douville, Herve; Colin, Jeanne] Meteo France, CNRM, Toulouse, France. [Cheruy, Frederique] Univ Paris 06, Ecole Polytech, Ecole Normale Super, LMD IPSL,CNRS, Paris, France. [Viovy, Nicholas] LSCE IPSL CEA CNRS UVSQ, Gif Sur Yvette, France. [Puma, Michael J.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Puma, Michael J.] Columbia Univ, Ctr Climate Syst Res, New York, NY USA. [Wada, Yoshihide] Int Inst Appl Syst Anal, Laxenburg, Austria. [Li, Weiping] China Meteorol Adm, Natl Climate Ctr, Lab Climate Studies, Beijing, Peoples R China. [Jia, Binghao] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Numer Modeling Atmospher Sci & Geop, Beijing, Peoples R China. [Alessandri, Andrea] Agenzia Nazl Nuove Tecnol Energia & Sviluppo Econ, Rome, Italy. [Lawrence, Dave M.] Natl Ctr Atmospher Res, Climate & Global Dynam Lab, POB 3000, Boulder, CO 80307 USA. [Weedon, Graham P.] Met Off JCHMR, Maclean Bldg, Wallingford, Oxon, England. [Ellis, Richard] Ctr Ecol & Hydrol, Maclean Bldg, Wallingford, Oxon, England. [Hagemann, Stefan] Max Planck Inst Meteorol, Hamburg, Germany. [Mao, Jiafu] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Mao, Jiafu] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Flanner, Mark G.] Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. [Zampieri, Matteo; Materia, Stefano] Euromediterranean Ctr Climate Change CMCC, Climate Simulat & Predict Div, Bologna, Italy. [Law, Rachel M.] CSIRO Oceans & Atmosphere, Aspendale, Vic, Australia. [Sheffield, Justin] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [Sheffield, Justin] Univ Southampton, Geog & Environm, Southampton, Hants, England. [Ducharne, Agnes] UPMC CNRS EPHE, Sorbonne Univ, UMR METIS 7619, Paris, France. RP van den Hurk, B (reprint author), KNMI, De Bilt, Netherlands. EM hurkvd@knmi.nl RI Oki, Taikan/E-5778-2010; Krinner, Gerhard/A-6450-2011; Weedon, Graham/B-7574-2008; Flanner, Mark/C-6139-2011; Mao, Jiafu/B-9689-2012; Law, Rachel/A-1969-2012; OI Oki, Taikan/0000-0003-4067-4678; Krinner, Gerhard/0000-0002-2959-5920; Weedon, Graham/0000-0003-1262-9984; Flanner, Mark/0000-0003-4012-174X; Mao, Jiafu/0000-0002-2050-7373; Law, Rachel/0000-0002-7346-0927; Seneviratne, Sonia/0000-0001-9528-2917 FU Joint UK DECC/Defra Met Office Hadley Climate Centre Programme [GA01101]; Biogeochemistry-Climate Feedbacks Scientific Focus Area project funded through the Regional and Global Climate Modeling Program in Climate and Environmental Sciences Division (CESD) of the (BER) Program in the; DOE [DE-AC05-00OR22725]; Japan Society for the Promotion of Science KAKENHI [16H06291] FX The authors thank the CMIP panel of the WCRP Working Group on Climate Modelling for their efforts in coordinating the CMIP6 enterprise. Graham R Weedon was supported by the Joint UK DECC/Defra Met Office Hadley Climate Centre Programme (GA01101). Jiafu Mao is supported by the Biogeochemistry-Climate Feedbacks Scientific Focus Area project funded through the Regional and Global Climate Modeling Program in Climate and Environmental Sciences Division (CESD) of the Biological and Environmental Research (BER) Program in the U.S. Department of Energy (DOE) Office of Science. Oak Ridge National Laboratory is managed by UT-BATTELLE for DOE under contract DE-AC05-00OR22725. H. Kim and T. Oki were supported by Japan Society for the Promotion of Science KAKENHI (16H06291). Hanna Lee (NorESM) has expressed intention to participate in LS3MIP when feasible, but has not contributed to this manuscript. NR 107 TC 1 Z9 1 U1 11 U2 11 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X EI 1991-9603 J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PD AUG 24 PY 2016 VL 9 IS 8 BP 2809 EP 2832 DI 10.5194/gmd-9-2809-2016 PG 24 WC Geosciences, Multidisciplinary SC Geology GA DW6ZQ UT WOS:000383800400002 ER PT J AU Liao, HC Tam, TLD Guo, PJ Wu, YL Manley, EF Huang, W Zhou, NJ Soe, CMM Wang, BH Wasielewski, MR Chen, LX Kanatzidis, MG Facchetti, A Chang, RPH Marks, TJ AF Liao, Hsueh-Chung Tam, Teck Lip Dexter Guo, Peijun Wu, Yilei Manley, Eric F. Huang, Wei Zhou, Nanjia Soe, Chan Myae Myae Wang, Binghao Wasielewski, Michael R. Chen, Lin X. Kanatzidis, Mercouri G. Facchetti, Antonio Chang, Robert P. H. Marks, Tobin J. TI Dopant-Free Hole Transporting Polymers for High Efficiency, Environmentally Stable Perovskite Solar Cells SO ADVANCED ENERGY MATERIALS LA English DT Article ID HIGH-PERFORMANCE; HALIDE PEROVSKITES; THIN-FILM; CONJUGATED POLYMER; CHARGE-TRANSPORT; LITHIUM-SALTS; SPIRO-OMETAD; CH3NH3PBI3; ELECTRON; LAYERS AB Over the past five years, a rapid progress in organometal-halide perovskite solar cells has greatly influenced emerging solar energy science and technology. In perovksite solar cells, the overlying hole transporting material (HTM) is critical for achieving high power conversion efficiencies (PCEs) and for protecting the air-sensitive perovskite active layer. This study reports the synthesis and implementation of a new polymeric HTM series based on semiconducting 4,8-dithien-2-yl-benzo[1,2-d;4,5-d']bistriazole-alt-benzo[1,2-b:4,5-b'] dithiophenes (pBBTa-BDTs), yielding high PCEs and environmentally-stable perovskite cells. These intrinsic (dopant-free) HTMs achieve a stabilized PCE of 12.3% in simple planar heterojunction cells-the highest value to date for a polymeric intrinsic HTM. This high performance is attributed to efficient hole extraction/collection (the most efficient pBBTa-BDT is highly ordered and orients pi-face-down on the perovskite surface) and balanced electron/hole transport. The smooth, conformal polymer coatings suppress aerobic perovskite film degradation, significantly enhancing the solar cell 85 degrees C/65% RH PCE stability versus typical molecular HTMs. C1 [Liao, Hsueh-Chung; Guo, Peijun; Wu, Yilei; Zhou, Nanjia; Chang, Robert P. H.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Liao, Hsueh-Chung; Tam, Teck Lip Dexter; Manley, Eric F.; Huang, Wei; Soe, Chan Myae Myae; Wang, Binghao; Wasielewski, Michael R.; Chen, Lin X.; Kanatzidis, Mercouri G.; Facchetti, Antonio; Marks, Tobin J.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Liao, Hsueh-Chung; Guo, Peijun; Zhou, Nanjia; Soe, Chan Myae Myae; Wasielewski, Michael R.; Chen, Lin X.] Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, Evanston, IL 60208 USA. [Tam, Teck Lip Dexter] ASTAR, IMRE, Fusionopolis Way,Innovis 08-03, Singapore 138634, Singapore. [Manley, Eric F.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Facchetti, Antonio] Polyera Corp, Skokie, IL 60077 USA. RP Chang, RPH (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.; Wasielewski, MR; Chen, LX; Kanatzidis, MG; Facchetti, A; Marks, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Wasielewski, MR; Chen, LX (reprint author), Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, Evanston, IL 60208 USA.; Chen, LX (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.; Facchetti, A (reprint author), Polyera Corp, Skokie, IL 60077 USA. EM m-wasielewski@northwestern.edu; lchen@anl.gov; m-kanatzidis@northwestern.edu; a-facchetti@northwestern.edu; r-chang@northwestern.edu; t-marks@northwestern.edu RI Guo, Peijun/I-1964-2013; WANG, BINGHAO/O-6881-2016; Wu, Yilei/O-5404-2014 OI Guo, Peijun/0000-0001-5732-7061; WANG, BINGHAO/0000-0002-9631-6901; Wu, Yilei/0000-0001-6756-1855 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-SC0001059]; Agency of Science, Technology and Research (A*STAR, Singapore); Ministry of Science and Technology of Taiwan; U.S. DOE [DE-AC02-06CH11357] FX H.-C.L. and T.L.D.T. contributed equally to this work. This research was supported by the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Award Number DE-SC0001059. T.L.D.T acknowledges the Agency of Science, Technology and Research (A*STAR, Singapore) for a postdoctoral fellowship. H.-C.L. acknowledges the Ministry of Science and Technology of Taiwan for a postdoctoral fellowship. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 72 TC 2 Z9 2 U1 69 U2 73 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD AUG 24 PY 2016 VL 6 IS 16 AR 1600502 DI 10.1002/aenm.201600502 PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DV9QS UT WOS:000383276600008 ER PT J AU Everroad, RC Stuart, RK Bebout, BM Detweiler, AM Lee, JZ Woebken, D Prufert-Bebout, L Pett-Ridge, J AF Everroad, R. Craig Stuart, Rhona K. Bebout, Brad M. Detweiler, Angela M. Lee, Jackson Z. Woebken, Dagmar Prufert-Bebout, Leslie Pett-Ridge, Jennifer TI Permanent draft genome of strain ESFC-1: ecological genomics of a newly discovered lineage of filamentous diazotrophic cyanobacteria SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Cyanobacteria; Nitrogen fixation; Hydrogenase; Intertidal microbial mat ID PHOTOSYNTHETIC MICROBIAL MATS; OXYGENIC PHOTOSYNTHESIS; HYDROGEN METABOLISM; MAXIMUM-LIKELIHOOD; DIVERSITY; IDENTIFICATION; PHYLOGENIES; ALGORITHMS; ORGANISMS; FIXATION AB The nonheterocystous filamentous cyanobacterium, strain ESFC-1, is a recently described member of the order Oscillatoriales within the Cyanobacteria. ESFC-1 has been shown to be a major diazotroph in the intertidal microbial mat system at Elkhorn Slough, CA, USA. Based on phylogenetic analyses of the 16S RNA gene, ESFC-1 appears to belong to a unique, genus-level divergence; the draft genome sequence of this strain has now been determined. Here we report features of this genome as they relate to the ecological functions and capabilities of strain ESFC-1. The 5,632,035 bp genome sequence encodes 4914 protein-coding genes and 92 RNA genes. One striking feature of this cyanobacterium is the apparent lack of either uptake or bi-directional hydrogenases typically expected within a diazotroph. Additionally, a large genomic island is found that contains numerous low GC-content genes and genes related to extracellular polysaccharide production and cell wall synthesis and maintenance. C1 [Everroad, R. Craig; Bebout, Brad M.; Detweiler, Angela M.; Lee, Jackson Z.; Woebken, Dagmar; Prufert-Bebout, Leslie] NASA, Exobiol Branch, Ames Res Ctr, Moffett Field, CA 94035 USA. [Everroad, R. Craig; Detweiler, Angela M.; Lee, Jackson Z.] Bay Area Environm Res Inst, Petaluma, CA 94952 USA. [Stuart, Rhona K.; Pett-Ridge, Jennifer] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA USA. [Woebken, Dagmar] Univ Vienna, Res Network Chem Meets Microbiol, Div Microbial Ecol, Dept Microbiol & Ecosyst Sci, Vienna, Austria. RP Everroad, RC (reprint author), NASA, Exobiol Branch, Ames Res Ctr, Moffett Field, CA 94035 USA.; Everroad, RC (reprint author), Bay Area Environm Res Inst, Petaluma, CA 94952 USA. EM craig.everroad@nasa.gov OI Woebken, Dagmar/0000-0002-1314-9926; Stuart, Rhona/0000-0001-5916-9693 FU US. DOE Genomic Science Program [SCW1039]; Community Sequencing Project 'Microbial Interactions in Extremophilic Mat Communities' at the DOE JGI [701]; Office of Science of the U.S. DOE [DE-AC02-05CH11231]; US DOE at Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Funding was provided by the US. DOE Genomic Science Program under contract SCW1039. Sequencing and support was provided by Community Sequencing Project #701 'Microbial Interactions in Extremophilic Mat Communities' at the DOE JGI. Work conducted by the U.S. DOE-JGI was supported by the Office of Science of the U.S. DOE Under Contract No. DE-AC02-05CH11231. Work at LLNL was performed under the auspices of the US DOE at Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. We thank Jeff Cann, Associate Wildlife Biologist, Central Region, California Department of Fish and Wildlife, for coordinating our access to the Moss Landing Wildlife Area. NR 45 TC 0 Z9 0 U1 5 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD AUG 24 PY 2016 VL 11 AR 53 DI 10.1186/s40793-016-0174-6 PG 8 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DW8PU UT WOS:000383918800002 PM 27559430 ER PT J AU Zarzar, LD Swartzentruber, BS Donovan, BF Hopkins, PE Kaehr, B AF Zarzar, Lauren D. Swartzentruber, B. S. Donovan, Brian F. Hopkins, Patrick E. Kaehr, Bryan TI Using Laser-Induced Thermal Voxels to Pattern Diverse Materials at the Solid-Liquid Interface SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE laser direct write; laser-induced heating Ni electrode; solvothermal synthesis; metals; microstructures ID INDUCED HYDROTHERMAL GROWTH; MULTIPHOTON LITHOGRAPHY; ONE-STEP; COPPER; NANOPARTICLE; DEPOSITION; POLYIMIDE; SURFACES; DESIGN; PHASE AB We describe a high-resolution patterning approach that combines the spatial control inherent to laser direct writing with the versatility of benchtop chemical synthesis. By taking advantage of the steep thermal gradient that occurs while laser heating a metal edge in contact with solution, diverse materials comprising transition metals are patterned with feature size resolution nearing 1 mu m. We demonstrate fabrication of reduced metallic nickel in one step and examine electrical properties and air stability through direct-write integration onto a device platform. This strategy expands the chemistries and materials that can be used in combination with laser direct writing. C1 [Zarzar, Lauren D.] Penn State Univ, Dept Mat Sci & Engn, Dept Chem, University Pk, PA 16802 USA. [Swartzentruber, B. S.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87545 USA. [Donovan, Brian F.; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Kaehr, Bryan] Sandia Natl Labs, Adv Mat Lab, POB 5800, Albuquerque, NM 87185 USA. [Kaehr, Bryan] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. RP Zarzar, LD (reprint author), Penn State Univ, Dept Mat Sci & Engn, Dept Chem, University Pk, PA 16802 USA.; Kaehr, B (reprint author), Sandia Natl Labs, Adv Mat Lab, POB 5800, Albuquerque, NM 87185 USA.; Kaehr, B (reprint author), Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. EM ldz4@psu.edu; bjkaehr@sandia.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Naval Research [N00014-15-12769]; U.S. Department of Energy's National Nuclear Security Administration [DE AC04-94AL85000] FX We thank Prof. Joanna Aizenberg for her support and helpful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. BFD and PEH appreciate funding from the Office of Naval Research, Grant #N00014-15-12769. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE AC04-94AL85000. NR 32 TC 1 Z9 1 U1 7 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 24 PY 2016 VL 8 IS 33 BP 21134 EP 21139 DI 10.1021/acsami.6b06625 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU4JR UT WOS:000382179400002 PM 27491598 ER PT J AU Zhang, Y Guo, XM Wu, F Yao, Y Yuan, YF Bi, XX Luo, XY Shahbazian-Yassar, R Zhang, CZ Amine, K AF Zhang, Yan Guo, Xingming Wu, Feng Yao, Ying Yuan, Yifei Bi, Xuanxuan Luo, Xiangyi Shahbazian-Yassar, Reza Zhang, Cunzhong Amine, Khalil TI Mesocarbon Microbead Carbon-Supported Magnesium Hydroxide Nanoparticles: Turning Spent Li-ion Battery Anode into a Highly Efficient Phosphate Adsorbent for Wastewater Treatment SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE spent Li-ion battery; phosphate; adsorption; magnesium hydroxide; anode ID LAYERED DOUBLE HYDROXIDES; SLOW-RELEASE FERTILIZER; SUGAR-BEET TAILINGS; AQUEOUS-SOLUTION; COIR-PITH; BIOCHAR NANOCOMPOSITES; POTENTIAL APPLICATION; SECONDARY BATTERIES; OXIDE NANOPARTICLES; ENHANCED ADSORPTION AB Phosphorus in water eutrophication has become a serious problem threatening the environment. However, the development of efficient adsorbents for phosphate removal from water is lagging. In this work, we recovered the waste material, graphitized carbon, from spent lithium ion batteries and modified it with nanostructured Mg(OH)(2) on the surface to treat excess phosphate. This phosphate adsorbent shows one of the highest phosphate adsorption capacities to date, 588.4 mg/g (1 order of magnitude higher than previously reported carbon-based adsorbents), and exhibits decent stability. A heterogeneous multilayer adsorption mechanism was proposed on the basis of multiple adsorption results. This highly efficient adsorbent from spent Li-ion batteries displays great potential to be utilized in industry, and the mechanism study paved a way for further design of the adsorbent for phosphate adsorption. C1 [Zhang, Yan; Guo, Xingming; Wu, Feng; Yao, Ying; Zhang, Cunzhong] Beijing Inst Technol, Beijing Key Lab Environm Sci & Engn, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Zhang, Yan; Guo, Xingming; Wu, Feng; Yao, Ying; Zhang, Cunzhong] Natl Dev Ctr High Technol Green Mat, Beijing 100081, Peoples R China. [Yuan, Yifei; Bi, Xuanxuan; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. [Luo, Xiangyi] Argonne Natl Lab, Div Mat Sci, 9700 South Cass Ave, Argonne, IL 60439 USA. [Yuan, Yifei; Shahbazian-Yassar, Reza] Michigan Technol Univ, Dept Mat Sci & Engn, 1400 Townsend Dr, Houghton, MI 49931 USA. [Bi, Xuanxuan] Ohio State Univ, Dept Chem & Biochem, 100 West 18th Ave, Columbus, OH 43210 USA. RP Yao, Y (reprint author), Beijing Inst Technol, Beijing Key Lab Environm Sci & Engn, Sch Mat Sci & Engn, Beijing 100081, Peoples R China.; Yao, Y (reprint author), Natl Dev Ctr High Technol Green Mat, Beijing 100081, Peoples R China. EM yaoying@bit.edu.cn FU National Natural Science Foundation of China (NSFC) [51402018]; National Key Program for Basic Research of China [2015CB251100]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This research was supported by the National Natural Science Foundation of China (NSFC) through Grant 51402018 and the National Key Program for Basic Research of China through Grant 2015CB251100. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 75 TC 0 Z9 0 U1 29 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 24 PY 2016 VL 8 IS 33 BP 21315 EP 21325 DI 10.1021/acsami.6b05458 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU4JR UT WOS:000382179400022 PM 27463402 ER PT J AU Bagheri, M Masoomi, MY Morsali, A Schoedel, A AF Bagheri, Minoo Masoomi, Mohammad Yaser Morsali, Ali Schoedel, Alexander TI Two Dimensional Host-Guest Metal-Organic Framework Sensor with High Selectivity and Sensitivity to Picric Acid SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE ratiometric fluorescent sensor; metal-organic frameworks; picric acid; sensitivity; selectivity ID EXPLOSIVE NITROAROMATIC COMPOUNDS; POROUS COORDINATION POLYMER; TUNABLE PHOTOLUMINESCENCE; GAS-SENSORS; LUMINESCENT; MOLECULES; CO2; PHOSPHORESCENCE; ADSORPTION; MORPHOLOGY AB A dye-sensitized metal organic framework, TMU-5S, was synthesized based on introducing the laser dye Rhodamine B into the porous framework TMU-5. TMU-5S was investigated as a ratiometric fluorescent sensor for the detection of explosive nitro aromatic compounds and showed four times greater selectivity to picric acid than any state-of-the-art luminescent-based sensor. Moreover, it can selectively discriminate picric acid concentrations in the presence of other nitro aromatics and volatile organic compounds. Our findings indicate that using this sensor in two dimensions leads to a greatly reduced environmental interference response and thus creates exceptional sensitivity toward explosive molecules with a fast response. C1 [Bagheri, Minoo; Masoomi, Mohammad Yaser; Morsali, Ali] Tarbiat Modares Univ, Dept Chem, Fac Sci, Tehran 1411713116, Iran. [Schoedel, Alexander] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Schoedel, Alexander] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Schoedel, Alexander] Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. RP Morsali, A (reprint author), Tarbiat Modares Univ, Dept Chem, Fac Sci, Tehran 1411713116, Iran. EM morsali_a@modares.ac.ir RI Schoedel, Alexander/B-3971-2013; OI Schoedel, Alexander/0000-0001-6548-9300; Masoomi, Mohammad Yaser/0000-0003-1329-5947 FU Tarbiat Modares University; German Research Foundation (DFG) [SCHO 1639/1-1] FX Support of this investigation by Tarbiat Modares University is gratefully acknowledged. A.S. gratefully acknowledges the German Research Foundation (DFG, SCHO 1639/1-1) for financial support. The authors would like to thank Zhe Ji (UC Berkeley) for producing the TOC graphics. NR 53 TC 5 Z9 5 U1 43 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 24 PY 2016 VL 8 IS 33 BP 21472 EP 21479 DI 10.1021/acsami.6b06955 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU4JR UT WOS:000382179400041 PM 27479837 ER PT J AU Siol, S Hellmann, JC Tilley, SD Graetzel, M Morasch, J Deuermeier, J Jaegermann, W Klein, A AF Siol, Sebastian Hellmann, Jan C. Tilley, S. David Graetzel, Michael Morasch, Jan Deuermeier, Jonas Jaegermann, Wolfram Klein, Andreas TI Band Alignment Engineering at Cu2O/ZnO Heterointerfaces SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE band alignment; Cu2O; ZnO; XPS; interface experiment; Fermi level pinning; band offset ID HETEROJUNCTION SOLAR-CELLS; SCHOTTKY-BARRIER FORMATION; FERMI-LEVEL; ELECTRICAL-PROPERTIES; INTERFACE; OXIDES; OFFSET; LAYER; TRANSITION; DIPOLES AB Energy band alignments at heterointerfaces play a crucial role in defining the functionality of semiconductor devices, yet the search for material combinations with suitable band alignments remains a challenge for numerous applications. In this work, we demonstrate how changes in deposition conditions can dramatically influence the functional properties of an interface, even within the same material system. The energy band alignment at the heterointerface between Cu2O and ZnO was studied using photoelectron spectroscopy with stepwise deposition of ZnO onto Cu2O and vice versa. A large variation of energy band alignment depending on the deposition conditions of the substrate and the film is observed, with valence band offsets in the range Delta E-VB = 1.45-2.7 eV. The variation of band alignment is accompanied by the occurrence or absence of band bending in either material. It can therefore be ascribed to a pinning of the Fermi level in ZnO and Cu2O, which can be traced back to oxygen vacancies in ZnO and to metallic precipitates in Cu2O. The intrinsic valence band offset for the interface, which is not modified by Fermi level pinning, is derived as Delta E-VB approximate to 1.5 eV, being favorable for solar cell applications. C1 [Siol, Sebastian; Hellmann, Jan C.; Morasch, Jan; Jaegermann, Wolfram; Klein, Andreas] Tech Univ Darmstadt, Inst Mat Sci, Div Surface Sci, Petersenstr 32, D-64287 Darmstadt, Germany. [Tilley, S. David; Graetzel, Michael] Ecole Polytech Fed Lausanne, Inst Sci & Ingn Chim, Lab Photon & Interfaces, Stn 6, CH-1015 Lausanne, Switzerland. [Deuermeier, Jonas] Univ Nova Lisboa, CENIMAT i3N, Campus Caparica, P-2829516 Caparica, Portugal. [Deuermeier, Jonas] CEMOP UNINOVA, Dept Mat Sci, Fac Sci & Technol, Campus Caparica, P-2829516 Caparica, Portugal. [Tilley, S. David] Univ Zurich, Dept Chem, Winterthurerstr 190, CH-8057 Zurich, Switzerland. [Siol, Sebastian] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Siol, S; Klein, A (reprint author), Tech Univ Darmstadt, Inst Mat Sci, Div Surface Sci, Petersenstr 32, D-64287 Darmstadt, Germany. EM siol.sebastian@googlemail.com; aklein@surface.tu-darmstadt.de RI Klein, Andreas/E-6081-2010; OI Klein, Andreas/0000-0001-7463-1495; Siol, Sebastian/0000-0002-0907-6525; Deuermeier, Jonas/0000-0002-2764-3124 FU German Ministry for Education and Research (BMBF) [03SF0358A]; European Commission FP7 project All-Oxide PV; Swiss Federal Office for Energy (PECHouse Competence Center) [SI/500090-02] FX This work was supported by German Ministry for Education and Research (BMBF) under contract number 03SF0358A, the European Commission FP7 project All-Oxide PV, and the Swiss Federal Office for Energy (PECHouse Competence Center, contract number SI/500090-02). NR 69 TC 3 Z9 3 U1 42 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 24 PY 2016 VL 8 IS 33 BP 21824 EP 21831 DI 10.1021/acsami.6b07325 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DU4JR UT WOS:000382179400081 PM 27452037 ER PT J AU Chappa, S Das, S Debnath, AK Sahu, M Saxena, MK Pandey, AK AF Chappa, Sankararao Das, Sadananda Debnath, A. K. Sahu, Manjulata Saxena, Manoj K. Pandey, Ashok K. TI Spacer Monomer in Polymer Chain Influencing Affinity of Ethylene Glycol Methacrylate Phosphate toward UO22+ and Pu4+ Ions SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SOLVENT-EXTRACTION SYSTEM; METAL-IONS; PHASE-TRANSITIONS; REVERSE MICELLES; ACID; DIGLYCOLAMIDES; AGGREGATION; PRECONCENTRATION; URANIUM(VI); SEPARATION AB The complexation behavior of ligating groups bearing ethylene glycol methacrylate phosphate (EGMP) units spaced in the polymer chain was studied to understand the coordination ability of segregated EGMP toward UO22+ and Pu4+ ions. The EGMP units in the polymer chain were copolymerized with a varying mol proportion of spacer monomer N-isopropylacylamide (NIPA) and methyl methacrylate (MMA) along with a cross-linker. These copolymer gels were characterized by FTIR, SEM/EDS, and thermal analysis. It was observed that the copolymer gels had homogeneity and concentration of phosphate groups systematically decreased with an increase in mol proportion of spacer monomer units. The hydrophlicity of (EGMP-co-MMA) copolymer gels decreased with an increase in mol proportion of MMA units whereas hydrophilicty of EGMP-co-NIPA copolymer increased with an increase in mol proportion of NIPA units in the copolymer gels. It was observed that UO22+ ions sorption decreased with an increase in MMA units in the polymer chain at higher HNO3 conc. (3 mol L-1) but did not affect Pu4+ ions sorption. This seems to suggest that EGMP units segregated sufficiently in the polymer chain by spacers exhibit a remarkable selectivity toward Pt4+ ions with respect to UO22+ ions at high HNO3 conc. Pu(IV) ions are known to have high affinity toward nitrate ions that help in the formation of a stable complex at higher acidity with a lesser number of coordination with phosphate groups. The experiments showed that the lower affinity of poly(EGMP-co-MMA) gel toward UO22+ ions was not due to dilution of phosphate groups concentration in the copolymer gel but could be attributed to the coordination requirement of UO22+ ions to form a stable complex at higher HNO3 concentration. The X-ray photoelectron spectroscopy (XPS) and time-resolved laser-induced fluorescence spectroscopy (TRLFS) studies of poly(EGMP) loaded with UO22+ ions from aqueous solution having pH 2 and 3 mol L-1 HNO3 indicated that (i) 1:2 and 1:4 (UO22+-EGMP) complexes are formed at lower acidity and higher acidity, respectively, (ii) UO22+ ion is coordinated with water molecules at pH range in addition to the ion-exchange, and (iii) the complex formed in pH range has higher stability with respect to that form at 3 mol L-1 conc. The higher hydrophilic poly(EGMP-co-NIPA) gels at 25 degrees C exhibit higher UO22+ uptake in 3 M HNO3, as phosphate units in hydrophilic gel are mobile and could form stable complex involving 3-4 phosphoryl oxygen, which is not possible in collapsed state due to hydophobicity of polymer net work above critical temperature. However, there was no effect of hydrophilicty/hydrophobicity on the UO22+ ions sorption in the copolymer gels from solutions having lower HNO3 conc. due to a requirement of lesser number of EGMP units to form a stable complex. C1 [Chappa, Sankararao; Pandey, Ashok K.] Bhabha Atom Res Ctr, Radiochem Div, Mumbai 400085, Maharashtra, India. [Chappa, Sankararao; Pandey, Ashok K.] Homi Bhabha Natl Inst, Bombay 400094, Maharashtra, India. [Das, Sadananda] Oak Ridge Natl Lab, Div Chem Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Debnath, A. K.] Bhabha Atom Res Ctr, Tech Phys Div, Bombay 400085, Maharashtra, India. [Sahu, Manjulata; Saxena, Manoj K.] Bhabha Atom Res Ctr, Radioanalyt Chem Div, Bombay 400085, Maharashtra, India. RP Pandey, AK (reprint author), Bhabha Atom Res Ctr, Radiochem Div, Mumbai 400085, Maharashtra, India.; Pandey, AK (reprint author), Homi Bhabha Natl Inst, Bombay 400094, Maharashtra, India.; Das, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM amisdas@gmail.com; ashokk@barc.gov.in OI chappa, sankararao/0000-0003-1351-2892 FU Department of Atomic Energy, India FX S.C. thanks Department of Atomic Energy, India for providing fellowship for the Doctoral studies at Homi Bhabha National Institute, Mumbai. The authors are thankful to Mr. Nimai Pathak, Radiochemistry Division, BARC for help in time resolved laser-induced fluorescence spectroscopy, and Dr. P. K. Pujari, Head Radiochemistry Division, BARC for his keen interest in the present work. NR 33 TC 0 Z9 0 U1 4 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD AUG 24 PY 2016 VL 55 IS 33 BP 8992 EP 9002 DI 10.1021/acs.iecr.6b01534 PG 11 WC Engineering, Chemical SC Engineering GA DU4KN UT WOS:000382181600009 ER PT J AU Zhu, HL Luo, W Ciesielski, PN Fang, ZQ Zhu, JY Henriksson, G Himmel, ME Hu, LB AF Zhu, Hongli Luo, Wei Ciesielski, Peter N. Fang, Zhiqiang Zhu, J. Y. Henriksson, Gunnar Himmel, Michael E. Hu, Liangbing TI Wood-Derived Materials for Green Electronics, Biological Devices, and Energy Applications SO CHEMICAL REVIEWS LA English DT Review ID TEMPO-MEDIATED OXIDATION; LITHIUM-ION BATTERIES; REGENERATED CELLULOSE FILMS; ENHANCED RAMAN-SCATTERING; PLANT-CELL WALL; HIGH-PERFORMANCE SUPERCAPACITORS; OPTICALLY TRANSPARENT WOOD; CHIRAL NEMATIC SUSPENSIONS; NAOH/UREA AQUEOUS-SOLUTION; PAPER-BASED MICROFLUIDICS AB With the arising of global climate change and resource shortage, in recent years, increased attention has been paid to environmentally friendly materials. Trees are sustainable and renewable materials, which give us shelter and oxygen and remove carbon dioxide from the atmosphere. Trees are a primary resource that human society depends upon every day, for example, homes, heating, furniture, and aircraft. Wood from trees gives us paper, cardboard, and medical supplies, thus impacting our homes, school, work, and play. All of the above-mentioned applications have been well developed over the past thousands of years. However, trees and wood have much more to offer us as advanced materials, impacting emerging high-tech fields, such as bioengineering, flexible electronics, and clean energy. Wood naturally has a hierarchical structure, composed of well-oriented microfibers and tracheids for water, ion, and oxygen transportation during metabolism. At higher magnification, the walls of fiber cells have an interesting morphology-a distinctly mesoporous structure. Moreover, the walls of fiber cells are composed of thousands of fibers (or macrofibrils) oriented in a similar angle. Nanofibrils and nanocrystals can be further liberated from macrofibrils by mechanical, chemical, and enzymatic methods. The obtained nanocellulose has unique optical, mechanical, and barrier properties and is an excellent candidate for chemical modification and reconfiguration. Wood is naturally a composite material, comprised of cellulose, hemicellulose, and lignin. Wood is sustainable, earth abundant, strong, biodegradable, biocompatible, and chemically accessible for modification; more importantly, multiscale natural fibers from wood have unique optical properties applicable to different kinds of optoelectronics and photonic devices. Today, the materials derived from wood are ready to be explored for applications in new technology areas, such as electronics, biomedical devices, and energy. The goal of this study is to review the fundamental structures and chemistries of wood and wood-derived materials, which are essential for a wide range of existing and new enabling technologies. The scope of the review covers multiscale materials and assemblies of cellulose, hemicellulose, and lignin as well as other biomaterials derived from wood, in regard to their major emerging applications. Structure properties application relationships will be investigated in detail. Understanding the fundamental properties of these structures is crucial for designing and manufacturing products for emerging applications. Today, a more holistic understanding of the interplay between the structure, chemistry, and performance of wood and wood-derived materials is advancing historical applications of these materials. This new level of understanding also enables a myriad of new and exciting applications, which motivate this review. There are excellent reviews already on the classical topic of woody materials, and some recent reviews also cover new understanding of these materials as well as potential applications. This review will focus on the uniqueness of woody materials for three critical applications: green electronics, biological devices, and energy storage and bioenergy. C1 [Zhu, Hongli; Luo, Wei; Fang, Zhiqiang; Hu, Liangbing] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Zhu, Hongli] Northeastern Univ, Dept Mech & Ind Engn, Boston, MA 02115 USA. [Ciesielski, Peter N.; Himmel, Michael E.] Natl Renewable Energy Lab, Biosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Zhu, J. Y.] US Forest Serv, Forest Prod Lab, USDA, Madison, WI 53726 USA. [Henriksson, Gunnar] KTH, Royal Inst Technol, Dept Fiber & Polymer Technol, Div Wood Chem & Pulp Technol, Stockholm, Sweden. RP Zhu, HL; Hu, LB (reprint author), Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA.; Zhu, HL (reprint author), Northeastern Univ, Dept Mech & Ind Engn, Boston, MA 02115 USA. EM h.zhu@neu.edu; binghu@umd.edu RI Luo, Wei/E-1582-2011; Hu, Liangbing/N-6660-2013; OI Luo, Wei/0000-0002-4019-4634; Fang, Zhiqiang/0000-0002-0844-7507 FU DOD (Air Force of Scientific Research) Young Investigator Program [FA95501310143]; 3M Non-Tenured Faculty; NSF-CBET Grant [1335979]; Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DESC0001160]; National Renewable Energy Laboratory's Laboratory Directed Research and Development (LDRD) Program; Northeastern University FX L.H. acknowledges support from the DOD (Air Force of Scientific Research) Young Investigator Program (FA95501310143) and 3M Non-Tenured Faculty and NSF-CBET Grant 1335979. This work also was supported as part of the Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award DESC0001160. Sections 2.1 and 6.2 were written with support from the National Renewable Energy Laboratory's Laboratory Directed Research and Development (LDRD) Program (MEH and PNC). H.Z. acknowledges the startup support from Northeastern University. We also acknowledge Mr. Jiaqi Dai from the University of Maryland for the help on figures. NR 519 TC 14 Z9 14 U1 220 U2 264 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD AUG 24 PY 2016 VL 116 IS 16 BP 9305 EP 9374 DI 10.1021/acs.chemrev.6b00225 PG 70 WC Chemistry, Multidisciplinary SC Chemistry GA DU4JO UT WOS:000382179100005 PM 27459699 ER PT J AU Wang, YG Cantu, DC Lee, MS Li, J Glezakou, VA Rousseau, R AF Wang, Yang-Gang Cantu, David C. Lee, Mal-Soon Li, Jun Glezakou, Vassiliki-Alexandra Rousseau, Roger TI CO Oxidation on Au/TiO2: Condition-Dependent Active Sites and Mechanistic Pathways SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID INITIO MOLECULAR-DYNAMICS; DENSITY-FUNCTIONAL THEORY; WATER-GAS SHIFT; SINGLE-ATOM CATALYSIS; SUPPORTED GOLD; AU CLUSTERS; HETEROGENEOUS CATALYSIS; CHEMISORBED OXYGEN; PERIMETER SITES; OXIDE SUPPORTS AB We present results of ab initio electronic structure and molecular dynamics simulations (AIMD), as well as a microkinetic model of CO oxidation catalyzed by TiO2 supported Au nanocatalysts. A coverage-dependent microkinetic analysis, based on energetics obtained with density functional methods, shows that the dominant kinetic pathway, activated oxygen species, and catalytic active sites are all strongly depended on both temperature and oxygen partial pressure. Under oxidizing conditions and T < 400 K, the prevalent pathway involves a dynamic single atom catalytic mechanism. This reaction is catalyzed by a transient Au CO species that migrates from the Au-cluster onto a surface oxygen adatom. It subsequently reacts with the TiO2 support via a Mars van Krevelen mechanism to form CO2 and finally the Au atom reintegrates back into the gold cluster to complete the catalytic cycle. At 300 <= T <= 600 K, oxygen-bound single O-ad-Au+-CO sites and the perimeter Au-sites of the nanoparticle work in tandem to optimally catalyze the reaction. Above 600 K, a variety of alternate pathways associated with both single-atom and the perimeter sites of the Au nanoparticle are found to be active. Under low oxygen pressures, O-ad-Au+-CO species can be a source of catalyst deactivation and the dominant pathway involves only Au-perimeter sites. A detailed comparison of the current model and the existing literature resolves many apparent inconsistencies in the mechanistic interpretations. C1 [Wang, Yang-Gang; Cantu, David C.; Lee, Mal-Soon; Glezakou, Vassiliki-Alexandra; Rousseau, Roger] Pacific Northwest Natl Lab, Inst Interfacial Catalysis, Richland, WA 99354 USA. [Li, Jun] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China. RP Rousseau, R (reprint author), Pacific Northwest Natl Lab, Inst Interfacial Catalysis, Richland, WA 99354 USA. EM roger.rousseau@pnnl.gov RI Rousseau, Roger/C-3703-2014; Lee, Mal-Soon/K-4161-2013 OI Lee, Mal-Soon/0000-0001-6851-177X FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research; National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory FX This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences and performed at the Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for Department of Energy by Battelle. Computational resources were provided at W. R. Wiley Environmental Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at PNNL and the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. NR 92 TC 2 Z9 2 U1 140 U2 163 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 24 PY 2016 VL 138 IS 33 BP 10467 EP 10476 DI 10.1021/jacs.6b04187 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DU4KQ UT WOS:000382181900020 PM 27480512 ER PT J AU Diroll, BT Jishkariani, D Cargnello, M Murray, CB Donnio, B AF Diroll, Benjamin T. Jishkariani, Davit Cargnello, Matteo Murray, Christopher B. Donnio, Bertrand TI Polycatenar Ligand Control of the Synthesis and Self-Assembly of Colloidal Nanocrystals SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BINARY NANOPARTICLE SUPERLATTICES; LIQUID-CRYSTALLINE NANOPARTICLES; GOLD NANOPARTICLES; STRUCTURAL DIVERSITY; INORGANIC LIGANDS; SURFACE LIGANDS; CLICK CHEMISTRY; PACKING; DESIGN; METAMATERIAL AB Hydrophobic colloidal nanocrystals are typically synthesized and manipulated with commercially available ligands, and surface functionalization is therefore typically limited to a small number of molecules. Here, we report the use of polycatenar ligands derived from polyalkylbenzoates for the direct synthesis of metallic, chalcogenide, pnictide, and oxide nanocrystals. Polycatenar molecules, branched structures bearing diverging chains in which the terminal substitution pattern, functionality, and binding group can be independently modified, offer a modular platform for the development of ligands with targeted properties. Not only are these ligands used for the direct synthesis of monodisperse nanocrystals, but nanocrystals coated with polycatenar ligands self assemble into softer bcc superlattices that deviate from conventional harder dose-packed structures (fcc or hcp) formed by the same nanocrystals coated with commercial ligands. Self-assembly experiments demonstrate that the molecular structure of polycatenar ligands encodes interparticle spacings and attractions, engineering self-assembly, which is tunable from hard sphere to soft sphere behavior. C1 [Diroll, Benjamin T.; Jishkariani, Davit; Cargnello, Matteo; Murray, Christopher B.] Univ Penn, Dept Chem, Philadelphia, PA 19104 USA. [Jishkariani, Davit; Donnio, Bertrand] Univ Penn, CNRS Solvay, UMI 3254, Complex Assemblies Soft Matter Lab COMPASS, Bristol, PA 19007 USA. [Murray, Christopher B.] Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. [Donnio, Bertrand] Univ Strasbourg, CNRS, UMR 7504, IPCMS, F-67034 Strasbourg 2, France. [Diroll, Benjamin T.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Cargnello, Matteo] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. RP Murray, CB (reprint author), Univ Penn, Dept Chem, Philadelphia, PA 19104 USA.; Donnio, B (reprint author), Univ Penn, CNRS Solvay, UMI 3254, Complex Assemblies Soft Matter Lab COMPASS, Bristol, PA 19007 USA.; Murray, CB (reprint author), Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA.; Donnio, B (reprint author), Univ Strasbourg, CNRS, UMR 7504, IPCMS, F-67034 Strasbourg 2, France. EM cbmurray@sas.upenn.edu; bdonnio@ipcms.unistra.fr RI Donnio, Bertrand/I-1305-2016; OI Donnio, Bertrand/0000-0001-5907-7705; Jishkariani, Davit/0000-0003-3771-2645; Cargnello, Matteo/0000-0002-7344-9031 FU CNRS-UPENN-SOLVAY through the Complex Assemblies of Soft Matter Laboratory (COMPASS); University of Pennsylvania's NSF MRSEC [DMR-112090] FX The authors thank A. Travesset for helpful discussions and access to prepublication data and python scripts and K. Weigandt for assistance running SANS experiments. This work was supported by the CNRS-UPENN-SOLVAY through the Complex Assemblies of Soft Matter Laboratory (COMPASS), in partnership with the University of Pennsylvania's NSF MRSEC under Award No. DMR-112090. C.B.M. acknowledges the Richard Perry University Professorship at the University of Pennsylvania. NR 51 TC 0 Z9 0 U1 44 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 24 PY 2016 VL 138 IS 33 BP 10508 EP 10515 DI 10.1021/jacs.6b04979 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DU4KQ UT WOS:000382181900025 PM 27472457 ER PT J AU Moonshiram, D Gimbert-Surinach, C Guda, A Picon, A Lehrnann, CS Zhang, XY Doumy, G March, AM Benet-Buchholz, J Soldatov, A Llobet, A Southworth, SH AF Moonshiram, Dooshaye Gimbert-Surinach, Carolina Guda, Alexander Picon, Antonio Lehrnann, C. Stefan Zhang, Xiaoyi Doumy, Gilles March, Anne Marie Benet-Buchholz, Jordi Soldatov, Alexander Llobet, Antoni Southworth, Stephen H. TI Tracking the Structural and Electronic Configurations of a Cobalt Proton Reduction Catalyst in Water SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ELECTROCATALYTIC HYDROGEN EVOLUTION; TRANSIENT ABSORPTION-SPECTROSCOPY; CHARGE SEPARATION; AQUEOUS-SOLUTION; MOLECULAR CATALYSTS; IRON COMPLEXES; H-2 EVOLUTION; K-EDGE; COBALOXIME; STATE AB X-ray transient absorption spectroscopy (X-TAS) has been used to study the light-induced hydrogen evolution reaction catalyzed by a tetradentate macrocyclic cobalt complex with the formula [(LCoCl2)-Cl-III](+) (L = macrocyclic ligand), [Ru(bpy)(3)](2+) photosensitizer, and an equimolar mixture of sodium ascorbate/ascorbic acid electron donor in pure water. X-ray absorption near edge structure ()CANES) and extended X-ray absorption fine structure (EXAFS) analysis of a binary mixture of the octahedral Co(III) precatalyst and [Ru(bpy)(3)](2+) after illumination revealed in situ formation of a Co(II) intermediate with significantly distorted geometry and electron-transfer kinetics of 51 ns. On the other hand, X-TAS experiments of the complete photocatalytic system in the presence of the electron donor showed the formation of a square planar Co(I) intermediate species within a few nanoseconds, followed by its decay in the microsecond time scale. The Co(I) structural assignment is supported by calculations based on density functional theory (DFT). At longer reaction times, we observe the formation of the initial Co(Ill) species concomitant to the decay of Co(I), thus dosing the catalytic cycle. The experimental X-ray absorption spectra of the molecular species formed along the catalytic cycle are modeled using a combination of molecular orbital DFT calculations (DFT-MO) and finite difference method (FDM). These findings allowed us to assign the full mechanistic pathway, followed by the catalyst as well as to determine the rate-limiting step of the process, which consists in the protonation of the Co(I) species. This study provides a complete kinetics scheme for the hydrogen evolution reaction by a cobalt catalyst, revealing unique information for the development of better catalysts for the reductive side of hydrogen fuel cells. C1 [Moonshiram, Dooshaye; Picon, Antonio; Lehrnann, C. Stefan; Doumy, Gilles; March, Anne Marie; Southworth, Stephen H.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. [Zhang, Xiaoyi] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Lemont, IL 60439 USA. [Gimbert-Surinach, Carolina; Benet-Buchholz, Jordi; Llobet, Antoni] Barcelona Inst Sci & Technol, Inst Chem Res Catalonia ICIQ, Avinguda Paisos Catalans 16, Tarragona 43007, Spain. [Guda, Alexander; Soldatov, Alexander] Southern Fed Univ, Int Res Ctr Smart Mat, Rostov Na Donu 344090, Russia. [Llobet, Antoni] Univ Autonoma Barcelona, Dept Quim, E-08193 Barcelona, Spain. RP Moonshiram, D (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA.; Gimbert-Surinach, C; Llobet, A (reprint author), Barcelona Inst Sci & Technol, Inst Chem Res Catalonia ICIQ, Avinguda Paisos Catalans 16, Tarragona 43007, Spain.; Llobet, A (reprint author), Univ Autonoma Barcelona, Dept Quim, E-08193 Barcelona, Spain. EM dmoonshi@gmail.com; cgimbert@iciq.es; allobet@iciq.es RI Guda, Alexander/A-3671-2015; Moonshiram, Dooshaye/J-5138-2014; Soldatov, Alexander/E-9323-2012; Gimbert Surinach, Carolina/S-7373-2016 OI Guda, Alexander/0000-0002-6941-4987; Moonshiram, Dooshaye/0000-0002-9075-3035; Soldatov, Alexander/0000-0001-8411-0546; Gimbert Surinach, Carolina/0000-0002-4412-7607 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division [DE-AC02-06CH11357]; DOE Office of Science [DE-AC02-06CH11357]; MINECO; "Fondo Europeo de Desarrollo Regional" (FEDER) [CTQ-2013-49075-R, SEV-2013-0319, CTQ-2014-52974-REDC]; EU COST actions [CM1202, CM1205]; AGAUR; Generalitat de Catalunya; Russian Ministry of Education and Science [14.587.21.0002, RFMEFI58714X0002] FX We acknowledge support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division under contract no. DE-AC02-06CH11357. This research uses resources of the Advanced Photon Source(APS), a U.S Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. We thank Dr. Chengjun Sun, Dr. Steve Heald, and Dr. Qingyu Kong for help with experiments at beamlines 20 BM and 11 ID-D, APS. We also acknowledge financial support from MINECO and the "Fondo Europeo de Desarrollo Regional" (FEDER) through grants CTQ-2013-49075-R, SEV-2013-0319, and CTQ-2014-52974-REDC. Financial support from the EU COST actions CM1202 and CM1205 are also acknowledged. C.G.S. is grateful to AGAUR and Generalitat de Catalunya for a "Beatriu de Pinos" postdoctoral grant. A.G. and A.S. would like to thank the Russian Ministry of Education and Science for the support (agreement no. 14.587.21.0002, unique identifier RFMEFI58714X0002). NR 71 TC 4 Z9 4 U1 40 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 24 PY 2016 VL 138 IS 33 BP 10586 EP 10596 DI 10.1021/jacs.6b05680 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA DU4KQ UT WOS:000382181900035 PM 27452370 ER PT J AU Yin, P Wu, B Li, T Bonnesen, PV Hong, KL Seifert, S Porcar, L Do, C Keum, JK AF Yin, Panchao Wu, Bin Li, Tao Bonnesen, Peter V. Hong, Kunlun Seifert, Soenke Porcar, Lionel Do, Changwoo Keum, Jong Kahk TI Reduction-Triggered Self-Assembly of Nanoscale Molybdenum Oxide Molecular Clusters SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID X-RAY; BUILDING-BLOCKS; NEUTRON-SCATTERING; DYNAMIC LIBRARY; ACIDIC-SOLUTION; FLEXIBLE PORES; CAPSULE; EXAFS; TOPOLOGY; XANES AB Understanding the formation mechanism of giant molecular clusters is essential for rational design and synthesis of cluster-based nanomaterials with required morphologies and functionalities. Here, typical synthetic reactions of a 2.9 nm spherical molybdenum oxide cluster, {Mo-132} (formula: [(Mo72Mo60O372)-Mo-VI-O-V(CH3COO)(30)(H2O)(72)](42-)), with systematically varied reaction parameters have been fully explored to determine the morphologies and concentration of products, reduction of metal centers, and chemical environments of the organic ligands. The growth of these clusters shows a typical sigmoid curve, suggesting a general multistep self-assembly mechanism for the formation of giant molecular clusters. The reaction starts with a lag phase period when partial Mo-VI centers of molybdate precursors are reduced to form {Mo-2(V)(acetate)} structures under the coordination effect of the acetate groups. Once the concentration of {Mo-2(V)(acetate)} reaches a critical value, it triggers the co assembly of Mo-V and Mo-VI species into the giant clusters. C1 [Yin, Panchao; Keum, Jong Kahk] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Wu, Bin] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Yin, Panchao; Wu, Bin] Oak Ridge Natl Lab, Shull Wollan Ctr, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Li, Tao; Seifert, Soenke] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Bonnesen, Peter V.; Hong, Kunlun; Keum, Jong Kahk] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Porcar, Lionel] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France. [Do, Changwoo] Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Yin, P (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA.; Yin, P (reprint author), Oak Ridge Natl Lab, Shull Wollan Ctr, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM yinp@ornl.gov RI Yin, Panchao/J-3322-2013; Do, Changwoo/A-9670-2011; Hong, Kunlun/E-9787-2015; OI Yin, Panchao/0000-0003-2902-8376; Do, Changwoo/0000-0001-8358-8417; Hong, Kunlun/0000-0002-2852-5111; Keum, Jong/0000-0002-5529-1373 FU Neutron Sciences Directorate of Oak Ridge National Laboratory; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; DOE Office of Science [DE-AC02-06CH11357] FX P.Y. is grateful for the support of the Clifford G. Shull Fellowship from Neutron Sciences Directorate of Oak Ridge National Laboratory. The research performed in BL-6 (EQ-SANS) at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). The sample preparation and initial SAXS study in the X-ray lab were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Oak Ridge National Laboratory is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. The synchrotron-based SAXS and XANES studies carried out in 12-ID-C used resources of the Advanced Photon Source, a U.S. Department of Energy Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors also thank the Institut Laue Langevin for neutron beamtime. The helpful discussions from Dr. Anibal J. Ramirez-Cuesta and Prof. Ira A. Weinstock are also acknowledged here. NR 40 TC 0 Z9 0 U1 14 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 24 PY 2016 VL 138 IS 33 BP 10623 EP 10629 DI 10.1021/jacs.6b05882 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DU4KQ UT WOS:000382181900039 PM 27459601 ER PT J AU Di Matteo, S Norman, MR AF Di Matteo, S. Norman, M. R. TI Magnetic ground state of Sr2IrO4 and implications for second-harmonic generation SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-SCATTERING; DICHROISM AB The currently accepted magnetic ground state of Sr2IrO4 (the -++- state) preserves inversion symmetry. This is at odds, though, with recent experiments that indicate a magnetoelectric ground state, leading to the speculation that orbital currents or more exotic magnetic multipoles might exist in this material. Here, we analyze various magnetic configurations and demonstrate that two of them, the magnetoelectric -+-+ state and the nonmagnetoelectric ++++ state, can explain these recent second-harmonic generation (SHG) experiments, obviating the need to invoke orbital currents. The SHG-probed magnetic order parameter has the symmetry of a parity-breaking multipole in the -+-+ state and of a parity-preserving multipole in the ++++ state. We speculate that either might have been created by the laser pump used in the experiments. An alternative is that the observed magnetic SHG signal is a surface effect. We suggest experiments that could be performed to test these various possibilities and also address the important issue of the suppression of the RXS intensity at the L-2 edge. C1 [Di Matteo, S.] Univ Rennes 1, Dept Mat Nanosci, Inst Phys Rennes, CNRS,UMR UR1 6251, F-35042 Rennes, France. [Norman, M. R.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Di Matteo, S (reprint author), Univ Rennes 1, Dept Mat Nanosci, Inst Phys Rennes, CNRS,UMR UR1 6251, F-35042 Rennes, France. RI Norman, Michael/C-3644-2013 FU Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, U.S. Dept. of Energy FX The authors would like to thank Dr. Liuyan Zhao and Prof. David Hsieh for providing the data plotted in Fig. 4 and for several discussions about this paper. They also thank Dr. Feng Ye for clarification concerning the neutron scattering results for Rh-doped samples, as well as Mark Dean for discussions about their pump-probe experiments. Finally, we would like to thank one of the referees for suggesting the possibility of surface magnetic SHG. Work by M.R.N. was supported by the Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, U.S. Dept. of Energy. NR 57 TC 1 Z9 1 U1 14 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 24 PY 2016 VL 94 IS 7 AR 075148 DI 10.1103/PhysRevB.94.075148 PG 25 WC Physics, Condensed Matter SC Physics GA DU0JO UT WOS:000381889400002 ER PT J AU Hurley, RC Hall, SA Andrade, JE Wright, J AF Hurley, R. C. Hall, S. A. Andrade, J. E. Wright, J. TI Quantifying Interparticle Forces and Heterogeneity in 3D Granular Materials SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY-DIFFRACTION; SAND AB Interparticle forces in granular materials are intimately linked to mechanical properties and are known to self-organize into heterogeneous structures, or force chains, under external load. Despite progress in understanding the statistics and spatial distribution of interparticle forces in recent decades, a systematic method for measuring forces in opaque, three-dimensional (3D), frictional, stiff granular media has yet to emerge. In this Letter, we present results from an experiment that combines 3D x-ray diffraction, x-ray tomography, and a numerical force inference technique to quantify interparticle forces and their heterogeneity in an assembly of quartz grains undergoing a one-dimensional compression cycle. Forces exhibit an exponential decay above the mean and partition into strong and weak networks. We find a surprising inverse relationship between macroscopic load and the heterogeneity of interparticle forces, despite the clear emergence of two force chains that span the system. C1 [Hurley, R. C.; Andrade, J. E.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Hall, S. A.] Lund Univ, Div Solid Mech, S-22100 Lund, Sweden. [Wright, J.] European Synchrotron Radiat Facil, F-38000 Grenoble, France. [Hurley, R. C.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Hall, SA (reprint author), Lund Univ, Div Solid Mech, S-22100 Lund, Sweden. EM stephen.hall@solid.lth.se RI Wright, Jonathan/A-4321-2010 OI Wright, Jonathan/0000-0002-8217-0884 FU U.S. Air Force Office of Scientific Research Grant [FA9550-12-1-0091]; U.S. Defense Threat Reduction Agency Grant [HDTRA1-12-1-0041]; Marie Curie FP7 integration grant within the 7th European Union Framework Programme; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors acknowledge the ESRF for synchrotron beam time for proposal ma1913. R. C. H. and J. E. A. acknowledge support from the U.S. Air Force Office of Scientific Research Grant No. FA9550-12-1-0091 and the U.S. Defense Threat Reduction Agency Grant No. HDTRA1-12-1-0041. S. A. H. acknowledges support from a Marie Curie FP7 integration grant within the 7th European Union Framework Programme. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Award No. DE-AC52-07NA27344. NR 19 TC 0 Z9 0 U1 6 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 24 PY 2016 VL 117 IS 9 AR 098005 DI 10.1103/PhysRevLett.117.098005 PG 5 WC Physics, Multidisciplinary SC Physics GA DU1YX UT WOS:000382008100016 PM 27610890 ER PT J AU Watanabe, H Po, HC Zaletel, MP Vishwanath, A AF Watanabe, Haruki Po, Hoi Chun Zaletel, Michael P. Vishwanath, Ashvin TI Filling-Enforced Gaplessness in Band Structures of the 230 Space Groups SO PHYSICAL REVIEW LETTERS LA English DT Article ID FERMI-SURFACE; CRYSTALS; TOPOLOGY; LATTICE AB Nonsymmorphic symmetries like screws and glides produce electron band touchings, obstructing the formation of a band insulator and leading, instead, to metals or nodal semimetals even when the number of electrons in the unit cell is an even integer. Here, we calculate the electron fillings compatible with being a band insulator for all 230 space groups, for noninteracting electrons with time-reversal symmetry. Our bounds are tight-that is, we can rigorously eliminate band insulators at any forbidden filling and produce explicit models for all allowed fillings-and stronger than those recently established for interacting systems. These results provide simple criteria that should help guide the search for topological semimetals and, also, have implications for both the nature and stability of the resulting nodal Fermi surfaces. C1 [Watanabe, Haruki] Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan. [Po, Hoi Chun; Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Zaletel, Michael P.] Microsoft Res, Stn Q, Santa Barbara, CA 93106 USA. [Vishwanath, Ashvin] Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA 94720 USA. RP Watanabe, H (reprint author), Univ Tokyo, Dept Appl Phys, Tokyo 1138656, Japan. FU Pappalardo Fellowship; Hellman Graduate Grant; Simons Investigator Grant; NSF [DMR-1411343] FX The work of H. W. was mainly performed at Massachusetts Institute of Technology, and he acknowledges financial support from the Pappalardo Fellowship. H. C. P. is supported by a Hellman Graduate Grant. A. V. acknowledges support from a Simons Investigator Grant. The work done at Berkeley (A. V. and H. C. P.) is supported by NSF Grant No. DMR-1411343. NR 34 TC 6 Z9 6 U1 5 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 24 PY 2016 VL 117 IS 9 AR 096404 DI 10.1103/PhysRevLett.117.096404 PG 5 WC Physics, Multidisciplinary SC Physics GA DU1YX UT WOS:000382008100012 PM 27610868 ER PT J AU Zhao, TZ Behm, K Dong, CF Davoine, X Kalmykov, SY Petrov, V Chvykov, V Cummings, P Hou, B Maksimchuk, A Nees, JA Yanovsky, V Thomas, AGR Krushelnick, K AF Zhao, T. Z. Behm, K. Dong, C. F. Davoine, X. Kalmykov, S. Y. Petrov, V. Chvykov, V. Cummings, P. Hou, B. Maksimchuk, A. Nees, J. A. Yanovsky, V. Thomas, A. G. R. Krushelnick, K. TI High-Flux Femtosecond X-Ray Emission from Controlled Generation of Annular Electron Beams in a Laser Wakefield Accelerator SO PHYSICAL REVIEW LETTERS LA English DT Article ID PLASMA; REGIME AB Annular quasimonoenergetic electron beams with a mean energy in the range 200-400 MeV and charge on the order of several picocoulombs were generated in a laser wakefield accelerator and subsequently accelerated using a plasma afterburner in a two-stage gas cell. Generation of these beams is associated with injection occurring on the density down ramp between the stages. This well-localized injection produces a bunch of electrons performing coherent betatron oscillations in the wakefield, resulting in a significant increase in the x-ray yield. Annular electron distributions are detected in 40% of shots under optimal conditions. Simultaneous control of the pulse duration and frequency chirp enables optimization of both the energy and the energy spread of the annular beam and boosts the radiant energy per unit charge by almost an order of magnitude. These well-defined annular distributions of electrons are a promising source of high-brightness laser plasma-based x rays. C1 [Zhao, T. Z.; Behm, K.; Chvykov, V.; Cummings, P.; Hou, B.; Maksimchuk, A.; Nees, J. A.; Yanovsky, V.; Thomas, A. G. R.; Krushelnick, K.] Univ Michigan, Ctr Ultrafast Opt Sci, Ann Arbor, MI 48109 USA. [Zhao, T. Z.; Behm, K.; Petrov, V.; Cummings, P.; Thomas, A. G. R.; Krushelnick, K.] Univ Michigan, Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Dong, C. F.] Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Davoine, X.] CEA DAM DIF, F-91297 Bruyeres Le Chatel, Arpajon, France. [Kalmykov, S. Y.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. RP Zhao, TZ (reprint author), Univ Michigan, Ctr Ultrafast Opt Sci, Ann Arbor, MI 48109 USA.; Zhao, TZ (reprint author), Univ Michigan, Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. RI Kalmykov, Serge/A-1991-2014; Dong, Chuanfei/E-6485-2010; OI Kalmykov, Serge/0000-0002-0946-857X; Dong, Chuanfei/0000-0002-8990-094X; Thomas, Alexander/0000-0003-3206-8512 FU U.S. Department of Energy/National Nuclear Security Administration Grant [DE-NA0002372]; National Science Foundation Career Grant [1054164]; Air Force Office of Scientific Research Young Investigator Program [FA9550-12-1-0310]; National Science Foundation [PHY-1535678] FX This work is supported by U.S. Department of Energy/National Nuclear Security Administration Grant No. DE-NA0002372, National Science Foundation Career Grant No. 1054164, and Air Force Office of Scientific Research Young Investigator Program Grant No. FA9550-12-1-0310. The work of S. Y. K. has been supported by the National Science Foundation Grant No. PHY-1535678. The authors would like to acknowledge the OSIRIS consortium for use of the OSIRIS2.0 framework. NR 40 TC 0 Z9 0 U1 8 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 24 PY 2016 VL 117 IS 9 AR 094801 DI 10.1103/PhysRevLett.117.094801 PG 5 WC Physics, Multidisciplinary SC Physics GA DU1YX UT WOS:000382008100007 PM 27610860 ER PT J AU Yang, YH Jing, LQ Zheng, B Hao, R Yin, WY Li, EP Soukoulis, CM Chen, HS AF Yang, Yihao Jing, Liqiao Zheng, Bin Hao, Ran Yin, Wenyan Li, Erping Soukoulis, Costas M. Chen, Hongsheng TI Full-Polarization 3D Metasurface Cloak with Preserved Amplitude and Phase SO ADVANCED MATERIALS LA English DT Article ID GROUND-PLANE CLOAK; BROAD-BAND; VISIBLE-LIGHT; INVISIBILITY CLOAK; METAMATERIALS; FREQUENCIES AB A full-polarization arbitrary-shaped 3D metasurface cloak with preserved amplitude and phase in microwave frequencies is experimentally demonstrated. By taking the unique feature of metasurfaces, it is shown that the cloak can completely restore the polarization, amplitude, and phase of light for full polarization as if light was incident on a flat mirror. C1 [Yang, Yihao; Jing, Liqiao; Zheng, Bin; Chen, Hongsheng] Zhejiang Univ, State Key Lab Modern Opt Instrumentat, Electromagnet Acad, Hangzhou 310027, Peoples R China. [Yang, Yihao; Jing, Liqiao; Zheng, Bin; Hao, Ran; Yin, Wenyan; Li, Erping; Chen, Hongsheng] Zhejiang Univ, Coll Informat Sci & Elect Engn, Hangzhou 310027, Peoples R China. [Yang, Yihao; Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Yang, Yihao; Soukoulis, Costas M.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Zheng, B (reprint author), Zhejiang Univ, State Key Lab Modern Opt Instrumentat, Electromagnet Acad, Hangzhou 310027, Peoples R China.; Zheng, B (reprint author), Zhejiang Univ, Coll Informat Sci & Elect Engn, Hangzhou 310027, Peoples R China. EM zhengbin@zju.edu.cn; liep@zju.edu.cn; soukoulis@ameslab.gov; hansomchen@zju.edu.cn RI Soukoulis, Costas/A-5295-2008 FU National Natural Science Foundation of China [61322501, 61275183, 61571395]; National Program for Special Support of Top-Notch Young Professionals; Program for New Century Excellent Talents in University [NCET-12-0489]; Fundamental Research Funds for the Central Universities; Innovation Joint Research Center for Cyber-Physical-Society Systems; U.S. Department of Energy, Office of Basic Energy U. Science, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX This work was sponsored by the National Natural Science Foundation of China under Grant Nos. 61322501, 61275183, and 61571395, the National Program for Special Support of Top-Notch Young Professionals, the Program for New Century Excellent Talents (NCET-12-0489) in University, the Fundamental Research Funds for the Central Universities, and the Innovation Joint Research Center for Cyber-Physical-Society Systems. Work at Ames Laboratory was partially supported by the U.S. Department of Energy, Office of Basic Energy U. Science, Division of Materials Sciences and Engineering (Ames Laboratory is operated for the S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358). NR 25 TC 4 Z9 4 U1 38 U2 46 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 24 PY 2016 VL 28 IS 32 BP 6866 EP + DI 10.1002/adma.201600625 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DU8RU UT WOS:000382482500007 PM 27218885 ER PT J AU Zhu, H Li, Q Ren, Y Fan, LL Chen, J Deng, JX Xing, XR AF Zhu, He Li, Qiang Ren, Yang Fan, Longlong Chen, Jun Deng, Jinxia Xing, Xianran TI Hydration and Thermal Expansion in Anatase Nanoparticles SO ADVANCED MATERIALS LA English DT Article ID SENSITIZED SOLAR-CELLS; TITANIUM-DIOXIDE NANOMATERIALS; TIO2; WATER; EFFICIENCY; SURFACES; FACETS; ZERO; DIFFRACTION; CRYSTALS AB A tunable thermal expansion is reported in nanosized anatase by taking advantage of surface hydration. The coefficient of thermal expansion of 4 nm TiO2 along alpha-axis is negative with a hydrated surface and is positive without a hydrated surface. High-energy synchrotron X-ray pair distribution function analysis combined with ab initio calculations on the specific hydrated surface are carried out to reveal the local structure distortion that is responsible for the unusual negative thermal expansion. C1 [Zhu, He; Li, Qiang; Fan, Longlong; Chen, Jun; Deng, Jinxia; Xing, Xianran] Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Xing, XR (reprint author), Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. EM xing@ustb.edu.cn FU National Natural Science Foundation of China [21590793, 91422301, 21231001]; Fundamental Research Funds for the Central Universities, China [FRF-SD-13-008A]; DOE Office of Science [DE-AC02-06CH11357] FX The authors thank Maohua Quan for the insightful discussion of TEM experiments. This work was supported by the National Natural Science Foundation of China (No. 21590793, 91422301, and 21231001) and the Fundamental Research Funds for the Central Universities, China (No. FRF-SD-13-008A). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 48 TC 0 Z9 0 U1 29 U2 39 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 24 PY 2016 VL 28 IS 32 BP 6894 EP + DI 10.1002/adma.201600973 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DU8RU UT WOS:000382482500011 PM 27270568 ER PT J AU Zhang, Q Wan, XJ Liu, F Kan, B Li, MM Feng, HR Zhang, HT Russell, TP Chen, YS AF Zhang, Qian Wan, Xiangjian Liu, Feng Kan, Bin Li, Miaomiao Feng, Huanran Zhang, Hongtao Russell, Thomas P. Chen, Yongsheng TI Evaluation of Small Molecules as Front Cell Donor Materials for High-Efficiency Tandem Solar Cells SO ADVANCED MATERIALS LA English DT Article ID POWER CONVERSION EFFICIENCY; ORGANIC TANDEM; 10-PERCENT EFFICIENCY; MORPHOLOGY CONTROL; POLYMER; PERFORMANCE; SINGLE; LAYER; ACCEPTOR; DITHIENOGERMOLE AB Three small molecules as front cell donors for tandem cells are thoroughly evaluated and a high power conversion effi ciency of 11.47% is achieved, which demonstrates that the oligomer-like small molecules offer a good choice for high-performance tandem solar cells. C1 [Zhang, Qian; Wan, Xiangjian; Kan, Bin; Li, Miaomiao; Feng, Huanran; Zhang, Hongtao; Chen, Yongsheng] Nankai Univ, State Key Lab, Collaborat Innovat Ctr Chem Sci & Engn, Sch Mat Sci & Engn, Tianjin 300071, Peoples R China. [Zhang, Qian; Wan, Xiangjian; Kan, Bin; Li, Miaomiao; Feng, Huanran; Zhang, Hongtao; Chen, Yongsheng] Nankai Univ, Inst Elementoorgan Chem, Collaborat Innovat Ctr Chem Sci & Engn, Sch Mat Sci & Engn, Tianjin 300071, Peoples R China. [Liu, Feng] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. RP Wan, XJ (reprint author), Nankai Univ, State Key Lab, Collaborat Innovat Ctr Chem Sci & Engn, Sch Mat Sci & Engn, Tianjin 300071, Peoples R China.; Wan, XJ (reprint author), Nankai Univ, Inst Elementoorgan Chem, Collaborat Innovat Ctr Chem Sci & Engn, Sch Mat Sci & Engn, Tianjin 300071, Peoples R China. EM xjwan@nankai.edu.cn; iamfengliu@gmail.com; russell@mail.pse.umass.edu; yschen99@nankai.edu.cn RI Zhang, Hongtao/O-8232-2016; Liu, Feng/J-4361-2014 OI Liu, Feng/0000-0002-5572-8512 FU MoST [2014CB643502]; NSFC [51373078, 51422304, 91433101]; PCSIRT [IRT1257]; Tianjin city [13RCGFGX01121] FX The authors gratefully acknowledge the financial support from MoST (2014CB643502), NSFC (51373078, 51422304, 91433101), PCSIRT (IRT1257) and Tianjin city (13RCGFGX01121). NR 48 TC 6 Z9 6 U1 40 U2 62 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 24 PY 2016 VL 28 IS 32 BP 7008 EP + DI 10.1002/adma.201601435 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DU8RU UT WOS:000382482500027 PM 27214707 ER PT J AU Miyauchi, S Navarro, D Grigoriev, IV Lipzen, A Riley, R Chevret, D Grisel, S Berrin, JG Henrissat, B Rosso, MN AF Miyauchi, Shingo Navarro, David Grigoriev, Igor V. Lipzen, Anna Riley, Robert Chevret, Didier Grisel, Sacha Berrin, Jean-Guy Henrissat, Bernard Rosso, Marie-Noelle TI Visual Comparative Omics of Fungi for Plant Biomass Deconstruction SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE self-organizing maps; data visualization; multi-omics integration; LPMOs; lignocellulosic biomass; biorefinery; CAZymes ID WOOD-DECAY FUNGI; LIGNIN DEGRADATION; GENOMES; REVEAL AB Wood-decay fungi contain the cellular mechanisms to decompose such plant cell wall components as cellulose, hemicellulose, and lignin. A multi-omics approach to the comparative analysis of wood-decay fungi gives not only new insights into their strategies for decomposing recalcitrant plant biomass, but also an understanding of how to exploit these mechanisms for biotechnological applications. We have developed an analytical workflow, Applied Biomass Conversion Design for Efficient Fungal Green Technology (ABCDEFGT), to simplify the analysis and interpretation of transcriptomic and secretomic data. ABCDEFGT utilizes self-organizing maps for grouping genes with similar transcription patterns, and an overlay with secreted proteins. The key feature of ABCDEFGT is simple graphic outputs of genome-wide transcriptomic and secretomic topographies, which enables visual inspection without a priori of the omics data and facilitates discoveries of co-regulated genes and proteins. Genome-wide omics landscapes were built with the newly sequenced fungal species Pycnoporus coccineus, Pycnoporus sanguineus, and Pycnoporus cinnabarinus grown on various carbon sources. Integration of the post-genomic data revealed a global overlap, confirming the pertinence of the genome-wide approach. ABCDEFGT was evaluated by comparison with the latest clustering method for ease of output interpretation, and ABCDEFGT gave a better biological representation of fungal behaviors. The genome-wide multi-omics strategy allowed us to determine the potential synergy of particular enzymes decomposing cellulose, hemicellulose, and lignin such as Lytic Polysaccharide Monooxygenases, modular enzymes associated with a cellulose binding modulel, and Class II Peroxidase isoforms co-regulated with oxido-reductases. Overall, ABCDEFGT was capable of visualizing genome-wide transcriptional and secretomic profiles for intuitive interpretations and is suitable for exploration of newly-sequenced organisms. C1 [Miyauchi, Shingo; Navarro, David; Grisel, Sacha; Berrin, Jean-Guy; Rosso, Marie-Noelle] Aix Marseille Univ, INRA, UMR1163, Biodiversite & Biotechnol Fong, Marseille, France. [Navarro, David] CIRM CF, Biodiversite & Biotechnol Fong UMR1163, Marseille, France. [Grigoriev, Igor V.; Lipzen, Anna; Riley, Robert] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Chevret, Didier] INRA, Plateforme Analyse Prote Paris Sud Ouest, UMR1319 Micalis, Jouy En Josas, France. [Henrissat, Bernard] Aix Marseille Univ, CNRS, Architecture & Fonct Macromol Biol, Marseille, France. [Henrissat, Bernard] INRA, USC AFMB 1408, Marseille, France. [Henrissat, Bernard] King Abdulaziz Univ, Dept Biol Sci, Jeddah, Saudi Arabia. RP Miyauchi, S; Rosso, MN (reprint author), Aix Marseille Univ, INRA, UMR1163, Biodiversite & Biotechnol Fong, Marseille, France. EM shingo.miyauchi@univ-amu.fr; marie-noelle.rosso@univ-amu.fr RI Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI berrin, jean-guy/0000-0001-7570-3745 FU Agence Nationale de la Recherche [ANR-14-CE06-0020]; Office of Science of the U.S. Department of Energy [DEAC02-05CH11231] FX The research was funded by the Agence Nationale de la Recherche (ANR-14-CE06-0020). The work by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported by the Office of Science of the U.S. Department of Energy under Contract No. DEAC02-05CH11231. NR 33 TC 0 Z9 0 U1 15 U2 20 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD AUG 24 PY 2016 VL 7 AR 1335 DI 10.3389/fmicb.2016.01335 PG 10 WC Microbiology SC Microbiology GA DT9BW UT WOS:000381791300001 PM 27605927 ER PT J AU Liang, JF Allmond, JM Gross, CJ Mueller, PE Shapira, D Varner, RL Dasgupta, M Hinde, DJ Simenel, C Williams, E Vo-Phuoc, K Brown, ML Carter, IP Evers, M Luong, DH Ebadi, T Wakhle, A AF Liang, J. F. Allmond, J. M. Gross, C. J. Mueller, P. E. Shapira, D. Varner, R. L. Dasgupta, M. Hinde, D. J. Simenel, C. Williams, E. Vo-Phuoc, K. Brown, M. L. Carter, I. P. Evers, M. Luong, D. H. Ebadi, T. Wakhle, A. TI Examining the role of transfer coupling in sub-barrier fusion of Ti-46,Ti-50+Sn-124 SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION FUSION; COULOMB BARRIER; CA-40+SN-124; FISSION; NUCLEI; ENERGY; STATE AB Background: The presence of neutron transfer channels with positive Q values can enhance sub-barrier fusion cross sections. Recent measurements of the fusion excitation functions for Ni-58+Sn-132,Sn-124 found that the fusion enhancement due to the influence of neutron transfer is smaller than that in Ca-40+Sn-132,Sn-124 although the Q values for multineutron transfer are comparable. Purpose: To investigate the differences observed between the fusion of Sn + Ni and Sn + Ca. Methods: Fusion excitation functions for Ti-46,Ti-50+Sn-124 have been measured at energies near the Coulomb barrier. Results: A comparison of the barrier distributions for Ti-46+Sn-124 and Ca-40+Sn-124 shows that the Ca-40+Sn-124 system has a barrier strength resulting from the coupling to the very collective octupole state in Ca-40 at an energy significantly lower than the uncoupled barrier. Conclusions: The large sub-barrier fusion enhancement in Ca-40 induced reactions is attributed to both couplings to neutron transfer and inelastic excitation, with the octupole vibration of Ca-40 playing a major role. C1 [Liang, J. F.; Allmond, J. M.; Gross, C. J.; Mueller, P. E.; Shapira, D.; Varner, R. L.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Dasgupta, M.; Hinde, D. J.; Simenel, C.; Williams, E.; Vo-Phuoc, K.; Brown, M. L.; Carter, I. P.; Evers, M.; Luong, D. H.; Ebadi, T.; Wakhle, A.] Australian Natl Univ, Dept Nucl Phys, Res Sch Phys Sci & Engn, Canberra, ACT 2601, Australia. [Liang, J. F.] FLIR Syst Inc, Wilsonville, OR USA. [Evers, M.] Australian Natl Univ, John Curtin Sch Med Res, Canberra, ACT, Australia. [Ebadi, T.] Seeing Machines, Canberra, ACT, Australia. [Wakhle, A.] MSU, Natl Superconducting Cyclotron Lab, Tirunelveli, Tamil Nadu, India. RP Liang, JF (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RI Simenel, Cedric/H-3705-2014; Hinde, David/D-5051-2013 OI Simenel, Cedric/0000-0002-2356-7769; Hinde, David/0000-0002-4595-0742 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics; Australian Research Council [DP130101569, FT120100760, DP140101337, FL110100098, DE140100784]; U.S. Department of Energy [DE-AC05-00OR22725]; United States Government FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics and this research used resources of the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory, which was a DOE Office of Science User Facility. Research at ANU was supported by the Australian Research Council Grants DP130101569, FT120100760, DP140101337, FL110100098, DE140100784 and by National Collaborative Research Infrastructure Strategy (NCRIS) for the operation of the Heavy Ion Accelerator Facility.; This manuscript was authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up irrevocable, worldwide license to publish or reproduce the published form of the manuscript, or allow others to do so, for United States Government purposes. NR 39 TC 1 Z9 1 U1 5 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 24 PY 2016 VL 94 IS 2 AR 024616 DI 10.1103/PhysRevC.94.024616 PG 9 WC Physics, Nuclear SC Physics GA DU0KP UT WOS:000381892700005 ER PT J AU Kim, JH Kong, K Lee, SJ Mohlabeng, G AF Kim, Jeong Han Kong, Kyoungchul Lee, Seung J. Mohlabeng, Gopolang TI Probing TeV scale top-philic resonances with boosted top-tagging at the high luminosity LHC SO PHYSICAL REVIEW D LA English DT Article ID COMPOSITE HIGGS; VACUUM MISALIGNMENT; BREAKING; PHYSICS; BOSONS; SU(2); PAIRS; JETS AB We investigate the discovery potential of singly produced top-philic resonances at the high luminosity (HL) LHC in the four-top final state. Our analysis spans over the fully hadronic, semileptonic, and samesign dilepton channels where we present concrete search strategies adequate to a boosted kinematic regime and high jet-multiplicity environments. We utilize the template overlap method with newly developed template observables for tagging boosted top quarks, a large-radius jet variable M-J, and customized b-tagging tactics for background discrimination. Our results show that the same-sign dilepton channel gives the best sensitivity among the considered channels, with an improvement of significance up to 10%-20% when combined with boosted top-tagging. Both the fully hadronic and semileptonic channels yield comparable discovery potential and contribute to further enhancements in the sensitivity by combining all channels. Finally, we show the sensitivity of a top-philic resonance at the LHC and HL-LHC by showing the 2 sigma exclusion limit and 5 sigma discovery reach, including a combination of all three channels. C1 [Kim, Jeong Han] Korea Adv Inst Sci & Technol, Dept Phys, 335 Gwahak Ro, Daejeon 305701, South Korea. [Kim, Jeong Han] Inst for Basic Sci Korea, Ctr Theoret Phys Universe, Daejeon 34051, South Korea. [Kong, Kyoungchul; Mohlabeng, Gopolang] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Lee, Seung J.] Korea Univ, Dept Phys, Seoul 136713, South Korea. [Lee, Seung J.] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea. [Mohlabeng, Gopolang] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. RP Kim, JH (reprint author), Korea Adv Inst Sci & Technol, Dept Phys, 335 Gwahak Ro, Daejeon 305701, South Korea.; Kim, JH (reprint author), Inst for Basic Sci Korea, Ctr Theoret Phys Universe, Daejeon 34051, South Korea.; Kong, K; Mohlabeng, G (reprint author), Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA.; Lee, SJ (reprint author), Korea Univ, Dept Phys, Seoul 136713, South Korea.; Lee, SJ (reprint author), Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea.; Mohlabeng, G (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. EM jeonghan.kim@kaist.ac.kr; kckong@ku.edu; sjjlee@korea.edu; gopolang.mohlabeng@ku.edu OI Lee, Seung J./0000-0002-7756-0407 FU IBS Center for Theoretical Physics of the Universe [IBS-R018-D1]; IBS Center for Axion and Precision Physics Research [IBS-R017-D1-2016-a00]; U.S. DOE [DE-FG02-12ER41809]; Fermilab Graduate Student Research Program in Theoretical Physics; National Research Foundation of South Africa [88614]; National Research Foundation of Korea - Korea government [NRF-2015R1A2A1A15052408] FX We would like to thank HTCaaS group of KISTI for providing useful cluster resources during the full course of this project. We are grateful to Chul Kim, Jae-Hyeok Yoo, and Hwidong Yoo for discussion and comments, and we would like to thank Michael Spannowsky for encouragement toward this study. J. H. K. is supported by the IBS Center for Theoretical Physics of the Universe (IBS-R018-D1) and Center for Axion and Precision Physics Research (IBS-R017-D1-2016-a00). K. K. is supported by the U.S. DOE under Grant No. DE-FG02-12ER41809. G. M. is supported by the Fermilab Graduate Student Research Program in Theoretical Physics and in part by the National Research Foundation of South Africa, Grant No. 88614. S. L. and J. H. K. (in part) have been supported by the National Research Foundation of Korea grant funded by the Korea government (NRF-2015R1A2A1A15052408). We also acknowledge the Korea Future Collider Study Group (KFCSG) for motivating us to proceed with this work. NR 93 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 24 PY 2016 VL 94 IS 3 AR 035023 DI 10.1103/PhysRevD.94.035023 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KU UT WOS:000381893500005 ER PT J AU Levallois, J Tran, MK Pouliot, D Presura, CN Greene, LH Eckstein, JN Uccelli, J Giannini, E Gu, GD Leggett, AJ van der Marel, D AF Levallois, J. Tran, M. K. Pouliot, D. Presura, C. N. Greene, L. H. Eckstein, J. N. Uccelli, J. Giannini, E. Gu, G. D. Leggett, A. J. van der Marel, D. TI Temperature-Dependent Ellipsometry Measurements of Partial Coulomb Energy in Superconducting Cuprates SO PHYSICAL REVIEW X LA English DT Article ID ELECTRONIC SPECIFIC-HEAT; T-C; CONDENSATION ENERGY; COLLECTIVE MODES; PSEUDOGAP STATE; PAIR FORMATION; HUBBARD-MODEL; SUM-RULE; PHASE; DENSITY AB We performed an experimental study of the temperature and doping dependence of the energy-loss function of the bilayer and trilayer bismuth cuprates family. The primary aim is to obtain information on the energy stored in the Coulomb interaction between the conduction electrons, on the temperature dependence thereof, and on the change of Coulomb interaction when Cooper pairs are formed. We performed temperature-dependent ellipsometry measurements on several Bi2Sr2CaCu2O8-x single crystals: under-doped with T-c = 60, 70, and 83 K; optimally doped with T-c = 91 K; overdoped with T-c = 84, 81, 70, and 58 K; as well as optimally doped Bi2Sr2Ca2Cu3O10+x with T-c = 110 K. Our first observation is that, as the temperature drops through T-c, the loss function in the range up to 2 eV displays a change of temperature dependence as compared to the temperature dependence in the normal state. This effect at-or close to-T-c depends strongly on doping, with a sign change for weak overdoping. The size of the observed change in Coulomb energy, using an extrapolation with reasonable assumptions about its q dependence, is about the same size as the condensation energy that has been measured in these compounds. Our results therefore lend support to the notion that the Coulomb energy is an important factor for stabilizing the superconducting phase. Because of the restriction to small momentum, our observations do not exclude a possible significant contribution to the condensation energy of the Coulomb energy associated with the region of q around (pi, pi). C1 [Levallois, J.; Tran, M. K.; Uccelli, J.; Giannini, E.; van der Marel, D.] Univ Geneva, Dept Quantum Matter Phys, Quai Ernest Ansermet 24, CH-1211 Geneva 4, Switzerland. [Pouliot, D.; Greene, L. H.; Eckstein, J. N.; Leggett, A. J.] Univ Illinois, Dept Phys, 1110 West Green St, Urbana, IL 61801 USA. [Presura, C. N.] Philips Res, Prof Holstlaan 4, NL-5656 AE Eindhoven, Netherlands. [Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Leggett, A. J.] Univ Waterloo, Inst Quantum Comp, Waterloo, ON N2L 3G1, Canada. RP Leggett, AJ (reprint author), Univ Illinois, Dept Phys, 1110 West Green St, Urbana, IL 61801 USA.; Leggett, AJ (reprint author), Univ Waterloo, Inst Quantum Comp, Waterloo, ON N2L 3G1, Canada. EM aleggett@illinois.edu; dirk.vandermarel@unige.ch RI van der Marel, Dirk/G-4618-2012 OI van der Marel, Dirk/0000-0001-5266-9847 FU Swiss National Science Foundation [200021-162628]; DOE [DE-SC00112704]; Center for Emergent Superconductivity, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-07CH11358] FX The authors thank Mehdi Brandt, Jeremie Teyssier, and Spiros Zanos for technical support. This project was supported by the Swiss National Science Foundation (Project No. 200021-162628). The work at Brookhaven is funded through DOE Contract No. DE-SC00112704. The work at the University of Illinois at Urbana-Champaign was supported as part of the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-AC02-07CH11358 NR 77 TC 1 Z9 1 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD AUG 24 PY 2016 VL 6 IS 3 AR 031027 DI 10.1103/PhysRevX.6.031027 PG 24 WC Physics, Multidisciplinary SC Physics GA DU0LS UT WOS:000381897200001 ER PT J AU Barnard, E Liu, J Yankova, E Cavalcanti, SM Magalhaes, M Li, HY Patrick, S McDowell, A AF Barnard, Emma Liu, Jared Yankova, Eliza Cavalcanti, Silvana M. Magalhaes, Marcelo Li, Huiying Patrick, Sheila McDowell, Andrew TI Strains of the Propionibacterium acnes type III lineage are associated with the skin condition progressive macular hypomelanosis SO SCIENTIFIC REPORTS LA English DT Article ID CONTAMINATION; PATHOGENESIS; POPULATIONS; SECRETION; SURGERY; TIME; PCR AB Progressive macular hypomelanosis (PMH) is a common skin disorder that causes hypopigmentation in a variety of skin types. Although the underlying aetiology of this condition is unclear, there is circumstantial evidence that links the skin bacterium Propionibacterium acnes to the condition. We now describe the first detailed population genetic analysis of P. acnes isolates recovered from paired lesional and non-lesional skin of PMH patients. Our results demonstrate a strong statistical association between strains from the type III phylogenetic lineage and PMH lesions (P = 0.0019), but not those representing other phylogroups, including those associated with acne (type IA(1)). We also demonstrate, based on in silico 16S rDNA analysis, that PMH isolates previously recovered from patients in Europe are also consistent with the type III lineage. Using comparative genome analysis, we identified multiple genomic regions that are specific for, or absent from, type III strains compared to other phylogroups. In the former case, these include open reading frames with putative functions in metabolism, transport and transcriptional regulation, as well as predicted proteins of unknown function. Further study of these genomic elements, along with transcriptional and functional analyses, may help to explain why type III strains are associated with PMH. C1 [Barnard, Emma; Patrick, Sheila; McDowell, Andrew] Queens Univ, Sch Med Dent & Biomed Sci, Ctr Infect & Immun, Belfast, Antrim, North Ireland. [Barnard, Emma; Liu, Jared; Li, Huiying] Univ Calif Los Angeles, David Geffen Sch Med, Dept Mol & Med Pharmacol, Crump Inst Mol Imaging, Los Angeles, CA 90095 USA. [Yankova, Eliza; McDowell, Andrew] Univ Ulster, Altnagelvin Area Hosp, Biomed Sci Res Inst, Northern Ireland Ctr Stratified Med, C TRIC Bldg, Coleraine BT52 1SA, Londonderry, North Ireland. [Cavalcanti, Silvana M.] Univ Pernambuco, Dept Dermatol, Recife, PE, Brazil. [Magalhaes, Marcelo] Univ Fed Pernambuco, Dept Microbiol, Recife, PE, Brazil. [Li, Huiying] UCLA DOE Inst Genom & Prote, Los Angeles, CA USA. RP McDowell, A (reprint author), Queens Univ, Sch Med Dent & Biomed Sci, Ctr Infect & Immun, Belfast, Antrim, North Ireland.; McDowell, A (reprint author), Univ Ulster, Altnagelvin Area Hosp, Biomed Sci Res Inst, Northern Ireland Ctr Stratified Med, C TRIC Bldg, Coleraine BT52 1SA, Londonderry, North Ireland. EM a.mcdowell@ulster.ac.uk OI McDowell, Andrew/0000-0002-9649-0504 FU R & D Division of Health and Social Care Northern Ireland [HSCNI RRG 9.41]; Department of Education and Learning (DEL); National Institutes of Health (NIH) grant from National Institute of General Medical Sciences (NIGMS) [R01GM099530]; European Union Regional Development Fund (ERDF) EU Sustainable Competitiveness Programme FX This work was supported by a R & D Division of Health and Social Care Northern Ireland grant (HSCNI RRG 9.41) awarded to SP, a Department of Education and Learning (DEL) Studentship award and an National Institutes of Health (NIH) grant (R01GM099530) from National Institute of General Medical Sciences (NIGMS) awarded to HL. A small portion of this work was also part-financed by a grant awarded to Prof A. J. Bjourson (University of Ulster) under the European Union Regional Development Fund (ERDF) EU Sustainable Competitiveness Programme for N. Ireland & the Northern Ireland Public Health Agency (HSC R & D). NR 33 TC 3 Z9 3 U1 1 U2 2 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 24 PY 2016 VL 6 AR 31968 DI 10.1038/srep31968 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9OM UT WOS:000381831400001 PM 27555369 ER PT J AU Kumar, P Sharma, V Reboredo, FA Yang, LM Pushpa, R AF Kumar, Pankaj Sharma, Vinit Reboredo, Fernando A. Yang, Li-Ming Pushpa, Raghani TI Tunable magnetism in metal adsorbed fluorinated nanoporous graphene SO SCIENTIFIC REPORTS LA English DT Article ID NITROGEN-DOPED GRAPHENE; AUGMENTED-WAVE METHOD; MONOLAYER GRAPHENE; ROOM-TEMPERATURE; ELECTRIC-FIELDS; ANISOTROPY; ATOM; NANOMAGNETICS; SPINTRONICS; TRANSPORT AB Developing nanostructures with tunable magnetic states is crucial for designing novel data storage and quantum information devices. Using density functional theory, we investigate the thermodynamic stability and magnetic properties of tungsten adsorbed tri-vacancy fluorinated (TVF) graphene. We demonstrate a strong structure-property relationship and its response to external stimuli via defect engineering in graphene-based materials. Complex interplay between defect states and the chemisorbed atom results in a large magnetic moment of 7 mu(B) along with high in-plane magneto-crystalline anisotropy energy (MAE) of 17 meV. Under the influence of electric field, spin crossover effect accompanied by a change in the MAE is observed. The ascribed change in spin-configuration is caused by the modification of exchange coupling between defect states and a change in the occupation of d-orbitals of the metal complex. Our predictions open a promising way towards controlling the magnetic properties in graphene based spintronic and non-volatile memory devices. C1 [Kumar, Pankaj; Pushpa, Raghani] Boise State Univ, Dept Phys, Boise, ID 83725 USA. [Sharma, Vinit; Reboredo, Fernando A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Yang, Li-Ming] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China. RP Pushpa, R (reprint author), Boise State Univ, Dept Phys, Boise, ID 83725 USA. EM pushparaghani@boisestate.edu RI Yang, Li-Ming/G-7467-2011 FU Research Corporation's Cottrell College Science award [20234]; NSF CAREER award [DMR-1255584]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This research is supported by the Research Corporation's Cottrell College Science award (Grant No. 20234) and NSF CAREER award (DMR-1255584). We are thankful to the HPC center of Idaho National Laboratory for computational support where, most of the calculations are performed. Work by VS and FAR was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. VS acknowledges the XSEDE computational resource allocation number TG-DMR160051. NR 69 TC 0 Z9 0 U1 27 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 24 PY 2016 VL 6 AR 31841 DI 10.1038/srep31841 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9OJ UT WOS:000381831100001 PM 27554975 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M De Barbaro, P Demortier, L Deninno, M Devoto, F d'Errico, M Di Canto, A Di Ruzza, B Dittmann, JR D'Onofrio, M Donati, S Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Eusebi, R Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SB Kim, SH Kim, YK Kim, YJ Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leone, S Lewis, JD Limosani, A Lipeles, E Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Prokoshin, F Pranko, A Ptohos, F Punzi, G Ranjan, N Fernandez, IR Renton, P Rescigno, M Riddick, T Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Safonov, A Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sinervo, P Sliwa, K Smith, JR Snider, FD Sorin, V Song, H Stancari, M Denis, RS Stelzer, B Stelzer-Chilton, O Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Warburton, A Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. Datta, M. De Barbaro, P. Demortier, L. Deninno, M. Devoto, F. d'Errico, M. Di Canto, A. Di Ruzza, B. Dittmann, J. R. D'Onofrio, M. Donati, S. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Elagin, A. Erbacher, R. Errede, S. Esham, B. Eusebi, R. Farrington, S. Fernandez Ramos, J. P. Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Giurgiu, G. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Gonzalez Lopez, O. Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grinstein, S. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. 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CA CDF Collaboration TI Measurement of the WW and WZ production cross section using final states with a charged lepton and heavy-flavor jets in the full CDF Run II data set SO PHYSICAL REVIEW D LA English DT Article ID ELECTROMAGNETIC CALORIMETER; ATLAS DETECTOR; PP COLLISIONS; ROOT-S=7 TEV; UPGRADE; COUPLINGS; EVENTS AB We present a measurement of the total WW and WZ production cross sections in p (p) over bar collision at root s = 1.96 TeV, in a final state consistent with leptonic W boson decay and jets originating from heavy-flavor quarks from either a W or a Z boson decay. This analysis uses the full data set collected with the CDF II detector during Run II of the Tevatron collider, corresponding to an integrated luminosity of 9.4 fb(-1). An analysis of the dijet mass spectrum provides 3.7 sigma evidence of the summed production processes of either WW or WZ bosons with a measured total cross section of sigma(WW+WZ) = 13.7 +/- 3.9 pb. Independent measurements of the WW and WZ production cross sections are allowed by the different heavy- flavor decay patterns of the W and Z bosons and by the analysis of secondary- decay vertices reconstructed within heavy- flavor jets. The productions of WW and of WZ dibosons are independently seen with significances of 2.9s and 2.1s, respectively, with total cross sections of sigma(WW) = 9.4 +/- 4.2 pb and sigma(WZ) = 3.7(-2.2)(+2.5) pb. The measurements are consistent with standard- model predictions. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece. [Camarda, S.; Cavalli-Sforza, M.; Grinstein, S.; Martinez, M.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, ICREA, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Bland, K. 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RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland.; Aaltonen, T (reprint author), Helsinki Inst Phys, FIN-00014 Helsinki, Finland. RI Marino, Pietro/N-7030-2015; Ruiz, Alberto/E-4473-2011; Warburton, Andreas/N-8028-2013; Canelli, Florencia/O-9693-2016; Grinstein, Sebastian/N-3988-2014; Prokoshin, Fedor/E-2795-2012; OI song, hao/0000-0002-3134-782X; Marino, Pietro/0000-0003-0554-3066; Ruiz, Alberto/0000-0002-3639-0368; Warburton, Andreas/0000-0002-2298-7315; Canelli, Florencia/0000-0001-6361-2117; Grinstein, Sebastian/0000-0002-6460-8694; Prokoshin, Fedor/0000-0001-6389-5399; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program, the National Research Foundation of Korea; Science and Technology Facilities Council; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); Programa Consolider-Ingenio, Spain; Royal Society, UK FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, UK; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; and the Australian Research Council (ARC). NR 60 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 23 PY 2016 VL 94 IS 3 AR 032008 DI 10.1103/PhysRevD.94.032008 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KT UT WOS:000381893400001 ER PT J AU Yuan, P Cai, CL Tang, JY Qin, YQ Jin, MY Fu, YB Li, ZH Ma, XH AF Yuan, Ping Cai, Chuanlin Tang, Jiayong Qin, Yuqi Jin, Mengyuan Fu, Yanbao Li, Zhenhua Ma, Xiaohua TI Anion Acceptors Dioxaborinane Contained in Solid State Polymer Electrolyte: Preparation, Characterization, and DFT Calculations SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; GRAPHENE; CONDUCTIVITY; OXIDE); SUPERCAPACITORS; PERFORMANCE; CAPACITORS; CARBON; POLYELECTROLYTE AB A novel dioxaborinane-contained solid state polymer electrolyte poly((-2phenyl-1, 3, 2-dioxaborolane-4-yl) methyl methacrylate) (P(GMMA-PBA)) for symmetrical capacitors (SCs) is prepared through solution casting technique. Due to the effect of electron withdrawing of dioxaborinane groups and irregular distributed porous microstructures, the solid polymer electrolyte (SPE) exhibits an optimal ionic conductivity of 0.5 mS cm(-1) at ambient conditions. The electronic properties of dioxaborinane groups and their interaction with anions of electrolyte salts are further studied with density functional theory calculations. SCs fabricated with this polymer film as electrolyte and reduced graphene oxide as electrodes provide a broad potential window of 2.5 V. The energy density of this capacitor ups to 22.49 Wh kg(-1) with a power density of 6.34 kW kg(-1) at 5 A g(-1). After 3000 charge-discharge cycles, the capacitance of the symmetrical SPE capacitor maintains 90% of its initial values. C1 [Yuan, Ping; Cai, Chuanlin; Tang, Jiayong; Qin, Yuqi; Jin, Mengyuan; Ma, Xiaohua] Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China. [Fu, Yanbao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Li, Zhenhua] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China. RP Ma, XH (reprint author), Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China. EM xhma@fudan.edu.cn FU State Key 973 Program of PRC [2011CB605704]; National Natural Science Foundation of China [U1201241, 51372041, 51202034, 51201035] FX P.Y. and C.C. contributed equally to this work. This work was financially supported by the State Key 973 Program of PRC (2011CB605704), and the National Natural Science Foundation of China (U1201241, 51372041, 51202034, and 51201035). The authors also thank Fudan University High-End Computing Center for computational resources. NR 53 TC 2 Z9 2 U1 24 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD AUG 23 PY 2016 VL 26 IS 32 BP 5930 EP 5939 DI 10.1002/adfm.201600888 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DW4JG UT WOS:000383608400016 ER PT J AU Wang, P Wang, YS Hang, B Zou, XP Mao, JH AF Wang, Pin Wang, Yunshan Hang, Bo Zou, Xiaoping Mao, Jian-Hua TI A novel gene expression-based prognostic scoring system to predict survival in gastric cancer SO ONCOTARGET LA English DT Article DE gene biomarkers; prognostic score; gastric cancer ID GROWTH-FACTOR; POOR-PROGNOSIS; PROTEIN; IDENTIFICATION; RECEPTOR; OVEREXPRESSION; INVASION; TUMORS; METASTASIS; CARCINOMA AB Analysis of gene expression patterns in gastric cancer (GC) can help to identify a comprehensive panel of gene biomarkers for predicting clinical outcomes and to discover potential new therapeutic targets. Here, a multi-step bioinformatics analytic approach was developed to establish a novel prognostic scoring system for GC. We first identified 276 genes that were robustly differentially expressed between normal and GC tissues, of which, 249 were found to be significantly associated with overall survival (OS) by univariate Cox regression analysis. The biological functions of 249 genes are related to cell cycle, RNA/ncRNA process, acetylation and extracellular matrix organization. A network was generated for view of the gene expression architecture of 249 genes in 265 GCs. Finally, we applied a canonical discriminant analysis approach to identify a 53-gene signature and a prognostic scoring system was established based on a canonical discriminant function of 53 genes. The prognostic scores strongly predicted patients with GC to have either a poor or good OS. Our study raises the prospect that the practicality of GC patient prognosis can be assessed by this prognostic scoring system. C1 [Wang, Pin; Zou, Xiaoping] Nanjing Med Univ, Dept Gastroenterol, Drum Tower Clin Med Sch, Nanjing 210008, Jiangsu, Peoples R China. [Wang, Yunshan; Hang, Bo; Mao, Jian-Hua] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. [Wang, Yunshan] Shandong Univ, Sch Ocean, Int Biotechnol R&D Ctr, Weihai 264209, Shandong, Peoples R China. RP Zou, XP (reprint author), Nanjing Med Univ, Dept Gastroenterol, Drum Tower Clin Med Sch, Nanjing 210008, Jiangsu, Peoples R China.; Mao, JH (reprint author), Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. EM zouxiaoping795@hotmail.com; JHMao@lbl.gov FU National Science Foundation of China [81472756, 81402193]; NIH, National Cancer Institute [R01 CA116481]; Low Dose Scientific Focus Area, Office of Biological and Environmental Research, U.S. Department of Energy [DE AC02-05CH11231]; China Postdoctoral International Exchange Program; Postdoctoral innovation project of Shandong Province; Postdoctoral Science Foundation of China FX This work was supported by National Science Foundation of China Grant no. 81472756. J.H.M. was supported by the NIH, National Cancer Institute grant R01 CA116481, and Low Dose Scientific Focus Area, Office of Biological and Environmental Research, U.S. Department of Energy under Contract No. DE AC02-05CH11231. Y.S.W. was supported by the China Postdoctoral International Exchange Program 2015, National Science Foundation of China Grant no. 81402193, Postdoctoral innovation project of Shandong Province, and Postdoctoral Science Foundation of China. NR 46 TC 0 Z9 0 U1 1 U2 1 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1949-2553 J9 ONCOTARGET JI Oncotarget PD AUG 23 PY 2016 VL 7 IS 34 BP 55343 EP 55351 DI 10.18632/oncotarget.10533 PG 9 WC Oncology; Cell Biology SC Oncology; Cell Biology GA DY9DY UT WOS:000385435000098 PM 27419373 ER PT J AU Ortega, I Coburn, S Berg, LK Lantz, K Michalsky, J Ferrare, RA Hair, J Hostetler, CA Volkamer, R AF Ortega, Ivan Coburn, Sean Berg, Larry K. Lantz, Kathy Michalsky, Joseph Ferrare, Richard A. Hair, JohnathanW. Hostetler, Chris A. Volkamer, Rainer TI The CU 2-D-MAX-DOAS instrument - Part 2: Raman scattering probability measurements and retrieval of aerosol optical properties SO ATMOSPHERIC MEASUREMENT TECHNIQUES LA English DT Article ID SKY BRIGHTNESS MEASUREMENTS; RADIATIVE-TRANSFER MODELS; SPECTROSCOPY MAX-DOAS; ABSORPTION SPECTROSCOPY; MULTIPLE-SCATTERING; SOLAR TRACKER; IN-SITU; AERONET; DEPTH; DISTRIBUTIONS AB The multiannual global mean of aerosol optical depth at 550 nm (AOD(550))over land is similar to 0.19, and that over oceans is similar to 0.13. About 45% of the Earth surface shows AOD550 smaller than 0.1. There is a need for measurement techniques that are optimized to measure aerosol optical properties under low AOD conditions. We present an inherently calibrated retrieval (i.e., no need for radiance calibration) to simultaneously measure AOD and the aerosol phase function parameter, g, based on measurements of azimuth distributions of the Raman scattering probability (RSP), the near-absolute rotational Raman scattering (RRS) intensity. We employ radiative transfer model simulations to show that for solar azimuth RSP measurements at solar elevation and solar zenith angle (SZA) smaller than 80 degrees, RSP is insensitive to the vertical distribution of aerosols and maximally sensitive to changes in AOD and g under near-molecular scattering conditions. The University of Colorado two-dimensional Multi-AXis Differential Optical Absorption Spectroscopy (CU 2-D-MAX-DOAS) instrument was deployed as part of the Two Column Aerosol Project (TCAP) at Cape Cod, MA, during the summer of 2012 to measure direct sun spectra and RSP from scattered light spectra at solar relative azimuth angles (SRAAs) between 5 and 170 degrees. During two case study days with (1) high aerosol load (17 July, 0.3 < AOD(430) < 0.6) and (2) near-molecular scattering conditions (22 July, AOD(430) < 0.13) we compare RSP-based retrievals of AOD(430) and g with data from a co-located CIMEL sun photometer, Multi-Filter Rotating Shadowband Radiometer (MFRSR), and an airborne High Spectral Resolution Lidar (HSRL-2). The average difference (relative to DOAS) for AOD(430) is + 0.012 +/- 0.023 (CIMEL), -0.012 +/- 0.024 (MFRSR), -0.011 +/- 0.014 (HSRL-2), and +0.023 +/- 0.013 (CIMELAOD - MFRSRAOD) and yields the following expressions for correlations between different instruments: DOAS(AOD) = -(0.019 +/- 0.006) + (1.03 +/- 0.02) X CIMELAOD (R-2 = 0.98), DOAS(AOD) = -(0.006 +/- 0.005) +. 1.08 +/- 0.02) x MFRSRAOD (R-2 = 0.98), and CIMELAOD = (0.013 +/- 0.004) + (1.05 +/- 0.01) x MFRSRAOD (R-2 = 0.99). The average g measured by DOAS on both days was 0.66 +/- 0.03, with a difference of 0.014 +/- 0.05 compared to CIMEL. Active steps to minimize the error in the RSP help to reduce the uncertainty in retrievals of AOD and g. As AOD decreases and SZA increases, the RSP signal-to-noise ratio increases. At AOD(430) similar to 0.4 and 0.10 the absolute AOD errors are similar to 0.014 and 0.003 at 70 degrees SZA and 0.02 and 0.004 at 35 degrees SZA. Inherently calibrated, precise AOD and g measurements are useful to better characterize the aerosol direct effect in urban polluted and remote pristine environments. C1 [Ortega, Ivan; Coburn, Sean; Volkamer, Rainer] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Ortega, Ivan; Coburn, Sean; Lantz, Kathy; Michalsky, Joseph; Volkamer, Rainer] CIRES, Boulder, CO 80309 USA. [Berg, Larry K.] Pacific Northwest Natl Lab, Richland, WA USA. [Lantz, Kathy; Michalsky, Joseph] NOAA, Global Monitoring Div, Earth Syst Res Lab, Boulder, CO USA. [Ferrare, Richard A.; Hair, JohnathanW.; Hostetler, Chris A.] NASA Langley Res Ctr, Hampton, VA USA. RP Volkamer, R (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA.; Volkamer, R (reprint author), CIRES, Boulder, CO 80309 USA. EM rainer.volkamer@colorado.edu RI Volkamer, Rainer/B-8925-2016 OI Volkamer, Rainer/0000-0002-0899-1369 FU NSF-CAREER [ATM-0847793]; US Department of Energy (DOE) [DE-SC0006080]; NASA Earth Science graduate fellowship; DOE Atmospheric System Research (ASR) Program; Battelle Memorial Institute [DE-AC06-76RLO 1830]; DOE ARM program: Interagency Agreement [DE-SC0006730] FX The instrument was developed with support from the NSF-CAREER award ATM-0847793; US Department of Energy (DOE) award DE-SC0006080 supported the TCAP deployment (RV). Ivan Ortega is the recipient of a NASA Earth Science graduate fellowship. Larry Berg is supported by the DOE Atmospheric System Research (ASR) Program. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. Support for the HSRL-2 light operations during TCAP was provided by the DOE ARM program: Interagency Agreement DE-SC0006730. We are grateful to Tim Deutschmann for providing support with the McArtim RTM. We thank Caroline Fayt and Michel van Roozendael for providing the WinDOAS software and Thomas Wagner for helpful discussions. NR 61 TC 0 Z9 0 U1 3 U2 3 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1867-1381 EI 1867-8548 J9 ATMOS MEAS TECH JI Atmos. Meas. Tech. PD AUG 23 PY 2016 VL 9 IS 8 BP 3893 EP 3910 DI 10.5194/amt-9-3893-2016 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DW6YI UT WOS:000383796900001 ER PT J AU Ge, J Yu, YJ Ke, WJ Li, J Tan, XX Wang, ZW Chu, JH Yan, YF AF Ge, Jie Yu, Yue Ke, Weijun Li, Jian Tan, Xinxuan Wang, Zhiwei Chu, Junhao Yan, Yanfa TI Improved Performance of Electroplated CZTS Thin-Film Solar Cells with Bifacial Configuration SO CHEMSUSCHEM LA English DT Article DE bifacial device; diffusion; indium tin oxide; kesterite; vapor annealing ID CONDUCTING OXIDE BACK; PHOTOVOLTAIC DEVICES; CONTACTS AB Annealing in S vapor greatly improves the performance of electroplated Cu2ZnSnS4 (CZTS) solar cells based on the bifacial configuration of Al-doped ZnO (AZO, front contact)/ZnO/CdS/CZTS/indium tin oxide (ITO, back contact), as compared to H2S annealing in our previous works. S-vapor annealing does not cause severe damage to the conductivity of the ITO back contact. The highest device efficiency of 5.8% was reached under 1sun illumination from the AZO side. The well-preformed devices based on the ITO back contact demonstrate smaller series resistances and better fill factors, as compared to our substrate-type devices using Mo back contacts. An interfacial reaction at the ITO back contact has been revealed in experiments, which contributes to the formation of SnO2-enriched interfacial layer and diffusion of In from ITO into CZTS through the Sn sites. Incorporation of In does not significantly change the optical and structural properties or the grain size of CZTS absorbers. C1 [Ge, Jie; Yu, Yue; Ke, Weijun; Li, Jian; Tan, Xinxuan; Wang, Zhiwei; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. [Wang, Zhiwei] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Chu, Junhao] Chinese Acad Sci, Natl Lab Infrared Phys, Shanghai Inst Tech Phys, Shanghai 800081, Peoples R China. RP Ge, J; Yan, YF (reprint author), Univ Toledo, Dept Phys & Astron, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. EM Jie.Ge@UToledo.edu; Yanfa.Yan@UToledo.edu FU National Science Foundation of USA [CHE-1230246, DMR-1534686]; Ohio Research Scholar Program FX The financial supports by the National Science Foundation of USA (Contract No. CHE-1230246 and DMR-1534686) and Ohio Research Scholar Program are acknowledged. The discussion with Prof. Jian V. Li in Texas State University is thanked. NR 50 TC 2 Z9 2 U1 20 U2 20 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD AUG 23 PY 2016 VL 9 IS 16 BP 2149 EP 2158 DI 10.1002/cssc.201600440 PG 10 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DV9NN UT WOS:000383267600019 PM 27400033 ER PT J AU Busato, L Boaga, J Peruzzo, L Himi, M Cola, S Bersan, S Cassiani, G AF Busato, Laura Boaga, Jacopo Peruzzo, Luca Himi, Mahjoub Cola, Simonetta Bersan, Silvia Cassiani, Giorgio TI Combined geophysical surveys for the characterization of a reconstructed river embankment SO ENGINEERING GEOLOGY LA English DT Article DE River embankment; Jet-grouting; ERT; MASW; GPR; Geophysical characterization ID GEOTECHNICAL CHARACTERIZATION; RESISTIVITY TOMOGRAPHY; ELECTRICAL-RESISTIVITY; SURFACE-WAVES; CONCRETE; DAM AB The managing and monitoring of natural and artificial river levees are crucial in order to reduce the hydrological risk. As these hydraulic structures are very extensive, the typically applied techniques (e.g. geotechnical soundings and visual inspections) provide only punctual information that are generally focused on areas already recognized as troublesome. To overcome these well-known issues, non-invasive and cost-effective geophysical measurements have been proposed (and used) to supply spatially extensive data that should be integrated with direct investigations. Therefore, in this paper we present the joint use of multichannel analysis of surface waves (MASW), electrical resistivity tomography (ERT), and ground penetrating radar (GPR) to characterize a reconstructed river embankment (made of concrete and tout-venant) prone to serious leakages. We compare common lengthwise ERT profiles, performed from the levee crest, with cross-embankment and cross-river profiles, showing how relying only on the first type of surveys may lead to misinterpretations. Furthermore, we take advantage of a land-streamer for the MASW surveys and of a trans-illumination approach to improve the GPR application. The comparison between geophysical and geotechnical data helps identify the spatial extent of the volume actually invaded by grouting injections, which appears as a highly electrically conductive mean. The lack of homogeneity within this domain, highlighted by the cross-embankment ERT profiles, can be related to the seepage phenomena affecting this artificial levee. Therefore, this case study demonstrates the effectiveness of combining direct and non-invasive investigations for the characterization of river embankments. (C) 2016 Elsevier B.V. All rights reserved. C1 [Busato, Laura; Boaga, Jacopo; Cassiani, Giorgio] Univ Padua, Dept Geosci, Via Giovanni Gradenigo 6-A, I-35131 Padua, Italy. [Peruzzo, Luca] Univ Bordeaux Montaigne, ENSEGID, Bordeaux INP EA4592, 1 Allee Daguin, Pessac, France. [Peruzzo, Luca] Lawrence Berkeley Natl Lab, Geosci Div, GO Energy, Bldg 74,Calvin Rd, Berkeley, CA USA. [Himi, Mahjoub] Univ Barcelona, Dept Mineral Petrol & Appl Geol, Marti i Franques S-N, Barcelona 08030, Spain. [Himi, Mahjoub] Univ Mohammed Premier, Ecole Natl Sci Appl ENSAH, Dept Genie Civil & Environm, Sidi Bouafif 32003, Morocco. [Cola, Simonetta; Bersan, Silvia] Univ Padua, Dept Civil Environm & Architectural Engn, Via Marzolo 9, I-35131 Padua, Italy. RP Busato, L (reprint author), Univ Padua, Dept Geosci, Via Giovanni Gradenigo 6-A, I-35131 Padua, Italy. OI Busato, Laura/0000-0003-0588-0847 NR 42 TC 0 Z9 0 U1 9 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0013-7952 EI 1872-6917 J9 ENG GEOL JI Eng. Geol. PD AUG 23 PY 2016 VL 211 BP 74 EP 84 DI 10.1016/j.enggeo.2016.06.023 PG 11 WC Engineering, Geological; Geosciences, Multidisciplinary SC Engineering; Geology GA DU6TM UT WOS:000382347500008 ER PT J AU Howe, K Knapen, S Robinson, DJ AF Howe, Kiel Knapen, Simon Robinson, Dean J. TI Diphotons from electroweak triplet-singlet mixing SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; HIGGS-BOSON; RESONANCE; LHC; EXCESS; SEARCH AB The neutral component of a real pseudoscalar electroweak (EW) triplet can produce a diphoton excess at 750 GeV, if it is somewhat mixed with an EW singlet pseudoscalar. This triplet-singlet mixing allows for greater freedom in the diboson branching ratios than the singlet-only case, but it is still possible to probe the parameter space extensively with 300 fb(-1). The charged component of the triplet is pair produced at the LHC, which results in a striking signal in the form of a pair of W gamma resonances with an irreducible rate of 0.27 fb. Other signatures include multiboson final states from cascade decays of the triplet-singlet neutral states. A large class of composite models feature both EW singlet and triplet pseudo-Nambu-Goldstone bosons in their spectrum, with the diboson couplings generated by axial anomalies. C1 [Howe, Kiel] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Knapen, Simon; Robinson, Dean J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Knapen, Simon; Robinson, Dean J.] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Knapen, Simon; Robinson, Dean J.] Univ Tokyo, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. RP Howe, K (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. OI Howe, Kiel/0000-0001-5044-6041 FU LDRD Program of LBNL under U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC02-07CH11359]; National Science Foundation (NSF) [PHY-1002399]; WPI, MEXT, Japan FX We thank Bogdan Dobrescu, Roni Hamik and Paddy Fox for the discussions which initiated this work. We are also grateful to Keiseke Harigaya, Jack Kearney, Zhen Liu, Tim Lou, Michele Papucci, and Diego Redigolo for useful discussions. We further thank Bogdan Dobrescu, Can Kilic and Diego Redigolo for valuable comments on the manuscript. The work of S. K. was supported by the LDRD Program of LBNL under U.S. Department of Energy Contract No. DE-AC02-05CH11231. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. The work of D. R. is supported by the National Science Foundation (NSF) under Grant No. PHY-1002399. The work of S. K. and D. R. is in part supported by WPI, MEXT, Japan. NR 75 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 23 PY 2016 VL 94 IS 3 AR 035021 DI 10.1103/PhysRevD.94.035021 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KT UT WOS:000381893400007 ER PT J AU Kotwal, AV Ramsey-Musolf, MJ No, JM Winslow, P AF Kotwal, Ashutosh V. Ramsey-Musolf, Michael J. No, Jose Miguel Winslow, Peter TI Singlet-catalyzed electroweak phase transitions in the 100 TeV frontier SO PHYSICAL REVIEW D LA English DT Article ID ATLAS DETECTOR; STANDARD-MODEL; PP COLLISIONS; HIGGS-BOSON; ROOT-S=8 TEV; ENERGY CALIBRATION; DARK-MATTER; LHC; SEARCH; MASS AB We study the prospects for probing a gauge singlet scalar driven strong first-order electroweak phase transition with a future proton-proton collider in the 100 TeV range. Singlet-Higgs mixing enables resonantly enhanced di-Higgs production, potentially aiding discovery prospects. We perform Monte Carlo scans of the parameter space to identify regions associated with a strong first-order electroweak phase transition, analyze the corresponding di-Higgs signal, and select a set of benchmark points that span the range of di-Higgs signal strengths. For the b (b) over bar gamma gamma and 4 tau final states, we investigate discovery prospects for each benchmark point for the high-luminosity phase of the Large Hadron Collider and for a future pp collider with root s = 50, 100, or 200 TeV. We find that any of these future collider scenarios could significantly extend the reach beyond that of the high-luminosity LHC, and that with root s = 100 TeV (200 TeV) and 30 ab(-1), the full region of parameter space favorable to strong first-order electroweak phase transitions is almost fully (fully) discoverable. C1 [Kotwal, Ashutosh V.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Kotwal, Ashutosh V.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Ramsey-Musolf, Michael J.; Winslow, Peter] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Ramsey-Musolf, Michael J.] CALTECH, Kellogg Radiat Lab, Pasadena, CA 91125 USA. [No, Jose Miguel] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. RP Kotwal, AV (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA.; Kotwal, AV (reprint author), Duke Univ, Dept Phys, Durham, NC 27708 USA. EM ashutosh.kotwal@duke.edu; mjrm@physics.umass.edu; J.M.No@sussex.ac.uk; pwinslow@physics.umass.edu FU Fermi National Accelerator Laboratory; United States Department of Energy [DE-AC02-07CH11359, DE-SC0011095]; National Science Foundation [NSF PHY11-25915]; People Programme (Marie Curie Actions) of the European Union Seventh Framework Programme (FP7) [PIEF-GA-2013-625809] FX The work of A. V. K. was supported by the Fermi National Accelerator Laboratory. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. The work of M. J. R. M. and P. W. was supported in part by U.S. Department of Energy Contract No. DE-SC0011095 and by the National Science Foundation under Grant No. NSF PHY11-25915. J. M. N. is supported by the People Programme (Marie Curie Actions) of the European Union Seventh Framework Programme (FP7/2007-2013) under REA grant agreement PIEF-GA-2013-625809. NR 65 TC 2 Z9 2 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 23 PY 2016 VL 94 IS 3 AR 035022 DI 10.1103/PhysRevD.94.035022 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KT UT WOS:000381893400008 ER PT J AU Negi, D Wiedeking, M Lanza, EG Litvinova, E Vitturi, A Bark, RA Bernstein, LA Bleuel, DL Bvumbi, S Bucher, TD Daub, BH Dinoko, TS Easton, JL Gorgen, A Guttormsen, M Jones, P Kheswa, BV Khumalo, NA Larsen, AC Lawrie, EA Lawrie, JJ Majola, SNT Masiteng, LP Nchodu, MR Ndayishimye, J Newman, RT Noncolela, SP Orce, JN Papka, P Pellegri, L Renstrom, T Roux, DG Schwengner, R Shirinda, O Siem, S AF Negi, D. Wiedeking, M. Lanza, E. G. Litvinova, E. Vitturi, A. Bark, R. A. Bernstein, L. A. Bleuel, D. L. Bvumbi, S. Bucher, T. D. Daub, B. H. Dinoko, T. S. Easton, J. L. Goergen, A. Guttormsen, M. Jones, P. Kheswa, B. V. Khumalo, N. A. Larsen, A. C. Lawrie, E. A. Lawrie, J. J. Majola, S. N. T. Masiteng, L. P. Nchodu, M. R. Ndayishimye, J. Newman, R. T. Noncolela, S. P. Orce, J. N. Papka, P. Pellegri, L. Renstrom, T. Roux, D. G. Schwengner, R. Shirinda, O. Siem, S. TI Nature of low-lying electric dipole resonance excitations in Ge-74 SO PHYSICAL REVIEW C LA English DT Article ID EVEN GERMANIUM ISOTOPES; INELASTIC-SCATTERING; BOUND-STATES; NUCLEI; ALPHA; STRENGTH; SN-124 AB Isospin properties of dipole excitations in Ge-74 are investigated using the (alpha,alpha'gamma) reaction and compared to (gamma,gamma') data. The results indicate that the dipole excitations in the energy region of 6 to 9MeV adhere to the scenario of the recently found splitting of the region of dipole excitations into two separated parts: one at low energy, being populated by both isoscalar and isovector probes, and the other at high energy, excited only by the electromagnetic probe. Relativistic quasiparticle time blocking approximation (RQTBA) calculations show a reduction in the isoscalar E1 strength with an increase in excitation energy, which is consistent with the measurement. C1 [Negi, D.; Wiedeking, M.; Bark, R. A.; Bucher, T. D.; Dinoko, T. S.; Easton, J. L.; Jones, P.; Kheswa, B. V.; Lawrie, E. A.; Lawrie, J. J.; Majola, S. N. T.; Nchodu, M. R.; Ndayishimye, J.; Noncolela, S. P.; Papka, P.; Pellegri, L.; Shirinda, O.] iThemba LABS, POB 722, ZA-7129 Somerset West, South Africa. [Negi, D.] UM DAE Ctr Excellence Basic Sci, Mumbai 400098, Maharashtra, India. [Lanza, E. G.] Ist Nazl Fis Nucl, Sez Catania, I-95123 Catania, Italy. [Litvinova, E.] Western Michigan Univ, Kalamazoo, MI 49008 USA. [Litvinova, E.] Michigan State Univ, Nat Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Vitturi, A.] Univ Padua, Dipartimento Fis Astron, Padua, Italy. [Vitturi, A.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Bernstein, L. A.; Bleuel, D. L.; Daub, B. H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bernstein, L. A.; Daub, B. H.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Bvumbi, S.; Masiteng, L. P.] Univ Johannesburg, ZA-2006 Auckland Pk, South Africa. [Dinoko, T. S.; Easton, J. L.; Khumalo, N. A.; Noncolela, S. P.; Orce, J. N.] Univ Western Cape, ZA-7535 Bellville, South Africa. [Goergen, A.; Guttormsen, M.; Larsen, A. C.; Renstrom, T.; Siem, S.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Kheswa, B. V.; Ndayishimye, J.; Newman, R. T.; Papka, P.; Shirinda, O.] Univ Stellenbosch, Dept Phys, ZA-7602 Matieland, South Africa. [Khumalo, N. A.] Univ Zululand, ZA-3886 Kwa Dlangezwa, South Africa. [Majola, S. N. T.] Univ Cape Town, ZA-7701 Rondebosch, South Africa. [Pellegri, L.] Univ Witwatersrand, ZA-2050 Johannesburg, South Africa. [Roux, D. G.] Rhodes Univ, ZA-6410 Grahamstown, South Africa. [Schwengner, R.] Helmholtz Zentrum Dresden Rossendorf, D-01328 Dresden, Germany. RP Negi, D (reprint author), iThemba LABS, POB 722, ZA-7129 Somerset West, South Africa.; Negi, D (reprint author), UM DAE Ctr Excellence Basic Sci, Mumbai 400098, Maharashtra, India. EM dinphysics@gmail.com; wiedeking@tlabs.ac.za RI Larsen, Ann-Cecilie/C-8742-2014 OI Larsen, Ann-Cecilie/0000-0002-2188-3709 FU National Research Foundation of South Africa [92789, 93500]; Research Council of Norway [205528, 213442, 210007]; US-NSF [PHY-1204486, PHY-1404343]; US Department of Energy [DE-AC52-07NA27344, DE-AC02-05CH11231]; ERC-STG [637686] FX The authors would like to thank the operational staff at iThemba LABS for providing excellent beam quality throughout the experiment and Lawrence Berkeley National Laboratory for making available the 74Ge target. This work was supported by the National Research Foundation of South Africa under Grants No. 92789, and No. 93500; by the Research Council of Norway, Project Grants No. 205528, No. 213442, and No. 210007; by US-NSF Grants No. PHY-1204486 and No. PHY-1404343; by the US Department of Energy under Contracts No. DE-AC52-07NA27344, and No. DE-AC02-05CH11231; and by ERC-STG-2014 Grant No. 637686. NR 56 TC 0 Z9 0 U1 4 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 23 PY 2016 VL 94 IS 2 AR 024332 DI 10.1103/PhysRevC.94.024332 PG 6 WC Physics, Nuclear SC Physics GA DU0KM UT WOS:000381892400002 ER PT J AU Madurga, M Paulauskas, SV Grzywacz, R Miller, D Bardayan, DW Batchelder, JC Brewer, NT Cizewski, JA Fijalkowska, A Gross, CJ Howard, ME Ilyushkin, SV Manning, B Matos, M Mendez, AJ Miernik, K Padgett, SW Peters, WA Rasco, BC Ratkiewicz, A Rykaczewski, KP Stracener, DW Wang, EH Wolinska-Cichocka, M Zganjar, EF AF Madurga, M. Paulauskas, S. V. Grzywacz, R. Miller, D. Bardayan, D. W. Batchelder, J. C. Brewer, N. T. Cizewski, J. A. Fijalkowska, A. Gross, C. J. Howard, M. E. Ilyushkin, S. V. Manning, B. Matos, M. Mendez, A. J., II Miernik, K. Padgett, S. W. Peters, W. A. Rasco, B. C. Ratkiewicz, A. Rykaczewski, K. P. Stracener, D. W. Wang, E. H. Wolinska-Cichocka, M. Zganjar, E. F. TI Evidence for Gamow-Teller Decay of Ni-78 Core from Beta-Delayed Neutron Emission Studies SO PHYSICAL REVIEW LETTERS LA English DT Article ID ENERGY-SPECTRA; SHELL-MODEL; PANDEMONIUM; SB-135; SYSTEM; AS-85; I-137 AB The beta-delayed neutron emission of Ga-83,Ga-84 isotopes was studied using the neutron time-of-flight technique. The measured neutron energy spectra showed emission from states at excitation energies high above the neutron separation energy and previously not observed in the beta decay of midmass nuclei. The large decay strength deduced from the observed intense neutron emission is a signature of Gamow-Teller transformation. This observation was interpreted as evidence for allowed beta decay to Ni-78 core-excited states in Ge-83,Ge-84 favored by shell effects. We developed shell model calculations in the proton f pg(9/2) and neutron extended f pg(9/2) + d(5/2) valence space using realistic interactions that were used to understand measured beta-decay lifetimes. We conclude that enhanced, concentrated beta-decay strength for neutron-unbound states may be common for very neutron-rich nuclei. This leads to intense beta-delayed high-energy neutron and strong multineutron emission probabilities that in turn affect astrophysical nucleosynthesis models. C1 [Madurga, M.; Paulauskas, S. V.; Grzywacz, R.; Miller, D.; Padgett, S. W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Madurga, M.] CERN, ISOLDE, EP Dept, CH-1211 Geneva, Switzerland. [Grzywacz, R.; Bardayan, D. W.; Brewer, N. T.; Gross, C. J.; Mendez, A. J., II; Miernik, K.; Rykaczewski, K. P.; Stracener, D. W.; Wolinska-Cichocka, M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37830 USA. [Batchelder, J. C.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94702 USA. [Cizewski, J. A.; Howard, M. E.; Manning, B.; Ratkiewicz, A.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. [Fijalkowska, A.; Miernik, K.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Ilyushkin, S. V.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Matos, M.; Rasco, B. C.; Zganjar, E. F.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Mendez, A. J., II] Austin Peay State Univ, Dept Phys & Astron, Clarksville, TN 37044 USA. [Peters, W. A.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Wang, E. H.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Wolinska-Cichocka, M.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. RP Madurga, M (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.; Madurga, M (reprint author), CERN, ISOLDE, EP Dept, CH-1211 Geneva, Switzerland. RI Peters, William/B-3214-2012 OI Peters, William/0000-0002-3022-4924 FU U.S. Department of Energy (DOE), Office of Science, Office of Nuclear Physics; DOE Office of Science User Facility; National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE [DE-FG52-08NA28552]; Office of Nuclear Physics, U.S. Department of Energy [DE-AC05-00OR22725, DE-FG02-96ER40983, DE-FG-05-88ER40407]; National Science Foundation FX We thank the HRIBF operations staff for providing the excellent quality radioactive ion beams necessary for this work. This material is based upon work supported by the U.S. Department of Energy (DOE), Office of Science, Office of Nuclear Physics and this research used resources of the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory, which was a DOE Office of Science User Facility. This research was sponsored in part by the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Award No. DE-FG52-08NA28552. This research was also sponsored by the Office of Nuclear Physics, U.S. Department of Energy under Awards No. DE-AC05-00OR22725 (ORNL), No. DE-FG02-96ER40983 (UTK), and No. DE-FG-05-88ER40407 (VU) and the National Science Foundation. NR 47 TC 2 Z9 2 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 23 PY 2016 VL 117 IS 9 AR 092502 DI 10.1103/PhysRevLett.117.092502 PG 6 WC Physics, Multidisciplinary SC Physics GA DU1YT UT WOS:000382007600004 PM 27610848 ER PT J AU Silvers, MA Pakhomova, S Neau, DB Silvers, WC Anzalone, N Taylor, CM Waldrop, GL AF Silvers, Molly A. Pakhomova, Svetlana Neau, David B. Silvers, William C. Anzalone, Nicholas Taylor, Carol M. Waldrop, Grover L. TI Crystal Structure of Carboxyltransferase from Staphylococcus aureus Bound to the Antibacterial Agent Moiramide B SO BIOCHEMISTRY LA English DT Article ID ACETYL-COA CARBOXYLASE; FATTY-ACID BIOSYNTHESIS; DRUG DISCOVERY; ESCHERICHIA-COLI; INHIBITORS; METABOLISM; PROSPECTS; COMPONENT; ENZYMES AB The dramatic increase in the prevalence of antibiotic-resistant bacteria has necessitated a search for new antibacterial agents against novel targets. Moiramide B is a natural product, broad-spectrum antibiotic that inhibits the carboxyltransferase component of acetyl-CoA carboxylase, which catalyzes the first committed step in fatty acid synthesis. Herein, we report the 2.6 angstrom resolution crystal structure of moiramide B bound to carboxyltransferase. An unanticipated but significant finding was that moiramide B bound as the enol/enolate. Crystallographic studies demonstrate that the (4S)-methyl succinimide moiety interacts with the oxyanion holes of the enzyme, supporting the notion that an anionic enolate is the active form of the antibacterial agent. Structure-activity studies demonstrate that the unsaturated fatty acid tail of moiramide B is needed only for entry into the bacterial cell. These results will allow the design of new antibacterial agents against the bacterial form of carboxyltransferase. C1 [Silvers, Molly A.; Pakhomova, Svetlana; Anzalone, Nicholas; Waldrop, Grover L.] Louisiana State Univ, Div Biochem & Mol Biol, Baton Rouge, LA 70803 USA. [Taylor, Carol M.] Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. [Neau, David B.] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. [Neau, David B.] Argonne Natl Lab, Northeastern Collaborat Access Team, 9700 S Cass Ave, Argonne, IL 60439 USA. [Silvers, William C.] Univ Texas Southwestern Med Ctr Dallas, Dept Radiol, Dallas, TX 75390 USA. RP Waldrop, GL (reprint author), Louisiana State Univ, 509 Choppin Hall, Baton Rouge, LA 70803 USA. EM gwaldro@lsu.edu RI Taylor, Carol/B-4841-2012; OI Taylor, Carol/0000-0002-6262-0796; Silvers, Molly/0000-0001-5544-8329 FU National Institute of General Medical Sciences from the National Institutes of Health (NIH) [P41 GM103403]; NIH-ORIP HEI grant [S10 RR029205]; DOE Office of Science [DE-AC02-06CH11357] FX This work is based upon research conducted at the Northeastern Collaborative Access Team beamlines, which are funded by the National Institute of General Medical Sciences from the National Institutes of Health (NIH) (P41 GM103403). The Pilatus 6M detector on beamline 24-ID-C is funded by a NIH-ORIP HEI grant (S10 RR029205). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. NR 34 TC 0 Z9 0 U1 6 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD AUG 23 PY 2016 VL 55 IS 33 BP 4666 EP 4674 DI 10.1021/acs.biochem.6b00641 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DU1HZ UT WOS:000381960100008 PM 27471863 ER PT J AU Yan, M Chakravarthy, S Tokuda, JM Pollack, L Bowman, GD Lee, YS AF Yan, Ming Chakravarthy, Srinivas Tokuda, Joshua M. Pollack, Lois Bowman, Gregory D. Lee, Young-Sam TI Succinyl-5-aminoimidazole-4-carboxamide-1-ribose 5 '-Phosphate (SAICAR) Activates Pyruvate Kinase Isoform M2 (PKM2) in Its Dimeric Form SO BIOCHEMISTRY LA English DT Article ID PROTEIN-KINASE; NUCLEAR TRANSLOCATION; GENE-TRANSCRIPTION; TUMOR-GROWTH; CANCER; PROMOTES; TUMORIGENESIS; CELLS; SAXS AB Human pyruvate kinase isoform M2 (PKM2) is a glycolytic enzyme isoform implicated in cancer. Malignant cancer cells have higher levels of dimeric PKM2, which is regarded as an inactive form of tetrameric pyruvate kinase. This perceived inactivity has fueled controversy about how the dimeric form of pyruvate kinase might contribute to cancer. Here we investigate enzymatic properties of PKM2(G415R), a variant derived from a cancer patient, which we show by size-exclusion chromatography and small-angle X-ray scattering to be a dimer that cannot form a tetramer in solution. Although PKM2(G415R) binds to fructose 1,6-bisphosphate (FBP), unlike the wild type this PKM2 variant shows no activation by FBP. In contrast, PKM2(G415R) is activated by succinyl-5-aminoimidazole-4-carboxamide-1-ribose 5'-phosphate (SAICAR), an endogenous metabolite that we previously showed correlates with an increased level of cell proliferation and promotes protein kinase activity of PKM2. Our results demonstrate an important and unexpected enzymatic activity of the PKM2 dimer that likely has a key role in cancer progression. C1 [Yan, Ming; Bowman, Gregory D.] Johns Hopkins Univ, TC Jenkins Dept Biophys, 3400 N Charles St, Baltimore, MD 21218 USA. [Yan, Ming; Lee, Young-Sam] Johns Hopkins Univ, Dept Biol, 3400 N Charles St, Baltimore, MD 21218 USA. [Chakravarthy, Srinivas] Argonne Natl Lab, Biophys Collaborat Access Team, 9700 S Cass Ave, Argonne, IL 60439 USA. [Tokuda, Joshua M.; Pollack, Lois] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. RP Bowman, GD (reprint author), Johns Hopkins Univ, TC Jenkins Dept Biophys, 3400 N Charles St, Baltimore, MD 21218 USA.; Lee, YS (reprint author), Johns Hopkins Univ, Dept Biol, 3400 N Charles St, Baltimore, MD 21218 USA. EM gdbowman@jhu.edu; ylee99@jhu.edu RI ID, BioCAT/D-2459-2012 FU National Institutes of Health [R21CA181751, R01CA168658]; DOE Office of Science [DE-AC02-06CH11357]; National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health [9 P41 GM103622]; NIGMS [1S10OD018090-01] FX This work was supported by National Institutes of Health Grants R21CA181751 to G.D.B. and Y.-S.L. and R01CA168658 to Y.-S.L. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. The SAXS experiment was supported by Grant 9 P41 GM103622 from the National Institute of General Medical Sciences (NIGMS) of the National Institutes of Health. Use of the Pilatus 3 1M detector was provided by Grant 1S10OD018090-01 from NIGMS. NR 29 TC 1 Z9 1 U1 1 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD AUG 23 PY 2016 VL 55 IS 33 BP 4731 EP 4736 DI 10.1021/acs.biochem.6b00658 PG 6 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DU1HZ UT WOS:000381960100014 PM 27481063 ER PT J AU Parija, A Liang, YF Andrews, JL De Jesus, LR Prendergast, D Banerjee, S AF Parija, Abhishek Liang, Yufeng Andrews, Justin L. De Jesus, Luis R. Prendergast, David Banerjee, Sarbajit TI Topochemically De-Intercalated Phases of V2O5 as Cathode Materials for Multivalent Intercalation Batteries: A First-Principles Evaluation SO CHEMISTRY OF MATERIALS LA English DT Article ID VANADIUM-OXIDE BRONZES; LITHIUM-ION BATTERIES; ELECTRONIC-STRUCTURE; LI INTERCALATION; MATERIALS DESIGN; MG; NANOWIRES; INSERTION; SPECTRA AB The scarce inventory of compounds that allow for diffusion of multivalent cations at reasonable rates poses a major impediment to the development of multivalent intercalation batteries. Here, we contrast the thermodynamics and kinetics of the insertion of Li, Na, Mg, and Al ions in two synthetically accessible metastable phases of V2O5, zeta- and epsilon-V2O5, with the relevant parameters for the thermodynamically stable alpha-phase of V2O5 using density functional theory calculations. The metastability of the frameworks results in a higher open circuit voltage for multivalent ions, exceeding 3 V for Mg-ion intercalation. Multivalent ions inserted within these structures encounter suboptimal coordination environments and expanded transition states, which facilitate easier ion diffusion. Specifically, a nudged elastic band examination of ion diffusion pathways suggests that migration barriers are substantially diminished for Na- and Mg-ion diffusion in the metastable polymorphs: the predicted migration barriers for Mg ions in zeta-V2O5 and epsilon-V2O5 are 0.62-0.86 and 0.21-0.24 eV, respectively. More generally, the results indicate that topochemically derived metastable polymorphs represent an interesting class of compounds for realizing multivalent cation diffusion because many such compounds place cations in "frustrated" coordination environments that are known to be useful for realizing low diffusion barriers. C1 [Parija, Abhishek; Andrews, Justin L.; De Jesus, Luis R.; Banerjee, Sarbajit] Texas A&M Univ, Dept Chem, College Stn, TX 77845 USA. [Parija, Abhishek; Andrews, Justin L.; De Jesus, Luis R.; Banerjee, Sarbajit] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77845 USA. [Liang, Yufeng; Prendergast, David] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Banerjee, S (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77845 USA.; Banerjee, S (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77845 USA.; Prendergast, D (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM dgprendergast@lbl.gov; banerjee@chem.tamu.edu FU National Science Foundation [DMR 1504702, 1252521]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported primarily by the National Science Foundation via Grant DMR 1504702. We also thank the Texas A&M Supercomputing Facility for computational resources. L.R.D.J. acknowledges support from a National Science Foundation Graduate Research Fellowship under Grant 1252521. Density functional theory simulations were performed as part of a User Project with Y.L. and D.G.P. at The Molecular Foundry (TMF), Lawrence Berkeley National Laboratory. TMF is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, under Contract DE-AC02-05CH11231. NR 47 TC 2 Z9 2 U1 36 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 23 PY 2016 VL 28 IS 16 BP 5611 EP 5620 DI 10.1021/acs.chemmater.6b01006 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DU1IB UT WOS:000381960300009 ER PT J AU Cooper, JK Scott, SB Ling, YC Yang, JH Hao, SJ Li, Y Toma, FM Stutzmann, M Lakshmi, KV Sharp, ID AF Cooper, Jason K. Scott, Soren B. Ling, Yichuan Yang, Jinhui Hao, Sijie Li, Yat Toma, Francesca M. Stutzmann, Martin Lakshmi, K. V. Sharp, Ian D. TI Role of Hydrogen in Defining the n-Type Character of BiVO4 Photoanodes SO CHEMISTRY OF MATERIALS LA English DT Article ID BISMUTH VANADATE PHOTOANODES; WATER OXIDATION; OPTICAL-ABSORPTION; METAL-OXIDE; SPECTROSCOPY; TEMPERATURE; TRANSPORT; GLASSES; IONS; PHOTOELECTRODES AB The roles of hydrogen impurity and oxygen vacancy defects on defining the conductivity, and hence photoelectrochemical (PEC) performance characteristics, of monoclinic scheelite bismuth vanadate (BiVO4) are investigated using a combination of experiment and theory. We find that elemental hydrogen is present as an impurity in as-synthesized if BiVO4 and that increasing its concentration by annealing in H-2 at temperatures up to 290 degrees C leads to near-complete elimination of majority carrier transport limitations, a beneficial shift in the photoanodic current onset potential, and improved fill factor. Magnetic resonance measurements reveal that hydrogen can be incorporated in at least two different chemical environments, which are assigned to interstitial and substitutional sites. Incorporation of hydrogen leads to a shift of the Fermi level toward the conduction band edge, indicating that n-type character is correlated with increased hydrogen content. This finding is in agreement with theory and reveals that hydrogen acts as a donor in BiVO4. Sub-bandgap photoluminescence is observed from as-synthesized material and is consistent with deep electronic states associated with oxygen vacancies. Hydrogen treatment leads to reduced emission from these states. These findings support the conclusion that hydrogen, rather than oxygen vacancies, is dominant in determining the n-type conductivity of BiVO4. These findings have important implications for controlling the electronic properties and functional characteristics of this promising photoanode material. C1 [Cooper, Jason K.; Scott, Soren B.; Yang, Jinhui; Toma, Francesca M.; Sharp, Ian D.] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Cooper, Jason K.; Yang, Jinhui; Toma, Francesca M.; Sharp, Ian D.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Ling, Yichuan; Li, Yat] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Hao, Sijie; Stutzmann, Martin] Tech Univ Munich, Walter Schottky Inst, Coulombwall 4, D-85748 Garching, Germany. [Hao, Sijie; Stutzmann, Martin] Tech Univ Munich, Phys Dept, Coulombwall 4, D-85748 Garching, Germany. [Lakshmi, K. V.] Rensselaer Polytech Inst, Dept Chem & Chem Biol, Troy, NY 12180 USA. [Lakshmi, K. V.] Rensselaer Polytech Inst, Baruch Ctr Biochem Solar Energy Res 60, Troy, NY 12180 USA. RP Sharp, ID (reprint author), Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.; Sharp, ID (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM idsharp@lbl.gov RI Lakshmi, K. V./A-9787-2017; OI Lakshmi, K. V./0000-0001-5443-9017; Li, Yat/0000-0002-8058-2084 FU Office of Science of the U.S. Department of Energy [DE-SC0004993, DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI); Office of Science, Basic Energy Sciences of the U.S. Department of Energy [DE-FG02-07ER15903]; NIH [1S10RR016634-01] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. SBS acknowledges support from the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI). KVL was supported by the Office of Science, Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-FG02-07ER15903. We acknowledge the UC Berkeley College of Chemistry NMR; the AV-500 was partially funded by NIH grant 1S10RR016634-01. The authors are grateful to Chris Canlas for his assistance with 1H NMR spectroscopy. Calculations were performed using the Hopper cluster at the National Energy Research Scientific Computing Center (NERSC) at the LBNL supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 58 TC 3 Z9 3 U1 36 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 23 PY 2016 VL 28 IS 16 BP 5761 EP 5771 DI 10.1021/acs.chemmater.6b01994 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DU1IB UT WOS:000381960300024 ER PT J AU Landry, AM Iglesia, E AF Landry, Alexandra M. Iglesia, Enrique TI Synthesis of Bimetallic AuPt Clusters with Clean Surfaces via Sequential Displacement-Reduction Processes SO CHEMISTRY OF MATERIALS LA English DT Article ID GOLD NANOPARTICLES; COLLOIDAL NANOPARTICLES; ELEMENTARY STEPS; PT NANOPARTICLES; CHARGE-TRANSFER; SIZE CONTROL; CATALYSIS; PLATINUM; NUCLEATION; OXIDATION AB We report the synthesis of bimetallic AuPt nanoparticles (3.3-4.3 nm) of uniform size and composition using colloidal methods and reagents containing only C, H, O, and N. These clusters were dispersed onto SiO2 and treated at low temperatures in the presence of reductants to remove all surface residues without concomitant agglomeration, thus leading to bimetallic structures suitable for mechanistic inquiries into bimetallic effects on surface reactivity. Synthesis protocols exploit and generalize galvanic displacement reduction (GDR) processes previously used to prepare AuPd clusters; these routes promote bimetallic mixing but become more challenging for systems (e.g., AuPt) with smaller reduction potential differences and less favorable mixing enthalpies than AuPd. These hurdles are addressed here through procedural modifications that inhibit the formation of large Au-rich clusters, which compromise size and compositional uniformity. In doing so, we extend GDR techniques to endothermic alloys with elements of more similar redox properties. Higher temperatures and lower Au3+ precursor concentrations promoted metal mixing and inhibited homogeneous and heterogeneous nucleation. Cluster size and compositional uniformity were confirmed by UV-visible spectroscopy during and after colloid formation, transmission electron microscopy, and high-angle annular dark-field (HAADF) imaging with energy-dispersive X-ray spectroscopy (EDS). Particle-by-particle EDS analysis and HAADF imaging demonstrated the prevalence of GDR processes in AuPd bimetallic cluster assembly. These methods also showed that size-dependent intracluster diffusion during AuPt cluster formation, driven by unfavorable AuPt mixing thermodynamics, leads to Au surface enrichment, thus promoting autocatalytic Au deposition. This rigorous mechanistic comparison of AuPt and AuPd systems provides essential guidance and specific control variables and procedures for the synthesis of other bimetallic systems based on the redox potential differences and mixing thermodynamics of their two components. C1 [Iglesia, Enrique] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. EO Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Iglesia, E (reprint author), Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. EM iglesia@berkeley.edu RI Iglesia, Enrique/D-9551-2017 OI Iglesia, Enrique/0000-0003-4109-1001 FU National Science Foundation Graduate Research Fellowship (NSF GRF); Achievement Rewards for College Scientists (ARCS) Fellowship; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Basic Energy Sciences, Chemical Sciences Division of the US Department of Energy [DE-AC02-05CH11231] FX The author acknowledges the National Science Foundation Graduate Research Fellowship (NSF GRF) and Achievement Rewards for College Scientists (ARCS) Fellowship for funding, as well as the Electron Microscopy Lab (EML) at the University of California, Berkeley for TEM facilities and the National Center for Electron Microscopy (NCEM) for EDS and HAADF facilities. NCEM is supported by the Office of Basic Energy Sciences of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. This work was supported by the Director, Office of Basic Energy Sciences, Chemical Sciences Division of the US Department of Energy under contract No. DE-AC02-05CH11231. NR 48 TC 3 Z9 3 U1 16 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 23 PY 2016 VL 28 IS 16 BP 5872 EP 5886 DI 10.1021/acs.chemmater.6b02346 PG 15 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DU1IB UT WOS:000381960300035 ER PT J AU Dedon, LR Saremi, S Chen, ZH Damodaran, AR Apgar, BA Gao, R Martin, LW AF Dedon, Liv R. Saremi, Sahar Chen, Zuhuang Damodaran, Anoop R. Apgar, Brent A. Gao, Ran Martin, Lane W. TI Nonstoichiometry, Structure, and Properties of BiFeO3 Films SO CHEMISTRY OF MATERIALS LA English DT Article ID THIN-FILMS; FERROELECTRIC PROPERTIES; EXCESS BI; GROWTH; STOICHIOMETRY; POLARIZATION; DEPOSITION; INTERFACE; EVOLUTION AB We explore the effect of growth conditions on the cation and anion chemistry, electrical leakage, conduction mechanisms, and ferroelectric and dielectric behavior of BiFeO3. Although it is possible to produce single-phase, coherently strained films in all cases, small variations in the pulsed-laser deposition growth process, specifically the laser repetition rate and target composition, result in films with chemistries ranging from 10% Bi-deficiency to 4% Bi-excess and films possessing Bi gradients as large a 6% across the film thickness. Corresponding variations and gradients in the O chemistry are also observed. As a result of the varying film chemistry, marked differences in surface and domain morphology are observed wherein Bi-deficiency stabilizes atomically smooth surfaces and ordered stripe domains. Subsequent investigation of the current voltage response reveals large differences in leakage current density arising from changes in both the overall stoichiometry and gradients. In turn, the film stoichiometry drives variations in the dominant conduction mechanism including examples of Schottky, Poole-Frenkel, and modified Poole-Frenkel emission depending on the film chemistry. Finally, slightly Bi-excess films are found to exhibit the best low-frequency ferroelectric and dielectric response while increasing Bi-deficiency worsens the low-frequency ferroelectric performance and reduces the dielectric permittivity. C1 [Dedon, Liv R.; Saremi, Sahar; Chen, Zuhuang; Damodaran, Anoop R.; Apgar, Brent A.; Gao, Ran; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Dedon, Liv R.; Martin, Lane W.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Martin, LW (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Martin, LW (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM lwmartin@berkeley.edu RI Martin, Lane/H-2409-2011; Chen, Zuhuang/E-7131-2011 OI Martin, Lane/0000-0003-1889-2513; Chen, Zuhuang/0000-0003-1912-6490 FU U.S. Department of Energy [DE-SC0012375]; National Science Foundation [CMMI-1434147, OISE-1545907, DMR-1451219]; Air Force Office of Scientific Research [FA9550-12-1-0471]; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; Army Research Office [W911NF-14-1-0104] FX L.R.D. acknowledges support from the U.S. Department of Energy under Grant No. DE-SC0012375. S.S. acknowledges support from the National Science Foundation under Grant CMMI-1434147. Z.C. acknowledges partial support from the Air Force Office of Scientific Research under Grant FA9550-12-1-0471 and the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231. A.R.D. acknowledges support from the Army Research Office under Grant W911NF-14-1-0104. R.G. acknowledges support from the National Science Foundation under Grant OISE-1545907. L.W.M. acknowledges support from the National Science Foundation under Grant DMR-1451219. NR 53 TC 0 Z9 0 U1 20 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD AUG 23 PY 2016 VL 28 IS 16 BP 5952 EP 5961 DI 10.1021/acs.chemmater.6b02542 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DU1IB UT WOS:000381960300043 ER PT J AU Murphy, RP Hong, KL Wagner, NJ AF Murphy, Ryan P. Hong, Kunlun Wagner, Norman J. TI Thermoreversible Gels Composed of Colloidal Silica Rods with Short Range Attractions SO LANGMUIR LA English DT Article ID PHASE-BEHAVIOR; GROWTH; MODEL; DISPERSIONS; GELATION; TEMPERATURE; SCATTERING; PARTICLES; RHEOLOGY; SPHERES AB Dynamic arrest transitions of colloidal suspensions containing nonspherical particles are of interest for the design and processing of various particle technologies. To better understand the effects of particle shape anisotropy and attraction strength on gel and glass formation, we present a colloidal model system of octadecyl-coated silica rods, termed as adhesive hard rods (AHR), which enables control of rod aspect ratio and temperature-dependent interactions. The aspect ratios of silica rods were controlled by varying the initial TEOS concentration following the work of Kuijk et al. (J. Am. Chem. Soc., 2011, 133, 2346-2349) and temperature-dependent attractions were introduced by coating the calcined silica rods with an octadecyl-brush and suspending in tetradecane. The rod length and aspect ratio were found to increase with TEOS concentration as expected, while other properties such as the rod diameter, coating coverage, density, and surface roughness were nearly independent of the aspect ratio. Ultrasmall angle X-ray scattering measurements revealed temperature-dependent attractions between octadecyl-coated silica rods in tetradecane, as characterized by a low-q upturn in the scattered intensity upon thermal quenching. Lastly, the rheology of a concentrated AHR suspension in tetradecane demonstrated thermoreversible gelation behavior, displaying a nearly 5 orders of magnitude change in the dynamic moduli as the temperature was cycled between 15 and 40 degrees C. The adhesive hard rod model system serves as a tunable platform to explore the combined influence of particle shape anisotropy and attraction strength on the dynamic arrest transitions in colloidal suspensions with thermoreversible, short-range attractions. C1 [Murphy, Ryan P.; Wagner, Norman J.] Univ Delaware, Ctr Mol & Engn Thermodynam, Newark, DE 19716 USA. [Murphy, Ryan P.; Wagner, Norman J.] Univ Delaware, Dept Chem & Biomol Engn, Ctr Neutron Sci, Newark, DE 19716 USA. [Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wagner, NJ (reprint author), Univ Delaware, Ctr Mol & Engn Thermodynam, Newark, DE 19716 USA.; Wagner, NJ (reprint author), Univ Delaware, Dept Chem & Biomol Engn, Ctr Neutron Sci, Newark, DE 19716 USA. EM wagnernj@udel.edu RI Wagner, Norman/B-6558-2012; Hong, Kunlun/E-9787-2015 OI Wagner, Norman/0000-0001-9565-619X; Hong, Kunlun/0000-0002-2852-5111 FU University of Delaware (UD); National Institute of Standards and Technology (NIST) [70NANB10H2S6, 70NANB12H239]; DOE Office of Science [DE-AC02-06CH11357]; DANSE project under NSF award [DMR-0520547] FX The authors acknowledge financial support of this work from the University of Delaware (UD) and the National Institute of Standards and Technology (NIST) under the cooperative agreements 70NANB10H2S6 and 70NANB12H239. Particle synthesis and characterization was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. X-ray scattering data was collected at the USAXS beamline 9-ID-C at the Advanced Photon Source, Argonne National Laboratory, with the assistance of Dr. Jan Ilavsky. This work benefitted from SasView software originally developed by the DANSE project under NSF award DMR-0520547. The authors also acknowledge the UD Keck Microscopy Laboratory and the UD Advanced Materials Characterization Laboratory for additional TEM and BET measurements. The authors thank Dr. Jan Ilaysky (APS), Dr. Jen Sloppy (UD), Dr. Chaoying Ni (UD), Gerald Poirier (UD), and Michelle Pawel (CNMS) for their technical assistance. NR 46 TC 1 Z9 1 U1 14 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD AUG 23 PY 2016 VL 32 IS 33 BP 8424 EP 8435 DI 10.1021/acs.langmuir.6b02107 PG 12 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DU1HQ UT WOS:000381959200015 PM 27466883 ER PT J AU Liu, S Xu, T AF Liu, Shuai Xu, Ting TI Ionic Liquids Containing Block Copolymer Based Supramolecules SO MACROMOLECULES LA English DT Article ID THIN-FILM TRANSISTORS; GEL GATE DIELECTRICS; PHYSICOCHEMICAL PROPERTIES; TRIBLOCK COPOLYMER; IMIDAZOLIUM CATION; CARBON CAPTURE; LENGTH SCALES; CONDUCTIVITY; SEPARATION; CONVERSION AB Block copolymer (BCP)-based supramolecules provide a versatile strategy to generate functional materials using noncovalent bond between small molecules and BCPs. Here, we report supramolecules composed of phenol-containing ionic liquids (ILs) hydrogen bonded to BCP, polystyrene-block-poly(4-vinyl-pyridine) (PS-b-P4VP). IL-containing supramolecules exhibit ordered structures in a wide range of IL loading and chemistry. Rheological behaviors and nanostructures of IL-containing supramolecules can be tuned by controlling the IL loading without losing ordered structure. The hydrogen bonds and nanostructures can be retained in a wide range of temperatures with different IL chemistry. Supramolecules provide a diverse platform toward IL materials with ordered structure and tunable properties with high tolerance of thermal treatment and processing. C1 [Liu, Shuai; Xu, Ting] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Xu, Ting] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Liu, Shuai; Xu, Ting] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Xu, T (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Xu, T (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Xu, T (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM tingxu@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 41 TC 0 Z9 0 U1 18 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD AUG 23 PY 2016 VL 49 IS 16 BP 6075 EP 6083 DI 10.1021/acs.macromol.6b01299 PG 9 WC Polymer Science SC Polymer Science GA DU1HU UT WOS:000381959600033 ER PT J AU Eisenberg, DS Sawaya, MR AF Eisenberg, David S. Sawaya, Michael R. TI Implications for Alzheimer's disease of an atomic resolution structure of amyloid-beta(1-42) fibrils SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Editorial Material ID BETA-AMYLOID FIBRILS; POLYMORPHISM; PLAQUES; PROTEIN C1 [Eisenberg, David S.; Sawaya, Michael R.] Univ Calif Los Angeles, UCLA DOE Inst, Los Angeles, CA 90095 USA. [Eisenberg, David S.; Sawaya, Michael R.] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA. [Eisenberg, David S.; Sawaya, Michael R.] Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. RP Eisenberg, DS (reprint author), Univ Calif Los Angeles, UCLA DOE Inst, Los Angeles, CA 90095 USA.; Eisenberg, DS (reprint author), Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA.; Eisenberg, DS (reprint author), Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. EM david@mbi.ucla.edu NR 16 TC 3 Z9 3 U1 16 U2 22 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 23 PY 2016 VL 113 IS 34 BP 9398 EP 9400 DI 10.1073/pnas.1610806113 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9ZK UT WOS:000381860800028 PM 27506787 ER PT J AU Kellogg, EH Howes, S Ti, SC Ramirez-Aportela, E Kapoor, TM Chacon, P Nogales, E AF Kellogg, Elizabeth H. Howes, Stuart Ti, Shih-Chieh Ramirez-Aportela, Erney Kapoor, Tarun M. Chacon, Pablo Nogales, Eva TI Near-atomic cryo-EM structure of PRC1 bound to the microtubule SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE PRC1; microtubules; cryo-EM; MAPs; cytoskeleton ID NDC80 KINETOCHORE COMPLEX; MITOTIC SPINDLE; MOLECULAR-DYNAMICS; CRYOELECTRON MICROSCOPY; ELECTRON-MICROSCOPY; PROTEIN-STRUCTURE; MIDZONE FORMATION; BINDING DOMAIN; TUBULIN; PREDICTION AB Proteins that associate with microtubules (MTs) are crucial to generate MT arrays and establish different cellular architectures. One example is PRC1 (protein regulator of cytokinesis 1), which cross-links antiparallel MTs and is essential for the completion of mitosis and cytokinesis. Here we describe a 4-angstrom-resolution cryo-EM structure of monomeric PRC1 bound to MTs. Residues in the spectrin domain of PRC1 contacting the MT are highly conserved and interact with the same pocket recognized by kinesin. We additionally found that PRC1 promotes MT assembly even in the presence of the MT stabilizer taxol. Interestingly, the angle of the spectrin domain on the MT surface corresponds to the previously observed cross-bridge angle between MTs cross-linked by full-length, dimeric PRC1. This finding, together with molecular dynamic simulations describing the intrinsic flexibility of PRC1, suggests that the MT-spectrin domain interface determines the geometry of the MT arrays cross-linked by PRC1. C1 [Kellogg, Elizabeth H.; Nogales, Eva] Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. [Kellogg, Elizabeth H.; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Howes, Stuart] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Ti, Shih-Chieh; Kapoor, Tarun M.] Rockefeller Univ, Lab Chem & Cell Biol, New York, NY 10065 USA. [Ramirez-Aportela, Erney; Chacon, Pablo] CSIC, Rocasolano Phys Chem Inst, Dept Biol Phys Chem, Plaza Murillo 2, E-28006 Madrid, Spain. [Nogales, Eva] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Howes, Stuart] Leiden Univ, Med Ctr, Dept Mol Cell Biol, NL-2333 ZC Leiden, Netherlands. RP Nogales, E (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. EM enogales@lbl.gov RI Chacon, Pablo/B-4211-2014 OI Chacon, Pablo/0000-0002-3168-4826 FU National Energy Research Scientific Computing Center [DE-AC02-05CH11231]; National Institute of General Medical Sciences [GM051487, GM65933]; Ministerio de Economia y Competitividad Grant [BFU2013-44306-P] FX We thank Patricia Grob and Tom Houweling for EM and computer support, respectively, and Peter Northcote and John Miller for their generous gift of peloruside. Computational resources for atomic model refinement were provided by the National Energy Research Scientific Computing Center under Grant DE-AC02-05CH11231. This work was supported by National Institute of General Medical Sciences Grants GM051487 (to E.N.) and GM65933 (to T.M.K.) and Ministerio de Economia y Competitividad Grant BFU2013-44306-P (to E.R.-A. and P.C.). The Gauss Centre for Supercomputing/Leibniz Supercomputing Centre provided high-performance computing resources for this project under a Partnership for Advanced Computing in Europe (PRACE) grant. E.N. is a Howard Hughes Medical Institute Investigator. NR 82 TC 2 Z9 3 U1 9 U2 16 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 23 PY 2016 VL 113 IS 34 BP 9430 EP 9439 DI 10.1073/pnas.1609903113 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9ZK UT WOS:000381860800034 PM 27493215 ER PT J AU Fay, AW Blank, MA Rebelein, JG Lee, CC Ribbe, MW Hedman, B Hodgson, KO Hu, YL AF Fay, Aaron W. Blank, Michael A. Rebelein, Johannes G. Lee, Chi Chung Ribbe, Markus W. Hedman, Britt Hodgson, Keith O. Hu, Yilin TI Assembly scaffold NifEN: A structural and functional homolog of the nitrogenase catalytic component SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE nitrogenase; catalysis; assembly; functional homolog; NifEN ID IRON-MOLYBDENUM COFACTOR; FEMO-COFACTOR; MOFE-PROTEIN; K-EDGE; PRECURSOR; EXAFS; MATURATION; RESOLUTION; INSIGHTS; CARBON AB NifEN is a biosynthetic scaffold for the cofactor of Mo-nitrogenase (designated the M-cluster). Previous studies have revealed the sequence and structural homology between NifEN and NifDK, the catalytic component of nitrogenase. However, direct proof for the functional homology between the two proteins has remained elusive. Here we show that, upon maturation of a cofactor precursor (designated the L-cluster) on NifEN, the cluster species extracted from NifEN is spectroscopically equivalent and functionally interchangeable with the native M-cluster extracted from NifDK. Both extracted clusters display nearly indistinguishable EPR features, X-ray absorption spectroscopy/extended X-ray absorption fine structure (XAS/EXAFS) spectra and reconstitution activities, firmly establishing the M-cluster-bound NifEN (designated NifENM) as the only protein other than NifDK to house the unique nitrogenase cofactor. Iron chelation experiments demonstrate a relocation of the cluster from the surface to its binding site within NifENM upon maturation, which parallels the insertion of M-cluster into an analogous binding site in NifDK, whereas metal analyses suggest an asymmetric conformation of NifENM with an M-cluster in one alpha beta-half and an empty cluster-binding site in the other alpha beta-half, which led to the proposal of a stepwise assembly mechanism of the M-cluster in the two alpha beta-dimers of NifEN. Perhaps most importantly, NifENM displays comparable ATP-independent substrate-reducing profiles to those of NifDK, which establishes the M-cluster-bound alpha beta-dimer of NifENM as a structural and functional mimic of one catalytic alpha beta-half of NifDK while suggesting the potential of this protein as a useful tool for further investigations of the mechanistic details of nitrogenase. C1 [Fay, Aaron W.; Rebelein, Johannes G.; Lee, Chi Chung; Ribbe, Markus W.; Hu, Yilin] Univ Calif Irvine, Dept Mol Biol & Biochem, Irvine, CA 92697 USA. [Blank, Michael A.; Hodgson, Keith O.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Ribbe, Markus W.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Hedman, Britt] Stanford Univ, Stanford Linear Accelerator Ctr, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Blank, Michael A.] Thermo Fisher Sci Inc, 335 River Oaks Pkwy, San Jose, CA 95134 USA. RP Ribbe, MW; Hu, YL (reprint author), Univ Calif Irvine, Dept Mol Biol & Biochem, Irvine, CA 92697 USA.; Hodgson, KO (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA.; Ribbe, MW (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.; Hedman, B (reprint author), Stanford Univ, Stanford Linear Accelerator Ctr, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. EM mribbe@uci.edu; hedman@slac.stanford.edu; hodgson@slac.stanford.edu; yilinh@uci.edu OI Rebelein, Johannes/0000-0003-2560-716X FU NIH [P41GM103393, GM67626]; Hellman Fellowship; US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393] FX This work was supported by NIH Grants P41GM103393 (to K.O.H.) and GM67626 (to M.W.R.) and a Hellman Fellowship (to Y.H.). Use of the Stanford Synchrotron Radiation Lightsource (SSRL), Stanford Linear Accelerator Center National Accelerator Laboratory, is supported by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, National Institute of General Medical Sciences, including Grant P41GM103393. NR 31 TC 0 Z9 0 U1 15 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 23 PY 2016 VL 113 IS 34 BP 9504 EP 9508 DI 10.1073/pnas.1609574113 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9ZK UT WOS:000381860800046 PM 27506795 ER PT J AU Bouchard, KE Brainard, MS AF Bouchard, Kristofer E. Brainard, Michael S. TI Auditory-induced neural dynamics in sensory-motor circuitry predict learned temporal and sequential statistics of birdsong SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE sequences; prediction; uncertainty; electrophysiology; birdsong ID SENSORIMOTOR CORTEX; CORTICAL ACTIVITY; DOPAMINE NEURONS; DECISION-MAKING; SPARSE CODE; SEQUENCES; SONG; GENERATION; BRAIN; ORGANIZATION AB Predicting future events is a critical computation for both perception and behavior. Despite the essential nature of this computation, there are few studies demonstrating neural activity that predicts specific events in learned, probabilistic sequences. Here, we test the hypotheses that the dynamics of internally generated neural activity are predictive of future events and are structured by the learned temporal-sequential statistics of those events. We recorded neural activity in Bengalese finch sensory-motor area HVC in response to playback of sequences from individuals' songs, and examined the neural activity that continued after stimulus offset. We found that the strength of response to a syllable in the sequence depended on the delay at which that syllable was played, with a maximal response when the delay matched the intersyllable gap normally present for that specific syllable during song production. Furthermore, poststimulus neural activity induced by sequence playback resembled the neural response to the next syllable in the sequence when that syllable was predictable, but not when the next syllable was uncertain. Our results demonstrate that the dynamics of internally generated HVC neural activity are predictive of the learned temporal-sequential structure of produced song and that the strength of this prediction is modulated by uncertainty. C1 [Bouchard, Kristofer E.] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. [Brainard, Michael S.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94158 USA. [Brainard, Michael S.] Univ Calif San Francisco, Ctr Integrat Neurosci, San Francisco, CA 94158 USA. [Brainard, Michael S.] Univ Calif San Francisco, Howard Hughes Med Inst, San Francisco, CA 94158 USA. RP Bouchard, KE (reprint author), Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. EM kebouchard@lbl.gov FU Howard Hughes Medical Institute, National Institutes of Health [DC006636]; National Science Foundation [IOS0951348] FX This work was supported by the Howard Hughes Medical Institute, National Institutes of Health Grant DC006636 (to M.S.B.), National Science Foundation Grant IOS0951348 (to M.S.B.), and a National Science Foundation predoctoral award (to K.E.B.). NR 50 TC 0 Z9 0 U1 8 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 23 PY 2016 VL 113 IS 34 BP 9641 EP 9646 DI 10.1073/pnas.1606725113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9ZK UT WOS:000381860800069 PM 27506786 ER PT J AU Walti, MA Ravotti, F Arai, H Glabe, CG Wall, JS Bockmann, A Guntert, P Meier, BH Riek, R AF Walti, Marielle Aulikki Ravotti, Francesco Arai, Hiromi Glabe, Charles G. Wall, Joseph S. Bockmann, Anja Guentert, Peter Meier, Beat H. Riek, Roland TI Atomic-resolution structure of a disease-relevant A beta(1-42) amyloid fibril SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE amyloid; solid-state NMR; Alzheimer's disease; protein structure ID NUCLEAR-MAGNETIC-RESONANCE; SOLID-STATE NMR; PROTEIN SECONDARY STRUCTURE; CHEMICAL-SHIFT INDEX; X-RAY-DIFFRACTION; ALZHEIMERS-DISEASE; A-BETA; EXPERIMENTAL CONSTRAINTS; 3-DIMENSIONAL STRUCTURE; MONOCLONAL-ANTIBODIES AB Amyloid-beta (A beta) is present in humans as a 39-to 42-amino acid residue metabolic product of the amyloid precursor protein. Although the two predominant forms, A beta(1-40) and A beta(1-42), differ in only two residues, they display different biophysical, biological, and clinical behavior. A beta(1-42) is the more neurotoxic species, aggre-gatesmuch faster, and dominates in senile plaque of Alzheimer's disease (AD) patients. Although small A beta oligomers are believed to be the neurotoxic species, A beta amyloid fibrils are, because of their presence in plaques, a pathological hallmark of AD and appear to play an important role in disease progression through cell-to-cell transmissibility. Here, we solved the 3D structure of a diseaserelevant A beta(1-42) fibril polymorph, combining data from solid-state NMR spectroscopy and mass-per-length measurements from EM. The 3D structure is composed of two molecules per fibril layer, with residues 15-42 forming a double-horseshoe-like cross-beta-sheet entity with maximally buried hydrophobic side chains. Residues 1-14 are partially ordered and in a beta-strand conformation, but do not display unambiguous distance restraints to the remainder of the core structure. C1 [Walti, Marielle Aulikki; Ravotti, Francesco; Guentert, Peter; Meier, Beat H.; Riek, Roland] ETH, Phys Chem Lab, CH-8093 Zurich, Switzerland. [Arai, Hiromi; Glabe, Charles G.] Univ Calif Irvine, Dept Mol Biol & Biochem, Irvine, CA 92697 USA. [Glabe, Charles G.] King Abdulaziz Univ, Fac Sci, Dept Biochem, Jeddah 21589, Saudi Arabia. [Glabe, Charles G.] King Abdulaziz Univ, Expt Biochem Unit, King Fahd Med Res Ctr, Jeddah 21589, Saudi Arabia. [Wall, Joseph S.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Bockmann, Anja] Univ Lyon, UMR CNRS 5086, Labex Ecofect, Inst Biol & Chim Prot,Bases Mol & Struct Syst Inf, F-69007 Lyon, France. [Guentert, Peter] Goethe Univ Frankfurt, Ctr Biomol Magnet Resonance, Inst Biophys Chem, D-60438 Frankfurt, Germany. [Guentert, Peter] Tokyo Metropolitan Univ, Grad Sch Sci & Engn, Dept Chem, Hachioji, Tokyo 1920397, Japan. RP Meier, BH; Riek, R (reprint author), ETH, Phys Chem Lab, CH-8093 Zurich, Switzerland.; Bockmann, A (reprint author), Univ Lyon, UMR CNRS 5086, Labex Ecofect, Inst Biol & Chim Prot,Bases Mol & Struct Syst Inf, F-69007 Lyon, France. EM a.bockmann@ibcp.fr; beme@ethz.ch; roland.riek@phys.chem.ethz.ch RI Meier, Beat/K-4066-2016; Guntert, Peter/L-5577-2013; Fachbereich14, Dekanat/C-8553-2015; Faculty of, Sciences, KAU/E-7305-2017 OI Meier, Beat/0000-0002-9107-4464; Guntert, Peter/0000-0002-2911-7574; FU Swiss National Science Foundation [200020_159707, 200020_146757]; French Agence Nationale de la Recherche [ANR-11-BSV8-021-01, ANR-11-BSV8-0013-01, ANR-14-CE09-0024B] FX We thank Beth Y. Lin (Brookhaven National Laboratory) for the STEM measurements; Frank Delaglio for support with NMRPipe; and Peter Tittmann (Scientific Center for Optical and Electron Microscopy of ETH) for support with electron microscopy. This work was supported by Swiss National Science Foundation Grants 200020_159707 and 200020_146757; and by French Agence Nationale de la Recherche Grants ANR-11-BSV8-021-01, 0013-01, and ANR-14-CE09-0024B. NR 65 TC 26 Z9 26 U1 32 U2 45 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 23 PY 2016 VL 113 IS 34 BP E4976 EP E4984 DI 10.1073/pnas.1600749113 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9ZK UT WOS:000381860800009 PM 27469165 ER PT J AU Chen, JY Liu, L Cao, CL Li, MJ Tan, KM Yang, XH Yun, CH AF Chen, Ji-Yun Liu, Liang Cao, Chun-Ling Li, Mei-Jun Tan, Kemin Yang, Xiaohan Yun, Cai-Hong TI Structure and function of human Naa60 (NatF), a Golgi-localized bi-functional acetyltransferase SO SCIENTIFIC REPORTS LA English DT Article ID N-TERMINAL ACETYLATION; HISTONE ACETYLTRANSFERASE; MOLECULAR-BASIS; CELLULAR-PROTEINS; AMPHIPATHIC HELIX; MEMBRANE; COMPLEX; ENZYMES; DOMAIN; ACTIVATION AB N-terminal acetylation (Nt-acetylation), carried out by N-terminal acetyltransferases (NATs), is a conserved and primary modification of nascent peptide chains. Naa60 (also named NatF) is a recently identified NAT found only in multicellular eukaryotes. This protein was shown to locate on the Golgi apparatus and mainly catalyze the Nt-acetylation of transmembrane proteins, and it also harbors lysine Ne-acetyltransferase (KAT) activity to catalyze the acetylation of lysine e-amine. Here, we report the crystal structures of human Naa60 (hNaa60) in complex with Acetyl-Coenzyme A (Ac-CoA) or Coenzyme A (CoA). The hNaa60 protein contains an amphipathic helix following its GNAT domain that may contribute to Golgi localization of hNaa60, and the beta 7-beta 8 hairpin adopted different conformations in the hNaa60(1-242) and hNaa60(1-199) crystal structures. Remarkably, we found that the side-chain of Phe 34 can influence the position of the coenzyme, indicating a new regulatory mechanism involving enzyme, co-factor and substrates interactions. Moreover, structural comparison and biochemical studies indicated that Tyr 97 and His 138 are key residues for catalytic reaction and that a non-conserved beta 3-beta 4 long loop participates in the regulation of hNaa60 activity. C1 [Chen, Ji-Yun; Liu, Liang; Cao, Chun-Ling; Li, Mei-Jun; Yun, Cai-Hong] Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Dept Biophys, Beijing 100191, Peoples R China. [Chen, Ji-Yun; Liu, Liang; Cao, Chun-Ling; Yun, Cai-Hong] Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Inst Syst Biomed, Beijing 100191, Peoples R China. [Chen, Ji-Yun; Liu, Liang; Cao, Chun-Ling; Yun, Cai-Hong] Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Beijing Key Lab Tumor Syst Biol, Beijing 100191, Peoples R China. [Tan, Kemin] Argonne Natl Lab, Biosci, Struct Biol Ctr, 9700 S Cass Ave, Argonne, IL 60439 USA. [Yang, Xiaohan] Peking Univ, Hlth Sci Ctr, Dept Biochem & Mol Biol, Key Lab Carcinogenesis & Translat Res,Minist Educ, Beijing 100191, Peoples R China. RP Yun, CH (reprint author), Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Dept Biophys, Beijing 100191, Peoples R China.; Yun, CH (reprint author), Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Inst Syst Biomed, Beijing 100191, Peoples R China.; Yun, CH (reprint author), Peking Univ, Hlth Sci Ctr, Sch Basic Med Sci, Beijing Key Lab Tumor Syst Biol, Beijing 100191, Peoples R China. EM yunch@hsc.pku.edu.cn FU National Basic Research Program of China (973 Program) [2012CB917202]; National Science Foundation of China [31270769]; Ministry of Science and Technology of China [NCET-12-0013]; U. S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX We thank the National Basic Research Program of China (973 Program, No. 2012CB917202), the National Science Foundation of China (No. 31270769), and the Ministry of Science and Technology of China (NCET-12-0013) for supporting this research. The use of Structural Biology Center 19-ID beamline at the Advanced Photon Source at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Biological and Environmental Research, under contract DE-AC02-06CH11357. NR 38 TC 0 Z9 0 U1 8 U2 8 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 23 PY 2016 VL 6 AR 31425 DI 10.1038/srep31425 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT8MK UT WOS:000381744600001 PM 27550639 ER PT J AU Fancher, CM Han, Z Levin, I Page, K Reich, BJ Smith, RC Wilson, AG Jones, JL AF Fancher, Chris M. Han, Zhen Levin, Igor Page, Katharine Reich, Brian J. Smith, Ralph C. Wilson, Alyson G. Jones, Jacob L. TI Use of Bayesian Inference in Crystallographic Structure Refinement via Full Diffraction Profile Analysis SO SCIENTIFIC REPORTS LA English DT Article ID CRYSTAL-STRUCTURE DETERMINATION; POWDER-DIFFRACTION; GENETIC ALGORITHM; STATISTICS AB A Bayesian inference method for refining crystallographic structures is presented. The distribution of model parameters is stochastically sampled using Markov chain Monte Carlo. Posterior probability distributions are constructed for all model parameters to properly quantify uncertainty by appropriately modeling the heteroskedasticity and correlation of the error structure. The proposed method is demonstrated by analyzing a National Institute of Standards and Technology silicon standard reference material. The results obtained by Bayesian inference are compared with those determined by Rietveld refinement. Posterior probability distributions of model parameters provide both estimates and uncertainties. The new method better estimates the true uncertainties in the model as compared to the Rietveld method. C1 [Fancher, Chris M.; Jones, Jacob L.] North Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. [Han, Zhen; Reich, Brian J.; Wilson, Alyson G.] North Carolina State Univ, Dept Stat, Raleigh, NC 27695 USA. [Levin, Igor] NIST, Mat Measurement Sci Div, Gaithersburg, MD 20899 USA. [Page, Katharine] Oak Ridge Natl Lab, Neutron Scattering Sci Directorate, Oak Ridge, TN 37831 USA. [Smith, Ralph C.] North Carolina State Univ, Dept Math, Raleigh, NC 27695 USA. RP Jones, JL (reprint author), North Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. EM jacob_jones@ncsu.edu RI Page, Katharine/C-9726-2009; Fancher, Chris/F-1293-2017; OI Page, Katharine/0000-0002-9071-3383; Fancher, Chris/0000-0002-3952-5168; Wilson, Alyson/0000-0003-1461-6212 FU Kenan Institute for Engineering, Technology and Science at NC State; Eastman Chemical Company - University Engagement Fund at NC State; National Science Foundation [DMR-1445926]; DOE Office of Science [DE-AC02-06CH11357] FX The authors acknowledge the support of the Kenan Institute for Engineering, Technology and Science at NC State and the Eastman Chemical Company - University Engagement Fund at NC State. JLJ acknowledges support from the National Science Foundation under DMR-1445926. This research used resources of the Advanced Photon Source, a US. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 38 TC 1 Z9 1 U1 5 U2 6 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 23 PY 2016 VL 6 AR 31625 DI 10.1038/srep31625 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT8NA UT WOS:000381746300001 PM 27550221 ER PT J AU Ji, J Colosimo, AM Anwand, W Boatner, LA Wagner, A Stepanov, PS Trinh, TT Liedke, MO Krause-Rehberg, R Cowan, TE Selim, FA AF Ji, J. Colosimo, A. M. Anwand, W. Boatner, L. A. Wagner, A. Stepanov, P. S. Trinh, T. T. Liedke, M. O. Krause-Rehberg, R. Cowan, T. E. Selim, F. A. TI ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy SO SCIENTIFIC REPORTS LA English DT Article ID ALPHA-PARTICLE DETECTORS; SINGLE-CRYSTALS; NANOSTRUCTURES; PERFORMANCE; DEFECTS; FILMS; GIPS AB The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials. C1 [Ji, J.; Colosimo, A. M.; Selim, F. A.] Bowling Green State Univ, Dept Phys & Astron, Bowling Green, OH 43403 USA. [Anwand, W.; Wagner, A.; Trinh, T. T.; Liedke, M. O.; Cowan, T. E.] Helmholtz Zentrum Dresden Rossendorf, Inst Radiat Phys, Bautzner Landstr 400, D-01328 Dresden, Germany. [Boatner, L. A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Stepanov, P. S.; Selim, F. A.] Bowling Green State Univ, Ctr Photochem Sci, Bowling Green, OH 43403 USA. [Trinh, T. T.; Cowan, T. E.] Tech Univ Dresden, D-01062 Dresden, Germany. [Krause-Rehberg, R.] Univ Halle Wittenberg, Dept Phys, D-06099 Halle, Germany. RP Selim, FA (reprint author), Bowling Green State Univ, Dept Phys & Astron, Bowling Green, OH 43403 USA.; Selim, FA (reprint author), Bowling Green State Univ, Ctr Photochem Sci, Bowling Green, OH 43403 USA. EM faselim@bgsu.edu RI Selim, Farida/N-8077-2016; Wagner, Andreas/G-3127-2013; Liedke, Maciej/R-3993-2016; Cowan, Thomas/A-8713-2011 OI Wagner, Andreas/0000-0001-7575-3961; Cowan, Thomas/0000-0002-5845-000X FU National Science Foundation [DMR1359523]; US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX The authors would like to thank M. Butterling for his contribution to GIPS setup and measurements. Funding for this work was provided by the National Science Foundation (DMR1359523 grant). Research at the Oak Ridge National Laboratory for one author (LAB) was sponsored by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 43 TC 2 Z9 2 U1 11 U2 18 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 23 PY 2016 VL 6 AR 31238 DI 10.1038/srep31238 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT8TE UT WOS:000381766600001 PM 27550235 ER PT J AU Lee, KS Spendelow, JS Choe, YK Fujimoto, C Kim, YS AF Lee, Kwan-Soo Spendelow, Jacob S. Choe, Yoong-Kee Fujimoto, Cy Kim, Yu Seung TI An operationally flexible fuel cell based on quaternary ammonium-biphosphate ion pairs SO NATURE ENERGY LA English DT Article ID POLYMER ELECTROLYTE; MEMBRANES; POLYAROMATICS; STABILITY; MODE; ACID AB Fuel cells are promising devices for clean power generation in a variety of economically and environmentally significant applications. Low-temperature proton exchange membrane (PEM) fuel cells utilizing Nafion require a high level of hydration, which limits the operating temperature to less than 100 degrees C. In contrast, high-temperature PEM fuel cells utilizing phosphoric acid-doped polybenzimidazole can operate effectively up to 180 degrees C;however, these devices degrade when exposed to water below 140 degrees C. Here we present a different class of PEM fuel cells based on quaternary ammonium-biphosphate ion pairs that can operate under conditions unattainable with existing fuel cell technologies. These fuel cells exhibit stable performance at 80-160 degrees C with a conductivity decay rate more than three orders of magnitude lower than that of a commercial hightemperature PEM fuel cell. By increasing the operational flexibility, this class of fuel cell can simplify the requirements for heat and water management, and potentially reduce the costs associated with the existing fully functional fuel cell systems. C1 [Lee, Kwan-Soo; Spendelow, Jacob S.; Kim, Yu Seung] Los Alamos Natl Lab, MPA Mat Synth & Integrated Devices 11, Los Alamos, NM 87545 USA. [Choe, Yoong-Kee] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. [Fujimoto, Cy] Sandia Natl Labs, Organ Mat Sci, Albuquerque, NM 87185 USA. [Lee, Kwan-Soo] Los Alamos Natl Lab, C CDE Chem Diagnost & Engn, Los Alamos, NM 87545 USA. RP Kim, YS (reprint author), Los Alamos Natl Lab, MPA Mat Synth & Integrated Devices 11, Los Alamos, NM 87545 USA. EM yskim@lanl.gov FU US Department of Energy, Energy Efficiency and Renewable Energy, Fuel Cell Technology Office; Ministry of Economy, Trade and Industry of Japan through the Japan-US Cooperation on Clean Energy Technology Program; Los Alamos National Security, LLC [DE-AC52-06NA25396]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the US Department of Energy, Energy Efficiency and Renewable Energy, Fuel Cell Technology Office. We thank E.S. De Castro for useful discussion and for supplying PBI samples. We also thank C. Kreller for helping with the polymer thermal analysis. Y.-K.C. acknowledges financial support from the Ministry of Economy, Trade and Industry of Japan through the Japan-US Cooperation on Clean Energy Technology Program. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC under Contract DE-AC52-06NA25396. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 22 TC 5 Z9 5 U1 4 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2058-7546 J9 NAT ENERGY JI Nat. Energy PD AUG 22 PY 2016 VL 1 AR 16120 DI 10.1038/NENERGY.2016.120 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary SC Energy & Fuels; Materials Science GA EK8ON UT WOS:000394183400001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Konig, A Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S De Wolf, EA Janssen, X Lauwers, J Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Lowette, S Moortgat, S Moreels, L Olbrechts, A Python, Q Tavernier, S Van Doninck, W Van Mulders, P Van Parijs, I Brun, H Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Luetic, J Maerschalk, T Marinov, A Randle-conde, A Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Cimmino, A Cornelis, T Dobur, D Fagot, A Garcia, G Gul, M Poyraz, D Salva, S Schofbeck, R Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L De Visscher, S Delaere, C Delcourt, M Forthomme, L Francois, B Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Magitteri, A Mertens, A Musich, M Nuttens, C Piotrzkowski, K Quertenmont, L Selvaggi, M Marono, MV Wertz, S Beliy, N Alda, WL Alves, FL Alves, GA Brito, L Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Da Silveira, GG Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Fang, W Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Chen, Y Cheng, T Jiang, CH Leggat, D Liu, Z Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Zhao, J Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Hernandez, CFG Alvarez, JDR Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Ferencek, D Kadija, K Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Jarrin, EC Abdelalim, AA El-khateeb, E Mahmoud, MA Radi, A Calpas, B Kadastik, M Murumaa, M Perrini, L Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Peltola, T Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Ghosh, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Kucher, I Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Abdulsalam, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Davignon, O de Cassagnac, RG Jo, M Lisniak, S Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Grenier, G 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Dolinska, G Eckerlin, G Eckstein, D Gallo, E Garcia, JG Geiser, A Gizhko, A Luyando, JMG Gunnellini, P Harb, A Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Keaveney, J Kieseler, J Kleinwort, C Korol, I Lange, W Lelek, A Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Ntomari, E Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Seitz, C Spannagel, S Stefaniuk, N Trippkewitz, KD Van Onsem, GP Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Dreyer, T Garutti, E Goebel, K Gonzalez, D Haller, J Hoffmann, M Junkes, A Klanner, R Kogler, R Kovalchuk, N Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Niedziela, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Poehlsen, J Sander, C Scharf, C Schleper, P Schmidt, A Schumann, S Schwandt, J Stadie, H Steinbruck, G Stober, FM Stover, M Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Vormwald, B 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CA CMS Collaboration TI Search for supersymmetry in pp collisions at root s=13 TeV in the single-lepton final state using the sum of masses of large-radius jets SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments); Supersymmetry ID GRAND UNIFIED THEORIES; SUPERGAUGE TRANSFORMATIONS; GLUINO PRODUCTION; NATURALNESS; MODEL; PREDICTIONS; UNIFICATION; EXTENSION; INVARIANT; NEUTRINO AB Results are reported from a search for supersymmetric particles in protonproton collisions in the final state with a single, high transverse momentum lepton; multiple jets, including at least one b-tagged jet; and large missing transverse momentum. The data sample corresponds to an integrated luminosity of 2: 3 fb(-1) at root s = 13TeV, recorded by the CMS experiment at the LHC. The search focuses on processes leading to high jet multiplicities, such as gluino pair production with (g) over tilde -> t (t) over bar(chi) over tilde (0)(1) . The quantity M-J, defined as the sum of the masses of the large-radius jets in the event, is used in conjunction with other kinematic variables to provide discrimination between signal and background and as a key part of the background estimation method. The observed event yields in the signal regions in data are consistent with those expected for standard model backgrounds, estimated from control regions in data. Exclusion limits are obtained for a simplified model corresponding to gluino pair production with three-body decays into top quarks and neutralinos. Gluinos with a mass below 1600 GeV are excluded at a 95% confidence level for scenarios with low (chi) over tilde (0)(1) mass, and neutralinos with a mass below 800 GeV are excluded for a gluino mass of about 1300 GeV. For models with two-body gluino decays producing on-shell top squarks, the excluded region is only weakly sensitive to the top squark mass. C1 [Khachatryan, V.; Sirunyan, A. 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A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Nardo, G.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [De Nardo, G.; Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Napoli Federico II, Naples, Italy. [Cavallo, N.; De Nardo, G.; Fabozzi, F.; Thyssen, F.] Univ Basilicata, Potenza, Italy. [De Nardo, G.; Di Guida, S.; Meola, S.; Thyssen, F.] Univ G Marconi, Rome, Italy. [Azzi, P.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Manzano, P. De Castro; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gonella, F.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Simonetto, F.; Torassa, E.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Zanetti, M.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Fedi, G.; Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Fedi, G.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Cipriani, M.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Cipriani, M.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bartosik, N.; Bellan, R.; Biino, C.; Cartiglia, N.; Cenna, F.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Shchelina, K.; Sola, V.; Solano, A.; Staiano, A.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Cenna, F.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Shchelina, K.; Solano, A.; Traczyk, P.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; La Licata, C.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Della Ricca, G.; La Licata, C.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Lee, S.; Lee, S. W.; Oh, Y. D.; Sekmen, S.; Son, D. C.; Yang, Y. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, H.; Lee, A.] Chonbuk Natl Univ, Jeonju, South Korea. [Cifuentes, J. A. Brochero; Kim, T. J.] Hanyang Univ, Seoul, South Korea. [Lee, S.; Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Ha, S.; Hong, B.; Jo, Y.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Almond, J.; Kim, J.; Oh, S. B.; Yang, U. K.; Yoo, H. D.; Yu, G. B.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Hwang, C.; Kim, D.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-De la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Oropeza Barrera, C.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.; Uribe Estrada, C.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Shah, M. A.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nemallapudi, M. V.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fisica Expt Particulas, Lisbon, Portugal. [Abdulsalam, A.; Khvedelidze, A.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Voytishin, N.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Chtchipounov, L.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Murzin, V.; Oreshkin, V.; Sulimov, V.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Matveev, V.; Chadeeva, M.; Danilov, M.; Markin, O.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Chadeeva, M.; Danilov, M.; Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Terkulov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Abdulsalam, A.; Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Elumakhov, D.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Romero, A.; Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Soares, M. S.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Gonzalez Caballero, I.; Gonzalez Fernandez, J. R.; Palencia Cortezon, E.; Sanchez Cruz, S.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Hartmann, F.; Mohanty, A. K.; Silvestris, L.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Pazzini, J.; Azzurri, P.; D'imperio, G.; Del Re, D.; Arcidiacono, R.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Fartoukh, S.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Girone, M.; Glege, F.; Gulhan, D.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Knuenz, V.; Kornmayer, A.; Kortelainen, M. J.; Kousouris, K.; Krammer, M.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Malgeri, L.; Mannelli, M.; Martelli, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Sauvan, J. B.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stoye, M.; Takahashi, Y.; Tosi, M.; Treille, D.; Triossi, A.; Tsirou, A.; Veckalns, V.; Veres, G. I.; Wardle, N.; Zagozdzinska, A.; Zeuner, W. D.; Virdee, T.] European Org Nucl Res, CERN, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Candelise, V.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Paganis, E.; Psallidas, A.; Tsai, J. f.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Kara, O.; Topaksu, A. Kayis; Kiminsu, U.; Oglakci, M.; Onengut, G.; Ozdemir, K.; Cerci, D. Sunar; Topakli, H.; Turkcapar, S.; Zorbakir, I. S.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Haddad, Y.; Hall, G.; Iles, G.; Lane, R.; Laner, C.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mastrolorenzo, L.; Nash, J.; Nikitenko, A.; Pela, J.; Penning, B.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Benelli, G.; Berry, E.; Cutts, D.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Spencer, E.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Burns, D.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Flores, C.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Paneva, M. I.; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Derdzinski, M.; Gerosa, R.; Holzner, A.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wood, J.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bhandari, R.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Heller, R.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Ovcharova, A.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Chen, Y.; Dubinin, M.; Anderson, D.; Apresyan, A.; Bendavid, J.; Bornheim, A.; Bunn, J.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.; Sun, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chaves, J.; Chu, J.; Dittmer, S.; Mcdermott, K.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Tan, S. M.; Tao, Z.; Thom, J.; Tucker, J.; Wittich, P.; Zientek, M.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cremonesi, M.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Magini, N.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holme, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Ristori, L.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Tavernier, S.; Kuznetsova, E.; Acosta, D.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Shchutska, L.; Sperka, D.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Martini, L.; Linn, S.; Markowitz, P.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adam, W.; Ackert, A.; Adams, J. R.; Askew, A.; Bein, S.; Diamond, B.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Santra, A.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Al-Bataineh, A.; Baringer, P.; Bean, A.; Bowen, J.; Bruner, C.; Castle, J.; Kenny, R. P.; Kropivnitskaya, A.; Majumder, D.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Takaki, J. D. Tapia; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Abercrombie, D.; Allen, B.; Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Hsu, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Chatterjee, R. M.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Rodrigues, A. Malta; Meier, F.; Monroy, J.; Siado, J. E.; Snow, G. R.; Stieger, B.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Parker, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M. H.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Anampa, K. Hurtado; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Alimena, J.; Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Francis, B.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Liu, B.; Luo, W.; Puigh, D.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Cooperstein, S.; Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Luo, J.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Folgueras, S.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Tan, S. M.; Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Duh, Y. T.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Gershtein, Y.; Espinosa, T. A. Gomez; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Kyriacou, S.; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Heideman, J.; Riley, G.; Rose, K.; Spanier, S.; Thapa, K.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Juska, E.; Kamon, T.; Krutelyov, V.; Mueller, R.; Pakhotin, Y.; Patel, R.; Perloff, A.; Pernie, L.; Rathjens, D.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Wang, Z.; Lee, S. W.; Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Barria, P.; Cox, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Schieck, J.; Wulz, C. -E.; Krammer, M.] Vienna Univ Technol, Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Chen, Y.] DESY, Hamburg, Germany. [Abdelalim, A. A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [El-khateeb, E.; Radi, A.] Ain Shams Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahmoud, M. A.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Nayak, A.] Inst Phys, Bhubaneswar, Orissa, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Chenarani, S.; Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. [Heredia-De la Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Orfanelli, S.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Veckalns, V.] Riga Tech Univ, Riga, Latvia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RI Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Konecki, Marcin/G-4164-2015; Puljak, Ivica/D-8917-2017; Lokhtin, Igor/D-7004-2012; TUVE', Cristina/P-3933-2015; Goh, Junghwan/Q-3720-2016 OI Della Ricca, Giuseppe/0000-0003-2831-6982; Konecki, Marcin/0000-0001-9482-4841; TUVE', Cristina/0000-0003-0739-3153; Goh, Junghwan/0000-0002-1129-2083 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican Funding Agency (BUAP); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (LNS); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretar a de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Mobility Plus program of the Ministry of Science and Higher Education (Poland); OPUS program of the National Science Center (Poland); Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Programa Clarin-COFUND del Principado de Asturias; Rachadapisek Sompot Fund for Postdoctoral Fellowship; Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (BUAP, CINVESTAV, CONACYT, LNS, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretar a de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Mobility Plus program of the Ministry of Science and Higher Education (Poland); the OPUS program of the National Science Center (Poland); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Programa Clarin-COFUND del Principado de Asturias; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 82 TC 1 Z9 1 U1 12 U2 12 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 22 PY 2016 IS 8 AR 122 DI 10.1007/JHEP08(2016)122 PG 49 WC Physics, Particles & Fields SC Physics GA EH4SW UT WOS:000391761900001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moortgat, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Parijs, I Brun, H Caillol, C Clerbaux, B 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CA CMS Collaboration TI Measurement of the differential cross section and charge asymmetry for inclusive pp -> W-+/- + X production at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID 3-LOOP SPLITTING FUNCTIONS; PARTON DISTRIBUTIONS; LEADING ORDER; LHC; QCD; SCATTERING; DENSITIES; EVOLUTION AB The differential cross section and charge asymmetry for inclusive pp -> W-+/- + X -> mu(+/-)nu + X production at root s = 8 TeV are measured as a function of muon pseudorapidity. The data sample corresponds to an integrated luminosity of 18.8 fb(-1) recorded with the CMS detector at the LHC. These results provide important constraints on the parton distribution functions of the proton in the range of the Bjorken scaling variable x from 10(-3) to 10(-1). C1 [Khachatryan, V. y; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. 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S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Niedziela, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Sander, C.; Scharf, C.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schumann, S.; Schwandt, J.; Stadie, H.; Steinbrueck, G.; Stober, F. M.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Schroeder, M.; Sieber, G.; Simonis, H. J.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Filipovic, N.; Vesztergombi, G.; Bartok, M.; Veres, G. I.] Eotvos Lorand Univ, MTA ELTE Lendulet CMS Particle & Nucl Phys Grp, Budapest, Hungary. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Choudhury, S.; Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Keshri, S.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Bhattacharya, R.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Ghosh, S.; Majumdar, N.; Modak, A.; Mondal, K.; Mukhopadhyay, S.; Nandan, S.; Purohit, A.; Roy, A.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay, Maharashtra, India. [Ghosh, S.; Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Guchait, M.; Gurtu, A.; Jain, Sa.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Bombay, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Rane, A.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Ist Nazl Fis Nucl, Sez Bolognaa, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, Catania, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Catania Univ, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenzea, Florence, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Pigazzini, S.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Milan, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Pigazzini, S.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.; Margaroli, F.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisac, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Rome, Rome, Italy. [Costa, S.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bartosik, N.; Bellan, R.; Biino, C.; Cartiglia, N.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Zanetti, M.; Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Lee, S. W.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Lee, S.; Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Guisao, J. Mejia; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Montoya, C. A. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Ibarguen, H. A. Salazar; Estrada, C. Uribe] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Pineda, A. Morelos] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Qazi, S.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Traczyk, P.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Da Cruz E Silva, C. Beirao; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Iglesias, L. Lloret; Nemallapudi, M. V.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Mitsyn, V. V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Tikhonenko, E.; Voytishin, N.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Matveev, V.; Chadeeva, M.; Chistov, R.; Danilov, M.; Markin, O.; Tarkovskii, E.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Troconiz, J. F. de; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Stahl, A.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Azzurri, P.; D'imperio, G.; Del Re, D.; Arcidiacono, R.; Palencia Cortezon, E.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Knunz, V.; Kortelainen, M. J.; Kousouris, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Sauvan, J. B.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veckalns, V.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Virdee, T.] CERN, European Org Nucl Res, Geneva, Switzerland. [Kuznetsova, E.; Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Chicago, Chicago, IL 60637 USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Castle, J.; Kenny, R. P.; Kropivnitskaya, A.; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.; Stieger, B.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Parker, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M. H.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Rupprecht, N.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Michlin, W. Li B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Heideman, J.; Riley, G.; Spanier, S.; Thapa, K.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Pernie, L.; Rathjens, D.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.; Wang, Z.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Barria, P.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [C., Clarke; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Wulz, C. -E.] Vienna Univ Technol, Vienna, Austria. [Chinellato, J.; Manganote, E. J. Tonelli] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Abdelalim, A. A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [El-Khateeb, E.; Elkafrawy, T.] Ain Shams Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahmoud, M. A.] British Univ Egypt, Cairo, Egypt. [Conte, E.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Grippo, M. T.] Univ Siena, Siena, Italy. [Kim, T. J.] Hanyang Univ, Seoul, South Korea. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Di Marco, E.] Univ Rome, Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Veckalns, V.] Riga Tech Univ, Riga, Latvia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Onengut, G.] Cag Univ, Mersin, Turkey. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. f.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Haddad, Y.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mastrolorenzo, L.; Nash, J.; Nikitenko, A.; Pela, J.; Penning, B.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bendavid, J.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Della Ricca, Giuseppe/B-6826-2013; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Goh, Junghwan/Q-3720-2016; Kirakosyan, Martin/N-2701-2015; Lokhtin, Igor/D-7004-2012; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Chadeeva, Marina/C-8789-2016; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Manganote, Edmilson/K-8251-2013; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Danilov, Mikhail/C-5380-2014; Konecki, Marcin/G-4164-2015 OI Della Ricca, Giuseppe/0000-0003-2831-6982; TUVE', Cristina/0000-0003-0739-3153; Goh, Junghwan/0000-0002-1129-2083; Paulini, Manfred/0000-0002-6714-5787; Chadeeva, Marina/0000-0003-1814-1218; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; Danilov, Mikhail/0000-0001-9227-5164; Konecki, Marcin/0000-0001-9482-4841 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union; Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Chulalongkorn Academic into Its Second Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its Second Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 55 TC 0 Z9 0 U1 18 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 22 PY 2016 VL 76 IS 8 AR 469 DI 10.1140/epjc/s10052-016-4293-4 PG 27 WC Physics, Particles & Fields SC Physics GA DU3TM UT WOS:000382135100001 PM 28303084 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fang, W Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L De Visscher, S Delaere, C Delcourt, M Favart, D Forthomme, L Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Leggat, D Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Assran, Y Kamel, AE Mahrous, A Mohamed, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Peltola, T Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Abdulsalam, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Davignon, O Filipovic, N de Cassagnac, RG Jo, M Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sordini, V Vander Donckt, M Verdier, P Viret, S Toriashvili, T Tsamalaidze, Z Autermann, C Beranek, S Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Mukherjee, S Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Borras, K Burgmeier, A Campbell, A Contreras-Campana, C Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Seitz, C Spannagel, S Stefaniuk, N Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Kovalchuk, N Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Sander, C Scharf, C Schleper, P Schlieckau, E Schmidt, A Schumann, S Schwandt, J Sola, V Stadie, H Steinbruck, G Stober, FM Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Vormwald, B Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T Colombo, F De Boer, W Descroix, A Dierlamm, A Fink, S Frensch, F Friese, R Giffels, M Gilbert, A Haitz, D Hartmann, F Heindl, SM Husemann, U Katkov, I Kornmayer, A Pardo, PL Maier, B Mildner, H Mozer, MU Muller, T Muller, T Plagge, M Quast, G Rabbertz, K Rocker, S Roscher, F Schroder, M Sieber, G Simonis, HJ Ulrich, R Wagner-Kuhr, J Wayand, S Weber, M Weiler, T Williamson, S Wohrmann, C Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Psallidas, A Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Tziaferi, E Evangelou, I Flouris, G Foudas, C Kokkas, P Loukas, N Manthos, N Papadopoulos, I Paradas, E Strologas, J Bencze, G Hajdu, C Hazi, A Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Szillasi, Z Bartok, M Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Choudhury, S Mal, P Mandal, K Sahoo, DK Sahoo, N Swain, SK Bansal, S Beri, SB Bhatnagar, V Chawla, R Gupta, R Bhawandeep, U Kalsi, AK Kaur, A Kaur, M Kumar, R Mehta, A Mittal, M Singh, JB Walia, G Kumar, A Bhardwaj, A Choudhary, BC Garg, RB Malhotra, S Naimuddin, M Nishu, N Ranjan, K Sharma, R Sharma, V Bhattacharya, S Chatterjee, K Dey, S Dutta, S Majumdar, N Modak, A Mondal, K Mukhopadhyay, S Roy, A Roy, D Chowdhury, SR Sarkar, S Sharan, M Chudasama, R Dutta, D Jha, V Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Banerjee, S Bhowmik, S Chatterjee, RM Dewanjee, RK Dugad, S Ganguly, S Ghosh, S Guchait, M Gurtu, A Jain, S Kole, G Kumar, S Mahakud, B Maity, M Majumder, G Mazumdar, K Mitra, S Mohanty, GB Parida, B Sarkar, T Sur, N Sutar, B Wickramage, N Chauhan, S Dube, S Kapoor, A Kothekar, K Rane, A Sharma, S Bakhshiansohi, H Behnamian, H Etesami, SM Fahim, A Khakzad, M Najafabadi, MM Naseri, M Mehdiabadi, SP Hosseinabadi, FR Safarzadeh, B Zeinali, M Felcini, M Grunewald, M Abbrescia, M Calabria, C Caputo, C 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CA CMS Collaboration TI Evidence for exclusive gamma gamma -> W (+) W (-) production and constraints on anomalous quartic gauge couplings in pp collisions at and 8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Forward physics; Hadron-Hadron scattering (experiments) ID CROSS-SECTION; HADRON COLLIDERS; BOSON COUPLINGS; HIGH-ENERGIES; LHC; LIMITS; EVENT; LEP AB A search for exclusive or quasi-exclusive gamma gamma -> W (+) W (-) production, via pp -> p ((*)) W (+) W (-) p ((*)) -> p ((*)) mu (+/-)e(a") p ((*)) at TeV, is reported using data corresponding to an integrated luminosity of 19.7 fb(-1). Events are selected by requiring the presence of an electron-muon pair with large transverse momentum p (T)(mu (+/-)e(a")) > 30 GeV, and no associated charged particles detected from the same vertex. The 8 TeV results are combined with the previous 7 TeV results (obtained for 5.05 fb(-1) of data). In the signal region, 13 (2) events are observed over an expected background of 3.9 +/- 0.6 (0.84 +/- 0.15) events for 8 (7) TeV, resulting in a combined excess of 3.4 sigma over the background-only hypothesis. The observed yields and kinematic distributions are compatible with the standard model prediction for exclusive and quasi-exclusive gamma gamma -> W (+) W (-) production. Upper limits on the anomalous quartic gauge coupling operators a (0,C) (W) (dimension-6) and f (M0,1,2,3) (dimension-8), the most stringent to date, are derived from the measured dilepton transverse momentum spectrum. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Barria, P.; Brun, H.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Fang, W.; Fasanella, G.; Favart, L.; Goldouzian, R.; Grebenyuk, A.; Karapostoli, G.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Marinov, A.; Pernie, L.; Randle-Conde, A.; Seva, T.; Vander Velde, C.; Vanlaer, P.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Caudron, A.; Ceard, L.; De Visscher, S.; Delaere, C.; Delcourt, M.; Favart, D.; Forthomme, L.; Giammanco, A.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Musich, M.; Nuttens, C.; Perrini, L.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Vidal Marono, M.] Catholic Univ Louvain, Louvain, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, Mons, Belgium. [Alda Junior, W. L.; Alves, F. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Hamer, M.; Hensel, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mora Herrera, C.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.; Romero Abad, D.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Leggat, D.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Spiezia, A.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Ribeiro Cipriano, P. M.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Inst Rudjer Boskov, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Kamel, A. Ellithi; Mahrous, A.; Mohamed, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Peltola, T.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM, IRFU, Gif Sur Yvette, France. [Abdulsalam, A.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Davignon, O.; Filipovic, N.; de Cassagnac, R. Granier; Jo, M.; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, Lab Leprince Ringuet, IN2P3, CNRS, Palaiseau, France. [Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] Inst Natl Phys Nucleaire & Phys Particules, Ctr Calcul, CNRS, IN2P3, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Claude Bernard Lyon 1, Univ Lyon, Inst Phys Nucl Lyon, CNRS,IN2P3, Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Tsamalaidze, Z.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Mukherjee, S.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inat A3, Aachen, Germany. Rhein Westfal TH Aachen, Phys Inat B3, Aachen, Germany. [Abdulsalam, A.; Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Borras, K.; Burgmeier, A.; Campbell, A.; Contreras-Campana, C.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe; Saxena, P.; Schoerner-Sadenius, T.; Seitz, C.; Spannagel, S.; Stefaniuk, N.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Sander, C.; Scharf, C.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schumann, S.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Stober, F. M.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Schroeder, M.; Sieber, G.; Simonis, H. J.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Choudhury, S.; Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Majumdar, N.; Modak, A.; Mondal, K.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Jain, Sa.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Rane, A.; Sharma, S.] Indian Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, Catania, Italy. [Hartmann, F.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] INFN, Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN, Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Maron, G.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.] INFN, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN, Sez Pavia, Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] INFN, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Abdulsalam, A.; Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] INFN, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] INFN, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Torino, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] INFN, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estud Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Traczyk, P.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; KarjJavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Chadeeva, M.; Chistov, R.; Danilov, M.; Rusinov, V.; Tarkovskii, E.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Ershov, A.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Lukina, O.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.; Hos, I.; Kangal, E. E.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.; Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Abdulsalam, A.; Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Rupprecht, N.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barker, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Kumar, A.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY USA. [Ciesielski, R.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Chou, J. P.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; Thapa, K.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Rathjens, D.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Woods, N.] Univ Wisconsin Madison, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, Vienna, Austria. [Rabady, D.; Merlin, J. A.; Pantaleo, F.; Kornmayer, A.; Szillasi, Z.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Azzurri, P.; D'imperio, G.; Del Re, D.; Arcidiacono, R.] CERN, European Org Nucl Res, Geneva, Switzerland. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Popov, A.; Zhukov, V.; Katkov, I.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Plestina, R.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, Palaiseau, France. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Assran, Y.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahrous, A.] Helwan Univ, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Toriashvili, T.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Borras, K.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Maron, G.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Kim, T. J.] Hanyang Univ, Seoul, South Korea. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.] Inst Nucl Res, Moscow, Russia. [Matveev, V.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Di Marco, E.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Di Marco, E.] Univ Rome, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Veres, G. I.] Eotvos Lorand Univ, MTA ELTE Lendulet CMS Particle & Nucl Phys Grp, Budapest, Hungary. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. 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[Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Danilov, Mikhail/C-5380-2014; Kirakosyan, Martin/N-2701-2015; Della Ricca, Giuseppe/B-6826-2013; Puljak, Ivica/D-8917-2017; Goh, Junghwan/Q-3720-2016; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Andreev, Vladimir/M-8665-2015; Yazgan, Efe/C-4521-2014; Konecki, Marcin/G-4164-2015; Chistov, Ruslan/B-4893-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Chadeeva, Marina/C-8789-2016; Smirnov, Vitaly/B-5001-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015 OI Danilov, Mikhail/0000-0001-9227-5164; Della Ricca, Giuseppe/0000-0003-2831-6982; Goh, Junghwan/0000-0002-1129-2083; Yazgan, Efe/0000-0001-5732-7950; Konecki, Marcin/0000-0001-9482-4841; Chistov, Ruslan/0000-0003-1439-8390; Paulini, Manfred/0000-0002-6714-5787; Chadeeva, Marina/0000-0003-1814-1218; Ogul, Hasan/0000-0002-5121-2893; FU Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; Mobility Plus program of the Ministry of Science and Higher Education (Poland); OPUS program of the National Science Center (Poland); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Mobility Plus program of the Ministry of Science and Higher Education (Poland); the OPUS program of the National Science Center (Poland); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 67 TC 3 Z9 3 U1 18 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 22 PY 2016 IS 8 AR 119 DI 10.1007/JHEP08(2016)119 PG 47 WC Physics, Particles & Fields SC Physics GA DV1DV UT WOS:000382661100001 ER PT J AU Aaboud, M Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V 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Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena in final states with an energetic jet and large missing transverse momentum in pp collisions at root s=13 TeV using the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID DARK-MATTER SEARCHES; PARTON DISTRIBUTIONS; SUPERGAUGE TRANSFORMATIONS; P(P)OVER-BAR COLLISIONS; FIELD-THEORY; LHC; PARTICLE; SUPERSYMMETRY; MODEL; CONSTRAINTS AB Results of a search for new phenomena in final states with an energetic jet and large missing transverse momentum are reported. The search uses proton-proton collision data corresponding to an integrated luminosity of 3.2 fb(-1) at root s = 13 TeV collected in 2015 with the ATLAS detector at the Large Hadron Collider. Events are required to have at least one jet with a transverse momentum above 250 GeV and no leptons. Several signal regions are considered with increasing missing-transverse-momentum requirements between E-T(miss) > 250 GeV and E-T(miss) > 700 GeV. Good agreement is observed between the number of events in data and Standard Model predictions. The results are translated into exclusion limits in models with large extra spatial dimensions, pair production of weakly interacting dark-matter candidates, and the production of supersymmetric particles in several compressed scenarios. C1 [Jackson, P.; Lee, L.; Petridis, A.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Czodrowski, P.; Dassoulas, J.; Dehghanian, N.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Berger, N.; Delmastro, M.; Di Ciaccio, L.; Grevtsov, K.; Koletsou, I.; Lafaye, R.; Leveque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Smart, B. H.; Spalla, M.] CNRS IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Grevtsov, K.; Guillemin, T.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Smart, B. H.; Todorov, T.] Univ Savoie Mt Blanc, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; LeCompte, T.; Love, J.; Malon, D.; Metcalfe, J.; Nguyen, D. 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H.; Casadei, D.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Foster, A. G.; Gonella, L.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys Engn, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; D'amen, G.; De Castro, S.; Fabbri, F.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. 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Alvarez; Anders, G.; Anghinolfi, F.; Avolio, G.; Boveia, A.; Burckhart, H.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Feng, E. J.; Francis, D.; Froidevaux, D.; Gorini, B.; Gumper, C.; Helsens, C.; Correia, A. M. Henriques; Hoecker, A.; Krasznahorkay, A.; Lapoire, C.; Miotto, G. Lehmann; Lenzi, B.; MandeIli, B.; Manousos, A.; Marzin, A.; Mornacchi, G.; Nairz, A. M.; Oide, H.; Pernegger, H.; Petersen, B. A.; Poppleton, A.; Poulard, G.; Rembser, C.; Ritsch, E.; Salzburger, A.; Schaefer, D.; Sforza, F.; Sanchez, C. A. Solans; Spalla, M.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Liang, Z.; Merino, J. Llorente; Lou, X.; Mansour, J. D.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Suzhou, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Ma, Y.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, PKU CHEP, Shanghai, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donin, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donin, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donin, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. 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P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX USA. [Behr, J. K.; Bertsche, C.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Bravo, A. Gascon; Glazov, A.; Gregor, I. 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[Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Gossling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phy 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Sinaone, A.; Gonella, G.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Nagel, M.; Pagacova, M.; Parzefal, U.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Spalla, M.; Sundermann, J. E.; Ta, D.; Temming, K. K.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Lionti, A. E.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Sfyrla, A.; Spalla, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.; Spalla, M.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Spalla, M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; De Maria, A.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Quadt, A.; Rieger, J.; Rosien, N. -A.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Trocme, B.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Spalla, M.; Starovoitov, P.; Suchek, S.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; de Lima, D. E. Ferreira; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salyucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Clear Water Bay, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Oren, H.; Penwell, J.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Milic, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Spalla, M.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichey, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Spalla, M.] JINR Dubna, Join Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Beddall, A.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Spalla, M.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Fox, H.; Grimm, K.; Hughes, G.; Muenstermann, D.; Parker, A. J.; Smizanska, M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Reale, M.; Spagnolo, S.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Reale, M.; Spagnolo, S.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Gwilliam, C. B.; Hayward, H. S.; King, B. T.; Kretzschmar, J.; Lehan, A.; Mehta, A.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lewis, D.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mefayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Spalla, M.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjommark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; De la Torre, H.; Del Peso, J.; Glasman, C.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Erte, E.; Fiedler, F.; Torregrosa, E. Fullana; Geisen, M.; Groh, S.; Heck, T.; Hulsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Yildirim, E.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schweiger, H.; Shaw, S. M.; Spalla, M.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Lu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Lu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Le, B.; McDonald, E. F.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spitler, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Dieh, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Citterio, M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Camplani, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Ducu, O. A.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Mochizuki, K.; Manh, T. Nguyen; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavritenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Hartmann, N. M.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Losel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Schachtner, B. M.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; McCarthy, T. G.; Menke, S.; Mueller, F.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schmidt-Sommerfeld, K. R.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izz, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Bruni, L. S.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Spalla, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Bruni, L. S.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Saha, P.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshey, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Cantero, J.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Pogioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Spalla, M.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris Saclay, Univ Paris Sud, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Spalla, M.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Leychenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, Kurchatov Inst, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Beddall, A.; Canepa, A.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Spalla, M.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Beddall, A.; Caforio, D.; Canepa, A.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Spalla, M.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Spalla, M.; Starchenko, E. A.; Vaniachine, A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emetiyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; MeMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Spalla, M.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.; Spalla, M.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Beddall, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Spalla, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassie, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Pinto Firmino Da Costa, J. Goncalves; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Spalla, M.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, Comm Energie Atom & Energies Alternat, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schier, S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Armbruster, A. J.; Bawa, H. S.; Beddall, A.; Black, J. E.; Garelli, N.; Ilic, N.; Kagan, M.; Kocian, M.; Malone, C.; Moss, J.; Nachman, B. P.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Spalla, M.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Dado, T.; Melo, M.; Plazak, L.; Smiesko, J.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Spalla, M.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY USA. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Beddall, A.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Miano, F.; Salvatore, F.; Castillo, L. Santoyo; Shehu, C. Y.; Spalla, M.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Saavedra, A. F.; Scarcella, M.; Spalla, M.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Beddall, A.; Canepa, A.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Pilkington, A. D.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Spalla, M.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Beddall, A.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Spalla, M.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Hod, N.; Jovicevic, J.; Codina, E. Perez; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. 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A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Dumancic, M.; Gross, E.; Kohler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Ravinovich, I.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Spalla, M.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw.; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Spalla, M.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beddall, A.; Boerner, D.; Braun, H. 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[Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pasztor, G.] Eotvos Lorand Univ, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Song, H. Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPh1, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. [Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] CNRS IN2P3, Marseille, France. RP Aaboud, M (reprint author), Univ Mohamed Premier, Fac Sci, Oujda, Morocco.; Aaboud, M (reprint author), LPTPM, Oujda, Morocco. RI Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Mitsou, Vasiliki/D-1967-2009; Gutierrez, Phillip/C-1161-2011; White, Ryan/E-2979-2015; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Doyle, Anthony/C-5889-2009; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Mashinistov, Ruslan/M-8356-2015; Lazzaroni, Massimo/N-3675-2015; Gladilin, Leonid/B-5226-2011; Warburton, Andreas/N-8028-2013; Brooks, William/C-8636-2013; Camarri, Paolo/M-7979-2015; Tikhomirov, Vladimir/M-6194-2015; Prokoshin, Fedor/E-2795-2012; Mindur, Bartosz/A-2253-2017; Owen, Mark/Q-8268-2016; Livan, Michele/D-7531-2012; Ventura, Andrea/A-9544-2015 OI Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Mitsou, Vasiliki/0000-0002-1533-8886; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; White, Ryan/0000-0003-3589-5900; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Doyle, Anthony/0000-0001-6322-6195; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; Mashinistov, Ruslan/0000-0001-7925-4676; Lazzaroni, Massimo/0000-0002-4094-1273; Gladilin, Leonid/0000-0001-9422-8636; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Prokoshin, Fedor/0000-0001-6389-5399; Mindur, Bartosz/0000-0002-5511-2611; Owen, Mark/0000-0001-6820-0488; Livan, Michele/0000-0002-5877-0062; Ventura, Andrea/0000-0002-3368-3413 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT,Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales; Aristeia programmes; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT,Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council,CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 100 TC 5 Z9 5 U1 32 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 22 PY 2016 VL 94 IS 3 AR 032005 DI 10.1103/PhysRevD.94.032005 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KR UT WOS:000381893100001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF 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CA ATLAS Collaboration TI Measurements of the charge asymmetry in top-quark pair production in the dilepton final state at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; PARTON DISTRIBUTIONS; RESUMMATION; LHC AB Measurements of the top-antitop quark pair production charge asymmetry in the dilepton channel, characterized by two high-p(T) leptons (electrons or muons), are presented using data corresponding to an integrated luminosity of 20.3 fb(-1) from pp collisions at a center-of-mass energy root s = 8 TeV collected with the ATLAS detector at the Large Hadron Collider at CERN. Inclusive and differential measurements as a function of the invariant mass, transverse momentum, and longitudinal boost of the tt system arc performed both in the full phase space and in a fiducial phase space closely matching the detector acceptance. Two observables are studied: A(c)(ll) based on the selected leptons and A(c)(tt) based on the reconstructed tt final state. The inclusive asymmetries are measured in the full phase space to be A(c)(ll)= 0.008 +/- 0.006 and A(c)(tt)= 0.021 +/- 0.016, which are in agreement with the Standard Model predictions of A(c)(ll)= 0.0064 +/- 0.0003 and A(c)(tt)= 0.0111 +/- 0.0004. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Jabbar, S.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Starz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Dassoulas, J.; Facini, G.; Gardner, R. W.; Kapliy, A.; Karamaoun, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Hanh, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, L.; Zhang, H.] Nanjing Univ, Dept Phys, Beijing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, PKU CHEP, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Phys Dept, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Phys Dept, Dallas, TX USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Albert Ludwigs Univ, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. 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A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Georg August Univ, Phys Inst 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchluff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, k.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Ducu, O. A.; Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kergevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kergevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; DemiIly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; DemiIly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; DemiIly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, A.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Dolgoshein, B. A.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; CavaIli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepan Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPH, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Kiryunin, A. E.; Kortner, O.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamatichi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamatichi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Igonkina, O.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] Northern Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nernethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris Saclay, Univ Paris Sud, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Leychenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, E-18071 Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, E-18071 Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Czech Tech Univ, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst Pr High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagilaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagilaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Farilla, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Goujdami, D.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Firmino Da Costa, J. Goncalves Pinto; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivemyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, DSM, IRFU, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Siolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Siolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jenssen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Riissenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Riissenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawanaoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawanaoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambience, Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Amadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Ides Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Ides Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Ides Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Ides Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Ides Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Kohler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kuechler, J. T.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Vogel, M.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachgrp Phys, Fak Math & Nat Wissensch, Wuppertal, Germany. [Baker, O. K.; Noccioli, E. Benhar; Cummings, J.; Demers, S.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Vasquez, J. G.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.; Oakham, F. G.] Azerbaijan Acad Sci, Inst Phys, Baku, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] Novosibirsk State Univ, Novosibirsk, Russia. Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, Barcelona, Spain. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, London, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Geng, C.; Guo, Y.; Li, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Govender, N.] Ctr High Performance Comp, Rosebank, CSIR Campus, Cape Town, South Africa. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Hanagaki, k.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. Acad Sinica, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Lin, S. C.; Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Moscow, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pasztor, G.] Eotvos Lorand Univ, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ South Carolina, Dept Phys & Astron, Columbia, SC USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Song, H. Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Mitsou, Vasiliki/D-1967-2009; Carvalho, Joao/M-4060-2013; Gutierrez, Phillip/C-1161-2011; White, Ryan/E-2979-2015; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Zhukov, Konstantin/M-6027-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Doyle, Anthony/C-5889-2009; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Lazzaroni, Massimo/N-3675-2015; Ventura, Andrea/A-9544-2015; Gladilin, Leonid/B-5226-2011; Warburton, Andreas/N-8028-2013; Mashinistov, Ruslan/M-8356-2015; Brooks, William/C-8636-2013; Camarri, Paolo/M-7979-2015; Tikhomirov, Vladimir/M-6194-2015; Prokoshin, Fedor/E-2795-2012; Mindur, Bartosz/A-2253-2017; Owen, Mark/Q-8268-2016; Livan, Michele/D-7531-2012 OI Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Mitsou, Vasiliki/0000-0002-1533-8886; Carvalho, Joao/0000-0002-3015-7821; Pina, Joao /0000-0001-8959-5044; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; White, Ryan/0000-0003-3589-5900; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Doyle, Anthony/0000-0001-6322-6195; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; Lazzaroni, Massimo/0000-0002-4094-1273; Ventura, Andrea/0000-0002-3368-3413; Gladilin, Leonid/0000-0001-9422-8636; Warburton, Andreas/0000-0002-2298-7315; Mashinistov, Ruslan/0000-0001-7925-4676; Brooks, William/0000-0001-6161-3570; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Prokoshin, Fedor/0000-0001-6389-5399; Mindur, Bartosz/0000-0002-5511-2611; Owen, Mark/0000-0001-6820-0488; Livan, Michele/0000-0002-5877-0062 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSIVI/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales; Aristeia programmes; EU-ESF; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSIVI/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America, In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom, The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN, the ATLAS Tier-I facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA), the Tier-2 facilities worldwide and large non-WLCG resource providers, Major contributors of computing resources are listed in Ref. [78]. NR 77 TC 0 Z9 0 U1 31 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 22 PY 2016 VL 94 IS 3 AR 032006 DI 10.1103/PhysRevD.94.032006 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KR UT WOS:000381893100002 ER PT J AU Adriani, O Berti, E Bonechi, L Bongi, M D'Alessandro, R Del Prete, M Haguenauer, M Itow, Y Iwata, T Kasahara, K Kawade, K Makino, Y Masuda, K Matsubayashi, E Menjo, H Mitsuka, G Muraki, Y Papini, P Perrot, AL Ricciarini, S Sako, T Sakurai, N Suzuki, T Tamura, T Tiberio, A Torii, S Tricomi, A Turner, WC Ueno, M Zhou, QD AF Adriani, O. Berti, E. Bonechi, L. Bongi, M. D'Alessandro, R. Del Prete, M. Haguenauer, M. Itow, Y. Iwata, T. Kasahara, K. Kawade, K. Makino, Y. Masuda, K. Matsubayashi, E. Menjo, H. Mitsuka, G. Muraki, Y. Papini, P. Perrot, A. -L. Ricciarini, S. Sako, T. Sakurai, N. Suzuki, T. Tamura, T. Tiberio, A. Torii, S. Tricomi, A. Turner, W. C. Ueno, M. Zhou, Q. D. CA LHCf Collaboration TI Measurements of longitudinal and transverse momentum distributions for neutral pions in the forward-rapidity region with the LHCf detector SO PHYSICAL REVIEW D LA English DT Article ID TELESCOPE ARRAY EXPERIMENT; PROTON-PROTON COLLISIONS; HIGH-ENERGY SCATTERING; COSMIC-RAYS; BARYON PRODUCTION; WORKING GROUP; FRAGMENTATION; ASTROPHYSICS; COLLIDER; SPECTRUM AB The differential cross sections for inclusive neutral pions as a function of transverse and longitudinal momentum in the very forward-rapidity region have been measured at the LHC with the LHC forward detector in proton-proton collisions at root s = 2.76 and 7 TeV and in proton-lead collisions at nucleon nucleon center-of-mass energies of root sNN = 5.02 TeV. Such differential cross sections in proton-proton collisions are compatible with the hypotheses of limiting fragmentation and Feynman scaling. Comparing proton-proton with proton-lead collisions, we find a sizable suppression of the production of neutral pions in the differential cross sections after subtraction of ultraperipheral proton-lead collisions. This suppression corresponds to the nuclear modification factor value of about 0.1-0.3. The experimental measurements presented in this paper provide a benchmark for the hadronic interaction Monte Carlo simulation codes that are used for the simulation of cosmic ray air showers. C1 [Adriani, O.; Berti, E.; Bonechi, L.; Bongi, M.; D'Alessandro, R.; Del Prete, M.; Papini, P.; Ricciarini, S.; Tiberio, A.] Ist Nazl Fis Nucl, Sect Florence, Florence, Italy. [Adriani, O.; Berti, E.; Bongi, M.; D'Alessandro, R.; Del Prete, M.; Mitsuka, G.; Tiberio, A.] Univ Florence, I-50121 Florence, Italy. [Haguenauer, M.] Ecole Polytech, Palaiseau, France. [Itow, Y.; Sako, T.] Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi, Japan. [Itow, Y.; Sako, T.; Sakurai, N.] Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univers, Nagoya, Aichi, Japan. [Iwata, T.; Kasahara, K.; Suzuki, T.; Torii, S.] Waseda Univ, RISE, Tokyo, Japan. [Kawade, K.; Makino, Y.; Masuda, K.; Matsubayashi, E.; Muraki, Y.; Ueno, M.; Zhou, Q. D.] Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi, Japan. [Menjo, H.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Perrot, A. -L.] CERN, CH-1211 Geneva 23, Switzerland. [Ricciarini, S.] CNR, IFAC, I-00185 Rome, Italy. [Tamura, T.] Kanagawa Univ, Yokohama, Kanagawa, Japan. [Tricomi, A.] Ist Nazl Fis Nucl, Sect Catania, Catania, Italy. [Tricomi, A.] Univ Catania, I-95124 Catania, Italy. [Turner, W. C.] LBNL, Berkeley, CA USA. [Mitsuka, G.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Sakurai, N.] Univ Tokushima, Inst Socioarts & Sci, Tokushima, Japan. RP Adriani, O (reprint author), Ist Nazl Fis Nucl, Sect Florence, Florence, Italy.; Adriani, O (reprint author), Univ Florence, I-50121 Florence, Italy. EM gaku.mitsuka@riken.jp FU MEXT; Istituto Nazionale di Fisica Nucleare (INFN) in Italy FX The LHCf Collaboration acknowledges CERN staff and the ATLAS Collaboration for their essential contributions to the successful operation of LHCf. We thank S. Ostapchenko and T. Pierog for numerous discussions and for confirming the results of the MC simulations. We are grateful to C. Baus, T. Pierog, and R. Ulrich for providing the CRMC program codes and useful comments. This work has been partly supported by a Grant-in-Aid for Scientific research by MEXT of Japan, a Grant-in-Aid for a JSPS Postdoctoral Fellowship for Research Abroad, a Grant-in-Aid for Nagoya University GCOE "QFPU" from MEXT, and Istituto Nazionale di Fisica Nucleare (INFN) in Italy. Part of this work was performed using the computer resources provided by the Institute for the Cosmic-Ray Research (University of Tokyo), CERN, and CNAF (INFN). NR 68 TC 4 Z9 4 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 22 PY 2016 VL 94 IS 3 AR 032007 DI 10.1103/PhysRevD.94.032007 PG 38 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DU0KR UT WOS:000381893100003 ER PT J AU Martinez, NJD Derose, CT Brock, RW Starbuck, AL Pomerene, AT Lentine, AL Trotter, DC Davids, PS AF Martinez, Nicholas J. D. Derose, Christopher T. Brock, Reinhard W. Starbuck, Andrew L. Pomerene, Andrew T. Lentine, Anthony L. Trotter, Douglas C. Davids, Paul S. TI High performance waveguide-coupled Ge-on-Si linear mode avalanche photodiodes SO OPTICS EXPRESS LA English DT Article ID GAIN-BANDWIDTH PRODUCT; LOW-VOLTAGE; 1550 NM; PHOTODETECTOR; DETECTORS; HYDROGEN; GROWTH; LIGHT AB We present experimental results for a selective epitaxially grown Ge-on-Si separate absorption and charge multiplication (SACM) integrated waveguide coupled avalanche photodiode (APD) compatible with our silicon photonics platform. Epitaxially grown Ge-on-Si waveguide-coupled linear mode avalanche photodiodes with varying lateral multiplication regions and different charge implant dimensions are fabricated and their illuminated device characteristics and high-speed performance is measured. We report a record gain-bandwidth product of 432 GHz for our highest performing waveguide-coupled avalanche photodiode operating at 1510nm. Bit error rate measurements show operation with BER < 10(-12), in the range from -18.3 dBm to -12 dBm received optical power into a 50 Omega load and open eye diagrams with 13 Gbps pseudo-random data at 1550 nm. (C) 2016 Optical Society of America C1 [Martinez, Nicholas J. D.; Derose, Christopher T.; Brock, Reinhard W.; Starbuck, Andrew L.; Pomerene, Andrew T.; Lentine, Anthony L.; Trotter, Douglas C.; Davids, Paul S.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Davids, PS (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pdavids@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia's Laboratory Directed Research and Development (LDRD) program; Department of Defense FX We would like to thank Chris Long for useful comments and Kate Musick of Sandia for SEM pictures of our devices. Funding for this work was provided by Sandia's Laboratory Directed Research and Development (LDRD) program and the Department of Defense. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 35 TC 1 Z9 1 U1 8 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD AUG 22 PY 2016 VL 24 IS 17 BP 19072 EP 19081 AR 268043 DI 10.1364/OE.24.019072 PG 10 WC Optics SC Optics GA DY6KV UT WOS:000385227100022 PM 27557187 ER PT J AU Kundu, S Stieber, SCE Ferrier, MG Kozimor, SA Bertke, JA Warren, TH AF Kundu, Subrata Stieber, S. Chantal E. Ferrier, Maryline G. Kozimor, Stosh A. Bertke, Jeffery A. Warren, Timothy H. TI Redox Non-Innocence of Nitrosobenzene at Nickel SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE nickel; nitric oxide; nitrosobenzene; redox-active ligands; X-ray spectroscopy ID COORDINATION-COMPLEXES; ELECTRONIC-STRUCTURE; ALLYLIC AMINATION; BOND ACTIVATION; METAL-COMPLEXES; HNO; REACTIVITY; CONVERSION; DIOXYGENASE; LIGAND AB Nitrosobenzene (PhNO) serves as a stable analogue of nitroxyl (HNO), a biologically relevant, redox-active nitric oxide derivative. Capture of nitrosobenzene at the electron-deficient beta-diketiminato nickel(I) complex [(Pr2NNF6)-Pr-i]Ni results in reduction of the PhNO ligand to a (PhNO)(./-) species coordinated to a square planar Ni-II center in [iPr(2)NN(F6)] Ni(eta(2)-ONPh). Ligand centered reduction leads to the (PhNO)(2-) moiety bound to NiII supported by XAS studies. Systematic investigation of structure-reactivity patterns of (PhNO)(./-) and (PhNO)(2-) ligands reveals parallels with superoxo (O-2)(./-) and peroxo (O-2)(2-) ligands, respectively, and forecasts reactivity patterns of the more transient HNO ligand. C1 [Kundu, Subrata; Bertke, Jeffery A.; Warren, Timothy H.] Georgetown Univ, Dept Chem, Box 571227, Washington, DC 20057 USA. [Stieber, S. Chantal E.; Ferrier, Maryline G.; Kozimor, Stosh A.] Los Alamos Natl Lab, Inorgan Isotope & Actinide Chem, Los Alamos, NM 87545 USA. [Stieber, S. Chantal E.] Calif State Polytech Univ Pomona, Dept Chem & Biochem, Pomona, CA 91768 USA. RP Kundu, S; Warren, TH (reprint author), Georgetown Univ, Dept Chem, Box 571227, Washington, DC 20057 USA.; Stieber, SCE (reprint author), Los Alamos Natl Lab, Inorgan Isotope & Actinide Chem, Los Alamos, NM 87545 USA.; Stieber, SCE (reprint author), Calif State Polytech Univ Pomona, Dept Chem & Biochem, Pomona, CA 91768 USA. EM skundu.chem@gmail.com; sestieber@cpp.edu; thw@georgetown.edu OI Kundu, Subrata/0000-0002-3533-3206 FU National Science Foundation [CHE-1459090, CHE-1337975]; Georgetown Environment Initiative; DOE, Office of Science, BES [DE-AC02-76SF00515] FX T.H.W. acknowledges funding from the National Science Foundation (CHE-1459090 and CHE-1337975) and the Georgetown Environment Initiative. S.A.K. acknowledges the Heavy Element Chemistry Program by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE), and Seaborg Institute Postdoctoral Fellowship (S.C.E.S., M.G.F.). LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. DOE (DE-AC52-06NA25396). Use of Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, supported by DOE, Office of Science, BES (DE-AC02-76SF00515). S.C.E.S. acknowledges CPP College of Science and NSF XSEDE (CHE-150060, ACI-1053575). NR 40 TC 3 Z9 3 U1 9 U2 9 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD AUG 22 PY 2016 VL 55 IS 35 BP 10321 EP 10325 DI 10.1002/anie.201605026 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DW0ZZ UT WOS:000383373700023 PM 27471147 ER PT J AU Albo, A Hu, Q Reno, JL AF Albo, Asaf Hu, Qing Reno, John L. TI Room temperature negative differential resistance in terahertz quantum cascade laser structures SO APPLIED PHYSICS LETTERS LA English DT Article AB The mechanisms that limit the temperature performance of GaAs/Al0.15GaAs-based terahertz quantum cascade lasers (THz-QCLs) have been identified as thermally activated LO-phonon scattering and leakage of charge carriers into the continuum. Consequently, the combination of highly diagonal optical transition and higher barriers should significantly reduce the adverse effects of both mechanisms and lead to improved temperature performance. Here, we study the temperature performance of highly diagonal THz-QCLs with high barriers. Our analysis uncovers an additional leakage channel which is the thermal excitation of carriers into bounded higher energy levels, rather than the escape into the continuum. Based on this understanding, we have designed a structure with an increased intersubband spacing between the upper lasing level and excited states in a highly diagonal THz-QCL, which exhibits negative differential resistance even at room temperature. This result is a strong evidence for the effective suppression of the aforementioned leakage channel. Published by AIP Publishing. C1 [Albo, Asaf; Hu, Qing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Albo, Asaf; Hu, Qing] MIT, Elect Res Lab, Cambridge, MA 02139 USA. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, MS 1303, Albuquerque, NM 87185 USA. RP Albo, A (reprint author), MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA.; Albo, A (reprint author), MIT, Elect Res Lab, Cambridge, MA 02139 USA. EM asafalbo@gmail.com RI Albo, Asaf/C-7774-2016 OI Albo, Asaf/0000-0002-7073-2958 FU NSF; Israel MoD; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Yuri V. Flores for helpful discussions and for his help in clarifying this manuscript. A.A. would like to acknowledge the generosity of the MIT-Technion and Andrew and Erna Finci Viterbi Fellowships and their support during this study. This work was supported by NSF and Israel MoD, and also performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 17 TC 3 Z9 3 U1 6 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081102 DI 10.1063/1.4961617 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000002 ER PT J AU Enriquez, E Zhang, YY Chen, AP Bi, ZX Wang, YQ Fu, EG Harrell, Z Lu, XJ Dowden, P Wang, HY Chen, CL Jia, QX AF Enriquez, Erik Zhang, Yingying Chen, Aiping Bi, Zhenxing Wang, Yongqiang Fu, Engang Harrell, Zachary Lu, Xujie Dowden, Paul Wang, Haiyan Chen, Chonglin Jia, Quanxi TI Epitaxial growth and physical properties of ternary nitride thin films by polymer-assisted deposition SO APPLIED PHYSICS LETTERS LA English DT Article ID LOW-FIELD MAGNETORESISTANCE; CHEMICAL-VAPOR-DEPOSITION; SOLID-STATE CHEMISTRY; MAGNETIC CHARACTERIZATION; METAL NITRIDES; FEWN2; EVOLUTION; ROUTE; FE AB Epitaxial layered ternary metal-nitride FeMoN2, (Fe0.33Mo0.67)MoN2, CoMoN2, and FeWN2 thin films have been grown on c-plane sapphire substrates by polymer-assisted deposition. The ABN(2) layer sits on top of the oxygen sublattices of the substrate with three possible matching configurations due to the significantly reduced lattice mismatch. The doping composition and elements affect not only the out-of-plane lattice parameters but also the temperature-dependent electrical properties. These films have resistivity in the range of 0.1-1 m Omega.cm, showing tunable metallic or semiconducting behaviors by adjusting the composition. A modified parallel connection channel model has been used to analyze the grain boundary and Coulomb blockade effect on the electrical properties. The growth of the high crystallinity layered epitaxial thin films provides an avenue to study the composition-structure-property relationship in ABN(2) materials through A and B-site substitution. Published by AIP Publishing. C1 [Enriquez, Erik; Chen, Aiping; Bi, Zhenxing; Wang, Yongqiang; Fu, Engang; Lu, Xujie; Dowden, Paul; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. [Zhang, Yingying] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China. [Harrell, Zachary; Chen, Chonglin] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Wang, Haiyan] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78539 USA. RP Enriquez, E (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. EM emenriquez@lanl.gov; yingyingzhang@mail.tsinghua.edu.cn; qxjia@lanl.gov RI Lu, Xujie/L-9672-2014; Chen, Aiping/F-3212-2011 OI Lu, Xujie/0000-0001-8402-7160; Chen, Aiping/0000-0003-2639-2797 FU NNSA's Laboratory Directed Research and Development Program; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX The work at Los Alamos National Laboratory was supported by the NNSA's Laboratory Directed Research and Development Program and was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy ( DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 38 TC 1 Z9 1 U1 15 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081907 DI 10.1063/1.4961880 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000016 ER PT J AU Gammer, C Kacher, J Czarnik, C Warren, OL Ciston, J Minor, AM AF Gammer, C. Kacher, J. Czarnik, C. Warren, O. L. Ciston, J. Minor, A. M. TI Local and transient nanoscale strain mapping during in situ deformation SO APPLIED PHYSICS LETTERS LA English DT Article ID ELECTRON-MICROSCOPY; TEM AB The mobility of defects such as dislocations controls the mechanical properties of metals. This mobility is determined both by the characteristics of the defect and the material, as well as the local stress and strain applied to the defect. Therefore, the knowledge of the stress and strain during deformation at the scale of defects is important for understanding fundamental deformation mechanisms. Here, we demonstrate a method of measuring local stresses and strains during continuous in situ deformation with a resolution of a few nanometers using nanodiffraction strain mapping. Our results demonstrate how large multidimensional data sets captured with high speed electron detectors can be analyzed in multiple ways after an in situ TEM experiment, opening the door for true multimodal analysis from a single electron scattering experiment. Published by AIP Publishing. C1 [Gammer, C.; Kacher, J.; Ciston, J.; Minor, A. M.] Lawrence Berkeley Natl Lab, Natl Ctr Elect Microscopy Mol Foundry, Berkeley, CA 94720 USA. [Kacher, J.; Minor, A. M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Czarnik, C.] Gatan Inc, Pleasanton, CA 94588 USA. [Warren, O. L.] Hysitron Inc, Minneapolis, MN 55344 USA. [Gammer, C.] Erich Schmid Inst Mat Sci, Jahnstr 12, Leoben, Austria. [Kacher, J.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. RP Gammer, C; Minor, AM (reprint author), Lawrence Berkeley Natl Lab, Natl Ctr Elect Microscopy Mol Foundry, Berkeley, CA 94720 USA.; Minor, AM (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Gammer, C (reprint author), Erich Schmid Inst Mat Sci, Jahnstr 12, Leoben, Austria. EM christoph.gammer@oeaw.ac.at; aminor@lbl.gov OI Gammer, Christoph/0000-0003-1917-4978 FU Austrian Science Fund (FWF) [J3397]; National Science Foundation CMMI/MoM program under GOALI Grant [1235610]; Molecular Foundry at Lawrence Berkeley National Laboratory; U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge support by the Austrian Science Fund (FWF): [J3397], the National Science Foundation CMMI/MoM program under GOALI Grant No. 1235610, and the Molecular Foundry at Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy under Contract No. #DE-AC02-05CH11231. We would also like to thank U. Dahmen for helpful discussions. NR 16 TC 0 Z9 0 U1 9 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081906 DI 10.1063/1.4961683 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000015 ER PT J AU Li, X Hua, WJ Wang, BY Pong, WF Glans, PA Guo, JH Luo, Y AF Li, Xin Hua, Weijie Wang, Bo-Yao Pong, Way-Faung Glans, Per-Anders Guo, Jinghua Luo, Yi TI Effects of domain size on x-ray absorption spectra of boron nitride doped graphenes SO APPLIED PHYSICS LETTERS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; CORE EXCITATIONS; CHEMICAL-SHIFTS; ATOMIC LAYERS; HETEROSTRUCTURES; APPROXIMATION; CARBON AB Doping is an efficient way to open the zero band gap of graphene. The control of the dopant domain size allows us to tailor the electronic structure and the properties of the graphene. We have studied the electronic structure of boron nitride doped graphenes with different domain sizes by simulating their near-edge X-ray absorption fine structure (NEXAFS) spectra at the N K-edge. Six different doping configurations (five quantum dot type and one phase-separated zigzag-edged type) were chosen, and N K-edge NEXAFS spectra were calculated with large truncated cluster models by using the density functional theory with hybrid functional and the equivalent core hole approximation. The opening of the band gap as a function of the domain size is revealed. We found that nitrogens in the dopant boundary contribute a weaker, red-shifted pi* peak in the spectra as compared to those in the dopant domain center. The shift is related to the fact that these interfacial nitrogens dominate the lowest conduction band of the system. Upon increasing the domain size, the ratio of interfacial atom decreases, which leads to a blue shift of the pi* peak in the total NEXAFS spectra. The spectral evolution agrees well with experiments measured at different BN-dopant concentrations and approaches to that of a pristine h-BN sheet. Published by AIP Publishing. C1 [Li, Xin; Luo, Yi] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Li, Xin; Hua, Weijie; Luo, Yi] KTH Royal Inst Technol, Dept Theoret Chem & Biol, Sch Biotechnol, S-10691 Stockholm, Sweden. [Li, Xin; Glans, Per-Anders; Guo, Jinghua] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Wang, Bo-Yao] Natl Changhua Univ Educ, Dept Phys, Changhua 500, Taiwan. [Pong, Way-Faung] Tamkang Univ, Dept Phys, Tamsui 251, Taiwan. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. RP Hua, WJ (reprint author), KTH Royal Inst Technol, Dept Theoret Chem & Biol, Sch Biotechnol, S-10691 Stockholm, Sweden. EM hua@theochem.kth.se; jguo@lbl.gov RI Luo, Yi/B-1449-2009; Hua, Weijie/F-3099-2010 OI Luo, Yi/0000-0003-0007-0394; Hua, Weijie/0000-0002-6706-651X FU Users with Excellence of the Hefei Science Center [2015HSC-UE008]; Knut and Alice Wallenberg Foundation [KAW-2013.0020]; Goran Gustafsson Foundation for Research in Natural Sciences and Medicine; Swedish Research Council (VR); Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge the financial support from the Users with Excellence of the Hefei Science Center (2015HSC-UE008), the Knut and Alice Wallenberg Foundation (Grant No. KAW-2013.0020) for the project "Strong Field Physics and New States of Matter," the Goran Gustafsson Foundation for Research in Natural Sciences and Medicine, and the Swedish Research Council (VR). The Swedish National Infrastructure for Computing (SNIC) and the National Energy Research Scientific Computing Center (NERSC) are acknowledged for the computational time. The work at BL8.0.1 of ALS and NERSC is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 0 Z9 0 U1 11 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081601 DI 10.1063/1.4961628 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000006 ER PT J AU Ren, F Schmidt, R Keum, JK Qian, BS Case, ED Littrell, KC An, K AF Ren, Fei Schmidt, Robert Keum, Jong K. Qian, Bosen Case, Eldon D. Littrell, Ken C. An, Ke TI In situ neutron scattering study of nanoscale phase evolution in PbTe-PbS thermoelectric material SO APPLIED PHYSICS LETTERS LA English DT Article ID HIGH-PERFORMANCE; THERMAL-EXPANSION; SEPARATION; DEVICES; MERIT AB Introducing nanostructural second phases has proved to be an effective approach to reduce the lattice thermal conductivity and thus enhances the figure of merit for many thermoelectric materials. Studies of the formation and evolution of these second phases are essential to understanding material temperature dependent behaviors, improving thermal stabilities, as well as designing new materials. In this study, powder samples of the PbTe-PbS thermoelectric material were examined using in situ neutron diffraction and small angle neutron scattering (SANS) techniques between room temperature and elevated temperature up to 663K, to explore quantitative information on the structure, weight fraction, and size of the second phase. Neutron diffraction data showed that the as-milled powder was primarily a solid solution prior to heat treatment. During heating, a PbS second phase precipitated out of the PbTe matrix around 500K, while re-dissolution started around 600K. The second phase remained separated from the matrix upon cooling. Furthermore, SANS data indicated that there are two populations of nanostructures. The size of the smaller nanostructure increased from initially 5 nm to approximately 25nm after annealing at 650 K, while the size of the larger one remained unchanged. This study demonstrated that in situ neutron techniques are effective means to obtain quantitative information on temperature-dependent nanostructural behavior of thermoelectrics and likely other high-temperature materials. Published by AIP Publishing. C1 [Ren, Fei; Qian, Bosen] Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA. [Schmidt, Robert; Case, Eldon D.] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Keum, Jong K.; Littrell, Ken C.; An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37830 USA. RP Ren, F (reprint author), Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA.; An, K (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37830 USA. EM renfei@temple.edu; kean@ornl.gov RI An, Ke/G-5226-2011; Keum, Jong/N-4412-2015; OI An, Ke/0000-0002-6093-429X; Keum, Jong/0000-0002-5529-1373; Schmidt, Robert/0000-0002-8838-8999; Littrell, Kenneth/0000-0003-2308-8618 FU Temple University faculty start-up fund; Department of Energy, "Revolutionary Materials for Solid State Energy Conversion Center"; Energy Frontier Research Center by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001054]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors acknowledge the financial support from Temple University faculty start-up fund and the Department of Energy, "Revolutionary Materials for Solid State Energy Conversion Center," an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001054. Research conducted at ORNL's Spallation Neutron Source and High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors also thank Dr. Dong Ma and Ms. Hui Yang of Oak Ridge National Laboratory for their technical assistance. NR 23 TC 0 Z9 0 U1 11 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081903 DI 10.1063/1.4961677 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000012 ER PT J AU Zheng, SJ Zhang, RF Huang, R Taniguchi, T Ma, XL Ikuhara, Y Beyerlein, IJ AF Zheng, Shijian Zhang, Ruifeng Huang, Rong Taniguchi, Takashi Ma, Xiuliang Ikuhara, Yuichi Beyerlein, Irene J. TI Structure and energetics of nanotwins in cubic boron nitrides SO APPLIED PHYSICS LETTERS LA English DT Article ID DEFORMATION MECHANISMS; MAXIMUM STRENGTH; TWIN BOUNDARIES; GROWTH TWINS; METALS; COPPER; DISLOCATIONS; COMPOSITES; NANOSCALE AB Recently, nanotwinned cubic boron nitrides (NT c-BN) have demonstrated extraordinary leaps in hardness. However, an understanding of the underlying mechanisms that enable nanotwins to give orders of magnitude increases in material hardness is still lacking. Here, using transmission electron microscopy, we report that the defect density of twin boundaries depends on nanotwin thickness, becoming defect-free, and hence more stable, as it decreases below 5 nm. Using ab initio density functional theory calculations, we reveal that the Shockley partials, which may dominate plastic deformation in c-BNs, show a high energetic barrier. We also report that the c-BN twin boundary has an asymmetrically charged electronic structure that would resist migration of the twin boundary under stress. These results provide important insight into possible nanotwin hardening mechanisms in c-BN, as well as how to design these nanostructured materials to reach their full potential in hardness and strength. Published by AIP Publishing. C1 [Zheng, Shijian; Ma, Xiuliang] Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China. [Zhang, Ruifeng] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Zhang, Ruifeng] Beihang Univ, Int Res Inst Multidisciplinary Sci, Beijing 100191, Peoples R China. [Huang, Rong] East China Normal Univ, Key Lab Polar Mat & Devices, Minist Educ, Shanghai 200062, Peoples R China. [Taniguchi, Takashi] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050044, Japan. [Ikuhara, Yuichi] Japan Fine Ceram Ctr, Nanostruct Res Lab, Nagoya, Aichi 4568587, Japan. [Ikuhara, Yuichi] Univ Tokyo, Inst Engn Innovat, Tokyo 1138656, Japan. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zheng, SJ (reprint author), Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China.; Zhang, RF (reprint author), Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China.; Zhang, RF (reprint author), Beihang Univ, Int Res Inst Multidisciplinary Sci, Beijing 100191, Peoples R China. EM sjzheng@imr.ac.cn; zrf@buaa.edu.cn RI Ikuhara, Yuichi/F-3066-2010; Huang, Rong/A-9684-2008 FU "Hundred Talents Project" of the Chinese Academy of Sciences; National Thousand Young Talents Program of China; Fundamental Research Funds for the Central Universities; National Natural Science Foundation of China [51471018]; Laboratory Directed Research and Development Program Award [20140348ER]; National Supercomputer Center at TianJin FX S.J.Z. wishes to acknowledge support from the "Hundred Talents Project" of the Chinese Academy of Sciences and the National Thousand Young Talents Program of China. R.F.Z. is supported by the Fundamental Research Funds for the Central Universities, National Natural Science Foundation of China (51471018), and the National Thousand Young Talents Program of China. I.J.B. would like to acknowledge support from a Laboratory Directed Research and Development Program Award, No. 20140348ER. We would like to thank Professor Dr. S. Veprek for constructive comments and suggestions. We also gratefully acknowledge the support from the National Supercomputer Center at TianJin. NR 36 TC 2 Z9 2 U1 17 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 22 PY 2016 VL 109 IS 8 AR 081901 DI 10.1063/1.4961240 PG 5 WC Physics, Applied SC Physics GA DW7RO UT WOS:000383849000010 ER PT J AU Kim, SK Chung, D Himmel, ME Bomble, YJ Westpheling, J AF Kim, Sun-Ki Chung, Daehwan Himmel, Michael E. Bomble, Yannick J. Westpheling, Janet TI Heterologous expression of family 10 xylanases from Acidothermus cellulolyticus enhances the exoproteome of Caldicellulosiruptor bescii and growth on xylan substrates SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Consolidated bioprocessing; Biomass deconstruction; Xylanase; Caldicellulosiruptor ID PLANT BIOMASS; SACCHAROMYCES-CEREVISIAE; DSM 6725; ETHANOL-PRODUCTION; BACILLUS-SUBTILIS; DECONSTRUCTION; DEGRADATION; BACTERIA; INSIGHTS; ENZYMES AB Background: The ability to deconstruct plant biomass without conventional pretreatment has made members of the genus Caldicellulosiruptor the target of investigation for the consolidated processing of lignocellulosic biomass to biofuels and bioproducts. These Gram-positive bacteria are hyperthermophilic anaerobes and the most thermophilic cellulolytic organisms so far described. They use both C5 and C6 sugars simultaneously and have the ability to grow well on xylan, a major component of plant cell walls. This is an important advantage for their use to efficiently convert biomass at yields sufficient for an industrial process. For commodity chemicals, yield from substrate is perhaps the most important economic factor. In an attempt to improve even further the ability of C. bescii to use xylan, we introduced two xylanases from Acidothermus cellulolyticus. Acel_0180 includes tandem carbohydrate-binding modules (CBM2 and CBM3) located at the C-terminus, one of which, CBM2, is not present in C. bescii. Also, the sequences of Xyn10A and Acel_0180 have very little homology with the GH10 domains present in C. bescii. For these reasons, we selected these xylanases as potential candidates for synergistic interaction with those in the C. bescii exoproteome. Results: Heterologous expression of two xylanases from Acidothermus cellulolyticus in Caldicellulosiruptor bescii resulted in a modest, but significant increase in the activity of the exoproteome of C. bescii on xylan substrates. Even though the increase in extracellular activity was modest, the ability of C. bescii to grow on these substrates was dramatically improved suggesting that the xylan substrate/microbe interaction substantially increased deconstruction over the secreted free enzymes alone. Conclusions: We anticipate that the ability to efficiently use xylan, a major component of plant cell walls for conversion of plant biomass to products of interest, will allow the conversion of renewable, sustainable, and inexpensive plant feedstocks to products at high yields. C1 [Kim, Sun-Ki; Westpheling, Janet] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Chung, Daehwan; Himmel, Michael E.; Bomble, Yannick J.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO USA. [Kim, Sun-Ki; Chung, Daehwan; Himmel, Michael E.; Bomble, Yannick J.; Westpheling, Janet] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Westpheling, J (reprint author), Univ Georgia, Dept Genet, Athens, GA 30602 USA.; Westpheling, J (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. EM janwest@uga.edu FU BioEnergy Science Center, US DOE Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; US DOE [DE-AC05-00OR22725] FX This work was supported by the BioEnergy Science Center, US DOE Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the US DOE under contract DE-AC05-00OR22725. The funders had no role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 43 TC 0 Z9 0 U1 2 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD AUG 22 PY 2016 VL 9 AR 176 DI 10.1186/s13068-016-0588-9 PG 10 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DV6BH UT WOS:000383015200003 PM 27555882 ER PT J AU Steinheimer, J Randrup, J AF Steinheimer, Jan Randrup, Jorgen TI Spinodal amplification and baryon number fluctuations in nuclear collisions at NICA SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article AB We discuss the effect of spinodal instabilities on the fluctuations of conserved flavors in nuclear collisions at NICA. We find that, when the system undergoes a phase transformation, baryon number clumping due to the mechanical instabilities in the spinodal phase occurs. This dynamical clumping enhances the cumulants of the net baryon number residing in a finite test volume of the total collision system. C1 [Steinheimer, Jan] Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. [Randrup, Jorgen] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Steinheimer, J (reprint author), Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. EM steinheimer@th.physik.uni-frankfurt.de FU GSI; LOEWE; Hessian initiative for excellence, through HIC for FAIR; Helmholtz International Center for FAIR; Office of Nuclear Physics in the U.S. Department of Energy's Office of Science [DE-AC02-05CH11231] FX This work was supported by GSI and LOEWE, the Hessian initiative for excellence, through HIC for FAIR, the Helmholtz International Center for FAIR (JS) and by the Office of Nuclear Physics in the U.S. Department of Energy's Office of Science under Contract No. DE-AC02-05CH11231 (JR). The computational resources were provided by LOEWE-CSC, the LOEWE Frankfurt Center for Scientific Computing. NR 12 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD AUG 22 PY 2016 VL 52 IS 8 AR 239 DI 10.1140/epja/i2016-16239-2 PG 5 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU7OB UT WOS:000382403100003 ER PT J AU Rasco, BC Wolinska-Cichocka, M Fijalkowska, A Rykaczewski, KP Karny, M Grzywacz, RK Goetz, KC Gross, CJ Stracener, DW Zganjar, EF Batchelder, JC Blackmon, JC Brewer, NT Go, S Heffron, B King, T Matta, JT Miernik, K Nesaraja, CD Paulauskas, SV Rajabali, MM Wang, EH Winger, JA Xiao, Y Zachary, CJ AF Rasco, B. C. Wolinska-Cichocka, M. Fijalkowska, A. Rykaczewski, K. P. Karny, M. Grzywacz, R. K. Goetz, K. C. Gross, C. J. Stracener, D. W. Zganjar, E. F. Batchelder, J. C. Blackmon, J. C. Brewer, N. T. Go, S. Heffron, B. King, T. Matta, J. T. Miernik, K. Nesaraja, C. D. Paulauskas, S. V. Rajabali, M. M. Wang, E. H. Winger, J. A. Xiao, Y. Zachary, C. J. TI Decays of the Three Top Contributors to the Reactor (nu)over-bar(e) High-Energy Spectrum, Rb-92, (96)gsY, and Cs-142, Studied with Total Absorption Spectroscopy SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEAR-DATA SHEETS; BETA-DECAY; SPECTROMETER; HRIBF AB We report total absorption spectroscopy measurements of Rb-92, (96)gsY, and Cs-142 beta decays, which are the most important contributors to the high energy (nu) over bar (e) spectral shape in nuclear reactors. These three beta decays contribute 43% of the (nu) over bar (e) flux near 5.5 MeV emitted by nuclear reactors. This (nu) over bar (e) energy is particularly interesting due to spectral features recently observed in several experiments including the Daya Bay, Double Chooz, and RENO Collaborations. Measurements were conducted at Oak Ridge National Laboratory by means of proton-induced fission of U-238 with on-line mass separation of fission fragments and the Modular Total Absorption Spectrometer. We observe a beta-decay pattern that is similar to recent measurements of Rb-92, with a ground-state to ground-state beta feeding of 91(3)%. We verify the 96gsY ground-state to ground-state beta feeding of 95.5(20)%. Our measurements substantially modify the beta-decay feedings of Cs-142, reducing the beta feeding to Ba-142 states below 2 MeV by 32% when compared with the latest evaluations. Our results increase the discrepancy between the observed and the expected reactor (nu) over bar (e) flux between 5 and 7 MeV, the maximum excess increases from similar to 10% to similar to 12%. C1 [Rasco, B. C.; Wolinska-Cichocka, M.; Karny, M.; Grzywacz, R. K.; Batchelder, J. C.; Brewer, N. T.; Miernik, K.] Oak Ridge Natl Lab, JINPA, Oak Ridge, TN 37831 USA. [Rasco, B. C.; Wolinska-Cichocka, M.; Rykaczewski, K. P.; Karny, M.; Grzywacz, R. K.; Gross, C. J.; Stracener, D. W.; Brewer, N. T.; Heffron, B.; Matta, J. T.; Nesaraja, C. D.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Rasco, B. C.; Fijalkowska, A.; Grzywacz, R. K.; Goetz, K. C.; Brewer, N. T.; Go, S.; Heffron, B.; King, T.; Paulauskas, S. V.; Xiao, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA. [Rasco, B. C.; Zganjar, E. F.; Blackmon, J. C.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Wolinska-Cichocka, M.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Fijalkowska, A.; Karny, M.; Miernik, K.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Goetz, K. C.] Univ Tennessee, CIRE Bredesen Ctr, Knoxville, TN 37966 USA. [Batchelder, J. C.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Rajabali, M. M.] Tennessee Technol Univ, Dept Phys, Cookeville, TN 38505 USA. [Wang, E. H.; Zachary, C. J.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Winger, J. A.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. RP Rasco, BC (reprint author), Oak Ridge Natl Lab, JINPA, Oak Ridge, TN 37831 USA.; Rasco, BC (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA.; Rasco, BC (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA.; Rasco, BC (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM brasco@utk.edu FU Office of Nuclear Physics, U.S. Department of Energy [DE-AC05-00OR22725, DE-FG02-96ER40983, DE-FG02-96ER40978, DE-FG02-96ER41006, DE-FG-05-88ER40407]; Polish National Science Center [UMO-2015/18/E/ST2/00217, UMO-2013/08/T/ST2/00624] FX We would like to thank the ORNL Tandem operations staff for providing the excellent quality proton beams necessary for this work. This research was also sponsored by the Office of Nuclear Physics, U.S. Department of Energy under Contracts No. DE-AC05-00OR22725 (ORNL), No. DE-FG02-96ER40983 (UTK), No. DE-FG02-96ER40978 (LSU), No. DE-FG02-96ER41006 (MSU), No. DE-FG-05-88ER40407 (VU), and by the Polish National Science Center under Contracts No. UMO-2015/18/E/ST2/00217 and No. UMO-2013/08/T/ST2/00624. NR 37 TC 3 Z9 3 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 22 PY 2016 VL 117 IS 9 AR 092501 DI 10.1103/PhysRevLett.117.092501 PG 6 WC Physics, Multidisciplinary SC Physics GA DU1YP UT WOS:000382007200001 PM 27610847 ER PT J AU Mert, A Fahjan, YM Hutchings, LJ Pinar, A AF Mert, Aydin Fahjan, Yasin M. Hutchings, Lawrence J. Pinar, Ali TI Physically based probabilistic seismic hazard analysis using broadband ground motion simulation: a case study for the Prince Islands Fault, Marmara Sea SO EARTH PLANETS AND SPACE LA English DT Article DE Simulation of strong ground motion; Probabilistic seismic hazard assessment; Empirical Green's function; Synthetic Green's function; Prince Island Fault ID NORTH ANATOLIAN FAULT; EMPIRICAL GREENS-FUNCTIONS; 17 AUGUST 1999; SOURCE PARAMETERS; TIME HISTORIES; REGION TURKEY; AEGEAN SEA; WAVE-FORM; NW TURKEY; EARTHQUAKE AB The main motivation for this study was the impending occurrence of a catastrophic earthquake along the Prince Island Fault (PIF) in the Marmara Sea and the disaster risk around the Marmara region, especially in Istanbul. This study provides the results of a physically based probabilistic seismic hazard analysis (PSHA) methodology, using broadband strong ground motion simulations, for sites within the Marmara region, Turkey, that may be vulnerable to possible large earthquakes throughout the PIF segments in the Marmara Sea. The methodology is called physically based because it depends on the physical processes of earthquake rupture and wave propagation to simulate earthquake ground motion time histories. We included the effects of all considerable-magnitude earthquakes. To generate the high-frequency (0.5-20 Hz) part of the broadband earthquake simulation, real, small-magnitude earthquakes recorded by a local seismic array were used as empirical Green's functions. For the frequencies below 0.5 Hz, the simulations were obtained by using synthetic Green's functions, which are synthetic seismograms calculated by an explicit 2D/3D elastic finite difference wave propagation routine. By using a range of rupture scenarios for all considerable-magnitude earthquakes throughout the PIF segments, we produced a hazard calculation for frequencies of 0.1-20 Hz. The physically based PSHA used here followed the same procedure as conventional PSHA, except that conventional PSHA utilizes point sources or a series of point sources to represent earthquakes, and this approach utilizes the full rupture of earthquakes along faults. Furthermore, conventional PSHA predicts ground motion parameters by using empirical attenuation relationships, whereas this approach calculates synthetic seismograms for all magnitudes of earthquakes to obtain ground motion parameters. PSHA results were produced for 2, 10, and 50 % hazards for all sites studied in the Marmara region. C1 [Mert, Aydin; Pinar, Ali] Bogazici Univ, Kandilli Observ & Earthquake Res Inst, Dept Earthquake Engn, Istanbul, Turkey. [Fahjan, Yasin M.] Gebze Tech Univ, Dept Earthquake & Struct Engn, Kocaeli, Turkey. [Hutchings, Lawrence J.] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. RP Mert, A (reprint author), Bogazici Univ, Kandilli Observ & Earthquake Res Inst, Dept Earthquake Engn, Istanbul, Turkey. EM mertay@boun.edu.tr FU Bogazici University Research Fund [10701]; Scientific and Technological Research Council of Turkey (TUBITAK) [2219, B.14.2.TBT.0.06.01-219-84] FX This work was supported by the Bogazici University Research Fund Grant Number 10701 and the Scientific and Technological Research Council of Turkey (TUBITAK) under the 2219 Postdoctoral Research Fellowship Program, number B.14.2.TBT.0.06.01-219-84. NR 100 TC 0 Z9 0 U1 4 U2 5 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1880-5981 J9 EARTH PLANETS SPACE JI Earth Planets Space PD AUG 22 PY 2016 VL 68 AR 146 DI 10.1186/s40623-016-0520-3 PG 26 WC Geosciences, Multidisciplinary SC Geology GA DT9FI UT WOS:000381800800001 ER PT J AU Stalzer, MM Telser, J Krzystek, J Motta, A Delferro, M Marks, TJ AF Stalzer, Madelyn M. Telser, Joshua Krzystek, Jurek Motta, Alessandro Delferro, Massimiliano Marks, Tobin J. TI A Neutrally Charged Trimethylmanganese(III) Complex: Synthesis, Characterization, and Disproportionation Chemistry SO ORGANOMETALLICS LA English DT Article ID VALENT ORGANOMANGANESE CHEMISTRY; ELECTRON-PARAMAGNETIC-RESONANCE; HIGH-SPIN MANGANESE(III); TRANSITION-METAL; HIGH-FREQUENCY; MAGNETIC-PROPERTIES; FIELD EPR; MOLECULAR-STRUCTURE; BASIS-SETS; LIGANDS AB The synthesis and properties of an unusual, neutrally charged and volatile N,N,N',N'-tetramethylethylenediamine trimethyl manganese(III) complex, (TMEDA)MnMe3, are described, along with its facile disproportionation to the corresponding Mn(II) and Mn(IV) complexes. Characterization by single-crystal XRD, UV-vis spectroscopy, high-frequency and-field EPR (HFEPR), magnetic susceptibility, and density functional theory (DFT) computations indicate that the (TMEDA)MnMe3 electronic structure can be described as largely square pyramidal Mn(III) centered. The paucity of manganese(III) polyalkyls and the simplicity and reactivity of this compound implicate it as a potentially useful synthetic building block. C1 [Stalzer, Madelyn M.; Marks, Tobin J.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Telser, Joshua] Roosevelt Univ, Dept Biol Chem & Phys Sci, Chicago, IL 60605 USA. [Krzystek, Jurek] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Motta, Alessandro] Univ Roma La Sapienza, Dipartimento Chim, Ple A Moro 5, I-00185 Rome, Italy. [Motta, Alessandro] Univ Roma La Sapienza, INSTM UdR Roma, Ple A Moro 5, I-00185 Rome, Italy. [Delferro, Massimiliano] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Marks, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Delferro, M (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM delferro@anl.gov; t-marks@northwestern.edu OI Delferro, Massimiliano/0000-0002-4443-165X FU Center for Electrochemical Energy Science, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-06CH11]; NHMFL; NSF [DMR 1157490]; State of Florida; U.S. Department of Energy; CINECA under the ISCRA [HP10CRFT69 2016] FX This work was supported as part of the Center for Electrochemical Energy Science, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under award number DE-AC02-06CH11. HFEPR studies were supported by the NHMFL, which is funded by the NSF through a Cooperative Agreement DMR 1157490, the State of Florida, and the U.S. Department of Energy. Computational resources supporting this work were provided by the Northwestern University Quest High Performance Computing cluster (M.D.) and CINECA award N. HP10CRFT69 2016 under the ISCRA initiative (A.M.). Dr. A. Ozarowski is acknowledged for his EPR simulation and fitting program SPIN. NR 57 TC 0 Z9 0 U1 5 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD AUG 22 PY 2016 VL 35 IS 16 BP 2683 EP 2688 DI 10.1021/acs.organomet.6b00422 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA DU0MQ UT WOS:000381899600014 ER PT J AU Huang, YL Wang, HP Rimmer, RA Wang, SH Guo, JQ AF Huang, Yulu Wang, Haipeng Rimmer, Robert A. Wang, Shaoheng Guo, Jiquan TI Ultrafast harmonic rf kicker design and beam dynamics analysis for an energy recovery linac based electron circulator cooler ring SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article AB An ultrafast kicker system is being developed for the energy recovery linac (ERL) based electron circulator cooler ring (CCR) in the proposed Jefferson Lab Electron Ion Collider (JLEIC, previously named MEIC). In the CCR, the injected electron bunches can be recirculated while performing ion cooling for 10-30 turns before the extraction, thus reducing the recirculation beam current in the ERL to 1/10 - 1/30 (150 mA - 50 mA) of the cooling beam current (up to 1.5 A). Assuming a bunch repetition rate of 476.3 MHz and a recirculating factor of 10 in the CCR, the kicker is required to operate at a pulse repetition rate of 47.63 MHz with pulse width of around 2 ns, so that only every 10th bunch in the CCR will experience a transverse kick while the rest of the bunches will not be disturbed. Such a kicker pulse can be synthesized by ten harmonic modes of the 47.63 MHz kicker pulse repetition frequency, using up to four quarter wavelength resonator (QWR) based deflecting cavities. In this paper, several methods to synthesize such a kicker waveform will be discussed and a comparison of their beamdynamics performance is made using ELEGANT. Four QWR cavities are envisaged with high transverse shunt impedance requiring less than 100 W of total rf power for a Flat-Top kick pulse. Multipole fields due to the asymmetry of this type of cavity are analyzed. The transverse emittance growth due to the sextupole component is simulated in ELEGANT. Off-axis injection and extraction issues and beam optics using a multicavity kick-drift scheme will also be discussed. C1 [Huang, Yulu] Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China. [Huang, Yulu; Wang, Haipeng; Rimmer, Robert A.; Wang, Shaoheng; Guo, Jiquan] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Huang, Yulu] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. RP Wang, HP (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM haipeng@jlab.org FU Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX Work supported by Jefferson Science Associates, LLC under U.S. DOE. Contract No. DE-AC05-06OR23177. The authors acknowledge the useful previous works on the harmonic kicker concept, and especially thank Amy Sy for the helpful discussion on the kicker waveform schemes and ELEGANT tracking, and Subashini de Silva for the help on the multipole field coefficient calculation. NR 28 TC 0 Z9 0 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD AUG 22 PY 2016 VL 19 IS 8 AR 084201 DI 10.1103/PhysRevAccelBeams.19.084201 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU1ZR UT WOS:000382010300001 ER PT J AU Mayers, MZ Hybertsen, MS Reichman, DR AF Mayers, Matthew Z. Hybertsen, Mark S. Reichman, David R. TI Description of quasiparticle and satellite properties via cumulant expansions of the retarded one-particle Green's function SO PHYSICAL REVIEW B LA English DT Article ID RANDOM-PHASE-APPROXIMATION; SELF-CONSISTENT GW; ELECTRON-GAS; SPECTRAL FUNCTIONS; ENERGIES; METALS; SOLIDS AB A cumulant-based GW approximation for the retarded one-particle Green's function is proposed, motivated by an exact relation between the improper Dyson self-energy and the cumulant generating function. Qualitative aspects of this method are explored within a simple one-electron independent phonon model, where it is seen that the method preserves the energy moment of the spectral weight while also reproducing the exact Green's function in the weak-coupling limit. For the three-dimensional electron gas, this method predicts multiple satellites at the bottom of the band, albeit with inaccurate peak spacing. However, its quasiparticle properties and correlation energies are more accurate than both previous cumulantmethods and standard G(0)W(0). Our results point to features that may be exploited within the framework of cumulant-based methods and suggest promising directions for future exploration and improvements of cumulant-based GW approaches. C1 [Mayers, Matthew Z.; Reichman, David R.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Hybertsen, Mark S.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Mayers, MZ (reprint author), Columbia Univ, Dept Chem, New York, NY 10027 USA. FU National Science Foundation [DGE-11-44155]; US DOE Office of Science User Facility at Brookhaven National Laboratory [DE-SC0012704] FX We thank J. Kas for numerous helpful discussions and aid with the implementation of numerics. M.Z.M. is supported by a fellowship from the National Science Foundation under Grant No. DGE-11-44155. Part of this work was done using resources from the Center for Functional Nanomaterials, which is a US DOE Office of Science User Facility at Brookhaven National Laboratory under Contract No. DE-SC0012704 (M.S.H.). NR 46 TC 1 Z9 1 U1 9 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 22 PY 2016 VL 94 IS 8 AR 081109 DI 10.1103/PhysRevB.94.081109 PG 6 WC Physics, Condensed Matter SC Physics GA DU0JQ UT WOS:000381889700001 ER PT J AU Daigle, S Kelly, KJ Champagne, AE Buckner, MQ Iliadis, C Howard, C AF Daigle, S. Kelly, K. J. Champagne, A. E. Buckner, M. Q. Iliadis, C. Howard, C. TI Measurement of the E-r(c.m.)=259 ke V resonance in the N-14(p,gamma)O-15 reaction SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; LIGHT-NUCLEI; SOLAR NEUTRINOS; CROSS-SECTION; ENERGY-LEVELS; S-FACTOR; GAMMA)O-15; N-14(P; DETECTOR; SYSTEM AB The N-14(p,gamma)(15) O reaction regulates the power generated by the CN cycle and thus impacts the structure and evolution of every star at some point in its life. The lowest positive-energy resonance in this reaction is located at E-r(c.m.) = 259 keV, too high in energy to strongly influence quiescent stellar burning. However, the strength of this resonance is used as a cross-section normalization for lower-energy measurements of this reaction. We report on new measurements of the energy, strength, and gamma-ray branching ratios for the 259-keV resonance, using different detection and data-analysis schemes. We have also reevaluated previous results, where possible. Our new recommended strength of omega gamma = 12.6(3) meV is in agreement with the previous value of 13.1(6) meV, but is more precise and thus provides a more reliable normalization for low-energy (p,gamma) measurements. C1 [Daigle, S.] Univ N Carolina, Chapel Hill, NC 27599 USA. Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Daigle, S.] NASA Marshall Space Flight Ctr, NASA Postdoctoral Program, Huntsville, AL 35812 USA. [Buckner, M. Q.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Howard, C.] Nordion, 447 March Rd, Kanata, ON K2K 1X8, Canada. RP Daigle, S (reprint author), Univ N Carolina, Chapel Hill, NC 27599 USA.; Daigle, S (reprint author), NASA Marshall Space Flight Ctr, NASA Postdoctoral Program, Huntsville, AL 35812 USA. EM stephen.daigle@nasa.gov FU US Department of Energy [DE-FG02-97ER41041]; U.S. Department of Energy National Nuclear Security Administration [DE-FC52-08NA28752] FX This work was supported in part by the US Department of Energy under Contract No. DE-FG02-97ER41041 and by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-FC52-08NA28752. We would like to thank J. R. Dermigny for his assistance with the fraction fits. NR 59 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 025803 DI 10.1103/PhysRevC.94.025803 PG 13 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200008 ER PT J AU Hoffman, CR Kay, BP Schiffer, JP AF Hoffman, C. R. Kay, B. P. Schiffer, J. P. TI Ordering of the 0d(5/2) and 1s(1/2) proton levels in light nuclei SO PHYSICAL REVIEW C LA English DT Article ID ENERGY-LEVELS; STATES; HALOS; N-13; B-9 AB A survey of the available single-proton data in A <= 17 nuclei was completed. These data, along with calculations using a Woods-Saxon potential, show that the ordering of the 0d(5/2) and 1s(1/2) proton orbitals are determined primarily by the proximity of the s-state proton energy to the Coulomb barrier. This is analogous to the dependence of the corresponding neutron orbitals in proximity to the neutron threshold, which was previously discussed. C1 [Hoffman, C. R.; Kay, B. P.; Schiffer, J. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Hoffman, CR (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM crhoffman@anl.gov; kay@anl.gov; schiffer@anl.gov RI Kay, Benjamin/F-3291-2011 OI Kay, Benjamin/0000-0002-7438-0208 FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX The authors thank a number of colleagues for helpful discussions. We also appreciate the helpful comments on the manuscript from P. W. Zhao, S. Bottoni, and D. Santiago-Gonzalez. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 38 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 024330 DI 10.1103/PhysRevC.94.024330 PG 8 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200002 ER PT J AU Hota, SS Tandel, SK Chowdhury, P Ahmad, I Carpenter, MP Chiara, CJ Greene, JP Hoffman, CR Jackson, EG Janssens, RVF Kay, BP Khoo, TL Kondev, FG Lakshmi, S Lalkovski, S Lauritsen, T Lister, CJ McCutchan, EA Moran, K Peterson, D Shirwadkar, U Seweryniak, D Stefanescu, I Toh, Y Zhu, S AF Hota, S. S. Tandel, S. K. Chowdhury, P. Ahmad, I. Carpenter, M. P. Chiara, C. J. Greene, J. P. Hoffman, C. R. Jackson, E. G. Janssens, R. V. F. Kay, B. P. Khoo, T. L. Kondev, F. G. Lakshmi, S. Lalkovski, S. Lauritsen, T. Lister, C. J. McCutchan, E. A. Moran, K. Peterson, D. Shirwadkar, U. Seweryniak, D. Stefanescu, I. Toh, Y. Zhu, S. TI Population and decay of a K-pi=8(-) two-quasineutron isomer in Pu-244 SO PHYSICAL REVIEW C LA English DT Article ID SUPERHEAVY ELEMENTS; HEAVY-ELEMENTS; IN-BEAM; NUCLEI; SPECTROSCOPY; PU; STABILITY; STATES AB The decay of a K-pi = 8(-) isomer in Pu-244 and the collective band structures populating the isomer were studied using deep inelastic excitations with Ti-47 and Pb-208 beams, respectively. Precise measurements of M1/E2 branching ratios in the band confirm a 9/2(-)[734](nu)circle times 7/2(+)[624](nu) configuration assignment for the isomer, validating the systematics of K-pi = 8(-), two-quasineutron isomers observed in even-Z, N = 150 isotones. These isomers around the deformed shell gap at N = 152 provide critical benchmarks for theoretical predictions of single-particle energies in this gateway region to superheavy nuclei. C1 [Hota, S. S.; Tandel, S. K.; Chowdhury, P.; Jackson, E. G.; Lakshmi, S.; Lister, C. J.; Moran, K.; Shirwadkar, U.] Univ Massachusetts, Dept Phys, Lowell, MA 01854 USA. [Ahmad, I.; Carpenter, M. P.; Chiara, C. J.; Greene, J. P.; Hoffman, C. R.; Lauritsen, T.; Lister, C. J.; McCutchan, E. A.; Peterson, D.; Seweryniak, D.; Stefanescu, I.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Chiara, C. J.; Janssens, R. V. F.; Kay, B. P.; Khoo, T. L.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Chiara, C. J.; Seweryniak, D.; Stefanescu, I.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Lalkovski, S.] Univ Sofia, Sofia 1164, Bulgaria. [Toh, Y.] Japan Atom Energy Agcy, Naka, Ibaraki 3191195, Japan. [Hota, S. S.] Australian Natl Univ, Dept Nucl Phys, RSPE, Canberra, ACT 2601, Australia. [Tandel, S. K.] UM DAE Ctr Excellence Basic Sci, Bombay 400098, Maharashtra, India. [Chiara, C. J.] Army Res Lab, Adelphi, MD 20783 USA. [Lakshmi, S.; Shirwadkar, U.] Radiat Monitoring Devices Inc, Watertown, MA 02472 USA. [McCutchan, E. A.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Chowdhury, P (reprint author), Univ Massachusetts, Dept Phys, Lowell, MA 01854 USA. EM partha_chowdhury@uml.edu RI Kay, Benjamin/F-3291-2011 OI Kay, Benjamin/0000-0002-7438-0208 FU Office of Basic Energy Science, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-94ER40848, DE-FG02-94ER40834, DE-AC02-06CH11357]; National Science Foundation [PHY-1203100] FX The trans-plutonium element production facilities at Oak Ridge National Laboratory, supported by the Office of Basic Energy Science, U.S. Department of Energy, is acknowledged for providing enriched isotopic material for the targets. This work is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Grants No. DE-FG02-94ER40848 and No. DE-FG02-94ER40834, and Contract No. DE-AC02-06CH11357, and the National Science Foundation under Grant No. PHY-1203100. This research used resources of the ATLAS facility at ANL, which is a DOE Office of Science user facility. NR 36 TC 0 Z9 0 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 021303 DI 10.1103/PhysRevC.94.021303 PG 5 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200001 ER PT J AU Loizides, C AF Loizides, C. TI Glauber modeling of high-energy nuclear collisions at the subnucleon level SO PHYSICAL REVIEW C LA English DT Article ID PROTON CROSS-SECTION; HEAVY-ION COLLISIONS; ROOT-S=7 TEV; ELECTRON-SCATTERING; INITIAL-STATE; FRAMEWORK; QUARK AB Glauber models based on nucleon-nucleon interactions are commonly used to characterize the initial state in high-energy nuclear collisions and the dependence of its properties on impact parameter or number of participating nucleons. In this paper, an extension to the Glauber model is presented, which accounts for an arbitrary number of effective subnucleon degrees of freedom, or active constituents, in the nucleons. Properties of the initial state, such as the number of constituent participants and collisions, as well as eccentricity and triangularity, are calculated and systematically compared for different assumptions of how to distribute the subnuclear degrees of freedom and for various collision systems. It is demonstrated that at high collision energy the number of produced particles scales with an average number of subnucleon degrees of freedom of between 3 and 5. The source codes for the constituent Monte Carlo Glauber extension, as well as for the calculation of the overlap area and participant density in a standard Glauber model, are made publicly available. C1 [Loizides, C.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Loizides, C (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-05CH11231] FX I would like to thank J. Schukraft and S. Sorensen for interesting discussions. This work is supported in part by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-05CH11231. NR 49 TC 5 Z9 5 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 024914 DI 10.1103/PhysRevC.94.024914 PG 12 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200005 ER PT J AU McGlinchey, D Nagle, JL Perepelitsa, DV AF McGlinchey, D. Nagle, J. L. Perepelitsa, D. V. TI Consequences of high-x proton size fluctuations in small collision systems at root S-NN=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR COLLISIONS; LEAD COLLISIONS; ATLAS DETECTOR; DEPENDENCE; CENTRALITY; TEV; PSEUDORAPIDITY AB Recent measurements of jet production rates at large transverse momentum (pT) in the collisions of small projectiles with large nuclei at the BNL Relativistic Heavy Ion Collider (RHIC) and the CERN Large Hadron Collider indicate that they have an unexpected relationship with estimates of the collision centrality. One compelling interpretation of the data is that they capture an x(p)-dependent decrease in the average interaction strength of the nucleon in the projectile undergoing a hard scattering. A weakly interacting or "shrinking" nucleon in the projectile strikes fewer nucleons in the nucleus, resulting in a particular pattern of centrality-dependent modifications to high-pT processes. We describe a simple one-parameter geometric implementation of this picture within a modified Monte Carlo Glauber model tuned to d + Au jet data, and explore two of its major consequences. First, the model predicts a particular projectile-species effect on the centrality dependence at high x(p), opposite to that expected from a final state energy loss effect. Second, we find that some of the large centrality dependence observed for forward dihadron production in d + Au collisions at RHIC may arise from the physics of the "shrinking" projectile nucleon, in addition to impact parameter dependent shadowing or saturation effects at low nuclear x. We conclude that analogous measurements in recently collected p + Au and He-3 + Au collision data at RHIC can provide a unique test of these predictions. C1 [McGlinchey, D.; Nagle, J. L.] Univ Colorado, Boulder, CO 80309 USA. [Perepelitsa, D. V.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP McGlinchey, D (reprint author), Univ Colorado, Boulder, CO 80309 USA. FU Division of Nuclear Physics of the U.S. Department of Energy [DE-FG02-03ER41244]; U.S. Department of Energy [DE-SC0012704] FX D.M. and J.L.N. acknowledge funding from the Division of Nuclear Physics of the U.S. Department of Energy under Grant No. DE-FG02-03ER41244. D.V.P. acknowledges funding from the U.S. Department of Energy under Contract No. DE-SC0012704. D.V.P. also acknowledges Mark Strikman for useful discussions. NR 34 TC 0 Z9 0 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 024915 DI 10.1103/PhysRevC.94.024915 PG 9 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200006 ER PT J AU Tveten, GM Spyrou, A Schwengner, R Naqvi, F Larsen, AC Eriksen, TK Garrote, FLB Bernstein, LA Bleuel, DL Campo, LC Guttormsen, M Giacoppo, F Gorgen, A Hagen, TW Hadynska-Klek, K Klintefjord, M Meyer, BS Nyhus, HT Renstrom, T Rose, SJ Sahin, E Siem, S Tornyi, TG AF Tveten, G. M. Spyrou, A. Schwengner, R. Naqvi, F. Larsen, A. C. Eriksen, T. K. Garrote, F. L. Bello Bernstein, L. A. Bleuel, D. L. Campo, L. Crespo Guttormsen, M. Giacoppo, F. Gorgen, A. Hagen, T. W. Hadynska-Klek, K. Klintefjord, M. Meyer, B. S. Nyhus, H. T. Renstrom, T. Rose, S. J. Sahin, E. Siem, S. Tornyi, T. G. TI Completing the nuclear reaction puzzle of the nucleosynthesis of Mo-92 SO PHYSICAL REVIEW C LA English DT Article ID GIANT-DIPOLE RESONANCE; P-PROCESS; LEVEL DENSITIES; MODEL-CALCULATIONS; STRENGTH FUNCTION; GAMMA; LIBRARY; STARS; ASTROPHYSICS; SYSTEMATICS AB One of the greatest questions for modern physics to address is how elements heavier than iron are created in extreme astrophysical environments. A particularly challenging part of that question is the creation of the so-called p-nuclei, which are believed to be mainly produced in some types of supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions. In this work, we present for the first time measurements on the nuclear level density and average gamma strength function of Mo-92. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. Our data provide stringent constraints on the Nb-91(p,gamma)Mo-92 reaction rate, which is the last unmeasured reaction in the nucleosynthesis puzzle of Mo-92. Based on our results, we conclude that the Mo-92 abundance anomaly is not due to the nuclear physics input to astrophysical model calculations. C1 [Tveten, G. M.; Larsen, A. C.; Eriksen, T. K.; Garrote, F. L. Bello; Campo, L. Crespo; Guttormsen, M.; Giacoppo, F.; Gorgen, A.; Hagen, T. W.; Hadynska-Klek, K.; Klintefjord, M.; Nyhus, H. T.; Renstrom, T.; Rose, S. J.; Sahin, E.; Siem, S.] Univ Oslo, Dept Phys, NO-0316 Oslo, Norway. [Spyrou, A.; Naqvi, F.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Spyrou, A.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Spyrou, A.; Naqvi, F.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Schwengner, R.] Helmholtz Zentrum Dresden Rossendorf, D-01328 Dresden, Germany. [Eriksen, T. K.; Tornyi, T. G.] Australian Natl Univ, Res Sch Phys & Engn, Dept Nucl Phys, Canberra, ACT 2601, Australia. [Bernstein, L. A.; Bleuel, D. L.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Giacoppo, F.] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Giacoppo, F.] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Hadynska-Klek, K.] Lab Nazl Legnaro Padova, INFN, I-35020 Legnaro, Italy. [Meyer, B. S.] Clemson Univ, Dept Phys & Astron, Clemson, SC 29634 USA. RP Tveten, GM (reprint author), Univ Oslo, Dept Phys, NO-0316 Oslo, Norway. EM g.m.tveten@fys.uio.no RI Larsen, Ann-Cecilie/C-8742-2014 OI Larsen, Ann-Cecilie/0000-0002-2188-3709 FU The Research Council of Norway [222287]; ERC-STG [637686]; National Science Foundation [PHY1102511, PHY 1430152, PHY 1350234]; U.S. Department of Energy [DE-AC52-07NA27344, DE-AC02-05CH11231] FX We give special thanks to J. C. Muller, A. Semchenkov, and J. C. Wikne for providing the high-quality beam and excellent experimental conditions. Lawrence Berkeley National Laboratory is thanked for lending us the 92Mo target. G.M.T. gratefully acknowledges funding of this research from The Research Council of Norway, Project Grant No. 222287. A.C.L. acknowledges funding from ERC-STG-2014 Grant Agreement No. 637686. This work was supported by the National Science Foundation under Grants No. PHY1102511 (NSCL), No. PHY 1430152 (JINA-CEE), and No. PHY 1350234 (CAREER). This work was performed under the auspices of the U.S. Department of Energy DE-AC52-07NA27344 (LLNL) and DE-AC02-05CH11231 (LBNL). NR 70 TC 0 Z9 0 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 22 PY 2016 VL 94 IS 2 AR 025804 DI 10.1103/PhysRevC.94.025804 PG 7 WC Physics, Nuclear SC Physics GA DU0KL UT WOS:000381892200009 ER PT J AU Zequine, C Ranaweera, CK Wang, Z Singh, S Tripathi, P Srivastava, ON Gupta, BK Ramasamy, K Kahol, PK Dvornic, PR Gupta, RK AF Zequine, Camila Ranaweera, C. K. Wang, Z. Singh, Sweta Tripathi, Prashant Srivastava, O. N. Gupta, Bipin Kumar Ramasamy, K. Kahol, P. K. Dvornic, P. R. Gupta, Ram K. TI High Performance and Flexible Supercapacitors based on Carbonized Bamboo Fibers for Wide Temperature Applications SO SCIENTIFIC REPORTS LA English DT Article ID HIGH-ENERGY DENSITY; DOUBLE-LAYER CAPACITORS; ACTIVATED CARBON; ELECTRODE MATERIALS; POROUS CARBON; PERFORMANCE; COMPOSITE; RESIDUE; LEAVES; WASTE AB High performance carbonized bamboo fibers were synthesized for a wide range of temperature dependent energy storage applications. The structural and electrochemical properties of the carbonized bamboo fibers were studied for flexible supercapacitor applications. The galvanostatic charge-discharge studies on carbonized fibers exhibited specific capacity of similar to 510F/g at 0.4 A/g with energy density of 54 Wh/kg. Interestingly, the carbonized bamboo fibers displayed excellent charge storage stability without any appreciable degradation in charge storage capacity over 5,000 charge-discharge cycles. The symmetrical supercapacitor device fabricated using these carbonized bamboo fibers exhibited an areal capacitance of similar to 1.55 F/cm(2) at room temperature. In addition to high charge storage capacity and cyclic stability, the device showed excellent flexibility without any degradation to charge storage capacity on bending the electrode. The performance of the supercapacitor device exhibited similar to 65% improvement at 70 degrees C compare to that at 10 degrees C. Our studies suggest that carbonized bamboo fibers are promising candidates for stable, high performance and flexible supercapacitor devices. C1 [Zequine, Camila; Ranaweera, C. K.; Wang, Z.; Dvornic, P. R.; Gupta, Ram K.] Pittsburg State Univ, Dept Chem, 1701 S Broadway, Pittsburg, KS 66762 USA. [Singh, Sweta; Tripathi, Prashant; Srivastava, O. N.] Banaras Hindu Univ, Dept Phys, Varanasi 221004, Uttar Pradesh, India. [Gupta, Bipin Kumar] Natl Phys Lab, CSIR, Dr KS Krishnan Rd, New Delhi 110012, India. [Ramasamy, K.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Kahol, P. K.] Pittsburg State Univ, Dept Phys, 1701 S Broadway, Pittsburg, KS 66762 USA. RP Gupta, RK (reprint author), Pittsburg State Univ, Dept Chem, 1701 S Broadway, Pittsburg, KS 66762 USA. EM ramguptamsu@gmail.com FU Polymer Chemistry Initiative, Pittsburg State University; National Science Foundation [EPS-0903806] FX Dr. Ram K. Gupta expresses his sincere acknowledgment to the Polymer Chemistry Initiative, Pittsburg State University for providing financial and research support. This material is based upon work partly supported by the National Science Foundation under Award No. EPS-0903806 and matching support from the State of Kansas through the Kansas Board of Regents. NR 29 TC 0 Z9 0 U1 27 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 22 PY 2016 VL 6 AR 31704 DI 10.1038/srep31704 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT7XM UT WOS:000381701600001 PM 27546225 ER PT J AU Li, ML Kim, DW Gu, S Parkinson, DY Barnard, H Tu, KN AF Li, Menglu Kim, Dong Wook Gu, Sam Parkinson, Dilworth Y. Barnard, Harold Tu, K. N. TI Joule heating induced thermomigration failure in un-powered microbumps due to thermal crosstalk in 2.5D IC technology SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SOLDER JOINTS; INTEGRATED-CIRCUITS AB Thermal-crosstalk induced thermomigration failure in un-powered microbumps has been found in 2.5D integrated circuit (IC) circuit. In 2.5D IC, a Si interposer was used between a polymer substrate and a device chip which has transistors. The interposer has no transistors. If transistors are added to the interposer chip, it becomes 3D IC. In our test structure, there are two Si chips placed horizontally on a Si interposer. The vertical connections between the interposer and the Si chips are through microbumps. We powered one daisy chain of the microbumps under one Si chip; however, the un-powered microbumps in the neighboring chip are failed with big holes in the solder layer. We find that Joule heating from the powered microbumps is transferred horizontally to the bottom of the neighboring un-powered microbumps, and creates a large temperature gradient, in the order of 1000 degrees C/cm, through the un-powered microbumps in the neighboring chip, so the latter failed by thermomigration. In addition, we used synchrotron radiation tomography to compare three sets of microbumps in the test structure: microbumps under electromigration, microbumps under thermomigration, and microbumps under a constant temperature thermal annealing. The results show that the microbumps under thermomigration have the largest damage. Furthermore, simulation of temperature distribution in the test structure supports the finding of thermomigration. Published by AIP Publishing. C1 [Li, Menglu; Tu, K. N.] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. [Kim, Dong Wook; Gu, Sam] Qualcomm, San Diego, CA 92121 USA. [Parkinson, Dilworth Y.; Barnard, Harold] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Tu, KN (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. EM kntu@ucla.edu OI Li, Menglu/0000-0001-9656-8087 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. All of the authors acknowledge the technical support of Sergey Prikhodko at MSE, UCLA for SEM and Noah Bodzin at nanolab, UCLA for FIB study. NR 22 TC 1 Z9 1 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2016 VL 120 IS 7 AR 075105 DI 10.1063/1.4961219 PG 10 WC Physics, Applied SC Physics GA DW6VA UT WOS:000383788300028 ER PT J AU Robinson, ZR Jernigan, GG Wheeler, VD Hernandez, SC Eddy, CR Mowll, TR Ong, EW Ventrice, CA Geisler, H Pletikosic, I Yang, H Valla, T AF Robinson, Zachary R. Jernigan, Glenn G. Wheeler, Virginia D. Hernandez, Sandra C. Eddy, Charles R., Jr. Mowll, Tyler R. Ong, Eng Wen Ventrice, Carl A., Jr. Geisler, Heike Pletikosic, Ivo Yang, Hongbo Valla, Tonica TI Growth and characterization of Al2O3 films on fluorine functionalized epitaxial graphene SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ATOMIC LAYER DEPOSITION; SILICON-CARBIDE; TRANSISTORS; OXIDES AB Intelligent engineering of graphene-based electronic devices on SiC(0001) requires a better understanding of processes used to deposit gate-dielectric materials on graphene. Recently, Al2O3 dielectrics have been shown to form conformal, pinhole-free thin films by functionalizing the top surface of the graphene with fluorine prior to atomic layer deposition (ALD) of the Al2O3 using a trimethylaluminum (TMA) precursor. In this work, the functionalization and ALD-precursor adsorption processes have been studied with angle-resolved photoelectron spectroscopy, low energy electron diffraction, and X-ray photoelectron spectroscopy. It has been found that the functionalization process has a negligible effect on the electronic structure of the graphene, and that it results in a twofold increase in the adsorption of the ALD-precursor. In situ TMA-dosing and XPS studies were also performed on three different Si(100) substrates that were terminated with H, OH, or dangling Si-bonds. This dosing experiment revealed that OH is required for TMA adsorption. Based on those data along with supportive in situ measurements that showed F-functionalization increases the amount of oxygen (in the form of adsorbed H2O) on the surface of the graphene, a model for TMA-adsorption on graphene is proposed that is based on a reaction of a TMA molecule with OH. Published by AIP Publishing. C1 [Robinson, Zachary R.] Coll Brockport, Dept Phys, Brockport, NY 14420 USA. [Jernigan, Glenn G.; Wheeler, Virginia D.; Hernandez, Sandra C.; Eddy, Charles R., Jr.] US Naval Res Lab, Washington, DC 20375 USA. [Mowll, Tyler R.; Ong, Eng Wen] SUNY Albany, Coll Nanoscale Sci & Engn, Albany, NY 12203 USA. [Ventrice, Carl A., Jr.] SUNY Polytech Inst, Coll Nanoscale Sci, Albany, NY 12203 USA. [Geisler, Heike] SUNY Coll Oneonta, Dept Chem & Biochem, Oneonta, NY 13820 USA. [Pletikosic, Ivo; Yang, Hongbo; Valla, Tonica] Brookhaven Natl Lab, Brookhaven, NY 11973 USA. RP Robinson, ZR (reprint author), Coll Brockport, Dept Phys, Brockport, NY 14420 USA. EM ZRobinso@Brockport.edu FU Office of Naval Research; National Science Foundation [DMR-1006411]; BNL [DE-SC0012704]; ASEE FX Work at the U.S. Naval Research Laboratory is supported by the Office of Naval Research. The NRL group and Z.R.R. acknowledge the postdoctoral for postdoctoral support. The SUNY Poly/UAlbany group acknowledges the support from the National Science Foundation (No. DMR-1006411). The ARPES experiments were performed under the BNL Grant No. DE-SC0012704. NR 20 TC 0 Z9 0 U1 17 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD AUG 21 PY 2016 VL 120 IS 7 AR 075302 DI 10.1063/1.4960803 PG 7 WC Physics, Applied SC Physics GA DW6VA UT WOS:000383788300030 ER PT J AU Hlova, IZ Castle, A Goldston, JF Gupta, S Prost, T Kobayashi, T Chumbley, LS Pruski, M Pecharsky, VK AF Hlova, Ihor Z. Castle, Andra Goldston, Jennifer F. Gupta, Shalabh Prost, Timothy Kobayashi, Takeshi Chumbley, L. Scott Pruski, Marek Pecharsky, Vitalij K. TI Solvent- and catalyst-free mechanochemical synthesis of alkali metal monohydrides SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID HYDRIDES; STORAGE; NMR; KINETICS AB Alkali metal monohydrides, AH (A = Li-Cs) have been synthesized in quantitative yields at room temperature by reactive milling of alkali metals in the presence of hydrogen gas at 200 bar or less. The mechanochemical approach reported here eliminates problems associated with the malleability of alkali metals especially Li, Na, and K - and promotes effective solid-gas reactions, ensuring their completion. This is achieved by incorporating a certain volume fraction of the corresponding hydride powder as a process control agent, which allows continuous and efficient milling primarily by coating the surface of metal particles, effectively blocking cold welding. Formation of high-purity crystalline monohydrides has been confirmed by powder X-ray diffraction, solid-state NMR spectroscopy, and volumetric analyses of reactively desorbed H-2 from as-milled samples. The proposed synthesis method is scalable and particularly effective for extremely air-sensitive materials, such as alkali and alkaline earth metal hydrides. The technique may also be favorable for production in continuous reactors operating at room temperature, thereby reducing the total processing time, energy consumption and, hence, the cost of production of these hydrides or their derivatives and composites. C1 [Hlova, Ihor Z.; Castle, Andra; Goldston, Jennifer F.; Gupta, Shalabh; Prost, Timothy; Kobayashi, Takeshi; Chumbley, L. Scott; Pruski, Marek; Pecharsky, Vitalij K.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Castle, Andra; Goldston, Jennifer F.; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Hlova, Ihor Z.; Prost, Timothy; Chumbley, L. Scott; Pecharsky, Vitalij K.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Gupta, S (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM Shalabh@ameslab.gov FU Division of Materials Sciences and Engineering of Basic Energy Sciences Program of the Office of Science of the U.S. Department of Energy [DE-AC02-07CH11358]; Iowa State University FX Research supported by the Division of Materials Sciences and Engineering of Basic Energy Sciences Program of the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-07CH11358 with Iowa State University. NR 32 TC 0 Z9 0 U1 12 U2 15 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 EI 2050-7496 J9 J MATER CHEM A JI J. Mater. Chem. A PD AUG 21 PY 2016 VL 4 IS 31 BP 12188 EP 12196 DI 10.1039/c6ta04391g PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA DU3FB UT WOS:000382095100025 ER PT J AU Bender, AN Kennedy, J Ade, PAR Basu, K Bertoldi, F Burkutean, S Clarke, J Dahlin, D Dobbs, M Ferrusca, D Flanigan, D Halverson, NW Holzapfel, WL Horellou, C Johnson, BR Kermish, ZD Klein, M Kneissl, R Lanting, T Lee, AT Mehl, J Menten, KM Muders, D Nagarajan, A Pacaud, F Reichardt, CL Richards, PL Schaaf, R Schwan, D Sommer, MW Spieler, H Tucker, C Westbrook, B AF Bender, A. N. Kennedy, J. Ade, P. A. R. Basu, K. Bertoldi, F. Burkutean, S. Clarke, J. Dahlin, D. Dobbs, M. Ferrusca, D. Flanigan, D. Halverson, N. W. Holzapfel, W. L. Horellou, C. Johnson, B. R. Kermish, Z. D. Klein, M. Kneissl, R. Lanting, T. Lee, A. T. Mehl, J. Menten, K. M. Muders, D. Nagarajan, A. Pacaud, F. Reichardt, C. L. Richards, P. L. Schaaf, R. Schwan, D. Sommer, M. W. Spieler, H. Tucker, C. Westbrook, B. TI Galaxy cluster scaling relations measured with APEX-SZ SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: clusters: general; cosmic background radiation; cosmology: observations ID SOUTH-POLE TELESCOPE; X-RAY OBSERVATIONS; SUNYAEV-ZELDOVICH; INTRACLUSTER MEDIUM; COSMOLOGICAL CONSTRAINTS; OBSERVED GROWTH; DATA REDUCTION; CHANDRA; SAMPLE; MASS AB We present thermal Sunyaev-Zel'dovich effect (SZE) measurements for 42 galaxy clusters observed at 150 GHz with the APEX-SZ experiment. For each cluster, we model the pressure profile and calculate the integrated Comptonization Y to estimate the total thermal energy of the intraclustermedium (ICM). We compare the measured Y values to X-ray observables of the ICM from the literature (cluster gas mass M-gas, temperature T-X, and Y-X = MgasTX) that relate to total cluster mass. We measure power-law scaling relations, including an intrinsic scatter, between the SZE and X-ray observables for three subsamples within the set of 42 clusters that have uniform X-ray analysis in the literature. We observe that differences between these X-ray analyses introduce significant variance into the measured scaling relations, particularly affecting the normalization. For all three subsamples, we find results consistent with a selfsimilarmodel of cluster evolution dominated by gravitational effects. Comparing to predictions from numerical simulations, these scaling relations prefer models that include cooling and feedback in the ICM. Lastly, we measure an intrinsic scatter of similar to 28 per cent in the Y - Y-X scaling relation for all three subsamples. C1 [Bender, A. N.; Kennedy, J.; Dobbs, M.; Lanting, T.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Bender, A. N.; Halverson, N. W.] Univ Colorado, Ctr Astrophys & Space Astron, Dept Astrophys & Planetary Sci, Campus Box 391, Boulder, CO 80309 USA. [Ade, P. A. R.; Tucker, C.] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3YB, S Glam, Wales. [Basu, K.; Bertoldi, F.; Burkutean, S.; Klein, M.; Nagarajan, A.; Pacaud, F.; Schaaf, R.; Sommer, M. W.] Univ Bonn, Argelander Inst Astron, D-53121 Bonn, Germany. [Clarke, J.; Flanigan, D.; Halverson, N. W.; Holzapfel, W. L.; Lee, A. T.; Mehl, J.; Reichardt, C. L.; Richards, P. L.; Schwan, D.; Westbrook, B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Clarke, J.] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Dahlin, D.; Horellou, C.] Chalmers, Onsala Space Observ, Dept Earth & Space Sci, SE-43992 Onsala, Sweden. [Ferrusca, D.] Inst Nacl Astrofis Opt & Electr, Luis Enrique Erro 1, Puebla 72840, Mexico. [Halverson, N. W.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Johnson, B. R.] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Kermish, Z. D.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Kneissl, R.] European Southern Observ, Alonso Cordova 3107, Santiago, Chile. [Kneissl, R.] Joint ALMA, Atacama Large Millimeter Submillimeter Array, Alonso Cordova 3107, Santiago, Chile. [Lee, A. T.; Spieler, H.] Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Menten, K. M.; Muders, D.] Max Planck Inst Radio Astron, D-53121 Bonn, Germany. RP Bender, AN (reprint author), McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada.; Bender, AN (reprint author), Univ Colorado, Ctr Astrophys & Space Astron, Dept Astrophys & Planetary Sci, Campus Box 391, Boulder, CO 80309 USA. EM abender@anl.gov OI Tucker, Carole/0000-0002-1851-3918 FU National Science Foundation [AST-0138348, AST-0709497]; Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Natural Sciences and Engineering Research Council of Canada; Canada Research Chairs programme; Canadian Institute for Advanced Research; DFG Transregio programme [TR33]; BMBF/DLR grant [50 OR 1117]; Barbro Osher pro Succia foundation; Swedish Research Council [2006-3356, 2009-4027]; German BMWi through the Verbundforschung [50 OR 1107]; Alfred P. Sloan Foundation FX We thank the staff at the APEX telescope site, at the time of observations led by David Rabanus and previously by Lars-Ake Nyman, for their dedicated and exceptional support. We also thank Bradford Benson for useful comments on a draft version of the manuscript as well as LBNL engineers John Joseph and Chinh Vu for their work on the readout electronics. APEX-SZ is funded by the National Science Foundation under Grant Nos. AST-0138348 and AST-0709497. Work at LBNL is supported by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Work at McGill is supported by the Natural Sciences and Engineering Research Council of Canada, the Canada Research Chairs programme, and the Canadian Institute for Advanced Research. This work has been partially supported by the DFG Transregio programme TR33 'The Dark Universe'. FP acknowledges support from the BMBF/DLR grant Nr. 50 OR 1117. CH acknowledges support from the Barbro Osher pro Succia foundation and from the Swedish Research Council under grants 2006-3356 and 2009-4027. MK acknowledges support by the German BMWi through the Verbundforschung under grant 50 OR 1107. NWH acknowledges support from the Alfred P. Sloan Foundation. NR 76 TC 1 Z9 1 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2016 VL 460 IS 4 BP 3432 EP 3446 DI 10.1093/mnras/stw1158 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DT8AV UT WOS:000381711100002 ER PT J AU Agarwal, B Johnson, JL Zackrisson, E Labbe, I van den Bosch, FC Natarajan, P Khochfar, S AF Agarwal, Bhaskar Johnson, Jarrett L. Zackrisson, Erik Labbe, Ivo van den Bosch, Frank C. Natarajan, Priyamvada Khochfar, Sadegh TI Detecting direct collapse black holes: making the case for CR7 SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: high-redshift; quasars: supermassive black holes; dark ages; reionization; first stars ID STAR-FORMATION RATES; DARK-MATTER HALOES; TO 8 GALAXIES; EARLY UNIVERSE; VIRIAL TEMPERATURES; SPECTRAL EVOLUTION; STELLAR MASSES; HIGH REDSHIFTS; RAPID GROWTH; 1ST STARS AB We propose that one of the sources in the recently detected system CR7 by Sobral et al. through spectrophotometric measurements at z=6.6 harbours a direct collapse black hole (DCBH). We argue that the LW radiation field required for direct collapse in source A is provided by sources B and C.By tracing the LW production history and star formation rate over cosmic time for the halo hosting CR7 in a ACDM universe, we demonstrate that a DCBH could have formed at z similar to 20. The spectrum of source A is well fit by nebular emission from primordial gas around a BH with MBH similar to 4.4x10(6)M(circle dot) accreting at a 40 per cent of the Eddington rate, which strongly supports our interpretation of the data. Combining these lines of evidence, we argue that CR7 might well be the first DCBH candidate. C1 [Agarwal, Bhaskar; van den Bosch, Frank C.; Natarajan, Priyamvada] Yale Univ, Dept Astron, 52 Hillhouse Ave,Steinbach Hall, New Haven, CT 06511 USA. [Johnson, Jarrett L.] Los Alamos Natl Lab, Theoret Div X, Los Alamos, NM 87545 USA. [Zackrisson, Erik] Uppsala Univ, Dept Phys & Astron, POB 515, SE-75120 Uppsala, Sweden. [Labbe, Ivo] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. [Khochfar, Sadegh] Univ Edinburgh, Inst Astron, Royal Observ, Edinburgh EH9 3HJ, Midlothian, Scotland. RP Agarwal, B (reprint author), Yale Univ, Dept Astron, 52 Hillhouse Ave,Steinbach Hall, New Haven, CT 06511 USA. EM bhaskar.agarwal@yale.edu FU NASA-NSF Theoretical and Computational Astrophysics Networks [1332858]; TCAN postdoctoral fellowship at Yale; Swedish Research Council [2011-5349]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX The authors would like to thank the anonymous referee whose suggestions greatly improved the paper. The authors would also like to thank David Sobral and Jorryt Matthee for their useful comments on the manuscript. BA would like to thank Pascal Oesch for his inputs that greatly helped in shaping the manuscript. BA would also like to thank Laura Morselli, Chervin Laporte and Jonny Elliott for their help during the preparation of this study. PN acknowledges support from a NASA-NSF Theoretical and Computational Astrophysics Networks award number 1332858. BA acknowledges support of a TCAN postdoctoral fellowship at Yale. E.Z. acknowledges research funding from the Swedish Research Council (project 2011-5349). Work at LANL was done under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract no. DE-AC52-06NA25396. NR 64 TC 7 Z9 7 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2016 VL 460 IS 4 BP 4003 EP 4010 DI 10.1093/mnras/stw1173 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DT8AV UT WOS:000381711100046 ER PT J AU Gil-Marin, H Percival, WJ Brownstein, JR Chuang, CH Grieb, JN Ho, S Kitaura, FS Maraston, C Prada, F Rodriguez-Torres, S Ross, AJ Samushia, L Schlegel, DJ Thomas, D Tinker, JL Zhao, GB AF Gil-Marin, Hector Percival, Will J. Brownstein, Joel R. Chuang, Chia-Hsun Grieb, Jan Niklas Ho, Shirley Kitaura, Francisco-Shu Maraston, Claudia Prada, Francisco Rodriguez-Torres, Sergio Ross, Ashley J. Samushia, Lado Schlegel, David J. Thomas, Daniel Tinker, Jeremy L. Zhao, Gong-Bo TI The clustering of galaxies in the SDSS-III Baryon Oscillation Spectroscopic Survey: RSD measurement from the LOS-dependent power spectrum of DR12 BOSS galaxies SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: haloes; cosmological parameters; cosmology: theory; large-scale structure of Universe ID DIGITAL SKY SURVEY; REDSHIFT SPACE DISTORTIONS; GROWTH-RATE; DATA RELEASE; ACOUSTIC-OSCILLATIONS; PERTURBATION-THEORY; GENERAL-RELATIVITY; CMASS GALAXIES; REAL-SPACE; FINAL DATA AB We measure and analyse the clustering of the Baryon Oscillation Spectroscopic Survey (BOSS) relative to the line of sight (LOS), for LOWZ and CMASS galaxy samples drawn from the final Data Release 12. The LOWZ sample contains 361 762 galaxies with an effective redshift of z(lowz) = 0.32, and the CMASS sample 777 202 galaxies with an effective redshift of z(cmass) = 0.57. From the power spectrum monopole and quadrupole moments around the LOS, we measure the growth of structure parameter f times the amplitude of dark matter density fluctuations sigma 8 by modelling the redshift-space distortion signal. When the geometrical Alcock-Paczynski effect is also constrained from the same data, we find joint constraints on f sigma(8), the product of the Hubble constant and the comoving sound horizon at the baryondrag epoch H(z) r(s)(z(d)), and the angular distance parameter divided by the sound horizon DA(z)/r(s)(zd). We find f(z(lowz)) sigma(8)(z(lowz)) = 0.394 +/- 0.062, D-A(zlowz)/r(s)(z(d)) = 6.35 +/- 0.19, H(z(lowz)) r(s)(z(d)) = (11.41 +/- 0.56) 103 km s(-1) for the LOWZ sample, and f( z(cmass)) sigma 8(z(cmass)) = 0.444 +/- 0.038, D-A(z(cmass))/r(s)(z(d)) = 9.42 +/- 0.15, H(z(cmass)) r(s)(z(d)) = (13.92 +/- 0.44) 103 km s-1 for the CMASS sample. We find general agreement with previous BOSS DR11 measurements. Assuming the Hubble parameter and angular distance parameter are fixed at fiducial +/- cold dark matter values, we find f( zlowz) sigma(8)( z(lowz))= 0.485 +/- 0.044 and f(z(cmass)) sigma(8)(z(cmass))= 0.436 +/- 0.022 for the LOWZ and CMASS samples, respectively. C1 [Gil-Marin, Hector; Percival, Will J.; Maraston, Claudia; Thomas, Daniel; Zhao, Gong-Bo] Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg, Portsmouth PO1 3FX, Hants, England. [Brownstein, Joel R.] Univ Utah, Dept Phys & Astron, 115 S 1400 E, Salt Lake City, UT 84112 USA. [Chuang, Chia-Hsun; Prada, Francisco; Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Inst Fis Teor UAM CSIC, E-28049 Madrid, Cantoblanco, Spain. [Grieb, Jan Niklas] Univ Munich, Univ Sternwarte Munchen, Scheiner Str 1, D-81679 Munich, Germany. [Grieb, Jan Niklas] Max Planck Inst Extraterr Phys, Postfach 1312,Giessenbachstr, D-85741 Garching, Germany. [Ho, Shirley] Carnegie Mellon Univ, McWilliams Ctr, Pittsburgh, PA 15213 USA. [Kitaura, Francisco-Shu] Leibniz Inst Astrophys AIP, Sternwarte 16, D-14482 Potsdam, Germany. [Prada, Francisco; Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Prada, Francisco] CSIC, Inst Astrofis Andalucia, Clorieta Astron, E-18080 Granada, Spain. [Rodriguez-Torres, Sergio] Campus Int Excellence UAM CSIC, E-28049 Madrid, Spain. [Ross, Ashley J.] Ohio State Univ, Ctr Cosmol & AstroParticle Phys, Columbus, OH 43210 USA. [Samushia, Lado] Kansas State Univ, Dept Phys, 116 Cardwell Hall, Manhattan, KS 66506 USA. [Samushia, Lado] Ilia State Univ, Natl Abastumani Astrophys Observ, 2A Kazbegi Ave, GE-1060 Tbilisi, Rep of Georgia. [Schlegel, David J.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Tinker, Jeremy L.] NYU, Ctr Cosmol & Particle Phys, Dept Phys, New York, NY 10003 USA. [Zhao, Gong-Bo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. RP Gil-Marin, H (reprint author), Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg, Portsmouth PO1 3FX, Hants, England. EM hector.gil@port.ac.uk RI Gil Marin, Hector/B-2013-2017 OI Gil Marin, Hector/0000-0003-0265-6217 FU UK Science and Technology Facilities Council [ST/I001204/1]; UK Science and Technology Facilities Research Council [ST/I001204/1]; European Research Council; Karl-Schwarzschild Program from the Leibniz Society; Spanish MICINNs Consolider-Ingenio Programme [MultiDark CSD2009-00064]; MINECO Centro de Excelencia Severo Ochoa Programme [SEV-2012-0249, AYA2014-60641-C2- 1-P]; Alfred P. Sloan Foundation; National Science Foundation; US Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX HGM is grateful for support from the UK Science and Technology Facilities Council through the grant ST/I001204/1. WJP is grateful for support from the UK Science and Technology Facilities Research Council through the grant ST/I001204/1, and the European Research Council through the grant 'Darksurvey'. FSK acknowledges the support of the Karl-Schwarzschild Program from the Leibniz Society. FSK, SRT, CC, and FP acknowledge support from the Spanish MICINNs Consolider-Ingenio 2010 Programme under grant MultiDark CSD2009-00064, MINECO Centro de Excelencia Severo Ochoa Programme under grant SEV-2012-0249, and grant AYA2014-60641-C2- 1-P. The massive production of all MultiDark Patchy BOSS DR12 mocks has been performed at the BSC Marenostrum supercomputer, the Hydra cluster at the Instituto de Fisica Teorica UAM/CSIC and NERSC at the Lawrence Berkeley National Laboratory.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the US Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 75 TC 12 Z9 12 U1 2 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2016 VL 460 IS 4 BP 4188 EP 4209 DI 10.1093/mnras/stw1096 PG 22 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DT8AV UT WOS:000381711100060 ER PT J AU Gil-Marin, H Percival, WJ Cuesta, AJ Brownstein, JR Chuang, CH Ho, S Kitaura, FS Maraston, C Prada, F Rodriguez-Torres, S Ross, AJ Schlegel, DJ Schneider, DP Thomas, D Tinker, JL Tojeiro, R Magana, MV Zhao, GB AF Gil-Marin, Hector Percival, Will J. Cuesta, Antonio J. Brownstein, Joel R. Chuang, Chia-Hsun Ho, Shirley Kitaura, Francisco-Shu Maraston, Claudia Prada, Francisco Rodriguez-Torres, Sergio Ross, Ashley J. Schlegel, David J. Schneider, Donald P. Thomas, Daniel Tinker, Jeremy L. Tojeiro, Rita Vargas Magana, Mariana Zhao, Gong-Bo TI The clustering of galaxies in the SDSS-III Baryon Oscillation Spectroscopic Survey: BAO measurement from the LOS-dependent power spectrum of DR12 BOSS galaxies SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: haloes; cosmological parameters; cosmology: theory; large-scale structure of Universe ID DIGITAL SKY SURVEY; ACOUSTIC-OSCILLATIONS; DATA RELEASE; FINAL DATA; RECONSTRUCTION; CATALOGS; SYSTEM; SPACE; PEAK AB We present an anisotropic analysis of the baryonic acoustic oscillation (BAO) scale in the twelfth and final data release of the Baryonic Oscillation Spectroscopic Survey (BOSS). We independently analyse the LOWZ and CMASS galaxy samples: the LOWZ sample contains contains 361 762 galaxies with an effective redshift of zLOWZ=0.32; the CMASS sample consists of 777 202 galaxies with an effective redshift of zCMASS=0.57. We extract the BAO peak position from the monopole power spectrum moment, a0, and from the 2 moment, a2, where is the cosine of the angle to the line-of-sight. The 2-moment provides equivalent information to that available in the quadrupole but is simpler to analyse. After applying a reconstruction algorithm to reduce the BAO suppression by bulk motions, we measure the BAO peak position in the monopole and 2-moment, which are related to radial and angular shifts in scale. We report H(zLOWZ)rs(zd)=(11.60 +/- 0.60) 103kms-1 and DA(zLOWZ)/rs(zd)=6.66 +/- 0.16 with a cross-correlation coefficient of rHDA=0.41, for the LOWZ sample; and H(zCMASS)rs(zd)=(14.56 +/- 0.37) 103kms-1 and DA(zCMASS)/rs(zd)=9.42 +/- 0.13 with a cross-correlation coefficient of rHDA=0.47, for the CMASS sample. We combine these results with the measurements of the BAO peak position in the monopole and quadrupole correlation function of the same dataset \citep[][companion paper]{Cuestaetal2015} and report the consensus values: H(zLOWZ)rs(zd)=(11.63 +/- 0.69) 103kms-1 and DA(zLOWZ)/rs(zd)=6.67 +/- 0.15 with rHDA=0.35 for the LOWZ sample; H(zCMASS)rs(zd)=(14.67 +/- 0.42) 103kms-1 and DA(zCMASS)/rs(zd)=9.47 +/- 0.12 with rHDA=0.52 for the CMASS sample. C1 [Gil-Marin, Hector; Percival, Will J.; Maraston, Claudia; Thomas, Daniel; Zhao, Gong-Bo] Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg, Portsmouth PO1 3FX, Hants, England. [Cuesta, Antonio J.] Univ Barcelona, Inst Ciencies Cosmos, IEEC UB, Marti & Franques 1, E-08028 Barcelona, Spain. [Brownstein, Joel R.] Univ Utah, Dept Phys & Astron, 115 S 1400 E, Salt Lake City, UT 84112 USA. [Chuang, Chia-Hsun; Prada, Francisco; Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Inst Fis Teo UAM CSIC, E-28049 Madrid, Cantobianco, Spain. [Ho, Shirley] Carnegie Mellon Univ, McWilliams Ctr, Pittsburgh, PA 15213 USA. [Kitaura, Francisco-Shu] Leibniz Inst Astrophys AIP, Sternwarte 16, D-14482 Potsdam, Germany. [Prada, Francisco; Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Prada, Francisco] Inst Astrofis Andalucia, CSIC, Glorieta Astronomia, E-18080 Granada, Spain. [Rodriguez-Torres, Sergio] Campus Int Excellence UAM CSIC, E-28049 Madrid, Spain. [Ross, Ashley J.] Ohio State Univ, Ctr Cosmol & AstroPanicle Phys, Columbus, OH 43210 USA. [Schlegel, David J.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Schlegel, David J.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Tinker, Jeremy L.] NYU, Ctr Cosmol & Particle Phys, Dept Phys, New York, NY 10003 USA. [Tojeiro, Rita] Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Vargas Magana, Mariana] Univ Nacl Autonoma Mexico, Inst Fis, Apdo 20364, Postal, Mexico. [Zhao, Gong-Bo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. RP Gil-Marin, H (reprint author), Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg, Portsmouth PO1 3FX, Hants, England. EM hector.gil@port.ac.uk RI Gil Marin, Hector/B-2013-2017; OI Gil Marin, Hector/0000-0003-0265-6217; Cuesta Vazquez, Antonio Jose/0000-0002-4153-9470 FU UK Science and Technology Facilities Council [ST/I001204/1]; UK Science and Technology Facilities Research Council [ST/I001204/1]; European Research Council [614030]; Karl-Schwarzschild Program from the Leibniz Society; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX HGM is grateful for support from the UK Science and Technology Facilities Council through the grant ST/I001204/1. WJP is grateful for support from the UK Science and Technology Facilities Research Council through the grant ST/I001204/1, and the European Research Council through the grant "Darksurvey", reference 614030. FSK acknowledges the support of the Karl-Schwarzschild Program from the Leibniz Society.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 8 Z9 8 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD AUG 21 PY 2016 VL 460 IS 4 BP 4210 EP 4219 DI 10.1093/mnras/stw1264 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DT8AV UT WOS:000381711100061 ER PT J AU Dau, PD Shuh, DK Sturzbecher-Hoehne, M Abergel, RJ Gibson, JK AF Dau, Phuong D. Shuh, David K. Sturzbecher-Hoehne, Manuel Abergel, Rebecca J. Gibson, John K. TI Divalent and trivalent gas-phase coordination complexes of californium: evaluating the stability of Cf(II) SO DALTON TRANSACTIONS LA English DT Article ID SOLID-STATE; STRUCTURAL-CHARACTERIZATION; MOLECULAR-COMPLEXES; OXIDATION-STATE; CHEMISTRY; SAMARIUM; STABILIZATION; LANTHANIDES; PLUTONYL; LIGANDS AB The divalent oxidation state is increasingly stable relative to the trivalent state for the later actinide elements, with californium the first actinide to exhibit divalent chemistry under moderate conditions. Although there is evidence for divalent Cf in solution and solid compounds, there are no reports of discrete complexes in which Cf-II is coordinated by anionic ligands. Described here is the divalent Cf methanesulfinate coordination complex, Cf-II(CH3SO2)(3-), prepared in the gas phase by reductive elimination of CH3SO2 from Cf-III(CH3SO2)(4-). Comparison with synthesis of the corresponding Sm and Cm complexes reveals reduction of Cf-III and Sm-III, and no evidence for reduction of Cm-III. This reflects the comparative 3+/2+ reduction potentials: Cf3+ (-1.60 V) approximate to Sm3+ (-1.55 V) >> Cm3+ (-3.7 V). Association of O-2 to the divalent complexes is attributed to formation of superoxides, with recovery of the trivalent oxidation state. The new gas-phase chemistry of californium, now the heaviest element to have been studied in this manner, provides evidence for Cf-II coordination complexes and similar chemistry of Cf and Sm. C1 [Dau, Phuong D.; Shuh, David K.; Sturzbecher-Hoehne, Manuel; Abergel, Rebecca J.; Gibson, John K.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Gibson, JK (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jkgibson@lbl.gov FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Heavy Element Chemistry Program at LBNL [DE-AC02-05CH11231] FX This work was fully supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Heavy Element Chemistry Program at LBNL under Contract No. DE-AC02-05CH11231. The 249Cf was provided through the US DOE Isotope Production Program at Oak Ridge National Laboratory. NR 39 TC 0 Z9 0 U1 9 U2 11 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PD AUG 21 PY 2016 VL 45 IS 31 BP 12338 EP 12345 DI 10.1039/c6dt02414a PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DT4WC UT WOS:000381480900011 PM 27424652 ER PT J AU Le, AT Hall, GE Sears, TJ AF Le, Anh T. Hall, Gregory E. Sears, Trevor J. TI The near-infrared spectrum of ethynyl radical SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID COLOR-CENTER LASER; VIBRATIONALLY EXCITED C2H; POLYCYCLIC AROMATIC-HYDROCARBONS; RATE-CONSTANT MEASUREMENTS; ABSOLUTE RATE COEFFICIENT; KINETIC SPECTROSCOPY; ABSORPTION SPECTRUM; THEORETICAL CALCULATION; TEMPERATURE; CCH AB Transient diode laser absorption spectroscopy has been used to measure three strong vibronic bands in the near infrared spectrum of the C2H, ethynyl, radical not previously observed in the gas phase. The radical was produced by ultraviolet excimer laser photolysis of either acetylene or (1,1,1)trifluoropropyne in a slowly flowing sample of the precursor diluted in inert gas, and the spectral resolution was Doppler-limited. The character of the upper states was determined from the rotational and fine structure in the observed spectra and assigned by measurement of ground state rotational combination differences. The upper states include a (2)Sigma(+) state at 6696 cm(-1), a second (2)Sigma(+) state at 7088 cm(-1), and a 2. state at 7110 cm(-1). By comparison with published calculations [R. Tarroni and S. Carter, J. Chem. Phys 119, 12878 (2003); Mol. Phys. 102, 2167 (2004)], the vibronic character of these levels was also assigned. The observed states contain both (2)Sigma(+) and Lambda(2). electronic characters. Several local rotational level perturbations were observed in the excited states. Kinetic measurements of the time-evolution of the ground state populations following collisional relaxation and reactive loss of the radicals formed in a hot, non-thermal, population distribution were made using some of the strong rotational lines observed. The case of C2H may be a good place to investigate the behavior at intermediate pressures of inert colliders, where the competition between relaxation and reaction can be tuned and observed to compare with master equation models, rather than deliberately suppressed to measure thermal rate constants. Published by AIP Publishing. C1 [Le, Anh T.; Hall, Gregory E.; Sears, Trevor J.] Brookhaven Natl Lab, Div Chem, Dept Energy & Photon Sci, Upton, NY 11973 USA. [Sears, Trevor J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Le, AT (reprint author), Brookhaven Natl Lab, Div Chem, Dept Energy & Photon Sci, Upton, NY 11973 USA. EM anhle@bnl.gov; gehall@bnl.gov; sears@bnl.gov OI Sears, Trevor/0000-0002-5559-0154; Hall, Gregory/0000-0002-8534-9783 FU U.S. Department of Energy, Office of Science [DE-SC0012704]; U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences FX Work at Brookhaven National Laboratory was carried out under Contract No. DE-SC0012704 with the U.S. Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences. We thank Stephen Klippenstein for productive discussions and exploratory calculations on the submerged barriers in the C2H + CF3C2H reaction. NR 74 TC 0 Z9 0 U1 6 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2016 VL 145 IS 7 AR 074306 DI 10.1063/1.4961019 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT7QG UT WOS:000381680700025 PM 27544104 ER PT J AU Mahalik, JP Muthukumar, M AF Mahalik, J. P. Muthukumar, M. TI Simulation of self-assembly of polyzwitterions into vesicles SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ZWITTERIONIC POLYMERS; DIBLOCK COPOLYMERS; AMPHIPHILIC MACROMOLECULES; MOLECULAR-DYNAMICS; BULK PROPERTIES; WATER; TRANSITION; BEHAVIOR; SURFACTANTS; SOLUBILITY AB Using the Langevin dynamics method and a coarse-grained model, we have studied the formation of vesicles by hydrophobic polymers consisting of periodically placed zwitterion side groups in dilute salt-free aqueous solutions. The zwitterions, being permanent charge dipoles, provide long-range electrostatic correlations which are interfered by the conformational entropy of the polymer. Our simulations are geared towards gaining conceptual understanding in these correlated dipolar systems, where theoretical calculations are at present formidable. A competition between hydrophobic interactions and dipole-dipole interactions leads to a series of self-assembled structures. As the spacing d between the successive zwitterion side groups decreases, single chains undergo globule -> disk -> worm-like structures. We have calculated the Flory-Huggins chi parameter for these systems in terms of d and monitored the radius of gyration, hydrodynamic radius, spatial correlations among hydrophobic and dipole monomers, and dipole-dipole orientational correlation functions. During the subsequent stages of self-assembly, these structures lead to larger globules and vesicles as d is decreased up to a threshold value, below which no large scale morphology forms. The vesicles form via a polynucleation mechanism whereby disk-like structures form first, followed by their subsequent merger. Published by AIP Publishing. C1 [Mahalik, J. P.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Mahalik, J. P.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Muthukumar, M.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. RP Mahalik, JP (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.; Mahalik, JP (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM mahalikjp@ornl.gov; muthu@polysci.umass.edu FU National Science Foundation [DMR 1404940]; AFOSR [FA9550-14-1-0164] FX Acknowledgment is made to the National Science Foundation (Grant No. DMR 1404940) and AFOSR (Grant No. FA9550-14-1-0164). NR 53 TC 0 Z9 0 U1 35 U2 35 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2016 VL 145 IS 7 AR 074907 DI 10.1063/1.4960774 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT7QG UT WOS:000381680700047 PM 27544126 ER PT J AU Rong, ZQ Kitchaev, D Canepa, P Huang, WX Ceder, G AF Rong, Ziqin Kitchaev, Daniil Canepa, Pieremanuele Huang, Wenxuan Ceder, Gerbrand TI An efficient algorithm for finding the minimum energy path for cation migration in ionic materials SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ELASTIC BAND METHOD; TRANSITION-STATE THEORY; AB-INITIO; 1ST-PRINCIPLES CALCULATIONS; DISSOCIATIVE ADSORPTION; DIFFUSION MECHANISMS; CHEMICAL-REACTIONS; 1ST PRINCIPLES; SADDLE-POINTS; INTERCALATION AB The Nudged Elastic Band (NEB) is an established method for finding minimum-energy paths and energy barriers of ion migration in materials, but has been hampered in its general application by its significant computational expense when coupled with density functional theory (DFT) calculations. Typically, an NEB calculation is initialized from a linear interpolation of successive intermediate structures (also known as images) between known initial and final states. However, the linear interpolation introduces two problems: (1) slow convergence of the calculation, particularly in cases where the final path exhibits notable curvature; (2) divergence of the NEB calculations if any intermediate image comes too close to a non-diffusing species, causing instabilities in the ensuing calculation. In this work, we propose a new scheme to accelerate NEB calculations through an improved path initialization and associated energy estimation workflow. We demonstrate that for cation migration in an ionic framework, initializing the diffusion path as the minimum energy path through a static potential built upon the DFT charge density reproduces the true NEB path within a 0.2 deviation and yields up to a 25mprovement in typical NEB runtiFurtherthermore, we find that the locally relaxed energy barrier derived from this initialization yields a good approximation of the NEB barrier, with errors within 20 meV of the true NEB value, while reducing computational expense by up to a factor of 5. Finally, and of critical importance for the automation of migration path calculations in high-throughput studies, we find that the new approach significantly enhances the stability of the calculation by avoiding unphysical image initialization. Our algorithm promises to enable efficient calculations of diffusion pathways, resolving a long-standing obstacle to the computational screening of intercalation compounds for Li-ion and multivalent batteries. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). C1 [Rong, Ziqin; Kitchaev, Daniil; Canepa, Pieremanuele; Huang, Wenxuan; Ceder, Gerbrand] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Canepa, Pieremanuele; Ceder, Gerbrand] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ceder, Gerbrand] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Ceder, G (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA.; Ceder, G (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM gceder@berkeley.edu RI Canepa, Pieremanuele/O-2344-2013; OI Canepa, Pieremanuele/0000-0002-5168-9253; /0000-0003-2309-3644 FU BES DOE Grant [EDCBEE]; Software Infrastructure for Sustained Innovation (SI2-SSI) Collaborative Research program of the National Science Foundation [OCI-1147503]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, and Basic Energy Sciences [3F-31144] FX We thank the Materials Project (BES DOE Grant No. EDCBEE) for infrastructure and algorithmic support. We would also like to thank Anubhav Jain for the help in implementing high-throughput ApproxNEB system with Fireworks. 65 The work of D.K. and G.C. on the development of the PathFinder algorithm was supported by the Software Infrastructure for Sustained Innovation (SI2-SSI) Collaborative Research program of the National Science Foundation under Award No. OCI-1147503. The work of Z.R., P.C., W.H., and G.C. on the ApproxNEB algorithm and the application to ionic diffusion in cathode materials was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, and Basic Energy Sciences, subcontract 3F-31144. We also thank the National Energy Research Scientific Computing Center (NERSC)64 for providing computing resources. NR 65 TC 0 Z9 0 U1 29 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD AUG 21 PY 2016 VL 145 IS 7 AR 074112 DI 10.1063/1.4960790 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT7QG UT WOS:000381680700013 PM 27544092 ER PT J AU Apresyan, A Los, S Pena, C Presutti, F Ronzhin, A Sphopulu, M Xie, S AF Apresyan, A. Los, S. Pena, C. Presutti, F. Ronzhin, A. Sphopulu, M. Xie, S. TI Direct tests of a pixelated microchannel plate as the active element of a shower maximum detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Microchannel plate photomultiplier; Shower maximum; Time resolution; Electromagnetic calorimeters; Collider experiments; Precision timing AB One possibility to make a fast and radiation resistant shower maximum detector is to use a secondary emitter as an active element. We report our studies of microchannel plate photomultipliers (MCPs) as the active element of a shower-maximum detector. We present test beam results obtained using Photonis XP85011 to detect secondary particles of an electromagnetic shower. We focus on the use of the multiple pixels on the Photonis MCP in order to find a transverse two-dimensional shower distribution. A spatial resolution of 0.8 mm was obtained with an 8 GeV electron beam. A method for measuring the arrival time resolution for electromagnetic showers is presented, and we show that time resolution better than 40 ps can be achieved. (C) 2016 Elsevier B.V. All rights reserved. C1 [Apresyan, A.; Pena, C.; Presutti, F.; Sphopulu, M.; Xie, S.] CALTECH, Pasadena, CA 91125 USA. [Los, S.; Ronzhin, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Apresyan, A (reprint author), CALTECH, Pasadena, CA 91125 USA. FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy; California Institute of Technology High Energy Physics [DE-SC0011925] FX This work is supported by funding from Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy, and from California Institute of Technology High Energy Physics under Contract DE-SC0011925 with the United States Department of Energy. NR 9 TC 0 Z9 0 U1 4 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 21 PY 2016 VL 828 BP 1 EP 7 DI 10.1016/j.nima.2016.05.015 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DN9KY UT WOS:000377399700001 ER PT J AU Abgrall, N Arnquist, IJ Avignone, FT Back, HO Barabash, AS Bertrand, FE Boswell, M Bradley, AW Brudanin, V Busch, M Buuck, M Byram, D Caldwell, AS Chan, YD Christofferson, CD Chu, PH Cuesta, C Detwiler, JA Dunmore, JA Efremenko, Y Ejiri, H Elliott, SR Finnerty, P Galindo-Uribarri, A Gehman, VM Gilliss, T Giovanetti, GK Goett, J Green, MP Gruszko, J Guinn, IS Guiseppe, VE Henning, R Hoppe, EW Howard, S Howe, MA Jasinski, BR Johnson, RA Keeter, KJ Kidd, MF Kochetov, O Konovalov, SI Kouzes, RT LaFerriere, BD Leon, J Loach, JC MacMullin, J MacMullin, S Martin, RD Massarczyk, R Meijer, S Mertens, S Miller, ML Orrell, JL O'Shaughnessy, C Overman, NR Poon, AWP Pushkin, K Radford, DC Rager, J Rielage, K Robertson, RGH Romero-Romero, E Ronquest, MC Schubert, AG Shanks, B Shirchenko, M Snavely, KJ Snyder, N Steele, D Suriano, AM Tedeschi, D Trimble, JE Varner, RL Vasilyev, S Vetter, K Vorren, K White, BR Wilkerson, JF Wiseman, C Xu, W Yakushev, E Yu, CH Yumatov, V Zhitnikov, I AF Abgrall, N. Arnquist, I. J. Avignone, F. T., III Back, H. O. Barabash, A. S. Bertrand, F. E. Boswell, M. Bradley, A. W. Brudanin, V. Busch, M. Buuck, M. Byram, D. Caldwell, A. S. Chan, Y. -D. Christofferson, C. D. Chu, P. -H. Cuesta, C. Detwiler, J. A. Dunmore, J. A. Efremenko, Yu Ejiri, H. Elliott, S. R. Finnerty, P. Galindo-Uribarri, A. Gehman, V. M. Gilliss, T. Giovanetti, G. K. Goett, J. Green, M. P. Gruszko, J. Guinn, I. S. Guiseppe, V. E. Henning, R. Hoppe, E. W. Howard, S. Howe, M. A. Jasinski, B. R. Johnson, R. A. Keeter, K. J. Kidd, M. F. Kochetov, O. Konovalov, S. I. Kouzes, R. T. LaFerriere, B. D. Leon, J. Loach, J. C. MacMullin, J. MacMullin, S. Martin, R. D. Massarczyk, R. Meijer, S. Mertens, S. Miller, M. L. Orrell, J. L. O'Shaughnessy, C. Overman, N. R. Poon, A. W. P. Pushkin, K. Radford, D. C. Rager, J. Rielage, K. Robertson, R. G. H. Romero-Romero, E. Ronquest, M. C. Schubert, A. G. Shanks, B. Shirchenko, M. Snavely, K. J. Snyder, N. Steele, D. Suriano, A. M. Tedeschi, D. Trimble, J. E. Varner, R. L. Vasilyev, S. Vetter, K. Vorren, K. White, B. R. Wilkerson, J. F. Wiseman, C. Xu, W. Yakushev, E. Yu, C. -H. Yumatov, V. Zhitnikov, I. TI The MAJORANA DEMONSTRATOR radioassay program SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Radiopurity; Trace analysis; Neutron activation analysis; Mass spectrometry; Mass spectroscopy; Germanium counting; Low background; Double beta decay; MAJORANA ID DOUBLE-BETA DECAY; UNDERGROUND RESEARCH FACILITY; PLASMA-MASS SPECTROMETRY; SAMPLE PREPARATION; COPPER; ASSAY; BACKGROUNDS; DETECTORS AB The MAJORANA collaboration is constructing the MAJORANA DEMONSTRATOR at the Sanford Underground Research Facility at the Homestake gold mine, in Lead, SD. The apparatus will use Ge detectors, enriched in isotope Ge-76, to demonstrate the feasibility of a large-scale Ge detector experiment to search for neutrinoless double beta decay. The long half-life of this postulated process requires that the apparatus be extremely low in radioactive isotopes whose decays may produce backgrounds to the search. The radioassay program conducted by the collaboration to ensure that the materials comprising the apparatus are sufficiently pure is described. The resulting measurements from gamma-ray counting, neutron activation and mass spectroscopy of the radioactive-isotope contamination for the materials studied for use in the detector are reported. We interpret these numbers in the context of the expected background for the experiment. (C) 2016 Elsevier B.V. All rights reserved. C1 [Abgrall, N.; Bradley, A. W.; Chan, Y. -D.; Mertens, S.; Poon, A. W. P.; Vetter, K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Arnquist, I. J.; Back, H. O.; Hoppe, E. W.; Kouzes, R. T.; LaFerriere, B. D.; Orrell, J. L.; Overman, N. R.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Avignone, F. T., III; Guiseppe, V. E.; Tedeschi, D.; Wiseman, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Avignone, F. T., III; Bertrand, F. E.; Galindo-Uribarri, A.; Green, M. P.; Radford, D. C.; Romero-Romero, E.; Varner, R. L.; White, B. R.; Wilkerson, J. F.; Yu, C. -H.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Back, H. O.; Green, M. P.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Back, H. O.; Busch, M.; Finnerty, P.; Gilliss, T.; Giovanetti, G. K.; Green, M. P.; Henning, R.; Howe, M. A.; MacMullin, J.; MacMullin, S.; Meijer, S.; O'Shaughnessy, C.; Rager, J.; Shanks, B.; Snavely, K. J.; Trimble, J. E.; Vorren, K.; Wilkerson, J. F.] Triangle Univ Nucl Lab, Durham, NC 27706 USA. [Barabash, A. S.; Konovalov, S. I.; Yumatov, V.] Kurchatov Inst Inst Theoret & Expt Phys, Natl Res Ctr, Moscow, Russia. [Boswell, M.; Chu, P. -H.; Elliott, S. R.; Gehman, V. M.; Goett, J.; Massarczyk, R.; Rielage, K.; Ronquest, M. C.; Steele, D.; Xu, W.] Los Alamos Natl Lab, Los Alamos, NM USA. [Brudanin, V.; Kochetov, O.; Shirchenko, M.; Yakushev, E.; Zhitnikov, I.] Joint Inst Nucl Res, Dubna, Russia. Duke Univ, Dept Phys, Durham, NC 27706 USA. [Byram, D.; Jasinski, B. R.; Martin, R. D.; Pushkin, K.; Snyder, N.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. [Caldwell, A. S.; Christofferson, C. D.; Howard, S.; Suriano, A. M.] South Dakota Sch Mines & Technol, Rapid City, SD USA. [Buuck, M.; Cuesta, C.; Detwiler, J. A.; Dunmore, J. A.; Gruszko, J.; Guinn, I. S.; Johnson, R. A.; Leon, J.; Miller, M. L.; Robertson, R. G. H.; Schubert, A. G.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA. [Buuck, M.; Cuesta, C.; Detwiler, J. A.; Dunmore, J. A.; Gruszko, J.; Guinn, I. S.; Johnson, R. A.; Leon, J.; Miller, M. L.; Robertson, R. G. H.; Schubert, A. G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Efremenko, Yu; Romero-Romero, E.; Vasilyev, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Ejiri, H.] Osaka Univ, Nucl Phys Res Ctr, Osaka, Japan. [Ejiri, H.] Osaka Univ, Dept Phys, Osaka, Japan. [Finnerty, P.; Gilliss, T.; Giovanetti, G. K.; Henning, R.; Howe, M. A.; MacMullin, J.; MacMullin, S.; Meijer, S.; O'Shaughnessy, C.; Rager, J.; Shanks, B.; Snavely, K. J.; Trimble, J. E.; Vorren, K.; Wilkerson, J. F.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC USA. [Keeter, K. J.] Black Hills State Univ, Dept Phys, Spearfish, SD 57799 USA. [Kidd, M. F.] Tennessee Technol Univ, Cookeville, TN USA. [Abgrall, N.; Loach, J. C.] Shanghai Jiao Tong Univ, Shanghai 200030, Peoples R China. [Finnerty, P.] Appl Res Associates Inc, 8537 Six Forks Rd,Suite 600, Raleigh, NC USA. [Johnson, R. A.] Microsoft Corp, One Microsoft Way, Redmond, WA USA. [MacMullin, S.; Steele, D.] Picarro Inc, 3105 Patrick Henry Dr, Santa Clara, CA USA. [Gehman, V. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Pushkin, K.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Ronquest, M. C.] CCRi, 1422 Sachem Pl 1, Charlottesville, VA USA. [Schubert, A. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Snavely, K. J.] IBM Cluodant, 200 State St, Boston, MA USA. [Martin, R. D.] Queens Univ, Dept Phys Engn Phys & Astron, Kingston, ON, Canada. [Vetter, K.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Elliott, SR (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM elliotts@lanl.gov RI Cuesta, Clara/L-5466-2014; Xu, Wenqin/H-7553-2014; Barabash, Alexander/S-8851-2016; Orrell, John/E-9313-2015; OI Cuesta, Clara/0000-0003-1190-7233; Xu, Wenqin/0000-0002-5976-4991; Orrell, John/0000-0001-7968-4051; Chu, Pinghan/0000-0003-1372-2910; Rielage, Keith/0000-0002-7392-7152 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-05CH11231, DE-AC52-06NA25396, DE-FG02-97ER41041, DE-FG02-97ER41033, DE-FG02-97ER41042, DE-SC0012612, DE-FG02-10ER41715, DE-SC0010254, DE-FG02-97ER41020]; National Science Foundation [PHY-0919270, PHY-1003940, 0855314, PHY-1202950, MRI 0923142, 1003399]; Russian Foundation for Basic Research [15-02-02919]; U.S. Department of Energy through the LANL/LDRD Program; DOE Office of Science User Facility [DE-AC02-05CH11231, DE-AC05-00OR22725]; Waste Isolation Pilot Plant; Kimballton Underground Research Facility at Oroville; Low Background Facility at Oroville; Berkeley Low Background Facility at SURF; Berkeley Low Background Facility at LBNL; McClellan Nuclear Radiation Center; North Carolina State University's PULSTAR research and teaching reactor; Radiation Safety Office at Virginia Tech; Radiation Safety Department at the University of Tennesse, Knoxville; Nu Instruments Limited in Wrexham, UK FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Award Numbers DE-AC02-05CH11231, DE-AC52-06NA25396, DE-FG02-97ER41041, DE-FG02-97ER41033, DE-FG02-97ER41042, DE-SC0012612, DE-FG02-10ER41715, DE-SC0010254, and DE-FG02-97ER41020. We acknowledge support from the Particle Astrophysics Program and Nuclear Physics Program of the National Science Foundation through grant numbers PHY-0919270, PHY-1003940, 0855314, PHY-1202950, MRI 0923142 and 1003399. We acknowledge support from the Russian Foundation for Basic Research, grant No. 15-02-02919. We acknowledge the support of the U.S. Department of Energy through the LANL/LDRD Program.; This research used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC05-00OR22725. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported under Contract No. DE-AC02-05CH11231. We thank our hosts and colleagues at the Sanford Underground Research Facility for their support. We acknowledge support from the facilities; the Waste Isolation Pilot Plant, the Kimballton Underground Research Facility and the Low Background Facility at Oroville, the Berkeley Low Background Facilities at SURF and at LBNL, the McClellan Nuclear Radiation Center, the North Carolina State University's PULSTAR research and teaching reactor, the Radiation Safety Office at Virginia Tech, the Radiation Safety Department at the University of Tennesse, Knoxville, and Nu Instruments Limited in Wrexham, UK. NR 43 TC 2 Z9 2 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 21 PY 2016 VL 828 BP 22 EP 36 DI 10.1016/j.nima.2016.04.070 PG 15 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DN9KY UT WOS:000377399700004 ER PT J AU Yang, X Huang, XB AF Yang, Xi Huang, Xiaobiao TI A method for simultaneous linear optics and coupling correction for storage rings with turn-by-turn beam position monitor data SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Optics correction; Turn-by-turn; BPM AB We propose a method to simultaneously correct linear optics errors and linear coupling for storage rings using turn-by-turn (TbT) beam position monitor (BPM) data. The independent component analysis (ICA) method is used to isolate the betatron normal modes from the measured TbT BPM data. The betatron amplitudes and phase advances of the projections of the normal modes on the horizontal and vertical planes are then extracted, which, combined with dispersion measurement, are used to fit the lattice model. The fitting results are used for lattice correction. The method has been successfully demonstrated on the NSLS-II storage ring. (C) 2016 Elsevier B.V. All rights reserved. C1 [Yang, Xi] Brookhaven Natl Lab, Upton, NY 11973 USA. [Huang, Xiaobiao] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Huang, XB (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM xiahuang@slac.stanford.edu FU U.S. DOE [DE-AC02-76SF00515, DE-AC02-98CH10886] FX We thank Yongjun Li for preparing the initial condition of the machine for the experiment. We thank James Safranek for reading the manuscript. Author X. Yang thanks Victor Smalyuk for many useful discussions. The study is supported by U.S. DOE under Contract No. DE-AC02-98CH10886 (BNL) and Contract No. DE-AC02-76SF00515 (SLAC). NR 22 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD AUG 21 PY 2016 VL 828 BP 97 EP 104 DI 10.1016/j.nima.2016.05.020 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DN9KY UT WOS:000377399700014 ER PT J AU Nelson, AF Marzari, F AF Nelson, Andrew F. Marzari, F. TI DYNAMICS OF CIRCUMSTELLAR DISKS III: THE CASE OF GG Tau A SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; binaries: general; protoplanetary disks; stars: formation; stars: variables: T Tauri; Herbig Ae/Be ID SELF-GRAVITATING DISCS; YOUNG BINARY-SYSTEM; COOLING TIME-SCALE; A NUMERICAL CODE; CIRCUMBINARY DISK; PLANET FORMATION; ACCRETION RATES; STELLAR-SYSTEM; MASS-RATIO; STARS AB We present two-dimensional hydrodynamic simulations using the Smoothed Particle Hydrodynamic code, VINE, to model a self-gravitating binary system. We model configurations in which a circumbinary torus+disk surrounds a pair of stars in orbit around each other and a circumstellar disk surrounds each star, similar to that observed for the GG Tau A system. We assume that the disks cool as blackbodies, using rates determined independently at each location in the disk by the time dependent temperature of the photosphere there. We assume heating due to hydrodynamical processes and to radiation from the two stars, using rates approximated from a measure of the radiation intercepted by the disk at its photosphere. We simulate a suite of systems configured with semimajor axes of either a = 62 AU ("wide") or a = 32 AU ("close"), and with assumed orbital eccentricity of either e = 0 or e = 0.3. Each simulation follows the evolution for similar to 6500-7500 yr, corresponding to about three orbits of the torus around the center of mass. Our simulations show that strong, sharply defined spiral structures are generated from the stirring action of the binary and that, in some cases, these structures fragment into 1-2 massive clumps. The torus quickly fragments into several dozen such fragments in configurations in which either the binary is replaced by a single star of equal mass, or radiative heating is neglected. The spiral structures extend inwards to the circumstellar environment as large scale material streams for which most material is found on trajectories that return it to the torus on a timescale of 1-200 yr, with only a small fraction accreting into the circumstellar environment. The spiral structures also propagate outwards through the torus, generating net outwards mass flow, and eventually losing coherence at large distances from the stars. The torus becomes significantly eccentric in shape over most of its evolution. In all configurations, accretion onto the stars occurs at a steady rate of a few x10(-8) M circle dot yr(-1), with the net result that, without replenishment, the disk lifetimes would be shorter than similar to 10(4) yr. Our simulations show that only wide orbit configurations are able to retain circumstellar disks, by virtue of accretion driven from the robust material streams generated in wide configurations, which are very weak in close configurations. In wide, eccentric orbit configurations, accretion is episodic and occurs preferentially onto the secondary, with rates strongly peaked near the binary periapse. Based on our results, we conclude that the GG Tau A torus is strongly self gravitating and that a major contribution to its thermal energy input is the shock dissipation associated with spiral structures generated both by self gravitating disturbances and by the stirring action of the binary. We interpret the sharply defined features observed in the torus as manifestations of such spiral structures. We interpret the low density disk surrounding it as an excretion disk created by the outward mass flux generated by the spiral arms as they propagate outwards. Typical eccentricities calculated for the shape of the tori modeled in our simulations are large enough to account for the supposed similar to 20 degrees mutual inclination between the stellar orbit plane of GG Tau A and its surrounding torus through a degeneracy between the interpretation of inclination of the torus and its eccentricity. We therefore interpret the observations in favor of a coplanar system with an eccentric torus. Because accretion onto the disks occurs at rates sufficient to sustain them only in wide orbit configurations, we conclude that the gas currently resident in the circumstellar disks of the GG Tau A system has been accreted from the torus within the past few thousand years. Although circumstellar disks will persist over time spans long enough to permit planet formation, the overall environment remains unfavorable due to high temperatures and other conditions. Given the presence of circumstellar disks, robust accretion streams, and our interpretation of the GG Tau A stellar orbit plane as coplanar with the torus surrounding it, we conclude that the GG Tau A system is in an eccentric, a similar to 62 AU orbit, resolving questions in the literature regarding its orbit parameters. C1 [Nelson, Andrew F.] Los Alamos Natl Lab, XCP 2,Mailstop T082, Los Alamos, NM 87545 USA. [Marzari, F.] Univ Padua, Dipartimento Fis, Via Marzolo 8, I-35131 Padua, Italy. RP Nelson, AF (reprint author), Los Alamos Natl Lab, XCP 2,Mailstop T082, Los Alamos, NM 87545 USA. EM andy.nelson@lanl.gov; francesco.marzari@pd.infn.it FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX We wish to thank the anonymous referee for comments which improved our manuscript. Portions of this work were carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396, for which this is publication LA-UR-16-23283. NR 71 TC 3 Z9 3 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2016 VL 827 IS 2 AR 93 DI 10.3847/0004-637X/827/2/93 PG 40 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW9SA UT WOS:000384001600005 ER PT J AU Sleator, CC Tomsick, JA King, AL Miller, JM Boggs, SE Bachetti, M Barret, D Chenevez, J Christensen, FE Craig, WW Hailey, CJ Harrison, FA Rahoui, F Stern, DK Walton, DJ Zhang, WW AF Sleator, Clio C. Tomsick, John A. King, Ashley L. Miller, Jon M. Boggs, Steven E. Bachetti, Matteo Barret, Didier Chenevez, Jerome Christensen, Finn E. Craig, William W. Hailey, Charles J. Harrison, Fiona A. Rahoui, Farid Stern, Daniel K. Walton, Dominic J. Zhang, William W. TI A NuSTAR OBSERVATION OF THE REFLECTION SPECTRUM OF THE LOW-MASS X-RAY BINARY 4U 1728-34 SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; stars: neutron; X-rays: binaries ID INNER ACCRETION DISKS; NEUTRON-STAR; BLACK-HOLES; AQUILA X-1; XMM-NEWTON; PULSARS; LINES; SPECTROSCOPY; CONSTRAINTS; TELESCOPE AB We report on a simultaneous NuSTAR and Swift observation of the neutron star low-mass X-ray binary 4U 1728-34. We identified and removed four Type I X-ray bursts during the observation in order to study the persistent emission. The continuum spectrum is hard and described well by a blackbody with kT = 1.5 keV and a cutoff power law with Gamma = 1.5, and a cutoff temperature of 25 keV. Residuals between 6 and 8 keV provide strong evidence of a broad Fe K alpha line. By modeling the spectrum with a relativistically blurred reflection model, we find an upper limit for the inner disk radius of R-in <= 2R(ISCO). Consequently, we find that R-NS <= 23 km, assuming M =1.4 M-circle dot and alpha = 0.15. We also find an upper limit on the magnetic field of B <= 2 x 10(8) G. C1 [Sleator, Clio C.; Tomsick, John A.; Boggs, Steven E.] Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA. [King, Ashley L.] Stanford Univ, KIPAC, 452 Lomita Mall, Stanford, CA 94305 USA. [Miller, Jon M.] Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA. [Bachetti, Matteo; Barret, Didier] Univ Toulouse, UPS OMP, Toulouse, France. [Bachetti, Matteo; Barret, Didier] CNRS, Inst Rech Astrophys & Planetol, 9 Av Colonel Roche,BP 44346, F-31028 Toulouse 4, France. [Chenevez, Jerome; Christensen, Finn E.] Tech Univ Denmark, DTU Space, Elektrovej 327-328, Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Craig, William W.; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, 550 West 120th St, New York, NY 10027 USA. [Craig, William W.; Hailey, Charles J.] Columbia Univ, Dept Astron, 550 West 120th St, New York, NY 10027 USA. [Harrison, Fiona A.; Walton, Dominic J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Rahoui, Farid] European Southern Observ, Karl Schwarzschild Str 2, D-85748 Garching, Germany. [Rahoui, Farid] Harvard Univ, Dept Astron, 60 Garden St, Cambridge, MA 02138 USA. [Stern, Daniel K.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Sleator, CC (reprint author), Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA. OI Bachetti, Matteo/0000-0002-4576-9337 FU ESA/PRODEX; NASA FX We thank Michael Parker and Andy Fabian for the particular version of the reflionx model used in this analysis. We thank Kristin Madsen for her help identifying the calibration issue in the NuSTAR data between 3-4.5 keV. J.C. thanks ESA/PRODEX for financial support. This work is based on data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. NR 45 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2016 VL 827 IS 2 AR 134 DI 10.3847/0004-637X/827/2/134 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW9SA UT WOS:000384001600046 ER PT J AU Sorini, D Onorbe, J Lukic, Z Hennawi, JF AF Sorini, Daniele Onorbe, Jose Lukic, Zarija Hennawi, Joseph F. TI MODELING THE Ly alpha FOREST IN COLLISIONLESS SIMULATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE intergalactic medium; methods: numerical ID PROBABILITY-DISTRIBUTION FUNCTION; BARYON ACOUSTIC-OSCILLATIONS; PARTICLE-MESH SIMULATIONS; SMALL-SCALE STRUCTURE; INTERGALACTIC MEDIUM; POWER SPECTRUM; HIGH-REDSHIFT; GRAVITATIONAL-INSTABILITY; HYDROGEN REIONIZATION; TRANSMITTED FLUX AB Cosmological hydrodynamic simulations can accurately predict the properties of the intergalactic medium (IGM), but only under the condition of retaining the high spatial resolution necessary to resolve density fluctuations in the IGM. This resolution constraint prohibits simulating large volumes, such as those probed by BOSS and future surveys, like DESI and 4MOST. To overcome this limitation, we present "Iteratively Matched Statistics" (IMS), a novel method to accurately model the Ly alpha forest with collisionless N-body simulations, where the relevant density fluctuations are unresolved. We use a small-box, high-resolution hydrodynamic simulation to obtain the probability distribution function (PDF) and the power spectrum of the real-space Lya. forest flux. These two statistics are iteratively mapped onto a pseudo-flux field of an N-body simulation, which we construct from the matter density. We demonstrate that our method can reproduce the PDF, line of sight and 3D power spectra of the Lya. forest with good accuracy (7%, 4%, and 7% respectively). We quantify the performance of the commonly used Gaussian smoothing technique and show that it has significantly lower accuracy (20%-80%), especially for N-body simulations with achievable mean inter-particle separations in large-volume simulations. In addition, we show that IMS produces reasonable and smooth spectra, making it a powerful tool for modeling the IGM in large cosmological volumes and for producing realistic "mock" skies for Ly alpha forest surveys. C1 [Sorini, Daniele; Onorbe, Jose; Hennawi, Joseph F.] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Lukic, Zarija] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Sorini, D (reprint author), Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. EM sorini@mpia-hd.mpg.de FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy Office of Advanced Scientific Computing Research; Office of High Energy Physics FX We are thankful to the anonymous referee for useful comments. We thank Martin White, Casey W. Stark, and the members of the ENIGMA group at the Max Planck Institute for Astronomy (MPIA) for helpful comments and discussions. We are grateful to Vetter's Alt Heidelberger for providing a. supportive and enriching environment for many of those discussions. We thank the Esalen Institute for kind hospitality. Calculations presented in this paper used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. Hydrodynamical runs in this paper were done under the ASCR Leadership Computing Challenge (ALCC) allocation. Z.L. acknowledges support from the Scientific Discovery through the Advanced Computing (SciDAC) program funded by U.S. Department of Energy Office of Advanced Scientific Computing Research and the Office of High Energy Physics. This work made extensive use of the NASA Astrophysics Data System and of the astro-ph preprint archive at arXiv.org. NR 74 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2016 VL 827 IS 2 AR 97 DI 10.3847/0004-637X/827/2/97 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW9SA UT WOS:000384001600009 ER PT J AU van Rossum, DR Kashyap, R Fisher, R Wollaeger, RT Garcia-Berro, E Aznar-Siguan, G Ji, SQ Loren-Aguilar, P AF van Rossum, Daniel R. Kashyap, Rahul Fisher, Robert Wollaeger, Ryan T. Garcia-Berro, Enrique Aznar-Siguan, Gabriela Ji, Suoqing Loren-Aguilar, Pablo TI LIGHT CURVES AND SPECTRA FROM A THERMONUCLEAR EXPLOSION OF A WHITE DWARF MERGER SO ASTROPHYSICAL JOURNAL LA English DT Article DE hydrodynamics; radiative transfer; supernovae: general; white dwarfs ID DELAY-TIME DISTRIBUTION; CORE-DEGENERATE SCENARIO; PARTICLE HYDRODYNAMICS SIMULATIONS; IA SUPERNOVAE; RADIATION TRANSPORT; NEBULAR SPECTRA; TRIPLE-SYSTEMS; GAMMA-RAYS; PROGENITORS; DETONATIONS AB Double-degenerate (DD) mergers of carbon-oxygen white dwarfs have recently emerged as a leading candidate for normal Type Ia supernovae (SNe Ia). However, many outstanding questions surround DD mergers, including the characteristics of their light curves and spectra. We have recently identified a spiral instability in the post-merger phase of DD mergers and demonstrated that this instability self-consistently leads to detonation in some cases. We call this the spiral merger SN. Ia model. Here, we utilize the SUPERNU radiative transfer software to calculate three-dimensional synthetic light curves and spectra of the spiral merger simulation with a system mass of 2.1 M-circle dot from Kashyap et al. Because of their large system masses, both violent and spiral merger light curves are slowly declining. The spiral merger resembles very slowly declining SNe Ia, including SN 2001ay, and provides a more natural explanation for its observed properties than other SN. Ia explosion models. Previous synthetic light curves and spectra of violent DD mergers demonstrate a strong dependence on viewing angle, which is in conflict with observations. Here, we demonstrate that the light curves and spectra of the spiral merger are less sensitive to the viewing angle than violent mergers, in closer agreement with observation. We find that the spatial distribution of Ni-56 and IMEs follows a characteristic hourglass shape. We discuss the implications of the asymmetric distribution of Ni-56 for the early-time gamma-ray observations of Ni-56 from SN 2014J. We suggest that DD mergers that agree with the light curves and spectra of normal SNe Ia will likely require a lower system mass. C1 [van Rossum, Daniel R.] Univ Chicago, Dept Astron & Astrophys, Flash Ctr Computat Sci, Chicago, IL 60637 USA. [Kashyap, Rahul; Fisher, Robert] Univ Massachusetts Dartmouth, Dept Phys, 285 Old Westport Rd, N Dartmouth, MA 02740 USA. [Wollaeger, Ryan T.] Los Alamos Natl Lab, Los Alamos, NM USA. [Garcia-Berro, Enrique; Aznar-Siguan, Gabriela] Univ Politecn Cataluna, Dept Fis, C Esteve Terrades 5, E-08860 Castelldefels, Spain. [Garcia-Berro, Enrique; Aznar-Siguan, Gabriela] Inst Estudis Espacials Catalunya, Ed Nexus 201,C Gran Capita 2-4, E-08034 Barcelona, Spain. [Ji, Suoqing] Univ Calif Santa Barbara, Dept Phys, Broida Hall, Santa Barbara, CA 93106 USA. [Loren-Aguilar, Pablo] Univ Exeter, Sch Phys, Stocker Rd, Exeter EX4 4QL, Devon, England. RP van Rossum, DR (reprint author), Univ Chicago, Dept Astron & Astrophys, Flash Ctr Computat Sci, Chicago, IL 60637 USA. OI van Rossum, Daniel/0000-0001-7772-6131; Fisher, Robert/0000-0001-8077-7255; Kashyap, Rahul/0000-0002-5700-282X; Wollaeger, Ryan/0000-0003-3265-4079; Ji, Suoqing/0000-0001-9658-0588 FU University of Chicago by National Science Foundation (JINA, Joint Institute for Nuclear Astrophysics) [AST-0909132, PHY-0822648]; University of Chicago by National Science Foundation (JINA-CEE, Joint Institute for Nuclear Astrophysics) [PHY-1430152]; NSF grant [CNS-0959382]; National Science Foundation [ACI-1053575]; AFOSR DURIP grant [FA9550-10-1-0354]; MINECO [AYA2014-59084P]; AGAUR FX We acknowledge useful discussions with Jerod Parrent, Marius Dan, and Brad Schaefer. This work is supported in part at the University of Chicago by the National Science Foundation under grants AST-0909132, PHY-0822648 (JINA, Joint Institute for Nuclear Astrophysics), and PHY-1430152 (JINA-CEE, Joint Institute for Nuclear Astrophysics). This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number ACI-1053575. Simulations at UMass Dartmouth were performed on a computer cluster supported by NSF grant CNS-0959382 and AFOSR DURIP grant FA9550-10-1-0354. The work of E.G.-B., G.A.-S., and P.L.-A. was partially funded by the MINECO AYA2014-59084P grant and by the AGAUR. This research has made use of NASA's Astrophysics Data System and the yt astrophysics analysis software suite (Turk et al. 2011). NR 79 TC 1 Z9 1 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD AUG 20 PY 2016 VL 827 IS 2 AR 128 DI 10.3847/0004-637X/827/2/128 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW9SA UT WOS:000384001600040 ER PT J AU Stephan, T Trappitsch, R Davis, AM Pellin, MJ Rost, D Savina, MR Yokochi, R Liu, N AF Stephan, Thomas Trappitsch, Reto Davis, Andrew M. Pellin, Michael J. Rost, Detlef Savina, Michael R. Yokochi, Reika Liu, Nan TI CHILI - the Chicago Instrument for Laser Ionization - a new tool for isotope measurements in cosmochemistry SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Resonance ionization mass spectrometry; Cosmochemistry; Isotopes; Isobaric interference ID PRESOLAR SIC GRAINS; GIANT BRANCH STARS; QUANTITATIVE SURFACE-ANALYSIS; MAINSTREAM SILICON CARBIDES; FLIGHT MASS-SPECTROMETRY; RESONANCE IONIZATION; TOF-SIMS; STARDUST; MURCHISON; ZIRCONIUM AB We describe CHILI, the Chicago Instrument for Laser Ionization, a new resonance ionization mass spectrometer developed for isotopic analysis at high spatial resolution and high sensitivity of small samples like contemporary interstellar dust grains returned by the Stardust spacecraft. We explain how CHILI addresses the technical challenges associated with such analyses by pushing most technical specifications towards their physical limits. As an initial demonstration, after many years of designing and developing CHILI, we have analyzed presolar silicon carbide grains for their isotopic compositions of strontium, zirconium, and barium. Subsequently, after further technical improvements, we have used CHILI to analyze, for the first time without interference, all stable isotopes of iron and nickel simultaneously in presolar silicon carbide grains. With a special timing scheme for the ionization lasers, we separated iron and nickel isotopes in the time-of-flight spectrum such that the isobaric interference between Fe-58 and Ni-58 was resolved. In-depth discussion of the astrophysical implications of the presolar grain results is deferred to dedicated later publications. Here we focus on the technical aspects of CHILI, its status quo, and further developments necessary to achieve CHILI's ultimate goals, similar to 10 nm lateral resolution and 30-40% useful yield. (C) 2016 Elsevier B.V. All rights reserved. C1 [Stephan, Thomas; Trappitsch, Reto; Davis, Andrew M.; Pellin, Michael J.; Rost, Detlef; Yokochi, Reika; Liu, Nan] Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. [Stephan, Thomas; Trappitsch, Reto; Davis, Andrew M.; Pellin, Michael J.; Rost, Detlef; Savina, Michael R.; Yokochi, Reika; Liu, Nan] Chicago Ctr Cosmochem, Chicago, IL USA. [Davis, Andrew M.; Pellin, Michael J.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Pellin, Michael J.; Savina, Michael R.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Rost, Detlef] Univ Auckland, Dept Phys, Auckland 1010, New Zealand. [Savina, Michael R.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94550 USA. [Liu, Nan] Carnegie Inst Sci, Dept Terr Magnetism, Washington, DC 20015 USA. RP Stephan, T (reprint author), Univ Chicago, Dept Geophys Sci, Chicago, IL 60637 USA. EM tstephan@uchicago.edu OI Trappitsch, Reto/0000-0002-0924-236X FU NASA Sample Return Laboratory Instruments and Data Analysis Program; Laboratory Analysis of Returned Samples Program [NNX07AL94G, NNX11AC21G, NNX15AF78G]; University of Chicago; Argonne National Laboratory; NASA Headquarters under NASA Earth and Space Science Fellowship Program [NNX12AL85H] FX Among the many people who directly or indirectly helped to build CHILI, we would like to emphasize the contribution by Gordon Ward from the central machine shop of the University of Chicago. His ingenuity was crucial for making CHILI. Construction and development of CHILI was supported by the NASA Sample Return Laboratory Instruments and Data Analysis Program and the Laboratory Analysis of Returned Samples Program through grants NNX07AL94G, NNX11AC21G, and NNX15AF78G, by the University of Chicago, and by Argonne National Laboratory. RT is supported by NASA Headquarters under the NASA Earth and Space Science Fellowship Program through grant NNX12AL85H. We appreciate thoughtful comments by one anonymous reviewer. NR 55 TC 0 Z9 0 U1 11 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD AUG 20 PY 2016 VL 407 BP 1 EP 15 DI 10.1016/j.ijms.2016.06.001 PG 15 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA DW0AW UT WOS:000383304300001 ER PT J AU Perciano, T Tupin, F Hirata, R Cesar, RM AF Perciano, T. Tupin, F. Hirata, R., Jr. Cesar, R. M., Jr. TI A two-level Markov random field for road network extraction and its application with optical, SAR, and multitemporal data SO INTERNATIONAL JOURNAL OF REMOTE SENSING LA English DT Article ID HIGH-RESOLUTION IMAGES; LINEAR FEATURES; AUTOMATIC EXTRACTION; MULTISENSOR DATA; FEATURE FUSION; URBAN AREAS; CLASSIFICATION; MODEL; COMBINATION; DETECTOR AB This article introduces a method for road network extraction from satellite images. The proposed approach covers a new fusion method (using data from multiple sources) and a new Markov random field (MRF) defined on connected components along with a multilevel application (two-level MRF). Our method allows the detection of roads with different characteristics and decreases by around 30% the size of the used graph model. Results for synthetic aperture radar (SAR) images and optical images obtained using the TerraSAR-X and Quickbird sensors, respectively, are presented demonstrating the improvement brought by the proposed approach. In a second part, an analysis of different types of data fusion combining optical/radar images, radar/radar images, and multitemporal SAR (TerraSAR-X and COSMO-SkyMed) images is described. The qualitative and quantitative results show that the fusion approach improves considerably the results of the road network extraction. C1 [Perciano, T.; Tupin, F.] Telecom ParisTech, Signal & Image Proc Dept, LTCI, Paris, France. [Perciano, T.; Hirata, R., Jr.; Cesar, R. M., Jr.] Univ Sao Paulo, Dept Comp Sci, Inst Math & Stat, BR-05508 Sao Paulo, SP, Brazil. RP Perciano, T (reprint author), Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. EM tperciano@lbl.gov RI Perciano, Talita/I-5977-2012; Cesar, Roberto/C-4120-2012 OI Perciano, Talita/0000-0002-2388-1803; Cesar, Roberto/0000-0003-2701-4288 FU Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior [0310-10-7]; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo [2011/50761-2]; Agence Nationale de la Recherche [ANR-2007-MCDC-04] FX This work was supported by Coordenacao de Aperfeicoamento de Pessoal de Nivel Superior under Grant #0310-10-7; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo under Grant #2011/50761-2; Agence Nationale de la Recherche under Grant #ANR-2007-MCDC-04. NR 53 TC 0 Z9 0 U1 10 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0143-1161 EI 1366-5901 J9 INT J REMOTE SENS JI Int. J. Remote Sens. PD AUG 20 PY 2016 VL 37 IS 16 BP 3584 EP 3610 DI 10.1080/01431161.2016.1201227 PG 27 WC Remote Sensing; Imaging Science & Photographic Technology SC Remote Sensing; Imaging Science & Photographic Technology GA DS8QT UT WOS:000381048600003 ER PT J AU Lei, W Han, LL Xuan, CJ Lin, RQ Liu, HF Xin, HLL Wang, DL AF Lei, Wen Han, Lili Xuan, Cuijuan Lin, Ruoqian Liu, Hongfang Xin, Huolin L. Wang, Deli TI Nitrogen-doped carbon nanofibers derived from polypyrrole coated bacterial cellulose as high-performance electrode materials for supercapacitors and Li-ion batteries SO ELECTROCHIMICA ACTA LA English DT Article DE supercapacitors; Li-ion batteries; polypyrrole; bacterial cellulose; nitrogen-doping ID HIERARCHICAL POROUS CARBON; ELECTROCHEMICAL CAPACITORS; GRAPHENE; NANOCOMPOSITES; OXIDE; DENSITY AB Nitrogen-doped carbon nanofiber (NDCN) was synthesized via carbonization of polypyrrole (PPy) coated bacterial cellulose (BC) composites, where BC serves as templates as well as precursor, and PPy serves as the nitrogen source. The synthesized NDCN was employed as electrode for both supercapacitors and Li-ion batteries. The large surface area exposed to electrolyte resulting from the 3D carbon networks leads to sufficient electrode/electrolyte interface and creates shorter transport paths of electrolyte ions and Li+ ion. Besides, the three types of N dopants in NDCN improve the electronic conductivity, as well as superior electrochemical performance. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Lei, Wen; Xuan, Cuijuan; Liu, Hongfang; Wang, Deli] Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Hubei Key Lab Mat Chem & Serv Failure, Key Lab Mat Chem Energy Convers & Storage,Minist, Wuhan 430074, Peoples R China. [Han, Lili; Lin, Ruoqian; Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Han, Lili] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China. [Lin, Ruoqian] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. RP Wang, DL (reprint author), Huazhong Univ Sci & Technol, Sch Chem & Chem Engn, Hubei Key Lab Mat Chem & Serv Failure, Key Lab Mat Chem Energy Convers & Storage,Minist, Wuhan 430074, Peoples R China. EM wangdl81125@hust.edu.cn RI Wang, Deli/K-5029-2012 FU National Natural Science Foundation [21306060, 21573083]; Program for New Century Excellent Talents in Universities of China [NCET-13-0237]; Doctoral Fund of Ministry of Education of China [20130142120039]; Fundamental Research Funds for the Central University [2013TS136, 2014YQ009]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX This work was supported by the National Natural Science Foundation (21306060, 21573083), the Program for New Century Excellent Talents in Universities of China (NCET-13-0237), the Doctoral Fund of Ministry of Education of China (20130142120039), the Fundamental Research Funds for the Central University (2013TS136, 2014YQ009). We thank Analytical and Testing Center of Huazhong University of Science and Technology for allowing us to use its facilities. S/TEM work was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No.DE-SC0012704. NR 33 TC 2 Z9 2 U1 33 U2 62 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD AUG 20 PY 2016 VL 210 BP 130 EP 137 DI 10.1016/j.electacta.2016.05.158 PG 8 WC Electrochemistry SC Electrochemistry GA DS4IZ UT WOS:000380746100018 ER PT J AU Dong, R Moore, L Ocola, LE Kuljanishvili, I AF Dong, Rui Moore, Logan Ocola, Leonidas E. Kuljanishvili, Irma TI Enabling Quality Interfaces with Mask-Free Approach to Selective Growth of MoS2/Graphene Stacked Structures SO ADVANCED MATERIALS INTERFACES LA English DT Article DE 2D atomic crystals; direct write patterning; mask-free fabrication; MoS2; Graphene stacked structures; residue-free interfaces ID DIP-PEN NANOLITHOGRAPHY; LARGE-AREA SYNTHESIS; 2-DIMENSIONAL MATERIALS; GRAPHENE; MOS2; FILMS; DECOMPOSITION; TRANSISTORS C1 [Dong, Rui; Moore, Logan; Kuljanishvili, Irma] St Louis Univ, Dept Phys, 3511 Laclede Ave, St Louis, MO 63103 USA. [Ocola, Leonidas E.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Kuljanishvili, I (reprint author), St Louis Univ, Dept Phys, 3511 Laclede Ave, St Louis, MO 63103 USA. EM ikuljani@slu.edu FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02 06CH11357]; NSF MRI program [1338021]; Saint Louis University seed funds FX Use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02 06CH11357. I.K. acknowledges support of NSF MRI program (Award No. 1338021), and the Saint Louis University seed funds. NR 22 TC 0 Z9 0 U1 14 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD AUG 19 PY 2016 VL 3 IS 16 AR 1600098 DI 10.1002/admi.201600098 PG 6 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DW6TD UT WOS:000383783200004 ER PT J AU Gearba, RI Kim, M Mueller, KM Veneman, PA Lee, K Holliday, BJ Chan, CK Chelikowsky, JR Tutuc, E Stevenson, KJ AF Gearba, Raluca I. Kim, Minjung Mueller, Kory M. Veneman, Peter A. Lee, Kayoung Holliday, Bradley J. Chan, Calvin K. Chelikowsky, James R. Tutuc, Emanuel Stevenson, Keith J. TI Atomically Resolved Elucidation of the Electrochemical Covalent Molecular Grafting Mechanism of Single Layer Graphene SO ADVANCED MATERIALS INTERFACES LA English DT Article DE angle resolved photoelectron spectroscopy; electronic properties in graphene; graphene covalent functionalization; scanning tunneling microscopy ID TRANSITION-METAL DICHALCOGENIDES; ORDERED PYROLYTIC-GRAPHITE; ARYL IODONIUM SALTS; ELECTRON-TRANSFER; HIGH-QUALITY; CHEMISTRY; FUNCTIONALIZATION; DEFECTS; SPECTROSCOPY; PERFORMANCE AB Engineering graphene at the atomic level via chemical doping, substrate interactions or lateral confinement opens up avenues for precise tuning of its electronic and magnetic properties. Chemical doping by covalent modification routes using electrochemical tools offers rich opportunities that are yet to be fully explored. The key to controlling graphene's physicochemical properties requires a detailed atomistic understanding of the geometry and mechanism of the covalent attachment process. By employing diaryliodonium salts instead of the commonly used diazonium salts, precise molecular grafting onto epitaxial graphene is achieved. Using atomically resolved imaging via scanning tunneling microscopy it is shown that for single layer, high quality, low defect graphene, the functionalization process is controlled by kinetics rather than thermodynamics in accord with Marcus-Gerisher theory. The predominance of the preferential pairwise attachment of molecular grafts specifically on the same graphene sublattice gives rise to ferromagnetic properties previously observed in nitrophenyl modified graphene. Furthermore, p-type doping has been quantified by electrical measurements and angle resolved photoelectron spectroscopy. Overall this electrochemical route for precise covalent functionalization of single layer graphene is general and can be straightforwardly extended to other 2D few-layer confined materials such as transition metal chalcogenides. C1 [Gearba, Raluca I.; Stevenson, Keith J.] Univ Texas Austin, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA. [Kim, Minjung; Chelikowsky, James R.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Kim, Minjung] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. [Mueller, Kory M.; Veneman, Peter A.; Holliday, Bradley J.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. [Lee, Kayoung; Tutuc, Emanuel] Univ Texas Austin, Microelect Res Ctr, Austin, TX 78758 USA. [Chan, Calvin K.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Chelikowsky, James R.] Univ Texas Austin, Ctr Computat Mat, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Stevenson, Keith J.] Ctr Electrochem Energy Storage, Skolkovo Inst Sci & Technol, Moscow 14306, Russia. RP Stevenson, KJ (reprint author), Univ Texas Austin, Ctr Nano & Mol Sci & Technol, Austin, TX 78712 USA.; Stevenson, KJ (reprint author), Ctr Electrochem Energy Storage, Skolkovo Inst Sci & Technol, Moscow 14306, Russia. EM stevenson@cm.utexas.edu FU Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences on "Understanding Charge Separation and Transfer at Interfaces in Energy Materials'' (EFRC:CST) [DESC0001091]; Sandia National Laboratories' Laboratory Directed Research; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy [DOE/DE-FG02-06ER46286, DE-AC02-05CH11231]; Welch Foundation [F-1529, F-1631] FX This work was supported by an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences on "Understanding Charge Separation and Transfer at Interfaces in Energy Materials'' (EFRC:CST, Award Number DESC0001091). The authors thank T. Ohta, G. Copeland, and L. Brunke for providing the graphene/SiC substrates. C.K.C. acknowledges support from Sandia National Laboratories' Laboratory Directed Research and Development Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. M.K. and J.R.C. acknowledge support on computational approaches to nanostructures by the U.S. Department of Energy under Award DOE/DE-FG02-06ER46286. K.J.S. and B.J.H. acknowledge additional funding by the Welch Foundation (Grants F-1529 and F-1631, respectively). The work at the Advanced Light Source (Berkeley) was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. R.I.G. would like to thank J. Denlinger for assistance during measurements on the 4.0.3 MERLIN beamline. NR 60 TC 0 Z9 0 U1 21 U2 21 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD AUG 19 PY 2016 VL 3 IS 16 AR 1600196 DI 10.1002/admi.201600196 PG 10 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DW6TD UT WOS:000383783200009 ER PT J AU Shen, X Pennycook, TJ Hernandez-Martin, D Perez, A Puzyrev, YS Liu, YH te Velthuis, SGE Freeland, JW Shafer, P Zhu, CH Varela, M Leon, C Sefrioui, Z Santamaria, J Pantelides, ST AF Shen, Xiao Pennycook, Timothy J. Hernandez-Martin, David Perez, Ana Puzyrev, Yevgeniy S. Liu, Yaohua te Velthuis, Suzanne G. E. Freeland, John W. Shafer, Padraic Zhu, Chenhui Varela, Maria Leon, Carlos Sefrioui, Zouhair Santamaria, Jacobo Pantelides, Sokrates T. TI High On/Off Ratio Memristive Switching of Manganite/Cuprate Bilayer by Interfacial Magnetoelectricity SO ADVANCED MATERIALS INTERFACES LA English DT Article DE DFT calculations; magnetoelectricity; memristive switching; oxide interface; transition metal ID ELECTRIC-FIELD CONTROL; TUNNEL-JUNCTIONS; OXIDE; MAGNETIZATION; MECHANISM; SYSTEMS; MEMORY; FILMS AB Memristive switching serves as the basis for a new generation of electronic devices. Conventional memristors are two-terminal devices in which the current is turned on and off by redistributing point defects, e.g., vacancies. Memristors based on alternative mechanisms have been explored, but achieving both high on/off ratio and low switching energy, as needed in applications, remains a challenge. This study reports memristive switching in La0.7Ca0.3MnO3/PrBa2Cu3O7 bilayers with an on/off ratio greater than 10(3) and results of density functional theory calculations in terms of which it is concluded that the phenomenon is likely the result of a new type of interfacial magnetoelectricity. More specifically, this study shows that an external electric field induces subtle displacements of the interfacial Mn ions, which switches on/off an interfacial magnetic dead layer, resulting in memristive behavior for spin-polarized electron transport across the bilayer. The interfacial nature of the switching entails low energy cost, about of a tenth of atto Joule for writing/erasing a bit. The results indicate new opportunities for manganite/cuprate systems and other transition metal oxide junctions in memristive applications. C1 [Shen, Xiao; Pennycook, Timothy J.; Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Shen, Xiao] Univ Memphis, Dept Phys & Mat Sci, Memphis, TN 38152 USA. [Pennycook, Timothy J.] SuperSTEM Lab, Daresbury WA4 4AD, Cheshire, England. [Pennycook, Timothy J.] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England. [Hernandez-Martin, David; Perez, Ana; Varela, Maria; Leon, Carlos; Sefrioui, Zouhair; Santamaria, Jacobo] Univ Complutense, Grp Fis Mat Complejos, E-28040 Madrid, Spain. [Liu, Yaohua] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Liu, Yaohua; te Velthuis, Suzanne G. E.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Shafer, Padraic; Zhu, Chenhui] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Varela, Maria; Pantelides, Sokrates T.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Santamaria, Jacobo] Univ Complutense, Inst Magnetismo Aplicado, E-28040 Madrid, Spain. [Pantelides, Sokrates T.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, 221 Kirkland Hall, Nashville, TN 37235 USA. RP Shen, X (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA.; Shen, X (reprint author), Univ Memphis, Dept Phys & Mat Sci, Memphis, TN 38152 USA. EM xshen1@memphis.edu RI Liu, Yaohua/B-2529-2009; te Velthuis, Suzanne/I-6735-2013; Leon, Carlos/A-5587-2008; Sefrioui, Zouhair/C-2728-2017; Varela, Maria/E-2472-2014 OI Liu, Yaohua/0000-0002-5867-5065; te Velthuis, Suzanne/0000-0002-1023-8384; Leon, Carlos/0000-0002-3262-1843; Sefrioui, Zouhair/0000-0002-6703-3339; Varela, Maria/0000-0002-6582-7004 FU National Science Foundation [DMR-1207241]; Department of Energy [DE-FG02-09ER46554]; McMinn Endowment at Vanderbilt University; NSF XSEDE [TG-DMR130121]; Spanish MICINN [MAT2014-52405-C02-01]; Consolider Ingenio [2010CSD2009-00013]; CAM through grant CAM [S2013/MIT-2740]; EPSRC; Division of Scientific User Facilities of the Office of Basic Energy Sciences, US Department of Energy; U.S. Department of Energy, Office of Science, Materials Science and Engineering Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy [DE-AC02-05CH11231] FX X.S., T.J.P., and D.H.-M. contributed equally to this work. The work at Vanderbilt was supported by National Science Foundation grant DMR-1207241, by Department of Energy grant DE-FG02-09ER46554, and by the McMinn Endowment at Vanderbilt University. Computational support was provided by the NSF XSEDE under Grant # TG-DMR130121. Research at UCM was supported by Spanish MICINN through grants MAT2014-52405-C02-01 and Consolider Ingenio 2010CSD2009-00013 (Imagine), by CAM through grant CAM S2013/MIT-2740. Research at SuperSTEM, the UK National Facility for Aberration-Corrected STEM was supported by the EPSRC. The work at ORNL was partially supported by the Division of Scientific User Facilities of the Office of Basic Energy Sciences, US Department of Energy. Work at Argonne National Laboratory (S.G.E.t.V.) was supported by the U.S. Department of Energy, Office of Science, Materials Science and Engineering Division. Work performed at the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No.DE-AC02-06CH11357. The Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 0 Z9 0 U1 18 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD AUG 19 PY 2016 VL 3 IS 16 AR 1600086 DI 10.1002/admi.201600086 PG 8 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DW6TD UT WOS:000383783200003 ER PT J AU Zhang, HH Wang, WJ Hagen, N Kuzmenko, I Akinc, M Travesset, A Mallapragada, S Vaknin, D AF Zhang, Honghu Wang, Wenjie Hagen, Noah Kuzmenko, Ivan Akinc, Mufit Travesset, Alex Mallapragada, Surya Vaknin, David TI Self-Assembly of DNA Functionalized Gold Nanoparticles at the Liquid-Vapor Interface SO ADVANCED MATERIALS INTERFACES LA English DT Article DE DNA-functionalization; GISAXS; gold nanoparticles; interfacial crystallization; X-ray fluorescence ID NANOCRYSTAL SUPERLATTICES; CAPPED NANOPARTICLES; CHARGED INTERFACES; CRYSTALLIZATION; MONOLAYERS; SYSTEMS; SURFACE AB Surface sensitive synchrotron X-ray scattering and spectroscopy are used to monitor and characterize the spontaneous formation of 2D Gibbs monolayers of thiolated single-stranded DNA-functionalized gold nanoparticles (ssDNA-AuNPs) at the vapor-solution interface by manipulating salt concentrations. Grazing incidence small-angle X-ray scattering and X-ray reflectivity show that the noncomplementary ssDNA-AuNPs dispersed in aqueous solution spontaneously accumulate at the vapor-liquid interface in the form of a single layer by increasing MgCl2 or CaCl2 concentrations. Furthermore, the monoparticle layer undergoes a transformation from short- to long-range (hexagonal) order above a threshold salt-concentration. Using various salts at similar ionic strength to those of MgCl2 or CaCl2 such as, NaCl or LaCl3, it is found that surface adsorbed NPs lack any order. X-ray fluorescence near total reflection of the same samples provides direct evidence of interfacial gold and more importantly a significant surface enrichment of the cations. Quantitative analysis reveals that divalent cations screen the charge of ssDNA, and that the hydrophobic hexyl-thiol group, commonly used to functionalize the ssDNA (for capping the AuNPs), is likely the driving force for the accumulation of the NPs at the interface. C1 [Zhang, Honghu; Wang, Wenjie; Hagen, Noah; Akinc, Mufit; Mallapragada, Surya; Vaknin, David] Ames Lab, Ames, IA 50011 USA. [Zhang, Honghu; Akinc, Mufit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kuzmenko, Ivan] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Travesset, Alex; Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Mallapragada, Surya] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. RP Vaknin, D (reprint author), Ames Lab, Ames, IA 50011 USA.; Vaknin, D (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM vaknin@ameslab.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering through Iowa State University [DE-AC02-07CH11358]; U.S. Department of Energy [DE-AC02-06CH11357] FX The authors thank Xiaobing Zuo for technical support with SAXS measurements conducted at the 12ID-B beamline at the Advanced Photon Source. Research in the Ames Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering through Iowa State University under Contract No. DE-AC02-07CH11358. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Argonne National Laboratory, is supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 38 TC 1 Z9 1 U1 16 U2 17 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD AUG 19 PY 2016 VL 3 IS 16 AR 1600180 DI 10.1002/admi.201600180 PG 9 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DW6TD UT WOS:000383783200007 ER PT J AU Alvarez-Castillo, D Benic, S Blaschke, D Han, S Typel, S AF Alvarez-Castillo, D. Benic, S. Blaschke, D. Han, Sophia Typel, S. TI Neutron star mass limit at 2 M-circle dot supports the existence of a CEP SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID QUARK NUCLEAR-MATTER; EQUATION-OF-STATE; COMPACT STARS; HYBRID STARS; CORES; MODEL; CONSTRAINTS; EOS AB We point out that the very existence of a "horizontal branch" in the mass-radius characteristics for neutron stars indicates a strong first-order phase transition and thus supports the existence of a critical endpoint (CEP) of first-order phase transitions in the QCD phase diagram. This branch would sample a sequence of hybrid stars with quark matter core, leading to the endpoint of stable compact star configurations with the highest possible baryon densities. Since we know of the existence of compact stars with 2 M-circle dot, this hypothetical branch has to lie in the vicinity of this mass value, if it exists. We report here a correlation between the maximal radius of the horizontal branch and the pressure at the onset of hadron-to-quark matter phase transition, which is likely to be a universal quantity of utmost relevance to the upcoming experiments with heavy-ion collisions at NICA and FAIR. C1 [Alvarez-Castillo, D.; Blaschke, D.] JINR Dubna, Bogoliubov Lab Theoret Phys, Dubna, Russia. [Benic, S.] Univ Zagreb, Dept Phys, Zagreb, Croatia. [Blaschke, D.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Blaschke, D.] Univ Wroclaw, Inst Theoret Phys, Wroclaw, Poland. [Han, Sophia] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Han, Sophia] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Typel, S.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Darmstadt, Germany. [Benic, S.] Univ Tokyo, Tokyo, Japan. RP Alvarez-Castillo, D (reprint author), JINR Dubna, Bogoliubov Lab Theoret Phys, Dubna, Russia. EM alvarez@theor.jinr.ru FU COST Action [MP 1304]; Polish NCN [UMO-2014/13/B/ST9/02621]; JINR Dubna; German Institutes; Croatian Science Foundation [8799]; Hessian LOEWE initiative through HIC for FAIR FX We acknowledge the partial support by the COST Action MP 1304 "NewCompStar" for our international networking activities in preparing this article. This work received support from the Polish NCN under grant No. UMO-2014/13/B/ST9/02621. DEAC and ST received support form the Heisenberg-Landau programme for scientist exchange between JINR Dubna and German Institutes. SB acknowledges partial support by the Croatian Science Foundation under Project No. 8799. DB was supported in part by the Hessian LOEWE initiative through HIC for FAIR. NR 52 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD AUG 19 PY 2016 VL 52 IS 8 AR 232 DI 10.1140/epja/i2016-16232-9 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DU4FJ UT WOS:000382167700004 ER PT J AU Mafi, E Tao, X Zhu, WG Gao, YF Wang, CM Gu, Y AF Mafi, Elham Tao, Xin Zhu, Wenguang Gao, Yanfei Wang, Chongmin Gu, Yi TI Generation and the role of dislocations in single-crystalline phase-change In2Se3 nanowires under electrical pulses SO NANOTECHNOLOGY LA English DT Article DE phase-change materials; transmission electron microscopy; scanning Kelvin probe microscopy ID AUGMENTED-WAVE METHOD; CHANGE MEMORY; TRANSFORMATION; AMORPHIZATION; SEMICONDUCTORS; VACANCIES; DRIVEN AB We report the observation of the generation of dislocations in single-crystal phase-change In2Se3 nanowires under electrical pulses and the impact of these dislocations on electrical properties. Particularly, we correlated the atomic-scale structural characteristics with local electrical resistance variations, by performing transmission electron microscopy and scanning Kelvin probe microscopy on the same nanowires. By coupling the experimental results with first-principles density functional theory calculations, we show that the immobile dislocations are generated via vacancy condensations. Importantly, these dislocations lead to several orders of magnitude increase in the electrical resistance, while maintaining the single crystallinity of the lattice. These results significantly advance the fundamental understanding of the structure-property relation in this phase-change material under transient electrical excitations. From a practical perspective, the significant increase in the electrical resistance, driven by the formation of dislocations, can be exploited as a new electronic state in the single-crystalline phase in this phase-change material. C1 [Mafi, Elham; Tao, Xin; Gu, Yi] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Zhu, Wenguang] Univ Sci & Technol China, Int Ctr Quantum Design Funct Mat ICQD, Hefei Natl Lab Phys Sci Microscale HFNL, Hefei 230026, Anhui, Peoples R China. [Zhu, Wenguang] Univ Sci & Technol China, Chinese Acad Sci, Sch Phys Sci, Key Lab Strongly Coupled Quantum Matter Phys, Hefei 230026, Anhui, Peoples R China. [Zhu, Wenguang] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. [Gao, Yanfei] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Gao, Yanfei] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Wang, Chongmin] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Gu, Y (reprint author), Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. EM yigu@wsu.edu RI Gao, Yanfei/F-9034-2010 OI Gao, Yanfei/0000-0003-2082-857X FU US National Science Foundation [DMR-1206960, CMMI-1300223]; National Natural Science Foundation of China [11374273, 11034006]; Fundamental Research Funds for the Central Universities [WK2090050027, WK2060190027, WK2340000063]; DOE's Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL) FX This work was supported by the US National Science Foundation DMR-1206960 (EM, XT, YG) and CMMI-1300223 (YFG), and by the National Natural Science Foundation of China 11374273, 11034006 (WZ) and the Fundamental Research Funds for the Central Universities WK2090050027, WK2060190027, WK2340000063 (WZ). The TEM work was conducted in the William R Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory (PNNL). NR 44 TC 1 Z9 1 U1 14 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD AUG 19 PY 2016 VL 27 IS 33 AR 335704 DI 10.1088/0957-4484/27/33/335704 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DW6SC UT WOS:000383780500020 PM 27389929 ER PT J AU Schoeniger, JS Hudson, CM Bent, ZW Sinha, A Williams, KP AF Schoeniger, Joseph S. Hudson, Corey M. Bent, Zachary W. Sinha, Anupama Williams, Kelly P. TI Experimental single-strain mobilomics reveals events that shape pathogen emergence SO NUCLEIC ACIDS RESEARCH LA English DT Article ID GENOMIC ISLANDS; REPLICATION AB Virulence genes on mobile DNAs such as genomic islands (GIs) and plasmids promote bacterial pathogen emergence. Excision is an early step in GI mobilization, producing a circular GI and a deletion site in the chromosome; circular forms are also known for some bacterial insertion sequences (ISs). The recombinant sequence at the junctions of such circles and deletions can be detected sensitively in high-throughput sequencing data, using new computational methods that enable empirical discovery of mobile DNAs. For the rich mobilome of a hospital Klebsiella pneumo-niae strain, circularization junctions (CJs) were detected for six GIs and seven IS types. Our methods revealed differential biology of multiple mobile DNAs, imprecision of integrases and transposases, and differential activity among identical IS copies for IS26, ISKpn18 and ISKpn21. Using the resistance of circular dsDNA molecules to exonuclease, internally calibrated with the native plasmids, showed that not all molecules bearing GI CJs were circular. Transpositions were also detected, revealing replicon preference (ISKpn18 prefers a conjugative IncA/C2 plasmid), local action (IS26), regional preferences, selection (against capsule synthesis) and IS polarity inversion. Efficient discovery and global characterization of numerous mobile elements per experiment improves accounting for the new gene combinations that arise in emerging pathogens. C1 [Schoeniger, Joseph S.; Hudson, Corey M.; Bent, Zachary W.; Sinha, Anupama; Williams, Kelly P.] Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94551 USA. RP Williams, KP (reprint author), Sandia Natl Labs, Dept Syst Biol, Livermore, CA 94551 USA. EM kpwilli@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories [DE-AC04-94AL85000]; Lockheed Martin Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This research was fully supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract [DE-AC04-94AL85000]. Funding for open access charge: Laboratory Directed Research and Development program at Sandia National Laboratories [DE-AC04-94AL85000]. NR 21 TC 0 Z9 0 U1 6 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 19 PY 2016 VL 44 IS 14 BP 6830 EP 6839 DI 10.1093/nar/gkw601 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DV5VX UT WOS:000382999900030 PM 27378783 ER PT J AU Wan, LCK Pillon, MC Thevakumaran, N Sun, YL Chakrabartty, A Guarne, A Kurinov, I Durocher, D Sicheri, F AF Wan, Leo C. K. Pillon, Monica C. Thevakumaran, Neroshan Sun, Yulong Chakrabartty, Avi Guarne, Alba Kurinov, Igor Durocher, Daniel Sicheri, Frank TI Structural and functional characterization of KEOPS dimerization by Pcc1 and its role in t(6)A biosynthesis SO NUCLEIC ACIDS RESEARCH LA English DT Article ID TRANSFER-RIBONUCLEIC-ACID; SMALL-ANGLE SCATTERING; TRANSFER-RNA; ESCHERICHIA-COLI; KINASE DOMAIN; PROTEIN; COMPLEX; N-(PURIN-6-YLCARBAMOYL)THREONINE; MECHANISM; SYSTEM AB KEOPS is an ancient protein complex required for the biosynthesis of N6-threonylcarbamoyladenosine (t(6)A), a universally conserved tRNA modification found on all ANN-codon recognizing tRNAs. KEOPS consist minimally of four essential subunits, namely the proteins Kae1, Bud32, Cgi121 and Pcc1, with yeast possessing the fifth essential subunit Gon7. Bud32, Cgi121, Pcc1 and Gon7 appear to have evolved to regulate the central t6A biosynthesis function of Kae1, but their precise function and mechanism of action remains unclear. Pcc1, in particular, binds directly to Kae1 and by virtue of its ability to form dimers in solution and in crystals, Pcc1 was inferred to function as a dimerization module for Kae1 and therefore KEOPS. We now present a 3.4 angstrom crystal structure of a dimeric Kae1-Pcc1 complex providing direct evidence that Pcc1 can bind and dimerize Kae1. Further biophysical analysis of a complete archaeal KEOPS complex reveals that Pcc1 facilitates KEOPS dimerization in vitro. Interestingly, while Pcc1-mediated dimerization of KEOPS is required to support the growth of yeast, it is dispensable for t6A biosynthesis by archaeal KEOPS in vitro, raising the question of how precisely Pcc1-mediated dimerization impacts cellular biology. C1 [Wan, Leo C. K.; Thevakumaran, Neroshan; Durocher, Daniel; Sicheri, Frank] Mt Sinai Hosp, Lunenfeld Tanenbaum Res Inst, Toronto, ON M5G 1X5, Canada. [Wan, Leo C. K.; Durocher, Daniel; Sicheri, Frank] Univ Toronto, Dept Mol Genet, Toronto, ON M5S 3E1, Canada. [Pillon, Monica C.; Guarne, Alba] McMaster Univ, Dept Biochem & Biomed Sci, Hamilton, ON L8S 4K1, Canada. [Thevakumaran, Neroshan; Chakrabartty, Avi; Sicheri, Frank] Univ Toronto, Dept Biochem, Toronto, ON M5S 1A8, Canada. [Sun, Yulong; Chakrabartty, Avi] Univ Toronto, Dept Med Biophys, Toronto, ON M5S 1L7, Canada. [Kurinov, Igor] Cornell Univ, Dept Chem & Chem Biol, NE CAT, Adv Photon Source, Bldg 436E,9700 S Cass Ave, Argonne, IL 60439 USA. RP Sicheri, F (reprint author), Mt Sinai Hosp, Lunenfeld Tanenbaum Res Inst, Toronto, ON M5G 1X5, Canada.; Sicheri, F (reprint author), Univ Toronto, Dept Mol Genet, Toronto, ON M5S 3E1, Canada.; Sicheri, F (reprint author), Univ Toronto, Dept Biochem, Toronto, ON M5S 1A8, Canada. EM sicheri@lunenfeld.ca RI Durocher, Daniel/A-7733-2010 OI Durocher, Daniel/0000-0003-3863-8635 FU Canadian Institutes of Health Research (CIHR) Foundation Grants [FDN 143277, FDN 143343]; CIHR Operating Grant [MOP-67189]; National Institutes of Health [P41 GM103403]; NIH-ORIP HEI Grant [S10 RR029205]; APS [DE-AC02-06CH11357]; CIHR Foundation Grant [FDN 143277] FX Canadian Institutes of Health Research (CIHR) Foundation Grants [FDN 143277 to F.S., FDN 143343 to D.D.]; CIHR Operating Grant [MOP-67189 to A.G.]; National Institutes of Health [P41 GM103403 to NE-CAT]; NIH-ORIP HEI Grant for Pilatus 6M detector on 24-IDC beam line [S10 RR029205]; APS funding [DE-AC02-06CH11357]. Funding for open access charge: CIHR Foundation Grant FDN 143277. NR 42 TC 1 Z9 1 U1 4 U2 4 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 19 PY 2016 VL 44 IS 14 BP 6971 EP 6980 DI 10.1093/nar/gkw542 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DV5VX UT WOS:000382999900041 PM 27302132 ER PT J AU Cambray, G Guimaraes, JC Mutalik, VK Lam, C Mai, QA Thimmaiah, T Carothers, JM Arkin, AP Endy, D AF Cambray, Guillaume Guimaraes, Joao C. Mutalik, Vivek K. Lam, Colin Quynh-Anh Mai Thimmaiah, Tim Carothers, James M. Arkin, Adam P. Endy, Drew TI Measurement and modeling of intrinsic transcription terminators (vol 41, pg 5139, 2013) SO NUCLEIC ACIDS RESEARCH LA English DT Correction C1 [Cambray, Guillaume; Guimaraes, Joao C.; Mutalik, Vivek K.; Lam, Colin; Quynh-Anh Mai; Arkin, Adam P.; Endy, Drew] BIOFAB Int Open Facil Adv Biotechnol BIOFAB, 5885 Hollis St, Emeryville, CA 94608 USA. [Cambray, Guillaume; Mutalik, Vivek K.; Lam, Colin; Quynh-Anh Mai; Arkin, Adam P.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Guimaraes, Joao C.; Thimmaiah, Tim; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Guimaraes, Joao C.] Univ Minho, Dept Informat, Comp Sci & Technol Ctr, Campus Gualtar, P-4700 Braga, Portugal. [Mutalik, Vivek K.; Carothers, James M.; Arkin, Adam P.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Endy, Drew] Stanford Univ, Dept Bioengn, Stanford, CA 94305 USA. RP Arkin, AP; Endy, D (reprint author), BIOFAB Int Open Facil Adv Biotechnol BIOFAB, 5885 Hollis St, Emeryville, CA 94608 USA.; Arkin, AP (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Arkin, AP (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.; Arkin, AP (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Endy, D (reprint author), Stanford Univ, Dept Bioengn, Stanford, CA 94305 USA. EM aparkin@lbl.gov; endy@stanford.edu NR 1 TC 0 Z9 0 U1 2 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD AUG 19 PY 2016 VL 44 IS 14 BP 7006 EP 7006 DI 10.1093/nar/gkw379 PG 1 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DV5VX UT WOS:000382999900044 PM 27131373 ER PT J AU Chandran, AKN Yoo, YH Cao, PJ Sharma, R Sharma, M Dardick, C Ronald, PC Jung, KH AF Chandran, Anil Kumar Nalini Yoo, Yo-Han Cao, Peijian Sharma, Rita Sharma, Manoj Dardick, Christopher Ronald, Pamela C. Jung, Ki-Hong TI Updated Rice Kinase Database RKD 2.0: enabling transcriptome and functional analysis of rice kinase genes SO RICE LA English DT Article DE Rice kinase database; Phylogenomics; Functional redundancy; Mutant analysis; Meta-analysis; Pearson correlation coefficient; Transcriptome ID PHYLOGENOMIC DATABASE; EXPRESSION; GENOME; IDENTIFICATION; RESOURCE AB Protein kinases catalyze the transfer of a phosphate moiety from a phosphate donor to the substrate molecule, thus playing critical roles in cell signaling and metabolism. Although plant genomes contain more than 1000 genes that encode kinases, knowledge is limited about the function of each of these kinases. A major obstacle that hinders progress towards kinase characterization is functional redundancy. To address this challenge, we previously developed the rice kinase database (RKD) that integrated omics-scale data within a phylogenetics context. An updated version of rice kinase database (RKD) that contains metadata derived from NCBI GEO expression datasets has been developed. RKD 2.0 facilitates in-depth transcriptomic analyses of kinase-encoding genes in diverse rice tissues and in response to biotic and abiotic stresses and hormone treatments. We identified 261 kinases specifically expressed in particular tissues, 130 that are significantly up- regulated in response to biotic stress, 296 in response to abiotic stress, and 260 in response to hormones. Based on this update and Pearson correlation coefficient (PCC) analysis, we estimated that 19 out of 26 genes characterized through loss-of-function studies confer dominant functions. These were selected because they either had paralogous members with PCC values of < 0.5 or had no paralog. Compared with the previous version of RKD, RKD 2.0 enables more effective estimations of functional redundancy or dominance because it uses comprehensive expression profiles rather than individual profiles. The integrated analysis of RKD with PCC establishes a single platform for researchers to select rice kinases for functional analyses. C1 [Chandran, Anil Kumar Nalini; Yoo, Yo-Han; Jung, Ki-Hong] Kyung Hee Univ, Grad Sch Biotechnol, Yongin 446701, South Korea. [Chandran, Anil Kumar Nalini; Yoo, Yo-Han; Jung, Ki-Hong] Kyung Hee Univ, Crop Biotech Inst, Yongin 446701, South Korea. [Cao, Peijian] Zhengzhou Tobacco Res Inst, China Tobacco Gene Res Ctr, Zhengzhou 450001, Peoples R China. [Sharma, Rita] Jawaharlal Nehru Univ, Sch Computat & Integrat Sci, New Delhi 110067, India. [Sharma, Manoj] Jawaharlal Nehru Univ, Sch Biotechnol, New Delhi 110067, India. [Dardick, Christopher] ARS, Appalachian Fruit Res Stn, USDA, 2217 Wiltshire Rd, Kearneysville, WV 25442 USA. [Ronald, Pamela C.] Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA. [Ronald, Pamela C.] Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. [Ronald, Pamela C.] Joint Bioenergy Inst, Emeryville, CA 95616 USA. RP Jung, KH (reprint author), Kyung Hee Univ, Grad Sch Biotechnol, Yongin 446701, South Korea.; Jung, KH (reprint author), Kyung Hee Univ, Crop Biotech Inst, Yongin 446701, South Korea.; Ronald, PC (reprint author), Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA.; Ronald, PC (reprint author), Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. EM pcronald@ucdavis.edu; khjung2010@khu.ac.kr FU Cooperative Research Program for Agriculture Science & Technology Development [PJ01182602]; Rural Development Administration, Republic of Korea; DOE Joint BioEnergy Institute by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory; U. S. Department of Energy FX This work was carried out with the support of "Cooperative Research Program for Agriculture Science & Technology Development ( Project No. PJ01182602)", Rural Development Administration, Republic of Korea, and was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U. S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 22 TC 0 Z9 0 U1 3 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1939-8425 EI 1939-8433 J9 RICE JI Rice PD AUG 19 PY 2016 VL 9 AR 40 DI 10.1186/s12284-016-0106-5 PG 16 WC Agronomy SC Agriculture GA DU1XQ UT WOS:000382004400001 PM 27540739 ER PT J AU Lee, S Kapustin, EA Yaghi, OM AF Lee, Seungkyu Kapustin, Eugene A. Yaghi, Omar M. TI Coordinative alignment of molecules in chiral metal-organic frameworks SO SCIENCE LA English DT Article ID CRYSTALLINE SPONGE METHOD; X-RAY-STRUCTURE; ABSOLUTE-CONFIGURATION; POROUS COMPLEXES AB A chiral metal-organic framework, MOF-520, was used to coordinatively bind and align molecules of varying size, complexity, and functionality. The reduced motional degrees of freedom obtained with this coordinative alignment method allowed the structures of molecules to be determined by single-crystal x-ray diffraction techniques. The chirality of the MOF backbone also served as a reference in the structure solution for an unambiguous assignment of the absolute configuration of bound molecules. Sixteen molecules representing four common functional groups (primary alcohol, phenol, vicinal diol, and carboxylic acid), ranging in complexity from methanol to plant hormones (gibberellins, containing eight stereocenters), were crystallized and had their precise structure determined. We distinguished single and double bonds in gibberellins, and we enantioselectively crystallized racemic jasmonic acid, whose absolute configuration had only been inferred from derivatives. C1 [Lee, Seungkyu; Kapustin, Eugene A.; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lee, Seungkyu; Kapustin, Eugene A.; Yaghi, Omar M.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lee, Seungkyu; Kapustin, Eugene A.; Yaghi, Omar M.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Lee, Seungkyu; Kapustin, Eugene A.; Yaghi, Omar M.] Berkeley Global Sci Inst, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Berkeley Global Sci Inst, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. EM yaghi@berkeley.edu OI Yaghi, Omar/0000-0002-5611-3325 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; NIH Shared Instrumentation grant [S10-RR027172] FX Supported by BASF SE (Ludwigshafen, Germany) for the synthesis, and by King Abdulaziz City for Science and Technology (Center of Excellence for Nanomaterials and Clean Energy Applications) for the characterization of compounds. We thank S. Teat for synchrotron x-ray diffraction data acquisition support at beamline 11.3.1 [Advanced Light Source (ALS), Lawrence Berkeley National Laboratory (LBNL)]; K. Gagnon for discussion of structure refinement; and H.-B. Burgi for invaluable discussions of structure refinement and editing of this manuscript. NMR data were acquired at the Molecular Foundry, LBNL. Work performed at ALS and the Molecular Foundry is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract DE-AC02-05CH11231 (ALS and Foundry). Use of CheXray facility at the College of Chemistry (UC Berkeley) is supported by NIH Shared Instrumentation grant S10-RR027172. Data reported in this paper are tabulated in the supplementary materials and archived at the Cambridge Crystallographic Data Centre under reference numbers CCDC 1488938 to 1488955. NR 16 TC 14 Z9 14 U1 126 U2 168 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD AUG 19 PY 2016 VL 353 IS 6301 BP 808 EP 811 DI 10.1126/science.aaf9135 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT5ZE UT WOS:000381561400042 PM 27540171 ER PT J AU Antonangeli, D Farber, DL Bosak, A Aracne, CM Ruddle, DG Krisch, M AF Antonangeli, Daniele Farber, Daniel L. Bosak, Alexei Aracne, Chantel M. Ruddle, David G. Krisch, Michael TI Phonon triggered rhombohedral lattice distortion in vanadium at high pressure SO SCIENTIFIC REPORTS LA English DT Article ID TRANSITION; DYNAMICS; NB AB In spite of the simple body-centered-cubic crystal structure, the elements of group V, vanadium, niobium and tantalum, show strong interactions between the electronic properties and lattice dynamics. Further, these interactions can be tuned by external parameters, such as pressure and temperature. We used inelastic x-ray scattering to probe the phonon dispersion of single-crystalline vanadium as a function of pressure to 45 GPa. Our measurements show an anomalous high-pressure behavior of the transverse acoustic mode along the (100) direction and a softening of the elastic modulus C-44 that triggers a rhombohedral lattice distortion occurring between 34 and 39 GPa. Our results provide the missing experimental confirmation of the theoretically predicted shear instability arising from the progressive intra-band nesting of the Fermi surface with increasing pressure, a scenario common to all transition metals of group V. C1 [Antonangeli, Daniele] UPMC, Univ Sorbonne, Museum Natl Hystoire Nat, IMPMC,UMR CNRS 7590,IRD, F-75252 Paris, France. [Farber, Daniel L.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, Santa Cruz, CA 95063 USA. [Bosak, Alexei] European Synchrotron Radiat Facil, F-38000 Grenoble, France. [Ruddle, David G.; Krisch, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Antonangeli, D (reprint author), UPMC, Univ Sorbonne, Museum Natl Hystoire Nat, IMPMC,UMR CNRS 7590,IRD, F-75252 Paris, France. EM daniele.antonangeli@impmc.upmc.fr FU Lawrence Livermore National Laboratory, U.S. Department of Energy [DE-AC52 07NA27344]; French National Research Agency (ANR) [2010-JCJC-604-01] FX This work was performed under the auspice of the Lawrence Livermore National Laboratory, U.S. Department of Energy, under contract DE-AC52 07NA27344 and supported by the French National Research Agency (ANR) grant no. 2010-JCJC-604-01 (to D.A.). NR 23 TC 0 Z9 0 U1 11 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD AUG 19 PY 2016 VL 6 AR 31887 DI 10.1038/srep31887 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT7NR UT WOS:000381674000001 PM 27539662 ER PT J AU Iqbal, MZ Abdala, AA Mittal, V Seifert, S Herring, AM Liberatore, MW AF Iqbal, Muhammad Z. Abdala, Ahmed A. Mittal, Vikas Seifert, Sonke Herring, Andrew M. Liberatore, Matthew W. TI Processable conductive graphene/polyethylene nanocomposites: Effects of graphene dispersion and polyethylene blending with oxidized polyethylene on rheology and microstructure SO POLYMER LA English DT Article DE Graphene; Polyethylene; Nanocomposites; SAXS; Rheology; Micromechanical models ID HIGH-DENSITY POLYETHYLENE; MECHANICAL-PROPERTIES; THERMAL-CONDUCTIVITY; ELASTIC PROPERTIES; (LLDPE)/CLAY NANOCOMPOSITES; FUNCTIONALIZED GRAPHENE; ELECTRICAL-PROPERTIES; EXPANDED GRAPHITE; CARBON NANOTUBES; MELT RHEOLOGY AB Poor dispersion of graphene in non-polar polymer matrices creates composites with limited applications. A method to improve the dispersion of graphene in polyethylene (PE) via blending PE with oxidized PE (OPE) is examined. Graphene was produced by simultaneous thermal exfoliation and reduction of graphite oxide. Nanocomposites of graphene with PE as well as graphene with PE/OPE-blends were prepared by solvent blending. Improved dispersion of graphene in PE/OPE blends substantially decreases percolation from both rheological (0.3 vol%) and electrical (0.13 vol%) measurements compared to neat PE nanocomposites (1 and 0.29 vol%), respectively. A universal Brownian dispersion of graphene in polymers was concluded similar to that of nanotubes, following the Doi-Edwards theory. Micromechanical models, such as Mori-Tanaka and Halpin-Tsai models, modeled the mechanical properties of the nanocomposites. The nanocomposites microstructure, studied by small angle x-ray scattering, confirmed better dispersion of graphene at lower loadings and the formation of surface fractals in the blend/graphene nanocomposites; whereas only mass fractals were observed in neat PE/graphene nanocomposites. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Iqbal, Muhammad Z.; Herring, Andrew M.; Liberatore, Matthew W.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Abdala, Ahmed A.] Hamad Bin Khalifa Univ, Qatar Environm & Energy Res Inst, Mat Sci & Engn Div, Doha, Qatar. [Abdala, Ahmed A.] Hamad Bin Khalifa Univ, Coll Sci & Engn, Doha, Qatar. [Mittal, Vikas] Petr Inst, Dept Chem Engn, Abu Dhabi, U Arab Emirates. [Seifert, Sonke] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Liberatore, Matthew W.] Univ Toledo, Dept Chem & Environm Engn, 2801 W Bancroft St, Toledo, OH 43606 USA. RP Liberatore, MW (reprint author), Univ Toledo, Dept Chem & Environm Engn, 2801 W Bancroft St, Toledo, OH 43606 USA. EM matthew.liberatore@utoledo.edu RI Liberatore, Matthew/B-6828-2008; OI Herring, Andrew/0000-0001-7318-5999 NR 79 TC 2 Z9 2 U1 38 U2 68 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD AUG 19 PY 2016 VL 98 SI SI BP 143 EP 155 DI 10.1016/j.polymer.2016.06.021 PG 13 WC Polymer Science SC Polymer Science GA DR1QE UT WOS:000379679200017 ER PT J AU Yu, J Mao, J Yuan, GC Satija, S Chen, W Tirrell, M AF Yu, Jing Mao, Jun Yuan, Guangcui Satija, Sushil Chen, Wei Tirrell, Matthew TI The effect of multivalent counterions to the structure of highly dense polystyrene sulfonate brushes SO POLYMER LA English DT Article DE Polyelectrolyte; Brush; Multivalentions; ATRP; Neutron; reflectivity ID POLYELECTROLYTE BRUSHES; POLYMER BRUSHES; SCALING RELATIONS; SALT-SOLUTIONS; COLLAPSE; FORCES; LUBRICATION; CHAINS; LAYERS; MEDIA AB Surface tethered polyelectrolyte brushes are scientifically interesting and technologically relevant to many applications, ranging from colloidal stabilization to responsive and tunable materials to lubrication. Many applications operate in environments containing multi-valent ions, media in which our scientific understanding is not yet well-developed. We synthesized high-density polystyrene sulfonate (PSS) brushes via surface initiated atom-transfer radical polymerization, and performed neutron reflectivity (NR) measurements to investigate and compare the effects of mono-valent Rb+ and tri-valent Y3+ counterions to the structure of the densely tethered PSS brushes. Our NR results show that in monovalent RbNO3 solution, the dense PSS brush retained its full thickness up to a salt concentration of 1 M, whereas it immediately collapsed upon adding 1.67 mM of tri-valent Y3+. Increasing the concentration of Y3+ beyond this level did not lead to any significant further structure change of the PSS brush. Our findings demonstrate that the presence of multi-valent counterions can significantly alter the structure of polyelectrolyte brushes, in a manner different from mono-valent ions, which has implications for the functionality of the brushes. (C) 2016 Published by Elsevier Ltd. C1 [Yu, Jing; Mao, Jun; Chen, Wei; Tirrell, Matthew] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Yu, Jing; Mao, Jun; Chen, Wei; Tirrell, Matthew] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Yuan, Guangcui; Satija, Sushil] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Yuan, Guangcui] Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. RP Tirrell, M (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA.; Chen, W (reprint author), Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. EM wchen@anl.gov; mtirrell@uchicago.edu RI Chen, Wei/G-6055-2011; Yu, Jing/C-4138-2017 OI Chen, Wei/0000-0001-8906-4278; Yu, Jing/0000-0002-4288-951X FU U.S. Department of Energy, Office of Science, Program in Basic Energy Sciences, Division of Materials Science and Engineering; NSF Award [NSF-DMR-1420709] FX This work was supported by the U.S. Department of Energy, Office of Science, Program in Basic Energy Sciences, Division of Materials Science and Engineering. We acknowledge the MRSEC Shared User Facilities at the University of Chicago supported by NSF Award NSF-DMR-1420709. NR 31 TC 6 Z9 6 U1 26 U2 43 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD AUG 19 PY 2016 VL 98 SI SI BP 448 EP 453 DI 10.1016/j.polymer.2016.02.053 PG 6 WC Polymer Science SC Polymer Science GA DR1QE UT WOS:000379679200050 ER PT J AU Wu, Y Kong, T Wang, LL Johnson, DD Mou, DX Huang, LN Schrunk, B Bud'ko, SL Canfield, PC Kaminski, A AF Wu, Yun Kong, Tai Wang, Lin-Lin Johnson, D. D. Mou, Daixiang Huang, Lunan Schrunk, Benjamin Bud'ko, S. L. Canfield, P. C. Kaminski, Adam TI Asymmetric mass acquisition in LaBi: Topological semimetal candidate SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WEYL FERMION SEMIMETAL; HGTE QUANTUM-WELLS; SINGLE DIRAC CONE; WAVE BASIS-SET; INSULATOR; SURFACE; ARCS; DISCOVERY; PHASE AB We use our high resolution He-lamp-based, tunable laser-based angle-resolved photoemission spectroscopy measurements and density functional theory calculations to study the electronic properties of LaBi, a binary system that was proposed to be a member of a new family of topological semimetals. Both bulk and surface bands are present in the spectra. The dispersion of the surface state is highly unusual. It resembles a Dirac cone, but upon closer inspection we can clearly detect an energy gap. The bottom band follows roughly a parabolic dispersion. The dispersion of the top band remains very linear, "V" -shape like, with the tip approaching very closely to the extrapolated location of Dirac point. Such asymmetric mass acquisition is highly unusual and opens a possibility of a new topological phenomenon that has yet to be understood. C1 [Wu, Yun; Kong, Tai; Wang, Lin-Lin; Johnson, D. D.; Mou, Daixiang; Huang, Lunan; Schrunk, Benjamin; Bud'ko, S. L.; Canfield, P. C.; Kaminski, Adam] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Wu, Yun; Kong, Tai; Johnson, D. D.; Mou, Daixiang; Huang, Lunan; Schrunk, Benjamin; Bud'ko, S. L.; Canfield, P. C.; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Johnson, D. D.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. RP Canfield, PC; Kaminski, A (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA.; Canfield, PC; Kaminski, A (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM canfield@ameslab.gov; kaminski@ameslab.gov OI Kong, Tai/0000-0002-5064-3464 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. Department of Energy [DE-AC02-07CH11358]; CEM, an NSF MRSEC [DMR-1420451] FX We acknowledge very useful discussions with Yuan-Ming Lu. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. L.H. was supported by CEM, an NSF MRSEC, under Contract No. DMR-1420451. NR 44 TC 3 Z9 3 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2016 VL 94 IS 8 AR 081108 DI 10.1103/PhysRevB.94.081108 PG 6 WC Physics, Condensed Matter SC Physics GA DT6NK UT WOS:000381600800002 ER PT J AU Hiranuma, N Mohler, O Kulkarni, G Schnaiter, M Vogt, S Vochezer, P Jarvinen, E Wagner, R Bell, DM Wilson, J Zelenyuk, A Cziczo, DJ AF Hiranuma, Naruki Moehler, Ottmar Kulkarni, Gourihar Schnaiter, Martin Vogt, Steffen Vochezer, Paul Jaervinen, Emma Wagner, Robert Bell, David M. Wilson, Jacqueline Zelenyuk, Alla Cziczo, Daniel J. TI Development and characterization of an ice-selecting pumped counterflow virtual impactor (IS-PCVI) to study ice crystal residuals SO ATMOSPHERIC MEASUREMENT TECHNIQUES LA English DT Article ID MIXED-PHASE CLOUDS; BIOLOGICAL AEROSOL-PARTICLES; SINGLE-PARTICLE; MASS-SPECTROMETRY; NUCLEATING PARTICLES; CONDENSATION NUCLEI; HEMATITE PARTICLES; SHIP TRACKS; DROPLET; CHAMBER AB Separation of particles that play a role in cloud activation and ice nucleation from interstitial aerosols has become necessary to further understand aerosol-cloud interactions. The pumped counterflow virtual impactor (PCVI), which uses a vacuum pump to accelerate the particles and increase their momentum, provides an accessible option for dynamic and inertial separation of cloud elements. However, the use of a traditional PCVI to extract large cloud hydrometeors is difficult mainly due to its small cut-size diameters (< 5 mu m). Here, for the first time we describe a development of an ice-selecting PCVI (IS-PCVI) to separate ice in controlled mixed-phase cloud system based on the particle inertia with the cut-off diameter >= 10 mu m. We also present its laboratory application demonstrating the use of the impactor under a wide range of temperature and humidity conditions. The computational fluid dynamics simulations were initially carried out to guide the design of the IS-PCVI. After fabrication, a series of validation laboratory experiments were performed coupled with the Aerosol Interaction and Dynamics in the Atmosphere (AIDA) expansion cloud simulation chamber. In the AIDA chamber, test aerosol particles were exposed to the ice supersaturation conditions (i.e., RHice > 100 %), where a mixture of droplets and ice crystals was formed during the expansion experiment. In parallel, the flow conditions of the IS-PCVI were actively controlled, such that it separated ice crystals from a mixture of ice crystals and cloud droplets, which were of diameter >= 10 mu m. These large ice crystals were passed through the heated evaporation section to remove the water content. Afterwards, the residuals were characterized with a suite of online and offline instruments downstream of the IS-PCVI. These results were used to assess the optimized operating parameters of the device in terms of (1) the critical cut-size diameter, (2) the transmission efficiency and (3) the counterflow-toinput flow ratio. Particle losses were characterized by comparing the residual number concentration to the rejected interstitial particle number concentration. Overall results suggest that the IS-PCVI enables inertial separation of particles with a volume-equivalent particle size in the range of similar to 10-30 mu m in diameter with small inadvertent intrusion (similar to 5%) of unwanted particles. C1 [Hiranuma, Naruki; Moehler, Ottmar; Schnaiter, Martin; Vogt, Steffen; Vochezer, Paul; Jaervinen, Emma; Wagner, Robert] Karlsruhe Inst Technol, Inst Meteorol & Climate Res Atmospher Aerosol Res, Karlsruhe, Germany. [Kulkarni, Gourihar; Bell, David M.; Wilson, Jacqueline; Zelenyuk, Alla] Pacific Northwest Natl Lab, Richland, WA USA. [Cziczo, Daniel J.] MIT, Civil & Environm Engn, Earth Atmospher & Planetary Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Hiranuma, N (reprint author), Karlsruhe Inst Technol, Inst Meteorol & Climate Res Atmospher Aerosol Res, Karlsruhe, Germany. EM seong.moon@kit.edu RI Schnaiter, Martin/A-2370-2013; Jarvinen, Emma/G-7120-2014 OI Jarvinen, Emma/0000-0001-5171-1759 FU Helmholtz Association through its research programme "Atmosphere and Climate (ATMO)"; Deutsche Forschungsgemeinschaft (DFG) through the Research Unit [FOR 1525, MO668/4-1, MO668/4-2]; DFG [SCHN 1140/2-1]; NSF [AGS-1461305]; US Department of Energy (DOE) Office of Biological and Environmental Research (OBER) Atmospheric Research Systems Program (ASR); DOE Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; DOE OBER; US DOE ASR; DOE by Battelle Memorial Institute [DE-AC05-76RLO 1830]; Centre of the Helmholtz Association FX We thank the Engineering and Infrastructure group at KIT IMK-AAF (Georg Scheurig, Tomasz Chudy and Rainer Buschbacher) for their support in constructing and operating the IS-PCVI. This work was funded by the Helmholtz Association through its research programme "Atmosphere and Climate (ATMO)" and the Deutsche Forschungsgemeinschaft (DFG) through the Research Unit FOR 1525 (INUIT, grant No MO668/4-1 and MO668/4-2). The valuable contributions of the FIN organizers, their institutions, and the FIN-1 Workshop science team are gratefully acknowledged. N. Hiranuma thanks A. Kiselev (KIT IMK-AAF) and K. Rabe (KIT IBG) for their support on the bacteria sample preparation. M. Schnaiter acknowledges the funding by DFG under grant SCHN 1140/2-1. The participation of G. Kulkarni, D. M. Bell, J. Wilson, A. Zelenyuk, and D. J. Cziczo was partially funded by NSF grant#AGS-1461305. Additional support (A. Zelenyuk, D. M. Bell, J. Wilson, and G. Kulkarni) was provided by the US Department of Energy (DOE) Office of Biological and Environmental Research (OBER) Atmospheric Research Systems Program (ASR). The development of miniS-PLAT was funded by the DOE Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences and EMSL User Facility sponsored by the DOE OBER and located at Pacific Northwest National Laboratory. G. Kulkarni acknowledges support from the US DOE ASR. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RLO 1830.; The article processing charges for this open-access publication were covered by a Research Centre of the Helmholtz Association. NR 74 TC 0 Z9 0 U1 14 U2 15 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1867-1381 EI 1867-8548 J9 ATMOS MEAS TECH JI Atmos. Meas. Tech. PD AUG 18 PY 2016 VL 9 IS 8 BP 3817 EP 3836 DI 10.5194/amt-9-3817-2016 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DW6VR UT WOS:000383790000002 ER PT J AU Bozovic, I He, X Wu, J Bollinger, AT AF Bozovic, I. He, X. Wu, J. Bollinger, A. T. TI Dependence of the critical temperature in overdoped copper oxides on superfluid density SO NATURE LA English DT Article ID MAGNETIC PENETRATION DEPTH; HIGH-T-C; MUON-SPIN-ROTATION; THIN-FILMS; SUPERCONDUCTING FILMS; MUTUAL INDUCTANCE; INTERFACE SUPERCONDUCTIVITY; FIELD PENETRATION; 2-COIL APPARATUS; CARRIER DENSITY AB The physics of underdoped copper oxide superconductors, including the pseudogap, spin and charge ordering and their relation to superconductivity(1-3), is intensely debated. The overdoped copper oxides are perceived as simpler, with strongly correlated fermion physics evolving smoothly into the conventional Bardeen-Cooper-Schrieffer behaviour. Pioneering studies on a few overdoped samples(4-11) indicated that the superfluid density was much lower than expected, but this was attributed to pair-breaking, disorder and phase separation. Here we report the way in which the magnetic penetration depth and the phase stiffness depend on temperature and doping by investigating the entire overdoped side of the La2-xSrxCuO4 phase diagram. We measured the absolute values of the magnetic penetration depth and the phase stiffness to an accuracy of one per cent in thousands of samples; the large statistics reveal clear trends and intrinsic properties. The films are homogeneous; variations in the critical superconducting temperature within a film are very small (less than one kelvin). At every level of doping the phase stiffness decreases linearly with temperature. The dependence of the zero-temperature phase stiffness on the critical superconducting temperature is generally linear, but with an offset; however, close to the origin this dependence becomes parabolic. This scaling law is incompatible with the standard Bardeen-Cooper-Schrieffer description. C1 [Bozovic, I.; He, X.; Wu, J.; Bollinger, A. T.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Bozovic, I.; He, X.] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. RP Bozovic, I (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.; Bozovic, I (reprint author), Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. EM bozovic@bnl.gov FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4410] FX A. Gozar, J. Zhang and J. Yoon contributed to developing the characterization techniques during the early stages of this work. R. Sundling developed the software for the inversion of the inductance data. We also benefited from the electrolyte-gating experiments and X-ray diffraction studies by X. Leng, and from numerical simulations by N. Bozovic. The research was done at BNL and was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. X.H. is supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through grant GBMF4410. I.B. acknowledges discussions with J. Zaanen, G. Deutscher, A. Leggett, P. Littlewood, C.-B. Eom, J. Mannhart, P. Coleman, R. Prozorov, D. van der Marel, A. McKenzie, V. Kogan, P. Armitage, J.-M. Triscone, P. Canfield, A. Chubukov, B. Halperin, P. Kim, T. Lemberger, M. V. Sadovskii, D. Pavuna, Z. Radovic and M. Vanevic. NR 60 TC 7 Z9 7 U1 43 U2 55 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 18 PY 2016 VL 536 IS 7616 BP 309 EP + DI 10.1038/nature19061 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9GN UT WOS:000381804900030 PM 27535534 ER PT J AU Tsai, HH Nie, WY Blancon, JC Toumpos, CCS Asadpour, R Harutyunyan, B Neukirch, AJ Verduzco, R Crochet, JJ Tretiak, S Pedesseau, L Even, J Alam, MA Gupta, G Lou, J Ajayan, PM Bedzyk, MJ Kanatzidis, MG Mohite, AD AF Tsai, Hsinhan Nie, Wanyi Blancon, Jean-Christophe Toumpos, Constantinos C. S. Asadpour, Reza Harutyunyan, Boris Neukirch, Amanda J. Verduzco, Rafael Crochet, Jared J. Tretiak, Sergei Pedesseau, Laurent Even, Jacky Alam, Muhammad A. Gupta, Gautam Lou, Jun Ajayan, Pulickel M. Bedzyk, Michael J. Kanatzidis, Mercouri G. Mohite, Aditya D. TI High-efficiency two-dimensional Ruddlesden-Popper perovskite solar cells SO NATURE LA English DT Article ID SOLUTION-PROCESSED PEROVSKITE; STABILITY; PERFORMANCE; ABSORBER; LAYERS; HYSTERESIS; AIR AB Three-dimensional organic-inorganic perovskites have emerged as one of the most promising thin-film solar cell materials owing to their remarkable photophysical properties(1-5), which have led to power conversion efficiencies exceeding 20 per cent(6,7), with the prospect of further improvements towards the Shockley-Queisser limit for a single-junction solar cell (33.5 per cent) (8). Besides efficiency, another critical factor for photovoltaics and other optoelectronic applications is environmental stability and photostability under operating conditions(9-15). In contrast to their three-dimensional counterparts, Ruddlesden-Popper phases-layered two-dimensional perovskite films-have shown promising stability, but poor efficiency at only 4.73 per cent(13,16,17). This relatively poor efficiency is attributed to the inhibition of out-of-plane charge transport by the organic cations, which act like insulating spacing layers between the conducting inorganic slabs. Here we overcome this issue in layered perovskites by producing thin films of near-single-crystalline quality, in which the crystallographic planes of the inorganic perovskite component have a strongly preferential out-of-plane alignment with respect to the contacts in planar solar cells to facilitate efficient charge transport. We report a photovoltaic efficiency of 12.52 per cent with no hysteresis, and the devices exhibit greatly improved stability in comparison to their three-dimensional counterparts when subjected to light, humidity and heat stress tests. Unencapsulated two-dimensional perovskite devices retain over 60 per cent of their efficiency for over 2,250 hours under constant, standard (AM1.5G) illumination, and exhibit greater tolerance to 65 per cent relative humidity than do three-dimensional equivalents. When the devices are encapsulated, the layered devices do not show any degradation under constant AM1.5G illumination or humidity. We anticipate that these results will lead to the growth of single-crystalline, solution-processed, layered, hybrid, perovskite thin films, which are essential for high-performance opto-electronic devices with technologically relevant long-term stability. C1 [Tsai, Hsinhan; Nie, Wanyi; Blancon, Jean-Christophe; Neukirch, Amanda J.; Crochet, Jared J.; Tretiak, Sergei; Gupta, Gautam; Mohite, Aditya D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Tsai, Hsinhan; Verduzco, Rafael; Lou, Jun; Ajayan, Pulickel M.] Rice Univ, Dept Mat Sci & Nanoengn, Houston, TX 77005 USA. [Toumpos, Constantinos C. S.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Toumpos, Constantinos C. S.; Harutyunyan, Boris; Bedzyk, Michael J.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Mat Sci, Evanston, IL 60208 USA. [Toumpos, Constantinos C. S.; Harutyunyan, Boris; Bedzyk, Michael J.; Kanatzidis, Mercouri G.] Northwestern Univ, Engn & Argonne Northwestern Solar Energy Res ANSE, Evanston, IL 60208 USA. [Asadpour, Reza; Alam, Muhammad A.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Verduzco, Rafael] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. [Pedesseau, Laurent; Even, Jacky] INSA Rennes, CNRS, UMR 6082, Fonct Opt Technol Informat,FOTON, F-35708 Rennes, France. RP Mohite, AD (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM amohite@lanl.gov RI Tretiak, Sergei/B-5556-2009; even, jacky/C-6212-2008; OI Tretiak, Sergei/0000-0001-5547-3647; even, jacky/0000-0002-4607-3390; Blancon, Jean-Christophe/0000-0002-3833-5792; Crochet, Jared/0000-0002-9570-2173; Stoumpos, Constantinos/0000-0001-8396-9578 FU ANSER Center, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; French national centres (GENCI/CINES/IDRIS grant) [2015-c2012096724]; Cellule Energie du CNRS (SOLHYBTRANS Project); University of Rennes 1 (Action Incitative, Defis Scientifique Emergents); Fondation d'entreprises banque Populaire de l'Ouest; Bay Area PV Consortium (a Department of Energy project with Prime Award) [DE-EE0004946]; NSF [DMR-1352099] FX This work at LANL was LANL LDRD programme (A.D.M., G.G., J.-C.B. and S.T.). Work at Northwestern University was supported as part of the ANSER Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001059. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Work at INSA de Rennes was performed using high-performance computational resources from the French national centres (GENCI/CINES/IDRIS grant 2015-c2012096724), Cellule Energie du CNRS (SOLHYBTRANS Project) and the University of Rennes 1 (Action Incitative,Defis Scientifique Emergents 2015). J.E.'s work is also supported by the Fondation d'entreprises banque Populaire de l'Ouest (Grant PEROPHOT 2015). The work at Purdue University was supported by the Bay Area PV Consortium (a Department of Energy project with Prime Award number DE-EE0004946). This work at LANL was done in part at the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnologies (CINT). R.V. acknowledges the support of the NSF DMR-1352099. NR 36 TC 62 Z9 62 U1 285 U2 323 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD AUG 18 PY 2016 VL 536 IS 7616 BP 312 EP + DI 10.1038/nature18306 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9GN UT WOS:000381804900031 ER PT J AU Bhat, R Chakraborty, M Glimm, T Stewart, TA Newman, SA AF Bhat, Ramray Chakraborty, Mahul Glimm, Tilmann Stewart, Thomas A. Newman, Stuart A. TI Deep phylogenomics of a tandem-repeat galectin regulating appendicular skeletal pattern formation SO BMC EVOLUTIONARY BIOLOGY LA English DT Article DE Galectin-8; Limb skeleton; Pattern formation; Mathematical modeling; Homology; Phylogeny ID CARBOHYDRATE-RECOGNITION DOMAINS; CELL-ADHESION; PHYLOGENETIC ANALYSIS; SEQUENCE ALIGNMENT; VERTEBRATE LIMB; HOX-GENES; NETWORK; FIN; BIOINFORMATICS; IDENTIFICATION AB Background: A multiscale network of two galectins Galectin-1 (Gal-1) and Galectin-8 (Gal-8) patterns the avian limb skeleton. Among vertebrates with paired appendages, chondrichthyan fins typically have one or more cartilage plates and many repeating parallel endoskeletal elements, actinopterygian fins have more varied patterns of nodules, bars and plates, while tetrapod limbs exhibit tandem arrays of few, proximodistally increasing numbers of elements. We applied a comparative genomic and protein evolution approach to understand the origin of the galectin patterning network. Having previously observed a phylogenetic constraint on Gal-1 structure across vertebrates, we asked whether evolutionary changes of Gal-8 could have critically contributed to the origin of the tetrapod pattern. Results: Translocations, duplications, and losses of Gal-8 genes in Actinopterygii established them in different genomic locations from those that the Sarcopterygii (including the tetrapods) share with chondrichthyans. The sarcopterygian Gal-8 genes acquired a potentially regulatory non-coding motif and underwent purifying selection. The actinopterygian Gal-8 genes, in contrast, did not acquire the non-coding motif and underwent positive selection. Conclusion: These observations interpreted through the lens of a reaction-diffusion-adhesion model based on avian experimental findings can account for the distinct endoskeletal patterns of cartilaginous, ray-finned, and lobe-finned fishes, and the stereotypical limb skeletons of tetrapods. C1 [Bhat, Ramray] Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Chakraborty, Mahul] Univ Calif Irvine, Dept Ecol & Evolutionary Biol, Irvine, CA 92697 USA. [Glimm, Tilmann] Western Washington Univ, Dept Math, Bellingham, WA 98229 USA. [Stewart, Thomas A.] Yale Univ, Dept Ecol & Evolutionary Biol, New Haven, CT 06520 USA. [Stewart, Thomas A.] Univ Minnesota, Minnesota Ctr Philosophy Sci, Minneapolis, MN 55455 USA. [Newman, Stuart A.] New York Med Coll, Dept Cell Biol & Anat, Valhalla, NY 10595 USA. [Bhat, Ramray] Indian Inst Sci, Dept Mol Reprod Dev & Genet, Bangalore 560012, Karnataka, India. RP Bhat, R (reprint author), Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA.; Newman, SA (reprint author), New York Med Coll, Dept Cell Biol & Anat, Valhalla, NY 10595 USA.; Bhat, R (reprint author), Indian Inst Sci, Dept Mol Reprod Dev & Genet, Bangalore 560012, Karnataka, India. EM ramray@mrdg.iisc.ernet.in; newman@nymc.edu NR 57 TC 0 Z9 0 U1 4 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2148 J9 BMC EVOL BIOL JI BMC Evol. Biol. PD AUG 18 PY 2016 VL 16 AR 162 DI 10.1186/s12862-016-0729-6 PG 11 WC Evolutionary Biology; Genetics & Heredity SC Evolutionary Biology; Genetics & Heredity GA DT9JC UT WOS:000381814200001 PM 27538950 ER PT J AU Chen, L Rago, NLD Bloom, ID Shaw, LL AF Chen, Lin Rago, Nancy L. Dietz Bloom, Ira D. Shaw, Leon L. TI New insights into the electrode mechanism of lithium sulfur batteries via air-free post-test analysis SO CHEMICAL COMMUNICATIONS LA English DT Article ID X-RAY-DIFFRACTION; IN-SITU; ION BATTERIES; ENERGY-STORAGE; CARBON; PERFORMANCE; CATHODE; SPECTROSCOPY; LI2S AB Effects of the volume expansion and shrinkage of Li2S cathodes on electrochemical cycle life are investigated via post-test analysis without exposure to air. The engineered electrodes that confine volume changes within micro-reactors have significantly longer life than the electrodes without the micro-reactor structure, providing the first unambiguous evidence of the importance of confining volume changes for improved battery performance. C1 [Chen, Lin; Shaw, Leon L.] IIT, Dept Mech Mat & Aerosp Engn, Chicago, IL 60616 USA. [Chen, Lin] Argonne Natl Lab, Div Energy Syst, Lemont, IL USA. [Rago, Nancy L. Dietz; Bloom, Ira D.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL USA. RP Shaw, LL (reprint author), IIT, Dept Mech Mat & Aerosp Engn, Chicago, IL 60616 USA. EM lshaw2@iit.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy (DOE), Office of Vehicle Technologies [DE-AC02-06CH11357] FX Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The work at Argonne National Laboratory was performed under the auspices of the U.S. Department of Energy (DOE), Office of Vehicle Technologies, under Contract No. DE-AC02-06CH11357. NR 33 TC 0 Z9 0 U1 16 U2 29 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 18 PY 2016 VL 52 IS 64 BP 9913 EP 9916 DI 10.1039/c6cc04401h PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DU3FC UT WOS:000382095200012 PM 27430393 ER PT J AU Pan, BF Feng, ZX Sa, NY Han, SD Ma, Q Fenter, P Vaughey, JT Zhang, ZC Liao, C AF Pan, Baofei Feng, Zhenxing Sa, Niya Han, Sang-Don Ma, Qing Fenter, Paul Vaughey, John T. Zhang, Zhengcheng Liao, Chen TI Advanced hybrid battery with a magnesium metal anode and a spinet LiMn2O4 cathode SO CHEMICAL COMMUNICATIONS LA English DT Article ID RECHARGEABLE MG BATTERIES; WIDE ELECTROCHEMICAL WINDOWS; ELECTROLYTE-SOLUTIONS; HIGH-VOLTAGE; MGCL2 AB Two Mg-Li dual salt hybrid electrolytes are developed, which exhibit excellent oxidative stability up to around 3.8 V (vs. Mg/Mg2+) on an aluminum current collector, enabling the successful coupling of several state-of-the-art lithium-ion intercalation cathodes (LiMn2O4, LiCoO2 and LiNi1/3Mn1/3Co1/3O2) with magnesium metal anodes. The Mg-LiMn2O4 battery delivers an initial discharge capacity of about 106 mA h g(-1) with a working voltage of around 2.8 V (vs. Mg/Mg2+), highlighting the highest working voltage of rechargeable batteries with magnesium metal anodes to date. C1 [Pan, Baofei; Feng, Zhenxing; Sa, Niya; Han, Sang-Don; Fenter, Paul; Vaughey, John T.; Zhang, Zhengcheng; Liao, Chen] Argonne Natl Lab, Chem Sci & Engn Div, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. [Ma, Qing] Argonne Natl Lab, Synchrotron Res Ctr, DND CAT, Lemont, IL 60439 USA. RP Pan, BF; Liao, C (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. EM panb@anl.gov; liaoc@anl.gov RI SA, NIYA/E-8521-2017 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Argonne National Laboratory (Advanced Photon Source), a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. Argonne National Laboratory (including Advanced Photon Source), a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. NR 30 TC 2 Z9 2 U1 52 U2 69 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 EI 1364-548X J9 CHEM COMMUN JI Chem. Commun. PD AUG 18 PY 2016 VL 52 IS 64 BP 9961 EP 9964 DI 10.1039/c6cc04133g PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DU3FC UT WOS:000382095200024 PM 27439946 ER PT J AU Wang, H Valkunas, L Cao, T Whittaker-Brooks, L Fleming, GR AF Wang, He Valkunas, Leonas Cao, Thu Whittaker-Brooks, Luisa Fleming, Graham R. TI Coulomb Screening and Coherent Phonon in Methylammonium Lead Iodide Perovskites SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITES; EXCITON BINDING-ENERGY; SOLAR-CELLS; CHARGE-CARRIERS; ORTHORHOMBIC PHASES; REFRACTIVE-INDEX; CH3NH3PBI3; RECOMBINATION; SPECTROSCOPY; TRANSITION AB Methylammonium lead iodide (CH3NH3PbI3) hybrid perovskite in the tetragonal and orthorhombic phases have different exciton binding energies and demonstrate different excitation kinetics. Here, we explore the role that crystal structure plays in the kinetics via fluence dependent transient absorption spectroscopy. We observe stronger saturation of the free carrier concentration under high pump energy density in the orthorhombic phase relative to the tetragonal phase. We attribute this phenomenon to small dielectric constant, large exciton binding energy, and weak Coulomb screening, which results in difficult exciton dissociation under high light intensity in the orthorhombic phase. At higher excitation intensities, we observe a coherent phonon with an oscillation frequency of 23.4 cm(-1) at 77 K, whose amplitude tracks the increase of the first-order lifetime. C1 [Wang, He; Cao, Thu; Fleming, Graham R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Wang, He; Cao, Thu; Fleming, Graham R.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Wang, He; Cao, Thu; Fleming, Graham R.] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Wang, He; Cao, Thu; Fleming, Graham R.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Valkunas, Leonas] Vilnius Univ, Theoret Phys Dept, LT-10222 Vilnius, Lithuania. [Valkunas, Leonas] Ctr Phys Sci & Technol, Mol Compound Phys Dept, LT-10222 Vilnius, Lithuania. [Whittaker-Brooks, Luisa] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. RP Fleming, GR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Fleming, GR (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA.; Fleming, GR (reprint author), Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA.; Fleming, GR (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM grfleming@lbl.gov FU National Science Foundation (NSF) [CHE-1012168, CHE-1362830]; Research Council of Lithuania (LMT) [MTP-080/2015] FX This work was supported by the National Science Foundation (NSF) under Awards CHE-1012168 and CHE-1362830. L.V. was supported by the Research Council of Lithuania (LMT Grant No. MTP-080/2015). NR 39 TC 1 Z9 1 U1 20 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD AUG 18 PY 2016 VL 7 IS 16 BP 3284 EP 3289 DI 10.1021/acs.jpclett.6b01425 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DT8YO UT WOS:000381781800035 PM 27485190 ER PT J AU Ma, CX Park, J Liu, L Kim, YS Yoon, M Baddorf, AP Gu, G Li, AP AF Ma, Chuanxu Park, Jewook Liu, Lei Kim, Yong-Sung Yoon, Mina Baddorf, Arthur P. Gu, Gong Li, An-Ping TI Interplay between intercalated oxygen superstructures and monolayer h-BN on Cu(100) SO PHYSICAL REVIEW B LA English DT Article ID HEXAGONAL BORON-NITRIDE; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; INDUCED RECONSTRUCTION; GRAPHENE EDGES; HIGH-QUALITY; BASIS-SET; OXIDATION; COPPER; HETEROSTRUCTURES AB The confinement effect of intercalated atoms in van der Waals heterostructures can lead to interesting interactions between the confined atoms or molecules and the overlaying two-dimensional (2D) materials. Here we report the formation of ordered Cu(100) p(2 x 2) oxygen superstructures by oxygen intercalation under the monolayer hexagonal boron nitride (h-BN) on Cu after annealing. By using scanning tunneling microscopy and x-ray photoelectron spectroscopy, we identify the superstructure and reveal its roles in passivating the exposed Cu surfaces, decoupling h-BN and Cu, and disintegrating h-BN monolayers. The oxygen superstructure appears as a 2D pattern on the exposed Cu surface or quasi-1D stripes of paired oxygen intercalated in the interface of h-BN and Cu predominantly oriented along the moire modulations. The oxygen superstructure is shown to etch the overlaying h-BN monolayer in a thermal annealing process. After extended annealing, the h-BN monolayer disintegrates into nanoislands with zigzag edges. We discuss the implications of these findings on the stability and oxidation resistance of h-BN and relate them to challenges in process integration and 2D heterostructures. C1 [Ma, Chuanxu; Park, Jewook; Kim, Yong-Sung; Yoon, Mina; Baddorf, Arthur P.; Li, An-Ping] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Liu, Lei; Kim, Yong-Sung; Yoon, Mina; Gu, Gong] Univ Tennessee, Knoxville, TN 37996 USA. [Kim, Yong-Sung] Korea Res Inst Stand & Sci, Yuseong 305340, Daejeon, South Korea. [Kim, Yong-Sung] Korea Univ Sci & Technol, Dept Nano Sci, Daejeon 305350, South Korea. RP Li, AP (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM apli@ornl.gov RI Li, An-Ping/B-3191-2012; OI Li, An-Ping/0000-0003-4400-7493; Ma, Chuanxu/0000-0001-6478-5917 FU NSF [ECCS-1231808]; DARPA [HR0011-13-2-0016]; National Energy Research Scientific Computing Center, a DOE Office of Science User Facility [DE-AC02-05CH11231] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. STM measurements by C.M. were supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U. S. DOE. The work at UTK was supported by NSF (Grant No. ECCS-1231808) and DARPA (Grant No. HR0011-13-2-0016). Computational research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility under Contract No. DE-AC02-05CH11231. NR 66 TC 1 Z9 1 U1 28 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2016 VL 94 IS 6 AR 064106 DI 10.1103/PhysRevB.94.064106 PG 8 WC Physics, Condensed Matter SC Physics GA DT6MV UT WOS:000381599300003 ER PT J AU Sirica, N Mo, SK Bondino, F Pis, I Nappini, S Vilmercati, P Yi, J Gai, Z Snijders, PC Das, PK Vobornik, I Ghimire, N Koehler, MR Li, L Sapkota, D Parker, DS Mandrus, DG Mannella, N AF Sirica, N. Mo, S. -K. Bondino, F. Pis, I. Nappini, S. Vilmercati, P. Yi, J. Gai, Z. Snijders, P. C. Das, P. K. Vobornik, I. Ghimire, N. Koehler, M. R. Li, L. Sapkota, D. Parker, D. S. Mandrus, D. G. Mannella, N. TI Electronic structure of the chiral helimagnet and 3d-intercalated transition metal dichalcogenide Cr1/3NbS2 SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-PROPERTIES; WEAK FERROMAGNETISM; VALLEY POLARIZATION; PHOTOEMISSION; 2H-NBSE2; SKYRMIONS; INTERCALATION; NIOBIUM; NBS2; MOS2 AB The electronic structure of the chiral helimagnet Cr1/3NbS2 has been studied with core level and angle-resolved photoemission spectroscopy (ARPES). Intercalated Cr atoms are found to be effective in donating electrons to the NbS2 layers but also cause significant modifications of the electronic structure of the host NbS2 material. In particular, the data provide evidence that a description of the electronic structure of Cr1/3NbS2 on the basis of a simple rigid band picture is untenable. The data also reveal substantial inconsistencies with the predictions of standard density functional theory. The relevance of these results to the attainment of a correct description of the electronic structure of chiral helimagnets, magnetic thin films/multilayers, and transition metal dichalcogenides intercalated with 3d magnetic elements is discussed. C1 [Sirica, N.; Vilmercati, P.; Snijders, P. C.; Ghimire, N.; Sapkota, D.; Mandrus, D. G.; Mannella, N.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Mo, S. -K.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bondino, F.; Pis, I.; Nappini, S.; Das, P. K.; Vobornik, I.] CNR, IOM, Lab TASC, SS 14 Km 163-5, I-34149 Basovizza, TS, Italy. [Pis, I.] Elettra Sincrotrone Trieste SCpA, SS 14 Km 163-5, I-34149 Basovizza, TS, Italy. [Das, P. K.] Abdus Salaam Int Ctr Theoret Phys, Str Costiera 11, I-34100 Trieste, Italy. [Yi, J.; Koehler, M. R.; Li, L.; Mandrus, D. G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Gai, Z.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Gai, Z.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Snijders, P. C.; Parker, D. S.; Mandrus, D. G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Mannella, N (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM nmannell@utk.edu RI Mo, Sung-Kwan/F-3489-2013; Gai, Zheng/B-5327-2012; Vobornik, Ivana/A-7461-2011; Vilmercati, Paolo/E-5655-2017; OI Mo, Sung-Kwan/0000-0003-0711-8514; Gai, Zheng/0000-0002-6099-4559; Vobornik, Ivana/0000-0001-9957-3535; Vilmercati, Paolo/0000-0002-3872-8828; Bondino, Federica/0000-0001-6505-9319 FU National Science Foundation, Division of Material Research [DMR-1151687]; National Science Foundation [DMR-1410428]; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Basic Energy Sciences of the DOE [DE-AC02-05CH1123] FX N.M. acknowledges that this work was supported by the National Science Foundation, Division of Material Research, Grant No. DMR-1151687. D.G.M. acknowledges support from National Science Foundation Award No. DMR-1410428. P.C.S. and D.S.P. are supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The Advanced Light Source is supported by the Office of Basic Energy Sciences of the DOE under Contract No. DE-AC02-05CH1123. The STM characterization was conducted at the Center for Nanophase Materials Science, which is a DOE office of Science User Facility. This work has been partly performed in the framework of the Nanoscience Foundry and Fine Analysis (NFFA-MIUR Italy) project. NR 63 TC 0 Z9 0 U1 21 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 18 PY 2016 VL 94 IS 7 AR 075141 DI 10.1103/PhysRevB.94.075141 PG 19 WC Physics, Condensed Matter SC Physics GA DT6NG UT WOS:000381600400002 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Aushev, V Aushev, Y Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brochmann, M Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cuth, J Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, A Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Franc, J Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schott, M Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stefaniuk, N Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhu, BZJ Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Aushev, V. Aushev, Y. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Borysova, M. Brandt, A. Brandt, O. Brochmann, M. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cuth, J. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, A. Evdokimov, V. N. Faure, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Franc, J. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Gogota, O. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Grunendahl, S. Grunewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kaur, M. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Savitskyi, M. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schott, M. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Snow, G. R. Snow, J. Snyder, S. Soldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stefaniuk, N. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of the top quark mass using the matrix element technique in dilepton final states SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; RUN-II; SEMILEPTONIC DECAYS; JET IDENTIFICATION; PAIR PRODUCTION; CROSS-SECTION; D0 EXPERIMENT; DETECTOR; COLLISIONS AB We present a measurement of the top quark mass in p (p) over bar collisions at a center-of-mass energy of 1.96 TeV at the Fermilab Tevatron collider. The data were collected by the D0 experiment corresponding to an integrated luminosity of 9.7 fb(-1). The matrix element technique is applied to t (t) over bar events in the final state containing leptons (electrons or muons) with high transverse momenta and at least two jets. The calibration of the jet energy scale determined in the lepton + jets final state of t (t) over bar decays is applied to jet energies. This correction provides a substantial reduction in systematic uncertainties. We obtain a top quark mass of m(t) = 173.93 +/- 1.84 GeV. C1 [Hensel, C.; Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, BR-22290 Rio De Janeiro, RJ, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550 Rio De Janeiro, RJ, Brazil. [Mercadante, P. G.] Univ Fed ABC, BR-09210 Sao Paulo, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota 111711, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague 11636 1, Czech Republic. [Augsten, K.; Franc, J.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, Prague 11636 6, Czech Republic. [Kupco, A.; Lokajicek, M.; Royon, C.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. [Hoeneisen, B.] Univ San Francisco Quito, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, CNRS IN2P3, LPC, F-63178 Aubiere, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS IN2P3, Inst Natl Polytech Grenoble, LPSC, F-38026 Grenoble, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CNRS IN2P3, CPPM, F-13288 Marseille 09, France. [Grivaz, J. -F.; Guillemin, T.; Jaffre, M.; Petroff, P.] Univ Paris Saclay, Univ Paris 11, CNRS IN2P3, LAL, F-91898 Orsay, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 06, LPNHE, CNRS IN2P3, F-75005 Paris, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 07, LPNHE, CNRS IN2P3, F-75005 Paris, France. [Bassler, U.; Besancon, M.; Chapon, E.; Couderc, F.; Deliot, F.; Faure, A.; Grohsjean, A.; Hubacek, Z.; Shary, V.; Titov, M.; Tuchming, B.; Vilanova, D.] CEA Saclay, Irfu, SPP, F-91191 Gif Sur Yvette, France. [Greder, S.; Miconi, F.; Ripp-Baudot, I.] Univ Strasbourg, CNRS IN2P3, IPHC, F-67037 Strasbourg, France. 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[Luna-Garcia, R.] Ctr Invest Computac IPN, Mexico City 07738, DF, Mexico. [Santos, A. S.] Univ Estadual Paulista, BR-01140 Sao Paulo, SP, Brazil. [Meyer, J.] SCC, KIT, D-76128 Karlsruhe, Germany. [Patwa, A.] US DOE, Washington, DC 20585 USA. [Cooke, M.] Amer Assoc Advancement Sci, Washington, DC 20005 USA. [Borysova, M.] KINR, UA-03680 Kiev, Ukraine. [Jabeen, S.] Univ Maryland, College Pk, MD 20742 USA. [Williams, M. R. J.] European Org Nucl Res CERN, CH-1211 Geneva, Switzerland. [Jung, A. W.] Purdue Univ, W Lafayette, IN 47907 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna 141980, Russia. RI Dudko, Lev/D-7127-2012; Gutierrez, Phillip/C-1161-2011; Li, Liang/O-1107-2015; OI Dudko, Lev/0000-0002-4462-3192; Li, Liang/0000-0001-6411-6107; Williams, Mark/0000-0001-5448-4213; Bertram, Iain/0000-0003-4073-4941 FU Department of Energy (United States of America); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); National Research Center "Kurchatov Institute" of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine); National Science Foundation (United States of America); Ministry of Education and Science of the Russian Federation (Russia); National Council for the Development of Science and Technology (Brazil); Science and Technology Facilities Council (United Kingdom) FX We thank the staffs at Fermilab and collaborating institutions and acknowledge support from the Department of Energy and National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center "Kurchatov Institute" of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council and The Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). NR 52 TC 1 Z9 1 U1 9 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 18 PY 2016 VL 94 IS 3 AR 032004 DI 10.1103/PhysRevD.94.032004 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DT6OL UT WOS:000381603500001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJ Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, B Piqueras, D Alviggi, MG Amadio, BT Amako, K Coutinho, Y Amelung, C Amidei, D Dos Santos, SP Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK 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Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. TI Measurement of fiducial differential cross sections of gluon-fusion production of Higgs bosons decaying to WW (au)-> e nu mu nu with the ATLAS detector at TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments) ID PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; LHC AB This paper describes a measurement of fiducial and differential cross sections of gluon-fusion Higgs boson production in the H -> W W (au)-> e nu mu nu channel, using 20.3 fb(-1) of proton-proton collision data. The data were produced at a centre-of-mass energy of TeV at the CERN Large Hadron Collider and recorded by the ATLAS detector in 2012. Cross sections are measured from the observed H -> W W (au)-> e nu mu nu signal yield in categories distinguished by the number of associated jets. The total cross section is measured in a fiducial region defined by the kinematic properties of the charged leptons and neutrinos. Differential cross sections are reported as a function of the number of jets, the Higgs boson transverse momentum, the dilepton rapidity, and the transverse momentum of the leading jet. The jet-veto efficiency, or fraction of events with no jets above a given transverse momentum threshold, is also reported. All measurements are compared to QCD predictions from Monte Carlo generators and fixed-order calculations, and are in agreement with the Standard Model predictions. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Duran Yildiz, H.] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Grevtsov, K.; Guillemin, T.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Levque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Smart, B. H.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mt Blanc, LAPP, CNRS IN2P, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; LeCompte, T.; Love, J.; Malon, D.; Metcalfe, J.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Ryu, S.; Stanek, R. 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[Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Istanbul Bilgi Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Beddall, A. J.] Bahcesehir Univ, Fac Engn & Nat Sci, Istanbul, Turkey. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Giacobbe, B.; Giorgi, F. M.; Negrini, M.; Polini, A.; Rinaldi, L.; Sbarra, C.; Spighi, R.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, F.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Lasagni Manghi, F.; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Ucchielli, G.; Valentinetti, S.; Villa, M.; Vittori, C.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Grefe, C.; Haefner, P.; Hagebock, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Kruger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; MijoviAO, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Yau Wong, K. H.; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Phys Inst, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio Janeiro COPPE EE, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.; Peralva, B. S.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Oliveira Damazio, D.; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Bossio Sola, J. D.; Marceca, G.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Valentino, D. Di; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Pasztor, G.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Alvarez Gonzalez, B.; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Capeans Garrido, M. D. M.; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Henriques Correia, A. M.; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Lehmann Miotto, G.; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Montejo Berlingen, J.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; PommSs, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Pozo Astigarraga, M. E.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Solans Sanchez, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Bryant, P.; Camacho Toro, R.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Barreiro Guimares da Costa, J.; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Hu, Q.; Jiang, Y.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Zaidan, R.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. 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C.; Gao, Y.; Garay Walls, F. M.; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Olivares Pino, S. A.; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; JavA-rek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagaova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Albert Ludwigs Univ, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Bilbao De Mendizabal, J.; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; RistiAO, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Darbo, G.; Gemme, C.; Morettini, P.; Passaggio, S.; Rossi, L. P.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Ferretto Parodi, A.; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Justus Liebig Univ Giessen, Phys Inst 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Breaden Madden, W. D.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Ferreira de Lima, D. E.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Moreno Llacer, M.; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Georg August Univ, Phys Inst 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Lopez Mateos, D.; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Meyer Zu Theenhausen, H.; Narrias Villar, D. I.; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Chan, Y. L.; Flores Castillo, L. R.; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Lorenzo Martinez, N.; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, CONICET, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Primavera, M.] INFN Sez Lecce, Lecce, Italy. [Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipi, A.; Goriek, A.; Kerevan, B. P.; Kramberger, G.; Maek, B.; MandiAO, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Dept Phys, Jozef Stefan Inst, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Faucci Giannelli, M.; George, S.; Gibson, S. M.; Kempster, J. J.; Panduro Vazquez, J. G.; Pastore, Fr.; Savage, G.; Sowden, B. C.; Span, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Gutierrez Ortiz, N. G.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Lopez Solis, A.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Lab Phys Nucl & Hautes Energies, UPMC, CNRS IN2P3, Paris, France. [kesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Fullana Torregrosa, E.; Groh, S.; Heck, T.; Hohlfeld, M.; Hulsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Iturbe Ponce, J. M.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Munoz Sanchez, F. J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Ticse Torres, R. E.; Tisserant, S.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Vazquez Schroeder, T.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Cavalli, D.; Costa, G.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Resconi, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Dallaire, F.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Rezvani, R.; Shoaleh Saadi, D.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Losel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Ludwig Maximilians Univ Munchen, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Carlino, G.; de Asmundis, R.; Doria, A.; Izzo, V.; Sekhniaidze, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Bogdanchikov, A. G.; Malyshev, V. M.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, LAL, CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Crispin Ortuzar, M.; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Ferrari, R.; Gaudio, G.; Lanza, A.; Polesello, G.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, Kurchatov Inst, BP Konstantinov Peterburg Nucl Phys Inst, St Petersburg, Russia. INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Araque, J. P.; Cantrill, R.; Lopes, L.; Oleiro Seabra, L. F.; Santos, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muio, P.; Cunha Sargedas De Sousa, M. J. Da; Jorge, P. M.; Machado Miguens, J.; Maneira, J.; Palma, A.; Pedro, R.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, CEFITEC, Fac Ciencias Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; De Pedis, D.; De Salvo, A.; Falciano, S.; Luminari, L.; Marzano, F.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Safai Tehrani, F.; Vari, R.; Veneziano, S.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Cardarelli, R.; Liberti, B.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Farilla, A.; Graziani, E.; Iodice, M.; Stanescu, C.] INFN Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Dano Hoffmann, M.; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Goncalves Pinto Firmino Da Costa, J.; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; Sales De Bruin, P. H.; Torr Pastor, E.; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Cuhadar Donszelmann, T.; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Lopez Paredes, B.; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Vickey Boeriu, O. E.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Black, J. E.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zeni, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Mellado Garcia, B. R.; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Bohm, C.; Silverstein, S. B.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; sman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia Bylund, O.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Valdes Santurio, E.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Chavez Barajas, C. A.; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Abdallah, J.; Hou, S.; Lee, S. C.; Li, B.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Sinervo, P.; Taenzer, J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Perez Codina, E.; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC, Canada. [Benitez Garcia, J. A.; Manjarres Ramos, J.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Bergeaas Kuutmann, E.; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Caminal Armadans, R.; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Hign-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Dept Fis Atom Mol & Nucl,CSIC, Dept Ingn Elect,Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Pearce, J.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Kohler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kuechler, J. T.; Mattig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Vogel, M.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fak Math & Nat Wissensch, Fachgrp Phys, Wuppertal, Germany. [Baker, O. K.; Benhar Noccioli, E.; Cummings, J.; Demers, S.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Paredes Hernandez, D.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particales IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Banerjee, Sw.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, Barcelona, Spain. [Castro, N. F.] Univ Porto, Dept Fis & Astron, Fac Ciencias, Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys IPP, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA USA. [Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. Aix Marseille Univ, CPPM, Marseille, France. CNRS IN2P3, Marseille, France. RI Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Prokoshin, Fedor/E-2795-2012; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Livan, Michele/D-7531-2012; Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Gladilin, Leonid/B-5226-2011; Garcia, Jose /H-6339-2015; Lazzaroni, Massimo/N-3675-2015; Mashinistov, Ruslan/M-8356-2015; Warburton, Andreas/N-8028-2013; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Tikhomirov, Vladimir/M-6194-2015; Doyle, Anthony/C-5889-2009 OI Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Prokoshin, Fedor/0000-0001-6389-5399; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Livan, Michele/0000-0002-5877-0062; Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Gladilin, Leonid/0000-0001-9422-8636; Lazzaroni, Massimo/0000-0002-4094-1273; Mashinistov, Ruslan/0000-0001-7925-4676; Warburton, Andreas/0000-0002-2298-7315; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Tikhomirov, Vladimir/0000-0002-9634-0581; Doyle, Anthony/0000-0001-6322-6195 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020 and Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex; Investissements d'Avenir Labex and Idex, ANR; Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes by EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society and Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. NR 89 TC 2 Z9 2 U1 28 U2 28 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD AUG 17 PY 2016 IS 8 AR 104 DI 10.1007/JHEP08(2016)104 PG 63 WC Physics, Particles & Fields SC Physics GA DU3JM UT WOS:000382106600001 ER PT J AU Huang, CL Sun, ZW Cui, MM Liu, F Helms, BA Russell, TP AF Huang, Caili Sun, Zhiwei Cui, Mengmeng Liu, Feng Helms, Brett A. Russell, Thomas P. TI Structured Liquids with pH-Triggered Reconfigurability SO ADVANCED MATERIALS LA English DT Article ID WATER/OIL INTERFACES; COLLOIDAL PARTICLES; GRAPHENE-OXIDE; EMULSIONS; DROPLETS; MICROCAPSULES; NANOPARTICLES; TEMPLATES; STABILITY; SILICA AB Through pH-tuning of electrostatic inter actions between polymer ligands and nano particles at structured-liquid interfaces, liquid droplets can be directed between a jammed nonequilibrium state and a dynamic reconfigurable state. The nanoparticle-surfactant dynamics highly depend on the pH, so that the liquids can be structured using an external field and under variation of pH, or alternatively being realized by remote photo-triggering. C1 [Huang, Caili; Liu, Feng; Russell, Thomas P.] Lawrence Berkeley Natl Lab, Div Mat Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. [Huang, Caili; Sun, Zhiwei; Cui, Mengmeng; Russell, Thomas P.] Univ Massachusetts, Polymer Sci & Engn Dept, Conte Ctr Polymer Res, 120 Governors Dr, Amherst, MA 01003 USA. [Helms, Brett A.] Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. [Russell, Thomas P.] Tohoku Univ, WPI AIMR, Aoba Ku, 2-1-1 Katahira, Sendai, Miyagi 9808577, Japan. RP Helms, BA (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. EM bahelms@lbl.gov; tom.p.russell@gmail.com RI Liu, Feng/J-4361-2014; OI Liu, Feng/0000-0002-5572-8512; Helms, Brett/0000-0003-3925-4174 FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231. B.A.H. and T.P.R. were supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 30 TC 0 Z9 0 U1 18 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD AUG 17 PY 2016 VL 28 IS 31 BP 6612 EP + DI 10.1002/adma.201600691 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DU8RJ UT WOS:000382481200011 PM 27214196 ER PT J AU Jorgensen, SW Johnson, TA Payzant, EA Bilheux, HZ AF Jorgensen, Scott W. Johnson, Terry A. Payzant, E. Andrew Bilheux, Hassina Z. TI Anisotropic storage medium development in a full-scale, sodium alanate-based, hydrogen storage system SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Sodium alanate; Neutron diffraction; Neutron computed tomography; Hydrogen storage; Vehicle scale; Catalyzed desorption ID NEUTRON-RADIOGRAPHY; ALUMINUM HYDRIDES; METAL; DESIGN; TANK AB Deuterium desorption in an automotive-scale hydrogen storage tube was studied in-situ using neutron diffraction. Gradients in the concentration of the various alanate phases were observed along the length of the tube but no significant radial anisotropy was present. In addition, neutron radiography and computed tomography showed large scale cracks and density fluctuations, confirming the presence of these structures in an undisturbed storage system. These results demonstrate that large scale storage structures are not uniform even after many absorption/desorption cycles and that movement of gaseous hydrogen cannot be properly modeled by a simple porous bed model. Furthermore, the evidence indicates that there is slow transformation of species at one end of the tube indicating loss of catalyst functionality. These observations explain the unusually fast movement of hydrogen in a full scale system and shows that loss of capacity is not occurring uniformly in this type of hydrogen-storage system. (C) 2016 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved. C1 [Jorgensen, Scott W.] Gen Motors R&D, MC 480-102-000,30500 Mound Rd, Warren, MI 48092 USA. [Johnson, Terry A.] Sandia Natl Lab Thermal Fluids Sci & Engn, 7011 East Ave, Livermore, CA 94551 USA. [Payzant, E. Andrew; Bilheux, Hassina Z.] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Jorgensen, SW (reprint author), GM R&D Labs, CMS Lab, 480-102-000,30500 Mound Rd, Warren, MI 48092 USA. EM scott.w.jorgensen@gm.com; tajohns@sandia.gov; payzanta@ornl.gov; bilheuxhn@ornl.gov RI Payzant, Edward/B-5449-2009; Bilheux, Hassina/H-4289-2012 OI Payzant, Edward/0000-0002-3447-2060; Bilheux, Hassina/0000-0001-8574-2449 FU GM hydrogen program; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, as part of the HTML User Program, Oak Ridge National Laboratory; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We wish to thank the GM hydrogen program that funded the development of the alanate based storage system and for supporting the program as a whole.; A portion of this research at ORNL's High Flux Isotope Reactor and Spallation Neutron Source, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, and by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, as part of the HTML User Program, Oak Ridge National Laboratory. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 34 TC 0 Z9 0 U1 7 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD AUG 17 PY 2016 VL 41 IS 31 BP 13557 EP 13574 DI 10.1016/j.ijhydene.2016.05.057 PG 18 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA DT5OW UT WOS:000381533500025 ER PT J AU Robinson, AE AF Robinson, Alan E. TI Reanalysis of radioisotope measurements of the Be-9(gamma, n)Be-8 cross section SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; INELASTIC ELECTRON-SCATTERING; 1ST EXCITED-STATE; ENERGY-LEVELS; GAMMA-RAYS; BE-9; THRESHOLD; DECAY; PHOTODISINTEGRATION; BERYLLIUM AB The Be-9(gamma, n)Be-8 reaction is enhanced by a near-threshold 1/2(+) state. Contradictions between existing measurements of this reaction cross section affect calculations of astrophysical r-process yields, dark matter detector calibrations, and the theory of the nuclear structure of Be-9. Select well-documented radioisotope Be-9(gamma, n) source yield measurements have been reanalyzed, providing a set of high-accuracy independently measured cross sections without the large systematic errors from recent beamline experiments [ Arnold, Clegg, Iliadis, Karwowski, Rich, Tompkins, and Howell, Phys. Rev. C 85, 044605 (2012); Utsunomiya, Katayama, Gheorghe, Imai, Yamaguchi, Kahl, Sakaguchi, Shima, Takahisa, and Miyamoto, ibid. 92, 064323 (2015)]. A single-level Breit-Wigner fit of these corrected measurement yields are E-R = 1736.8(18) keV, Gamma(gamma) = 0.742(25) eV, and Gamma(n) = 252(17) keV for the 1/2+ state, excluding a virtual state solution. C1 [Robinson, Alan E.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Robinson, AE (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM fbfree@fnal.gov FU Fermi Research Alliance, LLC [De-AC02-07CH-11359]; United States Department of Energy FX This work was derived from my thesis under the guidance of Juan Collar at the University of Chicago. I thank Juan Collar, Charles Arnold, and Hiroaki Utsonomiya for discussions about recent measurements of this cross section. This work was completed with the support of the Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH-11359 with the United States Department of Energy. NR 65 TC 1 Z9 1 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 17 PY 2016 VL 94 IS 2 AR 024613 DI 10.1103/PhysRevC.94.024613 PG 9 WC Physics, Nuclear SC Physics GA DT4ZJ UT WOS:000381489900006 ER PT J AU Van Isacker, P Macchiavelli, AO Fallon, P Zerguine, S AF Van Isacker, P. Macchiavelli, A. O. Fallon, P. Zerguine, S. TI Properties of isoscalar-pair condensates SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; SPIN AB It is pointed out that the ground state of n neutrons and n protons in a single-j shell, interacting through an isoscalar (T = 0) pairing force, is not paired, J = 0, but rather spin aligned, J = n. This observation is explained in the context of a model of isoscalar P (J = 1) pairs, which is mapped onto a system of p bosons, leading to an approximate analytic solution of the isoscalar-pairing limit in jj coupling. C1 [Van Isacker, P.] CEA DRF CNRS IN2P3, Grand Accelerateur Natl Ions Lourds, Bvd Henri Becquerel, F-14076 Caen, France. [Macchiavelli, A. O.; Fallon, P.] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Zerguine, S.] Univ Batna, PRIMALAB Lab, Dept Phys, Ave Boukhelouf M El Hadi, Batna 05000, Algeria. RP Van Isacker, P (reprint author), CEA DRF CNRS IN2P3, Grand Accelerateur Natl Ions Lourds, Bvd Henri Becquerel, F-14076 Caen, France. FU FUSTIPEN (French-U.S. Theory Institute for Physics with Exotic Nuclei) under U.S. DOE Grant [DE-FG02-10ER41700]; U.S. DOE Contract [DE-AC02-05CH11231] FX This work was supported in part by the FUSTIPEN (French-U.S. Theory Institute for Physics with Exotic Nuclei) under U.S. DOE Grant No. DE-FG02-10ER41700 and by the U.S. DOE Contract No. DE-AC02-05CH11231 (LBNL). NR 25 TC 0 Z9 0 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 17 PY 2016 VL 94 IS 2 AR 024324 DI 10.1103/PhysRevC.94.024324 PG 6 WC Physics, Nuclear SC Physics GA DT4ZJ UT WOS:000381489900004 ER PT J AU Cannatelli, MD Ragauskas, AJ AF Cannatelli, Mark D. Ragauskas, Arthur J. TI Ecofriendly syntheses of phenothiazones and related structures facilitated by laccase - a comparative study SO TETRAHEDRON LETTERS LA English DT Article DE Biocatalysis; Green chemistry; Laccase; Phenothiazones; Thiol-amine ID ONE-POT SYNTHESIS; FUNGAL LACCASES; KRAFT PULPS; BIOLOGICAL EVALUATION; CATALYZED SYNTHESIS; BACTERIAL LACCASES; ANTIFUNGAL AGENTS; P-HYDROQUINONES; DERIVATIVES; CATECHOLS AB The biocatalytic synthesis of phenothiazones and related compounds has been achieved in an aqueous system under mild conditions facilitated by laccase oxidation. It was found that by coupling 2-aminothiophenol directly with 1,4-quinones, the product yields could be significantly increased compared to generating the 1,4-quinones in situ from the corresponding hydroquinones via laccase oxidation. However, laccase still proved to be pivotal for achieving highest product yields by catalyzing the final oxidation step. Furthermore, a difference in reactivity of aromatic and aliphatic amines toward 1,4-naphthoquinone is observed. This study provides a sustainable approach to the synthesis of a biologically important class of compounds. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Cannatelli, Mark D.; Ragauskas, Arthur J.] Georgia Inst Technol, Sch Chem & Biochem, Renewable Bioprod Inst, Atlanta, GA 30332 USA. [Ragauskas, Arthur J.] Oak Ridge Natl Lab, Biosci Div, Joint Inst Biol Sci, Oak Ridge, TN 37831 USA. [Ragauskas, Arthur J.] Univ Tennessee, Dept Chem & Biomol Engn, Dept Forestry Wildlife & Fisheries, Knoxville, TN 37996 USA. RP Ragauskas, AJ (reprint author), Georgia Inst Technol, Sch Chem & Biochem, Renewable Bioprod Inst, Atlanta, GA 30332 USA.; Ragauskas, AJ (reprint author), Oak Ridge Natl Lab, Biosci Div, Joint Inst Biol Sci, Oak Ridge, TN 37831 USA.; Ragauskas, AJ (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Dept Forestry Wildlife & Fisheries, Knoxville, TN 37996 USA. EM aragausk@utk.edu FU Renewable Bioproducts Institute at Georgia Institute of Technology FX The authors are thankful for a student fellowship supported by the Renewable Bioproducts Institute at Georgia Institute of Technology. NR 71 TC 0 Z9 0 U1 6 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4039 J9 TETRAHEDRON LETT JI Tetrahedron Lett. PD AUG 17 PY 2016 VL 57 IS 33 BP 3749 EP 3753 DI 10.1016/j.tetlet.2016.07.016 PG 5 WC Chemistry, Organic SC Chemistry GA DT5QC UT WOS:000381536700017 ER PT J AU Gilmore, SF Blanchette, CD Scharadin, TM Hura, GL Rasley, A Corzett, M Pan, CX Fischer, NO Henderson, PT AF Gilmore, Sean F. Blanchette, Craig D. Scharadin, Tiffany M. Hura, Greg L. Rasley, Amy Corzett, Michele Pan, Chong-xian Fischer, Nicholas O. Henderson, Paul T. TI Lipid Cross-Linking of Nanolipoprotein Particles Substantially Enhances Serum Stability and Cellular Uptake SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE nanoparticles; drug delivery; rHDL; NLP; DiynePC; serum stability; cross-linking ID HIGH-DENSITY-LIPOPROTEINS; MEMBRANE-PROTEINS; SCATTERING SAXS; AMPHOTERICIN-B; CREMOPHOR-FREE; DRUG-DELIVERY; NANOPARTICLES; PACLITAXEL; NANODISCS; APOLIPOPROTEIN AB Nanolipoprotein particles (NLPs) consist of a discoidal phospholipid lipid bilayer confined by an apolipoprotein belt. NLPs are a promising platform for a variety of biomedical applications due to their biocompatibility, size, definable composition, and amphipathic characteristics. However, poor serum stability hampers the use of NLPs for in vivo applications such as drug formulation. In this study, NLP stability was enhanced upon the incorporation and subsequent UV-mediated intermolecular cross-linking of photoactive DiynePC phospholipids in the lipid bilayer, forming cross-linked nanoparticles (X-NLPs). Both the concentration of DiynePC in the bilayer and UV exposure time significantly affected the resulting X-NLP stability in 100% serum, as assessed by size exclusion chromatography (SEC) of fluorescently labeled particles. Cross-linking did not significantly impact the size of X-NLPs as determined by dynamic light scattering and SEC. X-NLPs had essentially no degradation over 48 h in 100% serum, which is a drastic improvement compared to non-cross-linked NLPs (50% degradation by similar to 10 min). X-NLPs had greater uptake into the human ATCC 5637 bladder Cancer cell line compared to non-cross-linked particles, indicating their potential utility for targeted drug delivery. X-NLPs also exhibited enhanced stability following intravenous administration in mice. These results collectively support the potential utility of X-NLPs for a variety of in vivo applications. C1 [Gilmore, Sean F.; Blanchette, Craig D.; Rasley, Amy; Corzett, Michele; Fischer, Nicholas O.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Livermore, CA 94551 USA. [Scharadin, Tiffany M.; Pan, Chong-xian; Henderson, Paul T.] Univ Calif Davis, Dept Internal Med, Div Hematol & Oncol, 4501 10 St,Room 3016, Sacramento, CA 95817 USA. [Scharadin, Tiffany M.; Pan, Chong-xian; Henderson, Paul T.] Univ Calif Davis, Ctr Comprehens Canc, Sacramento, CA 95817 USA. [Hura, Greg L.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Hura, Greg L.] Univ Calif Santa Cruz, Chem & Biochem, Santa Cruz, CA 95064 USA. RP Fischer, NO (reprint author), Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Livermore, CA 94551 USA.; Henderson, PT (reprint author), Univ Calif Davis, Dept Internal Med, Div Hematol & Oncol, 4501 10 St,Room 3016, Sacramento, CA 95817 USA.; Henderson, PT (reprint author), Univ Calif Davis, Ctr Comprehens Canc, Sacramento, CA 95817 USA. EM fischer29@llnl.gov; henderson84@gmail.com FU Lawrence Livermore National Laboratory [15-LW-023]; NIGMS [GM105404]; DOE BER IDAT; Lawrence Livermore National Laboratory; UC Davis Comprehensive Cancer Center; [NCI R01CA155642] FX This work was supported through Lawrence Livermore National Laboratory Research Award 15-LW-023. G.L.H. was supported by the NIGMS RO1MINOS (Grant GM105404) and DOE BER IDAT. S.F.G. was supported by a postdoctoral fellowship from the Lawrence Livermore National Laboratory and UC Davis Comprehensive Cancer Center Fitzpatrick Fund. P.T.H. and T.M.S. were supported by Grant NCI R01CA155642. We are grateful to Matthew Coleman of the Lawrence Livermore National Laboratory for advice on UV irradiation of NLPs. NR 50 TC 0 Z9 0 U1 10 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD AUG 17 PY 2016 VL 8 IS 32 BP 20549 EP 20557 DI 10.1021/acsami.6b04609 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DT8CF UT WOS:000381715900007 PM 27411034 ER PT J AU Levine, DJ Runcevski, T Kapelewski, MT Keitz, BK Oktawiec, J Reed, DA Mason, JA Jiang, HZH Colwell, KA Legendre, CM FitzGerald, SA Long, JR AF Levine, Dana J. Runcevski, Tomce Kapelewski, Matthew T. Keitz, Benjamin K. Oktawiec, Julia Reed, Douglas A. Mason, Jarad A. Jiang, Henry Z. H. Colwell, Kristen A. Legendre, Christina M. FitzGerald, Stephen A. Long, Jeffrey R. TI Olsalaiine-Based Metal-Organic Frameworks as Biocompatible Platforms for H2 Adsorption and Drug Delivery SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBON-DIOXIDE; HYDROGEN ADSORPTION; ULCERATIVE-COLITIS; COLORECTAL-CANCER; COORDINATION POLYMER; ANTICANCER DRUG; OLSALAZINE; SITES; ENCAPSULATION; RELEASE AB The drug olsalazine (H(4)olz) was employed as a ligand to synthesize a new series of mesoporous metal-organic frameworks that are expanded analogues of the well-known M-2(dobdc) materials (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate; M-MOF-74). The M-2(olz) frameworks (M = Mg, Fe, Co, Ni, and Zn) exhibit high surface areas with large hexagonal pore apertures that are approximately 27 angstrom in diameter. Variable temperature H-2 adsorption isotherms revealed strong adsorption at the open metal sites, and in situ infrared spectroscopy experiments on Mg-2(olz) and Ni-2(olz) were used to determine site-specific H-2 binding enthalpies. In addition to its capabilities for gas sorption, the highly biocompatible Mg-2(olz) framework was also evaluated as a platform for the delivery of olsalazine and Other encapsulated therapeutics. The Mg-2(olz) material (86 wt % olsalazine) was shown to release the therapeutic linker through dissolution of the framework under simulated physiological conditions. Furthermore, Mg-2(olz) was used to encapsulate phenethylamine (PEA), a model drug for a broad class of bioactive compounds. Under simulated physiological conditions, Mg-2(olz)(PEA)(2) disassembled to release PEA from the pores and olsalazine from the framework itself; demonstrating that multiple therapeutic components can be delivered together at different rates. The low toxicity, high surface areas, and coordinatively unsaturated metal sites make these M-2(olz) materials promising for a range of potential applications, including drug delivery in the treatment of gastrointestinal diseases. C1 [Levine, Dana J.; Runcevski, Tomce; Kapelewski, Matthew T.; Keitz, Benjamin K.; Oktawiec, Julia; Reed, Douglas A.; Mason, Jarad A.; Jiang, Henry Z. H.; Legendre, Christina M.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Colwell, Kristen A.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Runcevski, Tomce; Kapelewski, Matthew T.; Mason, Jarad A.; Jiang, Henry Z. H.; Long, Jeffrey R.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [FitzGerald, Stephen A.] Oberlin Coll, Dept Phys & Astron, Oberlin, OH 44074 USA. [Levine, Dana J.] CALTECH, Dept Chem Engn, Pasadena, CA 91125 USA. [Keitz, Benjamin K.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Mason, Jarad A.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Legendre, Christina M.] Univ Paris 06, Dept Chim, Ecole Normale Super Paris, F-75005 Paris, France. [Legendre, Christina M.] Univ Paris 06, Dept Chim, F-75005 Paris, France. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Long, JR (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu NR 77 TC 8 Z9 8 U1 98 U2 143 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 17 PY 2016 VL 138 IS 32 BP 10143 EP 10150 DI 10.1021/jacs.6b03523 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DT8CD UT WOS:000381715700020 PM 27486905 ER PT J AU Jiang, JC Furukawa, H Zhang, YB Yaghi, OM AF Jiang, Juncong Furukawa, Hiroyasu Zhang, Yue-Biao Yaghi, Omar M. TI High Methane Storage Working Capacity in Metal-Organic Frameworks with Acrylate Links SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NATURAL-GAS STORAGE; ADSORPTION; TOPOLOGY; POROSITY; ROUTE; SITES; CH4; CO2 AB High methane storage capacity in porous materials is important for the design and manufacture of vehicles powered by natural gas. Here, we report the synthesis, crystal structures and methane adsorption properties of five new zinc metal organic frameworks(MOFs), MOF-905, MOF-905-Me-2, MOF-905-Naph, MOF-905-NO2, and MOF905. All these MOFs consist of the Zn4O(-CO2)(6) secondary building units (SBUs) and benzene-1,3,5-tri-beta-acrylate, BTAC. The permanent porosity of all five materials was confirmed, and their methane adsorption measured up to 80 bar to reveal that MOF-905 is among the best performing methane storage materials with a volumetric working capacity (deorption at 5 bar) of 203 cm(3) cm(-3) at 80 bar and 298 K, a value rivaling that of H.KUST-1 (200 cm(3) cm(-3)), the benchmark compound for methane storage in MOFs. This study expands the scope of MOF materials with ultrahigh working capacity to include linkers having the common acrylate connectivity. C1 [Jiang, Juncong; Furukawa, Hiroyasu; Zhang, Yue-Biao; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Mat Sci Div,Kavli Energy NanoSciences Inst Berkel, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Mat Sci Div,Kavli Energy NanoSciences Inst Berkel, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. EM yaghi@berkeley.edu RI ZHANG, Yue-Biao/E-7870-2011; OI ZHANG, Yue-Biao/0000-0002-8270-1067; Yaghi, Omar/0000-0002-5611-3325 NR 41 TC 12 Z9 12 U1 58 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD AUG 17 PY 2016 VL 138 IS 32 BP 10244 EP 10251 DI 10.1021/jacs.6b05261 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DT8CD UT WOS:000381715700033 PM 27442620 ER PT J AU Pershoguba, SS Nakosai, S Balatsky, AV AF Pershoguba, Sergey S. Nakosai, Sho Balatsky, Alexander V. TI Skyrmion-induced bound states in a superconductor SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC SKYRMIONS; IMPURITY; LATTICE AB We consider a superconductor proximity coupled to a two-dimensional ferromagnetic film with a skyrmion texture. Using the T-matrix calculations and numerical modeling we calculate the spin-polarized local density of states in the superconductor in the vicinity of the skyrmion. We predict the skyrmion bound states that are induced in the superconductor, similar to the well-known Yu-Shiba-Rusinov states. The bound-state wave functions have spatial power-law decay. It is suggested that superconductivity could facilitate an effective long-range interaction between skyrmions when bound-state wave functions overlap. C1 [Pershoguba, Sergey S.; Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Pershoguba, Sergey S.; Nakosai, Sho; Balatsky, Alexander V.] KTH Royal Inst Technol, Ctr Quantum Mat, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Pershoguba, Sergey S.; Nakosai, Sho; Balatsky, Alexander V.] Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Nakosai, Sho] RIKEN, Condensed Matter Theory Lab, Wako, Saitama 3510198, Japan. RP Pershoguba, SS (reprint author), Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA.; Pershoguba, SS (reprint author), KTH Royal Inst Technol, Ctr Quantum Mat, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Pershoguba, SS (reprint author), Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. OI Pershoguba, Sergey/0000-0001-5003-3415 FU US DOE BES [E304]; [15H06858] FX We thank R. Wiesendanger, S. Fujimoto, J. Wiebe, J. Zang, A. Saxena, H. Hurst, Y. Tserkovnyak, S. Lin, and L. Bulaevskii for valuable discussions and comments. This work was supported by US DOE BES E304 (S.S.P. and A.V.B.) and by a Grant-in-Aid for Research Activity Start-up (No. 15H06858) (S.N.). NR 38 TC 1 Z9 1 U1 4 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 17 PY 2016 VL 94 IS 6 AR 064513 DI 10.1103/PhysRevB.94.064513 PG 8 WC Physics, Condensed Matter SC Physics GA DT4VW UT WOS:000381480300003 ER PT J AU Costantini, JM Lelong, G Guillaumet, M Weber, WJ Takaki, S Yasuda, K AF Costantini, Jean-Marc Lelong, Gerald Guillaumet, Maxime Weber, William J. Takaki, Seiya Yasuda, Kazuhiro TI Color-center production and recovery in electron-irradiated magnesium aluminate spinel and ceria SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE color centers; electron irradiation effects; optical absorption spectroscopy; spinel; ceria ID YTTRIA-STABILIZED ZIRCONIA; RADIATION-DAMAGE; DISLOCATION LOOPS; DEFECT CLUSTERS; MGAL2O4 SPINELS; POINT-DEFECTS; ION; CERAMICS; CEO2; SIMULATION AB Single crystals of magnesium aluminate spinel (MgAl2O4) with (1 0 0) or (1 1 0) orientations and cerium dioxide or ceria (CeO2) were irradiated by 1.0 MeV and 2.5 MeV electrons in a high-fluence range. Point-defect production was studied by off-line UV-visible optical spectroscopy after irradiation. For spinel, regardless of both crystal orientation and electron energy, two characteristic broad bands centered at photon energies of 5.4 eV and 4.9 eV were assigned to F and F+ centers (neutral and singly ionized oxygen vacancies), respectively, on the basis of available literature data. No clear differences in color-center formation were observed for the two crystal orientations. Using calculations from displacement cross sections by elastic collisions, these results are consistent with a very large threshold displacement energy (200 eV) for oxygen atoms at room temperature. A third very broad band centered at 3.7 eV might be attributed either to an oxygen hole center (V-type center) or an F-2 dimer center (oxygen di-vacancy). The onset of recovery of these color centers took place at 200 degrees C with almost full bleaching at 600 degrees C. Activation energies (similar to 0.3-0.4 eV) for defect recovery were deduced from the isochronal annealing data by using a first-order kinetics analysis. For ceria, a sub-band-gap absorption feature, which peaked at similar to 3.1 eV, was recorded for 2.5 MeV electron irradiation only. Assuming a ballistic process, we suggest that the latter defect might result from cerium atom displacement on the basis of computed cross sections. C1 [Costantini, Jean-Marc] CEA, DEN, SRMA, F-91191 Gif Sur Yvette, France. [Lelong, Gerald; Guillaumet, Maxime] Univ Paris 06, Sorbonne Univ, IMPMC, CNRS,Museum Natl Hist Nat,UMR 7590,IRD,UMR 206, 4 Pl Jussieu, F-75005 Paris, France. [Weber, William J.] Univ Tennessee Mat Sci & Engn, Knoxville, TN 37996 USA. [Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Takaki, Seiya; Yasuda, Kazuhiro] Kyushu Univ, Dept Appl Quantum Phys & Nucl Engn, Fukuoka, Japan. RP Costantini, JM (reprint author), CEA, DEN, SRMA, F-91191 Gif Sur Yvette, France. EM jean-marc.costantini@cea.fr RI Weber, William/A-4177-2008; OI Weber, William/0000-0002-9017-7365; Lelong, Gerald/0000-0002-3561-8228 FU French EMIR network; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division FX We thank the French EMIR network for supporting this research program. One of the authors (W J Weber) was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The authors are indebted to Lynn Boatner (Oak Ridge National Laboratory, USA) for providing the ceria single crystals, and to Bruno Boizot and Vincent Metayer (Ecole Polytechnique, Palaiseau, France) for their help during the irradiations. NR 42 TC 0 Z9 0 U1 6 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 17 PY 2016 VL 28 IS 32 AR 325901 DI 10.1088/0953-8984/28/32/325901 PG 9 WC Physics, Condensed Matter SC Physics GA DP9VO UT WOS:000378845900012 PM 27319289 ER PT J AU Krupin, O Dakovski, GL Kim, BJ Kim, JW Kim, J Mishra, S Chuang, YD Serrao, CR Lee, WS Schlotter, WF Minitti, MP Zhu, D Fritz, D Chollet, M Ramesh, R Molodtsov, SL Turner, JJ AF Krupin, O. Dakovski, G. L. Kim, B. J. Kim, J. W. Kim, Jungho Mishra, S. Chuang, Yi-De Serrao, C. R. Lee, W-S Schlotter, W. F. Minitti, M. P. Zhu, D. Fritz, D. Chollet, M. Ramesh, R. Molodtsov, S. L. Turner, J. J. TI Ultrafast dynamics of localized magnetic moments in the unconventional Mott insulator Sr2IrO4 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE iridates; spin-orbit coupling materials; free-electron laser science; resonant diffraction; ultra-fast x-ray studies; magnetism ID TRANSITION; STATE AB We report a time-resolved study of the ultrafast dynamics of the magnetic moments formed by the J(eff) = 1/2 states in Sr2IrO4 by directly probing the localized iridium 5d magnetic state through resonant x-ray diffraction. Using optical pump-hard x-ray probe measurements, two relaxation time scales were determined: a fast fluence-independent relaxation is found to take place on a time scale of 1.5 ps, followed by a slower relaxation on a time scale of 500 ps-1.5 ns. C1 [Krupin, O.; Dakovski, G. L.; Schlotter, W. F.; Minitti, M. P.; Zhu, D.; Fritz, D.; Chollet, M.; Turner, J. J.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94720 USA. [Krupin, O.; Molodtsov, S. L.] European XFEL, D-22761 Hamburg, Germany. [Kim, B. J.; Kim, J. W.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kim, Jungho] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Mishra, S.; Chuang, Yi-De] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Serrao, C. R.; Ramesh, R.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Lee, W-S] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Lee, W-S] Stanford Univ, Menlo Pk, CA 94025 USA. [Molodtsov, S. L.] TU Bergakad Freiberg, Inst Expt Phys, Leipziger Str 23, D-09599 Freiberg, Germany. [Molodtsov, S. L.] ITMO Univ, Kronoverskiy Pr 49, St Petersburg 197101, Russia. RP Dakovski, GL (reprint author), SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94720 USA. EM dakovski@slac.stanford.edu; joshuat@slac.stanford.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Science [DE-AC02-06CH11357] FX Use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. We also would like to acknowledge the LCLS 'In-House' program for the chance to access the X-ray Free Electon Laser for the 24 h of x-ray beamtime for this project. This research also used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 32 TC 0 Z9 0 U1 9 U2 40 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD AUG 17 PY 2016 VL 28 IS 32 AR 32LT01 DI 10.1088/0953-8984/28/32/32LT01 PG 4 WC Physics, Condensed Matter SC Physics GA DP9VO UT WOS:000378845900001 PM 27310659 ER PT J AU Khachatryan, V Sirunyan, A Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, V Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Suarez Gonzalez, J Alderweireldt, S Cornelis, T Wolf, E Janssen, X Knutsson, A Lauwers, J Luyckx, S Klundert, M Haevermaet, H Mechelen, P Remortel, N Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Doninck, W Mulders, P Onsem, G Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T L,onard, A Maerschalk, T Marinov, A PerniS, L Randle-conde, A Seva, T Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Ocampo Rios, A Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, G Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Vidal Marono, M Beliy, N Hammad, G Alda, WL Alves, F Alves, G Brito, L Correa Martins Junior, M Hamer, M Hensel, C Mora Herrera, C Moraes, A Pol, M Rebello Teles, P Belchior Batista Das Chagas, E Carvalho, W Chinellato, J Custdio, A Costa, E Jesus Damiao, D Oliveira Martins, C Fonseca De Souza, S Huertas Guativa, L Malbouisson, H Matos Figueiredo, D Mundim, L Nogima, H Prado Da Silva, W Santoro, A Sznajder, A Tonelli Manganote, E Vilela Pereira, A Ahuja, S Bernardes, C De Souza Santos, A Dogra, S Fernandez Perez Tomei, T Gregores, E Mercadante, P Moon, C Novaes, S Padula, S Romero Abad, D Ruiz Vargas, J Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, J Chen, G Chen, H Chen, M Cheng, T Du, R Jiang, C Plestina, R Romeo, F Shaheen, S Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, S Wang, D Xu, Z Avila, C Cabrera, A Chaparro Sierra, L Florez, C Gomez, J Gomez Moreno, B Sanabria, J Godinovic, N Lelas, D Puljak, I Ribeiro Cipriano, P Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, P Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y El Sawy, M Elgammal, S Ellithi Kamel, A Mahmoud, M Mahrous, A Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, J Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P Hamel de Monchenault, G Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Granier de Cassagnac, R Jo, M Lisniak, S Mastrolorenzo, L Mine, P Naranjo, I Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, J Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, J-L Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, E Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, J Skovpen, K Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Carrillo Montoya, C Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, I Lethuillier, M Mirabito, L Pequegnot, A Perries, S Ruiz Alvarez, J Sabes, D Sgandurra, L Sordini, V Donckt, M Verdier, P Viret, S Toriashvili, T Tsamalaidze, Z Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, M Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, J Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, 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Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Castaneda Hernandez, A. Celik, A. Dalchenko, M. Mattia, M. De Delgado, A. Dildick, S. Eusebi, R. Gilmore, J. Huang, T. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sinthuprasith, T. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Kottachchi Kankanamge Don, C. Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for direct pair production of supersymmetric top quarks decaying to all-hadronic final states in pp collisions at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SUPERSYMMETRIC THEORIES; PARTICLE PHYSICS; NATURALNESS; BREAKING; MODELS AB Results are reported from a search for the pair production of top squarks, the supersymmetric partners of top quarks, in final states with jets and missing transverse momentum. The data sample used in this search was collected by the CMS detector and corresponds to an integrated luminosity of 18.9 of proton-proton collisions at a centre-of-mass energy of 8 produced by the LHC. The search features novel background suppression and prediction methods, including a dedicated top quark pair reconstruction algorithm. The data are found to be in agreement with the predicted backgrounds. Exclusion limits are set in simplified supersymmetry models with the top squark decaying to jets and an undetected neutralino, either through a top quark or through a bottom quark and chargino. Models with the top squark decaying via a top quark are excluded for top squark masses up to 755 in the case of neutralino masses below 200. For decays via a chargino, top squark masses up to 620 are excluded, depending on the masses of the chargino and neutralino. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Ero, J.; Flechl, M.; Friedl, M.; Fruhwirth, R.; Ghete, V. 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M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Mattia, A. Di; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, INFN Sez Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Univ Firenze, INFN Sez Firenze, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] INFN Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Tabarelli de Fatis, T.] Univ Milano Bicocca, INFN Sez Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.; Pegoraro, M.] Univ Napoli Federico II, INFN Sez Napoli, Naples, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, INFN Sez Padova, Padua, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Univ Pavia, INFN Sez Pavia, Pavia, Italy. [Alunni Solestizi, L.; Bilei, G. M.; Ciangottini, D.; Fan, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Univ Perugia, INFN Sez Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Fo, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Univ Pisa, INFN Sez Pisa, Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Re, D. Del; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Univ Roma, INFN Sez Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Kiani, B.; Dellacasa, G.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Pinna Angioni, G. L.; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Univ Torino, INFN Sez Torino, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Licata, C. La; Marone, M.; Schizzi, A.; Zanetti, A.] Univ Trieste, INFN Sez Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Brochero Cifuentes, J. A.; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Md Ali, M. A. B.; Mohamad Idris, F.; Wan Abdullah, W. A. T.; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; Cruz-Burelo, E. De La; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autnoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Qazi, S.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Grski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Cruz E Silva, C. Beiro Da; Di Francesco, A.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, l.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys & Vinca, Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; Cruz, B. De La; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Ramos, J. P. Fernandez; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Yzquierdo, A. Prez-Calero; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; Trocniz, J. F. de; Missiroli, M.; Moran, D.] Univ Autnoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castieiras De Saa, J. R.; Castro Manzano, P. De; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; Gruttola, M. De; Guio, F. De; Roeck, A. De; Visscher, S. De; Marco, E. Di; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Doneg, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; Martinez Ruiz del Arbol, P.; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; Cosa, A. De; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.; Cardaci, M.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Miano Moya, M.; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Gecit, H.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Kayis Topaksu, A.; Onengut, G.; Ozcan, M.; Ozdemir, K.; Ozturk, S.; Sunar Cerci, D.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarlan, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; Seif El Nasr-storey, S.; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; Wit, A. De; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Vazquez Acosta, M.; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Barca Sanchez, M. Calderon De La; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Bravo, C.; Cousins, R.; Everaerts, P.; Farrell, C.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Schnaible, C.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Ivova Paneva, M.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Zevi Della Porta, G.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Franco Sevilla, M.; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Nicolas Kaufman, G.; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lopes De Sa, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Martinez Outschoorn, V. I.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.] Univ Florida, Gainesville, FL USA. [Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. 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RI Tuominen, Eija/A-5288-2017; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Lokhtin, Igor/D-7004-2012; Azarkin, Maxim/N-2578-2015; Konecki, Marcin/G-4164-2015; Kirakosyan, Martin/N-2701-2015; Dremin, Igor/K-8053-2015; Moraes, Arthur/F-6478-2010; Della Ricca, Giuseppe/B-6826-2013; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Goh, Junghwan/Q-3720-2016 OI Tuominen, Eija/0000-0002-7073-7767; Paulini, Manfred/0000-0002-6714-5787; Konecki, Marcin/0000-0001-9482-4841; Moraes, Arthur/0000-0002-5157-5686; Della Ricca, Giuseppe/0000-0003-2831-6982; TUVE', Cristina/0000-0003-0739-3153; Goh, Junghwan/0000-0002-1129-2083 NR 107 TC 1 Z9 1 U1 11 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD AUG 16 PY 2016 VL 76 IS 8 AR 460 DI 10.1140/epjc/s10052-016-4292-5 PG 46 WC Physics, Particles & Fields SC Physics GA DU1UX UT WOS:000381996600001 ER PT J AU Hirano, A Shi, G Jones, CR Lipzen, A Pennacchio, LA Xu, Y Hallows, WC McMahon, T Yamazaki, M PtAiAek, LJ Fu, YH AF Hirano, Arisa Shi, Guangsen Jones, Christopher R. Lipzen, Anna Pennacchio, Len A. Xu, Ying Hallows, William C. McMahon, Thomas Yamazaki, Maya PtAiAek, Louis J. Fu, Ying-Hui TI A Cryptochrome 2 mutation yields advanced sleep phase in humans SO ELIFE LA English DT Article ID MAMMALIAN CIRCADIAN CLOCK; CRYSTAL-STRUCTURE; UBIQUITIN LIGASE; PHOSPHORYLATION; PERIOD; REVEALS; RHYTHMS; FBXL3; CRY2; CONSEQUENCES AB Familial Advanced Sleep Phase (FASP) is a heritable human sleep phenotype characterized by very early sleep and wake times. We identified a missense mutation in the human Cryptochrome 2 (CRY2) gene that co-segregates with FASP in one family. The mutation leads to replacement of an alanine residue at position 260 with a threonine (A260T). In mice, the CRY2 mutation causes a shortened circadian period and reduced phase-shift to early-night light pulse associated with phase-advanced behavioral rhythms in the light-dark cycle. The A260T mutation is located in the phosphate loop of the flavin adenine dinucleotide (FAD) binding domain of CRY2. The mutation alters the conformation of CRY2, increasing its accessibility and affinity for FBXL3 (an E3 ubiquitin ligase), thus promoting its degradation. These results demonstrate that CRY2 stability controlled by FBXL3 plays a key role in the regulation of human sleep wake behavior. C1 [Hirano, Arisa; Shi, Guangsen; Hallows, William C.; McMahon, Thomas; Yamazaki, Maya; PtAiAek, Louis J.; Fu, Ying-Hui] Univ Calif San Francisco, Dept Neurol, San Francisco, CA 94143 USA. [Jones, Christopher R.] Univ Utah, Dept Neurol, Salt Lake City, UT USA. [Lipzen, Anna; Pennacchio, Len A.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Lipzen, Anna; Pennacchio, Len A.] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [Xu, Ying] Soochow Univ, Ctr Syst Biol, Suzhou, Peoples R China. [PtAiAek, Louis J.] Univ Calif San Francisco, Howard Hughes Med Inst, San Francisco, CA 94143 USA. RP PtAiAek, LJ; Fu, YH (reprint author), Univ Calif San Francisco, Dept Neurol, San Francisco, CA 94143 USA.; PtAiAek, LJ (reprint author), Univ Calif San Francisco, Howard Hughes Med Inst, San Francisco, CA 94143 USA. EM ljp@ucsf.edu; ying-hui.fu@ucsf.edu OI Xu, Ying/0000-0002-6689-7768 FU Japan Society for the Promotion of Science; Uehara Memorial Foundation; National Heart, Lung, and Blood Institute [HL059596]; William K. Bowes, Jr. Foundation; National Institute of General Medical Sciences [GM079180] FX Japan Society for the Promotion of Science Arisa Hirano; Uehara Memorial Foundation Arisa Hirano; National Heart, Lung, and Blood Institute HL059596 Louis J PtAiAek; William K. Bowes, Jr. Foundation Neurogenetics Fund Ying-Hui Fu; National Institute of General Medical Sciences GM079180 Ying-Hui Fu; The funders had no role in study design, data collection and interpretation, or the decision to submit the work for publication. NR 51 TC 2 Z9 2 U1 7 U2 7 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD AUG 16 PY 2016 VL 5 AR e16695 DI 10.7554/eLife.16695 PG 21 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DX1FZ UT WOS:000384112800001 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Bouchet, J Brandin, AV Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Cervantes, MC Chakaberia, I Chaloupka, P Chang, Z Chattopadhyay, S Chen, JH Chen, HF Cheng, J Cherney, M Christie, W Codrington, MJM Contin, G Crawford, HJ Cui, X Das, S De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD di Ruzza, B Didenko, L Dilks, C Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Eppley, G Esha, R Evdokimov, O Eyser, O Fatemi, R Fazio, S Federic, P Fedorisin, J Feng Filip, P Fisyak, Y Flores, CE Gagliardi, CA Garand, D Geurts, F Gibson, A Girard, M Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Hamad, A Hamed, A Han, LX Haque, R Harris, JW Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, X Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Klein, SR Koetke, DD Kollegger, T Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Li, ZM Li, X Li, W Li, Y Li, X Li, C Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, GL Ma, RM Ma, YG Magdy, N Mahapatra, DP Majka, R Manion, A Margetis, S Markert, C Masui, H Matis, HS McDonald, D Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Okorokov, V Olvitt, DL Page, BS Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Simko, M Skoby, MJ Smirnov, N Smirnov, D Solanki, D Song, L Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stock, R Strikhanov, M Stringfellow, B Sumbera, M Summa, BJ Sun, XM Sun, Z Sun, Y Sun, X Surrow, B Svirida, DN Szelezniak, MA Takahashi, J Tang, Z Tang, AH Tarnowsky, T Tawfik, AN Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Tripathy, SK Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Upsal, I Van Buren, G Van Nieuwenhuizen, G Vandenbroucke, M Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Voloshin, SA Vossen, A Wang, JS Wang, XL Wang, Y Wang, H Wang, F Wang, G Webb, G Webb, JC Wen, L Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, N Xu, Z Xu, H Xu, Y Xu, QH Yan, W Yang, Y Yang, C Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zbroszczyk, H Zha, W Zhang, XP Zhang, ZP Zhang, JB Zhang, JL Zhang, Y Zhang, S Zhao, F Zhao, J Zhong, C Zhu, YH Zhu, X Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Bouchet, J. Brandin, A. V. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Campbell, J. M. Cebra, D. Cervantes, M. C. Chakaberia, I. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, J. H. Chen, H. F. Cheng, J. Cherney, M. Christie, W. Codrington, M. J. M. Contin, G. Crawford, H. J. Cui, X. Das, S. De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Derradi de Souza, R. di Ruzza, B. Didenko, L. Dilks, C. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Eppley, G. Esha, R. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Federic, P. Fedorisin, J. Feng Filip, P. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Garand, D. Geurts, F. Gibson, A. Girard, M. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Hamad, A. Hamed, A. Han, L. -X. Haque, R. Harris, J. W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, X. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Klein, S. R. Koetke, D. D. Kollegger, T. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Li, Z. M. Li, X. Li, W. Li, Y. Li, X. Li, C. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, G. L. Ma, R. M. Ma, Y. G. Magdy, N. Mahapatra, D. P. Majka, R. Manion, A. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Okorokov, V. Olvitt, D. L., Jr. Page, B. S. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Simko, M. Skoby, M. J. Smirnov, N. Smirnov, D. Solanki, D. Song, L. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Summa, B. J. Sun, X. M. Sun, Z. Sun, Y. Sun, X. Surrow, B. Svirida, D. N. Szelezniak, M. A. Takahashi, J. Tang, Z. Tang, A. H. Tarnowsky, T. Tawfik, A. N. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Tripathy, S. K. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Upsal, I. Van Buren, G. Van Nieuwenhuizen, G. Vandenbroucke, M. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Voloshin, S. A. Vossen, A. Wang, J. S. Wang, X. L. Wang, Y. Wang, H. Wang, F. Wang, G. Webb, G. Webb, J. C. Wen, L. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, N. Xu, Z. Xu, H. Xu, Y. Xu, Q. H. Yan, W. Yang, Y. Yang, C. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I. -K. Yu, N. Zbroszczyk, H. Zha, W. Zhang, X. P. Zhang, Z. P. Zhang, J. B. Zhang, J. L. Zhang, Y. Zhang, S. Zhao, F. Zhao, J. Zhong, C. Zhu, Y. H. Zhu, X. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Beam-energy dependence of charge balance functions from Au plus Au collisions at energies available at the BNL Relativistic Heavy Ion Collider SO PHYSICAL REVIEW C LA English DT Article ID QUARK-GLUON PLASMA; BY-EVENT FLUCTUATIONS; TRANSVERSE-MOMENTUM; MEAN-P(T) FLUCTUATIONS; ROOT-S(NN)=200 GEV; PB COLLISIONS; HADRONIZATION; SIGNATURES; PHI; ETA AB Balance functions have been measured in terms of relative pseudorapidity (Delta(eta)) for charged particle pairs at the BNL Relativistic Heavy Ion Collider from Au + Au collisions at root s(NN) = 7.7 GeV to 200 GeV using the STAR detector. These results are compared with balance functions measured at the CERN Large Hadron Collider from Pb + Pb collisions at root s(NN) = 2.76 TeV by the ALICE Collaboration. The width of the balance function decreases as the collisions become more central and as the beam energy is increased. In contrast, the widths of the balance functions calculated using shuffled events show little dependence on centrality or beam energy and are larger than the observed widths. Balance function widths calculated using events generated by UrQMD are wider than the measured widths in central collisions and show little centrality dependence. The measured widths of the balance functions in central collisions are consistent with the delayed hadronization of a deconfined quark gluon plasma (QGP). The narrowing of the balance function in central collisions at root s(NN) = 7.7 GeV implies that a QGP is still being created at this relatively low energy. C1 [Adamczyk, L.; Przybycien, M.] AGH Univ Sci & Technol, PL-30059 Krakow, Poland. [Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Arkhipkin, D.; Aschenauer, E. C.; Bland, L. C.; Burton, T. P.; Chakaberia, I.; Christie, W.; Debbe, R. R.; di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; Li, X.; Ljubicic, T.; Longacre, R. S.; Ma, R. M.; Ogawa, A.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Ullrich, T.; Van Buren, G.; Videbaek, F.; Wang, H.; Webb, G.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Sanchez, M. Calderon de la Barca; Cebra, D.; Draper, J. E.; Flores, C. E.; Romero, J. L.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Esha, R.; Huang, H. Z.; Igo, G.; Landry, K. D.; Nasim, Md.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Wen, L.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, BR-13131 Sao Paulo, Brazil. [Feng; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Sun, X. M.; Wu, Y. F.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Huang, B.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Cherney, M.; De Silva, L. C.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Rusnakova, O.; Trzeciak, B. A.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Bielcikova, J.; Federic, P.; Rusnak, J.; Simko, M.; Sumbera, M.; Tlusty, D.; Vertesi, R.] Nucl Phys Inst AS CR, Rez 25068, Czech Republic. [Kisel, I.; Kollegger, T.; Kulakov, I.; Stock, R.; Zyzak, M.] FIAS, D-60438 Frankfurt, Germany. [Das, S.; Mahapatra, D. P.; Sahu, P. K.; Tripathy, S. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Sarkar, A.; Varma, R.] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Jacobs, W. W.; Page, B. S.; Skoby, M. J.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Kalinkin, D.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bhasin, A.; Gupta, A.; Gupta, S.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Alford, J.; Bouchet, J.; Hamad, A.; Kabana, S.; Keane, D.; Lomnitz, M.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Ramachandran, S.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Daejeon 305701, South Korea. [Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.] Inst Modern Phys, Lanzhou 730000, Peoples R China. [Contin, G.; Dong, X.; Greiner, L.; Klein, S. R.; Manion, A.; Masui, H.; Matis, H. S.; Mustafa, M. K.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, S. S.; Sichtermann, E. P.; Sun, X.; Szelezniak, M. A.; Thomas, J. H.; Wieman, H.; Xu, N.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Van Nieuwenhuizen, G.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kotchenda, L.; Kravtsov, P.; Nigmatkulov, G.; Okorokov, V.; Strikhanov, M.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Haque, R.; Mohanty, B.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Campbell, J. M.; Humanic, T. J.; Lisa, M. A.; Upsal, I.] Ohio State Univ, Columbus, OH 43210 USA. [Kycia, R. A.; Pawlik, B.; Turnau, J.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Pruthi, N. K.; Sharma, B.] Panjab Univ, Chandigarh 160014, India. [Dilks, C.; Heppelmann, S.; Summa, B. J.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Garand, D.; Hirsch, A.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zha, W.; Zhang, Z. P.; Zhang, Y.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Deng, J.; Xu, Q. H.; Zhang, J. L.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L. -X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D. L., Jr.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Hoffmann, G. W.; Markert, C.; Ray, R. L.; Schambach, J.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Song, L.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Roy, A.; Tribedy, P.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pawlak, T.; Pluta, J.; Poniatowska, K.; Sandacz, A.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Llope, W. J.; Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Magdy, N.; Tawfik, A. N.] World Lab Cosmol & Particle Phys WLCAPP, Cairo 11571, Egypt. [Caines, H.; Harris, J. W.; Horvat, S.; Majka, R.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Kycia, Radoslaw/J-4397-2015; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; Takahashi, Jun/B-2946-2012; Derradi de Souza, Rafael/M-4791-2013 OI Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Kycia, Radoslaw/0000-0002-6390-4627; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Takahashi, Jun/0000-0002-4091-1779; Derradi de Souza, Rafael/0000-0002-2084-7001 FU Office of NP within the U.S. DOE Office of Science; Office of HEP within the U.S. DOE Office of Science; U.S. NSF [CNRS/IN2P3]; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; MSMT of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3, FAPESP CNPq of Brazil, the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST and MoE of China, the Korean Research Foundation, GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and CSIR of India, the National Science Centre of Poland, National Research Foundation (NRF-2012004024), the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 46 TC 0 Z9 0 U1 13 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD AUG 16 PY 2016 VL 94 IS 2 AR 024909 DI 10.1103/PhysRevC.94.024909 PG 7 WC Physics, Nuclear SC Physics GA DT4ZD UT WOS:000381489300001 ER PT J AU Turner, DL Fennell, JF Blake, JB Clemmons, JH Mauk, BH Cohen, IJ Jaynes, AN Craft, JV Wilder, FD Baker, DN Reeves, GD Gershman, DJ Avanov, LA Dorelli, JC Giles, BL Pollock, CJ Schmid, D Nakamura, R Strangeway, RJ Russell, CT Artemyev, AV Runov, A Angelopoulos, V Spence, HE Torbert, RB Burch, JL AF Turner, D. L. Fennell, J. F. Blake, J. B. Clemmons, J. H. Mauk, B. H. Cohen, I. J. Jaynes, A. N. Craft, J. V. Wilder, F. D. Baker, D. N. Reeves, G. D. Gershman, D. J. Avanov, L. A. Dorelli, J. C. Giles, B. L. Pollock, C. J. Schmid, D. Nakamura, R. Strangeway, R. J. Russell, C. T. Artemyev, A. V. Runov, A. Angelopoulos, V. Spence, H. E. Torbert, R. B. Burch, J. L. TI Energy limits of electron acceleration in the plasma sheet during substorms: A case study with the Magnetospheric Multiscale (MMS) mission SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE energetic particle injections; particle acceleration; magnetotail; plasma sheet; reconnection; substorm ID BURSTY BULK FLOWS; DIPOLARIZATION EVENTS; PARTICLE INJECTIONS; RECONNECTION; SIMULATION; FIELD AB We present multipoint observations of earthward moving dipolarization fronts and energetic particle injections from NASA's Magnetospheric Multiscale mission with a focus on electron acceleration. From a case study during a substorm on 02 August 2015, we find that electrons are only accelerated over a finite energy range, from a lower energy threshold at similar to 7-9keV up to an upper energy cutoff in the hundreds of keV range. At energies lower than the threshold energy, electron fluxes decrease, potentially due to precipitation by strong parallel electrostatic wavefields or initial sources in the lobes. Electrons at energies higher than the threshold are accelerated cumulatively by a series of impulsive magnetic dipolarization events. This case demonstrates how the upper energy cutoff increases, in this case from similar to 130keV to >500keV, with each dipolarization/injection during sustained activity. We also present a simple model accounting for these energy limits that reveals that electron energization is dominated by betatron acceleration. C1 [Turner, D. L.; Fennell, J. F.; Blake, J. B.; Clemmons, J. H.] Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. [Mauk, B. H.; Cohen, I. J.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. [Jaynes, A. N.; Craft, J. V.; Wilder, F. D.; Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Gershman, D. J.; Avanov, L. A.; Dorelli, J. C.; Giles, B. L.; Pollock, C. J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Pollock, C. J.] Denali Sci, Healy, AK USA. [Schmid, D.; Nakamura, R.] Austrian Acad Sci, Space Res Inst, Graz, Austria. [Strangeway, R. J.; Russell, C. T.; Artemyev, A. V.; Runov, A.; Angelopoulos, V.] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA USA. [Spence, H. E.; Torbert, R. B.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Burch, J. L.] Southwest Res Inst, San Antonio, TX USA. RP Turner, DL (reprint author), Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. EM drew.lawson.turner@gmail.com RI NASA MMS, Science Team/J-5393-2013; Cohen, Ian/K-3038-2015; Mauk, Barry/E-8420-2017; OI NASA MMS, Science Team/0000-0002-9504-5214; Cohen, Ian/0000-0002-9163-6009; Mauk, Barry/0000-0001-9789-3797; Clemmons, James/0000-0002-5298-5222 FU NASA (MMS) [NNG04EB99C]; International Space Science Institute's International Teams program FX The authors are thankful to all of the MMS, THEMIS, Van Allen Probes, ACE, Wind, and OMNI teams for making their data available to the public. In addition to coauthors' contributions, we thank from THEMIS, K.H. Glassmeier, U. Auster, and W. Baumjohann (under contract 50 OC 0302); D. Larson and R. P. Lin; and C. W. Carlson and J. P. McFadden for FGM, SST, and ESA data, respectively; from Van Allen Probes, C. Kletzing and team for EMFISIS data; from ACE, Wind, and OMNI, J. H. King, N. Papatashvilli, and team for OMNI solar wind data; the SPEDAS team and contributors for their open source library of data analysis tools; and NASA CDAWeb and mission specific online databases. MMS data are available at < https://lasp.colorado.edu/mms/sdc >; data from this particular event, which occurred during commissioning, may be requested from the authors or from the SDC. THEMIS data and SPEDAS tools are freely available at < http://themis.ssl.berkeley.edu/index.shtml >. Van Allen Probes data are available at < http://rbspgway.jhuapl.edu/data_instrumentationSOC >. This work was primarily supported by funding from NASA (MMS contract NNG04EB99C) and research supported by the International Space Science Institute's International Teams program. NR 40 TC 1 Z9 1 U1 16 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2016 VL 43 IS 15 BP 7785 EP 7794 DI 10.1002/2016GL069691 PG 10 WC Geosciences, Multidisciplinary SC Geology GA DV9VM UT WOS:000383290300001 ER PT J AU Yue, C An, X Bortnik, J Ma, QL Li, W Thorne, RM Reeves, GD Gkioulidou, M Mitchell, DG Kletzing, CA AF Yue, Chao An, Xin Bortnik, Jacob Ma, Qianli Li, Wen Thorne, Richard M. Reeves, Geoffrey D. Gkioulidou, Matina Mitchell, Donald G. Kletzing, Craig A. TI The relationship between the macroscopic state of electrons and the properties of chorus waves observed by the Van Allen Probes SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE electron temperature anisotropy; whistler mode chorus waves; beta parallel; marginally stable state; quasi-parallel waves; oblique waves ID INSTABILITY; PARTICLE; RADIATION AB Plasma kinetic theory predicts that a sufficiently anisotropic electron distribution will excite whistler mode waves, which in turn relax the electron distribution in such a way as to create an upper bound on the relaxed electron anisotropy. Here using whistler mode chorus wave and plasma measurements by Van Allen Probes, we confirm that the electron distributions are well constrained by this instability to a marginally stable state in the whistler mode chorus waves generation region. Lower band chorus waves are organized by the electron (vertical bar e) into two distinct groups: (i) relatively large-amplitude, quasi-parallel waves with vertical bar e0.025 and (ii) relatively small-amplitude, oblique waves with vertical bar e less than or similar to 0.025. The upper band chorus waves also have enhanced amplitudes close to the instability threshold, with large-amplitude waves being quasi-parallel whereas small-amplitude waves being oblique. These results provide important insight for studying the excitation of whistler mode chorus waves. C1 [Yue, Chao; An, Xin; Bortnik, Jacob; Ma, Qianli; Li, Wen; Thorne, Richard M.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. [Yue, Chao] Univ Corp Atmospheric Res, Boulder, CO 80307 USA. [Reeves, Geoffrey D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Reeves, Geoffrey D.] New Mexico Consortium, Div Space Sci, Los Alamos, NM USA. [Gkioulidou, Matina; Mitchell, Donald G.] Johns Hopkins Univ, Appl Phys Lab, Dept Space, Laurel, MD USA. [Kletzing, Craig A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. RP Yue, C; An, X (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA.; Yue, C (reprint author), Univ Corp Atmospheric Res, Boulder, CO 80307 USA. EM yuechao@atmos.ucla.edu; xinan@atmos.ucla.edu RI Yue, Chao/C-2535-2015; OI Yue, Chao/0000-0001-9720-5210; An, Xin/0000-0003-2507-8632; Ma, Qianli/0000-0001-5452-4756; Reeves, Geoffrey/0000-0002-7985-8098 FU NASA Living With a Star Jack Eddy Postdoctoral Fellowship Program; Department of Energy and the National Science Foundation [DE-SC0010578]; NASA [NNX13AI61G, NNX15AF61G, NNX14AI18G, NAS5-01072]; NSF [AGS-1405054] FX This work was supported by the NASA Living With a Star Jack Eddy Postdoctoral Fellowship Program, administered by the UCAR Visiting Scientist Programs. The research was also funded by the Department of Energy and the National Science Foundation by grant DE-SC0010578, which was awarded to UCLA through the NSF/DOE Plasma Partnership program, and NASA grants NNX13AI61G, NNX15AF61G, and NNX14AI18G, and NSF grant AGS-1405054. We acknowledge use of Van Allen Probes data, made publicly available through NASA prime contract NAS5-01072, including the Level 3 HOPE omni-dimensional data obtained from the RBSP-ECT website (www.rbsp-ect.lanl.gov/data_pub/rbspb/hope/level3/PA/); the Level 3 RBSPICE omni-dimensional flux data obtained from the RBSPICE website (http://rbspicea.ftecs.com/Level_3PAP/); the Level 3 magnetic field and wave data obtained from the RBSP EMFISIS website (emfisis.physics.uiowa.edu/Flight/RBSP-B/L3). We thank the Space Physics Data Facility at the NASA Goddard Space Flight Center for providing the OMNI data (ftp://spdf.gsfc.nasa.gov/pub/data/omni/omni_cdaweb/). NR 29 TC 2 Z9 2 U1 3 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2016 VL 43 IS 15 BP 7804 EP 7812 DI 10.1002/2016GL070084 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DV9VM UT WOS:000383290300003 ER PT J AU Ozaki, M Shiokawa, K Miyoshi, Y Kataoka, R Yagitani, S Inoue, T Ebihara, Y Jun, CW Nomura, R Sakaguchi, K Otsuka, Y Shoji, M Schofield, I Connors, M Jordanova, VK AF Ozaki, M. Shiokawa, K. Miyoshi, Y. Kataoka, R. Yagitani, S. Inoue, T. Ebihara, Y. Jun, C. -W Nomura, R. Sakaguchi, K. Otsuka, Y. Shoji, M. Schofield, I. Connors, M. Jordanova, V. K. TI Fast modulations of pulsating proton aurora related to subpacket structures of Pc1 geomagnetic pulsations at subauroral latitudes SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE pulsating proton aurora; Pc1 geomagnetic pulsations; subpacket structure; fast modulation; wave-particle interactions ID ION-CYCLOTRON WAVES; 1-2 MAGNETIC PULSATIONS; DAWN-DUSK ASYMMETRY; MODE CHORUS WAVES; VAN ALLEN PROBES; EQUATORIAL MAGNETOSPHERE; PEARL PULSATIONS; EMIC WAVES; EMISSIONS; PRECIPITATION AB To understand the role of electromagnetic ion cyclotron (EMIC) waves in determining the temporal features of pulsating proton aurora (PPA) via wave-particle interactions at subauroral latitudes, high-time-resolution (1/8s) images of proton-induced N-2(+) emissions were recorded using a new electron multiplying charge-coupled device camera, along with related Pc1 pulsations on the ground. The observed Pc1 pulsations consisted of successive rising-tone elements with a spacing for each element of 100s and subpacket structures, which manifest as amplitude modulations with a period of a few tens of seconds. In accordance with the temporal features of the Pc1 pulsations, the auroral intensity showed a similar repetition period of 100s and an unpredicted fast modulation of a few tens of seconds. These results indicate that PPA is generated by pitch angle scattering, nonlinearly interacting with Pc1/EMIC waves at the magnetic equator. C1 [Ozaki, M.; Yagitani, S.; Inoue, T.] Kanazawa Univ, Grad Sch Nat Sci & Technol, Kanazawa, Ishikawa, Japan. [Shiokawa, K.; Miyoshi, Y.; Jun, C. -W; Otsuka, Y.; Shoji, M.] Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi, Japan. [Kataoka, R.] Natl Inst Polar Res, Tachikawa, Tokyo, Japan. [Kataoka, R.] Grad Univ Adv Studies SOKENDAI, Dept Polar Sci, Tachikawa, Tokyo, Japan. [Ebihara, Y.] Kyoto Univ, Res Inst Sustainable Humanosphere, Uji, Kyoto, Japan. [Nomura, R.] Japan Aerosp Explorat Agcy, Inst Space & Astronaut Sci, Sagamihara, Kanagawa, Japan. [Sakaguchi, K.] Natl Inst Informat & Communicat Technol, Koganei, Tokyo, Japan. [Schofield, I.; Connors, M.] Athabasca Univ, Ctr Sci, Athabasca, AB, Canada. [Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Ozaki, M (reprint author), Kanazawa Univ, Grad Sch Nat Sci & Technol, Kanazawa, Ishikawa, Japan. EM ozaki@is.t.kanazawa-u.ac.jp RI Ebihara, Yusuke/D-1638-2013; Miyoshi, Yoshizumi/B-5834-2015 OI Ebihara, Yusuke/0000-0002-2293-1557; Miyoshi, Yoshizumi/0000-0001-7998-1240 FU Japan Society for the Promotion of Science [25247080, 25302006, 15H05747, 15H05815, 16H06286]; Canada Foundation for Innovation FX This work was supported by Grants-in-Aid for Scientific Research (25247080, 25302006, 15H05747, 15H05815, and 16H06286) from the Japan Society for the Promotion of Science. The observations at the Athabasca University Geospace Observatory were supported by the Canada Foundation for Innovation, and the authors wish to thank Kyle Reiter of Athabasca University Geospace Observatory for his helpful support in the operation of the induction magnetometer and optical observations. The induction magnetometer data at ATH are available at http://stdb2.stelab.nagoya-u.ac.jp/magne/index.html. The all-sky EMCCD data taken with a BG3 glass filter at ATH are available through ISEE, Nagoya University. The all-sky EMCCD data for Hbeta emissions at ATH are obtained from http://autumn.athabascau.ca/magdata/. The AE index was provided by the WDC for Geomagnetism in Kyoto (http://wdc.kugi.kyoto-u.ac.jp/). NR 49 TC 0 Z9 0 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2016 VL 43 IS 15 BP 7859 EP 7866 DI 10.1002/2016GL070008 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DV9VM UT WOS:000383290300009 ER PT J AU Burrows, SM Gobrogge, E Fu, L Link, K Elliott, SM Wang, HF Walker, R AF Burrows, Susannah M. Gobrogge, Eric Fu, Li Link, Katie Elliott, Scott M. Wang, Hongfei Walker, Rob TI OCEANFILMS-2: Representing coadsorption of saccharides in marine films and potential impacts on modeled marine aerosol chemistry SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE sea surface microlayer; marine aerosol; surfactant interactions; sea spray aerosol; organic aerosol; marine biofilms ID SEA SPRAY AEROSOL; ORGANIC-MATTER ENRICHMENT; CENTRAL ARCTIC-OCEAN; AIR-WATER-INTERFACE; SURFACE MICROLAYER; GLOBAL DISTRIBUTION; CHLOROPHYLL-A; ADRIATIC SEA; PARTICLES; FRACTIONATION AB Here we show that the addition of chemical interactions between soluble monosaccharides and an insoluble lipid surfactant monolayer improves agreement of modeled sea spray chemistry with observed marine aerosol chemistry. In particular, the alkane:hydroxyl mass ratio in modeled sea spray organic matter is reduced from a median of 2.73 to a range of 0.41-0.69, reducing the discrepancy with previous Fourier transform infrared spectroscopy (FTIR) observations of clean marine aerosol (ratio: 0.24-0.38). The overall organic fraction of submicron sea spray also increases, allowing organic mass fractions in the range 0.5-0.7 for submicron sea spray particles over highly active phytoplankton blooms. Sum frequency generation experiments support the modeling approach by demonstrating that soluble monosaccharides can strongly adsorb to a lipid monolayer likely via Coulomb interactions under appropriate conditions. These laboratory findings motivate further research to determine the relevance of coadsorption mechanisms for real-world, sea spray aerosol production. C1 [Burrows, Susannah M.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Gobrogge, Eric; Link, Katie; Walker, Rob] Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA. [Fu, Li; Wang, Hongfei] Pacific Northwest Natl Lab, Environm & Mol Sci Lab, Richland, WA USA. [Elliott, Scott M.] Los Alamos Natl Lab, Climate Ocean & Sea Ice Modelling Grp, Los Alamos, NM USA. RP Burrows, SM (reprint author), Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM susannah.burrows@pnnl.gov RI Wang, Hongfei/B-1263-2010; Burrows, Susannah/A-7429-2011 OI Wang, Hongfei/0000-0001-8238-1641; Burrows, Susannah/0000-0002-0745-7252 FU Regional and Global Climate Modeling program of the Office of Biological and Environmental Research in the DOE Office of Science; National Science Foundation [CHE-1026870]; DOE [DE-AC05-76RL01830] FX S.M.B. and S.M.E. were supported by the Regional and Global Climate Modeling program of the Office of Biological and Environmental Research in the DOE Office of Science. R.A.W., E.A.G., and K.A.L. acknowledge support from the National Science Foundation (CHE-1026870). A portion of the research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL), under EMSL User proposal 48281. PNNL is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. All original data underlying analyses in this paper are available from the authors upon request. NR 52 TC 2 Z9 2 U1 13 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD AUG 16 PY 2016 VL 43 IS 15 BP 8306 EP 8313 DI 10.1002/2016GL069070 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DV9VM UT WOS:000383290300060 ER PT J AU Thompson, DR McCubbin, I Gao, BC Green, RO Matthews, AA Mei, F Meyer, KG Platnick, S Schmid, B Tomlinson, J Wilcox, E AF Thompson, David R. McCubbin, Ian Gao, Bo Cai Green, Robert O. Matthews, Alyssa A. Mei, Fan Meyer, Kerry G. Platnick, Steven Schmid, Beat Tomlinson, Jason Wilcox, Eric TI Measuring cloud thermodynamic phase with shortwave infrared imaging spectroscopy SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE imaging spectroscopy; remote sensing; cloud phase; shortwave infrared; AVIRIS-C; Arm Airborne Facility ID RADIATIVE-TRANSFER; OPTICAL-THICKNESS; SPECTROMETER DATA; EFFECTIVE RADIUS; LIQUID WATER; MU-M; ICE; AIRBORNE; RETRIEVAL; WAVELENGTHS AB Shortwave Infrared imaging spectroscopy enables accurate remote mapping of cloud thermodynamic phase at high spatial resolution. We describe a measurement strategy to exploit signatures of liquid and ice absorption in cloud top apparent reflectance spectra from 1.4 to 1.8m. This signal is generally insensitive to confounding factors such as solar angles, view angles, and surface albedo. We first evaluate the approach in simulation and then apply it to airborne data acquired in the Calwater-2/ACAPEX campaign of Winter 2015. Here NASA's Classic Airborne Visible Infrared Imaging Spectrometer (AVIRIS-C) remotely observed diverse cloud formations while the U.S. Department of Energy ARM Aerial Facility G-1 aircraft measured cloud integral and microphysical properties in situ. The coincident measurements demonstrate good separation of the thermodynamic phases for relatively homogeneous clouds. C1 [Thompson, David R.; McCubbin, Ian; Green, Robert O.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91125 USA. [McCubbin, Ian; Wilcox, Eric] Desert Res Inst, Reno, NV USA. [Gao, Bo Cai] Naval Res Lab, Washington, DC 20375 USA. [Matthews, Alyssa A.; Mei, Fan; Schmid, Beat; Tomlinson, Jason] Pacific Northwest Natl Lab, Richland, WA USA. [Meyer, Kerry G.] Univ Space Res Assoc, Goddard Earth Sci Technol & Res, Columbia, MD USA. [Meyer, Kerry G.; Platnick, Steven] NASA Goddard Space Flight Ctr, Greenland, MD USA. RP Thompson, DR (reprint author), CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91125 USA. EM david.r.thompson@jpl.nasa.gov RI Platnick, Steven/J-9982-2014; Meyer, Kerry/E-8095-2016; OI Platnick, Steven/0000-0003-3964-3567; Meyer, Kerry/0000-0001-5361-9200; Thompson, David/0000-0003-1100-7550 FU National Oceanographic and Atmospheric Administration; Department of Energy; Scripps Institute for Oceanography; California Energy Commission FX The data used in this paper are available from http://aviris.jpl.nasa.gov/publications/. The research described in this paper was performed by the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. Copyright 2016 California Institute of Technology. Government sponsorship acknowledged. We appreciate the vital assistance of the DOE Atmospheric Radiation Measurement (ARM) program and the ARM Airborne Facility (AAF) team. We specifically acknowledge the WCM-2000 sensor team including John Hubbe (deployment and calibration). We also acknowledge and thank Jennifer Comstock of PNNL and Chris Roden of SPEC. David Diner and Felix Seidel led the ER-2 observations and coordinated the AAF and the ER-2 flights. We thank the ER-2 aircraft team at the NASA Armstrong Flight Research Laboratory, and the Jet Propulsion Laboratory AVIRIS-C instrument team including Michael Eastwood, Chuck Sarture, Scott Nolte, Mark Helmlinger, Sarah Lundeen, and others. We acknowledge the help and support of NASA Earth Science and the joint Calwater-2/ACAPEX investigation sponsored by the National Oceanographic and Atmospheric Administration, the Department of Energy, Scripps Institute for Oceanography, and the California Energy Commission. NR 47 TC 0 Z9 0 U1 5 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD AUG 16 PY 2016 VL 121 IS 15 BP 9174 EP 9190 DI 10.1002/2016JD024999 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DW0ZN UT WOS:000383372400026 ER PT J AU Dumontier, M Gray, AJG Marshall, MS Alexiev, V Ansell, P Bader, G Baran, J Bolleman, JT Callahan, A Cruz-Toledo, J Gaudet, P Gombocz, EA Gonzalez-Beltran, AN Groth, P Haendel, M Ito, M Jupp, S Juty, N Katayama, T Kobayashi, N Krishnaswami, K Laibe, C Le Novere, N Lin, S Malone, J Miller, M Mungall, CJ Rietveld, L Wimalaratne, SM Yamaguchi, A AF Dumontier, Michel Gray, Alasdair J. G. Marshall, M. Scott Alexiev, Vladimir Ansell, Peter Bader, Gary Baran, Joachim Bolleman, Jerven T. Callahan, Alison Cruz-Toledo, Jose Gaudet, Pascale Gombocz, Erich A. Gonzalez-Beltran, Alejandra N. Groth, Paul Haendel, Melissa Ito, Maori Jupp, Simon Juty, Nick Katayama, Toshiaki Kobayashi, Norio Krishnaswami, Kalpana Laibe, Camille Le Novere, Nicolas Lin, Simon Malone, James Miller, Michael Mungall, Christopher J. Rietveld, Laurens Wimalaratne, Sarala M. Yamaguchi, Atsuko TI The health care and life sciences community profile for dataset descriptions SO PEERJ LA English DT Article DE Data profiling; Dataset descriptions; Metadata; Provenance; FAIR data ID ONTOLOGY AB Access to consistent, high-quality metadata is critical to finding, understanding, and reusing scientific data. However, while there are many relevant vocabularies for the annotation of a dataset, none sufficiently captures all the necessary metadata. This prevents uniform indexing and querying of dataset repositories. Towards providing a practical guide for producing a high quality description of biomedical datasets, the W3C Semantic Web for Health Care and the Life Sciences Interest Group (HCLSIG) identified Resource Description Framework (RDF) vocabularies that could be used to specify common metadata elements and their value sets. The resulting guideline covers elements of description, identification, attribution, versioning, provenance, and content summarization. This guideline reuses existing vocabularies, and is intended to meet key functional requirements including indexing, discovery, exchange, query, and retrieval of datasets, thereby enabling the publication of FAIR data. The resulting metadata profile is generic and could be used by other domains with an interest in providing machine readable descriptions of versioned datasets. C1 [Dumontier, Michel; Baran, Joachim; Callahan, Alison] Stanford Univ, Stanford Ctr Biomed Informat Res, Stanford, CA 94305 USA. [Gray, Alasdair J. G.] Heriot Watt Univ, Dept Comp Sci, Edinburgh, Midlothian, Scotland. [Marshall, M. Scott] MAASTRO Clin, GROW Sch Oncol & Dev Biol, Dept Radiat Oncol MAASTRO, Maastricht, Netherlands. [Alexiev, Vladimir] Ontotext Corp, Sofia, Bulgaria. [Ansell, Peter] CSIRO, Canberra, ACT, Australia. [Bader, Gary] Univ Toronto, Donnelly Ctr, Toronto, ON, Canada. [Bolleman, Jerven T.] SIB Swiss Inst Bioinformat, Swiss Prot Grp, Geneva, Switzerland. [Cruz-Toledo, Jose] Carleton Univ, Ottawa, ON K1S 5B6, Canada. [Gaudet, Pascale] SIB Swiss Inst Bioinformat, CALIPHO Grp, Geneva, Switzerland. [Gombocz, Erich A.] IO Informat, Berkeley, CA USA. [Gonzalez-Beltran, Alejandra N.] Univ Oxford, Oxford E Res Ctr, Oxford, Oxon, England. [Groth, Paul] Elsevier Labs, Amsterdam, Netherlands. [Haendel, Melissa] Oregon Hlth & Sci Univ, Dept Med Informat & Epidemiol, Portland, OR USA. [Ito, Maori] Pharmaceut & Med Devices Agcy, Off Med Informat & Epidemiol, Chiyoda Ku, Tokyo, Japan. [Jupp, Simon; Juty, Nick; Laibe, Camille; Malone, James; Wimalaratne, Sarala M.] European Bioinformat Inst, EMBL, Saffron Walden, Essex, England. [Katayama, Toshiaki; Yamaguchi, Atsuko] Database Ctr Life Sci, Kashiwa, Chiba, Japan. [Kobayashi, Norio] RIKEN, Adv Ctr Comp & Commun, Wako, Saitama, Japan. [Krishnaswami, Kalpana] Cerenode Inc, Wilmington, DE USA. [Le Novere, Nicolas] Babraham Inst, Cambridge, England. [Lin, Simon] Nationwide Childrens Hosp, Columbus, OH USA. [Miller, Michael] Inst Syst Biol, Seattle, WA USA. [Mungall, Christopher J.] Lawrence Berkeley Natl Lab, Environm Genom & Syst Biol, Berkeley, CA USA. [Rietveld, Laurens] Vrije Univ Amsterdam, Dept Exact Sci, Amsterdam, Netherlands. RP Dumontier, M (reprint author), Stanford Univ, Stanford Ctr Biomed Informat Res, Stanford, CA 94305 USA.; Gray, AJG (reprint author), Heriot Watt Univ, Dept Comp Sci, Edinburgh, Midlothian, Scotland.; Marshall, MS (reprint author), MAASTRO Clin, GROW Sch Oncol & Dev Biol, Dept Radiat Oncol MAASTRO, Maastricht, Netherlands. EM micheldumontier@gmail.com; A.J.G.Gray@hw.ac.uk; mscottmarshall@gmail.com RI KOBAYASHI, Norio/C-5685-2017; OI KOBAYASHI, Norio/0000-0002-2962-0073; Wimalaratne, Sarala/0000-0002-5355-2576; Juty, Navtej/0000-0002-2036-8350 FU NIAID, trans-NIH Big Data to Knowledge (BD2K) initiative [U54 HG008033-01]; European Union's Seventh Framework Programme (FP7) [115191]; Open PHACTS project; European Commission through the EURECA [FP7-ICT-2012-6-270253]; US National Institutes of Health grant [U41 HG006623]; Swiss Federal Government through the State Secretariat for Education, Research and Innovation; BBSRC Institute Strategic Programme [BB/J004456/1]; Integrated Database Project (Ministry of Education, Culture, Sports Science and Technology, Japan); National Bioscience Database Center (NBDC - Japan); Database Center for Life Sciences (DBCLS - Japan) FX Funding for Michel Dumontier was provided in part by grant U54 HG008033-01 awarded by NIAID through funds provided by the trans-NIH Big Data to Knowledge (BD2K) initiative. Alasdair J.G. Gray was partly funded by the Open PHACTS project and Innovative Medicines Initiative Joint Undertaking under grant agreement number 115191, the resources of which are composed of financial contribution from the European Union's Seventh Framework Programme (FP7/2007-2013) and EFPIA companies' in kind contribution. M. Scott Marshall was funded by the European Commission through the EURECA (FP7-ICT-2012-6-270253) project. Gary Bader was supported by the US National Institutes of Health grant (U41 HG006623). Jerven Bollenman's Swiss-Prot group activities are supported by the Swiss Federal Government through the State Secretariat for Education, Research and Innovation. Nicolas Le Novere was funded by the BBSRC Institute Strategic Programme BB/J004456/1. The BioHackathon series is supported by the Integrated Database Project (Ministry of Education, Culture, Sports Science and Technology, Japan), the National Bioscience Database Center (NBDC - Japan), and the Database Center for Life Sciences (DBCLS - Japan). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 26 TC 1 Z9 1 U1 2 U2 2 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD AUG 16 PY 2016 VL 4 AR e2331 DI 10.7717/peerj.2331 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT2XK UT WOS:000381344900009 PM 27602295 ER PT J AU Gando, A Gando, Y Hachiya, T Hayashi, A Hayashida, S Ikeda, H Inoue, K Ishidoshiro, K Karino, Y Koga, M Matsuda, S Mitsui, T Nakamura, K Obara, S Oura, T Ozaki, H Shimizu, I Shirahata, Y Shirai, J Suzuki, A Takai, T Tamae, K Teraoka, Y Ueshima, K Watanabe, H Kozlov, A Takemoto, Y Yoshida, S Fushimi, K Banks, TI Berger, BE Fujikawa, BK O'Donnell, T Winslow, LA Efremenko, Y Karwowski, HJ Markoff, DM Tornow, W Detwiler, JA Enomoto, S Decowski, MP AF Gando, A. Gando, Y. Hachiya, T. Hayashi, A. Hayashida, S. Ikeda, H. Inoue, K. Ishidoshiro, K. Karino, Y. Koga, M. Matsuda, S. Mitsui, T. Nakamura, K. Obara, S. Oura, T. Ozaki, H. Shimizu, I. Shirahata, Y. Shirai, J. Suzuki, A. Takai, T. Tamae, K. Teraoka, Y. Ueshima, K. Watanabe, H. Kozlov, A. Takemoto, Y. Yoshida, S. Fushimi, K. Banks, T. I. Berger, B. E. Fujikawa, B. K. O'Donnell, T. Winslow, L. A. Efremenko, Y. Karwowski, H. J. Markoff, D. M. Tornow, W. Detwiler, J. A. Enomoto, S. Decowski, M. P. CA KamLAND-Zen Collaboration TI Search for Majorana Neutrinos Near the Inverted Mass Hierarchy Region with KamLAND-Zen SO PHYSICAL REVIEW LETTERS LA English DT Article AB We present an improved search for neutrinoless double-beta (0 nu beta beta) decay of Xe-136 in the KamLAND-Zen experiment. Owing to purification of the xenon-loaded liquid scintillator, we achieved a significant reduction of the Ag-110m contaminant identified in previous searches. Combining the results from the first and second phase, we obtain a lower limit for the 0 nu beta beta decay half-life of T-1/2(0 nu) > 1.07 x 10(26) yr at 90% C.L., an almost sixfold improvement over previous limits. Using commonly adopted nuclear matrix element calculations, the corresponding upper limits on the effective Majorana neutrino mass are in the range 61-165 meV. For the most optimistic nuclear matrix elements, this limit reaches the bottom of the quasidegenerate neutrino mass region. C1 [Gando, A.; Gando, Y.; Hachiya, T.; Hayashi, A.; Hayashida, S.; Ikeda, H.; Inoue, K.; Ishidoshiro, K.; Karino, Y.; Koga, M.; Matsuda, S.; Mitsui, T.; Nakamura, K.; Obara, S.; Oura, T.; Ozaki, H.; Shimizu, I.; Shirahata, Y.; Shirai, J.; Suzuki, A.; Takai, T.; Tamae, K.; Teraoka, Y.; Ueshima, K.; Watanabe, H.] Tohoku Univ, Res Ctr Neutrino Sci, Sendai, Miyagi 9808578, Japan. [Inoue, K.; Koga, M.; Nakamura, K.; Kozlov, A.; Takemoto, Y.; Berger, B. E.; Fujikawa, B. K.; Efremenko, Y.; Tornow, W.; Detwiler, J. A.; Enomoto, S.; Decowski, M. P.] Univ Tokyo, Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Yoshida, S.] Osaka Univ, Grad Sch Sci, Toyonaka, Osaka 5600043, Japan. [Fushimi, K.] Univ Tokushima, Fac Integrated Arts & Sci, Tokushima 7708502, Japan. [Banks, T. I.; Berger, B. E.; Fujikawa, B. K.; O'Donnell, T.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Banks, T. I.; Berger, B. E.; Fujikawa, B. K.; O'Donnell, T.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Winslow, L. A.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Efremenko, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Karwowski, H. J.; Markoff, D. M.; Tornow, W.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Karwowski, H. J.; Markoff, D. M.; Tornow, W.] Duke Univ, Dept Phys, Durham, NC 27705 USA. [Karwowski, H. J.; Markoff, D. M.; Tornow, W.] North Carolina Cent Univ, Durham, NC 27701 USA. [Detwiler, J. A.; Enomoto, S.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA. [Decowski, M. P.] Nikhef, Sci Pk, NL-1098 XG Amsterdam, Netherlands. [Decowski, M. P.] Univ Amsterdam, Sci Pk, NL-1098 XG Amsterdam, Netherlands. RP Gando, A (reprint author), Tohoku Univ, Res Ctr Neutrino Sci, Sendai, Miyagi 9808578, Japan. FU JSPS KAKENHI [21000001, 26104002]; World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan; Stichting FOM in the Netherlands; U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; DOE grant; NSF grant; NII for SINET4 FX The authors wish to acknowledge Professor A. Piepke for providing radioactive sources for KamLAND. The KamLAND-Zen experiment is supported by JSPS KAKENHI Grants No. 21000001 and No. 26104002; the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan; Stichting FOM in the Netherlands; and under the U.S. Department of Energy (DOE) Contract No. DE-AC02-05CH11231, as well as other DOE and NSF grants to individual institutions. The Kamioka Mining and Smelting Company has provided service for activities in the mine. We acknowledge the support of NII for SINET4. NR 31 TC 27 Z9 27 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 16 PY 2016 VL 117 IS 8 AR 082503 DI 10.1103/PhysRevLett.117.082503 PG 6 WC Physics, Multidisciplinary SC Physics GA DT5BO UT WOS:000381495900001 PM 27588852 ER PT J AU Harrison, N AF Harrison, N. TI Number of holes contained within the Fermi surface volume in underdoped high-temperature superconductors SO PHYSICAL REVIEW B LA English DT Article ID T-C SUPERCONDUCTOR; DENSITY-WAVE ORDER; QUANTUM OSCILLATIONS; CUPRATE SUPERCONDUCTOR; CHARGE ORDER; YBA2CU3O6.67; TRANSITION; PSEUDOGAP; TRANSPORT; INSULATOR AB We provide a potential solution to the longstanding problem relating Fermi surface reconstruction to the number of holes contained within the Fermi surface volume in underdoped high T-c superconductors. On considering uniaxial and biaxial charge-density wave order, we show that there exists a relationship between the ordering wave vector, the hole doping, and the cross-sectional area of the reconstructed Fermi surface whose precise form depends on the volume of the starting Fermi surface. We consider a "large" starting Fermi surface comprising 1 + p hole carriers, as predicted by band structure calculations, and a "small" starting Fermi surface comprising p hole carriers, as proposed in models in which the Coulomb repulsion remains the dominant energy. Using the reconstructed Fermi surface cross-sectional area obtained in quantum oscillation experiments in YBa2Cu3O6+x and HgBa2CuO4+x and the established methods for estimating the chemical hole doping, we find the ordering vectors obtained from x-ray scattering measurements to show a close correspondence with those expected for the small starting Fermi surface. We therefore show the quantum oscillation frequency and charge-density wave vectors provide accurate estimates for the number of holes contributing to the Fermi surface volume in the pseudogap regime. C1 [Harrison, N.] Los Alamos Natl Labs, Mail Stop E536, Los Alamos, NM 87545 USA. RP Harrison, N (reprint author), Los Alamos Natl Labs, Mail Stop E536, Los Alamos, NM 87545 USA. OI Harrison, Neil/0000-0001-5456-7756 FU U.S. Department of Energy BES "Science at 100 T" [LANLF100]; National Science Foundation; State of Florida FX This work is supported by the U.S. Department of Energy BES "Science at 100 T" Grant No. LANLF100, the National Science Foundation, and the State of Florida. N.H. thanks Mun Chan for useful comments. NR 55 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 16 PY 2016 VL 94 IS 8 AR 085129 DI 10.1103/PhysRevB.94.085129 PG 6 WC Physics, Condensed Matter SC Physics GA DT4XP UT WOS:000381485000002 ER PT J AU Bhat, R Belardi, B Mori, H Kuo, PW Tam, A Hines, WC Le, QT Bertozzi, CR Bissell, MJ AF Bhat, Ramray Belardi, Brian Mori, Hidetoshi Kuo, Peiwen Tam, Andrew Hines, William C. Quynh-Thu Le Bertozzi, Carolyn R. Bissell, Mina J. TI Nuclear repartitioning of galectin-1 by an extracellular glycan switch regulates mammary morphogenesis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE galectin-1; sialic acid; mammary gland; breast cancer; glycobiology ID BREAST-CANCER CELLS; BRANCHING MORPHOGENESIS; CARCINOMA-CELLS; SIALIC-ACID; EXPRESSION; LECTIN; GLYCOSYLATION; SPECIFICITY; PROGRESSION; ACTIVATION AB Branching morphogenesis in the mammary gland is achieved by the migration of epithelial cells through a microenvironment consisting of stromal cells and extracellular matrix (ECM). Here we show that galectin-1 (Gal-1), an endogenous lectin that recognizes glycans bearing N-acetyllactosamine (LacNAc) epitopes, induces branching migration of mammary epithelia in vivo, ex vivo, and in 3D organotypic cultures. Surprisingly, Gal-1's effects on mammary patterning were independent of its glycan-binding ability and instead required localization within the nuclei of mammary epithelia. Nuclear translocation of Gal-1, in turn, was regulated by discrete cell-surface glycans restricted to the front of the mammary end buds. Specifically, alpha 2,6-sialylation of terminal LacNAc residues in the end buds masked Gal-1 ligands, thereby liberating the protein for nuclear translocation. Within mammary epithelia, Gal-1 localized within nuclear Gemini bodies and drove epithelial invasiveness. Conversely, unsialylated LacNAc glycans, enriched in the epithelial ducts, sequestered Gal-1 in the extracellular environment, ultimately attenuating invasive potential. We also found that malignant breast cells possess higher levels of nuclear Gal-1 and alpha 2,6-SA and lower levels of LacNAc than nonmalignant cells in culture and in vivo and that nuclear localization of Gal-1 promotes a transformed phenotype. Our findings suggest that differential glycosylation at the level of tissue microanatomy regulates the nuclear function of Gal-1 in the context of mammary gland morphogenesis and in cancer progression. C1 [Bhat, Ramray; Mori, Hidetoshi; Tam, Andrew; Hines, William C.; Bissell, Mina J.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Belardi, Brian] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mori, Hidetoshi] Univ Calif Davis, Ctr Comparat Med, Dept Pathol, Davis, CA 95616 USA. [Kuo, Peiwen; Quynh-Thu Le] Stanford Univ, Sch Med, Dept Radiat Oncol, Stanford, CA 94305 USA. [Bertozzi, Carolyn R.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Bertozzi, Carolyn R.] Stanford Univ, Howard Hughes Med Inst, Stanford, CA 94305 USA. [Bhat, Ramray] Indian Inst Sci, Dept Mol Reprod Dev & Genet, Bangalore 560012, Karnataka, India. RP Bhat, R; Bissell, MJ (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA.; Bertozzi, CR (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA.; Bertozzi, CR (reprint author), Stanford Univ, Howard Hughes Med Inst, Stanford, CA 94305 USA. EM ramray@mrdg.iisc.ernet.in; bertozzi@stanford.edu; mjbissell@lbl.gov FU US Department of Energy, Office of Biological and Environmental Research, and Low Dose Scientific Focus Area; National Cancer Institute; Breast Cancer Research Foundation; US Department of Defense; NIH [GM059907, R01CA161585-05]; Susan G. Komen for the Cure [KG111229]; National Science Foundation predoctoral fellowship FX We thank Jason Hudak, Chin Thi, and Angelica Maciel Gomes for helpful discussions and for critical reading of the manuscript. The work from the M.J.B. laboratory has been supported by grants from the US Department of Energy, Office of Biological and Environmental Research, and Low Dose Scientific Focus Area; by multiple grants from the National Cancer Institute; by a grant from the Breast Cancer Research Foundation; and by two "Innovator awards" from the US Department of Defense. The work from the C.R.B. laboratory was funded by a grant from the NIH (GM059907). The work from the Q.-T.L. laboratory was supported by a grant from the NIH (R01CA161585-05). R.B. was supported by a postdoctoral fellowship from Susan G. Komen for the Cure (KG111229), and B.B. was supported by a National Science Foundation predoctoral fellowship. NR 42 TC 2 Z9 2 U1 8 U2 12 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD AUG 16 PY 2016 VL 113 IS 33 BP E4820 EP E4827 DI 10.1073/pnas.1609135113 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT3RS UT WOS:000381399200011 PM 27496330 ER PT J AU Miller, CJ Chadha, U Ulibarri-Sanchez, JR Dickie, DA Kemp, RA AF Miller, Christopher J. Chadha, Ujwal Ulibarri-Sanchez, Jordan R. Dickie, Diane A. Kemp, Richard A. TI Structure and Lewis-base reactivity of bicyclic low-valent germanium and tin complexes bridged by bis(diisopropylphosphino)amine SO POLYHEDRON LA English DT Article DE Group 14 elements; Phosphine ligands; X-ray crystallography; Multinuclear NMR; Small molecule activation ID CARBON-DIOXIDE; DIHYDROGEN ACTIVATION; SMALL MOLECULES; CARBENE-BORANE; NMR-SPECTRA; N BONDS; CO2; INSERTION; PAIR; ADDUCT AB Lithium bis(diisopropylphosphino)amide LiN[P(i-Pr)(2)](2) reacts with SnCl2 or GeCl2 dioxane in the presence of excess n-BuLi to produce the bicyclic compounds {MN[P(i-Pr)(2)](2))(2) (M = Sn, Ge) which feature Sn-2(2+) or Ge-2(2+) units bridged by phosphorus. When paired with B(C6F5)(3) in THF, the Lewis-basic M-2(2+) complexes participate in a THF ring-opening reaction. Quite surprisingly, in the absence of THF one para-F atom from B(C6F5)(3) is activated and displaced to B while a new M-C bond is formed. Each of these complexes, as well as Cl2Sn{N[P(i-Pr)(2)](2)}(2) and {ClSnN[P(i-Pr)(2)](2))(2) were characterized by a combination of multi-nuclear NMR spectroscopy and single-crystal X-ray diffraction. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Miller, Christopher J.; Chadha, Ujwal; Ulibarri-Sanchez, Jordan R.; Dickie, Diane A.; Kemp, Richard A.] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. [Kemp, Richard A.] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. RP Kemp, RA (reprint author), Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA.; Kemp, RA (reprint author), Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. EM rakemp@unm.edu OI Dickie, Diane/0000-0003-0939-3309 FU National Science Foundation [CHE12-13529]; National Science Foundation CRIF:MU [CHE04-43580]; NSF [CHE08-40523, CHE09-46690]; United States Department of Energy [DE-AC04-94AL85000] FX This work was financially supported by the National Science Foundation (Grant CHE12-13529). The Bruker X-ray diffractometer was purchased via a National Science Foundation CRIF:MU award to the University of New Mexico (CHE04-43580), and the NMR spectrometers were upgraded via grants from the NSF (CHE08-40523 and CHE09-46690). Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94AL85000. Prof. Roger Cramer (University of Hawaii) provided helpful discussions about the polymorphs of 4. Mr. Jeremiah Sears (Sandia National Laboratories) performed the elemental analyses of compounds 1 and 6. NR 60 TC 1 Z9 1 U1 5 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD AUG 16 PY 2016 VL 114 SI SI BP 351 EP 359 DI 10.1016/j.poly.2016.01.028 PG 9 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DQ9YE UT WOS:000379564400050 ER PT J AU Supej, MJ Volkov, A Darko, L West, RA Darmon, JM Schulz, CE Wheeler, KA Hoyt, HM AF Supej, Michael J. Volkov, Alexander Darko, Louisa West, Ryan A. Darmon, Jonathan M. Schulz, Charles E. Wheeler, Kraig A. Hoyt, Helen M. TI Aryl-substituted BIAN complexes of iron dibromide: Synthesis, X-ray and electronic structure, and catalytic hydrosilylation activity SO POLYHEDRON LA English DT Article DE Iron; alpha-Diimine; Hydrosilylation; Catalysis; Bis(imino)acenaphthene ID APPROXIMATE COULOMB POTENTIALS; LIGAND COPPER(II) COMPLEXES; ZETA VALENCE QUALITY; AUXILIARY BASIS-SETS; GAUSSIAN-BASIS SETS; BIOINORGANIC CHEMISTRY; ALKENE HYDROSILYLATION; DIRADICAL CHARACTER; MOSSBAUER-SPECTRA; NICKEL-COMPLEXES AB Anhydrous iron dibromide complexes bearing bidentate alpha-diimine ligands N-Ar=C(Me) (Me)C=N-Ar and (Ar)BIAN (BIAN = bis(imino)acenaphthene; Ar = dpp and Mes; dpp = 2,6-diisopropylphenyl; Mes = 2,4,6-trimethylphenyl) have been prepared, and characterized by H-1 NMR spectroscopy. The aryl-substituted BIAN complexes were structurally characterized by single-crystal X-ray diffraction, and their metrical parameters are consistent with a redox-innocent chelating ligand. A high-spin iron(II) electronic structure description for the ArBIAN iron complexes is supported by Mossbauer spectroscopy, solution state magnetic measurements, and quantum-chemical calculations. Upon reduction, the iron complexes promote catalytic hydrosilylation of 1-hexene with phenylsilane at 22 degrees C. Under optimized conditions, 1 mol% of the (dPP)BIANFeBr(2) precatalyst was activated in situ to produce 1-hexylphenylsilane in high yield from a 1:1 ratio of 1-hexene:PhSiH3 in solvent-free conditions at 22 degrees C in 24 h. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Supej, Michael J.; Volkov, Alexander; Darko, Louisa; Hoyt, Helen M.] Knox Coll, Dept Chem, 2 E South St, Galesburg, IL 61401 USA. [West, Ryan A.] Knox Coll, Dept Phys, 2 E South St, Galesburg, IL 61401 USA. [Darmon, Jonathan M.] Pacific NW Natl Lab, Ctr Mol Electrocatalysis, Div Phys Sci, POB 999,K2-57, Richland, WA 99352 USA. [Wheeler, Kraig A.] Eastern Illinois Univ, Dept Chem, Charleston, IL 61920 USA. RP Hoyt, HM (reprint author), Knox Coll, Dept Chem, 2 E South St, Galesburg, IL 61401 USA. EM msupej@knox.edu; avolkov@knox.edu; lodarko@knox.edu; rwest@knox.edu; jonathan.darmon@pnnl.gov; cschulz@knox.edu; kawheeler@eiu.edu; hhoyt@knox.edu FU American Chemical Society Petroleum Research Fund [54044-UNI3]; National Science Foundation NSF-MRI [CHE-1427411]; NSF-MRI [CHE-0722547]; Knox College; Scripps Foundation; Paul K. Richter & Evalyn E. Cook Memorial Trust; Ford Fellowship program FX We acknowledge the donors of the American Chemical Society Petroleum Research Fund #54044-UNI3 (H.M.H.), National Science Foundation NSF-MRI award CHE-1427411 for the 400 MHz NMR spectrometer (H.M.H.), and NSF-MRI award CHE-0722547 for the X-ray diffractometer (K.A.W.). We also acknowledge funding from Knox College, The Scripps Foundation for the Mossbauer spectrometer (C.E.S.) and the IR spectrometer (H.M.H.), the Paul K. Richter & Evalyn E. Cook Memorial Trust (M.J.S., A.V., and L.D.), and the Ford Fellowship program (M.J.S.) for support of this research. We thank Carsten Milsmann for productive discussions of the computations and Marika Takemura for her initial preparation of 4a. NR 59 TC 1 Z9 1 U1 10 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD AUG 16 PY 2016 VL 114 SI SI BP 403 EP 414 DI 10.1016/j.poly.2016.02.020 PG 12 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DQ9YE UT WOS:000379564400057 ER PT J AU Ryu, SG Kim, E Allen, FI Hwang, DJ Minor, AM Grigoropoulos, CP AF Ryu, Sang-gil Kim, Eunpa Allen, Frances I. Hwang, David J. Minor, Andrew M. Grigoropoulos, Costas P. TI Incubation behavior of silicon nanowire growth investigated by laser-assisted rapid heating SO APPLIED PHYSICS LETTERS LA English DT Article ID LIQUID-SOLID GROWTH; SMALL PARTICLES; BINARY-SYSTEMS; PHASE-DIAGRAMS; KINETICS; SIZE; INTEGRATION; NUCLEATION; EPITAXY; SILANE AB We investigate the early stage of silicon nanowire growth by the vapor-liquid-solid mechanism using laser-localized heating combined with ex-situ chemical mapping analysis by energy-filtered transmission electron microscopy. By achieving fast heating and cooling times, we can precisely determine the nucleation times for nanowire growth. We find that the silicon nanowire nucleation process occurs on a time scale of similar to 10 ms, i.e., orders of magnitude faster than the times reported in investigations using furnace processes. The rate-limiting step for silicon nanowire growth at temperatures in the vicinity of the eutectic temperature is found to be the gas reaction and/or the silicon crystal growth process, whereas at higher temperatures it is the rate of silicon diffusion through the molten catalyst that dictates the nucleation kinetics. Published by AIP Publishing. C1 [Ryu, Sang-gil; Kim, Eunpa; Grigoropoulos, Costas P.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Allen, Frances I.; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Allen, Frances I.; Minor, Andrew M.] Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Hwang, David J.] SUNY Stony Brook, Dept Mech Engn, Stony Brook, NY 11794 USA. RP Grigoropoulos, CP (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM cgrigoro@berkeley.edu FU DARPA/MTO [N66001-08-1-2041]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge support by DARPA/MTO under Grant No. N66001-08-1-2041. The VLS growth experiments were carried out at the Laser Assisted Chemical Vapor Deposition (LACVD) setup in the UC Berkeley Marvell Nanolab. EFTEM analysis was performed at the Molecular Foundry at Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 31 TC 0 Z9 0 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 15 PY 2016 VL 109 IS 7 AR 073106 DI 10.1063/1.4961374 PG 5 WC Physics, Applied SC Physics GA DW6UR UT WOS:000383787400043 ER PT J AU Ying, MJ Blythe, HJ Dizayee, W Heald, SM Gerriu, FM Fox, AM Gehring, GA AF Ying, Minju Blythe, Harry J. Dizayee, Wala Heald, Steve M. Gerriu, Fatma M. Fox, A. Mark Gehring, Gillian A. TI Advantageous use of metallic cobalt in the target for pulsed laser deposition of cobalt-doped ZnO films SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETIC SEMICONDUCTOR; INDUCED FERROMAGNETISM; ROOM-TEMPERATURE; SPINTRONICS; CO AB We investigate the magnetic properties of ZnCoO thin films grown by pulsed laser deposition (PLD) from targets made containing metallic Co or CoO precursors instead of the usual Co3O4. We find that the films grown from metallic Co precursors in an oxygen rich environment contain negligible amounts of Co metal and have a large magnetization at room temperature. Structural analysis by X-ray diffraction and magneto-optical measurements indicate that the enhanced magnetism is due, in part, from Zn vacancies that partially compensate the naturally occurring n-type defects. We conclude that strongly magnetic films of Zn0.95Co0.05O that do not contain metallic cobalt can be grown by PLD from Co-metal-precursor targets if the films are grown in an oxygen atmosphere. Published by AIP Publishing. C1 [Ying, Minju; Blythe, Harry J.; Dizayee, Wala; Gerriu, Fatma M.; Fox, A. Mark; Gehring, Gillian A.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England. [Ying, Minju] Beijing Normal Univ, Minist Educ, Key Lab Beam Technol & Mat Modificat, Coll Nucl Sci & Technol, Beijing 100875, Peoples R China. [Dizayee, Wala] Salahaddin Univ, Dept Sci, Erbil, Iraq. [Heald, Steve M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Ying, MJ; Gehring, GA (reprint author), Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England.; Ying, MJ (reprint author), Beijing Normal Univ, Minist Educ, Key Lab Beam Technol & Mat Modificat, Coll Nucl Sci & Technol, Beijing 100875, Peoples R China. EM mjying@bnu.edu.cn; g.gehring@sheffield.ac.uk RI Fox, Mark/F-1096-2010 OI Fox, Mark/0000-0002-9025-2441 FU Fundamental Research Funds for the Central Universities; Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics [KF201404]; China Scholarship Council; U.K. Engineering and Physical Sciences Research [EP/D070406/1]; U.S. DOE [DE-AC02-06CH11357] FX M.Y. thanks the Fundamental Research Funds for the Central Universities, the Open Research Fund Program of the State Key Laboratory of Low-Dimensional Quantum Physics (KF201404), the China Scholarship Council for a scholarship and Sheffield University for hospitality. The SQUID and MCD measurements were taken on apparatus initially funded by the U.K. Engineering and Physical Sciences Research EP/D070406/1. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 34 TC 1 Z9 1 U1 15 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD AUG 15 PY 2016 VL 109 IS 7 AR 072403 DI 10.1063/1.4961223 PG 5 WC Physics, Applied SC Physics GA DW6UR UT WOS:000383787400028 ER PT J AU Olsen, A Key, RM van Heuven, S Lauvset, SK Velo, A Lin, XH Schirnick, C Kozyr, A Tanhua, T Hoppema, M Jutterstrom, S Steinfeldt, R Jeansson, E Ishii, M Perez, FF Suzuki, T AF Olsen, Are Key, Robert M. van Heuven, Steven Lauvset, Siv K. Velo, Anton Lin, Xiaohua Schirnick, Carsten Kozyr, Alex Tanhua, Toste Hoppema, Mario Jutterstrom, Sara Steinfeldt, Reiner Jeansson, Emil Ishii, Masao Perez, Fiz F. Suzuki, Toru TI The Global Ocean Data Analysis Project version 2 (GLODAPv2) - an internally consistent data product for the world ocean SO EARTH SYSTEM SCIENCE DATA LA English DT Article ID DISSOLVED INORGANIC CARBON; NORTH PACIFIC-OCEAN; POTENTIAL TEMPERATURE; HYDROGRAPHIC DATA; TIME-SERIES; SEA-WATER; SEAWATER; SOLUBILITY; CO2; EQUILIBRIUM AB Version 2 of the Global Ocean Data Analysis Project (GLODAPv2) data product is composed of data from 724 scientific cruises covering the global ocean. It includes data assembled during the previous efforts GLODAPv1.1 ( Global Ocean Data Analysis Project version 1.1) in 2004, CARINA (CARbon IN the Atlantic) in 2009/2010, and PACIFICA (PACIFic ocean Interior CArbon) in 2013, as well as data from an additional 168 cruises. Data for 12 core variables ( salinity, oxygen, nitrate, silicate, phosphate, dissolved inorganic carbon, total alkalinity, pH, CFC-11, CFC-12, CFC-113, and CCl4) have been subjected to extensive quality control, including systematic evaluation of bias. The data are available in two formats: (i) as submitted but updated to WOCE exchange format and (ii) as a merged and internally consistent data product. In the latter, adjustments have been applied to remove significant biases, respecting occurrences of any known or likely time trends or variations. Adjustments applied by previous efforts were re-evaluated. Hence, GLODAPv2 is not a simple merging of previous products with some new data added but a unique, internally consistent data product. This compiled and adjusted data product is believed to be consistent to better than 0.005 in salinity, 1% in oxygen, 2% in nitrate, 2% in silicate, 2% in phosphate, 4 mu mol kg(-1) in dissolved inorganic carbon, 6 mu mol kg(-1) in total alkalinity, 0.005 in pH, and 5% for the halogenated transient tracers. The original data and their documentation and doi codes are available at the Carbon Dioxide Information Analysis Center (http://cdiac.ornl.gov/oceans/GLODAPv2/). This site also provides access to the calibrated data product, which is provided as a single global file or four regional ones - the Arctic, Atlantic, Indian, and Pacific oceans - under the doi: 10.3334/CDIAC/OTG.NDP093_GLODAPv2. The product files also include significant ancillary and approximated data. These were obtained by interpolation of, or calculation from, measured data. This paper documents the GLODAPv2 methods and products and includes a broad overview of the secondary quality control results. The magnitude of and reasoning behind each adjustment is available on a per-cruise and per-variable basis in the online Adjustment Table. C1 [Olsen, Are; Lauvset, Siv K.] Univ Bergen, Inst Geophys, Allegaten 70, N-5007 Bergen, Norway. [Olsen, Are; Lauvset, Siv K.] Bjerknes Ctr Climate Res, Allegaten 70, N-5007 Bergen, Norway. [Key, Robert M.] Princeton Univ, Atmospher & Ocean Sci, 300 Forrestal Rd,Sayre Hall, Princeton, NJ 08544 USA. [van Heuven, Steven] Royal Netherlands Inst Sea Res NIOZ, Marine Geol & Chem Oceanog, POB 59, NL-1790 AB Den Burg, Netherlands. [Lauvset, Siv K.; Jeansson, Emil] Bjerknes Ctr Climate Res, Uni Res Climate, Nygardsgaten 112, N-5007 Bergen, Norway. [Velo, Anton; Perez, Fiz F.] CSIC, Inst Invest Marinas, Eduardo Cabello 6, Vigo 36208, Spain. [Schirnick, Carsten; Tanhua, Toste] GEOMAR Helmholtz Ctr Ocean Res Kiel, Dusternbrooker Weg 20, D-24105 Kiel, Germany. [Kozyr, Alex] US DOE, Carbon Dioxide Informat Anal Ctr, Div Environm Sci, Oak Ridge Natl Lab, Bldg 4500N,Mail Stop 6290, Oak Ridge, TN 37831 USA. [Hoppema, Mario] Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, Bussestr 24, D-27570 Bremerhaven, Germany. [Jutterstrom, Sara] IVL Swedish Environm Res Inst, Ascheberggatan 44, S-41133 Gothenburg, Sweden. [Steinfeldt, Reiner] Univ Bremen, Inst Environm Phys, Otto Hahn Allee, D-28359 Bremen, Germany. [Ishii, Masao] Japan Meteorol Agcy, Meteorol Res Inst, Oceanog & Geochem Res Dept, 1-1 Nagamine, Tsukuba, Ibaraki 3050052, Japan. [Suzuki, Toru] Japan Hydrog Assoc, Marine Informat Res Ctr, Ota Ku, 1-6-6-6F Hanedakuko, Tokyo 1440041, Japan. RP Olsen, A (reprint author), Univ Bergen, Inst Geophys, Allegaten 70, N-5007 Bergen, Norway.; Olsen, A (reprint author), Bjerknes Ctr Climate Res, Allegaten 70, N-5007 Bergen, Norway. EM are.olsen@gfi.uib.no RI Olsen, Are/A-1511-2011; OI Olsen, Are/0000-0003-1696-9142; Hoppema, Mario/0000-0002-2326-619X; Fernandez Perez, Fiz/0000-0003-4836-8974 FU EU-IP CARBOCHANGE (FP7) [264878]; FRAM - High North Research Centre for Climate and the Environment; Centre for Climate Dynamics at the Bjerknes Centre for Climate Research; EU AtlantOS project [633211]; Norwegian Research Council project SNACS [229752]; KeyCrafts [2012-001]; CICS [NA08OAR4320752, NA14OAR4320106]; NASA [NNX12AQ22G]; NSF [OCE-0825163, C119245, PLR-1425989, 4000133565]; DOE [DE-AC05-00OR2272]; Norwegian Research Council [214513, 229791]; U.S. National Science Foundation [OCE-1243377]; BOCATS project [CTM2013-41048-P]; Spanish Government and the Fondo Europeo de Desarrollo Regional (FEDER); AtlantOS project - EU H2020 research and innovation programme [633211] FX The GLODAPv2 project itself received support from a number of agencies and projects. Importantly, the EU-IP CARBOCHANGE (FP7 264878) provided funding for A. Olsen, M. Hoppema, S. van Heuven, and T. Tanhua as well as travel support for R. Key and the project framework that instigated GLODAPv2. A. Olsen further acknowledges generous support from the FRAM - High North Research Centre for Climate and the Environment, the Centre for Climate Dynamics at the Bjerknes Centre for Climate Research, the EU AtlantOS (grant agreement no. 633211) project, and the Norwegian Research Council project SNACS (229752). R. Key was supported by KeyCrafts grant 2012-001, CICS grants NA08OAR4320752 and NA14OAR4320106, NASA grant NNX12AQ22G, NSF grants OCE-0825163 (with a supplement via WHOI P.O. C119245) and PLR-1425989, and Battelle contract #4000133565 to CDIAC. A. Kozyr was supported by DOE contract DE-AC05-00OR2272 to UT-Battelle, operators of CDIAC under ORNL. S. K. Lauvset and E. Jeansson appreciate support from the Norwegian Research Council (projects DECApH, 214513 and VENTILATE, 229791). The International Ocean Carbon Coordination Project (IOCCP) also supported this activity through the U.S. National Science Foundation grant (OCE-1243377) to the Scientific Committee on Oceanic Research. A. Velo and F. F. Perez acknowledge the support provided by BOCATS project (CTM2013-41048-P) co-funded by the Spanish Government and the Fondo Europeo de Desarrollo Regional (FEDER), and the AtlantOS project (grant agreement no. 633211) funded by EU H2020 research and innovation programme. Benjamin Pfeil (University of Bergen) provided help with some of the data management issues during the preparation of GLODAPv2 and Karel Bakker (NIOZ) shared his invaluable insight with us, helping with the secondary quality control of the nutrient data. NR 61 TC 5 Z9 5 U1 7 U2 9 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1866-3508 EI 1866-3516 J9 EARTH SYST SCI DATA JI Earth Syst. Sci. Data PD AUG 15 PY 2016 VL 8 IS 2 BP 297 EP 323 DI 10.5194/essd-8-297-2016 PG 27 WC Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Geology; Meteorology & Atmospheric Sciences GA DV9AW UT WOS:000383232700001 ER PT J AU Lauvset, SK Key, RM Olsen, A van Heuven, S Velo, A Lin, XH Schirnick, C Kozyr, A Tanhua, T Hoppema, M Jutterstrom, S Steinfeldt, R Jeansson, E Ishii, M Perez, FF Suzuki, T Watelet, S AF Lauvset, Siv K. Key, Robert M. Olsen, Are van Heuven, Steven Velo, Anton Lin, Xiaohua Schirnick, Carsten Kozyr, Alex Tanhua, Toste Hoppema, Mario Jutterstrom, Sara Steinfeldt, Reiner Jeansson, Emil Ishii, Masao Perez, Fiz F. Suzuki, Toru Watelet, Sylvain TI A new global interior ocean mapped climatology: the 1 degrees x 1 degrees GLODAP version 2 SO EARTH SYSTEM SCIENCE DATA LA English DT Article ID CO2 ATLAS SOCAT; VARIATIONAL ANALYSIS DIVA; ANTHROPOGENIC CO2; CARBON CONTENT; ERROR FIELDS; SEA-WATER; UPDATE; MODELS AB We present a mapped climatology (GLODAPv2.2016b) of ocean biogeochemical variables based on the new GLODAP version 2 data product (Olsen et al., 2016; Key et al., 2015), which covers all ocean basins over the years 1972 to 2013. The quality- controlled and internally consistent GLODAPv2 was used to create global 1 degrees x 1 degrees mapped climatologies of salinity, temperature, oxygen, nitrate, phosphate, silicate, total dissolved inorganic carbon (TCO2), total alkalinity (TAlk), pH, and CaCO3 saturation states using the DataInterpolating Variational Analysis (DIVA) mapping method. Improving on maps based on an earlier but similar dataset, GLODAPv1.1, this climatology also covers the Arctic Ocean. Climatologies were created for 33 standard depth surfaces. The conceivably confounding temporal trends in TCO2 and pH due to anthropogenic influence were removed prior to mapping by normalizing these data to the year 2002 using first- order calculations of anthropogenic carbon accumulation rates. We additionally provide maps of accumulated anthropogenic carbon in the year 2002 and of preindustrial TCO2. For all parameters, all data from the full 1972- 2013 period were used, including data that did not receive full secondary quality control. The GLODAPv2.2016b global 1 degrees x 1 degrees mapped climatologies, including error fields and ancillary information, are available at the GLODAPv2 web page at the Carbon Dioxide Information Analysis Center (CDIAC; doi: 10.3334/ CDIAC/ OTG. NDP093_ GLODAPv2). C1 [Lauvset, Siv K.; Olsen, Are] Univ Bergen, Inst Geophys, Allegaten 70, N-5007 Bergen, Norway. [Lauvset, Siv K.; Olsen, Are] Bjerknes Ctr Climate Res, Allegaten 70, N-5007 Bergen, Norway. [Lauvset, Siv K.; Olsen, Are; Jeansson, Emil] Bjerknes Ctr Climate Res, Uni Res Climate, Allegt 55, N-5007 Bergen, Norway. [Key, Robert M.; Lin, Xiaohua] Princeton Univ, Atmospher & Ocean Sci, 300 Forrestal Rd,Sayre Hall, Princeton, NJ 08544 USA. [van Heuven, Steven] Royal Netherlands Inst Sea Res NIOZ, Marine Geol & Chem Oceanog, POB 59, NL-1790 AB Den Burg, Netherlands. [Velo, Anton; Perez, Fiz F.] CSIC, Inst Invest Marinas, Eduardo Cabello 6, Vigo 36208, Spain. [Schirnick, Carsten; Tanhua, Toste] GEOMAR Helmholtz Ctr Ocean Res Kiel, Dusternbrooker Weg 20, D-24105 Kiel, Germany. [Kozyr, Alex] US DOE, Carbon Dioxide Informat Anal Ctr, Div Environm Sci, Oak Ridge Natl Lab, Bldg 4500N,Mail Stop 6290, Oak Ridge, TN 37831 USA. [Hoppema, Mario] Alfred Wegener Inst, Helmholtz Ctr Polar & Marine Res, Bussestr 24, D-27570 Bremerhaven, Germany. [Jutterstrom, Sara] IVL Swedish Environm Res Inst, Ascheberggatan 44, S-41133 Gothenburg, Sweden. [Steinfeldt, Reiner] Univ Bremen, Inst Environm Phys, Otto Hahn Allee, D-28359 Bremen, Germany. [Ishii, Masao] Japan Meteorol Agcy, Oceanog & Geochem Res Dept, Meteorol Res Inst, 1-1 Nagamine, Tsukuba, Ibaraki 3050052, Japan. [Suzuki, Toru] Japan Hydrog Assoc, Marine Informat Res Ctr, Ota Ku, 1-6-6-6F Hanedakuko, Tokyo 1440041, Japan. [Watelet, Sylvain] Univ Liege, Dept Astrophys Geophys & Oceanog, Liege, Belgium. RP Lauvset, SK (reprint author), Univ Bergen, Inst Geophys, Allegaten 70, N-5007 Bergen, Norway.; Lauvset, SK (reprint author), Bjerknes Ctr Climate Res, Allegaten 70, N-5007 Bergen, Norway. EM siv.lauvset@uib.no RI Olsen, Are/A-1511-2011 OI Olsen, Are/0000-0003-1696-9142 FU Norwegian Research Council [214513/F20, 229752, 229791]; EU-IP CARBOCHANGE (FP7) [264878]; FRAM - High North Research Centre for Climate and the Environment; Centre for Climate Dynamics at the Bjerknes Centre for Climate Research; EU AtlantOS project [633211]; KeyCrafts grant [2012-001]; CICS [NA08OAR4320752, NA14OAR4320106]; NASA [NNX12AQ22G]; NSF [OCE-0825163, C119245, PLR-1425989, 4000133565]; US Department of Energy; project MEXT [24121003]; BOCATS project [CTM20134410484P]; Spanish government and the Fondo Europeo de Desarrollo Regional (FEDER); U.S. National Science Foundation [OCE-1243377] FX The work of S. K. Lauvset was funded by the Norwegian Research Council through the projects DECApH (214513/F20). The EU-IP CARBOCHANGE (FP7 264878) project provided funding for A. Olsen, S. van Heuven, T. Tanhua, R. Steinfeldt, and M. Hoppema and is the project framework that instigated GLODAPv2. A. Olsen additionally acknowledges generous support from the FRAM - High North Research Centre for Climate and the Environment, the Centre for Climate Dynamics at the Bjerknes Centre for Climate Research, the EU AtlantOS (grant agreement no. 633211) project, and the Norwegian Research Council project SNACS (229752). Emil Jeansson appreciates support from the Norwegian Research Council project VENTILATE (229791). R. Key was supported by KeyCrafts grant 2012-001, CICS grants NA08OAR4320752 and NA14OAR4320106, NASA grant NNX12AQ22G, NSF grants OCE-0825163 (with a supplement via WHOI P.O. C119245) and PLR-1425989, and Battelle contract #4000133565 to CDIAC. A. Kozyr acknowledges funding from the US Department of Energy. M. Ishii acknowledges the project MEXT 24121003. A. Velo and F. F. Perez were supported by the BOCATS (CTM20134410484P) project cofounded by the Spanish government and the Fondo Europeo de Desarrollo Regional (FEDER). The International Ocean Carbon Coordination Project (IOCCP) partially supported this activity through the U.S. National Science Foundation grant (OCE-1243377) to the Scientific Committee on Oceanic Research.; The research leading to the last developments of DIVA has received funding from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 283607, SeaDataNet 2, and from the project EMODNET (MARE/2012/10 - Lot 4 Chemistry - SI2.656742) from the Directorate-General for Maritime Affairs and Fisheries. NR 32 TC 1 Z9 1 U1 3 U2 3 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1866-3508 EI 1866-3516 J9 EARTH SYST SCI DATA JI Earth Syst. Sci. Data PD AUG 15 PY 2016 VL 8 IS 2 BP 325 EP 340 DI 10.5194/essd-8-325-2016 PG 16 WC Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Geology; Meteorology & Atmospheric Sciences GA DV9AZ UT WOS:000383233000001 ER PT J AU DeGraffenreid, AJ Feng, YT Wycoff, DE Morrow, R Phipps, MD Cutler, CS Ketring, AR Barnes, CL Jurisson, SS AF DeGraffenreid, Anthony J. Feng, Yutian Wycoff, Donald E. Morrow, Ryan Phipps, Michael D. Cutler, Cathy S. Ketring, Alan R. Barnes, Charles L. Jurisson, Silvia S. TI Dithiol Aryl Arsenic Compounds as Potential Diagnostic and Therapeutic Radiopharmaceuticals SO INORGANIC CHEMISTRY LA English DT Article ID IN-VITRO; CHROMATOGRAPHIC-SEPARATION; SE-72/AS-72 GENERATOR; CHEMISTRY; ANTIDOTES; GERMANIUM; PROTEIN; AS-72 AB Arsenic-72 (As-72) and As-77 have nuclear properties useful for positron emission tomography (PET) and radiotherapy, respectively. The thiophilic nature of arsenic led to the evaluation of dithioarylarsines for potential use in radiopharmaceuticals. Several dithioarylarsines were synthesized from their arylarsonic acids and dithiols and were fully characterized by NMR, ESI-MS, and X-ray crystallography. This chemistry was translated to the no-carrier-added (nca) As-77 level. Because arsenic was available at the nca nanomolar level only as [As-77]arsenate, this required addition of an aryl group directly to the As to form the [As-77]arylarsonic acid. The [As-77]arsenate was reduced from As-77 (V) to As-77 (III), and a modified Bart reaction was used to incorporate the aryl ring onto the As-77, which was followed by dithiol addition. Various modifications and optimizations resulted in 95% radiochemical yield of nca [As-77]p-ethoxyphenyl-1,2-ethanedithiolatoarsine. C1 [DeGraffenreid, Anthony J.; Feng, Yutian; Wycoff, Donald E.; Morrow, Ryan; Phipps, Michael D.; Barnes, Charles L.; Jurisson, Silvia S.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Cutler, Cathy S.; Ketring, Alan R.; Jurisson, Silvia S.] Univ Missouri, Res Reactor Ctr MURK, Columbia, MO 65211 USA. [DeGraffenreid, Anthony J.; Cutler, Cathy S.] Brookhaven Natl Lab, Collider Accelerator Dept, Med Isotope Res & Prod Program MIRP, POB 5000,Bldg 801, Upton, NY 11973 USA. RP Jurisson, SS (reprint author), Univ Missouri, Dept Chem, Columbia, MO 65211 USA.; Jurisson, SS (reprint author), Univ Missouri, Res Reactor Ctr MURK, Columbia, MO 65211 USA. EM jurissons@missouri.edu FU NIBIB training grant [5T32-EB004822]; DOE [DE-SC0003851, DE-SC0010283] FX This work was supported by NIBIB training grant 5T32-EB004822 (A.J.D.) and DOE grants DE-SC0003851 and DE-SC0010283. Special thanks to Dr. Nathan Leigh, University of Missouri, for the collection of ESI-MS data, and Dr. Wei Wycoff, University of Missouri, for assistance with NMR and the respective facilities used. NR 41 TC 1 Z9 1 U1 4 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD AUG 15 PY 2016 VL 55 IS 16 BP 8091 EP 8098 DI 10.1021/acs.inorgchem.6b01175 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DT6KW UT WOS:000381594100038 PM 27453472 ER PT J AU Misichronis, K Chen, JH Kahk, JK Imel, A Dadmun, M Hong, KL Hadjichristidis, N Mays, JW Avgeropoulos, A AF Misichronis, Konstantinos Chen, Jihua Kahk, Jong K. Imel, Adam Dadmun, Mark Hong, Kunlun Hadjichristidis, Nikos Mays, Jimmy W. Avgeropoulos, Apostolos TI Diblock Copolymers of Polystyrene-b-Poly(1,3-cyclohexadiene) Exhibiting Unique Three-Phase Microdomain Morphologies SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE anionic polymerization; diblock copolymers; differential scanning calorimetry (DSC); TEM; SAXS ID COIL BLOCK-COPOLYMERS; LINEAR TRIBLOCK TERPOLYMERS; CONFORMATIONAL ASYMMETRY; ANIONIC-POLYMERIZATION; 1,3-CYCLOHEXADIENE POLYMERS; MICROPHASE SEPARATION; PHASE-BEHAVIOR; POLY(CYCLOHEXADIENE); THERMODYNAMICS; MICELLES AB The synthesis and molecular characterization of series of conformationally asymmetric polystyrene-blockpoly(1,3-cyclohexadiene) (PS-b-PCHD) diblock copolymers (PCHD: 90% 1,4 and similar to 10% 1,2), by sequential anionic copolymerization high vacuum techniques, is reported. A vvide range of volume fractions (0.27 <= (phi PS) <= 0.91) was studied by transmission electron microscopy and small-angle X-ray scattering in order to explore in detail the microphase separation behavior of these flexiblefsemiflexible diblock copolymers. Unusual morphologies, consisting of PCHD core(PCHD-1,4)-shell(PCHD-1,2) cylinders in PS matrix and three-phase (PS, PCHD-1,4, PCHD-1,2) four-layer lamellae, were observed suggesting that the chain stiffness of the PCHD block and the strong dependence of the interaction parameter chi on the PCHD microstructures are important factors for the formation of this unusual microphase separation behavior irk PS-b-PCHD diblock copolymers (C) 2016 Wile Periodicals Inc. C1 [Misichronis, Konstantinos; Chen, Jihua; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Misichronis, Konstantinos; Imel, Adam; Dadmun, Mark; Mays, Jimmy W.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Misichronis, Konstantinos; Avgeropoulos, Apostolos] Univ Ioannina, Dept Mat Sci Engn, Univ Campus Dourouti, GR-45110 Ioannina, Greece. [Kahk, Jong K.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Hadjichristidis, Nikos; Avgeropoulos, Apostolos] King Abdullah Univ Sci & Technol KAUST, KAUST Catalysis Ctr, Phys Sci & Engn Div, Polymer Synth Lab, Thuwal 23955, Saudi Arabia. RP Avgeropoulos, A (reprint author), Univ Ioannina, Dept Mat Sci Engn, Univ Campus Dourouti, GR-45110 Ioannina, Greece.; Avgeropoulos, A (reprint author), King Abdullah Univ Sci & Technol KAUST, KAUST Catalysis Ctr, Phys Sci & Engn Div, Polymer Synth Lab, Thuwal 23955, Saudi Arabia. EM aavger@cc.uoi.gr RI Hong, Kunlun/E-9787-2015; OI Hong, Kunlun/0000-0002-2852-5111; Keum, Jong/0000-0002-5529-1373; Misichronis, Konstantinos/0000-0002-2620-1738 FU Materials Science and Engineering Division, U.S. Department of Energy (DoE), Office of Basic Energy Sciences (BES) [DEAC05-00OR22725]; UT-Battelle, LLC at Oak Ridge National Laboratory (ORNL); Scientific User Facilities Division of DoE; King Abdullah University of Science and Technology (KAUST) FX This work was supported by the Materials Science and Engineering Division, U.S. Department of Energy (DoE), Office of Basic Energy Sciences (BES) under contract No. DEAC05-00OR22725 with UT-Battelle, LLC at Oak Ridge National Laboratory (ORNL). Part of the research was done at the Center for Nanophase Materials Sciences, which is sponsored by the Scientific User Facilities Division of DoE through a user project to J. W. Mays. A. Avgeropoulos also thank the nuclear magnetic resonance spectroscopy and the electron microscopy facilities of the University of Ioannina. The research reported in this publication was partially supported by funding from King Abdullah University of Science and Technology (KAUST). NR 56 TC 1 Z9 1 U1 7 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD AUG 15 PY 2016 VL 54 IS 16 BP 1564 EP 1572 DI 10.1002/polb.24050 PG 9 WC Polymer Science SC Polymer Science GA DT2FE UT WOS:000381295400003 ER PT J AU Capps, N Montgomery, R Sunderland, D Pytel, M Wirth, BD AF Capps, Nathan Montgomery, Robert Sunderland, Dion Pytel, Martin Wirth, Brian D. TI Evaluation of missing pellet surface geometry on cladding stress distribution and magnitude SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID FUEL PELLETS; INTERACTION PCI; SIMULATION; EXPANSION; BEHAVIOR AB Missing pellet surface (MPS) defects are local geometric defects in nuclear fuel pellets that result from pellet mishandling or manufacturing. The presence of MPS defects can cause significant clad stress concentrations that can lead to through-wall cladding failure for certain combinations of fuel burnup, and reactor power level or power change. Consequently, the impact of MPS defects has limited the rate of power increase, or ramp rate, in both pressurized and boiling water reactors (PWRs and BWRs, respectively). Improved three-dimensional (3-D) fuel performance models of MPS defect geometry can provide better understanding of the probability for pellet clad mechanical interaction (PCMI), and correspondingly the available margin against cladding failure by stress corrosion cracking (SCC). The Consortium of Advanced Simulations of Light Water Reactors (CASL) has been developing the Bison-CASL fuel performance code to consider the inherently multi-physics and multi-dimensional mechanisms that control fuel behavior, including cladding stress concentrations resulting from MPS defects. This paper evaluates the cladding hoop stress distributions as a function of MPS defect geometry with discrete pellet radial cracks for a set of typical operating conditions in a PWR fuel rod. The results provide a first step toward a probabilistic approach to assess cladding failure during power maneuvers. This analysis provides insight into how varying pellet defect geometries affect the distribution of the cladding stress, as well as the temperature distributions within the fuel and clad; and are used to develop stress concentration factors for comparing 2-D and 3-D models. Published by Elsevier B.V. C1 [Capps, Nathan; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Montgomery, Robert; Sunderland, Dion] Pacific Northwest Natl Lab, Richland, WA 99354 USA. [Sunderland, Dion] ANATECH Corp, San Diego, CA 92121 USA. [Pytel, Martin] Elect Power Res Inst, 3412 Hillview Ave, Palo Alto, CA 94304 USA. RP Capps, N (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. FU Consortium for Advanced Simulation of Light Water Reactors; Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy [DE-AC05-00OR2272] FX This research was supported by the Consortium for Advanced Simulation of Light Water Reactors (http://www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-00OR2272. NR 25 TC 1 Z9 1 U1 5 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD AUG 15 PY 2016 VL 305 BP 51 EP 63 DI 10.1016/j.nucengdes.2016.04.039 PG 13 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DV5XG UT WOS:000383003400006 ER PT J AU Lillo, TM van Rooyen, IJ Wu, YQ AF Lillo, T. M. van Rooyen, I. J. Wu, Y. Q. TI Precession electron diffraction for SiC grain boundary characterization in unirradiated TRISO fuel SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID COATED PARTICLES; AGR-1 EXPERIMENT; SILVER; MICROSTRUCTURE; TEMPERATURE; PALLADIUM; EBSD AB Precession electron diffraction (PED), a transmission electron microscopy-based technique, has been evaluated for the suitability for evaluating grain boundary character in the SiC layer of tristructural isotropic(TRISO) fuel. This work reports the effect of transmission electron microscope (TEM) lamella thickness on the quality of data and establishes a baseline comparison to SiC grain boundary characteristics, in an unirradiated TRISO particle, determined previously using a conventional electron backscatter diffraction (EBSD) scanning electron microscope (SEM)-based technique. In general, it was determined that the lamella thickness produced using the standard focused ion beam (FIB) fabrication process (similar to 80 nm), is sufficient to provide reliable PED measurements, although thicker lamellae (similar to 120 nm) were found to produce higher quality orientation data. Also, analysis of SiC grain boundary character from the TEM-based PED data showed a much lower fraction of low-angle grain boundaries compared to SEM-based EBSD data from the SiC layer of a TRISO-coated particle made using the same fabrication parameters and a SiC layer deposited at a slightly lower temperature from a surrogate TRISO particle. However, the fractions of high-angle and coincident site lattice (CSL)-related grain boundaries determined by PED are similar to those found using SEM-based EBSD. Since the grain size of the SiC layer of TRSIO fuel can be as small as 250 nm (Kirchhofer et al., 2013), depending on the fabrication parameters, and since grain boundary fission product precipitates in irradiated TRISO fuel can be nano-sized, the TEM-based PED orientation data collection method is preferred to determine an accurate representation of the relative fractions of low-angle, high-angle, and CSL-related grain boundaries. It was concluded that although the resolution of the PED data is better by more than an order of magnitude, data acquisition times may be significantly longer or the number of areas analyzed needs to be significantly greater than the SEM-based method to obtain a statistically relevant distribution. Also, grain size could be accurately determined but significantly larger analysis areas would be required than those used in this study. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lillo, T. M.] Idaho Natl Lab, Dept Mat Sci & Engn, Idaho Falls, ID 83415 USA. [van Rooyen, I. J.] Idaho Natl Lab, Fuel Performance & Design Dept, Idaho Falls, ID 83415 USA. [Wu, Y. Q.] Boise State Univ, Micron Sch Mat Sci & Engn, Boise, ID 83725 USA. [Wu, Y. Q.] Ctr Adv Energy Studies, Idaho Falls, ID 83401 USA. RP Lillo, TM (reprint author), Idaho Natl Lab, Dept Mat Sci & Engn, Idaho Falls, ID 83415 USA. EM thomas.lillo@inl.gov RI Lilllo, Thomas/S-5031-2016 OI Lilllo, Thomas/0000-0002-7572-7883 FU US Department of Energy, Office of Nuclear Energy, under DOE Idaho Operations Office, as part of Very High Temperature Reactor Development Program [DEAC07051D14517]; National Science Users Facility Program FX This work was sponsored by the US Department of Energy, Office of Nuclear Energy, under DOE Idaho Operations Office Contract DEAC07051D14517, as part of the Very High Temperature Reactor Development Program as well as the National Science Users Facility Program. The authors would like to acknowledge the efforts of Mr. James Madden in the FIB-fabrication of the TEM samples as well as other staff at the Materials and Fuels Complex at INL and those at the Center for Advanced Energy Studies. NR 21 TC 0 Z9 0 U1 5 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD AUG 15 PY 2016 VL 305 BP 277 EP 283 DI 10.1016/j.nucengdes.2016.05.027 PG 7 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DV5XG UT WOS:000383003400027 ER PT J AU Puig, F Dennis, H AF Puig, Francesc Dennis, Haile TI Neutron fluence effects on SLOWPOKE-2 beryllium reflector composition and reactivity SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article AB Within the scope of the conversion process from HEU to LEU of the Jamaican SLOWPOKE-2 reactor (JM-1), the effects of the neutron fluence on the beryllium reflector composition, and the corresponding effect on reactivity throughout the life of the reactor core, have been studied. Two different methods have been used and compared involving MCNP5, ORIGEN2.2, ORIGEN-S and COUPLE codes, reaching excellent agreement between them. The neutron flux profile and energy spectrum specific to the beryllium reflectors of this reactor design have been taken into account to analyze several scenarios, comprising both real and hypothetical conditions and involving different initial reflector compositions and reactor burnups. The analysis has been extended to provide estimates for the similar MNSR reactor design and compared with previously published predictions for the Syrian MNSR. The results show small overall reactivity effects in most cases, being dominated by impurity depletion as opposed to poison buildup, contrarily to what generally occurs in beryllium reflected reactors of far higher power and to MNSR predictions. The resulting reactivity increases are typically of less than 0.4 mk for usual impurity levels and maximum HEU core burnup achievable. (C) 2016 Elsevier B.V. All rights reserved. C1 [Puig, Francesc] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Dennis, Haile] Univ West Indies, Int Ctr Environm & Nucl Sci, 2 Anguilla Close, Kingston 7, Jamaica. RP Puig, F (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM fpuig@anl.gov; haile.dennis02@uwimona.edu.jm OI Puig, Francesc/0000-0002-9370-5880 FU U.S. Department of Energy, National Nuclear Safety Administration (NNSA), Office of Material Management and Minimization Reactor Conversion Program [NA-23]; Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This work is sponsored by the U.S. Department of Energy, National Nuclear Safety Administration (NNSA), Office of Material Management and Minimization (NA-23) Reactor Conversion Program.; The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 12 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD AUG 15 PY 2016 VL 305 BP 451 EP 460 DI 10.1016/j.nucengdes.2016.05.033 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DV5XG UT WOS:000383003400042 ER PT J AU Mohanty, S Soppet, WK Majumdar, S Natesan, K AF Mohanty, Subhasish Soppet, William K. Majumdar, Saurindranath Natesan, Krishnamurti TI Chaboche-based cyclic material hardening models for 316 SS-316 SS weld under in-air and pressurized water reactor water conditions SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article AB This paper discusses a material hardening models for welds made from 316 stainless steel (SS) to 316 SS. The model parameters were estimated from the strain-versus-stress curves obtained from tensile and fatigue tests conducted under different conditions (air at room temperature, air at 300 degrees C, and primary loop water conditions for a pressurized water reactor). These data were used to check the fatigue cycle dependency of the material hardening parameters (yield stress, parameters related to Chaboche-based linear and nonlinear kinematic hardening models, etc.). The details of the experimental results, material hardening models, and associated calculated results are published in an Argonne report (ANL/LWRS-15/2). This paper summarizes the reported material parameters for 316 SS-316 SS welds and their dependency on fatigue cycles and other test conditions. (C) 2016 Elsevier B.V. All rights reserved. C1 [Mohanty, Subhasish; Soppet, William K.; Majumdar, Saurindranath; Natesan, Krishnamurti] Argonne Natl Lab, Lemont, IL 60439 USA. RP Mohanty, S (reprint author), Argonne Natl Lab, Lemont, IL 60439 USA. EM smohanty@anl.gov FU U.S. Department of Energy FX This research was supported through the U.S. Department of Energy's Light Water Reactor Sustainability program under the work package of environmental fatigue study, program manager Dr Jeremy Busby (FY 2015) and Dr. Keith Leonard (FY 2016). NR 17 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD AUG 15 PY 2016 VL 305 BP 524 EP 530 DI 10.1016/j.nucengdes.2016.05.031 PG 7 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DV5XG UT WOS:000383003400049 ER PT J AU Mohanty, S Majumdar, S Natesan, K AF Mohanty, Subhasish Majumdar, Saurin Natesan, Ken TI Steam generator tube rupture simulation using extended finite element method SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID ARBITRARY EVOLVING CRACKS; THROUGH-WALL CRACKS; MESHFREE METHOD; MESHLESS METHODS; COALESCENCE; FRACTURE; PROPAGATION; PREDICTION; GROWTH AB A steam generator (SG) is an important component of any pressurized water reactor. Steam generator tubes represent a primary pressure boundary whose integrity is vital to the safe operation of the reactor. SG tubes may rupture due to propagation of a crack created by mechanisms such as stress corrosion cracking, fatigue, etc. It is thus important to estimate the rupture pressures of cracked tubes for structural integrity evaluation of SGs. The objective of the present paper is to demonstrate the use of extended finite element method capability of commercially available ABAQUS software, to model SG tubes with preexisting flaws and to estimate their rupture pressures. For the purpose, elastic-plastic finite element models were developed for different SG tubes made from Alloy 600 material. The simulation results were compared with experimental results available from the steam generator tube integrity program (SGTIP) sponsored by the United States Nuclear Regulatory Commission (NRC) and conducted at Argonne National Laboratory (ANL). A reasonable correlation was found between extended finite element model results and experimental results. (C) 2016 Elsevier B.V. All rights reserved. C1 [Mohanty, Subhasish; Majumdar, Saurin; Natesan, Ken] Argonne Natl Lab, Nucl Engn Div, Lemont, IL USA. RP Mohanty, S (reprint author), Argonne Natl Lab, Nucl Engn Div, Lemont, IL USA. EM smohanty@anl.gov FU Department of Energy of United States of America; Light Water Reactor Sustainability Research and Development effort; US-NRC-sponsored SGTIP program FX This research was sponsored by the Department of Energy of United States of America, for the Light Water Reactor Sustainability Research and Development effort, under the program manager Dr. Jeremy Busby. Test results from the US-NRC-sponsored SGTIP program were used to validate the finite element model results. NR 35 TC 2 Z9 2 U1 4 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD AUG 15 PY 2016 VL 305 BP 697 EP 705 DI 10.1016/j.nucengdes.2016.06.031 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DV5XG UT WOS:000383003400064 ER PT J AU Chu, PH Kim, YJ Savukov, I AF Chu, P. -H. Kim, Y. J. Savukov, I. TI Search for exotic spin-dependent interactions with a spin-exchange relaxation-free magnetometer SO PHYSICAL REVIEW D LA English DT Article ID ATOMIC MAGNETOMETER; DC SQUID; FORCES; PARTICLES; ELECTRONS; AXIONS; LIMITS AB We propose a novel experimental approach to explore exotic spin-dependent interactions using a spin-exchange relaxation-free (SERF) magnetometer, the most sensitive noncryogenic magnetic-field sensor. This approach studies the interactions between optically polarized electron spins located inside a vapor cell of the SERF magnetometer and unpolarized or polarized particles of external solid-state objects. The coupling of spin-dependent interactions to the polarized electron spins of the magnetometer induces the tilt of the electron spins, which can be detected with high sensitivity by a probe laser beam similarly as an external magnetic field. We estimate that by moving unpolarized or polarized objects next to the SERF Rb vapor cell, the experimental limit to the spin-dependent interactions can be significantly improved over existing experiments, and new limits on the coupling strengths can be set in the interaction range below 10(-2) m. C1 [Chu, P. -H.; Kim, Y. J.; Savukov, I.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chu, PH; Kim, YJ (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM pchu@lanl.gov; youngjin@lanl.gov OI Savukov, Igor/0000-0003-4190-5335 FU U.S. DOE through the LANL/LDRD program FX The authors thank H. Gao, J. Long, and W. M. Snow for useful discussions. The authors gratefully acknowledge this work was supported by the U.S. DOE through the LANL/LDRD program. NR 58 TC 1 Z9 1 U1 14 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 15 PY 2016 VL 94 IS 3 AR 036002 DI 10.1103/PhysRevD.94.036002 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DT4ZO UT WOS:000381490500005 ER PT J AU Bohm, V Schmittfull, M Sherwin, BD AF Boehm, Vanessa Schmittfull, Marcel Sherwin, Blake D. TI Bias to CMB lensing measurements from the bispectrum of large-scale structure SO PHYSICAL REVIEW D LA English DT Article ID PRIMORDIAL NON-GAUSSIANITY; MATTER POWER SPECTRUM; POLARIZATION ANISOTROPIES; COSMOLOGICAL PARAMETERS; REDUCED SHEAR; DARK-MATTER; MICROWAVE; TEMPERATURE; RECONSTRUCTION; MODEL AB The rapidly improving precision of measurements of gravitational lensing of the cosmic microwave background (CMB) also requires a corresponding increase in the precision of theoretical modeling. A commonly made approximation is to model the CMB deflection angle or lensing potential as a Gaussian random field. In this paper, however, we analytically quantify the influence of the non-Gaussianity of large-scale structure (LSS) lenses, arising from nonlinear structure formation, on CMB lensing measurements. In particular, evaluating the impact of the nonzero bispectrum of large-scale structure on the relevant CMB four-point correlation functions, we find that there is a bias to estimates of the CMB lensing power spectrum. For temperature-based lensing reconstruction with CMB stage III and stage IV experiments, we find that this lensing power spectrum bias is negative and is of order 1% of the signal. This corresponds to a shift of multiple standard deviations for these upcoming experiments. We caution, however, that our numerical calculation only evaluates two of the largest bias terms and, thus, only provides an approximate estimate of the full bias. We conclude that further investigation into lensing biases from nonlinear structure formation is required and that these biases should be accounted for in future lensing analyses. C1 [Boehm, Vanessa] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85748 Garching, Germany. [Schmittfull, Marcel; Sherwin, Blake D.] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Schmittfull, Marcel; Sherwin, Blake D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sherwin, Blake D.] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. RP Bohm, V (reprint author), Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85748 Garching, Germany. EM vboehm@mpa-garching.mpg.de NR 66 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD AUG 15 PY 2016 VL 94 IS 4 AR 043519 DI 10.1103/PhysRevD.94.043519 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DT4ZW UT WOS:000381491300006 ER PT J AU Belopolski, I Xu, SY Ishida, Y Pan, XC Yu, P Sanchez, DS Zheng, H Neupane, M Alidoust, N Chang, GQ Chang, TR Wu, Y Bian, G Huang, SM Lee, CC Mou, DX Huang, LN Song, Y Wang, BG Wang, GH Yeh, YW Yao, N Rault, JE Le Fevre, P Bertran, F Jeng, HT Kondo, T Kaminski, A Lin, H Liu, Z Song, FQ Shin, S Hasan, MZ AF Belopolski, Ilya Xu, Su-Yang Ishida, Yukiaki Pan, Xingchen Yu, Peng Sanchez, Daniel S. Zheng, Hao Neupane, Madhab Alidoust, Nasser Chang, Guoqing Chang, Tay-Rong Wu, Yun Bian, Guang Huang, Shin-Ming Lee, Chi-Cheng Mou, Daixiang Huang, Lunan Song, You Wang, Baigeng Wang, Guanghou Yeh, Yao-Wen Yao, Nan Rault, Julien E. Le Fevre, Patrick Bertran, Francois Jeng, Horng-Tay Kondo, Takeshi Kaminski, Adam Lin, Hsin Liu, Zheng Song, Fengqi Shin, Shik Hasan, M. Zahid TI Fermi arc electronic structure and Chern numbers in the type-II Weyl semimetal candidate MoxW1-xTe2 SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; WANNIER FUNCTIONS; BASIS-SET; METALS AB It has recently been proposed that electronic band structures in crystals can give rise to a previously overlooked type of Weyl fermion, which violates Lorentz invariance and, consequently, is forbidden in particle physics. It was further predicted that MoxW1-xTe2 may realize such a type-II Weyl fermion. Here, we first show theoretically that it is crucial to access the band structure above the Fermi level epsilon(F) to show a Weyl semimetal in MoxW1-xTe2. Then, we study MoxW1-xTe2 by pump-probe ARPES and we directly access the band structure > 0.2 eV above epsilon(F) in experiment. By comparing our results with ab initio calculations, we conclude that we directly observe the surface state containing the topological Fermi arc. We propose that a future study of MoxW1-xTe2 by pump-probe ARPES may directly pinpoint the Fermi arc. Our work sets the stage for the experimental discovery of the first type-II Weyl semimetal in MoxW1-xTe2. C1 [Belopolski, Ilya; Xu, Su-Yang; Sanchez, Daniel S.; Zheng, Hao; Alidoust, Nasser; Bian, Guang; Hasan, M. Zahid] Princeton Univ, Dept Phys, Lab Topol Quantum Matter & Spect B7, Princeton, NJ 08544 USA. [Ishida, Yukiaki; Kondo, Takeshi; Shin, Shik] Univ Tokyo, ISSP, Kashiwa, Chiba 2778581, Japan. [Pan, Xingchen; Wang, Baigeng; Wang, Guanghou; Song, Fengqi] Nanjing Univ, Natl Lab Solid State Microstruct, Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Pan, Xingchen; Wang, Baigeng; Wang, Guanghou; Song, Fengqi] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Yu, Peng; Liu, Zheng] Nanyang Technol Univ, Sch Mat Sci & Engn, Ctr Programmable Mat, Singapore 639798, Singapore. [Neupane, Madhab] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Chang, Guoqing; Lee, Chi-Cheng; Lin, Hsin] Natl Univ Singapore, Ctr Adv Mat 2D, 6 Sci Dr 2, Singapore 117546, Singapore. [Chang, Guoqing; Lee, Chi-Cheng; Lin, Hsin] Natl Univ Singapore, Graphene Res Ctr, 6 Sci Dr 2, Singapore 117546, Singapore. [Chang, Guoqing; Lee, Chi-Cheng; Lin, Hsin] Natl Univ Singapore, Dept Phys, 2 Sci Dr 3, Singapore 117546, Singapore. [Chang, Tay-Rong; Jeng, Horng-Tay] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Wu, Yun; Mou, Daixiang; Huang, Lunan; Kaminski, Adam] US DOE, Ames Lab, Ames, IA 50011 USA. [Wu, Yun; Mou, Daixiang; Huang, Lunan; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Huang, Shin-Ming] Natl Sun Yat Sen Univ, Dept Phys, Kaohsiung 80424, Taiwan. [Song, You] Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Sch Chem & Chem Engn, State Key Lab Coordinat Chem, Nanjing 210093, Jiangsu, Peoples R China. [Yeh, Yao-Wen; Yao, Nan; Hasan, M. Zahid] Princeton Univ, Princeton Inst Sci & Technol Mat, Princeton, NJ 08544 USA. [Rault, Julien E.; Le Fevre, Patrick; Bertran, Francois] Synchrotron SOLEIL, Orme Merisiers, St Aubin BP 48, F-91192 Gif Sur Yvette, France. [Jeng, Horng-Tay] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Liu, Zheng] Nanyang Technol Univ, NOVITAS, Nanoelect Ctr Excellence, Sch Elect & Elect Engn, Singapore 639798, Singapore. [Liu, Zheng] CINTRA CNRS NTU THALES, UMI 3288, Res Techno Plaza,50 Nanyang Dr,Border 10 Block, Singapore 637553, Singapore. RP Belopolski, I (reprint author), Princeton Univ, Dept Phys, Lab Topol Quantum Matter & Spect B7, Princeton, NJ 08544 USA. EM ilyab@princeton.edu; z.liu@ntu.edu.sg; songfengqi@nju.edu.cn; mzhasan@princeton.edu RI Chang, Tay-Rong/K-3943-2015; Song, Fengqi/E-7474-2010; BERTRAN, Francois/B-7515-2008; Lin, Hsin/F-9568-2012; ISHIDA, Yukiaki/D-4261-2016; zheng, hao/H-8636-2015 OI Chang, Tay-Rong/0000-0003-1222-2527; BERTRAN, Francois/0000-0002-2416-0514; Lin, Hsin/0000-0002-4688-2315; zheng, hao/0000-0002-6495-874X FU U.S. DOE/BES [DE-FG-02-05ER46200]; US National Science Foundation GRFP; Japan Society for the Promotion of Science [KAKENHI 26800165]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. Department of Energy [DE-AC02-07CH11358]; University of Central Florida; National Key Projects for Basic Research of China [2013CB922100, 2011CB922103]; National Natural Science Foundation of China [91421109, 11522432, 21571097]; Singapore National Research Foundation (NRF) under NRF RF Award [NRF-RF2013-08]; Nanyang Technological University [M4081137.070]; National Science Council, Taiwan; Singapore NRF [NRF-NRFF2013-03] FX Work at Princeton and Princeton-led ARPES measurements were supported by the U.S. DOE/BES under DE-FG-02-05ER46200. I.B. and D.S. thank Moritz Hoesch and Timur Kim for support during synchrotron ARPES measurements at Beamline I05 of Diamond Lightsource in Didcot, UK. I.B. acknowledges the support of the US National Science Foundation GRFP. Y.I. is supported by the Japan Society for the Promotion of Science, KAKENHI 26800165. The ARPES measurements at Ames Lab were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. M.N. is supported by start-up funds from the University of Central Florida. X.C.P., Y.S., B.G.W., G.H.W., and F.Q.S. thank the National Key Projects for Basic Research of China (Grant Nos. 2013CB922100 and 2011CB922103), the National Natural Science Foundation of China (Grant Nos. 91421109, 11522432, and 21571097) and the NSF of Jiangsu province (No. BK20130054). This work is also financially supported by the Singapore National Research Foundation (NRF) under NRF RF Award No. NRF-RF2013-08, the start-up funding from Nanyang Technological University (M4081137.070). T.-R.C. and H.-T.J. were supported by the National Science Council, Taiwan. H.-T.J. also thanks the National Center for High-Performance Computing, Computer and Information Network Center National Taiwan University, and the National Center for Theoretical Sciences, Taiwan, for technical support. H.L. acknowledges the Singapore NRF under Award No. NRF-NRFF2013-03. NR 44 TC 20 Z9 20 U1 29 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 15 PY 2016 VL 94 IS 8 AR 085127 DI 10.1103/PhysRevB.94.085127 PG 7 WC Physics, Condensed Matter SC Physics GA DT4XJ UT WOS:000381484400004 ER PT J AU Hung, LD da Jornada, FH Souto-Casares, J Chelikowsky, JR Louie, SG Ogut, S AF Hung, Linda da Jornada, Felipe H. Souto-Casares, Jaime Chelikowsky, James R. Louie, Steven G. Ogut, Serdar TI Excitation spectra of aromatic molecules within a real-space GW-BSE formalism: Role of self-consistency and vertex corrections SO PHYSICAL REVIEW B LA English DT Article ID QUASI-PARTICLE; GREENS-FUNCTION; ELECTRON-GAS; PHOTOELECTRON-SPECTRUM; OPTICAL-PROPERTIES; EXCITED-STATES; APPROXIMATION; ENERGIES; IONIZATION; NANOSTRUCTURES AB We present first-principles calculations on the vertical ionization potentials (IPs), electron affinities (EAs), and singlet excitation energies on an aromatic-molecule test set (benzene, thiophene, 1,2,5-thiadiazole, naphthalene, benzothiazole, and tetrathiafulvalene) within the GW and Bethe-Salpeter equation (BSE) formalisms. Our computational framework, which employs a real-space basis for ground-state and a transition-space basis for excited-state calculations, is well suited for high-accuracy calculations on molecules, as we show by comparing against G(0)W(0) calculations within a plane-wave-basis formalism. We then generalize our framework to test variants of the GW approximation that include a local density approximation (LDA)-derived vertex function (Gamma(LDA)) and quasiparticle-self-consistent (QS) iterations. We find that Gamma(LDA) and quasiparticle self-consistency shift IPs and EAs by roughly the same magnitude, but with opposite sign for IPs and the same sign for EAs. G(0)W(0) and QSGW Gamma(LDA) are more accurate for IPs, while G(0)W(0)Gamma(LDA) and QSGW are best for EAs. For optical excitations, we find that perturbative GW-BSE underestimates the singlet excitation energy, while self-consistent GW-BSE results in good agreement with previous best-estimate values for both valence and Rydberg excitations. Finally, our work suggests that a hybrid approach, in which G0W0 energies are used for occupied orbitals and G(0)W(0)Gamma(LDA) for unoccupied orbitals, also yields optical excitation energies in good agreement with experiment but at a smaller computational cost. C1 [Hung, Linda; Ogut, Serdar] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Hung, Linda] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [da Jornada, Felipe H.; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [da Jornada, Felipe H.; Louie, Steven G.] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Souto-Casares, Jaime; Chelikowsky, James R.] Univ Texas Austin, Ctr Computat Mat, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. RP Hung, LD (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA.; Hung, LD (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM linda.hung@nist.gov; ogut@uic.edu OI Hung, Linda/0000-0002-1578-6152 FU US Department of Energy [DE-FG02-09ER16072]; Scientific Discovery through Advanced Computing (SciDAC) Program on Excited State Phenomena in Energy Materials - US Department of Energy, Office of Basic Energy Sciences; Advanced Scientific Computing Research at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; National Science Foundation [DMR-1508412]; SciDAC program - US Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences [DE-SC0008877]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX L.H. and S.O. would like to thank the US Department of Energy, Grant No. DE-FG02-09ER16072, for support. Part of this research (F.H.J. and S.G.L.) was supported by the Scientific Discovery through Advanced Computing (SciDAC) Program on Excited State Phenomena in Energy Materials funded by the US Department of Energy, Office of Basic Energy Sciences, and by Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory, which provided algorithm and code developments and simulations, and by the National Science Foundation under Grant No. DMR-1508412, which provided basic theoretical analyses. J.S.C. and J.R.C. also acknowledge support provided by the SciDAC program funded by the US Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences, under Award No. DE-SC0008877. All authors used resources at the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 90 TC 2 Z9 2 U1 9 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 15 PY 2016 VL 94 IS 8 AR 085125 DI 10.1103/PhysRevB.94.085125 PG 13 WC Physics, Condensed Matter SC Physics GA DT4XJ UT WOS:000381484400002 ER PT J AU Yamada, T Takakura, H Kong, T Das, P Jayasekara, WT Kreyssig, A Beutier, G Canfield, PC de Boissieu, M Goldman, AI AF Yamada, T. Takakura, H. Kong, T. Das, P. Jayasekara, W. T. Kreyssig, A. Beutier, G. Canfield, P. C. de Boissieu, M. Goldman, A. I. TI Atomic structure of the i-R-Cd quasicrystals and consequences for magnetism SO PHYSICAL REVIEW B LA English DT Article ID ANTIFERROMAGNETIC ORDER; PENROSE LATTICE; ZN; APPROXIMANT; ALLOYS; TB; HO AB We report on the six-dimensional (6D) structural refinement of three members of the i-R-Cd quasicrystals (R = Gd, Dy, Tm) via synchrotron x-ray diffraction from single-grain samples, and show that this series is isostructural to the i-YbCd5.7 quasicrystal. However, our refinements suggest that the R occupancy on the Yb icosahedron sites within the Tsai-type atomic cluster is approximately 80%, with the balance taken up by Cd. Similarities between the i-R-Cd series and i-ScZn7.33, and their differences with i-YbCd5.7 and i-Ca15Cd85, indicate that there are at least two subclasses of Tsai-type icosahedral quasicrystals. We further show from x-ray resonant magnetic scattering (XRMS) measurements on a set of closely related Tb1-xYxCd6 1/1 approximants that the dilution of themagnetic R ions on the icosahedron within the Tsai-type cluster by nonmagnetic Y disrupts the commensurate magnetic ordering in the approximant phase. C1 [Yamada, T.] Tohoku Univ, Inst Multidisciplinary Res Adv Materials, Sendai, Miyagi 9809870, Japan. [Takakura, H.] Hokkaido Univ, Fac Engn, Div Appl Phys, Sapporo, Hokkaido 0608628, Japan. [Kong, T.; Das, P.; Jayasekara, W. T.; Kreyssig, A.; Canfield, P. C.; Goldman, A. I.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Kong, T.; Das, P.; Jayasekara, W. T.; Kreyssig, A.; Canfield, P. C.; Goldman, A. I.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Beutier, G.; de Boissieu, M.] Univ Grenoble Alpes, SIMaP, F-38000 Grenoble, France. [Beutier, G.; de Boissieu, M.] CNRS, SIMaP, F-38000 Grenoble, France. RP Yamada, T (reprint author), Tohoku Univ, Inst Multidisciplinary Res Adv Materials, Sendai, Miyagi 9809870, Japan. FU U.S. DOE [DE-AC02-06CH11357]; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-07CH11358]; JSPS KAKENHI [15K04659]; ANR [2011-BS04-004-01]; [26-2924] FX We thank the synchrotron SOLEIL for the allowance of beam time for the structural measurements and P. Fertey for his help in setting up the experiment on the CRISTAL beamline. Figures 2 and 3 were obtained using VESTA software [42]. Use of the Advanced Photon Source was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Work at the Ames Laboratory was supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-07CH11358. Work at Tohoku University was supported by a Grant-in-Aid for JSPS Research Fellows No. 26-2924. Work at Hokkaido University was supported by JSPS KAKENHI No. 15K04659. Work at University Grenoble Alpes was supported by ANR 2011-BS04-004-01. Part of this study was carried out within the European C-MAC network. NR 41 TC 1 Z9 1 U1 13 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD AUG 15 PY 2016 VL 94 IS 6 AR 060103 DI 10.1103/PhysRevB.94.060103 PG 5 WC Physics, Condensed Matter SC Physics GA DT4VG UT WOS:000381478700001 ER PT J AU Ba, Y Liu, HH Li, Q Kang, QJ Sun, JJ AF Ba, Yan Liu, Haihu Li, Qing Kang, Qinjun Sun, Jinju TI Multiple-relaxation-time color-gradient lattice Boltzmann model for simulating two-phase flows with high density ratio SO PHYSICAL REVIEW E LA English DT Article ID IMMISCIBLE FLUIDS; VARIABLE-DENSITY; POROUS-MEDIA; DROP IMPACT; EQUATION; DISPLACEMENT; COMPONENTS; INTERFACE; DYNAMICS; SURFACES AB In this paper we propose a color-gradient lattice Boltzmann (LB) model for simulating two-phase flows with high density ratio and high Reynolds number. The model applies a multirelaxation-time (MRT) collision operator to enhance the stability of the simulation. A source term, which is derived by the Chapman-Enskog analysis, is added into the MRT LB equation so that the Navier-Stokes equations can be exactly recovered. Also, a form of the equilibrium density distribution function is used to simplify the source term. To validate the proposed model, steady flows of a static droplet and the layered channel flow are first simulated with density ratios up to 1000. Small values of spurious velocities and interfacial tension errors are found in the static droplet test, and improved profiles of velocity are obtained by the present model in simulating channel flows. Then, two cases of unsteady flows, Rayleigh-Taylor instability and droplet splashing on a thin film, are simulated. In the former case, the density ratio of 3 and Reynolds numbers of 256 and 2048 are considered. The interface shapes and spike and bubble positions are in good agreement with the results of previous studies. In the latter case, the droplet spreading radius is found to obey the power law proposed in previous studies for the density ratio of 100 and Reynolds number up to 500. C1 [Ba, Yan; Liu, Haihu; Sun, Jinju] Xi An Jiao Tong Univ, Sch Energy & Power Engn, 28 West Xianning Rd, Xian 710049, Peoples R China. [Ba, Yan; Kang, Qinjun] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Li, Qing] Cent S Univ, Sch Energy Sci & Engn, Changsha 410083, Hunan, Peoples R China. [Sun, Jinju] Collaborat Innovat Ctr Adv Aeroengine CICAAE, Beijing, Peoples R China. RP Sun, JJ (reprint author), Xi An Jiao Tong Univ, Sch Energy & Power Engn, 28 West Xianning Rd, Xian 710049, Peoples R China.; Sun, JJ (reprint author), Collaborat Innovat Ctr Adv Aeroengine CICAAE, Beijing, Peoples R China. EM jjsun@mail.xjtu.edu.cn RI Liu, Haihu/B-2097-2013 OI Liu, Haihu/0000-0002-0295-1251 FU National Natural Science Foundation of China [51576148, 51506168]; LANL's LDRD Program; Institutional Computing Program; China Scholarship Council; "Young Thousand Talents Program" of China FX The authors acknowledge the support from National Natural Science Foundation of China under Grants No. 51576148 and No. 51506168, and from LANL's LDRD Program and Institutional Computing Program. Y.B. would like to acknowledge the financial support from the China Scholarship Council. H.L. gratefully acknowledges the support from the "Young Thousand Talents Program" of China. NR 54 TC 2 Z9 2 U1 13 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 15 PY 2016 VL 94 IS 2 AR 023310 DI 10.1103/PhysRevE.94.023310 PG 15 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DT5AF UT WOS:000381492200017 PM 27627415 ER PT J AU Johnson, MG Knauer, JP Cerjan, CJ Eckart, MJ Grim, GP Hartouni, EP Hatarik, R Kilkenny, JD Munro, DH Sayre, DB Spears, BK Bionta, RM Bond, EJ Caggiano, JA Callahan, D Casey, DT Doppner, T Frenje, JA Glebov, VY Hurricane, O Kritcher, A LePape, S Ma, T Mackinnon, A Meezan, N Patel, P Petrasso, RD Ralph, JE Springer, PT Yeamans, CB AF Johnson, M. Gatu Knauer, J. P. Cerjan, C. J. Eckart, M. J. Grim, G. P. Hartouni, E. P. Hatarik, R. Kilkenny, J. D. Munro, D. H. Sayre, D. B. Spears, B. K. Bionta, R. M. Bond, E. J. Caggiano, J. A. Callahan, D. Casey, D. T. Doppner, T. Frenje, J. A. Glebov, V. Yu. Hurricane, O. Kritcher, A. LePape, S. Ma, T. Mackinnon, A. Meezan, N. Patel, P. Petrasso, R. D. Ralph, J. E. Springer, P. T. Yeamans, C. B. TI Indications of flow near maximum compression in layered deuterium-tritium implosions at the National Ignition Facility SO PHYSICAL REVIEW E LA English DT Article ID INERTIAL-CONFINEMENT FUSION; SPECTRA; TARGETS; OMEGA AB An accurate understanding of burn dynamics in implosions of cryogenically layered deuterium (D) and tritium (T) filled capsules, obtained partly through precision diagnosis of these experiments, is essential for assessing the impediments to achieving ignition at the National Ignition Facility. We present measurements of neutrons from such implosions. The apparent ion temperatures T-ion are inferred from the variance of the primary neutron spectrum. Consistently higher DT than DD T-ion are observed and the difference is seen to increase with increasing apparent DT T-ion. The line-of-sight rms variations of both DD and DT T-ion are small, similar to 150 eV, indicating an isotropic source. The DD neutron yields are consistently high relative to the DT neutron yields given the observed T-ion. Spatial and temporal variations of the DT temperature and density, DD-DT differential attenuation in the surrounding DT fuel, and fluid motion variations contribute to a DT T-ion greater than the DD T-ion, but are in a one-dimensional model insufficient to explain the data. We hypothesize that in a three-dimensional interpretation, these effects combined could explain the results. C1 [Johnson, M. Gatu; Frenje, J. A.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Knauer, J. P.; Glebov, V. Yu.] Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. [Cerjan, C. J.; Eckart, M. J.; Grim, G. P.; Hartouni, E. P.; Hatarik, R.; Munro, D. H.; Sayre, D. B.; Spears, B. K.; Bionta, R. M.; Bond, E. J.; Caggiano, J. A.; Callahan, D.; Casey, D. T.; Doppner, T.; Hurricane, O.; Kritcher, A.; LePape, S.; Ma, T.; Mackinnon, A.; Meezan, N.; Patel, P.; Ralph, J. E.; Springer, P. T.; Yeamans, C. B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kilkenny, J. D.] Gen Atom Co, San Diego, CA 92186 USA. RP Johnson, MG (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM gatu@psfc.mit.edu RI Patel, Pravesh/E-1400-2011 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors sincerely thank the NIF operations staff, who supported this work. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 53 TC 0 Z9 0 U1 6 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD AUG 15 PY 2016 VL 94 IS 2 AR 021202 DI 10.1103/PhysRevE.94.021202 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DT5AF UT WOS:000381492200001 PM 27627237 ER PT J AU Huang, ZS Balatsky, AV AF Huang, Zhoushen Balatsky, Alexander V. TI Dynamical Quantum Phase Transitions: Role of Topological Nodes in Wave Function Overlaps SO PHYSICAL REVIEW LETTERS LA English DT Article ID STATISTICAL-MECHANICS; CHERN NUMBER; ENERGY; THERMALIZATION; LOCALIZATION; SYSTEMS; STATES; GASES AB A sudden quantum quench of a Bloch band from one topological phase toward another has been shown to exhibit an intimate connection with the notion of a dynamical quantum phase transition (DQPT), where the returning probability of the quenched state to the initial state-i.e., the Loschmidt echo-vanishes at critical times {t*}. Analytical results to date are limited to two-band models, leaving the exact relation between topology and DQPT unclear. In this Letter, we show that, for a general multiband system, a robust DQPT relies on the existence of nodes (i.e., zeros) in the wave function overlap between the initial band and the postquench energy eigenstates. These nodes are topologically protected if the two participating wave functions have distinctive topological indices. We demonstrate these ideas in detail for both one and two spatial dimensions using a three-band generalized Hofstadter model. We also discuss possible experimental observations. C1 [Huang, Zhoushen; Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] NORDITA, Roslagstullsbacken 23, SE-10691 Stockholm, Sweden. RP Huang, ZS (reprint author), Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. EM zsh@lanl.gov; avb@nordita.org FU U.S. DOE [BES E304/E3B7]; ERC [DM 321031] FX We are grateful to D. P. Arovas, A. Alexandradinata, and A. Saxena for the useful discussions. We thank J. M. Zhang for communications regarding a recent work [62]. Work at LANL was supported by U.S. DOE Grant No. BES E304/E3B7. Work at NORDITA was supported by ERC Grant No. DM 321031. NR 59 TC 2 Z9 2 U1 6 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 15 PY 2016 VL 117 IS 8 AR 086802 DI 10.1103/PhysRevLett.117.086802 PG 6 WC Physics, Multidisciplinary SC Physics GA DT5BH UT WOS:000381495100021 PM 27588874 ER PT J AU Lovato, A Gandolfi, S Carlson, J Pieper, SC Schiavilla, R AF Lovato, A. Gandolfi, S. Carlson, J. Pieper, Steven C. Schiavilla, R. TI Electromagnetic Response of C-12: A First-Principles Calculation SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRON-SCATTERING; LIGHT-NUCLEI; MONTE-CARLO; FORM-FACTORS; TRANSITION AB The longitudinal and transverse electromagnetic response functions of C-12 are computed in a "first-principles" Green's function Monte Carlo calculation, based on realistic two- and three-nucleon interactions and associated one-and two-body currents. We find excellent agreement between theory and experiment and, in particular, no evidence for the quenching of the measured versus calculated longitudinal response. This is further corroborated by a reanalysis of the Coulomb sum rule, in which the contributions from the low-lying J(pi) = 2(+), 0(2)(+) (Hoyle), and 4(+) states in C-12 are accounted for explicitly in evaluating the total inelastic strength. C1 [Lovato, A.; Pieper, Steven C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Gandolfi, S.; Carlson, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Schiavilla, R.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. [Schiavilla, R.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. RP Lovato, A (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC52-06NA25396, DE-AC05-06OR23177]; NUCLEI SciDAC program; LANL LDRD program; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357, DE-AC02-05CH11231] FX A critical reading of the manuscript by Ingo Sick is gratefully acknowledged. We also thank P. von Neumann-Cosel for providing us with the data on the form factor for the transition from the ground state in 12C to the Hoyle state. This research is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 (A. L. and S. C. P.), No. DE-AC52-06NA25396 (S. G. and J. C.), and No. DE-AC05-06OR23177 (R. S.), and by the NUCLEI SciDAC and LANL LDRD programs. Under an award of computer time provided by the INCITE program, this research used resources of the Argonne Leadership Computing Facility at Argonne National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. It also used resources provided by Los Alamos Open Supercomputing, by Argonne LCRC, and by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 42 TC 2 Z9 2 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 15 PY 2016 VL 117 IS 8 AR 082501 DI 10.1103/PhysRevLett.117.082501 PG 5 WC Physics, Multidisciplinary SC Physics GA DT5BH UT WOS:000381495100006 PM 27588850 ER PT J AU Shao, JH Shi, JR Antipov, SP Baryshev, SV Chen, HB Conde, M Gai, W Ha, GH Jing, CG Wang, FY Wisniewski, E AF Shao, Jiahang Shi, Jiaru Antipov, Sergey P. Baryshev, Sergey V. Chen, Huaibi Conde, Manoel Gai, Wei Ha, Gwanghui Jing, Chunguang Wang, Faya Wisniewski, Eric TI In Situ Observation of Dark Current Emission in a High Gradient rf Photocathode Gun SO PHYSICAL REVIEW LETTERS LA English DT Article ID FIELD-EMISSION; ELECTRON-EMISSION; CATHODES AB Undesirable electron field emission (also known as dark current) in high gradient rf photocathode guns deteriorates the quality of the photoemission current and limits the operational gradient. To improve the understanding of dark current emission, a high-resolution (similar to 100 mu m) dark current imaging experiment has been performed in an L-band photocathode gun operating at similar to 100 MV/m of surface gradient. Scattered strong emission areas with high current have been observed on the cathode. The field enhancement factor beta of selected regions on the cathode has been measured. The postexaminations with scanning electron microscopy and white light interferometry reveal the origins of similar to 75% strong emission areas overlap with the spots where rf breakdown has occurred. C1 [Shao, Jiahang; Shi, Jiaru; Chen, Huaibi] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Shao, Jiahang; Antipov, Sergey P.; Baryshev, Sergey V.; Conde, Manoel; Gai, Wei; Ha, Gwanghui; Jing, Chunguang; Wisniewski, Eric] Argonne Natl Lab, Lemont, IL 60439 USA. [Antipov, Sergey P.; Baryshev, Sergey V.; Jing, Chunguang] Euclid Techlabs LLC, Bolingbrook, IL 60440 USA. [Wang, Faya] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Shao, JH (reprint author), Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China.; Shao, JH (reprint author), Argonne Natl Lab, Lemont, IL 60439 USA. EM shaojh07@mails.tsinghua.edu.cn; jingchg@anl.gov FU U.S. Department of Energy Office of Science [DE-AC02-06CH11357]; National Natural Science Foundation of China [11135004]; U.S. Department of Energy Early Career Research Program [LAB 11-572]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We would like to thank the Tsinghua University machine shop for preparing the new shaped cathodes, all staff in the AWA group for their work in the experiment, Dr. Klaus Flottmann from DESY for his great help with the ASTRA code and other useful discussions, and Paul Schoessow of Euclid TechLabs for his valuable comments on the manuscript. The work by the AWA group is funded through the U.S. Department of Energy Office of Science under Contract No. DE-AC02-06CH11357. The work at Tsinghua University is supported by National Natural Science Foundation of China under Grant No. 11135004. The work by F. Wang is supported by the U.S. Department of Energy Early Career Research Program under Contract Code LAB 11-572. SEM measurements were conducted in the Electron Microscopy Center of the Center for Nanoscale Materials at Argonne National Laboratory. Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 29 TC 0 Z9 0 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 15 PY 2016 VL 117 IS 8 AR 084801 DI 10.1103/PhysRevLett.117.084801 PG 5 WC Physics, Multidisciplinary SC Physics GA DT5BH UT WOS:000381495100013 PM 27588860 ER PT J AU Surh, MP Benedict, LX Sadigh, B AF Surh, Michael P. Benedict, Lorin X. Sadigh, Babak TI Magnetostructural Transition Kinetics in Shocked Iron SO PHYSICAL REVIEW LETTERS LA English DT Article ID AUGMENTED-WAVE METHOD; PHASE-TRANSITION; AB-INITIO; PRESSURE; MAGNETISM; FE AB A generalized Heisenberg model is implemented to study the effect of thermal magnetic disorder on kinetics of the Fe alpha-epsilon transition. The barrier to bulk martensitic displacement remains large in alpha-Fe shocked well past the phase line but is much reduced in the [001] alpha-epsilon boundary. The first result is consistent with observed overdriving to metastable alpha, while the second suggests structural instability, as implied by observation of a [001] shock transformation front without plastic relaxation. Reconciling both behaviors may require concurrent treatment of magnetic and structural order. C1 [Surh, Michael P.; Benedict, Lorin X.; Sadigh, Babak] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Surh, MP (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM surh1@llnl.gov; benedict5@llnl.gov; sadigh1@llnl.gov FU Laboratory Directed Research and Development (LDRD) Program at LLNL [13-ERD-044]; U.S. Department of Energy [DE-AC52-07NA27344] FX The authors thank Hector Lorenzana for helpful collaboration, and Jon Belof for informative discussions. We also thank Timothy Germann for providing the Fe interatomic potential in Ref. [12]. This work was supported by the Laboratory Directed Research and Development (LDRD) Program at LLNL under tracking code No. 13-ERD-044. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 32 TC 1 Z9 1 U1 4 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 15 PY 2016 VL 117 IS 8 AR 085701 DI 10.1103/PhysRevLett.117.085701 PG 5 WC Physics, Multidisciplinary SC Physics GA DT5BH UT WOS:000381495100018 PM 27588867 ER PT J AU Waitz, M Metz, D Lower, J Schober, C Keiling, M Pitzer, M Mertens, K Martins, M Viefhaus, J Klumpp, S Weber, T Schmidt-Bocking, H Schmidt, LPH Morales, F Miyabe, S Rescigno, TN McCurdy, CW Martin, F Williams, JB Schoffler, MS Jahnke, T Dorner, R AF Waitz, M. Metz, D. Lower, J. Schober, C. Keiling, M. Pitzer, M. Mertens, K. Martins, M. Viefhaus, J. Klumpp, S. Weber, T. Schmidt-Boecking, H. Schmidt, L. Ph. H. Morales, F. Miyabe, S. Rescigno, T. N. McCurdy, C. W. Martin, F. Williams, J. B. Schoeffler, M. S. Jahnke, T. Doerner, R. TI Two-Particle Interference of Electron Pairs on a Molecular Level SO PHYSICAL REVIEW LETTERS LA English DT Article ID DOUBLE-SLIT; MOMENTUM SPECTROSCOPY; RECOIL-ION; PHOTOIONIZATION AB We investigate the photodouble ionization of H-2 molecules with 400 eV photons. We find that the emitted electrons do not show any sign of two-center interference fringes in their angular emission distributions if considered separately. In contrast, the quasiparticle consisting of both electrons (i.e., the "dielectron") does. The work highlights the fact that nonlocal effects are embedded everywhere in nature where many-particle processes are involved. C1 [Waitz, M.; Metz, D.; Lower, J.; Schober, C.; Keiling, M.; Schmidt-Boecking, H.; Schmidt, L. Ph. H.; Schoeffler, M. S.; Jahnke, T.; Doerner, R.] Goethe Univ Frankfurt, Inst Kernphys, Max von Laue Str 1, D-60438 Frankfurt, Germany. [Pitzer, M.] Univ Kassel, Heinr Plett Str 40, D-34132 Kassel, Germany. [Mertens, K.; Martins, M.] Univ Hamburg, Inst Expt Phys, Luruper Chaussee 149, D-22761 Hamburg, Germany. [Viefhaus, J.] DESY, FS PE, Notkestr 85, D-22607 Hamburg, Germany. [Klumpp, S.] DESY, FS FL, Notkestr 85, D-22607 Hamburg, Germany. [Weber, T.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Morales, F.] Max Born Inst, Max Born Str 2 A, D-12489 Berlin, Germany. [Miyabe, S.] RIKEN Ctr Adv Photon, Attosecond Sci Res Team, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Rescigno, T. N.; McCurdy, C. W.] Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA. [McCurdy, C. W.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Martin, F.] Univ Autonoma Madrid, Dept Quim, E-28049 Madrid, Spain. [Martin, F.] Inst Madrileno Estudios Avanzados Nanociencia, Madrid 28049, Spain. [Martin, F.] Univ Autonoma Madrid, Condensed Matter Phys Ctr IFIMAC, E-28049 Madrid, Spain. [Williams, J. B.] Univ Nevada, Dept Phys, 1664 North Virginia St, Reno, NV 89557 USA. RP Dorner, R (reprint author), Goethe Univ Frankfurt, Inst Kernphys, Max von Laue Str 1, D-60438 Frankfurt, Germany. EM doerner@atom.uni-frankfurt.de RI Doerner, Reinhard/A-5340-2008; Martin, Fernando/C-3972-2014; OI Doerner, Reinhard/0000-0002-3728-4268; Martin, Fernando/0000-0002-7529-925X; Martins, Michael/0000-0002-1228-5029 FU Deutsche Forschungsgemeinschaft (DFG); BMBF; European COST Action [XLIC CM1204]; European Research Council Advanced XCHEM [290853]; MINECO Project [FIS2013-42002-R]; DFG FX This work was funded by the Deutsche Forschungsgemeinschaft (DFG), the BMBF, the European COST Action Grant No. XLIC CM1204, the European Research Council Advanced XCHEM Grant No. 290853, and the MINECO Project Grant No. FIS2013-42002-R. J. L. thanks the DFG for support. We are grateful to the staff of PETRA III for excellent support during the beam time. Raw data are archived at the Goethe-University Frankfurt am Main and are available on request. NR 23 TC 0 Z9 0 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD AUG 15 PY 2016 VL 117 IS 8 AR 083002 DI 10.1103/PhysRevLett.117.083002 PG 5 WC Physics, Multidisciplinary SC Physics GA DT5BH UT WOS:000381495100009 PM 27588854 ER PT J AU Antinao, JL McDonald, E Rhodes, EJ Brown, N Barrera, W Gosse, JC Zimmermann, S AF Antinao, Jose Luis McDonald, Eric Rhodes, Edward J. Brown, Nathan Barrera, Wendy Gosse, John C. Zimmermann, Susan TI Late Pleistocene-Holocene alluvial stratigraphy of southern Baja California, Mexico SO QUATERNARY SCIENCE REVIEWS LA English DT Article DE Late Pleistocene; Holocene; Alluvial fans; Tropical cyclones; Baja California; North America; Sonoran desert; Mexico ID GULF-OF-CALIFORNIA; SEA-SURFACE TEMPERATURES; SOUTHWEST UNITED-STATES; NORTH-AMERICAN MONSOON; CYCLONE JULIETTE 2001; LAST GLACIAL MAXIMUM; SAN-ANDREAS FAULT; TROPICAL CYCLONES; COSMOGENIC NUCLIDES; MID-WISCONSIN AB A late Pleistocene to Holocene alluvial stratigraphy has been established for the basins of La Paz and San Jose del Cabo, in the southern tip of the Baja California peninsula, Mexico. Six discrete alluvial units (Qt1 through Qt6) were differentiated across the region using a combination of geomorphologic mapping, sedimentological analysis, and soil development. These criteria were supported using radiocarbon, optically stimulated luminescence and cosmogenic depth-profile geochronology. Major aggradation started shortly after similar to 70 ka (Qt2), and buildup of the main depositional units ended at similar to 10 ka (Qt4). After deposition of Qt4, increasing regional incision of older units and the progressive development of a channelized alluvial landscape coincide with deposition of Qt5 and Qt6 units in a second, incisional phase. All units consist of multiple 1-3 m thick alluvial packages deposited as upper-flow stage beds that represent individual storms. Main aggradational units (Qt2-Qt4) occurred across broad (>2 km) channels in the form of sheetflood deposition while incisional stage deposits are confined to channels of similar to 0.5 -2 km width. Continuous deposition inside the thicker (>10 m) pre-Qt5 units is demonstrated by closely spaced dates in vertical profiles. In a few places, disconformities between these major units are nevertheless evident and indicated by partly eroded buried soils. The described units feature sedimentological traits similar to historical deposits formed by large tropical cyclone events, but also include characteristics of upper-regime flow sedimentation not shown by historical sediments, like long (>10 m) wavelength antidunes and transverse ribs. We interpret the whole sequence as indicating discrete periods during the late Pleistocene and Holocene when climatic conditions allowed larger and more frequent tropical cyclone events than those observed historically. These discrete periods are associated with times when insolation at the tropics was higher than the present-day conditions, determined by precessional cycles, and modulated by the presence of El Nino-like conditions along the tropical and northeastern Pacific. The southern Baja California alluvial record is the first to document a precession-driven alluvial chronology for the region, and it constitutes a strong benchmark for discrimination of direct tropical influence on any other alluvial record in southwestern North America. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Antinao, Jose Luis; McDonald, Eric] Desert Res Inst, Div Earth & Ecosyst Sci, 2215 Raggio Pkwy, Reno, NV 89512 USA. [Antinao, Jose Luis] CIGIDEN, Natl Res Ctr Integrated Nat Disaster Management, Santiago 7820436, Chile. [Rhodes, Edward J.; Brown, Nathan; Barrera, Wendy] Univ Calif Los Angeles, Dept Earth & Space Sci, Los Angeles, CA 90095 USA. [Gosse, John C.] Dalhousie Univ, Dalhousie Geochronol Ctr, Halifax, NS B3H 4J1, Canada. [Zimmermann, Susan] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. RP Antinao, JL (reprint author), Desert Res Inst, Div Earth & Ecosyst Sci, 2215 Raggio Pkwy, Reno, NV 89512 USA. EM jantinao@dri.edu OI Brown, Nathan/0000-0002-7385-8679; Antinao, Jose Luis/0000-0003-2826-8917 FU U.S. National Science Foundation NSF EAR [1123481]; US Army Research Office [DAAD19-03-1-0159]; Division of Earth and Ecosystem Sciences (DEES) of the Desert Research Institute (DRI); National Research Center for Integrated Natural Disaster Management (Chile) [FONDAP CONICYT 15110017] FX We thank two anonymous reviewers for their helpful comments on an earlier version of our manuscript. U.S. National Science Foundation NSF EAR 1123481 grant to J.L.A., E.M., and E.R. and US Army Research Office Contract No. DAAD19-03-1-0159 to E.M. supported this research. J.L.A. was also funded by postdoctoral support funds from the Division of Earth and Ecosystem Sciences (DEES) of the Desert Research Institute (DRI) and by the National Research Center for Integrated Natural Disaster Management (grant FONDAP CONICYT 15110017, Chile). L. Farfan and S. Mayer (CICESE, Unidad La Paz) provided partial logistical support for field activities. Discussions with G. Martinez (UABCS), K.-b. Liu (LSU), A. Hidy (LLNL), and thorough reviews by two anonymous reviewers improved the manuscript. S. Baker (DRI) helped with figure design. G. Yang (Dalhousie) and E. Huenupi (DRI) performed all analytical work for cosmogenic isotope extraction. This manuscript is contribution LLNL-JRNL-676762. NR 105 TC 0 Z9 0 U1 12 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-3791 J9 QUATERNARY SCI REV JI Quat. Sci. Rev. PD AUG 15 PY 2016 VL 146 BP 161 EP 181 DI 10.1016/j.quascirev.2016.06.008 PG 21 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA DT1ID UT WOS:000381234000010 ER PT J AU Dalcin, L Collier, N Vignal, P Cortes, AMA Calo, VM AF Dalcin, L. Collier, N. Vignal, P. Cortes, A. M. A. Calo, V. M. TI PetIGA: A framework for high-performance isogeometric analysis SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING LA English DT Article DE Isogeometric analysis; High-performance computing; Finite element method; Open-source software ID NAVIER-STOKES EQUATIONS; FINITE-ELEMENT-METHOD; HYPERELASTIC MATERIALS; DIRECT SOLVERS; CONTINUITY; LIBRARY; NURBS; COST; PRECONDITIONERS; REFINEMENT AB We present PetIGA, a code framework to approximate the solution of partial differential equations using isogeometric analysis. PetIGA can be used to assemble matrices and vectors which come from a Galerkin weak form, discretized with Non-Uniform Rational B-spline basis functions. We base our framework on PETSc, a high-performance library for the scalable solution of partial differential equations, which simplifies the development of large-scale scientific codes, provides a rich environment for prototyping, and separates parallelism from algorithm choice. We describe the implementation of PetIGA, and exemplify its use by solving a model nonlinear problem. To illustrate the robustness and flexibility of PetIGA, we solve some challenging nonlinear partial differential equations that include problems in both solid and fluid mechanics. We show strong scaling results on up to 4096 cores, which confirm the suitability of PetIGA for large scale simulations. (C) 2016 Elsevier B.V. All rights reserved. C1 [Dalcin, L.] King Abdullah Univ Sci & Technol, Extreme Comp Res Ctr, Thuwal, Saudi Arabia. [Dalcin, L.; Cortes, A. M. A.; Calo, V. M.] King Abdullah Univ Sci & Technol, Ctr Numer Porous Media NumPor Comp Elect & Math S, Thuwal, Saudi Arabia. [Dalcin, L.] Ctr Invest Metodos Computac CIMEC, Santa Fe, Argentina. [Dalcin, L.] Consejo Nacl Invest Cient & Tecn, Santa Fe, Argentina. [Collier, N.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN USA. [Vignal, P.] King Abdullah Univ Sci & Technol, Ctr Numer Porous Media NumPor Mat Sci & Engn, Thuwal, Saudi Arabia. RP Dalcin, L (reprint author), 4700 King Abdullah Univ Sci & Technol Al Khawariz, Thuwal 239556900, Saudi Arabia. EM dalcinl@gmail.com; nathaniel.collier@gmail.com; philippe.vignal@kaust.edu.sa; adrimacortes@gmail.com; vmcalo@gmail.com OI Dalcin, Lisandro/0000-0001-8086-0155; Calo, Victor Manuel/0000-0002-1805-4045 FU European Union's Horizon 2020 research and innovation programme of the Marie Sklodowska-Curie grant [644602]; Center for Numerical Porous Media at King Abdullah University of Science and Technology; Agencia Nacional de Promocion Cientifica y Tecnologica [PICT 0938-13, PICT 2660-14, PICT-E 0191-14] FX This work is part of the European Union's Horizon 2020 research and innovation programme of the Marie Sklodowska-Curie grant agreement No. 644602. This work was also supported by the Center for Numerical Porous Media at King Abdullah University of Science and Technology and Agencia Nacional de Promocion Cientifica y Tecnologica grants PICT 0938-13, PICT 2660-14 and PICT-E 0191-14. NR 72 TC 4 Z9 4 U1 4 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0045-7825 EI 1879-2138 J9 COMPUT METHOD APPL M JI Comput. Meth. Appl. Mech. Eng. PD AUG 15 PY 2016 VL 308 BP 151 EP 181 DI 10.1016/j.cma.2016.05.011 PG 31 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA DS2AA UT WOS:000380512800008 ER PT J AU Knezevic, M Zecevic, M Beyerlein, IJ Lebensohn, RA AF Knezevic, Marko Zecevic, Miroslav Beyerlein, Irene J. Lebensohn, Ricardo A. TI A numerical procedure enabling accurate descriptions of strain rate-sensitive flow of polycrystals within crystal visco-plasticity theory SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING LA English DT Article DE Dislocations; Microstructure; Crystal plasticity; Rate-dependent material; Numerical methods ID IMPLICIT FINITE-ELEMENTS; TANTALUM-TUNGSTEN ALLOYS; TEXTURE EVOLUTION; CRYSTALLOGRAPHIC TEXTURE; MECHANICAL THRESHOLD; DEFORMATION-BEHAVIOR; DISLOCATION DENSITY; HCP/BCC COMPOSITES; ALPHA-TITANIUM; PATH CHANGES AB The plastic deformation of polycrystalline metals is carried by the motion of dislocations on specific crystallographic glide planes. According to the thermodynamics theory of slip, in the regime of strain rates, roughly from 10(-5)/s to 10(5)/s, dislocation motion is thermally activated. Dislocations must overcome barriers in order to move, and this concept defines critical activation stresses tau(s)(c) on a slip system s that evolve as a function of strain rate and temperature. The fundamental flow rule in crystal visco-plasticity theory that involves tau(s)(c) in order to activate slip has a power-law form: (gamma) over dot(s) = (gamma) over dot(0) (vertical bar tau(s)vertical bar/tau(s)(c))(n) sign (tau(s)). This form is desirable because it provides uniqueness of solution for the active slip systems that accommodate an imposed strain rate; however, it also introduces a strain rate dependence, which in order to represent the actual behavior of polycrystalline materials deforming in relevant conditions of temperature and strain-rate usually needs to be described by a high value of the exponent n. However, since until now the highest value of n was limited by numerical tractability, the use of the power-law flow rule frequently introduced an artificially high rate-sensitivity. All prior efforts to correct this extraneous rate sensitivity have only lessened its effect and unfortunately also at the expense of substantial increases in computation time. To this day, a solution for the power-law exponent reflecting true material behavior is still sought. This article provides a novel method enabling the use of realistic material strain rate-sensitivity exponents to be used within the crystal visco-plasticity theory without increasing computation time involved in polycrystal simulations. Calculations are performed for polycrystalline pure Cu and excellent agreement with experimental measurement is demonstrated. (C) 2016 Elsevier B.V. All rights reserved. C1 [Knezevic, Marko; Zecevic, Miroslav] Univ New Hampshire, Dept Mech Engn, 33 Acad Way,Kingsbury Hall,W119, Durham, NH 03824 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Lebensohn, Ricardo A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, 33 Acad Way,Kingsbury Hall,W119, Durham, NH 03824 USA. EM marko.knezevic@unh.edu RI Lebensohn, Ricardo/A-2494-2008 OI Lebensohn, Ricardo/0000-0002-3152-9105 FU National Science Foundation [CMMI-1541918]; Los Alamos National Laboratory Directed Research and Development (LDRD) project [ER20140348] FX This work is based upon project supported by the National Science Foundation under Grant No. CMMI-1541918. The authors gratefully acknowledge this support. IJB would like to acknowledge support through a Los Alamos National Laboratory Directed Research and Development (LDRD) project ER20140348. NR 72 TC 1 Z9 1 U1 4 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0045-7825 EI 1879-2138 J9 COMPUT METHOD APPL M JI Comput. Meth. Appl. Mech. Eng. PD AUG 15 PY 2016 VL 308 BP 468 EP 482 DI 10.1016/j.cma.2016.05.025 PG 15 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA DS2AA UT WOS:000380512800020 ER PT J AU Mosby, MA Engle, JW Jackman, KR Nortier, FM Birnbaum, ER AF Mosby, M. A. Engle, J. W. Jackman, K. R. Nortier, F. M. Birnbaum, E. R. TI Determination of spallation neutron flux through spectral adjustment techniques SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Spallation neutrons; Isotope production; Proton irradiation; Spectral unfolding ID CROSS-SECTIONS AB The Los Alamos Isotope Production Facility (IPF) creates medical isotopes using a proton beam impinged on a target stack. Spallation neutrons are created in the interaction of the beam with target. The use of these spallation neutrons to produce additional radionuclides has been proposed. However, the energy distribution and magnitude of the flux is not well understood. A modified SAND-II spectral adjustment routine has been used with radioactivation foils to determine the differential neutron fluence for these spallation neutrons during a standard IPF production run. (C) 2016 Elsevier B.V. All rights reserved. C1 [Mosby, M. A.; Engle, J. W.; Jackman, K. R.; Nortier, F. M.; Birnbaum, E. R.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Mosby, MA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM mosbym@lanl.gov OI Nortier, Francois/0000-0002-7549-8101 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA253996]; U.S. DOE Office of Science via from the Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics FX This study was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA253996 with partial funding by the U.S. DOE Office of Science via funding from the Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics. NR 12 TC 1 Z9 1 U1 0 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD AUG 15 PY 2016 VL 381 BP 29 EP 33 DI 10.1016/j.nimb.2016.04.041 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DR7MB UT WOS:000380082700005 ER PT J AU Zong, HX Ding, XD Lookman, T Sun, J AF Zong, Hongxiang Ding, Xiangdong Lookman, Turab Sun, Jun TI Twin boundary activated alpha -> omega phase transformation in titanium under shock compression SO ACTA MATERIALIA LA English DT Article DE Deformation twinning; Martensitic transformation; Shock compression; Titanium ID GRAIN-BOUNDARY; MOLECULAR-DYNAMICS; DISLOCATIONS; DEFORMATION; MIGRATION; STRESS; MOTION; SHEAR; REORIENTATION; MECHANISMS AB The role of grain boundary structures on the shock response of hexagonal-close-packed (hcp) metals is little understood. We use molecular dynamics simulations to investigate deformation mechanisms in shock compressed Ti bicrystals with three types of grain boundary (GB) microstructure. Our results show the shock response of phase Ti polycrystals are influenced by the GB characteristics, i.e., elastic shock wave induced inelastic deformation occurs on both sides of the {10 (1) over bar2} coherent twin boundaries (CTBs) but only on one-side of the symmetric incoherent twin boundaries (ITB) or {1 (2) over bar 10} tilt grain boundaries regions. In particular, we find that the elastic shock wave can readily trigger the alpha -> omega to transformation at {10 (1) over bar2} CTBs but not the other two GBs, and the alpha -> omega transformation at CTBs leads to considerable wave attenuation (i.e., the elastic precursor decay). Combined with first principle calculations, we find that CTBs can facilitate the overcoming of the energy barrier for the alpha -> omega transformation. Our findings have the potential to influence interface engineering and materials design under extreme conditions. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Zong, Hongxiang; Ding, Xiangdong; Sun, Jun] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. [Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zong, HX; Ding, XD (reprint author), Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. EM zonghust@mail.xjtu.edu.cn; Dingxd@mail.xjtu.edu.cn FU US DOE at LANL [DE-AC52-06NA25396]; National Natural Science Foundation of China [51320105014, 51321003, 51501141]; China Postdoctoral Science Foundation [2015M580843]; 973 Program of China [2012CB619402] FX This work was supported by the US DOE at LANL (DE-AC52-06NA25396) as well as by the National Natural Science Foundation of China (51320105014, 51321003 and 51501141), the China Postdoctoral Science Foundation (2015M580843), and the 973 Program of China (2012CB619402). NR 42 TC 0 Z9 0 U1 22 U2 63 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 1 EP 9 DI 10.1016/j.actamat.2016.05.037 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400001 ER PT J AU Yu, C Aoun, B Cui, LS Liu, YN Yang, H Jiang, XH Cai, S Jiang, DQ Liu, ZP Brown, DE Ren, Y AF Yu, Cun Aoun, Bachir Cui, Lishan Liu, Yinong Yang, Hong Jiang, Xiaohua Cai, Song Jiang, Daqiang Liu, Zunping Brown, Dennis E. Ren, Yang TI Synchrotron high energy X-ray diffraction study of microstructure evolution of severely cold drawn NiTi wire during annealing SO ACTA MATERIALIA LA English DT Article DE Shape memory alloy; Structural relaxation; Crystallization; In-situ synchrotron high energy X ray diffraction ID SHAPE-MEMORY ALLOYS; SEVERE PLASTIC-DEFORMATION; TRANSMISSION ELECTRON-MICROSCOPY; MARTENSITIC-TRANSFORMATION; PHASE-TRANSFORMATIONS; FREE-VOLUME; TEXTURE; LIQUIDS AB Microstructure evolution of a cold-drawn NiTi shape memory alloy wire was investigated by means of in situ synchrotron high-energy X-ray diffraction during continuous heating. The cold-drawn wire contained amorphous regions and nano-crystalline domains in its microstructure. Pair distribution function analysis revealed that the amorphous regions underwent structural relaxation via atomic rearrangement when heated above 100 degrees C. The nano-crystalline domains were found to exhibit a strong cold work induced lattice strain anisotropy along 111 , which coincides with the crystallographic fiber orientation of the domains along the wire axial direction. The lattice strain anisotropy systematically decreased upon heating above 200 degrees C, implying a structural recovery. Crystallization of the amorphous phase led to a broadening of the angular distribution of 111 preferential orientations of grains along the axial direction as relative to the original 111 axial fiber texture of the nanocrystalline domains produced by the severe cold wire drawing deformation. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Yu, Cun; Cui, Lishan; Jiang, Xiaohua; Jiang, Daqiang] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Yu, Cun; Cui, Lishan; Jiang, Xiaohua; Jiang, Daqiang] China Univ Petr, Dept Mat Sci & Engn, Beijing 102249, Peoples R China. [Aoun, Bachir; Liu, Zunping; Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Liu, Yinong; Yang, Hong; Jiang, Daqiang] Univ Western Australia, Sch Mech & Chem Engn, Crawley, WA 6009, Australia. [Yu, Cun] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Cai, Song] Ft Wayne Met Res Prod Corp, 9609 Ardmore Ave, Ft Wayne, IN 46809 USA. [Brown, Dennis E.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Cui, LS (reprint author), China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China.; Cui, LS (reprint author), China Univ Petr, Dept Mat Sci & Engn, Beijing 102249, Peoples R China.; Liu, YN (reprint author), Univ Western Australia, Sch Mech & Chem Engn, Crawley, WA 6009, Australia. EM lscui@cup.edu.cn RI Jiang, Daqiang /G-5511-2014; OI , Cun/0000-0002-2822-2583; Yu, Cun/0000-0003-0084-6746 FU National Natural Science Foundation of China [51231008, 11474362, 51401240]; National 973 program of China [2012CB619403]; Australian Research Council [DP140103805]; Institute for NanoScience, Engineering, and Technology (INSET) of Northern Illinois University; U.S. Department of Energy [DE-AC02-06CH11357] FX The authors wish to thank Prof. R. Wenk, Prof. L. Lutterotti and Dr. W Kanitpanyacharoen for their help with texture analysis. This work was supported by the National Natural Science Foundation of China (51231008, 11474362 and 51401240), the National 973 program of China (2012CB619403), the Australian Research Council (Grant No. DP140103805), and the Institute for NanoScience, Engineering, and Technology (INSET) of Northern Illinois University. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy under contract No. DE-AC02-06CH11357. NR 33 TC 1 Z9 1 U1 12 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 35 EP 44 DI 10.1016/j.actamat.2016.05.039 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400004 ER PT J AU Lange, AP Tan, XL Palley, CS Mahajan, S AF Lange, A. P. Tan, X. L. Palley, C. S. Mahajan, S. TI Structure and chemistry of aluminum predose layers in AlN epitaxy on (111) silicon SO ACTA MATERIALIA LA English DT Article DE AlN on (111) silicon; GaN on (111) silicon; Aluminum predose; AlN XPS; Meltback etching ID MOLECULAR-BEAM EPITAXY; HIGH-QUALITY GAN; SI SUBSTRATE; INTERMEDIATE LAYER; SI(111); GROWTH; DIFFUSION; SURFACES; AMMONIA AB In this study, (111) silicon substrates were exposed to varied trimethylaluminum predoses and ammonia using metalorganic chemical vapor deposition and the resulting deposits were examined using AFM, SEM, TEM, STEM, EDXS, and XPS. Growth patches were observed with facets in the both the vertical and lateral directions. The width of these patches increased with increasing total volume of deposited aluminum. Their structure was found to be diamond cubic silicon with dilute concentrations of aluminum. Small, rounded AlN islands were observed on the surface of these patches which had electron diffraction patterns consistent with both strained wurtzite and zinc blende structures. A model is proposed in which silicon diffuses into liquid aluminum prior to ammonia exposure and the resulting liquid Al-Si alloy is converted into AlN and silicon upon nitridation. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Lange, A. P.; Mahajan, S.] Univ Calif Davis, Dept Mat Sci & Engn, Davis, CA 95616 USA. [Tan, X. L.; Palley, C. S.] Univ Calif Davis, Dept Phys, Davis, CA USA. [Tan, X. L.; Palley, C. S.] Lawrence Berkeley Natl Lab, Div Mat Sci, Lawrence, KS USA. RP Lange, AP (reprint author), Univ Calif Davis, Dept Mat Sci & Engn, Davis, CA 95616 USA. EM aplange@ucdavis.edu FU University of California, Davis College of Engineering FX Financial support for this work was provided by the University of California, Davis College of Engineering. NR 25 TC 0 Z9 0 U1 16 U2 35 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 94 EP 103 DI 10.1016/j.actamat.2016.05.036 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400010 ER PT J AU Taylor, CA Patel, MK Aguiar, JA Zhang, YW Crespillo, ML Wen, J Xue, HZ Wang, YG Weber, WJ AF Taylor, Caitlin A. Patel, Maulik K. Aguiar, Jeffery A. Zhang, Yanwen Crespillo, Miguel L. Wen, Juan Xue, Haizhou Wang, Yonggiang Weber, William J. TI Bubble formation and lattice parameter changes resulting from He irradiation of defect-fluorite Gd2Zr2O7 SO ACTA MATERIALIA LA English DT Article DE Pyrochlore; Helium bubble; Radiation damage; Nuclear waste; Lattice swelling ID LEVEL NUCLEAR-WASTE; DAMAGE EVOLUTION; IMMOBILIZATION; PLUTONIUM; CERAMICS; BEHAVIOR; FORM AB Pyrochlores have long been considered as potential candidates for advanced ceramic waste-forms for the immobilization of radioactive waste nuclides. This work provides evidence that Gd2Zr2O7, often considered the most radiation tolerant pyrochlore, could be susceptible to radiation damage in the form of bubble nucleation at the highest He doses expected over geological time. Ion irradiations were utilized to experimentally simulate the radiation damage and He accumulation produced by alpha-decay. Samples were pre-damaged using 7 MeV Au3+ to induce the pyrochlore to defect-fluorite phase transformation, which would occur due to alpha-recoil damage within several hundred years of storage in a Gd2Zr2O7 waste form. These samples were then implanted to various He concentrations in order to study the long-term effects of He accumulation. Helium bubbles 1-3 nm in diameter were observed in TEM at a concentration of 4.6 at.% He. Some bubbles remained isolated, while others formed chains 10-30 nm in length parallel to the surface. GIXRD measurements showed lattice swelling after irradiating pristine Gd2Zr2O7 with 7 MeV Au3+ to a fluence of 2.2 x 10(15) Au/cm(2). An increase in lattice swelling was also measured after 2.2 x 10(15) Au/cm(2) + 2 x 10(15) He/cm(2) and 2.2 x 10(15) Au/cm(2) + 2 x 10(16) He/cm(2). A decrease in lattice swelling was measured after irradiation with 2.2 x 1015 Au/cm2 + 2 x 1017 He/cm2, the fluence where bubbles and bubble chains were observed in TEM. Bubble chains are thought to form in order to reduce lattice strain normal to the surface, which is produced by the Au and He irradiation damage. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Taylor, Caitlin A.; Patel, Maulik K.; Zhang, Yanwen; Crespillo, Miguel L.; Xue, Haizhou; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Aguiar, Jeffery A.] Idaho Natl Lab, Fuel Performance & Design Dept, Idaho Falls, ID 83415 USA. [Aguiar, Jeffery A.] Natl Renewable Energy Lab, Ctr Mat Sci, Golden, CO 80220 USA. [Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Wen, Juan] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Gansu, Peoples R China. [Wen, Juan; Wang, Yonggiang] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Taylor, CA (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM ctayl105@vols.utk.edu RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy (DOE) Office of Science by Los Alamos National Laboratory [DE-AC52-06NA25396]; National Renewable Energy Laboratory; U.S. Department of Energy; DOE-Nuclear Energy University Program [DE-NE0000693]; Nuclear Engineering University Program (NEUP) [12-3528]; Sandia National Laboratories [DE-AC04-94AL85000] FX First, the authors would like to thank Kurt Sickafus for helpful discussions and use of his laboratory facilities. Helium implantations were performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). This research was also in part supported by the National Renewable Energy Laboratory, where part of the transmission electron microscopy work was performed, which is sponsored by U.S. Department of Energy. Some initial electron microscopy was conducted as part of a user proposal at Oak Ridge National Laboratory's Center for Nano phase Materials Sciences, which is a Department of Energy Office of Science User Facility. X-ray diffraction experiments were performed using the instruments that were procured through the general infrastructure grant of DOE-Nuclear Energy University Program (DE-NE0000693). This work was supported by the Nuclear Engineering University Program (NEUP) Award Number 12-3528. NR 28 TC 0 Z9 0 U1 8 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 115 EP 122 DI 10.1016/j.actamat.2016.05.045 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400012 ER PT J AU Owen, LR Playford, HY Stone, HJ Tucker, MG AF Owen, L. R. Playford, H. Y. Stone, H. J. Tucker, M. G. TI A new approach to the analysis of short-range order in alloys using total scattering SO ACTA MATERIALIA LA English DT Article DE Atomic ordering; Diffraction; Pair correlation function; Short-range order; Short-range ordering ID BINARY-ALLOYS; SYSTEMS AB In spite of its influence on a number of physical properties, short-range order in crystalline alloys has received little recent attention, largely due to the complexity of the experimental methods involved. In this work, a novel approach that could be used for the analysis of ordering transitions and short-range order in crystalline alloys using total scattering and reverse Monte Carlo (RMC) refinements is presented. Calculated pair distribution functions representative of different types of short-range order are used to illustrate the level of information contained within these experimentally accessible functions and the insight into ordering which may be obtained using this new method. Key considerations in the acquisition of data of sufficient quality for successful analysis are also discussed. It is shown that the atomistic models obtained from RMC refinements may be analysed to identify directly the Clapp configurations that are present. It is further shown how these configurations can be enhanced compared with a random structure, and how their degradation pathways and the distribution of Warren-Cowley parameters, can then be used to obtain a detailed, quantitative structural description of the short-range order occurring in crystalline alloys. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Owen, L. R.; Stone, H. J.] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Owen, L. R.; Playford, H. Y.; Tucker, M. G.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Tucker, M. G.] Diamond Light Source Ltd, Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England. [Tucker, M. G.] Spallat Neutron Source, One Bethel Valley Rd, Oak Ridge, TN USA. RP Playford, HY (reprint author), STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. EM helen.playford@stfc.ac.uk OI Owen, Lewis/0000-0003-2311-3908 FU STFC ISIS Facility; Rolls-Royce plc/EPSRC Strategic Partnership [EP/H022309/1, EP/M005607/1] FX This work was supported by the STFC ISIS Facility and the Rolls-Royce plc/EPSRC Strategic Partnership under EP/H022309/1 and EP/M005607/1. The authors gratefully acknowledge STFC for the provision of beamtime at Diamond Light Source Ltd (EE10354, EE11665) and the ISIS Facility (RB1510579, RB1520332), and thank Dr Stephen Hull for useful discussions. NR 33 TC 2 Z9 2 U1 9 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 155 EP 166 DI 10.1016/j.actamat.2016.05.031 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400016 ER PT J AU Moore, AP Deo, C Baskes, MI Okuniewski, MA AF Moore, A. P. Deo, C. Baskes, M. I. Okuniewski, M. A. TI Atomistic mechanisms of morphological evolution and segregation in U-Zr alloys SO ACTA MATERIALIA LA English DT Article DE Microstructure evolution; Metal alloys; Uranium; Zirconium; Atomistic simulations ID URANIUM-ZIRCONIUM SYSTEM; MOLECULAR-DYNAMICS; DELTA-PHASE; STABILITY; TEMPERATURES; SIMULATIONS AB In many metallic alloys, complex microstructures form as a consequence of local atomic ordering that depends on the processing path. This research uses an atomistic approach to study microstructural morphology and evolution in order to investigate how temperature and alloy concentration affect ordering. A semi-empirical Modified Embedded Atom Method (MEAM) is used in conjunction with molecular dynamics (MD) and Monte Carlo (MC) simulations to investigate the properties and equilibrium configurations of the high temperature body-centered-cubic (bcc) uranium-zirconium (U-Zr) alloys. Atomic simulations conducted with the MEAM potential show the thermodynamic driving force to the lamellar structure for the melt-casted U-rich alloys and the finely acicular microstructure of the water quenched U-rich alloys. In addition, when the U-rich U-Zr alloy is equilibrated at a lower temperature, the lamellar/acicular microstructures begin to spheroidize, as observed in experiments. In the intermediate Zr concentration region, the ordering seen is able to facilitate the structure to the partially ordered delta-UZr2 phase seen experimentally. Lastly, the Zr-rich region is able to successfully show the thermodynamic driving force to the acicular, Widmanstatten, and martensitic needles type microstructures observed experimentally. These simulations are able to successfully replicate some of the fundamental thermo-physical and microstructural characteristics following fabrication and irradiation of the U-Zr metallic fuels. Published by Elsevier Ltd on behalf of Acta Materialia Inc. C1 [Moore, A. P.; Deo, C.] Georgia Inst Technol, 770 State St, Atlanta, GA 30332 USA. [Baskes, M. I.] Mississippi State Univ, 105 Lee Blvd, Mississippi State, MS 39762 USA. [Baskes, M. I.] Univ Calif San Diego, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Baskes, M. I.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Okuniewski, M. A.] Purdue Univ, 610 Purdue Mall, W Lafayette, IN 47907 USA. [Okuniewski, M. A.] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. RP Moore, AP (reprint author), Georgia Inst Technol, 770 State St, Atlanta, GA 30332 USA. EM safeacount@gmail.com FU Idaho National Laboratory (INL) [00123590]; National Science Foundation - Domestic Nuclear Detection Office (NSF-DNDO) Academic Research grant [2014-DN-077-ARI072-02]; Department of Energy Nuclear Energy University Program (DOE-NEUP) FX Authors acknowledge support from an Idaho National Laboratory (INL) subcontract (00123590), a National Science Foundation - Domestic Nuclear Detection Office (NSF-DNDO) Academic Research grant (2014-DN-077-ARI072-02), and from the Department of Energy Nuclear Energy University Program (DOE-NEUP). NR 52 TC 1 Z9 1 U1 9 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 178 EP 188 DI 10.1016/j.actamat.2016.05.052 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400018 ER PT J AU Ardeljan, M Savage, DJ Kumar, A Beyerlein, IJ Knezevic, M AF Ardeljan, Milan Savage, Daniel J. Kumar, Anil Beyerlein, Irene J. Knezevic, Marko TI The plasticity of highly oriented nano-layered Zr/Nb composites SO ACTA MATERIALIA LA English DT Article DE Zirconium; Niobium; Crystal plasticity; Accumulative roll bonding; Interfaces ID CRYSTALLOGRAPHIC TEXTURE EVOLUTION; POLYCRYSTALLINE HCP/BCC COMPOSITES; FINITE-ELEMENT MODELS; AUGMENTED-WAVE METHOD; STRAIN-PATH CHANGES; X-RAY-DIFFRACTION; ALPHA-URANIUM; DEFORMATION-BEHAVIOR; DISLOCATION DENSITY; MECHANICAL RESPONSE AB In prior work, bulk lamellar composites of pure zirconium and niobium (Zr/Nb) were manufactured by accumulative roll bonding (ARB). After the substantial amounts of straining required to refine the layers to nanoscale dimensions, formation of highly oriented Zr crystals was observed. In this work, we employ a spatially resolved multiscale crystal plasticity based model in 3D to study the orientational stability of Zr single crystals and Zr/Nb bicrystals during rolling deformation. The analysis reveals that predominant texture components arise due to substantially reduced ratios of slip resistances among the prismatic, pyramidal I , and basal slip systems. In support, density functional theory (DFT) calculations of generalized stacking fault energy curves on these three slip systems suggest that the ratio of critical stresses to form these dislocations are within 2.5 times. This finding of reduced anisotropy in Zr at the nanoscale can provide insight into the design of nano-structuring processes for target textures, such as those containing highly oriented grains. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Ardeljan, Milan; Savage, Daniel J.; Knezevic, Marko] Univ New Hampshire, Dept Mech Engn, 33 Acad Way, Durham, NH 03824 USA. [Kumar, Anil; Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ardeljan, M; Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, 33 Acad Way, Durham, NH 03824 USA. EM milan.ardeljan@gmail.com; marko.knezevic@unh.edu FU National Science Foundation [CMMI-1541918]; Los Alamos National Laboratory Directed Research and Development (LDRD) project [ER20140348] FX This work is based upon project supported by the National Science Foundation under grant. No. CMMI-1541918. The authors gratefully acknowledge this support. IJB and AK would like to acknowledge support through a Los Alamos National Laboratory Directed Research and Development (LDRD) project ER20140348. NR 82 TC 3 Z9 3 U1 14 U2 29 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 189 EP 203 DI 10.1016/j.actamat.2016.05.058 PG 15 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400019 ER PT J AU Osetsky, YN Beland, LK Stoller, RE AF Osetsky, Yuri N. Beland, Laurent K. Stoller, Roger E. TI Specific features of defect and mass transport in concentrated fcc alloys SO ACTA MATERIALIA LA English DT Article DE Diffusion; Concentrated alloys; Tracer diffusion coefficient; Ni-Fe alloys ID FE-CR ALLOYS; PHENOMENOLOGICAL COEFFICIENTS; COMPUTER-SIMULATION; ATOM DIFFUSION; ALPHA-FE; IRRADIATION; DILUTE AB Diffusion and mass transport are basic properties that control materials performance, such as phase stability, solute decomposition and radiation tolerance. While understanding diffusion in dilute alloys is a mature field, concentrated alloys are much less studied. Here, atomic-scale diffusion and mass transport via vacancies and interstitial atoms are compared in fcc Ni, Fe and equiatomic Ni-Fe alloy. High temperature properties were determined using conventional molecular dynamics on the microsecond timescale, whereas the kinetic activation-relaxation (k-ART) approach was applied at low temperatures. The k-ART was also used to calculate transition states in the alloy and defect transport coefficients. The calculations reveal several specific features. For example, vacancy and interstitial defects migrate via different alloy components, diffusion is more sluggish in the alloy and, notably, mass transport in the concentrated alloy cannot be predicted on the basis of diffusion in its pure metal counterparts. The percolation threshold for the defect diffusion in the alloy is discussed and it is suggested that this phenomenon depends on the properties and diffusion mechanisms of specific defects. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Osetsky, Yuri N.; Beland, Laurent K.; Stoller, Roger E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Osetsky, YN (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM osetskiyyn@ornl.gov OI Osetskiy, Yury/0000-0002-8109-0030 FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Fonds Quebecois de recherche Nature et Technologies FX This work was supported as part of the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. LKB acknowledges additional support from a fellowship awarded by the Fonds Quebecois de recherche Nature et Technologies. The authors thank Dr. A. Barashev for numerous discussions. NR 33 TC 1 Z9 1 U1 8 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 364 EP 371 DI 10.1016/j.actamat.2016.06.018 PG 8 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400037 ER PT J AU Gwalani, B Alam, T Miller, C Rojhirunsakool, T Kim, YS Kim, SS Kaufman, MJ Ren, Y Banerjee, R AF Gwalani, B. Alam, T. Miller, C. Rojhirunsakool, T. Kim, Y. S. Kim, S. S. Kaufman, M. J. Ren, Yang Banerjee, R. TI Experimental investigation of the ordering pathway in a Ni-33 at.%Cr alloy SO ACTA MATERIALIA LA English DT Article DE Ni-based superalloy; Atomic ordering; Synchrotron XRD; Orientation specific APT ID PHASE PRECIPITATION; NI2CR; TRANSFORMATIONS; SUSCEPTIBILITY; SYSTEM AB The present study involves a detailed experimental investigation of the concurrent compositional clustering and long-range ordering tendencies in a Ni-33 at.%Cr alloy, carried out by coupling synchrotron-based X-ray diffraction (XRD), transmission electron microscopy (TEM), and atom probe tomography (APT). Synchrotron-based XRD results clearly exhibited progressively increasing lattice contraction in the matrix with increasing isothermal aging time, at 475 degrees C, eventually leading to the development of long-range ordering (LRO) of the Pt2Mo-type. Detailed TEM and APT investigations revealed that this LRO in the matrix is manifested in the form of nanometer-scale ordered domains, and the spatial distribution, size, morphology and compositional evolution of these domains have been carefully investigated. APT results also revealed the early stages of compositional clustering prior to the onset of long-range ordering in this alloy and such compositional clustering can potentially be correlated to the lattice contraction and previously proposed short-range ordering tendencies. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Gwalani, B.; Alam, T.; Rojhirunsakool, T.; Banerjee, R.] Univ North Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. [Miller, C.; Kaufman, M. J.] Colorado Sch Mines, Dept Met & Mat & Engn, Golden, CO 80401 USA. [Kim, Y. S.; Kim, S. S.] Korean Atom Energy Res Inst, Daejeon, South Korea. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Banerjee, R (reprint author), Univ North Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. EM rajarshi.banerjee@unt.edu FU U.S. Department of Energy (DOE) under the International Nuclear Energy Research Initiative (INERI) [2011-01-K]; Korean Atomic Energy Research Institute (KAERI) FX This work has been supported by the U.S. Department of Energy (DOE) under the International Nuclear Energy Research Initiative (INERI) (2011-01-K), in partnership with the Korean Atomic Energy Research Institute (KAERI). The authors would also like to acknowledge the DOE's Advanced Proton Source at the Argonne National Lab for providing access and user time on the beam line for x-ray diffraction experiments. The authors would also like to acknowledge the Center for Advanced Research and Technology at the University of North Texas. NR 32 TC 0 Z9 0 U1 8 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD AUG 15 PY 2016 VL 115 BP 372 EP 384 DI 10.1016/j.actamat.2016.06.014 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DR7MI UT WOS:000380083400038 ER PT J AU Hodgkins, SB Tfaily, MM Podgorski, DC McCalley, CK Saleska, SR Crill, PM Rich, VI Chanton, JP Cooper, WT AF Hodgkins, Suzanne B. Tfaily, Malak M. Podgorski, David C. McCalley, Carmody K. Saleska, Scott R. Crill, Patrick M. Rich, Virginia I. Chanton, Jeffrey P. Cooper, William T. TI Elemental composition and optical properties reveal changes in dissolved organic matter along a permafrost thaw chronosequence in a subarctic peatland SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Dissolved organic matter; FT-ICR MS; UV/Vis; EEMS; Peatlands; Permafrost ID RESOLUTION MASS-SPECTROMETRY; PHENOL OXIDASE ACTIVITY; SOLID-PHASE EXTRACTION; FLUORESCENCE SPECTROSCOPY; CLIMATE-CHANGE; CARBON-CYCLE; CHEMICAL-COMPOSITION; NORTHERN PEATLANDS; ACCUMULATION RATES; METHANE PRODUCTION AB The fate of carbon stored in permafrost-zone peatlands represents a significant uncertainty in global climate modeling. Given that the breakdown of dissolved organic matter (DOM) is often a major pathway for decomposition in peatlands, knowledge of DOM reactivity under different permafrost regimes is critical for determining future climate feedbacks. To explore the effects of permafrost thaw and resultant plant succession on DOM reactivity, we used a combination of Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR MS), UV/Vis absorbance, and excitation-emission matrix spectroscopy (EEMS) to examine the DOM elemental composition and optical properties of 27 pore water samples gathered from various sites along a permafrost thaw sequence in Stordalen Mire, a thawing subarctic peatland in northern Sweden. The presence of dense Sphagnum moss, a feature that is dominant in the intermediate thaw stages, appeared to be the main driver of variation in DOM elemental composition and optical properties at Stordalen. Specifically, DOM from sites with Sphagnum had greater aromaticity, higher average molecular weights, and greater O/C, consistent with a higher abundance of phenolic compounds that likely inhibit decomposition. These compounds are released by Sphagnum and may accumulate due to inhibition of phenol oxidase activity by the acidic pH at these sites. In contrast, sites without Sphagnum, specifically fully-thawed rich fens, had more saturated, more reduced compounds, which were high in N and S. Optical properties at rich fens indicated the presence of microbially-derived DOM, consistent with the higher decomposition rates previously measured at these sites. These results indicate that Sphagnum acts as an inhibitor of rapid decomposition and CH4 release in thawing subarctic peatlands, consistent with lower rates of CO2 and CH4 production previously observed at these sites. However, this inhibitory effect may disappear if Sphagnum-dominated bogs transition to more waterlogged rich fens that contain very little to no living Sphagnum. Release of this inhibition allows for higher levels of microbial activity and potentially greater CH4 release, as has been observed in these fen sites. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Hodgkins, Suzanne B.; Chanton, Jeffrey P.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Tfaily, Malak M.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Tfaily, Malak M.] Pacific Northwest Natl Lab, Div Biol Sci, Richland, WA 99354 USA. [Podgorski, David C.] Florida State Univ, Future Fuels Inst, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [McCalley, Carmody K.] Rochester Inst Technol, Thomas H Gosnell Sch Life Sci, Rochester, NY 14623 USA. [Saleska, Scott R.] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ 85716 USA. [Crill, Patrick M.] Stockholm Univ, Dept Geol Sci, S-10691 Stockholm, Sweden. [Rich, Virginia I.] Ohio State Univ, Dept Microbiol, Columbus, OH 43210 USA. [Cooper, William T.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. RP Hodgkins, SB (reprint author), Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. EM sbh10c@fsu.edu OI Hodgkins, Suzanne/0000-0002-0489-9207 FU US Department of Energy Office of Biological and Environmental Research under the Genomic Science program [DE-SC0004632, DE-SC0010580]; NSF [DMR-1157490]; FSU Future Fuels Institute; Ecosystem Genomics Initiative from the University of Arizona Technology and Research Initiative Fund, via the program in Water, Environmental and Energy Solutions FX This research was funded by the US Department of Energy Office of Biological and Environmental Research under the Genomic Science program (Awards DE-SC0004632 and DE-SC0010580). Infrastructure for sampling was provided by the Abisko Scientific Research Station, and mass spectra were obtained at the National High Magnetic Field Laboratory FT-ICR Facility in Tallahassee, FL (Project NSF DMR-1157490). David Podgorski received support from the FSU Future Fuels Institute. Scott Saleska and Virginia Rich received additional support through the Ecosystem Genomics Initiative from the University of Arizona Technology and Research Initiative Fund, via the program in Water, Environmental and Energy Solutions. NR 96 TC 1 Z9 1 U1 40 U2 60 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2016 VL 187 BP 123 EP 140 DI 10.1016/j.gca.2016.05.015 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DR2ME UT WOS:000379737800006 ER PT J AU Cadieux, SB White, JR Sauer, PE Peng, YB Goldman, AE Pratt, LM AF Cadieux, Sarah B. White, Jeffrey R. Sauer, Peter E. Peng, Yongbo Goldman, Amy E. Pratt, Lisa M. TI Large fractionations of C and H isotopes related to methane oxidation in Arctic lakes SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Methane; Hydrogen isotopes; Carbon isotopes; Arctic; Lakes ID FRESH-WATER LAKE; ATMOSPHERIC METHANE; BACTERIAL METHANE; WEST GREENLAND; METHANOTROPHIC DIVERSITY; ACETATE FERMENTATION; MICROBIAL OXIDATION; ANAEROBIC OXIDATION; MASS-SPECTROMETRY; RECEDING GLACIER AB Microbial oxidation of methane (CH4) plays a central role in carbon cycling in Arctic lakes, reducing potential CH4 emissions associated with warming. Isotopic signatures of CH4 (delta C-13 and delta H-2) are indicators of microbial oxidation, wherein the process strongly enriches C-13 and H-2 in residual CH4. We present delta C-13 and delta H-2 measurements obtained from sampling the water column and sediment for dissolved CH4 from three, small Arctic lakes in western Greenland under both open-water and ice-covered conditions from 2013 to 2014. Despite substantial variations in aquatic chemistry among the lakes, delta C-13 and delta H-2 of CH4 suggested that CH4 was produced predominantly by acetoclastic methanogenesis in the littoral sediments and hydrogenotrophic methanogenesis in the profundal sediments in all of the lakes. Surprisingly large variations for both delta C-13 and delta H-2 of CH4 were observed, with delta C-13 extending from -72 parts per thousand to + 7.4 parts per thousand and delta H-2 from -390 parts per thousand to +250 parts per thousand. The CH4 isotopic values reported here were significantly more enriched (p < 0.0001) in both C-13 and H-2 than values reported from other Arctic freshwater environments. As is characteristic of methanotrophy, the enrichment in C-13 and H-2 was associated with low CH4 concentrations. We suggest that the CH4 most enriched in C-13 and H-2 may reflect unusually efficient methanotrophic communities in Arctic ice-margin lakes. This study provides the first measurement of delta H-2 for CH4 in an Arctic freshwater environment at concentrations <10 mu M. The extreme enrichment of C-13 and H-2 of CH4 from Arctic methanotrophy has significant implications for interpreting sources and sinks of CH4. Without knowledge of local geology, stable isotope values of CH4 higher than -30 parts per thousand for delta C-13 and -150 parts per thousand for delta H-2 could be misinterpreted as thermogenic, geothermal, or abiogenic origins. Given crystalline bedrock and the strong positive correlation between delta C-13 and delta H-2 throughout the water columns in three Arctic lakes confirms that CH4 heavily enriched in C-13 and H-2 is the result of methanotrophy. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Cadieux, Sarah B.; Sauer, Peter E.; Peng, Yongbo; Goldman, Amy E.; Pratt, Lisa M.] Indiana Univ, Dept Geol Sci, Bloomington, IN 47405 USA. [White, Jeffrey R.; Goldman, Amy E.] Indiana Univ, Sch Publ & Environm Affairs, Bloomington, IN 47405 USA. [Peng, Yongbo] Louisiana State Univ, Dept Geol & Geophys, Baton Rouge, LA 70803 USA. [Goldman, Amy E.] Pacific Northwest Natl Lab, Richland, WA 99352 USA. RP Cadieux, SB (reprint author), Univ Illinois, Dept Earth & Environm Sci, Chicago, IL 60607 USA. RI White, Jeffrey/A-6965-2017 FU NASA Astrobiology Technology for Exploring Planets (ASTEP) Grant [NNX11AJ01G] FX Funding for this work was provided by NASA Astrobiology Technology for Exploring Planets (ASTEP) Grant #NNX11AJ01G. Thanks to Seth Young, Jennifer Stern and Caroline Freissinet for assistance with sample collection, David Finkelstein for isotopic analysis of hydrogen from water. For logistical support, we thank Polar Field Services, Inc., Kangerlussuaq International Science Support, and Ruth Droppo. Reference materials for delta13C and delta2H of CH4 were provided by Arndt Schimmelmann. NR 85 TC 3 Z9 3 U1 22 U2 36 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2016 VL 187 BP 141 EP 155 DI 10.1016/j.gca.2016.05.004 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DR2ME UT WOS:000379737800007 ER PT J AU Shiel, AE Johnson, TM Lundstrom, CC Laubach, PG Long, PE Williams, KH AF Shiel, A. E. Johnson, T. M. Lundstrom, C. C. Laubach, P. G. Long, P. E. Williams, K. H. TI Reactive transport of uranium in a groundwater bioreduction study: Insights from high-temporal resolution U-238/U-235 data SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Uranium isotopes; Isotope fractionation; Uranium reduction; MC-ICP-MS; Bioremediation ID STABLE-ISOTOPE FRACTIONATION; SHALLOW ALLUVIAL AQUIFER; EARLY SOLAR-SYSTEM; CHEMICAL-EXCHANGE; HEAVY-ELEMENTS; REDUCTION; BIOREMEDIATION; U(VI); ADSORPTION; DEPENDENCE AB We conducted a detailed investigation of U isotopes in conjunction with a broad geochemical investigation during field-scale biostimulation and desorption experiments. This investigation was carried out in the uranium-contaminated alluvial aquifer of the Rifle field research site. In this well-characterized setting, a more comprehensive understanding of U isotope geochemistry is possible. Our results indicate that U isotope fractionation is consistently observed across multiple experiments at the Rifle site. Microbially-mediated reduction is suggested to account for most or all of the observed fractionation as abiotic reduction has been demonstrated to impart much smaller, often near-zero, isotopic fractionation or isotopic fractionation in the opposite direction. Data from some time intervals are consistent with a simple model for transport and U(VI) reduction, where the fractionation factor (epsilon = +0.65 parts per thousand to +0.85 parts per thousand) is consistent with experimental studies. However, during other time intervals the observed patterns in our data indicate the importance of other processes in governing U concentrations and U-238/U-235 ratios. For instance, we demonstrate that departures from Rayleigh behavior in groundwater systems arise from the presence of adsorbed species. We also show that isotope data are sensitive to the onset of oxidation after biostimulation ends, even in the case where reduction continues to remove contaminant uranium downstream. Our study and the described conceptual model support the use of U-238/U-235 ratios as a tool for evaluating the efficacy of biostimulation and potentially other remedial strategies employed at Rifle and other uranium-contaminated sites. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Shiel, A. E.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, 104 CEOAS Adm Bldg,101 SW 26th St, Corvallis, OR 97331 USA. [Johnson, T. M.; Lundstrom, C. C.; Laubach, P. G.] Univ Illinois, Dept Geol, 156 Comp Applicat Bldg,605 E Springfield, Champaign, IL 61820 USA. [Long, P. E.; Williams, K. H.] Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Shiel, AE (reprint author), Oregon State Univ, Coll Earth Ocean & Atmospher Sci, 104 CEOAS Adm Bldg,101 SW 26th St, Corvallis, OR 97331 USA. EM ashiel@ceoas.oregonstate.edu RI Long, Philip/F-5728-2013; Williams, Kenneth/O-5181-2014 OI Long, Philip/0000-0003-4152-5682; Williams, Kenneth/0000-0002-3568-1155 FU U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research [DE-SC0006755, DE-AC02-05CH11231] FX We thank Alison Montgomery and Mark Robbins for help collecting groundwater samples and Joern Larsen for quantifying dissolved U concentrations in groundwater samples. Funding was provided through the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research under contracts DE-SC0006755 (University of Illinois at Urbana-Champaign) and DE-AC02-05CH11231 (Lawrence Berkeley National Laboratory; operated by the University of California). This material is based upon work equally supported through the Integrated Field Research Challenge Site (IFRC) at Rifle, Colorado and the Lawrence Berkeley National Laboratory's Sustainable Systems Scientific Focus Area. We are greatly appreciative of the constructive reviews by three anonymous reviewers and to Claudine Stirling for editorial handling. NR 54 TC 1 Z9 1 U1 10 U2 15 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2016 VL 187 BP 218 EP 236 DI 10.1016/j.gca.2016.05.020 PG 19 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DR2ME UT WOS:000379737800011 ER PT J AU Cassata, WS Borg, LE AF Cassata, W. S. Borg, L. E. TI A new approach to cosmogenic corrections in Ar-40/Ar-39 chronometry: Implications for the ages of Martian meteorites SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article DE Mars; Shergottite; Ar-40/Ar-39; Chronology; Cosmogenic ID NOBLE-GASES; EXCESS AR-40; ISOTOPIC COMPOSITION; THERMAL HISTORY; SHERGOTTITES; ARGON; ORIGIN; AR; ALH84001; AFRICA AB Anomalously old Ar-40/Ar-39 ages are commonly obtained from Shergottites and are generally attributed to uncertainties regarding the isotopic composition of the trapped component and/or the presence of excess Ar-40. Old ages can also be obtained if inaccurate corrections for cosmogenic Ar-36 are applied. Current methods for making the cosmogenic correction require simplifying assumptions regarding the spatial homogeneity of target elements for cosmogenic production and the distribution of cosmogenic nuclides relative to trapped and reactor-derived Ar isotopes. To mitigate uncertainties arising from these assumptions, a new cosmogenic correction approach utilizing the exposure age determined on an un-irradiated aliquot and step-wise production rate estimates that account for spatial variations in Ca and K is described. Data obtained from NWA 4468 and an unofficial pairing of NWA 2975, which yield anomalously old ages when corrected for cosmogenic Ar-36 using conventional techniques, are used to illustrate the efficacy of this new approach. For these samples, anomalous age determinations are rectified solely by the improved cosmogenic correction technique described herein. Ages of 188 +/- 17 and 184 +/- 17 Ma are obtained for NWA 4468 and NWA 2975, respectively, both of which are indistinguishable from ages obtained by other radioisotopic systems. For other Shergottites that have multiple trapped components, have experienced diffusive loss of Ar, or contain excess Ar, more accurate cosmogenic corrections may aid in the interpretation of anomalous ages. The trapped Ar-40/Ar-36 ratios inferred from inverse isochron diagrams obtained from NWA 4468 and NWA 2975 are significantly lower than the Martian atmospheric value, and may represent upper mantle or crustal components. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Cassata, W. S.; Borg, L. E.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, 7000 East Ave, Livermore, CA 94550 USA. RP Cassata, WS (reprint author), Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, 7000 East Ave, Livermore, CA 94550 USA. EM cassata2@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; NASA Cosmochemistry program [NH12AT84I]; NASA Mars Fundamental Research Program [NNH14AX56I] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The authors acknowledge financial support from the NASA Cosmochemistry program (Grant NH12AT84I to L.E.B). Financial support was provided by the NASA Mars Fundamental Research Program (Grant NNH14AX56I to W.S. Cassata). The anonymous reviewers are thanked for thoughtful and constructive reviews of the manuscript, and C. Hall is thanked for handling the manuscript. NR 50 TC 0 Z9 0 U1 7 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD AUG 15 PY 2016 VL 187 BP 279 EP 293 DI 10.1016/j.gca.2016.04.045 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DR2ME UT WOS:000379737800014 ER PT J AU Liu, SL Yang, RJ Pan, YZ Ren, B Chen, QB Li, X Xiong, X Tao, JJ Cheng, QS Ma, MD AF Liu, Shiliang Yang, Rongjie Pan, Yuanzhi Ren, Bo Chen, Qibing Li, Xi Xiong, Xi Tao, Jianjun Cheng, Qingsu Ma, Mingdong TI Beneficial behavior of nitric oxide in copper-treated medicinal plants SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Amino acids; Antitumor alkaloids; Catharanthus roseus L.; Copper stress; Phenolic metabolism ID SCENEDESMUS-QUADRICAUDA CHLOROPHYCEAE; REPENS L. PLANTS; FREE AMINO-ACIDS; CATHARANTHUS-ROSEUS; HYDROGEN-PEROXIDE; OXIDATIVE STRESS; CUCUMIS-SATIVUS; PROTEIN-KINASES; CADMIUM STRESS; PROTON PUMPS AB Despite numerous reports implicating nitric oxide (NO) in the environmental-stress responses of plants, the specific metabolic and ionic mechanisms of NO-mediated adaptation to metal stress remain unclear. Here, the impacts of copper (Cu) and NO donor (SNP, 50 mu M) alone or in combination on the well-known medicinal plant Catharanthus roseus L. were investigated. Our results showed that Cu markedly increased Cu2+ accumulation, decreased NO production, and disrupted mineral equilibrium and proton pumps, thereby stimulating a burst of ROS; in addition, SNP ameliorates the negative toxicity of Cu, and cPTIO reverses this action. Furthermore, the accumulations of ROS and NO resulted in reciprocal changes. Interestingly, nearly all of the investigated amino acids and the total phenolic content in the roots were promoted by the SNP treatment but were depleted by the Cu + SNP treatment, which is consistent with the self-evident increases in phenylalanine ammonia-lyase activity and total soluble phenol content induced by SNP. Unexpectedly, leaf vincristine and vinblastine as well as the total alkaloid content (ca. 1.5-fold) were decreased by Cu but markedly increased by SNP (+38% and +49% of the control levels). This study provides the first evidence of the beneficial behavior of NO, rather than other compounds, in depleting Cu toxicity by regulating mineral absorption, reestablishing ATPase activities, and stimulating secondary metabolites. (C) 2016 Elsevier B.V. All rights reserved. C1 [Liu, Shiliang; Yang, Rongjie; Pan, Yuanzhi; Chen, Qibing; Li, Xi; Tao, Jianjun; Ma, Mingdong] Sichuan Agr Univ, Coll Landscape Architecture, Chengdu 611130, Sichuan, Peoples R China. [Ren, Bo] Sichuan Acad Forestry, Inst Biotechnol & Breeding, Chengdu 610081, Sichuan, Peoples R China. [Xiong, Xi] Univ Missouri, Coll Agr Food & Nat Resources, Columbia, MO 65211 USA. [Cheng, Qingsu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Cheng, Qingsu] Univ Nevada, Dept Elect & Biomed Engn, Reno, NV 89557 USA. RP Ma, MD (reprint author), Sichuan Agr Univ, Coll Landscape Architecture, Chengdu 611130, Sichuan, Peoples R China. EM liushiliang9@163.com; 610245498@qq.com FU National Natural Science Foundation of China (NSFC) [31570700]; National Science and Technology Supporting Program in Eleventh Five Year Plan of China (NSTSP) [2006BA031002] FX This study was partially supported by the National Natural Science Foundation of China (NSFC, No. 31570700) and the National Science and Technology Supporting Program in the Eleventh Five Year Plan of China (NSTSP, No. 2006BA031002). The authors acknowledge Prof. H.X. Song (SICAU, Chengdu, China) for his constructive suggestions on this manuscript. Special thanks are given to associate Prof. S.R. Pu (SICAU, Dujiangyan, China) for his technical assistance in the HPLC determinations, and Dr. J.Z. Zhang (Sichuan University, Chengdu, China) for the fluorescence detections. The authors are also grateful to the editors and three anonymous reviewers for their comments and suggestions on an earlier manuscript. NR 55 TC 1 Z9 2 U1 6 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD AUG 15 PY 2016 VL 314 BP 140 EP 154 DI 10.1016/j.jhazmat.2016.04.042 PG 15 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DO4FX UT WOS:000377738300016 PM 27131454 ER PT J AU Sa, NY Wang, H Proffit, DL Lipson, AL Key, B Liu, M Feng, ZX Fister, TT Ren, Y Sun, CJ Vaughey, JT Fenter, PA Persson, KA Burrell, AK AF Sa, Niya Wang, Hao Proffit, Danielle L. Lipson, Albert L. Key, Baris Liu, Miao Feng, Zhenxing Fister, Timothy T. Ren, Yang Sun, Cheng-Jun Vaughey, John T. Fenter, Paul A. Persson, Kristin A. Burrell, Anthony K. TI Is alpha-V2O5 a cathode material for Mg insertion batteries? SO JOURNAL OF POWER SOURCES LA English DT Article DE Mg battery; Non-aqueous Mg electrolyte; Mg anode; Full cell; Proton intercalation; Solid state NMR ID RECHARGEABLE MAGNESIUM BATTERIES; WIDE ELECTROCHEMICAL WINDOWS; ELECTROLYTE-SOLUTIONS; APROTIC ELECTROLYTES; LITHIUM BATTERIES; INTERCALATION; V2O5; STABILITY; ISSUES; OXIDES AB When designing a high energy density battery, one of the critical features is a high voltage, high capacity cathode material. In the development of Mg batteries, oxide cathodes that can reversibly intercalate Mg, while at the same time being compatible with an electrolyte that can deposit Mg reversibly are rare. Herein, we report the compatibility of Mg anodes with alpha-V2O5 by employing magnesium bis(trifluoromethane sulfonyl)imide in diglyme electrolytes at very low water levels. Electrolytes that contain a high water level do not reversibly deposit Mg, but interestingly these electrolytes appear to enable much higher capacities for an alpha-V2O5 cathode. Solid state NMR indicates that the major source of the higher capacity in high water content electrolytes originates from reversible proton insertion. In contrast, we found that lowering the water level of the magnesium bis(trifluoromethane sulfonyl)imide in diglyme electrolyte is critical to achieve reversible Mg deposition and direct evidence for reversible Mg intercalation is shown. Findings we report here elucidate the role of proton intercalation in water-containing electrolytes and clarify numerous conflicting reports of Mg insertion into alpha-V2O5. (C) 2016 Elsevier B.V. All rights reserved. C1 [Sa, Niya; Wang, Hao; Proffit, Danielle L.; Lipson, Albert L.; Key, Baris; Feng, Zhenxing; Fister, Timothy T.; Vaughey, John T.; Fenter, Paul A.; Burrell, Anthony K.] Argonne Natl Lab, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. [Sa, Niya; Wang, Hao; Proffit, Danielle L.; Lipson, Albert L.; Key, Baris; Feng, Zhenxing; Fister, Timothy T.; Vaughey, John T.; Fenter, Paul A.; Burrell, Anthony K.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Liu, Miao; Persson, Kristin A.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Ren, Yang; Sun, Cheng-Jun] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Sa, NY; Burrell, AK (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. EM san@anl.gov; burrell@anl.gov RI SA, NIYA/E-8521-2017; OI Liu, Miao/0000-0002-1843-9519 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; DOE Office of Science [DE-AC02-06CH11357] FX This work was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. This research used resources at the Electron Microscopy Center in the Center for Nanoscale Materials and the Advanced Photon Source (beamline 11-ID-C and 20-BM-B), two U.S. Department of Energy (DOE) Office of Science User Facilities operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 40 TC 9 Z9 9 U1 39 U2 114 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2016 VL 323 BP 44 EP 50 DI 10.1016/j.jpowsour.2016.05.028 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DP0PQ UT WOS:000378192100007 ER PT J AU Devaux, D Chang, YH Villaluenga, I Chen, XC Chintapalli, M DeSimone, JM Balsara, NP AF Devaux, Didier Chang, Yu H. Villaluenga, Irune Chen, X. Chelsea Chintapalli, Mahati DeSimone, Joseph M. Balsara, Nitash P. TI Conductivity of carbonate- and perfluoropolyether-based electrolytes in porous separators SO JOURNAL OF POWER SOURCES LA English DT Article DE Perfluoropolyether; Conductivity; Separators; Battery; Polyolefin; Polytetrafluoroethylene ID BLOCK-COPOLYMER ELECTROLYTES; LITHIUM-ION BATTERIES; POLYMER ELECTROLYTES; MOLECULAR-WEIGHT; TEMPERATURE; MEMBRANES; SALT; ELECTRODES; COMPLEXES; VISCOSITY AB In lithium batteries, a porous separator filled with an electrolyte is placed in between the electrodes. Properties of the separator such as porosity and wettability strongly influence the conductivity of the electrolyte-separator composite. This study focuses on three commercial separators: a single layer polypropylene (Celgard 2500), a trilayer polypropylene-polyethylene-polypropylene (PP-PE-PP), and a porous polytetrafluoroethylene (PTFE). Electron microscopy was used to characterize the pore structure, and these experiments reveal large differences in pore morphology. The separators were soaked in both carbonate- and perfluoropolyether-based electrolytes. The conductivity of the neat electrolytes (sigma(0)) varied from 6.46 x 10(-6) to 1.76 x 10(-2) S cm(-1). The porosity and wettability of the separator affect the electrolyte uptake that in turn affect the conductivity of electrolyte-separator composites. The conductivity of the electrolyte-separator composites (sigma) was found to follow a master equation, sigma = 0.51. sigma(0).phi(3.2 +/- 0.2)(c), where phi(c) is the volume fraction of the electrolyte in each separator. (C) 2016 Elsevier B.V. All rights reserved. C1 [Devaux, Didier; Chang, Yu H.; Villaluenga, Irune; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Devaux, Didier; Villaluenga, Irune; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCESR, Berkeley, CA 94720 USA. [Devaux, Didier; Chang, Yu H.; Villaluenga, Irune; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Chen, X. Chelsea; Chintapalli, Mahati; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Chintapalli, Mahati] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [DeSimone, Joseph M.] Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA. [DeSimone, Joseph M.] N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Chem Engn, 201 Gilman Hall, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu FU Center for Mesoscale Transport Properties, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012673] FX This work was supported as part of the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under award #DE-SC0012673. NR 37 TC 0 Z9 0 U1 12 U2 47 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD AUG 15 PY 2016 VL 323 BP 158 EP 165 DI 10.1016/j.jpowsour.2016.05.039 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DP0PQ UT WOS:000378192100020 ER PT J AU Das, S Brown, S Mayes, RT Janke, CJ Tsouris, C Kuo, LJ Gill, G Dai, S AF Das, S. Brown, S. Mayes, R. T. Janke, C. J. Tsouris, C. Kuo, L. -J. Gill, G. Dai, S. TI Novel poly(imide dioxime) sorbents: Development and testing for enhanced extraction of uranium from natural seawater SO CHEMICAL ENGINEERING JOURNAL LA English DT Article DE Polymer; Grafting; Amidoxime; Imide dioxime; Uranium adsorption; Seawater ID SEA-WATER; SPECTROPHOTOMETRIC DETERMINATION; AQUEOUS-SOLUTION; ACRYLIC-ACID; AMIDOXIME; POLYACRYLONITRILE; ACRYLONITRILE; RECOVERY; COMPLEXATION; ADSORPTION AB A new series of amidoxime-based polymer adsorbents were synthesized at the Oak Ridge National Laboratory (ORNL) by electron beam induced grafting of acrylonitrile and itaconic acid onto polyethylene fiber. Hydroxylamine derivatives of poly(acrylonitrile) (PAN) moiety are demonstrated to possess two kinds of functional groups: open-chain amidoxime and cyclic imide dioxime. The open-chain amidoxime is shown to convert to imide dioxime on heat treatment in the presence of an aprotic solvent, like dimethylsulfoxide (DMSO). The formation of amidoxime and imide dioxime was confirmed by C-13 CP-MAS spectra. The adsorbents were evaluated for uranium adsorption efficiency at ORNL with simulated seawater spiked with 8 ppm uranium and 5 gallon seawater in a batch reactor, and in flow-through columns with natural seawater at the Marine Science Laboratory (MSL) of Pacific Northwest National Laboratory (PNNL) at Sequim Bay, WA. The DMSO-heat-treated sorbents adsorbed uranium as high as 4.48 g-U/kg-ads. from seawater. Experimental evidence is presented that the poly(imide dioxime) is primarily responsible for enhanced uranium adsorption capacity from natural seawater. The conjugated system in the imide dioxime ligand possesses increased electron donation ability, which is believed to significantly enhance the uranyl coordination in seawater. (C) 2016 Elsevier B.V. All rights reserved. C1 [Das, S.; Mayes, R. T.; Janke, C. J.; Tsouris, C.; Dai, S.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Brown, S.; Dai, S.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Kuo, L. -J.; Gill, G.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Das, S (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM dass1@ornl.gov; dais@ornl.gov RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027 FU US Department of Energy, Office of Nuclear Energy; US Department of Energy [DE-AC05-000R22725]; Department of Energy FX This work was sponsored by the US Department of Energy, Office of Nuclear Energy. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-000R22725 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 39 TC 4 Z9 4 U1 35 U2 85 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 1385-8947 EI 1873-3212 J9 CHEM ENG J JI Chem. Eng. J. PD AUG 15 PY 2016 VL 298 BP 125 EP 135 DI 10.1016/j.cej.2016.04.013 PG 11 WC Engineering, Environmental; Engineering, Chemical SC Engineering GA DN8DQ UT WOS:000377309800014 ER PT J AU Simos, N Elbakhshwan, M Zhong, Z Ghose, S Savkliyildiz, I AF Simos, Nikolaos Elbakhshwan, Mohamed Zhong, Zhong Ghose, Sanjit Savkliyildiz, Ilyas TI High-temperature annealing of proton irradiated beryllium - A dilatometry-based study SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Irradiation damage; High temperature annealing; Oxidation; Transmutation gas; Beryllium ID NEUTRON-IRRADIATION; MICROSTRUCTURE; OXIDATION; DEUTERIUM; OXYGEN; IONS AB S-200 F grade beryllium has been irradiated with 160 MeV protons up to 1.2 10(20) cm(-2) peak fluence and irradiation temperatures in the range of 100-200 degrees C. To address the effect of proton irradiation on dimensional stability, an important parameter in its consideration in fusion reactor applications, and to simulate high temperature irradiation conditions, multi-stage annealing using high precision dilatometry to temperatures up to 740 degrees C were conducted in air. X-ray diffraction studies were also performed to compliment the macroscopic thermal study and offer a microscopic view of the irradiation effects on the crystal lattice. The primary objective was to qualify the competing dimensional change processes occurring at elevated temperatures namely manufacturing defect annealing, lattice parameter recovery, transmutation He-4 and H-3 diffusion and swelling and oxidation kinetics. Further, quantification of the effect of irradiation dose and annealing temperature and duration on dimensional changes is sought. The study revealed the presence of manufacturing porosity in the beryllium grade, the oxidation acceleration effect of irradiation including the discontinuous character of oxidation advancement, the effect of annealing duration on the recovery of lattice parameters recovery and the triggering temperature for transmutation gas diffusion leading to swelling. (C) 2016 Published by Elsevier B.V. C1 [Simos, Nikolaos; Elbakhshwan, Mohamed; Zhong, Zhong; Ghose, Sanjit] Brookhaven Natl Lab, Upton, NY 11973 USA. [Savkliyildiz, Ilyas] Rutgers State Univ, Piscataway, NJ 08855 USA. RP Simos, N (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM simos@bnl.gov OI Elbakhshwan, Mohamed/0000-0002-3995-4173 FU US DOE [DE-AC02-CH10886] FX Work performed under the auspices of the US DOE.; Work at the NSLS is supported under US DOE contract DE-AC02-CH10886. NR 21 TC 0 Z9 0 U1 2 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 1 EP 17 DI 10.1016/j.jnucmat.2016.04.001 PG 17 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000001 ER PT J AU Lim, HC Rudman, K Krishnan, K McDonald, R Dickerson, P Gong, BW Peralta, P AF Lim, Harn Chyi Rudman, Karin Krishnan, Kapil McDonald, Robert Dickerson, Patricia Gong, Bowen Peralta, Pedro TI Effects of microstructural constraints on the transport of fission products in uranium dioxide at low burnups SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID GRAIN-BOUNDARY DIFFUSION; GAS RELEASE; POLYCRYSTALLINE UO2; MOLECULAR-DYNAMICS; NUCLEAR-FUEL; SIZE; IRRADIATION; SIMULATION; ANISOTROPY; NETWORKS AB Diffusion of fission gases in UO2 is studied at low burnups, before bubble growth and coalescence along grain boundaries (GBs) become dominant, using a 3-D finite element model that incorporates actual UO2 microstructures. Grain boundary diffusivities are assigned based on crystallography with lattice and GB diffusion coupled with temperature to account for temperature gradients. Heterogeneity of GB properties and connectivity can induce regions where concentration is locally higher than without GB diffusion. These regions are produced by "bottlenecks" in the GB network because of lack of connectivity among high diffusivity GBs due to crystallographic constraints, and they can lead to localized swelling. Effective diffusivities were calculated assuming a uniform distribution of high diffusivity among GBs. Results indicate an increase over the bulk diffusivity with a clear grain size effect and that connectivity and properties of different GBs become important factors on the variability of fission product concentration at the microscale. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lim, Harn Chyi; Rudman, Karin; Krishnan, Kapil; McDonald, Robert; Gong, Bowen; Peralta, Pedro] Arizona State Univ, Tempe, AZ USA. [Dickerson, Patricia] Los Alamos Natl Lab, Los Alamos, NM USA. RP Peralta, P (reprint author), Arizona State Univ, Tempe, AZ USA. EM pperalta@asu.edu FU Fulton Schools of Engineering at Arizona State University; DOE/NE [DE-NE-0000670000, DE-NE-0000134] FX Modeling work was supported by a graduate fellowship to H. Lim from the Fulton Schools of Engineering at Arizona State University and microstructural reconstruction was supported by DOE/NE under grants # DE-NE-0000670000 and DE-NE-0000134. We are also grateful to D. Byler and K. McClellan at Los Alamos National Laboratory for providing the UO2 pellets used to gather the 3-D microstructural data for this work. NR 41 TC 0 Z9 0 U1 6 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 24 EP 36 DI 10.1016/j.jnucmat.2016.04.032 PG 13 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000003 ER PT J AU Backman, M Juslin, N Huang, GY Wirth, BD AF Backman, Marie Juslin, Niklas Huang, Guiyang Wirth, Brian D. TI A W-Ne interatomic potential for simulation of neon implantation in tungsten SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID TRANSITION-METALS; DYNAMICS; HE AB An interatomic pair potential for W-Ne is developed for atomistic molecular dynamics simulations of neon implantation in tungsten. The new potential predicts point defect energies and binding energies of small clusters that are in good agreement with electronic structure calculations. Molecular dynamics simulations of small neon clusters in tungsten show that trap mutation, in which an interstitial neon cluster displaces a tungsten atom from its lattice site, occurs for clusters of three or more neon atoms. However, near a free surface, trap mutation can occur at smaller sizes, including even a single neon interstitial in close proximity to a (100) or (110) surface. (C) 2016 Published by Elsevier B.V. C1 [Backman, Marie; Juslin, Niklas; Huang, Guiyang; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Wirth, Brian D.] Oak Ridge Natl Lab, POB 2008,MS-6003, Oak Ridge, TN 37831 USA. RP Wirth, BD (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. EM bdwirth@utk.edu FU Scientific Discovery through Advanced Computing (SciDAC) project on Plasma-Surface Interactions - U. S. Department of Energy, Offices of Science, Advanced Scientific Computing Research, and Fusion Energy Sciences; Plasma-Surface Interactions Science Center - U. S. Department of Energy, Office of Fusion Energy Sciences [DE-SC00-02060]; U.S. Department of Energy, Office of Fusion Energy Sciences [DE-SC0006661] FX Partial financial support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) project on Plasma-Surface Interactions, funded by the U. S. Department of Energy, Offices of Science, Advanced Scientific Computing Research, and Fusion Energy Sciences. Additional funding was provided through the Plasma-Surface Interactions Science Center, funded by the U. S. Department of Energy, Office of Fusion Energy Sciences under award DE-SC00-02060 and by the U.S. Department of Energy, Office of Fusion Energy Sciences under award DE-SC0006661. NR 17 TC 1 Z9 1 U1 4 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 37 EP 41 DI 10.1016/j.jnucmat.2016.05.002 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000004 ER PT J AU Steiner, MA Calhoun, CA Klein, RW An, K Garlea, E Agnew, SR AF Steiner, M. A. Calhoun, C. A. Klein, R. W. An, K. Garlea, E. Agnew, S. R. TI alpha-Phase transformation kinetics of U-8 wt% Mo established by in situ neutron diffraction SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE U-Mo alloys; Neutron diffraction; Time-temperature-transformation diagram; Transformation kinetics; Eutectoid decomposition ID THERMOMECHANICAL PROCESS OPTIMIZATION; MICROSTRUCTURE; NUCLEATION; ALLOYS; GROWTH AB The a-phase transformation kinetics of as-cast U - 8 wt% Mo below the eutectoid temperature have been established by in situ neutron diffraction. alpha-phase weight fraction data acquired through Rietveld refinement at five different isothermal hold temperatures can be modeled accurately utilizing a simple Johnson-Mehl-Avrami-Kolmogorov impingement-based theory, and the results are validated by a corresponding evolution in the g-phase lattice parameter during transformation that follows Vegard's law. Neutron diffraction data is used to produce a detailed Time-Temperature-Transformation diagram that improves upon inconsistencies in the current literature, exhibiting a minimum transformation start time of 40 min at temperatures between 500 degrees C and 510 degrees C. The transformation kinetics of U - 8 wt% Mo can vary significantly from as-cast conditions after extensive heat treatments, due to homogenization of the typical dendritic microstructure which possesses non-negligible solute segregation. (C) 2016 Elsevier B.V. All rights reserved. C1 [Steiner, M. A.; Calhoun, C. A.; Klein, R. W.; Agnew, S. R.] Univ Virginia, Mat Sci & Engn, 395 McCormick Rd, Charlottesville, VA 22904 USA. [An, K.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Garlea, E.] Y-12 Natl Secur Complex, Oak Ridge, TN 37831 USA. RP Steiner, MA (reprint author), Univ Virginia, Mat Sci & Engn, 395 McCormick Rd, Charlottesville, VA 22904 USA. EM mas4cw@virginia.edu RI An, Ke/G-5226-2011 OI An, Ke/0000-0002-6093-429X FU Y-12 National Security Complex's Plant Directed Research, Development, and Demonstration program; Scientific User Facilities Division, the Office of Basic Energy Sciences, the U.S. Department of Energy; agency of the United States Government [DE NA0001942]; U.S. Department of Energy/National Nuclear Security Administration [DE-NA-0001942] FX Funding for this research was provided by the Y-12 National Security Complex's Plant Directed Research, Development, and Demonstration program. The Spallation Neutron Source (SNS) user facility, Oak Ridge National Laboratory, is supported by the Scientific User Facilities Division, the Office of Basic Energy Sciences, the U.S. Department of Energy. This work of authorship and those incorporated herein were prepared by Consolidated Nuclear Security, LLC (CNS) Pantex Plant/Y-12 National Security Complex as accounts of work sponsored by an agency of the United States Government under contract DE NA0001942. Neither the United States Government nor any agency thereof, nor CNS, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility to any non-governmental recipient hereof for the accuracy, completeness, use made, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency or contractor thereof, or by CNS. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency or contractor ( other than the authors) thereof. This document has been authored by Consolidated Nuclear Security, LLC, under Contract DE-NA-0001942 with the U.S. Department of Energy/National Nuclear Security Administration, or a subcontractor thereof. The United States Government retains and the publisher, by accepting the document for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this document, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U.S. Government purposes. The authors would like to thank Matt Frost of Oak Ridge National Laboratory for his logistical help throughout this experiment. NR 35 TC 0 Z9 0 U1 3 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 149 EP 156 DI 10.1016/j.jnucmat.2016.05.016 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000018 ER PT J AU Perez, E Keiser, DD Sohn, YH AF Perez, E. Keiser, D. D. Sohn, Y. H. TI Microstructural development from interdiffusion and reaction between U-Mo and AA6061 alloys annealed at 600 degrees and 550 degrees C SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Fuel development; Nuclear fuel; Research reactor; Uranium molybdenum; Aluminum alloy; Interdiffusion; Intermetallic; Phase development; U-Mo; 6061; AA6061 ID MO/AL DISPERSION FUEL; URANIUM-MOLYBDENUM ALLOYS; TRANSMISSION ELECTRON-MICROSCOPY; NUCLEAR-RESEARCH REACTORS; HEAVY-ION IRRADIATION; X-RAY-DIFFRACTION; AL A356 ALLOY; DIFFUSION COUPLES; INTERACTION LAYER; HIGH-DENSITY AB The U.S. Material Management and Minimization Reactor Conversion Program is developing low enrichment fuel systems encased in Al-alloy for use in research and test reactors. Monolithic fuel plates have local regions where the U-Mo fuel plate may come into contact with the Al-alloy 6061 (AA6061) cladding. This results in the development of interdiffusion zones with complex microstructures with multiple phases. In this study, the microstructural development of diffusion couples, U-7 wt% Mo, U-10 wt% Mo, and U-12 wt% Mo vs. AA6061, annealed at 600 degrees C for 24 h and at 550 degrees C for 1, 5, and 20 h, were analyzed by scanning electron microscopy with x-ray energy dispersive spectroscopy. The microstructural development and kinetics were compared to diffusion couples U-Mo vs. high purity Al and binary Al-Si alloys. The diffusion couples developed complex interaction regions where phase development was influenced by the alloying additions of the AA6061. Published by Elsevier B.V. C1 [Perez, E.; Keiser, D. D.] Idaho Natl Lab, Nucl Fuels & Mat Div, POB 1625, Idaho Falls, ID 83415 USA. [Sohn, Y. H.] Univ Cent Florida, Dept Mat Sci & Engn, 4000 Cent Florida Blvd, Orlando, FL 32816 USA. RP Perez, E (reprint author), Idaho Natl Lab, Nucl Fuels & Mat Div, POB 1625, Idaho Falls, ID 83415 USA. EM Emmanuel.Perez@inl.gov; dennis.keiser@inl.gov; yongho.sohn@ucf.edu RI Sohn, Yongho/A-8517-2010; OI Sohn, Yongho/0000-0003-3723-4743; Perez, Emmanuel/0000-0001-5546-4978 FU U.S. Department of Energy [DE-AC07-05ID14517] FX This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 72 TC 0 Z9 0 U1 6 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 178 EP 192 DI 10.1016/j.jnucmat.2016.05.019 PG 15 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000022 ER PT J AU Wood, ES Terrani, KA Nelson, AT AF Wood, E. Sooby Terrani, K. A. Nelson, A. T. TI Sensitivity of measured steam oxidation kinetics to atmospheric control and impurities SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID HIGH-TEMPERATURE OXIDATION; REFRACTORY METALS; FLOWING STEAM; WATER-VAPOR; MOLYBDENUM; ZIRCALOY-4 AB The most direct means of improving the ability of water cooled reactors to withstand excessive cladding oxidation during a loss of coolant accident is to either modify or replace zirconium cladding. It is important to understand what level of agreement is to be expected as a function of systematic differences in steam oxidation testing techniques and instrumentation among testing facilities. The present study was designed to assess the sensitivities of some of the current and proposed reactor cladding materials. Steam oxidation sensitivity of Zircaloy-2, FeCrAl and Mo to O-2 impurities in steam were examined. It was shown that the effect of O-2 impurities is negligible for the two former materials while significant in the case of Mo. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wood, E. Sooby; Nelson, A. T.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Terrani, K. A.] Oak Ridge Natl Lab, Nucl Fuels Mat Grp, Oak Ridge, TN USA. RP Wood, ES (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM sooby@lanl.gov OI Nelson, Andrew/0000-0002-4071-3502 FU U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle Research and Development program FX This work was supported by the U.S. Department of Energy, Office of Nuclear Energy Fuel Cycle Research and Development program. NR 17 TC 0 Z9 0 U1 3 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD AUG 15 PY 2016 VL 477 BP 228 EP 233 DI 10.1016/j.jnucmat.2016.05.023 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DN8KD UT WOS:000377327000027 ER EF