FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Chaston, CC Bonnell, JW Reeves, GD Skoug, RM AF Chaston, C. C. Bonnell, J. W. Reeves, G. D. Skoug, R. M. TI Driving ionospheric outflows and magnetospheric O+ energy density with Alfven waves SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID FIELD LINE RESONANCES; INNER MAGNETOSPHERE; RING CURRENT; GEOSYNCHRONOUS ORBIT; ION-ACCELERATION; SMALL-SCALE; PLASMA; FREQUENCY; MAGNETOPAUSE; TURBULENCE AB We show how dispersive Alfven waves observed in the inner magnetosphere during geomagnetic storms can extract O+ ions from the topside ionosphere and accelerate these ions to energies exceeding 50 keV in the equatorial plane. This occurs through wave trapping, a variant of "shock" surfing, and stochastic ion acceleration. These processes in combination with the mirror force drive field-aligned beams of outflowing ionospheric ions into the equatorial plane that evolve to provide energetic O+ distributions trapped near the equator. These waves also accelerate preexisting/injected ion populations on the same field lines. We show that the action of dispersive Alfven waves over several minutes may drive order of magnitude increases in O+ ion pressure to make substantial contributions to magnetospheric ion energy density. These wave accelerated ions will enhance the ring current and play a role in the storm time evolution of the magnetosphere. C1 [Chaston, C. C.; Bonnell, J. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Chaston, C. C.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Reeves, G. D.; Skoug, R. M.] Los Alamos Natl Lab, Los Alamos, NM USA. [Reeves, G. D.] New Mexico Consortium, Space Sci Div, Los Alamos, NM USA. RP Chaston, CC (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.; Chaston, CC (reprint author), Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. EM ccc@ssl.berkeley.edu OI Reeves, Geoffrey/0000-0002-7985-8098 FU NASA [NNX11AD78G, NNX15AF57G, NNX16AG69G]; Van Allen Probes (RBSP) under NASA [NAS5-01072]; RBSP-ECT JHU/APL [967399]; Australian Research Council [FT110100316]; University of Sydney FX This research was supported by the NASA grants NNX11AD78G, NNX15AF57G, and NNX16AG69G and Van Allen Probes (RBSP) funding provided under NASA prime contract NAS5-01072, including the EFW investigation (PI: J.R. Wygant, University of Minnesota), RBSP-ECT JHU/APL under contract 967399. Chris Chaston also received support from the Australian Research Council through fellowship FT110100316 and a University of Sydney bridging grant. Simulation generated data are stored on Linux workstations at the Space Sciences Laboratory at UC Berkeley and can be accessed by contacting the first author. All observational data used in this study can be obtained at http://www.rbsp-ect.lanl.gov/science/DataDirectories.php. NR 34 TC 1 Z9 1 U1 1 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 28 PY 2016 VL 43 IS 10 BP 4825 EP 4833 DI 10.1002/2016GL069008 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DP2UC UT WOS:000378347500020 ER PT J AU Atchley, AL Coon, ET Painter, SL Harp, DR Wilson, CJ AF Atchley, Adam L. Coon, Ethan T. Painter, Scott L. Harp, Dylan R. Wilson, Cathy J. TI Influences and interactions of inundation, peat, and snow on active layer thickness SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID LAND-SURFACE MODEL; 3-PHASE NUMERICAL-MODEL; ARCTIC COASTAL-PLAIN; EARTH SYSTEM MODELS; CLIMATE-CHANGE; THERMAL-CONDUCTIVITY; PERMAFROST DYNAMICS; WATER-BALANCE; ORGANIC SOIL; CARBON AB Active layer thickness (ALT), the uppermost layer of soil that thaws on an annual basis, is a direct control on the amount of organic carbon potentially available for decomposition and release to the atmosphere as carbon-rich Arctic permafrost soils thaw in a warming climate. We investigate how key site characteristics affect ALT using an integrated surface/subsurface permafrost thermal hydrology model. ALT is most sensitive to organic layer thickness followed by snow depth but is relatively insensitive to the amount of water on the landscape with other conditions held fixed. The weak ALT sensitivity to subsurface saturation suggests that changes in Arctic landscape hydrology may only have a minor effect on future ALT. However, surface inundation amplifies the sensitivities to the other parameters and under large snowpacks can trigger the formation of near-surface taliks. C1 [Atchley, Adam L.; Coon, Ethan T.; Harp, Dylan R.; Wilson, Cathy J.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Painter, Scott L.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Painter, Scott L.] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Atchley, AL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM aatchley@lanl.gov RI Painter, Scott/C-2586-2016; OI Painter, Scott/0000-0002-0901-6987; Harp, Dylan/0000-0001-9777-8000; Atchley, Adam/0000-0003-2203-1994 FU Los Alamos National Laboratory, Laboratory Direction Research and Development project [LDRD201200068DR]; Next Generation Ecosystem Experiment (NGEE-Arctic) project; Office of Biological and Environmental Research in the DOE Office of Science FX This work was supported by the Los Alamos National Laboratory, Laboratory Direction Research and Development project LDRD201200068DR and by the Next Generation Ecosystem Experiment (NGEE-Arctic) project. NGEE-Arctic is supported by the Office of Biological and Environmental Research in the DOE Office of Science. Model input files and result can be accessed at 10.5440/1240734. In addition, we wish to extend our thanks to GRL Editor Julienne Stroeve and two anonymous reviewers and who provided thoughtful commentary resulting in a quality manuscript. NR 60 TC 3 Z9 3 U1 7 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 28 PY 2016 VL 43 IS 10 BP 5116 EP 5123 DI 10.1002/2016GL068550 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DP2UC UT WOS:000378347500056 ER PT J AU Mlynczak, MG Daniels, TS Kratz, DP Feldman, DR Collins, WD Mlawer, EJ Alvarado, MJ Lawler, JE Anderson, LW Fahey, DW Hunt, LA Mast, JC AF Mlynczak, Martin G. Daniels, Taumi S. Kratz, David P. Feldman, Daniel R. Collins, William D. Mlawer, Eli J. Alvarado, Matthew J. Lawler, James E. Anderson, L. W. Fahey, David W. Hunt, Linda A. Mast, Jeffrey C. TI The spectroscopic foundation of radiative forcing of climate by carbon dioxide SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID LINE-SHAPE; TRANSFER MODEL; CO2; DATABASE; SPECTRA; BANDS; TEMPERATURE; PARAMETERS; SOFTWARE; 15-MU-M AB The radiative forcing (RF) of carbon dioxide (CO2) is the leading contribution to climate change from anthropogenic activities. Calculating CO2 RF requires detailed knowledge of spectral line parameters for thousands of infrared absorption lines. A reliable spectroscopic characterization of CO2 forcing is critical to scientific and policy assessments of present climate and climate change. Our results show that CO2 RF in a variety of atmospheres is remarkably insensitive to known uncertainties in the three main CO2 spectroscopic parameters: the line shapes, line strengths, and half widths. We specifically examine uncertainty in RF due to line mixing as this process is critical in determining line shapes in the far wings of CO2 absorption lines. RF computed with a Voigt line shape is also examined. Overall, the spectroscopic uncertainty in present-day CO2 RF is less than 1%, indicating a robust foundation in our understanding of how rising CO2 warms the climate system. C1 [Mlynczak, Martin G.; Daniels, Taumi S.; Kratz, David P.] NASA Langley Res Ctr, Hampton, VA 23666 USA. [Feldman, Daniel R.; Collins, William D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Mlawer, Eli J.; Alvarado, Matthew J.] Atmospher & Environm Res Inc, Lexington, MA USA. [Lawler, James E.; Anderson, L. W.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Fahey, David W.] NOAA Environm Syst Res Lab, Boulder, CO USA. [Hunt, Linda A.; Mast, Jeffrey C.] Sci Syst & Applicat Inc, Hampton, VA USA. RP Mlynczak, MG (reprint author), NASA Langley Res Ctr, Hampton, VA 23666 USA. EM m.g.mlynczak@nasa.gov RI Fahey, David/G-4499-2013; Richards, Amber/K-8203-2015; Collins, William/J-3147-2014; Feldman, Daniel/N-8703-2013; Manager, CSD Publications/B-2789-2015 OI Fahey, David/0000-0003-1720-0634; Collins, William/0000-0002-4463-9848; Feldman, Daniel/0000-0003-3365-5233; FU National Aeronautics and Space Administration Climate Absolute Radiance and Refractivity Observatory (CLARREO) project at Langley Research Center FX This work was supported with funding from the National Aeronautics and Space Administration Climate Absolute Radiance and Refractivity Observatory (CLARREO) project at Langley Research Center. This article has been contributed to by US Government employees and their work is in the public domain in the USA. I. Gordon and L. Rothman of Smithsonian Astrophysical Observatory provided helpful discussions on spectral line uncertainties. The LBLRTM model can be obtained online at http://rtweb.aer.com and the atmospheric profile data used to perform the calculations contained in this paper are available NR 27 TC 1 Z9 1 U1 8 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 28 PY 2016 VL 43 IS 10 BP 5318 EP 5325 DI 10.1002/2016GL068837 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DP2UC UT WOS:000378347500080 ER PT J AU Ivashchenko, VI Turchi, PEA Veprek, S Shevchenko, VI Leszczynski, J Gorb, L Hill, F AF Ivashchenko, V. I. Turchi, P. E. A. Veprek, S. Shevchenko, V. I. Leszczynski, Jerzy Gorb, Leonid Hill, Frances TI First-principles study of crystalline and amorphous AlMgB14-based materials SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID 1ST PRINCIPLES; THIN-FILMS; BORON; BORIDES; DIFFRACTION AB We report first-principles investigations of crystalline and amorphous boron and M1(x)M2(y)X(z)B(14-z) (M1, M2 = Al, Mg, Li, Na, Y; X = Ti, C, Si) phases (so-called "BAM" materials). Phase stability is analyzed in terms of formation energy and dynamical stability. The atomic configurations as well as the electronic and phonon density states of these phases are compared. Amorphous boron consists of distorted icosahedra, icosahedron fragments, and dioctahedra, connected by an amorphous network. The presence of metal atoms in amorphous BAM materials precludes the formation of icosahedra. For all the amorphous structures considered here, the Fermi level is located in the mobility gap independent of the number of valence electrons. The intra-icosahedral vibrations are localized in the range of 800 cm(-1), whereas the inter-icosahedral vibrations appear at higher wavenumbers. The amorphization leads to an enhancement of the vibrations in the range of 1100-1250 cm(-1). The mechanical properties of BAM materials are investigated at equilibrium and under shear and tensile strain. The anisotropy of the ideal shear and tensile strengths is explained in terms of a layered structure of the B-12 units. The strength of amorphous BAM materials is lower than that of the crystalline counterparts because of the partial fragmentation of the boron icosahedra in amorphous structures. The strength enhancement found experimentally for amorphous boron-based films is very likely related to an increase in film density, and the presence of oxygen impurities. For crystalline BAM materials, the icosahedra are preserved during elongation upon tension as well as upon shear in the (010)[100] slip system. Published by AIP Publishing. C1 [Ivashchenko, V. I.; Shevchenko, V. I.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, Krzhyzhanosky Str 3, UA-03142 Kiev, Ukraine. [Turchi, P. E. A.] Lawrence Livermore Natl Lab, L-352,POB 808, Livermore, CA 94551 USA. [Veprek, S.] Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85747 Garching, Germany. [Leszczynski, Jerzy; Gorb, Leonid] Jackson State Univ, Dept Chem & Biochem, Interdisciplinary Ctr Nanotox, Jackson, MS 39217 USA. [Gorb, Leonid] Badger Tech Serv LLC, Vicksburg, MS 39180 USA. [Hill, Frances] US Army, Erdc, Vicksburg, MS 39180 USA. RP Shevchenko, VI (reprint author), Natl Acad Sci Ukraine, Inst Problems Mat Sci, Krzhyzhanosky Str 3, UA-03142 Kiev, Ukraine. EM shev@materials.kiev.ua RI Veprek, Stan/C-1248-2008 OI Veprek, Stan/0000-0002-6016-3093 FU STCU [5964]; U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Company SHM s.r.o. (Czech Republic) FX This work was supported by the STCU Contract No. 5964. The work of P.T. was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. The authors are grateful to the directorate of the Summer Institute at Jackson State University for the opportunity to perform large-scale calculations. S.V. thanks the Company SHM s.r.o. (Czech Republic) for financial support. We also thank Dr. M.G.J. Veprek-Heijman for critical reading of the manuscript and many useful comments. NR 48 TC 2 Z9 2 U1 4 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 28 PY 2016 VL 119 IS 20 AR 205105 DI 10.1063/1.4952391 PG 13 WC Physics, Applied SC Physics GA DO3YM UT WOS:000377718700037 ER PT J AU Joshya, RS Rajaji, V Narayana, C Mascarenhas, A Kini, RN AF Joshya, R. S. Rajaji, V. Narayana, Chandrabhas Mascarenhas, A. Kini, R. N. TI Anharmonicity in light scattering by optical phonons in GaAs1-xBix SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID BAND-GAP; GAASBI ALLOYS; RAMAN; NITROGEN; BI; SEMICONDUCTORS; SPECTROSCOPY; TEMPERATURE; DEPENDENCE; ABSORPTION AB We present a Raman spectroscopic study of GaAs1-xBix epilayers grown by molecular beam epitaxy. We have investigated the anharmonic effect on the GaAs-like longitudinal optical phonon mode (LOGaAs') of GaAs1-xBix for different Bi concentrations at various temperatures. The results are analyzed in terms of the anharmonic damping effect induced by thermal and compositional disorder. We have observed that the anharmonicity increases with Bi concentration in GaAs1-xBix as evident from the increase in the anharmonicity constants. In addition, the anharmonic lifetime of the optical phonon decreases with increasing Bi concentration in GaAs1-xBix. Published by AIP Publishing. C1 [Joshya, R. S.; Kini, R. N.] Indian Inst Sci Educ & Res Thiruvananthapuram IIS, CET Campus, Thiruvananthapuram 695016, Kerala, India. [Rajaji, V.; Narayana, Chandrabhas] JNCASR, Bangalore 560064, Karnataka, India. [Mascarenhas, A.] NREL, 1617 Cole Blvd, Golden, CO 80401 USA. RP Joshya, RS; Kini, RN (reprint author), Indian Inst Sci Educ & Res Thiruvananthapuram IIS, CET Campus, Thiruvananthapuram 695016, Kerala, India. EM joshya@iisertvm.ac.in; rajeevkini@iisertvm.ac.in OI Kini, Rajeev/0000-0002-3305-9346 FU Science and Engineering Research Board, Department of Science and Technology, India through the Fast Track Scheme for Young Scientists; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC36-08GO28308] FX Research at IISER-TVM was supported by Science and Engineering Research Board, Department of Science and Technology, India through the Fast Track Scheme for Young Scientists and the work at NREL was supported by U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC36-08GO28308. NR 39 TC 0 Z9 0 U1 6 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 28 PY 2016 VL 119 IS 20 AR 205706 DI 10.1063/1.4952381 PG 5 WC Physics, Applied SC Physics GA DO3YM UT WOS:000377718700055 ER PT J AU Perez, D Sandoval, L Uberuaga, BP Voter, AF AF Perez, Danny Sandoval, Luis Uberuaga, Blas P. Voter, Arthur F. TI The thermodynamic and kinetic interactions of He interstitial clusters with bubbles in W SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LOW-ENERGY; HELIUM BUBBLES; TUNGSTEN; METALS; RETENTION; PLASMA; IRRADIATION; SIMULATION; HYDROGEN; SURFACE AB Due to its enviable properties, tungsten is a leading candidate plasma facing material in nuclear fusion reactors. However, like many other metals, tungsten is known to be affected by the high doses of helium atoms incoming from the plasma. Indeed, the implanted interstitial helium atoms cluster together and, upon reaching a critical cluster size, convert into substitutional nanoscale He bubbles. These bubbles then grow by absorbing further interstitial clusters from the matrix. This process can lead to deleterious changes in microstructure, degradation of mechanical properties, and contamination of the plasma. In order to better understand the growth process, we use traditional and accelerated molecular dynamics simulations to investigate the interactions between interstitial He clusters and pre-existing bubbles. These interactions are characterized in terms of thermodynamics and kinetics. We show that the proximity of the bubble leads to an enhancement of the trap mutation rate and, consequently, to the nucleation of satellite bubbles in the neighborhood of existing ones. We also uncover a number of mechanisms that can lead to the subsequent annihilation of such satellite nanobubbles. Published by AIP Publishing. C1 [Perez, Danny; Sandoval, Luis; Voter, Arthur F.] Los Alamos Natl Lab, Theoret Div T1, POB 1663, Los Alamos, NM 87545 USA. [Uberuaga, Blas P.] Los Alamos Natl Lab, Mat Sci & Technol MST 8, POB 1663, Los Alamos, NM 87545 USA. RP Perez, D (reprint author), Los Alamos Natl Lab, Theoret Div T1, POB 1663, Los Alamos, NM 87545 USA. EM danny_perez@lanl.gov OI Voter, Arthur/0000-0001-9788-7194; Sandoval, Luis/0000-0002-1172-7972 FU United States Department of Energy (U.S. DOE) SciDAC program; Office of Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the United States Department of Energy (U.S. DOE) SciDAC program (DP, LS, BPU) and by the Office of Basic Energy Sciences, Materials Sciences and Engineering Division (AFV). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract No. DE-AC52-06NA25396. This research was enabled by computational resources from the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 2 Z9 2 U1 12 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 28 PY 2016 VL 119 IS 20 AR 203301 DI 10.1063/1.4951706 PG 10 WC Physics, Applied SC Physics GA DO3YM UT WOS:000377718700010 ER PT J AU Mosquera, MA Chen, LX Ratner, MA Schatz, GC AF Mosquera, Martin A. Chen, Lin X. Ratner, Mark A. Schatz, George C. TI Sequential double excitations from linear-response time-dependent density functional theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ABSORPTION FINE-STRUCTURE; EXTENDED X-RAY; TRANSIENT ABSORPTION; FOURIER-ANALYSIS; STATE; SPECTROSCOPY AB Traditional UV/vis and X-ray spectroscopies focus mainly on the study of excitations starting exclusively from electronic ground states. However there are many experiments where transitions from excited states, both absorption and emission, are probed. In this work we develop a formalism based on linear-response time-dependent density functional theory to investigate spectroscopic properties of excited states. We apply our model to study the excited-state absorption of a diplatinum(II) complex under X-rays, and transient vis/UV absorption of pyrene and azobenzene. Published by AIP Publishing. C1 [Mosquera, Martin A.; Chen, Lin X.; Ratner, Mark A.; Schatz, George C.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Lemont, IL 60439 USA. RP Schatz, GC (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM g-schatz@northwestern.edu OI Mosquera, Martin/0000-0003-2170-5651; Schatz, George/0000-0001-5837-4740 FU Ultrafast Initiative of the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, through Argonne National Laboratory [DE-AC02-06CH11357]; DOE [DOE DE-FG02-10ER16153] FX We acknowledge support for this work from the Ultrafast Initiative of the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, through Argonne National Laboratory under Contract No. DE-AC02-06CH11357. For vis-UV development we acknowledge the DOE, under Grant No. DOE DE-FG02-10ER16153. M.A.M. is grateful to Carlos Borca, Nicholas Jackson, and Dr. Inkoo Kim and Dr. Amrit Poudel, for productive discussions. NR 23 TC 1 Z9 1 U1 2 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 28 PY 2016 VL 144 IS 20 AR 204105 DI 10.1063/1.4950876 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WI UT WOS:000377712700007 PM 27250277 ER PT J AU Pabit, SA Katz, AM Tolokh, IS Drozdetski, A Baker, N Onufriev, AV Pollack, L AF Pabit, Suzette A. Katz, Andrea M. Tolokh, Igor S. Drozdetski, Aleksander Baker, Nathan Onufriev, Alexey V. Pollack, Lois TI Understanding nucleic acid structural changes by comparing wide-angle x-ray scattering (WAXS) experiments to molecular dynamics simulations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID B-DNA; FORCE-FIELD; A-DNA; PROTEINS; WATER; SAXS; CONDENSATION; ASSOCIATION AB Wide-angle x-ray scattering (WAXS) is emerging as a powerful tool for increasing the resolution of solution structure measurements of biomolecules. Compared to its better known complement, small angle x-ray scattering (SAXS), WAXS targets higher scattering angles and can enhance structural studies of molecules by accessing finer details of solution structures. Although the extension from SAXS to WAXS is easy to implement experimentally, the computational tools required to fully harness the power of WAXS are still under development. Currently, WAXS is employed to study structural changes and ligand binding in proteins; however, the methods are not as fully developed for nucleic acids. Here, we show how WAXS can qualitatively characterize nucleic acid structures as well as the small but significant structural changes driven by the addition of multivalent ions. We show the potential of WAXS to test all-atom molecular dynamics (MD) simulations and to provide insight into understanding how the trivalent ion cobalt(III) hexammine (CoHex) affects the structure of RNA and DNA helices. We find that MD simulations capture the RNA structural change that occurs due to addition of CoHex. Published by AIP Publishing. C1 [Pabit, Suzette A.; Katz, Andrea M.; Pollack, Lois] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Tolokh, Igor S.; Onufriev, Alexey V.] Virginia Tech, Dept Comp Sci, Blacksburg, VA 24061 USA. [Drozdetski, Aleksander; Onufriev, Alexey V.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Baker, Nathan] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Pabit, SA (reprint author), Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. OI Baker, Nathan/0000-0002-5892-6506 FU NIH [R01 GM-099450]; NSF [CNS-0960081]; HokieSpeed supercomputer at Virginia Tech; NSF Graduate Research Fellowship [DGE-1144153]; NSF; NIH/NIGMS via NSF [DMR-1332208]; NIGMS [GM-103485] FX We acknowledge funding support from NIH Grant No. R01 GM-099450 and, in part, by NSF Grant No. CNS-0960081 and the HokieSpeed supercomputer at Virginia Tech. A.M.K. was supported by the NSF Graduate Research Fellowship Grant No. DGE-1144153. We thank Arthur Woll, Steve Meisburger, Huimin Chen, and Pollack Lab Members for experimental assistance. WAXS data were acquired at the Cornell High Energy Synchrotron Source (CHESS). CHESS is supported by the NSF and NIH/NIGMS via NSF Award No. DMR-1332208, and the MacCHESS resource is supported by NIGMS Award No. GM-103485. NR 34 TC 2 Z9 2 U1 5 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 28 PY 2016 VL 144 IS 20 AR 205102 DI 10.1063/1.4950814 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WI UT WOS:000377712700060 PM 27250330 ER PT J AU de Souza, GB Serbena, FC Jurelo, AR da Silva, SA Pinheiro, LBLG Dias, FT Mikowski, A Bud'ko, SL Thaler, A Canfield, PC AF de Souza, Gelson B. Serbena, Francisco C. Jurelo, Alcione R. da Silva, Simone A. Pinheiro, Lincoln B. L. G. Dias, Fabio T. Mikowski, Alexandre Bud'ko, Sergey L. Thaler, Alex Canfield, Paul C. TI On the determination of hardness and elastic modulus in BaFe2As2 lamellar-like material SO JOURNAL OF MATERIALS RESEARCH LA English DT Article DE crystal growth; layered; nano-indentation ID MECHANICAL-PROPERTIES; LAYERED SUPERCONDUCTOR; BIOLOGICAL-MATERIALS; FRACTURE-TOUGHNESS; SINGLE-CRYSTALS; NANOSCRATCH AB The mechanical behavior of superconductor lamellar-like BaFe2As2 single crystals was investigated at nanoscale by instrumented indentation. The unique responses of the ab- and a(b)c-crystallographic planes were discussed based on their influence in hardness (H) and elastic modulus (E). The results allowed two main conclusions. (i) The choice of testing parameters strongly affected the scaling of mechanical properties on the lamellar surfaces. Lamellar cracking was the leading mechanism of deformation, featuring a brittle-like behavior and affecting considerably H and E. However, the plastic deformation history allowed different elastic-plastic responses on the ab-plane owing to the compaction of the material. Threshold loads for cracking depended on both loading rate and penetration velocity, pointing out to time-dependent plastic deformation mechanisms. (ii) Proper estimates were achieved for H in multiple loading tests [3.4 GPa for ab- and approximate to 1 GPa for a(b)c-planes], and for E under loads less than 3 mN (approximate to 55 GPa for both planes). C1 [de Souza, Gelson B.; Serbena, Francisco C.; Jurelo, Alcione R.; da Silva, Simone A.] Univ Estadual Ponta Grossa, Dept Phys, BR-84030000 Ponta Grossa, PR, Brazil. [Pinheiro, Lincoln B. L. G.] Inst Fed Sao Paulo, BR-13565905 Sao Carlos, SP, Brazil. [Dias, Fabio T.] Univ Fed Pelotas, Dept Phys, BR-96010900 Pelotas, RS, Brazil. [Mikowski, Alexandre] Univ Fed Santa Catarina, BR-89218035 Joinville, SC, Brazil. [Bud'ko, Sergey L.; Thaler, Alex; Canfield, Paul C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Bud'ko, Sergey L.; Thaler, Alex; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP de Souza, GB (reprint author), Univ Estadual Ponta Grossa, Dept Phys, BR-84030000 Ponta Grossa, PR, Brazil. EM gelsonbs@uepg.br FU CNPq/Brazil [472.746/2013-8]; US Department of Energy Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX The authors thank Prof. Dr. C.M. Lepienski (DEFIS/UFPR) for the use of the instrumented indentation facilities, Prof. Dr. A.L. Chinelatto (DEMA/UEPG) for some of the SEM images, the CME/UFPR for the use of SEM facilities, and C-LABMU/UEPG for the use of AFM. This work was partially financed by CNPq/Brazil under contract no. 472.746/2013-8. Work at the Ames Laboratory was supported by the US Department of Energy Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. NR 34 TC 0 Z9 0 U1 4 U2 7 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAY 28 PY 2016 VL 31 IS 10 BP 1413 EP 1422 DI 10.1557/jmr.2016.166 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA DO4KZ UT WOS:000377752900005 ER PT J AU Filippetto, D Qian, H AF Filippetto, D. Qian, H. TI Design of a high-flux instrument for ultrafast electron diffraction and microscopy SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE ultrafast electron diffraction; high flux; electron sources; femtosecond beams; nanodiffraction; electron coherence ID TEMPORAL RESOLUTION; MOLECULES; DYNAMICS; PULSES; GUN AB We present the design and optimization of a new instrument for ultrafast electron diffraction and imaging. The proposed instrument merges the high peak current and relativistic electron energies of radio-frequency guns, with the high average electron flux of static electron microscopes, extending the beam parameter space achievable with relativistic electrons by many orders of magnitude. An immediate consequence of this work is a broader range of accessible science by using electron probes, enabling techniques as femtosecond nano-diffraction and coherent diffraction imaging, and paving the way to direct observation of ultrafast dynamics in complex and isolated samples, from nanocrystals, to nano/micro droplets and organic molecules. C1 [Filippetto, D.; Qian, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Filippetto, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. EM DFilippetto@lbl.gov FU US Department of Energy [DE-AC02-05CH11231] FX The authors are grateful to F Sannibale, M Zolotorev, P Musumeci, R K Li and H Rasool for fruitful discussions. We also would like to acknowledge R Wells for his suggestions and help in the beamline installation, together with all the HiRES installation team, and L Doolittle and G Huang for their insights on LLRF and feedback systems. This work was supported by the US Department of Energy Contract No. DE-AC02-05CH11231. NR 38 TC 1 Z9 1 U1 8 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAY 28 PY 2016 VL 49 IS 10 AR 104003 DI 10.1088/0953-4075/49/10/104003 PG 12 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DN0KW UT WOS:000376753800006 ER PT J AU Fears, TM Doucet, M Browning, JF Baldwin, JKS Winiarz, JG Kaiser, H Taub, H Sacci, RL Veith, GM AF Fears, T. M. Doucet, M. Browning, J. F. Baldwin, J. K. S. Winiarz, J. G. Kaiser, H. Taub, H. Sacci, R. L. Veith, G. M. TI Evaluating the solid electrolyte interphase formed on silicon electrodes: a comparison of ex situ X-ray photoelectron spectroscopy and in situ neutron reflectometry SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID LITHIUM-ION BATTERIES; FLUORINATED ELECTROLYTES; DIFFRACTION; CHEMISTRY; LITHIATION; STABILITY; SOLVENTS; ANODE; FILM; MORPHOLOGY AB This work details the in situ characterization of the interface between a silicon electrode and an electrolyte using a linear fluorinated solvent molecule, 0.1 M lithium bis(trifluoromethanesulfonyl) imide (LiTFSI) in deuterated dimethyl perfluoroglutarate (d(6)-PF5M(2)) (1.87 x 10(-2) mS cm(-1)). The solid electrolyte interphase (SEI) composition and thickness determined via in situ neutron reflectometry (NR) and ex situ X-ray photoelectron spectroscopy (XPS) were compared. The data show that SEI expansion and contraction (breathing) during electrochemical cycling were observed via both techniques; however, ex situ XPS suggests that the SEI thickness increases during Si lithiation and decreases during delithiation, while in situ NR suggests the opposite. The most likely cause of this discrepancy is the selective removal of SEI components (top 20 nm of the SEI) during the electrode rinse process, which is required to remove the electrolyte residue prior to ex situ analysis, demonstrating the necessity of performing SEI characterization in situ. C1 [Fears, T. M.; Winiarz, J. G.] Missouri Univ Sci & Technol, Dept Chem, 400 W 11th St, Rolla, MO 65409 USA. [Doucet, M.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Browning, J. F.] Oak Ridge Natl Lab, Dept Chem & Mat Engn, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Baldwin, J. K. S.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Kaiser, H.] Univ Missouri, Res Reactor, 1513 Res Pk Dr, Columbia, MO 65211 USA. [Taub, H.] Univ Missouri, Dept Phys & Astron, Columbia, MO 65211 USA. [Sacci, R. L.; Veith, G. M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Fears, T. M.] US DOE, Oak Ridge Natl Lab, Off Sci Grad Student Res Program Fellow, Washington, DC 20585 USA. RP Fears, TM (reprint author), Missouri Univ Sci & Technol, Dept Chem, 400 W 11th St, Rolla, MO 65409 USA.; Doucet, M (reprint author), Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.; Browning, JF (reprint author), Oak Ridge Natl Lab, Dept Chem & Mat Engn, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA.; Veith, GM (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM fears1@llnl.gov; doucetm@ornl.gov; browningjf@ornl.gov; veithgm@ornl.gov RI Doucet, Mathieu/A-5333-2010; Fears, Tyler/L-1338-2016 OI Doucet, Mathieu/0000-0002-5560-6478; Fears, Tyler/0000-0001-8648-7582 FU U.S. National Science Foundation [DGE-1069091]; DOE [DE-AC05-06OR23100]; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; UT-Battelle, LLC; Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (RLS - Conductivity, ATR-IR); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; UT-Battelle, LLC [DEAC05-00OR22725]; U.S. Department of Energy; Department of Energy; DOE Public Access Plan FX Student support and materials for ester synthesis and scattering profiles are provided by the U.S. National Science Foundation under Grant No. DGE-1069091. Student support for the electrochemical, XPS, and ATR-IR studies performed at Oak Ridge National Laboratory provided by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists, Office of Science Graduate Student Research (SCGSR) program is acknowledged. The SCGSR program is administered by the Oak Ridge Institute for Science and Education for the DOE under contract number DE-AC05-06OR23100. The equipment, materials and technical guidance at ORNL, was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy under contract with UT-Battelle, LLC (GMV - XPS, ATR-IR, electrochemical) and the Fluid Interface Reactions, Structures, and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (RLS - Conductivity, ATR-IR). Neutron reflectometry measurements were carried out on the Liquids Reflectometer at the Spallation Neutron Source which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (J. F. B., M. D., Data collection and analysis). Sample preparation (J. K. B.) was performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. This manuscript has been authored by UT-Battelle, LLC under Contract No. DEAC05-00OR22725 with the U.S. Department of Energy. By accepting this article, the publisher acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). T. M. F. would like to thank Dr C. Sotiriou-Leventis for help in formulating the perfluorocarboxylate ester synthesis. NR 43 TC 0 Z9 0 U1 19 U2 53 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAY 28 PY 2016 VL 18 IS 20 BP 13927 EP 13940 DI 10.1039/c6cp00978f PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN4MW UT WOS:000377042400022 PM 27149427 ER PT J AU Boyle, TJ Neville, ML Parkes, MV AF Boyle, Timothy J. Neville, Michael L. Parkes, Marie V. TI Synthesis and characterization of a series of Group 4 phenoxy-thiol derivatives SO POLYHEDRON LA English DT Article DE Alkoxides; Thiols; Titanium; Zirconium; Hafnium ID EFFECTIVE CORE POTENTIALS; DENSITY-FUNCTIONAL THEORY; MOLECULAR-ORBITAL METHODS; ELECTRONIC-STRUCTURE; ALKOXIDES; POLYMERIZATION; APPROXIMATION; NANOPARTICLES; COMPLEXES; ENERGIES AB A series of Group 4 phenoxy-thiols were developed from the reaction products of a series of metal tertbutoxides ([M(OBut)(4)]) with four equivalents of 4-mercaptophenol (H-4MP). The products were found by single crystal X-ray diffraction to adopt the general structure [(HOBut)(4MP)(3)M(mu-MP)](2) [where M = Ti (1), Zr (2), Hf (3)] from toluene and [(py)(2)M(4MP)] where M = Ti (4), Zr (5) and [(py)(4MP)(3)Hf (mu-4MP)](2) (6) from pyridine (py). Varying the [Ti(OR)(4)] precursors (OR = iso-propoxide (OPri) or neo-pentoxide (ONep)) in toluene led to [(HOR)(4MP)(3)Ti(mu-4MP)](2) (OR = OPri (7), ONep (8)), which were structurally similar to 1. Lower stoichiometric reactions in toluene led to partial substitution by the 4MP ligands yielding [H][Ti(mu-4MP)(4MP)(ONep)(3)](2) (9). Independent of the stoichiometry, all of the Ti derivatives were found to be red in color, whereas the heavier congeners were colorless. Attempts to understand this phenomenon led to investigation with a series of varied-SH substituted phenols. From the reaction of H-2MP and H-3MP (2-mercaptophenol and 3-mercaptophenol, respectively), the isolated products had identical arrangements: [(ONep)(2)(2MP)Ti(mu,eta(2)-2MP)](2) (10) and [(HOR)(3MP)M(mu-3MP)](2) (M/OR=Ti/ONep (11); Zr/OBut (12)) with a similar red color. Based on the simulated and observed UV-Vis spectra, it was reasoned that the color was generated due to a ligand-to-metal charge transfer for Ti that was not available for the larger congeners. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Boyle, Timothy J.; Neville, Michael L.; Parkes, Marie V.] Sandia Natl Labs, Adv Mat Lab, 1001 Univ Blvd SE, Albuquerque, NM 87106 USA. [Neville, Michael L.] Univ Calif San Diego, Dept Chem, 9500 Gilman Dr, La Jolla, CA USA. [Parkes, Marie V.] Sandia Natl Labs, Geochem Dept, POB 5800, Albuquerque, NM 87185 USA. RP Boyle, TJ (reprint author), Sandia Natl Labs, Adv Mat Lab, 1001 Univ Blvd SE, Albuquerque, NM 87106 USA. EM tjboyle@Sandia.gov FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; National Science Foundation CRIF:MU award [CHE04-43580]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Mr. J. M. Sears (Sandia) for technical assistance, the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories for support of this program, and the use of the Bruker X-ray diffractometer purchased via the National Science Foundation CRIF:MU award to Prof Kemp of the University of New Mexico (CHE04-43580). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 39 TC 0 Z9 0 U1 7 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD MAY 28 PY 2016 VL 110 BP 1 EP 13 DI 10.1016/j.poly.2016.02.019 PG 13 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DL3FF UT WOS:000375518900001 ER PT J AU Liu, X Gonzalez-Castro, A Mutikainen, I Pevec, A Teat, SJ Gamez, P Costa, JS Bouwman, E Reedijk, J AF Liu, Xue Gonzalez-Castro, Adriana Mutikainen, Ilpo Pevec, Andrej Teat, Simon J. Gamez, Patrick Costa, Jose Sanchez Bouwman, Elisabeth Reedijk, Jan TI Zinc and cadmium halide compounds with the tridentate ligand 2-(methylsulfanyl)-N-(pyridin-2-ylmethylidene)aniline showing yellow luminescence SO POLYHEDRON LA English DT Article DE Zinc(II); Cadmium(II); Chloride; Bromide; Luminescence ID SCHIFF-BASE COMPLEXES; METAL-COMPLEXES; CRYSTAL; BEHAVIOR; ZN(II); SENSOR; IONS AB Five mononuclear complexes, i.e. ZnLCl2 (1), [ZnLBr2](CH3CN) (2), ZnLBr2 (3), CdLCl2 (4), and CdLBr2 (5), with L = 2-(methylsulfany1)-N-(pyridin-2-ylmethylidene)aniline, have been synthesized and characterized. For [ZnLBr2](CH3CN) only a few crystals were obtained from the main batch of ZnLBr2. Their crystal structures and solid-state luminescence properties both at room temperature and 77 K have been investigated. All compounds contain 5-coordinated Zn(II) or Cd(II) ions in a square-pyramidal geometry, distorted towards trigonal bipyramidal. The phase purity of all compounds has been evaluated by Powder XRD and IR. All five compounds show photoluminescent properties both at room temperature and 77 K. In the solid state, the compounds exhibit yellow luminescence with the maximum of emission at around 540 nm. By cooling down to 77 K, the shape and position of the emission spectra of all these compounds remains more or less constant. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Liu, Xue; Gonzalez-Castro, Adriana; Gamez, Patrick; Costa, Jose Sanchez; Bouwman, Elisabeth; Reedijk, Jan] Leiden Univ, Leiden Inst Chem, Gorlaeus Labs, POB 9502, NL-2300 RA Leiden, Netherlands. [Mutikainen, Ilpo] Univ Helsinki, Dept Chem, POB 55 AI Virtasenaukio 1, FI-00014 Helsinki, Finland. [Pevec, Andrej] Univ Ljubljana, Fac Chem & Chem Technol, Vecna Pot 113, Ljubljana, Slovenia. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Gamez, Patrick] Catalan Inst Res & Adv Studies ICREA, Passeig Lluis Co 23, Barcelona 08010, Spain. [Costa, Jose Sanchez] IMDEA Nanosci C Faraday 9, Campus Cantoblanco, Madrid 28049, Spain. RP Bouwman, E (reprint author), Leiden Univ, Leiden Inst Chem, Gorlaeus Labs, POB 9502, NL-2300 RA Leiden, Netherlands. EM bouwman@chem.leidenuniv.nl RI Gamez, Patrick/B-3610-2012; Bouwman, Elisabeth/D-1637-2010; Sanchez Costa, Jose/N-9085-2014 OI Gamez, Patrick/0000-0003-2602-9525; Bouwman, Elisabeth/0000-0001-7762-3968; Sanchez Costa, Jose/0000-0001-5426-7956 FU Chinese Scholarship Council [201206250014]; Slovenian Research Agency [P1-0175]; U.S. Department of Energy [DE-AC02-05CH11231] FX X. Liu gratefully acknowledges a grant from the Chinese Scholarship Council (no. 201206250014). Andrej Pevec thanks the Slovenian Research Agency for support (Grant P1-0175). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 2 Z9 2 U1 2 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD MAY 28 PY 2016 VL 110 BP 100 EP 105 DI 10.1016/j.poly.2016.02.030 PG 6 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DL3FF UT WOS:000375518900012 ER PT J AU Ching, J Zaveri, RA Easter, RC Riemer, N Fast, JD AF Ching, Joseph Zaveri, Rahul A. Easter, Richard C. Riemer, Nicole Fast, Jerome D. TI A three-dimensional sectional representation of aerosol mixing state for simulating optical properties and cloud condensation nuclei SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID SOURCE-ORIENTED MODEL; BLACK CARBON; LABORATORY EVALUATION; COMBUSTION AEROSOLS; CLIMATE MODELS; WRF-CHEM; ON-ROAD; PART 2; SIZE; EMISSIONS AB Light absorption by black carbon (BC) particles emitted from fossil fuel combustion depends on their size and how thickly they are coated with nonrefractory species such as ammonium, sulfate, nitrate, organics, and water. The cloud condensation nuclei (CCN) activation behavior of a particle depends on its dry size and the hygroscopicities of all the individual species mixed together. It is therefore necessary to represent both size and mixing state of aerosols to reliably predict their climate-relevant properties in atmospheric models. Here we describe and evaluate a novel sectional framework in the Model for Simulating Aerosol Interactions and Chemistry (box model), referred to as MOSAIC-mix, that represents the mixing state by resolving aerosol dry size (D-dry), BC dry mass fraction (w(BC)), and hygroscopicity (k). Using 10 idealized urban plume scenarios in which different types of aerosols evolve over 24 h under a range of atmospherically relevant conditions, we examine errors in CCN concentrations and optical properties with respect to the level of detail of the aerosol mixing state representation. We find that a small number of wBC and k bins can achieve significant reductions in the errors and propose a configuration with 24 D-dry bins, 2 w(BC) bins, and 2 k bins that give average errors of about 5% or less in CCN concentrations and optical properties, 3-4 times lower than those from size-only resolved (i.e., internally mixed) simulations. These results suggest that MOSAIC-mix is suitable for use in regional and global models to examine the effects of mixing state on aerosol-radiation-cloud feedbacks. C1 [Ching, Joseph; Zaveri, Rahul A.; Easter, Richard C.; Fast, Jerome D.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Riemer, Nicole] Univ Illinois, Dept Atmospher Sci, Urbana, IL USA. RP Ching, J; Zaveri, RA (reprint author), Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM pingpui.ching@pnnl.gov; rahul.zaveri@pnnl.gov FU U.S. Department of Energy (DOE) under Atmospheric System Research (ASR) program of the Office of Science; DOE [DE-AC05-76RL01830]; DOE ASR grant [DE-SC0011771] FX We thank Elaine Chapman at PNNL for reviewing the manuscript. This research was supported by the U.S. Department of Energy (DOE) under the auspices of the Atmospheric System Research (ASR) program of the Office of Science. Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. Nicole Riemer acknowledges funding from DOE ASR grant DE-SC0011771. Model output data can be obtained by contacting Joseph Ching (pingpui.ching@pnnl.gov) or Rahul Zaveri (rahul.zaveri@pnnl.gov). NR 62 TC 0 Z9 0 U1 11 U2 13 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 27 PY 2016 VL 121 IS 10 BP 5912 EP 5929 DI 10.1002/2015JD024323 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DT6YB UT WOS:000381629900048 ER PT J AU Ching, J Riemer, N West, M AF Ching, J. Riemer, N. West, M. TI Black carbon mixing state impacts on cloud microphysical properties: Effects of aerosol plume and environmental conditions SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID ATMOSPHERIC AEROSOLS; SPECTRAL DISPERSION; OPTICAL-PROPERTIES; DROPLET FORMATION; EFFECTIVE RADIUS; CLIMATE MODELS; PARAMETERIZATION; CONDENSATION; CCN; STRATOCUMULUS AB Black carbon (BC) is usually mixed with other aerosol species within individual aerosol particles. This mixture, along with the particles' size and morphology, determines the particles' optical and cloud condensation nuclei properties, and hence black carbon's climate impacts. In this study, the particle-resolved aerosol model PartMC-MOSAIC (Particle Monte Carlo-Model for Simulating Aerosol Interactions and Chemistry) was used to quantify the importance of black carbon mixing state for predicting cloud microphysical quantities. Based on a set of about 100 cloud parcel simulations a process-level analysis framework was developed to attribute the response in cloud microphysical properties to changes in the underlying aerosol population ("plume effect") and the cloud parcel cooling rate ("parcel effect"). In most of the simulations the plume and parcel effects had opposite signs, with the plume effect dominating. The response of cloud droplet number concentration to changes in BC emissions depended on the BC mixing state. When the aerosol population contained mainly aged BC, an increase in BC emission increased cloud droplet number concentrations ("additive effect"). In contrast, when the aerosol population contained mainly fresh BC particles, they act as sinks for condensable gaseous species, resulting in decreasing cloud droplet number concentration as BC emissions were increased ("competition effect"). Additionally, we quantified the error in cloud microphysical quantities when neglecting the information on BC mixing state. The errors ranged from -12% to +45% for the cloud droplet number fraction, from 0% to +1022% for the nucleation-scavenged BC mass fraction, from -12% to +4% for the effective radius, and from -30% to +60% for the relative dispersion. C1 [Ching, J.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA USA. [Riemer, N.] Univ Illinois, Dept Atmospher Sci, Urbana, IL 61801 USA. [West, M.] Univ Illinois, Dept Mech Sci & Engn, Urbana, IL USA. RP Riemer, N (reprint author), Univ Illinois, Dept Atmospher Sci, Urbana, IL 61801 USA. EM nriemer@illinois.edu OI West, Matthew/0000-0002-7605-0050 FU National Science Foundation [NSF ATM 07-39404, NSF ATM 09-34491]; U.S. Department of Energy, Office of Science, Biological and Environmental Research as part of the Atmospheric System Research program [DE-SC0003921, DE-SC0011771]; DOE [DE-AC05-76RL01830] FX The authors acknowledge funding from the National Science Foundation under grants NSF ATM 07-39404 and NSF ATM 09-34491. A portion of this research was supported by the U.S. Department of Energy, Office of Science, Biological and Environmental Research as part of the Atmospheric System Research program under grants DE-SC0003921 and DE-SC0011771. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. Model output data can be obtained by contacting N. Riemer (nriemer@illinois.edu). NR 59 TC 0 Z9 0 U1 10 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 27 PY 2016 VL 121 IS 10 BP 5990 EP 6013 DI 10.1002/2016JD024851 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DT6YB UT WOS:000381629900052 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Beringer, J Berlendis, S Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertram, IA Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Broughton, JH de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, BH Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Camplani, A Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, I Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavallaro, E Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chan, SK Chan, YL Chang, P Chapman, JD Charlton, DG Chatterjee, A Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, S Chen, S Chen, X Cheng, HC Cheng, HJ Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chitan, A Chizhov, MV Choi, K Chomont, AR Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, MR Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cormier, KJR Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dado, T Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Dann, NS Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, M Davison, P Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Denysiuk, D Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Clemente, WK Di Donato, C Di Girolamo, A Di Girolamo, B Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Du, Y Duarte-Campderros, J Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dumancic, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dutta, B Dyndal, M Eckardt, C Ecker, KM Edgar, RC Edwards, NC Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellajosyula, V Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Ennis, JS Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, F Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farina, C Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fawcett, WJ Fayard, L Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiedler, F Filipcic, A Filipuzzi, M Filthaut, F Fincke-Keeler, M Finelli, KD Fiolhais, MCN Fiorini, L Firan, A Fischer, A Fischer, C Fischer, J Fisher, WC Flaschel, N Fleck, I Fleischmann, P Fletcher, GT Fletcher, RRM Flick, T Floderus, A Castillo, LRF Flowerdew, MJ Forcolin, GT Formica, A Forti, A Foster, AG Fournier, D Fox, H Fracchia, S Francavilla, P Franchini, M Francis, D Franconi, L Franklin, M Frate, M Fraternali, M Freeborn, D Fressard-Batraneanu, SM Friedrich, F Froidevaux, D Frost, JA Fukunaga, C Torregrosa, EF Fusayasu, T Fuster, J Gabaldon, C Gabizon, O Gabrielli, A Gabrielli, A Gach, GP Gadatsch, S Gadomski, S Gagliardi, G Gagnon, LG Gagnon, P Galea, C Galhardo, B Gallas, EJ Gallop, BJ Gallus, P Galster, G Gan, KK Gao, J Gao, Y Gao, YS Walls, FMG Garcia, C Navarro, JEG Garcia-Sciveres, M Gardner, RW Garelli, N Garonne, V Bravo, AG Gatti, C Gaudiello, A Gaudio, G Gaur, B Gauthier, L Gavrilenko, IL Gay, C Gaycken, G 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Greenwood, ZD Grefe, C Gregersen, K Gregor, IM Grenier, P Grevtsov, K Griffiths, J Grillo, AA Grimm, K Grinstein, S Gris, P Grivaz, JF Groh, S Grohs, JP Gross, E Grosse-Knetter, J Grossi, GC Grout, ZJ Guan, L Guan, W Guenther, J Guescini, F Guest, D Gueta, O Guido, E Guillemin, T Guindon, S Gul, U Gumpert, C Guo, J Guo, Y Gupta, S Gustavino, G Gutierrez, P Ortiz, NGG Gutschow, C Guyot, C Gwenlan, C Gwilliam, CB Haas, A Haber, C Hadavand, HK Haddad, N Hadef, A Haefner, P Hagebock, S Hajduk, Z Hakobyan, H Haleem, M Haley, J Halladjian, G Hallewell, GD Hamacher, K Hamal, P Hamano, K Hamilton, A Hamity, GN Hamnett, PG Han, L Hanagaki, K Hanawa, K Hance, M Haney, B Hanke, P Hanna, R Hansen, JB Hansen, JD Hansen, MC Hansen, PH Hara, K Hard, AS Harenberg, T Hariri, F Harkusha, S Harrington, RD Harrison, PF Hartjes, F Hasegawa, M Hasegawa, Y Hasib, A Hassani, S Haug, S Hauser, R Hauswald, L Havranek, M Hawkes, CM Hawkings, RJ Hawkins, AD Hayden, D Hays, CP Hays, JM Hayward, HS Haywood, SJ 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T Konoplich, R Konstantinidis, N Kopeliansky, R Koperny, S Kopke, L Kopp, AK Korcyl, K Kordas, K Korn, A Korol, AA Korolkov, I Korolkova, EV Kortner, O Kortner, S Kosek, T Kostyukhin, VV Kotwal, A Kourkoumeli-Charalampidi, A Kourkoumelis, C Kouskoura, V Kowalewska, AB Kowalewski, R Kowalski, TZ Kozanecki, W Kozhin, AS Kramarenko, VA Kramberger, G Krasnopevtsev, D Krasny, MW Krasznahorkay, A Kraus, JK Kravchenko, A Kretz, M Kretzschmar, J Kreutzfeldt, K Krieger, P Krizka, K Kroeninger, K Kroha, H Kroll, J Kroseberg, J Krstic, J Kruchonak, U Kruger, H Krumnack, N Kruse, A Kruse, MC Kruskal, M Kubota, T Kucuk, H Kuday, S Kuechler, JT Kuehn, S Kugel, A Kuger, F Kuhl, A Kuhl, T Kukhtin, V Kukla, R Kulchitsky, Y Kuleshov, S Kuna, M Kunigo, T Kupco, A Kurashige, H Kurochkin, YA Kus, V Kuwertz, ES Kuze, M Kvita, J Kwan, T Kyriazopoulos, D La Rosa, A Navarro, JLL La Rotonda, L Lacasta, C Lacava, F Lacey, J Lacker, H Lacour, D Lacuesta, VR Ladygin, E Lafaye, R Laforge, B Lagouri, T Lai, S 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Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Ya, Y. C. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for the Standard Model Higgs boson decaying into b(b)over-bar produced in association with top quarks decaying hadronically in pp collisions at root s=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments) ID MONTE-CARLO; PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; PAIR; LHC; NLO; CONSTRAINTS; COLLIDERS AB A search for Higgs boson production in association with a pair of top quarks (t (t) over barH) is performed, where the Higgs boson decays to b (b) over bar, and both top quarks decay hadronically. The data used correspond to an integrated luminosity of 20.3 fb(-1) of pp collisions at root s = 8 TeV collected with the ATLAS detector at the Large Hadron Collider. The search selects events with at least six energetic jets and uses a boosted decision tree algorithm to discriminate between signal and Standard Model background. The dominant multijet background is estimated using a dedicated data-driven technique. For a Higgs boson mass of 125 GeV, an upper limit of 6.4 (5.4) times the Standard Model cross section is observed (expected) at 95% confidence level. The best-fit value for the signal strength is mu = 1.6 +/- 2.6 times the Standard Model expectation for m(H) = 125 GeV. Combining all t (t) over barH searches carried out by ATLAS at root s = 8 and 7 TeV, an observed (expected) upper limit of 3.1 (1.4) times the Standard Model expectation is obtained at 95% confidence level, with a signal strength mu = 1.7 +/- 0.8. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. 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H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ruiz-Martinez, A.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Starz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheplakov, A.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Tapia Araya, S.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, Y.; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Huainan, Anhui, Peoples R China. [Chen, S.; Guo, J.; Yang, H.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Li, L.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Bret, M. Cano; Li, L.] PKU CHEP, Beijing 100084, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN Grp Collegato Cosenza, Lab Nazl Frascati, I-87036 Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; de Lima, D. E. Ferreira; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheremushkina, E.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Cheng, H. C.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Ya, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Ya, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Ya, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. J.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Li, B.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, INFN Sez Milano, Milan, Italy. [Andreazza, A.; Camplani, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Ducu, O. A.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Nguyen Manh, T.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Igonkina, O.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris Saclay, Univ Paris 11, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, P-3000 Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; El Moursli, R. Cherkaoui; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, INFN Sez Roma, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Univ Rome Tre, INFN Sez Roma Tre, I-00146 Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univ, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Dado, T.; Melo, M.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellm, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellm, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Hod, N.; Jovicevic, J.; Oakham, F. G.; Codina, E. Perez; Savard, P.; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; McPherson, R. A.; Pearce, J.; Seuster, R.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Dumancic, M.; Gross, E.; Kohler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kuechler, J. T.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Vogel, M.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachgrp Phys, Fak Mathemat & Naturwissensch, Wuppertal, Germany. [Baker, O. K.; Noccioli, E. Benhar; Cummings, J.; Demers, S.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Vasquez, J. G.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Banerjee, Sw.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Castro, N. F.; McPherson, R. A.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Victoria, BC, Canada. [Ducu, O. A.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Govender, N.] Ctr High Performance Comp, CSIR Campus, Cape Town, South Africa. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellenic Open Univ, Patras, Greece. [Lin, S. C.; Myagkov, A. G.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pasztor, G.] Eotvos Lorand Univ, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS IN2P3, Marseille, France. RI Garcia, Jose /H-6339-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Lazzaroni, Massimo/N-3675-2015; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Shulga, Evgeny/R-1759-2016; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Gladilin, Leonid/B-5226-2011; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Carvalho, Joao/M-4060-2013; Warburton, Andreas/N-8028-2013; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016; Mitsou, Vasiliki/D-1967-2009 OI Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Lazzaroni, Massimo/0000-0002-4094-1273; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Shulga, Evgeny/0000-0001-5099-7644; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Gladilin, Leonid/0000-0001-9422-8636; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Carvalho, Joao/0000-0002-3015-7821; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620; Mitsou, Vasiliki/0000-0002-1533-8886 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, Region Auvergne and Fondation Partager le Savoir, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 82 TC 1 Z9 1 U1 20 U2 51 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 27 PY 2016 IS 5 AR 160 DI 10.1007/JHEP05(2016)160 PG 51 WC Physics, Particles & Fields SC Physics GA DO2II UT WOS:000377602900001 ER PT J AU Abbott, D Adderley, P Adeyemi, A Aguilera, P Ali, M Areti, H Baylac, M Benesch, J Bosson, G Cade, B Camsonne, A Cardman, LS Clark, J Cole, P Covert, S Cuevas, C Dadoun, O Dale, D Dong, H Dumas, J Fanchini, E Forest, T Forman, E Freyberger, A Froidefond, E Golge, S Grames, J Gueye, P Hansknecht, J Harrell, P Hoskins, J Hyde, C Josey, B Kazimi, R Kim, Y Machie, D Mahoney, K Mammei, R Marton, M McCarter, J McCaughan, M McHugh, M McNulty, D Mesick, KE Michaelides, T Michaels, R Moffit, B Moser, D Camacho, CM Muraz, JF Opper, A Poelker, M Real, JS Richardson, L Setiniyaz, S Stutzman, M Suleiman, R Tennant, C Tsai, C Turner, D Ungaro, M Variola, A Voutier, E Wang, Y Zhang, Y AF Abbott, D. Adderley, P. Adeyemi, A. Aguilera, P. Ali, M. Areti, H. Baylac, M. Benesch, J. Bosson, G. Cade, B. Camsonne, A. Cardman, L. S. Clark, J. Cole, P. Covert, S. Cuevas, C. Dadoun, O. Dale, D. Dong, H. Dumas, J. Fanchini, E. Forest, T. Forman, E. Freyberger, A. Froidefond, E. Golge, S. Grames, J. Gueye, P. Hansknecht, J. Harrell, P. Hoskins, J. Hyde, C. Josey, B. Kazimi, R. Kim, Y. Machie, D. Mahoney, K. Mammei, R. Marton, M. McCarter, J. McCaughan, M. McHugh, M. McNulty, D. Mesick, K. E. Michaelides, T. Michaels, R. Moffit, B. Moser, D. Camacho, C. Munoz Muraz, J-F Opper, A. Poelker, M. Real, J-S Richardson, L. Setiniyaz, S. Stutzman, M. Suleiman, R. Tennant, C. Tsai, C. Turner, D. Ungaro, M. Variola, A. Voutier, E. Wang, Y. Zhang, Y. CA PEPPo Collaboration TI Production of Highly Polarized Positrons Using Polarized Electrons at MeV Energies SO PHYSICAL REVIEW LETTERS LA English DT Article AB The Polarized Electrons for Polarized Positrons experiment at the injector of the Continuous Electron Beam Accelerator Facility has demonstrated for the first time the efficient transfer of polarization from electrons to positrons produced by the polarized bremsstrahlung radiation induced by a polarized electron beam in a high-Z target. Positron polarization up to 82% have been measured for an initial electron beam momentum of 8.19 MeV/c, limited only by the electron beam polarization. This technique extends polarized positron capabilities from GeV to MeV electron beams, and opens access to polarized positron beam physics to a wide community. C1 [Abbott, D.; Adderley, P.; Aguilera, P.; Ali, M.; Areti, H.; Benesch, J.; Cade, B.; Camsonne, A.; Cardman, L. S.; Clark, J.; Covert, S.; Cuevas, C.; Dong, H.; Dumas, J.; Forman, E.; Freyberger, A.; Grames, J.; Hansknecht, J.; Harrell, P.; Kazimi, R.; Kim, Y.; Machie, D.; Mahoney, K.; Mammei, R.; McCaughan, M.; Michaelides, T.; Michaels, R.; Moffit, B.; Moser, D.; Poelker, M.; Richardson, L.; Stutzman, M.; Suleiman, R.; Tennant, C.; Turner, D.; Ungaro, M.; Wang, Y.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Baylac, M.; Bosson, G.; Dumas, J.; Fanchini, E.; Froidefond, E.; Marton, M.; Muraz, J-F; Real, J-S; Voutier, E.] Univ Grenoble Alpes, CNRS IN2P3, LPSC, F-38026 Grenoble, France. [Adeyemi, A.; Gueye, P.] Hampton Univ, Hampton, VA 23668 USA. [Cole, P.; Dale, D.; Forest, T.; Kim, Y.; McNulty, D.; Setiniyaz, S.] Idaho State Univ, Pocatello, ID 83209 USA. [Dadoun, O.; Variola, A.] Univ Paris 11, LAL, F-91898 Orsay, France. [Dadoun, O.; Variola, A.] Univ Paris Saclay, CNRS IN2P3, F-91898 Orsay, France. [Camacho, C. Munoz; Voutier, E.] Univ Paris 11, IPN, F-91406 Orsay, France. [Camacho, C. Munoz; Voutier, E.] Univ Paris Saclay, CNRS IN2P3, F-91406 Orsay, France. [Golge, S.] N Carolina Cent Univ, Durham, NC 27707 USA. [Hyde, C.] Old Dominion Univ, Norfolk, VA 23529 USA. [Mesick, K. E.; Zhang, Y.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Hoskins, J.] Coll William & Mary, Williamsburg, VA 23187 USA. [McCarter, J.] Univ Virginia, Charlottesville, VA 22901 USA. [Tsai, C.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Josey, B.] Univ New Mexico, Albuquerque, NM 87131 USA. [McHugh, M.; Opper, A.] George Washington Univ, Washington, DC 20052 USA. RP Voutier, E (reprint author), Univ Grenoble Alpes, CNRS IN2P3, LPSC, F-38026 Grenoble, France.; Voutier, E (reprint author), Univ Paris 11, IPN, F-91406 Orsay, France.; Voutier, E (reprint author), Univ Paris Saclay, CNRS IN2P3, F-91406 Orsay, France. EM voutier@ipno.in2p3.fr OI Mesick, Katherine/0000-0001-6138-1474 FU U.S. Department of Energy; French Centre National de la Recherche Scientifique; International Linear Collider RD program; DOE [DE-AC05-06OR23177] FX We are deeply grateful to the SLAC E-166 Collaboration, particularly K. Laihem, K. McDonald, S. Riemann, A. Schalicke, P. Schuler, J. Sheppard, and A. Stahl for loan of fundamental equipment parts and support in GEANT4 modeling. We also thank N. Smirnov for delivery of critical hardware. This work was supported in part by the U.S. Department of Energy, the French Centre National de la Recherche Scientifique, and the International Linear Collider R&D program. Jefferson Science Associates operates the Thomas Jefferson National Accelerator Facility under DOE Contract No. DE-AC05-06OR23177. NR 21 TC 0 Z9 0 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 27 PY 2016 VL 116 IS 21 AR 214801 DI 10.1103/PhysRevLett.116.214801 PG 5 WC Physics, Multidisciplinary SC Physics GA DM8QK UT WOS:000376628800007 PM 27284661 ER PT J AU Wakeham, N Bauer, ED Neupane, M Ronning, F AF Wakeham, N. Bauer, E. D. Neupane, M. Ronning, F. TI Large magnetoresistance in the antiferromagnetic semimetal NdSb SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-PROPERTIES; PHASE; FIELD AB There has been considerable interest in topological semimetals that exhibit extreme magnetoresistance (XMR). These have included materials lacking inversion symmetry such as TaAs, as well Dirac semimetals such as Cd3As2. However, it was reported recently that LaSb and LaBi also exhibit XMR, even though the rocksalt structure of these materials has inversion symmetry, and the band-structure calculations do not show a Dirac dispersion in the bulk. Here, we present magnetoresistance and specific-heat measurements on NdSb, which is isostructural with LaSb. NdSb has an antiferromagnetic ground state and, in analogy with the lanthanum monopnictides, is expected to be a topologically nontrivial semimetal. We show that NdSb has an XMR of similar to 10(4)%, even within the antiferromagnetic state, illustrating that XMR can occur independently of the absence of time-reversal symmetry breaking in zero magnetic field. The persistence of XMR in a magnetic system offers the promise of new functionality when combining topological matter with electronic correlations. We also find that in an applied magnetic field below the Neel temperature there is a first-order transition, consistent with evidence from previous neutron scattering work. C1 [Wakeham, N.; Bauer, E. D.; Ronning, F.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Neupane, M.] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. RP Wakeham, N (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU U.S. Department of Energy, Office of Science; Los Alamos National Laboratory LDRD program FX We thank Y. Luo for many helpful discussions. Synthesis and measurements of the crystals were performed under the auspices of the U.S. Department of Energy, Office of Science. Electronic structure calculations were performed with the support of the Los Alamos National Laboratory LDRD program. NR 27 TC 0 Z9 0 U1 20 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 27 PY 2016 VL 93 IS 20 AR 205152 DI 10.1103/PhysRevB.93.205152 PG 5 WC Physics, Condensed Matter SC Physics GA DM8UC UT WOS:000376639000004 ER PT J AU Searcy, J Huang, LL Pleier, MA Zhu, JJ AF Searcy, Jacob Huang, Lillian Pleier, Marc-Andre Zhu, Junjie TI Determination of the WW polarization fractions in pp -> W-+/- W(+/-)jj using a deep machine learning technique SO PHYSICAL REVIEW D LA English DT Article ID HIGGS-BOSON MASS; WEAK INTERACTIONS; HIGH-ENERGIES; PARTICLE; PHYSICS; LHC AB The unitarization of the longitudinal vector boson scattering (VBS) cross section by the Higgs boson is a fundamental prediction of the Standard Model which has not been experimentally verified. One of the most promising ways to measure VBS uses events containing two leptonically decaying same-electric-charge W bosons produced in association with two jets. However, the angular distributions of the leptons in the W boson rest frame, which are commonly used to fit polarization fractions, are not readily available in this process due to the presence of two neutrinos in the final state. In this paper we present a method to alleviate this problem by using a deep machine learning technique to recover these angular distributions from measurable event kinematics and demonstrate how the longitudinal-longitudinal scattering fraction could be studied. We show that this method doubles the expected sensitivity when compared to previous proposals. C1 [Searcy, Jacob; Huang, Lillian; Zhu, Junjie] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Pleier, Marc-Andre] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Searcy, J (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. FU U.S. DOE Early Career Grant [DE-SC0008062]; U.S. DOE [DE-SC0012704] FX We would like to thank our colleagues Sally Dawson, Frank Paige, and Olivier Mattelaer for their help and guidance while preparing this manuscript. The contributions from J. S., L. H., and J. Z. are supported by the U.S. DOE Early Career Grant under Contract No. DE-SC0008062. The work of M.-A. P. is supported by U.S. DOE Contract No. DE-SC0012704. We would also like to acknowledge the role of the U.S. ATLAS Scholar program for fostering collaboration between Michigan and Brookhaven National Laboratory. NR 32 TC 0 Z9 0 U1 5 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 27 PY 2016 VL 93 IS 9 AR 094033 DI 10.1103/PhysRevD.93.094033 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8VL UT WOS:000376642500003 ER PT J AU Martin-Albo, J Vidal, JM Ferrario, P Nebot-Guinot, M Gomez-Cadenas, JJ Alvarez, V Azevedo, CDR Borges, FIG Carcel, S Carrion, JV Cebrian, S Cervera, A Conde, CAN Diaz, J Diesburg, M Esteve, R Fernandes, LMP Ferreira, AL Freitas, EDC Goldschmidt, A Gonzalez-Diaz, D Gutierrez, RM Hauptman, J Henriques, CAO Morata, JAH Herrero, V Labarga, L Laing, A Lebrun, P Liubarsky, I Lopez-March, N Lorca, D Losada, M Martinez-Lema, G Martinez, A Monrabal, F Monteiro, CMB Mora, FJ Moutinho, LM Novella, P Nygren, D Palmeiro, B Para, A Querol, M Renner, J Ripoll, L Rodriguez, J Santos, FP dos Santos, JMF Serra, L Shuman, D Simon, A Sofka, C Sorel, M Stiegler, T Toledo, JF Torrent, J Tsamalaidze, Z Veloso, JFCA Webb, R White, JT Yahlali, N Yepes-Ramirez, H AF Martin-Albo, J. Munoz Vidal, J. Ferrario, P. Nebot-Guinot, M. Gomez-Cadenas, J. J. Alvarez, V. Azevedo, C. D. R. Borges, F. I. G. Carcel, S. Carrion, J. V. Cebrian, S. Cervera, A. Conde, C. A. N. Diaz, J. Diesburg, M. Esteve, R. Fernandes, L. M. P. Ferreira, A. L. Freitas, E. D. C. Goldschmidt, A. Gonzalez-Diaz, D. Gutierrez, R. M. Hauptman, J. Henriques, C. A. O. Hernando Morata, J. A. Herrero, V. Labarga, L. Laing, A. Lebrun, P. Liubarsky, I. Lopez-March, N. Lorca, D. Losada, M. Martinez-Lema, G. Martinez, A. Monrabal, F. Monteiro, C. M. B. Mora, F. J. Moutinho, L. M. Novella, P. Nygren, D. Palmeiro, B. Para, A. Querol, M. Renner, J. Ripoll, L. Rodriguez, J. Santos, F. P. dos Santos, J. M. F. Serra, L. Shuman, D. Simon, A. Sofka, C. Sorel, M. Stiegler, T. Toledo, J. F. Torrent, J. Tsamalaidze, Z. Veloso, J. F. C. A. Webb, R. White, J. T. Yahlali, N. Yepes-Ramirez, H. CA NEXT Collaboration TI Sensitivity of NEXT-100 to neutrinoless double beta decay SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Dark Matter and Double Beta Decay (experiments); Rare decay ID NUCLEAR-DATA SHEETS; EXO-200; SEARCH; TESTS; MASS AB NEXT-100 is an electroluminescent high-pressure xenon gas time projection chamber that will search for the neutrinoless double beta (0v beta beta) decay of Xe-136. The detector possesses two features of great value for 0v beta beta searches: energy resolution better than 1% FWHM at the Q value of Xe-136 and track reconstruction for the discrimination of signal and background events. This combination results in excellent sensitivity, as discussed in this paper. Material-screening measurements and a detailed Monte Carlo detector simulation predict a background rate for NEXT-100 of at most 4 x 10(-4) counts keV(-1) kg(-1) yr(-1). Accordingly, the detector will reach a sensitivity to the 0v beta beta-decay half-life of 2.8 x 10(25) years (90% CL) for an exposure of 100 kg.year, or 6.0 x 10(25) years after a run of 3 effective years. C1 [Martin-Albo, J.; Munoz Vidal, J.; Ferrario, P.; Nebot-Guinot, M.; Gomez-Cadenas, J. J.; Alvarez, V.; Carcel, S.; Carrion, J. V.; Cervera, A.; Diaz, J.; Laing, A.; Liubarsky, I.; Lopez-March, N.; Lorca, D.; Martinez, A.; Novella, P.; Palmeiro, B.; Querol, M.; Renner, J.; Rodriguez, J.; Serra, L.; Simon, A.; Sorel, M.; Yahlali, N.] CSIC, Inst Fis Corpuscular IFIC, Calle Catedrat Jose Beltran 2, Valencia 46980, Spain. [Martin-Albo, J.; Munoz Vidal, J.; Ferrario, P.; Nebot-Guinot, M.; Gomez-Cadenas, J. J.; Alvarez, V.; Carcel, S.; Carrion, J. V.; Cervera, A.; Diaz, J.; Laing, A.; Liubarsky, I.; Lopez-March, N.; Lorca, D.; Martinez, A.; Novella, P.; Palmeiro, B.; Querol, M.; Renner, J.; Rodriguez, J.; Serra, L.; Simon, A.; Sorel, M.; Yahlali, N.; NEXT Collaboration] Univ Valencia, Calle Catedrat Jose Beltran 2, Valencia 46980, Spain. [Azevedo, C. D. R.; Ferreira, A. L.; Moutinho, L. M.; Veloso, J. F. C. A.] Univ Aveiro, I3N, Campus Santiago, P-3810193 Aveiro, Portugal. [Borges, F. I. G.; Conde, C. A. N.; Santos, F. P.] Univ Coimbra, Dept Fis, LIP, Rua Larga, P-3004516 Coimbra, Portugal. [Cebrian, S.] Univ Zaragoza, Lab Fis Nucl & Astroparticulas, Calle Pedro Cerbuna 12, E-50009 Zaragoza, Spain. [Diesburg, M.; Lebrun, P.; Para, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Esteve, R.; Herrero, V.; Mora, F. J.; Toledo, J. F.] Univ Politecn Valencia, I3M, Camino Vera S-N,Edificio 8B, E-46022 Valencia, Spain. [Fernandes, L. M. P.; Freitas, E. D. C.; Henriques, C. A. O.; Monteiro, C. M. B.; dos Santos, J. M. F.] Univ Coimbra, Dept Phys, LIBPhys, Rua Larga, P-3004516 Coimbra, Portugal. [Goldschmidt, A.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Gonzalez-Diaz, D.] European Org Nucl Res CERN, CH-1211 Geneva 23, Switzerland. [Gutierrez, R. M.; Losada, M.; Yepes-Ramirez, H.] Univ Antonio Narino Sede Circunvalar, Ctr Investi Ciencias Basicas & Aplicadas, Carretera 3 Este 47 A-15, Bogota, Colombia. [Hauptman, J.] Iowa State Univ, Dept Phys & Astron, 12 Phys Hall, Ames, IA 50011 USA. [Hernando Morata, J. A.; Martinez-Lema, G.] Univ Santiago de Compostela, Inst Gallego Fis Altas Energias, Campus Sur,Rua Xose Maria Suarez Nunez S-N, Santiago De Compostela 15782, Spain. [Labarga, L.] Univ Autonoma Madrid, Dept Fis Teor, Campus Cantoblanco, E-28049 Madrid, Spain. [Monrabal, F.; Nygren, D.; Shuman, D.] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Ripoll, L.; Torrent, J.] Univ Girona, Escola Politecn Super, Ave Montilivi S-N, Girona 17071, Spain. [Sofka, C.; Stiegler, T.; Webb, R.; White, J. T.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Tsamalaidze, Z.] Joint Inst Nucl Res, Joliot Curie 6, Dubna 141980, Russia. [Martin-Albo, J.] Univ Oxford, Oxford, England. RP Martin-Albo, J (reprint author), CSIC, Inst Fis Corpuscular IFIC, Calle Catedrat Jose Beltran 2, Valencia 46980, Spain.; Martin-Albo, J (reprint author), Univ Valencia, Calle Catedrat Jose Beltran 2, Valencia 46980, Spain.; Martin-Albo, J (reprint author), Univ Oxford, Oxford, England. EM justo.martin-albo@ific.uv.es OI Santos, Filomena/0000-0002-0214-4185; Munoz Vidal, Javier/0000-0002-9649-2251; Toledo Alarcon, Jose Francisco/0000-0002-9782-4510; Freitas, Elisabete/0000-0001-8235-3229; Azevedo, Carlos/0000-0002-0012-9918; Martin-Albo, Justo/0000-0002-7318-1469; Veloso, Joao/0000-0002-7107-7203 FU European Research Council (ERC) [339787-NEXT]; Ministerio de Economia y Competitividad of Spain [2010 CSD2008-0037, FIS2014-53371-C04]; Severo Ochoa Program [SEV-2014-0398]; Portuguese FCT; FEDER through the program COMPETE [PTDC/FIS/103860/2008]; U.S. Department of Energy [DE-AC02-07CH11359, DE-FG02-13ER42020]; University of Texas at Arlington FX The NEXT Collaboration acknowledges support from the following agencies and institutions: the European Research Council (ERC) under the Advanced Grant 339787-NEXT; the Ministerio de Economia y Competitividad of Spain under grants CONSOLIDER-Ingenio 2010 CSD2008-0037 (CUP), FIS2014-53371-C04 and the Severo Ochoa Program SEV-2014-0398; the Portuguese FCT and FEDER through the program COMPETE, project PTDC/FIS/103860/2008; the U.S. Department of Energy under contracts number DE-AC02-07CH11359 (Fermi National Accelerator Laboratory) and DE-FG02-13ER42020 (Texas A & and the University of Texas at Arlington. We thank Joshua B. Albert for useful discussions regarding the cosmogenic backgrounds. NR 75 TC 3 Z9 3 U1 6 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 26 PY 2016 IS 5 AR 159 DI 10.1007/JHEP05(2016)159 PG 30 WC Physics, Particles & Fields SC Physics GA EH4ML UT WOS:000391745200003 ER PT J AU Chatterjee, S Kapoor, A Akiyama, J Auer, D Berrios, C Pennacchio, L Chakravarti, A AF Chatterjee, S. Kapoor, A. Akiyama, J. Auer, D. Berrios, C. Pennacchio, L. Chakravarti, A. TI Multiple enhancer variants disrupt gene regulatory network in Hirschsprung disease SO HUMAN GENOMICS LA English DT Meeting Abstract C1 [Chatterjee, S.; Kapoor, A.; Auer, D.; Berrios, C.; Chakravarti, A.] Johns Hopkins Univ, Inst Med Genet, Baltimore, MD 21218 USA. [Akiyama, J.; Pennacchio, L.] Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1473-9542 EI 1479-7364 J9 HUM GENOMICS JI Hum. Genomics PD MAY 26 PY 2016 VL 10 SU 1 MA O8 PG 1 WC Genetics & Heredity SC Genetics & Heredity GA DW5LM UT WOS:000383686700009 ER PT J AU Dolen, J Harris, P Marzani, S Rappoccio, S Tran, N AF Dolen, James Harris, Philip Marzani, Simone Rappoccio, Salvatore Nhan Tran TI Thinking outside the ROCs: Designing Decorrelated Taggers (DDT) for jet substructure SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; QCD Phenomenology ID RESONANCES; COLLISIONS; SEARCH; TEV AB We explore the scale-dependence and correlations of jet substructure observables to improve upon existing techniques in the identification of highly Lorentz-boosted objects. Modified observables are designed to remove correlations from existing theoretically well-understood observables, providing practical advantages for experimental measurements and searches for new phenomena. We study such observables in W jet tagging and provide recommendations for observables based on considerations beyond signal and background efficiencies. C1 [Dolen, James; Marzani, Simone; Rappoccio, Salvatore] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. [Harris, Philip] European Org Nucl Res, CERN, Geneva, Switzerland. [Nhan Tran] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Dolen, J (reprint author), SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. EM james.william.dolen@cern.ch; philip.coleman.harris@cern.ch; smarzani@buffalo.edu; srrappoc@buffalo.edu; ntran@fnal.gov FU CERN; LHC Theory Initiative; Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy; U.S. National Science Foundation [PHY-1401223, PHY-0969510] FX We thank Andrew Larkoski and Petar Maksimovic for their critical reading of the manuscript. The authors would also like to thank Matteo Cremonesi, Matthew Low, Cristina Mantilla Suarez, Siddharth Narayanan, Gavin Salam, Gregory Soyez, and Michael Spannowsky for useful discussion and inputs. JD and SR are partially supported by the U.S. National Science Foundation, under grant PHY-1401223. PH is supported by CERN. The work of SM is partly supported by the U.S. National Science Foundation, under grant PHY-0969510, the LHC Theory Initiative. NT is supported by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 56 TC 3 Z9 3 U1 1 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 26 PY 2016 IS 5 AR 156 DI 10.1007/JHEP05(2016)156 PG 19 WC Physics, Particles & Fields SC Physics GA DU0OI UT WOS:000381904000001 ER PT J AU Craig, PR Havlas, Z Trujillo, M Rempala, P Kirby, JP Miller, JR Noll, BC Michl, J AF Craig, Peter R. Havlas, Zdenek Trujillo, Marianela Rempala, Pawel Kirby, James P. Miller, John R. Noll, Bruce C. Michl, Josef TI Electronic Spectra of the Tetraphenylcyclobutadienecyclopentadienylnickel(II) Cation and Radical SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CYCLOBUTADIENE-METAL COMPLEXES; TETRAGONAL STAR CONNECTORS; SQUARE-GRID POLYMER; HALIDES AB Properties of the tetraphenylcyclobutadienecyclopentadienylnickel(II) cation 1 and its tetra-o-fluoro derivative la have been measured and calculated. The B3LYP/TZP optimized geometry of the free cation 1 agrees with a single-crystal X-ray diffraction structure except that in the crystal one of the phenyl substituents is strongly twisted to permit a close-packing interaction of two of its hydrogens with a nearby BF4- anion. The low-energy parts of the solution electronic absorption and magnetic circular dichroism (MCD) spectra of 1 and la have been interpreted by comparison with TD-DFT (B3LYP/TZP) results. Reduction or pulse radiolysis lead to a neutral 19-electron radical, whose visible absorption and MCD spectra have been recorded and interpreted as well. The reduction is facilitated by similar to 0.1 V upon going from 1 to la. Unsuccessful attempts to prepare several other aryl substituted derivatives of 1 by the classical synthetic route are described in the Supporting Information. C1 [Craig, Peter R.; Trujillo, Marianela; Rempala, Pawel; Noll, Bruce C.; Michl, Josef] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Havlas, Zdenek; Michl, Josef] Acad Sci Czech Republic, Inst Organ Chem & Biochem, Flemingovo Nam 2, CR-16610 Prague 6, Czech Republic. [Kirby, James P.; Miller, John R.] Brookhaven Natl Lab, Dept Chem, Bldg 555A, Upton, NY 11973 USA. RP Michl, J (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA.; Michl, J (reprint author), Acad Sci Czech Republic, Inst Organ Chem & Biochem, Flemingovo Nam 2, CR-16610 Prague 6, Czech Republic. RI Michl, Josef/G-9376-2014 FU National Science Foundation [CHE-1265922]; Institute of Organic Chemistry and Biochemistry [RVO:61388963]; Czech Science Foundation [GBP208/12/G016] FX This material is based upon work supported by the National Science Foundation under Grant No. CHE-1265922. We are grateful to Mr. Justin M. Ray, Mr. David J. Koditek, and Mr. Kamal Gala for technical assistance. Work in Prague was supported by the Institute of Organic Chemistry and Biochemistry (RVO:61388963) and the Czech Science Foundation (GBP208/12/G016). NR 12 TC 0 Z9 0 U1 8 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 26 PY 2016 VL 120 IS 20 BP 3456 EP 3462 DI 10.1021/acs.jpca.6b00648 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN1QS UT WOS:000376841100008 PM 27136127 ER PT J AU Schrauben, JN Akdag, A Wen, J Havlas, Z Ryerson, JL Smith, MB Michl, J Johnson, JC AF Schrauben, Joel N. Akdag, Akin Wen, Jin Havlas, Zdenek Ryerson, Joseph L. Smith, Millie B. Michl, Josef Johnson, Justin C. TI Excitation Localization/Delocalization Isomerism in a Strongly Coupled Covalent Dimer of 1,3-Diphenylisobenzofuran SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INTRAMOLECULAR SINGLET FISSION; DENSITY-FUNCTIONAL THEORY; EXCITON FISSION; TETRACENE DIMER; THIN-FILM; STATES; PHOTOPHYSICS; DELOCALIZATION; CONFORMATIONS; MOLECULES AB Two isomers of both the lowest excited singlet (S-1) and triplet (T-1) states of the directly para, para'-connected covalent dimer of the singlet-fission chromophore 1,3-diphenylisobenzofuran have been observed. In one isomer, excitation is delocalized over both halves of the dimer, and in the other, it is localized on one or the other half. For a covalent dimer in solution, such "excitation isomerism" is extremely rare. The vibrationally relaxed isomers do not interconvert, and their photophysical properties, including singlet fission, differ significantly. C1 [Schrauben, Joel N.; Ryerson, Joseph L.; Johnson, Justin C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ryerson, Joseph L.; Michl, Josef] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Akdag, Akin] Middle E Tech Univ, Dept Chem, TR-06800 Ankara, Turkey. [Wen, Jin; Havlas, Zdenek; Michl, Josef] Acad Sci Czech Republic, Inst Organ Chem & Biochem, Flemingovo Nam 2, CR-16610 Prague, Czech Republic. RP Johnson, JC (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. RI Michl, Josef/G-9376-2014 FU NREL [DE-AC36-08GO28308]; DOE [DE-SC0007004]; post-doctoral program of the IOCB (ASCR) [RVO: 61388963]; Grant Agency of the Czech Republic [15-19143S]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences FX This material is based on work supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences, and Geosciences. J.N.S., J.L.R., and J.C.J acknowledge Contract DE-AC36-08GO28308 with NREL, and J.M. and A.A. acknowledge Award DOE DE-SC0007004. J.W. acknowledges the post-doctoral program of the IOCB (ASCR, RVO: 61388963). Z.H., J.M., and J.W. acknowledge support from the Grant Agency of the Czech Republic (Grant 15-19143S). NR 44 TC 1 Z9 1 U1 18 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 26 PY 2016 VL 120 IS 20 BP 3473 EP 3483 DI 10.1021/acs.jpca.6b00826 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN1QS UT WOS:000376841100010 PM 27158903 ER PT J AU Pakhira, S Singh, RI Olatunji-Ojo, O Frenklach, M Lester, WA AF Pakhira, Srimanta Singh, Ravi I. Olatunji-Ojo, Olayinka Frenklach, Michael Lester, William A., Jr. TI Quantum Monte Carlo Study of the Reactions of CH with Acrolein: Major and Minor Channels SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATES; PRODUCT DETECTION; WAVE-FUNCTIONS; MOLECULES; DENSITY; IMPLEMENTATION; DISSOCIATIONS; SIMULATIONS; LOOSENESS; ENERGIES AB Acrolein is an important unsaturated hydrocarbon, containing both C=O and C=C bonds, and responsible for atmospheric pollution. A recent study of major reactions of CH with acrolein has been supplemented with computations of other reactions of the system. Similar to the previous approach, the quantum Monte Carlo (QMC) method in the accurate diffusion Monte Carlo (DMC) method was implemented. Single determinant wave functions were used as trial functions for the random walks. Rate coefficients and product branching ratios were computed by solving master equations using the MultiWell software suite. At room temperature, the dominant product channels are 2-methylvinyl + CO (P6), 1,3-butadienal + H (P2), and furan + H (P1). At elevated temperatures, 2,3-butadienal + H (P10) is also a major product. The chain decomposition pathway to form C3H4 + HCO was not competitive with the cyclization pathway at any of the temperatures studied. The DMC branching fractions of the products formed in the subject reaction are in reasonable accord with previous experimental and theoretical values. The computed rate coefficients were found to be independent of pressure at temperatures relevant to combustion (1500-2500 K). C1 [Pakhira, Srimanta; Lester, William A., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Singh, Ravi I.; Frenklach, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Pakhira, Srimanta; Lester, William A., Jr.] Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. [Singh, Ravi I.; Frenklach, Michael] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Olatunji-Ojo, Olayinka] Univ Calif Berkeley, Coll Chem, Berkeley, CA 94720 USA. [Pakhira, Srimanta] Nagoya Univ, Grad Sch Informat Sci, Chikusa Ku, Furo Cho, Nagoya, Aichi 4648601, Japan. RP Lester, WA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Lester, WA (reprint author), Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. EM walester@berkeley.edu FU U.S. Department of Energy [DE-AC03-76F00098]; U.S. Army Corps of Engineers, Humphreys Engineering Center Support Activity [W912HQ-07-C-0044]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Srimanta Pakhira and William A. Lester, Jr., were supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the U.S. Department of Energy, under Contract No. DE-AC03-76F00098. Srimanta Pakhira thanks the Japan Society for the Promotion of Science (JSPS). Ravi I. Singh and Michael Frenklach were supported by the U.S. Army Corps of Engineers, Humphreys Engineering Center Support Activity, under Contract No. W912HQ-07-C-0044. This research used computational resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We are grateful to Brian M. Austin, Advanced Technology Group, NERSC, Lawrence Berkeley National Laboratory, Berkeley, CA, USA, and to Benjamin Sanchez Lengeling, Department of Chemistry and Chemical Biology, Harvard University, Cambridge, MA, USA, for helpful discussions. NR 39 TC 0 Z9 0 U1 8 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 26 PY 2016 VL 120 IS 20 BP 3602 EP 3612 DI 10.1021/acs.jpca.5b11527 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN1QS UT WOS:000376841100026 PM 27046018 ER PT J AU Knudsen, KB Nichols, JE Vegge, T Luntz, AC McCloskey, BD Hjelm, J AF Knudsen, Kristian B. Nichols, Jessica E. Vegge, Tejs Luntz, Alan C. McCloskey, Bryan D. Hjelm, Johan TI An Electrochemical Impedance Study of the Capacity Limitations in Na-O-2 Cells SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID NONAQUEOUS LI-O-2 BATTERIES; POROUS FILM ELECTRODES; CONSTANT-PHASE-ELEMENT; SODIUM SUPEROXIDE; GROWTH; LI2O2; STABILITY; TRANSPORT; DISCHARGE; SOLVENTS AB Electrochemical impedance spectroscopy, pressure change measurements, and scanning electron microscopy were used to investigate the nonaqueous Na-O-2 cell potential decrease and rise (sudden deaths) on discharge and charge, respectively. To fit the impedance spectra from operating cells, an equivalent circuit model was used that takes into account the porous nature of the positive electrode and is able to distinguish between the electrolyte resistance in the pores and the charge-transfer resistance of the pore walls. The results obtained indicate that sudden death on discharge is caused by, depending on the current density, either accumulation of large NaO2 crystals that eventually block the electrode surface and/or a thin film of NaO2 forming on the cathode surface at the end of discharge, which limits charge-transfer. The commonly observed sudden rise in potential toward the end of charge may be caused by a concentration depletion of NaO2 dissolved in the electrolyte near the cathode surface and/or an accumulation of degradation products on the cathode surface. C1 [Knudsen, Kristian B.; Vegge, Tejs; Hjelm, Johan] Tech Univ Denmark, Dept Energy Convers & Storage, DK-4000 Roskilde, Denmark. [Knudsen, Kristian B.; Nichols, Jessica E.; McCloskey, Bryan D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Nichols, Jessica E.; McCloskey, Bryan D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Luntz, Alan C.] Stanford Univ, Dept Chem Engn, SUNCAT Ctr Interface Sci & Catalysis, 443 Via Ortega, Stanford, CA 94305 USA. [Luntz, Alan C.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Hjelm, J (reprint author), Tech Univ Denmark, Dept Energy Convers & Storage, DK-4000 Roskilde, Denmark.; McCloskey, BD (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; McCloskey, BD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. EM bmcclosk@berkeley.edu; johh@dtu.dk RI Vegge, Tejs/A-9419-2011; OI Vegge, Tejs/0000-0002-1484-0284; Hjelm, Johan/0000-0003-0072-5784 FU ReLiable project - Danish Council for Strategic Research, Program Commission on Sustainable Energy and Environment [11-116792]; National Science Foundation Graduate Research Fellowship Program [DGE-1106400] FX We gratefully acknowledge financial support from the ReLiable project (project no. 11-116792) funded by the Danish Council for Strategic Research, Program Commission on Sustainable Energy and Environment. This material is based upon work supported by the National Science Foundation Graduate Research Fellowship Program under Grant no. DGE-1106400. Torben Jacobsen is acknowledged for valuable discussions of porous electrode theory. NR 30 TC 3 Z9 3 U1 3 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2016 VL 120 IS 20 BP 10799 EP 10805 DI 10.1021/acs.jpcc.6602788 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DN1QQ UT WOS:000376840900007 ER PT J AU Grinter, DC Muryn, C Sala, A Yim, CM Pang, CL Mentes, TO Locatelli, A Thornton, G AF Grinter, David C. Muryn, Chris Sala, Alessandro Yim, Chi-Ming Pang, Chi L. Mentes, Tevfik O. Locatelli, Andrea Thornton, Geoff TI Spillover Reoxidation of Ceria Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOELECTRON MICROSCOPY; RESONANT PHOTOEMISSION; SINGLE-CRYSTALS; GROWTH; FILMS; SPECTROSCOPY; DESORPTION; MORPHOLOGY; REDUCTION; CATALYSIS AB Interest in resolving the mechanisms behind ceria's activity has been intense due to the numerous industrial applications including those in heterogeneous catalysis. In this work, we study the reduction and reoxidation of ultrathin CeO2(111) nanoislands on Rh(111) and Pt(111) substrates, so-called inverse model catalysts, with a combination of real and reciprocal space techniques based on X-ray photoemission electron microscopy (XPEEM) and low energy electron microscopy. Soft X-ray microfocused illumination was employed to reduce the ceria islands, which we are able to control by varying the oxygen partial pressure within the measurement chamber. Low energy electron diffraction measurements of the irradiated ceria films demonstrate the formation of an ordered array of oxygen vacancies leading to a (/7 x root 7)R19.1 degrees superstructure attributed to the i-phase (Ce7O12)(111). Resonant photoelectron spectroscopy provides the required high sensitivity to detect small changes in Ce3+ concentration. The high spatial resolution of the XPEEM allows us to determine that the reduction of the ceria occurs initially at the interface of the islands with the Rh support. Reoxidation of the CeO2-x(111) to CeO2(111) proceeds via spillover of activated oxygen adsorbed on the Rh(111) surface as a (2 x 2) overlayer. Our results highlight the important role that the noble metal plays in the regeneration of the stoichiometric ceria surface, a vital step in many reactions on ceria. This differs from the commonly proposed Mars van Krevelen model in which reoxidation involves direct reaction of the ceria with O-2. C1 [Grinter, David C.; Yim, Chi-Ming; Pang, Chi L.; Thornton, Geoff] UCL, Dept Chem, London WC1H 0AJ, England. [Grinter, David C.; Yim, Chi-Ming; Pang, Chi L.; Thornton, Geoff] UCL, Ctr Nanotechnol, London WC1H 0AJ, England. [Grinter, David C.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Muryn, Chris] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England. [Muryn, Chris] Univ Manchester, Photon Sci Inst, Manchester M13 9PL, Lancs, England. [Mentes, Tevfik O.; Locatelli, Andrea] Elettra Sincrotrone Trieste SCpA, I-34149 Trieste, Italy. RP Thornton, G (reprint author), UCL, Dept Chem, London WC1H 0AJ, England.; Thornton, G (reprint author), UCL, Ctr Nanotechnol, London WC1H 0AJ, England. EM g.thornton@ucl.ac.uk RI COST, CM1104/I-8057-2015; Pang, Chi Lun/M-1105-2016; OI Pang, Chi Lun/0000-0002-5222-9734; Grinter, David/0000-0001-6089-119X; Locatelli, Andrea/0000-0002-8072-7343 FU European Research Council; EU COST Action [CM1104]; Royal Society; EPSRC (U.K.) FX This work was supported by the European Research Council Advanced Grant ENERGYSURF (G.T.), the EU COST Action CM1104, the Royal Society, and the EPSRC (U.K.). NR 51 TC 1 Z9 1 U1 14 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2016 VL 120 IS 20 BP 11037 EP 11044 DI 10.1021/acs.jpcc.6b03670 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DN1QQ UT WOS:000376840900033 ER PT J AU Kim, M Adamska, L Hartmann, NF Kwon, H Liu, J Velizhanin, KA Piao, YM Powell, LR Meany, B Doorn, SK Tretiak, S Wang, YH AF Kim, Mijin Adamska, Lyudmyla Hartmann, Nicolai F. Kwon, Hyejin Liu, Jin Velizhanin, Kirill A. Piao, Yanmei Powell, Lyndsey R. Meany, Brendan Doorn, Stephen K. Tretiak, Sergei Wang, YuHuang TI Fluorescent Carbon Nanotube Defects Manifest Substantial Vibrational Reorganization SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELECTRONIC-STRUCTURE; PHOTOLUMINESCENCE; TEMPERATURE; EXCITON; SPECTROSCOPY; GENERATION; STATES AB Fluorescent defects have opened up exciting new opportunities to chemically tailor semiconducting carbon nanotubes for imaging, sensing, and photonics needs such as lasing, single photon emission, and photon upconversion. However, experimental measurements on the trap depths of these defects show a puzzling energy mismatch between the optical gap (difference in emission energies between the native exciton and defect trap states) and the thermal detrapping energy determined by application of the van 't Hoff equation. To resolve this fundamentally important problem, here we synthetically incorporated a series of fluorescent aryl defects into semiconducting single-walled carbon nanotubes and experimentally determined their energy levels by temperature-dependent and chemically correlated evolution of exciton population and photoluminescence. We found that depending on the chemical nature and density of defects, the exciton detrapping energy is 14-77% smaller than the optical gap determined from photoluminescence. For the same type of defect, the detrapping energy increases with defect density from 76 to 131 meV for 4-nitroaryl defects in (6,5) single-walled carbon nanotubes, whereas the optical gap remains nearly unchanged (<5 meV). These experimental findings are corroborated by quantum-chemical simulations of the chemically functionalized carbon nanotubes. Our results suggest that the energy mismatch arises from vibrational reorganization due to significant deformation of the nanotube geometry upon exciton trapping at the defect site. An unexpectedly large reorganization energy (on the order of 100 meV) is found between ground and excited states of the defect tailored nanostructures. This finding reveals a molecular picture for description of these synthetic defects and suggests significant potential for tailoring the electronic properties of carbon nanostructures through chemical engineering. C1 [Kim, Mijin; Kwon, Hyejin; Piao, Yanmei; Powell, Lyndsey R.; Meany, Brendan; Wang, YuHuang] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Adamska, Lyudmyla; Hartmann, Nicolai F.; Doorn, Stephen K.; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. [Adamska, Lyudmyla; Velizhanin, Kirill A.; Tretiak, Sergei] Los Alamos Natl Lab, Div Theoret, Phys & Chem Mat, T-1, Los Alamos, NM 87545 USA. RP Wang, YH (reprint author), Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA.; Doorn, SK (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. EM skdoorn@lan1.gov; yhw@umd.edu RI Velizhanin, Kirill/C-4835-2008; Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Hartmann, Nicolai/0000-0002-4174-532X; Powell, Lyndsey/0000-0002-7133-7546 FU National Science Foundation [CHE-1507974, CAREER CHE-1055514]; AFOSR through MURI [FA9550-16-1-0150]; LANL LDRD program; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Science user facility [U2015A0059] FX This work was supported by the National Science Foundation (CHE-1507974, CAREER CHE-1055514). CNT sorting is supported by AFOSR through MURI grant FA9550-16-1-0150. S.K.D. and S.T. acknowledge partial support from the LANL LDRD program. This work was performed in part at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Science user facility, as part of User Project U2015A0059. The authors also acknowledge the LANL Institutional Computing (IC) Program for providing computational resources. NR 41 TC 3 Z9 3 U1 6 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 26 PY 2016 VL 120 IS 20 BP 11268 EP 11276 DI 10.1021/acs.jpcc.6b02538 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DN1QQ UT WOS:000376840900060 ER PT J AU Abhyankar, VV Wu, MY Koh, CY Hatch, AV AF Abhyankar, Vinay V. Wu, Meiye Koh, Chung-Yan Hatch, Anson V. TI A Reversibly Sealed, Easy Access, Modular (SEAM) Microfluidic Architecture to Establish In Vitro Tissue Interfaces SO PLOS ONE LA English DT Article ID ORGANS-ON-CHIPS; PEPTIDE-AMPHIPHILE NANOFIBERS; CELL-CULTURE; EXTRACELLULAR-MATRIX; MOLECULAR-MECHANISMS; DRUG DISCOVERY; MEMBRANES; DEVICES; MICROFABRICATION; PURIFICATION AB Microfluidic barrier tissue models have emerged as advanced in vitro tools to explore interactions with external stimuli such as drug candidates, pathogens, or toxins. However, the procedures required to establish and maintain these systems can be challenging to implement for end users, particularly those without significant in-house engineering expertise. Here we present a module-based approach that provides an easy-to-use workflow to establish, maintain, and analyze microscale tissue constructs. Our approach begins with a removable culture insert that is magnetically coupled, decoupled, and transferred between standalone, prefabricated microfluidic modules for simplified cell seeding, culture, and downstream analysis. The modular approach allows several options for perfusion including standard syringe pumps or integration with a self-contained gravity-fed module for simple cell maintenance. As proof of concept, we establish a culture of primary human microvascular endothelial cells (HMVEC) and report combined surface protein imaging and gene expression after controlled apical stimulation with the bacterial endotoxin lipopolysaccharide (LPS). We also demonstrate the feasibility of incorporating hydrated biomaterial interfaces into the microfluidic architecture by integrating an ultra-thin (<1 mu m), self-assembled hyaluronic acid/peptide amphiphile culture membrane with brain-specific Young's modulus (similar to 1kPa). To highlight the importance of including biomimetic interfaces into microscale models we report multi-tiered readouts from primary rat cortical cells cultured on the self-assembled membrane and compare a panel of mRNA targets with primary brain tissue signatures. We anticipate that the modular approach and simplified operational workflows presented here will enable a wide range of research groups to incorporate microfluidic barrier tissue models into their work. C1 [Abhyankar, Vinay V.; Wu, Meiye; Koh, Chung-Yan; Hatch, Anson V.] Sandia Natl Labs, Dept Biotechnol & Bioengn, Livermore, CA 94551 USA. [Abhyankar, Vinay V.] Univ Texas Arlington, Res Inst, Biol Microsyst, Ft Worth, TX 76118 USA. RP Abhyankar, VV; Hatch, AV (reprint author), Sandia Natl Labs, Dept Biotechnol & Bioengn, Livermore, CA 94551 USA.; Abhyankar, VV (reprint author), Univ Texas Arlington, Res Inst, Biol Microsyst, Ft Worth, TX 76118 USA. EM vinay.abhyankar@gmail.com; ahatch@sandia.gov FU Laboratory Directed Research and Development (LDRD) at Sandia National Laboratories; Defense Threat Reduction Agency Joint Science and Technology Office for Chemical and Biological Defense (IAA) [DTRA 10027IA-3167]; NIAID [R01AI98853]; US Department of Energy [DE-AC04-94AL85000] FX This work was funded under Laboratory Directed Research and Development (LDRD) at Sandia National Laboratories and by the Defense Threat Reduction Agency Joint Science and Technology Office for Chemical and Biological Defense (IAA number DTRA 10027IA-3167). CK was supported by NIAID grant R01AI98853. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US Department of Energy under contract DE-AC04-94AL85000. Illustrations contained vector art designed by Freepik. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 65 TC 1 Z9 1 U1 9 U2 15 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2016 VL 11 IS 5 AR e0156341 DI 10.1371/journal.pone.0156341 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN2GQ UT WOS:000376882500118 PM 27227828 ER PT J AU Stromberg, LR Hengartner, NW Swingle, KL Moxley, RA Graves, SW Montano, GA Mukundan, H AF Stromberg, Loreen R. Hengartner, Nicolas W. Swingle, Kirstie L. Moxley, Rodney A. Graves, Steven W. Montano, Gabriel A. Mukundan, Harshini TI Membrane Insertion for the Detection of Lipopolysaccharides: Exploring the Dynamics of Amphiphile-in-Lipid Assays SO PLOS ONE LA English DT Article ID LINKED-IMMUNOSORBENT-ASSAY; HIGH-DENSITY-LIPOPROTEIN; ESCHERICHIA-COLI O26; TOLL-LIKE RECEPTORS; BINDING-PROTEIN; (LPS)-BINDING PROTEIN; BIOLOGICAL-ACTIVITIES; BACTERIAL-ENDOTOXINS; PATHOGEN DETECTION; MOLECULAR-BASIS AB Shiga toxin-producing Escherichia coli is an important cause of foodborne illness, with cases attributable to beef, fresh produce and other sources. Many serotypes of the pathogen cause disease, and differentiating one serotype from another requires specific identification of the O antigen located on the lipopolysaccharide (LPS) molecule. The amphiphilic structure of LPS poses a challenge when using classical detection methods, which do not take into account its lipoglycan biochemistry. Typically, detection of LPS requires heat or chemical treatment of samples and relies on bioactivity assays for the conserved lipid A portion of the molecule. Our goal was to develop assays to facilitate the direct and discriminative detection of the entire LPS molecule and its O antigen in complex matrices using minimal sample processing. To perform serogroup identification of LPS, we used a method called membrane insertion on a waveguide biosensor, and tested three serogroups of LPS. The membrane insertion technique allows for the hydrophobic association of LPS with a lipid bilayer, where the exposed O antigen can be targeted for specific detection. Samples of beef lysate were spiked with LPS to perform O antigen specific detection of LPS from E. coli O157. To validate assay performance, we evaluated the biophysical interactions of LPS with lipid bilayers both in-and outside of a flow cell using fluorescence microscopy and fluorescently doped lipids. Our results indicate that membrane insertion allows for the qualitative and reliable identification of amphiphilic LPS in complex samples like beef homogenates. We also demonstrated that LPS-induced hole formation does not occur under the conditions of the membrane insertion assays. Together, these findings describe for the first time the serogroup-specific detection of amphiphilic LPS in complex samples using a membrane insertion assay, and highlight the importance of LPS molecular conformations in detection architectures. C1 [Stromberg, Loreen R.; Graves, Steven W.; Mukundan, Harshini] Univ New Mexico, Ctr Biomed Engn, Albuquerque, NM 87131 USA. [Stromberg, Loreen R.; Mukundan, Harshini] Los Alamos Natl Lab, Phys Chem & Appl Spect, Los Alamos, NM USA. [Stromberg, Loreen R.; Graves, Steven W.; Mukundan, Harshini] New Mexico Consortium, Los Alamos, NM USA. [Hengartner, Nicolas W.] Los Alamos Natl Lab, Theoret Biol & Biophys, Los Alamos, NM USA. [Swingle, Kirstie L.; Montano, Gabriel A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM USA. [Moxley, Rodney A.] Univ Nebraska, Sch Vet Med & Biomed Sci, Lincoln, NE USA. RP Mukundan, H (reprint author), Univ New Mexico, Ctr Biomed Engn, Albuquerque, NM 87131 USA. EM harshini@lanl.gov OI Moxley, Rodney/0000-0002-5377-7716; Stromberg, Loreen/0000-0003-1715-1211 FU National Institute of Food and Agriculture, U.S. Department of Agriculture [2012-68003-30155]; National Nuclear Security Administration of the United States Department of Energy [DE-AC52-06NA25396]; Photosynthetic Antenna Research Center, an Energy Frontier Research Center - United States Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001035]; Los Alamos National Laboratory Directed Research and Development (LDRD); Agriculture and Food Research Initiative Competitive from the United States Department of Agriculture's National Institute of Food and Agriculture [2012-68003-30155]; Los Alamos National Laboratory Directed Research Award, Integrative Biosurveillance FX LRS RAM SWG HM were supported in part by the National Institute of Food and Agriculture, U.S. Department of Agriculture, under award number 2012-68003-30155. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the United States Department of Energy under contract No. DE-AC52-06NA25396. Work by G.A.M and K.L.S. was supported by Photosynthetic Antenna Research Center, an Energy Frontier Research Center funded by the United States Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0001035. Nicholas Hengartner was supported by a Los Alamos National Laboratory Directed Research and Development (LDRD) award (project title, Integrative Biosurveillance, PI Mukundan and McMahon). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the United States Department of Energy's Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the United States Department of Energy under contract No. DE-AC52-06NA25396. Work by G.A.M and K.L.S. was supported by Photosynthetic Antenna Research Center, an Energy Frontier Research Center funded by the United States Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0001035. H.M., R.A.M, S.W.G and L.R.S. were supported by Agriculture and Food Research Initiative Competitive Grant No. 2012-68003-30155 from the United States Department of Agriculture's National Institute of Food and Agriculture. N.H. was supported by Los Alamos National Laboratory Directed Research Award, Integrative Biosurveillance (Mukundan and McMahon). NR 86 TC 0 Z9 0 U1 6 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 26 PY 2016 VL 11 IS 5 AR e0156295 DI 10.1371/journal.pone.0156295 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN2GQ UT WOS:000376882500105 PM 27227979 ER PT J AU Cass, CL Lavell, AA Santoro, N Foster, CE Karlen, SD Smith, RA Ralph, J Garvin, DF Sedbrook, JC AF Cass, Cynthia L. Lavell, Anastasiya A. Santoro, Nicholas Foster, Cliff E. Karlen, Steven D. Smith, Rebecca A. Ralph, John Garvin, David F. Sedbrook, John C. TI Cell Wall Composition and Biomass Recalcitrance Differences Within a Genotypically Diverse Set of Brachypodium distachyon Inbred Lines SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE bioenergy; grass; polysaccharide; hemicellulose; lignin; digestibility; vernalization; Pooideae ID BROMIDE SPECTROPHOTOMETRIC METHOD; ARABIDOPSIS-THALIANA; LIGNIN CONCENTRATION; NATURAL VARIATION; FLOWERING TIME; MODEL SYSTEM; GRASS; SACCHARIFICATION; CONVERSION; QUALITY AB Brachypodium distachyon (Brachypodium) has emerged as a useful model system for studying traits unique to graminaceous species including bioenergy crop grasses owing to its amenability to laboratory experimentation and the availability of extensive genetic and germplasm resources. Considerable natural variation has been uncovered for a variety of traits including flowering time, vernalization responsiveness, and above-ground growth characteristics. However, cell wall composition differences remain underexplored. Therefore, we assessed cell wall-related traits relevant to biomass conversion to biofuels in seven Brachypodium inbred lines that were chosen based on their high level of genotypic diversity as well as available genome sequences and recombinant inbred line (RIL) populations. Senesced stems plus leaf sheaths from these lines exhibited significant differences in acetyl bromide soluble lignin (ABSL), cell wall polysaccharide-derived sugars, hydroxycinnamates content, and syringyl:guaiacyl:p-hydroxyphenyl (S:G:H) lignin ratios. Free glucose, sucrose, and starch content also differed significantly in senesced stems, as did the amounts of sugars released from cell wall polysaccharides (digestibility) upon exposure to a panel of thermochemical pretreatments followed by hydrolytic enzymatic digestion. Correlations were identified between inbred line lignin compositions and plant growth characteristics such as biomass accumulation and heading date (HD), and between amounts of cell wall polysaccharides and biomass digestibility. Finally, stem cell wall p-coumarate and ferulate contents and free-sugars content changed significantly with increased duration of vernalization for some inbred lines. Taken together, these results show that Brachypodium displays substantial phenotypic variation with respect to cell wall composition and biomass digestibility, with some compositional differences correlating with growth characteristics. Moreover, besides influencing HD and biomass accumulation, vernalization was found to affect cell wall composition and free sugars accumulation in some Brachypodium inbred lines, suggesting genetic differences in how vernalization affects carbon flux to polysaccharides. The availability of related RIL populations will allow for the genetic and molecular dissection of this natural variation, the knowledge of which may inform ways to genetically improve bioenergy crop grasses. C1 [Cass, Cynthia L.; Sedbrook, John C.] Illinois State Univ, Sch Biol Sci, Normal, IL 61761 USA. [Cass, Cynthia L.; Karlen, Steven D.; Smith, Rebecca A.; Ralph, John; Sedbrook, John C.] Univ Wisconsin, US DOE, Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Lavell, Anastasiya A.; Garvin, David F.] Univ Minnesota, Dept Agron & Plant Genet, St Paul, MN USA. [Lavell, Anastasiya A.; Garvin, David F.] USDA ARS, Plant Sci Res Ctr, St Paul, MN 55108 USA. [Santoro, Nicholas; Foster, Cliff E.] Michigan State Univ, US DOE, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Ralph, John] Univ Wisconsin, Dept Biochem, 420 Henry Mall, Madison, WI 53705 USA. RP Sedbrook, JC (reprint author), Illinois State Univ, Sch Biol Sci, Normal, IL 61761 USA.; Sedbrook, JC (reprint author), Univ Wisconsin, US DOE, Great Lakes Bioenergy Res Ctr, Madison, WI USA. EM jcsedbr@ilstu.edu FU Department of Energy's Great Lakes Bioenergy Research Center (Department of Energy, Biological and Environmental Research, Office of Science) [DE FCO2-07ER64494]; USDA-ARS CRIS Project [5062-21000-030-00D] FX This work was supported by the Department of Energy's Great Lakes Bioenergy Research Center (Department of Energy, Biological and Environmental Research, Office of Science grant no. DE FCO2-07ER64494), and by USDA-ARS CRIS Project 5062-21000-030-00D NR 54 TC 2 Z9 2 U1 7 U2 11 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAY 26 PY 2016 VL 7 AR 708 DI 10.3389/fpls.2016.00708 PG 16 WC Plant Sciences SC Plant Sciences GA DN0KR UT WOS:000376753300001 PM 27303415 ER PT J AU Klein, S AF Klein, Spencer TI Invest in neutrino astronomy SO NATURE LA English DT Editorial Material ID ICECUBE C1 [Klein, Spencer] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Klein, Spencer] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Klein, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Klein, S (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM srklein@lbl.gov NR 9 TC 0 Z9 0 U1 2 U2 2 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 26 PY 2016 VL 533 IS 7604 BP 462 EP 464 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM6EJ UT WOS:000376443100015 PM 27225103 ER PT J AU Katmis, F Lauter, V Nogueira, FS Assaf, BA Jamer, ME Wei, P Satpati, B Freeland, JW Eremin, I Heiman, D Jarillo-Herrero, P Moodera, JS AF Katmis, Ferhat Lauter, Valeria Nogueira, Flavio S. Assaf, Badih A. Jamer, Michelle E. Wei, Peng Satpati, Biswarup Freeland, John W. Eremin, Ilya Heiman, Don Jarillo-Herrero, Pablo Moodera, Jagadeesh S. TI A high-temperature ferromagnetic topological insulating phase by proximity coupling SO NATURE LA English DT Article ID MAJORANA FERMIONS; SURFACE AB Topological insulators are insulating materials that display conducting surface states protected by time-reversal symmetry(1,)2, wherein electron spins are locked to their momentum. This unique property opens up new opportunities for creating next-generation electronic, spintronic and quantum computation devices(3-5). Introducing ferromagnetic order into a topological insulator system without compromising its distinctive quantum coherent features could lead to the realization of several predicted physical phenomena(6,7). In particular, achieving robust long-range magnetic order at the surface of the topological insulator at specific locations without introducing spin-scattering centres could open up new possibilities for devices. Here we use spin-polarized neutron reflectivity experiments to demonstrate topologically enhanced interface magnetism by coupling a ferromagnetic insulator (EuS) to a topological insulator (Bi2Se3) in a bilayer system. This interfacial ferromagnetism persists up to room temperature, even though the ferromagnetic insulator is known to order ferromagnetically only at low temperatures (<17 K). The magnetism induced at the interface resulting from the large spin-orbit interaction and the spin-momentum locking of the topological insulator surface greatly enhances the magnetic ordering (Curie) temperature of this bilayer system. The ferromagnetism extends similar to 2 nm into the Bi2Se3 from the interface. Owing to the short-range nature of the ferromagnetic exchange interaction, the time-reversal symmetry is broken only near the surface of a topological insulator, while leaving its bulk states unaffected. The topological magneto-electric response originating in such an engineered topological insulator(2,8) could allow efficient manipulation of the magnetization dynamics by an electric field, providing an energy-efficient topological control mechanism for future spin-based technologies. C1 [Katmis, Ferhat; Wei, Peng; Jarillo-Herrero, Pablo; Moodera, Jagadeesh S.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Katmis, Ferhat; Wei, Peng; Moodera, Jagadeesh S.] MIT, Francis Bitter Magnet Lab, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Katmis, Ferhat; Wei, Peng; Moodera, Jagadeesh S.] MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Lauter, Valeria] Oak Ridge Natl Lab, Neutron Sci Directorate, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Nogueira, Flavio S.; Eremin, Ilya] Ruhr Univ Bochum, Inst Theoret Phys 3, D-44801 Bochum, Germany. [Nogueira, Flavio S.] Inst Festkoerper & Werkstoffforsch Dresden, Inst Theoret Solid State Phys, D-01069 Dresden, Germany. [Assaf, Badih A.; Jamer, Michelle E.; Heiman, Don] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Assaf, Badih A.] Paris Sci & Lettres Res Univ, CNRS, Ecole Normale Super, Dept Phys, F-75005 Paris, France. [Satpati, Biswarup] Saha Inst Nucl Phys, 1-AF Bidhannagar, Kolkata 64, India. [Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Katmis, F; Moodera, JS (reprint author), MIT, Dept Phys, Cambridge, MA 02139 USA.; Katmis, F; Moodera, JS (reprint author), MIT, Francis Bitter Magnet Lab, 77 Massachusetts Ave, Cambridge, MA 02139 USA.; Katmis, F; Moodera, JS (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM katmis@mit.edu; moodera@mit.edu RI Nogueira, Flavio/G-1064-2012; Eremin, Ilya /M-2079-2016 OI Jamer, Michelle/0000-0001-5316-8817; Nogueira, Flavio/0000-0001-7296-5096; Eremin, Ilya /0000-0003-0557-8015 FU Scientific User Facilities Division, Office of Basic Energy Sciences; US Department of Energy; MIT MRSEC through the MRSEC Program of the National Science Foundation [DMR-0819762]; National Science Foundation [DMR-1207469, DMR-0907007, ECCS-1402738]; Office of Naval Research [N00014-13-1-0301]; STC Center for Integrated Quantum Materials under National Science Foundation [DMR-1231319]; US Department of Energy, Basic Energy Sciences Office, Division of Material Sciences and Engineering [DE-SC0006418]; Agence Nationale de la Recherche LabEx grants ENS-ICFP [ANR-10-LABX-0010/ANR-10-IDEX-0001-02 PSL]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; German Research Council (DFG) under the collaborative research centre [SFB TR 12]; German Research Council (DFG) under the priority programme SPP 1666 [ER 463/9] FX F.K. thanks L. Fu, V. Madhavan, N. Gedik, B. Sinkovic, Y. Wang and H. Lin for discussions. V.L. thanks S. Nagler for discussions, and H. Ambaye, A. Glavic and the Spallation Neutron Source staff for support. The research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, and the US Department of Energy. F.K., P.J.-H., and J.S.M. thank the MIT MRSEC through the MRSEC Program of the National Science Foundation under award number DMR-0819762 (upgrade of the molecular beam epitaxy system) for support. J.S.M. thanks the National Science Foundation (DMR-1207469), Office of Naval Research (N00014-13-1-0301) and the STC Center for Integrated Quantum Materials under National Science Foundation grant DMR-1231319 for support, and the thin-film growth and characterization of the materials used. The hetero-structure characterization was supported by the US Department of Energy, Basic Energy Sciences Office, Division of Material Sciences and Engineering under award number DE-SC0006418 (F.K. and P.J.-H.). B.A.A., M.E.J. and D.H. thank the National Science Foundation under award numbers DMR-0907007 and ECCS-1402738 (for SQUID magnetometry characterization) for support. B.A.A. is also supported in part by the Agence Nationale de la Recherche LabEx grants ENS-ICFP (ANR-10-LABX-0010/ANR-10-IDEX-0001-02 PSL). The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract number DE-AC02-06CH11357. I.E. and F.S.N. acknowledge the German Research Council (DFG) for the financial support under the collaborative research centre SFB TR 12 and the priority programme SPP 1666 (grant number ER 463/9). NR 36 TC 11 Z9 11 U1 51 U2 115 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 26 PY 2016 VL 533 IS 7604 BP 513 EP + DI 10.1038/nature17635 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM6EJ UT WOS:000376443100036 PM 27225124 ER PT J AU Jones, CF Bernando, C Tanyag, RMP Bacellar, C Ferguson, KR Gomez, LF Anielski, D Belkacem, A Boll, R Bozek, J Carron, S Cryan, J Englert, L Epp, SW Erk, B Foucar, L Hartmann, R Neumark, DM Rolles, D Rudenko, A Siefermann, KR Weise, F Rudek, B Sturm, FP Ullrich, J Bostedt, C Gessner, O Vilesov, AF AF Jones, Curtis F. Bernando, Charles Tanyag, Rico Mayro P. Bacellar, Camila Ferguson, Ken R. Gomez, Luis F. Anielski, Denis Belkacem, Ali Boll, Rebecca Bozek, John Carron, Sebastian Cryan, James Englert, Lars Epp, Sascha W. Erk, Benjamin Foucar, Lutz Hartmann, Robert Neumark, Daniel M. Rolles, Daniel Rudenko, Artem Siefermann, Katrin R. Weise, Fabian Rudek, Benedikt Sturm, Felix P. Ullrich, Joachim Bostedt, Christoph Gessner, Oliver Vilesov, Andrey F. TI Coupled motion of Xe clusters and quantum vortices in He nanodroplets SO PHYSICAL REVIEW B LA English DT Article ID FREELY ROTATING SUPERFLUID; HELIUM NANODROPLETS; QUANTIZED VORTICES; VORTEX; VISUALIZATION; SPECTROSCOPY; MOLECULES; DROPLETS; DYNAMICS AB Single He nanodroplets doped with Xe atoms are studied via ultrafast coherent x-ray diffraction imaging. The diffraction images show that rotating He nanodroplets about 200 nm in diameter contain a small number of symmetrically arranged quantum vortices decorated with Xe clusters. Unexpected large distances of the vortices from the droplet center (approximate to 0.7-0.8 droplet radii) are explained by a significant contribution of the Xe dopants to the total angular momentum of the droplets and a stabilization of widely spaced vortex configurations by the trapped Xe clusters. C1 [Jones, Curtis F.; Tanyag, Rico Mayro P.; Gomez, Luis F.; Vilesov, Andrey F.] Univ So Calif, Dept Chem, Los Angeles, CA 90089 USA. [Bernando, Charles; Vilesov, Andrey F.] Univ So Calif, Dept Phys & Astron, Los Angeles, CA 90089 USA. [Bacellar, Camila; Belkacem, Ali; Cryan, James; Neumark, Daniel M.; Siefermann, Katrin R.; Weise, Fabian; Sturm, Felix P.; Gessner, Oliver] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Bacellar, Camila; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ferguson, Ken R.; Bozek, John; Carron, Sebastian; Bostedt, Christoph] SLAC Natl Accelerator Lab, LCLS, Linac Coherent Light Source, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Ferguson, Ken R.] Stanford Univ, Dept Appl Phys, Stanford, CA 94063 USA. [Anielski, Denis; Boll, Rebecca; Erk, Benjamin; Foucar, Lutz; Rolles, Daniel; Rudenko, Artem; Rudek, Benedikt; Ullrich, Joachim] Ctr Free Electron Laser Sci CFEL, Max Planck Adv Study Grp, Notkestr 85, D-22607 Hamburg, Germany. [Anielski, Denis; Boll, Rebecca; Erk, Benjamin; Rudenko, Artem; Rudek, Benedikt; Ullrich, Joachim] Max Planck Inst Kernphys, Saupfercheckweg 1, D-69117 Heidelberg, Germany. [Boll, Rebecca; Erk, Benjamin; Rolles, Daniel] Deutsch Elektronen Synchrotron DESY, Notkestr 85, D-22607 Hamburg, Germany. [Englert, Lars] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85741 Garching, Germany. [Epp, Sascha W.] Max Planck Inst Struktur & Dynam Mat, Luruper Chaussee 149, D-22761 Hamburg, Germany. [Foucar, Lutz; Rolles, Daniel] Max Planck Inst Med Res, Jahnstr 29, D-69120 Heidelberg, Germany. [Hartmann, Robert] PNSensor GmbH, Otto Hahn Ring 6, D-81739 Munich, Germany. [Rudek, Benedikt; Ullrich, Joachim] Phys Tech Bundesanstalt, Bundesallee 100, D-38116 Braunschweig, Germany. [Bostedt, Christoph] Stanford Univ, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Bostedt, Christoph] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Bostedt, Christoph] Argonne Natl Lab, 9700 South Cass Ave B109, Argonne, IL 60439 USA. [Bostedt, Christoph] Northwestern Univ, Dept Phys & Astron, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Gomez, Luis F.] IPG Photon, 3930 Freedom Circle,Ste 130, Santa Clara, CA 95054 USA. [Rolles, Daniel; Rudenko, Artem] Kansas State Univ, Dept Phys, JR MacDonald Lab, Manhattan, KS 66506 USA. [Siefermann, Katrin R.] Leibniz Inst Surface Modificat IOM, Permoserstr 15, D-04318 Leipzig, Germany. [Weise, Fabian] Berliner Glas KGaA Herbert Kubatz GmbH & Co, Waldkraiburger Str 5, D-12347 Berlin, Germany. RP Vilesov, AF (reprint author), Univ So Calif, Dept Chem, Los Angeles, CA 90089 USA.; Vilesov, AF (reprint author), Univ So Calif, Dept Phys & Astron, Los Angeles, CA 90089 USA.; Gessner, O (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Bostedt, C (reprint author), SLAC Natl Accelerator Lab, LCLS, Linac Coherent Light Source, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Bostedt, C (reprint author), Stanford Univ, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Bostedt, C (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Bostedt, C (reprint author), Argonne Natl Lab, 9700 South Cass Ave B109, Argonne, IL 60439 USA. EM cbostedt@anl.gov; ogessner@lbl.gov; vilesov@usc.edu RI Neumark, Daniel/B-9551-2009; Bozek, John/E-9260-2010; Rudek, Benedikt/A-5100-2017; Rudenko, Artem/C-7412-2009; OI Neumark, Daniel/0000-0002-3762-9473; Bozek, John/0000-0001-7486-7238; Rudenko, Artem/0000-0002-9154-8463; Epp, Sascha/0000-0001-6366-9113; Boll, Rebecca/0000-0001-6286-4064 FU NSF at USC [DMR-1501276]; US Department of Energy, Office of Basic Energy Sciences (DOE, OBES) Chemical Sciences, Geosciences and Biosciences Division [DE-AC02-05CH11231, DE-AC02-06CH11357, DE-AC02-76SF00515]; Max Planck Society FX This work was supported by NSF Grant DMR-1501276 (A.F.V.) at USC, by the US Department of Energy, Office of Basic Energy Sciences (DOE, OBES) Chemical Sciences, Geosciences and Biosciences Division, through Contracts No. DE-AC02-05CH11231, No. DE-AC02-06CH11357, and No. DE-AC02-76SF00515 and by the Max Planck Society by funding the development and operation of the CAMP instrument within the ASG at CFEL. Portions of this research were carried out at the Linac Coherent Light Source, a national user facility operated by Stanford University on behalf of the US DOE, OBES under beamtime grant L549: Imaging of quantum vortices in superfluid helium droplets. Sebastian Schorb took part in and provided valuable expertise for the measurements taken during LCLS AMO 54912 beamtime of July 2012 as part of the AMO team. Martin Seifrid and Justin Kwok participated as part of the USC team. NR 36 TC 3 Z9 3 U1 6 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2016 VL 93 IS 18 AR 180510 DI 10.1103/PhysRevB.93.180510 PG 6 WC Physics, Condensed Matter SC Physics GA DM8TD UT WOS:000376636500001 ER PT J AU Wang, M Yi, M Sun, HL Valdivia, P Kim, MG Xu, ZJ Berlijn, T Christianson, AD Chi, SX Hashimoto, M Lu, DH Li, XD Bourret-Courchesne, E Dai, PC Lee, DH Maier, TA Birgeneau, RJ AF Wang, Meng Yi, M. Sun, H. L. Valdivia, P. Kim, M. G. Xu, Z. J. Berlijn, T. Christianson, A. D. Chi, Songxue Hashimoto, M. Lu, D. H. Li, X. D. Bourret-Courchesne, E. Dai, Pengcheng Lee, D. H. Maier, T. A. Birgeneau, R. J. TI Experimental elucidation of the origin of the 'double spin resonances' in Ba(Fe1-xCox)(2)As-2 SO PHYSICAL REVIEW B LA English DT Article ID IRON-BASED SUPERCONDUCTORS; T-C SUPERCONDUCTORS; NEUTRON-SCATTERING; EXCITATIONS AB We report a combined study of the spin resonances and superconducting gaps for underdoped (T-c = 19 K), optimally doped (T-c = 25 K), and overdoped (T-c = 19 K) Ba(Fe1-xCox)(2)As-2 single crystalswith inelastic neutron scattering and angle resolved photoemission spectroscopy. We find a quasi-two-dimensional spin resonance whose energy scales with the superconducting gap in all three compounds. In addition, anisotropic low energy spin excitation enhancements in the superconducting state have been deduced and characterized for the under and optimally doped compounds. Our data suggest that the quasi-two-dimensional spin resonance is a spin exciton that corresponds to the spin singlet-triplet excitations of the itinerant electrons. However, the intensity enhancements of the anisotropic spin excitations are dominated by the out-of-plane spin excitations of the ordered moments due to the suppression of damping in the superconducting state. Hence we offer an interpretation of the double energy scales differing from previous interpretations based on anisotropic superconducting energy gaps and systematically explain the doping-dependent trend across the phase diagram. C1 [Wang, Meng; Yi, M.; Valdivia, P.; Xu, Z. J.; Lee, D. H.; Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sun, H. L.; Li, X. D.] Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Inst High Energy Phys, Beijing 100049, Peoples R China. [Kim, M. G.; Bourret-Courchesne, E.; Lee, D. H.; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Berlijn, T.; Maier, T. A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Berlijn, T.; Maier, T. A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Christianson, A. D.; Chi, Songxue] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Hashimoto, M.; Lu, D. H.] SLAS Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Wang, M; Yi, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM wangm@berkeley.edu; mingyi@berkeley.edu RI Dai, Pengcheng /C-9171-2012; Maier, Thomas/F-6759-2012; xu, zhijun/A-3264-2013; Kim, Min Gyu/B-8637-2012; christianson, andrew/A-3277-2016; Chi, Songxue/A-6713-2013; Wang, Meng/E-6595-2012 OI Dai, Pengcheng /0000-0002-6088-3170; Maier, Thomas/0000-0002-1424-9996; xu, zhijun/0000-0001-7486-2015; Kim, Min Gyu/0000-0001-7676-454X; christianson, andrew/0000-0003-3369-5884; Chi, Songxue/0000-0002-3851-9153; Wang, Meng/0000-0002-8232-2331 FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of US Department of Energy [DE-AC02-05-CH11231]; Quantum Materials Program [KC2202]; Office of Basic Energy Sciences U.S. DOE [DE-AC03-76SF008]; U.S. NSF [DMR-1308603, DMR-1362219]; Robert A. Welch Foundation [C-1839]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05-CH11231 with the Quantum Materials Program (KC2202) and the Office of Basic Energy Sciences U.S. DOE Grant No. DE-AC03-76SF008. The RPA calculations were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. The work at Rice was supported by the U.S. NSF-DMR-1308603 and DMR-1362219 (P.D.), and by Robert A. Welch Foundation Grant No. C-1839 (P.D.). The neutron scattering experiments at Oak Ridge National Laboratory's High-Flux Isotope Reactor were sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The ARPES work was performed at the Stanford Synchrotron Radiation Lightsource, which is operated by the Office of Basic Energy Science, U.S. Department of Energy. NR 45 TC 1 Z9 1 U1 4 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2016 VL 93 IS 20 AR 205149 DI 10.1103/PhysRevB.93.205149 PG 7 WC Physics, Condensed Matter SC Physics GA DM8TZ UT WOS:000376638700003 ER PT J AU Williams, SC Johnson, RD Freund, F Choi, S Jesche, A Kimchi, I Manni, S Bombardi, A Manuel, P Gegenwart, P Coldea, R AF Williams, S. C. Johnson, R. D. Freund, F. Choi, Sungkyun Jesche, A. Kimchi, I. Manni, S. Bombardi, A. Manuel, P. Gegenwart, P. Coldea, R. TI Incommensurate counterrotating magnetic order stabilized by Kitaev interactions in the layered honeycomb alpha-Li2IrO3 SO PHYSICAL REVIEW B LA English DT Article ID IRIDATE; LI2IRO3 AB The layered honeycomb magnet alpha-Li2IrO3 has been theoretically proposed as a candidate to display unconventional magnetic behaviour associated with Kitaev interactions between spin-orbit entangled j(eff) = 1/2 magnetic moments on a honeycomb lattice. Here we report single crystal magnetic resonant x-ray diffraction combined with powder magnetic neutron diffraction to reveal an incommensurate magnetic order in the honeycomb layers with Ir magnetic moments counterrotating on nearest-neighbor sites. This unexpected type of magnetic structure for a honeycomb magnet cannot be explained by a spin Hamiltonian with dominant isotropic (Heisenberg) couplings. The magnetic structure shares many key features with the magnetic order in the structural polytypes beta- and gamma-Li2IrO3, understood theoretically to be stabilized by dominant Kitaev interactions between Ir moments located on the vertices of three-dimensional hyperhoneycomb and stripyhoneycomb lattices, respectively. Based on this analogy and a theoretical soft-spin analysis of magnetic ground states for candidate spin Hamiltonians, we propose that Kitaev interactions also dominate in alpha-Li2IrO3, indicative of universal Kitaev physics across all three members of the harmonic honeycomb family of Li2IrO3 polytypes. C1 [Williams, S. C.; Johnson, R. D.; Choi, Sungkyun; Coldea, R.] Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. [Johnson, R. D.; Manuel, P.] Rutherford Appleton Lab STFC, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Freund, F.; Jesche, A.; Manni, S.; Gegenwart, P.] Univ Augsburg, Ctr Elect Correlat & Magnetism, EP VI, D-86159 Augsburg, Germany. [Kimchi, I.] MIT, Dept Phys, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Bombardi, A.] Diamond Light Source Ltd, Harwell Sci & Innovat Campus, Cambridge OX11 0DE, England. [Choi, Sungkyun] Max Planck Inst Solid State Res, Heisenbergstr 1, D-70569 Stuttgart, Germany. [Manni, S.] Iowa State Univ, Ames Lab, Dept Phys & Astron, Ames, IA 50010 USA. RP Williams, SC (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. RI Gegenwart, Philipp/A-7291-2017; Manni, Soham/G-1455-2016 OI Manni, Soham/0000-0001-6279-3497 FU EPSRC (U.K.) [EP/H014934/1, EP/M020517/1]; Royal Society University Research Fellowship; MIT Pappalardo Fellowship; Helmholtz Virtual Institute 521 ("New states of matter and their excitations"); German Science Foundation [TRR-80] FX Work at Oxford was partially supported by the EPSRC (U.K.) under Grants No. EP/H014934/1 and No. EP/M020517/1. R.D.J. acknowledges support from a Royal Society University Research Fellowship. I.K. acknowledges support from an MIT Pappalardo Fellowship. Work at Augsburg was supported by the Helmholtz Virtual Institute 521 ("New states of matter and their excitations") and the German Science Foundation through TRR-80. We thank Diamond Light Source for access to beamline I16 (under proposal MT12028-1) that contributed to the results presented here. In accordance with the EPSRC policy framework on research data, access to the data will be made available from Ref. [32]. NR 27 TC 5 Z9 5 U1 10 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 26 PY 2016 VL 93 IS 19 AR 195158 DI 10.1103/PhysRevB.93.195158 PG 12 WC Physics, Condensed Matter SC Physics GA DM8TP UT WOS:000376637700001 ER PT J AU Greif, M Greiner, C Denicol, GS AF Greif, Moritz Greiner, Carsten Denicol, Gabriel S. TI Electric conductivity of a hot hadron gas from a kinetic approach SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; TRANSPORT MODEL; FLAVOR; COLLABORATION; PERSPECTIVE; DYNAMICS; MATTER; FLOW AB We calculate the electric conductivity of a gas of relativistic particles with isotropic cross sections using the Boltzmann equation as the starting point. Our analysis is restricted to elastic collisions. We show the perfect agreement with previously published numerical results for a massless quark-gluon plasma, and give results for the electric conductivity of an interacting hadron gas, employing realistic resonance cross sections. These results for the electric conductivity of a hot hadron gas, as created in ( ultra) relativistic heavy-ion collisions, are of rich phenomenological as well as theoretical interest and can be compared to, e.g., lattice quantum field theory calculations. C1 [Greif, Moritz; Greiner, Carsten] Goethe Univ Frankfurt, Inst Theoret Phys, Max von Laue Str 1, D-60438 Frankfurt, Germany. [Denicol, Gabriel S.] Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. RP Greif, M (reprint author), Goethe Univ Frankfurt, Inst Theoret Phys, Max von Laue Str 1, D-60438 Frankfurt, Germany. EM greif@th.physik.uni-frankfurt.de RI Silveira Denicol, Gabriel/L-5048-2016 FU DOE [DE-SC0012704]; Helmholtz International Center for FAIR FX M. G. is grateful to "Helmhotz Graduate School for Heavy Ion research." G. S. D. is supported under DOE Contract No. DE-SC0012704. The authors are grateful to the Center for Scientific Computing (CSC) Frankfurt for the computing resources. This work was supported by the Helmholtz International Center for FAIR within the framework of the LOEWE program launched by the State of Hesse. NR 73 TC 2 Z9 2 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 26 PY 2016 VL 93 IS 9 AR 096012 DI 10.1103/PhysRevD.93.096012 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8VE UT WOS:000376641800013 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Frohwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fang, W Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Seva, T Velde, CV Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Delaere, C Delcourt, M Favart, D Forthomme, L Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Leggat, D Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA 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CA CMS Collaboration TI Search for supersymmetry in pp collisions at root s=8 TeV in final states with boosted W bosons and b jets using razor variables SO PHYSICAL REVIEW D LA English DT Article ID PARTON DISTRIBUTIONS; SQUARK; EXTENSION; NEUTRINO; HIGGS; LHC AB A search for supersymmetry in hadronic final states with highly boosted W bosons and b jets is presented, focusing on compressed scenarios. The search is performed using proton-proton collision data at a center-of-mass energy of 8 TeV, collected by the CMS experiment at the LHC, corresponding to an integrated luminosity of 19.7 fb(-1). Events containing candidates for hadronic decays of boosted W bosons are identified using jet substructure techniques, and are analyzed using the razor variables M-R and R-2, which characterize a possible signal as a peak on a smoothly falling background. The observed event yields in the signal regions are found to be consistent with the expected contributions from standard model processes, which are predicted using control samples in the data. The results are interpreted in terms of gluino-pair production followed by their exclusive decay into top squarks and top quarks. The analysis excludes gluino masses up to 1.1 TeV for light top squarks decaying solely to a charm quark and a neutralino, and up to 700 GeV for heavier top squarks decaying solely to a top quark and a neutralino. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Froehwirth, R.; Ghete, V. 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[Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. 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[Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Rome, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Gulmini, M.; Lacaprara, S.; Margoni, M.; Meneguzzo, T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. 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[Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Roma, Rome, Italy. [Aleksandrov, A.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. 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Casimiro; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno; Vazquez Valencia, F.; Salazar Ibarguen, H. A.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Morelos Pineda, A.; Krofcheck, D.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Butler, P. H.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Ahmad, A.] Univ Auckland, Auckland 1, New Zealand. [Ahmad, M.] Univ Canterbury, Christchurch 1, New Zealand. [Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. 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Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Szillasi, Z.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Bonacorsi, D.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Del Re, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, I.; Wardle, N.; Whri, K.; Zagozdzinska, A.; Zeuner, D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Aleksandrov, A.; Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Cerati, G. B.; Holzner, A.; Klein, D.; Olivito, D.; Vartak, A.; Welke, C.; Wurthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Yoo, J.; Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.; Acosta, J. G.] Univ Minnesota, Minneapolis, MN USA. [Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Pirou, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Kumar, A.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.] Univ Tennessee, Knoxville, TN USA. [Thapa, K.; Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.] Univ Wisconsin, Madison, WI USA. [Froehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.; Savoy-Navarro, A.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.; Elgammal, S.; Mahmoud, M. A.] British Univ Egypt, Cairo, Egypt. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J-L; Conte, E.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. Wigner Res Ctr Phys, Budapest, Hungary. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.; Azzurri, P.; Ulmer, K. A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Gulmini, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, A.; Grippo, T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Md Ali, B.] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Madagascar. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Di Marco, E.] Univ Rome, INFN Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens 11528, Greece. [Veres, I.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. 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RI Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Chistov, Ruslan/B-4893-2014; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Chadeeva, Marina/C-8789-2016; Danilov, Mikhail/C-5380-2014; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Lokhtin, Igor/D-7004-2012; Mora Herrera, Maria Clemencia/L-3893-2016; Della Ricca, Giuseppe/B-6826-2013; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; OI Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Chistov, Ruslan/0000-0003-1439-8390; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Chadeeva, Marina/0000-0003-1814-1218; Danilov, Mikhail/0000-0001-9227-5164; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie-Curie program; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science - European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR Project (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Chulalongkorn University (Thailand); Chulalongkorn Academic into its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and the National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and the Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and the National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, Contract No. C-1845. NR 87 TC 1 Z9 1 U1 17 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 26 PY 2016 VL 93 IS 9 AR 092009 DI 10.1103/PhysRevD.93.092009 PG 31 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8VE UT WOS:000376641800001 ER PT J AU Denicol, G Monnai, A Schenke, B AF Denicol, Gabriel Monnai, Akihiko Schenke, Bjorn TI Moving Forward to Constrain the Shear Viscosity of QCD Matter SO PHYSICAL REVIEW LETTERS LA English DT Article ID NONLINEAR GLUON EVOLUTION; COLOR GLASS CONDENSATE; HEAVY-ION COLLISIONS; RENORMALIZATION-GROUP; HIGH-ENERGIES; SCATTERING; EQUATION; FLOW; PROTON; QUARK AB We demonstrate that measurements of rapidity differential anisotropic flow in heavy-ion collisions can constrain the temperature dependence of the shear viscosity to entropy density ratio eta/s of QCD matter. Comparing results from hydrodynamic calculations with experimental data from the RHIC, we find evidence for a small eta/s approximate to 0.04 in the QCD crossover region and a strong temperature dependence in the hadronic phase. A temperature independent eta/s is disfavored by the data. We further show that measurements of the event-by-event flow as a function of rapidity can be used to independently constrain the initial state fluctuations in three dimensions and the temperature dependent transport properties of QCD matter. C1 [Denicol, Gabriel; Schenke, Bjorn] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Monnai, Akihiko] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Denicol, G (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RI Silveira Denicol, Gabriel/L-5048-2016 FU RIKEN Special Postdoctoral Researcher program; U.S. DOE [DE-SC0012704]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE Office of Science Early Career grant FX A. M. is supported by the RIKEN Special Postdoctoral Researcher program. G. S. D. and B. P. S. are supported under U.S. DOE Contract No. DE-SC0012704. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B. P. S. acknowledges receipt of a DOE Office of Science Early Career grant. NR 65 TC 5 Z9 5 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 26 PY 2016 VL 116 IS 21 AR 212301 DI 10.1103/PhysRevLett.116.212301 PG 6 WC Physics, Multidisciplinary SC Physics GA DM8PZ UT WOS:000376627700004 PM 27284652 ER PT J AU Mohanty, D Dahlberg, K King, DM David, LA Sefat, AS Wood, DL Daniel, C Dhar, S Mahajan, V Lee, M Albano, F AF Mohanty, Debasish Dahlberg, Kevin King, David M. David, Lamuel A. Sefat, Athena S. Wood, David L. Daniel, Claus Dhar, Subhash Mahajan, Vishal Lee, Myongjai Albano, Fabio TI Modification of Ni-Rich FCG NMC and NCA Cathodes by Atomic Layer Deposition: Preventing Surface Phase Transitions for High-Voltage Lithium-Ion Batteries SO SCIENTIFIC REPORTS LA English DT Article ID HIGH-ENERGY; CYCLING PERFORMANCE; STRUCTURAL-CHANGES; HIGH-CAPACITY; HIGH-POWER; FADE; LINI0.4MN0.4CO0.2O2; TRANSFORMATION; DIFFRACTION; PERSPECTIVE AB The energy density of current lithium-ion batteries (LIBs) based on layered LiMO2 cathodes (M = Ni, Mn, Co: NMC; M = Ni, Co, Al: NCA) needs to be improved significantly in order to compete with internal combustion engines and allow for widespread implementation of electric vehicles (EVs). In this report, we show that atomic layer deposition (ALD) of titania (TiO2) and alumina (Al2O3) on Ni-rich FCG NMC and NCA active material particles could substantially improve LIB performance and allow for increased upper cutoff voltage (UCV) during charging, which delivers significantly increased specific energy utilization. Our results show that Al2O3 coating improved the NMC cycling performance by 40% and the NCA cycling performance by 34% at 1 C/-1 C with respectively 4.35 V and 4.4 V UCV in 2 Ah pouch cells. High resolution TEM/SAED structural characterization revealed that Al2O3 coatings prevented surface-initiated layered-to-spinel phase transitions in coated materials which were prevalent in uncoated materials. EIS confirmed that Al2O3-coated materials had significantly lower increase in the charge transfer component of impedance during cycling. The ability to mitigate degradation mechanisms for Ni-rich NMC and NCA illustrated in this report provides insight into a method to enable the performance of high-voltage LIBs. C1 [Mohanty, Debasish; David, Lamuel A.; Wood, David L.; Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN USA. [Dahlberg, Kevin; Dhar, Subhash] Energy Power Syst LLC, Pontiac, MI USA. [King, David M.] PneumatiCoat Technol LLC, Broomfield, CO USA. [Sefat, Athena S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. [Wood, David L.; Daniel, Claus] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN USA. [Dhar, Subhash; Mahajan, Vishal; Lee, Myongjai] XALT Energy LLC, Midland, MI USA. [Albano, Fabio] Univ Michigan, Dept Mat Sci & Engn, 2300 Hayward St, Ann Arbor, MI 48109 USA. RP Mohanty, D; Wood, DL (reprint author), Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN USA.; Dahlberg, K (reprint author), Energy Power Syst LLC, Pontiac, MI USA.; Wood, DL (reprint author), Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN USA. EM debasisdm1@gmail.com; kdahlberg@energypowersystems.com; wooddl@ornl.gov RI Daniel, Claus/A-2060-2008; Sefat, Athena/R-5457-2016; OI Daniel, Claus/0000-0002-0571-6054; Sefat, Athena/0000-0002-5596-3504; David, Lamuel/0000-0002-6407-7897; Wood, David/0000-0002-2471-4214 FU U.S. Department of Energy (DOE) [DE-EE0005384, NFE-11-03678, TSA 14-587, LS-111201A-MMW]; Office of Energy Efficiency and Renewable Energy for the Vehicle Technologies Office; Vehicle Technologies Office [DE-SC0010230]; DOE Basic Energy Sciences (BES), Materials Sciences and Engineering Division FX The research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the U.S. Department of Energy (DOE) under contract No. DE-EE0005384, subcontracts Nos NFE-11-03678, TSA 14-587 and LS-111201A-MMW, was sponsored by the Office of Energy Efficiency and Renewable Energy for the Vehicle Technologies Office (Program Managers: Dave Howell and Peter Faguy). Work performed at PneumatiCoat Technologies under contract No. DE-SC0010230 was also sponsored by the Vehicle Technologies Office (Program Manager: Brian Cunningham). Microscopy was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Part of this research was supported by the DOE Basic Energy Sciences (BES), Materials Sciences and Engineering Division. The authors also acknowledge BASF for supply of the electrolyte for pouch cell scale up. NR 36 TC 4 Z9 4 U1 70 U2 138 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 26 PY 2016 VL 6 AR 26532 DI 10.1038/srep26532 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM7ZQ UT WOS:000376580500001 PM 27226071 ER PT J AU Wang, WJ Zhang, HH Kuzmenko, I Mallapragada, S Vaknin, D AF Wang, Wenjie Zhang, Honghu Kuzmenko, Ivan Mallapragada, Surya Vaknin, David TI Assembling Bare Au Nanoparticles at Positively Charged Templates SO SCIENTIFIC REPORTS LA English DT Article ID DNA-CAPPED NANOPARTICLES; AIR-LIQUID INTERFACE; COLLOIDAL CRYSTALS; PHASE-TRANSITIONS; REAL-TIME; CRYSTALLIZATION; MONOLAYERS; PROTEIN; SALT AB In-situ X-ray reflectivity (XRR) and grazing incidence X-ray small-angle scattering (GISAXS) reveal that unfunctionalized (bare) gold nanoparticles (AuNP) spontaneously adsorb to a cationic lipid template formed by a Langmuir monolayer of DPTAP (1,2-dihexadecanoyl-3-trimethylammonium-propane) at vapor/aqueous interfaces. Analysis of the XRR yields the electron density profile across the charged-interfaces along the surface normal showing the AuNPs assemble with vertical thickness comparable to the particle size. The GISAXS analysis indicates that the adsorbed mono-particle layer exhibits short-range in-plane correlations. By contrast, single-stranded DNA-functionalized AuNPs, while attracted to the positively charged surface (more efficiently with the addition of salt to the solution), display less in-plane regular packing compared to bare AuNPs. C1 [Wang, Wenjie; Zhang, Honghu; Mallapragada, Surya; Vaknin, David] US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Zhang, Honghu] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kuzmenko, Ivan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Lemont, IL 60439 USA. [Mallapragada, Surya] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Wang, WJ; Vaknin, D (reprint author), US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA.; Vaknin, D (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM wwang@ameslab.gov; vaknin@ameslab.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358]; U.S. DOE [DE-AC02-06CH11357] FX We thank Xiaobin Zuo at beamline 12ID-B, APS, for technical support in measuring bulk SAXS. H. Z. thanks Prof. Mufit Akinc (Ames Laboratory and Iowa State University) for discussion on functionalization of AuNPs with DNA. Research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 42 TC 2 Z9 2 U1 9 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 26 PY 2016 VL 6 AR 26462 DI 10.1038/srep26462 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM7GP UT WOS:000376525900001 PM 27225047 ER PT J AU Brunk, E George, KW Alonso-Gutierrez, J Thompson, M Baidoo, E Wang, G Petzold, CJ McCloskey, D Monk, J Yang, L O'Brien, EJ Batth, TS Martin, HG Feist, A Adams, PD Keasling, JD Palsson, BO Lee, TS AF Brunk, Elizabeth George, Kevin W. Alonso-Gutierrez, Jorge Thompson, Mitchell Baidoo, Edward Wang, George Petzold, Christopher J. McCloskey, Douglas Monk, Jonathan Yang, Laurence O'Brien, Edward J. Batth, Tanveer S. Martin, Hector Garcia Feist, Adam Adams, Paul D. Keasling, Jay D. Palsson, Bernhard O. Lee, Taek Soon TI Characterizing Strain Variation in Engineered E.coli Using a Multi-Omics-Based Workflow SO CELL SYSTEMS LA English DT Article ID HETEROLOGOUS MEVALONATE PATHWAY; ESCHERICHIA-COLI; SYNTHETIC BIOLOGY; ADVANCED BIOFUELS; SYSTEMS BIOLOGY; PROTEOMICS; PROTEINS; EXPRESSION; POLY(3-HYDROXYBUTYRATE); BIOTECHNOLOGY AB Understanding the complex interactions that occur between heterologous and native biochemical pathways represents a major challenge in metabolic engineering and synthetic biology. We present a workflow that integrates metabolomics, proteomics, and genome-scale models of Escherichia coli metabolism to study the effects of introducing a heterologous pathway into a microbial host. This workflow incorporates complementary approaches from computational systems biology, metabolic engineering, and synthetic biology; provides molecular insight into how the host organism microenvironment changes due to pathway engineering; and demonstrates how biological mechanisms underlying strain variation can be exploited as an engineering strategy to increase product yield. As a proof of concept, we present the analysis of eight engineered strains producing three biofuels: isopentenol, limonene, and bisabolene. Application of this workflow identified the roles of candidate genes, pathways, and biochemical reactions in observed experimental phenomena and facilitated the construction of a mutant strain with improved productivity. The contributed workflow is available as an open-source tool in the form of iPython notebooks. C1 [Brunk, Elizabeth; George, Kevin W.; Alonso-Gutierrez, Jorge; Thompson, Mitchell; Baidoo, Edward; Wang, George; Petzold, Christopher J.; Batth, Tanveer S.; Martin, Hector Garcia; Adams, Paul D.; Keasling, Jay D.; Lee, Taek Soon] JBEI, Joint Bioenergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. [Brunk, Elizabeth; McCloskey, Douglas; Monk, Jonathan; Yang, Laurence; O'Brien, Edward J.; Feist, Adam; Palsson, Bernhard O.] Univ Calif San Diego, Dept Bioengn, San Diego, CA 92093 USA. [Brunk, Elizabeth; George, Kevin W.; Alonso-Gutierrez, Jorge; Baidoo, Edward; Wang, George; Petzold, Christopher J.; Martin, Hector Garcia; Feist, Adam; Keasling, Jay D.; Lee, Taek Soon] Lawrence Berkeley Natl Lab, Biol Syst Engn Div, Berkeley, CA 94720 USA. [Thompson, Mitchell] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Keasling, Jay D.; Palsson, Bernhard O.] Tech Univ Denmark, Novo Nordisk Fdn Ctr Biosustainabil, DK-2970 Horsholm, Denmark. [Adams, Paul D.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [George, Kevin W.] Amyris, 5885 Hollis St, Emeryville, CA 94608 USA. RP Lee, TS (reprint author), JBEI, Joint Bioenergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA.; Palsson, BO (reprint author), Univ Calif San Diego, Dept Bioengn, San Diego, CA 92093 USA.; Lee, TS (reprint author), Lawrence Berkeley Natl Lab, Biol Syst Engn Div, Berkeley, CA 94720 USA.; Palsson, BO (reprint author), Tech Univ Denmark, Novo Nordisk Fdn Ctr Biosustainabil, DK-2970 Horsholm, Denmark. EM palsson@eng.ucsd.edu; tslee@lbl.gov OI Garcia Martin, Hector/0000-0002-4556-9685 FU Joint BioEnergy Institute; US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Swiss National Science Foundation [p2elp2_148961]; National Institutes of Health [GM057089]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Joint BioEnergy Institute (http://www.jbei.org/), which is supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy (to K.W.G., J.A.-G., M.T., H.G.M., E.B., C.J.P., P.D.A., J.D.K., and T.S.L.); the Swiss National Science Foundation (grant p2elp2_148961 to E.B.); and the National Institutes of Health (grant GM057089 to B.O.P.). This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also gratefully acknowledge Dr. Daniel Zielinski, Dr. Aarash Bordbar, Chris Shymansky, Jennifer Gin, Dr. Josh Lerman, and Professor Vassily Hatzimanikatis for early input in the project as well as Ali Ebrahim for technical support. The United States Government retains, and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 53 TC 4 Z9 4 U1 3 U2 4 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 2405-4712 EI 2405-4720 J9 CELL SYST JI Cell Syst. PD MAY 25 PY 2016 VL 2 IS 5 BP 335 EP 346 DI 10.1016/j.cels.2016.04.004 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA EL1DG UT WOS:000394360100008 PM 27211860 ER PT J AU Zhang, W Bock, DC Pelliccione, CJ Li, Y Wu, LJ Zhu, YM Marschilok, AC Takeuchi, ES Takeuchi, KJ Wang, F AF Zhang, Wei Bock, David C. Pelliccione, Christopher J. Li, Yan Wu, Lijun Zhu, Yimei Marschilok, Amy. C. Takeuchi, Esther S. Takeuchi, Kenneth J. Wang, Feng TI Insights into Ionic Transport and Structural Changes in Magnetite during Multiple-Electron Transfer Reactions SO ADVANCED ENERGY MATERIALS LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; RECHARGEABLE LITHIUM BATTERIES; CRYSTALLITE SIZE CONTROL; X-RAY; NANOCRYSTALLINE MAGNETITE; CONVERSION REACTIONS; SPINEL ELECTRODES; CATHODE MATERIALS; ANODE MATERIAL; FINE-STRUCTURE AB Metal oxides, such as Fe3O4, hold promise for future battery applications due to their abundance, low cost, and opportunity for high lithium storage capacity. In order to better understand the mechanisms of multiple-electron transfer reactions leading to high capacity in Fe3O4, a comprehensive investigation on local ionic transport and ordering is made by probing site occupancies of anions (O2-) and cations (Li+, Fe3+ /Fe2+) using multiple synchrotron X-ray and electron-beam techniques, in combination with ab-initio calculations. Results from this study provide the first experimental evidence that the cubic-close-packed (ccp) O-anion array in Fe3O4 is sustained throughout the lithiation and delithiation processes, thereby enabling multiple lithium intercalation and conversion reactions. Cation displacement/reordering occurs within the ccp O-anion framework, which leads to a series of phase transformations, starting from the inverse spinel phase and turning into intermediate rock-salt-like phases (LixFe3O4; 0 < x < 2), then into a cation-segregated phase (Li O-2 center dot FeO), and finally converting into metallic Fe and Li2O. Subsequent delithiation and lithiation processes involve interconversion between metallic Fe and FeO-like phases. These results may offer new insights into the structure-determined ionic transport and electrochemical reactions in metal oxides, and those of other compounds sharing a ccp anion framework, reminiscent of magnetite. C1 [Zhang, Wei; Bock, David C.; Pelliccione, Christopher J.; Wu, Lijun; Zhu, Yimei; Takeuchi, Esther S.; Wang, Feng] Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. [Li, Yan] Amer Phys Soc, Ridge, NY 11961 USA. [Marschilok, Amy. C.; Takeuchi, Esther S.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11974 USA. [Marschilok, Amy. C.; Takeuchi, Esther S.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11974 USA. RP Wang, F (reprint author), Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA.; Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11974 USA.; Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11974 USA. EM kenneth.takeuchi.1@stonybrook.edu; fwang@bnl.gov FU Center for Mesoscale Transport Properties, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012673]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Use Facilities Division; Materials Science and Engineering Division [DE-SC0012704] FX This work was supported as part of the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under award #DE-SC0012673. Work at Brookhaven, including the use of the National Synchrotron Light Source I, was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Use Facilities Division, as well as Materials Science and Engineering Division under Contract No. DE-SC0012704. The authors gratefully acknowledge Dr. Melissa C. Menard for the original collection of the XAS data. NR 69 TC 4 Z9 4 U1 15 U2 27 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY 25 PY 2016 VL 6 IS 10 AR 1502471 DI 10.1002/aenm.201502471 PG 11 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DQ6JH UT WOS:000379310200007 ER PT J AU Dumitrescu, CE Mueller, CJ Kurtz, E AF Dumitrescu, Cosmin E. Mueller, Charles J. Kurtz, Eric TI Investigation of a tripropylene-glycol monomethyl ether and diesel blend for soot-free combustion in an optical direct-injection diesel engine SO APPLIED THERMAL ENGINEERING LA English DT Article DE Diesel; Soot-free combustion; Oxygenate; LLFC AB Natural luminosity and chemiluminescence imaging diagnostics were employed to investigate if a 50/50 blend by volume of tripropylene-glycol monomethyl ether (TPGME) and ultra-low sulfur #2 diesel certification fuel (CF) could enable leaner-lifted flame combustion (LLFC), a non-sooting mode of mixing controlled combustion associated with equivalence ratios below approximately 2. The experiments were performed in a single-cylinder heavy-duty optical compression-ignition engine at three injection pressures and three dilution levels. Results indicate that TPGME addition effectively eliminated engine-out smoke emissions by curtailing soot production and/or increasing soot oxidation during and after the end of fuel injection. TPGME greatly reduced soot luminosity when compared with neat CF, but did not enable LLFC because the equivalence ratios at the lift-off length, phi(H), never reached the non-sooting limit and incandescence from hot soot within the combustion chambered remained visible. Concerning other engine out emissions, injection pressure influenced the effects of TPGME addition on NO. emissions. HC and CO emissions were higher compared to the baseline fuel, likely due to the lower net heat of combustion of TPGME and the need to limit fuel-injection duration for valid optical measurements. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Dumitrescu, Cosmin E.] West Virginia Univ, 275 Engn Sci Bldg, Morgantown, WV 26506 USA. [Mueller, Charles J.] Sandia Natl Labs, 7011 East Ave, Livermore, CA 94550 USA. [Kurtz, Eric] Ford Motor Co, 1 Amer Rd, Dearborn, MI 48126 USA. RP Dumitrescu, CE (reprint author), West Virginia Univ, 275 Engn Sci Bldg, Morgantown, WV 26506 USA. EM cosmin.dumitrescu@mail.wvu.edu FU U.S. Department of Energy (DOE); West Virginia University FX The experimental data were acquired while author Dumitrescu was employed by Sandia National Laboratories and funded by the U.S. Department of Energy (DOE). Preparation of this manuscript was performed while author Dumitrescu was employed and funded by West Virginia University. NR 36 TC 2 Z9 2 U1 5 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-4311 J9 APPL THERM ENG JI Appl. Therm. Eng. PD MAY 25 PY 2016 VL 101 BP 639 EP 646 DI 10.1016/j.applthermaleng.2015.12.068 PG 8 WC Thermodynamics; Energy & Fuels; Engineering, Mechanical; Mechanics SC Thermodynamics; Energy & Fuels; Engineering; Mechanics GA DR0ZU UT WOS:000379636500062 ER PT J AU Weiner, RG Chen, DP Unocic, RR Skrabalak, SE AF Weiner, Rebecca G. Chen, Dennis P. Unocic, Raymond R. Skrabalak, Sara E. TI Impact of Membrane-Induced Particle Immobilization on Seeded Growth Monitored by In Situ Liquid Scanning Transmission Electron Microscopy SO SMALL LA English DT Article ID AU; NANOPARTICLES; NANOCRYSTALS; NANOSTRUCTURES; SIZE; MORPHOLOGY; KINETICS C1 [Weiner, Rebecca G.; Chen, Dennis P.; Skrabalak, Sara E.] Indiana Univ, Dept Chem, 800 E Kirkwood Ave, Bloomington, IN 47405 USA. [Unocic, Raymond R.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Skrabalak, SE (reprint author), Indiana Univ, Dept Chem, 800 E Kirkwood Ave, Bloomington, IN 47405 USA. EM sskrabal@indiana.edu FU Indiana University; National Science Foundation (NSF) [CHE-1306853] FX R.G.W. and D.P.C. contributed equally to this work. This work was supported by start-up funds from Indiana University and National Science Foundation (NSF) Award CHE-1306853. Electron microscopy was conducted as part of a user proposal at Oak Ridge National Laboratory's Center for Nanophase Materials Sciences (CNMS), a U.S. Department of Energy Office of Science User Facility. The authors thank Dr. Koczkur for his assistance in video processing. NR 30 TC 4 Z9 4 U1 7 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD MAY 25 PY 2016 VL 12 IS 20 BP 2701 EP 2706 DI 10.1002/smll.201502974 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DP3VQ UT WOS:000378424400003 PM 27038413 ER PT J AU Chang, CJ AF Chang, Christopher J. TI A Triple Crown of Sustainable Synthesis SO ACS CENTRAL SCIENCE LA English DT Editorial Material C1 [Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Howard Hughes Med Inst, Dept Chem, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Howard Hughes Med Inst, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Helen Wills Neurosci Inst, Div Chem Sci, Berkeley, CA 94720 USA. RP Chang, CJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Howard Hughes Med Inst, Dept Chem, Berkeley, CA 94720 USA.; Chang, CJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Howard Hughes Med Inst, Dept Mol & Cell Biol, Berkeley, CA 94720 USA.; Chang, CJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Helen Wills Neurosci Inst, Div Chem Sci, Berkeley, CA 94720 USA. EM chrischang@berkeley.edu NR 4 TC 0 Z9 0 U1 3 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD MAY 25 PY 2016 VL 2 IS 5 BP 266 EP 267 DI 10.1021/acscentsci.6b00144 PG 2 WC Chemistry, Multidisciplinary SC Chemistry GA DO5LW UT WOS:000377825600001 PM 27280158 ER PT J AU Hartwig, JF Larsen, MA AF Hartwig, John F. Larsen, Matthew A. TI Undirected, Homogeneous C-H Bond Functionalization: Challenges and Opportunities SO ACS CENTRAL SCIENCE LA English DT Article ID LATE-STAGE FUNCTIONALIZATION; CATALYZED DIRECT ARYLATION; ALKYL ISOMERIZATION EQUILIBRIA; ALKANE DEHYDROGENATION; ASYMMETRIC-SYNTHESIS; OMEGA-HYDROXYLATION; ORGANIC-SYNTHESIS; METHYL ARYLDIAZOACETATES; C(SP(3))-H AMINATION; DIOXYGEN ACTIVATION AB The functionalization of C-H bonds has created new approaches to preparing organic molecules by enabling new strategic "disconnections" during the planning of a synthetic route. Such functionalizations also have created the ability to derivatize complex molecules by modifying one or more of the many C-H bonds. For these reasons, researchers are developing new types of functionalization reactions of C-H bonds and new applications of these processes. These C-H bond functionalization reactions can be divided into two general classes: those directed by coordination to an existing functional group prior to the cleavage of the C-H bond (directed) and those occurring without coordination prior to cleavage of the C-H bond (undirected). The undirected functionalizations of C-H bonds are much less common and more challenging to develop than the directed reactions. This outlook will focus on undirected C-H bond functionalization, as well as related reactions that occur by a noncovalent association of the catalyst prior to C-H bond cleavage. The inherent challenges of conducting undirected functionalizations of C-H bonds and the methods for undirected functionalization that are being developed will be presented, along with the factors that govern selectivity in these reactions. Finally, this outlook discusses future directions for research on undirected C-H functionalization, with an emphasis on the limitations that must be overcome if this type of methodology is to become widely used in academia and in industry. C1 [Hartwig, John F.; Larsen, Matthew A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hartwig, John F.; Larsen, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Hartwig, JF (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Hartwig, JF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jhartwig@berkeley.edu FU NIGMS NIH HHS [R29 GM055382, R01 GM055382, R01 GM115812, R37 GM055382] NR 142 TC 24 Z9 24 U1 36 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD MAY 25 PY 2016 VL 2 IS 5 BP 281 EP 292 DI 10.1021/acscentsci.6b00032 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA DO5LW UT WOS:000377825600006 PM 27294201 ER PT J AU Fuemmeler, EG Sanders, SN Pun, AB Kumarasamy, E Zeng, T Miyata, K Steigerwald, ML Zhu, XY Sfeir, MY Campos, LM Ananth, N AF Fuemmeler, Eric G. Sanders, Samuel N. Pun, Andrew B. Kumarasamy, Elango Zeng, Tao Miyata, Kiyoshi Steigerwald, Michael L. Zhu, X. -Y. Sfeir, Matthew Y. Campos, Luis M. Ananth, Nandini TI A Direct Mechanism of Ultrafast Intramolecular Singlet Fission in Pentacene Dimers SO ACS CENTRAL SCIENCE LA English DT Article ID EXCITON FISSION; ELECTRONIC-STRUCTURE; CRYSTALLINE TETRACENE; THIN-FILMS; BASIS-SETS; STATES; MOLECULES; MODEL; DYNAMICS; PHOTOVOLTAICS AB Interest in materials that undergo singlet fission (SF) has been catalyzed by the potential to exceed the Shockley-Queisser limit of solar power conversion efficiency. In conventional materials, the mechanism of SF is an intermolecular process (xSF), which is mediated by charge transfer (CT) states and depends sensitively on crystal packing or molecular collisions. In contrast, recently reported covalently coupled pentacenes yield similar to 2 triplets per photon absorbed in individual molecules: the hallmark of intramolecular singlet fission (iSF). However, the mechanism of iSF is unclear. Here, using multireference electronic structure calculations and transient absorption spectroscopy, we establish that iSF can occur via a direct coupling mechanism that is independent of CT states. We show that a near-degeneracy in electronic state energies induced by vibronic coupling to intramolecular modes of the covalent dimer allows for strong mixing between the correlated triplet pair state and the local excitonic state, despite weak direct coupling. C1 [Fuemmeler, Eric G.; Zeng, Tao; Ananth, Nandini] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. [Sanders, Samuel N.; Pun, Andrew B.; Kumarasamy, Elango; Miyata, Kiyoshi; Steigerwald, Michael L.; Zhu, X. -Y.; Campos, Luis M.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Zeng, Tao] Carleton Univ, Dept Chem, Ottawa, ON K1S 5B6, Canada. RP Ananth, N (reprint author), Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA.; Campos, LM (reprint author), Columbia Univ, Dept Chem, New York, NY 10027 USA.; Sfeir, MY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM msfeir@bnl.gov; lcampos@columbia.edu; ananth@cornell.edu RI Miyata, Kiyoshi/L-2358-2016; OI Miyata, Kiyoshi/0000-0001-6748-1337; Kumarasamy, Elango/0000-0002-7995-6894 NR 71 TC 12 Z9 12 U1 25 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD MAY 25 PY 2016 VL 2 IS 5 BP 316 EP 324 DI 10.1021/acscentsci.6b00063 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DO5LW UT WOS:000377825600010 PM 27280166 ER PT J AU Mahmoud, ME Nabil, GM El-Mallah, NM Bassiouny, HI Kumar, S Abdel-Fattah, TM AF Mahmoud, Mohamed E. Nabil, Gehan M. El-Mallah, Nabila M. Bassiouny, Heba I. Kumar, Sandeep Abdel-Fattah, Tarek M. TI Kinetics, isotherm, and thermodynamic studies of the adsorption of reactive red 195 A dye from water by modified Switchgrass Biochar adsorbent SO JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY LA English DT Article DE Reactive red 195 A dye; Switchgrass Biochar; Thermodynamic parameters; Kinetic study; Adsorption isotherm models ID ACTIVATED CARBON; AQUEOUS-SOLUTION; METHYLENE-BLUE; COMPONENT SYSTEMS; MALACHITE GREEN; REMOVAL; EQUILIBRIUM; ACID; MECHANISM; 2,4,6-TRICHLOROPHENOL AB A method is described for efficient decolorization of reactive red 195 A dye (RR-195A) from aqueous and wastewater samples using modified Switchgrass Biochar (SB) by tetradecyltrimethyl ammonium bromide (TTAB) as a cationic surfactant for the formation of a novel SB-TTAB adsorbent. The different controlling experimental conditions such as solution pH, initial dye concentration, contact time, adsorbent mass, interfering ions and temperature have been investigated and optimized. Adsorption equilibrium using Langmuir, Freundlich, Temkin and Dubinin-Radushkevich (D-R) isotherm models have been also studied and the best fit was related to the Langmuir adsorption isotherm. Adsorption kinetics have been tested and illustrated using pseudo first-order, pseudo-second-order, intraparticle diffusion and Elovich models. The collected results confirmed that the pseudo-second order kinetic model exhibited the best fit with the experimental data. Thermodynamic parameters were calculated and the results referred to an exothermic nature and spontaneity of the adsorption process. Improved decolorization of reactive red 195 A dye from textile industrial wastewater and other water samples were successfully established. Excellent recovery values of RR-195A dye by SB-TTAB adsorbent were determined in the ranges of 96.61-98.76%, 97.79-99.26%, 94.24-100.0% and 90.98-92.96% (+/- 1.0-4.0%) from tap water, raw water, wastewater and sea water, respectively. (C) 2016 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved. C1 [Mahmoud, Mohamed E.; Nabil, Gehan M.; El-Mallah, Nabila M.; Bassiouny, Heba I.] Univ Alexandria, Dept Chem, Fac Sci, POB 426, Alexandria, Egypt. [Kumar, Sandeep] Old Dominion Univ, Dept Civil & Environm Engn, Norfolk, VA 23529 USA. [Abdel-Fattah, Tarek M.] Christopher Newport Univ, Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. [Abdel-Fattah, Tarek M.] Christopher Newport Univ, Dept Mol Biol & Chem, Newport News, VA 23606 USA. RP Abdel-Fattah, TM (reprint author), Christopher Newport Univ, Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA.; Abdel-Fattah, TM (reprint author), Christopher Newport Univ, Dept Mol Biol & Chem, Newport News, VA 23606 USA. EM fattah@cnu.edu NR 36 TC 5 Z9 5 U1 12 U2 23 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1226-086X EI 1876-794X J9 J IND ENG CHEM JI J. Ind. Eng. Chem. PD MAY 25 PY 2016 VL 37 BP 156 EP 167 DI 10.1016/j.jiec.2016.03.020 PG 12 WC Chemistry, Multidisciplinary; Engineering, Chemical SC Chemistry; Engineering GA DO4FL UT WOS:000377737100022 ER PT J AU Ibanez, GC Senanayake, S Kubacka, A AF Colon Ibanez, Gerardo Senanayake, Sanjaya Kubacka, Anna TI Hydrogen from oxygenated molecules Preface SO APPLIED CATALYSIS A-GENERAL LA English DT Editorial Material C1 [Colon Ibanez, Gerardo] Inst Mat Sevilla, C Amer Vespucio 49, Seville 41092, Spain. [Senanayake, Sanjaya] Brookhaven Natl Lab, Dept Chem, Bldg 555, Upton, NY 11973 USA. [Kubacka, Anna] CSIC, Inst Catalisis & Petr Quim, C Marie Curie 2, Madrid 28049, Spain. RP Kubacka, A (reprint author), CSIC, Inst Catalisis & Petr Quim, C Marie Curie 2, Madrid 28049, Spain. EM ak@icp.csic.es RI Senanayake, Sanjaya/D-4769-2009 OI Senanayake, Sanjaya/0000-0003-3991-4232 NR 0 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD MAY 25 PY 2016 VL 518 BP 1 EP 1 DI 10.1016/j.apcata.2016.03.003 PG 1 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA DN8DO UT WOS:000377309600001 ER PT J AU Nguyen-Phan, TD Baber, AE Rodriguez, JA Senanayake, SD AF Thuy-Duong Nguyen-Phan Baber, Ashleigh E. Rodriguez, Jose A. Senanayake, Sanjaya D. TI Au and Pt nanoparticle supported catalysts tailored for H-2 production: From models to powder catalysts SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Gold; Platinum; Supported catalyst; Water-gas shift; Steam reforming; Water splitting ID WATER-GAS-SHIFT; PHOTOCATALYTIC HYDROGEN-PRODUCTION; NOBLE-METAL CATALYSTS; TEMPERATURE CO OXIDATION; GOLD NANOPARTICLES; VISIBLE-LIGHT; PARTICLE-SIZE; SPECTROSCOPIC CHARACTERIZATION; OXYGENATED HYDROCARBONS; ETHYLENE HYDROGENATION AB The use of metal nanoparticles (NPs), including Au and Pt, supported over oxides has been pivotal, and is ever increasing in enabling catalytic reactions which target the production of hydrogen. We review here the most recent works pertaining to the fundamental understanding of the structure, morphology, growth, characterization, and intrinsic phenomenological properties of Au- and Pt-based catalysts that influence the reactivity and selectivity to target hydrogen production. We draw on surface science and theoretical methods of model and powder catalysts using high resolution imaging, spectroscopy, scattering experiments, and theoretical studies. Based on these insights we identify key aspects of studies of supported metal nanoparticle (NP) catalysts for several reactions. The main focus of this review is on the intersection of catalytic chemistry related to the water-gas shift (WGS), oxygenate steam reforming (OSR), and solar-assisted reactions (SAR). (C) 2015 Elsevier B.V. All rights reserved. C1 [Thuy-Duong Nguyen-Phan; Rodriguez, Jose A.; Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Baber, Ashleigh E.] James Madison Univ, Dept Chem & Biochem, Harrisonburg, VA 22807 USA. [Rodriguez, Jose A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Nguyen-Phan, TD; Senanayake, SD (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM nguyenphanthuyduong@gmail.com; ssenanay@bnl.gov RI Nguyen Phan, Thuy Duong/C-8751-2014; Senanayake, Sanjaya/D-4769-2009 OI Senanayake, Sanjaya/0000-0003-3991-4232 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and Catalysis Science Program [DE-SC0012704] FX The work carried out at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and Catalysis Science Program under contract No. DE-SC0012704. NR 213 TC 1 Z9 1 U1 18 U2 52 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD MAY 25 PY 2016 VL 518 BP 18 EP 47 DI 10.1016/j.apcata.2015.12.012 PG 30 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA DN8DO UT WOS:000377309600003 ER PT J AU Brady, MP Leonard, DN Meyer, HM Thomson, JK Unocic, KA Elsentriecy, HH Song, GL Kitchen, K Davis, B AF Brady, M. P. Leonard, D. N. Meyer, H. M., III Thomson, J. K. Unocic, K. A. Elsentriecy, H. H. Song, G. -L. Kitchen, K. Davis, B. TI Advanced characterization study of commercial conversion and electrocoating structures on magnesium alloys AZ31B and ZE10A SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Magnesium; Conversion coating; Electrocoating; Corrosion; Transmission electron microscopy ID MG ALLOY; AUTOMOTIVE APPLICATIONS; FLUORIDE SOLUTIONS; ALUMINUM-ALLOY; SURFACE-FILMS; CORROSION; COATINGS; MECHANISM; PRETREATMENT; PERFORMANCE AB The local metal-coating interface microstructure and chemistry formed on commercial magnesium alloys Mg-3Al-1Zn (AZ31B) and Mg-1Zn-0.25Zr-<0.5Nd (ZE10A, ZEK100 type) were analyzed as-chemical conversion coated with a commercial hexafluoro-titanate/zirconate type + organic polymer based treatment (Bonderite (R) 5200) and a commercial hexafluoro-zirconate type + trivalent chromium Cr3+ type treatment (Surtec (R) 650), and after the same conversion coatings followed by electrocoating with an epoxy based coating, Cathoguard (R) 525. Characterization techniques included scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS), and cross-section scanning transmission electron microscopy (STEM). Corrosion behavior was assessed in room temperature saturated aqueous Mg(OH)(2) solution with 1 wt.% NaCl. The goal of the effort was to assess the degree to which substrate alloy additions become enriched in the conversion coating, and how the conversion coating was impacted by subsequent electrocoating. Key findings included the enrichment of Al from AZ31B and Zr from ZE10A, respectively, into the conversion coating, with moderate corrosion resistance benefits for AZ31B when Al was incorporated. Varying degrees of increased porosity and modification of the initial conversion coating chemistry at the metal-coating interface were observed after electrocoating. These changes were postulated to result in degraded electrocoating protectiveness. These observations highlight the challenges of coating Mg, and the need to tailor electrocoating in light of potential degradation of the initial as-conversion coated Mg alloy surface. (C) 2016 Elsevier B.V. All rights reserved. C1 [Brady, M. P.; Leonard, D. N.; Meyer, H. M., III; Thomson, J. K.; Unocic, K. A.; Elsentriecy, H. H.; Song, G. -L.] Oak Ridge Natl Lab, MS 6156, Oak Ridge, TN 37831 USA. [Elsentriecy, H. H.] Cent Met Res & Dev Inst, Cairo, Egypt. [Kitchen, K.; Davis, B.] Magnesium Elektron North Amer, Madison, IL USA. [Song, G. -L.] Xiamen Univ, Coll Mat, Fujian 361005, Peoples R China. RP Brady, MP (reprint author), Oak Ridge Natl Lab, MS 6156, Oak Ridge, TN 37831 USA. EM bradymp@ornl.gov RI Brady, Michael/A-8122-2008 OI Brady, Michael/0000-0003-1338-4747 FU U.S. DOE EERE Vehicle Technologies Office [DE-AC05-00OR22725] FX The authors thank D.W. Coffey, T.M. Lowe, T. Geer and T.L. Jordan for assistance with the experimental work. M. Lance, B. Armstrong, and B.A. Pint provided helpful comments for this manuscript. This research was sponsored by the U.S. DOE EERE (DE-AC05-00OR22725) Vehicle Technologies Office. TEM/STEM characterization work made use of capabilities at the ORNL Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 51 TC 0 Z9 0 U1 9 U2 26 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD MAY 25 PY 2016 VL 294 BP 164 EP 176 DI 10.1016/j.surfcoat.2016.03.066 PG 13 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DN8FV UT WOS:000377315500023 ER PT J AU Wilfong, WC Kail, BW Jones, CW Pacheco, C Gray, ML AF Wilfong, Walter Christopher Kail, Brian W. Jones, Christopher W. Pacheco, Carlos Gray, McMahan L. TI Spectroscopic Investigation of the Mechanisms Responsible for the Superior Stability of Hybrid Class 1/Class 2 CO2 Sorbents: A New Class 4 Category SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE CO2 capture; hybrid; Class 4; amine sorbent; infrared spectroscopy; NMR ID CARBON-DIOXIDE CAPTURE; TEMPERATURE SWING ADSORPTION; SUPPORTED AMINE SORBENTS; HOLLOW-FIBER SORBENTS; SILICA-GEL; FLUIDIZED-BED; ADSORBED CO2; OXIDATIVE-DEGRADATION; SOLID SORBENTS; AMBIENT AIR AB Hybrid Class 1/Class 2 supported amine CO2 sorbents demonstrate superior performance under practical steam conditions, yet their amine immobilization and stabilization mechanisms are unclear. Uncovering the interactions responsible for the sorbents' robust features is critical for further improvements and can facilitate practical applications. We employ solid state Si-29 CP-MAS and 2-D FSLG H-1-C-13 CP HETCOR NMR spectroscopies to probe the overall molecular interactions of aminosilane/silica, polyamine [poly(ethylenimine), PEI]/silica, and hybrid aminosilane/PEI/silica sorbents. A unique, sequential impregnation sorbent preparation method is executed in a diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS) setup to decouple amine binding mechanisms at the amine silica interfacefrom those within bulk amine layers. These mechanisms are correlated with each sorbents' resistance to accelerated liquid H2O and TGA steam treatments (H2O stability) and to oxidative degradation (thermal stability). High percentages of CO2 capture retained (PCR) and organic content retained (OCR) values after H2O testing of N-(3-(trimethoxysilyl)propyl)ethylenediamine (TMPED)/PEI and (3-aminopropyl)trimethoxysilane (APTMS)/PEI hybrid sorbents are associated with a synergistic stabilizing effect of the amine species observed during oxidative degradation (thermal gravimetric analysis-differential scanning calorimetry, TGA-DSC). Solid state NMR spectroscopy reveals that the synergistic effect of the TMPED/PEI mixture is manifested by the formation of hydrogen-bonded PEI NH2 center dot center dot center dot NH2 TMPED and PEI NH2 HO Si/O Si-O (TMPED, T-2) linkages within the sorbent. DRIFTS further determines that PEI enhances the grafting of TMPED to silica and that PEI is dispersed among a stable network of polymerized TMPED in the bulk, utilizing H-bonded linkages. These findings provide the scientific basis for establishing a Class 4 category for aminosilane/polyamine/silica hybrid sorbents. C1 [Wilfong, Walter Christopher; Gray, McMahan L.] US DOE, Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Wilfong, Walter Christopher] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Kail, Brian W.] AECOM, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Pacheco, Carlos] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Jones, Christopher W.] Georgia Inst Technol, Sch Chem & Biomol Engn, 311 Ferst Dr, Atlanta, GA 30332 USA. RP Wilfong, WC; Gray, ML (reprint author), US DOE, Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA.; Wilfong, WC (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM Walter.Wilfong@netl.doe.gov; Mac.Gray@netl.doe.gov OI Pacheco, Carlos/0000-0002-5607-5517 FU Department of Energy, National Energy Technology Laboratory, an agency of the United States Government; AECOM; U.S. Department of Energy; National Energy Technology Laboratory under the RES [DE-FE0004000]; NSF [CBET-1403239] FX This project was funded by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with AECOM. This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. A portion of this technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. C.W.J. acknowledges support from NSF via CBET-1403239. NR 66 TC 4 Z9 4 U1 7 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 25 PY 2016 VL 8 IS 20 BP 12780 EP 12791 DI 10.1021/acsami.6b02062 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DN1KX UT WOS:000376825800027 PM 27145200 ER PT J AU Mei, DL Yuan, XX Ma, Z Wei, P Yu, XB Yang, J Ma, ZF AF Mei, Delong Yuan, Xianxia Ma, Zhong Wei, Ping Yu, Xuebin Yang, Jun Ma, Zi-Feng TI A SnO2-Based Cathode Catalyst for Lithium-Air Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE tin dioxide; carbon coated tin dioxide; cathode catalyst; microstructure; Li-air batteries ID RECHARGEABLE LI-O-2 BATTERIES; ION BATTERIES; EFFICIENT ELECTROCATALYST; SNO2 NANOPARTICLES; STORAGE PROPERTIES; OXYGEN-ELECTRODE; CARBON CATHODE; PERFORMANCE; NANOWIRES; COMPOSITE AB SnO2 and SnO2@C have been successfully synthesized with a simple hydrothermal procedure combined with heat treatment, and their performance as cathode catalysts of Li-air batteries has been comparatively evaluated and discussed. The results show that both SnO2 and SnO2@C are capable of catalyzing oxygen reduction reactions (ORR) and oxygen evolution reactions (OER) at the cathode of Li-air batteries, but the battery with SnO2@C displays better performance due to its unique higher conductivity, larger surface area, complex pore distribution, and huge internal space. C1 [Mei, Delong; Yuan, Xianxia; Ma, Zhong; Yang, Jun; Ma, Zi-Feng] Shanghai Jiao Tong Univ, Dept Chem Engn, Shanghai 200240, Peoples R China. [Wei, Ping] Nanning Univ, Sch Mech Elect & Qual Technol Engn, Nanning 532999, Guangxi, Peoples R China. [Yu, Xuebin] Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China. [Ma, Zhong] Brookhaven Natl Lab, Energy & Photon Sci Directorate, Upton, NY 11973 USA. RP Yuan, XX (reprint author), Shanghai Jiao Tong Univ, Dept Chem Engn, Shanghai 200240, Peoples R China. EM yuanxx@sjtu.edu.cn RI Yuan, Xianxia/A-4256-2009; Yu, Xuebin/E-9785-2012 FU National Key Basic Research Program of China [2014CB932303]; National Natural Science Foundation of China [21176155, 21476138] FX The authors are grateful for the financial support of this work by National Key Basic Research Program of China (2014CB932303) and the National Natural Science Foundation of China (21176155 and 21476138). NR 48 TC 2 Z9 2 U1 16 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 25 PY 2016 VL 8 IS 20 BP 12804 EP 12811 DI 10.1021/acsami.6602402 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DN1KX UT WOS:000376825800030 PM 27152996 ER PT J AU Ding, H Dwaraknath, SS Garten, L Ndione, P Ginley, D Persson, KA AF Ding, Hong Dwaraknath, Shyam S. Garten, Lauren Ndione, Paul Ginley, David Persson, Kristin A. TI Computational Approach for Epitaxial Polymorph Stabilization through Substrate Selection SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE epitaxy; substrate selection; topology; elastic energy; homoepitaxy; heteroepitaxy ID AUGMENTED-WAVE METHOD; PHASE-TRANSITION; VANADIUM-OXIDE; GROWTH; VO2; HETEROEPITAXY; SPECTROSCOPY; BROOKITE AB With the ultimate goal of finding new polymorphs through targeted synthesis conditions and techniques, we outline a computational framework to select optimal substrates for epitaxial growth using first principle calculations of formation energies, elastic strain energy, and topological information. To demonstrate the approach, we study the stabilization of metastable VO2 compounds which provides a rich chemical and structural polymorph space. We find that common polymorph statistics, lattice matching, and energy above hull considerations recommends homostructural growth on TiO2 substrates, where the VO2 brookite phase would be preferentially grown on the a-c TiO2 brookite plane while the columbite and anatase structures favor the a-b plane on the respective TiO2 phases. Overall, we find that a model which incorporates a geometric unit cell area matching between the substrate and the target film as well as the resulting strain energy density of the film provide qualitative agreement with experimental observations for the heterostructural growth of known VO2 polymorphs: rutile, A and B phases. The minimal interfacial geometry matching and estimated strain energy criteria provide several suggestions for substrates and substrate film orientations for the heterostructural growth of the hitherto hypothetical anatase, brookite, and columbite polymorphs. These criteria serve as a preliminary guidance for the experimental efforts stabilizing new materials and/or polymorphs through epitaxy. The current screening algorithm is being integrated within the Materials Project online framework and data and hence publicly available. C1 [Ding, Hong; Dwaraknath, Shyam S.; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol, Berkeley, CA 94720 USA. [Garten, Lauren; Ndione, Paul; Ginley, David] Natl Renewable Energy Lab, Mat Chem Sci & Technol, Golden, CO 80401 USA. [Persson, Kristin A.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94704 USA. RP Persson, KA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol, Berkeley, CA 94720 USA.; Persson, KA (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94704 USA. EM kapersson@lbl.gov OI Dwaraknath, Shyam/0000-0003-0289-2607 FU Center for Next Generation Materials by Design an Energy Frontier Research Center - the U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-05CH11231, DE-AC36-089028308]; Office of Science of the U.S. Department of Energy FX This work was supported as part of the Center for Next Generation Materials by Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Awards DE-AC02-05CH11231 and DE-AC36-089028308. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy. The Materials Project (BES DOE Grant EDCBEE) is acknowledged for infrastructure and algorithmic support. We gratefully acknowledge Dr. John Perkins for his helpful discussion in compiling this manuscript. NR 41 TC 4 Z9 4 U1 15 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 25 PY 2016 VL 8 IS 20 BP 13086 EP 13093 DI 10.1021/acsami.6b01630 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DN1KX UT WOS:000376825800063 PM 27145398 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connellb, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDCS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadellid, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Du, Y Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunforda, M Yildiz, HD Duren, M Durglishvili, A Duschinger, D Dutta, B Dyndala, M Eckardt, C Ecker, KM Edgar, RC Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Elliot, AA Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Erdmann, J Ereditato, A Ernis, G Ernst, J Ernst, M Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Giannelli, MF Favareto, A Fayard, L Fedin, OL Fedorko, W Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Feremenga, L Martinez, PF Perez, SF Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M 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Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Reconstruction of hadronic decay products of tau leptons with the ATLAS experiment SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PP COLLISIONS; ROOT-S=7 TEV; CROSS-SECTION; HIGGS-BOSON; DETECTOR; SEARCH; LHC; MASS AB This paper presents a new method of reconstructing the individual charged and neutral hadrons in tau decays with the ATLAS detector. The reconstructed hadrons are used to classify the decay mode and to calculate the visible four-momentum of reconstructed tau candidates, significantly improving the resolution with respect to the calibration in the existing tau reconstruction. The performance of the reconstruction algorithm is optimised and evaluated using simulation and validated using samples of Z -> tau tau and Z(-> mu mu)+jets events selected from proton-proton collisions at a centre-of-mass energy root s = 8 TeV, corresponding to an integrated luminosity of 5 fb(-1). C1 [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; TenKate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.; ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Corriveau, F.; Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; LeCompte, T.; Love, J.; Malon, D.; Metcalfe, J.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Stanek, R. W.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Webster, J. S.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E. St.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-Zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Barcelona Inst Sci & Technol, IFAE, Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin dit; Sjursen, T. B.; Smestad, L.; Stugu, B.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Invalidenstr 110, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Gach, G. P.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Abdinov, O.; Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Khalil-Zada, F.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadellid, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurerb, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Araya, S. Tapia] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Geng, C.; Jin, S.; Li, B.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndala, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Aloisio, A.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Kneke, K.; Kopp, A. 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Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gaudiello, A.; Gemme, C.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. 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W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunforda, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. 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[Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandi, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. 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A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; TicseTorres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; TicseTorres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. 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P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Alonso, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst Russian, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. 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A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Knig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Marti, L. F.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Marti, L. F.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, CNRS, IN2P3,LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Recherches Lois Fondamentales Unive, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Salvatore, F.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connellb, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron & Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Shi, L.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. 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[Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. 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RI Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Boyko, Igor/J-3659-2013; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Shulga, Evgeny/R-1759-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Stabile, Alberto/L-3419-2016; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Gladilin, Leonid/B-5226-2011; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016 OI Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Shulga, Evgeny/0000-0001-5099-7644; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Robson, Aidan/0000-0002-1659-8284; Beck, Hans Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Terzo, Stefano/0000-0003-3388-3906; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Cristinziani, Markus/0000-0003-3893-9171; Galhardo, Bruno/0000-0003-0641-301X; Pina, Joao /0000-0001-8959-5044; Farrington, Sinead/0000-0001-5350-9271; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694; Stabile, Alberto/0000-0002-6868-8329; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Gladilin, Leonid/0000-0001-9422-8636; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 43 TC 0 Z9 0 U1 17 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 25 PY 2016 VL 76 IS 5 AR 295 DI 10.1140/epjc/s10052-016-4110-0 PG 26 WC Physics, Particles & Fields SC Physics GA DN2YP UT WOS:000376929300001 ER PT J AU Hosseinzadeh, P Tian, SL Marshall, NM Hemp, J Mullen, T Nilges, MJ Gao, YG Robinson, H Stahl, DA Gennis, RB Lu, Y AF Hosseinzadeh, Parisa Tian, Shiliang Marshall, Nicholas M. Hemp, James Mullen, Timothy Nilges, Mark J. Gao, Yi-Gui Robinson, Howard Stahl, David A. Gennis, Robert B. Lu, Yi TI A Purple Cupredoxin from Nitrosopumilus maritimus Containing a Mononuclear Type 1 Copper Center with an Open Binding Site SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PSEUDOMONAS-AERUGINOSA AZURIN; AMMONIA-OXIDIZING ARCHAEA; ELECTRON-TRANSFER; NITROSOMONAS-EUROPAEA; NITRIC-OXIDE; BLUE; PROTEINS; OXIDATION; DIVERSITY; COMMUNITY AB Mononuclear cupredoxin proteins usually contain a coordinately saturated type 1 copper (T1Cu) center and function exclusively as electron carriers. Here we report a cupredoxin isolated from the nitrifying archaeon Nitrosopumilus maritimus SCM1, called Nmar1307, that contains a T1Cu center with an open binding site containing water. It displays a deep purple color due to strong absorptions around 413 nm (1880 M-1 cm(-1)) and 558 nm (2290 M-1 cm(-1)) in the UV-vis electronic spectrum. EPR studies suggest the protein contains two Cu(II) species of nearly equal population, one nearly axial, with hyperfine constant A(parallel to) = 98 x 10(-4) cm(-1), and another more rhombic, with a smaller value of 69 x 10(-4) cm(-1). The X-ray crystal structure at 1.6 angstrom resolution confirms that it contains a Cu atom coordinated by two His and one Cys in a trigonal plane, with an axial H2O at 2.25 angstrom. Both UV-vis absorption and EPR spectroscopic studies suggest that the Nmar1307 can oxidize NO to nitrite, an activity that is attributable to the high reduction potential (354 mV vs SHE) of the copper site. These results suggest that mononuclear cupredoxins can have a wide range of structural features, including an open binding site containing water, making this class of proteins even more versatile. C1 [Hosseinzadeh, Parisa; Hemp, James; Gennis, Robert B.; Lu, Yi] Univ Illinois, Dept Biochem, Urbana, IL 61801 USA. [Tian, Shiliang; Marshall, Nicholas M.; Mullen, Timothy; Gennis, Robert B.; Lu, Yi] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Gao, Yi-Gui] Univ Illinois, Biocrystallizat Facil, Urbana, IL 61801 USA. [Nilges, Mark J.] Univ Illinois, EPR Ctr, Urbana, IL 61801 USA. [Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Stahl, David A.] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. RP Gennis, RB; Lu, Y (reprint author), Univ Illinois, Dept Biochem, Urbana, IL 61801 USA.; Gennis, RB; Lu, Y (reprint author), Univ Illinois, Dept Chem, Urbana, IL 61801 USA. EM r-gennis@illinois.edu; yi-lu@illinois.edu RI Lu, Yi/B-5461-2010; OI Lu, Yi/0000-0003-1221-6709; Hemp, James/0000-0001-7193-0553 FU National Science Foundation [CHE-1413328]; National Institutes of Health [NIH HL16101]; NSF from Molecular and Cellular Biosciences [MCB-06044482, MCB-0949807]; NSF from Biological Oceanography [OCE-1046017] FX This Communication is based on work supported by the National Science Foundation under Award CHE-1413328 (to Y.L.) and the National Institutes of Health under Award NIH HL16101 (to R.B.G.), with partial support by NSF Awards from Molecular and Cellular Biosciences MCB-06044482 and MCB-0949807, and Biological Oceanography OCE-1046017 (to D.A.S.). The authors acknowledge Mr. Jason Varnell and Prof. Andrew Gewirth for their help in electrochemistry experiments. The authors would also like to thanks Mr. Junjie Li for his help with protein purificaiton. The authors also thank Dr. Igor Petrik for his help in crystal structure deposition to PDB. NR 58 TC 2 Z9 2 U1 6 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2016 VL 138 IS 20 BP 6324 EP 6327 DI 10.1021/jacs.5b13128 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DN1KY UT WOS:000376825900002 PM 27120678 ER PT J AU Liu, JL Lucci, FR Yang, M Lee, S Marcinkowski, MD Therrien, AJ Williams, CT Sykes, ECH Flytzani-Stephanopoulos, M AF Liu, Jilei Lucci, Felicia R. Yang, Ming Lee, Sungsik Marcinkowski, Matthew D. Therrien, Andrew J. Williams, Christopher T. Sykes, E. Charles H. Flytzani-Stephanopoulos, Maria TI Tackling CO Poisoning with Single-Atom Alloy Catalysts SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBON-MONOXIDE OXIDATION; SELECTIVE HYDROGENATION; CU(111); CU3PT(111); ADSORPTION; PALLADIUM; SURFACES AB Platinum catalysts are extensively used in the chemical industry and as electrocatalysts in fuel cells. Pt is notorious for its sensitivity to poisoning by strong CO adsorption. Here we demonstrate that the single-atom alloy (SAA) strategy applied to Pt reduces the binding strength of CO while maintaining catalytic performance. By using surface sensitive studies, we determined the binding strength of CO to different Pt ensembles, and this in turn guided the preparation of PtCu alloy nanoparticles (NPs). The atomic ratio Pt:Cu = 1:125 yielded a SAA which exhibited excellent CO tolerance in H-2 activation, the key elementary step for hydrogenation and hydrogen electro-oxidation. As a probe reaction, the selective hydrogenation of acetylene to ethene was performed under flow conditions on the SAA NPs supported on alumina without activity loss in the presence of CO. The ability to maintain reactivity in the presence of CO is vital to other industrial reaction systems, such as hydrocarbon oxidation, electrochemical methanol oxidation, and hydrogen fuel cells. C1 [Liu, Jilei; Yang, Ming; Flytzani-Stephanopoulos, Maria] Tufts Univ, Dept Chem & Biol Engn, 4 Colby St, Medford, MA 02155 USA. [Lucci, Felicia R.; Marcinkowski, Matthew D.; Therrien, Andrew J.; Sykes, E. Charles H.] Tufts Univ, Dept Chem, 62 Talbot Ave, Medford, MA 02155 USA. [Lee, Sungsik] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Williams, Christopher T.] Univ S Carolina, Dept Chem Engn, 301 Main St, Columbia, SC 29208 USA. RP Flytzani-Stephanopoulos, M (reprint author), Tufts Univ, Dept Chem & Biol Engn, 4 Colby St, Medford, MA 02155 USA.; Sykes, ECH (reprint author), Tufts Univ, Dept Chem, 62 Talbot Ave, Medford, MA 02155 USA. EM charles.sykes@tufts.edu; maria.flytzani-stephanopoulos@tufts.edu FU National Science Foundation [CBET-1159882]; U.S. Department of Energy [DE-FG02-05ER15730, DE-FG02-10ER16170]; Tufts University Department of Chemistry; DOE Office of Science [DE-AC02-06CH11357] FX We dedicate this work to the memory of Howard Saltsburg. We thank the National Science Foundation (CBET-1159882 to J.L.), and the U.S. Department of Energy (DE-FG02-05ER15730 to A.J.T. and M.F-S. and DE-FG02-10ER16170 to F.R.L. and E.C.H.S.) for the financial support of this work. M.D.M. thanks the Tufts University Department of Chemistry for an Illumina Fellowship. J.L. thanks Prof. Terry Haas (Tufts University) for assistance with the IR analysis. The XAS research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE), Office of Science, User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 23 TC 7 Z9 7 U1 71 U2 138 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2016 VL 138 IS 20 BP 6396 EP 6399 DI 10.1021/jacs.6b03339 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DN1KY UT WOS:000376825900020 PM 27167705 ER PT J AU Ziegler, MS Levine, DS Lakshmi, KV Tilley, TD AF Ziegler, Micah S. Levine, Daniel S. Lakshmi, K. V. Tilley, T. Don TI Aryl Group Transfer from Tetraarylborato Anions to an Electrophilic Dicopper(I) Center and Mixed-Valence mu-Aryl Dicopper(I,II) Complexes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NUCLEAR MAGNETIC-RESONANCE; DENSITY-FUNCTIONAL THEORY; COPPER(I) COMPLEXES; X-RAY; MACROCYCLIC LIGANDS; REACTION-MECHANISMS; EXCITED-STATES; BOND-CLEAVAGE; COORDINATION; OXIDATION AB The synthesis of discrete, cationic binuclear mu-aryl dicopper complexes [Cu-2(mu-eta(1):eta(1)-Ar)DPFN]X (Ar = C6H5, 3,5-(CF3)(2)C6H3, and C6F5; DPFN = 2,7-bis(fluoro-di(2-pyridy1)methyl)-1,8-naphthyridine; X = BAr4- and NTf2-; Tf = SO2CF3) was achieved by treatment of a dicopper complex [Cu-2(mu-eta(1):eta(1)-NCCH3)DPFN]X-2 (X = PF6- and NTf2-) with tetraarylborates. Structural characterization revealed symmetrically bridging aryl groups, and H-1 NMR spectroscopy evidenced the same structure in solution at 24 degrees C. Electrochemical investigation of the resulting arylcopper complexes uncovered reversible redox events that led to the synthesis and isolation of a rare mixed-valence organocopper complex [Cu-2(mu-eta(1):eta(1)--Ph)DPFN](NTf2)(2) in high yield. The solid-state structure of the mixed-valence mu-phenyl complex exhibits inequivalent copper centers, despite a short Cu center dot center dot center dot Cu distance. Electronic and variable-temperature electron paramagnetic resonance spectroscopy of the mixed-valence mu-phenyl complex suggest that the degree of spin localization is temperature-dependent, with a high degree of spin localization observed at lower temperatures. Electronic structure calculations agree with the experimental results and suggest that the spin is localized almost entirely on one metal center. C1 [Ziegler, Micah S.; Levine, Daniel S.; Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ziegler, Micah S.; Tilley, T. Don] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Lakshmi, K. V.] Rensselaer Polytech Inst, Dept Chem & Chem Biol, Troy, NY 12180 USA. [Lakshmi, K. V.] Rensselaer Polytech Inst, Baruch Ctr Biochem Solar Energy Res 60, Troy, NY 12180 USA. RP Tilley, TD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Tilley, TD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM tdtilley@berkeley.edu RI Lakshmi, K. V./A-9787-2017 OI Lakshmi, K. V./0000-0001-5443-9017 FU Office of Science, Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231, DE-FG02-07ER15903]; National Institutes of Health [S10-RR027172, SRR023679A, 1S10RR016634-01]; Joint Center for Artificial Photosynthesis, a U.S. Department of Energy, Office of Science, Basic Energy Sciences Innovation Hub [DE-SC0004993]; National Science Foundation (NSF) [DGE 1106400]; Philomathia Graduate Student Fellowship in the Environmental Sciences; NSF FX We thank Allegra L. Liberman-Martin, Timothy C. Davenport, Hyun S. Ahn, Teera Chantarojsiri, Rebecca A. Green, Jennifer E. Laaser, Hsueh-Ju Liu, Andy I. Nguyen, Patrick W. Smith, Narbe Mardirossian, and James P. Dombrowski for useful conversations. We also thank Michael L. Aubrey for electrochemical equipment and Philip C. Bunting for assistance with UV-vis-NIR spectroscopy. Finally, we thank Antonio G. DiPasquale for X-ray crystallography advice and Hasan Celik, Jeffery G. Pelton, and Chris Canlas for NMR spectroscopy advice. This work was supported by the Director, Office of Science, Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (T.D.T.) and DE-FG02-07ER15903 (K.V.L.). We acknowledge the National Institutes of Health for funding the UC Berkeley CheXray X-ray crystallographic facility under Grant No. S10-RR027172 and the UC Berkeley College of Chemistry NMR facility under Grant Nos. SRR023679A and 1S10RR016634-01, as well as the Joint Center for Artificial Photosynthesis, a U.S. Department of Energy, Office of Science, Basic Energy Sciences Innovation Hub, under Grant No. DE-SC0004993, for EPR facilities. In addition, M.S.Z. was supported by a National Science Foundation (NSF) Graduate Research Fellowship (Grant No: DGE 1106400) and Philomathia Graduate Student Fellowship in the Environmental Sciences, and D.S.L. was also supported by a NSF Graduate Research Fellowship. We thank Boulder Scientific Company for a donation of KBArF20. NR 65 TC 2 Z9 2 U1 9 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 25 PY 2016 VL 138 IS 20 BP 6484 EP 6491 DI 10.1021/jacs.6b00802 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DN1KY UT WOS:000376825900034 PM 27176131 ER PT J AU Keiter, DA Cunningham, FL Rhodes, OE Irwin, BJ Beasley, JC AF Keiter, David A. Cunningham, Fred L. Rhodes, Olin E., Jr. Irwin, Brian J. Beasley, James C. TI Optimization of Scat Detection Methods for a Social Ungulate, the Wild Pig, and Experimental Evaluation of Factors Affecting Detection of Scat SO PLOS ONE LA English DT Article ID BOAR SUS-SCROFA; POPULATION-SIZE; SOUTH-CAROLINA; FECAL DNA; DEER; SELECTION; GENETICS; IMPACT; RANGE; FECES AB Collection of scat samples is common in wildlife research, particularly for genetic capture-mark-recapture applications. Due to high degradation rates of genetic material in scat, large numbers of samples must be collected to generate robust estimates. Optimization of sampling approaches to account for taxa-specific patterns of scat deposition is, therefore, necessary to ensure sufficient sample collection. While scat collection methods have been widely studied in carnivores, research to maximize scat collection and noninvasive sampling efficiency for social ungulates is lacking. Further, environmental factors or scat morphology may influence detection of scat by observers. We contrasted performance of novel radial search protocols with existing adaptive cluster sampling protocols to quantify differences in observed amounts of wild pig (Sus scrofa) scat. We also evaluated the effects of environmental (percentage of vegetative ground cover and occurrence of rain immediately prior to sampling) and scat characteristics (fecal pellet size and number) on the detectability of scat by observers. We found that 15- and 20-m radial search protocols resulted in greater numbers of scats encountered than the previously used adaptive cluster sampling approach across habitat types, and that fecal pellet size, number of fecal pellets, percent vegetative ground cover, and recent rain events were significant predictors of scat detection. Our results suggest that use of a fixed-width radial search protocol may increase the number of scats detected for wild pigs, or other social ungulates, allowing more robust estimation of population metrics using noninvasive genetic sampling methods. Further, as fecal pellet size affected scat detection, juvenile or smaller-sized animals may be less detectable than adult or large animals, which could introduce bias into abundance estimates. Knowledge of relationships between environmental variables and scat detection may allow researchers to optimize sampling protocols to maximize utility of noninvasive sampling for wild pigs and other social ungulates. C1 [Keiter, David A.; Rhodes, Olin E., Jr.; Beasley, James C.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC USA. [Keiter, David A.; Beasley, James C.] Univ Georgia, DB Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. [Cunningham, Fred L.] US Anim & Plant Hlth Inspect Serv, Natl Wildlife Res Ctr, USDA, Starkville, MS USA. [Rhodes, Olin E., Jr.] Univ Georgia, Odum Sch Ecol, Athens, GA 30602 USA. [Irwin, Brian J.] Univ Georgia, DB Warnell Sch Forestry & Nat Resources, Georgia Cooperat Fish & Wildlife Res Unit, US Geol Survey, Athens, GA 30602 USA. RP Keiter, DA (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC USA.; Keiter, DA (reprint author), Univ Georgia, DB Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. EM david.keiter@gmail.com FU United States Department of Energy [DE-FC09-07SR22506]; United States Department of Agriculture, Animal and Plant Health Inspection Service, Wildlife Services, National Wildlife Research Center; U.S. Geological Survey; Georgia Department of Natural Resources; U.S. Fish and Wildlife Service; University of Georgia; Wildlife Management Institute; United States Government FX Funding for this research was provided by the United States Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation and the United States Department of Agriculture, Animal and Plant Health Inspection Service, Wildlife Services, National Wildlife Research Center (https://www.aphis.usda.gov/wps/portal/aphis/ourfocus/wildlifedamage?uri le=wcm%3Apath%3A%2FAPHIS_Content_Library%2FSA_Our_Focus%2FSA_Wildlife_Da mage%2FSA_Programs%2FSA_NWRC). Researchers at the USDA-APHIS National Wildlife Research Center participated in design of this study and preparation of the manuscript.; We thank the volunteers in the fall 2014 Wildlife Techniques course at the University of Georgia who assisted with this research and L. Lee for her photograph of bottomland hardwood habitat at the Savannah River Site. All other photographs were provided by D. Keiter. The Georgia Cooperative Fish and Wildlife Research Unit is sponsored jointly by the U.S. Geological Survey, the Georgia Department of Natural Resources, the U.S. Fish and Wildlife Service, the University of Georgia, and the Wildlife Management Institute. This paper was prepared as an account of work sponsored by an agency of the United States Government. Neither the U.S. Department of Agriculture, nor any of its employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the U.S. Government. The views and opinions of authors expressed herein do not necessarily state or reflect those of the U.S. Department of Agriculture. Although these data have been processed successfully on a computer system at the U.S. Geological Survey (USGS), no warranty expressed or implied is made regarding the display or utility of the data or associated code on any other system or for general or scientific purposes, nor shall the act of distribution constitute any such warranty. The USGS or the U.S. Government shall not be held liable for improper or incorrect use of the data or code described and/or contained herein. NR 43 TC 0 Z9 0 U1 6 U2 15 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 25 PY 2016 VL 11 IS 5 AR e0155615 DI 10.1371/journal.pone.0155615 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN2GI UT WOS:000376881700023 PM 27224453 ER PT J AU Jasieniak, JJ Treat, ND McNeill, CR de Villers, BJT Della Gaspera, E Chabinyc, ML AF Jasieniak, Jacek J. Treat, Neil D. McNeill, Christopher R. de Villers, Bertrand J. Tremolet Della Gaspera, Enrico Chabinyc, Michael L. TI Interfacial Characteristics of Efficient Bulk Heterojunction Solar Cells Fabricated on MoOx Anode Interlayers SO ADVANCED MATERIALS LA English DT Article ID POLYMER PHOTOVOLTAIC CELLS; VERTICAL PHASE-SEPARATION; SELF-ORGANIZATION; THIN-FILMS; SURFACE; BLENDS; POLY(3-HEXYLTHIOPHENE); MORPHOLOGY; STRATIFICATION; SEMICONDUCTORS AB The role of the interface between an MoOx anode interlayer and a polymer: fullerene bulk heterojunction is investigated. Processing differences in the MoOx induce large variations in the vertical stratification of the bulk heterojunction films. These variations are found to be inconsistent in predicting device performance, with a much better gauge being the quantity of polymer chemisorbed to the anode interlayer. C1 [Jasieniak, Jacek J.; McNeill, Christopher R.] Monash Univ, Dept Mat Sci & Engn, Clayton, Vic 3800, Australia. [Treat, Neil D.] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2ZA, England. [de Villers, Bertrand J. Tremolet] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Della Gaspera, Enrico] Commonwealth Sci & Res Org, Mfg Flagship, Clayton, Vic 3168, Australia. [Chabinyc, Michael L.] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. RP Jasieniak, JJ (reprint author), Monash Univ, Dept Mat Sci & Engn, Clayton, Vic 3800, Australia. EM Jacek.Jasieniak@monash.edu RI McNeill, Christopher/B-4530-2008; Della Gaspera, Enrico/H-3085-2013 OI McNeill, Christopher/0000-0001-5221-878X; Della Gaspera, Enrico/0000-0001-9948-5893 NR 53 TC 2 Z9 2 U1 14 U2 43 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAY 25 PY 2016 VL 28 IS 20 SI SI BP 3944 EP + DI 10.1002/adma.201503309 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM6RZ UT WOS:000376481400009 PM 26468898 ER PT J AU Kelly, LL Racke, DA Kim, H Ndione, P Sigdel, AK Berry, JJ Graham, S Nordlund, D Monti, OLA AF Kelly, Leah L. Racke, David A. Kim, Hyungchul Ndione, Paul Sigdel, Ajaya K. Berry, Joseph J. Graham, Samuel Nordlund, Dennis Monti, Oliver L. A. TI Hybridization-Induced Carrier Localization at the C-60/ZnO Interface SO ADVANCED MATERIALS LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; CHARGE-TRANSFER DYNAMICS; ULTRAFAST ELECTRON-TRANSFER; SOLID C-60; RESONANT PHOTOEMISSION; SOLAR-CELLS; SEMICONDUCTOR; HETEROJUNCTION; OXIDE; AUTOIONIZATION AB Electronic coupling and ground-state charge transfer at the C-60/ZnO hybrid interface is shown to localize carriers in the C-60 phase. This effect, revealed by resonant X-ray photoemission, arises from interfacial hybridization between C-60 and ZnO. Such localization at carrier-selective electrodes and interlayers may lead to severely reduced carrier harvesting efficiencies and increased recombination rates in organic electronic devices. C1 [Kelly, Leah L.; Racke, David A.; Monti, Oliver L. A.] Univ Arizona, Dept Chem & Biochem, 1306 E Univ Blvd, Tucson, AZ 85721 USA. [Kim, Hyungchul; Graham, Samuel] Georgia Inst Technol, Sch Mech Engn, Atlanta, GA 30332 USA. [Kim, Hyungchul; Graham, Samuel] Georgia Inst Technol, Ctr Organ Photon & Elect, Atlanta, GA 30332 USA. [Ndione, Paul; Sigdel, Ajaya K.; Berry, Joseph J.] Natl Ctr Photovolta, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Nordlund, Dennis] Stanford Synchrotron Lab, Stanford Linear Accelerator Campus, Menlo Pk, CA 94025 USA. [Monti, Oliver L. A.] Univ Arizona, Dept Phys, 118 E Fourth St, Tucson, AZ 85721 USA. RP Monti, OLA (reprint author), Univ Arizona, Dept Chem & Biochem, 1306 E Univ Blvd, Tucson, AZ 85721 USA.; Monti, OLA (reprint author), Univ Arizona, Dept Phys, 118 E Fourth St, Tucson, AZ 85721 USA. EM monti@u.arizona.edu NR 33 TC 2 Z9 2 U1 12 U2 32 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAY 25 PY 2016 VL 28 IS 20 SI SI BP 3960 EP + DI 10.1002/adma.201503694 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM6RZ UT WOS:000376481400011 PM 26596518 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahmad, S Ahn, SU Aiola, S Akindinov, A Alam, SN Albuquerque, DSD Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Balasubramanian, S Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Benacek, P Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biro, G Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Cabala, J Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chauvin, A Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danisch, MC Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Conti, C de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E Deplano, C Dhankher, P Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Endress, E Engel, H Epple, E Erazmus, B Erdemir, I Erhardt, F Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fronze, GG Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, AS Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hamon, JC Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Hellbar, E Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hillemanns, H Hippolyte, B Horak, D Hosokawa, R Hristov, P Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Inaba, M Incani, E Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacazio, N Jacobs, PM Jadhav, MB Jadlovska, S Jadlovsky, J Jahnke, C Jakubowska, MJ Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, DW Kim, DJ Kim, D Kim, H Kim, JS Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Klewin, S Kluge, A Knichel, ML Knospe, AG Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kostarakis, P Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kralik, I Kravcakova, A Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kuhn, C Kuijer, PG Kumar, A Kumar, J Kumar, L Kumar, S Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P de Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Vargas, HL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Lutz, TH Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV Margotti, A Margutti, J Marin, A Markert, C Marquard, M Martin, NA Blanco, JM Martinengo, P Martinez, MI Garcia, GM Pedreira, MM Mas, A Masciocchi, S Masera, M Masoni, A Mastroserio, A Matyja, A Mayer, C Mazer, J Mazzoni, MA Mcdonald, D Meddi, F Melikyan, Y Menchaca-Rocha, A Meninno, E Perez, JM Meres, M Miake, Y Mieskolainen, MM Mikhaylov, K Milano, L Milosevic, J Mischke, A Mishra, AN Miskowiec, D Mitra, J Mitu, CM Mohammadi, N Mohanty, B Molnar, L Zetina, LM Montes, E De Godoy, DAM Moreno, LAP Moretto, S Morreale, A Morsch, A Muccifora, V Mudnic, E Muhlheim, D Muhuri, S Mukherjee, M Mulligan, JD Munhoz, MG Munzer, RH Murakami, H Murray, S Musa, L Musinsky, J Naik, B Nair, R Nandi, BK Nania, R Nappi, E Naru, MU da Luz, HN Nattrass, C Navarro, SR Nayak, K Nayak, R Nayak, TK Nazarenko, S Nedosekin, A Nellen, L Ng, F Nicassio, M Niculescu, M Niedziela, J Nielsen, BS Nikolaev, S Nikulin, S Nikulin, V Noferini, F Nomokonov, P Nooren, G Noris, JCC Norman, J Nyanin, A Nystrand, J Oeschler, H Oh, S Oh, SK Ohlson, A Okatan, A Okubo, T Olah, L Oleniacz, J Da Silva, ACO Oliver, MH Onderwaater, J Oppedisano, C Orava, R Oravec, M Velasquez, AO Oskarsson, A Otwinowski, J Oyama, K Ozdemir, M Pachmayer, Y Pagano, D Pagano, P Paic, G Pal, SK Pan, J Pandey, AK Papikyan, V Pappalardo, GS Pareek, P Park, WJ Parmar, S Passfeld, A Paticchio, V Patra, RN Paul, B Pei, H Peitzmann, T Da Costa, HP Peresunko, D Lara, CEP Lezama, EP Peskov, V Pestov, Y Petracek, V Petrov, V Petrovici, M Petta, C Piano, S Pikna, M Pillot, P Pimentel, LODL Pinazza, O Pinsky, L Piyarathna, DB Ploskon, M Planinic, M Pluta, J Pochybova, S Podesta-Lerma, PLM Poghosyan, MG Polichtchouk, B Poljak, 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CA ALICE Collaboration TI Particle identification in ALICE: a Bayesian approach SO EUROPEAN PHYSICAL JOURNAL PLUS LA English DT Article ID PB COLLISIONS; TEV; PP; PERFORMANCE AB We present a Bayesian approach to particle identification (PID) within the ALICE experiment. The aim is to more effectively combine the particle identification capabilities of its various detectors. After a brief explanation of the adopted methodology and formalism, the performance of the Bayesian PID approach for charged pions, kaons and protons in the central barrel of ALICE is studied. PID is performed via measurements of specific energy loss (dE/dx) and time of flight. PID efficiencies and misidentification probabilities are extracted and compared with Monte Carlo simulations using high-purity samples of identified particles in the decay channels K-S(0) -> pi(-)pi(+), phi -> K-K+, and A -> p pi(-) in p-Pb collisions at root sNN = 5.02 TeV. In order to thoroughly assess the validity of the Bayesian approach, this methodology was used to obtain corrected p(T) spectra of pions, kaons, protons, and D-0 mesons in pp collisions at root s = 7TeV. In all cases, the results using Bayesian PID were found to be consistent with previous measurements performed by ALICE using a standard PID approach. For the measurement of D-0 -> K-pi(+), it was found that a Bayesian PID approach gave a higher signal-to-background ratio and a similar or larger statistical significance when compared with standard PID selections, despite a reduced identification efficiency. Finally, we present an exploratory study of the measurement of A(c)(+) -> pK(-)pi(+) in pp collisions at root s = 7TeV, using the Bayesian approach for the identification of its decay products. C1 [Rinella, G. Aglieri; Augustinus, A.; Barth, K.; Berzano, D.; Betev, L.; Bufalino, S.; Buncic, P.; Caffarri, D.; Carena, F.; Carena, W.; Chapeland, S.; Barroso, V. 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[Bartke, J.; Bhom, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Monzon, I. Leon; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Gimenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Mas, A.; Munhoz, M. G.; Natal da Luz, H.; Oliveira Da Silva, A. C.; Suaide, A. A. P.; Szanto de Toledo, A.; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Albuquerque, D. S. D.; Chinellato, D. D.; de Souza, R. D.; Takahashi, J.] Univ Estadual Campinas, UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Knospe, A. G.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Murakami, H.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Sadhu, S.; Saini, J.; Sarkar, D.; Sarkar, N.; Sheikh, A. I.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. Wayne State Univ, Detroit, MI 48202 USA. [Barnafoeldi, G. 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RP Adam, J (reprint author), Benemerita Univ Autonoma Puebla, Puebla, Mexico.; Adam, J (reprint author), Univ Padua, Dipartimento Fis & Astron, Padua, Italy. RI Vechernin, Vladimir/J-5832-2013; Pshenichnov, Igor/A-4063-2008; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Derradi de Souza, Rafael/M-4791-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Bregant, Marco/I-7663-2012; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Chinellato, David/D-3092-2012; Cosentino, Mauro/L-2418-2014 OI Vechernin, Vladimir/0000-0003-1458-8055; Pshenichnov, Igor/0000-0003-1752-4524; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Derradi de Souza, Rafael/0000-0002-2084-7001; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Giubilato, Piero/0000-0003-4358-5355; De Pasquale, Salvatore/0000-0001-9236-0748; Murray, Sean/0000-0003-0548-588X; Fernandez Tellez, Arturo/0000-0001-5092-9748; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Read, Kenneth/0000-0002-3358-7667; Riggi, Francesco/0000-0002-0030-8377; Melikyan, Yury/0000-0002-4165-505X; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Chinellato, David/0000-0002-9982-9577; Cosentino, Mauro/0000-0002-7880-8611 FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Escudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung and Technologic (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nationale di Fisica Nucleate (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direction General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (EOM); Nederlandse Organisatie voor Wet Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Education); Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN); Cubaenergia; Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut AMP; Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STEC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catalica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; r The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Escudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire", "Region Alsace", "Region Auvergne" and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung and Technologic (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nationale di Fisica Nucleate (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direction General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (EOM) and the Nederlandse Organisatie voor Wet Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Education), Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STEC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catalica del Peru. NR 26 TC 1 Z9 1 U1 9 U2 32 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 2190-5444 J9 EUR PHYS J PLUS JI Eur. Phys. J. Plus PD MAY 25 PY 2016 VL 131 IS 5 AR 168 DI 10.1140/epjp/i2016-16168-5 PG 24 WC Physics, Multidisciplinary SC Physics GA DM8CH UT WOS:000376587700004 ER PT J AU Beniwal, S Zhang, X Mu, S Naim, A Rosa, P Chastanet, G Letard, JF Liu, J Sterbinsky, GE Arena, DA Dowben, PA Enders, A AF Beniwal, S. Zhang, X. Mu, S. Naim, A. Rosa, P. Chastanet, G. Letard, J-F Liu, J. Sterbinsky, G. E. Arena, D. A. Dowben, P. A. Enders, A. TI Surface-induced spin state locking of the [Fe(H2B(pz)(2))(2)(bipy)] spin crossover complex SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE spin-crossover; Fe(II) spin-crossover; molecular magnetism; spin state locking ID PHOTOELECTRON-SPECTROSCOPY; MOLECULAR ADSORBATE; MULTIPLET STRUCTURE; MAGNETIC-PROPERTIES; SINGLE MOLECULES; FE(II) COMPLEXES; VACANCY LEVELS; XPS SPECTRA; OXIDE-FILMS; THIN-FILMS AB Temperature-and coverage-dependent studies of the Au(1 1 1)-supported spin crossover Fe(II) complex (SCO) of the type [Fe(H2B(pz)(2))(2)(bipy)] with a suite of surface-sensitive spectroscopy and microscopy tools show that the substrate inhibits thermally induced transitions of the molecular spin state, so that both high-spin and low-spin states are preserved far beyond the spin transition temperature of free molecules. Scanning tunneling microscopy confirms that [Fe(H2B(pz) 2) 2(bipy)] grows as ordered, molecular bilayer islands at sub-monolayer coverage and as disordered film at higher coverage. The temperature dependence of the electronic structure suggest that the SCO films exhibit a mixture of spin states at room temperature, but upon cooling below the spin crossover transition the film spin state is best described as a mix of high-spin and low-spin state molecules of a ratio that is constant. This locking of the spin state is most likely the result of a substrate-induced conformational change of the interfacial molecules, but it is estimated that also the intra-atomic electron-electron Coulomb correlation energy, or Hubbard correlation energy U, could be an additional contributing factor. C1 [Beniwal, S.; Zhang, X.; Mu, S.; Dowben, P. A.; Enders, A.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Naim, A.; Rosa, P.; Chastanet, G.; Letard, J-F] Univ Bordeaux, CNRS, ICMCB, UPR 9048, 87 Ave Dr A Schweitzer, F-33608 Pessac, France. [Liu, J.] Northeastern Univ, Dept Chem Engn, Boston, MA 02115 USA. [Liu, J.; Sterbinsky, G. E.; Arena, D. A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Enders, A (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM a.enders@me.com FU National Science Foundation through the Nebraska MRSEC [DMR-1420645]; Agence Nationale de la Recherche [11-BS08-06, 11-LABX-0058_NIE, ANR-10-IDEX-0002-02, 11-JS07-013-01]; International Center for Frontier Research in Chemistry (icFRC, Strasbourg); U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This research was primarily supported by the National Science Foundation through the Nebraska MRSEC (DMR-1420645). Partial financial support of the Agence Nationale de la Recherche (MULTISELF 11-BS08-06, Labex NIE 11-LABX-0058_NIE within the Investissement d'Avenir program ANR-10-IDEX-0002-02, CHIROTS 11-JS07-013-01) and the International Center for Frontier Research in Chemistry (icFRC, Strasbourg) are also gratefully acknowledged. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 46 TC 3 Z9 3 U1 7 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 25 PY 2016 VL 28 IS 20 AR 206002 DI 10.1088/0953-8984/28/20/206002 PG 8 WC Physics, Condensed Matter SC Physics GA DM5RZ UT WOS:000376409000008 PM 27121917 ER PT J AU Alkauskas, A Dreyer, CE Lyons, JL Van de Walle, CG AF Alkauskas, Audrius Dreyer, Cyrus E. Lyons, John L. Van de Walle, Chris G. TI Role of excited states in Shockley-Read-Hall recombination in wide-band-gap semiconductors SO PHYSICAL REVIEW B LA English DT Article ID MULTIPHONON CAPTURE COEFFICIENTS; IONIZATION RATES; NEUTRAL CENTERS; COUPLING SCHEME; DEEP-LEVEL AB Defect-assisted recombination is an important limitation on efficiency of optoelectronic devices. However, since nonradiative capture rates decrease exponentially with the energy of the transition, the mechanisms by which such recombination can take place in wide-band-gap materials are unclear. Using electronic structure calculations we uncover the crucial role of electronic excited states in nonradiative recombination processes. The impact is elucidated with examples for the group-III nitrides, for which accumulating experimental evidence indicates that defect-assisted recombination limits efficiency. Our work provides insights into the physics of nonradiative recombination, and the mechanisms are suggested to be ubiquitous in wide-band-gap semiconductors. C1 [Alkauskas, Audrius] Ctr Phys Sci & Technol, LT-01108 Vilnius, Lithuania. [Dreyer, Cyrus E.; Lyons, John L.; Van de Walle, Chris G.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Dreyer, Cyrus E.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08845 USA. [Lyons, John L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Alkauskas, A (reprint author), Ctr Phys Sci & Technol, LT-01108 Vilnius, Lithuania. EM audrius.alkauskas@ftmc.lt RI Alkauskas, Audrius/I-3245-2012 OI Alkauskas, Audrius/0000-0002-4228-6612 FU Marie Sklodowska-Curie Action of the European Union (project NITRIDE-SRH) [657054]; US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-SC0010689]; DOE Office of Science [DE-AC02-05CH11231] FX We acknowledge M. W. Doherty, M. A. Reshchikov, J. S. Speck, C. Weisbuch, and Q. Yan for fruitful interactions. A. A. was supported by Marie Sklodowska-Curie Action of the European Union (project NITRIDE-SRH, Grant No. 657054). Work at UCSB was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) under Award No. DE-SC0010689. Computational resources were provided by the National Energy Research Scientific Computing Center, which is supported by the DOE Office of Science under Contract No. DE-AC02-05CH11231. NR 40 TC 2 Z9 2 U1 12 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2016 VL 93 IS 20 AR 201304 DI 10.1103/PhysRevB.93.201304 PG 5 WC Physics, Condensed Matter SC Physics GA DM8TY UT WOS:000376638600002 ER PT J AU McDannald, A dela Cruz, CR Seehra, MS Jain, M AF McDannald, A. dela Cruz, C. R. Seehra, M. S. Jain, M. TI Negative exchange bias in single-phase Dy1-xNdxCrO3 induced by Nd doping SO PHYSICAL REVIEW B LA English DT Article AB Observation of significant negative exchange bias ( HE) is reported in solid solutions of single-phase samples of Dy1-xNdxCrO3 for x = 0.33, 0.67, and 1 with corresponding Neel temperatures at T-N(Cr) = 175K, 200K, and 225 K, respectively, and the spin-reorientation transitions T-SR at 48 K, 58 K, and 38 K, respectively. In contrast, no HE was observed for the sample with x = 0 (i.e., DyCrO3) shows no HE below its T-N(Cr) = 145 K, and no reorientation of spins at lower temperatures was observed. More importantly, the (negative) HE for the x = 0.33, 0.67, and 1 samples is observed only in the temperature range between T-N and TSR with the corresponding observation of magnetic coercivity. These results show that the canted antiferromagnetic Gamma(7),(Cr) structure of the Cr3+ moments present between T-N(Cr) and TSR is essential for the observed HE. By comparing this result to the literature, common features of single-phase materials with HE were identified. The present bulk powder samples were prepared by the citrate method and structurally characterized by x-ray diffraction and Raman spectroscopy techniques. Neutron diffraction measurements for the x = 0.33, 0.67, and 1 samples at select temperatures were done to verify the presence of the Gamma(7,Cr) structure between T-N(Cr) and TSR and the Gamma(1,Cr) structure (with no canting of Cr3+ moments) below TSR C1 [McDannald, A.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [dela Cruz, C. R.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Seehra, M. S.] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. [Jain, M.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Jain, M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP McDannald, A (reprint author), Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. RI dela Cruz, Clarina/C-2747-2013 OI dela Cruz, Clarina/0000-0003-4233-2145 FU National Science Foundation [DMR-1310149]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This paper is based in part upon work supported by the National Science Foundation under Grant DMR-1310149. Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 30 TC 2 Z9 2 U1 6 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 25 PY 2016 VL 93 IS 18 AR 184430 DI 10.1103/PhysRevB.93.184430 PG 8 WC Physics, Condensed Matter SC Physics GA DM8TC UT WOS:000376636400007 ER PT J AU Vogt, A Birkenbach, B Reiter, P Blazhev, A Siciliano, M Valiente-Dobon, JJ Wheldon, C Bazzacco, D Bowry, M Bracco, A Bruyneel, B Chakrawarthy, RS Chapman, R Cline, D Corradi, L Crespi, FCL Cromaz, M de Angelis, G Eberth, J Fallon, P Farnea, E Fioretto, E Freeman, SJ Gadea, A Geibel, K Gelletly, W Gengelbach, A Giaz, A Gorgen, A Gottardo, A Hayes, AB Hess, H Hua, H John, PR Jolie, J Jungclaus, A Korten, W Lee, IY Leoni, S Liang, X Lunardi, S Macchiavelli, AO Menegazzo, R Mengoni, D Michelagnoli, C Mijatovic, T Montagnoli, G Montanari, D Napoli, D Pearson, CJ Pellegri, L Podolyak, Z Pollarolo, G Pullia, A Radeck, F Recchia, F Regan, PH Sahin, E Scarlassara, F Sletten, G Smith, JF Soderstrom, PA Stefanini, AM Steinbach, T Stezowski, O Szilner, S Szpak, B Teng, R Ur, C Vandone, V Ward, D Warner, DD Wiens, A Wu, CY AF Vogt, A. Birkenbach, B. Reiter, P. Blazhev, A. Siciliano, M. Valiente-Dobon, J. J. Wheldon, C. Bazzacco, D. Bowry, M. Bracco, A. Bruyneel, B. Chakrawarthy, R. S. Chapman, R. Cline, D. Corradi, L. Crespi, F. C. L. Cromaz, M. de Angelis, G. Eberth, J. Fallon, P. Farnea, E. Fioretto, E. Freeman, S. J. Gadea, A. Geibel, K. Gelletly, W. Gengelbach, A. Giaz, A. Gorgen, A. Gottardo, A. Hayes, A. B. Hess, H. Hua, H. John, P. R. Jolie, J. Jungclaus, A. Korten, W. Lee, I. Y. Leoni, S. Liang, X. Lunardi, S. Macchiavelli, A. O. Menegazzo, R. Mengoni, D. Michelagnoli, C. Mijatovic, T. Montagnoli, G. Montanari, D. Napoli, D. Pearson, C. J. Pellegri, L. Podolyak, Zs. Pollarolo, G. Pullia, A. Radeck, F. Recchia, F. Regan, P. H. Sahin, E. Scarlassara, F. Sletten, G. Smith, J. F. Soderstrom, P. -A. Stefanini, A. M. Steinbach, T. Stezowski, O. Szilner, S. Szpak, B. Teng, R. Ur, C. Vandone, V. Ward, D. Warner, D. D. Wiens, A. Wu, C. Y. TI High-spin structure of Xe-134 SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; HEAVY-ION DETECTOR; MAGNETIC-MOMENTS; N=80 ISOTONES; STATE; GAMMASPHERE; ISOMERS AB Detailed spectroscopic information on the N similar to 82 nuclei is necessary to benchmark shell-model calculations in the region. The nuclear structure above long-lived isomers in Xe-134 is investigated after multinucleon transfer (MNT) and actinide fission. Xenon-134 was populated as (i) a transfer product in Xe-136 + U-238 and Xe-136 + Pb-208 MNT reactions and (ii) as a fission product in the Xe-136 + U-238 reaction employing the high-resolution Advanced Gamma Tracking Array (AGATA). Trajectory reconstruction has been applied for the complete identification of beamlike transfer products with the magnetic spectrometer PRISMA. The Xe-136 + Pt-198 MNT reaction was studied with the gamma-ray spectrometer GAMMASPHERE in combination with the gas detector array Compact Heavy Ion Counter (CHICO). Several high-spin states in Xe-134 on top of the two long-lived isomers are discovered based on gamma gamma-coincidence relationships and information on the gamma-ray angular distributions as well as excitation energies from the total kinetic energy loss and fission fragments. The revised level scheme of Xe-134 is extended up to an C1 [Vogt, A.; Birkenbach, B.; Reiter, P.; Blazhev, A.; Eberth, J.; Geibel, K.; Hess, H.; Jolie, J.; Radeck, F.; Steinbach, T.; Wiens, A.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Siciliano, M.; John, P. R.; Lunardi, S.; Mengoni, D.; Michelagnoli, C.; Montagnoli, G.; Montanari, D.; Recchia, F.; Scarlassara, F.] Univ Padua, Dipartimento Fis & Astron, I-35131 Padua, Italy. [Siciliano, M.; Valiente-Dobon, J. J.; Corradi, L.; de Angelis, G.; Fioretto, E.; Gottardo, A.; Napoli, D.; Sahin, E.; Stefanini, A. M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Wheldon, C.] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Bowry, M.; Gelletly, W.; Pearson, C. J.; Podolyak, Zs.; Regan, P. H.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Bracco, A.; Crespi, F. C. L.; Giaz, A.; Leoni, S.; Pellegri, L.; Pullia, A.; Vandone, V.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Bracco, A.; Crespi, F. C. L.; Giaz, A.; Leoni, S.; Pellegri, L.; Pullia, A.; Vandone, V.] INFN, Sez Milano, I-20133 Milan, Italy. [Bruyneel, B.] CEA Saclay, Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Chakrawarthy, R. S.; Freeman, S. J.] Univ Manchester, Dept Phys & Astron, Schuster Lab, Manchester M13 9PL, Lancs, England. [Chapman, R.] Univ West Scotland, Sch Engn & Comp, SUPA, Paisley PA1 2BE, Renfrew, Scotland. [Cline, D.; Hayes, A. B.; Hua, H.; Teng, R.; Wu, C. Y.] Univ Rochester, Dept Phys, 601 Elmwood Ave, Rochester, NY 14627 USA. [Cromaz, M.; Fallon, P.; Gorgen, A.; Lee, I. Y.; Macchiavelli, A. O.; Ward, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gadea, A.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain. [Gengelbach, A.; Soderstrom, P. -A.] Uppsala Univ, Dept Phys & Astron, SE-75121 Uppsala, Sweden. [Gorgen, A.; Sahin, E.] Univ Oslo, Dept Phys, POB 1048 Blindern, N-0316 Oslo, Norway. [Gorgen, A.; Korten, W.] Ctr CEA Saclay, DSM, CEA, IRFU, F-91191 Gif Sur Yvette, France. [Jungclaus, A.] CSIC, Inst Estruct Mat, Serrano 119, E-28006 Madrid, Spain. [Liang, X.; Mengoni, D.; Smith, J. F.] Univ West Scotland, Nucl Phys Res Grp, High St, Paisley PA1 2BE, Renfrew, Scotland. [Mijatovic, T.; Szilner, S.] Rudjer Boskovic Inst, HR-10002 Zagreb, Croatia. [Pollarolo, G.] Univ Turin, Dipartimento Fis Teor, Via P Giuria 1, I-10125 Turin, Italy. [Pollarolo, G.] Ist Nazl Fis Nucl, I-10125 Turin, Italy. [Regan, P. H.] Natl Phys Lab, Radioact Grp, Teddington TW11 0LW, Middx, England. [Sletten, G.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Stezowski, O.] Univ Lyon 1, CNRS, IN2P3, UMR5822,IPNL, F-69622 Villeurbanne, France. [Szpak, B.] Henryk Niewodniczanski Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Warner, D. D.] CCLRC Daresbury Lab, Warrington WA4 4AD, Cheshire, England. [Michelagnoli, C.] CNRS, IN2P3, CEA, DSM,GANIL, F-14076 Caen, France. [Montanari, D.] Univ Strasbourg, CNRS, IPHC, USIAS, F-67037 Strasbourg 2, France. [Pearson, C. J.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Soderstrom, P. -A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Wu, CY (reprint author), Univ Rochester, Dept Phys, 601 Elmwood Ave, Rochester, NY 14627 USA. EM andreas.vogt@ikp.uni-koeln.de RI Freeman, Sean/B-1280-2010; Gadea, Andres/L-8529-2014; Napoli, Daniel R./D-9863-2012; Menegazzo, Roberto/J-5853-2012 OI Freeman, Sean/0000-0001-9773-4921; Gadea, Andres/0000-0002-4233-1970; Napoli, Daniel R./0000-0002-8154-6958; Menegazzo, Roberto/0000-0002-3060-5276 FU German BMBF [05P12PKFNE TP4]; European Union [262010 ENSAR]; Spanish Ministerio de Ciencia e Innovacion [FPA2011-29854-C04]; Spanish Ministerio de Economia y Competitividad [FPA2014-57196-C5]; Bonn-Cologne Graduate School of Physics and Astronomy (BCGS); UK Science and Technology Facilities Council (STFC); US National Science Foundation (NSF); Generalitat Valenciana, Spain [PROMETEOII/2014/019]; EU under the FEDER program FX The research leading to these results has received funding from the German BMBF under Contract No. 05P12PKFNE TP4, from the European Union Seventh Framework Programme FP7/2007-2013 under Grant Agreement No. 262010 ENSAR, from the Spanish Ministerio de Ciencia e Innovacion under Contract No. FPA2011-29854-C04, from the Spanish Ministerio de Economia y Competitividad under Contract No. FPA2014-57196-C5, from the Bonn-Cologne Graduate School of Physics and Astronomy (BCGS), from the UK Science and Technology Facilities Council (STFC), and from the US National Science Foundation (NSF). One of the authors (A. Gadea) has been supported by the Generalitat Valenciana, Spain, under Grant No. PROMETEOII/2014/019 and EU under the FEDER program. NR 51 TC 1 Z9 1 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 25 PY 2016 VL 93 IS 5 AR 054325 DI 10.1103/PhysRevC.93.054325 PG 12 WC Physics, Nuclear SC Physics GA DM8UM UT WOS:000376640000002 ER PT J AU Bazavov, A Bernard, C Brown, N Komijani, J Detar, C Foley, J Levkova, L Gottlieb, S Heller, UM Laiho, J Sugar, RL Toussaint, D Van de Water, RS AF Bazavov, A. Bernard, C. Brown, N. Komijani, J. Detar, C. Foley, J. Levkova, L. Gottlieb, Steven Heller, U. M. Laiho, J. Sugar, R. L. Toussaint, D. Van de Water, R. S. TI Gradient flow and scale setting on MILC HISQ ensembles SO PHYSICAL REVIEW D LA English DT Article ID LATTICE QCD; ALPHA(S); QUARKS AB We report on a scale determination with gradient-flow techniques on the N-f = 2 + 1 + 1 highly improved staggered quark ensembles generated by the MILC Collaboration. The ensembles include four lattice spacings, ranging from approximately 0.15 to 0.06 fm, and both physical and unphysical values of the quark masses. The scales root t(0)/a and their tree-level improvements, root t(0,imp) and root w(0,imp), are computed on each ensemble using Symanzik flow and the cloverleaf definition of the energy density E. Using a combination of continuum chiral-perturbation theory and a Taylor-series ansatz for the latticespacing and strong-coupling dependence, the results are simultaneously extrapolated to the continuum and interpolated to physical quark masses. We determine the scales root t(0) = 0.171416((18)(-5)) fm, and w(0) =.174 ((-15)(-12)), where the errors are sums, in quadrature, of statistical and all systematic errors. The precision of w(0) and root t(0) is comparable to or more precise than the best previous estimates, respectively. We then find the continuum mass dependence of root t(0) and w(0), which will be useful for estimating the scales of new ensembles. We also estimate the integrated autocorrelation length of < E(t)>. For long flow times, the autocorrelation length of < E > appears to be comparable to that of the topological charge. C1 [Bazavov, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Bernard, C.; Brown, N.; Komijani, J.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Detar, C.; Foley, J.; Levkova, L.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Gottlieb, Steven] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Heller, U. M.] Amer Phys Soc, One Res Rd, Ridge, NY 11961 USA. [Laiho, J.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Sugar, R. L.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Toussaint, D.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Van de Water, R. S.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Bazavov, A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. RP Brown, N (reprint author), Washington Univ, Dept Phys, St Louis, MO 63130 USA. EM brownnathan@wustl.edu FU Office of Science of the U.S. Department of Energy; National Science Foundation's Teragrid/XSEDE Program; NSF [OCI-0725070, ACI-1238993]; State of Illinois; National Science Foundation [OCI-0832315, PHY-1067881, PHY-10034278, PHYS-1417805, PHY-1316748]; U.S. Department of Energy [DE-FG02-91ER40628, DE-FC02-12ER41879, DE-FG02-91ER40661, DE-SC0010120, DE-FG02-13ER-41976, DE-AC02-98CH10886, DE-AC02-07CH11359] FX Computations for this work were carried out with resources provided by the USQCD Collaboration, the Argonne Leadership Computing Facility, and the National Energy Research Scientific Computing Center, which are funded by the Office of Science of the U.S. Department of Energy; and with resources provided by the National Center for Atmospheric Research, the National Center for Supercomputing Applications, the National Institute for Computational Science, and the Texas Advanced Computing Center, which are funded through the National Science Foundation's Teragrid/XSEDE Program; and with resources provided by the Blue Waters Computing Project, which is funded by NSF Grants No. OCI-0725070 and No. ACI-1238993 and the State of Illinois. This work is also part of the "Lattice QCD on Blue Waters" PRAC allocation supported by National Science Foundation Grant No. OCI-0832315. This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG02-91ER40628 (C. B., N. B., J. K.), No. DE-FC02-12ER41879 (C. D., J. F., L. L.), No. DE-FG02-91ER40661 (S. G.), No. DE-SC0010120 (S. G.), No. DE-FG02-13ER-41976 (D. T.), by the National Science Foundation under Grants No. PHY-1067881 (C. D., J. F., L. L.), No. PHY-10034278 (C. D.), No. PHYS-1417805 (J. L.), and No. PHY-1316748 (R. S.). This manuscript has been coauthored by an employee of Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 33 TC 3 Z9 3 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 25 PY 2016 VL 93 IS 9 AR 094510 DI 10.1103/PhysRevD.93.094510 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8UY UT WOS:000376641200003 ER PT J AU Martinez, AJ Yasuda, H Kim, E Kevrekidis, PG Porter, MA Yang, J AF Martinez, Alejandro J. Yasuda, Hiromi Kim, Eunho Kevrekidis, P. G. Porter, Mason A. Yang, Jinkyu TI Scattering of waves by impurities in precompressed granular chains SO PHYSICAL REVIEW E LA English DT Article ID SOLITARY WAVES; PULSE-PROPAGATION; FANO RESONANCES; METAMATERIALS; CRYSTALS; MEDIA AB We study scattering of waves by impurities in strongly precompressed granular chains. We explore the linear scattering of plane waves and identify a closed-form expression for the reflection and transmission coefficients for the scattering of the waves from both a single impurity and a double impurity. For single-impurity chains, we show that, within the transmission band of the host granular chain, high-frequency waves are strongly attenuated (such that the transmission coefficient vanishes as the wavenumber k -> +/-pi), whereas low-frequency waves are well-transmitted through the impurity. For double-impurity chains, we identify a resonance-enabling full transmission at a particular frequency-in a manner that is analogous to the Ramsauer-Townsend (RT) resonance from quantum physics. We also demonstrate that one can tune the frequency of the RT resonance to any value in the pass band of the host chain. We corroborate our theoretical predictions both numerically and experimentally, and we directly observe almost complete transmission for frequencies close to the RT resonance frequency. Finally, we show how this RT resonance can lead to the existence of reflectionless modes in granular chains ( including disordered ones) with multiple double impurities. C1 [Martinez, Alejandro J.; Porter, Mason A.] Univ Oxford, Math Inst, Oxford Ctr Ind & Appl Math, Oxford OX2 6GG, England. [Yasuda, Hiromi; Kim, Eunho; Yang, Jinkyu] Univ Washington, Aeronaut & Astronaut, Seattle, WA 98195 USA. [Kim, Eunho] Chonbuk Natl Univ, Div Mech Syst Engn, Automot Hitechnol Res Ctr, 567 Baeje Daero, Jeonju Si 54896, Jeollabuk Do, South Korea. [Kevrekidis, P. G.] Los Alamos Natl Lab, Ctr Nonlinear Studies, POB 1663, Los Alamos, NM 87544 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. [Kevrekidis, P. G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Porter, Mason A.] Univ Oxford, CABDyN Complex Ctr, Oxford OX1 1HP, England. RP Porter, MA (reprint author), Univ Oxford, Math Inst, Oxford Ctr Ind & Appl Math, Oxford OX2 6GG, England.; Yang, J (reprint author), Univ Washington, Aeronaut & Astronaut, Seattle, WA 98195 USA.; Porter, MA (reprint author), Univ Oxford, CABDyN Complex Ctr, Oxford OX1 1HP, England. EM porterm@maths.ox.ac.uk; jkyang@uw.washington.edu FU CONICYT [BCH72130485/2013]; ONR [N000141410388]; NSF [CMMI-1414748, CMMI-1553202]; ADD of Korea [UD140059JD]; US-AFOSR [FA9550-12-1-0332]; ERC under FP7, Marie Curie Actions, People, International Research Staff Exchange Scheme [IRSES-605096]; US-ARO [W911NF-15-1-0604] FX A.J.M. acknowledges partial support from CONICYT (Grant No. BCH72130485/2013). J.Y. and H.Y. acknowledge the support of ONR(Grant No. N000141410388), NSF (Grants No. CMMI-1414748 and No. CMMI-1553202), and ADD of Korea (Grant No. UD140059JD). P.G.K gratefully acknowledges support from US-AFOSR under Grant No. FA9550-12-1-0332 and the ERC under FP7, Marie Curie Actions, People, International Research Staff Exchange Scheme (Grant No. IRSES-605096). J.Y. and P.G.K. also acknowledge support from US-ARO under Grant No. W911NF-15-1-0604. NR 58 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 25 PY 2016 VL 93 IS 5 AR 052224 DI 10.1103/PhysRevE.93.052224 PG 12 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DM8WT UT WOS:000376645900002 PM 27300897 ER PT J AU Zhu, M Peng, J Zou, T Prokes, K Mahanti, SD Hong, T Mao, ZQ Liu, GQ Ke, X AF Zhu, M. Peng, J. Zou, T. Prokes, K. Mahanti, S. D. Hong, T. Mao, Z. Q. Liu, G. Q. Ke, X. TI Colossal Magnetoresistance in a Mott Insulator via Magnetic Field-Driven Insulator-Metal Transition SO PHYSICAL REVIEW LETTERS LA English DT Article ID PHASE-SEPARATION; SUPERCONDUCTIVITY; CA3RU2O7; CRYSTAL; SYSTEMS; PHYSICS AB We present a new type of colossal magnetoresistance (CMR) arising from an anomalous collapse of the Mott insulating state via a modest magnetic field in a bilayer ruthenate, Ti-doped Ca3Ru2O7. Such an insulator-metal transition is accompanied by changes in both lattice and magnetic structures. Our findings have important implications because a magnetic field usually stabilizes the insulating ground state in a Mott-Hubbard system, thus calling for a deeper theoretical study to reexamine the magnetic field tuning of Mott systems with magnetic and electronic instabilities and spin-lattice-charge coupling. This study further provides a model approach to search for CMR systems other than manganites, such as Mott insulators in the vicinity of the boundary between competing phases. C1 [Zhu, M.; Zou, T.; Mahanti, S. D.; Ke, X.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Peng, J.; Mao, Z. Q.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. [Prokes, K.] Helmholtz Zentrum Berlin, D-14109 Berlin, Germany. [Hong, T.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Liu, G. Q.] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China. RP Ke, X (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM ke@pa.msu.edu RI Zou, Tao/A-1761-2013 OI Zou, Tao/0000-0002-6510-5749 FU Michigan State University; NSF [DMR-1205469]; Scientific User Facilities Division, Office of Basic Energy Sciences, DOE; National Natural Science Foundation of China [11204326, 11474296] FX X. K. is grateful for Dr. Matas in HZB for help during the neutron experiment. X. K. acknowledges the start-up funds from Michigan State University. Work at Tulane University was supported by the NSF under Grant No. DMR-1205469 and work at ORNL was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. G. L. was supported by the National Natural Science Foundation of China (Grants No. 11204326 and No. 11474296). NR 42 TC 2 Z9 2 U1 18 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 25 PY 2016 VL 116 IS 21 AR 216401 DI 10.1103/PhysRevLett.116.216401 PG 5 WC Physics, Multidisciplinary SC Physics GA DM8PS UT WOS:000376627000004 PM 27284665 ER PT J AU Pathak, AK Gschneidner, KA Khan, M McCallum, RW Pecharsky, VK AF Pathak, Arjun K. Gschneidner, K. A., Jr. Khan, M. McCallum, R. W. Pecharsky, V. K. TI High performance Nd-Fe-B permanent magnets without critical elements SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Permanent magnet; Coercivity; Maximum energy product; Nd2Fe14B; Cerium ID COBALT SITE PREFERENCES; CE-SUBSTITUTION; MICROSTRUCTURE; ND2FE14B; RIBBONS; CERIUM AB Scanning electron microscopy, and magnetization measurements reveal that as cast (Nd1-xCex)(2)Fe14B alloys contain significant amounts of alpha-Fe that can be dramatically reduced by annealing the alloys at 1000 degrees C for 3 days. The room temperature intrinsic coercivity, Hci, of (Nd0.8Ce0.2)(2.2)Fe14B melt spun ribbons was found to be 11 kOe, which is similar to 32-similar to 10% higher in comparison to that of Nd2Fe14B (Hci = 8.3 kOe), and (Nd0.8Ce0.2)(2.0)Fe14B (Hci = 10 kOe), respectively. The substitution of Co for Fe in (Nd0.8Ce0.2)(2)Fe14-zCozB significantly increases both T-C and the maximum energy product, (BH)max. Our study shows that both Co-containing and Co-free Ce-substituted Nd2Fe14B alloys have excellent magnetic properties at room temperature and above. The experimental results also demonstrate the potential of Nd-Ce-Fe-TM-B based alloys as alternative to expensive Dy-containing high performance rare earth magnets. (C) 2016 Elsevier B.V. All rights reserved. C1 [Pathak, Arjun K.; Gschneidner, K. A., Jr.; Khan, M.; McCallum, R. W.; Pecharsky, V. K.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Gschneidner, K. A., Jr.; Pecharsky, V. K.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Khan, M.] Miami Univ, Dept Phys, Oxford, OH 45056 USA. [McCallum, R. W.] McCallum Consulting LLC, 1948 Cerros Colorados, Santa Fe, NM 87501 USA. RP Pathak, AK (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM pathak138@ameslab.gov FU U.S. Department of Energy (DOE), Advanced Research Projects Agency-Energy (ARPA-E), Rare Earth Alternatives in Critical Technologies for Energy (REACT); U.S. DOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Advanced Research Projects Agency-Energy (ARPA-E), Rare Earth Alternatives in Critical Technologies for Energy (REACT). The research was performed at the Ames Laboratory which is operated for the U.S. DOE by Iowa State University under contract #DE-AC02-07CH11358. The authors would like to thank Matthew Abben, Matthew Kenney, and Matthew Wheaton for their help preparing melt spun ribbon samples. NR 28 TC 3 Z9 3 U1 15 U2 69 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD MAY 25 PY 2016 VL 668 BP 80 EP 86 DI 10.1016/j.jallcom.2016.01.194 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA DG0OE UT WOS:000371763700012 ER PT J AU Zhang, RB Abtew, TA Quackenbush, NF Wanioh, LW Huie, M Brady, AB Bock, D Efstathiadis, H Whittingham, MS Marschilok, AC Takeuch, KJ Takeuchi, ES Zhang, PH Piper, LFJ AF Zhang, Ruibo Abtew, Tesfaye A. Quackenbush, Nicholas F. Wanioh, Linda W. Huie, Matthew Brady, Alexander B. Bock, David Efstathiadis, Harry Whittingham, M. Stanley Marschilok, Amy C. Takeuch, Kenneth J. Takeuchi, Esther S. Zhang, Peihong Piper, Louis F. J. TI Electrode Reaction Mechanism of Ag2VO2PO4 Cathode SO CHEMISTRY OF MATERIALS LA English DT Article ID VANADIUM PHOSPHORUS OXIDE; X-RAY-DIFFRACTION; ELECTROCHEMICAL REDUCTION; SPECTROSCOPY; CONDUCTIVITY; DISSOLUTION; BATTERIES; PHOSPHATE; DISCHARGE; KINETICS AB The high capacity of primary lithium-ion cathode Ag2VO2PO4 is facilitated by both displacement and insertion reaction mechanisms. Whether the Ag extrusion (specifically, Ag reduction with Ag metal displaced from the host crystal) and V reduction are sequential or concurrent remains unclear. A microscopic description of the reaction mechanism is required for developing design rules for new multimechanism cathodes, combining both displacement and insertion reactions. However, the amorphization of Ag2VO2PO4 during lithiation makes the investigation of the electrode reaction mechanism difficult with conventional characterization tools. For addressing this issue, a combination of local probes of pair-distribution function and X-ray spectroscopy were used to obtain a description of the discharge reaction. We determine that the initial reaction is dominated by silver extrusion with vanadium playing a supporting role. Once sufficient Ag has been displaced, the residual Ag+ in the host can no longer stabilize the host structure and V-O environment (i.e., onset of amorphization). After amorphization, silver extrusion continues but the vanadium reduction dominates the reaction. As a result, the crossover from primarily silver reduction displacement to vanadium reduction is facilitated by the amorphization that makes vanadium reduction increasingly more favorable. C1 [Zhang, Ruibo; Whittingham, M. Stanley] SUNY Binghamton, Inst Mat Res, Binghamton, NY 13902 USA. [Whittingham, M. Stanley] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. [Zhang, Ruibo; Quackenbush, Nicholas F.; Wanioh, Linda W.; Piper, Louis F. J.] SUNY Binghamton, Dept Chem, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Abtew, Tesfaye A.] SUNY Buffalo, Dept Phys, Buffalo, NY 14260 USA. [Huie, Matthew; Brady, Alexander B.; Marschilok, Amy C.; Takeuch, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Marschilok, Amy C.; Takeuch, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bock, David; Takeuch, Kenneth J.] Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. [Efstathiadis, Harry] SUNY Albany, Polytech Inst, Coll Nanoscale Sci, Albany, NY 12203 USA. [Efstathiadis, Harry] SUNY Albany, Polytech Inst, Coll Engn, Albany, NY 12203 USA. RP Piper, LFJ (reprint author), SUNY Binghamton, Dept Chem, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. EM lpiper@binghamton.edu RI Zhang, Peihong/D-2787-2012; OI Hayward, Michael/0000-0002-6248-2063; Piper, Louis/0000-0002-3421-3210 FU SUNY Research Foundation as part of the Network of Excellence in Materials and Advanced Manufacturing; DOE Office of Science [DE-AC02-06CH11357, DE-SC0012704]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Drs. Peter Chupas, Karena Chapman, Olaf Borkiewicz, and Kamila Wiaderek for their help at APS beamline 11-ID-B. We thank Drs. Eric Dooryhee, Sanjit Ghose, and Jianming Bai for their help at NSLS II beamline 28-ID. We also thank Drs. Jinghua Guo and Anders Glans for their help at ALS beamline 6.3.1.2 ISAAC. This research was funded by the SUNY Research Foundation as part of the Network of Excellence in Materials and Advanced Manufacturing. We acknowledge the computational support provided by the Center for Computational Research at the University at Buffalo, SUNY. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. This research used resources [beamline 28 ID] of the National Synchrotron Light Source II, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Brookhaven National Laboratory under Contract No. DE-SC0012704. The use of Advanced Light Source, Lawrence Berkeley National Laboratory, is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 31 TC 1 Z9 1 U1 8 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2016 VL 28 IS 10 BP 3428 EP 3434 DI 10.1021/acs.chemmater.6b00828 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DN1KW UT WOS:000376825700025 ER PT J AU Roy, UN Mundle, RM Camarda, GS Cui, Y Gul, R Hossain, A Yang, G Pradhan, AK James, RB AF Roy, U. N. Mundle, R. M. Camarda, G. S. Cui, Y. Gul, R. Hossain, A. Yang, G. Pradhan, A. K. James, R. B. TI Novel ZnO:Al contacts to CdZnTe for X- and gamma-ray detectors SO SCIENTIFIC REPORTS LA English DT Article ID RADIATION DETECTOR; CDTE; CRYSTALS AB CdZnTe (CZT) has made a significant impact as a material for room-temperature nuclear-radiation detectors due to its potential impact in applications related to nonproliferation, homeland security, medical imaging, and gamma-ray telescopes. In all such applications, common metals, such as gold, platinum and indium, have been used as electrodes for fabricating the detectors. Because of the large mismatch in the thermal-expansion coefficient between the metal contacts and CZT, the contacts can undergo stress and mechanical degradation, which is the main cause for device instability over the long term. Here, we report for the first time on our use of Al-doped ZnO as the preferred electrode for such detectors. The material was selected because of its better contact properties compared to those of the metals commonly used today. Comparisons were conducted for the detector properties using different contacts, and improvements in the performances of ZnO: Al-coated detectors are described in this paper. These studies show that Al:ZnO contacts to CZT radiation detectors offer the potential of becoming a transformative replacement for the common metallic contacts due to the dramatic improvements in the performance of detectors and improved long-term stability. C1 [Roy, U. N.; Camarda, G. S.; Cui, Y.; Gul, R.; Hossain, A.; Yang, G.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Mundle, R. M.; Pradhan, A. K.] Norfolk State Univ, Dept Engn, Norfolk, VA 23504 USA. RP Roy, UN (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM uroy@bnl.gov FU U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and Development, DNN RD; Department of Defense (DoD) [W911NF-11-1-0209]; NSF-CREST Grant [HRD 1036494] FX This work was supported primarily by the U.S. Department of Energy, Office of Defense Nuclear Nonproliferation Research and Development, DNN R&D. AKP and RM were partially supported by the Department of Defense (DoD), Grant Numbers W911NF-11-1-0209 and NSF-CREST Grant Number HRD 1036494. NR 21 TC 0 Z9 0 U1 3 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 24 PY 2016 VL 6 AR 26384 DI 10.1038/srep26384 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EH8ZD UT WOS:000392060400001 PM 27216387 ER PT J AU Sava Gallis, DF Chapman, KW Rodriguez, MA Greathouse, JA Parkes, MV Nenoff', TM AF Sava Gallis, Dorina F. Chapman, Karena W. Rodriguez, Mark A. Greathouse, Jeffery A. Parkes, Marie V. Nenoff', Tina M. TI Selective O-2 Sorption at Ambient Temperatures via Node Distortions in Sc-MIL-100 SO CHEMISTRY OF MATERIALS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; ADSORPTION; SIMULATIONS; SITES; EQUILIBRIA; SEPARATION; DETECTOR; GASES; PORES; OXIDE AB An open pored metal organic framework (MOF) with oxygen selectivity at exceptionally high temperatures is confirmed by synthesis, sorption, and synchrotron structural analyses. The large-pore MIL-100 framework with access to the metal center (e.g., Sc and Fe) resulted in preferential O-2 over N-2 gas uptake at temperatures ranging from 77 K to ambient temperatures (258, 298, and 313 K). Most notably, Sc-MIL-100 shows exceptional O-2 sorption; pair distribution function analyses indicate that this is due to distortions in the framework owing to the size of Sc atoms, in particular in the trimer metal cluster. Experimental studies also correlate very well with GCMC simulations, confirming more favorable O-2-framework interactions at pressures up to 1 bar, due to the close proximity of O-2 to the high density of metal centers in the small tetrahedral cages. Both materials maintain their crystallinity upon gas adsorption cycling, are regenerable, and show exceptional promise for use in energy efficient oxygen purification processes, such as Pressure Swing Adsorption. C1 [Sava Gallis, Dorina F.] Sandia Natl Labs, Nanoscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. [Rodriguez, Mark A.] Sandia Natl Labs, Mat Characterizat & Performance Dept, POB 5800, Albuquerque, NM 87185 USA. [Nenoff', Tina M.] Sandia Natl Labs, Phys Chem & Nano Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. [Greathouse, Jeffery A.; Parkes, Marie V.] Sandia Natl Labs, Dept Geochem, POB 5800, Albuquerque, NM 87185 USA. [Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Nenoff', TM (reprint author), Sandia Natl Labs, Phys Chem & Nano Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM tmnenof@sandia.gov RI Sava Gallis, Dorina/D-2827-2015 FU Laboratory Directed Research and Development Program at Sandia National Laboratories; US DOE's NNSA [DE-AC04-94AL85000]; US DOE [DE-AC02-06CH11357] FX The authors would like to thank Dr. David Fairen-Jimenez for helpful discussions and for providing the atomic charges for MIL-100(Cr) and to Kenneth Croes for help with synthesis and TGA-MS experiments. This work is supported by the Laboratory Directed Research and Development Program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram lab managed and operated by Sandia Corp., a wholly owned subsidiary of Lockheed Martin Corporation, for the US DOE's NNSA under contract DE-AC04-94AL85000). Work done at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE/Office of Science by Argonne National Laboratory, was supported by the US DOE, Contract No. DE-AC02-06CH11357. NR 42 TC 0 Z9 0 U1 21 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2016 VL 28 IS 10 BP 3327 EP 3336 DI 10.1021/acs.chemmater.6b00249 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DN1KW UT WOS:000376825700013 ER PT J AU Cheng, YW Shao, YY Raju, V Ji, XL Mehdi, BL Han, KS Engelhard, MH Li, GS Browning, ND Mueller, KT Liu, J AF Cheng, Yingwen Shao, Yuyan Raju, Vadivukarasi Ji, Xiulei Mehdi, B. Layla Han, Kee Sung Engelhard, Mark H. Li, Guosheng Browning, Nigel D. Mueller, Karl T. Liu, Jun TI Molecular Storage of Mg Ions with Vanadium Oxide Nanoclusters SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID RECHARGEABLE MAGNESIUM BATTERIES; ELECTROCHEMICAL ENERGY-STORAGE; CATHODE MATERIALS; INTERCALATION PROPERTIES; ELECTROLYTE-SOLUTIONS; INSERTION; V2O5; CARBON; NANOCOMPOSITES; DEPOSITION AB Mg batteries have potential advantages in terms of safety, cost, and reliability over existing battery technologies, but their practical implementations are hindered by the lack of amenable high-voltage cathode materials. The development of cathode materials is complicated by limited understandings of the unique divalent Mg2+ ion electrochemistry and the interaction/transportation of Mg2+ ions with host materials. Here, it is shown that highly dispersed vanadium oxide (V2O5) nanoclusters supported on porous carbon frameworks are able to react with Mg2+ ions reversibly in electrolytes that are compatible with Mg metal, and exhibit high capacities and good reaction kinetics. They are able to deliver initial capacities exceeding 300 mAh g(-1) at 40 mA g(-1) in the voltage window of 0.5 to 2.8 V. The combined electron microscope, spectroscopy, and electrochemistry characterizations suggest a surface-controlled pseudocapacitive electrochemical reaction, and may be best described as a molecular energy storage mechanism. This work can provide a new approach of using the molecular mechanism for pseudocapacitive storage of Mg2+ for Mg batteries cathode materials. C1 [Cheng, Yingwen; Shao, Yuyan; Li, Guosheng; Liu, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Shao, Yuyan; Mehdi, B. Layla; Han, Kee Sung; Browning, Nigel D.; Mueller, Karl T.; Liu, Jun] Pacific NW Natl Lab, JCESR, Richland, WA 99352 USA. [Raju, Vadivukarasi; Ji, Xiulei] Oregon State Univ, Dept Chem, Gilbert Hall 153, Corvallis, OR 97331 USA. [Mehdi, B. Layla; Browning, Nigel D.; Mueller, Karl T.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Han, Kee Sung; Engelhard, Mark H.; Mueller, Karl T.] Pacific NW Natl Lab, EMSL, Richland, WA 99352 USA. [Browning, Nigel D.] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. RP Shao, YY; Liu, J (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA.; Shao, YY; Liu, J (reprint author), Pacific NW Natl Lab, JCESR, Richland, WA 99352 USA. EM yuyan.shao@pnnl.gov; jun.liu@pnnl.gov RI Shao, Yuyan/A-9911-2008; Cheng, Yingwen/B-2202-2012 OI Shao, Yuyan/0000-0001-5735-2670; Cheng, Yingwen/0000-0002-0778-5504 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Material Sciences and Engineering [KC020105-FWP12152]; Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; DOE's Office of Biological and Environmental Research; Department of Energy [DE-AC05-76RLO1830]; Oregon State University Venture Development Fund FX This research was supported by U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Material Sciences and Engineering, under Award KC020105-FWP12152. The (S) TEM and NMR studies were supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. (S) TEM, XPS, NMR, and Raman experiments were conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the Department of Energy under Contract No. DE-AC05-76RLO1830. V.R. and X.J. acknowledge support from the Oregon State University Venture Development Fund. NR 48 TC 2 Z9 2 U1 33 U2 84 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 24 PY 2016 VL 26 IS 20 BP 3446 EP 3453 DI 10.1002/adfm.201505501 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO2FP UT WOS:000377595600007 ER PT J AU Zhao, LC Luo, DY Wu, J Hu, Q Zhang, W Chen, K Liu, TH Liu, Y Zhang, YF Liu, F Russell, TP Snaith, HJ Zhu, R Gong, QH AF Zhao, Lichen Luo, Deying Wu, Jiang Hu, Qin Zhang, Wei Chen, Ke Liu, Tanghao Liu, Yi Zhang, Yifei Liu, Feng Russell, Thomas P. Snaith, Henry J. Zhu, Rui Gong, Qihuang TI High-Performance Inverted Planar Heterojunction Perovskite Solar Cells Based on Lead Acetate Precursor with Efficiency Exceeding 18% SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITES; THIN-FILMS; SEQUENTIAL DEPOSITION; TRIHALIDE PEROVSKITES; CH3NH3PBI3; IODIDE; LAYERS; CRYSTALLIZATION; HYSTERESIS; QUALITY AB Organic-inorganic lead halide perovskites are emerging materials for the next-generation photovoltaics. Lead halides are the most commonly used lead precursors for perovskite active layers. Recently, lead acetate (Pb(Ac)(2)) has shown its superiority as the potential replacement for traditional lead halides. Here, we demonstrate a strategy to improve the efficiency for the perovskite solar cell based on lead acetate precursor. We utilized methylammonium bromide as an additive in the Pb(Ac)(2) and methylammonium iodide precursor solution, resulting in uniform, compact and pinhole-free perovskite films. We observed enhanced charge carrier extraction between the perovskite layer and charge collection layers and delivered a champion power conversion efficiency of 18.3% with a stabilized output efficiency of 17.6% at the maximum power point. The optimized devices also exhibited negligible current density-voltage (J-V) hysteresis under the scanning conditions. C1 [Zhao, Lichen; Luo, Deying; Wu, Jiang; Hu, Qin; Chen, Ke; Liu, Tanghao; Liu, Yi; Zhang, Yifei; Zhu, Rui; Gong, Qihuang] Peking Univ, Dept Phys, State Key Lab Artificial Microstruct & Mesoscop P, Beijing 100871, Peoples R China. [Hu, Qin; Zhu, Rui; Gong, Qihuang] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Hu, Qin; Liu, Feng; Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhang, Wei; Snaith, Henry J.] Univ Oxford, Clarendon Lab, Dept Phys, Parks Rd, Oxford OX1 3PU, England. [Zhang, Wei] Lincoln Univ, Sch Chem, Beevor St, Lincoln LN6 7DL, England. [Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Zhu, Rui; Gong, Qihuang] Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China. RP Russell, TP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Russell, TP (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. EM russell@mail.pse.umass.edu; iamzhurui@pku.edu.cn RI Zhu, Rui/F-5244-2011; Zhu, Rui/E-7572-2010; Snaith, Henry/A-7367-2016; ZHANG, WEI/A-6955-2016; Hu, Qin/N-3493-2014; Liu, Feng/J-4361-2014 OI Zhu, Rui/0000-0001-7631-3589; Zhu, Rui/0000-0001-7631-3589; Snaith, Henry/0000-0001-8511-790X; ZHANG, WEI/0000-0002-2678-8372; Hu, Qin/0000-0003-3089-1070; Liu, Feng/0000-0002-5572-8512 FU 973 Program of China [2015CB932203]; National Natural Science Foundation of China [61377025, 91433203, 11121091]; Young 1000 Talents Global Recruitment Program of China; U.S. Office of Naval Research [N00014-15-1-2244]; Advanced Light Source Doctoral Fellowship in Residence at the Lawrence Berkeley National Laboratory FX L.Z. and D.L. contributed equally to this work. This work was financially supported by the 973 Program of China (2015CB932203), the National Natural Science Foundation of China (61377025, 91433203, and 11121091), and the Young 1000 Talents Global Recruitment Program of China. F.L. and T.P.R. were supported by the U.S. Office of Naval Research under contract N00014-15-1-2244. Q.H. also received support from the Advanced Light Source Doctoral Fellowship in Residence at the Lawrence Berkeley National Laboratory. The authors thank Prof. Shufeng Wang and Mr. Yu Li for the photoluminescence measurements. NR 44 TC 11 Z9 11 U1 74 U2 209 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 24 PY 2016 VL 26 IS 20 BP 3508 EP 3514 DI 10.1002/adfm.201601175 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO2FP UT WOS:000377595600014 ER PT J AU Mehra, S Bergerud, A Milliron, DJ Chan, EM Salleo, A AF Mehra, Saahil Bergerud, Amy Milliron, Delia J. Chan, Emory M. Salleo, Alberto TI Core/Shell Approach to Dopant Incorporation and Shape Control in Colloidal Zinc Oxide Nanorods SO CHEMISTRY OF MATERIALS LA English DT Article ID TUNABLE INFRARED-ABSORPTION; SURFACE-PLASMON RESONANCE; DOPED ZNO NANOCRYSTALS; CATION-EXCHANGE; THIN-FILMS; SEMICONDUCTOR NANOCRYSTALS; ALUMINUM; CHEMISTRY; DESIGN; IONS AB Tunable aliovalent doping is critical to controlling the optoelectronic properties of semiconductor nanocrystal systems. However, unintentional dopant-induced shape evolution and kinetically limited doping reactions in low temperature nanocrystal syntheses make it difficult to independently control shape and incorporate dopants in colloidal metal oxide nanocrystals. Here, we demonstrate a synthetic strategy for achieving simultaneous control of both nanorod shape and dopant concentration in colloidal zinc oxide nanorods. We show that this approach succeeds in doping zinc oxide nanorods using Group III dopants (indium or aluminum) in varying concentrations, and we quantify the effects of dopant incorporation on the structural, optical, and plasmonic properties of the nanorods. The synthesis of undoped zinc oxide nanorod templates and subsequent addition of dopant salts to the ongoing reaction enables both shape retention and dopant incorporation. Subsequent growth of an undoped shell on the nanorods incorporates surface segregated dopants with high efficiency. This "core/shell" doping strategy presents a general route to achieving controlled dopant incorporation and morphological retention in anisotropic metal oxide nanocrystal systems. C1 [Mehra, Saahil; Salleo, Alberto] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Bergerud, Amy] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Milliron, Delia J.; Chan, Emory M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Milliron, Delia J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. RP Salleo, A (reprint author), Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. EM asalleo@stanford.edu FU National Science Foundation [DMR1007886, DGE1106400]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge the National Science Foundation Award No. DMR1007886 for financial support. All experiments were performed as part of the Molecular Foundry User Program, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. A.B. was supported by a National Science Foundation Graduate Research Fellowship under Grant No. DGE1106400. NR 45 TC 2 Z9 2 U1 15 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 24 PY 2016 VL 28 IS 10 BP 3454 EP 3461 DI 10.1021/acs.chemmater.6b00981 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DN1KW UT WOS:000376825700028 ER PT J AU Mohoric, T Kokot, G Osterman, N Snezhko, A Vilfan, A Babic, D Dobnikar, J AF Mohoric, Tomaz Kokot, Gasper Osterman, Natan Snezhko, Alexey Vilfan, Andrej Babic, Dusan Dobnikar, Jure TI Dynamic Assembly of Magnetic Colloidal Vortices SO LANGMUIR LA English DT Article ID FIELDS; EQUILIBRIUM; COMPOSITES; DROPLETS; TORQUE; FLUIDS AB Magnetic colloids in external time-dependent fields are subject to complex induced many-body interactions governing their self-assembly into a variety of equilibrium and out-of-equilibrium structures such as chains, networks, suspended membranes, and colloidal foams. Here, we report experiments, simulations, and theory probing the dynamic assembly of superparamagnetic colloids in precessing external magnetic fields. Within a range of field frequencies, we observe dynamic large-scale structures such as ordered phases composed of precessing chains, ribbons, and rotating fluidic vortices. We show that the structure formation is inherently coupled to the buildup of torque, which originates from internal relaxation of induced dipoles and from transient correlations among the particles as a result of short-lived chain formation. We discuss in detail the physical properties of the vortex phase and demonstrate its potential in particle-coating applications. C1 [Mohoric, Tomaz; Dobnikar, Jure] Beijing Univ Chem Technol, Int Res Ctr Soft Matter, Beijing 100029, Peoples R China. [Mohoric, Tomaz] Univ Ljubljana, Dept Chem, Vecna Pot 113, Ljubljana 1000, Slovenia. [Babic, Dusan] Dept Math & Phys, Jadranska 19, Ljubljana 1000, Slovenia. [Kokot, Gasper; Osterman, Natan; Vilfan, Andrej] Univ Ljubljana, Jozef Stefan Inst, Jamova Cesta 39, Ljubljana 1000, Slovenia. [Snezhko, Alexey] Argonne Natl Lab, 9700 Cass Ave, Lemont, IL 60439 USA. [Dobnikar, Jure] Univ Cambridge, Dept Chem, Cambridge CB2 1TN, England. RP Dobnikar, J (reprint author), Beijing Univ Chem Technol, Int Res Ctr Soft Matter, Beijing 100029, Peoples R China.; Dobnikar, J (reprint author), Univ Cambridge, Dept Chem, Cambridge CB2 1TN, England. EM jd489@cam.ac.uk RI Vilfan, Andrej/B-1042-2008 OI Vilfan, Andrej/0000-0001-8985-6072 FU Fundamental Research Funds for the Central Universities of P. R. China [buctrc201422]; ERC [227758]; European ITN grant [234810]; Slovenian Research Agency (ARRS) funds through the Young Researchers Program [ARRS J1-5437]; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE AC02-06CH11357] FX We acknowledge inspiring discussions with Ignacio Pagonabarraga, Jim E. Martin, Emanuela Del Gado, Igor Aranson, and Daan Frenkel. This research was supported by the Fundamental Research Funds for the Central Universities of P. R. China under the project buctrc201422, ERC Advanced Grant 227758 (COLSTRUCTION), European ITN grant 234810 (COMPLOIDS), and Slovenian Research Agency (ARRS) funds through the Young Researchers Program, ARRS J1-5437 in P1-0099 grants. The research of A.S. was supported by the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under contract no. DE AC02-06CH11357. NR 53 TC 1 Z9 1 U1 11 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 24 PY 2016 VL 32 IS 20 BP 5094 EP 5101 DI 10.1021/acs.langmuir.6b00722 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DN1LB UT WOS:000376826200008 PM 27128501 ER PT J AU Heberle, FA Marquardt, D Doktorova, M Geier, B Standaert, RF Heftberger, P Kollmitzer, B Nickels, JD Dick, RA Feigenson, GW Katsaras, J London, E Pabst, G AF Heberle, Frederick A. Marquardt, Drew Doktorova, Milka Geier, Barbara Standaert, Robert F. Heftberger, Peter Kollmitzer, Benjamin Nickels, Jonathan D. Dick, Robert A. Feigenson, Gerald W. Katsaras, John London, Erwin Pabst, Georg TI Subnanometer Structure of an Asymmetric Model Membrane: Interleaflet Coupling Influences Domain Properties SO LANGMUIR LA English DT Article ID SMALL-ANGLE NEUTRON; GIANT UNILAMELLAR VESICLES; LIPID PHASES; CHAIN-LENGTH; BILAYERS; TEMPERATURE; SCATTERING; RAFTS; CHOLESTEROL; MIXTURES AB Cell membranes possess a complex three-dimensional architecture, including nonrandom lipid lateral organization within the plane of a bilayer leaflet, and compositional asymmetry between the two leaflets. As a result, delineating the membrane structure function relationship has been a highly challenging task. Even in simplified model systems, the interactions between bilayer leaflets are poorly understood, due in part to the difficulty of preparing asymmetric model membranes that are free from the effects of residual organic solvent or osmotic stress. To address these problems, we have modified a technique for preparing asymmetric large unilamellar vesicles (aLUVs) via cyclodextrin-mediated lipid exchange in order to produce tensionless, solvent-free aLUVs suitable for a range of biophysical studies. Leaflet composition and structure were characterized using isotopic labeling strategies, which allowed us to avoid the use of bulky labels. NMR and gas chromatography provided precise quantification of the extent of lipid exchange and bilayer asymmetry, while small-angle neutron scattering (SANS) was used to resolve bilayer structural features with subnanometer resolution. Isotopically asymmetric POPC vesicles were found to have the same bilayer thickness and area per lipid as symmetric POPC vesicles, demonstrating that the modified exchange protocol preserves native bilayer structure. Partial exchange of DPPC into the outer leaflet of POPC vesicles produced chemically asymmetric vesicles with a gel/fluid phase-separated outer leaflet and a uniform, POPC-rich inner leaflet. SANS was able to separately resolve the thicknesses and areas per lipid of coexisting domains, revealing reduced lipid packing density of the outer leaflet DPPC-rich phase compared to typical gel phases. Our finding that a disordered inner leaflet can partially fluidize ordered outer leaflet domains indicates some degree of interleaflet coupling, and invites speculation on a role for bilayer asymmetry in modulating membrane lateral organization. C1 [Heberle, Frederick A.; Nickels, Jonathan D.; Katsaras, John] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Heberle, Frederick A.; Nickels, Jonathan D.; Katsaras, John] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Standaert, Robert F.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Marquardt, Drew; Geier, Barbara; Heftberger, Peter; Kollmitzer, Benjamin; Pabst, Georg] Graz Univ, NAWI Graz, Inst Mol Biosci, Div Biophys, A-8010 Graz, Austria. [Marquardt, Drew; Geier, Barbara; Heftberger, Peter; Kollmitzer, Benjamin; Pabst, Georg] BioTechMed Graz, A-8010 Graz, Austria. [Doktorova, Milka] Weill Cornell Med Coll, Triinst PhD Program Computat Biol & Med, New York, NY 10065 USA. [Doktorova, Milka; Dick, Robert A.; Feigenson, Gerald W.] Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. [Standaert, Robert F.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [London, Erwin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Kollmitzer, Benjamin] Infineon Technol Austria AG, Dev Ctr Graz, Babenbergerstr 10, A-8010 Graz, Austria. RP Heberle, FA (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.; Heberle, FA (reprint author), Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA.; Marquardt, D; Pabst, G (reprint author), Graz Univ, NAWI Graz, Inst Mol Biosci, Div Biophys, A-8010 Graz, Austria.; Marquardt, D; Pabst, G (reprint author), BioTechMed Graz, A-8010 Graz, Austria. EM heberlefa@ornl.gov; drew.marquardt@uni-graz.at; georg.pabst@uni-graz.at RI Nickels, Jonathan/I-1913-2012; OI Nickels, Jonathan/0000-0001-8351-7846; Marquardt, Drew/0000-0001-6848-2497; Pabst, Georg/0000-0003-1967-1536 FU Austrian Science Fund (FWF) [P27083]; U.S. National Science Foundation [DMR 1404985]; U.S. National Institutes of Health [GM105684]; U.S. Department of Energy (DOE) Office of Basic Energy Sciences (BES) through the EPSCoR [DE-FG02-08ER46528]; University of Tennessee-Oak Ridge National Laboratory (ORNL) Joint Institute for Biological Sciences; Laboratory Directed Research and Development Program of ORNL; Scientific User Facilities Division of the DOE BES; US DOE [DE-AC05-00OR22725] FX We thank Lance Gill, Edward Hagaman, Thad Harroun, Qingqing Lin, Gerald Rechberger, Mijin Son, Chris Stanley, and Klaus Zangger for technical assistance and helpful discussions. This work acknowledges support from the Austrian Science Fund (FWF) project P27083 (to G.P.); U.S. National Science Foundation Grant DMR 1404985 (to E.L.); U.S. National Institutes of Health Grant GM105684 (to G.W.F.); the U.S. Department of Energy (DOE) Office of Basic Energy Sciences (BES) through the EPSCoR Grant DE-FG02-08ER46528 (to J.D.N.); the University of Tennessee-Oak Ridge National Laboratory (ORNL) Joint Institute for Biological Sciences (to F.A.H.); the Laboratory Directed Research and Development Program of ORNL (to J.K., R.F.S., J.D.N., and F.A.H.), managed by UT-Battelle, LLC, for the DOE; and from the Scientific User Facilities Division of the DOE BES, for the EQ-SANS instrument at the ORNL Spallation Neutron Source, managed by UT-Battelle, LLC under US DOE Contract No. DE-AC05-00OR22725. NR 31 TC 3 Z9 3 U1 12 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 24 PY 2016 VL 32 IS 20 BP 5195 EP 5200 DI 10.1021/acs.langmuir.5b04562 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DN1LB UT WOS:000376826200019 PM 27128636 ER PT J AU Mapas, JKD Thomay, T Cartwright, AN Ilavsky, J Rzayev, J AF Mapas, Jose Kenneth D. Thomay, Tim Cartwright, Alexander N. Ilavsky, Jan Rzayev, Javid TI Ultrahigh Molecular Weight Linear Block Copolymers: Rapid Access by Reversible-Deactivation Radical Polymerization and Self Assembly into Large Domain Nanostructures SO MACROMOLECULES LA English DT Article ID DIBLOCK COPOLYMERS; PHOTONIC CRYSTALS; MOLAR-MASS; TRIBLOCK COPOLYMERS; METHYL-METHACRYLATE; PHASE-BEHAVIOR; HIGH-PRESSURE; POLYDISPERSITY; POLYMERS; ATRP AB Block copolymer (BCP) derived periodic nanostructures with domain sizes larger than 150 nm present a versatile platform for the fabrication of photonic materials. So far, the access to such materials has been limited to highly synthetically involved protocols. Herein, we report a simple, "user-friendly" method for the preparation of ultrahigh molecular weight linear poly(solketal methacrylate-b-styrene) block copolymers by a combination of Cu-wire-mediated ATRP and RAFT polymerizations. The synthesized copolymers with molecular weights up to 1.6 million g/mol and moderate dispersities readily assemble into highly ordered cylindrical or lamella microstructures with domain sizes as large as 292 nm, as determined by ultrasmall-angle X-ray scattering and scanning electron microscopy analyses. Solvent cast films of the synthesized block copolymers exhibit stop bands in the visible spectrum correlated to their domain spacings. The described method opens new avenues for facilitated fabrication and the advancement of fundamental understanding of BCP-derived photonic nanomaterials for a variety of applications. C1 [Mapas, Jose Kenneth D.; Rzayev, Javid] SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. [Thomay, Tim; Cartwright, Alexander N.] SUNY Buffalo, Dept Elect Engn, Buffalo, NY 14260 USA. [Ilavsky, Jan] Argonne Natl Lab, Adv Photon Source Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Rzayev, J (reprint author), SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. EM jrzayev@buffalo.edu RI Ilavsky, Jan/D-4521-2013 OI Ilavsky, Jan/0000-0003-1982-8900 FU National Science Foundation [DMR-1409467]; University at Buffalo; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We acknowledge financial support from the National Science Foundation (DMR-1409467) and the University at Buffalo. The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 57 TC 2 Z9 2 U1 22 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 24 PY 2016 VL 49 IS 10 BP 3733 EP 3738 DI 10.1021/acs.macromol.6b00863 PG 6 WC Polymer Science SC Polymer Science GA DN1KT UT WOS:000376825400009 ER PT J AU Berger, EL Gao, J Li, CS Liu, ZL Zhu, HX AF Berger, Edmond L. Gao, Jun Li, Chong Sheng Liu, Ze Long Zhu, Hua Xing TI Charm-Quark Production in Deep-Inelastic Neutrino Scattering at Next-to-Next-to-Leading Order in QCD SO PHYSICAL REVIEW LETTERS LA English DT Article ID JET CROSS-SECTIONS; NNLO; DISTRIBUTIONS; DECAY; LHC AB We present a fully differential next-to-next-to-leading order calculation of charm-quark production in charged-current deep-inelastic scattering, with full charm-quark mass dependence. The next-to-next-to-leading order corrections in perturbative quantum chromodynamics are found to be comparable in size to the next-to-leading order corrections in certain kinematic regions. We compare our predictions with data on dimuon production in (anti)neutrino scattering from a heavy nucleus. Our results can be used to improve the extraction of the parton distribution function of a strange quark in the nucleon. C1 [Berger, Edmond L.; Gao, Jun] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Li, Chong Sheng; Liu, Ze Long] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Li, Chong Sheng; Liu, Ze Long] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Li, Chong Sheng] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. [Zhu, Hua Xing] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. RP Berger, EL; Gao, J (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.; Li, CS; Liu, ZL (reprint author), Peking Univ, Dept Phys, Beijing 100871, Peoples R China.; Li, CS; Liu, ZL (reprint author), Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.; Li, CS (reprint author), Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China.; Zhu, HX (reprint author), MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. EM berger@anl.gov; jgao@anl.gov; csli@pku.edu.cn; liuzelong@pku.edu.cn; zhuhx@mit.edu RI Gao, Jun/C-9777-2017 FU U.S. Department of Energy [DE-AC02-06CH11357]; Office of Nuclear Physics of the U.S. DOE [DE-SC0011090]; National Nature Science Foundation of China [11375013, 11135003] FX Work at the Argonne National Laboratory (ANL) is supported in part by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. H. X. Z. was supported by the Office of Nuclear Physics of the U.S. DOE under Contract No. DE-SC0011090. This work was also supported in part by the National Nature Science Foundation of China, under Grants No. 11375013 and No. 11135003. We thank Pavel Nadolsky for his valuable comments and Southern Methodist University for the use of the High Performance Computing facility ManeFrame. NR 59 TC 6 Z9 6 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2016 VL 116 IS 21 AR 212002 DI 10.1103/PhysRevLett.116.212002 PG 6 WC Physics, Multidisciplinary SC Physics GA DM8PO UT WOS:000376626600005 PM 27284650 ER PT J AU Cuevas-Maraver, J Kevrekidis, PG Saxena, A Comech, A Lan, RM AF Cuevas-Maraver, Jesus Kevrekidis, Panayotis G. Saxena, Avadh Comech, Andrew Lan, Ruomeng TI Stability of Solitary Waves and Vortices in a 2D Nonlinear Dirac Model SO PHYSICAL REVIEW LETTERS LA English DT Article ID LOCALIZED SOLUTIONS; SCHRODINGER-EQUATION; ORBITAL STABILITY; STATIONARY STATES; FIELD-THEORIES; SOLITONS; EXISTENCE; POINTS AB We explore a prototypical two-dimensional massive model of the nonlinear Dirac type and examine its solitary wave and vortex solutions. In addition to identifying the stationary states, we provide a systematic spectral stability analysis, illustrating the potential of spinor solutions to be neutrally stable in a wide parametric interval of frequencies. Solutions of higher vorticity are generically unstable and split into lower charge vortices in a way that preserves the total vorticity. These conclusions are found not to be restricted to the case of cubic two-dimensional nonlinearities but are found to be extended to the case of quintic nonlinearity, as well as to that of three spatial dimensions. Our results also reveal nontrivial differences with respect to the better understood nonrelativistic analogue of the model, namely the nonlinear Schrodinger equation. C1 [Cuevas-Maraver, Jesus] Univ Seville, Escuela Politecn Super, Dept Fis Aplicada 1, Grp Fis No Lineal, C Virgen Africa 7, Seville 41011, Spain. [Cuevas-Maraver, Jesus] IMUS, Edificio Celestino Mutis Avda Reina Mercedes S-N, Seville 41012, Spain. [Kevrekidis, Panayotis G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Kevrekidis, Panayotis G.; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Kevrekidis, Panayotis G.; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Comech, Andrew; Lan, Ruomeng] Texas A&M Univ, Dept Math, College Stn, TX 77843 USA. [Comech, Andrew] Inst Informat Transmiss Problems, Moscow 127994, Russia. RP Cuevas-Maraver, J (reprint author), Univ Seville, Escuela Politecn Super, Dept Fis Aplicada 1, Grp Fis No Lineal, C Virgen Africa 7, Seville 41011, Spain.; Cuevas-Maraver, J (reprint author), IMUS, Edificio Celestino Mutis Avda Reina Mercedes S-N, Seville 41012, Spain. EM jcuevas@us.es RI Cuevas-Maraver, Jesus/A-1255-2008 OI Cuevas-Maraver, Jesus/0000-0002-7162-5759 FU Russian Foundation for Sciences [14-50-00150]; U.S. Department of Energy; U.S.-NSF [DMS-1312856]; ERC [IRSES-605096] FX The research of A. C. was carried out at the Institute for Information Transmission Problems of the Russian Academy of Sciences at the expense of the Russian Foundation for Sciences (Project No. 14-50-00150). A. S. was supported by the U.S. Department of Energy. P. G. K. gratefully acknowledges the support of the U.S.-NSF under Award No. DMS-1312856, and of the ERC under FP7, Marie Curie Actions, People, International Research Staff Exchange Scheme (IRSES-605096). NR 54 TC 0 Z9 0 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2016 VL 116 IS 21 AR 214101 DI 10.1103/PhysRevLett.116.214101 PG 6 WC Physics, Multidisciplinary SC Physics GA DM8PO UT WOS:000376626600006 PM 27284659 ER PT J AU Ding, Y Yang, LX Chen, CC Kim, HS Han, MJ Luo, W Feng, ZX Upton, M Casa, D Kim, J Gog, T Zeng, ZD Cao, G Mao, HK van Veenendaal, M AF Ding, Yang Yang, Liuxiang Chen, Cheng-Chien Kim, Heung-Sik Han, Myung Joon Luo, Wei Feng, Zhenxing Upton, Mary Casa, Diego Kim, Jungho Gog, Thomas Zeng, Zhidan Cao, Gang Mao, Ho-kwang van Veenendaal, Michel TI Pressure-Induced Confined Metal from the Mott Insulator Sr3Ir2O7 SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY-SCATTERING; SUPERCONDUCTIVITY; TRANSITIONS AB The spin-orbit Mott insulator Sr3Ir2O7 provides a fascinating playground to explore insulator-metal transition driven by intertwined charge, spin, and lattice degrees of freedom. Here, we report high-pressure electric resistance and resonant inelastic x-ray scattering measurements on single-crystal Sr3Ir2O7 up to 63-65 GPa at 300 K. The material becomes a confined metal at 59.5 GPa, showing metallicity in the ab plane but an insulating behavior along the c axis. Such an unusual phenomenon resembles the strange metal phase in cuprate superconductors. Since there is no sign of the collapse of spin-orbit or Coulomb interactions in x-ray measurements, this novel insulator-metal transition is potentially driven by a first-order structural change at nearby pressures. Our discovery points to a new approach for synthesizing functional materials. C1 [Ding, Yang; Yang, Liuxiang; Zeng, Zhidan; Mao, Ho-kwang] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Ding, Yang; Chen, Cheng-Chien; Upton, Mary; Casa, Diego; Kim, Jungho; Gog, Thomas; van Veenendaal, Michel] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Ding, Yang; Yang, Liuxiang; Zeng, Zhidan; Mao, Ho-kwang] Carnegie Inst Sci, Geophys Lab, HPSynC, Argonne, IL 60439 USA. [Chen, Cheng-Chien] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Kim, Heung-Sik; Han, Myung Joon] Korea Adv Inst Sci & Technol, Dept Phys, Daejeon 305701, South Korea. [Luo, Wei] Condensed Matter Theory Grp, Box 530, SE-75121 Uppsala, Sweden. [Feng, Zhenxing] Argonne Natl Lab, Chem Sci & Engn, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cao, Gang] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [Mao, Ho-kwang] Carnegie Inst Sci, Geophys Lab, Washington, DC USA. [van Veenendaal, Michel] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Ding, Y (reprint author), Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China.; Ding, Y (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.; Ding, Y (reprint author), Carnegie Inst Sci, Geophys Lab, HPSynC, Argonne, IL 60439 USA. EM yang.ding@hpstar.ac.cn RI Han, Myung Joon/H-7104-2012 OI Han, Myung Joon/0000-0002-8089-7991 FU U.S. DOE [DE-AC02-06CH11357, DE-FG02-03ER46097]; Aneesur Rahman Postdoctoral Fellowship at ANL; Basic Science Research Program through NRF [2014R1A1A2057202]; Samsung Advanced Institute of Technology (SAIT); NSF [DMR1265162]; DOE-BES [DE-FG02-99ER45775]; NSFC [U1530402]; Institute for Nanoscience, Engineering, and Technology at Northern Illinois University FX The authors acknowledge useful discussions with Elizabeth Nowadnick. The RIXS measurements are performed at sectors 30 ID-B and 27 ID-B of Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science user facility operated by Argonne National Laboratory (ANL) supported by the U.S. DOE Award No. DE-AC02-06CH11357. C. C. C. is supported by the Aneesur Rahman Postdoctoral Fellowship at ANL. H.-S. K. and M. J. H. were supported by the Basic Science Research Program through NRF (Grant No. 2014R1A1A2057202) and by Samsung Advanced Institute of Technology (SAIT). G. C. acknowledges NSF support via Grant No. DMR1265162. H.-k. M. acknowledges the support of DOE-BES under Award No. DE-FG02-99ER45775 and NSFC Grant No. U1530402. M. v. V. is supported by the U.S. DOE under Award No. DE-FG02-03ER46097, and by the Institute for Nanoscience, Engineering, and Technology at Northern Illinois University. NR 57 TC 3 Z9 3 U1 12 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2016 VL 116 IS 21 AR 216402 DI 10.1103/PhysRevLett.116.216402 PG 6 WC Physics, Multidisciplinary SC Physics GA DM8PO UT WOS:000376626600007 PM 27284666 ER PT J AU Garmash, A Abdesselam, A Adachi, I Aihara, H Asner, DM Aushev, T Ayad, R Aziz, T Babu, V Badhrees, I Bakich, AM Behera, P Bhardwaj, V Bhuyan, B Bobrov, A Bondar, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chilikin, K Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Danilov, M Dash, N Dolezal, Z Drutskoy, A Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Ferber, T Fulsom, BG Gaur, V Gabyshev, N Gillard, R Goh, YM Goldenzweig, P Golob, B Hara, T Hayasaka, K Hayashii, H Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Joffe, D Joo, KK Julius, T Kang, KH Kato, E Kawasaki, T Kim, DY Kim, JB Kim, KT Kim, MJ Kim, SH Kim, YJ Kinoshita, K Korpar, S Krizan, P Krokovny, P Kuhr, T Kuzmin, A Kwon, YJ Lange, JS Lee, IS Li, C Li, H Li, L Gioi, LL Libby, J Liventsev, D Lukin, P Masuda, M Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Mori, T Mussa, R Nakano, E Nakao, M Nanut, T Natkaniec, Z Nishida, S Olsen, SL Pakhlov, P Pakhlova, G Pal, B Park, H Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Ribezl, E Ritter, M Rostomyan, A Sahoo, H Sakai, Y Sandilya, S Sanuki, T Savinov, V Schneider, O Schnell, G Schwanda, C Seino, Y Semmler, D Senyo, K Seong, IS Sevior, ME Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Simon, F Sohn, YS Solovieva, E Staric, M Sumiyoshi, T Tamponi, U Tanida, K Teramoto, Y Trabelsi, K Uchida, M Uehara, S Uglov, T Uno, S Van Hulse, C Vanhoefer, P Varner, G Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Watanabe, Y Williams, KM Won, E Yamamoto, H Yamaoka, J Yashchenko, S Yelton, J Yook, Y Yuan, CZ Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Garmash, A. Abdesselam, A. Adachi, I. Aihara, H. Asner, D. M. Aushev, T. Ayad, R. Aziz, T. Babu, V. Badhrees, I. Bakich, A. M. Behera, P. Bhardwaj, V. Bhuyan, B. Bobrov, A. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Danilov, M. Dash, N. Dolezal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Ferber, T. Fulsom, B. G. Gaur, V. Gabyshev, N. Gillard, R. Goh, Y. M. Goldenzweig, P. Golob, B. Hara, T. Hayasaka, K. Hayashii, H. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Joffe, D. Joo, K. K. Julius, T. Kang, K. H. Kato, E. Kawasaki, T. Kim, D. Y. Kim, J. B. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Kinoshita, K. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, I. S. Li, C. Li, H. Li, L. Gioi, L. Li Libby, J. Liventsev, D. Lukin, P. Masuda, M. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Mori, T. Mussa, R. Nakano, E. Nakao, M. Nanut, T. Natkaniec, Z. Nishida, S. Olsen, S. L. Pakhlov, P. Pakhlova, G. Pal, B. Park, H. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Ribezl, E. Ritter, M. Rostomyan, A. Sahoo, H. Sakai, Y. Sandilya, S. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Seino, Y. Semmler, D. Senyo, K. Seong, I. S. Sevior, M. E. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Simon, F. Sohn, Y. -S. Solovieva, E. Staric, M. Sumiyoshi, T. Tamponi, U. Tanida, K. Teramoto, Y. Trabelsi, K. Uchida, M. Uehara, S. Uglov, T. Uno, S. Van Hulse, C. Vanhoefer, P. Varner, G. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Watanabe, Y. Williams, K. M. Won, E. Yamamoto, H. Yamaoka, J. Yashchenko, S. Yelton, J. Yook, Y. Yuan, C. Z. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Observation of Z(b)(10610) and Z(b)(10650) Decaying to B Mesons SO PHYSICAL REVIEW LETTERS LA English DT Article AB We report the analysis of the three-body e(+)e(-) -> B (B) over bar pi(+/-), B (B) over bar*pi(+/-), and B*(B) over bar* pi(+/-) processes, including the first observations of the Z(b)(+/-)(10610) -> [B (B) over bar* + c.c.](+/-) and Z(b)(+/-)(10650) -> [B*(B) over bar*](+/-) transitions that are found to dominate the corresponding final states. We measure Born cross sections for the three-body production of sigma(e(+)e(-) -> [B (B) over bar* + c.c.](+/-)pi(-/+)) = [17.4 +/- 1.6(stat) +/- 1.9(syst)]pb and sigma(e(+)e(-) -> [B*(B) over bar*](+/-)pi(-/+)) = [8.75 +/- 1.15(stat) +/- 1.04(syst)] pb and set a 90% C.L. upper limit of sigma(e(+)e(-) -> [B (B) over bar](+/-)pi(-/+)) < 2.9 pb. The results are based on a 121.4 fb(-1) data sample collected with the Belle detector at a center-of-mass energy near the Upsilon(10860) peak. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Shen, C. P.; Zupanc, A.] Beihang Univ, Beijing 100191, Peoples R China. [Garmash, A.; Bobrov, A.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] RAS, SB, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Kinoshita, K.; Pal, B.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Yelton, J.] Univ Florida, Gainesville, FL 32611 USA. [Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Adachi, I.; Hara, T.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uehara, S.; Uno, S.] Grad Univ Adv Studies, SOKENDAI, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Seong, I. S.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Hara, T.; Itoh, R.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uehara, S.; Uno, S.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Basque Fdn Sci, Bilbao 48013, Spain. [Dash, N.] Indian Inst Technol Bhubaneswar, Satya Nagar 751007, India. [Bhuyan, B.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Behera, P.; Libby, J.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Li, H.] Indiana Univ, Bloomington, IN 47408 USA. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruher Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Cho, K.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kang, K. H.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.; Vanhoefer, P.] Univ Munich, Marchioninistr 15, D-80539 Munich, Germany. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Li, C.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Chilikin, K.; Danilov, M.; Drutskoy, A.; Mizuk, R.; Pakhlov, P.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Aushev, T.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Mori, T.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Natkaniec, Z.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Seino, Y.] Niigata Univ, Niigata 9502181, Japan. [Garmash, A.; Bobrov, A.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Fulsom, B. G.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Li, L.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Olsen, S. L.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Ayad, R.; Badhrees, I.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Aziz, T.; Babu, V.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Sandilya, S.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ishikawa, A.; Kato, E.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.; Epifanov, D.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Liventsev, D.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Garmash, A (reprint author), RAS, SB, Budker Inst Nucl Phys, Novosibirsk 630090, Russia.; Garmash, A (reprint author), Novosibirsk State Univ, Novosibirsk 630090, Russia. RI Pakhlov, Pavel/K-2158-2013; Aihara, Hiroaki/F-3854-2010; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014; Uglov, Timofey/B-2406-2014; Chilikin, Kirill/B-4402-2014; Drutskoy, Alexey/C-8833-2016; Mizuk, Roman/B-3751-2014; Danilov, Mikhail/C-5380-2014; Pakhlova, Galina/C-5378-2014 OI Krizan, Peter/0000-0002-4967-7675; Pakhlov, Pavel/0000-0001-7426-4824; Aihara, Hiroaki/0000-0002-1907-5964; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059; Uglov, Timofey/0000-0002-4944-1830; Chilikin, Kirill/0000-0001-7620-2053; Drutskoy, Alexey/0000-0003-4524-0422; Danilov, Mikhail/0000-0001-9227-5164; Pakhlova, Galina/0000-0001-7518-3022 FU MEXT (Japan); JSPS (Japan); Nagoya's TLPRC (Japan); ARC (Australia); DIISR (Australia); FWF (Austria); NSFC (China); MSMT (Czechia); CZF (Germany); DFG (Germany); VS (Germany); DST (India); INFN (Italy); MEST (Korea); NRF (Korea); GSDC of KISTI (Korea); WCU (Korea); MNiSW (Poland); NCN (Poland); MES (Russia); RFAAE (Russia); ARRS (Slovenia); IKERBASQUE (Spain); UPV/EHU (Spain); SNSF (Switzerland); NSC (Taiwan); MOE (Taiwan); DOE (U.S.); NSF (U.S.) FX We thank the KEKB group for excellent operation of the accelerator; the KEK cryogenics group for efficient solenoid operations; and the KEK computer group, the NII, and PNNL/EMSL for valuable computing and SINET4 network support. We acknowledge support from MEXT, JSPS, and Nagoya's TLPRC (Japan); ARC and DIISR (Australia); FWF (Austria); NSFC (China); MSMT (Czechia); CZF, DFG, and VS (Germany); DST (India); INFN (Italy); MEST, NRF, GSDC of KISTI, and WCU (Korea); MNiSW and NCN (Poland); MES and RFAAE (Russia); ARRS (Slovenia); IKERBASQUE and UPV/EHU (Spain); SNSF (Switzerland); NSC and MOE (Taiwan); and DOE and NSF (U.S.). NR 19 TC 7 Z9 7 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 24 PY 2016 VL 116 IS 21 AR 212001 DI 10.1103/PhysRevLett.116.212001 PG 7 WC Physics, Multidisciplinary SC Physics GA DM8PO UT WOS:000376626600004 PM 27284649 ER PT J AU Yang, Z Swedlund, P Gu, QF Hemar, Y Chaieb, S AF Yang, Zhi Swedlund, Peter Gu, Qinfen Hemar, Yacine Chaieb, Sahraoui TI Retrogradation of Maize Starch after High Hydrostatic Pressure Gelation: Effect of Amylose Content and Depressurization Rate SO PLOS ONE LA English DT Article ID X-RAY-DIFFRACTION; WAXY MAIZE; CORN STARCH; RHEOLOGICAL PROPERTIES; INFRARED-SPECTROSCOPY; IN-SITU; RICE; GELATINIZATION; AMYLOPECTIN; BEHAVIOR AB High hydrostatic pressure (HHP) has been employed to gelatinize or physically modify starch dispersions. In this study, waxy maize starch, normal maize starch, and two high amylose content starch were processed by a HHP of the order of 600 MPa, at 25 degrees C for 15min. The effect of HHP processing on the crystallization of maize starches with various amylose content during storage at 4 degrees C was investigated. Crystallization kinetics of HHP treated starch gels were investigated using rheology and FTIR. The effect of crystallization on the mechanical properties of starch gel network were evaluated in terms of dynamic complex modulus (G*). The crystallization induced increase of short-range helices structures were investigated using FTIR. The pressure releasing rate does not affect the starch retrogradation behaviour. The rate and extent of retrogradation depends on the amylose content of amylose starch. The least retrogradation was observed in HHP treated waxy maize starch. The rate of retrogradation is higher for HHP treated high amylose maize starch than that of normal maize starch. A linear relationship between the extent of retrogradation (phase distribution) measured by FTIR and G* is proposed. C1 [Yang, Zhi; Swedlund, Peter; Hemar, Yacine] Univ Auckland, Sch Chem Sci, Private Bag 92019, Auckland 1142, New Zealand. [Gu, Qinfen] Australian Synchrotron, 800 Blackburn Rd, Clayton, Vic 3168, Australia. [Chaieb, Sahraoui] KAUST, Div Biol & Environm Sci & Engn, Thuwal 23955, Saudi Arabia. [Chaieb, Sahraoui] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,Mailstop 6R-2100, Berkeley, CA 94720 USA. RP Chaieb, S (reprint author), KAUST, Div Biol & Environm Sci & Engn, Thuwal 23955, Saudi Arabia.; Chaieb, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,Mailstop 6R-2100, Berkeley, CA 94720 USA. EM sahraoui.chaieb@kaust.edu.sa FU KAUST FX We acknowledge the support of the plant and food research institute in providing the high pressure equipment used in this work. We thank Mr. Graeme Summers from Plant & Food Research Ltd. for his technical assistance. SC thanks KAUST for support. NR 46 TC 0 Z9 0 U1 12 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 24 PY 2016 VL 11 IS 5 AR e0156061 DI 10.1371/journal.pone.0156061 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN2FY UT WOS:000376880700038 PM 27219066 ER PT J AU Seinfeld, JH Bretherton, C Carslaw, KS Coe, H DeMott, PJ Dunlea, EJ Feingold, G Ghan, S Guenther, AB Kahn, R Kraucunas, I Kreidenweis, SM Molina, MJ Nenes, A Penner, JE Prather, KA Ramanathan, V Ramaswamy, V Rasch, PJ Ravishankara, AR Rosenfeld, D Stephens, G Wood, R AF Seinfeld, John H. Bretherton, Christopher Carslaw, Kenneth S. Coe, Hugh DeMott, Paul J. Dunlea, Edward J. Feingold, Graham Ghan, Steven Guenther, Alex B. Kahn, Ralph Kraucunas, Ian Kreidenweis, Sonia M. Molina, Mario J. Nenes, Athanasios Penner, Joyce E. Prather, Kimberly A. Ramanathan, V. Ramaswamy, Venkatachalam Rasch, Philip J. Ravishankara, A. R. Rosenfeld, Daniel Stephens, Graeme Wood, Robert TI Improving our fundamental understanding of the role of aerosol-cloud interactions in the climate system SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE climate; aerosol-cloud effects; general circulation models; radiative forcing; satellite observations ID HETEROGENEOUS ICE NUCLEATION; COMMUNITY ATMOSPHERE MODEL; ANTHROPOGENIC AEROSOLS; CONDENSATION NUCLEI; CONVECTIVE CLOUDS; BOUNDARY-LAYER; MIXING STATE; CCN ACTIVITY; VOCALS-REX; SATELLITE AB The effect of an increase in atmospheric aerosol concentrations on the distribution and radiative properties of Earth's clouds is the most uncertain component of the overall global radiative forcing from preindustrial time. General circulation models (GCMs) are the tool for predicting future climate, but the treatment of aerosols, clouds, and aerosol-cloud radiative effects carries large uncertainties that directly affect GCM predictions, such as climate sensitivity. Predictions are hampered by the large range of scales of interaction between various components that need to be captured. Observation systems (remote sensing, in situ) are increasingly being used to constrain predictions, but significant challenges exist, to some extent because of the large range of scales and the fact that the various measuring systems tend to address different scales. Fine-scale models represent clouds, aerosols, and aerosol-cloud interactions with high fidelity but do not include interactions with the larger scale and are therefore limited from a climatic point of view. We suggest strategies for improving estimates of aerosol-cloud relationships in climate models, for new remote sensing and in situ measurements, and for quantifying and reducing model uncertainty. C1 [Seinfeld, John H.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Seinfeld, John H.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Bretherton, Christopher; Wood, Robert] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. [Carslaw, Kenneth S.] Univ Leeds, Sch Earth & Environm, Leeds L32 9JT, W Yorkshire, England. [Coe, Hugh] Univ Manchester, Sch Earth Atmospher & Environm Sci, Manchester M13 9PL, Lancs, England. [DeMott, Paul J.; Kreidenweis, Sonia M.; Ravishankara, A. R.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Dunlea, Edward J.] Natl Acad Sci Engn & Med, Board Atmospher Sci & Climate, Washington, DC 20001 USA. [Feingold, Graham] NOAA, Earth Syst Res Lab, Boulder, CO 80523 USA. [Ghan, Steven; Kraucunas, Ian; Rasch, Philip J.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Guenther, Alex B.] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Kahn, Ralph] NASA, Goddard Space Flight Ctr, Sci & Explorat Directorate, Greenbelt, MD 20771 USA. [Molina, Mario J.; Prather, Kimberly A.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Molina, Mario J.; Prather, Kimberly A.; Ramanathan, V.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Nenes, Athanasios] Georgia Inst Technol, Dept Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Nenes, Athanasios] Georgia Inst Technol, Dept Chem & Biol Engn, Atlanta, GA 30332 USA. [Nenes, Athanasios] Fdn Res & Technol Hellas, Inst Chem Engn Sci, GR-26504 Patras, Greece. [Nenes, Athanasios] Natl Observ Athens, Inst Environm Res & Sustainable Dev, GR-15236 Palea Pendeli, Greece. [Penner, Joyce E.] Univ Michigan, Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. [Ramaswamy, Venkatachalam] Princeton Univ, Geophys Fluid Dynam Lab, Princeton, NJ 08540 USA. [Ramaswamy, Venkatachalam] NOAA, Princeton, NJ 08540 USA. [Rosenfeld, Daniel] Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. [Stephens, Graeme] NASA, Jet Prop Lab, Ctr Climate Sci, Pasadena, CA 91109 USA. RP Seinfeld, JH (reprint author), CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.; Seinfeld, JH (reprint author), CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. EM seinfeld@caltech.edu RI Ghan, Steven/H-4301-2011; DeMott, Paul/C-4389-2011; Rosenfeld, Daniel/F-6077-2016; Carslaw, Ken/C-8514-2009; Feingold, Graham/B-6152-2009; Wood, Robert/A-2989-2008; Kreidenweis, Sonia/E-5993-2011; Prather, Kimberly/A-3892-2008; Manager, CSD Publications/B-2789-2015; OI Ghan, Steven/0000-0001-8355-8699; DeMott, Paul/0000-0002-3719-1889; Rosenfeld, Daniel/0000-0002-0784-7656; Carslaw, Ken/0000-0002-6800-154X; Wood, Robert/0000-0002-1401-3828; Kreidenweis, Sonia/0000-0002-2561-2914; Prather, Kimberly/0000-0003-3048-9890; Coe, Hugh/0000-0002-3264-1713 FU US Department of Energy (DOE) [DE-AC06-76RLO 1830]; US DOE Decadal and Regional Climate Prediction; US DOE Earth System Modeling program FX The authors acknowledge Dr. Kristina Pistone for taking meticulous notes during the Colloquium. The Pacific Northwest National Laboratory (PNNL) is operated for the US Department of Energy (DOE) by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. Work at PNNL was supported by the US DOE Decadal and Regional Climate Prediction using Earth System Models program and by the US DOE Earth System Modeling program. NR 84 TC 10 Z9 10 U1 34 U2 83 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2016 VL 113 IS 21 BP 5781 EP 5790 DI 10.1073/pnas.1514043113 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN0UD UT WOS:000376779900033 PM 27222566 ER PT J AU DeMott, PJ Hill, TCJ McCluskey, CS Prather, KA Collins, DB Sullivan, RC Ruppel, MJ Mason, RH Irish, VE Lee, T Hwang, CY Rhee, TS Snider, JR McMeeking, GR Dhaniyala, S Lewis, ER Wentzell, JJB Abbatt, J Lee, C Sultana, CM Ault, AP Axson, JL Martinez, MD Venero, I Santos-Figueroa, G Stokes, MD Deane, GB Mayol-Bracero, OL Grassian, VH Bertram, TH Bertram, AK Moffett, BF Franc, GD AF DeMott, Paul J. Hill, Thomas C. J. McCluskey, Christina S. Prather, Kimberly A. Collins, Douglas B. Sullivan, Ryan C. Ruppel, Matthew J. Mason, Ryan H. Irish, Victoria E. Lee, Taehyoung Hwang, Chung Yeon Rhee, Tae Siek Snider, Jefferson R. McMeeking, Gavin R. Dhaniyala, Suresh Lewis, Ernie R. Wentzell, Jeremy J. B. Abbatt, Jonathan Lee, Christopher Sultana, Camille M. Ault, Andrew P. Axson, Jessica L. Martinez, Myrelis Diaz Venero, Ingrid Santos-Figueroa, Gilmarie Stokes, M. Dale Deane, Grant B. Mayol-Bracero, Olga L. Grassian, Vicki H. Bertram, Timothy H. Bertram, Allan K. Moffett, Bruce F. Franc, Gary D. TI Sea spray aerosol as a unique source of ice nucleating particles SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE marine aerosols; ice nucleation; clouds ID HYGROSCOPIC GROWTH; MARINE AIR; CHEMICAL-COMPOSITION; NUCLEI POPULATIONS; SIZE-DISTRIBUTION; FORMING NUCLEI; CLOUD; DUST; PRECIPITATION; RAIN AB Ice nucleating particles (INPs) are vital for ice initiation in, and precipitation from, mixed-phase clouds. A source of INPs from oceans within sea spray aerosol (SSA) emissions has been suggested in previous studies but remained unconfirmed. Here, we show that INPs are emitted using real wave breaking in a laboratory flume to produce SSA. The number concentrations of INPs from laboratory-generated SSA, when normalized to typical total aerosol number concentrations in the marine boundary layer, agree well with measurements from diverse regions over the oceans. Data in the present study are also in accord with previously published INP measurements made over remote ocean regions. INP number concentrations active within liquid water droplets increase exponentially in number with a decrease in temperature below 0 degrees C, averaging an order of magnitude increase per 5 degrees C interval. The plausibility of a strong increase in SSA INP emissions in association with phytoplankton blooms is also shown in laboratory simulations. Nevertheless, INP number concentrations, or active site densities approximated using "dry" geometric SSA surface areas, are a few orders of magnitude lower than corresponding concentrations or site densities in the surface boundary layer over continental regions. These findings have important implications for cloud radiative forcing and precipitation within low-level and midlevel marine clouds unaffected by continental INP sources, such as may occur over the Southern Ocean. C1 [DeMott, Paul J.; Hill, Thomas C. J.; McCluskey, Christina S.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Prather, Kimberly A.; Collins, Douglas B.; Ruppel, Matthew J.; Lee, Christopher; Sultana, Camille M.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Prather, Kimberly A.; Stokes, M. Dale; Deane, Grant B.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Sullivan, Ryan C.] Carnegie Mellon Univ, Ctr Atmospher Particle Studies, Pittsburgh, PA 15213 USA. [Mason, Ryan H.; Irish, Victoria E.; Bertram, Allan K.] Univ British Columbia, Dept Chem, 2036 Main Mall, Vancouver, BC V6T 1Z1, Canada. [Lee, Taehyoung] Hankuk Univ Foreign Studies, Dept Environm Sci, Yongin 449791, South Korea. [Hwang, Chung Yeon; Rhee, Tae Siek] Korea Polar Res Inst, Inchon 406840, South Korea. [Snider, Jefferson R.] Univ Wyoming, Dept Atmospher Sci, Laramie, WY 82071 USA. [McMeeking, Gavin R.] Handix Sci, Boulder, CO 80301 USA. [Dhaniyala, Suresh] Clarkson Univ, Dept Mech & Aeronaut Engn, Potsdam, NY 13699 USA. [Lewis, Ernie R.] Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA. [Wentzell, Jeremy J. B.] Environm Canada, Air Qual Processes Res Sect, Toronto, ON M3H 5T4, Canada. [Abbatt, Jonathan] Univ Toronto, Dept Chem, Toronto, ON M5S 3H6, Canada. [Ault, Andrew P.] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. [Ault, Andrew P.; Axson, Jessica L.] Univ Michigan, Dept Environm Hlth Sci, Ann Arbor, MI 48109 USA. [Martinez, Myrelis Diaz; Venero, Ingrid; Santos-Figueroa, Gilmarie; Mayol-Bracero, Olga L.] Univ Puerto Rico, Dept Environm Sci, San Juan, PR 00931 USA. [Grassian, Vicki H.] Univ Iowa, Dept Chem, Iowa City, IA 52242 USA. [Bertram, Allan K.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. [Moffett, Bruce F.] Fishguard Harbour, Ocean Lab, Goodwick SA64 0DE, Pembroke, Wales. [Franc, Gary D.] Univ Wyoming, Dept Plant Sci, Laramie, WY 82071 USA. [Ruppel, Matthew J.] High Tech High, San Marcos, CA 92078 USA. RP DeMott, PJ (reprint author), Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. EM Paul.Demott@colostate.edu RI Sullivan, Ryan/B-4674-2008; DeMott, Paul/C-4389-2011; Collins, Douglas/B-2788-2015; Prather, Kimberly/A-3892-2008; Ault, Andrew/E-4594-2011 OI Sullivan, Ryan/0000-0003-0701-7158; DeMott, Paul/0000-0002-3719-1889; Collins, Douglas/0000-0002-6248-9644; Prather, Kimberly/0000-0003-3048-9890; Ault, Andrew/0000-0002-7313-8559 FU National Science Foundation (NSF) [ATM0841602, AGS1036028, AGS-1358495, ATM0841542, AGS-0936879, ATM-0548036, AGS-1121915, AGS-1034858]; NSF Center for Chemical Innovation, Center for Aerosol Impacts on Climate and the Environment (CAICE) [CHE1305427]; National Aeronautics and Space Administration (NASA) Space Grant Consortium for Research Experiences for Undergraduates; Office of Biological and Environmental Research (OBER) of the US Department of Energy as part of the Atmospheric Radiation Measurement Climate Research Facility; US Department of Energy's Atmospheric System Research Program (Office of Science, OBER) [DE-SC00112704]; Korean Polar Research Program [PE13410]; NSF; Natural Sciences and Engineering Research Council of Canada FX We thank Horizon Lines and the captain and crew of the Spirit for their support and hospitality during MAGIC. Thanks to Benjamin Murray for sharing his previously published data for use in Fig. 3. Various authors acknowledge support for data collections used in this research from the National Science Foundation (NSF), including Grants ATM0841602, AGS1036028, and AGS-1358495 (to P.J.D.), ATM0841542 (to T.C.J.H.), AGS-0936879 (to O.L.M.-B.), ATM-0548036 and AGS-1121915 (to S.D.), and AGS-1034858 (to J.R.S.). Laboratory studies were supported via the NSF Center for Chemical Innovation, Center for Aerosol Impacts on Climate and the Environment (CAICE) under Grant CHE1305427 (to K.A.P.). O.L.M.-B. acknowledges the National Aeronautics and Space Administration (NASA) Space Grant Consortium for Research Experiences for Undergraduates funding of M.D.M. and I.V. Measurements during the MAGIC study were supported by the Office of Biological and Environmental Research (OBER) of the US Department of Energy as part of the Atmospheric Radiation Measurement Climate Research Facility. E.R.L. was supported by the US Department of Energy's Atmospheric System Research Program (Office of Science, OBER) under Contract DE-SC00112704. Support for data collected during SHIPPO was provided by the Korean Polar Research Program (PE13410). ICE-T aircraft data were provided by National Center for Atmospheric Research (NCAR)/Earth Observing Laboratory (EOL) under sponsorship of the NSF. The Natural Sciences and Engineering Research Council of Canada funded the MOUDI-DFT measurements carried out at CAICE and supported the ambient ice nucleating particle (INP) measurements onboard the icebreaker CGSS Amundsen through the NETCARE Project. NR 64 TC 19 Z9 19 U1 28 U2 64 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2016 VL 113 IS 21 BP 5797 EP 5803 DI 10.1073/pnas.1514034112 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN0UD UT WOS:000376779900035 PM 26699469 ER PT J AU Ghan, S Wang, MH Zhang, SP Ferrachat, S Gettelman, A Griesfeller, J Kipling, Z Lohmann, U Morrison, H Neubauer, D Partridge, DG Stier, P Takemura, T Wang, HL Zhang, K AF Ghan, Steven Wang, Minghuai Zhang, Shipeng Ferrachat, Sylvaine Gettelman, Andrew Griesfeller, Jan Kipling, Zak Lohmann, Ulrike Morrison, Hugh Neubauer, David Partridge, Daniel G. Stier, Philip Takemura, Toshihiko Wang, Hailong Zhang, Kai TI Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE aerosol radiative forcing; cloud-aerosol interactions; constraints; factors ID COMMUNITY ATMOSPHERE MODEL; GENERAL-CIRCULATION MODEL; GLOBAL CLIMATE MODEL; VERSION-3 CAM3; TECHNICAL NOTE; SATELLITE DATA; 2 SENSITIVITY; PHASE CLOUDS; PARAMETERIZATION; MICROPHYSICS AB A large number of processes are involved in the chain from emissions of aerosol precursor gases and primary particles to impacts on cloud radiative forcing. Those processes are manifest in a number of relationships that can be expressed as factors dlnX/dlnY driving aerosol effects on cloud radiative forcing. These factors include the relationships between cloud condensation nuclei (CCN) concentration and emissions, droplet number and CCN concentration, cloud fraction and droplet number, cloud optical depth and droplet number, and cloud radiative forcing and cloud optical depth. The relationship between cloud optical depth and droplet number can be further decomposed into the sum of two terms involving the relationship of droplet effective radius and cloud liquid water path with droplet number. These relationships can be constrained using observations of recent spatial and temporal variability of these quantities. However, we are most interested in the radiative forcing since the preindustrial era. Because few relevant measurements are available from that era, relationships from recent variability have been assumed to be applicable to the preindustrial to present-day change. Our analysis of Aerosol Comparisons between Observations and Models (AeroCom) model simulations suggests that estimates of relationships from recent variability are poor constraints on relationships from anthropogenic change for some terms, with even the sign of some relationships differing in many regions. Proxies connecting recent spatial/temporal variability to anthropogenic change, or sustained measurements in regions where emissions have changed, are needed to constrain estimates of anthropogenic aerosol impacts on cloud radiative forcing. C1 [Ghan, Steven; Wang, Minghuai; Wang, Hailong; Zhang, Kai] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Wang, Minghuai; Zhang, Shipeng] Nanjing Univ, Inst Climate & Global Change Res, Nanjing 210023, Jiangsu, Peoples R China. [Wang, Minghuai; Zhang, Shipeng] Nanjing Univ, Sch Atmospher Sci, Nanjing 210023, Jiangsu, Peoples R China. [Wang, Minghuai; Zhang, Shipeng] Collaborat Innovat Ctr Climate Change, Nanjing 210023, Peoples R China. [Ferrachat, Sylvaine; Lohmann, Ulrike; Neubauer, David] ETH, Inst Atmospher & Climate Sci, CH-8092 Zurich, Switzerland. [Gettelman, Andrew; Morrison, Hugh] Natl Ctr Atmospher Res, Boulder, CO 80305 USA. [Griesfeller, Jan] Norwegian Meteorol Inst, Informat Technol Div, N-0313 Oslo, Norway. [Kipling, Zak; Partridge, Daniel G.; Stier, Philip] Univ Oxford, Dept Phys, Atmospher Ocean & Planetary Phys, Oxford OX1 3PU, England. [Partridge, Daniel G.] Stockholm Univ, Dept Environm Sci & Analyt Chem, SE-10691 Stockholm, Sweden. [Partridge, Daniel G.] Stockholm Univ, Bert Bolin Ctr Climate Res, SE-10691 Stockholm, Sweden. [Takemura, Toshihiko] Kyushu Univ, Res Inst Appl Mech, Fukuoka 8168580, Japan. RP Ghan, S (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM Steve.Ghan@pnnl.gov RI Ghan, Steven/H-4301-2011; Kyushu, RIAM/F-4018-2015; Takemura, Toshihiko/C-2822-2009; Zhang, Kai/F-8415-2010; Stier, Philip/B-2258-2008; Wang, Hailong/B-8061-2010 OI Ghan, Steven/0000-0001-8355-8699; Takemura, Toshihiko/0000-0002-2859-6067; Zhang, Kai/0000-0003-0457-6368; Stier, Philip/0000-0002-1191-0128; Wang, Hailong/0000-0002-1994-4402 FU Department of Energy (DOE) [DE-AC06-76RLO 1830]; US DOE Decadal and Regional Climate Prediction; US DOE Earth System Modeling program; One Thousand Young Talent Program; Jiangsu Province Specially-Appointed Professor Grant; National Natural Science Foundation of China [41575073]; Austrian Science Fund [J 3402-N29]; Swiss National Supercomputing Centre [s431]; United Kingdom (UK) Natural Environment Research Council [NE/I020148/1]; European Research Council (ERC) [FP7-280025]; National Environmental Research Council (NERC); Joint Department of Energy & Climate Change/Department for Environment, Food & Rural Affairs Meteorology Office Hadley Centre Climate Programme; Environment Research and Technology Development Fund of the Ministry of the Environment, Japan [S-12-3]; Japan Society for the Promotion of Science KAKENHI [15H01728, 15K12190]; US National Science Foundation FX Peter Caldwell prodded our thinking on factorization, Rob Wood coaxed us to explore the role of cloud fraction, and Nicolas Bellouin provided helpful comments. Reviewer comments were also helpful. The Pacific Northwest National Laboratory (PNNL) is operated for the Department of Energy (DOE) by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. Work at PNNL was supported by the US DOE Decadal and Regional Climate Prediction using Earth System Models program and by the US DOE Earth System Modeling program. Work of M.W. and S.Z. performed at Nanjing University was supported by the One Thousand Young Talent Program, Jiangsu Province Specially-Appointed Professor Grant, and the National Natural Science Foundation of China (41575073). A portion of this research was performed using PNNL Institutional Computing resources. The ECHAM6-HAM model was developed by a consortium composed of ETH Zurich, Max Planck Institut fur Meteorologie, Forschungszentrum Julich, University of Oxford, the Finnish Meteorological Institute, and the Leibniz Institute for Tropospheric Research, and is managed by the Center for Climate Systems Modeling (C2SM) at ETH Zurich. D.N. acknowledges support by the Austrian Science Fund (J 3402-N29, Erwin Schrodinger Fellowship Abroad). C2SM at ETH Zurich is acknowledged for providing technical and scientific support. This work was also supported by a grant from the Swiss National Supercomputing Centre under Project ID s431. D.G.P. and P.S. acknowledge support from the United Kingdom (UK) Natural Environment Research Council Grant NE/I020148/1. P.S. and Z.K. acknowledge funding from the European Research Council (ERC) under the European Union's Seventh Framework Programme (FP7/2007-2013) ERC project ACCLAIM (Grant Agreement FP7-280025). The development of modal version of the GLObal Model of Aerosol Processes (GLOMAP-mode) within Hadley Center Global Environmental Mode (HadGEM) is part of the United Kingdom Chemistry and Aerosols (UKCA) project, which is supported by both National Environmental Research Council (NERC) and the Joint Department of Energy & Climate Change/Department for Environment, Food & Rural Affairs Meteorology Office Hadley Centre Climate Programme. We acknowledge use of the Met Office and NERC MONSooN high performance computing system, a collaborative facility supplied under the Joint Weather and Climate Research Programme, a strategic partnership between the Met Office and the NERC. Simulations by SPRINTARS were executed with the supercomputer system SX-9/ACE of the National Institute for Environmental Studies, Japan. SPRINTARS is partly supported by the Environment Research and Technology Development Fund (S-12-3) of the Ministry of the Environment, Japan and Japan Society for the Promotion of Science KAKENHI Grants-in-Aid for Scientific Research 15H01728 and 15K12190. Computing resources for CAM5-MG2 simulations were provided by the Climate Simulation Laboratory at National Center for Atmospheric Research (NCAR) Computational and Information Systems Laboratory. NCAR is sponsored by the US National Science Foundation. NR 71 TC 10 Z9 10 U1 5 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2016 VL 113 IS 21 BP 5804 EP 5811 DI 10.1073/pnas.1514036113 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN0UD UT WOS:000376779900036 PM 26921324 ER PT J AU Wolf, S Keenan, TF Fisher, JB Baldocchi, DD Desai, AR Richardson, AD Scott, RL Law, BE Litvak, ME Brunsell, NA Peters, W van der Laan-Luijkx, IT AF Wolf, Sebastian Keenan, Trevor F. Fisher, Joshua B. Baldocchi, Dennis D. Desai, Ankur R. Richardson, Andrew D. Scott, Russell L. Law, Beverly E. Litvak, Marcy E. Brunsell, Nathaniel A. Peters, Wouter van der Laan-Luijkx, Ingrid T. TI Warm spring reduced carbon cycle impact of the 2012 US summer drought SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE seasonal climate anomalies; carbon uptake; ecosystem fluxes; biosphere; atmosphere feedbacks; eddy covariance ID EDDY-COVARIANCE; SOIL-MOISTURE; CLIMATE; FOREST; REDUCTION; EXCHANGE; DIOXIDE; HEAT; PREDICTABILITY; FEEDBACKS AB The global terrestrial carbon sink offsets one-third of the world's fossil fuel emissions, but the strength of this sink is highly sensitive to large-scale extreme events. In 2012, the contiguous United States experienced exceptionally warm temperatures and the most severe drought since the Dust Bowl era of the 1930s, resulting in substantial economic damage. It is crucial to understand the dynamics of such events because warmer temperatures and a higher prevalence of drought are projected in a changing climate. Here, we combine an extensive network of direct ecosystem flux measurements with satellite remote sensing and atmospheric inverse modeling to quantify the impact of the warmer spring and summer drought on biosphere-atmosphere carbon and water exchange in 2012. We consistently find that earlier vegetation activity increased spring carbon uptake and compensated for the reduced uptake during the summer drought, which mitigated the impact on net annual carbon uptake. The early phenological development in the Eastern Temperate Forests played a major role for the continental-scale carbon balance in 2012. The warm spring also depleted soilwater resources earlier, and thus exacerbated water limitations during summer. Our results show that the detrimental effects of severe summer drought on ecosystem carbon storage can be mitigated by warming-induced increases in spring carbon uptake. However, the results also suggest that the positive carbon cycle effect of warm spring enhances water limitations and can increase summer heating through biosphere-atmosphere feedbacks. C1 [Wolf, Sebastian; Baldocchi, Dennis D.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Wolf, Sebastian] ETH, Dept Environm Syst Sci, CH-8092 Zurich, Switzerland. [Keenan, Trevor F.] Macquarie Univ, Dept Biol Sci, Sydney, NSW 2109, Australia. [Fisher, Joshua B.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Desai, Ankur R.] Univ Wisconsin, Atmospher & Ocean Sci, Madison, WI 53706 USA. [Richardson, Andrew D.] Harvard Univ, Dept Organism & Evolutionary Biol, Cambridge, MA 02138 USA. [Scott, Russell L.] USDA ARS, Southwest Watershed Res Ctr, Tucson, AZ 85719 USA. [Law, Beverly E.] Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. [Litvak, Marcy E.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. [Brunsell, Nathaniel A.] Univ Kansas, Dept Geog, Lawrence, KS 66045 USA. [Peters, Wouter; van der Laan-Luijkx, Ingrid T.] Wageningen Univ, Dept Meteorol & Air Qual, NL-6708 PB Wageningen, Netherlands. [Peters, Wouter] Univ Groningen, Ctr Isotope Res, NL-9747 AG Groningen, Netherlands. [Keenan, Trevor F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci, Berkeley, CA 94720 USA. RP Wolf, S (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA.; Wolf, S (reprint author), ETH, Dept Environm Syst Sci, CH-8092 Zurich, Switzerland. EM sewolf@ethz.ch RI van der Laan-Luijkx, Ingrid/G-9169-2011; Wolf, Sebastian/B-4580-2010; Keenan, Trevor/B-2744-2010; Baldocchi, Dennis/A-1625-2009; Law, Beverly/G-3882-2010; OI van der Laan-Luijkx, Ingrid/0000-0002-3990-6737; Wolf, Sebastian/0000-0001-7717-6993; Keenan, Trevor/0000-0002-3347-0258; Baldocchi, Dennis/0000-0003-3496-4919; Law, Beverly/0000-0002-1605-1203; Desai, Ankur/0000-0002-5226-6041; Fisher, Joshua/0000-0003-4734-9085 FU Carbon Dioxide Information Analysis Center at the Oak Ridge National Laboratory; European Commission [300083]; US Department of Energy's Office of Science [DE-AC02-05CH11231]; Macquarie University Research Fellowship; National Aeronautics and Space Administration; NASA's Terrestrial Hydrology Program; National Science Foundation (NSF), through the Macrosystems Biology program [EF-1065029]; LTER program [DEB-1114804]; NASA ROSES [0486V-874F]; NSF EPSCoR program [EPS-0553722, EPS-0919443]; LTER program at the Konza Prairie Biological Station [DEB-0823341]; NWO [SH-060-13]; OCW/NWO for ICOS-NL FX We acknowledge support from the Carbon Dioxide Information Analysis Center at the Oak Ridge National Laboratory, particularly B. Yang. We thank D. M. Ricciuto for assistance with the gap-filling of climate data and M. Sikka for remote-sensing data processing. We thank all data contributors for this synthesis study, particularly P. Blanken, G. Bohrer, D. Bowling, S. Burns, K. L. Clark, D. Hollinger, S. Ma, Q. Mu, K. A. Novick, S. A. Papuga, F. Rahman, and M. Zhao. We thank K. A. Novick, G. Bohrer, E. van Gorsel, and E. Paul-Limoges for helpful comments on the manuscript. We also appreciate the constructive comments of the reviewers and the editor. This research was supported by the European Commission's FP7 Marie Curie International Outgoing Fellowship Grant 300083 (to S.W.). Funding for the AmeriFlux Management Project was provided by the US Department of Energy's Office of Science (Contract DE-AC02-05CH11231). T.F.K. acknowledges support from a Macquarie University Research Fellowship. J.B.F. carried out the research at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration, and acknowledges support from NASA's Terrestrial Hydrology Program. A.D.R. acknowledges support from the National Science Foundation (NSF), through the Macrosystems Biology program (Award EF-1065029) and the LTER program (DEB-1114804). M. E. L. acknowledges support from NASA ROSES (Award 0486V-874F). N.A.B. acknowledges support from the NSF EPSCoR program (EPS-0553722 and EPS-0919443) and the LTER program at the Konza Prairie Biological Station (DEB-0823341). W. P. and I.T.v.d.L.-L. acknowledge funding from NWO (SH-060-13) for computing time. I.T.v.d.L.-L. received financial support from OCW/NWO for ICOS-NL. NR 39 TC 9 Z9 9 U1 16 U2 51 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2016 VL 113 IS 21 BP 5880 EP 5885 DI 10.1073/pnas.1519620113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN0UD UT WOS:000376779900048 PM 27114518 ER PT J AU Ghan, S Wang, MH Zhang, SP Ferrachat, S Gettelman, A Griesfeller, J Kipling, Z Lohmann, U Morrison, H Neubauer, D Partridge, DG Stier, P Takemura, T Wang, HL Zhang, K AF Ghan, Steven Wang, Minghuai Zhang, Shipeng Ferrachat, Sylvaine Gettelman, Andrew Griesfeller, Jan Kipling, Zak Lohmann, Ulrike Morrison, Hugh Neubauer, David Partridge, Daniel G. Stier, Philip Takemura, Toshihiko Wang, Hailong Zhang, Kai TI Challenges in constraining anthropogenic aerosol effects on cloud radiative forcing using present-day spatiotemporal variability (vol 113, pg 5804, 2016) SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Correction C1 [Ghan, Steven; Wang, Minghuai; Wang, Hailong; Zhang, Kai] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Wang, Minghuai; Zhang, Shipeng] Nanjing Univ, Inst Climate & Global Change Res, Nanjing 210023, Jiangsu, Peoples R China. [Wang, Minghuai; Zhang, Shipeng] Nanjing Univ, Sch Atmospher Sci, Nanjing 210023, Jiangsu, Peoples R China. [Wang, Minghuai; Zhang, Shipeng] Collaborat Innovat Ctr Climate Change, Nanjing 210023, Jiangsu, Peoples R China. [Ferrachat, Sylvaine; Lohmann, Ulrike; Neubauer, David] ETH, Inst Atmospher & Climate Sci, CH-8092 Zurich, Switzerland. [Gettelman, Andrew; Morrison, Hugh] Natl Ctr Atmospher Res, Boulder, CO 80305 USA. [Griesfeller, Jan] Norwegian Meteorol Inst, Informat Technol Div, N-0313 Oslo, Norway. [Kipling, Zak; Partridge, Daniel G.; Stier, Philip] Univ Oxford, Dept Phys, Atmospher Ocean & Planetary Phys, Oxford OX1 3PU, England. [Partridge, Daniel G.] Stockholm Univ, Dept Environm Sci & Analyt Chem, SE-10691 Stockholm, Sweden. [Partridge, Daniel G.] Stockholm Univ, Bert Bolin Ctr Climate Res, SE-10691 Stockholm, Sweden. [Takemura, Toshihiko] Kyushu Univ, Res Inst Appl Mech, Fukuoka 8168580, Japan. RP Ghan, S (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RI Kyushu, RIAM/F-4018-2015 NR 1 TC 0 Z9 0 U1 0 U2 2 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 24 PY 2016 VL 113 IS 21 BP E3049 EP E3049 DI 10.1073/pnas.1604888113 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DN0UD UT WOS:000376779900024 ER PT J AU Lecot, P Alimirah, F Desprez, PY Campisi, J Wiley, C AF Lecot, Pacome Alimirah, Fatouma Desprez, Pierre-Yves Campisi, Judith Wiley, Christopher TI Context-dependent effects of cellular senescence in cancer development SO BRITISH JOURNAL OF CANCER LA English DT Review DE immunosurveillance; inflammation; oncogene; senescence-associated secretory phenotype; tumour progression; tumour suppression ID SECRETORY PHENOTYPE; TUMOR SUPPRESSION; MITOCHONDRIAL DYSFUNCTION; DAMAGE RESPONSE; CELLS; P53; RESTORATION; CLEARANCE; REGULATOR; APOPTOSIS AB Cellular senescence is an established tumour-suppressive mechanism that prevents the proliferation of premalignant cells. However, several lines of evidence show that senescent cells, which often persist in vivo, can also promote tumour progression in addition to other age-related pathologies via the senescence-associated secretory phenotype (SASP). Moreover, new insights suggest the SASP can facilitate tissue repair. Here, we review the beneficial and detrimental roles of senescent cells, highlighting conditions under which the senescence response does and does not promote pathology, particularly cancer. By better understanding the context-dependent effects of cellular senescence, it may be feasible to limit its detrimental properties while preserving its beneficial effects, and develop novel therapeutic strategies to prevent or treat cancer and possibly other age-associated diseases. C1 [Lecot, Pacome; Alimirah, Fatouma; Desprez, Pierre-Yves; Campisi, Judith; Wiley, Christopher] Buck Inst Res Aging, 8001 Redwood Blvd, Novato, CA 94945 USA. [Desprez, Pierre-Yves] Calif Pacific Med Ctr, 475 Brannan St, San Francisco, CA 94107 USA. [Campisi, Judith] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Wiley, C (reprint author), Buck Inst Res Aging, 8001 Redwood Blvd, Novato, CA 94945 USA. EM cwiley@buckinstitute.org NR 40 TC 2 Z9 2 U1 4 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0007-0920 EI 1532-1827 J9 BRIT J CANCER JI Br. J. Cancer PD MAY 24 PY 2016 VL 114 IS 11 BP 1180 EP 1184 DI 10.1038/bjc.2016.115 PG 5 WC Oncology SC Oncology GA DM6AE UT WOS:000376431200007 PM 27140310 ER PT J AU Collier, R Bragg, J Hernandez, BT Vogel, JP Thilmony, R AF Collier, Ray Bragg, Jennifer Hernandez, Bryan T. Vogel, John P. Thilmony, Roger TI Use of Agrobacterium rhizogenes Strain 18r12v and Paromomycin Selection for Transformation of Brachypodium distachyon and Brachypodium sylvaticum SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE transformation; Brachypodium; Agrobacterium rhizogenes; paromomycin; tissue culture; callus ID SELECTABLE MARKER GENES; MEDIATED TRANSFORMATION; PLANT TRANSFORMATION; PARTICLE BOMBARDMENT; POLYUBIQUITIN GENES; PROMOTER ACTIVITY; EXPRESSION; L.; ELECTROPORATION; PROTOPLASTS AB The genetic transformation of monocot grasses is a resource intensive process, the quality and efficiency of which is dependent in part upon the method of DNA introduction, as well as the ability to effectively separate transformed from wildtype tissue. Agrobacterium-mediated transformation of Brachypodium has relied mainly on Agrobacterium tumefaciens strain AGL1. Currently the antibiotic hygromycin B has been the selective agent of choice for robust identification of transgenic calli in Brachypodium distachyon and Brachypodium sylvaticum but few other chemicals have been shown to work as well for selection of transgenic Brachypodium cells in tissue culture. This study demonstrates that Agrobacterium rhizogenes strain 18r12v and paromomycin selection can be successfully used for the efficient generation of transgenic B. distachyon and B. sylvaticurn. Additionally we observed that the transformation rates were similar to or higher than those obtained with A. turnefaciens strain AGL1 and hygromycin selection. The A. rhizogenes strain 18r12v harboring the pARS1 binary vector and paromomycin selection is an effective means of generating transgenic Brachypodium plants. This novel approach will facilitate the transgenic complementation of T-DNA knockout mutants of B. distachyon which were created using hygromycin selection, as well as aid the implementation of more complex genome manipulation strategies which require multiple rounds of transformation. C1 [Collier, Ray; Bragg, Jennifer; Vogel, John P.; Thilmony, Roger] USDA ARS, Crop Improvement & Genet Res Unit, Western Reg Res Ctr, Albany, CA USA. [Hernandez, Bryan T.] Univ Calif Davis, Dept Plant Sci, Davis, CA 95616 USA. [Vogel, John P.] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. RP Thilmony, R (reprint author), USDA ARS, Crop Improvement & Genet Res Unit, Western Reg Res Ctr, Albany, CA USA. EM roger.thilmony@ars.usda.gov FU USDA Agricultural Research Service CRIS project [2030-21000-020-00D]; Office of Biological and Environmental Research, Office of Science, US Department of Energy [DE-SC0001526]; U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231] FX RC, BH, and RT were supported by USDA Agricultural Research Service CRIS project 2030-21000-020-00D. JB and JV were supported by Office of Biological and Environmental Research, Office of Science, US Department of Energy, interagency agreement DE-SC0001526. The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-AC02-05CH11231. Mention of trade names or commercial products is solely for the purpose of providing specific information and does not imply recommendation or endorsement by the US Department of Agriculture. USDA is an equal opportunity provider and employer. NR 32 TC 0 Z9 0 U1 7 U2 12 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAY 24 PY 2016 VL 7 AR 716 DI 10.3389/fpls.2016.00716 PG 9 WC Plant Sciences SC Plant Sciences GA DN0HD UT WOS:000376744100001 PM 27252729 ER PT J AU Aytac, Y Olson, BV Kim, JK Shaner, EA Hawkins, SD Klem, JF Flatte, ME Boggess, TF AF Aytac, Y. Olson, B. V. Kim, J. K. Shaner, E. A. Hawkins, S. D. Klem, J. F. Flatte, M. E. Boggess, T. F. TI Evidence of a Shockley-Read-Hall Defect State Independent of Band-Edge Energy in InAs/In(As,Sb) Type-II Superlattices SO PHYSICAL REVIEW APPLIED LA English DT Article AB A set of seven InAs/In(As, Sb) type-II superlattices (T2SLs) are designed to have specific band-gap energies between 290 meV (4.3 mu m) and 135 meV (9.2 mu m) in order to study the effects of the T2SL band-gap energy on the minority-carrier lifetime. A temperature-dependent optical pump-probe technique is used to measure the carrier lifetimes, and the effect of a midgap defect level on the carrier-recombination dynamics is reported. The Shockley-Read-Hall (SRH) defect state is found to be at energy of approximately -250 +/- 12 meV relative to the valence-band edge of bulk GaSb for the entire set of T2SL structures, even though the T2SL valence-band edge shifts by 155 meV on the same scale. These results indicate that the SRH defect state in InAs/In(As, Sb) T2SLs is singular and is nearly independent of the exact position of the T2SL band-gap or band-edge energies. They also suggest the possibility of engineering the T2SL structure such that the SRH state is removed completely from the band gap, a result that should significantly increase the minority-carrier lifetime. C1 [Aytac, Y.; Flatte, M. E.; Boggess, T. F.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Aytac, Y.; Flatte, M. E.; Boggess, T. F.] Univ Iowa, Opt Sci & Technol Ctr, Iowa City, IA 52242 USA. [Olson, B. V.; Kim, J. K.; Shaner, E. A.; Hawkins, S. D.; Klem, J. F.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Aytac, Y (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA.; Aytac, Y (reprint author), Univ Iowa, Opt Sci & Technol Ctr, Iowa City, IA 52242 USA. EM yigit-aytac@uiowa.edu FU U.S. government; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This research is funded by the U.S. government. NR 25 TC 3 Z9 3 U1 10 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD MAY 24 PY 2016 VL 5 IS 5 AR 054016 DI 10.1103/PhysRevApplied.5.054016 PG 6 WC Physics, Applied SC Physics GA DM8XL UT WOS:000376647700001 ER PT J AU Gan, Y de la Pena, GA Kogar, A Uchoa, B Casa, D Gog, T Fradkin, E Abbamonte, P AF Gan, Yu de la Pena, Gilberto A. Kogar, Anshul Uchoa, Bruno Casa, Diego Gog, Thomas Fradkin, Eduardo Abbamonte, Peter TI Reexamination of the effective fine structure constant of graphene as measured in graphite SO PHYSICAL REVIEW B LA English DT Article ID TOPOLOGICAL INSULATORS AB We present a refined and improved study of the influence of screening on the effective fine structure constant of graphene, alpha*, as measured in graphite using inelastic x-ray scattering. This followup to our previous study [J. P. Reed et al., Science 330, 805 (2010)] was carried out with two times better energy resolution, five times better momentum resolution, and an improved experimental setup with lower background. We compare our results to random-phase approximation (RPA) calculations and evaluate the relative importance of interlayer hopping, excitonic corrections, and screening from high energy excitations involving the sigma bands. We find that the static, limiting value of alpha* falls in the range 0.25-0.35, which is higher than our previous result of 0.14, but still below the value expected from RPA. We show the reduced value is not a consequence of interlayer hopping effects, which were ignored in our previous analysis, but of a combination of excitonic effects in the pi -> pi* particle-hole continuum, and background screening from the sigma-bonded electrons. We find that sigma-band screening is extremely strong at distances of less than a few nanometers, and should be highly effective at screening out short-distance, Hubbard-like interactions in graphene as well as other carbon allotropes. C1 [Gan, Yu; de la Pena, Gilberto A.; Kogar, Anshul; Fradkin, Eduardo; Abbamonte, Peter] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Gan, Yu; de la Pena, Gilberto A.; Kogar, Anshul; Fradkin, Eduardo; Abbamonte, Peter] Univ Illinois, Federick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Uchoa, Bruno] Univ Oklahoma, Dept Phys & Astron, Norman, OK 73019 USA. [Casa, Diego; Gog, Thomas; Abbamonte, Peter] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Gan, Y (reprint author), Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA.; Gan, Y (reprint author), Univ Illinois, Federick Seitz Mat Res Lab, Urbana, IL 61801 USA. FU US Department of Energy [DE-FG02-06ER46285]; NSF CAREER Grant [DMR-1352604]; DOE [DE-SC001236]; EPiQS Initiative of the Gordon and Betty Moore Foundation [GBMF4542]; [DEAC02-06CH11357] FX The authors acknowledge helpful discussions with L. K. Wagner. This work was supported by the US Department of Energy Grant No. DE-FG02-06ER46285, with use of the Advanced Photon Source supported by DEAC02-06CH11357. B.U. acknowledges NSF CAREER Grant No. DMR-1352604 for support. E.F. acknowledges support from DOE award No. DE-SC001236. P.A. acknowledges support from the EPiQS Initiative of the Gordon and Betty Moore Foundation, through Grant No. GBMF4542. NR 25 TC 0 Z9 0 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 24 PY 2016 VL 93 IS 19 AR 195150 DI 10.1103/PhysRevB.93.195150 PG 10 WC Physics, Condensed Matter SC Physics GA DM8TK UT WOS:000376637200002 ER PT J AU Ochi, M Arita, R Trivedi, N Okamoto, S AF Ochi, Masayuki Arita, Ryotaro Trivedi, Nandini Okamoto, Satoshi TI Strain-induced topological transition in SrRu2O6 and CaOs2O6 SO PHYSICAL REVIEW B LA English DT Article ID LOCALIZED WANNIER FUNCTIONS; AUGMENTED-WAVE METHOD; INSULATOR; SURFACE; OXIDES AB The topological property of SrRu2O6 and isostructural CaOs2O6 under various strain conditions is investigated using density functional theory. Based on an analysis of parity eigenvalues, we anticipate that a three-dimensional strong topological insulating state should be realized when band inversion is induced at the A point in the hexagonal Brillouin zone. For SrRu2O6, such a transition requires rather unrealistic tuning, where only the c axis is reduced while other structural parameters are unchanged. However, given the larger spin-orbit coupling and smaller lattice constants in CaOs2O6, the desired topological transition does occur under uniform compressive strain. Our study paves a way to realize a topological insulating state in a complex oxide, which has not been experimentally demonstrated so far. C1 [Ochi, Masayuki] Osaka Univ, Grad Sch Sci, Dept Phys, Osaka 5650043, Japan. [Ochi, Masayuki; Arita, Ryotaro] RIKEN, CEMS, Wako, Saitama 3510198, Japan. [Trivedi, Nandini] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Okamoto, Satoshi] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Okamoto, S (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM okapon@ornl.gov RI Okamoto, Satoshi/G-5390-2011; Ochi, Masayuki/B-1933-2015; Arita, Ryotaro/D-5965-2012 OI Okamoto, Satoshi/0000-0002-0493-7568; Arita, Ryotaro/0000-0001-5725-072X FU National Science Foundation [NSF PHY11-25915]; JSPS KAKENHI Grants [15K17724, 15H05883]; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; US Department of Energy [DE-AC05-00OR22725]; DOE Public Access Plan; [NSF-DMR1309461] FX This research was initiated at the Kavli Institute for Theoretical Physics (KITP), the University of California, Santa Barbara, where three of the authors (R.A., N.T., and S.O.) attended the program "New Phases and Emergent Phenomena in Correlated Materials with Strong Spin-Orbit Coupling." R.A., N.T., and S.O. thank the KITP, which is supported in part by the National Science Foundation under Grant No. NSF PHY11-25915, for hospitality. S.O. thanks V. R. Cooper for useful discussions. This work was supported by JSPS KAKENHI Grants No. 15K17724 (M.O.) and 15H05883 (R.A.). N.T. acknowledges funding from Grant No. NSF-DMR1309461. The research by S.O. is supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division.; Copyright notice: This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 49 TC 1 Z9 1 U1 6 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 24 PY 2016 VL 93 IS 19 AR 195149 DI 10.1103/PhysRevB.93.195149 PG 6 WC Physics, Condensed Matter SC Physics GA DM8TK UT WOS:000376637200001 ER PT J AU Potapkin, V Dubrovinsky, L Sergueev, I Ekholm, M Kantor, I Bessas, D Bykova, E Prakapenka, V Hermann, RP Ruffer, R Cerantola, V Jonsson, HJM Olovsson, W Mankovsky, S Ebert, H Abrikosov, IA AF Potapkin, V. Dubrovinsky, L. Sergueev, I. Ekholm, M. Kantor, I. Bessas, D. Bykova, E. Prakapenka, V. Hermann, R. P. Rueffer, R. Cerantola, V. Joensson, H. J. M. Olovsson, W. Mankovsky, S. Ebert, H. Abrikosov, I. A. TI Magnetic interactions in NiO at ultrahigh pressure SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METAL OXIDES; MOSSBAUER-SPECTROSCOPY; MOTT TRANSITION; COLLAPSE; MNO AB Magnetic properties of NiO have been studied in the multimegabar pressure range by nuclear forward scattering of synchrotron radiation using the 67.4 keV Mossbauer transition of Ni-61. The observed magnetic hyperfine splitting confirms the antiferromagnetic state of NiO up to 280 GPa, the highest pressure where magnetism has been observed so far, in any material. Remarkably, the hyperfine field increases from 8.47 T at ambient pressure to similar to 24 T at the highest pressure, ruling out the possibility of a magnetic collapse. A joint x-ray diffraction and extended x-ray-absorption fine structure investigation reveals that NiO remains in a distorted sodium chloride structure in the entire studied pressure range. Ab initio calculations support the experimental observations, and further indicate a complete absence of Mott transition in NiO up to at least 280 GPa. C1 [Potapkin, V.; Hermann, R. P.] Forschungszentrum Julich, JCNS, JARA FIT, D-52425 Julich, Germany. [Potapkin, V.; Hermann, R. P.] Forschungszentrum Julich, PGI, JARA FIT, D-52425 Julich, Germany. [Dubrovinsky, L.; Bykova, E.; Cerantola, V.] Univ Bayreuth, Bayer Geoinst, POB 101251, D-95440 Bayreuth, Germany. [Sergueev, I.] DESY, D-22607 Hamburg, Germany. [Ekholm, M.; Abrikosov, I. A.] Linkoping Univ, Swedish E Sci Res Ctr SeRC, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. [Kantor, I.; Bessas, D.; Rueffer, R.] European Synchrotron Radiat Facil, Boite Postale 220, F-38043 Grenoble, France. [Prakapenka, V.] Univ Chicago, CARS, Chicago, IL 60437 USA. [Hermann, R. P.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Joensson, H. J. M.; Olovsson, W.] Linkoping Univ, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. [Mankovsky, S.; Ebert, H.] Univ Munich, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany. [Abrikosov, I. A.] Natl Univ Sci & Technol MISIS, Mat Modeling & Dev Lab, Moscow 119049, Russia. [Abrikosov, I. A.] Tomsk State Univ, LACOMAS Lab, Tomsk 634050, Russia. RP Potapkin, V (reprint author), Forschungszentrum Julich, JCNS, JARA FIT, D-52425 Julich, Germany.; Potapkin, V (reprint author), Forschungszentrum Julich, PGI, JARA FIT, D-52425 Julich, Germany. EM potapkinv@gmail.com RI Hermann, Raphael/F-6257-2013; OI Hermann, Raphael/0000-0002-6138-5624; Olovsson, Weine/0000-0002-2904-0108 FU National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-GeoSciences [DE-FG02-94ER14466]; DOE Office of Science [DE-AC02-06CH11357]; Helmholtz Association; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; Swedish Government Strategic Research Area Grants Swedish e-Science Research Center (SeRC) and in Materials Science on Functional Materials at Linkoping University [2009 00971]; Knut and Alice Wallenbergs Foundation project Strong Field Physics and New States of Matter; Swedish Foundation for Strategic Research program SRL Grant [10-0026]; Swedish Research Council (VR) [2015-04391]; Grant of Ministry of Education and Science of the Russian Federation [14.Y26.31.0005]; Tomsk State University Academic D.I. Mendeleev Fund Program FX The European Synchrotron Radiation Facility is acknowledged for provision of synchrotron radiation beam time and the beamlines ID18 and ID09. The authors thank A. Chumakov and M. Hanfland for their help with ID18 and ID09 experiments, respectively. Portions of this work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (Grant No. EAR-1128799) and Department of Energy-GeoSciences (Grant No. DE-FG02-94ER14466). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. V.Pt. would like to acknowledge Helmholtz Association for support in the framework of the Helmholtz Postdoctoral Program. R.P.H. acknowledges support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. M.E., J.J., W.O., and I.A.A. acknowledge support from the Swedish Government Strategic Research Area Grants Swedish e-Science Research Center (SeRC) and in Materials Science on Functional Materials at Linkoping University (Faculty Grant SFO-Mat-LiU No 2009 00971), as well as from Knut and Alice Wallenbergs Foundation project Strong Field Physics and New States of Matter 2014-2019 (COTXS). I.A.A. is grateful for the support provided by the Swedish Foundation for Strategic Research program SRL Grant No. 10-0026: the Swedish Research Council (VR) Grant No 2015-04391, the Grant of Ministry of Education and Science of the Russian Federation (Grant No. 14.Y26.31.0005), and Tomsk State University Academic D.I. Mendeleev Fund Program. The simulations were carried out using supercomputer resources provided by the Swedish National Infrastructure for Computing (SNIC). NR 25 TC 0 Z9 0 U1 5 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 24 PY 2016 VL 93 IS 20 AR 201110 DI 10.1103/PhysRevB.93.201110 PG 5 WC Physics, Condensed Matter SC Physics GA DM8TW UT WOS:000376638400001 ER PT J AU Binosi, D Chang, L Papavassiliou, J Qin, SX Roberts, CD AF Binosi, Daniele Chang, Lei Papavassiliou, Joannis Qin, Si-Xue Roberts, Craig D. TI Symmetry preserving truncations of the gap and Bethe-Salpeter equations SO PHYSICAL REVIEW D LA English DT Article ID DYSON-SCHWINGER EQUATIONS; GREEN-TAKAHASHI IDENTITIES; LADDER APPROXIMATION; HADRON PHYSICS; RAINBOW-LADDER; MESONS; QCD; SPECTRUM; VERTEX; THEOREM AB Ward-Green-Takahashi (WGT) identities play a crucial role in hadron physics, e.g. imposing stringent relationships between the kernels of the one-and two-body problems, which must be preserved in any veracious treatment of mesons as bound states. In this connection, one may view the dressed gluon-quark vertex, Gamma(alpha)(mu), as fundamental. We use a novel representation of Gamma(alpha)(mu), in terms of the gluon-quark scattering matrix, to develop a method capable of elucidating the unique quark-antiquark Bethe-Salpeter kernel, K, that is symmetry consistent with a given quark gap equation. A strength of the scheme is its ability to expose and capitalize on graphic symmetries within the kernels. This is displayed in an analysis that reveals the origin of H-diagrams in K, which are two-particle-irreducible contributions, generated as two-loop diagrams involving the three-gluon vertex, that cannot be absorbed as a dressing of Gamma(alpha)(mu) in a Bethe-Salpeter kernel nor expressed as a member of the class of crossed-box diagrams. Thus, there are no general circumstances under which the WGT identities essential for a valid description of mesons can be preserved by a Bethe-Salpeter kernel obtained simply by dressing both gluon-quark vertices in a ladderlike truncation; and, moreover, adding any number of similarly dressed crossed-box diagrams cannot improve the situation. C1 [Binosi, Daniele] European Ctr Theoret Studies Nucl Phys & Related, Str Tabarelle 286, I-38123 Villazzano, TN, Italy. [Binosi, Daniele] Fdn Bruno Kessler Villa Tambosi, Str Tabarelle 286, I-38123 Villazzano, TN, Italy. [Chang, Lei] Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China. [Papavassiliou, Joannis] Univ Valencia, Dept Theoret Phys, E-46100 Valencia, Spain. [Papavassiliou, Joannis] Univ Valencia, IFIC, E-46100 Valencia, Spain. [Papavassiliou, Joannis] CSIC, E-46100 Valencia, Spain. [Qin, Si-Xue; Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Binosi, D (reprint author), European Ctr Theoret Studies Nucl Phys & Related, Str Tabarelle 286, I-38123 Villazzano, TN, Italy.; Binosi, D (reprint author), Fdn Bruno Kessler Villa Tambosi, Str Tabarelle 286, I-38123 Villazzano, TN, Italy. FU Spanish MEYC Grants [FPA2014-53631-C2-1-P, SEV-2014-0398]; Generalitat Valenciana [PrometeoII/2014/066]; Argonne National Laboratory Office of the Director; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX We are grateful for constructive remarks from A. Bashir, S. J. Brodsky, I. C. Cloet, B. El-Bennich, G. Krein, C. Mezrag, J. Rodriguez-Quintero, and J. Segovia. Research supported by: Spanish MEYC Grants No. FPA2014-53631-C2-1-P and No. SEV-2014-0398; Generalitat Valenciana under Grant No. PrometeoII/2014/066; Argonne National Laboratory Office of the Director, through the Named Postdoctoral Fellowship Program; and U.S. Department of Energy, Office of Science, Office of Nuclear Physics, Contract No. DE-AC02-06CH11357. NR 61 TC 8 Z9 8 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 24 PY 2016 VL 93 IS 9 AR 096010 DI 10.1103/PhysRevD.93.096010 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8UW UT WOS:000376641000007 ER PT J AU Herklotz, A Wong, AT Meyer, T Biegalski, MD Lee, HN Ward, TZ AF Herklotz, A. Wong, A. T. Meyer, T. Biegalski, M. D. Lee, H. N. Ward, T. Z. TI Controlling Octahedral Rotations in a Perovskite via Strain Doping SO SCIENTIFIC REPORTS LA English DT Article ID EPITAXIAL THIN-FILMS; SRRUO3; HETEROSTRUCTURES; TRANSITION; ANISOTROPY; ENERGY AB The perovskite unit cell is the fundamental building block of many functional materials. The manipulation of this crystal structure is known to be of central importance to controlling many technologically promising phenomena related to superconductivity, multiferroicity, mangetoresistivity, and photovoltaics. The broad range of properties that this structure can exhibit is in part due to the centrally coordinated octahedra bond flexibility, which allows for a multitude of distortions from the ideal highly symmetric structure. However, continuous and fine manipulation of these distortions has never been possible. Here, we show that controlled insertion of He atoms into an epitaxial perovskite film can be used to finely tune the lattice symmetry by modifying the local distortions, i.e., octahedral bonding angle and length. Orthorhombic SrRuO3 films coherently grown on SrTiO3 substrates are used as a model system. Implanted He atoms are confirmed to induce out-of-plane strain, which provides the ability to controllably shift the bulk-like orthorhombically distorted phase to a tetragonal structure by shifting the oxygen octahedra rotation pattern. These results demonstrate that He implantation offers an entirely new pathway to strain engineering of perovskite-based complex oxide thin films, useful for creating new functionalities or properties in perovskite materials. C1 [Herklotz, A.; Wong, A. T.; Meyer, T.; Lee, H. N.; Ward, T. Z.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Wong, A. T.] Univ Tennessee, Mat Sci & Engn, Knoxville, TN 37996 USA. [Biegalski, M. D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Ward, TZ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM wardtz@ornl.gov RI Ward, Thomas/I-6636-2016; Lee, Ho Nyung/K-2820-2012 OI Ward, Thomas/0000-0002-1027-9186; Lee, Ho Nyung/0000-0002-2180-3975 FU US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division. The temperature dependent XRD was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 35 TC 4 Z9 4 U1 14 U2 44 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 24 PY 2016 VL 6 AR 26491 DI 10.1038/srep26491 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM5AN UT WOS:000376358900002 PM 27215804 ER PT J AU Comes, RB Spurgeon, SR Heald, SM Kepaptsoglou, DM Jones, L Ong, PV Bowden, ME Ramasse, QM Sushko, PV Chambers, SA AF Comes, Ryan B. Spurgeon, Steven R. Heald, Steve M. Kepaptsoglou, Despoina M. Jones, Lewys Phuong Vu Ong Bowden, Mark E. Ramasse, Quentin M. Sushko, Peter V. Chambers, Scott A. TI Interface-Induced Polarization in SrTiO3-LaCrO3 Superlattices SO ADVANCED MATERIALS INTERFACES LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; AUGMENTED-WAVE METHOD; SRTIO3 THIN-FILMS; ELECTRON-GAS; OXIDE; HETEROSTRUCTURES; ENHANCEMENT; STRAIN; FERROELECTRICITY; DISORDER AB Epitaxial interfaces and superlattices comprised of polar and non-polar perovskite oxides have generated considerable interest because they possess a range of desirable properties for functional devices. In this work, emergent polarization in superlattices of SrTiO3 (STO) and LaCrO3 (LCO) is demonstrated. By controlling the interfaces between polar LCO and non-polar STO, polarization is induced throughout the STO layers of the superlattice. Using X-ray absorption near-edge spectroscopy and aberration-corrected scanning transmission electron microscopy displacements of the Ti cations off-center within TiO6 octahedra along the superlattice growth direction are measured. This distortion gives rise to built-in potential gradients within the STO and LCO layers, as measured by in situ X-ray photoelectron spectroscopy. Density functional theory models explain the mechanisms underlying this behavior, revealing the existence of both an intrinsic polar distortion and a built-in electric field, which are due to alternately positively and negatively charged interfaces in the superlattice. This study paves the way for controllable polarization for carrier separation in multilayer materials and highlights the crucial role that interface structure plays in governing such behavior. C1 [Comes, Ryan B.; Spurgeon, Steven R.; Phuong Vu Ong; Sushko, Peter V.; Chambers, Scott A.] Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Heald, Steve M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Kepaptsoglou, Despoina M.; Ramasse, Quentin M.] SuperSTEM, SciTech Daresbury Campus, Daresbury WA4 4AD, Cheshire, England. [Jones, Lewys] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [Bowden, Mark E.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Comes, RB; Chambers, SA (reprint author), Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. EM ryan.comes@pnnl.gov; sa.chambers@pnnl.gov RI Jones, Lewys/R-3501-2016; ONG, PHUONG VU/B-5651-2016; Sushko, Peter/F-5171-2013; OI Jones, Lewys/0000-0002-6907-0731; ONG, PHUONG VU/0000-0001-8613-1690; Sushko, Peter/0000-0001-7338-4146; Comes, Ryan/0000-0002-5304-6921 FU Linus Pauling Distinguished Post-doctoral Fellowship at Pacific Northwest National Laboratory [PNNL LDRD PN13100/2581]; U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Division of Materials Sciences and Engineering [10122]; LDRD Program at PNNL; DOE Office of Biological and Environmental Research; U.S. DOE BES; Canadian Light Source; University of Washington; APS; DOE [DE-AC02-06CH11357]; Engineering and Physical Sciences Research Council (EPSRC); European Union [312483] FX R.B.C. was supported by the Linus Pauling Distinguished Post-doctoral Fellowship at Pacific Northwest National Laboratory (PNNL LDRD PN13100/2581). S.R.S., M.E.B., and S.A.C. were supported by the U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Division of Materials Sciences and Engineering under Award No. 10122. P.V.S. and P.V.O. were supported by the LDRD Program at PNNL. PNNL work was performed in the Environmental Molecular Sciences Laboratory, a National Science User Facility sponsored by the DOE Office of Biological and Environmental Research. Sector 20 facilities at the Advanced Photon Source (APS), and research at these facilities, were supported by the U.S. DOE BES, the Canadian Light Source and its funding partners, the University of Washington, and the APS. Use of the APS, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, was supported by the DOE under Contract No. DE-AC02-06CH11357. Electron microscopy was carried out in parts at the SuperSTEM Laboratory, the U.K. National Facility for Aberration-Corrected STEM, which was supported by the Engineering and Physical Sciences Research Council (EPSRC). The research leading to these results received funding from the European Union Seventh Framework Programme under Grant Agreement No. 312483-ESTEEM2 (Integrated Infrastructure Initiative (I3)). NR 54 TC 5 Z9 5 U1 18 U2 34 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD MAY 23 PY 2016 VL 3 IS 10 AR 1500779 DI 10.1002/admi.201500779 PG 8 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR6ZZ UT WOS:000380051100005 ER PT J AU Yoo, CG Pu, YQ Li, M Ragauskas, AJ AF Yoo, Chang Geun Pu, Yunqiao Li, Mi Ragauskas, Arthur J. TI Elucidating Structural Characteristics of Biomass using Solution-State 2D NMR with a Mixture of Deuterated Dimethylsulfoxide and Hexamethylphosphoramide SO CHEMSUSCHEM LA English DT Article DE biomass; characterization; hexamethylphosphoramide; NMR spectroscopy; whole cell wall ID ORGANIC LIQUIDS; CELLULOSE; LIGNIN; WOOD; GRAIN; CORN AB Recent developments of NMR methods for characterization of lignocellulosic biomass allow improved understanding of plant cell-wall structures with minimal deconstruction and modification of biomass. This study introduces a new NMR solvent system composed of dimethylsulfoxide (DMSO-d(6)) and hexamethylphosphoramide (HMPA-d(18)). HMPA as a co-solvent enhanced swelling and mobility of the biomass samples; thereby it allowed enhancing signals of NMR spectra. The structural information of biomass was successfully analyzed by the proposed NMR solvent system (DMSO-d(6)/HMPA-d(18); 4:1, v/v) with different biomass. The proposed bi-solvent system does not require derivatization or isolation of biomass, facilitating a facile sample preparation and involving with no signals overlapping with biomass peaks. It also allows analyzing biomass with a room-temperature NMR probe instead of cryo-probes, which are traditionally used for enhancing signal intensities. C1 [Yoo, Chang Geun; Pu, Yunqiao; Li, Mi; Ragauskas, Arthur J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Yoo, Chang Geun; Pu, Yunqiao; Li, Mi; Ragauskas, Arthur J.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. [Yoo, Chang Geun; Pu, Yunqiao; Li, Mi; Ragauskas, Arthur J.] Oak Ridge Natl Lab, UT ORNL Joint Inst Biol Sci, Oak Ridge, TN 37831 USA. [Ragauskas, Arthur J.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Ragauskas, Arthur J.] Univ Tennessee, Dept Forestry Wildlife & Fisheries, Knoxville, TN 37996 USA. RP Ragauskas, AJ (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA.; Ragauskas, AJ (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA.; Ragauskas, AJ (reprint author), Oak Ridge Natl Lab, UT ORNL Joint Inst Biol Sci, Oak Ridge, TN 37831 USA.; Ragauskas, AJ (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA.; Ragauskas, AJ (reprint author), Univ Tennessee, Dept Forestry Wildlife & Fisheries, Knoxville, TN 37996 USA. EM aragauskas@utk.edu RI LI, Mi/Q-4261-2016; OI LI, Mi/0000-0001-7523-1266; Ragauskas, Arthur/0000-0002-3536-554X; Yoo, Chang Geun/0000-0002-6179-2414 FU U.S. Department of Energy [DE-AC05-00OR22725]; BioEnergy Science Center (BESC); Office of Biological and Environmental Research in the DOE Office of Science FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. This study was supported and performed as part of the BioEnergy Science Center (BESC). The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 35 TC 1 Z9 1 U1 6 U2 15 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD MAY 23 PY 2016 VL 9 IS 10 BP 1090 EP 1095 DI 10.1002/cssc.201600135 PG 6 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DP6UV UT WOS:000378635500006 PM 27116696 ER PT J AU Palo, M Eller, M Uin, J Tamm, E AF Palo, Maris Eller, Meelis Uin, Janek Tamm, Eduard TI Electric wind in a Differential Mobility Analyzer SO BOREAL ENVIRONMENT RESEARCH LA English DT Article ID SIZE RANGE; AEROSOLS; STANDARD; HISTORY AB Electric wind - the movement of gas, induced by ions moving in an electric field - can be a distorting factor in size distribution measurements using Differential Mobility Analyzers (DMAs). The aim of this study was to determine the conditions under which electric wind occurs in the locally-built VLDMA (Very Long Differential Mobility Analyzer) and TSI Long-DMA (3081) and to describe the associated distortion of the measured spectra. Electric wind proved to be promoted by the increase of electric field strength, aerosol layer thickness, particle number concentration and particle size. The measured size spectra revealed three types of distortion: widening of the size distribution, shift of the mode of the distribution to smaller diameters and smoothing out the peaks of the multiply charged particles. Electric wind may therefore be a source of severe distortion of the spectrum when measuring large particles at high concentrations. C1 [Palo, Maris; Eller, Meelis; Tamm, Eduard] Univ Tartu, Inst Phys, Lab Environm Phys, Ulikooli 18, EE-50090 Tartu, Estonia. [Uin, Janek] Brookhaven Natl Lab, Biol Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Palo, M (reprint author), Univ Tartu, Inst Phys, Lab Environm Phys, Ulikooli 18, EE-50090 Tartu, Estonia. FU Estonian Ministry of Education and Research [IUT20-11] FX This work was supported by institutional research funding IUT20-11 of the Estonian Ministry of Education and Research. NR 20 TC 0 Z9 0 U1 4 U2 4 PU FINNISH ENVIRONMENT INST PI HELSINKI PA P O BOX 140, FIN-00251 HELSINKI, FINLAND SN 1239-6095 EI 1797-2469 J9 BOREAL ENVIRON RES JI Boreal Environ. Res. PD MAY 23 PY 2016 VL 21 IS 3-4 BP 221 EP 229 PG 9 WC Environmental Sciences SC Environmental Sciences & Ecology GA DO8FY UT WOS:000378019700003 ER PT J AU Chen, X Tamura, N MacDowell, A James, RD AF Chen, Xian Tamura, Nobumichi MacDowell, Alastair James, Richard D. TI In-situ characterization of highly reversible phase transformation by synchrotron X-ray Laue microdiffraction SO APPLIED PHYSICS LETTERS LA English DT Article ID SHAPE-MEMORY ALLOYS; MARTENSITIC-TRANSFORMATION; HYSTERESIS; CRYSTALS; ENERGY AB The alloy Cu25Au30Zn45 undergoes a huge first-order phase transformation (6% strain) and shows a high reversibility under thermal cycling and an unusual martensitc microstructure in sharp contrast to its nearby compositions. This alloy was discovered by systematically tuning the composition so that its lattice parameters satisfy the cofactor conditions (i.e., the kinematic conditions of compatibility between phases). It was conjectured that satisfaction of these conditions is responsible for the enhanced reversibility as well as the observed unusual fluid-like microstructure during transformation, but so far, there has been no direct evidence confirming that these observed microstructures are those predicted by the cofactor conditions. To verify this hypothesis, we use synchrotron X-ray Laue microdiffraction to measure the orientations and structural parameters of variants and phases near the austenite/martensite interface. The areas consisting of both austenite and multivariants of martensite are scanned by microLaue diffraction. The cofactor conditions have been examined from the kinematic relation of lattice vectors across the interface. The continuity condition of the interface is precisely verified from the correspondent lattice vectors between two phases. Published by AIP Publishing. C1 [Chen, Xian] Hong Kong Univ Sci & Technol, Dept Mech & Aerosp Engn, Clear Water Bay, Hong Kong, Peoples R China. [Chen, Xian; Tamura, Nobumichi; MacDowell, Alastair] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [James, Richard D.] Univ Minnesota, Dept Aerosp Engn & Mech, Minneapolis, MN 55455 USA. RP Chen, X (reprint author), Hong Kong Univ Sci & Technol, Dept Mech & Aerosp Engn, Clear Water Bay, Hong Kong, Peoples R China.; Chen, X (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. OI Tamura, Nobumichi/0000-0002-3698-2611 FU MURI [FA9550-12-1-0458]; XC's Start-up Fund by UGC [B002-0172-R9358]; AFOSR [FA9550-15-1-0207]; ONR [N00014-14-0714]; NSF/PIRE [OISE-0967140]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX X.C. and R.D.J. acknowledge the financial support of MURI Project No. FA9550-12-1-0458 (administered by AFOSR). This research is also benefited from the support of XC's Start-up Fund B002-0172-R9358 (by UGC) and from the support of AFOSR (FA9550-15-1-0207), ONR (N00014-14-0714), and NSF/PIRE (OISE-0967140) to R.D.J. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The data analysis used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 24 TC 2 Z9 2 U1 6 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 23 PY 2016 VL 108 IS 21 AR 211902 DI 10.1063/1.4951001 PG 5 WC Physics, Applied SC Physics GA DN4HH UT WOS:000377024400015 ER PT J AU Kiraly, B Mannix, AJ Jacobberger, RM Fisher, BL Arnold, MS Hersam, MC Guisinger, NP AF Kiraly, Brian Mannix, Andrew J. Jacobberger, Robert M. Fisher, Brandon L. Arnold, Michael S. Hersam, Mark C. Guisinger, Nathan P. TI Sub-5 nm, globally aligned graphene nanoribbons on Ge(001) SO APPLIED PHYSICS LETTERS LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; ELECTRONIC-PROPERTIES; ROOM-TEMPERATURE; BAND-GAP; TRANSPORT; TRANSISTORS; GERMANIUM; SURFACE; GROWTH AB Graphene nanoribbons (GNRs) hold great promise for future electronics because of their edge and width dependent electronic bandgaps and exceptional transport properties. While significant progress toward GNR devices has been made, the field has been limited by difficulties achieving narrow widths, global alignment, and atomically pristine GNR edges on technologically relevant substrates. A recent advance has challenged these limits by using Ge(001) substrates to direct the bottom-up growth of GNRs with nearly pristine armchair edges and widths near similar to 10 nm via atmospheric pressure chemical vapor deposition. In this work, the growth of GNRs on Ge(001) is extended to ultra-high vacuum conditions, resulting in the realization of GNRs with widths narrower than 5 nm. Armchair graphene nanoribbons oriented along Ge < 110 > surface directions are achieved with excellent width control and relatively large bandgaps. The bandgap magnitude and electronic uniformity of these sub-5 nm GNRs are well-suited for emerging nanoelectronic applications. Published by AIP Publishing. C1 [Kiraly, Brian; Mannix, Andrew J.; Fisher, Brandon L.; Guisinger, Nathan P.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave,Bldg 440, Argonne, IL 60439 USA. [Kiraly, Brian; Mannix, Andrew J.; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. [Jacobberger, Robert M.; Arnold, Michael S.] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Hersam, Mark C.] Northwestern Univ, Dept Chem, 2220 Campus Dr, Evanston, IL 60208 USA. RP Guisinger, NP (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave,Bldg 440, Argonne, IL 60439 USA.; Hersam, MC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA.; Hersam, MC (reprint author), Northwestern Univ, Dept Chem, 2220 Campus Dr, Evanston, IL 60208 USA. EM m-hersam@northwestern.edu; nguisinger@anl.gov RI Hersam, Mark/B-6739-2009; Arnold, Michael/L-9112-2015 FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; U.S. Department of Energy SISGR [DE-FG02-09ER16109]; Office of Naval Research [N00014-14-1-0669]; National Science Foundation Graduate Fellowship [DGE-1324585, DGE-0824162]; Department of Energy (DOE) Office of Science Early Career Research Program through the Office of Basic Energy Sciences [DE-SC0006414]; Department of Defense (DOD) Air Force Office of Scientific Research through the National Defense Science and Engineering Graduate Fellowship [32 CFR 168a] FX This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. This work was supported by the U.S. Department of Energy SISGR Contract No. DE-FG02-09ER16109, the Office of Naval Research (Grant No. N00014-14-1-0669), and the National Science Foundation Graduate Fellowship (DGE-1324585 and DGE-0824162). R.M.J. and M.S.A. acknowledge support from the Department of Energy (DOE) Office of Science Early Career Research Program through the Office of Basic Energy Sciences (No. DE-SC0006414) for graphene synthesis, and R.M.J. also acknowledges support from the Department of Defense (DOD) Air Force Office of Scientific Research through the National Defense Science and Engineering Graduate Fellowship (No. 32 CFR 168a). NR 30 TC 1 Z9 1 U1 21 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. 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Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Muon reconstruction performance of the ATLAS detector in proton-proton collision data at root s=13 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article AB This article documents the performance of the ATLAS muon identification and reconstruction using the LHC dataset recorded at root s = 13 TeVin 2015. Using a large sample of J/.psi -> mu mu and Z -> mu mu decays from 3.2 fb(-1) of pp collision data, measurements of the reconstruction efficiency, as well as of the momentum scale and resolution, are presented and compared to Monte Carlo simulations. The reconstruction efficiency is measured to be close to 99 % over most of the covered phase space (vertical bar eta vertical bar < 2.5 and 5 < p(T) < 100 GeV). The isolation efficiency varies between 93 and 100 % depending on the selection applied and on the momentum of the muon. Both efficiencies are well reproduced in simulation. In the central region of the detector, the momentum resolution is measured to be 1.7 % (2.3 %) for muons from J/psi -> mu mu(Z -> mu mu) decays, and the momentum scale is known with an uncertainty of 0.05 %. In the region vertical bar eta vertical bar > 2.2, the p(T) resolution for muons from Z -> mu decays is 2.9 % while the precision of the momentum scale for low-p(T) muons from J/psi -> mu mu decays is about 0.2 %. C1 [ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. 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A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Marceca, G.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ruiz-Martinez, A.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Solans Sanchez, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Peng, C.; Ren, H.; Shana, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhao, Z.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] PKU CHEP, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darboa, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Aloisio, A.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; de Lima, D. E. Ferreira; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Aloisio, A.; Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Ticse Torres, R. E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Ticse Torres, R. E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Vazquez Schroeder, T.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Brochu, F. M.; Dawe, E.; Jennens, D.; Kubota, T.; Le, B.; McDonald, E. F.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Citterio, M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Villaplana Perez, M.] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Camplani, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Ducu, O. A.; Gagnon, L. 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[Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Koehler, N. M.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef, Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Fac Sci, Columbus, OH 43210 USA. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. 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L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Scarcella, M.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Britzger, D.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Thomson, E.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, NRC KI, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anullia, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Nisatia, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Safai Tehrani, F.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Facini, G.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ghazlane, H.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ghazlane, H.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, IRFU, DSM, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; Sales De Bruin, P. H.; Torro Pastor, E.; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Dado, T.; Melo, M.; Plazak, L.; Sykora, I.; Tokara, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohma, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Ughetto, M.; Valdes Santurio, E.; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Ughetto, M.; Valdes Santurio, E.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Morley, A. K.; Saavedra, A. F.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Hod, N.; Jovicevic, J.; Codina, E. Perez; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualaha, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Cobal, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Giordani, M. P.; Pinamonti, M.; Soualaha, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Cheplakov, A.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. 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RI Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Gladilin, Leonid/B-5226-2011; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Lazzaroni, Massimo/N-3675-2015; Warburton, Andreas/N-8028-2013; Ippolito, Valerio/L-1435-2016; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015 OI Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Gladilin, Leonid/0000-0001-9422-8636; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Lazzaroni, Massimo/0000-0002-4094-1273; Warburton, Andreas/0000-0002-2298-7315; Ippolito, Valerio/0000-0001-5126-1620; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario InnovationTrust, Canada; EPLANET; ERC; Horizon; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF; GIF; Minerva, Israel; BRF, Norway; Generalitat de Catalunya; Generalitat Valenciana, Spain; Royal Society; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario InnovationTrust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 28 TC 0 Z9 0 U1 14 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 23 PY 2016 VL 76 IS 5 AR 292 DI 10.1140/epjc/s10052-016-4120-y PG 30 WC Physics, Particles & Fields SC Physics GA DM9IP UT WOS:000376679200003 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaitia, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedraa, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghia, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costaa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM 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Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the transverse momentum and phi(eta)*. distributions of Drell-Yan lepton pairs in proton-proton collisions at root s=8 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CROSS-SECTION; RESONANCE REGION; MONTE-CARLO; BOSON; DECAY AB Distributions of transverse momentum p(T)(ll) and the related angular variable phi(eta)*. of Drell-Yan lepton pairs are measured in 20.3 fb(-1) of proton-proton collisions at root s = 8 TeV with the ATLAS detector at the LHC. Measurements in electron-pair and muon-pair final states are corrected for detector effects and combined. Compared to previous measurements in proton-proton collisions at root s = 7 TeV, these new measurements benefit from a larger data sample and improved control of systematic uncertainties. Measurements are performed in bins of lepton-pair mass above, around and below the Z-boson mass peak. The data are compared to predictions from perturbative and resummed QCD calculations. For values of phi(eta)*. < 1 the predictions from the Monte Carlo generator ResBos are generally consistent with the data within the theoretical uncertainties. However, at larger values of phi(eta)*. this is not the case. Monte Carlo generators based on the parton-shower approach are unable to describe the data over the full range of p(T)(ll) while the fixed-order prediction of Dynnlo falls below the data at high values of p(T)(ll). 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Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Bruckman de Renstrom, P. A.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Garay Walls, F. M.; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; Bilbao De Mendizabal, J.; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nackenhorst, O.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darboa, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Ferreira de Lima, D. E.; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dunford, M.; Geisler, M. P.; Hankea, P.; Jongmanns, J.; Klugea, E-E.; Langa, V. S.; Meier, K.; Meyer Zu Theenhausen, H.; Narrias Villar, D. I.; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretzc, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Flores Castillo, L. R.; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Lorenzo Martinez, N.; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Gutierrez Ortiz, N. G.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Phys Theor & Hautes Energies Lab, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Caudron, J.; Cuth, J.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Kaluza, A.; Meyer, C.; Sander, H. G.; Schmitt, C.; Simioni, E.; Valderanis, C.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Iturbe Ponce, J. M.; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Munoz Sanchez, F. J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. 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[Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Vazquez Schroeder, T.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; McKee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Villaplana Perez, M.] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. 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S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karakostas, K.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. 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J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. 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M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedraa, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedraa, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Czech Tech Univ, Fac Math & Phys, CR-16635 Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, NRC KI, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. 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[Aielli, G.; Bai, Y.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaouid, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaouid, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Mourslie, R.; Fassie, F.; Haddade, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Dano Hoffmann, M.; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Goncalves Pinto Firmino Da Costa, J.; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lanon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; Sales De Bruin, P. H.; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Cuhadar Donszelmann, T.; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Vickey Boeriu, O. E.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Canale, V.; Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamiltona, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Mellado Garciac, B. R.; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaitia, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia Bylund, O.; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaitia, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bessidskaia Bylund, O.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Perez Codina, E.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Benitez Garcia, J. A.; Manjarres Ramos, J.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Caminal Armadans, R.; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Bergeaas Kuutmann, E.; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, CNM, IMB, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Macek, B.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Banerjee, Sw] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Chen, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Conventi, F.; Corriveau, F.; Della Pietra, M.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Toronto, ON, Canada. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytechn Univ, Dept Phys, St Petersburg, Russia. [Geng, C.; Guo, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Taipei, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Li, B.; Song, H. Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS, IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Livan, Michele/D-7531-2012; Ippolito, Valerio/L-1435-2016; Carvalho, Joao/M-4060-2013; Gladilin, Leonid/B-5226-2011; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015 OI Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694; Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Livan, Michele/0000-0002-5877-0062; Ippolito, Valerio/0000-0001-5126-1620; Carvalho, Joao/0000-0002-3015-7821; Gladilin, Leonid/0000-0001-9422-8636; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario InnovationTrust, Canada; EPLANET; ERC; FP7; Horizon 2020; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF; GIF; Minerva; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario InnovationTrust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 68 TC 4 Z9 4 U1 17 U2 49 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 23 PY 2016 VL 76 IS 5 AR 291 DI 10.1140/epjc/s10052-016-4070-4 PG 61 WC Physics, Particles & Fields SC Physics GA DM9IP UT WOS:000376679200002 ER PT J AU van Dam, HJJ AF van Dam, Hubertus J. J. TI Generalization of the Kohn-Sham system that can represent arbitrary one-electron density matrices SO PHYSICAL REVIEW A LA English DT Article ID MOLECULAR-ORBITAL METHODS; BASIS-SETS AB Density functional theory is currently the most widely applied method in electronic structure theory. The Kohn-Sham method, based on a fictitious system of noninteracting particles, is the workhorse of the theory. The particular form of the Kohn-Sham wave function admits only idempotent one-electron density matrices whereas wave functions of correlated electrons in post-Hartree-Fock methods invariably have fractional occupation numbers. Here we show that by generalizing the orbital concept and introducing a suitable dot product as well as a probability density, a noninteracting system can be chosen that can represent the one-electron density matrix of any system, even one with fractional occupation numbers. This fictitious system ensures that the exact electron density is accessible within density functional theory. It can also serve as the basis for reduced density matrix functional theory. Moreover, to aid the analysis of the results the orbitals may be assigned energies from a mean-field Hamiltonian. This produces energy levels that are akin to Hartree-Fock orbital energies such that conventional analyses based on Koopmans' theorem are available. Finally, this system is convenient in formalisms that depend on creation and annihilation operators as they are trivially applied to single-determinant wave functions. C1 [van Dam, Hubertus J. J.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP van Dam, HJJ (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. FU U.S. Department of Energy [DESC0012704]; Office of Biological and Environmental Research FX This manuscript has been authored by employees of Brookhaven Science Associates, LLC under Contract No. DESC0012704 with the U.S. Department of Energy. A portion of the research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 13 TC 0 Z9 0 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 23 PY 2016 VL 93 IS 5 AR 052512 DI 10.1103/PhysRevA.93.052512 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DM8RL UT WOS:000376631500004 ER PT J AU Di Stefano, D Nazarov, R Hickel, T Neugebauer, J Mrovec, M Elsasser, C AF Di Stefano, Davide Nazarov, Roman Hickel, Tilmann Neugebauer, Joerg Mrovec, Matous Elsaesser, Christian TI First-principles investigation of hydrogen interaction with TiC precipitates in alpha-Fe SO PHYSICAL REVIEW B LA English DT Article ID HIGH-STRENGTH STEELS; THERMAL-DESORPTION SPECTROSCOPY; TOTAL-ENERGY CALCULATIONS; LATH MARTENSITIC STEEL; WAVE BASIS-SET; 1ST PRINCIPLES; MECHANICAL-PROPERTIES; QUANTITATIVE-ANALYSIS; FERRITIC STEEL; IRON AB A correct description of hydrogen diffusion and trapping is the prerequisite for an understanding of the phenomenon of hydrogen embrittlement. In this study, we carried out extensive first-principles calculations based on density functional theory to investigate the interaction of H with TiC precipitates that are assumed to be efficient trapping agents mitigating HE in advanced high-strength steels. We found that there exists a large variety of possible trapping sites for H associated with different types of interfaces between the TiC particle and the Fe matrix, with misfit dislocations and other defects at these interfaces, and with carbon vacancies in TiC. The most efficient trapping by more than 1 eV occurs at carbon vacancies in the interior of TiC particles. However, these traps are difficult to populate at ambient temperatures since the energy barrier for H entering the particles is high. H trapping at the semicoherent interfaces between the TiC particles and the Fe matrix is moderate, ranging from 0.3 to 0.5 eV. However, a sufficiently large concentration of the carbide particles can significantly reduce the amount of H segregated at dislocation cores in the Fe matrix. A systematic comparison of the obtained theoretical results with available experimental observations reveals a consistent picture of hydrogen trapping at the TiC particles that is expected to be qualitatively valid also for other carbide precipitates with the rock-salt crystal structure. C1 [Di Stefano, Davide; Mrovec, Matous; Elsaesser, Christian] Fraunhofer Inst Werkstoffmech IWM, Wohlerstr 11, D-79108 Freiburg, Germany. [Nazarov, Roman; Hickel, Tilmann; Neugebauer, Joerg] Max Planck Inst Eisenforsch GmbH, D-40237 Dusseldorf, Germany. [Nazarov, Roman] Lawrence Livermore Natl Lab, Livermore, CA USA. [Mrovec, Matous] Karlsruher Inst Technol, IAM, Engelbert Arnold Str 4, D-76131 Karlsruhe, Germany. [Elsaesser, Christian] Univ Freiburg, FMF, Stefan Meier Str 21, D-79104 Freiburg, Germany. RP Di Stefano, D; Mrovec, M (reprint author), Fraunhofer Inst Werkstoffmech IWM, Wohlerstr 11, D-79108 Freiburg, Germany. EM distefanodav@gmail.com; matous.mrovec@iwm.fraunhofer.de RI Mrovec, Matous/C-1315-2009 OI Mrovec, Matous/0000-0001-8216-2254 FU European Union [263335, RFCS-CT-2010-00020]; Helmholtz Portfolio Project Energy Materials EMR; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the European Union under the Seventh Framework Programme, grant number 263335, MultiHy (Multiscale Modeling of Hydrogen Embrittlement), and under the Research Fund for Coal and Steel (RFCS) within the project HYDRAMICROS (RFCS-CT-2010-00020). MM was partly supported by the Helmholtz Portfolio Project Energy Materials EMR. The work of RN has been performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 74 TC 0 Z9 0 U1 13 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 18 AR 184108 DI 10.1103/PhysRevB.93.184108 PG 14 WC Physics, Condensed Matter SC Physics GA DM8SX UT WOS:000376635900003 ER PT J AU Ghimire, NJ Cary, SK Eley, S Wakeham, NA Rosa, PFS Albrecht-Schmitt, T Lee, Y Janoschek, M Brown, CM Civale, L Thompson, JD Ronning, F Bauer, ED AF Ghimire, N. J. Cary, S. K. Eley, S. Wakeham, N. A. Rosa, P. F. S. Albrecht-Schmitt, T. Lee, Y. Janoschek, M. Brown, C. M. Civale, L. Thompson, J. D. Ronning, F. Bauer, E. D. TI Physical properties of the Ce2MAl7Ge4 heavy-fermion compounds (M = Co, Ir, Ni, Pd) SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM PHASE-TRANSITIONS; METALS; SUPERCONDUCTIVITY; MAGNETISM AB We report the synthesis, crystal structure, and characterization by means of single-crystal x-ray diffraction, neutron powder diffraction, and magnetic, thermal, and transport measurements of the new heavy-fermion compounds Ce2MAl7Ge4 (M = Co, Ir, Ni, Pd). These compounds crystallize in a noncentrosymmetric tetragonal space group P (4) over bar2(1)m, consisting of layers of square nets of Ce atoms separated by Ge-Al and M-Al-Ge blocks. Ce2CoAl7Ge4, Ce2IrAl7Ge4, and Ce2NiAl7Ge4 order magnetically below T-M = 1.8, 1.6, and 0.8 K, respectively. There is no evidence of magnetic ordering in Ce2PdAl7Ge4 down to 0.4 K. The small amount of entropy released in the magnetic state of Ce2MAl7Ge4 (M = Co, Ir, Ni) and the reduced specific heat jump at TM suggest a strong Kondo interaction in these materials. Ce2PdAl7Ge4 shows non-Fermi liquid behavior, possibly due to the presence of a nearby quantum critical point. C1 [Ghimire, N. J.; Eley, S.; Wakeham, N. A.; Rosa, P. F. S.; Janoschek, M.; Civale, L.; Thompson, J. D.; Ronning, F.; Bauer, E. D.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Cary, S. K.; Albrecht-Schmitt, T.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Lee, Y.] POSTECH Pohang, Dept Phys, Inst Basic Sci, Ctr Artificial Low Dimens Elect Syst, Pohang 790784, South Korea. [Brown, C. M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20878 USA. RP Ghimire, NJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM nghimire@lanl.gov RI Brown, Craig/B-5430-2009; OI Brown, Craig/0000-0002-9637-9355; Ronning, Filip/0000-0002-2679-7957; Janoschek, Marc/0000-0002-2943-0173; Civale, Leonardo/0000-0003-0806-3113; Bauer, Eric/0000-0003-0017-1937; Ferrari Silveira Rosa, Priscila/0000-0002-3437-548X; Eley, Serena/0000-0002-2928-5316 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC52-06NA25396]; Los Alamos LDRD program; Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, Heavy Elements Chemistry Program, U.S. Department of Energy [DE-FG02-13ER16414]; Institute of Basic Sciences (IBS) [IBS-R014-D1]; National Institute of Standards and Technology, U.S. Department of Commerce FX We thank Z. Fisk, J. Lawrence, and A. Mar for stimulating discussion. Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The EDS measurements were performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. P.F.S.R. acknowledges a Director's Postdoctoral Fellowship supported through the Los Alamos LDRD program. Support for T.E.A.S. and S.K.C. was provided by the Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, Heavy Elements Chemistry Program, U.S. Department of Energy, under Grant No. DE-FG02-13ER16414. Y.L. was supported by the Institute of Basic Sciences (IBS), Grant No. IBS-R014-D1. We acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the neutron research facilities used in this work. NR 32 TC 0 Z9 0 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 20 AR 205141 DI 10.1103/PhysRevB.93.205141 PG 10 WC Physics, Condensed Matter SC Physics GA DM8TU UT WOS:000376638200005 ER PT J AU Hmiel, A Winey, JM Gupta, YM Desjarlais, MP AF Hmiel, A. Winey, J. M. Gupta, Y. M. Desjarlais, M. P. TI Nonlinear elastic response of strong solids: First-principles calculations of the third-order elastic constants of diamond SO PHYSICAL REVIEW B LA English DT Article ID AB-INITIO AB Accurate theoretical calculations of the nonlinear elastic response of strong solids (e.g., diamond) constitute a fundamental and important scientific need for understanding the response of such materials and for exploring the potential synthesis and design of novel solids. However, without corresponding experimental data, it is difficult to select between predictions from different theoretical methods. Recently the complete set of third-order elastic constants (TOECs) for diamond was determined experimentally, and the validity of various theoretical approaches to calculate the same may now be assessed. We report on the use of density functional theory (DFT) methods to calculate the six third-order elastic constants of diamond. Two different approaches based on homogeneous deformations were used: (1) an energy-strain fitting approach using a prescribed set of deformations, and (2) a longitudinal stress-strain fitting approach using uniaxial compressive strains along the [100], [110], and [111] directions, together with calculated pressure derivatives of the second-order elastic constants. The latter approach provides a direct comparison to the experimental results. The TOECs calculated using the energy-strain approach differ significantly from the measured TOECs. In contrast, calculations using the longitudinal stress-uniaxial strain approach show good agreement with the measured TOECs and match the experimental values significantly better than the TOECs reported in previous theoretical studies. Our results on diamond have demonstrated that, with proper analysis procedures, first-principles calculations can indeed be used to accurately calculate the TOECs of strong solids. C1 [Hmiel, A.; Winey, J. M.; Gupta, Y. M.] Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. [Hmiel, A.; Winey, J. M.; Gupta, Y. M.] Washington State Univ, Dept Phys, Pullman, WA 99164 USA. [Desjarlais, M. P.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Hmiel, A (reprint author), Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA.; Hmiel, A (reprint author), Washington State Univ, Dept Phys, Pullman, WA 99164 USA. OI Hmiel, Abraham/0000-0002-8390-7470 FU Department of Energy/NNSA [DE-NA0002007]; Washington State University FX This work was supported by the Department of Energy/NNSA through the Cooperative Agreement No. DE-NA0002007 with Washington State University. NR 29 TC 0 Z9 0 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 17 AR 174113 DI 10.1103/PhysRevB.93.174113 PG 7 WC Physics, Condensed Matter SC Physics GA DM8SM UT WOS:000376634800001 ER PT J AU Jiang, S Liu, L Schutt, M Hallas, AM Shen, B Tian, W Emmanouilidou, E Shi, AS Luke, GM Uemura, YJ Fernandes, RM Ni, N AF Jiang, Shan Liu, Lian Schutt, Michael Hallas, Alannah M. Shen, Bing Tian, Wei Emmanouilidou, Eve Shi, Aoshuang Luke, Graeme M. Uemura, Yasutomo J. Fernandes, Rafael M. Ni, Ni TI Effect of interlayer coupling on the coexistence of antiferromagnetism and superconductivity in Fe pnictide superconductors: A study of Ca0.74(1)La0.26(1)(Fe1-xCox)As-2 single crystals SO PHYSICAL REVIEW B LA English DT Article ID ORDER AB We report the transport, thermodynamic, muon spin relaxation, and neutron study of the Ca0.74(1)La0.26(1)(Fe1-xCox)As-2 single crystals, mapping out the temperature-doping level phase diagram. Upon Co substitution on the Fe site, the structural and magnetic phase transitions in this 112 compound are suppressed and superconductivity up to 20 K occurs. Our measurements of the superconducting and magnetic volume fractions show that these two phases coexist microscopically in the underdoped region, in contrast to the related Ca-10(Pt3As8)((Fe1-xPtx)(2)As-2)(5) (10-3-8) compound, where coexistence is absent. Supported by model calculations, we discuss the differences in the phase diagrams of the 112 and 10-3-8 compounds in terms of the FeAs interlayer coupling, whose strength is affected by the character of the spacer layer, which is metallic in the 112 compound and insulating in the 10-3-8 compound. C1 [Jiang, Shan; Shen, Bing; Emmanouilidou, Eve; Shi, Aoshuang; Ni, Ni] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Jiang, Shan; Shen, Bing; Emmanouilidou, Eve; Shi, Aoshuang; Ni, Ni] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA. [Liu, Lian; Uemura, Yasutomo J.] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Schutt, Michael; Fernandes, Rafael M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Hallas, Alannah M.; Luke, Graeme M.] McMaster Univ, Dept Phys, Hamilton, ON L8S 4M1, Canada. [Hallas, Alannah M.; Luke, Graeme M.] Canadian Inst Adv Res, 180 Dundas St W, Toronto, ON M5G 1Z7, Canada. [Tian, Wei] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Ni, N (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA.; Ni, N (reprint author), Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA. EM nini@physics.ucla.edu RI Schuett, Michael/J-6870-2015; Luke, Graeme/A-9094-2010; Fernandes, Rafael/E-9273-2010; Tian, Wei/C-8604-2013 OI Schuett, Michael/0000-0002-3114-1119; Tian, Wei/0000-0001-7735-3187 FU NSF DMREF [DMR-1435672, DMR-1436095]; Scientific User Facilities Division, BES, DOE; PIRE [IIA 0968226, DMR-1105961]; JAEA REIMEI; Humboldt Foundation; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012336]; Natural Sciences and Engineering Research Council of Canada; Vanier Canada Graduate Scholarship program FX Work at UCLA was supported by the NSF DMREF Grant No. DMR-1435672. Work at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, BES, DOE. Work at Columbia and TRIUMF was supported by the NSF DMREF Grant No. DMR-1436095, PIRE Project No. IIA 0968226, Grant No. DMR-1105961, and JAEA REIMEI. M.S. acknowledges the support from the Humboldt Foundation. R.M.F. is supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0012336. Work at McMaster was supported by the Natural Sciences and Engineering Research Council of Canada. A.M.H. acknowledges support from the Vanier Canada Graduate Scholarship program. N.N. thanks useful discussion with G. Kotliar. NR 37 TC 2 Z9 2 U1 11 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 17 AR 174513 DI 10.1103/PhysRevB.93.174513 PG 5 WC Physics, Condensed Matter SC Physics GA DM8SM UT WOS:000376634800008 ER PT J AU Kedem, Y Zhu, JX Balatsky, AV AF Kedem, Yaron Zhu, Jian-Xin Balatsky, Alexander V. TI Unusual superconducting isotope effect in the presence of a quantum criticality SO PHYSICAL REVIEW B LA English DT Article ID TEMPERATURE SUPERCONDUCTOR; TRANSITION-TEMPERATURE; MECHANISM AB The isotope effect in superconductivity (SC) is used to make a concrete connection to a quantum critical point (QCP) that is tunable by isotopic mass substitution. We find a distinct contribution to the isotope exponent in SC and derive an explicit relation to the critical exponent of a QCP. The relation between the two exponents is general and can be used as an experimental signature for the connection between SC and a QCP. We demonstrate it in a scenario where the SC pairing is due to modes related to a structural instability. Within this model the isotope exponent is derived in terms of microscopic parameters. C1 [Kedem, Yaron; Balatsky, Alexander V.] KTH Royal Inst Technol, Ctr Quantum Mat, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Kedem, Yaron; Balatsky, Alexander V.] Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, POB 1663, Los Alamos, NM 87545 USA. RP Kedem, Y (reprint author), KTH Royal Inst Technol, Ctr Quantum Mat, NORDITA, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Kedem, Y (reprint author), Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. FU U.S. DOE [BES E304]; ERC [DM 321031] FX We are grateful to C. Triola, S. Pershoguba, J. Edge, U. Aschauer, and N. A. Spaldin. This work was supported by U.S. DOE BES E304. The work of Y.K. was supported by ERC DM 321031 and VR. Y.K. acknowledges the hospitality of LANL. NR 27 TC 1 Z9 1 U1 3 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 18 AR 184507 DI 10.1103/PhysRevB.93.184507 PG 4 WC Physics, Condensed Matter SC Physics GA DM8SX UT WOS:000376635900006 ER PT J AU Pribram-Jones, A Burke, K AF Pribram-Jones, A. Burke, K. TI Connection formulas for thermal density functional theory SO PHYSICAL REVIEW B LA English DT Article ID ADIABATIC CONNECTION; CORRELATION ENERGIES; ELECTRON-GAS; EXCHANGE; MOLECULES; SYSTEMS; PLASMAS; SURFACE; FORCES; VIRIAL AB The adiabatic connection formula of ground-state density functional theory relates the correlation energy to a coupling-constant integral over a purely potential contribution, and is widely used to understand and improve approximations. The corresponding formula for thermal density functional theory is cast as an integral over temperatures instead, ranging upward from the system's physical temperature. We also show how to relate different correlation components to each other, either in terms of temperature or coupling-constant integrations. We illustrate our results on the uniform electron gas. C1 [Pribram-Jones, A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pribram-Jones, A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Burke, K.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. RP Pribram-Jones, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.; Pribram-Jones, A (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM pribramjones1@llnl.gov FU NSF [CHE-1464795]; DOE [DE-FG02-97ER25308]; University of California President's Postdoctoral Fellowship; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX K.B. thanks NSF Grant No. CHE-1464795, and A.P.J. thanks DOE Grant No. DE-FG02-97ER25308 and the University of California President's Postdoctoral Fellowship. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 30 TC 1 Z9 1 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 23 PY 2016 VL 93 IS 20 AR 205140 DI 10.1103/PhysRevB.93.205140 PG 5 WC Physics, Condensed Matter SC Physics GA DM8TU UT WOS:000376638200004 ER PT J AU Mitchell, JT Perepelitsa, DV Tannenbaum, MJ Stankus, PW AF Mitchell, J. T. Perepelitsa, D. V. Tannenbaum, M. J. Stankus, P. W. TI Tests of constituent-quark generation methods which maintain both the nucleon center of mass and the desired radial distribution in Monte Carlo Glauber models SO PHYSICAL REVIEW C LA English DT Article ID HIGH-ENERGIES; CENTRALITY DEPENDENCE; COLLISIONS; MULTIPLICITY; QCD AB Several methods of generating three constituent quarks in a nucleon are evaluated which explicitly maintain the nucleon's center of mass and desired radial distribution and can be used within Monte Carlo Glauber frameworks. The geometric models provided by each method are used to generate distributions over the number of constituent quark participants (N-qp) in p + p, d + Au, and Au + Au collisions. The results are compared with each other and to a previous result of N-qp calculations, without this explicit constraint, used in measurements of root s(NN) = 200 GeV p + p, d + Au, and Au + Au collisions at the BNL Relativistic Heavy Ion Collider. C1 [Mitchell, J. T.; Perepelitsa, D. V.; Tannenbaum, M. J.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Stankus, P. W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Mitchell, JT (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. FU US Department of Energy [DE-SC0012704, DE-AC05-00OR22725] FX BNL research is supported by US Department of Energy, Contract No. DE-SC0012704. ORNL research is supported by US Department of Energy, Contract No. DE-AC05-00OR22725. NR 30 TC 4 Z9 4 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 23 PY 2016 VL 93 IS 5 AR 054910 DI 10.1103/PhysRevC.93.054910 PG 14 WC Physics, Nuclear SC Physics GA DM8UJ UT WOS:000376639700006 ER PT J AU Schmittfull, M Vlah, Z McDonald, P AF Schmittfull, Marcel Vlah, Zvonimir McDonald, Patrick TI Fast large scale structure perturbation theory using one-dimensional fast Fourier transforms SO PHYSICAL REVIEW D LA English DT Article ID MICROWAVE BACKGROUND ANISOTROPIES; GRAVITATIONAL-INSTABILITY; LOOP CORRECTIONS; POWER SPECTRUM; MODES AB The usual fluid equations describing the large-scale evolution of mass density in the universe can be written as local in the density, velocity divergence, and velocity potential fields. As a result, the perturbative expansion in small density fluctuations, usually written in terms of convolutions in Fourier space, can be written as a series of products of these fields evaluated at the same location in configuration space. Based on this, we establish a new method to numerically evaluate the 1-loop power spectrum (i.e., Fourier transform of the 2-point correlation function) with one-dimensional fast Fourier transforms. This is exact and a few orders of magnitude faster than previously used numerical approaches. Numerical results of the new method are in excellent agreement with the standard quadrature integration method. This fast model evaluation can in principle be extended to higher loop order where existing codes become painfully slow. Our approach follows by writing higher order corrections to the 2-point correlation function as, e.g., the correlation between two second-order fields or the correlation between a linear and a third-order field. These are then decomposed into products of correlations of linear fields and derivatives of linear fields. The method can also be viewed as evaluating three-dimensional Fourier space convolutions using products in configuration space, which may also be useful in other contexts where similar integrals appear. C1 [Schmittfull, Marcel] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Schmittfull, Marcel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Vlah, Zvonimir] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94306 USA. [Vlah, Zvonimir] Stanford Univ, Dept Phys, Stanford, CA 94306 USA. [Vlah, Zvonimir] SLAC, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Vlah, Zvonimir] Stanford Univ, Menlo Pk, CA 94025 USA. [McDonald, Patrick] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Schmittfull, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA.; Schmittfull, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. OI McDonald, Patrick/0000-0001-8346-8394 FU U.S. Department of Energy [DE-AC02-76SF00515] FX We thank Uros Seljak and Martin White for useful discussions. Z. V. is supported in part by the U.S. Department of Energy contract to SLAC No. DE-AC02-76SF00515. NR 34 TC 5 Z9 5 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 23 PY 2016 VL 93 IS 10 AR 103528 DI 10.1103/PhysRevD.93.103528 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM8VR UT WOS:000376643100006 ER PT J AU Jesse, S Chi, M Belianinov, A Beekman, C Kalinin, SV Borisevich, AY Lupini, AR AF Jesse, S. Chi, M. Belianinov, A. Beekman, C. Kalinin, S. V. Borisevich, A. Y. Lupini, A. R. TI Big Data Analytics for Scanning Transmission Electron Microscopy Ptychography SO SCIENTIFIC REPORTS LA English DT Article ID Z-CONTRAST; OCTAHEDRAL TILTS; COMPLEX OXIDE; BIFEO3 FILMS; POLARIZATION; INTERFACES; RESOLUTION; GROWTH; IMAGES; SERIES AB Electron microscopy is undergoing a transition; from the model of producing only a few micrographs, through the current state where many images and spectra can be digitally recorded, to a new mode where very large volumes of data (movies, ptychographic and multi-dimensional series) can be rapidly obtained. Here, we discuss the application of so-called "big-data" methods to high dimensional microscopy data, using unsupervised multivariate statistical techniques, in order to explore salient image features in a specific example of BiFeO3 domains. Remarkably, k-means clustering reveals domain differentiation despite the fact that the algorithm is purely statistical in nature and does not require any prior information regarding the material, any coexisting phases, or any differentiating structures. While this is a somewhat trivial case, this example signifies the extraction of useful physical and structural information without any prior bias regarding the sample or the instrumental modality. Further interpretation of these types of results may still require human intervention. However, the open nature of this algorithm and its wide availability, enable broad collaborations and exploratory work necessary to enable efficient data analysis in electron microscopy. C1 [Jesse, S.; Chi, M.; Belianinov, A.; Kalinin, S. V.; Borisevich, A. Y.; Lupini, A. R.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Jesse, S.; Chi, M.; Belianinov, A.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Beekman, C.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Beekman, C.] Natl High Magnet Field Lab, 1800 E Paul Dirac Dr, Tallahassee, FL 32310 USA. [Borisevich, A. Y.; Lupini, A. R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Jesse, S (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA.; Jesse, S (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM sjesse@ornl.gov RI Chi, Miaofang/Q-2489-2015 OI Chi, Miaofang/0000-0003-0764-1567 FU Oak Ridge National Laboratory's Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Division of Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. DOE FX Research supported by Oak Ridge National Laboratory's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (M.C., S.V.K.), and by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy (S.J., A.Be.), and by Division of Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. DOE (A.R.L., A.Bo.). NR 51 TC 4 Z9 4 U1 8 U2 25 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 23 PY 2016 VL 6 AR 26348 DI 10.1038/srep26348 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM3IM UT WOS:000376240100001 PM 27211523 ER PT J AU Zhang, WW Oganov, AR Zhu, Q Lobanov, SS Stavrou, E Goncharov, AF AF Zhang, Weiwei Oganov, Artem R. Zhu, Qiang Lobanov, Sergey S. Stavrou, Elissaios Goncharov, Alexander F. TI Stability of numerous novel potassium chlorides at high pressure SO SCIENTIFIC REPORTS LA English DT Article ID CRYSTAL-STRUCTURE PREDICTION; INDUCED PHASE-TRANSFORMATION; STATE; TRANSITION; EQUATIONS; HALIDES; LITHIUM; NACL; KCL AB K-Cl is a simple system displaying all four main types of bonding, as it contains (i) metallic potassium, (ii) elemental chlorine made of covalently bonded Cl-2 molecules held together by van der Waals forces, and (iii) an archetypal ionic compound KCl. The charge balance rule, assigning classical charges of "+1" to K and "-1" to Cl, predicts that no compounds other than KCl are possible. However, our quantum-mechanical variable-composition evolutionary simulations predict an extremely complex phase diagram, with new thermodynamically stable compounds K3Cl, K2Cl, K3Cl2, K4Cl3, K5Cl4, K3Cl5, KCl3 and KCl7. Of particular interest are 2D-metallic homologs Kn+1Cln, the presence of positively charged Cl atoms in KCl7, and the predicted stability of KCl3 already at nearly ambient pressures at zero Kelvin. We have synthesized cubic Pm (3) over barn -KCl3 at 40-70 GPa and trigonal P (3) over bar c1 -KCl3 at 20-40 GPa in a laser-heated diamond anvil cell (DAC) at temperature exceeding 2000 K from KCl and Cl-2. These phases were identified using in situ synchrotron X-ray diffraction and Raman spectroscopy. Upon unloading to 10 GPa, P (3) over bar c1 -KCl3 transforms to a yet unknown structure before final decomposition to KCl and Cl-2 at near-ambient conditions. C1 [Zhang, Weiwei] China Agr Univ, Dept Appl Phys, Beijing 100080, Peoples R China. [Zhang, Weiwei; Oganov, Artem R.; Zhu, Qiang] SUNY Stony Brook, Dept Geosci, Ctr Mat Design, Stony Brook, NY 11794 USA. [Zhang, Weiwei; Oganov, Artem R.; Zhu, Qiang] SUNY Stony Brook, Inst Adv Computat Sci, Stony Brook, NY 11794 USA. [Oganov, Artem R.] Skolkovo Innovat Ctr, Skolkovo Inst Sci & Technol, 3 Nobel St, Moscow 143026, Russia. [Oganov, Artem R.] Moscow Inst Phys & Technol, 9 Inst Skiy Lane, Dolgoprudnyi 141700, Moscow Region, Russia. [Oganov, Artem R.] Northwestern Polytech Univ, Xian 710072, Peoples R China. [Lobanov, Sergey S.; Stavrou, Elissaios; Goncharov, Alexander F.] Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd, Washington, DC 20015 USA. [Lobanov, Sergey S.] SB RAS, VS Sobolev Inst Geol & Mineral, 3 Pr Ac Koptyga, Novosibirsk 630090, Russia. [Stavrou, Elissaios] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, POB 808 L-350, Livermore, CA 94550 USA. [Goncharov, Alexander F.] Chinese Acad Sci, Key Lab Mat Phys, Inst Solid State Phys, Hefei 230031, Peoples R China. [Goncharov, Alexander F.] Univ Sci & Technol China, Hefei 230026, Peoples R China. RP Zhang, WW (reprint author), China Agr Univ, Dept Appl Phys, Beijing 100080, Peoples R China.; Zhang, WW; Oganov, AR (reprint author), SUNY Stony Brook, Dept Geosci, Ctr Mat Design, Stony Brook, NY 11794 USA.; Zhang, WW; Oganov, AR (reprint author), SUNY Stony Brook, Inst Adv Computat Sci, Stony Brook, NY 11794 USA.; Oganov, AR (reprint author), Skolkovo Innovat Ctr, Skolkovo Inst Sci & Technol, 3 Nobel St, Moscow 143026, Russia.; Oganov, AR (reprint author), Moscow Inst Phys & Technol, 9 Inst Skiy Lane, Dolgoprudnyi 141700, Moscow Region, Russia.; Oganov, AR (reprint author), Northwestern Polytech Univ, Xian 710072, Peoples R China. EM zwwjennifer@gmail.com; artem.oganov@stonybrook.edu RI Lobanov, Sergey/D-9405-2017; OI Lobanov, Sergey/0000-0001-9728-2363; Oganov, Artem R./0000-0001-7082-9728 FU NSFC [11474355, 21403297, 61474142, 21473211]; Chinese Universities Scientific Fund [2015LX002]; DaBeiNong Young Scholars Research Plan, the Government of Russian Federation [14.A12.31.0003]; Foreign Talents Introduction and Academic Exchange Program [B08040]; Army Research Office; NSF-EAR; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-Geosciences [DE-FG02-94ER14466]; European Community's Seventh Framework Programme (FP7) [312284]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Ministry of Education and Science of Russian Federation [14. B25.31.0032]; U.S. Department of Energy [DE-AC52-07NA27344] FX We thank X. Dong, V. Prakapenka and Z. Konopkova for technical support and discussions. This work is funded by NSFC (Nos 11474355, 21403297, 61474142), Chinese Universities Scientific Fund (No. 2015LX002), DaBeiNong Young Scholars Research Plan, the Government of Russian Federation (No. 14.A12.31.0003) and Foreign Talents Introduction and Academic Exchange Program (No. B08040). A.F.G. acknowledges support from the Army Research Office and NSF-EAR. X-ray diffraction experiments were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory and Petra III, DESY, Hamburg, Germany. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-Geosciences (DE-FG02-94ER14466). The research leading to these results has received funding from NSFC (No. 21473211) and the European Community's Seventh Framework Programme (FP7/2007-2013) under grant agreement No. 312284. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. PETRA III at DESY is a member of the Helmholtz Association (HGF). S.S.L. was partly supported by the Ministry of Education and Science of Russian Federation (No. 14. B25.31.0032). Work of E.S. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Security, LLC under Contract DE-AC52-07NA27344. NR 28 TC 2 Z9 2 U1 9 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 23 PY 2016 VL 6 AR 26265 DI 10.1038/srep26265 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM3GC UT WOS:000376233800001 PM 27211847 ER PT J AU Pacold, JI Lukens, WW Booth, CH Shuh, DK Knight, KB Eppich, GR Holliday, KS AF Pacold, J. I. Lukens, W. W. Booth, C. H. Shuh, D. K. Knight, K. B. Eppich, G. R. Holliday, K. S. TI Chemical speciation of U, Fe, and Pu in melt glass from nuclear weapons testing SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ABSORPTION FINE-STRUCTURE; NEAR-EDGE STRUCTURE; NEVADA TEST-SITE; IRON OXIDATION-STATES; STRUCTURE SPECTROSCOPY; SILICATE GLASS; STRUCTURAL ENVIRONMENTS; BOROSILICATE GLASSES; URANIUM SPECIATION; LOCAL-STRUCTURE AB Nuclear weapons testing generates large volumes of glassy materials that influence the transport of dispersed actinides in the environment and may carry information on the composition of the detonated device. We determine the oxidation state of U and Fe (which is known to buffer the oxidation state of actinide elements and to affect the redox state of groundwater) in samples of melt glass collected from three U.S. nuclear weapons tests. For selected samples, we also determine the coordination geometry of U and Fe, and we report the oxidation state of Pu from one melt glass sample. We find significant variations among the melt glass samples and, in particular, find a clear deviation in one sample from the expected buffering effect of Fe(II)/Fe(III) on the oxidation state of uranium. In the first direct measurement of Pu oxidation state in a nuclear test melt glass, we obtain a result consistent with existing literature that proposes Pu is primarily present as Pu(IV) in post-detonation material. In addition, our measurements imply that highly mobile U(VI) may be produced in significant quantities when melt glass is quenched rapidly following a nuclear detonation, though these products may remain immobile in the vitrified matrices. The observed differences in chemical state among the three samples show that redox conditions can vary dramatically across different nuclear test conditions. The local soil composition, associated device materials, and the rate of quenching are all likely to affect the final redox state of the glass. The resulting variations in glass chemistry are significant for understanding and interpreting debris chemistry and the later environmental mobility of dispersed material. Published by AIP Publishing. C1 [Pacold, J. I.; Lukens, W. W.; Booth, C. H.; Shuh, D. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Knight, K. B.; Eppich, G. R.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94550 USA. [Holliday, K. S.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. RP Pacold, JI (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. FU Office of Defense Nuclear Nonproliferation Research and Development within the U.S. Department of Energy's National Nuclear Security Administration [DE-AC02-05CH11231, DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX We thank Pat Allen and Tim Rose for useful insights and discussion. This work was funded by the Office of Defense Nuclear Nonproliferation Research and Development within the U.S. Department of Energy's National Nuclear Security Administration, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory and under Contract No. DE-AC52-07NA27344 at Lawrence Livermore National Laboratory. Use of SSRL, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. NR 81 TC 0 Z9 0 U1 16 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 21 PY 2016 VL 119 IS 19 AR 195102 DI 10.1063/1.4948942 PG 11 WC Physics, Applied SC Physics GA DO3YH UT WOS:000377718100030 ER PT J AU Hale, LM Zimmerman, JA Wong, BM AF Hale, Lucas M. Zimmerman, Jonathan A. Wong, Bryan M. TI Large-scale atomistic simulations of helium-3 bubble growth in complex palladium alloys SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID EMBEDDED-ATOM METHOD; MOLECULAR-DYNAMICS; TRITIUM STORAGE; PD NANOPARTICLES; HELIUM RELEASE; HYDROGEN; THERMODYNAMICS; ABSORPTION; STABILITY; PRESSURE AB Palladium is an attractive material for hydrogen and hydrogen-isotope storage applications due to its properties of large storage density and high diffusion of lattice hydrogen. When considering tritium storage, the material's structural and mechanical integrity is threatened by both the embrittlement effect of hydrogen and the creation and evolution of additional crystal defects (e.g., dislocations, stacking faults) caused by the formation and growth of helium-3 bubbles. Using recently developed inter-atomic potentials for the palladium-silver-hydrogen system, we perform large-scale atomistic simulations to examine the defect-mediated mechanisms that govern helium bubble growth. Our simulations show the evolution of a distribution of material defects, and we compare the material behavior displayed with expectations from experiment and theory. We also present density functional theory calculations to characterize ideal tensile and shear strengths for these materials, which enable the understanding of how and why our developed potentials either meet or confound these expectations. Published by AIP Publishing. C1 [Hale, Lucas M.] NIST, Gaithersburg, MD 20899 USA. [Zimmerman, Jonathan A.] Sandia Natl Labs, Livermore, CA 94550 USA. [Wong, Bryan M.] Univ Calif Riverside, Riverside, CA 92521 USA. RP Hale, LM (reprint author), NIST, Gaithersburg, MD 20899 USA. EM lucas.hale@nist.gov; jzimmer@sandia.gov; bryan.wong@ucr.edu RI Wong, Bryan/B-1663-2009 OI Wong, Bryan/0000-0002-3477-8043 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Robert Kolasinski for providing data on the equation of state for He at room temperature. In addition, the authors appreciate the following individuals for their helpful discussions and guidance: Xiaowang Zhou, Michael Foster, Wilhelm Wolfer, Donald Cowgill, and Steven Rice. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 47 TC 1 Z9 1 U1 7 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2016 VL 144 IS 19 AR 194705 DI 10.1063/1.4948789 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WH UT WOS:000377712600037 PM 27208963 ER PT J AU Lam, RK Smith, JW Saykally, RJ AF Lam, Royce K. Smith, Jacob W. Saykally, Richard J. TI Communication: Hydrogen bonding interactions in water-alcohol mixtures from X-ray absorption spectroscopy SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; METHANOL MIXTURES; AQUEOUS-SOLUTION; LIQUID METHANOL; THERMODYNAMIC PROPERTIES; WATER/METHANOL MIXTURES; DIELECTRIC-PROPERTIES; HYDRATION STRUCTURE; BINARY-SOLUTIONS; FREE-ENERGY AB While methanol and ethanol are macroscopically miscible with water, their mixtures exhibit negative excess entropies of mixing. Despite considerable effort in both experiment and theory, there remains significant disagreement regarding the origin of this effect. Different models for the liquid mixture structure have been proposed to address this behavior, including the enhancement of the water hydrogen bonding network around the alcohol hydrophobic groups and microscopic immiscibility or clustering. We have investigated mixtures of methanol, ethanol, and isopropanol with water by liquid microjet X-ray absorption spectroscopy on the oxygen K-edge, an atom-specific probe providing details of both inter-and intra-molecular structure. The measured spectra evidence a significant enhancement of hydrogen bonding originating from the methanol and ethanol hydroxyl groups upon the addition of water. These additional hydrogen bonding interactions would strengthen the liquid-liquid interactions, resulting in additional ordering in the liquid structures and leading to a reduction in entropy and a negative enthalpy of mixing, consistent with existing thermodynamic data. In contrast, the spectra of the isopropanol-water mixtures exhibit an increase in the number of broken alcohol hydrogen bonds for mixtures containing up to 0.5 water mole fraction, an observation consistent with existing enthalpy of mixing data, suggesting that the measured negative excess entropy is a result of clustering or micro-immiscibility. Published by AIP Publishing. C1 [Saykally, Richard J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Saykally, RJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM saykally@berkeley.edu OI SAYKALLY, RICHARD/0000-0001-8942-3656; Lam, Royce/0000-0003-2878-038X FU Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) through the Chemical Sciences Division of the Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 through the Chemical Sciences Division of the Lawrence Berkeley National Laboratory (LBNL). The authors thank Craig P. Schwartz, Janel S. Uejio, Alice H. England, and Andrew M. Duffin for assistance with taking the data and Wanli Yang and Jon Spear for beamline support at the Advanced Light Source. The data presented are available upon request to saykally@berkeley.edu. NR 53 TC 2 Z9 2 U1 13 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2016 VL 144 IS 19 AR 191103 DI 10.1063/1.4951010 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WH UT WOS:000377712600003 PM 27208929 ER PT J AU Witte, J Neaton, JB Head-Gordon, M AF Witte, Jonathon Neaton, Jeffrey B. Head-Gordon, Martin TI Push it to the limit: Characterizing the convergence of common sequences of basis sets for intermolecular interactions as described by density functional theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CONSISTENT BASIS-SETS; MOLECULAR-ORBITAL METHODS; GAUSSIAN-BASIS SETS; GENERALIZED GRADIENT APPROXIMATION; DIFFUSE BASIS FUNCTIONS; POLARIZATION-CONSISTENT; SUPERPOSITION ERROR; NONCOVALENT INTERACTIONS; COUNTERPOISE CORRECTION; WAVE-FUNCTIONS AB With the aim of systematically characterizing the convergence of common families of basis sets such that general recommendations for basis sets can be made, we have tested a wide variety of basis sets against complete-basis binding energies across the S22 set of intermolecular interactions-noncovalent interactions of small and medium-sized molecules consisting of first-and second-row atoms-with three distinct density functional approximations: SPW92, a form of local-density approximation; B3LYP, a global hybrid generalized gradient approximation; and B97M-V, a meta-generalized gradient approximation with nonlocal correlation. We have found that it is remarkably difficult to reach the basis set limit; for the methods and systems examined, the most complete basis is Jensen's pc-4. The Dunning correlation-consistent sequence of basis sets converges slowly relative to the Jensen sequence. The Karlsruhe basis sets are quite cost effective, particularly when a correction for basis set superposition error is applied: counterpoise-corrected def2-SVPD binding energies are better than corresponding energies computed in comparably sized Dunning and Jensen bases, and on par with uncorrected results in basis sets 3-4 times larger. These trends are exhibited regardless of the level of density functional approximation employed. A sense of the magnitude of the intrinsic incompleteness error of each basis set not only provides a foundation for guiding basis set choice in future studies but also facilitates quantitative comparison of existing studies on similar types of systems. Published by AIP Publishing. C1 [Witte, Jonathon; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Witte, Jonathon; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy Nanosci Inst Berkeley, Berkeley, CA 94720 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Head-Gordon, M (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Head-Gordon, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-FG02-12ER16362]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-05CH11231] FX This research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences under Award No. DE-FG02-12ER16362. Work at the Molecular Foundry was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-05CH11231. NR 88 TC 3 Z9 3 U1 7 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 21 PY 2016 VL 144 IS 19 AR 194306 DI 10.1063/1.4949536 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WH UT WOS:000377712600022 PM 27208948 ER PT J AU Bittner, DM Stephens, SL Zaleski, DP Tew, DP Walker, NR Legon, AC AF Bittner, Dror M. Stephens, Susanna L. Zaleski, Daniel P. Tew, David P. Walker, Nicholas R. Legon, Anthony C. TI Gas phase complexes of H3N center dot center dot center dot CuF and H3N center dot center dot center dot CuI studied by rotational spectroscopy and ab initio calculations: the effect of X (X = F, Cl, Br, I) in OC center dot center dot center dot CuX and H3N center dot center dot center dot CuX SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID DEPENDENCE MOLECULAR-STRUCTURES; AUXILIARY BASIS-SETS; HYPERFINE CONSTANTS; MICROWAVE-SPECTRA; RI-CC2 CALCULATIONS; PULSED-JET; GEOMETRIES; PSEUDOPOTENTIALS; CHEMISTRY; CHARACTER AB Complexes of H3N center dot center dot center dot CuF and H3N center dot center dot center dot CuI have been synthesised in the gas phase and characterized by microwave spectroscopy. The rotational spectra of 4 isotopologues of H3N center dot center dot center dot CuF and 5 isotopologues of H3N center dot center dot center dot CuI have been measured in the 6.5-18.5 GHz frequency range using a chirped-pulse Fourier transform microwave spectrometer. Each complex is generated from a gas sample containing NH3 and a halogen-containing precursor diluted in Ar. Copper is introduced by laser ablation of a solid target prior to supersonic expansion of the sample into the vacuum chamber of the microwave spectrometer. The spectrum of each complex is characteristic of a symmetric rotor and a C-3v geometry in which the N, Cu and X atoms (where X is F or I) lie on the C-3(a) axis. The rotational constant (B-0), centrifugal distortion constants (D-J and D-JK), nuclear spin-rotation (C-bb(Cu) = C-cc(Cu)) constant (for H3N center dot center dot center dot CuF only) and nuclear quadrupole coupling constants (chi(aa)(X) where (X = N, Cu, I)) are fitted to the observed transition frequencies. Structural parameters are determined from the measured rotational constants and also calculated ab initio at the CCSD(T)(F12*)/AVQZ level of theory. Force constants describing the interaction between ammonia and each metal halide are determined from D-J for each complex. Trends in the interaction strengths and geometries of B center dot center dot center dot CuX (B = NH3, CO) (X = F, Cl, Br, I) are discussed. C1 [Bittner, Dror M.; Stephens, Susanna L.; Zaleski, Daniel P.; Walker, Nicholas R.] Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Tew, David P.; Legon, Anthony C.] Univ Bristol, Sch Chem, Bristol BS8 1TS, Avon, England. [Stephens, Susanna L.] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada. [Zaleski, Daniel P.] Argonne Natl Lab, Chem Sci & Engn, 9700 S Cass Ave,Bldg 200, Lemont, IL 60439 USA. RP Walker, NR (reprint author), Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England.; Legon, AC (reprint author), Univ Bristol, Sch Chem, Bristol BS8 1TS, Avon, England. EM nick.walker@newcastle.ac.uk; a.c.legon@bristol.ac.uk RI Walker, Nicholas /E-6180-2011; Tew, David/E-1458-2011 OI Walker, Nicholas /0000-0002-9450-305X; Tew, David/0000-0002-3220-4177 FU EPSRC; School of Chemistry at Newcastle University; European Research Council [CPFTMW-307000]; Newcastle University; University of Bristol; Royal Society FX The authors thank the EPSRC and the School of Chemistry at Newcastle University for the award of a DTA postgraduate studentship to D. M. B., the European Research Council for the postdoctoral fellowships awarded to S. L. S. and D. P. Z., and for project funding (Grant No. CPFTMW-307000). D. P. Z. also thanks Newcastle University for a SAgE Research Fellowship. A. C. L. thanks the University of Bristol for a Senior Research Fellowship and Newcastle University for a Visiting Professor award. D. P. T. is pleased to acknowledge the Royal Society for the award of a University Research Fellowship. We are also grateful to the EPSRC UK National Service for Computational Chemistry Software (NSCCS) at Imperial College London. NR 64 TC 1 Z9 1 U1 2 U2 4 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAY 21 PY 2016 VL 18 IS 19 BP 13638 EP 13645 DI 10.1039/c6cp01368f PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DM1WQ UT WOS:000376138000054 PM 27139221 ER PT J AU Prentice, SJ Mazzali, PA Pian, E Gal-Yam, A Kulkarni, SR Rubin, A Corsi, A Fremling, C Sollerman, J Yaron, O Arcavi, I Zheng, W Kasliwal, MM Filippenko, AV Cenko, SB Cao, Y Nugent, PE AF Prentice, S. J. Mazzali, P. A. Pian, E. Gal-Yam, A. Kulkarni, S. R. Rubin, A. Corsi, A. Fremling, C. Sollerman, J. Yaron, O. Arcavi, I. Zheng, W. Kasliwal, M. M. Filippenko, A. V. Cenko, S. B. Cao, Y. Nugent, P. E. TI The bolometric light curves and physical parameters of stripped-envelope supernovae SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE supernovae: general ID GAMMA-RAY BURST; CORE-COLLAPSE SUPERNOVAE; 25 APRIL 1998; IIB SUPERNOVA; IC SUPERNOVA; IB/C SUPERNOVAE; X-RAY; SUPERGIANT PROGENITOR; COMPACT PROGENITOR; OPTICAL PHOTOMETRY AB The optical and optical/near-infrared pseudo-bolometric light curves of 85 stripped-envelope supernovae (SNe) are constructed using a consistent method and a standard cosmology. The light curves are analysed to derive temporal characteristics and peak luminosity L-p, enabling the construction of a luminosity function. Subsequently, the mass of Ni-56 synthesized in the explosion, along with the ratio of ejecta mass to ejecta kinetic energy, are found. Analysis shows that host-galaxy extinction is an important factor in accurately determining luminosity values as it is significantly greater than Galactic extinction in most cases. It is found that broad-lined SNe Ic (SNe Ic-BL) and gamma-ray burst SNe are the most luminous subtypes with a combined median L-p, in erg s(-1), of log(L-p)= 43.00 compared to 42.51 for SNe Ic, 42.50 for SNe Ib, and 42.36 for SNe IIb. It is also found that SNe Ic-BL synthesize approximately twice the amount of 56Ni compared with SNe Ic, Ib, and IIb, with median M-Ni = 0.34, 0.16, 0.14, and 0.11 M-circle dot, respectively. SNe Ic-BL, and to a lesser extent SNe Ic, typically rise from L-p/2 to L-p more quickly than SNe Ib/IIb; consequently, their light curves are not as broad. C1 [Prentice, S. J.; Mazzali, P. A.] Liverpool John Moores Univ, IC2, Astrophys Res Inst, Liverpool Sci Pk,146 Brownlow Hill, Liverpool L3 5RF, Merseyside, England. [Mazzali, P. A.] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85748 Garching, Germany. [Pian, E.] Inst Space Astrophys & Cosm Phys, Via P Gobetti 101, I-40129 Bologna, Italy. [Pian, E.] Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, Italy. [Gal-Yam, A.; Rubin, A.; Yaron, O.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Kulkarni, S. R.; Kasliwal, M. M.; Cao, Y.] CALTECH, Div Phys Math & Astron, 1200 E Calif Blvd, Pasadena, CA 91125 USA. [Corsi, A.] Texas Tech Univ, Dept Phys, Box 41051, Lubbock, TX 79409 USA. [Fremling, C.; Sollerman, J.] Univ Stockholm, Oskar Klein Ctr, Dept Astron, S-10691 Stockholm, Sweden. [Arcavi, I.] Las Cumbres Observ Global Telescope Network, 6740 Cortona Dr,Suite 102, Goleta, CA 93111 USA. [Arcavi, I.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Zheng, W.; Filippenko, A. V.; Nugent, P. E.] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Kasliwal, M. M.] Carnegie Inst Sci, The Observ, 813 Santa Barbara St, Pasadena, CA 91101 USA. [Cenko, S. B.] NASA, Astrophys Sci Div, Goddard Space Flight Ctr, Mail Code 661, Greenbelt, MD 20771 USA. [Nugent, P. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Prentice, SJ (reprint author), Liverpool John Moores Univ, IC2, Astrophys Res Inst, Liverpool Sci Pk,146 Brownlow Hill, Liverpool L3 5RF, Merseyside, England. EM S.J.Prentice@2014.ljmu.ac.uk OI Sollerman, Jesper/0000-0003-1546-6615 FU Office of Science of the US Department of Energy [DE-AC02-05CH11231]; NSF [AST-1211916]; TABASGO Foundation; Christopher R. Redlich Fund; EU/FP7 via ERC [307260]; "The Quantum Universe" I-Core program by the Israeli Committee for planning and budgeting; ISF; Minerva; Weizmann-UK "making connections" program; Kimmel award; YeS award FX This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. AVF's research was funded by NSF grant AST-1211916, the TABASGO Foundation, and the Christopher R. Redlich Fund. A.G.Y. is supported by the EU/FP7 via ERC grant no. 307260, "The Quantum Universe" I-Core program by the Israeli Committee for planning and budgeting and the ISF; by Minerva and ISF grants; by the Weizmann-UK "making connections" program; and by Kimmel and YeS awards. NR 102 TC 4 Z9 4 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAY 21 PY 2016 VL 458 IS 3 BP 2973 EP 3002 DI 10.1093/mnras/stw299 PG 30 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DL7DC UT WOS:000375799000052 ER PT J AU Halavanau, A Piot, P AF Halavanau, A. Piot, P. TI Simulation of a cascaded longitudinal space charge amplifier for coherent radiation generation SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Linear accelerator; Electron beams; Space charge; Micro-bunching instabilities; N-body tree algorithm ID ALGORITHM; CODE AB Longitudinal space charge (LSC) effects are generally considered as harmful in free-electron lasers as they can seed unfavorable energy modulations that can result in density modulations with associated emittance dilution. This "micro-bunching instabilities" is naturally broadband and could possibly support the generation of coherent radiation over a broad region of the spectrum. Therefore there has been an increasing interest in devising accelerator beam lines capable of controlling LSC induced density modulations. In the present paper we refine these previous investigations by combining a grid-less space charge algorithm with the popular particle-tracking program ELEGANT. This high-fidelity model of the space charge is used to benchmark conventional LSC models. We finally employ the developed model to investigate the performance of a cascaded LSC amplifier using beam parameters comparable to the ones achievable at Fermilab Accelerator Science & Technology (FAST) facility currently under commissioning at Fermilab. (C) 2016 Elsevier B.V. All rights reserved. C1 [Halavanau, A.; Piot, P.] No Illinois Univ, Ctr Accelerator & Detector Dev, Dept Phys & Northern Illinois, De Kalb, IL 60115 USA. [Halavanau, A.; Piot, P.] Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, POB 500, Batavia, IL 60510 USA. RP Halavanau, A (reprint author), No Illinois Univ, Ctr Accelerator & Detector Dev, Dept Phys & Northern Illinois, De Kalb, IL 60115 USA.; Halavanau, A (reprint author), Fermilab Natl Accelerator Lab, Accelerator Phys Ctr, POB 500, Batavia, IL 60510 USA. EM aliaksei.halavanau@gmail.com FU US Department of Energy (DOE) [DE-SC0011831]; Northern Illinois University; US DOE [DE-AC02-07CH11359] FX We are grateful to Dr. J. Barnes (U. Hawaii) for granting us the use of his open-source version of the BH algorithm and to Dr. M. Borland (ANL) for his help with ELEGANT. We thank Dr. J. Wu (SLAC) for discussing some of the results presented in his paper [25], and Dr. R. Li OLab) and Dr. V. Litvinenko (BNL) for their interests and comments on our work. This work was supported by the US Department of Energy (DOE) under contract DE-SC0011831 with Northern Illinois University. Fermilab is operated by the Fermi Research Alliance LLC under US DOE contract DE-AC02-07CH11359. NR 37 TC 0 Z9 0 U1 3 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 21 PY 2016 VL 819 BP 144 EP 153 DI 10.1016/j.nima.2016.03.002 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DG8FQ UT WOS:000372318800019 ER PT J AU Granstrom, CR Fridman, I Lei, HC Petrovic, C Wei, JYT AF Granstrom, C. R. Fridman, I. Lei, H. -C. Petrovic, C. Wei, J. Y. T. TI Point-contact Andreev reflection spectroscopy on Bi2Se3 single crystals SO INTERNATIONAL JOURNAL OF MODERN PHYSICS B LA English DT Article; Proceedings Paper CT International Conference on Electron Correlation in Nanostructures (ECN) CY SEP 03-06, 2015 CL Odessa, UKRAINE DE Andreev reflection; topological insulator; superconductor ID TOPOLOGICAL INSULATORS; SPIN POLARIZATION; SUPERCONDUCTORS; TRANSITION; SURFACE AB To study how Andreev reflection (AR) occurs between a superconductor and a threedimensional topological insulator (TI), we use superconducting Nb tips to perform point-contact AR spectroscopy at 4.2 K on as-grown single crystals of Bi2Se3. Scanning tunneling spectroscopy and scanning tunneling microscopy are also used to characterize the superconducting tip and both the doping level and surface condition of the TI sample. The point-contact measurements show clear spectral signatures of AR, as well as a depression of zero-bias conductance with decreasing junction impedance. The latter observation can be attributed to interfacial Rashba spin-orbit coupling, and the presence of bulk bands at the Fermi level in our samples suggests that bulk states of Bi2Se3 are involved in the observed AR. C1 [Granstrom, C. R.; Fridman, I.; Wei, J. Y. T.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Lei, H. -C.; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Wei, J. Y. T.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. RP Wei, JYT (reprint author), Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada.; Wei, JYT (reprint author), Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. EM wei@physics.utoronto.ca NR 32 TC 2 Z9 2 U1 8 U2 19 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-9792 EI 1793-6578 J9 INT J MOD PHYS B JI Int. J. Mod. Phys. B PD MAY 20 PY 2016 VL 30 IS 13 SI SI AR 1642002 DI 10.1142/S0217979216420029 PG 7 WC Physics, Applied; Physics, Condensed Matter; Physics, Mathematical SC Physics GA DP5LZ UT WOS:000378540300003 ER PT J AU Adrian-Martinez, S Albert, A Andre, M Anton, G Ardid, M Aubert, JJ Baret, B Barrios-Marti, J Basa, S Bertin, V Biagi, S Bormuth, R Bouwhuis, MC Bruijn, R Brunner, J Busto, J Capone, A Caramete, L Carr, J Chiarusi, T Circella, M Coniglione, R Costantini, H Coyle, P Creusot, A Dekeyser, I Deschamps, A De Bonis, G Distefano, C Donzaud, C Dornic, D Drouhin, D Dumas, A Eberl, T Elsasser, D Enzenhofer, A Fehn, K Felis, I Fermani, P Folger, F Fusco, LA Galata, S Gay, P Geisselsoder, S Geyer, K Giordano, V Gleixner, A Gracia-Ruiz, R Graf, K Hallmann, S van Haren, H Heijboer, AJ Hello, Y Hernandez-Rey, JJ Hossl, J Hofestadt, J Hugon, C James, CW de Jong, M Kadler, M Kalekin, O Katz, U Kiessling, D Kooijman, P Kouchner, A Kreter, M Kreykenbohm, I Kulikovskiy, V Lahmann, R Lefevre, D Leonora, E Loucatos, S Marcelin, M Margiotta, A Marinelli, A Martinez-Mora, JA Mathieu, A Michael, T Migliozzi, P Moussa, A Mueller, C Nezri, E Pavalas, GE Pellegrino, C Perrina, C Piattelli, P Popa, V Pradier, T Racca, C Riccobene, G Richter, R Roensch, K Saldana, M Samtleben, DFE Sanchez-Losa, A Sanguineti, M Sapienza, P Schmid, J Schnabel, J Schussler, F Seitz, T Sieger, C Spurio, M Steijger, JJM Stolarczyk, T Taiuti, M Tamburini, C Trovato, A Tselengidou, M Tonnis, C Vallage, B Vallee, C Van Elewyck, V Visser, E Vivolo, D Wagner, S Wilms, J Zornoza, JD Zuniga, J Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Ansseau, I Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Clark, K Classen, L Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Rosendo, ED Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M De Young, T Diaz-Velez, JC di Lorenzo, V Dumm, JP Dunkman, M Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fahey, S Fazely, AR Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Fosig, CC Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Glagla, M Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Gora, D Grant, D Griffith, Z Gross, A Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansen, E Hansmann, B Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jeong, M Jero, K Jurkovic, M Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohnen, G Koirala, R Kolanoski, H Konietz, R Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kruckl, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lesiak-Bzdak, M Leuermann, M Leuner, J Lu, L Lunemann, J Madsen, J Maggi, G Mahn, KBM Mandelartz, M Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Neer, G Niederhausen, H Nowicki, SC Nygren, DR Pollmann, AO Olivas, A Omairat, A O'Murchadha, A Palczewski, T Pandya, H Pankova, DV Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Raab, C Radel, L Rameez, M Rawlins, K Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ryckbosch, D Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Scheriau, F Schimp, M Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schulte, L Schumacher, L Seckel, D Seunarine, S Soldin, D Song, M Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stasik, A Steuer, A Stezelberger, T Stokstad, RG Stossl, A Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Tatar, J Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Toscano, S Tosi, D Tselengidou, M Turcati, A Unger, E Usner, M Vallecorsa, S Vandenbroucke, J van Eijndhoven, N Vanheule, S van Santen, J Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallace, A Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Wiebe, K Wiebusch, CH Wille, L Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zoll, M AF Adrian-Martinez, S. Albert, A. Andre, M. Anton, G. Ardid, M. Aubert, J. -J. Baret, B. Barrios-Marti, J. Basa, S. Bertin, V. Biagi, S. Bormuth, R. Bouwhuis, M. C. Bruijn, R. Brunner, J. Busto, J. Capone, A. Caramete, L. Carr, J. Chiarusi, T. Circella, M. Coniglione, R. Costantini, H. Coyle, P. Creusot, A. Dekeyser, I. Deschamps, A. De Bonis, G. Distefano, C. Donzaud, C. Dornic, D. Drouhin, D. Dumas, A. Eberl, T. Elsaesser, D. Enzenhoefer, A. Fehn, K. Felis, I. Fermani, P. Folger, F. Fusco, L. A. Galata, S. Gay, P. Geisselsoeder, S. Geyer, K. Giordano, V. Gleixner, A. Gracia-Ruiz, R. Graf, K. Hallmann, S. van Haren, H. Heijboer, A. J. Hello, Y. Hernandez-Rey, J. J. Hoessl, J. Hofestaedt, J. Hugon, C. James, C. W. de Jong, M. Kadler, M. Kalekin, O. Katz, U. Kiessling, D. Kooijman, P. Kouchner, A. Kreter, M. Kreykenbohm, I. Kulikovskiy, V. Lahmann, R. Lefevre, D. Leonora, E. Loucatos, S. Marcelin, M. Margiotta, A. Marinelli, A. Martinez-Mora, J. A. Mathieu, A. Michael, T. Migliozzi, P. Moussa, A. Mueller, C. Nezri, E. Pavalas, G. E. Pellegrino, C. Perrina, C. Piattelli, P. Popa, V. Pradier, T. Racca, C. Riccobene, G. Richter, R. Roensch, K. Saldana, M. Samtleben, D. F. E. Sanchez-Losa, A. Sanguineti, M. Sapienza, P. Schmid, J. Schnabel, J. Schussler, F. Seitz, T. Sieger, C. Spurio, M. Steijger, J. J. M. Stolarczyk, Th. Taiuti, M. Tamburini, C. Trovato, A. Tselengidou, M. Tonnis, C. Vallage, B. Vallee, C. Van Elewyck, V. Visser, E. Vivolo, D. Wagner, S. Wilms, J. Zornoza, J. D. Zuniga, J. Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Ansseau, I. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Clark, K. Classen, L. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Rosendo, E. del Pino Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. De Young, T. Diaz-Velez, J. C. di Lorenzo, V. Dumm, J. P. Dunkman, M. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fahey, S. Fazely, A. R. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Foesig, C. -C. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Glagla, M. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Gora, D. Grant, D. Griffith, Z. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansen, E. Hansmann, B. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jeong, M. Jero, K. Jurkovic, M. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Kohnen, G. Koirala, R. Kolanoski, H. Konietz, R. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Krueckl, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Lu, L. Lunemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Mandelartz, M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Neer, G. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Pollmann, A. Obertacke Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Pandya, H. Pankova, D. V. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raab, C. Raedel, L. Rameez, M. Rawlins, K. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ryckbosch, D. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Scheriau, F. Schimp, M. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schulte, L. Schumacher, L. Seckel, D. Seunarine, S. Soldin, D. Song, M. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stasik, A. Steuer, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strom, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Tatar, J. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Toscano, S. Tosi, D. Tselengidou, M. Turcati, A. Unger, E. Usner, M. Vallecorsa, S. Vandenbroucke, J. van Eijndhoven, N. Vanheule, S. van Santen, J. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallace, A. Wallraff, M. Wandkowsky, N. Weaver, Ch. Wendt, C. Westerhoff, S. Whelan, B. J. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zoll, M. CA ANTARES Collaboration IceCube Collaboration TI THE FIRST COMBINED SEARCH FOR NEUTRINO POINT-SOURCES IN THE SOUTHERN HEMISPHERE WITH THE ANTARES AND ICECUBE NEUTRINO TELESCOPES SO ASTROPHYSICAL JOURNAL LA English DT Article DE astroparticle physics; neutrinos ID HIGH-ENERGY NEUTRINOS; SUPERNOVA-REMNANTS; FLUX PREDICTIONS; ASTRONOMY; TEV; ASTROPHYSICS; MICROQUASARS; PERFORMANCE; EMISSION; DETECTOR AB We present the results of searches for point-like sources of neutrinos based on the first combined analysis of data from both the ANTARES and IceCube neutrino telescopes. The combination of both detectors, which differ in size and location, forms a window in the southern sky where the sensitivity to point sources improves by up to a factor of 2 compared with individual analyses. Using data recorded by ANTARES from 2007 to 2012, and by IceCube from 2008 to 2011, we search for sources of neutrino emission both across the southern sky and from a preselected list of candidate objects. No significant excess over background has been found in these searches, and flux upper limits for the candidate sources are presented for E-2.5 and E-2 power-law spectra with different energy cut-offs. C1 [Adrian-Martinez, S.; Ardid, M.; Felis, I.; Martinez-Mora, J. A.; Saldana, M.] Univ Politecn Valencia, Inst Invest Gestio Integrada Zones Costaneres IGI, C Paranimf 1, E-46730 Gandia, Spain. [Albert, A.; Drouhin, D.; Racca, C.] Univ Haute Alsace, GRPHE, Inst Univ Technol Colmar, 34 Rue Grillenbreit BP, F-50568 Colmar, France. 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[Dumas, A.; Gay, P.] Univ Clermont Ferrand, Univ Blaise Pascal, CNRS, Phys Corpusculaire Lab,IN2P3, BP 10448, F-63000 Clermont Ferrand, France. [Elsaesser, D.; Kadler, M.; Kreter, M.; Mueller, C.] Univ Wurzburg, Inst Theoret Phys & Astrophys, Emil Fischer Str 31, D-97074 Wrzburg, Germany. [Fusco, L. A.; Margiotta, A.; Pellegrino, C.; Spurio, M.] Univ Bologna, Dipartimento Fis & Astron, Viale Berti Pichat 6-2, I-40127 Bologna, Italy. [Giordano, V.; Leonora, E.] Ist Nazl Fis Nucl, Sez Catania, Viale Andrea Doria 6, I-95125 Catania, Italy. [van Haren, H.] Royal Netherlands Inst Sea Res NIOZ, Landsdiep 4, NL-1797 SZ Texel, Netherlands. [Hugon, C.; Sanguineti, M.; Taiuti, M.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Hugon, C.; Sanguineti, M.; Taiuti, M.] Univ Genoa, Dipartimento Fis, Via Dodecaneso 33, I-16146 Genoa, Italy. [Kooijman, P.] Univ Utrecht, Fac Betawetenschappen, Princetonplein 5, NL-3584 CC Utrecht, Netherlands. [Kreykenbohm, I.; Wilms, J.] Univ Erlangen Nurnberg, Dr Remeis Sternwarte, Sternwartstr 7, D-96049 Bamberg, Germany. [Kreykenbohm, I.; Wilms, J.] Univ Erlangen Nurnberg, ECAP, Sternwartstr 7, D-96049 Bamberg, Germany. [Kulikovskiy, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. [Leonora, E.] Univ Catania, Dipartimento Fis & Astron, Viale Andrea Doria 6, I-95125 Catania, Italy. [Loucatos, S.; Schussler, F.; Stolarczyk, Th.; Vallage, B.] CEA Saclay, Serv Phys Particules, Inst Rech Fondament Univers, Direct Sci Matiere, F-91191 Gif Sur Yvette, France. [Marinelli, A.] Ist Nazl Fis Nucl, Sez Pisa, Largo B Pontecorvo 3, I-56127 Pisa, Italy. [Marinelli, A.] Univ Pisa, Dipartimento Fis, Largo B Pontecorvo 3, I-56127 Pisa, Italy. [Migliozzi, P.; Vivolo, D.] Ist Nazl Fis Nucl, Sez Napoli, Via Cintia, I-80126 Naples, Italy. [Moussa, A.] Univ Mohammed 1, Lab Phys Matter & Radiat, BP 717, Oujda 6000, Morocco. 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[Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Koirala, R.; Pandya, H.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Koirala, R.; Pandya, H.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Lu, L.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Hansen, E.; Koskinen, D. J.; Larson, M. J.; Medici, M.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Inst Phys, Nussallee 12, D-53115 Bonn, Germany. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Kurahashi, N.; Richman, M.] Drexel Univ, Dept Phys, 3141 Chestnut St, Philadelphia, PA 19104 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.; Toale, P. A.; Williams, D. R.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Palczewski, T.; Pepper, J. A.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, 3211 Providence Dr, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Adrian-Martinez, S (reprint author), Univ Politecn Valencia, Inst Invest Gestio Integrada Zones Costaneres IGI, C Paranimf 1, E-46730 Gandia, Spain. RI Sarkar, Subir/G-5978-2011; Koskinen, David/G-3236-2014; James, Clancy/G-9178-2015; Migliozzi, Pasquale/I-6427-2015; Zuniga, Juan/P-4385-2014; Hernandez-Rey, Juan Jose/N-5955-2014; Capone, Antonio/F-1098-2010; Maruyama, Reina/A-1064-2013; Wilms, Joern/C-8116-2013; Eberl, Thomas/J-4826-2016; Anton, Gisela/C-4840-2013; Tjus, Julia/G-8145-2012; Beatty, James/D-9310-2011; Schussler, Fabian/G-5313-2013; Caramete, Laurentiu/C-2328-2011; Katz, Uli/E-1925-2013; Wiebusch, Christopher/G-6490-2012 OI Kadler, Matthias/0000-0001-5606-6154; Sarkar, Subir/0000-0002-3542-858X; Koskinen, David/0000-0002-0514-5917; James, Clancy/0000-0002-6437-6176; Migliozzi, Pasquale/0000-0001-5497-3594; Zuniga, Juan/0000-0002-1041-6451; Sanguineti, Matteo/0000-0002-7206-2097; Sanchez Losa, Agustin/0000-0001-9596-7078; Fusco, Luigi Antonio/0000-0001-8254-3372; Perez de los Heros, Carlos/0000-0002-2084-5866; Hernandez-Rey, Juan Jose/0000-0002-1527-7200; Maruyama, Reina/0000-0003-2794-512X; Wilms, Joern/0000-0003-2065-5410; Eberl, Thomas/0000-0002-5301-9106; Anton, Gisela/0000-0003-2039-4724; Beatty, James/0000-0003-0481-4952; Schussler, Fabian/0000-0003-1500-6571; Katz, Uli/0000-0002-7063-4418; Wiebusch, Christopher/0000-0002-6418-3008 FU Centre National de la Recherche Scientifique (CNRS), France; Commissariat a l'energie atomique et aux energies alternatives (CEA), France; Commission Europeenne, France; Region Ile-de-France (DIM-ACAV) Region Alsace, France; Region Provence-Alpes-Cote d'Azur, France; Departement du Var, France; Ville de La Seyne-sur-Mer, France; Bundesministerium fur Bildung und Forschung (BMBF), Germany; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Stichting voor Fundamenteel Onderzoek der Materie (FOM), the Netherlands; Nederlandse organisatie voor Wetenschappelijk Onderzoek (NWO), the Netherlands; Council of the President of the Russian Federation for young scientists and leading scientific schools supporting grants, Russia; National Authority for Scientific Research (ANCS), Romania; Ministerio de Economia y Competitividad (MINECO), Spain; Prometeo and Grisolia programs of Generalitat Valenciana, Spain; MultiDark, Spain; Agence de l'Oriental, Morocco; CNRST, Morocco; U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; WestGrid; Compute/Calcul Canada, Sweden; Swedish Research Council, Sweden; Swedish Polar Research Secretariat, Sweden; Swedish National Infrastructure for Computing (SNIC), Sweden; Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Germany; Deutsche Forschungsgemeinschaft (DFG), Germany; Helmholtz Alliance for Astroparticle Physics (HAP), Germany; Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX The authors of the ANTARES collaboration acknowledge the financial support of the funding agencies: Centre National de la Recherche Scientifique (CNRS), Commissariat a l'energie atomique et aux energies alternatives (CEA), Commission Europeenne (FEDER fund and Marie Curie Program), Region Ile-de-France (DIM-ACAV) Region Alsace (contrat CPER), Region Provence-Alpes-Cote d'Azur, Departement du Var and Ville de La Seyne-sur-Mer, France; Bundesministerium fur Bildung und Forschung (BMBF), Germany; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Stichting voor Fundamenteel Onderzoek der Materie (FOM), Nederlandse organisatie voor Wetenschappelijk Onderzoek (NWO), the Netherlands; Council of the President of the Russian Federation for young scientists and leading scientific schools supporting grants, Russia; National Authority for Scientific Research (ANCS), Romania; Ministerio de Economia y Competitividad (MINECO), Prometeo and Grisolia programs of Generalitat Valenciana and MultiDark, Spain; Agence de l'Oriental and CNRST, Morocco. We also acknowledge the technical support of Ifremer, AIM and Foselev Marine for the sea operation and the CC-IN2P3 for the computing facilities.; The authors of the IceCube collaboration acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 74 TC 5 Z9 5 U1 6 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 20 PY 2016 VL 823 IS 1 AR 65 DI 10.3847/0004-637X/823/1/65 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN6WD UT WOS:000377216300065 ER PT J AU Bhagia, S Muchero, W Kumar, R Tuskan, GA Wyman, CE AF Bhagia, Samarthya Muchero, Wellington Kumar, Rajeev Tuskan, Gerald A. Wyman, Charles E. TI Natural genetic variability reduces recalcitrance in poplar SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Rare poplar variants; Liquid hot water pretreatment; High-throughput pretreatment and co-hydrolysis; Poplar ranks; Lignin comparators ID LIGNOCELLULOSIC BIOMASS; ENZYMATIC-HYDROLYSIS; POPULUS-TRICHOCARPA; BIOFUEL PRODUCTION; CELLULOSE; ACID; PRETREATMENT; INHIBITION; CONVERSION; SUGARS AB Background: Lignin content and structure are known to affect recalcitrance of lignocellulosic biomass to chemical/biochemical conversion. Previously, we identified rare Populus trichocarpa natural variants with significantly reduced lignin content. Because reduced lignin content may lower recalcitrance, 18 rare variants along with 4 comparators, and BESC standard Populus was analyzed for composition of structural carbohydrates and lignin. Sugar yields from these plants were measured at 5 process conditions: one for just enzymatic hydrolysis without pretreatment and four via our combined high-throughput hot water pretreatment and co-hydrolysis (HTPH) technique. Results: Mean of glucan + xylan yields and the best glucan + xylan yield from rare natural poplar variants were 34 and 50 relative percent higher than the high lignin comparator (BESC-316) at the highest severity HTPH condition, respectively. The ability of HTPH to solubilize a large portion of xylan from solids led to small differences in xylan yields among poplar variants. However, HTPH showed large differences in glucan yields, and hence glucan + xylan yields, among the poplar variants. The high lignin comparator did not display lowest glucan + xylan yields with HTPH at moderate pretreatment severity compared to rare variants, but on the other hand, the low lignin comparator was a consistent top performer at all 5 process conditions. Furthermore, the low lignin comparator (GW-11012) showed a 15 absolute percent increase in glucan + xylan yield compared to the high lignin comparator at the most severe HTPH condition. Overall, relative variant rankings varied greatly with pretreatment severity, but poplar deconstruction was significantly enhanced when the pretreatment temperature was increased from 140 and 160 to 180 degrees C at the same pretreatment severity factor. Conclusions: Glucan yields from high severity HTPH of rare natural poplar variants with reduced lignin content were significantly higher than from the high lignin comparator. Because of the significant effect of processing conditions on the performance rankings, selection of the best performing biofuel feedstocks should be based on sugar yields tested at conditions that represent industrial practice. From a feedstock perspective, the most consistent variants, SKWE-24-2 and GW-11012, provide key insights into the genetic improvement of versatile lignocellulosic biofuels feedstock varieties. C1 [Bhagia, Samarthya; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, 900 Univ Ave, Riverside, CA 92521 USA. [Bhagia, Samarthya; Kumar, Rajeev; Wyman, Charles E.] Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol, 1084 Columbia Ave, Riverside, CA 92507 USA. [Tuskan, Gerald A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Bhagia, Samarthya; Muchero, Wellington; Kumar, Rajeev; Tuskan, Gerald A.; Wyman, Charles E.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, POB 2008, Oak Ridge, TN 37831 USA. RP Wyman, CE (reprint author), Univ Calif Riverside, Bourns Coll Engn, Dept Chem & Environm Engn, 900 Univ Ave, Riverside, CA 92521 USA.; Wyman, CE (reprint author), Univ Calif Riverside, Bourns Coll Engn, Ctr Environm Res & Technol, 1084 Columbia Ave, Riverside, CA 92507 USA.; Wyman, CE (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, POB 2008, Oak Ridge, TN 37831 USA. EM cewyman@engr.ucr.edu RI Tuskan, Gerald/A-6225-2011; OI Tuskan, Gerald/0000-0003-0106-1289; muchero, wellington/0000-0002-0200-9856 FU Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BioEnergy Science Center (BESC) at Oak Ridge National Laboratory [DE-PS02-06ER64304] FX This work was supported by Office of Biological and Environmental Research in the Department of Energy (DOE) Office of Science through the BioEnergy Science Center (BESC) at Oak Ridge National Laboratory (Contract DE-PS02-06ER64304). NR 33 TC 4 Z9 4 U1 4 U2 9 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 20 PY 2016 VL 9 AR 106 DI 10.1186/s13068-016-0521-2 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DN7LV UT WOS:000377258300001 PM 27213013 ER PT J AU McCallum, M Tammam, S Little, DJ Robinson, H Koo, J Shah, M Calmettes, C Moraes, TF Burrows, LL Howell, PL AF McCallum, Matthew Tammam, Stephanie Little, Dustin J. Robinson, Howard Koo, Jason Shah, Megha Calmettes, Charles Moraes, Trevor F. Burrows, Lori L. Howell, P. Lynne TI PilN Binding Modulates the Structure and Binding Partners of the Pseudomonas aeruginosa Type IVa Pilus Protein PilM SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE ligand-binding protein; protein chimera; Pseudomonas aeruginosa (P; aeruginosa); type IV pili; x-ray crystallography; PilM; PilN ID BACTERIAL 2-HYBRID SYSTEM; INNER MEMBRANE PLATFORM; II SECRETION SYSTEM; TWITCHING MOTILITY; CYTOPLASMIC DOMAIN; ESCHERICHIA-COLI; THERMUS-THERMOPHILUS; BIOFILM FORMATION; Z-RING; BIOGENESIS AB Pseudomonas aeruginosa is an opportunistic bacterial pathogen that expresses type IVa pili. The pilus assembly system, which promotes surface-associated twitching motility and virulence, is composed of inner and outer membrane subcomplexes, connected by an alignment subcomplex composed of PilMNOP. PilM binds to the N terminus of PilN, and we hypothesize that this interaction causes functionally significant structural changes in PilM. To characterize this interaction, we determined the crystal structures of PilM and a PilM chimera where PilM was fused to the first 12 residues of PilN (PilMPilN(1-12)). Structural analysis, multiangle light scattering coupled with size exclusion chromatography, and bacterial two-hybrid data revealed that PilM forms dimers mediated by the binding of a novel conserved motif in the N terminus of PilM, and binding PilN abrogates this binding interface, resulting in PilM monomerization. Structural comparison of PilM with PilMPilN(1-12) revealed that upon PilN binding, there is a large domain closure in PilM that alters its ATP binding site. Using biolayer interferometry, we found that the association rate of PilN with PilM is higher in the presence of ATP compared with ADP. Bacterial two-hybrid data suggested the connectivity of the cytoplasmic and inner membrane components of the type IVa pilus machinery in P. aeruginosa, with PilM binding to PilB, PilT, and PilC in addition to PilN. Pull-down experiments demonstrated direct interactions of PilM with PilB and PilT. We propose a working model in which dynamic binding of PilN facilitates functionally relevant structural changes in PilM. C1 [McCallum, Matthew; Little, Dustin J.; Shah, Megha; Calmettes, Charles; Moraes, Trevor F.; Howell, P. Lynne] Univ Toronto, Dept Biochem, Toronto, ON M5S 1A8, Canada. [McCallum, Matthew; Tammam, Stephanie; Little, Dustin J.; Koo, Jason; Howell, P. Lynne] Hosp Sick Children, Peter Gilgan Ctr Res & Learning, Program Mol Struct & Funct, 686 Bay St, Toronto, ON M5G 0A4, Canada. [Robinson, Howard] Brookhaven Natl Lab, Photon Sci Div, Upton, NY 11973 USA. [Burrows, Lori L.] McMaster Univ, Dept Biochem & Biomed Sci, Hamilton, ON L8N 3Z5, Canada. [Burrows, Lori L.] McMaster Univ, Michael G DeGroote Inst Infect Dis Res, Hamilton, ON L8N 3Z5, Canada. RP Howell, PL (reprint author), Hosp Sick Children, Peter Gilgan Ctr Res & Learning, Program Mol Struct & Funct, 686 Bay St, Toronto, ON M5G 0A4, Canada.; Burrows, LL (reprint author), McMaster Univ, Dept Biochem & Biomed Sci, Hamilton, ON L8N 3Z5, Canada.; Burrows, LL (reprint author), McMaster Univ, Michael G DeGroote Inst Infect Dis Res, Hamilton, ON L8N 3Z5, Canada. EM burrowl@mcmaster.ca; howell@sickkids.ca FU Department of Energy; National Institutes of Health National Center for Research Resources; Canadian Foundation for Innovation FX We thank Patrick Yip for technical assistance and Liliana Sampaleanu, Ryan Buensuceso, Tiffany Leighton, Hanjeong Harvey, and Daniel Yong for generation of initial PilM vectors and several BACTH constructs and for helpful discussions. Beamline X29 at the National Synchrotron Light Source, Brookhaven National Laboratory, is supported by the Department of Energy and by a grant from the National Institutes of Health National Center for Research Resources. Funds for the x-ray facilities at the Hospital for Sick Children were provided, in part, by the Canadian Foundation for Innovation. NR 69 TC 3 Z9 3 U1 2 U2 7 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 20 PY 2016 VL 291 IS 21 BP 11003 EP 11015 DI 10.1074/jbc.M116.718353 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DN4MT UT WOS:000377042100005 PM 27022027 ER PT J AU Li, HG Hwang, Y Perry, K Bushman, F Van Duyne, GD AF Li, Huiguang Hwang, Young Perry, Kay Bushman, Frederic Van Duyne, Gregory D. TI Structure and Metal Binding Properties of a Poxvirus Resolvase SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE enzyme structure; Holliday junction; metalloenzyme; poxvirus; viral replication; resolvase ID HOLLIDAY JUNCTION RESOLVASE; CRYSTAL-STRUCTURE; ESCHERICHIA-COLI; VACCINIA VIRUS; DNA JUNCTIONS; SUBSTRATE-SPECIFICITY; RNASE-H; GENETIC-RECOMBINATION; T7 ENDONUCLEASE; RUVC RESOLVASE AB Poxviruses replicate their linear genomes by forming concatemers that must be resolved into monomeric units to produce new virions. A viral resolvase cleaves DNA four-way junctions extruded at the concatemer junctions to produce monomeric genomes. This cleavage reaction is required for viral replication, so the resolvase is an attractive target for small molecule inhibitors. To provide a platform for understanding resolvase mechanism and designing inhibitors, we have determined the crystal structure of the canarypox virus (CPV) resolvase. CPV resolvase is dimer of RNase H superfamily domains related to Escherichia coli RuvC, with an active site lined by highly conserved acidic residues that bind metal ions. There are several intriguing structural differences between resolvase and RuvC, and a model of the CPV resolvaseHolliday junction complex provides insights into the consequences of these differences, including a plausible explanation for the weak sequence specificity exhibited by the poxvirus enzymes. The model also explains why the poxvirus resolvases are more promiscuous than RuvC, cleaving a variety of branched, bulged, and flap-containing substrates. Based on the unique active site structure observed for CPV resolvase, we have carried out a series of experiments to test divalent ion usage and preferences. We find that the two resolvase metal binding sites have different preferences for Mg(2+)versus Mn2+. Optimal resolvase activity is maintained with 5 mu m Mn2+ and 100 mu m Mg2+, concentrations that are well below those required for either metal alone. Together, our findings provide biochemical insights and structural models that will facilitate studying poxvirus replication and the search for efficient poxvirus inhibitors. C1 [Li, Huiguang; Van Duyne, Gregory D.] Univ Penn, Perelman Sch Med, Dept Biochem & Biophys, Philadelphia, PA 19104 USA. [Li, Huiguang] Univ Penn, Perelman Sch Med, Grad Grp Biochem & Mol Biophys, Philadelphia, PA 19104 USA. [Hwang, Young; Bushman, Frederic] Univ Penn, Perelman Sch Med, Dept Microbiol, Philadelphia, PA 19104 USA. [Perry, Kay] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14850 USA. [Perry, Kay] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Van Duyne, GD (reprint author), Univ Penn, Perelman Sch Med, Dept Biochem & Biophys, Philadelphia, PA 19104 USA.; Bushman, F (reprint author), Univ Penn, Perelman Sch Med, Dept Microbiol, Philadelphia, PA 19104 USA. EM bushman@mail.med.upenn.edu; vanduyne@mail.med.upenn.edu FU NIAID; National Institutes of Health Mid-Atlantic Regional Center of Excellence for Biodefense Research Grants [U54 AI057168, U01 AI 082015]; National Institutes of Health [P41 GM103403]; Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported in part by NIAID, National Institutes of Health Mid-Atlantic Regional Center of Excellence for Biodefense Research Grants U54 AI057168 and U01 AI 082015 and National Institutes of Health Grant P41 GM103403 (to the NE-CAT beamlines). The Advanced Photon Source is a U.S. Department of Energy Office of Science User Facility operated by Argonne National Laboratory under Contract DE-AC02-06CH11357. The authors declare that they have no conflicts of interest with the contents of this article. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. NR 52 TC 2 Z9 2 U1 0 U2 1 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 20 PY 2016 VL 291 IS 21 BP 11094 EP 11104 DI 10.1074/jbc.M115.709139 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DN4MT UT WOS:000377042100013 PM 27013661 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK 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CA ATLAS Collaboration TI Measurement of the differential cross-sections of prompt and non-prompt production of J/psi and psi(2S) in pp collisions at root s=7 and 8 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID P(P)OVER-BAR COLLISIONS; S=1.8 TEV; QUARKONIUM PRODUCTION; HADRONIC COLLISIONS; HEAVY-QUARKONIUM; J-PSI; POLARIZATION; CHI(C); GLUONS; HADROPRODUCTION AB The production rates of prompt and non-prompt J/psi and psi(2S) mesons in their dimuon decay modes are measured using 2.1 and 11.4 fb(-1) of data collected with the ATLAS experiment at the Large Hadron Collider, in proton-proton collisions at root s = 7 and 8 respectively. Production cross-sections for prompt as well as non-prompt sources, ratios of psi(2S) to J/psi production, and the fractions of non-prompt production for J/psi and psi(2S) are measured as a function of meson transverse momentum and rapidity. The measurements are compared to theoretical predictions. 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P.; Maidantchik, C.; Marroquim, F.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, San Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero y; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Sanchez, C. A. Solans; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiangb, Y.; Lib, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Songb, H. Y.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] PKU CHEP, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Penwell, J.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Ouchrif, M.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Coll Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindura, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA, Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Lindquist, B. E.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Geneva, Switzerland. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Geneva, Switzerland. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubuab, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Staerz, S.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmittb, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Bai, Y.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Ahmadov, F.; Aleksandrov, I. N.; Dos Santos, S. P. Amor; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. 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[Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primaveraa, M.; Spagnolo, S.; Vazeille, F.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Vazeille, F.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandio, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandio, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Calderini, G.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Derue, F.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Crescioli, F.; De Cecco, S.; Demilly, A.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Crescioli, F.; De Cecco, S.; Demilly, A.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. 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[Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Nechaeva, P. Yu.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, LAL, CNRS IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bernius, C.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Kreiss, S.; Lewis, A.; Nagai, K.; Neves, R. M.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguensb, J. Machado; Meyer, C.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Castro, N. F.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Varouchas, D.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Galhardo, B.; Gomes, A.; Jorge, P. M.; Miguensb, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Varouchas, D.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Voka, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys Protvino, Moscow NRC KI, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchia, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Pedis, D. De; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Giordani, M. P.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrania, F. Safai; Vanadia, M.; Vari, R.; Varvell, K. 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[Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fa Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Pinto Firmino Da Costa, J. Goncalves; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tayalati, Y.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondament Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Johannesburg, South Africa. [Bristow, K.; Hsuc, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoein, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoein, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Dao, V.; Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [AbouZeid, O. S.; Azuelos, G.; Batista, S. J.; Canepa, A.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Gingrich, D. M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Oakham, F. G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Miglioranzi, S.; Pinamonti, M.; Plazak, L.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Miglioranzi, S.; Pinamonti, M.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Veatch, J.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Soualah, R.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. 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[Guo, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubuab, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lib, B.; Songb, H. Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris Saclay, Univ Paris 11, LAL, CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Villa, Mauro/C-9883-2009; Warburton, Andreas/N-8028-2013; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Gladilin, Leonid/B-5226-2011; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Zhukov, Konstantin/M-6027-2015; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016 OI Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Gladilin, Leonid/0000-0001-9422-8636; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, The Netherlands; NWO, The Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; Investissement d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, The Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (The Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 61 TC 0 Z9 0 U1 16 U2 41 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 20 PY 2016 VL 76 IS 5 AR 283 DI 10.1140/epjc/s10052-016-4050-8 PG 47 WC Physics, Particles & Fields SC Physics GA DM8IU UT WOS:000376606500003 PM 28280433 ER PT J AU Badziak, M Wagner, CEM AF Badziak, Marcin Wagner, Carlos E. M. TI Enhancing the Higgs associated production with a top quark pair SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Higgs Physics; Supersymmetric Standard Model ID ATLAS DETECTOR; STANDARD MODEL; PP COLLISIONS; ROOT-S=8 TEV; FINAL-STATES; SEARCH; BOSON; LHC; CONSTRAINTS; BREAKING AB It is pointed out that in a wide class of models reminiscent of type-II Two-Higgs-Doublet Models (2HDM) the signal of the Higgs produced in association with a top-antitop quark pair (tth) and decaying into gauge bosons can be significantly larger than the Standard Model (SM) prediction without violating any experimental constraints. The crucial feature of these models is enhanced (suppressed) Higgs coupling to top (bottom) quarks and existence of light colored particles that give negative contribution to the effective Higgs coupling to gluons resulting in the gluon fusion rates in the gauge boson decay channels close to SM predictions. We demonstrate this mechanism in NMSSM with light stops and show that tth signal in the WW decay channel can be two times larger than the SM prediction, as suggested by the excesses observed by ATLAS and CMS, provided that the Higgs-singlet superpotential coupling lambda greater than or similar to 0.8 and the MSSM-like Higgs boson masses are in the range of 160 to 300 GeV. C1 [Badziak, Marcin] Univ Warsaw, Fac Phys, Inst Theoret Phys, Ul Pasteura 5, PL-02093 Warsaw, Poland. [Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Badziak, M (reprint author), Univ Warsaw, Fac Phys, Inst Theoret Phys, Ul Pasteura 5, PL-02093 Warsaw, Poland.; Wagner, CEM (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Wagner, CEM (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.; Wagner, CEM (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. EM mbadziak@fuw.edu.pl; cwagner@hep.anl.gov RI Badziak, Marcin/G-3382-2011 FU National Science Centre [DEC-2014/15/B/ST2/02157]; Polish Ministry of Science and Higher Education [1266/MOB/IV/2015/0]; U.S. Department of Energy, Office of High Energy Physics [DE-AC02-06CH11357]; U.S. Department of Energy [DE-FG02-13ER41958]; Galileo Galilei Institute for Theoretical Physics; INFN; National Science Foundation [PHYS-1066293] FX This work has been partially supported by National Science Centre under research grant DEC-2014/15/B/ST2/02157. MB acknowledges support from the Polish Ministry of Science and Higher Education (decision no. 1266/MOB/IV/2015/0). Work at ANL is supported in part by the U.S. Department of Energy, Office of High Energy Physics, under Contract No. DE-AC02-06CH11357. Work at the University of Chicago is supported in part by U.S. Department of Energy grant number DE-FG02-13ER41958. MB would like to thank Cyril Hugonie, Ulrich Ellwanger and Tim Stefaniak for useful correspondence about NMSSMTools and HiggsBounds. MB thanks the Galileo Galilei Institute for Theoretical Physics and INFN for hospitality and partial support during the completion of this work. C.W thanks the hospitality of the Aspen Center for Physics, which is supported by the National Science Foundation under Grant No. PHYS-1066293. NR 61 TC 2 Z9 2 U1 1 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 20 PY 2016 IS 5 AR 123 DI 10.1007/JHEP05(2016)123 PG 21 WC Physics, Particles & Fields SC Physics GA DM9NC UT WOS:000376692000001 ER PT J AU Chien, YT Kang, ZB Ringer, F Vitew, I Xing, HX AF Chien, Yang-Ting Kang, Zhong-Bo Ringer, Felix Vitew, Ivan Xing, Hongxi TI Jet fragmentation functions in proton-proton collisions using soft-collinear effective theory SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; QCD Phenomenology ID PB COLLISIONS; DISTRIBUTIONS; SUBSTRUCTURE; LHC; TEV AB The jet fragmentation function describes the longitudinal momentum distribution of hadrons inside a reconstructed jet. We study the jet fragmentation function in proton-proton collisions in the framework of soft-collinear effective theory (SCET). We find that, up to power corrections, the jet fragmentation function can be expressed as the ratio of the fragmenting jet function and the unmeasured jet function. Using renormalization group techniques, we are able to resum large logarithms of jet radii R in the perturbative expansion of the cross section. We use our theoretical formalism to describe the jet fragmentation functions for light hadron and heavy meson production measured at the Large Hadron Collider (LHC). Our calculations agree very well with the experimental data for the light hadron production. On the other hand, although our calculations for the heavy meson production inside jets are consistent with the PYTHIA simulation, they fail to describe the LHC data. We find that the jet fragmentation function for heavy meson production is very sensitive to the gluon-to-heavy-meson fragmentation function. C1 [Chien, Yang-Ting; Kang, Zhong-Bo; Ringer, Felix; Vitew, Ivan; Xing, Hongxi] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Chien, YT; Kang, ZB; Ringer, F; Vitew, I; Xing, HX (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM ytchien@lanl.gov; zkang@lanl.gov; f.ringer@lanl.gov; ivitev@lanl.gov; hxing@lanl.gov RI Kang, Zhongbo/P-3645-2014 FU U.S. Department of Energy [DE-AC52-06NA25396]; Office of Science Early Career Award program; LDRD program at Los Alamos National Laboratory FX We would like to thank Emanuele Mereghetti for his collaboration at the early stage of the project, and for many useful discussions and comments throughout the project. We also thank Andrew Hornig, Daekyoung Kang, Christopher Lee, Adam Leibovich, Thomas Mehen, Werner Vogelsang, and Wouter Waalewijn for helpful discussions and comments. This work is supported by the U.S. Department of Energy under Contract No. DE-AC52-06NA25396, the Office of Science Early Career Award program, and in part by the LDRD program at Los Alamos National Laboratory. NR 65 TC 5 Z9 5 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 20 PY 2016 IS 5 AR 125 DI 10.1007/JHEP05(2016)125 PG 26 WC Physics, Particles & Fields SC Physics GA DM6KB UT WOS:000376459500002 ER PT J AU Zhu, CZ Guo, ZH Mu, AU Liu, Y Wheeler, SE Fang, L AF Zhu, Congzhi Guo, Zi-Hao Mu, Anthony U. Liu, Yi Wheeler, Steven E. Fang, Lei TI Low Band Gap Coplanar Conjugated Molecules Featuring Dynamic Intramolecular Lewis Acid-Base Coordination SO JOURNAL OF ORGANIC CHEMISTRY LA English DT Article ID FIELD-EFFECT TRANSISTORS; HIGH-ELECTRON-MOBILITY; BN HETEROSUPERBENZENES; CHARGE-TRANSFER; CROCONATE DYES; POLYMERS; ABSORPTION; SYSTEMS; DERIVATIVES; ACCEPTOR AB Ladder-type conjugated molecules with a low band gap and low LUMO level were synthesized through an N-directed borylation reaction of pyrazine-derived donor-acceptor-donor precursors. The intramolecular boron-nitrogen coordination bonds played a key role in rendering the rigid and coplanar conformation of these molecules and their corresponding electronic structures. Experimental investigation and theoretical simulation revealed the dynamic nature of such coordination, which allowed for active manipulation of the optical properties of these molecules by using competing Lewis basic solvents. C1 [Zhu, Congzhi; Guo, Zi-Hao; Mu, Anthony U.; Wheeler, Steven E.; Fang, Lei] Texas A&M Univ, Dept Chem, 3255 TAMU, College Stn, TX 77843 USA. [Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Fang, L (reprint author), Texas A&M Univ, Dept Chem, 3255 TAMU, College Stn, TX 77843 USA. EM fang@chem.tamu.edu RI Liu, yi/A-3384-2008; Wheeler, Steven/G-5834-2011; Guo, Zi-Hao/K-5163-2015 OI Liu, yi/0000-0002-3954-6102; Wheeler, Steven/0000-0001-7824-6906; Guo, Zi-Hao/0000-0001-7948-2919 FU Texas AM University; National Science Foundation [CHE-1254897]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Dr. Jodie Lutkenhaus and Dr. Fei Li at TAMU for help with the cyclic voltammetry experiments. Funding is gratefully acknowledged from Texas A&M University and the National Science Foundation (Grant CHE-1254897). Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 64 TC 5 Z9 5 U1 14 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0022-3263 J9 J ORG CHEM JI J. Org. Chem. PD MAY 20 PY 2016 VL 81 IS 10 BP 4347 EP 4352 DI 10.1021/acs.joc.6b00238 PG 6 WC Chemistry, Organic SC Chemistry GA DM6QB UT WOS:000376476400041 PM 27096728 ER PT J AU Gao, F Chen, J Liu, YX Qin, SX Roberts, CD Schmidt, SM AF Gao, Fei Chen, Jing Liu, Yu-Xin Qin, Si-Xue Roberts, Craig D. Schmidt, Sebastian M. TI Phase diagram and thermal properties of strong-interaction matter SO PHYSICAL REVIEW D LA English DT Article ID DYSON-SCHWINGER EQUATIONS; CHIRAL-SYMMETRY BREAKING; QUANTUM CHROMODYNAMICS; ASYMPTOTIC FREEDOM; OF-STATE; QCD; CONFINEMENT; CONTINUUM; LATTICE; PROPAGATORS AB We introduce a novel method for computing the (mu, T)-dependent pressure in continuum QCD, from which we obtain a complex phase diagram and predictions for thermal properties of the dressed-quark component of the system, providing the in-medium behavior of the related trace anomaly, speed of sound, latent heat, and heat capacity. C1 [Gao, Fei; Chen, Jing; Liu, Yu-Xin] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Gao, Fei; Chen, Jing; Liu, Yu-Xin] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Liu, Yu-Xin] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Liu, Yu-Xin] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. [Qin, Si-Xue; Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Schmidt, Sebastian M.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Schmidt, Sebastian M.] JARA, D-52425 Julich, Germany. RP Liu, YX (reprint author), Peking Univ, Dept Phys, Beijing 100871, Peoples R China.; Liu, YX (reprint author), Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China.; Liu, YX (reprint author), Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China.; Liu, YX (reprint author), Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China.; Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM yxliu@pku.edu.cn; cdroberts@anl.gov FU National Natural Science Foundation of China [11435001, 11175004]; National Key Basic Research Program of China [G2013CB834400, 2015CB956900]; Office of the Director at Argonne National Laboratory through the Named Postdoctoral Fellowship Program; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC0206CH11357] FX This work was supported by the National Natural Science Foundation of China under Contracts No. 11435001 and No. 11175004; the National Key Basic Research Program of China under Contracts No. G2013CB834400 and No. 2015CB956900; the Office of the Director at Argonne National Laboratory through the Named Postdoctoral Fellowship Program; and the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC0206CH11357. NR 69 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 20 PY 2016 VL 93 IS 9 AR 094019 DI 10.1103/PhysRevD.93.094019 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM3OS UT WOS:000376256400003 ER PT J AU Malapi-Wight, M Demers, JE Veltri, D Marra, RE Crouch, JA AF Malapi-Wight, Martha Demers, Jill E. Veltri, Daniel Marra, Robert E. Crouch, Jo Anne TI LAMP Detection Assays for Boxwood Blight Pathogens: A Comparative Genomics Approach SO SCIENTIFIC REPORTS LA English DT Article ID MEDIATED ISOTHERMAL AMPLIFICATION; CALONECTRIA-PSEUDONAVICULATA; CYLINDROCLADIUM-BUXICOLA; VIRUS DIAGNOSTICS; VISUAL DETECTION; PLANT-PATHOGENS; STEM BLIGHT; BOX BLIGHT; 1ST REPORT; DNA AB Rapid and accurate molecular diagnostic tools are critical to efforts to minimize the impact and spread of emergent pathogens. The identification of diagnostic markers for novel pathogens presents several challenges, especially in the absence of information about population diversity and where genetic resources are limited. The objective of this study was to use comparative genomics datasets to find unique target regions suitable for the diagnosis of two fungal species causing a newly emergent blight disease of boxwood. Candidate marker regions for loop-mediated isothermal amplification (LAMP) assays were identified from draft genomes of Calonectria henricotiae and C. pseudonaviculata, as well as three related species not associated with this disease. To increase the probability of identifying unique targets, we used three approaches to mine genome datasets, based on (i) unique regions, (ii) polymorphisms, and (iii) presence/absence of regions across datasets. From a pool of candidate markers, we demonstrate LAMP assay specificity by testing related fungal species, common boxwood pathogens, and environmental samples containing 445 diverse fungal taxa. This comparative-genomics-based approach to the development of LAMP diagnostic assays is the first of its kind for fungi and could be easily applied to diagnostic marker development for other newly emergent plant pathogens. C1 [Malapi-Wight, Martha; Demers, Jill E.; Veltri, Daniel; Crouch, Jo Anne] ARS, USDA, Systemat Mycol & Microbiol Lab, Beltsville, MD 20705 USA. [Veltri, Daniel] ARS, Oak Ridge Inst Sci & Educ, Res Participat Program, Oak Ridge, TN 37831 USA. [Marra, Robert E.] Connecticut Agr Expt Stn, Dept Plant Pathol & Ecol, New Haven, CT 06504 USA. [Malapi-Wight, Martha] Anim & Plant Hlth Inspect Serv, USDA, Plant Germplasm Quarantine Program, Beltsville, MD 20705 USA. RP Crouch, JA (reprint author), ARS, USDA, Systemat Mycol & Microbiol Lab, Beltsville, MD 20705 USA. EM joanne.crouch@ars.usda.gov OI Crouch, Jo Anne/0000-0001-6886-8090; Veltri, Daniel/0000-0002-6101-6693; Malapi-Wight, Martha/0000-0003-2249-6257 FU USDA-APHIS Farm Bill [10201, 10004]; USDA-ARS Floricultural and Nursery Research Fund; Class of USDA-ARS Headquarters Research Associate Award; DOE [DE-AC05-06OR23100] FX This work was supported by funds from the USDA-APHIS 2012 Farm Bill 10201 to JAC and REM, and funds from the USDA-ARS Floricultural and Nursery Research Fund to JAC. MMW is supported by a Class of 2013 USDA-ARS Headquarters Research Associate Award to JAC; JED is supported by a Class of 2012 USDA-ARS Headquarters Research Associate Award to Lisa Castlebury; and DV is supported through 2013 and 2014 USDA-APHIS Farm Bill 10201 and 10004 grants to JAC. We thank Lisa Castlebury for helpful discussion of this manuscript; Kurt Heungens and Bjorn Gehesquiere for sharing fungal isolates; and Richard Buckley for the landscape images. This research was supported in part by an appointment to the Agricultural Research Service (ARS) Research Participation Program administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. Department of Energy (DOE) and the U.S. Department of Agriculture (USDA). ORISE is managed by ORAU under DOE contract number DE-AC05-06OR23100. Mention of trade names or commercial products in this publication is solely for the purpose of providing specific information and does not imply recommendation or endorsement by the USDA. USDA is an equal opportunity provider and employer. NR 47 TC 1 Z9 1 U1 5 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 20 PY 2016 VL 6 AR 26140 DI 10.1038/srep26140 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM7QC UT WOS:000376554100001 PM 27199028 ER PT J AU Yang, Y Burghoff, D Hayton, DJ Gao, JR Reno, JL Hu, Q AF Yang, Yang Burghoff, David Hayton, Darren J. Gao, Jian-Rong Reno, John L. Hu, Qing TI Terahertz multiheterodyne spectroscopy using laser frequency combs SO OPTICA LA English DT Article ID QUANTUM-CASCADE-LASER AB The terahertz region is of great importance for spectroscopy since many molecules have absorption fingerprints there. Frequency combs based on terahertz quantum cascade lasers feature broadband coverage and high output powers in a compact package, making them an attractive option for broadband spectroscopy. Here, we demonstrate the first multiheterodyne spectroscopy using two terahertz quantum cascade laser combs. Over a spectral range of 250 GHz, we achieve average signal-to-noise ratios of 34 dB using cryogenic detectors and 24 dB using room-temperature detectors, all in just 100 mu s. As a proof of principle, we use these combs to measure the broadband transmission spectrum of etalon samples and show that, with proper signal processing, it is possible to extend the multiheterodyne spectroscopy to quantum cascade laser combs operating in pulsed mode. This greatly expands the range of quantum cascade lasers that could be suitable for these techniques and allows for the creation of completely solid-state terahertz laser spectrometers. (C) 2016 Optical Society of America C1 [Yang, Yang; Burghoff, David; Hu, Qing] MIT, Dept Elect Engn & Comp Sci, Elect Res Lab, Cambridge, MA 02139 USA. [Hayton, Darren J.; Gao, Jian-Rong] SRON Netherlands Inst Space Res, NL-9747 AD Groningen, Netherlands. [Gao, Jian-Rong] Delft Univ Technol, Kavli Inst NanoSci, Lorentzweg 1, NL-2628 CJ Delft, Netherlands. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87123 USA. RP Yang, Y (reprint author), MIT, Dept Elect Engn & Comp Sci, Elect Res Lab, Cambridge, MA 02139 USA. EM yang_y@mit.edu FU Defense Advanced Research Projects Agency (DARPA) [W31P4Q-16-1-0001]; National Science Foundation (NSF); North Atlantic Treaty Organization (NATO) (NATO-SFP); European Commission (EC) (RadioNet); Netherlands Organisation for Scientific Research (NWO); Sandia National Laboratories; U.S. Department of Energy (DOE) [DE-AC04-94AL85000] FX Defense Advanced Research Projects Agency (DARPA) (W31P4Q-16-1-0001); National Science Foundation (NSF); North Atlantic Treaty Organization (NATO) (NATO-SFP); European Commission (EC) (RadioNet); Netherlands Organisation for Scientific Research (NWO); Sandia National Laboratories; U.S. Department of Energy (DOE) (DE-AC04-94AL85000). NR 31 TC 7 Z9 7 U1 3 U2 7 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2334-2536 J9 OPTICA JI Optica PD MAY 20 PY 2016 VL 3 IS 5 BP 499 EP 502 DI 10.1364/OPTICA.3.000499 PG 4 WC Optics SC Optics GA DM5NE UT WOS:000376395400007 ER PT J AU Garcia, A Wang, J Windus, TL Sadow, AD Evans, JW AF Garcia, Andres Wang, Jing Windus, Theresa L. Sadow, Aaron D. Evans, James W. TI Catalytic conversion reactions in nanoporous systems with concentration-dependent selectivity: Statistical mechanical modeling SO PHYSICAL REVIEW E LA English DT Article ID SINGLE-FILE DIFFUSION; TRACER EXCHANGE; ZEOLITE; MOLECULES; KINETICS AB Statistical mechanical modeling is developed to describe a catalytic conversion reaction A -> B-c or B-t with concentration-dependent selectivity of the products, B-c or B-t, where reaction occurs inside catalytic particles traversed by narrow linear nanopores. The associated restricted diffusive transport, which in the extreme case is described by single-file diffusion, naturally induces strong concentration gradients. Furthermore, by comparing kinetic Monte Carlo simulation results with analytic treatments, selectivity is shown to be impacted by strong spatial correlations induced by restricted diffusivity in the presence of reaction and also by a subtle clustering of reactants, A. C1 [Garcia, Andres; Wang, Jing; Windus, Theresa L.; Sadow, Aaron D.; Evans, James W.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Garcia, Andres; Evans, James W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Wang, Jing; Evans, James W.] Iowa State Univ, Dept Math, Ames, IA 50011 USA. [Windus, Theresa L.; Sadow, Aaron D.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Wang, Jing] Amer Inst Res, 1000 Thomas Jefferson St NW, Washington, DC 20007 USA. RP Garcia, A (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.; Garcia, A (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; USDOE [DE-AC02-07CH11358] FX We thank Sanjeevi Sivasankar for instructive comments on the form of concentration profiles inside the pore. This work was supported by the U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program for the theory and modeling studies. The work was performed at Ames Laboratory which is operated for the USDOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 32 TC 1 Z9 1 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 20 PY 2016 VL 93 IS 5 AR 052137 DI 10.1103/PhysRevE.93.052137 PG 12 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DM3RE UT WOS:000376263100001 PM 27300859 ER PT J AU Hatta, Y Xiao, BW Yuan, F AF Hatta, Yoshitaka Xiao, Bo-Wen Yuan, Feng TI Probing the Small-x Gluon Tomography in Correlated Hard Diffractive Dijet Production in Deep Inelastic Scattering SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTON DISTRIBUTIONS; IMPACT PARAMETER; JETS; HERA; DISSOCIATION; SINGULARITY; SATURATION; POMERON AB We investigate the close connection between the quantum phase space Wigner distribution of small-x gluons and the color dipole scattering amplitude, and we propose studying it experimentally in the hard diffractive dijet production at the planned electron-ion collider. The angular correlation between the nucleon recoiled momentum and the dijet transverse momentum probes the nontrivial correlation in the phase space Wigner distribution. This experimental study not only provides us with three-dimensional tomographic pictures of gluons inside high energy protons-it gives a unique and interesting signal for the small-x dynamics with QCD evolution effects. C1 [Hatta, Yoshitaka] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Xiao, Bo-Wen] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Xiao, Bo-Wen] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Hatta, Y (reprint author), Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-05CH11231]; U.S. National Science Foundation [PHY-0855561, PHY-1417326]; NSFC [11575070] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-05CH11231, and by the U.S. National Science Foundation under Grants No. PHY-0855561 and No. PHY-1417326, as well as by the NSFC under Grant No. 11575070. B. X. acknowledges his interesting discussion with A. Mueller and wishes to thank Dr. X. N. Wang and the nuclear theory group at LBNL for their hospitality and support during his visit while this work was finalized. NR 53 TC 2 Z9 2 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 20 PY 2016 VL 116 IS 20 AR 202301 DI 10.1103/PhysRevLett.116.202301 PG 6 WC Physics, Multidisciplinary SC Physics GA DM3SR UT WOS:000376267300006 PM 27258865 ER PT J AU Wongnate, T Sliwa, D Ginovska, B Smith, D Wolf, MW Lehnert, N Raugei, S Ragsdale, SW AF Wongnate, Thanyaporn Sliwa, Dariusz Ginovska, Bojana Smith, Dayle Wolf, Matthew W. Lehnert, Nicolai Raugei, Simone Ragsdale, Stephen W. TI The radical mechanism of biological methane synthesis by methyl-coenzyme M reductase SO SCIENCE LA English DT Article ID ANAEROBIC OXIDATION; ALKYL-NICKEL; CATALYTIC CYCLE; LIQUID FUELS; METHANOGENESIS; ENZYME; ARCHAEA; F430; BOND; ACTIVATION AB Methyl-coenzyme M reductase, the rate-limiting enzyme in methanogenesis and anaerobic methane oxidation, is responsible for the biological production of more than 1 billion tons of methane per year. The mechanism of methane synthesis is thought to involve either methyl-nickel(III) or methyl radical/Ni(II)-thiolate intermediates. We employed transient kinetic, spectroscopic, and computational approaches to study the reaction between the active Ni(I) enzyme and substrates. Consistent with the methyl radical-based mechanism, there was no evidence for a methyl-Ni(III) species; furthermore, magnetic circular dichroism spectroscopy identified the Ni(II)-thiolate intermediate. Temperature-dependent transient kinetics also closely matched density functional theory predictions of the methyl radical mechanism. Identifying the key intermediate in methanogenesis provides fundamental insights to develop better catalysts for producing and activating an important fuel and potent greenhouse gas. C1 [Wongnate, Thanyaporn; Sliwa, Dariusz; Ragsdale, Stephen W.] Univ Michigan, Dept Biol Chem, Ann Arbor, MI 48109 USA. [Ginovska, Bojana; Smith, Dayle; Raugei, Simone] Pacific NW Natl Lab, Phys Sci Div, POB 999,K1-83, Richland, WA 99352 USA. [Wolf, Matthew W.; Lehnert, Nicolai] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. [Wolf, Matthew W.; Lehnert, Nicolai] Univ Michigan, Dept Biophys, Ann Arbor, MI 48109 USA. [Sliwa, Dariusz] Appl Photophys Inc, Cummings Ctr 100, Suite 440C, Beverly, MA 01915 USA. [Smith, Dayle] Intel Corp, 2111 NW 25th Ave,JF5-202, Hillsboro, OR 97124 USA. RP Ragsdale, SW (reprint author), Univ Michigan, Dept Biol Chem, Ann Arbor, MI 48109 USA. EM sragsdal@umich.edu FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-FG02-08ER15931]; U.S. DOE, Advanced Research Projects Agency - Energy [DE-AR0000426]; DOE's Office of Biological and Environmental Research FX Data presented here are available through the Ragsdale LabGuru portal (https://my.labguru.com/knowledge/projects/361/milestones/711). This work was supported by U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under award DE-FG02-08ER15931 and by U.S. DOE, Advanced Research Projects Agency - Energy, under award number DE-AR0000426. Computer resources were provided by the W. R. Wiley Environmental Molecular Sciences Laboratory, a DOE Office of Science User Facility located at Pacific Northwest National Laboratory and sponsored by DOE's Office of Biological and Environmental Research. Computer resources were also provided by the National Energy Research Computing Center at the Lawrence Berkeley National Laboratory. Author contributions: T.W. generated the data, performed the data analysis, and prepared Figs. 2, A and B, and 4, and Table 1; and performed the data analysis and generated Fig. 2, C and D, and figs. S1, S4, and S6. D. Sliwa prepared CoBSH substrates and enzyme; generated the data and performed preliminary data analysis for Fig. 2, C and D, and fig. S1; and prepared the samples for the MCD measurements described in Fig. 3 and fig. S2. B.G. and S.R. performed and interpreted the computational studies described in Fig. 5; figs. S5, S7, S8, and S9; and tables S1 to S3. D. Smith performed initial computational experiments on the MCR mechanisms. M.W. and N.L. performed, analyzed, and interpreted the MCD spectroscopic experiments and prepared Fig. 3 and fig. S2. S.W.R. conceptualized and refined the research idea; prepared Figs. 1 and 6 and fig. S3; and coordinated the various collaborations and guided analysis and interpretation of the biochemical experiments. All authors were involved to varying degrees in writing and/or editing the manuscript. NR 48 TC 12 Z9 12 U1 31 U2 63 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 20 PY 2016 VL 352 IS 6288 SI SI BP 953 EP 958 DI 10.1126/science.aaf0616 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM2AK UT WOS:000376147800039 PM 27199421 ER PT J AU Wang, YL Xiao, ZL Snezhko, A Xu, J Ocola, LE Divan, R Pearson, JE Crabtree, GW Kwok, WK AF Wang, Yong-Lei Xiao, Zhi-Li Snezhko, Alexey Xu, Jing Ocola, Leonidas E. Divan, Ralu Pearson, John E. Crabtree, George W. Kwok, Wai-Kwong TI Rewritable artificial magnetic charge ice SO SCIENCE LA English DT Article ID DOT CELLULAR-AUTOMATA; SPIN-ICE; LOGIC GATE; FRUSTRATION; ELECTRONS; LATTICE AB Artificial ices enable the study of geometrical frustration by design and through direct observation. However, it has proven difficult to achieve tailored long-range ordering of their diverse configurations, limiting both fundamental and applied research directions. We designed an artificial spin structure that produces a magnetic charge ice with tunable long-range ordering of eight different configurations. We also developed a technique to precisely manipulate the local magnetic charge states and demonstrate write-read-erase multifunctionality at room temperature. This globally reconfigurable and locally writable magnetic charge ice could provide a setting for designing magnetic monopole defects, tailoring magnonics, and controlling the properties of other two-dimensional materials. C1 [Wang, Yong-Lei; Xiao, Zhi-Li; Snezhko, Alexey; Xu, Jing; Pearson, John E.; Crabtree, George W.; Kwok, Wai-Kwong] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wang, Yong-Lei] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Xiao, Zhi-Li; Xu, Jing] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Ocola, Leonidas E.; Divan, Ralu] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. [Crabtree, George W.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Crabtree, George W.] Univ Illinois, Dept Elect & Comp Engn, Chicago, IL 60607 USA. [Crabtree, George W.] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA. RP Wang, YL; Xiao, ZL (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Wang, YL (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA.; Xiao, ZL (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. EM ylwang@anl.gov; xiao@anl.gov RI Wang, Yong-Lei/N-7940-2013 OI Wang, Yong-Lei/0000-0003-0391-7757 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; NSF [DMR-1407175]; DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank W. J. Jiang, S. Zhang, W. Zhang, and M. P. Smylie for critical comments. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. Z.-L.X. and J.X. were supported by NSF grant no. DMR-1407175. Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the DOE, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 36 TC 9 Z9 9 U1 22 U2 39 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 20 PY 2016 VL 352 IS 6288 SI SI BP 962 EP 966 DI 10.1126/science.aad8037 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM2AK UT WOS:000376147800041 PM 27199423 ER PT J AU Ben-Naim, E Krapivsky, PL Randon-Furling, J AF Ben-Naim, E. Krapivsky, P. L. Randon-Furling, J. TI Maxima of two random walks: universal statistics of lead changes SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE random walks; statistics of maxima; Levy flights AB We investigate statistics of lead changes of the maxima of two discrete-time random walks in one dimension. We show that the average number of lead changes grows as pi(-1) ln t in the long-time limit. We present theoretical and numerical evidence that this asymptotic behavior is universal. Specifically, this behavior is independent of the jump distribution: the same asymptotic underlies standard Brownian motion and symmetric Levy flights. We also show that the probability to have at most n lead changes behaves as t(-1/4)(lnt)(n) for Brownian motion and as t(-beta(mu))(ln t)(n) for symmetric Levy flights with index mu. The decay exponent beta equivalent to beta(mu) varies continuously with the Levy index when 0 < mu < 2, and remains constant beta = 1/4 for mu > 2. C1 [Ben-Naim, E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ben-Naim, E.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Krapivsky, P. L.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Krapivsky, P. L.] Univ Paris Saclay, Inst Phys Theor, F-91191 Gif Sur Yvette, France. [Krapivsky, P. L.] CNRS, F-91191 Gif Sur Yvette, France. [Randon-Furling, J.] Univ Paris 01, SAMM EA 4543, F-75013 Paris, France. RP Ben-Naim, E (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Ben-Naim, E (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. EM pkrapivsky@gmail.com RI Ben-Naim, Eli/C-7542-2009; Krapivsky, Pavel/A-4612-2014 OI Ben-Naim, Eli/0000-0002-2444-7304; FU INFN; US-DOE [DE-AC52-06NA25396] FX We benefited from discussions with S N Majumdar. We are grateful to the referee for extremely helpful comments and suggestions. Two of us (PLK and JRF) thank the Galileo Galilei Institute for Theoretical Physics for hospitality during the program on 'Statistical Mechanics, Integrability and Combinatorics' and the INFN for partial support. The work of EBN was supported through US-DOE grant DE-AC52-06NA25396. NR 40 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD MAY 20 PY 2016 VL 49 IS 20 AR 205003 DI 10.1088/1751-8113/49/20/205003 PG 13 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA DK2SP UT WOS:000374765000005 ER PT J AU Friar, JL Goldman, T Perez-Mercader, J AF Friar, J. L. Goldman, T. Perez-Mercader, J. TI Ubiquity of Benford's law and emergence of the reciprocal distribution SO PHYSICS LETTERS A LA English DT Article DE Benford/Reciprocal distribution; Information/Communication theory; Iteration theory ID NUMBERS AB We apply the Law of Total Probability to the construction of scale-invariant probability distribution functions (pdfs), and require that probability measures be dimensionless and unitless under a continuous change of scales. If the scale-change distribution function is scale invariant then the constructed distribution will also be scale invariant. Repeated application of this construction on an arbitrary set of (normalizable) pdfs results again in scale-invariant distributions. The invariant function of this procedure is given uniquely by the reciprocal distribution, suggesting a kind of universality. We separately demonstrate that the reciprocal distribution results uniquely from requiring maximum entropy for size class distributions with uniform bin sizes. (C) 2016 Elsevier B.V. All rights reserved. C1 [Friar, J. L.; Goldman, T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Perez-Mercader, J.] Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA. [Perez-Mercader, J.] Santa Fe Inst, 1399 Hyde Pk Rd, Santa Fe, NM 87501 USA. RP Perez-Mercader, J (reprint author), Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA. EM friar@lanl.gov; tjgoldman@post.harvard.edu; jperezmercader@fas.harvard.edu OI Perez-Mercader, Juan/0000-0001-6278-9068 FU everis Foundation; Repsol; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396] FX One of us (JP-M) would like to thank the everis Foundation and Repsol for generous support, and the Theoretical Division of Los Alamos National Laboratory for its hospitality. This work was carried out in part under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 31 TC 0 Z9 0 U1 2 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9601 EI 1873-2429 J9 PHYS LETT A JI Phys. Lett. A PD MAY 20 PY 2016 VL 380 IS 22-23 BP 1895 EP 1899 DI 10.1016/j.physleta.2016.03.045 PG 5 WC Physics, Multidisciplinary SC Physics GA DL3EC UT WOS:000375516000002 ER PT J AU Kong, LB Hasanbeigi, A Price, L AF Kong, Lingbo Hasanbeigi, Ali Price, Lynn TI Assessment of emerging energy-efficiency technologies for the pulp and paper industry: a technical review SO JOURNAL OF CLEANER PRODUCTION LA English DT Review DE Emerging energy-efficiency technology; Energy saving; CO2 emissions; Pulp and paper industry ID DISK MEMBRANE MODULE; KRAFT BLACK LIQUOR; PRE-EXTRACTION; HEMICELLULOSE EXTRACTION; PROCESS INTEGRATION; BIOFUEL PRODUCTION; BIOREFINERY; ULTRAFILTRATION; MILLS; BOARD AB The pulp and paper industry accounts for approximately 5% of total industrial energy consumption and contributes 2% of direct carbon dioxide (CO2) emissions from industries. World paper and paperboard demand and production are increasing significantly, leading to an increase in this sector's energy use and CO2 emissions. Although current studies identify a wide range of energy-efficiency technologies that have already been commercialized for the pulp and paper industry, information is limited or scattered regarding new energy-efficiency technologies that are not yet fully commercialized. Development of emerging or advanced energy-efficiency technologies and their deployment in the market will be crucial for this industry's mid- and long-term energy saving and climate change mitigation strategies. This paper compiles available information on energy savings, environmental and other benefits, costs, and commercialization status for 25 emerging technologies to reduce the energy use and CO2 emissions. The purpose is to provide a well-structured comprehensive review on these emerging energy-efficiency technologies for engineers, researchers, investors, policy makers, pulp and/or paper companies, and other interested parties. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Kong, Lingbo] Tianjin Univ Sci & Technol, Tianjin Key Lab Pulp & Paper, Tianjin 300457, Peoples R China. [Kong, Lingbo; Hasanbeigi, Ali; Price, Lynn] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, Berkeley, CA 94720 USA. [Kong, Lingbo] S China Univ Technol, State Key Lab Pulp & Paper Engn, Guangzhou 510640, Guangdong, Peoples R China. RP Kong, LB (reprint author), Tianjin Univ Sci & Technol, Tianjin Key Lab Pulp & Paper, Tianjin 300457, Peoples R China. EM Lingbo.Kung@gmail.com; AHasanbeigi@lbl.gov; LKPrice@lbl.gov RI Kong, Lingbo/E-1209-2013 OI Kong, Lingbo/0000-0002-6067-3763 FU China Sustainable Energy Program of the Energy Foundation; Dow Chemical Company (through a charitable contribution) through the U.S. Department of Energy [DE-AC02-05CH11231]; State Key Laboratory of Pulp and Paper Engineering, South China University of Technology [201422] FX This work was supported by the China Sustainable Energy Program of the Energy Foundation and Dow Chemical Company (through a charitable contribution) through the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, was also acknowledged for the project (201422). We are thankful to Ron Brown from Agenda 2020 Technology Alliance, Reid Miner and Barry Malmberg from National Council for Air and Steam Improvement, and Bhima Sastri from the U.S. Department of Energy for their valuable comments on the earlier version of this study. We also would like to thank the four anonymous reviewers for their helpful comments and suggestions. NR 176 TC 9 Z9 9 U1 14 U2 29 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-6526 EI 1879-1786 J9 J CLEAN PROD JI J. Clean Prod. PD MAY 20 PY 2016 VL 122 BP 5 EP 28 DI 10.1016/j.jclepro.2015.12.116 PG 24 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental; Environmental Sciences SC Science & Technology - Other Topics; Engineering; Environmental Sciences & Ecology GA DK8FM UT WOS:000375162600003 ER PT J AU Neuhauser, D Rabani, E Cytter, Y Baer, R AF Neuhauser, Daniel Rabani, Eran Cytter, Yael Baer, Roi TI Stochastic Optimally Tuned Range-Separated Hybrid Density Functional Theory SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID BAND-GAPS; ENERGY; APPROXIMATION; SEMICONDUCTORS; NANOCRYSTALS; EXCITATIONS; INSULATORS; ELECTRONS; SYSTEMS; CHARGE AB We develop a stochastic formulation of the optimally tuned range-separated hybrid density functional theory that enables significant reduction of the computational effort and scaling of the nonlocal exchange, operator at the price of introducing a controllable statistical error. Our method is based on stochastic representations of the Coulomb convolution integral and of the generalized Kohn-Sham density matrix. The computational cost of the approach is similar to that of usual Kohn-Sham density functional theory, yet it provides a much more accurate description of the quasiparticle energies for the frontier orbitals. This is illustrated for a series of silicon nanocrystals up to sizes exceeding 3000 electrons. Comparison with the stochastic GW many-body perturbation technique indicates excellent agreement for the fundamental band gap energies, good agreement for the band edge quasiparticle excitations, and very low statistical errors in the total energy for large systems. The present approach has a major advantage over one-shot GW by providing a self-consistent Hamiltonian that is central for additional postprocessing, for example, in the stochastic Bethe-Salpeter approach. C1 [Neuhauser, Daniel] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Rabani, Eran] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Rabani, Eran] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Rabani, Eran] Tel Aviv Univ, Sadder Ctr Computat Mol & Mat Sci, IL-69978 Tel Aviv, Israel. [Cytter, Yael; Baer, Roi] Hebrew Univ Jerusalem, Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel. RP Neuhauser, D (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.; Rabani, E (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Rabani, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Rabani, E (reprint author), Tel Aviv Univ, Sadder Ctr Computat Mol & Mat Sci, IL-69978 Tel Aviv, Israel.; Baer, R (reprint author), Hebrew Univ Jerusalem, Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel. EM dxn@chem.ucla.edu; eran.rabani@berkeley.edu; roi.baer@huji.ac.il FU Israel Science Foundation-FIRST Program [1700/14]; NSF [CHE-1112500, CHE-1465064] FX R.B. and E.R. gratefully thank the Israel Science Foundation-FIRST Program (Grant No. 1700/14). R.B. gratefully acknowledges support for his sabbatical visit by the Pitzer Center and the Kavli Institute of the University of California, Berkeley. D.N. and E.R. acknowledge support by the NSF, Grants CHE-1112500 and CHE-1465064, respectively. We dedicate this paper to Prof. Ronnie Kosloff from the Hebrew University to acknowledge his important contributions to the field of computational/theoretical chemistry. Kosloff has been our teacher and mentor for many years and his methods, such as the Chebyshev expansions and Fourier grids, were used extensively in our present work as well. NR 72 TC 1 Z9 1 U1 4 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2016 VL 120 IS 19 BP 3071 EP 3078 DI 10.1021/acs.jpca.5b10573 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DM5VC UT WOS:000376417300015 PM 26651840 ER PT J AU Zaster, S Bittner, ER Piryatinski, A AF Zaster, Svitlana Bittner, Eric R. Piryatinski, Andrei TI Quantum Symmetry Breaking of Exciton/Polaritons in a Metal-Nanorod Plasmonic Array SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SEMICONDUCTOR MICROCAVITY; EXCITON-POLARITONS; COHERENCE; SUPERRADIANCE; CRYSTALS AB We study the collective, superradiant behavior in the system of emitter-dressed Ag nanorods. Starting from the Drude model for the plasmon oscillations, we arrive at a semiempirical Hamiltonian describing the coupling between quantized surface plasmon modes and the quantum emitters that can be controlled by manipulating their geometry, spacing, and orientation. Further, identifying the lowest polariton mode as SP-states dressed by excitons in the vicinity of k = 0, we examine conditions allowing for the polariton quantum-phase transition. Though the system is formally a 1D array, we show that the polariton states of interest can undergo a quantum-phase transition to form a Bose condensate at finite temperatures for physically accessible parameter ranges. C1 [Zaster, Svitlana; Bittner, Eric R.] Univ Houston, Dept Chem, Univ Pk, Houston, TX 77204 USA. [Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Bittner, ER (reprint author), Univ Houston, Dept Chem, Univ Pk, Houston, TX 77204 USA.; Piryatinski, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM bittner@uh.edu; apiryat@lanl.gov RI Piryatinski, Andrei/B-5543-2009 FU National Science Foundation [CHE-1362006]; Robert A. Welch Foundation [E-1337]; Los Alamos Directed Research and Development (LDRD) funds FX The work at the University of Houston was funded in part by the National Science Foundation (CHE-1362006) and the Robert A. Welch Foundation (E-1337). The work at Los Alamos National Lab was funded by the Los Alamos Directed Research and Development (LDRD) funds. NR 38 TC 0 Z9 0 U1 9 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2016 VL 120 IS 19 BP 3109 EP 3116 DI 10.1021/acs.jpca.5b10726 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DM5VC UT WOS:000376417300019 PM 26905014 ER PT J AU Warrick, ER Cao, W Neumark, DM Leone, SR AF Warrick, Erika R. Cao, Wei Neumark, Daniel M. Leone, Stephen R. TI Probing the Dynamics of Rydberg and Valence States of Molecular Nitrogen with Attosecond Transient Absorption Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID POTENTIAL-ENERGY CURVES; THRESHOLD PHOTOELECTRON; LASER CONTROL; AB-INITIO; PULSES; SPECTRUM; N-2; LIGHT; N2; PHOTOABSORPTION AB An attosecond pulse is used to create a wavepacket in molecular nitrogen composed of multiple-bound and autoionizing electronic states of Rydberg and valence character between 12 and 16.7 eV. A time-delayed,, few-femtosecond, near-infrared (NIR) laser pulse is used to couple individual state in the wavepacket to multiple neighboring states, resulting in time-dependent modification of the absorption spectrum and revealing both individual quantum beats of the wavepacket and the energy shifts of the excited states in the presence of the strong NIR field: The broad bandwidth of the attosecond pulse and high energy,resolution of the extreme ultraviolet spectrometer allow the simultaneous Observation of time-dependent dynamics cot many, individual vibrational levels in each electronic state. Quantum beating with periods from. 1.3 to 12 fs and transient line shape changes are observed among vibrational levels of a progression of electronically autoionizing Rydberg states leading to the excited A (IIu)-I-2 N-2(+) ion core. Vibrational levels in the valence b (IIu)-I-1 state exhibit 50 fs oscillation periods, revealing superpositions between individual vibrational levels within this state. Comparisons are, made to previous studies of electronic wavepackets in atoms that highlight similarities to atomic behavior yet illustrate unique contributions of the diatomic molecular structure to the wavepacket, including the influence of different electronic potentials and vibrational-level-specific electronic dynamics. C1 [Warrick, Erika R.; Cao, Wei; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Warrick, Erika R.; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Neumark, DM; Leone, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Neumark, DM; Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Leone, SR (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu; srl@berkeley.edu RI cao, wei/D-9643-2015; Neumark, Daniel/B-9551-2009; OI Neumark, Daniel/0000-0002-3762-9473; Warrick, Erika/0000-0003-0637-7645 FU Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under contract no. DE-AC02-05CH11231. NR 68 TC 8 Z9 8 U1 7 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2016 VL 120 IS 19 BP 3165 EP 3174 DI 10.1021/acs.jpca.5b11570 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DM5VC UT WOS:000376417300024 PM 26862883 ER PT J AU Sapir, L Stanley, CB Harries, D AF Sapir, Liel Stanley, Christopher B. Harries, Daniel TI Properties of Polyvinylpyrrolidone in a Deep Eutectic Solvent SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ANGLE NEUTRON-SCATTERING; AQUEOUS POLYMER-SOLUTIONS; EQUATION-OF-STATE; IONIC LIQUIDS; THERMODYNAMIC PROPERTIES; CHOLINE CHLORIDE; LIGHT-SCATTERING; FLEXIBLE POLYMERS; MIXTURES; DNA AB Deep eutectic solvents (DES) are mixtures of two or more components with high melting temperatures, which form a liquid at room temperature. These DES hold great promise as green solvents for chemical processes, as they are inexpensive and environmentally friendly. Specifically, they present a unique solvating environment to polymers that is different from water. Here, we use small angle neutron scattering to study the polymer properties of the common, water-soluble, polyvinylpyrrolidone (PVP) in the prominent DES formed by a 1:2 molar mixture of choline chloride and urea. We find that the polymer adopts a slightly different structure in DES than in water, so that at higher concentrations the polymer favors a more expanded conformation compared to the same concentration in water. Yet, the osmotic pressure of PVP solutions in DES is very similar to that in water, indicating that both solvents are of comparable quality and that the DES components interact favorably with PVP. The osmotic pressure measurements within this novel class of promising solvents should be of value toward future technological applications as well as for osmotic stress experiments in nonaqueous environments. C1 [Sapir, Liel; Harries, Daniel] Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel. [Sapir, Liel; Harries, Daniel] Hebrew Univ Jerusalem, Fritz Haber Res Ctr, IL-91904 Jerusalem, Israel. [Stanley, Christopher B.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Harries, D (reprint author), Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel.; Harries, D (reprint author), Hebrew Univ Jerusalem, Fritz Haber Res Ctr, IL-91904 Jerusalem, Israel.; Stanley, CB (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM stanleycb@ornl.gov; daniel.harries@mail.huji.ac.il OI Stanley, Christopher/0000-0002-4226-7710 FU International Network Grant of the Leverhulme Trust; Aharon and Ephraim Katzir Fellowship of the Batsheva de Rothschild Fund; US Israel Binational Science Foundation (BSF); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Israel Academy of Sciences and Humanities; Minerva Foundation, Munich, Germany FX We thank Werner Kunz for introducing us to DES. The authors thank Uri Raviv for allowing us use of the osmometer and for his continuing support. This project was supported by the International Network Grant of the Leverhulme Trust. L.S.'s travel to ORNL was funded through the Aharon and Ephraim Katzir Fellowship of the Batsheva de Rothschild Fund and through the R. Rahamimoff travel grant program of the US Israel Binational Science Foundation (BSF). A portion of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. L.S. is supported by the Adams Fellowship Program of the Israel Academy of Sciences and Humanities. The Fritz Haber Research Center is supported by the Minerva Foundation, Munich, Germany. NR 51 TC 0 Z9 0 U1 11 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 19 PY 2016 VL 120 IS 19 BP 3253 EP 3259 DI 10.1021/acs.jpca.5b11927 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DM5VC UT WOS:000376417300034 PM 26963367 ER PT J AU Ye, YF Kawase, A Song, MK Feng, BM Liu, YS Marcus, MA Feng, J Fang, HT Cairns, EJ Zhu, JF Guo, JH AF Ye, Yifan Kawase, Ayako Song, Min-Kyu Feng, Bingmei Liu, Yi-Sheng Marcus, Matthew A. Feng, Jun Fang, Haitao Cairns, Elton J. Zhu, Junfa Guo, Jinghua TI X-ray Absorption Spectroscopic Characterization of the Synthesis Process: Revealing the Interactions in Cetyltrimethylammonium Bromide-Modified Sulfur-Graphene Oxide Nanocomposites SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-S BATTERIES; LITHIUM/SULFUR BATTERIES; PERFORMANCE; CATHODE; CELL; TEMPERATURE; SPECIATION; ANODE; ION AB We have investigated the chemical bonding interaction of S in a CTAB (cetyltrimethylammonium bromide, CH3(CH2)(15)N+(CH3)(3)Br-)-modified sulfur-graphene oxide (S-GO) nanocomposite used as the cathode material for Li/S cells by S K-edge X-ray absorption spectroscopy (XAS). The results show that the introduction of CTAB to the S-GO nanocomposite and changes in the synthesis recipe including alteration of the S precursor ratios and the sequence of mixing ingredients lead to the formation of different S species. CTAB modifies the cathode materials through bonding with Na2Sx in the precursor solution, which is subsequently converted to C-S bonds during the heat treatment at 155 degrees C. Moreover, GO bonds with CTAB and acts as the nucleation center for S precipitation. All these interactions among S, CTAB, and GO help to immobilize the sulfur in the cathode and may be responsible for the enhanced cell cycle life of CTAB-S-GO nanocomposite-based Li/S cells. C1 [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. [Ye, Yifan; Zhu, Junfa] Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Peoples R China. [Ye, Yifan; Feng, Bingmei; Liu, Yi-Sheng; Marcus, Matthew A.; Feng, Jun; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kawase, Ayako; Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Kawase, Ayako; Cairns, Elton J.] Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA. [Song, Min-Kyu] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Feng, Bingmei; Fang, Haitao] Harbin Inst Technol, Sch Mat Sci & Engn, Harbin 150001, Peoples R China. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. RP Zhu, JF (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China.; Zhu, JF (reprint author), Univ Sci & Technol China, Collaborat Innovat Ctr Suzhou Nano Sci & Technol, Hefei 230029, Peoples R China.; Guo, JH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.; Cairns, EJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA.; Cairns, EJ (reprint author), Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA.; Guo, JH (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. EM ejcairns@lbl.gov; jfzhu@ustc.edu.cn; jguo@lbl.gov RI Zhu, Junfa/E-4020-2010; OI Zhu, Junfa/0000-0003-0888-4261; Cairns, Elton/0000-0002-1179-7591 FU National Basic Research Program of China [2013CB834605]; National Natural Science Foundation of China [U1232102, 21173200, 21473178]; Scientific Research and Users with Potential Grants of Hefei Science Center of CAS [2015SRG-HSC031, 2015HSC-UP022]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; ALS Doctoral Fellowship FX We thank Wayne Stolte, Josep Roque-Rosell, Sirine Fakra, and Richard Celestre for the technical support at the ALS beamlines. J.Z. gratefully acknowledges the financial support from the National Basic Research Program of China (2013CB834605), the National Natural Science Foundation of China (U1232102, 21173200, 21473178), and Scientific Research and Users with Potential Grants of Hefei Science Center of CAS (2015SRG-HSC031, 2015HSC-UP022). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Y.Y. thanks the support of ALS Doctoral Fellowship. NR 30 TC 1 Z9 1 U1 15 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2016 VL 120 IS 19 BP 10111 EP 10117 DI 10.1021/acs.jpcc.6b00751 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DM5VE UT WOS:000376417500001 ER PT J AU Boschen, JS Lee, J Windus, TL Evans, JW Liu, DJ AF Boschen, Jeffery S. Lee, Jiyoung Windus, Theresa L. Evans, James W. Liu, Da-Jiang TI Size Dependence of S-bonding on (111) Facets of Cu Nanoclusters SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EFFECTIVE CORE POTENTIALS; AUGMENTED-WAVE METHOD; SIMPLE METAL-CLUSTERS; MOLECULAR CALCULATIONS; BASIS-SET; DENSITY; SULFUR; NANOPARTICLES; ENERGY; ATOMS AB We demonstrate a strong damped oscillatory size dependence of the adsorption energy for sulfur on the (111) facets of tetrahedral Cu nanoclusters up to sizes of similar to 300 atoms. This behavior reflects quantum size effects. Consistent results are obtained from density functional theory analyses utilizing either atomic orbital or plane-wave bases and using the same Perdew-Burke-Ernzerhof functional. Behavior is interpreted via molecular orbitals (MO), density of states (DOS), and crystal orbital Hamilton population (COHP) analyses. C1 [Boschen, Jeffery S.; Lee, Jiyoung; Windus, Theresa L.; Evans, James W.; Liu, Da-Jiang] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Boschen, Jeffery S.; Lee, Jiyoung; Windus, Theresa L.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Evans, James W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Liu, DJ (reprint author), Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. EM dajiang@ameslab.gov FU U.S. Department of Energy (U.S. DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program; U.S. DOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (U.S. DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program. We acknowledge use of NERSC computational resources. The work was performed at Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 55 TC 2 Z9 2 U1 6 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2016 VL 120 IS 19 BP 10268 EP 10274 DI 10.1021/acs.jpcc.6b00829 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DM5VE UT WOS:000376417500019 ER PT J AU Dholabhai, PP Perriot, R Uberuaga, BP AF Dholabhai, Pratik P. Perriot, Romain Uberuaga, Blas P. TI Atomic-Scale Structure and Stability of the Low-Index Surfaces of Pyrochlore Oxides SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID IONIC-ELECTRONIC CONDUCTION; VAPOR-SOLID REACTION; RADIATION TOLERANCE; COMPLEX OXIDES; NUCLEAR-WASTE; FUEL-CELLS; SIMULATION; TEMPERATURE; ADSORPTION; CHEMISTRY AB The multifunctional properties of complex ternary oxides such as pyrochlores are often influenced by surface structure. Optimizing the surface-driven attributes of these materials necessitates a detailed understanding of the structure and chemical composition of those surfaces. Here we report atomistic simulations elucidating the diverse atomic-scale structures of a set of low-index surfaces [(100), (110), (111), and (112)] in pyrochlore compounds as a function of both A and B cation chemistry. In pyrochlores, the low-index facets are all dipolar, requiring the introduction of surface defects to eliminate the surface dipole. We find that, due to the corresponding higher coordination of the surface cations, the (110) facet is the most energetically stable in all of the compounds considered, an interesting contrast to fluorite, in which the (111) surface is most stable. We also reveal a correlation between the surface energy and the energy to disorder the pyrochlore as a function of B cation chemistry, implying a similar physical origin for the two phenomena. Further, we find that surface rumpling is common across all pyrochlore compounds. An even more interesting feature emerging at these surfaces is the formation of extended structural defects such as steps and trenches, which are found to be stable after high-temperature annealing. As the formation of these features is a consequence of surface defects introduced to eliminate the surface dipole, we propose that the superior surface properties of materials of pyrochlores are due to these extended structural features, which are a direct consequence of the inherent dipole at the surfaces. C1 [Dholabhai, Pratik P.; Perriot, Romain; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87545 USA. RP Dholabhai, PP (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87545 USA. EM pdholabhai@lanl.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [2013LANL8400]; UC Lab Fees Research Program [12-LF-239032]; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396] FX The authors are grateful to Christopher R. Stanek, David A. Andersson, and Kurt E. Sickafus for insightful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Award Number 2013LANL8400. P.P.D. acknowledges support by UC Lab Fees Research Program 12-LF-239032. This research used resources provided by the LANL Institutional Computing Program. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. NR 88 TC 1 Z9 1 U1 9 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2016 VL 120 IS 19 BP 10485 EP 10499 DI 10.1021/acs.jpcc.6b02847 PG 15 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DM5VE UT WOS:000376417500041 ER PT J AU Kwizera, EA Chaffin, E Shen, X Chen, JY Zou, Q Wu, ZM Gai, Z Bhana, S O'Connor, R Wang, LJ Adhikari, H Mishra, SR Wang, YM Huang, XH AF Kwizera, Elyahb Allie Chaffin, Elise Shen, Xiao Chen, Jingyi Zou, Qiang Wu, Zhiming Gai, Zheng Bhana, Saheel O'Connor, Ryan Wang, Lijia Adhikari, Hitesh Mishra, Sanjay R. Wang, Yongmei Huang, Xiaohua TI Size- and Shape-Controlled Synthesis and Properties of Magnetic-Plasmonic Core-Shell Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENHANCED RAMAN-SCATTERING; DISCRETE-DIPOLE APPROXIMATION; COATED IRON NANOPARTICLES; FE-AT-AU; GOLD NANORODS; MULTIFUNCTIONAL NANOPARTICLES; OPTICAL-PROPERTIES; CANCER-CELLS; PHOTOTHERMAL DESTRUCTION; OXIDE NANOPARTICLES AB Magnetic-plasmonic core-shell nanomaterials offer a wide range of applications across science, engineering, and biomedical disciplines. However, the ability to synthesize and understand magnetic plasmonic core-shell nanoparticles with tunable sizes and shapes remains very limited. This work reports experimental and computational studies on the synthesis and properties of iron oxide gold core-shell nanoparticles of three different shapes (sphere, popcorn, and star) with controllable sizes (70 to 250 nm). The nanoparticles were synthesized via a seed-mediated growth method in which newly formed gold atoms were added onto gold-seeded iron oxide octahedrons to form a gold shell. The evolution of the shell into different shapes was found to occur after the coalescence of gold seeds, which was achieved by controlling the amount of additive (silver nitrate) and reducing agent (ascorbic acid) in the growth solution. First-principles calculation, together with experimental results, elucidated the intimate roles of thermodynamic and kinetic parameters in the shape-controlled synthesis. Both discrete dipole approximation calculation and experimental results showed that the nanopopcorns and nanostars exhibited red-shifted plasmon resonance compared with the nanospheres, with the nanostars giving multispectral feature. This research has made a great step further in manipulating and understanding magnetic plasmonic hybrid nanostructures and will make an important impact in many different fields. C1 [Kwizera, Elyahb Allie; Chaffin, Elise; Bhana, Saheel; O'Connor, Ryan; Wang, Yongmei; Huang, Xiaohua] Univ Memphis, Dept Chem, Memphis, TN 38152 USA. [Shen, Xiao; Wang, Lijia; Adhikari, Hitesh; Mishra, Sanjay R.] Univ Memphis, Dept Phys & Mat Sci, Memphis, TN 38152 USA. [Chen, Jingyi] Univ Arkansas, Dept Chem, Fayetteville, AR 72071 USA. [Zou, Qiang; Wu, Zhiming; Gai, Zheng] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wang, YM; Huang, XH (reprint author), Univ Memphis, Dept Chem, Memphis, TN 38152 USA. EM ywang@memphis.edu; xhuang4@memphis.edu RI Gai, Zheng/B-5327-2012; Wang, Yongmei/B-7071-2008; Chen, Jingyi/E-7168-2010; OI Gai, Zheng/0000-0002-6099-4559; Chen, Jingyi/0000-0003-0012-9640; Zou, Qiang/0000-0002-0912-6895 FU National Institutes of Health [1R15 CA 195509-01] FX We gratefully acknowledge the support from the National Institutes of Health (Grant No. 1R15 CA 195509-01). NR 80 TC 2 Z9 2 U1 28 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2016 VL 120 IS 19 BP 10530 EP 10546 DI 10.1021/acs.jpcc.6b00875 PG 17 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DM5VE UT WOS:000376417500046 PM 27239246 ER PT J AU Alam, TM Liao, ZL Nyman, M Yates, J AF Alam, Todd M. Liao, Zuolei Nyman, May Yates, Jonathan TI Insight into Hydrogen Bonding of Uranyl Hydroxide Layers and Capsules by Use of H-1 Magic-Angle Spinning NMR Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PROTON-MAGNETIC-RESONANCE; X-RAY-DIFFRACTION; SOLID-STATE; AQUEOUS-SOLUTION; CHEMICAL-SHIFTS; DEHYDRATED SCHOEPITE; CRYSTAL-STRUCTURE; HIGH-TEMPERATURE; PEROXIDE; DYNAMICS AB Solid-state H-1 magic-angle spinning (MAS) NMR was used to investigate local proton environments in anhydrous [UO2(OH)(2)] (alpha-UOH) and hydrated uranyl hydroxide [(UO2)(4)O(OH)(6)center dot 5H(2)O (metaschoepite). For the metaschoepite material, proton resonances of the mu(2)-OH hydroxyl and interlayer waters were resolved, with two-dimensional (2D) double-quantum (DQ) H-1-H-1 NMR correlation experiments revealing strong dipolar interactions between these different proton species. The experimental NMR results were combined with first-principles CASTEP GIPAW (gauge including projector-augmented wave) chemical shift calculations to develop correlations between hydrogen bond strength and observed H-1 NMR chemical shifts. These NMR correlations allowed characterization of local hydrogen-bond environments in uranyl U-24 capsules and of changes in hydrogen bonding that occurred during thermal dehydration of metaschoepite. C1 [Alam, Todd M.] Sandia Natl Labs, Dept Organ Mat Sci, Albuquerque, NM 87185 USA. [Liao, Zuolei; Nyman, May] Oregon State Univ, Dept Chem & Mat, Corvallis, OR 97331 USA. [Yates, Jonathan] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England. RP Alam, TM (reprint author), Sandia Natl Labs, Dept Organ Mat Sci, Albuquerque, NM 87185 USA. EM tmalam@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Materials Science of Actinides, an Energy Frontier Research Center - Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001089] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, of the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The work at Oregon State University was funded by the Materials Science of Actinides, an Energy Frontier Research Center funded by the Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001089. We are also indebted to Professor Sergey Ostanin for providing the ab initio relaxed schoepite structure from ref 40, used for GIPAW NMR calculations. NR 52 TC 0 Z9 0 U1 11 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 19 PY 2016 VL 120 IS 19 BP 10675 EP 10685 DI 10.1021/acs.jpcc.6b02692 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DM5VE UT WOS:000376417500061 ER PT J AU Dowgiallo, AM Mistry, KS Johnson, JC Reid, OG Blackburn, JL AF Dowgiallo, Anne-Marie Mistry, Kevin S. Johnson, Justin C. Reid, Obadiah G. Blackburn, Jeffrey L. TI Probing Exciton Diffusion and Dissociation in Single-Walled Carbon Nanotube-C-60 Heterojunctions SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID THIN-FILM PHOTOVOLTAICS; SOLAR-CELLS; C-60; LENGTH AB The efficiency of thin-film organic photovoltaic (OPV) devices relies heavily upon the transport of excitons to type-II heterojunction interfaces, where there is sufficient driving force for exciton dissociation and ultimately the formation of charge carriers. Semiconducting single-walled carbon nanotubes (SWCNTs) are strong near-infrared absorbers that form type-II heterojunctions with fullerenes such as C-60. Although the efficiencies of SWCNT-fullerene OPV devices have climbed over the past few years, questions remain regarding the fundamental factors that currently limit their performance. In this study, we determine the exciton diffusion length in the C-60 layer of SWCNT-C-60 bilayer active layers using femtosecond transient absorption measurements. We demonstrate that hole transfer from photoexcited C-60 molecules to SWCNTs can be tracked by the growth of narrow spectroscopic signatures of holes in the SWCNT "reporter layer". In bilayers with thick C-60 layers, the SWCNT charge-related signatures display a slow rise over hundreds of picoseconds, reflecting exciton diffusion through the C-60 layer to the interface. A model based on exciton diffusion with a Beer-Lambert excitation profile, as well as Monte Carlo simulations, gives the best fit to the data as a function of C-60 layer thickness using an exciton diffusion length of approximately 5 nm. C1 [Dowgiallo, Anne-Marie; Mistry, Kevin S.; Johnson, Justin C.; Reid, Obadiah G.; Blackburn, Jeffrey L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Mistry, Kevin S.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Reid, Obadiah G.] Univ Colorado, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. RP Blackburn, JL (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Jeffrey.Blackburn@nrel.gov OI REID, OBADIAH/0000-0003-0646-3981 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC36-08GO28308] FX This work was supported by the Solar Photochemistry Program of the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, under Contract No. DE-AC36-08GO28308 to NREL. NR 33 TC 7 Z9 7 U1 8 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2016 VL 7 IS 10 BP 1794 EP 1799 DI 10.1021/acs.jpclett.6b00604 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM5WL UT WOS:000376421200007 PM 27127916 ER PT J AU Xie, W Lee, YL Shao-Horn, Y Morgan, D AF Xie, Wei Lee, Yueh-Lin Shao-Horn, Yang Morgan, Dane TI Oxygen Point Defect Chemistry in Ruddlesden-Popper Oxides (La1-xSrx)(2)MO4 +/-delta (M = Co, Ni, Cu) SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID NEUTRON-DIFFRACTION; SURFACE EXCHANGE; IONIC TRANSPORT; NONSTOICHIOMETRY; LA2CUO4+DELTA; ENERGETICS; LA2-XSRXNIO4+DELTA; LA2-XSRXCUO4-Y; LA2NIO4+DELTA; STABILITY AB Stability of oxygen point defects in Ruddlesden-Popper oxides (La1-xSrx)(2)MO4 +/-delta (M = Co, Ni, Cu) is studied with density functional theory calculations to determine their stable sites, charge states, and energetics as functions of Sr content (x), transition metal (M), and defect concentration (delta). We demonstrate that the dominant O point defects can change between oxide interstitials, peroxide interstitials, and vacancies. In general, increasing x and atomic number of M stabilizes peroxide over oxide interstitials as well as vacancies over both peroxide and oxide interstitials; increasing delta destabilizes both oxide interstitials and vacancies but barely affects peroxide interstitials. We also demonstrate that the O 2p-band center is a powerful descriptor for these materials and correlates linearly with the formation energy of all defects. The trends of formation energy versus x, M, and delta and the correlation with O 2p-band center are explained in terms of oxidation chemistry and electronic structure. C1 [Xie, Wei; Lee, Yueh-Lin; Morgan, Dane] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Lee, Yueh-Lin; Shao-Horn, Yang] MIT, Electrochem Energy Lab, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Xie, Wei] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Lee, Yueh-Lin] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Morgan, D (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM ddmorgan@wisc.edu RI LEE, YUEH-LIN/F-6274-2011; OI LEE, YUEH-LIN/0000-0003-2477-6412; Xie, Wei/0000-0003-1501-896X FU U.S. Department of Energy (DOE), National Energy Technology Laboratory (NETL), Solid State Energy Conversion Alliance (SECA) Core Technology Program [FE0009435]; NSF Software Infrastructure for Sustained Innovation (SI2) [1148011]; U.S. National Science Foundation [ACI-1053575] FX Initial calculations for this work by Y.-L.L. were supported by the U.S. Department of Energy (DOE), National Energy Technology Laboratory (NETL), Solid State Energy Conversion Alliance (SECA) Core Technology Program with award number FE0009435. The bulk of the calculations, all manuscript development, and all activities by W.X. and D.M. were supported by the NSF Software Infrastructure for Sustained Innovation (SI2) award no. 1148011. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by U.S. National Science Foundation with grant number ACI-1053575. NR 35 TC 2 Z9 2 U1 16 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 19 PY 2016 VL 7 IS 10 BP 1939 EP 1944 DI 10.1021/acs.jpclett.6b00739 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM5WL UT WOS:000376421200031 PM 27157124 ER PT J AU Currier, JM Cheng, WY Menendez, D Conolly, R Chorley, BN AF Currier, Jenna M. Cheng, Wan-Yun Menendez, Daniel Conolly, Rory Chorley, Brian N. TI Developing a Gene Biomarker at the Tipping Point of Adaptive and Adverse Responses in Human Bronchial Epithelial Cells SO PLOS ONE LA English DT Article ID TOXCAST PROGRAM; IN-VITRO; ANTIOXIDANT RESPONSE; RISK-ASSESSMENT; BEAS-2B CELLS; CANCER-CELLS; ZINC; P53; TOXICITY; APOPTOSIS AB Determining mechanism-based biomarkers that distinguish adaptive and adverse cellular processes is critical to understanding the health effects of environmental exposures. Shifting from in vivo, low-throughput toxicity studies to high-throughput screening (HTS) paradigms and risk assessment based on in vitro and in silico testing requires utilizing toxicity pathway information to distinguish adverse outcomes from recoverable adaptive events. Little work has focused on oxidative stresses in human airway for the purposes of predicting adverse responses. We hypothesize that early gene expression-mediated molecular changes could be used to delineate adaptive and adverse responses to environmentally-based perturbations. Here, we examined cellular responses of the tracheobronchial airway to zinc (Zn) exposure, a model oxidant. Airway derived BEAS-2B cells exposed to 2-10 mu M Zn2+ elicited concentration-and time-dependent cytotoxicity. Normal, adaptive, and cytotoxic Zn2+ exposure conditions were determined with traditional apical endpoints, and differences in global gene expression around the tipping point of the responses were used to delineate underlying molecular mechanisms. Bioinformatic analyses of differentially expressed genes indicate early enrichment of stress signaling pathways, including those mediated by the transcription factors p53 and NRF2. After 4 h, 154 genes were differentially expressed (p < 0.01) between the adaptive and cytotoxic Zn2+ concentrations. Nearly 40% of the biomarker genes were related to the p53 signaling pathway with 30 genes identified as likely direct targets using a database of p53 ChIP-seq studies. Despite similar p53 activation profiles, these data revealed widespread dampening of p53 and NRF2-related genes as early as 4 h after exposure at higher, unrecoverable Zn2+ exposures. Thus, in our model early increased activation of stress response pathways indicated a recoverable adaptive event. Overall, this study highlights the importance of characterizing molecular mechanisms around the tipping point of adverse responses to better inform HTS paradigms. C1 [Currier, Jenna M.; Cheng, Wan-Yun] US EPA, Oak Ridge Inst Sci & Educ, Res Triangle Pk, NC 27711 USA. [Menendez, Daniel] NIEHS, Genome Integr & Struct Biol Lab, NIH, POB 12233, Res Triangle Pk, NC 27709 USA. [Conolly, Rory; Chorley, Brian N.] US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC 27711 USA. RP Chorley, BN (reprint author), US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC 27711 USA. EM chorley.brian@epa.gov FU United States Environmental Protection Agency, Office of Research and Development; Oak Ridge Institute for Science and Education Research/Participation Program at the US Environmental Protection Agency FX This work was supported by intramural funding by the United States Environmental Protection Agency, Office of Research and Development.; JMC and W-YC were supported by the Oak Ridge Institute for Science and Education Research/Participation Program at the US Environmental Protection Agency. This manuscript has been reviewed by the National Health and Environmental Effects Research Laboratory and approved for publication. The content does not necessarily reflect the views of the US EPA nor does mention of trade names or commercial products constitute endorsement or recommendation for use. NR 64 TC 0 Z9 0 U1 1 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 19 PY 2016 VL 11 IS 5 AR e0155875 DI 10.1371/journal.pone.0155875 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM4BR UT WOS:000376291100124 PM 27195669 ER PT J AU Colegrove, E Harvey, SP Yang, JH Burst, JM Albin, DS Wei, SH Metzger, WK AF Colegrove, Eric Harvey, Steven P. Yang, Ji-Hui Burst, James M. Albin, David S. Wei, Su-Huai Metzger, Wyatt K. TI Phosphorus Diffusion Mechanisms and Deep Incorporation in Polycrystalline and Single-Crystalline CdTe SO PHYSICAL REVIEW APPLIED LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; SOLAR-CELLS; EFFICIENCY; SEMICONDUCTORS; ACCEPTOR AB A key challenge in cadmium-telluride (CdTe) semiconductors is obtaining stable and high hole density. Group-I elements substituting Cd can form acceptors but easily self-compensate and diffuse quickly. For example, CdTe photovoltaics have relied on copper as a dopant, but this creates stability problems and hole density that has not exceeded 10(15) cm(-3). If hole density can be increased beyond 10(16) cm(-3), CdTe solar technology can exceed multicrystalline silicon performance and provide levelized costs of electricity below conventional energy sources. Group-V elements substituting Te offer a solution, but they are very difficult to incorporate. Using time-of-flight secondary-ion mass spectrometry, we examine bulk and grain-boundary diffusion of phosphorus (P) in CdTe in Cd-rich conditions. We find that in addition to slow bulk diffusion and fast grain-boundary diffusion, there is a critical fast bulk-diffusion component that enables deep P incorporation in CdTe. Detailed first-principle calculations indicate the slow bulk-diffusion component is caused by substitutional P diffusion through the Te sublattice, whereas the fast bulk-diffusion component is caused by P diffusing through interstitial lattice sites following the combination of a kick-out step and two rotation steps. The latter is limited in magnitude by high formation energy, but is sufficient to manipulate P incorporation. In addition to an increased physical understanding, these results open up experimental possibilities for group-V doping in CdTe applications. C1 [Colegrove, Eric; Harvey, Steven P.; Yang, Ji-Hui; Burst, James M.; Albin, David S.; Metzger, Wyatt K.] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Wei, Su-Huai] Beijing Computat Sci Res Ctr, Beijing 100193, Peoples R China. RP Colegrove, E (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. FU U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy [DE-AC36-08GO28308] FX This work is supported by the U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, under Contract No. DE-AC36-08GO28308. NR 35 TC 4 Z9 4 U1 7 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD MAY 19 PY 2016 VL 5 IS 5 AR 054014 DI 10.1103/PhysRevApplied.5.054014 PG 7 WC Physics, Applied SC Physics GA DM3VS UT WOS:000376275400001 ER PT J AU Bi, W Lim, J Fabbris, G Zhao, J Haskel, D Alp, EE Hu, MY Chow, P Xiao, Y Xu, W Schilling, JS AF Bi, W. Lim, J. Fabbris, G. Zhao, J. Haskel, D. Alp, E. E. Hu, M. Y. Chow, P. Xiao, Y. Xu, W. Schilling, J. S. TI Magnetism of europium under extreme pressures SO PHYSICAL REVIEW B LA English DT Article ID ANTIFERROMAGNETIC TRANSITION; HYPERFINE INTERACTIONS; SYNCHROTRON-RADIATION; QUANTUM CRITICALITY; HEAVY FERMIONS; METAL YBRH2SI2; SUPERCONDUCTIVITY; MOSSBAUER; SCATTERING; VALENCE AB Using synchrotron-based Mossbauer and x-ray emission spectroscopies, we explore the evolution of magnetism in elemental (divalent) europium as it gives way to superconductivity at extreme pressures. Magnetic order in Eu is observed to collapse just above 80 GPa as superconductivity emerges, even though Eu cations retain their strong local 4f(7) magnetic moments up to 119 GPa with no evidence for an increase in valence. We speculate that superconductivity in Eu may be unconventional and have its origin in magnetic fluctuations, as has been suggested for high-T-c cuprates, heavy fermions, and iron-pnictides. C1 [Bi, W.; Fabbris, G.; Zhao, J.; Haskel, D.; Alp, E. E.; Hu, M. Y.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Bi, W.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA. [Lim, J.; Fabbris, G.; Schilling, J. S.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Lim, J.] Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. [Lim, J.] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Fabbris, G.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. [Chow, P.; Xiao, Y.] Carnegie Inst Sci, Geophys Lab, High Pressure Collaborat Access Team, Argonne, IL 60439 USA. [Xu, W.] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil, Beijing 100049, Peoples R China. RP Bi, W (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA.; Bi, W (reprint author), Univ Illinois, Dept Geol, Urbana, IL 61801 USA. EM wbi@aps.anl.gov RI Xu, Wei/E-2261-2011; Fabbris, Gilberto/F-3244-2011 OI Xu, Wei/0000-0001-8006-2399; Fabbris, Gilberto/0000-0001-8278-4985 FU Consortium for Materials Properties Research in Earth Sciences (COMPRES); National Science Foundation (NSF) [DMR-1104742]; Carnegie/DOE Alliance Center (CDAC) through NNSA/Department of Energy (DOE) Grant [DE-FC52-08NA28554]; DOE Office of Science [DE-AC02-06CH11357] FX We thank M. M. Abd-Elmeguid and W. Sturhahn for helpful discussion. Support by Consortium for Materials Properties Research in Earth Sciences (COMPRES), the National Science Foundation (NSF) through Grant No. DMR-1104742 and by the Carnegie/DOE Alliance Center (CDAC) through NNSA/Department of Energy (DOE) Grant No. DE-FC52-08NA28554 is gratefully acknowledged. This research used resources of the APS, a US DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 61 TC 1 Z9 1 U1 6 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 19 PY 2016 VL 93 IS 18 AR 184424 DI 10.1103/PhysRevB.93.184424 PG 6 WC Physics, Condensed Matter SC Physics GA DM3LJ UT WOS:000376247600003 ER PT J AU Ulvestad, A Tripathi, A Hruszkewycz, SO Cha, W Wild, SM Stephenson, GB Fuoss, PH AF Ulvestad, A. Tripathi, A. Hruszkewycz, S. O. Cha, W. Wild, S. M. Stephenson, G. B. Fuoss, P. H. TI Coherent diffractive imaging of time-evolving samples with improved temporal resolution SO PHYSICAL REVIEW B LA English DT Article ID STRAIN; DYNAMICS; NANOPARTICLES; NANOCRYSTAL; PALLADIUM; HYDROGEN AB Bragg coherent x-ray diffractive imaging is a powerful technique for investigating dynamic nanoscale processes in nanoparticles immersed in reactive, realistic environments. Its temporal resolution is limited, however, by the oversampling requirements of three-dimensional phase retrieval. Here, we show that incorporating the entire measurement time series, which is typically a continuous physical process, into phase retrieval allows the oversampling requirement at each time step to be reduced, leading to a subsequent improvement in the temporal resolution by a factor of 2-20 times. The increased time resolution will allow imaging of faster dynamics and of radiation-dose-sensitive samples. This approach, which we call "chrono CDI," may find use in improving the time resolution in other imaging techniques. C1 [Ulvestad, A.; Hruszkewycz, S. O.; Cha, W.; Stephenson, G. B.; Fuoss, P. H.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Tripathi, A.; Wild, S. M.] Argonne Natl Lab, Div Math & Comp Sci, Lemont, IL 60439 USA. RP Ulvestad, A (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. FU US Department of Energy, Office of Science [DE-AC02-06CH11357]; Office of Basic Energy Sciences (BES); Basic Energy Sciences, Division of Materials Sciences and Engineering; Office of Advanced Scientific Computing Research; ROMPR project; Argonne Director's postdoctoral fellowship FX This material was based upon work supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. This research used resources of the Advanced Photon Source, which is a DOE Office of Science User Facility. Work at the Advanced Photon Source was supported by the Office of Basic Energy Sciences (BES). P.H.F., S.O.H., and G.B.S. were supported by Basic Energy Sciences, Division of Materials Sciences and Engineering. A.T. and S.M.W. were supported by the Office of Advanced Scientific Computing Research and the ROMPR project. A.U. was supported by an Argonne Director's postdoctoral fellowship. The authors thank Jesse N. Clark for insightful discussions. NR 27 TC 1 Z9 1 U1 10 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 19 PY 2016 VL 93 IS 18 AR 184105 DI 10.1103/PhysRevB.93.184105 PG 7 WC Physics, Condensed Matter SC Physics GA DM3LJ UT WOS:000376247600001 ER PT J AU Mukhopadhyay, S Sun, JF Subedi, A Siegrist, T Singh, DJ AF Mukhopadhyay, Saikat Sun, Jifeng Subedi, Alaska Siegrist, Theo Singh, David J. TI Competing covalent and ionic bonding in Ge-Sb-Te phase change materials SO SCIENTIFIC REPORTS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; CHANGE MEMORY; ELECTRON-DIFFRACTION; LOCAL-STRUCTURE; CHAIN-STRUCTURE; GE2SB2TE5; AMORPHIZATION; CRYSTALLINE; SEMICONDUCTORS AB Ge2Sb2Te5 and related phase change materials are highly unusual in that they can be readily transformed between amorphous and crystalline states using very fast melt, quench, anneal cycles, although the resulting states are extremely long lived at ambient temperature. These states have remarkably different physical properties including very different optical constants in the visible in strong contrast to common glass formers such as silicates or phosphates. This behavior has been described in terms of resonant bonding, but puzzles remain, particularly regarding different physical properties of crystalline and amorphous phases. Here we show that there is a strong competition between ionic and covalent bonding in cubic phase providing a link between the chemical basis of phase change memory property and origins of giant responses of piezoelectric materials (PbTi3, BiFeO3). This has important consequences for dynamical behavior in particular leading to a simultaneous hardening of acoustic modes and softening of high frequency optic modes in crystalline phase relative to amorphous. This different bonding in amorphous and crystalline phases provides a direct explanation for different physical properties and understanding of the combination of long time stability and rapid switching and may be useful in finding new phase change compositions with superior properties. C1 [Mukhopadhyay, Saikat; Sun, Jifeng] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Sun, Jifeng; Siegrist, Theo] FAMU FSU Coll Engn, Dept Chem & Biomed Engn, Tallahassee, FL 32310 USA. [Subedi, Alaska] Max Planck Inst Struct & Dynam Matter, Hamburg, Germany. [Singh, David J.] Univ Missouri, Dept Phys & Astron, Columbia, MO 65211 USA. RP Mukhopadhyay, S (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM mukhopadhyas@ornl.gov RI Mukhopadhyay, Saikat/B-4402-2011 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; S3TEC an Energy Frontier Research Center - Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001299/DE-FG02-09ER46577]; Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division through the ORNL GO! program; Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0008832] FX SM gratefully acknowledges support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. This work was partially supported as part of S3TEC an Energy Frontier Research Center funded by the Department of Energy, Office of Science, Basic Energy Sciences under award # DE-SC0001299/DE-FG02-09ER46577(DJS). J.S. acknowledges a graduate student fellowship, funded by the Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division through the ORNL GO! program. SM thankfully acknowledges computing resources from Research Services at Boston College and Texas Advanced Computing Center (TACC) at The University of Texas at Austin. Helpful discussions with Dr. Mao-Hua Du are greatly acknowledged. T.S. acknowledges funding by the Department of Energy, Office of Science, Basic Energy Sciences under award #DE-SC0008832. NR 59 TC 2 Z9 2 U1 14 U2 26 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 19 PY 2016 VL 6 AR 25981 DI 10.1038/srep25981 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM5FX UT WOS:000376374200001 PM 27193531 ER PT J AU Ozaki, N Nellis, WJ Mashimo, T Ramzan, M Ahuja, R Kaewmaraya, T Kimura, T Knudson, M Miyanishi, K Sakawa, Y Sano, T Kodama, R AF Ozaki, N. Nellis, W. J. Mashimo, T. Ramzan, M. Ahuja, R. Kaewmaraya, T. Kimura, T. Knudson, M. Miyanishi, K. Sakawa, Y. Sano, T. Kodama, R. TI Dynamic compression of dense oxide (Gd3Ga5O12) from 0.4 to 2.6 TPa: Universal Hugoniot of fluid metals SO SCIENTIFIC REPORTS LA English DT Article ID OF-STATE MEASUREMENTS; AUGMENTED-WAVE METHOD; PRESSURE; CONDUCTIVITY; HYDROGEN; MBAR; GPA AB Materials at high pressures and temperatures are of great current interest for warm dense matter physics, planetary sciences, and inertial fusion energy research. Shock-compression equation-of-state data and optical reflectivities of the fluid dense oxide, Gcl(3)Ga(5)O(12) (GGG), were measured at extremely high pressures up to 2.6TPa (26 Mbar) generated by high-power laser irradiation and magnetically driven hypervelocity impacts. Above 0.75TPa, the GGG Hugoniot data approach/reach a universal linear line of fluid metals, and the optical reflectivity most likely reaches a constant value indicating that GGG undergoes a crossover from fluid semiconductor to poor metal with minimum metallic conductivity (MMC). These results suggest that most fluid compounds, e.g., strong planetary oxides, reach a common state on the universal Hugoniot of fluid metals (UHFM) with MMC at sufficiently extreme pressures and temperatures. The systematic behaviors of warm dense fluid would be useful benchmarks for developing theoretical equation-of-state and transport models in the warm dense matter regime in determining computational predictions. C1 [Ozaki, N.; Kodama, R.] Osaka Univ, Grad Sch Engn, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan. [Ozaki, N.; Miyanishi, K.; Kodama, R.] Osaka Univ, Photon Pioneers Ctr, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan. [Nellis, W. J.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Mashimo, T.] Kumamoto Univ, Shock Wave & Condensed Matter Res Ctr, Kumamoto 8608555, Japan. [Ramzan, M.; Ahuja, R.; Kaewmaraya, T.] Uppsala Univ, Dept Phys & Astron, Condensed Matter Theory Grp, Box 516, SE-75120 Uppsala, Sweden. [Ahuja, R.] KTH Royal Inst Technol, Dept Mat Sci & Engn, Appl Mat Phys, SE-10044 Stockholm, Sweden. [Kimura, T.] Ehime Univ, Geodynam Res Ctr, Matsuyama, Ehime 7908577, Japan. [Knudson, M.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Knudson, M.] Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. [Sakawa, Y.; Sano, T.] Osaka Univ, Inst Laser Engn, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan. [Kodama, R.] Osaka Univ, Inst Acad Initiat, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan. RP Ozaki, N (reprint author), Osaka Univ, Grad Sch Engn, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan.; Ozaki, N (reprint author), Osaka Univ, Photon Pioneers Ctr, 2-2 Yamadaoka, Suita, Osaka 5650871, Japan. EM norimasa.ozaki@eei.eng.osaka-u.ac.jp RI Sano, Takayoshi/E-7860-2010; Kodama, Ryosuke/G-2627-2016; Sakawa, Youichi/J-5707-2016 OI Sakawa, Youichi/0000-0003-4165-1048 FU JSPS KAKENHI [22224012, 25707041]; JSPS; High Power Laser; XFEL; X-ray Free Electron Laser Priority Strategy Program at Osaka University from the Ministry of Education, Culture, Sports, Science and Technology (MEXT); Genesis Research Institute, Inc. (Konpon-ken, TOYOTA); Global COE Programs at the Kumamoto University (Global Initiative Center for High-Rate Impulse-Energy Engineering) from the MEXT; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Y. Kimura for her support with target fabrication. Laser-shock experiments were conducted under the joint research project of the Institute of Laser Engineering, Osaka University. This work was supported in part by JSPS KAKENHI (Grant Nos 22224012 and 25707041), JSPS core-to-core program on International Alliance for Material Science in Extreme States with High Power Laser and XFEL, and the X-ray Free Electron Laser Priority Strategy Program at Osaka University from the Ministry of Education, Culture, Sports, Science and Technology (MEXT). This work was also partially supported by the Genesis Research Institute, Inc. (Konpon-ken, TOYOTA) and by the Global COE Programs at the Kumamoto University (Global Initiative Center for High-Rate Impulse-Energy Engineering) from the MEXT. Sandia Corporation is a wholly owned subsidiary of Lockheed Martin Corporation operated for the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 38 TC 1 Z9 1 U1 3 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 19 PY 2016 VL 6 AR 26000 DI 10.1038/srep26000 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM5FZ UT WOS:000376374400001 PM 27193942 ER PT J AU Pandya, S Damodaran, AR Xu, RJ Hsu, SL Agar, JC Martin, LW AF Pandya, Shishir Damodaran, Anoop R. Xu, Ruijuan Hsu, Shang-Lin Agar, Joshua C. Martin, Lane W. TI Strain-induced growth instability and nanoscale surface patterning in perovskite thin films SO SCIENTIFIC REPORTS LA English DT Article ID LAYER-BY-LAYER; MISFIT DISLOCATIONS; MISMATCHED LAYERS; STEP-FLOW; MORPHOLOGY; DIFFUSION; EPITAXY; NUCLEATION; DEFECTS; PT(111) AB Despite extensive studies on the effects of epitaxial strain on the evolution of the lattice and properties of materials, considerably less work has explored the impact of strain on growth dynamics. In this work, we demonstrate a growth-mode transition from 2D-step flow to self-organized, nanoscale 3D-island formation in PbZr0.2Ti0.8O3/SrRuO3/SrTiO3(001) heterostructures as the kinetics of the growth process respond to the evolution of strain. With increasing heterostructure thickness and misfit dislocation formation at the buried interface, a periodic, modulated strain field is generated that alters the adatom binding energy and, in turn, leads to a kinetic instability that drives a transition from 2D growth to ordered, 3D-island formation. The results suggest that the periodically varying binding energy can lead to inhomogeneous adsorption kinetics causing preferential growth at certain sites. This, in conjunction with the presence of an Ehrlich-Schwoebel barrier, gives rise to long-range, periodically-ordered arrays of so-called "wedding cake" 3D nanostructures which self-assemble along the [100] and [010]. C1 [Pandya, Shishir; Damodaran, Anoop R.; Xu, Ruijuan; Hsu, Shang-Lin; Agar, Joshua C.; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Martin, LW (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Martin, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM lwmartin@berkeley.edu RI Martin, Lane/H-2409-2011 OI Martin, Lane/0000-0003-1889-2513 FU Army Research Office [W911NF-14-1-0104]; National Science Foundation [DMR-1124696, DMR-1451219, CMMI-1434147] FX S.P. and A.R.D. acknowledge support from the Army Research Office under grant W911NF-14-1-0104. R.X. acknowledges support from the National Science Foundation under grant DMR-1124696. J.C.A. acknowledges support from the National Science Foundation under grant DMR-1451219. L.W.M. acknowledges support from the National Science Foundation under grant CMMI-1434147. NR 43 TC 1 Z9 1 U1 17 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 19 PY 2016 VL 6 AR 26075 DI 10.1038/srep26075 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM5GC UT WOS:000376374700001 PM 27194595 ER PT J AU Zwolak, M Riedel, CJ Zurek, WH AF Zwolak, Michael Riedel, C. Jess Zurek, Wojciech H. TI Amplification, Decoherence, and the Acquisition of Information by Spin Environments SO SCIENTIFIC REPORTS LA English DT Article ID QUANTUM DARWINISM; DIAMOND; EINSELECTION; CENTERS AB Quantum Darwinism recognizes the role of the environment as a communication channel: Decoherence can selectively amplify information about the pointer states of a system of interest (preventing access to complementary information about their superpositions) and can make records of this information accessible to many observers. This redundancy explains the emergence of objective, classical reality in our quantum Universe. Here, we demonstrate that the amplification of information in realistic spin environments can be quantified by the quantum Chernoff information, which characterizes the distinguishability of partial records in individual environment subsystems. We show that, except for a set of initial states of measure zero, the environment always acquires redundant information. Moreover, the Chernoff information captures the rich behavior of amplification in both finite and infinite spin environments, from quadratic growth of the redundancy to oscillatory behavior. These results will considerably simplify experimental testing of quantum Darwinism, e.g., using nitrogen vacancies in diamond. C1 [Zwolak, Michael] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. [Riedel, C. Jess] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Riedel, C. Jess] IBM Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Zurek, Wojciech H.] Los Alamos Natl Lab, Div Theoret, MS B213, Los Alamos, NM 87545 USA. RP Zwolak, M (reprint author), Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. EM mpzwolak@gmail.com RI Zwolak, Michael/G-2932-2013 OI Zwolak, Michael/0000-0001-6443-7816 FU Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation; US Department of Energy through the LANL/LDRD Program; John Templeton Foundation; Foundational Questions Institute Grant on "Physics of What Happens" [2015-144057] FX We would like to thank Salomon for color-scheme inspiration and the Center for Integrated Quantum Science and Technology (IQST) and the University of Ulm, where part of this work was carried out. Research at the Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. This research was supported in part by the US Department of Energy through the LANL/LDRD Program and, in part, by the John Templeton Foundation and the Foundational Questions Institute Grant No. 2015-144057 on "Physics of What Happens". NR 38 TC 1 Z9 1 U1 0 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 19 PY 2016 VL 6 AR 25277 DI 10.1038/srep25277 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM5FA UT WOS:000376371900001 PM 27193389 ER PT J AU He, Y Yan, CL Fang, J Inouye, C Tjian, R Ivanov, I Nogales, E AF He, Yuan Yan, Chunli Fang, Jie Inouye, Carla Tjian, Robert Ivanov, Ivaylo Nogales, Eva TI Near-atomic resolution visualization of human transcription promoter opening SO NATURE LA English DT Article ID RNA-POLYMERASE-II; ELONGATION-FACTOR TFIIS; STRUCTURAL BASIS; GENERAL TRANSCRIPTION; PREINITIATION COMPLEX; ELECTRON-MICROSCOPY; INITIATION COMPLEX; CRYSTAL-STRUCTURE; CRYO-EM; CONFORMATIONAL-CHANGES AB In eukaryotic transcription initiation, a large multi-subunit pre-initiation complex (PIC) that assembles at the core promoter is required for the opening of the duplex DNA and identification of the start site for transcription by RNA polymerase II. Here we use cryo-electron microscropy (cryo-EM) to determine near-atomic resolution structures of the human PIC in a closed state (engaged with duplex DNA), an open state (engaged with a transcription bubble), and an initially transcribing complex (containing six base pairs of DNA-RNA hybrid). Our studies provide structures for previously uncharacterized components of the PIC, such as TFIIE and TFIIH, and segments of TFIIA, TFIIB and TFIIF. Comparison of the different structures reveals the sequential conformational changes that accompany the transition from each state to the next throughout the transcription initiation process. This analysis illustrates the key role of TFIIB in transcription bubble stabilization and provides strong structural support for a translocase activity of XPB. C1 [He, Yuan; Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. [He, Yuan] Northwestern Univ, Dept Mol Biosci, Evanston, IL 60208 USA. [Yan, Chunli; Ivanov, Ivaylo] Georgia State Univ, Ctr Diagnost & Therapeut, Dept Chem, Atlanta, GA 30302 USA. [Fang, Jie; Tjian, Robert; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Inouye, Carla; Tjian, Robert] Univ Calif Berkeley, Li Ka Shing Ctr Biomed & Hlth Sci, Berkeley, CA 94720 USA. [Tjian, Robert; Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. RP He, Y; Nogales, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA.; He, Y (reprint author), Northwestern Univ, Dept Mol Biosci, Evanston, IL 60208 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM yuanhe@northwestern.edu; ENogales@lbl.gov OI Ivanov, Ivaylo/0000-0002-5306-1005; He, Yuan/0000-0002-1455-3963 FU NIGMS [GM63072, GM110387]; National Science Foundation [MCB-1149521] FX We thank S. Zheng for providing XPB mAb, D. King for providing peptides, P. Grob and T. Houweling for electron microscopy and computer support, respectively; S. Scheres for advice on image processing, S. Kassube for providing TFIIS, and G. Cardone for advice concerning filtering according to local resolution. This work was funded by NIGMS (GM63072 to E.N. and GM110387 to I. I.) and the National Science Foundation (MCB-1149521 to I. I.). Computational resources were provided in part by XSEDE (CHE110042) and the National Energy Research for Scientific Computing Center (DE-AC02-05CH11231). E.N. and R.T are Howard Hughes Medical Institute Investigators. NR 92 TC 19 Z9 19 U1 8 U2 26 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 19 PY 2016 VL 533 IS 7603 BP 359 EP + DI 10.1038/nature17970 PG 21 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM0AH UT WOS:000376004300041 PM 27193682 ER PT J AU Sauter, NK Echols, N Adams, PD Zwart, PH Kern, J Brewster, AS Koroidov, S Alonso-Mori, R Zouni, A Messinger, J Bergmann, U Yano, J Yachandra, VK AF Sauter, Nicholas K. Echols, Nathaniel Adams, Paul D. Zwart, Petrus H. Kern, Jan Brewster, Aaron S. Koroidov, Sergey Alonso-Mori, Roberto Zouni, Athina Messinger, Johannes Bergmann, Uwe Yano, Junko Yachandra, Vittal K. TI No observable conformational changes in PSII SO NATURE LA English DT Letter ID PHOTOSYSTEM-II; THERMOSYNECHOCOCCUS-ELONGATUS; EVOLUTION C1 [Sauter, Nicholas K.; Echols, Nathaniel; Adams, Paul D.; Zwart, Petrus H.; Kern, Jan; Brewster, Aaron S.; Yano, Junko; Yachandra, Vittal K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Kern, Jan; Alonso-Mori, Roberto; Bergmann, Uwe] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. [Koroidov, Sergey; Messinger, Johannes] Umea Univ, Kemiskt Biol Ctr, Inst Kemi, S-90187 Umea, Sweden. [Zouni, Athina] Humboldt Univ, Inst Biol, D-10099 Berlin, Germany. [Koroidov, Sergey; Bergmann, Uwe] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. RP Sauter, NK; Yachandra, VK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. EM NKSauter@lbl.gov; VKYachandra@lbl.gov RI Sauter, Nicholas/K-3430-2012 NR 11 TC 4 Z9 4 U1 21 U2 45 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 19 PY 2016 VL 533 IS 7603 BP E1 EP E2 DI 10.1038/nature17983 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM0AH UT WOS:000376004300001 PM 27193689 ER PT J AU Henriksson, K Foucart, F Kidder, LE Teukolsky, SA AF Henriksson, Katherine Foucart, Francois Kidder, Lawrence E. Teukolsky, Saul A. TI Initial data for high-compactness black hole-neutron star binaries SO CLASSICAL AND QUANTUM GRAVITY LA English DT Article DE neutron stars; initial value problem; black holes; relativity and gravitation; relativistic binaries ID GAMMA-RAY BURSTS; GRAVITATIONAL-RADIATION; DENSE MATTER; MERGERS; EQUATION; SIMULATIONS; RELATIVITY; HOT AB For highly compact neutron stars, constructing numerical initial data for black hole-neutron star binary evolutions is very difficult. We describe improvements to an earlier method that enable it to handle these more challenging cases. These improvements were found by invoking a general relaxation principle that may be helpful in improving robustness in other initial data solvers. We examine the case of a 6: 1 mass ratio system in inspiral close to merger, where the star is governed by a polytropic Gamma = 2, an SLy, or an LS220 equation of state (EOS). In particular, we are able to obtain a solution with a realistic LS220 EOS for a star with compactness 0.26 and mass 1.98Me, which is representative of the highest reliably determined neutron star masses. For the SLy EOS, we can obtain solutions with a comparable compactness of 0.25, while for a family of polytropic equations of state, we obtain solutions with compactness up to 0.21, the largest compactness that is stable in this family. These compactness values are significantly higher than any previously published results. C1 [Henriksson, Katherine; Kidder, Lawrence E.; Teukolsky, Saul A.] Cornell Univ, Ctr Radiophys & Space Res, Ithaca, NY 14853 USA. [Foucart, Francois] Univ Toronto, Canadian Inst Theoret Astrophys, 60 St George St, Toronto, ON M5S 3H8, Canada. [Foucart, Francois] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Henriksson, Katherine] Google Inc, 747 6th St S, Kirkland, WA 98033 USA. RP Henriksson, K (reprint author), Cornell Univ, Ctr Radiophys & Space Res, Ithaca, NY 14853 USA. EM kth48@cornell.edu FU NSF [PHY-1306125, AST-1333129]; Sherman Fairchild Foundation; Vincent and Beatrice Tremaine Postdoctoral Fellowship; NSERC Canada; NASA through Einstein Postdoctoral Fellowship - Chandra X-ray Center [PF4-150122]; NASA [NAS8-03060]; NSF MRI [PHY-0960291] FX K H would like to thank Geoffrey Lovelace, Curran Muhlberger, Harald Pfeiffer, and David Chernoff for useful discussions, and Andy Bohn for the use of computing resources. This work was supported in part by NSF Grants PHY-1306125 and AST-1333129 at Cornell University, and by a grant from the Sherman Fairchild Foundation. F F gratefully acknowledges support from the Vincent and Beatrice Tremaine Postdoctoral Fellowship and NSERC Canada. Support for this work was provided by NASA through Einstein Postdoctoral Fellowship grant number PF4-150122 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. This research was performed in part using the Zwicky computer system operated by the Caltech Center for Advanced Computing Research and funded by NSF MRI No. PHY-0960291 and the Sherman Fairchild Foundation. NR 49 TC 1 Z9 1 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0264-9381 EI 1361-6382 J9 CLASSICAL QUANT GRAV JI Class. Quantum Gravity PD MAY 19 PY 2016 VL 33 IS 10 AR 105009 DI 10.1088/0264-9381/33/10/105009 PG 22 WC Astronomy & Astrophysics; Physics, Multidisciplinary; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK3QY UT WOS:000374833700009 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moortgat, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Parijs, I Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Randle-conde, A Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Schofbeck, R Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L De Visscher, S Delaere, C Delcourt, M Forthomme, L Francois, B Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Magitteri, A Mertens, A Musich, M Nuttens, C Piotrzkowski, K Quertenmont, L Selvaggi, M Marono, MV Wertz, S Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Fang, W Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Leggat, D Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Ferencek, D Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Jarrin, EC Awad, A 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Woods, N. CA CMS Collaboration TI Measurement of the top quark mass using charged particles in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID FRAGMENTATION FUNCTION; DECAYS; MODEL AB A novel technique for measuring the mass of the top quark that uses only the kinematic properties of its charged decay products is presented. Top quark pair events with final states with one or two charged leptons and hadronic jets are selected from the data set of 8 TeV proton-proton collisions, corresponding to an integrated luminosity of 19.7 fb(-1). By reconstructing secondary vertices inside the selected jets and computing the invariant mass of the system formed by the secondary vertex and an isolated lepton, an observable is constructed that is sensitive to the top quark mass that is expected to be robust against the energy scale of hadronic jets. The main theoretical systematic uncertainties, concerning the modeling of the fragmentation and hadronization of b quarks and the reconstruction of secondary vertices from the decays of b hadrons, are studied. A top quark mass of 173.68 +/- 0.20(stat)(-0.97)(+1.58) (syst) GeV is measured. The overall systematic uncertainty is dominated by the uncertainty in the b quark fragmentation and the modeling of kinematic properties of the top quark. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Pigazzini, S.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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De Castro; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trent, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bartosik, N.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.; Traczyk, P.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; La Licata, C.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Lee, S. W.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Yang, Y. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, Y.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Guisao, J. Mejia; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.; Uribe Estrada, C.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nemallapudi, M. V.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Voytishin, N.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Matveev, V.; Chadeeva, M.; Chistov, R.; Danilov, M.; Markin, O.; Popova, E.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Korneeva, N.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Merlin, J. A.; Stahl, A.; Pantaleo, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Pazzini, J.; Azzurri, P.; D'imperio, G.; Del Re, D.; Arcidiacono, R.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Fartoukh, S.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Knunz, V.; Kortelainen, M. J.; Kousouris, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Sauvan, J. B.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veckalns, V.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Virdee, T.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.; Chen, K. H.] Univ Zurich, Zurich, Switzerland. [Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Tsai, J. F.; Tzeng, Y. M.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Cerci, D. Sunar; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Haddad, Y.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mastrolorenzo, L.; Nash, J.; Nikitenko, A.; Pela, J.; Penning, B.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Flores, C.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Paneva, M. I.; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Gerosa, R.; Holzner, A.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wood, J.; Wurthwein, F.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bendavid, J.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cremonesi, M.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Kuznetsova, E.; Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Santra, A.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Castle, J.; Kenny, R. P., III; Kropivnitskaya, A.; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Hsu, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.; Stieger, B.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Parker, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M. H.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Rupprecht, N.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Duh, Y. T.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Gershtein, Y.; Espinosa, T. A. Gomez; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Kyriacou, S.; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Heideman, J.; Riley, G.; Rose, K.; Spanier, S.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Pernie, L.; Rathjens, D.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.; Wang, Z.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Elgammal, S.; Salama, E.] British Univ Egypt, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Salama, E.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Kim, T. J.] Hanyang Univ, Seoul 133791, South Korea. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. [Heredia-De La Cruz, I.; Zagozdzinska, A.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Di Marco, E.] Univ Rome, Sez Roma, Ist Nazl Fis Nucl, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Pisa, Italy. [Veckalns, V.] Riga Tech Univ, Riga, Latvia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, CA USA. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Chistov, Ruslan/B-4893-2014; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Ogul, Hasan/S-7951-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Chadeeva, Marina/C-8789-2016; Danilov, Mikhail/C-5380-2014; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Lokhtin, Igor/D-7004-2012; Seixas, Joao/F-5441-2013; Della Ricca, Giuseppe/B-6826-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Mora Herrera, Maria Clemencia/L-3893-2016; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016 OI ciocci, maria agnese /0000-0003-0002-5462; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Chistov, Ruslan/0000-0003-1439-8390; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Chadeeva, Marina/0000-0003-1814-1218; Danilov, Mikhail/0000-0001-9227-5164; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Seixas, Joao/0000-0002-7531-0842; Della Ricca, Giuseppe/0000-0003-2831-6982; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Center, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR Project (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund, Chulalongkorn University (Thailand); Welch Foundation [C-1845]; Ministry of Science and Technology; Programa Consolider-Ingenio, Spain FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Center, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, Contract No. C-1845. NR 75 TC 2 Z9 2 U1 13 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 18 PY 2016 VL 93 IS 9 AR 092006 DI 10.1103/PhysRevD.93.092006 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM3ON UT WOS:000376255900001 ER PT J AU Arnou, P van Hest, MFAM Cooper, CS Malkov, AV Walls, JM Bowers, JW AF Arnou, Panagiota van Hest, Maikel F. A. M. Cooper, Carl S. Malkov, Andrei V. Walls, John M. Bowers, Jake W. TI Hydrazine-Free Solution-Deposited CuIn(S,Se)(2) Solar Cells by Spray Deposition of Metal Chalcogenides SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE CIGS; thin film; solar cells; chalcopyrite; atmospheric process ID THIN-FILMS; SEMICONDUCTORS; CUINSE2 AB Solution processing of semiconductors, such as CuInSe2 and its alloys (CIGS), can significantly reduce the manufacturing costs of thin film solar cells. Despite the recent success of solution deposition approaches for CIGS, toxic reagents such as hydrazine are usually involved, which introduce health and safety concerns. Here, we present a simple and safer methodology for the preparation of high-quality CuIn(S, Se)(2) absorbers from metal sulfide solutions in a diamine/dithiol mixture. The solutions are sprayed in air, using a chromatography atomizer, followed by a postdeposition selenization step. Two different selenization methods are explored resulting in power conversion efficiencies of up to 8%. C1 [Arnou, Panagiota; Cooper, Carl S.; Walls, John M.; Bowers, Jake W.] Univ Loughborough, Wolfson Sch Mech Elect & Mfg Engn, CREST, Loughborough LE11 3TU, Leics, England. [Cooper, Carl S.; Malkov, Andrei V.] Univ Loughborough, Dept Chem, Loughborough LE11 3TU, Leics, England. [van Hest, Maikel F. A. M.] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Arnou, P; Bowers, JW (reprint author), Univ Loughborough, Wolfson Sch Mech Elect & Mfg Engn, CREST, Loughborough LE11 3TU, Leics, England. EM P.Arnou@lboro.ac.uk; J.W.Bowers@lboro.ac.uk RI Malkov, Andrei/F-4908-2013; OI Malkov, Andrei/0000-0001-6072-2353; Arnou, Panagiota/0000-0001-7992-0632 FU EPSRC Supergen SuperSolar Hub [EP/J017361/1]; EPSRC PVTEAM [EP/L017792/1]; EPRSRC [EP/N508457/1]; SuperSolar Hub FX The authors thank Dr. Stephen Whitelegg, Nanoco Technologies plc (UK) for the EQE measurements, and Dr. Ali. Abbas (Loughborough University), for the SEM images. Authors P.A, C.S.C, J.M.W., and J.W.B. are grateful for funding from EPSRC Supergen SuperSolar Hub (EP/J017361/1); EPSRC PVTEAM (EP/L017792/1) and EPRSRC grant EP/N508457/1 to support this project. P.A. also thanks the SuperSolar Hub for funding a 3 month secondment at the National Renewable Energy Laboratory in Colorado, USA. NR 20 TC 3 Z9 3 U1 10 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 18 PY 2016 VL 8 IS 19 BP 11893 EP 11897 DI 10.1021/acsami.6b01541 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DM4QC UT WOS:000376330800001 PM 27135679 ER PT J AU Xia, Y Lee, E Hu, H Gharbi, MA Beller, DA Fleischmann, EK Kamien, RD Zentel, R Yang, S AF Xia, Yu Lee, Elaine Hu, Hao Gharbi, Mohamed Amine Beller, Daniel A. Fleischmann, Eva-Kristina Kamien, Randall D. Zentel, Rudolf Yang, Shu TI Better Actuation Through Chemistry: Using Surface Coatings to Create Uniform Director Fields in Nematic Liquid Crystal Elastomers SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE liquid crystal elastomer; surface chemistry; monodomain; soft lithography; actuator ID WRINKLED ELASTOMERS; ARTIFICIAL MUSCLES; LIGHT; ADHESIVE; CONTACT; ARRAYS; WINDOW AB Controlling the molecular alignment of liquid crystal monomers (LCMs) within nano and microstructures is essential in manipulating the actuation behavior of nematic liquid crystal elastomers (NLCEs). Here, we study how to induce uniformly vertical alignment of nematic LCMs within a micropillar array to maximize the macroscopic shape change using surface chemistry. Landau-de Gennes numerical modeling suggests that it is difficult to perfectly align LCMs vertically in every pore within a poly(dimethylsiloxane) (PDMS) mold with porous channels during soft lithography. In an untreated PDMS mold that provides homeotropic anchoring of LCMs, a radially escaped configuration of LCMs is observed. Vertically aligned LCMs, a preferred configuration for actuation, are only observed when using a PDMS mold with planar anchoring. Guided by the numerical modeling, we coat the PDMS mold with a thin layer of poly(2-hydroxyethyl methacrylate) (PHEMA), leading to planar anchoring of LCM. Confirmed by polarized optical microscopy, we observe monodomains of vertically aligned LCMs within the mold, in agreement with modeling. After curing and peeling off the mold, the resulting NLCE micropillars showed a relatively large and reversible radial strain (similar to 30%) when heated above the nematic to isotropic transition temperature. C1 [Xia, Yu; Lee, Elaine; Hu, Hao; Gharbi, Mohamed Amine; Yang, Shu] Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. [Lee, Elaine] Lawrence Livermore Natl Lab, Engn Directorate, 7000 East Ave, Livermore, CA 94550 USA. [Gharbi, Mohamed Amine; Kamien, Randall D.] Univ Penn, Dept Phys & Astron, 209 South 33rd St, Philadelphia, PA 19104 USA. [Beller, Daniel A.] Harvard Univ, Paulson Sch Engn & Appl Sci, 29 Oxford St, Cambridge, MA 02138 USA. [Fleischmann, Eva-Kristina; Zentel, Rudolf] Johannes Gutenberg Univ Mainz, Inst Organ Chem, Duesbergweg 10-14, D-55128 Mainz, Germany. RP Yang, S (reprint author), Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. EM shuyang@seas.upenn.edu RI Yang, Shu/D-9758-2011; Zentel, Rudolf/D-4542-2011 FU National Science Foundation (NSF) Materials Science and Engineering Center (MRSEC) Grant [DMR-1120901, DMR-1410253, DMR12-62047]; Simons Investigator grant from the Simons Foundation; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344, LLNL-ABS-678248] FX We acknowledge support by the National Science Foundation (NSF) Materials Science and Engineering Center (MRSEC) Grant to University of Pennsylvania, DMR-1120901, DMR-1410253 (S.Y.), and DMR12-62047 (R.D.K.). This work is also partially supported by a Simons Investigator grant from the Simons Foundation to R.D.K. We also acknowledge Dr. Simon Copar for providing POV-Ray scene file generator for visualizations of numerical results. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344, LLNL-ABS-678248. NR 38 TC 0 Z9 0 U1 19 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 18 PY 2016 VL 8 IS 19 BP 12466 EP 12472 DI 10.1021/acsami.6b02789 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DM4QC UT WOS:000376330800064 PM 27152975 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahmad, S Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Balasubramanian, S Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Benacek, P Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biro, G Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chauvin, A Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danisch, MC Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Conti, C de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E Deplano, C Dhankher, P Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Endress, E Engel, H Epple, E Erazmus, B Erdemir, I Erhardt, F Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fronze, GG Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hamon, JC Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hillemanns, H Hippolyte, B Horak, D Hosokawa, R Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Inaba, M Incani, E Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacazio, N Jacobs, PM Jadhav, MB Jadlovska, S Jadlovsky, J Jahnke, C Jakubowska, MJ Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, DW Kim, DJ Kim, D Kim, H Kim, JS Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Klewin, S Kluge, A Knichel, ML Knospe, AG Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kostarakis, P Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kralik, I Kravcakova, A Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kuhn, C Kuijer, PG Kumar, A Kumar, J Kumar, L Kumar, S Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P de Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Vargas, HL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Lutz, TH Maevskaya, A 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CA ALICE Collaboration TI Multipion Bose-Einstein correlations in pp, p-Pb, and Pb-Pb collisions at energies available at the CERN Large Hadron Collider SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; 3-PION INTERFEROMETRY; COULOMB CORRECTIONS; CONDENSATION; INTERFERENCE; THERMINATOR; GENERATOR; SYSTEMS; 2-PION; STATES AB Three- and four-pionBose-Einstein correlations are presented in pp, p-Pb, and Pb-Pb collisions at the LHC. We compare our measured four-pion correlations to the expectation derived from two-and three-pion measurements. Such a comparison provides a method to search for coherent pion emission. We also present mixed-charge correlations in order to demonstrate the effectiveness of several analysis procedures such as Coulomb corrections. Same-charge four-pion correlations in pp and p-Pb appear consistent with the expectations from three-pion measurements. However, the presence of non-negligible background correlations in both systems prevent a conclusive statement. In Pb-Pb collisions, we observe a significant suppression of three-and four-pion Bose-Einstein correlations compared to expectations from two-pionmeasurements. There appears to be no centrality dependence of the suppression within the 0%-50% centrality interval. The origin of the suppression is not clear. However, by postulating either coherent pion emission or large multibody Coulomb effects, the suppression may be explained. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Moreno, L. A. P.; Navarro, S. R.; Noris, J. C. C.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Limon, S. Vergara; Tello, A. Villatoro] Benemerita Univ Autonoma Puebla, Puebla, Mexico. 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M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Gimenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Fernandes, C. Lagana; Mas, A.; Munhoz, M. G.; da Luz, H. Natal; Da Silva, A. C. Oliveira; Suaide, A. A. P.; de Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; de Souza, R. D.; Takahashi, J.] Univ Estadual Campinas, UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Murakami, H.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Biro, G.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Balasubramanian, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Lutz, T. H.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Fachhsch Worms, ZTT, Worms, Germany. [Adam, J.; Akindinov, A.; Alici, A.; Alkin, A.; Connors, M. E.] Georgia State Univ, Atlanta, GA 30303 USA. [Khan, M. Mohisin] Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-16635 Prague, Czech Republic.; Adam, J (reprint author), Georgia State Univ, Atlanta, GA 30303 USA.; Adam, J (reprint author), Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. RI Bregant, Marco/I-7663-2012; Peitzmann, Thomas/K-2206-2012; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Chinellato, David/D-3092-2012; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Vechernin, Vladimir/J-5832-2013; Pshenichnov, Igor/A-4063-2008; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Derradi de Souza, Rafael/M-4791-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; OI Peitzmann, Thomas/0000-0002-7116-899X; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Chinellato, David/0000-0002-9982-9577; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Vechernin, Vladimir/0000-0003-1458-8055; Pshenichnov, Igor/0000-0003-1752-4524; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Derradi de Souza, Rafael/0000-0002-2084-7001; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Read, Kenneth/0000-0002-3358-7667; Riggi, Francesco/0000-0002-0030-8377; Melikyan, Yury/0000-0002-4165-505X; Giubilato, Piero/0000-0003-4358-5355; Brucken, Jens Erik/0000-0001-6066-8756; Murray, Sean/0000-0003-0548-588X; Fernandez Tellez, Arturo/0000-0001-5092-9748 FU Grid centers; Worldwide LHC Computing Grid (WLCG) collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organizatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX We would like to thank Richard Lednicky and Tamas Csorgo for numerous helpful discussions. The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centers and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organizatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 54 TC 5 Z9 5 U1 3 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 18 PY 2016 VL 93 IS 5 AR 054908 DI 10.1103/PhysRevC.93.054908 PG 20 WC Physics, Nuclear SC Physics GA DM3NS UT WOS:000376253800002 ER PT J AU Tian, XC Shaw, S Lind, KR Cademartiri, L AF Tian, Xinchun Shaw, Santosh Lind, Kara R. Cademartiri, Ludovico TI Thermal Processing of Silicones for Green, Scalable, and Healable Superhydrophobic Coatings SO ADVANCED MATERIALS LA English DT Article ID SUPEROLEOPHOBIC SURFACES; EMERGING APPLICATIONS; OIL/WATER SEPARATION; SLIPPERY SURFACES; ROBUST; FABRICATION; MEMBRANES; COMPATIBILITY; TRANSPARENT; DEGRADATION AB The thermal degradation of silicones is exploited and engineered to make super-hydrophobic coatings that are scalable, healable, and ecofriendly for various outdoor applications. The coatings can be generated and regenerated at the rate of 1 m(2) min(-1) using premixed flames, adhere to a variety of substrates, and tolerate foot traffic (>1000 steps) after moderate wear and healing. C1 [Tian, Xinchun; Shaw, Santosh; Lind, Kara R.; Cademartiri, Ludovico] Iowa State Univ Sci & Technol, Dept Mat Sci & Engn, 2220 Hoover Hall, Ames, IA 50011 USA. [Cademartiri, Ludovico] Iowa State Univ Sci & Technol, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Cademartiri, Ludovico] US DOE, Ames Lab, Ames, IA 50011 USA. RP Cademartiri, L (reprint author), Iowa State Univ Sci & Technol, Dept Mat Sci & Engn, 2220 Hoover Hall, Ames, IA 50011 USA.; Cademartiri, L (reprint author), Iowa State Univ Sci & Technol, Dept Chem & Biol Engn, Ames, IA 50011 USA.; Cademartiri, L (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM lcademar@iastate.edu RI Cademartiri, Ludovico/A-4142-2008 OI Cademartiri, Ludovico/0000-0001-8805-9434 FU Iowa State University of Science and Technology; Chinese Scholarship Committee FX The research has been supported by Iowa State University of Science and Technology through a startup grant to LC. X.C.T is grateful to the Chinese Scholarship Committee for a scholarship. The authors thank Jerry Carney & Son Inc. for assistance with the large-scale experiments. The authors are also grateful to Martin Thuo for access to a goniometer and to Stephanie Oyola, Sarah Cady, Dapeng Jing, and Warren Straszheim for assistance with CA, SSNMR, XPS, and SEM characterizations. NR 53 TC 10 Z9 11 U1 64 U2 144 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAY 18 PY 2016 VL 28 IS 19 BP 3677 EP 3682 DI 10.1002/adma.201506446 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM6RQ UT WOS:000376480500006 PM 27008206 ER PT J AU Sliwiak, J Dauter, Z Jaskolski, M AF Sliwiak, Joanna Dauter, Zbigniew Jaskolski, Mariusz TI Crystal Structure of Hyp-1, a Hypericum perforatum PR-10 Protein, in Complex with Melatonin SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE pathogenesis-related protein; PR-10; phytohormone; ligand binding; cytokinin ID PATHOGENESIS-RELATED PROTEINS; BET V 1; X-RAY; CYTOKININ; BINDING; BIOSYNTHESIS; PLANTS; L.; ALLERGEN; EXPRESSION AB Hyp-1, a PR-10-fold protein from Hypericum perforatum, was crystallized in complex with melatonin (MEL). The structure confirms the conserved protein fold and the presence of three unusual ligand binding sites, two of which are internal chambers (1,2), while the third one (3) is formed as an invagination of the protein surface. The MEL ligand in site 1 is well defined while that in site 3 seems to be rotating between the side chains of Lys33 and Tyr150 that act as a molecular vise. The patch of electron density in site 2 does not allow unambiguous modeling of a melatonin molecule but suggests a possible presence of its degradation product. This pattern of ligand occupation is reproducible in repeated crystallization/structure determination experiments. Although the binding of melatonin by Hyp-1 does not appear to be very strong (for example, MEL cannot displace the artificial fluorescence probe ANS), it is strong enough to suggest a physiological role of this interaction. For example, trans-zeatin, which is a common ligand of PR-10 proteins, does not overcompete melatonin for binding to Hyp-1 as it does not affect the crystallization process of the Hyp-1/MEL complex, and among a number of potential natural mediators tested, melatonin was the only one to form a crystalline complex with Hyp-1 with the use of standard crystallization screens. Hyp-1 is the second protein in the Protein Data Bank for which melatonin binding has been demonstrated crystallographically, the first one being human quinone reductase. C1 [Sliwiak, Joanna; Jaskolski, Mariusz] Polish Acad Sci, Inst Bioorgan Chem, Ctr Biocrystallog Res, Poznan, Poland. [Dauter, Zbigniew] Argonne Natl Lab, Synchrotron Radiat Res Sect, NCI, 9700 S Cass Ave, Argonne, IL 60439 USA. [Jaskolski, Mariusz] Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, Grunwaldzka 6, PL-60780 Poznan, Poland. RP Jaskolski, M (reprint author), Polish Acad Sci, Inst Bioorgan Chem, Ctr Biocrystallog Res, Poznan, Poland.; Jaskolski, M (reprint author), Adam Mickiewicz Univ, Fac Chem, Dept Crystallog, Grunwaldzka 6, PL-60780 Poznan, Poland. EM mariuszj@amu.edu.pl FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38]; European Union within the European Regional Developmental Fund; Polish National Science Centre [2013/10/M/NZ1/00251]; Polish Ministry of Science and Higher Education under the KNOW program FX X-Ray diffraction data were collected at the Southeast Regional Collaborative Access Team (SER-CAT) beamline of the APS/ANL. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38. Financial support of the project was provided by the European Union within the European Regional Developmental Fund and by the Polish National Science Centre (grant No. 2013/10/M/NZ1/00251). This publication was supported by the Polish Ministry of Science and Higher Education under the KNOW program. NR 44 TC 0 Z9 0 U1 1 U2 8 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAY 18 PY 2016 VL 7 AR 668 DI 10.3389/fpls.2016.00668 PG 10 WC Plant Sciences SC Plant Sciences GA DL9QF UT WOS:000375977100003 PM 27242869 ER PT J AU Thaner, RV Eryazici, I Macfarlane, RJ Brown, KA Lee, B Nguyen, ST Mirkin, CA AF Thaner, Ryan V. Eryazici, Ibrahim Macfarlane, Robert J. Brown, Keith A. Lee, Byeongdu Nguyen, SonBinh T. Mirkin, Chad A. TI The Significance of Multivalent Bonding Motifs and "Bond Order" in DNA-Directed Nanoparticle Crystallization SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OLIGONUCLEOTIDE DENDRIMERS; MOLECULAR-DYNAMICS; MELTING PROPERTIES; NANOSTRUCTURES; SUPERLATTICES; DUPLEXES; ASSEMBLIES; HYBRIDS; DIMERS AB Multivalent oligonucleotide-based bonding elements have been synthesized and studied for the assembly and crystallization of gold nanoparticles. Through the use of organic branching points, divalent and trivalent DNA linkers were readily incorporated into the oligonucleotide shells that define DNA-nanoparticles and compared to monovalent linker systems. These multivalent bonding motifs enable the change of "bond strength" between particles and therefore modulate the effective "bond order." In addition, the improved accessibility of strands between neighboring particles, either due to multivalency or modifications to increase strand flexibility, gives rise to superlattices with less strain in the crystallites compared to traditional designs. Furthermore, the increased availability and number of binding modes also provide a new variable that allows previously unobserved crystal structures to be synthesized, as evidenced by the formation of a thorium phosphide superlattice. C1 [Thaner, Ryan V.; Eryazici, Ibrahim; Macfarlane, Robert J.; Brown, Keith A.; Nguyen, SonBinh T.; Mirkin, Chad A.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Thaner, Ryan V.; Eryazici, Ibrahim; Macfarlane, Robert J.; Brown, Keith A.; Nguyen, SonBinh T.; Mirkin, Chad A.] Northwestern Univ, Int Inst Nanotechnol, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, X Ray Sci Div, Argonne, IL 60439 USA. RP Nguyen, ST; Mirkin, CA (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Nguyen, ST; Mirkin, CA (reprint author), Northwestern Univ, Int Inst Nanotechnol, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM stn@northwestern.edu; chadnano@northwestern.edu RI Nguyen, SonBinh/C-1682-2014; Mirkin, Chad/E-3911-2010 OI Nguyen, SonBinh/0000-0002-6977-3445; FU Air Force Office of Scientific Research [FA9550-11-1-0275, FA9550-12-1-0280]; Center for Cancer Nanotechnology Excellence initiative of the National Institutes of Health [U54CA151880, U54CA199091]; NSF; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This material is based upon work supported by the following awards: Air Force Office of Scientific Research FA9550-11-1-0275 and FA9550-12-1-0280; the Center for Cancer Nanotechnology Excellence initiative of the National Institutes of Health U54CA151880 and U54CA199091. R.V.T. gratefully acknowledges an NSF Graduate Research Fellowship. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. NR 41 TC 1 Z9 1 U1 20 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2016 VL 138 IS 19 BP 6119 EP 6122 DI 10.1021/jacs.6b02479 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DM4QE UT WOS:000376331000008 PM 27148838 ER PT J AU von Kugelgen, S Bellone, DE Cloke, RR Perkins, WS Fischer, FR AF von Kugelgen, Stephen Bellone, Donatela E. Cloke, Ryan R. Perkins, Wade S. Fischer, Felix R. TI Initiator Control of Conjugated Polymer Topology in Ring-Opening Alkyne Metathesis Polymerization SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ARYLENE-ETHYNYLENE MACROCYCLES; POLY(PHENYLENE ETHYNYLENE)S; ENHANCED FLUORESCENCE; CATALYSTS; SENSOR; FILMS AB Molybdenum carbyne complexes [RC=Mo(OC(CH3)(CF3)(2))(3)] featuring a mesityl (R = Mes) or an ethyl (R = Et) substituent initiate the living ring-opening alkyne metathesis polymerization of the strained cyclic alkyne, 5,6,11,12-tetradehyoltobenzo[a,e] [8]annulene, to yield fully conjugated poly(o-phenylene ethynylene). The difference in the steric demand of the polymer end-group (Mes vs Et) transferred during the initiation step determines the topology of the resulting polymer chain. While [MesC Mo(OC(CH3)(CF3)(2))(3)] exclusively yields linear poly(o-phenylene ethynylene), polymerization initiated by [EtC Mo(OC(CH3)(CF3)(2))(3)] results in cyclic polymers ranging in size from n = 5 to 20 monomer units. Kinetic studies reveal that the propagating. species emerging from [EtC Mo(OC(CH3)(CF3)(2))(3)] undergoes a highly selective intramblecular backbiting into C1 [von Kugelgen, Stephen; Bellone, Donatela E.; Cloke, Ryan R.; Perkins, Wade S.; Fischer, Felix R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. [Fischer, Felix R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Fischer, FR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Fischer, FR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Fischer, FR (reprint author), Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA.; Fischer, FR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM ffischer@berkeley.edu FU National Science Foundation [CHE-1455289]; NIH [SRR023679A]; NIH Shared Instrumentation Grant [S10-RR027172]; Abramson Foundation FX This research is supported by the National Science Foundation under contract number CHE-1455289, Berkeley NMR Facility is supported in part by NIH Grant SRR023679A, and the X-Ray Facility is supported in part by NIH Shared Instrumentation Grant S10-RR027172. D.B. acknowledges fellowship support through the Abramson Foundation. The authors acknowledge Dr. Christian Canlas and Dr. Hasan Celik for support with NMR acquisition and Dr. Antonio DiPasquale for assistance with X-ray analysis. NR 39 TC 2 Z9 2 U1 19 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 18 PY 2016 VL 138 IS 19 BP 6234 EP 6239 DI 10.1021/jacs.6b02422 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DM4QE UT WOS:000376331000025 PM 27120088 ER PT J AU Pontzen, A Slosar, A Roth, N Peiris, HV AF Pontzen, Andrew Slosar, Anze Roth, Nina Peiris, Hiranya V. TI Inverted initial conditions: Exploring the growth of cosmic structure and voids SO PHYSICAL REVIEW D LA English DT Article ID MATTER POWER SPECTRUM; EXCURSION SET FORMALISM; N-BODY SIMULATIONS; PERTURBATION-THEORY; ZELDOVICH APPROXIMATION; MASS FUNCTIONS; FLUCTUATIONS; GALAXIES; OSCILLATIONS; EVOLUTION AB We introduce and explore "paired" cosmological simulations. A pair consists of an A and B simulation with initial conditions related by the inversion delta(A)(x, t(initial)) = -delta(B)(x, t(initial)) (underdensities substituted for overdensities and vice versa). We argue that the technique is valuable for improving our understanding of cosmic structure formation. The A and B fields are by definition equally likely draws from Lambda CDM initial conditions, and in the linear regime evolve identically up to the overall sign. As nonlinear evolution takes hold, a region that collapses to form a halo in simulation A will tend to expand to create a void in simulation B. Applications include (i) contrasting the growth of A-halos and B-voids to test excursion-set theories of structure formation, (ii) cross-correlating the density field of the A and B universes as a novel test for perturbation theory, and (iii) canceling error terms by averaging power spectra between the two boxes. Generalizations of the method to more elaborate field transformations are suggested. C1 [Pontzen, Andrew; Roth, Nina; Peiris, Hiranya V.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Slosar, Anze] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Pontzen, A (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM a.pontzen@ucl.ac.uk FU Royal Society; European Research Council under the European Community's Seventh Framework Programme (FP7)/ERC grant [306478]; INFN; BIS National E-Infrastructure capital grant [ST/K000373/1]; STFC DiRAC Operations grant [ST/K0003259/1] FX A. P. acknowledges financial support from the Royal Society. N. R. and H. V. P. were supported by the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement No. 306478-CosmicDawn. A. S. thanks the Department of Physics and Astronomy at University College London for hospitality during completion of this work. H. V. P. thanks the Galileo Galilei Institute for Theoretical Physics for hospitality and the INFN for partial support during the completion of this work. This work used the DiRAC Complexity system, operated by the University of Leicester IT Services, which forms part of the STFC DiRAC HPC Facility (www.dirac.ac.uk). This equipment is funded by BIS National E-Infrastructure capital grant ST/K000373/1 and STFC DiRAC Operations grant ST/K0003259/1. DiRAC is part of the National E-Infrastructure. NR 53 TC 1 Z9 1 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 18 PY 2016 VL 93 IS 10 AR 103519 DI 10.1103/PhysRevD.93.103519 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM3PO UT WOS:000376258700004 ER PT J AU Turnbull, D Michel, P Chapman, T Tubman, E Pollock, BB Chen, CY Goyon, C Ross, JS Divol, L Woolsey, N Moody, JD AF Turnbull, D. Michel, P. Chapman, T. Tubman, E. Pollock, B. B. Chen, C. Y. Goyon, C. Ross, J. S. Divol, L. Woolsey, N. Moody, J. D. TI High Power Dynamic Polarization Control Using Plasma Photonics SO PHYSICAL REVIEW LETTERS LA English DT Article ID LASER-BEAMS; ACCELERATOR; COMPRESSION; SCATTERING; BRILLOUIN; RAMAN AB We report the first experimental demonstration of a plasma wave plate based on laser-induced birefringence. An elliptically polarized input was converted into a nearly ideal circularly polarized beam using an optical system composed of a second laser beam and a plasma. The results are in excellent agreement with linear theory and three-dimensional simulations up to phase delays exceeding pi/4, thus establishing the feasibility of laser-plasma photonic devices that are ultrafast, damage-resistant, and easily tunable. C1 [Turnbull, D.; Michel, P.; Chapman, T.; Pollock, B. B.; Goyon, C.; Ross, J. S.; Divol, L.; Moody, J. D.] Lawrence Livermore Natl Lab, Natl Ignit Facil, Livermore, CA 94550 USA. [Tubman, E.; Woolsey, N.] Univ York, York Plasma Inst, York YO10 5DQ, N Yorkshire, England. [Chen, C. Y.] Cornell Univ, Sch Elect & Comp Engn, Ithaca, NY 14853 USA. RP Turnbull, D (reprint author), Lawrence Livermore Natl Lab, Natl Ignit Facil, Livermore, CA 94550 USA. EM turnbull2@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LLNL-LDRD Program [42074]; Grand Challenge program at Lawrence Livermore National laboratory; EPSRC Grant [EP/K504178/1, EP/L000644/1] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. This work was supported by the LLNL-LDRD Program under Project No. 42074. We acknowledge the allocation of computational resources under the Grand Challenge program at Lawrence Livermore National laboratory, as well as EPSRC Grant No. EP/K504178/1 and No. EP/L000644/1. Finally, we thank the staff of the Jupiter Laser Facility and Suzanne Ali for enabling a successful experimental campaign. NR 18 TC 4 Z9 4 U1 6 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 18 PY 2016 VL 116 IS 20 AR 205001 DI 10.1103/PhysRevLett.116.205001 PG 5 WC Physics, Multidisciplinary SC Physics GA DM3SK UT WOS:000376266500002 PM 27258871 ER PT J AU Bhandari, R Peters, NA AF Bhandari, Ramesh Peters, Nicholas A. TI On the general constraints in single qubit quantum process tomography SO SCIENTIFIC REPORTS LA English DT Article AB We briefly review single-qubit quantum process tomography for trace-preserving and nontrace-preserving processes, and derive explicit forms of the general constraints for fitting experimental data. These forms provide additional insight into the structure of the process matrix. We illustrate this with several examples, including a discussion of qubit leakage error models and the intuition which can be gained from their process matrices. C1 [Bhandari, Ramesh] Lab Phys Sci, 8050 Greenmead Dr, College Pk, MD 20740 USA. [Peters, Nicholas A.] Oak Ridge Natl Lab, One Bethel Valley Rd,POB 2008,MS-6418, Oak Ridge, TN 37831 USA. RP Bhandari, R (reprint author), Lab Phys Sci, 8050 Greenmead Dr, College Pk, MD 20740 USA. EM rbhandari@lps.umd.edu RI Peters, Nicholas/F-2530-2010 OI Peters, Nicholas/0000-0002-7215-9630 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX One of us (NAP) acknowledges research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. RB acknowledges useful communications with Joel Wallman, Joseph Emerson, Andrzej Veitia, and Robin Blume-Kahout. NR 13 TC 0 Z9 0 U1 6 U2 10 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 18 PY 2016 VL 6 AR 26004 DI 10.1038/srep26004 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL9TN UT WOS:000375986000002 PM 27188691 ER PT J AU Sales, BC Jin, K Bei, HB Stocks, GM Samolyuk, GD May, AF McGuire, MA AF Sales, Brian C. Jin, Ke Bei, Hongbin Stocks, G. Malcolm Samolyuk, German D. May, Andrew F. McGuire, Michael A. TI Quantum Critical Behavior in a Concentrated Ternary Solid Solution SO SCIENTIFIC REPORTS LA English DT Article ID FERMI-LIQUID BEHAVIOR; LINEAR MAGNETORESISTANCE; MAGNETIC-PROPERTIES; PHASE-TRANSITIONS; SOLUTION ALLOYS; CRITICAL-POINT; DISORDER; SYSTEMS AB The face centered cubic (fcc) alloy NiCoCrx with x approximate to 1 is found to be close to the Cr concentration where the ferromagnetic transition temperature, T-c, goes to 0. Near this composition these alloys exhibit a resistivity linear in temperature to 2 K, a linear magnetoresistance, an excess - TlnT (or power law) contribution to the low temperature heat capacity, and excess low temperature entropy. All of the low temperature electrical, magnetic and thermodynamic properties of the alloys with compositions near x approximate to 1 are not typical of a Fermi liquid and suggest strong magnetic fluctuations associated with a quantum critical region. The limit of extreme chemical disorder in this simple fcc material thus provides a novel and unique platform to study quantum critical behavior in a highly tunable system. C1 [Sales, Brian C.; Jin, Ke; Bei, Hongbin; Stocks, G. Malcolm; Samolyuk, German D.; May, Andrew F.; McGuire, Michael A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Sales, BC (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM salesbc@ornl.gov RI McGuire, Michael/B-5453-2009; May, Andrew/E-5897-2011; Stocks, George Malcollm/Q-1251-2016; OI McGuire, Michael/0000-0003-1762-9406; May, Andrew/0000-0003-0777-8539; Stocks, George Malcollm/0000-0002-9013-260X; Bei, Hongbin/0000-0003-0283-7990 FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, BES FX This research was supported primarily by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (B.C.S, A.F.M., M.A.M.). K.J., H.B., G.D.S. and G.M.S. were supported by the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, BES. NR 33 TC 2 Z9 2 U1 8 U2 22 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 18 PY 2016 VL 6 AR 26179 DI 10.1038/srep26179 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL9WE UT WOS:000375993300001 PM 27188715 ER PT J AU Aji, LBB Wallace, JB Shao, L Kucheyev, SO AF Aji, L. B. Bayu Wallace, J. B. Shao, L. Kucheyev, S. O. TI Effective defect diffusion lengths in Ar-ion bombarded 3C-SiC SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article DE defect diffusion length; radiation damage; SiC ID QUANTITATIVE APPROACH AB Above room temperature, SiC exhibits pronounced processes of diffusion and interaction of radiation-generated point defects. Here, we use the recently developed pulsed ion beam method to measure effective defect diffusion lengths in 3C-SiC bombarded in the temperature range of 25-200 degrees C with 500 keV Ar ions. Results reveal a diffusion length of similar to 10 nm, which exhibits a weak temperature dependence, changing from 9 to 13 nm with increasing temperature. These results have important implications for understanding and predicting radiation damage in SiC and for the development of radiation-resistant materials via interface-mediated defect reactions. C1 [Aji, L. B. Bayu; Wallace, J. B.; Kucheyev, S. O.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Wallace, J. B.; Shao, L.] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. RP Aji, LBB (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM bayuaji1@llnl.gov FU Nuclear Energy Enabling Technology (NEET) Program of the U.S. DOE, Office of Nuclear Energy; US DOE by LLNL [DE-AC52-07NA27344]; LGSP FX This work was funded by the Nuclear Energy Enabling Technology (NEET) Program of the U.S. DOE, Office of Nuclear Energy and performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344. JBW acknowledges the LGSP for funding. NR 18 TC 1 Z9 1 U1 3 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD MAY 18 PY 2016 VL 49 IS 19 AR 19LT01 DI 10.1088/0022-3727/49/19/19LT01 PG 4 WC Physics, Applied SC Physics GA DK9MW UT WOS:000375255500001 ER PT J AU Tait, EW Ratcliff, LE Payne, MC Haynes, PD Hine, NDM AF Tait, E. W. Ratcliff, L. E. Payne, M. C. Haynes, P. D. Hine, N. D. M. TI Simulation of electron energy loss spectra of nanomaterials with linear-scaling density functional theory SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE EELS; ELNES; linear scaling; defects; titanium dioxide; theoretical spectroscopy; electron energy loss spectroscopy ID MATRIX; ELNES; PHASE; STATE AB Experimental techniques for electron energy loss spectroscopy (EELS) combine high energy resolution with high spatial resolution. They are therefore powerful tools for investigating the local electronic structure of complex systems such as nanostructures, interfaces and even individual defects. Interpretation of experimental electron energy loss spectra is often challenging and can require theoretical modelling of candidate structures, which themselves may be large and complex, beyond the capabilities of traditional cubic-scaling density functional theory. In this work, we present functionality to compute electron energy loss spectra within the onetep linear-scaling density functional theory code. We first demonstrate that simulated spectra agree with those computed using conventional plane wave pseudopotential methods to a high degree of precision. The ability of onetep to tackle large problems is then exploited to investigate convergence of spectra with respect to supercell size. Finally, we apply the novel functionality to a study of the electron energy loss spectra of defects on the (1 0 1) surface of an anatase slab and determine concentrations of defects which might be experimentally detectable. C1 [Tait, E. W.; Payne, M. C.] Univ Cambridge, Cavendish Lab, Condensed Matter Theory Grp, 19 JJ Thomson Ave, Cambridge CB3 0HE, England. [Ratcliff, L. E.] Argonne Natl Lab, Leadership Comp Facil, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. [Haynes, P. D.] Univ London Imperial Coll Sci Technol & Med, Dept Mat, Exhibit Rd, London SW7 2AZ, England. [Hine, N. D. M.] Univ Warwick, Dept Phys, Theory Grp, Coventry CV4 7AL, W Midlands, England. RP Tait, EW (reprint author), Univ Cambridge, Cavendish Lab, Condensed Matter Theory Grp, 19 JJ Thomson Ave, Cambridge CB3 0HE, England. EM ewt23@cam.ac.uk RI Hine, Nicholas/D-4109-2011 OI Hine, Nicholas/0000-0001-5613-3679 FU Higher Education Funding Council for England; Science and Technology Facilities Council; EPSRC Cambridge NanoDTC [EP/G037221/1]; DOE Office of Science User Facility [DE-AC02-06CH11357]; Winton Programme for the Physics of Sustainability; EPSRC [EP/J015059/1] FX This work was performed using the Darwin Supercomputer of the University of Cambridge High Performance Computing Service (www.hpc.cam.ac.uk/), provided by Dell Inc. using Strategic Research Infrastructure Funding from the Higher Education Funding Council for England and funding from the Science and Technology Facilities Council. EWT was supported by the EPSRC Cambridge NanoDTC, EP/G037221/1. LER was supported, in part, by DOE Office of Science User Facility under Contract DE-AC02-06CH11357. NDMH Acknowledges the support of the Winton Programme for the Physics of Sustainability. ONETEP development is supported by EPSRC platform grant EP/J015059/1. We wish to acknowledge the use of the EPSRC's Chemical Database Service at Daresbury. The authors thank Dr Caterina Ducati for useful discussions. The underlying data of this publication can be accessed via the following persistent URI:www.repository.cam.ac.uk/handle/1810/253717 NR 39 TC 1 Z9 1 U1 3 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 18 PY 2016 VL 28 IS 19 AR 195202 DI 10.1088/0953-8984/28/19/195202 PG 10 WC Physics, Condensed Matter SC Physics GA DJ7ME UT WOS:000374394700006 PM 27094207 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahmad, S Ahn, SU Aiola, S Akindinov, A Alam, SN Albuquerque, DSD Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Balasubramanian, S Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK 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CA ALICE Collaboration TI Centrality dependence of charged jet production in p-Pb collisions at root(NN)-N-S=5.02 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID TRANSVERSE-MOMENTUM DEPENDENCE; RANGE ANGULAR-CORRELATIONS; ROOT-S(NN)=5.02 TEV; ATLAS DETECTOR; LONG-RANGE; PARTICLE PRODUCTION; ROOT-S-NN=5.02 TEV; PPB COLLISIONS; SUPPRESSION; MATTER AB Measurements of charged jet production as a function of centrality are presented for p-Pb collisions recorded a root(NN)-N-S = 5.02 TeV with the ALICE detector. Centrality classes are determined via the energy deposit in neutron calorimeters at zero degree, close to the beam direction, to minimise dynamical biases of the selection. The corresponding number of participants or binary nucleon-nucleon collisions is determined based on the particle production in the Pb-going rapidity region. Jets have been reconstructed in the central rapidity region from charged particles with the anti-k(T) algorithm for resolution parameters R = 0.2 and R = 0.4 in the transverse momentum range 20 to 120 GeV/c. The reconstructed jet momentum and yields have been corrected for detector effects and underlying-event background. In the five centrality bins considered, the charged jet production in p-Pb collisions is consistent with the production expected from binary scaling from pp collisions. The ratio of jet yields reconstructed with the two different resolution parameters is also independent of the centrality selection, demonstrating the absence of major modifications of the radial jet structure in the reported centrality classes. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Bello Martinez, H.; Cortes Maldonado, I.; Fernandez Tellez, A.; Martinez, M. I.; Moreno, L. A. P.; Navarro, S. R.; Noris, J. C. 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[Barbera, R.; La Rocca, P.; Petta, C.; Riggi, F.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.] Univ Padua, Dipartimento Fis & Astron, Padua, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Girard, M. Fusco; Meninno, E.; Pagano, P.; Virgili, T.] Univ Salerno, Dipartimento Fis ER Caianiello, Salerno, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Girard, M. Fusco; Meninno, E.; Pagano, P.; Virgili, T.] Ist Nazl Fis Nucl, Grp Collegato, Salerno, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Ist Nazl Fis Nucl, Grp Collegato, Alessandria, Italy. 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S.; Grigoras, A.; Grigoras, C.; Grosse-Oetringhaus, J. F.; Haake, R.; Hillemanns, H.; Hristov, P.; Kalweit, A.; Keil, M.; Klein, J.; Kluge, A.; Kofarago, M.; Kouzinopoulos, C.; Kryshen, E.; Lakomov, I.; Laudi, E.; Mager, M.; Manzari, V.; Martinengo, P.; Pedreira, M. Martinez; Milano, L.; Morsch, A.; Musa, L.; Niedziela, J.; Ohlson, A.; Pinazza, O.; Preghenella, R.; Reidt, F.; Riedler, P.; Riegler, W.; Ronchetti, F.; Rossi, A.; Safarik, K.; Schukraft, J.; Schutz, Y.; Senyukov, S.; Shahoyan, R.; Sielewicz, K. M.; Simonetti, G.; Szczepankiewicz, A.; Tauro, A.; Telesca, A.; Van Hoorne, J. W.; Vande Vyvre, P.; von Haller, B.; Vranic, D.; Weber, M.; Zampolli, C.; Zimmermann, M. B.] European Org Nucl Res CERN, Geneva, Switzerland. [Arnold, O. W.; Bilandzic, A.; Chauvin, A.; Dahms, T.; Epple, E.; Fabbietti, L.; Gasik, P.; Lapidus, K.; Munzer, R. H.; Doce, O. Vazquez; Vorobyev, I.] Tech Univ Munich, Excellence Cluster Univ, Munich, Germany. [Alme, J.; Helstrup, H.; Hetland, K. F.; Kileng, B.] Bergen Univ Coll, Fac Engn, Mons, Norway. [Meres, M.; Pikna, M.; Sitar, B.; Strmen, P.; Szabo, A.; Szarka, I.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Adam, J.; Bielcik, J.; Broz, M.; Cepila, J.; Contreras, J. G.; Eyyubova, G.; Horak, D.; Petracek, V.; Schulc, M.; Spacek, M.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, Prague, Czech Republic. [Bombara, M.; Kravcakova, A.; Sefcik, M.; Vrlakova, J.] Safarik Univ, Fac Sci, Kosice, Slovakia. [Langoy, R.; Lien, J.] Buskerud & Vestfold Univ Coll, Fac Technol, Vestfold, Norway. [Alt, T.; de Cuveland, J.; Gorbunov, S.; Hutter, D.; Kirsch, S.; Kisel, I.; Krzewicki, M.; Lindenstruth, V.; Rohr, D.; Zyzak, M.] Goethe Univ Frankfurt, Frankfurt Inst Adv Studies, Frankfurt, Germany. [Bhattacharjee, B.; Hussain, N.; Sarma, P.] Gauhati Univ, Dept Phys, Kangnung, South Korea. [Brucken, E. J.; Mieskolainen, M. M.; Orava, R.; Rasanen, S. S.; Saarinen, S.] Helsinki Inst Phys HIP, Helsinki, Finland. [Okubo, T.; Sekihata, D.; Shigaki, K.; Sugitate, T.; Yano, S.] Hiroshima Univ, Hiroshima, Japan. [Agrawal, N.; Dash, S.; Dhankher, P.; Jadhav, M. B.; Meethaleveedu, G. Koyithatta; Kumar, J.; Kumar, S.; Naik, B.; Nandi, B. K.; Nayak, R.; Pandey, A. K.; Varma, R.] Indian Inst Technol Bombay IIT, Mumbai, Maharashtra, India. [Behera, N. K.; Mishra, A. N.; Pareek, P.; Roy, A.; Sahoo, P.; Sahoo, R.; Thakur, D.] Indian Inst Technol Indore IITI, Indore, Madhya Pradesh, India. [Sumowidagdo, S.] Indonesian Inst Sci, Jakarta, Indonesia. [Behera, N. K.; Cho, S.; Kweon, M. J.; Yoon, J. H.] Inha Univ, Incheon, South Korea. [del Valle, Z. Conesa; Espagnon, B.; Hadjidakis, C.; Suire, C.; Tarhini, M.] Univ Paris 11, CNRS, Inst Phys Nucl Orsay IPNO, IN2P3, Orsay, France. [Breitner, T.; Engel, H.; Ramirez, A. Gomez; Kebschull, U.; Lara, C.] Goethe Univ Frankfurt, Inst Informat, Frankfurt, Germany. [Appelshaeuser, H.; Arslandok, M.; Bailhache, R.; Bartsch, E.; Beck, H.; Blume, C.; Book, J.; Broker, T. A.; Buesching, H.; Dillenseger, P.; Doenigus, B.; Drozhzhova, T.; Erdemir, I.; Heckel, S. T.; Hellbaer, E.; Kamin, J.; Klein, C.; Luettig, P.; Marquard, M.; Munzer, R. H.; Ozdemir, M.; Lezama, E. Perez; Peskov, V.; Rascanu, B. T.; Reichelt, P.; Renfordt, R.; Sahlmuller, B.; Schuchmann, S.; Toia, A.] Goethe Univ Frankfurt, Inst Kernphys, Frankfurt, Germany. [Bathen, B.; Cunqueiro, L.; Feldkamp, L.; Klein-Boesing, C.; De Godoy, D. A. Moreira; Muehlheim, D.; Passfeld, A.; Wessels, J. P.; Westerhoff, U.; Zimmermann, M. B.] Westtlil Wilhelms Univ Munster, Inst Kernphys, Munster, Germany. [Belikov, I.; Hamon, J. C.; Hippolyte, B.; Kuhn, C.; Maire, A.; Molnar, L.; Rami, F.; Roy, C.] Univ Strasbourg, CNRS IN2P3, Inst Pluridisciplinaire Hubert Curien IPHC, Strasbourg, France. [Finogeev, D.; Furs, A.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A.; Kurepin, A. B.; Maevskaya, A.; Pshenichnov, I.; Reshetin, A.; Shabanov, A.; Tikhonov, A.] Acad Sci, Inst Nucl Res, Moscow, Russia. [Bertens, R. A.; Bjelogrlic, S.; Caliva, A.; Dubla, A.; Grelli, A.; Keijdener, D. L. D.; Leogrande, E.; Lodato, D. F.; Margutti, J.; Mischke, A.; Mohammadi, N.; Nooren, G.; Peitzmann, T.; Rocco, E.; Snellings, R. J. M.; Van der Maarel, J.; van Leeuwen, M.; Veen, A. M.; Veldhoen, M.; Wang, H.; Zhang, C.] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Akindinov, A.; Kiselev, S.; Mal'Kevich, D.; Mikhaylov, K.; Nedosekin, A.; Sultanov, R.; Voloshin, K.; Zhigareva, N.] Inst Theoret & Expt Phys, Moscow, Russia. [Colella, D.; Jadlovsky, J.; Kalinak, P.; Kralik, I.; Krivda, M.; Musinsky, J.; Sandor, L.; Vala, M.] Slovak Acad Sci, Inst Expt Phys, Kosice, Slovakia. [Mares, J.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Baral, R. C.; Sahoo, S.; Sahu, P. K.] Inst Phys, Bhubaneswar, Orissa, India. [Danu, A.; Dobrin, A.; Gheata, M.; Haiduc, M.; Mitu, C. M.; Niculescu, M.; Ristea, C.; Sevcenco, A.; Stan, I.; Zgura, I. S.] Inst Space Sci ISS, Bucharest, Romania. [Cuautle, E.; Maldonado Cervantes, I.; Nellen, L.; Ortiz Velasquez, A.; Paic, G.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City, DF, Mexico. [Alfaro Molina, R.; Belmont-Moreno, E.; Gomez Coral, D. M.; Grabski, V.; Leon Vargas, H.; Menchaca-Rocha, A.; Sandoval, A.; Serradilla, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City, DF, Mexico. [Bossu, F.; Buthelezi, Z.; Foertsch, S.; Marchisone, M.; Murray, S.; Senosi, K.; Steyn, G.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Rogochaya, E.; Vodopyanov, A.] Joint Inst Nucl Res JINR, Dubna, Russia. [Baek, Y. W.; Oh, S. K.] Konkuk Univ, Seoul, South Korea. [Ahn, S. U.; Jang, H. J.] Korea Inst Sci & Technol Informat, Daejeon, South Korea. [Uysal, A. Karasu; Okatan, A.] KTO Karatay Univ, Konya, Turkey. [Barret, V.; Bastid, N.; Camejo, A. Batista; Crochet, P.; Dupieux, P.; Feuillard, V. J. G.; Li, S.; Lopez, X.; Manso, F.; Porteboeuf-Houssais, S.; Rosnet, P.; Palomo, L. Valencia; Vulpescu, B.] Clermont Univ, Univ Blaise Pascal, CNRS IN2P3, Lab Phys Corpusculaire LPC, Clermont Ferrand, France. [Balbastre, G. Conesa; Faivre, J.; Furget, C.; Guernane, R.; Silvestre, C.; Vauthier, A.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatotm & Cosmol, Grenoble, France. [Bianchi, N.; Diaz, L. Calero; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, A. R.; Ronchetti, F.; Sakai, S.; Spiriti, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Ricci, R. A.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Legnaro, Italy. [Bock, F.; Collu, A.; Fasel, M.; Gangadharan, D. R.; Jacobs, P. M.; Loizides, C.; Milano, L.; Ploskon, M.; Porter, J.; Thaeder, J.; Zhang, X.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Belyaev, V.; Bogdanov, A.; Grigoriev, V.; Ippolitov, M.; Kaplin, V.; Kondratyeva, N.; Loginov, V.; Melikyan, Y.; Peresunko, D.] Moscow Engn Phys Inst, Moscow, Russia. [Oyama, K.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Deloff, A.; Kovalenko, O.; Kurashvili, P.; Nair, R.; Redlich, K.; Siemiarczuk, T.; Wilk, G.] Natl Ctr Nucl Studies, Warsaw, Poland. [Andrei, C.; Berceanu, I.; Bercuci, A.; Herghelegiu, A.; Petrovici, M.; Pop, A.; Schiaua, C.; Tarzila, M. G.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Biswas, S.; Dash, A.; Mohanty, B.; Nayak, K.; Singh, R.; Singha, S.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Aleksandrov, D.; Blau, D.; Fokin, S.; Ippolitov, M.; Manko, V.; Nikolaev, S.; Nikulin, S.; Nyanin, A.; Peresunko, D.; Ryabinkin, E.; Sibiriak, Y.; Vasiliev, A.; Vinogradov, A.] Kurchatov Inst, Natl Res Ctr, Moscow, Russia. [Bearden, I. G.; Bilandzic, A.; Boggild, H.; Bourjau, C.; Chojnacki, M.; Christensen, C. H.; Gaardhoje, J. J.; Gulbrandsen, K.; Nielsen, B. S.; Pimentel, L. O. D. L.; Zaccolo, V.; Zhou, Y.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Christakoglou, P.; Deplano, C.; Dobrin, A.; Kuijer, P. G.; Lehas, F.; Manso, A. Rodriguez] Natl Inst subatomaire Fys, Nikhef, Amsterdam, Netherlands. [Borri, M.; Lemmon, R. C.] STFC Daresbury Lab, Nucl Phys Grp, Daresbury, England. [Adamova, D.; Bielcikova, J.; Ferencei, J.; Krizek, F.; Kucera, V.; Pospisil, J.; Sumbera, M.; Vanat, T.] Acad Sci Czech Republic, Inst Nucl Phys, Rez, Czech Republic. [Cormier, T. M.; Poghosyan, M. G.; Read, K. F.; Stankus, P.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Berdnikov, Y.; Ivanov, V.; Khanzadeev, A.; Kryshen, E.; Malaev, M.; Nikulin, V.; Riabov, V.; Ryabov, Y.; Samsonov, V.; Zhalov, M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Cherney, M.; Poghosyan, M. G.; Seger, J. E.] Creighton Univ, Dept Phys, Omaha, NE USA. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Parmar, S.; Rathee, D.] Panjab Univ, Dept Phys, Chandigarh, India. [Ganoti, P.; Kostarakis, P.; Roukoutakis, F.; Spyropoulou-Stassinaki, M.; Vasileiou, M.] Univ Athens, Dept Phys, Athens, Greece. [Bhasin, A.; Bhat, I. R.; Gupta, A.; Kour, M.; Kumar, A.; Sharma, A.; Sharma, M.] Univ Jammu, Dept Phys, Jammu, India. [Raniwala, R.; Raniwala, S.] Univ Rajasthan, Dept Phys, Jaipur, Rajasthan, India. [Arnold, O. W.; Bilandzic, A.; Chauvin, A.; Dahms, T.; Epple, E.; Fabbietti, L.; Gasik, P.; Lapidus, K.; Munzer, R. H.; Doce, O. Vazquez; Vorobyev, I.] Tech Univ Munich, Dept Phys, Munich, Germany. [Anguelov, V.; Beck, H.; Bock, F.; Danisch, M. C.; Deisting, A.; Fleck, M. G.; Glaessel, P.; Karayan, L.; Klewin, S.; Knichel, M. L.; Leardini, L.; Perez, J. Mercado; Oeschler, H.; Oyama, K.; Pachmayer, Y.; Reidt, F.; Reygers, K.; Schicker, R.; Stachel, J.; Stiller, J. H.; Voelkl, M. A.; Weiser, D. F.; Wilkinson, J.; Windelband, B.; Winn, M.; Zimmermann, A.] Heidelberg Univ, Physikal Inst, Heidelberg, Germany. [Browning, T. A.] Purdue Univ, W Lafayette, IN USA. [Borissov, A.; Choi, K.; Chunng, S. U.; Eum, J.; Song, J.; Yoo, I. -K.] Pusan Natl Univ, Pusan, South Korea. [Andronic, A.; Averbeck, R.; Braun-Munzinger, P.; Deisting, A.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Gronefeld, J. M.; Grosso, R.; Ivanov, M.; Bustamante, R. T. Jimenez; Karayan, L.; Kollegger, T.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Sozzi, F.; Vranic, D.; Wagner, J.; Weber, S. G.] GSI Helmholtzzentrum Schwerionenforschung, Res Div & ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, T.] Rudjer Boskovie Inst, Zagreb, Croatia. [Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Chattopadhyay, S.; Das, D.; Das, I.; Khan, P.; Paul, B.; Roy, P.; Sinha, T.] Saha Inst Nucl Phys, Kolkata, India. [Alexandre, D.; Barnby, L. S.; Evans, D.; Graham, K. L.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lictava, R.; Baillie, O. Villalobos; Zardoshti, N.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Calvo Villar, E.; Endress, E.; Gago, A. M.] Pontificia Univ Catel Peru, Dept Ciencias, Sec Fis, Lima, Peru. [de Cataldo, G.; Elia, D.; Lenti, V.; Manzari, V.; Nappi, E.; Paticchio, V.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Alici, A.; Antonioli, P.; Cindolo, F.; Hatzifotiadou, D.; Margotti, A.; Nania, R.; Noferini, F.; Pinazza, O.; Preghenella, R.; Scapparone, E.; Williams, M. C. S.; Zampolli, C.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Cicalo, C.; Masoni, A.; Siddhanta, S.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Badala, A.; Pappalardo, G. S.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Antinori, F.; Dainese, A.; Fabris, D.; Ruzza, B. D.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Bedda, C.; Bruna, E.; Cerello, P.; Morales, Y. Corrales; De Marco, N.; Feliciello, A.; Giubellino, P.; La Pointe, S. L.; Oppedisano, C.; Paul, B.; Prino, F.; Scomparin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] SSC THEP NRC Kurchatov Inst, Protvino, Russia. [Lehner, S.; Weber, M.] Stefan Meyer Inst Subatomare Phys SMI, Vienna, Austria. [Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Blanco, J. Martin; Martinez Garcia, G.; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, CNRS IN2P3, Ecole Mines Nantes, SUBATECH, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cabala, J.; Cerkala, J.; Jadlovska, S.; Jadlovsky, J.; Kopcik, M.; Oravec, M.] Tech Univ Kosice, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vinogradov, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Bhom, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas, Dept Phys, Austin, TX USA. [Almaraz, J. R. M.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Domenicis Gimenez, D.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Mas, A.; Munhoz, M. G.; Natal da Luz, H.; Oliveira Da Silva, A. C.; Suaide, A. A. P.; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Albuquerque, D. S. D.; Chinellato, D. D.; de Souza, R. D.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Knospe, A. G.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.] Univ Liverpool, Liverpool, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Murakami, H.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, Univ Lyon, IPN Lyon, CNRS IN2P3, Villeurbanne, France. [Pagano, D.] Univ Brescia, Brescia, Italy. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Sadhu, S.; Saini, J.; Sarkar, D.; Sarkar, N.; Sheikh, A. I.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Biro, G.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Balasubramanian, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Lutz, T. H.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul, South Korea. [Keidel, R.] Fachhochschule Worms, Zentrum Technologietransfer & Telekommunikat ZTT, Worms, Germany. [Connors, M. E.] Georgia State Univ, Atlanta, GA USA. [Khan, M. Mohisin] Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, Prague, Czech Republic. RI Kovalenko, Vladimir/C-5709-2013 OI Kovalenko, Vladimir/0000-0001-6012-6615 FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology; Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi, Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; apan Society for the Promotion of Science (JSPS) KAKENHI; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique, European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian FederalAgency of Atomic Energy; Russian FederalAgency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, SouthAfrica; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones TecnolA, sgicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut and AliceWallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial-Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi, Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique, European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian FederalAgency of Atomic Energy, Russian FederalAgency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, SouthAfrica; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones TecnolA, sgicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut and AliceWallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial-Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 58 TC 1 Z9 1 U1 2 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAY 17 PY 2016 VL 76 IS 5 DI 10.1140/epjc/s10052-016-4107-8 PG 16 WC Physics, Particles & Fields SC Physics GA EO2KS UT WOS:000396526000001 ER PT J AU He, Y Gu, M Xiao, HY Luo, LL Shao, YY Gao, F Du, YG Mao, SX Wang, CM AF He, Yang Gu, Meng Xiao, Haiyan Luo, Langli Shao, Yuyan Gao, Fei Du, Yingge Mao, Scott X. Wang, Chongmin TI Atomistic Conversion Reaction Mechanism of WO3 in Secondary Ion Batteries of Li, Na, and Ca SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE conversion; in situ TEM; intercalation; ion batteries; WO3 ID TRANSMISSION ELECTRON-MICROSCOPY; ELECTROCHEMICAL LITHIATION; LITHIUM BATTERIES; OXIDE; NANOPARTICLES; SODIATION; INSERTION; CATHODES; LIXWO3; ANODE AB Intercalation and conversion are two fundamental chemical processes for battery materials in response to ion insertion. The interplay between these two chemical processes has never been directly seen and understood at atomic scale. Here, using in situ HRTEM, we captured the atomistic conversion reaction processes during Li, Na, Ca insertion into a WO3 single crystal model electrode. An intercalation step prior to conversion is explicitly revealed at atomic scale for the first time for Li, Na, Ca. Nanoscale diffraction and ab initio molecular dynamic simulations revealed that after intercalation, the inserted ion-oxygen bond formation destabilizes the transition-metal framework which gradually shrinks, distorts and finally collapses to an amorphous W and MxO (M = Li, Na, Ca) composite structure. This study provides a full atomistic picture of the transition from intercalation to conversion, which is of essential importance for both secondary ion batteries and electrochromic devices. C1 [He, Yang; Luo, Langli; Du, Yingge; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [He, Yang; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Xiao, Haiyan] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Shao, Yuyan] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Gao, Fei] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. RP Du, YG; Wang, CM (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.; Mao, SX (reprint author), Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA.; Gao, F (reprint author), Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. EM gaofeium@umich.edu; yingge.du@pnnl.gov; sxm2@pitt.edu; chongmin.wang@pnnl.gov RI Shao, Yuyan/A-9911-2008; Luo, Langli/B-5239-2013; OI Shao, Yuyan/0000-0001-5735-2670; Luo, Langli/0000-0002-6311-051X FU Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231, 6951379]; Office of Basic Energy Sciences, Division of Materials Science and Engineering [10122]; U.S. Department of Energy (DOE) [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 6951379 under the advanced Battery Materials Research (BMR) program. Y.D. acknowledges support on film growth by the Office of Basic Energy Sciences, Division of Materials Science and Engineering under Award 10122 and EMSL's Intramural Research and Capability Development Program. PNNL is a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy (DOE) under Contract DE-AC05-76RL01830. The research was performed using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. NR 25 TC 3 Z9 3 U1 49 U2 97 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY 17 PY 2016 VL 55 IS 21 BP 6244 EP 6247 DI 10.1002/anie.201601542 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DO6UG UT WOS:000377918400019 PM 27071488 ER PT J AU Bielicki, JM Pollak, MF Deng, H Wilson, EJ Fitts, JP Peters, CA AF Bielicki, Jeffrey M. Pollak, Melisa F. Deng, Hang Wilson, Elizabeth J. Fitts, Jeffrey P. Peters, Catherine A. TI The Leakage Risk Monetization Model for Geologic CO2 Storage SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CARBON-DIOXIDE SEQUESTRATION; AQUIFERS; IMPACTS; CAPTURE; CEMENT; GROUNDWATER; INTEGRITY; MIGRATION; FRAMEWORK; HEALTH AB We developed the Leakage Risk Monetization Model (LRiMM) which integrates simulation of CO2 leakage from geologic CO, storage reservoirs with estimation of monetized leakage risk (MLR). Using geospatial data, LRiMM quantifies financial responsibility if leaked CO2 or brine interferes with subsurface resources, and estimates the MLR reduction achievable by remediating leaks. We demonstrate LRiMM with simulations of 30 years of injection into the Mt. Simon sandstone at two locations that differ primarily in their proximity to existing wells that could be leakage pathways. The peak MLR for the site nearest the leakage pathways ($7.5/tCO(2)) was 190x larger than for the farther injection site, illustrating how careful siting would minimize MLR in heavily used sedimentary basins. Our MLR projections are at least an order of magnitude below overall CO2 storage costs at well-sited locations, but some stakeholders may incur substantial costs. Reliable methods to detect and remediate leaks could further minimize MLR For both sites, the risk of CO2 migrating to potable aquifers or reaching the atmosphere was negligible due to secondary trapping, whereby multiple impervious sedimentary layers trap CO2 that has leaked through the primary seal of the storage formation. C1 [Bielicki, Jeffrey M.] Ohio State Univ, Dept Civil Environm & Geodet Engn, Columbus, OH 43210 USA. [Bielicki, Jeffrey M.] Ohio State Univ, John Glenn Coll Publ Affairs, Columbus, OH 43210 USA. [Pollak, Melisa F.; Wilson, Elizabeth J.] Univ Minnesota, Hubert H Humphrey Sch Publ Affairs, Minneapolis, MN 55455 USA. [Deng, Hang; Fitts, Jeffrey P.; Peters, Catherine A.] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [Pollak, Melisa F.] Barr Engn Co, 4700 West 77th St, Minneapolis, MN 55435 USA. [Deng, Hang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Geosci Div, 1 Cyclotron Rd Mailstop 74R316C, Berkeley, CA 94720 USA. RP Bielicki, JM (reprint author), Ohio State Univ, Dept Civil Environm & Geodet Engn, Columbus, OH 43210 USA.; Bielicki, JM (reprint author), Ohio State Univ, John Glenn Coll Publ Affairs, Columbus, OH 43210 USA. EM bielicki.2@osu.edu RI Deng, Hang/E-5302-2015; Bielicki, Jeffrey/D-4239-2016 OI Deng, Hang/0000-0001-5784-996X; Bielicki, Jeffrey/0000-0001-8449-9328 FU U.S. Department of Energy, Office of Fossil Energy [DE-FE-0000749]; National Science Foundation under Sustainable Energy Pathways program [1230691]; [CBET-1133849] FX This research was funded by the U.S. Department of Energy, Office of Fossil Energy (Grant DE-FE-0000749), and by the National Science Foundation under Sustainable Energy Pathways program (Grant 1230691) and Grant CBET-1133849. NR 48 TC 0 Z9 0 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 4923 EP 4931 DI 10.1021/acs.est.5b05329 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500004 PM 27052112 ER PT J AU Salter-Blanc, AJ Bylaska, EJ Lyon, MA Ness, SC Tratnyek, PG AF Salter-Blanc, Alexandra J. Bylaska, Eric J. Lyon, Molly A. Ness, Stuart C. Tratnyek, Paul G. TI Structure-Activity Relationships for Rates of Aromatic Amine Oxidation by Manganese Dioxide SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ONE-ELECTRON OXIDATION; SEDIMENT-ASSOCIATED REACTIONS; SUBSTITUTED ANILINES; NITROAROMATIC COMPOUNDS; AQUEOUS-SOLUTION; RATE CONSTANTS; ORGANIC CONTAMINANTS; FLASH-PHOTOLYSIS; REDUCTION; REACTIVITY AB New energetic compounds are designed to minimize their potential environmental impacts, which includes their transformation and the fate and effects of their transformation products. The nitro groups of energetic compounds are readily reduced to amines, and the resulting aromatic amines are subject to oxidation and coupling reactions. Manganese dioxide (MnO2) is a common environmental oxidant and model system for kinetic studies of aromatic amine oxidation. In this study, a training set of new and previously reported kinetic data for the oxidation of model and energetic-derived aromatic amines was assembled and subjected to correlation analysis against descriptor variables that ranged from general purpose [Hammett sigma constants (sigma(-)), pK(a)s of the amines, and energies of the highest occupied molecular orbital (E-HOMO)] to specific for the likely rate-limiting step [one-electron oxidation potentials (E-ox]. The selection of calculated descriptors (pK(a), E-HOMO, and E-ox) was based on validation with experimental data. All of the correlations gave satisfactory quantitative structure-activity relationships (QSARs), but they improved with the specificity of the descriptor. The scope of correlation analysis was extended beyond MnO2 to include literature data on aromatic amine oxidation by other environmentally relevant oxidants (ozone, chlorine dioxide, and phosphate and carbonate radicals) by correlating relative rate constants (normalized to 4-chloroaniline) to E-HOMO (calculated with a modest level of theory). C1 [Salter-Blanc, Alexandra J.; Lyon, Molly A.; Ness, Stuart C.; Tratnyek, Paul G.] Oregon Hlth & Sci Univ, Inst Environm Hlth, 3181 SW Sam Jackson Pk Rd, Portland, OR 97239 USA. [Bylaska, Eric J.] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. RP Tratnyek, PG (reprint author), Oregon Hlth & Sci Univ, Inst Environm Hlth, 3181 SW Sam Jackson Pk Rd, Portland, OR 97239 USA. EM tratnyek@ohsu.edu FU Strategic Environmental Research and Development Program (SERDP) [ER-1735]; DOE's Office of Biological and Environmental Research [DE-AC06-76RLO 1830] FX This work was supported by the Strategic Environmental Research and Development Program (SERDP) under ER-1735. This report has not been subject to review by SERDP and therefore does not necessarily reflect their views, and no official endorsement should be inferred. A. J. S.-B. was supported as an OHSU Graduate Research Scholar during a portion of this study. A portion of this research was performed using the Institutional Computing facility (PIC) at the Pacific Northwest National Laboratory (PNNL) and the Chinook, Barracuda, and Cascade computing resources at the Environmental Molecular Sciences Laboratory (EMSL). PNNL is operated by Battelle Memorial Institute for the U.S. Department of Energy (DOE). EMSL is a national scientific user facility located at PNNL and sponsored by the DOE's Office of Biological and Environmental Research (DE-AC06-76RLO 1830). We also acknowledge EMSL for supporting the development of NWChem. Structure database management and some property prediction was performed using Instant JChem (Instant JChem 5.9.4, 2012, ChemAxon [http://www.chemaxon.com]). Anne Bentley (Lewis & Clark College) performed the X-ray diffraction on the MnO2. NR 70 TC 1 Z9 1 U1 16 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 5094 EP 5102 DI 10.1021/acs.est.6b00924 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500023 PM 27074054 ER PT J AU Burant, A Thompson, C Lowry, GV Karamalidis, AK AF Burant, Aniela Thompson, Christopher Lowry, Gregory V. Karamalidis, Athanasios K. TI New Linear Partitioning Models Based on Experimental Water: Supercritical CO2 Partitioning Data of Selected Organic Compounds SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID STRUCTURE-PROPERTY RELATIONSHIPS; GEOLOGICAL SEQUESTRATION; AQUEOUS SOLUBILITY; CARBON-DIOXIDE; COEFFICIENTS; MIXTURES; CONTAMINANTS; PREDICTION; EXTRACTION; SOLUTES AB Partitioning coefficients of organic compounds between water and supercritical CO2 (sc-CO2) are necessary to assess the risk of migration of these chemicals from subsurface CO2 storage sites. Despite the large number of potential organic contaminants, the current data set of published water sc-CO2 partitioning coefficients is very limited. Here, the partitioning coefficients of thiophene, pyrrole, and anisole were measured in situ over a range of temperatures and pressures using a novel pressurized batch-reactor system with dual spectroscopic detectors: a near-infrared spectrometer for measuring the organic analyte in the CO2 phase and a UV detector for quantifying the analyte in the aqueous phase. Our measured partitioning coefficients followed expected trends based on volatility and aqueous solubility. The partitioning coefficients and literature data were then used to update a published poly parameter linear free-energy relationship and to develop five new linear free-energy relationships for predicting water sc-CO2 partitioning coefficients. A total of four of the models targeted a single class of organic compounds. Unlike models that utilize Abraham solvation parameters, the new relationships use vapor pressure and aqueous solubility of the organic compound at 25 degrees C and CO2 density to predict partitioning coefficients over a range of temperature and pressure conditions. The compound class models provide better estimates of partitioning behavior for compounds in that class than does the model built for the entire data set. C1 [Burant, Aniela; Lowry, Gregory V.; Karamalidis, Athanasios K.] Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA. [Thompson, Christopher] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Karamalidis, AK (reprint author), Carnegie Mellon Univ, Dept Civil & Environm Engn, Pittsburgh, PA 15213 USA. EM akaramal@andrew.cmu.edu FU National Energy Technology Laboratory; Department of Energy by Battelle Memorial Institute [DE-AC05-76RLO-1830]; Jared and Maureen Cohon Fellowship in Environmental Engineering; Bradford and Diane Smith Fellowship in Engineering FX This work was funded under the National Energy Technology Laboratory's former Regional University Alliance. Part of this research was performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility at PNNL that is managed by the DOE's Office of Biological and Environmental Research. PNNL is operated for the Department of Energy by Battelle Memorial Institute under contract no. DE-AC05-76RLO-1830. Zheming Wang and John Loring provided useful assistance with the FTIR. The Jared and Maureen Cohon Fellowship in Environmental Engineering and the Bradford and Diane Smith Fellowship in Engineering are acknowledged for additional support. NR 29 TC 1 Z9 1 U1 11 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 5135 EP 5142 DI 10.1021/acs.est.6b00301 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500028 PM 27081725 ER PT J AU Piens, DS Kelly, ST Harder, TH Petters, MD O'Brien, RE Wang, BB Teske, K Dowell, P Laskin, A Gilles, MK AF Piens, Dominique S. Kelly, Stephen T. Harder, Tristan H. Petters, Markus D. O'Brien, Rachel E. Wang, Bingbing Teske, Ken Dowell, Pat Laskin, Alexander Gilles, Mary K. TI Measuring Mass-Based Hygroscopicity of Atmospheric Particles through in Situ Imaging SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID LIQUID PHASE-SEPARATION; BURNING AEROSOL-PARTICLES; X-RAY SPECTROMICROSCOPY; ACTIVITY-COEFFICIENTS; WATER-UPTAKE; CHEMICAL-COMPOSITION; THERMODYNAMIC MODEL; AMMONIUM-SULFATE; ACID PARTICLES; TRANSMISSION AB Quantifying how atmospheric particles interact with water vapor is critical for understanding the effects of aerosols on climate. We present a novel method to measure the mass-based hygroscopicity of particles while characterizing their elemental and carbon functional group compositions. Since mass-based hygroscopicity is insensitive to particle geometry, it is advantageous for probing the hygroscopic behavior of atmospheric particles, which can have irregular morphologies. Combining scanning electron microscopy with energy dispersive X-ray analysis (SEM/EDX), scanning transmission X-ray microscopy (STXM) analysis, and in situ STXM humidification experiments, this method was validated using laboratory-generated, atmospherically relevant particles. Then, the hygroscopicity and elemental composition of 15 complex atmospheric particles were analyzed by leveraging quantification of C, N, and O from STXM, and complementary elemental quantification from SEM/EDX. We found three types of hygroscopic responses, and correlated high hygroscopicity with Na and Cl content. The mixing state of 158 other particles from the sample broadly agreed with those of the humidified particles, indicating the potential to infer atmospheric hygroscopic behavior from a selected subset of particles. These methods offer unique quantitative capabilities to characterize and correlate the hygroscopicity and chemistry of individual submicrometer atmospheric particles. C1 [Piens, Dominique S.; Harder, Tristan H.; O'Brien, Rachel E.; Gilles, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Harder, Tristan H.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Petters, Markus D.] N Carolina State Univ, Dept Marine Earth & Atmospher Sci, Box 8208, Raleigh, NC 27695 USA. [Wang, Bingbing; Laskin, Alexander] Pacific NW Natl Lab, William R Wiley Environm & Mol Sci Lab, Richland, WA 99352 USA. [Teske, Ken; Dowell, Pat] Atmospher Radiat Monitoring Southern Great Plains, 109596 Coal Rd, Billings, OK 74630 USA. [Piens, Dominique S.] Stanford Univ, Stanford, CA 94305 USA. [Kelly, Stephen T.] Carl Zeiss Xray Microscopy Inc, Pleasanton, CA 94588 USA. [O'Brien, Rachel E.] MIT, Dept Civil & Environm Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Wang, Bingbing] Xiamen Univ, Coll Ocean & Earth Sci, State Key Lab Marine Environm Sci, Xiamen 361102, Peoples R China. RP Piens, DS; Gilles, MK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Piens, DS (reprint author), Stanford Univ, Stanford, CA 94305 USA. EM dpiens@stanford.edu; mkgilles@lbl.gov RI Laskin, Alexander/I-2574-2012; Harder, Tristan/H-8186-2016; Petters, Markus/D-2144-2009 OI Laskin, Alexander/0000-0002-7836-8417; Harder, Tristan/0000-0001-8352-6494; Petters, Markus/0000-0002-4082-1693 FU Atmospheric Systems Research (ASR) of the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research (OBER) program; DOE, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program; DOE ASR; Office of Science, Office of Basic Energy Sciences (BES) of the U.S. DOE [DE-AC02-05CH11231]; Chemical Imaging Initiative of the Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL); DOE OBER; U.S. DOE by Battelle Memorial Institute [DE-AC06-76RL0 1830] FX STXM/NEXAFS dry characterization experiments (MKG, STK, THH) were supported by the Atmospheric Systems Research (ASR) of the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research (OBER) program. Dry STXM/NEXAFS analysis of the field samples (T.H.H.) was partially supported by the German National Academic Foundation. Development of the MATLAB scripts and analysis for the mass-based water vapor uptake analysis (D.S.P.) was supported through the DOE, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internship (SULI) program. R.E.O. (supported by DOE ASR) provided analysis guidance to both D.S.P. and T.H.H. The experimental portion of the water vapor uptake experiments (S.T.K., M.K.G.) and assistance with the interpretation of the data (M.P.) was supported by the ASR DOE OBER program. STXM/NEXAFS measurements were done with the assistance of Tolek Tyliszczak at Beamline 11.0.2 of the Advanced Light Source (ALS) at Lawrence Berkeley National Laboratory (LBNL). The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences (BES), of the U.S. DOE under Contract No. DE-AC02-05CH11231. Beamline 11.0.2 is supported under the same contract as well as the Condensed Phase and Interfacial Molecular Sciences Program of DOE BES. A.L. and B.W. acknowledge support from the Chemical Imaging Initiative of the Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL). The preparation of laboratory samples and SEM/EDX measurements were performed at the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL) - a national scientific user facility located at PNNL, and sponsored by DOE OBER. PNNL is operated for U.S. DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RL0 1830. Samples were collected (K.T., P.D.) at the Atmospheric Radiation Monitoring (ARM) site located at Southern Great Plains and sponsored by DOE OBER. NR 47 TC 2 Z9 2 U1 8 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 5172 EP 5180 DI 10.1021/acs.est.6b00793 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500032 PM 27088454 ER PT J AU Lee, J Im, J Kim, U Loffler, FE AF Lee, Jaejin Im, Jeongdae Kim, Ungtae Loeffler, Frank E. TI A Data Mining Approach to Predict In Situ Detoxification Potential of Chlorinated Ethenes SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID REDUCTIVE DECHLORINATION; SOURCE ZONE; CONTAMINATED GROUNDWATER; ANAEROBIC BIOREMEDIATION; BACTERIAL COMMUNITY; VINYL-CHLORIDE; PH CONTROL; ROC CURVE; DEHALOCOCCOIDES; BIOAUGMENTATION AB Despite advances in physicochemical remediation technologies, in situ bioremediation treatment based on Dehalococcoides mccartyi (Dhc) reductive dechlorination activity remains a cornerstone approach to remedy sites impacted with chlorinated ethenes. Selecting the best remedial strategy is challenging due to uncertainties and complexity associated with biological and geochemical factors influencing Dhc activity. Guidelines based on measurable biogeochemical parameters have been proposed, but contemporary efforts fall short of meaningfully integrating the available information. Extensive groundwater monitoring data sets have been collected for decades, but have not been systematically analyzed and used for developing tools to guide decision-making. In the present study, geochemical and microbial data sets collected from 35 wells at five contaminated sites were used to demonstrate that a data mining prediction model using the classification and regression tree (CART) algorithm can provide improved predictive understanding of a site's reductive dechlorination potential. The CART model successfully predicted the 3-month-ahead reductive dechlorination potential with 75.8% and 69.5% true positive rate (i.e:,sensitivity) for the training set and the test set, respectively. The machine learning algorithm ranked parameters by relative importance for assessing in situ reductive dechlorination potential. The abundance of Dhc 16S rRNA genes, CH4, Fe2+, NO3-, NO2-, and SO42- concentrations, total organic carbon (TOC) amounts, and oxidation reduction potential (ORP) displayed significant correlations (p < 0.01) with dechlorination potential, with NO3-, NO2-, and Fe2+ concentrations. exhibiting precedence over other parameters. Contrary to prior efforts, the power of data mining approaches lies in the ability to discern synergetic effects between multiple parameters that affect reductive dechlorination activity. Overall, these findings demonstrate that data mining techniques (e.g., machine learning algorithms) effectively utilize groundwater monitoring,data to derive predictive understanding of contaminant degradation, and thus have great potential for improving decision-making, tools, A major need for realizing the predictive capabilities of data mining approaches is a curated, open-access, up-to-date and comprehensive collection of biogeochemical groundwater monitoring data. C1 [Lee, Jaejin; Im, Jeongdae; Loeffler, Frank E.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Lee, Jaejin; Im, Jeongdae; Loeffler, Frank E.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA. [Kim, Ungtae] Cleveland State Univ, Dept Civil & Environm Engn, Cleveland, OH 44115 USA. [Loeffler, Frank E.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Loeffler, Frank E.] Univ Tennessee, Oak Ridge, TN 37831 USA. [Loeffler, Frank E.] Oak Ridge Natl Lab UT ORNL, JIBS, Oak Ridge, TN 37831 USA. [Loeffler, Frank E.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Im, Jeongdae] Univ Massachusetts, Dept Microbiol, Amherst, MA 01002 USA. RP Loffler, FE (reprint author), Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA.; Loffler, FE (reprint author), Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37996 USA.; Loffler, FE (reprint author), Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA.; Loffler, FE (reprint author), Univ Tennessee, Oak Ridge, TN 37831 USA.; Loffler, FE (reprint author), Oak Ridge Natl Lab UT ORNL, JIBS, Oak Ridge, TN 37831 USA.; Loffler, FE (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM frank.loeffler@utk.edu FU Strategic Environmental Research and Development Program (SERDP) [ER-2312]; Environmental Security Technology Certification Program (ESTCP) [ER-1129] FX Funding for this study was provided by the Strategic Environmental Research and Development Program (SERDP) under Project ER-2312 and the Environmental Security Technology Certification Program (ESTCP) under Project ER-1129. The content of this manuscript has not been subject to agency review and does not necessarily represent the view of the sponsoring agency. We are grateful to Microbial Insights, Inc. (MI) and Chicago Bridge & Iron Company (CB&I) for providing us with biogeochemical data sets enabling the development of the data mining approach. NR 62 TC 1 Z9 1 U1 9 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 5181 EP 5188 DI 10.1021/acs.est.5b05090 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500033 PM 27116079 ER PT J AU Smith, FN Um, W Taylor, CD Kim, DS Schweiger, MJ Kruger, AA AF Smith, Frances N. Um, Wooyong Taylor, Christopher D. Kim, Dong-Sang Schweiger, Michael J. Kruger, Albert A. TI Computational Investigation of Technetium(IV) Incorporation into Inverse Spinels: Magnetite (Fe3O4) and Trevorite (NiFe2O4) SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID TITANOMAGNETITE FE3-XTIXO4 NANOPARTICLES; DENSITY-FUNCTIONAL THEORY; HEMATITE ALPHA-FE2O3; HETEROGENEOUS REDUCTION; POWDER DIFFRACTION; GLASSY MATERIALS; STEEL SURFACES; ATOM EXCHANGE; FERROUS IRON; WASTE FORM AB Iron oxides and oxyhydroxides play an important role in minimizing the mobility of redox-sensitive elements in engineered and natural environments. For the radionuclide technetium-99 (Tc), these phases hold promise as primary hosts for increasing Tc loading into glass waste form matrices, or as secondary sinks during the long-term storage of nuclear materials. Recent experiments show that the inverse spinel, magnetite [Fe(II)Fe(III)(2)O-4], can incorporate Tc(IV) into its octahedral sublattice. In that same class of materials, trevorite [Ni(II)Fe(III)(2)O-4] is also being investigated for its ability to host Tc(IV). However, questions remain regarding the most energetically favorable charge compensation mechanism for Tc(IV) incorporation in each structure, which will affect Tc behavior under changing waste processing or storage conditions. Here, quantum-mechanical methods were used to evaluate incorporation energies and optimized lattice bonding environments for three different, charge-balanced Tc(IV) incorporation mechanisms in magnetite and trevorite (similar to 5 wt % Tc). For both phases, the removal of two octahedral Fen or Ni(II) ions upon the addition of Tc(IV) in an octahedral site is the most stable mechanism, relative to the creation of octahedral Fe(III) defects or increasing octahedral Fe(II) content. Following hydration-energy corrections, Tc(IV) incorporation into magnetite is energetically favorable while an energy barrier exists for trevorite. C1 [Smith, Frances N.; Um, Wooyong; Kim, Dong-Sang; Schweiger, Michael J.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. [Um, Wooyong] Pohang Univ Sci & Technol POSTECH, Pohang, South Korea. [Taylor, Christopher D.] Ohio State Univ, Fontana Corros Ctr Mat Sci & Engn, Columbus, OH 43210 USA. [Taylor, Christopher D.] DNV GL, Strateg Res & Innovat, Dublin, OH 43017 USA. [Kruger, Albert A.] US DOE, Off River Protect, POB 450, Richland, WA 99352 USA. RP Um, W (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99354 USA. EM Wooyong.um@pnnl.gov FU U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Project of the Office of River Protection FX This research was supported by the U.S. Department of Energy's (DOE) Waste Treatment and Immobilization Plant Project of the Office of River Protection. This research was performed using PNNL Institutional Computing at Pacific Northwest National Laboratory. We gratefully acknowledge T.S. Carlson, K.R. Glaesemann for computational support and E. Kim for guidance and discussion. NR 60 TC 6 Z9 6 U1 15 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 17 PY 2016 VL 50 IS 10 BP 5216 EP 5224 DI 10.1021/acs.est.6b00200 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DM4QJ UT WOS:000376331500037 PM 27049925 ER PT J AU Morrow, BM Kozar, RW Anderson, KR Mills, MJ AF Morrow, B. M. Kozar, R. W. Anderson, K. R. Mills, M. J. TI Substructure evolution of Zircaloy-4 during creep and implications for the Modified Jogged-Screw model SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Creep; Strain evolution; Jogged-screw dislocation; Mechanistic modeling; Zirconium; Zircaloy ID HIGH-TEMPERATURE CREEP; MICROSTRUCTURAL EVOLUTION; BEHAVIOR AB Several specimens of Zircaloy-4 were creep tested at a single stress-temperature condition, and interrupted at different accumulated strain levels. Substructural observations were performed using bright field scanning transmission electron microscopy (BF STEM). The dislocation substructure was characterized to ascertain how creep strain evolution impacts the Modified Jogged-Screw (MJS) model, which has previously been utilized to predict steady-state strain rates in Zircaloy-4. Special attention was paid to the evolution of individual model parameters with increasing strain. Results of model parameter measurements are reported and discussed, along with possible extensions to the MJS model. Published by Elsevier B.V. C1 [Morrow, B. M.; Mills, M. J.] Ohio State Univ, 2041 Coll Rd,477 Watts Hall, Columbus, OH 43210 USA. [Morrow, B. M.] Los Alamos Natl Lab, POB 1663,MS G755, Los Alamos, NM 87545 USA. [Kozar, R. W.; Anderson, K. R.] Bechtel Marine Prop Corp, Bettis Lab, West Mifflin, PA 15122 USA. RP Morrow, BM (reprint author), Los Alamos Natl Lab, POB 1663,MS G755, Los Alamos, NM 87545 USA. EM morrow@lanl.gov; millsmj@mse.osu.edu OI Morrow, Benjamin/0000-0003-1925-4302 NR 20 TC 1 Z9 1 U1 1 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 17 PY 2016 VL 665 BP 90 EP 97 DI 10.1016/j.msea.2016.04.014 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DN0WO UT WOS:000376788000011 ER PT J AU Zecevic, M Knezevic, M Beyerlein, IJ McCabe, RJ AF Zecevic, Miroslav Knezevic, Marko Beyerlein, Irene J. McCabe, Rodney J. TI Origin of texture development in orthorhombic uranium SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Orthorhombic structure; Uranium; Texture; Rolling; Crystal plasticity ID POLYCRYSTALLINE HCP/BCC COMPOSITES; IMPLICIT FINITE-ELEMENTS; STRAIN-PATH CHANGES; ZINC ALLOY SHEET; ALPHA-URANIUM; HEXAGONAL MATERIALS; DISLOCATION DENSITY; MECHANICAL RESPONSE; PLASTICITY MODEL; FAST COMPUTATION AB We study texture evolution of alpha-uranium (alpha-U) during plane strain compression and uniaxial compression to high strains at different temperatures. We combine a multiscale polycrystal constitutive model and detailed analysis of texture data to uncover the slip and twinning modes responsible for the formation of individual texture components. The analysis indicates that during plane strain compression, floor slip (001)[100] results in the formation of two pronounced {001} texture peaks tilted 10-15 degrees away from the normal toward the rolling direction. During both high-temperature (573 K) through-thickness compression and plane strain compression, the active slip modes are floor slip (001)[100] and chimney slip 1/2{110}< 1 (1) over bar0 > with slightly different ratios. {130}< 3 (1) over bar0 > deformation twinning is profuse during rolling and in-plane compression and decreases with increasing temperature, but is not as active for through-thickness compression. Finally, we comment on some similarities between rolling textures of cc U, which has a c/a ratio of 1.734, and those that develop in hexagonal close packed metals with similarly high c/a ratios like Zn (1.856) and Cd (1.885) and are dominated by basal slip. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zecevic, Miroslav; Knezevic, Marko] Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [McCabe, Rodney J.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Knezevic, M (reprint author), Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. EM marko.knezevic@unh.edu OI McCabe, Rodney /0000-0002-6684-7410 FU CEPS Graduate Fellowships program at the University of New Hampshire (UNH); Los Alamos National Laboratory [277871]; Laboratory Directed Research and Development grant [20140630ER] FX M.Z. acknowledges support from the CEPS Graduate Fellowships program at the University of New Hampshire (UNH). M.K. acknowledges subcontract, No. 277871, granted by Los Alamos National Laboratory to UNH. I.J.B. and R. J. M. acknowledge support by a Laboratory Directed Research and Development grant 20140630ER. NR 72 TC 3 Z9 3 U1 6 U2 12 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 17 PY 2016 VL 665 BP 108 EP 124 DI 10.1016/j.msea.2016.04.018 PG 17 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DN0WO UT WOS:000376788000013 ER PT J AU Insel, PS Mattsson, N Mackin, RS Scholl, M Nosheny, RL Tosun, D Donohue, MC Aisen, PS Jagust, WJ Weiner, MW AF Insel, Philip S. Mattsson, Niklas Mackin, R. Scott Scholl, Michael Nosheny, Rachel L. Tosun, Duygu Donohue, Michael C. Aisen, Paul S. Jagust, William J. Weiner, Michael W. CA Alzheimer's Dis Neuroimaging TI Accelerating rates of cognitive decline and imaging markers associated with -amyloid pathology SO NEUROLOGY LA English DT Article ID POSITRON-EMISSION-TOMOGRAPHY; ALZHEIMERS-DISEASE; CEREBROSPINAL-FLUID; HYPOTHETICAL MODEL; DYNAMIC BIOMARKERS; BRAIN ACTIVITY; BETA; DEMENTIA; TRIALS; ADULTS AB Objective:To estimate points along the spectrum of -amyloid pathology at which rates of change of several measures of neuronal injury and cognitive decline begin to accelerate.Methods:In 460 patients with mild cognitive impairment (MCI), we estimated the points at which rates of florbetapir PET, fluorodeoxyglucose (FDG) PET, MRI, and cognitive and functional decline begin to accelerate with respect to baseline CSF A(42). Points of initial acceleration in rates of decline were estimated using mixed-effects regression.Results:Rates of neuronal injury and cognitive and even functional decline accelerate substantially before the conventional threshold for amyloid positivity, with rates of florbetapir PET and FDG PET accelerating early. Temporal lobe atrophy rates also accelerate prior to the threshold, but not before the acceleration of cognitive and functional decline.Conclusions:A considerable proportion of patients with MCI would not meet inclusion criteria for a trial using the current threshold for amyloid positivity, even though on average, they are experiencing cognitive/functional decline associated with prethreshold levels of CSF A(42). Future trials in early Alzheimer disease might consider revising the criteria regarding -amyloid thresholds to include the range of amyloid associated with the first signs of accelerating rates of decline. C1 [Insel, Philip S.; Mackin, R. Scott; Nosheny, Rachel L.; Tosun, Duygu; Weiner, Michael W.] Dept Vet Affairs Med Ctr, Ctr Imaging Neurodegenerat Dis, San Francisco, CA USA. [Insel, Philip S.; Tosun, Duygu; Weiner, Michael W.] Univ Calif San Francisco, Dept Radiol & Biomed Imaging, San Francisco, CA 94143 USA. [Mackin, R. Scott] Univ Calif San Francisco, Dept Psychiat, San Francisco, CA USA. [Insel, Philip S.; Mattsson, Niklas] Lund Univ, Clin Memory Res Unit, Fac Med, S-22100 Lund, Sweden. [Mattsson, Niklas] Lund Univ, Skane Univ Hosp, Memory Clin, S-22100 Lund, Sweden. [Mattsson, Niklas] Lund Univ, Skane Univ Hosp, Dept Neurol, S-22100 Lund, Sweden. [Scholl, Michael] Univ Gothenburg, MedTech West, Gothenburg, Sweden. [Scholl, Michael] Univ Gothenburg, Dept Clin Neurosci & Rehabil, Gothenburg, Sweden. [Donohue, Michael C.; Aisen, Paul S.] Univ So Calif, Keck Sch Med, Dept Neurol, Los Angeles, CA 90033 USA. [Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Scholl, Michael; Jagust, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Insel, PS (reprint author), Dept Vet Affairs Med Ctr, Ctr Imaging Neurodegenerat Dis, San Francisco, CA USA.; Insel, PS (reprint author), Univ Calif San Francisco, Dept Radiol & Biomed Imaging, San Francisco, CA 94143 USA.; Insel, PS (reprint author), Lund Univ, Clin Memory Res Unit, Fac Med, S-22100 Lund, Sweden. EM philipinsel@gmail.com FU Alzheimer's Disease Neuroimaging Initiative (ADNI) (NIH) [U01 AG024904]; National Institute on Aging; National Institute of Biomedical Imaging and Bioengineering; ADNI clinical sites in Canada; NIH [P30 AG010129, K01 AG030514] FX Data collection and sharing for this project was funded by the Alzheimer's Disease Neuroimaging Initiative (ADNI) (NIH grant U01 AG024904). ADNI is funded by the National Institute on Aging, the National Institute of Biomedical Imaging and Bioengineering, and through contributions from the following: Alzheimer's Association; Alzheimer's Drug Discovery Foundation; BioClinica, Inc.; Biogen Idec Inc.; Bristol-Myers Squibb Company; Eisai Inc.; Elan Pharmaceuticals, Inc.; Eli Lilly and Company; F. Hoffmann-La Roche Ltd. and its affiliated company Genentech, Inc.; GE Healthcare; Innogenetics, N.V.; IXICO Ltd.; Janssen Alzheimer Immunotherapy Research & Development, LLC; Johnson & Johnson Pharmaceutical Research & Development LLC; Medpace, Inc.; Merck & Co., Inc.; Meso Scale Diagnostics, LLC; NeuroRx Research; Novartis Pharmaceuticals Corporation; Pfizer Inc.; Piramal Imaging; Servier; Synarc Inc.; and Takeda Pharmaceutical Company. The Canadian Institutes of Health Research is providing funds to support ADNI clinical sites in Canada. Private sector contributions are facilitated by the Foundation for the NIH (www.fnih.org). The grantee organization is the Northern California Institute for Research and Education, and the study is coordinated by the Alzheimer's Disease Cooperative Study at the University of California, San Diego. ADNI data are disseminated by the Laboratory for Neuroimaging at the University of Southern California. This research was also supported by NIH grants P30 AG010129 and K01 AG030514. NR 38 TC 3 Z9 3 U1 3 U2 4 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0028-3878 EI 1526-632X J9 NEUROLOGY JI Neurology PD MAY 17 PY 2016 VL 86 IS 20 BP 1887 EP 1896 DI 10.1212/WNL.0000000000002683 PG 10 WC Clinical Neurology SC Neurosciences & Neurology GA DN0US UT WOS:000376782000010 PM 27164667 ER PT J AU Burke, K Smith, JC Grabowski, PE Pribram-Jones, A AF Burke, K. Smith, J. C. Grabowski, P. E. Pribram-Jones, A. TI Exact conditions on the temperature dependence of density functionals SO PHYSICAL REVIEW B LA English DT Article ID ELECTRON LIQUID; EXCHANGE AB Universal exact conditions guided the construction of most ground-state density functional approximations in use today. We derive the relation between the entropy and Mermin free energy density functionals for thermal density functional theory. Both the entropy and sum of kinetic and electron-electron repulsion functionals are shown to be monotonically increasing with temperature, while the Mermin functional is concave downwards. Analogous relations are found for both exchange and correlation. The importance of these conditions is illustrated in two extremes: the Hubbard dimer and the uniform gas. C1 [Burke, K.; Smith, J. C.; Grabowski, P. E.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Burke, K.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Pribram-Jones, A.] Lawrence Livermore Natl Lab, 7000 East Ave,L-413, Livermore, CA 94550 USA. [Pribram-Jones, A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Burke, K (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA.; Burke, K (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. FU National Science Foundation (NSF) under grant CHE [1464795]; NSF Graduate Research fellowship program [DGE-1321846]; Department of Energy (DOE) [DE14-017426]; U.S. Department of Energy by Lawrence Livermore National Laboratory [AC52-07NA27344]; University of California President's Postdoctoral Fellowship FX The authors acknowledge support from the National Science Foundation (NSF) under grant CHE - 1464795. J.C.S. acknowledges support through the NSF Graduate Research fellowship program under Award No. DGE-1321846. P.E.G. acknowledges support from the Department of Energy (DOE) under Grant No. DE14-017426. A.P.J.' s work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. A.P.J. was supported in part by the University of California President's Postdoctoral Fellowship. NR 40 TC 2 Z9 2 U1 3 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2016 VL 93 IS 19 AR 195132 DI 10.1103/PhysRevB.93.195132 PG 5 WC Physics, Condensed Matter SC Physics GA DM3LT UT WOS:000376248600002 ER PT J AU Santos, B Rybicki, M Zasada, I Starodub, E McCarty, KF Cerda, JI Puerta, JM de la Figuera, J AF Santos, B. Rybicki, M. Zasada, I. Starodub, E. McCarty, K. F. Cerda, J. I. Puerta, J. M. de la Figuera, J. TI Structure and stability of ultrathin Fe films on W(110) SO PHYSICAL REVIEW B LA English DT Article ID ENERGY ELECTRON-DIFFRACTION; HYPERFINE INTERACTIONS; MAGNETIC-PROPERTIES; SURFACE RELAXATION; METAL-SURFACES; FE(110); ADSORPTION; DISLOCATIONS; TRANSITION; INTERFACES AB The growth of one and two atomic layers of iron on a W(110) substrate was followed by low-energy electron microscopy. The near-surface structural properties of the perfectly flat pseudomorphic films were studied by quantitative low-energy electron diffraction analysis from areas of uniform thickness as well as by the density functional theory. A strong relaxation of the outermost atomic layers was found in Fe mono-and bilayers on W(110). By calculating the phonon dispersion relations and phonon density of states, the stability of the pseudomorphic iron bilayer on a tungsten substrate has been addressed. To complete the physical picture, an iron trilayer has also been analyzed in order to identify the source of instability for its pseudomorphic phase. Our results show that the surface instability originates from the softening of the in-plane surface modes along the [1 (1) over bar 0] direction, although the soft modes were not observed. The enhanced magnetic moments calculated within the density functional theory are in good agreement with experimental findings reported for these systems. C1 [Santos, B.; de la Figuera, J.] CSIC, Inst Quim Fis Rocasolano, Madrid 28006, Spain. [Santos, B.] European Qual Assurance Spain SL, Madrid 28023, Spain. [Rybicki, M.; Zasada, I.] Univ Lodz, Dept Solid State Phys, Ul Pomorska 149-153, PL-90131 Lodz, Poland. [Starodub, E.; McCarty, K. F.] Sandia Natl Labs, Livermore, CA 94550 USA. [Cerda, J. I.; Puerta, J. M.] CSIC, Inst Ciencia Mat Madrid, Madrid 28049, Spain. RP Zasada, I (reprint author), Univ Lodz, Dept Solid State Phys, Ul Pomorska 149-153, PL-90131 Lodz, Poland. EM izasada@wfis.uni.lodz.pl RI Cerda, Jorge/F-4043-2010; de la Figuera, Juan/E-7046-2010 OI Cerda, Jorge/0000-0001-6176-0191; de la Figuera, Juan/0000-0002-7014-4777 FU Polish Ministry of Science and Higher Education [N N202 259539]; Spanish Ministry of Innovation and Science [MAT2010-18432, MAT2012-38045-C04-01]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy [DE-AC04-94AL85000]; University of Warsaw [G53-11] FX This work was financially supported by the Polish Ministry of Science and Higher Education in the frame of Grant No. N N202 259539 and partially by the Spanish Ministry of Innovation and Science under Contracts No. MAT2010-18432 and No. MAT2012-38045-C04-01, and by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, U.S. Department of Energy under Contract No. DE-AC04-94AL85000. Parts of the numerical calculations reported in this work have been performed at the Interdisciplinary Center for Mathematical and Computational Modeling (ICM) of the University of Warsaw within Grant No. G53-11. NR 51 TC 0 Z9 0 U1 5 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2016 VL 93 IS 19 AR 195423 DI 10.1103/PhysRevB.93.195423 PG 8 WC Physics, Condensed Matter SC Physics GA DM3LT UT WOS:000376248600006 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S 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Wickens, F. J. Wiedenmann, W. Wielers, M. Wienemann, P. Wiglesworth, C. Wiik-Fuchs, L. A. M. Wildauer, A. Wilkens, H. G. Williams, H. H. Williams, S. Willis, C. Willocq, S. Wilson, A. Wilson, J. A. Wingerter-Seez, I. Winklmeier, F. Winter, B. T. Wittgen, M. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamada, M. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yao, W-M. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yurkewicz, A. Mm, I. Yusuff Zabinski, B. Zaidan, R. Zaitsev, A. M. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for the standard model Higgs boson produced in association with a vector boson and decaying into a tau pair in pp collisions at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID MASSLESS PARTICLES; BROKEN SYMMETRIES; HADRON COLLIDERS; LHC; STRAHLUNG AB A search for the standard model Higgs boson produced in association with a vector boson with the decay H -> tau tau is presented. The data correspond to 20.3 fb(-1) of integrated luminosity from proton-proton collisions at root s = 8 TeV recorded by the ATLAS experiment at the LHC during 2012. The data agree with the background expectation, and 95% confidence-level upper limits are placed on the cross section of this process. The observed (expected) limit, expressed in terms of the signal strength mu= sigma/sigma(SM) for m(H) = 125 GeV, is mu < 5.6 (3.7). The measured value of the signal strength is mu = 2.3 +/- 1.6. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Duran Yildiz, H.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. 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A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Garzon, G. Otero Y.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Mm, I. Yusuff] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Fac Fis, Casilla 6177, Santiago 22, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; White, R.] Univ Tecn Federico Santa Maria, Fac Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; De Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Monig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gssling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kopeliansky, R.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; De Lima, D. E. 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H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Ishitsuka, M.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Zu Theenhausen, H. Meyer; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Physik, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.; Shaw, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Nucl Res Inst, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris 06, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Phys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; Caputo, R.; De la Torre, H.; Del Peso, J.; Francavilla, P.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Milic, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shatalov, P. B.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. 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A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Havranek, M.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr Kurchatov Inst, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Dos Santos, S. P. Amor; Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Carvalho, J.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Fis, P-3000 Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torr; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, ZA-2050 Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjlin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjlin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Hh, L. Shi; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Musto, E.; Rozen, Y.; Tarem, S.; Van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Javadov, N.; Jovicevic, J.; Koutsman, A.; Nessi, M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, CNM, IMB, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernndez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. 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[Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Guo, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Hh, L. Shi; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Mm, I. Yusuff] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Ippolito, Valerio/L-1435-2016; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015; Gladilin, Leonid/B-5226-2011; Villa, Mauro/C-9883-2009; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; BESSON, NATHALIE/L-6250-2015; Warburton, Andreas/N-8028-2013; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015 OI Lacasta, Carlos/0000-0002-2623-6252; Belanger-Champagne, Camille/0000-0003-2368-2617; Ippolito, Valerio/0000-0001-5126-1620; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581; Gladilin, Leonid/0000-0001-9422-8636; Villa, Mauro/0000-0002-9181-8048; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Pina, Joao /0000-0001-8959-5044; Veneziano, Stefano/0000-0002-2598-2659; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; Investissement d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos program - EU-ESF; Thales program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020, and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne, and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales, and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; BSF, GIF, and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 53 TC 0 Z9 0 U1 15 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 17 PY 2016 VL 93 IS 9 AR 092005 DI 10.1103/PhysRevD.93.092005 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM3OI UT WOS:000376255400001 ER PT J AU Fraga, CG Bronk, K Dockendorff, BP Heredia-Langner, A AF Fraga, Carlos G. Bronk, Krys Dockendorff, Brian P. Heredia-Langner, Alejandro TI Organic Chemical Attribution Signatures for the Sourcing of a Mustard Agent and Its Starting Materials SO ANALYTICAL CHEMISTRY LA English DT Article ID CHROMATOGRAPHY MASS-SPECTROMETRY; PRINCIPAL COMPONENT ANALYSIS; GAS-CHROMATOGRAPHY; NERVE-AGENT; FEATURE-SELECTION; CHEMOMETRICS; IMPURITIES; DISCOVERY; PRECURSOR; RESIDUES AB Chemical attribution signatures (CAS) are being investigated for the sourcing of chemical warfare (CW) agents and their starting materials that may be implicated in chemical attacks or CW proliferation. The work reported here demonstrates for the first time trace impurities from the synthesis of tris(2-chloroethyl)amine (HN3) that point to the reagent and the specific reagent stocks used in the synthesis of this CW agent. Thirty batches of HN3 were synthesized using different combinations of commercial stocks of triethanolamine (TEA), thionyl chloride, chloroform, and acetone. The HN3 batches and reagent stocks were then analyzed for impurities by gas chromatography/mass spectrometry. All the reagent stocks had impurity profiles that differentiated them from one another. This was demonstrated by building classification models with partial least-squares discriminant analysis (PLSDA) and obtaining average stock classification errors of 2.4, 2.8, 2.8, and 11% by cross-validation for chloroform (7 stocks), thionyl chloride (3 stocks), acetone (7 stocks), and TEA (3 stocks), respectively, and 0% for a validation set of chloroform samples. In addition, some reagent impurities indicative of reagent type were batches that were originally present in the reagent stocks and presumably not altered during synthesis. More intriguing, impurities in HN3 batches that were apparently produced by side reactions of impurities unique to specific TEA and chloroform stocks, and thus indicative of their use, were observed. C1 [Fraga, Carlos G.; Bronk, Krys; Dockendorff, Brian P.; Heredia-Langner, Alejandro] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Fraga, CG (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM carlos.fraga@pnnl.gov FU Science and Technology Directorate, U.S. Department of Homeland Security [HSHQPM-11-X-00040] FX The authors would like to thank Sedric B. Granger, Michael D. Crenshaw, and Greg Kastner from Battelle for information and guidance regarding CW agent handling. Helen W. Kreuzer and Nikhil S. Mirjankar from PNNL are also thanked for helpful edits and suggestions in the writing of this paper. Funding for this work was provided by the Science and Technology Directorate, U.S. Department of Homeland Security under Contract HSHQPM-11-X-00040. NR 27 TC 0 Z9 0 U1 6 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD MAY 17 PY 2016 VL 88 IS 10 BP 5406 EP 5413 DI 10.1021/acs.analchem.6b00766 PG 8 WC Chemistry, Analytical SC Chemistry GA DM3CD UT WOS:000376223500053 PM 27116337 ER PT J AU Le Roux, X Bouskill, NJ Niboyet, A Barthes, L Dijkstra, P Field, CB Hungate, BA Lerondelle, C Pommier, T Tang, JY Terada, A Tourna, M Poly, F AF Le Roux, Xavier Bouskill, Nicholas J. Niboyet, Audrey Barthes, Laure Dijkstra, Paul Field, Chris B. Hungate, Bruce A. Lerondelle, Catherine Pommier, Thomas Tang, Jinyun Terada, Akihiko Tourna, Maria Poly, Franck TI Predicting the Responses of Soil Nitrite-Oxidizers to Multi-Factorial Global Change: A Trait-Based Approach SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE bacterial functional traits; elevated CO2; nitrifiers; nitrogen fertilisation; trait-based modeling ID WATER TREATMENT PLANTS; GRASSLAND RESPONSES; NITRIFYING BACTERIA; MICROBIAL DIVERSITY; COMMUNITY STRUCTURE; AMMONIA-OXIDIZERS; ELEVATED CO2; NITROSPIRA; NITROBACTER; BIOGEOGRAPHY AB Soil microbial diversity is huge and a few grams of soil contain more bacterial taxa than there are bird species on Earth. This high diversity often makes predicting the responses of soil bacteria to environmental change intractable and restricts our capacity to predict the responses of soil functions to global change. Here, using a long-term field experiment in a California grassland, we studied the main and interactive effects of three global change factors (increased atmospheric CO2 concentration, precipitation and nitrogen addition, and all their factorial combinations, based on global change scenarios for central California) on the potential activity, abundance and dominant taxa of soil nitrite-oxidizing bacteria (NOB). Using a trait-based model, we then tested whether categorizing NOB into a few functional groups unified by physiological traits enables understanding and predicting how soil NOB respond to global environmental change. Contrasted responses to global change treatments were observed between three main NOB functional types. In particular, putatively mixotrophic Nitrobacter, rare under most treatments, became dominant under the 'High CO2+Nitrogen+Precipitation' treatment. The mechanistic trait-based model, which simulated ecological niches of NOB types consistent with previous ecophysiological reports, helped predicting the observed effects of global change on NOB and elucidating the underlying biotic and abiotic controls. Our results are a starting point for representing the overwhelming diversity of soil bacteria by a few functional types that can be incorporated into models of terrestrial ecosystems and biogeochemical processes. C1 [Le Roux, Xavier; Lerondelle, Catherine; Pommier, Thomas; Tourna, Maria; Poly, Franck] Univ Lyon 1, Ctr Microbial Ecol, UMR INRA 1418, INRA,CNRS,UMR CNRS 5557, F-69622 Villeurbanne, France. [Bouskill, Nicholas J.; Tang, Jinyun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Niboyet, Audrey; Barthes, Laure] Univ Paris 11, CNRS, UMR 8079, AgroParisTech,Ecol Systemat & Evolut Lab, F-91405 Orsay, France. [Dijkstra, Paul; Hungate, Bruce A.] No Arizona Univ, Dept Biol Sci, Ecosyst Sci & Soc Ctr, Box 5640, Flagstaff, AZ 86011 USA. [Field, Chris B.] Stanford Univ, Carnegie Inst, Dept Global Ecol, Stanford, CA 94305 USA. [Terada, Akihiko] Tech Univ Denmark, Dept Environm Engn, DK-2800 Lyngby, Denmark. [Niboyet, Audrey] Univ Paris 06, CNRS, AgroParis Tech, Inst Ecol & Environm Sci,UMR 7618, Thiverval Grignon, France. [Terada, Akihiko] Tokyo Univ Agr & Technol, Dept Chem Engn, Tokyo, Japan. [Tourna, Maria] Univ Thessaly, Dept Biochem, Larisa, Greece. RP Le Roux, X (reprint author), Univ Lyon 1, Ctr Microbial Ecol, UMR INRA 1418, INRA,CNRS,UMR CNRS 5557, F-69622 Villeurbanne, France. EM xavier.le-roux@univ-lyon1.fr RI Tang, Jinyun/M-4922-2013; Bouskill, Nick/G-2390-2015; Terada, Akihiko/C-5749-2012 OI Tang, Jinyun/0000-0002-4792-1259; Terada, Akihiko/0000-0002-9258-6912 FU INRA; CNRS; EC2CO program; US Department of Energy; US NSF [DEB-0092642/0145324]; Packard Foundation; Morgan Family Foundation FX This work was supported by grants from INRA, CNRS, EC2CO program, the US Department of Energy, the US NSF (DEB-0092642/0145324), the Packard Foundation, and the Morgan Family Foundation. NR 59 TC 2 Z9 2 U1 25 U2 36 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAY 17 PY 2016 VL 7 AR 628 DI 10.3389/fmicb.2016.00628 PG 13 WC Microbiology SC Microbiology GA DL9YT UT WOS:000376000100001 PM 27242680 ER PT J AU Seck, CM Kokish, MG Dietrich, MR Odom, BC AF Seck, Christopher M. Kokish, Mark G. Dietrich, Matthew R. Odom, Brian C. TI Raman sideband cooling of a Ba-138(+) ion using a Zeeman interval SO PHYSICAL REVIEW A LA English DT Article ID ELECTROMAGNETICALLY INDUCED TRANSPARENCY; GROUND-STATE; TRAPPED IONS; QUANTUM LOGIC; LASER; SPECTROSCOPY; VIOLATION; SHIFT; LIGHT AB Motional ground state cooling and internal state preparation are important elements for quantum logic spectroscopy (QLS), a class of quantum information processing. Since QLS does not require the high gate fidelities usually associated with quantum computation and quantum simulation, it is possible to make simplifying choices in ion species and quantum protocols at the expense of some fidelity. Here, we report sideband cooling and motional state detection protocols for Ba-138(+) of sufficient fidelity for QLS without an extremely narrow-band laser or the use of a species with hyperfine structure. We use the two S-1/2 Zeeman sublevels of Ba-138(+) to Raman sideband cool a single ion to the motional ground state. Because of the small Zeeman splitting, continuous near-resonant Raman sideband cooling of Ba-138(+) requires only the Doppler cooling lasers and two additional acousto-optic modulators. Observing the near-resonant Raman optical pumping fluorescence, we extract relevant experimental parameters and demonstrate a final average motional quantum number (n) over bar << 1. We additionally employ a second, far-off-resonant laser driving Raman pi pulses between the two Zeeman sublevels to provide motional state detection for QLS and to confirm the sideband cooling efficiency, measuring a final (n) over bar = 0.15(6). C1 [Seck, Christopher M.; Kokish, Mark G.; Dietrich, Matthew R.; Odom, Brian C.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Dietrich, Matthew R.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Odom, BC (reprint author), Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. EM b-odom@northwestern.edu FU AFOSR [FA9550-13-1-0116]; NSF [PHY-1404455]; NSF GRFP [DGE-1324585]; U.S. DOE, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This work was supported by AFOSR Grant No. FA9550-13-1-0116, NSF Grant No. PHY-1404455, and NSF GRFP DGE-1324585. This work was partially supported by U.S. DOE, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. NR 46 TC 0 Z9 0 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 17 PY 2016 VL 93 IS 5 AR 053415 DI 10.1103/PhysRevA.93.053415 PG 10 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DM3IN UT WOS:000376240200004 ER PT J AU Chikara, S Singleton, J Bowlan, J Yarotski, DA Lee, N Choi, HY Choi, YJ Zapf, VS AF Chikara, S. Singleton, J. Bowlan, J. Yarotski, D. A. Lee, N. Choi, H. Y. Choi, Y. J. Zapf, V. S. TI Electric polarization observed in single crystals of multiferroic Lu2MnCoO6 SO PHYSICAL REVIEW B LA English DT Article ID FERROELECTRICITY AB We report electric polarization and magnetization measurements in single crystals of double perovskite Lu2MnCoO6 using pulsed magnetic fields and optical second harmonic generation in dc magnetic fields. We observe well-resolved magnetic field-induced changes in the electric polarization in single crystals and thereby resolve the question about whether multiferroic behavior is intrinsic to these materials or is an extrinsic feature of polycrystals. We find electric polarization along the crystalline b axis, that is suppressed by applying a magnetic fields along the c axis, and advance a model for the origin of magnetoelectric coupling. We furthermore map the phase diagram using both capacitance and electric polarization to identify regions of ordering and regions of magnetoelectric hysteresis. This compound is a rare example of coupled hysteretic behavior in the magnetic and electric properties. The ferromagneticlike magnetic hysteresis loop that couples to hysteretic electric polarization can be attributed not to ordinary ferromagnetic domains, but to the rich physics of magnetic frustration of Ising-like spins in the axial next-nearest-neighbor interaction model. C1 [Chikara, S.; Singleton, J.; Zapf, V. S.] Los Alamos Natl Lab, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. [Bowlan, J.; Yarotski, D. A.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. [Lee, N.; Choi, H. Y.; Choi, Y. J.] Yonsei Univ, Dept Phys, Seoul 120749, South Korea. [Lee, N.; Choi, H. Y.; Choi, Y. J.] Yonsei Univ, IPAP, Seoul 120749, South Korea. RP Chikara, S (reprint author), Los Alamos Natl Lab, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. EM schikara@lanl.gov RI Chikara, Shalinee/E-4654-2017; OI Bowlan, John/0000-0002-2051-1778; Zapf, Vivien/0000-0002-8375-4515 FU Laboratory-Directed Research and Development program (LDRD); US National Science Foundation [DMR-1157490]; State of Florida; US Department of Energy; National Research Foundation of Korea (NRF) [NRF-2013R1A1A2058155, NRF-2014S1A2A2028481, NRF-2015R1C1A1A02037744]; Yonsei University Future-leading Research Initiative [2014-22-0123] FX Work at LANL was supported by the Laboratory-Directed Research and Development program (LDRD). The NHMFL Pulsed-Field Facility is funded by the US National Science Foundation through Cooperative Grant No. DMR-1157490, the State of Florida, and the US Department of Energy. Work at Yonsei University was supported by the National Research Foundation of Korea (NRF) Grants No. NRF-2013R1A1A2058155, No. NRF-2014S1A2A2028481, and No. NRF-2015R1C1A1A02037744, and partially by the Yonsei University Future-leading Research Initiative of 2014 (2014-22-0123). NR 24 TC 0 Z9 0 U1 11 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2016 VL 93 IS 18 AR 180405 DI 10.1103/PhysRevB.93.180405 PG 5 WC Physics, Condensed Matter SC Physics GA DM3LD UT WOS:000376247000001 ER PT J AU Ochapski, M Urbain, E Djeghloul, F Speisser, V Majjad, H Spor, D Vu, AD Coraux, J Rougemaille, N Chen, G Schmid, AK Suzuki, M Yasue, T Koshikawa, T Bulou, H Weber, W AF Ochapski, M. Urbain, E. Djeghloul, F. Speisser, V. Majjad, H. Spor, D. Vu, A. D. Coraux, J. Rougemaille, N. Chen, G. Schmid, A. K. Suzuki, M. Yasue, T. Koshikawa, T. Bulou, H. Weber, W. TI Breakdown of the electron-spin motion upon reflection at metal-organic or metal-carbon interfaces. II. SO PHYSICAL REVIEW B LA English DT Article ID W(110); FILMS; FE(110) AB A breakdown of the spin dependence of the electron reflection due to organic molecules or amorphous carbon deposited onto a metallic film has been observed in the past. The goal of the present work is to further elucidate the physics of this phenomenon by studying it in ways not yet studied in the past. The most intriguing observation of the present study is that the breakdown phenomenon appears in a relatively well defined electron energy range between 2 and about 200 eV kinetic energy. Outside this energy range the breakdown phenomenon is not observed. However, an explanation of the breakdown phenomenon is still missing. C1 [Ochapski, M.; Urbain, E.; Djeghloul, F.; Speisser, V.; Majjad, H.; Spor, D.; Bulou, H.; Weber, W.] CNRS UdS, UMR 7504, Inst Phys & Chim Mat Strasbourg, 23 Rue Loess,BP 43, F-67034 Strasbourg 2, France. [Vu, A. D.; Coraux, J.; Rougemaille, N.] CNRS, Inst NEEL, F-38000 Grenoble, France. [Vu, A. D.; Coraux, J.; Rougemaille, N.] Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France. [Chen, G.; Schmid, A. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, NCEM, Berkeley, CA 94720 USA. [Suzuki, M.; Yasue, T.; Koshikawa, T.] Osaka Electrocommun Univ, Fundamental Elect Res Inst, Neyagawa, Osaka 5728530, Japan. [Djeghloul, F.] Univ Ferhat Abbas Setif 1, Fac Technol, Setif, Algeria. RP Ochapski, M (reprint author), CNRS UdS, UMR 7504, Inst Phys & Chim Mat Strasbourg, 23 Rue Loess,BP 43, F-67034 Strasbourg 2, France. RI Chen, Gong/H-3074-2015; Speisser, Virginie/H-9914-2016 OI Speisser, Virginie/0000-0001-5920-3599 FU ANR Grant [ANR-12-BS-1000-401-NANOCELLS] FX We acknowledge support from ANR Grant ANR-12-BS-1000-401-NANOCELLS. We thank F. Scheurer, M. Alouani, and P. Panissod for discussions on the work. NR 16 TC 0 Z9 0 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 17 PY 2016 VL 93 IS 17 AR 174411 DI 10.1103/PhysRevB.93.174411 PG 7 WC Physics, Condensed Matter SC Physics GA DM3KI UT WOS:000376244900003 ER PT J AU Strickler, TS Langin, TK McQuillen, P Daligault, J Killian, TC AF Strickler, T. S. Langin, T. K. McQuillen, P. Daligault, J. Killian, T. C. TI Experimental Measurement of Self-Diffusion in a Strongly Coupled Plasma SO PHYSICAL REVIEW X LA English DT Article ID ONE-COMPONENT PLASMA; BROWNIAN-MOTION; LIQUIDS; VELOCITY; MATTER; DEGENERATE; PHYSICS; MODES AB We present a study of the collisional relaxation of ion velocities in a strongly coupled, ultracold neutral plasma on short time scales compared to the inverse collision rate. The measured average velocity of a tagged population of ions is shown to be equivalent to the ion-velocity autocorrelation function. We thus gain access to fundamental aspects of the single-particle dynamics in strongly coupled plasmas and to the ion self-diffusion constant under conditions where experimental measurements have been lacking. Nonexponential decay towards equilibrium of the average velocity heralds non-Markovian dynamics that are not predicted by traditional descriptions of weakly coupled plasmas. This demonstrates the utility of ultracold neutral plasmas for studying the effects of strong coupling on collisional processes, which is of interest for dense laboratory and astrophysical plasmas. C1 [Strickler, T. S.; Langin, T. K.; McQuillen, P.; Killian, T. C.] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Daligault, J.] Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. RP Strickler, TS (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. FU Air Force Office of Scientific Research [FA9550-12-1-0267]; Department of Energy, Fusion Energy Sciences [DE-SC0014455]; Department of Defense through the National Defense Science and Engineering Graduate Fellowship; Department of Energy Office of Fusion Energy Sciences FX This work was supported by the Air Force Office of Scientific Research (FA9550-12-1-0267), Department of Energy, Fusion Energy Sciences (DE-SC0014455), and Department of Defense through the National Defense Science and Engineering Graduate Fellowship. The work of J. D. was supported by the Department of Energy Office of Fusion Energy Sciences. NR 56 TC 2 Z9 2 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAY 17 PY 2016 VL 6 IS 2 AR 021021 DI 10.1103/PhysRevX.6.021021 PG 11 WC Physics, Multidisciplinary SC Physics GA DM3RI UT WOS:000376263500001 ER PT J AU Yuan, R Beyerlein, IJ Zhou, CZ AF Yuan, Rui Beyerlein, Irene J. Zhou, Caizhi TI Coupled crystal orientation-size effects on the strength of nano crystals SO SCIENTIFIC REPORTS LA English DT Article ID STRAIN-RATE SENSITIVITY; NANOCRYSTALLINE NICKEL; MECHANICAL-PROPERTIES; ELECTRODEPOSITED NICKEL; PLASTIC ANISOTROPY; TENSILE BEHAVIOR; METALS; COPPER; CU; DEFORMATION AB We study the combined effects of grain size and texture on the strength of nanocrystalline copper (Cu) and nickel (Ni) using a crystal-plasticity based mechanics model. Within the model, slip occurs in discrete slip events exclusively by individual dislocations emitted statistically from the grain boundaries. We show that a Hall-Petch relationship emerges in both initially texture and non-textured materials and our values are in agreement with experimental measurements from numerous studies. We find that the Hall-Petch slope increases with texture strength, indicating that preferred orientations intensify the enhancements in strength that accompany grain size reductions. These findings reveal that texture is too influential to be neglected when analyzing and engineering grain size effects for increasing nanomaterial strength. C1 [Yuan, Rui; Zhou, Caizhi] Missouri Univ Sci & Technol, Dept Mat Sci & Engn, Rolla, MO 65409 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zhou, CZ (reprint author), Missouri Univ Sci & Technol, Dept Mat Sci & Engn, Rolla, MO 65409 USA. EM zhouc@mst.edu FU University of Missouri Research Board; MRC at Missouri University of Science and Technology; Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program [LDRD 20140348ER] FX R.Y. and C.Z. gratefully acknowledge financial support from The University of Missouri Research Board and MRC at Missouri University of Science and Technology. I.J.B. gratefully acknowledges support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program through project number LDRD 20140348ER. NR 43 TC 1 Z9 1 U1 8 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 17 PY 2016 VL 6 AR 26254 DI 10.1038/srep26254 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL9QU UT WOS:000375978600001 PM 27185364 ER PT J AU Winkler, PM McGraw, RL Bauer, PS Rentenberger, C Wagner, PE AF Winkler, P. M. McGraw, R. L. Bauer, P. S. Rentenberger, C. Wagner, P. E. TI Direct determination of three-phase contact line properties on nearly molecular scale SO SCIENTIFIC REPORTS LA English DT Article ID HETEROGENEOUS NUCLEATION; TENSION; NUCLEUS; SIZE; NANOPARTICLES; PARTICLES; SURFACES; WATER; ANGLE; WORK AB Wetting phenomena in multi-phase systems govern the shape of the contact line which separates the different phases. For liquids in contact with solid surfaces wetting is typically described in terms of contact angle. While in macroscopic systems the contact angle can be determined experimentally, on the molecular scale contact angles are hardly accessible. Here we report the first direct experimental determination of contact angles as well as contact line curvature on a scale of the order of 1nm. For water nucleating heterogeneously on Ag nanoparticles we find contact angles around 15 degrees compared to 90 degrees for the corresponding macroscopically measured equilibrium angle. The obtained microscopic contact angles can be attributed to negative line tension in the order of -10(-10) J/m that becomes increasingly dominant with increasing curvature of the contact line. These results enable a consistent theoretical description of heterogeneous nucleation and provide firm insight to the wetting of nanosized objects. C1 [Winkler, P. M.; Bauer, P. S.; Rentenberger, C.; Wagner, P. E.] Univ Vienna, Fac Phys, Waehringer Guertel 18, A-1090 Vienna, Austria. [McGraw, R. L.] Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Winkler, PM (reprint author), Univ Vienna, Fac Phys, Waehringer Guertel 18, A-1090 Vienna, Austria. EM paul.winkler@univie.ac.at OI Rentenberger, Christian/0000-0002-3385-8850 FU European Research Council under the European Community's Seventh Framework Programme (FP7)/ERC [616075]; Austrian Science Fund (FWF) [P19546, L593]; Atmospheric Systems Research (ASR) Program of the US Department of Energy FX We thank Dr. R. Thalman (BNL) for connecting Eq. 9 with the Gumbel extreme-value distribution. This work was supported by the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement No. 616075, and the Austrian Science Fund (FWF) (project no. P19546, L593). Work at Brookhaven was supported by the Atmospheric Systems Research (ASR) Program of the US Department of Energy. NR 41 TC 1 Z9 1 U1 5 U2 9 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 17 PY 2016 VL 6 AR 26111 DI 10.1038/srep26111 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL8ZN UT WOS:000375931000001 PM 27183880 ER PT J AU Sayer, AM Hsu, NC Bettenhausen, C Lee, J Redemann, J Schmid, B Shinozuka, Y AF Sayer, A. M. Hsu, N. C. Bettenhausen, C. Lee, J. Redemann, J. Schmid, B. Shinozuka, Y. TI Extending "Deep Blue" aerosol retrieval coverage to cases of absorbing aerosols above clouds: Sensitivity analysis and first case studies SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID BIOMASS BURNING PARTICLES; GROUND-BASED MEASUREMENTS; OPTICAL-DEPTH; ACE-ASIA; SOUTHEAST-ASIA; SOURCE REGIONS; WATER-VAPOR; MODIS; SATELLITE; OCEAN AB Cases of absorbing aerosols above clouds (AACs), such as smoke or mineral dust, are omitted from most routinely processed space-based aerosol optical depth (AOD) data products, including those from the Moderate Resolution Imaging Spectroradiometer (MODIS). This study presents a sensitivity analysis and preliminary algorithm to retrieve above-cloud AOD and liquid cloud optical depth (COD) for AAC cases from MODIS or similar sensors, for incorporation into a future version of the "Deep Blue" AOD data product. Detailed retrieval simulations suggest that these sensors should be able to determine AAC AOD with a typical level of uncertainty similar to 25-50% (with lower uncertainties for more strongly absorbing aerosol types) and COD with an uncertainty similar to 10-20%, if an appropriate aerosol optical model is known beforehand. Errors are larger, particularly if the aerosols are only weakly absorbing, if the aerosol optical properties are not known, and the appropriate model to use must also be retrieved. Actual retrieval errors are also compared to uncertainty envelopes obtained through the optimal estimation (OE) technique; OE-based uncertainties are found to be generally reasonable for COD but larger than actual retrieval errors for AOD, due in part to difficulties in quantifying the degree of spectral correlation of forward model error. The algorithm is also applied to two MODIS scenes (one smoke and one dust) for which near-coincident NASA Ames Airborne Tracking Sun photometer (AATS) data were available to use as a ground truth AOD data source, and found to be in good agreement, demonstrating the validity of the technique with real observations. C1 [Sayer, A. M.; Hsu, N. C.; Bettenhausen, C.; Lee, J.] NASA Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Sayer, A. M.] Univ Space Res Assoc, Goddard Earth Sci Technol & Res, Greenbelt, MD USA. [Bettenhausen, C.] Sci Syst & Applicat Inc, Lanham, MD USA. [Lee, J.] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. [Redemann, J.] NASA Ames Res Ctr, Moffett Field, CA USA. [Schmid, B.] Pacific Northwest Natl Lab, Richland, WA USA. [Shinozuka, Y.] Bay Area Environm Res Inst, Petaluma, CA USA. RP Sayer, AM (reprint author), NASA Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. EM andrew.sayer@nasa.gov RI Sayer, Andrew/H-2314-2012; OI Sayer, Andrew/0000-0001-9149-1789; Lee, Jaehwa/0000-0002-5029-476X FU NASA ROSES program FX Further information about Deep Blue is available at http://deepblue.gsfc.nasa.gov. The NASA Ames Sunphotometer-Satellite Team page is https://earthscience.arc.nasa.gov/sunsat. This research was funded under the NASA ROSES program. AERONET data are available from http://aeronet.gsfc.nasa.gov/; the AERONET team and PIs, led by B. Holben, are thanked for the creation and stewardship of these data records. CPL data are available from http://cpl.gsfc.nasa.gov/. R. Frey and K. Meyer are thanked for their useful discussions about the MODIS cloud data products. Z. Zhang and two anonymous reviewers are thanked for their insightful reviews. NR 91 TC 3 Z9 3 U1 8 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAY 16 PY 2016 VL 121 IS 9 BP 4830 EP 4854 DI 10.1002/2015JD024729 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DR2DS UT WOS:000379715800026 ER PT J AU Sun, YW Carrigan, CR AF Sun, Yunwei Carrigan, Charles R. TI Thermally driven advection for radioxenon transport from an underground nuclear explosion SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID NETWORKS AB Barometric pumping is a ubiquitous process resulting in migration of gases in the subsurface that has been studied as the primary mechanism for noble gas transport from an underground nuclear explosion (UNE). However, at early times following a UNE, advection driven by explosion residual heat is relevant to noble gas transport. A rigorous measure is needed for demonstrating how, when, and where advection is important. In this paper three physical processes of uncertain magnitude (oscillatory advection, matrix diffusion, and thermally driven advection) are parameterized by using boundary conditions, system properties, and source term strength. Sobol' sensitivity analysis is conducted to evaluate the importance of all physical processes influencing the xenon signals. This study indicates that thermally driven advection plays a more important role in producing xenon signals than oscillatory advection and matrix diffusion at early times following a UNE, and xenon isotopic ratios are observed to have both time and spatial dependence. C1 [Sun, Yunwei; Carrigan, Charles R.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Sun, YW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA. EM sun4@llnl.gov FU Office of Proliferation Detection [NA-221]; U.S. Department of Energy; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank anonymous reviewers and the editor for their constructive reviews and helpful comments that led to an improved manuscript. This research was funded by Office of Proliferation Detection (NA-221), U.S. Department of Energy, and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 25 TC 0 Z9 0 U1 8 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAY 16 PY 2016 VL 43 IS 9 BP 4418 EP 4425 DI 10.1002/2016GL068290 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DP2RS UT WOS:000378339200041 ER PT J AU Weck, PF Kim, E Wang, YF AF Weck, Philippe F. Kim, Eunja Wang, Yifeng TI van der Waals forces and confinement in carbon nanopores: Interaction between CH4, COOH, NH3, OH, SH and single-walled carbon nanotubes SO CHEMICAL PHYSICS LETTERS LA English DT Article DE Nanotubes; Carbon nanopores; Density functional theory ID BRILLOUIN-ZONE INTEGRATIONS; AUGMENTED-WAVE METHOD; FLOW AB Interactions between CH4, COOH, NH3, OH, SH and armchair (n, n) (n = 4, 7,14) and zigzag (n, 0) (n = 7,12, 25) single-walled carbon nanotubes (SWCNTs) have been systematically investigated within the framework of dispersion-corrected density functional theory (DFT-D2). Endohedral and exohedral molecular adsorption on SWCNT walls is energetically unfavorable or weak, despite the use of C6/16 pair wise London-dispersion corrections. The effects of pore size and chirality on the molecule/SWCNTs interaction were also assessed. Chemisorption of COOH, NH3, OH and SH at SWCNT edge sites was examined using a H-capped (7, 0) SWCNT fragment and its impact on electrophilic, nucleophilic and radical attacks was predicted by means of Fukui functions. (C) 2016 Elsevier B.V. All rights reserved. C1 [Weck, Philippe F.; Wang, Yifeng] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Kim, Eunja] Univ Nevada, Dept Phys & Astron, 4505 Maryland Pkwy, Las Vegas, NV 89154 USA. RP Weck, PF (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pfweck@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Energy Technology Laboratory (NETL); Laboratory Directed Research and Development (LDRD) from Sandia National Laboratories FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was supported by the National Energy Technology Laboratory (NETL) and by Laboratory Directed Research and Development (LDRD) funding from Sandia National Laboratories. NR 25 TC 0 Z9 0 U1 4 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAY 16 PY 2016 VL 652 BP 22 EP 26 DI 10.1016/j.cplett.2016.04.012 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN6RS UT WOS:000377204100005 ER PT J AU Hinnefeld, JH Xu, RJ Rogers, S Pandya, S Shim, M Martin, LW Mason, N AF Hinnefeld, J. Henry Xu, Ruijuan Rogers, Steven Pandya, Shishir Shim, Moonsub Martin, Lane W. Mason, Nadya TI Single gate p-n junctions in graphene-ferroelectric devices SO APPLIED PHYSICS LETTERS LA English DT Article ID FIELD-EFFECT TRANSISTORS; DENSITY AB Graphene's linear dispersion relation and the attendant implications for bipolar electronics applications have motivated a range of experimental efforts aimed at producing p-n junctions in graphene. Here we report electrical transport measurements of graphene p-n junctions formed via simple modifications to a PbZr0.2Ti0.8O3 substrate, combined with a self-assembled layer of ambient environmental dopants. We show that the substrate configuration controls the local doping region, and that the p-n junction behavior can be controlled with a single gate. Finally, we show that the ferroelectric substrate induces a hysteresis in the environmental doping which can be utilized to activate and deactivate the doping, yielding an "on-demand" p-n junction in graphene controlled by a single, universal backgate. Published by AIP Publishing. C1 [Hinnefeld, J. Henry; Mason, Nadya] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Xu, Ruijuan; Pandya, Shishir; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Xu, Ruijuan; Pandya, Shishir; Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Rogers, Steven; Shim, Moonsub] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. RP Mason, N (reprint author), Univ Illinois, Dept Phys, Urbana, IL 61801 USA. EM nadya@illinois.edu RI Shim, Moonsub/A-7875-2009; Martin, Lane/H-2409-2011; OI Shim, Moonsub/0000-0001-7781-1029; Martin, Lane/0000-0003-1889-2513; Hinnefeld, John/0000-0002-3566-9340 FU National Science Foundation; Nanoelectronics Research Initiative under NSF-NEB [DMR-1124696]; Army Research Office [W911NF-14-1-0104]; National Science Foundation [ENG-1434147] FX J.H.H., R.X., S.R., and M.S. acknowledge support from the National Science Foundation and the Nanoelectronics Research Initiative under NSF-NEB Grant No. DMR-1124696. S.P. acknowledges support from the Army Research Office under Grant No. W911NF-14-1-0104. N.M. and L.W.M. acknowledge support from the National Science Foundation under Grant No. ENG-1434147. This work was carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities at the University of Illinois. NR 44 TC 2 Z9 2 U1 16 U2 32 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2016 VL 108 IS 20 AR 203109 DI 10.1063/1.4950975 PG 5 WC Physics, Applied SC Physics GA DN4HE UT WOS:000377024000046 ER PT J AU Li, JJ Yu, Q Zhang, ZJ Xu, W Sun, X AF Li, Jingjing Yu, Qian Zhang, Zijiao Xu, Wei Sun, Xin TI Formation mechanism for the nanoscale amorphous interface in pulse-welded Al/Fe bimetallic systems SO APPLIED PHYSICS LETTERS LA English DT Article ID METALLIC-GLASS FORMATION; ALUMINUM; ALLOYS; STEEL; MICROSTRUCTURE; DIFFUSION; FE AB Pulse or impact welding traditionally has been referred to as "solid-state" welding. By integrating advanced interface characterizations and diffusion calculations, we report that the nanoscale amorphous interface in the pulse-welded Al/Fe bimetallic system is formed by rapid heating and melting of a thin Al layer at the interface, diffusion of iron atoms in the liquid aluminum, and subsequent rapid quenching with diffused iron atoms in solution. This finding challenges the commonly held belief regarding the solid-state nature of the impact-based welding process for dissimilar metals. Elongated ultra-fine grains with high dislocation density and ultra-fine equiaxed grains also are observed in the weld interface vicinity on the steel and aluminum sides, respectively, which further confirms that melting and the subsequent recrystallization occurred on the aluminum side of the interface. Published by AIP Publishing. C1 [Li, Jingjing] Univ Hawaii Manoa, Dept Mech Engn, Honolulu, HI 96822 USA. [Yu, Qian; Zhang, Zijiao] Zhejiang Univ, Dept Mat Sci & Engn, Ctr Electron Microscope, Hangzhou 310027, Zhejiang, Peoples R China. [Xu, Wei; Sun, Xin] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Sun, X (reprint author), Pacific NW Natl Lab, Richland, WA 99354 USA. EM xin.sun@pnnl.gov FU U.S. Department of Energy (DOE) [DE-AC05-76RL01830]; DOE's Office of FreedomCAR and Vehicle Technologies under the Automotive Lightweighting Materials Program; National Science Foundation Civil, Mechanical and Manufacturing Innovation [1554748] FX Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy (DOE) under Contract No. DE-AC05-76RL01830. This work was funded by the DOE's Office of FreedomCAR and Vehicle Technologies under the Automotive Lightweighting Materials Program managed by Dr. William Joost. University of Hawaii at Manoa's work was supported by National Science Foundation Civil, Mechanical and Manufacturing Innovation Grant No. 1554748. NR 32 TC 0 Z9 0 U1 15 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2016 VL 108 IS 20 AR 201606 DI 10.1063/1.4947465 PG 5 WC Physics, Applied SC Physics GA DN4HE UT WOS:000377024000013 ER PT J AU Morishige, AE Jensen, MA Hofstetter, J Yen, PXT Wang, CL Lai, B Fenning, DP Buonassisi, T AF Morishige, Ashley E. Jensen, Mallory A. Hofstetter, Jasmin Yen, Patricia X. T. Wang, Chenlei Lai, Barry Fenning, David P. Buonassisi, Tonio TI Synchrotron-based investigation of transition-metal getterability in n-type multicrystalline silicon SO APPLIED PHYSICS LETTERS LA English DT Article ID SOLAR-CELLS; CRYSTALLINE SILICON; CARRIER LIFETIME; EXTENDED DEFECTS; IRON; EFFICIENCY; DIFFUSION; IMPACT; PRECIPITATION; SOLUBILITY AB Solar cells based on n-type multicrystalline silicon (mc-Si) wafers are a promising path to reduce the cost per kWh of photovoltaics; however, the full potential of the material and how to optimally process it are still unknown. Process optimization requires knowledge of the response of the metal-silicide precipitate distribution to processing, which has yet to be directly measured and quantified. To supply this missing piece, we use synchrotron-based micro-X-ray fluorescence (mu-XRF) to quantitatively map >250 metal-rich particles in n-type mc-Si wafers before and after phosphorus diffusion gettering (PDG). We find that 820 degrees C PDG is sufficient to remove precipitates of fast-diffusing impurities and that 920 degrees C PDG can eliminate precipitated Fe to below the detection limit of mu-XRF. Thus, the evolution of precipitated metal impurities during PDG is observed to be similar for n-and p-type mc-Si, an observation consistent with calculations of the driving forces for precipitate dissolution and segregation gettering. Measurements show that minority-carrier lifetime increases with increasing precipitate dissolution from 820 degrees C to 880 degrees C PDG, and that the lifetime after PDG at 920 degrees C is between the lifetimes achieved after 820 degrees C and 880 degrees C PDG. Published by AIP Publishing. C1 [Morishige, Ashley E.; Jensen, Mallory A.; Yen, Patricia X. T.; Fenning, David P.; Buonassisi, Tonio] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Wang, Chenlei] Supreme Inc, Sunnyvale, CA 94085 USA. [Lai, Barry] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Fenning, David P.] Univ Calif San Diego, La Jolla, CA 92093 USA. RP Morishige, AE; Buonassisi, T (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM aemorish@alum.mit.edu; buonassisi@mit.edu FU National Science Foundation (NSF); Department of Energy (DOE) under NSF CA [EEC-1041895]; DOE Office of Science [DE-AC02-06CH11357]; NSF [ECS-0335765, 1122374]; Department of Defense through the NDSEG fellowship program; Martin Family Society of Fellows for Sustainability; University of California, San Diego FX We thank S. Meyer, S. Wahl, S. Ramanathan, S. A. McHugo, and H. S. Laine. Funding provided by the National Science Foundation (NSF) and the Department of Energy (DOE) under NSF CA No. EEC-1041895. mu-XRF was performed at the Advanced Photon Source, a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. EBSD and ALD performed at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network, which is supported by NSF Award No. ECS-0335765. CNS is part of Harvard University. A.E.M. acknowledges the Department of Defense through the NDSEG fellowship program. M.A.J. and P.X.T.Y. acknowledge support by the NSF Graduate Research Fellowship under Grant No. 1122374. D.P.F. acknowledges support by the Martin Family Society of Fellows for Sustainability and the University of California, San Diego. NR 34 TC 2 Z9 2 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 16 PY 2016 VL 108 IS 20 AR 202104 DI 10.1063/1.4950765 PG 5 WC Physics, Applied SC Physics GA DN4HE UT WOS:000377024000023 ER PT J AU Hochberg, Y Kuflik, E Murayama, H AF Hochberg, Yonit Kuflik, Eric Murayama, Hitoshi TI SIMP spectroscopy SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Chiral Lagrangians ID INTERACTING DARK-MATTER; GALAXY CLUSTER 1E-0657-56; INTERACTION CROSS-SECTION; COSMOLOGICAL SIMULATIONS; CURRENT-ALGEBRA; ABELL 3827; CONSTRAINTS; SUBHALOES; MILKY AB We study the interactions between strongly interacting massive particle dark matter and the Standard Model via a massive vector boson that is kinetically mixed with the hypercharge gauge boson. The relic abundance is set by 3 -> 2 self-interactions of the dark matter, while the interactions with the vector mediator enable kinetic equilibrium between the dark and visible sectors. We show that a wide range of parameters is phenomenologically viable and can be probed in various ways. Astrophysical and cosmological constraints are evaded due to the p-wave nature of dark matter annihilation into visible particles, while direct detection methods using electron recoils can be sensitive to parts of the parameter space. In addition, we propose performing spectroscopy of the strongly coupled dark sector at e(+)e(-) colliders, where the energy of a mono-photon can track the resonance structure of the dark sector. Alternatively, some resonances may decay back into Standard Model leptons or jets, realizing 'hidden valley' phenomenology at the LHC and ILC in a concrete fashion. C1 [Hochberg, Yonit; Murayama, Hitoshi] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Hochberg, Yonit; Murayama, Hitoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kuflik, Eric] Cornell Univ, Dept Phys, LEPP, Ithaca, NY 14853 USA. [Murayama, Hitoshi] Univ Tokyo, Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Murayama, Hitoshi] Univ Calif Berkeley, Ctr Japanese Studies, Berkeley, CA 94720 USA. RP Hochberg, Y; Murayama, H (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Hochberg, Y; Murayama, H (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Kuflik, E (reprint author), Cornell Univ, Dept Phys, LEPP, Ithaca, NY 14853 USA.; Murayama, H (reprint author), Univ Tokyo, Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan.; Murayama, H (reprint author), Univ Calif Berkeley, Ctr Japanese Studies, Berkeley, CA 94720 USA. EM yonit.hochberg@berkeley.edu; kuflik@cornell.edu; hitoshi@berkeley.edu FU U.S. National Science Foundation [PHY-1002399]; NSF [PHY-1002399, PHY-1316222, PHY-1316783, PHYS-1066293]; Hans Bethe Postdoctoral Fellowship at Cornell; U.S. DOE [DE-AC02-05CH11231]; JSPS [26400241, 15H05887]; WPI, MEXT, Japan FX We thank Zoltan Fodor, Tongyan Lin, Takeo Higuchi, Kenkichi Miyabayashi, Yu-Dai Tsai for useful discussions, and Tomer Volansky and Jay Wacker for helpful conversations and comments on the manuscript. We thank the journal referee for an important comment on thermal tails. We are especially grateful to Jay Wacker for contributions to parts of this manuscript. The work of YH is supported by the U.S. National Science Foundation under Grant No. PHY-1002399. YH is an Awardee of the Weizmann Institute of Science - National Postdoctoral Award Program for Advancing Women in Science. EK is supported by the NSF under Grant No. PHY-1316222 and by a Hans Bethe Postdoctoral Fellowship at Cornell. HM was supported by the U.S. DOE under Contract DE-AC02-05CH11231, and by the NSF under grants PHY-1002399 and PHY-1316783. HM was also supported by the JSPS Grant-in-Aid for Scientific Research (C) (No. 26400241), Scientific Research on Innovative Areas (No. 15H05887), and by WPI, MEXT, Japan. This work was supported in part by the NSF under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. NR 80 TC 5 Z9 5 U1 2 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 16 PY 2016 IS 5 AR 090 DI 10.1007/JHEP05(2016)090 PG 37 WC Physics, Particles & Fields SC Physics GA DM5OQ UT WOS:000376399600003 ER PT J AU Feigenbaum, E Raman, RN Cross, D Carr, CW Matthews, MJ AF Feigenbaum, Eyal Raman, Rajesh N. Cross, David Carr, C. W. Matthews, Manyalibo J. TI Laser-induced Hertzian fractures in silica initiated by metal micro-particles on the exit surface SO OPTICS EXPRESS LA English DT Article ID INDUCED DAMAGE SITES; FUSED-SILICA; OPTICAL-COMPONENTS; PRECURSORS; ABLATION; PULSES; GROWTH; MODEL; POWER; NM AB Laser-induced Hertzian fractures on the exit surface of silica glass are found to result from metal surface-bound micro particles. Two types of metal micro-spheres are studied (stainless-steel and Al) using ultraviolet laser light. The fracture initiation probability curve as a function of fluence is obtained, resulting in an initiation threshold fluence of 11.1 +/- 4.7 J/cm(2) and 16.5 +/- 4.5 J/cm(2) for the SS and Al particles, accordingly. The modified damage density curve is calculated based on the fracture probability. The calculated momentum coupling coefficient linking incident laser fluence to the resulting plasma pressure is found to be similar for both particles: 32.6 +/- 15.4 KN/J and 28.1 +/- 10.4 KN/J for the SS and Al cases accordingly. (C) 2016 Optical Society of America C1 [Feigenbaum, Eyal] Lawrence Livermore Natl Lab, Natl Ignit Facil, 7000 East Ave, Livermore, CA 94550 USA. Lawrence Livermore Natl Lab, Photon Sci, 7000 East Ave, Livermore, CA 94550 USA. RP Feigenbaum, E (reprint author), Lawrence Livermore Natl Lab, Natl Ignit Facil, 7000 East Ave, Livermore, CA 94550 USA. EM eyal@llnl.gov FU U.S. Department of Energy [DE-AC52-07NA27344]; Laboratory Directed Research and Development [14-ERD-098. LLNL-JRNL-686277] FX We would like to acknowledge W. A. Steele and the optical sciences laboratory (OSL) staff for the experiment support and also to J. D. Bude, T. I. Suratwala, A. M. Rubenchik, P. E. Miller, and Z. Liao for the useful conversations. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. We would like to acknowledge the funding from Laboratory Directed Research and Development grant 14-ERD-098. LLNL-JRNL-686277. NR 36 TC 1 Z9 1 U1 6 U2 12 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAY 16 PY 2016 VL 24 IS 10 AR UNSP 261529 DI 10.1364/OE.24.010527 PG 10 WC Optics SC Optics GA DM5IE UT WOS:000376380700056 ER PT J AU Kweon, KE Aberg, D Lordi, V AF Kweon, Kyoung E. Aberg, Daniel Lordi, Vincenzo TI First-principles study of atomic and electronic structures of 60 degrees perfect and 30 degrees/90 degrees partial glide dislocations in CdTe SO PHYSICAL REVIEW B LA English DT Article ID SEMI-INSULATED CDTE; CADMIUM TELLURIDE; CDZNTE; SPECTROSCOPY; MICROSCOPY; DETECTORS; DEFECTS; CRYSTAL; ENERGY; CORES AB The atomic and electronic structures of 60 degrees glide perfect and 30 degrees/90 degrees glide partial dislocations in CdTe are studied using combined semi-empirical and density functional theory calculations. The calculations predict that the dislocation cores tend to undergo significant reconstructions along the dislocation lines from the singly-periodic (SP) structures, yielding either doubly-periodic (DP) ordering by forming a dimer or quadruply-periodic (QP) ordering by alternating a dimer and a missing dimer. Charge modulation along the dislocation line, accompanied by the QP reconstruction for the Cd-/Te-core 60 degrees perfect and 30 degrees partials or the DP reconstruction for the Cd-core 90 degrees partial, results in semiconducting character, as opposed to the metallic character of the SP dislocation cores. Dislocation-induced defect states for the 60 degrees Cd-/Te-core are located relatively close to the band edges, whereas the defect states lie in the middle of the band gap for the 30 degrees Cd-/Te-core partial dislocations. In addition to the intracore charge modulation within each QP core, the possibility of intercore charge transfer between two different dislocation cores when they are paired together in the same system is discussed. The analysis of the electronic structures reveals the potential role of the dislocations on charge transport in CdTe, particularly in terms of charge trapping and recombination. C1 [Kweon, Kyoung E.; Aberg, Daniel; Lordi, Vincenzo] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Kweon, KE; Lordi, V (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kweon1@llnl.gov; lordi2@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE National Nuclear Security Administration Office of Defense Nuclear Nonproliferation Research and Development [LL13-MatModelRadDetect-PD3YJ] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, with support from the DOE National Nuclear Security Administration Office of Defense Nuclear Nonproliferation Research and Development (project LL13-MatModelRadDetect-PD3YJ). Helpful contributions by Eunae Cho and Michael Skarlinski are warmly acknowledged. NR 41 TC 0 Z9 0 U1 9 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2016 VL 93 IS 17 AR 174109 DI 10.1103/PhysRevB.93.174109 PG 11 WC Physics, Condensed Matter SC Physics GA DM3KG UT WOS:000376244700001 ER PT J AU Parker, DS Herklotz, A Ward, TZ McGuire, MA Singh, DJ AF Parker, David S. Herklotz, Andreas Ward, T. Z. McGuire, Michael A. Singh, David J. TI Enhanced ferroelectric polarization and possible morphotrophic phase boundary in PZT-based alloys SO PHYSICAL REVIEW B LA English DT Article ID FREE PIEZOELECTRIC CERAMICS; 1ST-PRINCIPLES; FILMS AB We present a combined theoretical and experimental study of alloys of the high performance piezoelectric PZT (PbZr0.5Ti0.5O3) with BZnT (BiZn0.5Ti0.5O3) and BZnZr (BiZn0.5Zr0.5O3), focusing on atomic displacements, ferroelectric polarization, and elastic stability. From theory we find that the 75-25 PZT-BZnT alloy has substantially larger cation displacements, and hence ferroelectric polarization than the PZT base material, on the tetragonal side of the phase diagram. We also find a possible morphotrophic phase boundary in this system by comparing displacement patterns and optimized c/a ratios. Elastic stability calculations find the structures to be essentially stable. Experiments indicate the feasibility of sample synthesis within this alloy system, although measurements do not find significant polarization, probably due to a large coercive field. C1 [Parker, David S.; Herklotz, Andreas; Ward, T. Z.; McGuire, Michael A.] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Singh, David J.] Univ Missouri, Dept Phys & Astron, Columbia, MO 65211 USA. RP Parker, DS (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RI McGuire, Michael/B-5453-2009; OI McGuire, Michael/0000-0003-1762-9406; Ward, Thomas/0000-0002-1027-9186 FU U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Vehicle Technologies, Propulsion Materials program; DOE Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy, Vehicle Technologies, Propulsion Materials program (DP, MAM), and the DOE Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (A.H., T.Z.W.). NR 23 TC 0 Z9 0 U1 2 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2016 VL 93 IS 17 AR 174307 DI 10.1103/PhysRevB.93.174307 PG 9 WC Physics, Condensed Matter SC Physics GA DM3KG UT WOS:000376244700002 ER PT J AU Sturza, M Bugaris, DE Malliakas, CD Han, F Chung, DY Kanatzidis, MG AF Sturza, Mihai Bugaris, Daniel E. Malliakas, Christos D. Han, Fei Chung, Duck Young Kanatzidis, Mercouri G. TI Mixed-Valent NaCu4Se3: A Two-Dimensional Metal SO INORGANIC CHEMISTRY LA English DT Article ID COPPER CHALCOGENIDES; PHASE TRANSITIONS; DIMENSIONAL METAL; CRYSTAL-STRUCTURE; LAYERED COMPOUND; SALTS; POLYCHALCOGENIDE; SYSTEM; SUPERCONDUCTORS; SELENIDES AB The new ternary copper selenide NaCu4Se3 crystallizes in the RbCd4As3 structure type with the trigonal space group R3m and lattice constants a = 4.0316(4) angstrom and c = 31.438(8) angstrom. Its structure is built from two-dimensional slabs of 2/infinity [Cu4Se3] separated by Na+ cations. The compound is formally mixed-valent with Se2-/Se- atoms and exhibits metallic properties. It is a hole conductor with an electrical conductivity of similar to 300 S cm(-1) at room temperature and a thermopower of similar to 10 mu V K-1. Hall effect measurements indicate holes as the dominant carrier with a concentration of similar to 6.12(1) X 10(21) cm(-3) at 300 K. Density functional theory electronic structure calculations indicate p -type metallic behavior for the 2/infinity [Cu4Se3] framework, which is in a good agreement with the experimental metallic conductivity and Pauli paramagnetism. C1 [Sturza, Mihai; Bugaris, Daniel E.; Malliakas, Christos D.; Han, Fei; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Sturza, Mihai] Leibniz Inst Solid State & Mat Res Dresden IFW, Inst Solid State Res, D-01069 Dresden, Germany. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. RP Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013 OI Han, Fei/0000-0001-7782-2713 FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. Use of the Center for Nanoscale Materials, including resources in the Electron Microscopy Center where we performed EDS/SEM for elemental analysis, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 64 TC 1 Z9 1 U1 10 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2016 VL 55 IS 10 BP 4884 EP 4890 DI 10.1021/acs.inorgchem.6b00400 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DM1YY UT WOS:000376144000022 PM 27143407 ER PT J AU Borycz, J Paier, J Verma, P Darago, LE Xiao, DJ Truhlar, DG Long, JR Gagliardi, L AF Borycz, Joshua Paier, Joachim Verma, Pragya Darago, Lucy E. Xiao, Dianne J. Truhlar, Donald G. Long, Jeffrey R. Gagliardi, Laura TI Structural and Electronic Effects on the Properties of Fe-2(dobdc) upon Oxidation with N2O SO INORGANIC CHEMISTRY LA English DT Article ID METAL-ORGANIC FRAMEWORK; DENSITY-FUNCTIONAL THEORY; IRON(II) COORDINATION SITES; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CO2 ADSORPTION; FORCE-FIELDS; M-MOF-74 M; BASIS-SET; EXCHANGE AB We report electronic-vibrational, and magnetic properties, together with their structural dependences, for the metal organic framework Fe-2(dobdc) (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate) and its derivatives, Fe-2(O)(2)(dobdc) and Fe-2(OH)(2)(dobdc)-species arising in the previously proposed mechanism for the oxidation of ethane to ethanol using N2O as an oxidant. Magnetic susceptibility measurements reported for Fe-2(dobdc) in an earlier study and reported in the current study for Fe-0.26(II)[Fe-II(OH)](1.74)(dobdc)(DMF)(0.15)(THF)(0.22), which is more simply referred to as Fe-2(OH)(2)(dobdc), were used to confirm the computational results. Theory was also compared to experiment for infrared spectra and powder X-ray diffraction structures. Structural and magnetic properties were computed by using Kohn-Sham density functional theory both with periodic boundary conditions and with cluster models. In addition, we studied the effects of different treatments of the exchange interactions on the magnetic coupling parameters by comparing several approaches to the exchange-correlation functional: generalized gradient approximation (GGA), GGA with empirical Coulomb and exchange integrals for 3d electrons (GGA+U), nonseparable gradient approximation (NGA) with empirical Coulomb and exchange integrals for 3d electrons (NGA+U), hybrid GGA, meta-GGA, and hybrid meta-GGA. We found the coupling between the metal centers along a chain to be ferromagnetic in the case Of Fe2(dobdc) and antiferromagnetic in the cases of Fe-2(O)(2)(dobdc) and Fe-2(OH)(2)(dobdc). The shift in magnetic coupling behavior correlates with the changing electronic structure of the framework, which derives from both structural and electronic changes that occur upon metal oxidation and addition of the charge-balancing oxo and hydroxo ligands. C1 [Borycz, Joshua; Verma, Pragya; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Minnesota Supercomp Inst, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Borycz, Joshua; Verma, Pragya; Truhlar, Donald G.; Gagliardi, Laura] Univ Minnesota, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Borycz, Joshua; Verma, Pragya; Darago, Lucy E.; Xiao, Dianne J.; Truhlar, Donald G.; Long, Jeffrey R.; Gagliardi, Laura] Univ Minnesota, Nanoporous Mat Genome Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Paier, Joachim] Humboldt Univ, Inst Chem, Unter Linden 6, D-10099 Berlin, Germany. [Darago, Lucy E.; Xiao, Dianne J.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Truhlar, DG; Gagliardi, L (reprint author), Univ Minnesota, Minnesota Supercomp Inst, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA.; Truhlar, DG; Gagliardi, L (reprint author), Univ Minnesota, Chem Theory Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA.; Truhlar, DG; Long, JR; Gagliardi, L (reprint author), Univ Minnesota, Nanoporous Mat Genome Ctr, 207 Pleasant St SE, Minneapolis, MN 55455 USA.; Paier, J (reprint author), Humboldt Univ, Inst Chem, Unter Linden 6, D-10099 Berlin, Germany.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM joachim.paier@chemie.hu-berlin.de; truhlar@umn.edu; jrlong@berkeley.edu; gagliard@umn.edu RI Paier, Joachim/E-5850-2012; OI Darago, Lucy/0000-0001-7515-5558; Truhlar, Donald/0000-0002-7742-7294 FU U.S. DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-FG02-12ER16362]; Fonds der Chemischen Industrie (FCI); Doctoral Dissertation Fellowship; National Science Foundation (NSF) FX We thank Professor Joachim Sauer for insightful discussions and comments on the manuscript. This work was supported by the U.S. DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences (Award No. DE-FG02-12ER16362). This work has been carried out using the Minnesota Supercomputing Institute computational resources and National Energy Research Scientific Computing center resources and using computing time granted by the high-performance computer centers HLRN (North-German Supercomputing Alliance in Berlin and Hannover) and JUROPA (Forschungszentrum Julich). J.P. acknowledges financial support by the Fonds der Chemischen Industrie (FCI). P.V. and J.B. acknowledge financial support by the Doctoral Dissertation Fellowship. L.E.D. and D.J.X. thank the National Science Foundation (NSF) for providing graduate fellowship support. NR 85 TC 2 Z9 2 U1 18 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2016 VL 55 IS 10 BP 4924 EP 4934 DI 10.1021/acs.inorgchem.6b00467 PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DM1YY UT WOS:000376144000027 PM 27136308 ER PT J AU Browne, KP Maerzke, KA Travia, NE Morris, DE Scott, BL Henson, NJ Yang, P Kiplinger, JL Veauthier, JM AF Browne, Kevin P. Maerzke, Katie A. Travia, Nicholas E. Morris, David E. Scott, Brian L. Henson, Neil J. Yang, Ping Kiplinger, Jaqueline L. Veauthier, Jacqueline M. TI Synthesis, Characterization, and Density Functional Theory Analysis of Uranium and Thorium Complexes Containing Nitrogen-Rich 5-Methyltetrazolate Ligands SO INORGANIC CHEMISTRY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; COORDINATION POLYMERS; ORGANOURANIUM COMPLEXES; CRYSTAL-STRUCTURES; GAS-ADSORPTION; BASIS-SETS; AZIDE; MOLECULES; CHEMISTRY; NITRIDE AB Two nitrogen-rich, isostructural complexes of uranium and thorium, (C5Me5)(2)U[eta(2)-(N,N')-tetrazolate](2), (7) and (C5Me5)(2)Th[eta(2)-(NnN'-tetrazolate], (8), containing 5methyltetrazolate) have been synthesized and structurally characterized by single-crystal X-ray diffraction, electro-chemical methods, UV-visible near-IR spectroscopy, and variable-temperature H-1 NMR spectroscopy. Density functional theory (DFT) calculations yield favorable free energies of formation (approximately -375 kJ/mol) and optimized structures in good agreement with the experimental crystal structures. Additionally, calculated NMR chemical shifts of 7 and 8 are in good agreement with the variable -temperature H-1 NMR. experiments. Time-dependent DFT calculations of both complexes yield UV visible spectroscopic features that are consistent with experiment and provide assignments of the corresponding electronic transitions. The electronic transitions in the UV visible spectroscopic region are attributed to C5Me5 ligand-to-metal charge transfer. The low-lying molecular orbitals of the tetrazolate ligands (similar to 2 eV below the HOMO) do not contribute appreciably to experimentally observed electronic transitiohsrThe combined experimental and theoretical analysis of these new nitrogen-rich uranium and thorium complexes indicates the tetrazolate ligand 'behaves primarily as a sigma-donor. C1 [Browne, Kevin P.; Maerzke, Katie A.; Travia, Nicholas E.; Morris, David E.; Scott, Brian L.; Henson, Neil J.; Yang, Ping; Kiplinger, Jaqueline L.; Veauthier, Jacqueline M.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Henson, NJ; Yang, P; Kiplinger, JL; Veauthier, JM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM Veauthier@lanl.gov RI Kiplinger, Jaqueline/B-9158-2011; Scott, Brian/D-8995-2017; OI Kiplinger, Jaqueline/0000-0003-0512-7062; Scott, Brian/0000-0003-0468-5396; Henson, Neil/0000-0002-1842-7884; Veauthier, Jacqueline/0000-0003-2206-7786; Yang, Ping/0000-0003-4726-2860 FU U.S. Department of Energy through the LANL LDRD Program; LANL G.T. Seaborg Institute for Transactinium Science; Office of Basic Energy Sciences, Heavy Element Chemistry Program; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX For financial support of this work, we acknowledge the U.S. Department of Energy through the LANL LDRD Program (K.P.B., K.A.M., B.L.S., N.E.T., N.J.H, P.Y., J.L.K., J.M.V., materials and supplies), the LANL G.T. Seaborg Institute for Transactinium Science (PD Fellowships to K.P.B., N.E.T.), and the Office of Basic Energy Sciences, Heavy Element Chemistry Program (P.Y., J.L.K., B.L.S., materials and supplies). This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy (contract DE-AC52-06NA25396). NR 71 TC 4 Z9 4 U1 9 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2016 VL 55 IS 10 BP 4941 EP 4950 DI 10.1021/acs.inorgchem.6b00492 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DM1YY UT WOS:000376144000029 PM 27110650 ER PT J AU Kelley, MP Yang, P Clark, SB Clark, AE AF Kelley, Morgan P. Yang, Ping Clark, Sue B. Clark, Aurora E. TI Structural and Thermodynamic Properties of the Cm-III Ion Solvated by Water and Methanol SO INORGANIC CHEMISTRY LA English DT Article ID INDUCED FLUORESCENCE SPECTROSCOPY; DENSITY-FUNCTIONAL THEORY; PREFERENTIAL SOLVATION; MIXED-SOLVENTS; MOLECULAR-DYNAMICS; BASIS-SETS; ELECTRONIC-STRUCTURE; AQUEOUS-SOLUTION; 1ST PRINCIPLES; PAIR FORMATION AB The geometric and electronic structures of the 9-coordinate Cm3+ ion solvated with both water and methanol are systematically investigated in the gas phase at each possible solvent-shell composition and configuration using density functional theory and second-order Moller-Plesset perturbation theory. Ab initio molecular dynamics simulations are employed to assess the effects of second and third solvent shells on the gas phase structure. The ion solvent dissociation energy for methanol is greater than that of water, potentially because of increased charge donation to the ion made possible by the electron-rich methyl group. Further, the ion solvent dissociation energy and the ion solvent distance are shown to be dependent on the solvent-shell composition. This has implications for solvent exchange, which is generally the rate-limiting step in complexation reactions utilized in the separation of curium from complex metal mixtures that derive from the advanced nuclear fuel cycle. C1 [Kelley, Morgan P.; Clark, Sue B.; Clark, Aurora E.] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Kelley, Morgan P.; Yang, Ping] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. RP Kelley, MP; Clark, AE (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA.; Kelley, MP; Yang, P (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. EM m.kelley@wsu.edu; pyang@lanl.gov; auclark@wsu.edu OI Yang, Ping/0000-0003-4726-2860 FU G. T. Seaborg Institute, Los Alamos National Laboratory; Department of Energy Office of Science; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry Program, at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy, Office of Science, Heavy Elements Program [DE-SC-000-4102, DE-SC-000-1815]; U.S. Department of Energy, Biological and Environmental Research FX M.P.K. acknowledges support from the G. T. Seaborg Institute, Los Alamos National Laboratory, and a Department of Energy Office of Science Graduate Student Research Fellowship. P.Y. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry Program, at Los Alamos National Laboratory under Contract DE-AC52-06NA25396 (operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy). S.B.C. acknowledges support from the U.S. Department of Energy, Office of Science, Heavy Elements Program (Grant DE-SC-000-4102). A.E.C. acknowledges support from the U.S. Department of Energy, Office of Science, Heavy Elements Program (Grant DE-SC-000-1815). Calculations were performed using the Molecular Science Computing Facilities at William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy, Biological and Environmental Research, and located at Pacific Northwest National Laboratory. NR 66 TC 0 Z9 0 U1 5 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2016 VL 55 IS 10 BP 4992 EP 4999 DI 10.1021/acs.inorgchem.6b00477 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DM1YY UT WOS:000376144000034 PM 27120717 ER PT J AU Lin, QS Zhu, R Miller, GJ AF Lin, Qisheng Zhu, Ran Miller, Gordon J. TI Tuning Complexity by Lithiation: A Family of Intergrowth Structures Using Condensed hypho-Icosahedra in the Li-Doped Ca-Zn System SO INORGANIC CHEMISTRY LA English DT Article ID INTERMETALLIC COMPOUNDS; CRYSTAL-STRUCTURES; ZINTL PHASES; ALLOYS; SRMG4; EARTH AB Cluster chemistry of intermetallics with valence electron counts (VECs) in the range of 2,0-3.0 is intriguing. Lithiation of polar intermetallics in this VEC region is found to be an effective chemical route to produce new, complex structures with different stability mechanisms. In this work, two new complex intermetallic structures have been discovered in the Ca-Li-zn system: Ca(12)Li(x)Zn(59-)x, and Ca15LixZn75-x,. Ca12LixZn5-x_, x approximate to 5.65(3)-14.95(3), forms in the trigonal space group R3m, with a = 9.074(1)-9.1699(2) angstrom, c = 53,353(1)753.602(1) angstrom, and Z = 3. In comparison, Ca15LixZn75-x, x approximate to 19.07(2), crystallizes in the Space group P63/mmc, with a 9.183(1) A, c 45.191(5) A), and.Z = 2. Both structures are members of a large dritergrowth family featuring (.3m) slabs Of dimers (D) and trimers (T) stacking along [001], with the sequences DTDDTDDTD for- Ca15LixZn59-x and TDDDTDDD for Ca15LixZn75-x Each dimer consists of two face -sharing Zn-centered hypho-icosahedra, and each trimer comprises a Li -centered icosahedron sandwiched by two hypho-icosahedra. This intergrowth family includes several known intermetallic structure types involving very electropositive metals, e.g, SrMg5.2, Ba2Li421Al4.79, and Sr9Li17.5Al25.5. Because of cluster defects and condensation, both Ca12LixZn59-x, and Ca15LixZn75-x, are electronically akin to close -packed metals, and their structural stabilities can be interpreted by a Hume-Rothery mechanism rather than the Zintl Klemm concept. C1 [Lin, Qisheng; Miller, Gordon J.] US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Zhu, Ran; Miller, Gordon J.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Lin, QS (reprint author), US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. EM qslin@ameslab.gov FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX The research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract DE-AC02-07CH11358. R.Z. was an undergraduate student participant of the Department of Chemistry, Iowa State University. NR 35 TC 0 Z9 0 U1 3 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 16 PY 2016 VL 55 IS 10 BP 5041 EP 5050 DI 10.1021/acs.inorgchem.6b00612 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DM1YY UT WOS:000376144000039 PM 27115056 ER PT J AU Droghetti, A Rungger, I Das Pemmaraju, C Sanvito, S AF Droghetti, Andrea Rungger, Ivan Das Pemmaraju, Chaitanya Sanvito, Stefano TI Fundamental gap of molecular crystals via constrained density functional theory SO PHYSICAL REVIEW B LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; DERIVATIVE DISCONTINUITIES; GROUND-STATES; BAND-GAP; ENERGY; SYSTEMS; NUMBER; CHARGE AB The energy gap of a molecular crystal is one of the most important properties since it determines the crystal charge transport when the material is utilized in electronic devices. This is, however, a quantity difficult to calculate and standard theoretical approaches based on density functional theory (DFT) have proven unable to provide accurate estimates. In fact, besides the well-known band-gap problem, DFT completely fails in capturing the fundamental gap reduction occurring when molecules are packed in a crystal structures. The failure has to be associated with the inability of describing the electronic polarization and the real space localization of the charged states. Here we describe a scheme based on constrained DFT, which can improve upon the shortcomings of standard DFT. The method is applied to the benzene crystal, where we show that accurate results can be achieved for both the band gap and also the energy level alignment. C1 [Droghetti, Andrea] Univ Pais Vasco CFM CSIC UPV EHU MPC, Nanobio Spect Grp, Ave Tolosa 72, E-20018 San Sebastian, Spain. [Droghetti, Andrea] Univ Pais Vasco CFM CSIC UPV EHU MPC, ETSF, Ave Tolosa 72, E-20018 San Sebastian, Spain. [Droghetti, Andrea] DIPC, Ave Tolosa 72, E-20018 San Sebastian, Spain. [Rungger, Ivan] Natl Phys Lab, Mat Div, Teddington TW11 0LW, Middx, England. [Das Pemmaraju, Chaitanya] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Das Pemmaraju, Chaitanya] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Sanvito, Stefano] Univ Dublin Trinity Coll, Sch Phys, AMBER & CRANN Inst, Dublin 2, Ireland. RP Droghetti, A (reprint author), Univ Pais Vasco CFM CSIC UPV EHU MPC, Nanobio Spect Grp, Ave Tolosa 72, E-20018 San Sebastian, Spain.; Droghetti, A (reprint author), Univ Pais Vasco CFM CSIC UPV EHU MPC, ETSF, Ave Tolosa 72, E-20018 San Sebastian, Spain.; Droghetti, A (reprint author), DIPC, Ave Tolosa 72, E-20018 San Sebastian, Spain. RI DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; Droghetti, Andrea/F-8058-2016; CSIC-UPV/EHU, CFM/F-4867-2012 OI Droghetti, Andrea/0000-0003-4106-7327; FU European Union [618082 ACMOL]; "Ministerio de Economia y Competitividad" (Mineco) of Spain [FPDI-2013-16641]; European Research Council FX The authors are grateful to S. Refaely-Abramson for useful discussions. A.D. and I.R. were sponsored by the European Union through Project No. 618082 ACMOL. A.D. received additional support from the "Ministerio de Economia y Competitividad" (Mineco) of Spain (Grant No. FPDI-2013-16641). S.S. acknowledges the Quest project funded by European Research Council. Computational resources were provided by the Trinity Centre for High Performance Computing (TCHPC) and the Irish Centre for High-End Computing (ICHEC). NR 61 TC 1 Z9 1 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2016 VL 93 IS 19 AR 195208 DI 10.1103/PhysRevB.93.195208 PG 8 WC Physics, Condensed Matter SC Physics GA DM3LP UT WOS:000376248200003 ER PT J AU Zou, K Mandal, S Albright, SD Peng, R Pu, YJ Kumah, D Lau, C Simon, GH Dagdeviren, OE He, X Bozovic, I Schwarz, UD Altman, EI Feng, DL Walker, FJ Ismail-Beigi, S Ahn, CH AF Zou, Ke Mandal, Subhasish Albright, Stephen D. Peng, Rui Pu, Yujia Kumah, Divine Lau, Claudia Simon, Georg H. Dagdeviren, Omur E. He, Xi Bozovic, Ivan Schwarz, Udo D. Altman, Eric I. Feng, Donglai Walker, Fred J. Ismail-Beigi, Sohrab Ahn, Charles H. TI Role of double TiO2 layers at the interface of FeSe/SrTiO3 superconductors SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; SINGLE-LAYER; FESE FILMS; PHASE-DIAGRAM; THIN-FILMS; SRTIO3; ORIGIN; SYSTEM; GAP AB We determine the surface reconstruction of SrTiO3 used to achieve superconducting FeSe films in experiments, which is different from the 1 x 1 TiO2-terminated SrTiO3 assumed by most previous theoretical studies. In particular, we identify the existence of a double TiO2 layer at the FeSe/SrTiO3 interface that plays two important roles. First, it facilitates the epitaxial growth of FeSe. Second, ab initio calculations reveal a strong tendency for electrons to transfer from an oxygen deficient SrTiO3 surface to FeSe when the double TiO2 layer is present. The double layer helps to remove the hole pocket in the FeSe at the Gamma point of the Brillouin zone and leads to a band structure characteristic of superconducting samples. The characterization of the interface structure presented here is a key step towards the resolution of many open questions about this superconductor. C1 [Zou, Ke; Mandal, Subhasish; Kumah, Divine; He, Xi; Bozovic, Ivan; Walker, Fred J.; Ismail-Beigi, Sohrab; Ahn, Charles H.] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. [Zou, Ke; Mandal, Subhasish; Albright, Stephen D.; Kumah, Divine; Lau, Claudia; Simon, Georg H.; Dagdeviren, Omur E.; Schwarz, Udo D.; Altman, Eric I.; Walker, Fred J.; Ismail-Beigi, Sohrab; Ahn, Charles H.] Yale Univ, CRISP, New Haven, CT 06520 USA. [Albright, Stephen D.; Lau, Claudia; Ahn, Charles H.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Peng, Rui; Pu, Yujia; Feng, Donglai] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Peng, Rui; Pu, Yujia; Feng, Donglai] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China. [Simon, Georg H.; Dagdeviren, Omur E.; Schwarz, Udo D.; Ahn, Charles H.] Yale Univ, Dept Mech Engn & Mat Sci, New Haven, CT 06520 USA. [He, Xi; Bozovic, Ivan] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Schwarz, Udo D.; Altman, Eric I.] Yale Univ, Dept Chem & Environm Engn, New Haven, CT 06520 USA. RP Zou, K (reprint author), Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA.; Zou, K (reprint author), Yale Univ, CRISP, New Haven, CT 06520 USA. RI Zou, Ke/D-2322-2014; Kumah, Divine/A-7031-2011 OI Zou, Ke/0000-0002-1181-1779; Kumah, Divine/0000-0003-0715-1285 FU DMR NSF MRSEC [1119826]; AFOSR [FA9550-15-1-0472]; National Science Foundation of China; National Basic Research Program of China (973 Program) [2012CB921402]; US Department of Energy; US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; NSF [CNS 08-21132]; NSF XSEDE resources [TG-MCA08 x 007] FX This research is sponsored by the DMR NSF MRSEC 1119826 and the AFOSR under Grant No. FA9550-15-1-0472. R.P., Y.P., and D.F. acknowledge support from the National Science Foundation of China, and the National Basic Research Program of China (973 Program) under Grant No. 2012CB921402. The work at Argonne National Laboratory is supported by the US Department of Energy. Magnetic measurements (X.H. and I.B.) at BNL were supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Computational facilities are supported by NSF Grant No. CNS 08-21132 and by the facilities and staff of the Yale University Faculty of Arts and Sciences High Performance Computing Center. Additional computations were carried out via the NSF XSEDE resources through Grant No. TG-MCA08 x 007. NR 54 TC 3 Z9 3 U1 12 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 16 PY 2016 VL 93 IS 18 AR 180506 DI 10.1103/PhysRevB.93.180506 PG 6 WC Physics, Condensed Matter SC Physics GA DM3LA UT WOS:000376246700001 ER PT J AU Matters, DA Lerch, AG Hurst, AM Szentmiklosi, L Carroll, JJ Detwiler, B Revay, Z McClory, JW McHale, SR Firestone, RB Sleaford, BW Krticka, M Belgya, T AF Matters, D. A. Lerch, A. G. Hurst, A. M. Szentmiklosi, L. Carroll, J. J. Detwiler, B. Revay, Zs. McClory, J. W. McHale, S. R. Firestone, R. B. Sleaford, B. W. Krticka, M. Belgya, T. TI Investigation of Re-186 via radiative thermal-neutron capture on Re-185 SO PHYSICAL REVIEW C LA English DT Article ID GAMMA ACTIVATION-ANALYSIS; BUDAPEST RESEARCH REACTOR; CROSS-SECTIONS; NUCLEAR-DATA; RESONANCES; STRENGTH; STANDARDIZATION; WIDTHS; PGAA AB Partial gamma-ray production cross sections and the total radiative thermal-neutron capture cross section for the Re-185(n,gamma) Re-186 reaction were measured using the Prompt Gamma Activation Analysis facility at the Budapest Research Reactor with an enriched Re-185 target. The Re-186 cross sections were standardized using well-known Cl-35(n,gamma) Cl-36 cross sections from irradiation of a stoichiometric (ReCl3)-Re-nat target. The resulting cross sections for transitions feeding the Re-186 ground state from low-lying levels below a cutoff energy of E-c = 746 keV were combined with a modeled probability of ground-state feeding from levels above E-c to arrive at a total cross section of sigma(0) = 111(6) b for radiative thermal-neutron capture on Re-185. A comparison of modeled discrete-level populations with measured transition intensities led to proposed revisions for seven tentative spin-parity assignments in the adopted level scheme for Re-186. Additionally, 102 primary gamma rays were measured, including 50 previously unknown. A neutron-separation energy of S-n = 6179.59(5) keV was determined from a global least-squares fit of the measured gamma-ray energies to the known Re-186 decay scheme. The total capture cross section and separation energy results are comparable to earlier measurements of these values. C1 [Matters, D. A.; McClory, J. W.] US Air Force, Inst Technol, Wright Patterson AFB, OH 45433 USA. [Lerch, A. G.; McHale, S. R.] Def Threat Reduct Agcy, Ft Belvoir, VA 22060 USA. [Hurst, A. M.; Firestone, R. B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Hurst, A. M.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Szentmiklosi, L.; Belgya, T.] Hungarian Acad Sci, Ctr Energy Res, H-1525 Budapest, Hungary. [Carroll, J. J.] US Army Res Lab, Adelphi, MD 20783 USA. [Detwiler, B.] Youngstown State Univ, Youngstown, OH 44555 USA. [Revay, Zs.] Tech Univ Munich, Heinz Maier Leibnitz Zentrum MLZ 7, Garching, Germany. [Sleaford, B. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Krticka, M.] Charles Univ Prague, Fac Math & Phys, CZ-18000 Prague, Czech Republic. RP Matters, DA (reprint author), US Air Force, Inst Technol, Wright Patterson AFB, OH 45433 USA. EM david.a.matters.mil@mail.mil RI Szentmiklosi, Laszlo/F-5362-2015 OI Szentmiklosi, Laszlo/0000-0001-7747-8545 FU Defense Threat Reduction Agency Grant [HDTRA1-08-1-0014]; University of California - Office of Science, Office of Basic Energy Sciences, of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy at Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Domestic Nuclear Detection Office of the Department of Homeland Security; NAP VENEUS08 grant [OMFB-00184/2006]; Czech Science Foundation [13-07117S] FX This work was initiated under Defense Threat Reduction Agency Grant No. HDTRA1-08-1-0014 (YSU). Later work was performed under the auspices of the University of California, supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231, and at Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Additional funding was provided by the Domestic Nuclear Detection Office of the Department of Homeland Security. Access to the Budapest PGAA facility was financially supported by the NAP VENEUS08 grant under Contract No. OMFB-00184/2006. This work was also supported by the Czech Science Foundation under Grant No. 13-07117S. The authors gratefully acknowledge the support of the operations staff at the Budapest Research Reactor. D.M. thanks Dr. C.J. Chiara for help reviewing the manuscript. NR 70 TC 0 Z9 0 U1 8 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 16 PY 2016 VL 93 IS 5 AR 054319 DI 10.1103/PhysRevC.93.054319 PG 19 WC Physics, Nuclear SC Physics GA DM3NN UT WOS:000376253300001 ER PT J AU Finnell, J AF Finnell, Joshua TI The Sport of Kings SO LIBRARY JOURNAL LA English DT Book Review C1 [Finnell, Joshua] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Finnell, J (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. NR 1 TC 0 Z9 0 U1 0 U2 0 PU REED BUSINESS INFORMATION PI NEW YORK PA 360 PARK AVENUE SOUTH, NEW YORK, NY 10010 USA SN 0363-0277 J9 LIBR J JI Libr. J. PD MAY 15 PY 2016 VL 141 IS 9 BP 69 EP 69 PG 1 WC Information Science & Library Science SC Information Science & Library Science GA DM3EC UT WOS:000376228600137 ER PT J AU Conaway, CH Thordsen, JJ Manning, MA Cook, PJ Trautz, RC Thomas, B Kharaka, YK AF Conaway, Christopher H. Thordsen, James J. Manning, Michael A. Cook, Paul J. Trautz, Robert C. Thomas, Burt Kharaka, Yousif K. TI Comparison of geochemical data obtained using four brine sampling methods at the SECARB Phase III Anthropogenic Test CO2 injection site, Citronelle Oil Field, Alabama SO INTERNATIONAL JOURNAL OF COAL GEOLOGY LA English DT Article DE Brine; Carbon capture and storage; Produced water; U-tube; Wireline fluid sampling ID POTENTIAL ENVIRONMENTAL-ISSUES; WATER-ROCK INTERACTIONS; STATES GULF-COAST; SEDIMENTARY BASINS; SALINE AQUIFERS; FRIO-FORMATION; STORAGE; SEQUESTRATION; USA; CARBON AB The chemical composition of formation water and associated gases from the lower Cretaceous Paluxy Formation was determined using four different sampling methods at a characterization well in the Citronelle Oil Field, Alabama, as part of the Southeast Regional Carbon Sequestration Partnership (SECARB) Phase III Anthropogenic Test, which is an integrated carbon capture and storage project. In this study, formation water and gas samples were obtained from well D-9-8 #2 at Citronelle using gas lift, electric submersible pump, U-tube, and a downhole vacuum sampler (VS) and subjected to both field and laboratory analyses. Field chemical analyses included electrical conductivity, dissolved sulfide concentration, alkalinity, and pH; laboratory analyses included major, minor and trace elements, dissolved carbon, volatile fatty acids, free and dissolved gas species. The formation water obtained from this well is a Na-Ca-Cl-type brine with a salinity of about 200,000 mg/L total dissolved solids. Differences were evident between sampling methodologies, particularly in pH, Fe and alkalinity. There was little gas in samples, and gas composition results were strongly influenced by sampling methods. The results of the comparison demonstrate the difficulty and importance of preserving volatile analytes in samples, with the VS and U-tube system performing most favorably in this aspect. Published by Elsevier B.V. C1 [Conaway, Christopher H.; Thordsen, James J.; Thomas, Burt; Kharaka, Yousif K.] USGS Natl Res Program, Menlo Pk, CA 94025 USA. [Manning, Michael A.] USGS Lower Mississippi Gulf Water Sci Ctr, Jackson, MS USA. [Cook, Paul J.] Lawrence Berkeley Natl Labs, Div Earth Sci, Berkeley, CA USA. [Trautz, Robert C.] Elect Power Res Inst, Palo Alto, CA USA. [Thomas, Burt] Willamette Univ, Dept Environm & Earth Sci, Salem, OR 97301 USA. RP Conaway, CH (reprint author), USGS Natl Res Program, Menlo Pk, CA 94025 USA. EM cconaway@usgs.gov RI Cook, Paul/I-4788-2016 FU US Department of Energy's (DOE) National Energy Technology Laboratory (NETL); DOE FX This project was conducted as part of the Southeast Regional Carbon Sequestration Partnership (SECARB) Phase III Anthropogenic Test, which is managed by the Southern States Energy Board in partnership with Southern Company, the Electric Power Research Institute (EPRI), and Advanced Resources International (ARI). The test is an integrated capture and storage project funded in part by the US Department of Energy's (DOE) National Energy Technology Laboratory (NETL), with Bruce M. Brown and Mary A. Sullivan as Program Coordinators. R. Burt Thomas was supported in part by an appointment to the NETL Research Participation Program, sponsored by the DOE and administered by the Oak Ridge Institute for Science and Education (ORISE). Barry M. Freifeld from the Lawrence Berkeley National Laboratory (LBNL) provided engineering expertise for the U-tube installation, and Tom Daley (LBNL) provided geophysical support. We thank Gil Ambats, Atosa Abedni, Brent Topping, John Fitzpatrick, and Michael Murphy (USGS) for analytical support. Determinations of NORMs by gamma spectroscopy were performed by Peter Swarzenski (USGS). The U-tube sampler was operated in 2013 by RDH Environmental Services. Gas samples were analyzed by W.C. Evans (USGS). We thank Allen Roberts (USGS), Steve Bumgardner and Hunter Jonsson (ARI), and host-site workers at Denbury Onshore Inc. We thank Mark A. Engle, Gerald R. Hill, and Scott C. Wehner, and two anonymous reviewers for providing comments to improve the manuscript. Any use of trade names is for descriptive purposes only and does not imply endorsement by the U.S. Government. NR 41 TC 0 Z9 0 U1 3 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0166-5162 EI 1872-7840 J9 INT J COAL GEOL JI Int. J. Coal Geol. PD MAY 15 PY 2016 VL 162 BP 85 EP 95 DI 10.1016/j.coal.2016.06.001 PG 11 WC Energy & Fuels; Geosciences, Multidisciplinary SC Energy & Fuels; Geology GA DR7KT UT WOS:000380079200009 ER PT J AU Cohen, I Kayode, O Hockla, A Sankaran, B Radisky, DC Radisky, ES Papo, N AF Cohen, Itay Kayode, Olumide Hockla, Alexandra Sankaran, Banumathi Radisky, Derek C. Radisky, Evette S. Papo, Niv TI Combinatorial protein engineering of proteolytically resistant mesotrypsin inhibitors as candidates for cancer therapy SO BIOCHEMICAL JOURNAL LA English DT Article DE cancer therapy; directed evolution; enzyme inhibition; mesotrypsin; protease inhibitor; protein engineering; proteolysis; X-ray structure ID KUNITZ DOMAIN INHIBITORS; YEAST SURFACE-DISPLAY; FACTOR-FACTOR VIIA; DIRECTED EVOLUTION; PHAGE DISPLAY; ITERATIVE OPTIMIZATION; TRYPSIN-INHIBITORS; PLASMA KALLIKREIN; PROSTATE-CANCER; GROWTH-FACTOR AB Engineered protein therapeutics offer advantages, including strong target affinity, selectivity and low toxicity, but like natural proteins can be susceptible to proteolytic degradation, thereby limiting their effectiveness. A compelling therapeutic target is mesotrypsin, a protease up-regulated with tumour progression, associated with poor prognosis, and implicated in tumour growth and progression of many cancers. However, with its unique capability for cleavage and inactivation of proteinaceous inhibitors, mesotrypsin presents a formidable challenge to the development of biological inhibitors. We used a powerful yeast display platform for directed evolution, employing a novel multi-modal library screening strategy, to engineer the human amyloid precursor protein Kunitz protease inhibitor domain (APPI) simultaneously for increased proteolytic stability, stronger binding affinity and improved selectivity for mesotrypsin inhibition. We identified a triple mutant APPI(M17G/I18F/F34V), with a mesotrypsin inhibition constant (K-i) of 89 pM, as the strongest mesotrypsin inhibitor yet reported; this variant displays 1459-fold improved affinity, up to 350 000-fold greater specificity and 83-fold improved proteolytic stability compared with wildtype APPI. We demonstrated that APPI(M17G/I18F/F34V) acts as a functional inhibitor in cell-based models of mesotrypsin-dependent prostate cancer cellular invasiveness. Additionally, by solving the crystal structure of the APPI(M17G/I18F/F34V)-mesotrypsin complex, we obtained new insights into the structural and mechanistic basis for improved binding and proteolytic resistance. Our study identifies a promising mesotrypsin inhibitor as a starting point for development of anticancer protein therapeutics and establishes proof-of-principle for a novel library screening approach that will be widely applicable for simultaneously evolving proteolytic stability in tandem with desired functionality for diverse protein scaffolds. C1 [Cohen, Itay; Papo, Niv] Ben Gurion Univ Negev, Dept Biotechnol Engn, IL-84105 Beer Sheva, Israel. [Cohen, Itay; Papo, Niv] Ben Gurion Univ Negev, Natl Inst Biotechnol Negev, IL-84105 Beer Sheva, Israel. [Kayode, Olumide; Hockla, Alexandra; Radisky, Derek C.; Radisky, Evette S.] Mayo Clin, Ctr Comprehens Canc, Dept Canc Biol, Jacksonville, FL 32224 USA. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. RP Papo, N (reprint author), Ben Gurion Univ Negev, Dept Biotechnol Engn, IL-84105 Beer Sheva, Israel.; Papo, N (reprint author), Ben Gurion Univ Negev, Natl Inst Biotechnol Negev, IL-84105 Beer Sheva, Israel.; Radisky, ES (reprint author), Mayo Clin, Ctr Comprehens Canc, Dept Canc Biol, Jacksonville, FL 32224 USA. EM radisky.evette@mayo.edu; papo@bgu.ac.il FU European Research Council [336041]; Prostate Cancer Foundation [13YOUN020]; National Institutes of Health [R01CA154387] FX This work was supported by the European Research Council 'Ideas programme' ERC-2013-StG [grant number 336041]; the Prostate Cancer Foundation [grant number 13YOUN020 (to N.P.); and the National Institutes of Health [grant number R01CA154387 (to E.S.R.)]. NR 51 TC 2 Z9 2 U1 2 U2 4 PU PORTLAND PRESS LTD PI LONDON PA CHARLES DARWIN HOUSE, 12 ROGER STREET, LONDON WC1N 2JU, ENGLAND SN 0264-6021 EI 1470-8728 J9 BIOCHEM J JI Biochem. J. PD MAY 15 PY 2016 VL 473 BP 1329 EP 1341 DI 10.1042/BJ20151410 PN 10 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DN6TI UT WOS:000377208700004 PM 26957636 ER PT J AU Hayami, S Kusunose, H Motome, Y AF Hayami, Satoru Kusunose, Hiroaki Motome, Yukitoshi TI Asymmetric Magnon Excitation by Spontaneous Toroidal Ordering SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID CRYSTALS AB The effects of spontaneous toroidal ordering on magnetic excitation are theoretically investigated for a localized spin model that includes a staggered Dzyaloshinsky-Moriya interaction and anisotropic exchange interactions, which arise from the antisymmetric spin-orbit coupling and the multiorbital correlation effect. We show that the model exhibits a Neel-type antiferromagnetic order, which simultaneously accompanies a ferroic toroidal order. We find that the occurrence of toroidal order modulates the magnon dispersion in an asymmetric way with respect to the wave number: a toroidal dipole order on the zigzag chain leads to a band-bottom shift, while a toroidal octupole order on the honeycomb lattice gives rise to a valley splitting. These asymmetric magnon excitations could be a source of unusual magnetic responses, such as nonreciprocal magnon transport. A variety of modulations are discussed while changing the lattice and magnetic symmetries. The implications regarding candidate materials for asymmetric magnon excitations are presented. C1 [Hayami, Satoru] Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA. [Hayami, Satoru] Los Alamos Natl Lab, CNLS, POB 1663, Los Alamos, NM 87545 USA. [Hayami, Satoru; Motome, Yukitoshi] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Kusunose, Hiroaki] Meiji Univ, Dept Phys, Kawasaki, Kanagawa 2148571, Japan. [Hayami, Satoru] Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. RP Hayami, S (reprint author), Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA.; Hayami, S (reprint author), Los Alamos Natl Lab, CNLS, POB 1663, Los Alamos, NM 87545 USA.; Hayami, S (reprint author), Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan.; Hayami, S (reprint author), Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. FU U.S. DOE through LDRD program [DE-AC52-06NA25396]; Strategic Programs for Innovative Research (SPIRE), MEXT [24340076, 15K05176, 15H05885]; Computational Materials Science Initiative (CMSI), Japan FX The authors thank T. Arima for enlightening discussions. They also thank K. Matan, Y. Onose, and T. J. Sato for fruitful discussions on the experimental situations. Work at LANL was performed under the auspices of the U.S. DOE contract No. DE-AC52-06NA25396 through the LDRD program. This work was supported by Grants-in-Aid for Scientific Research (Nos. 24340076 and 15K05176), a Grant-in-Aid for Scientific Research on Innovative Areas (No. 15H05885), the Strategic Programs for Innovative Research (SPIRE), MEXT, and the Computational Materials Science Initiative (CMSI), Japan. NR 31 TC 1 Z9 1 U1 6 U2 7 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD MAY 15 PY 2016 VL 85 IS 5 AR 053705 DI 10.7566/JPSJ.85.053705 PG 5 WC Physics, Multidisciplinary SC Physics GA DN0PX UT WOS:000376766900004 ER PT J AU Wu, CC Duan, JC Liu, T Smith, RD Qian, WJ AF Wu, Chaochao Duan, Jicheng Liu, Tao Smith, Richard D. Qian, Wei-Jun TI Contributions of immunoaffinity chromatography to deep proteome profiling of human biofluids SO JOURNAL OF CHROMATOGRAPHY B-ANALYTICAL TECHNOLOGIES IN THE BIOMEDICAL AND LIFE SCIENCES LA English DT Article DE Biofluid; Immunoaffinity chromatography; Plasma/Serum; Immunodepletion; Immunoenrichment; Biomarker discovery; Proteomics; Affinity proteomics ID HUMAN PLASMA PROTEOME; LECTIN AFFINITY-CHROMATOGRAPHY; TARGETED MASS-SPECTROMETRY; HUMAN CEREBROSPINAL-FLUID; HIGH-ABUNDANCE PROTEINS; LUNG-CANCER PATIENTS; BIOMARKER DISCOVERY; QUANTITATIVE PROTEOMICS; OVARIAN-CANCER; HUMAN SERUM AB Human biofluids, especially blood plasma or serum, hold great potential as the sources of candidate biomarkers for various diseases; however, the enormous dynamic range of protein concentrations in biofluids represents a significant analytical challenge for detecting promising low-abundance proteins. Over the last decade, various immunoaffinity chromatographic methods have been developed and routinely applied for separating low-abundance proteins from the high- and moderate-abundance proteins, thus enabling much more effective detection of low-abundance proteins. Herein, we review the advances of immunoaffinity separation methods and their contributions to the proteomic applications in human biofluids. The limitations and future perspectives of immunoaffinity separation methods are also discussed. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wu, Chaochao; Duan, Jicheng; Liu, Tao; Smith, Richard D.; Qian, Wei-Jun] Pacific NW Natl Lab, Div Biol Sci, POB 999,MSIN K8-98, Richland, WA 99352 USA. RP Qian, WJ (reprint author), Pacific NW Natl Lab, Div Biol Sci, POB 999,MSIN K8-98, Richland, WA 99352 USA. EM weijun.qian@pnnl.gov RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; QIAN, Wei-Jun/0000-0002-5393-2827 FU NIH grant from National Cancer Institute Clinical Proteomic Tumor Analysis Consortium (CPTAC) [U24-CA-160019]; NIGMS Biomedical Technology Research Resource [P41GM103493] FX Portions of this work were supported by the NIH grant U24-CA-160019 from the National Cancer Institute Clinical Proteomic Tumor Analysis Consortium (CPTAC), and NIGMS Biomedical Technology Research Resource P41GM103493. NR 161 TC 2 Z9 2 U1 3 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1570-0232 EI 1873-376X J9 J CHROMATOGR B JI J. Chromatogr. B PD MAY 15 PY 2016 VL 1021 SI SI BP 57 EP 68 DI 10.1016/j.jchromb.2016.01.015 PG 12 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA DM7MV UT WOS:000376545600006 PM 26868616 ER PT J AU Li, ZG Qiu, F Wang, JH AF Li, Zhigang Qiu, Feng Wang, Jianhui TI Data-driven real-time power dispatch for maximizing variable renewable generation SO APPLIED ENERGY LA English DT Article DE Data-driven; Real-time dispatch; Renewable energy generation; Uncertainty ID UNIT COMMITMENT; OPTIMIZATION; CONSTRAINTS AB Traditional power dispatch methods have difficulties in accommodating large-scale variable renewable generation (VRG) and have resulted in unnecessary VRG spillage in the practical industry. The recent dispatchable-interval-based methods have the potential to reduce VRG curtailment, but the dispatchable intervals are not allocated effectively due to the lack of exploiting historical dispatch records of VRG units. To bridge this gap, this paper proposes a novel data-driven real-time dispatch approach to maximize VRG utilization by using do-not-exceed (DNE) limits. This approach defines the maximum generation output ranges that the system can accommodate without compromising reliability. The DNE limits of VRG units and operating base points of conventional units are co-optimized by hybrid stochastic and robust optimization, and the decision models are formulated as mixed-integer linear programs by the sample average approximation technique exploiting historical VRG data. A strategy for selecting historical data samples is also proposed to capture the VRG uncertainty more accurately under variant prediction output levels. Computational experiments show the effectiveness of the proposed methods. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Li, Zhigang] Tsinghua Univ, Dept Elect Engn, Beijing 100084, Peoples R China. [Qiu, Feng; Wang, Jianhui] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Li, ZG (reprint author), Tsinghua Univ, Rm 3-120,West Main Bldg, Beijing 100084, Peoples R China. EM lizg163@126.com NR 22 TC 1 Z9 1 U1 7 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD MAY 15 PY 2016 VL 170 BP 304 EP 313 DI 10.1016/j.apenergy.2016.02.125 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DK0KJ UT WOS:000374601400027 ER PT J AU Mo, DL Fang, HB Niu, KF Liu, J Wu, M Li, SY Zhu, TEN Aleskandarany, MA Arora, A Lobo, DN Madhusudan, S Balajee, AS Chi, ZF Zhao, YL AF Mo, Dongliang Fang, Hongbo Niu, Kaifeng Liu, Jing Wu, Meng Li, Shiyou Zhu, Tienian Aleskandarany, Mohammed A. Arora, Arvind Lobo, Dileep N. Madhusudan, Srinivasan Balajee, Adayabalam S. Chi, Zhenfen Zhao, Yongliang TI Human Helicase RECQL4 Drives Cisplatin Resistance in Gastric Cancer by Activating an AKT-YB1-MDR1 Signaling Pathway SO CANCER RESEARCH LA English DT Article ID ROTHMUND-THOMSON-SYNDROME; BOX BINDING-PROTEIN; BREAST-CANCER; CHROMOSOMAL INSTABILITY; GASTROESOPHAGEAL CANCER; MOLECULAR-MECHANISMS; NUCLEAR-LOCALIZATION; DRUG-RESISTANCE; GENE-EXPRESSION; FACTOR YB-1 AB Elevation of the DNA-unwinding helicase RECQL4, which participates in various DNA repair pathways, has been suggested to contribute to the pathogenicity of various human cancers, including gastric cancer. In this study, we addressed the prognostic and chemotherapeutic significance of RECQL4 in human gastric cancer, which has yet to be determined. We observed significant increases in RECQL4 mRNA or protein in >70% of three independent sets of human gastric cancer specimens examined, relative to normal gastric tissues. Strikingly, high RECQL4 expression in primary tumors correlated well with poor survival and gastric cancer lines with high RECQL4 expression displayed increased resistance to cisplatin treatment. Mechanistic investigations revealed a novel role for RECQL4 in transcriptional regulation of the multidrug resistance gene MDR1, through a physical interaction with the transcription factor YB1. Notably, ectopic expression of RECQL4 in cisplatin-sensitive gastric cancer cells with low endogenous RECQL4 was sufficient to render them resistant to cisplatin, in a manner associated with YB1 elevation and MDR1 activation. Conversely, RECQL4 silencing in cisplatin-resistant gastric cancer cells with high endogenous RECQL4 suppressed YB1 phosphorylation, reduced MDR1 expression, and resensitized cells to cisplatin. In establishing RECQL4 as a critical mediator of cisplatin resistance in gastric cancer cells, our findings provide a therapeutic rationale to target RECQL4 or the downstream AKT-YB1-MDR1 axis to improve gastric cancer treatment. (C) 2016 AACR. C1 [Mo, Dongliang; Fang, Hongbo; Niu, Kaifeng; Liu, Jing; Li, Shiyou; Chi, Zhenfen; Zhao, Yongliang] Chinese Acad Sci, Key Lab Genom & Precis Med, Gastrointestinal Canc Res Ctr, Beijing Inst Genom, Beijing 100101, Peoples R China. [Mo, Dongliang; Niu, Kaifeng; Liu, Jing] Univ Chinese Acad Sci, Beijing, Peoples R China. [Wu, Meng] Hebei Acad Sci, Biol Inst, Shijiazhuang, Peoples R China. [Zhu, Tienian] Bethune Int Peace Hosp, Dept Med Oncol, Shijiazhuang, Peoples R China. [Aleskandarany, Mohammed A.; Arora, Arvind; Madhusudan, Srinivasan] Univ Nottingham, Sch Med, Univ Nottingham Hosp, Div Canc & Stem Cells, City Hosp Campus, Nottingham, England. [Lobo, Dileep N.] Univ Nottingham Hosp, Gastrointestinal Surg, Natl Inst Hlth Res, Nottingham Digest Dis Ctr,Biomed Res Unit, Nottingham NG7 2UH, England. [Lobo, Dileep N.] Univ Nottingham, Queens Med Ctr, Nottingham NG7 2RD, England. [Balajee, Adayabalam S.] Oak Ridge Associated Univ, Oak Ridge Inst Sci & Educ, REAC TS, Oak Ridge, TN USA. RP Zhao, YL (reprint author), Chinese Acad Sci, Beijing Inst Genom, Beijing 100101, Peoples R China. EM chizf@big.ac.cn; zhaoyongliang@big.ac.cn OI Madhusudan, Srinivasan/0000-0002-5354-5480; Lobo, Dileep/0000-0003-1187-5796 NR 41 TC 3 Z9 3 U1 5 U2 10 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD MAY 15 PY 2016 VL 76 IS 10 BP 3057 EP 3066 DI 10.1158/0008-5472.CAN-15-2361 PG 10 WC Oncology SC Oncology GA DL7SS UT WOS:000375841000023 PM 27013200 ER PT J AU Mahalik, JP Yang, YB Deodhar, C Ankner, JF Lokitz, BS Kilbey, SM Sumpter, BG Kumar, R AF Mahalik, J. P. Yang, Yubo Deodhar, Chaitra Ankner, John F. Lokitz, Bradley S. Kilbey, S. Michael, II Sumpter, Bobby G. Kumar, Rajeev TI Monomer Volume Fraction Profiles in pH Responsive Planar Polyelectrolyte Brushes SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE charge regulation; field theory; neutron reflectivity; polyelectrolyte brushes ID CONSISTENT-FIELD THEORY; GRAFTED POLYMER BRUSH; WEAK POLYACID BRUSHES; POLY(METHACRYLIC ACID); NEUTRON REFLECTIVITY; SWELLING BEHAVIOR; SCALING THEORY; MOLECULAR-DYNAMICS; DENSITY PROFILE; IONIC-STRENGTH AB Spatial dependencies of monomer volume fraction profiles of pH responsive polyelectrolyte brushes were investigated using field theories and neutron reflectivity experiments. In particular, planar polyelectrolyte brushes in good solvent were studied and direct comparisons between predictions of the theories and experimental measurements are presented. The comparisons between the theories and the experimental data reveal that solvent entropy and ion-pairs resulting from adsorption of counterions from the added salt play key roles in affecting the monomer distribution and must be taken into account in modeling polyelectrolyte brushes. Furthermore, the utility of this physics-based approach based on these theories for the prediction and interpretation of neutron reflectivity profiles in the context of pH responsive planar polyelectrolyte brushes such as polybasic poly(2-(dimethylamino)ethyl methacrylate) (PDMAEMA) and polyacidic poly(methacrylic acid) (PMAA) brushes is demonstrated. The approach provides a quantitative way of estimating molecular weights of the polymers polymerized using surface-initiated atom transfer radical polymerization. (C) 2016 Wiley Periodicals, Inc. C1 [Mahalik, J. P.; Sumpter, Bobby G.; Kumar, Rajeev] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Yang, Yubo] Denison Univ, Granville, OH 43023 USA. [Deodhar, Chaitra; Kilbey, S. Michael, II] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ankner, John F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Mahalik, J. P.; Lokitz, Bradley S.; Sumpter, Bobby G.; Kumar, Rajeev] Oak Ridge Natl Lab, Ctr Nanophase Materials Sci, Oak Ridge, TN 37831 USA. RP Mahalik, JP; Kumar, R (reprint author), Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA.; Mahalik, JP; Kumar, R (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Materials Sci, Oak Ridge, TN 37831 USA. EM mahalikjp@ornl.gov; kumarr@ornl.gov RI Sumpter, Bobby/C-9459-2013; Kumar, Rajeev/Q-2255-2015; mahalik, jyoti/A-9258-2016 OI Sumpter, Bobby/0000-0001-6341-0355; Kumar, Rajeev/0000-0001-9494-3488; mahalik, jyoti/0000-0003-4448-4126 FU National Science Foundation [0840249, 1133320] FX BSL, BGS, and RK acknowledge work performed at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility. JPM, JFA, BGS, and RK acknowledge support for aspects of code development from the ORNL Laboratory Directed Research and Development. SMKII and CD acknowledge funding from the National Science Foundation (Award Nos. 0840249 and 1133320) that supported experimental efforts. NR 73 TC 6 Z9 6 U1 8 U2 23 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD MAY 15 PY 2016 VL 54 IS 10 BP 956 EP 964 DI 10.1002/polb.24008 PG 9 WC Polymer Science SC Polymer Science GA DK1UX UT WOS:000374701300003 ER PT J AU Landauer, AK Barnhill, WC Qu, J AF Landauer, Alexander K. Barnhill, William C. Qu, Jun TI Correlating mechanical properties and anti-wear performance of tribofilms formed by ionic liquids, ZDDP and their combinations SO WEAR LA English DT Article DE Nanoindentation; Ionic liquid; ZDDP; Tribofilm; Hardness; Resistance-to-plastic-deformation ID LUBRICANT ADDITIVES; TRIBOLOGICAL BEHAVIOR; FILMS; NANOINDENTATION; STEEL; ORGANOPHOSPHATE; INDENTATION; DEPTH AB This article examines the elasticity, hardness, and resistance-to-plastic-deformation (P/S-2) measured via nanoindentation of several tribofilms and correlates these properties to friction and wear behavior. The tribofilms were generated by ball-on-plate reciprocating sliding lubricated by a base oil containing an ionic liquid, phosphonium-organophosphate or ammonium-organophosphate, zinc dialkyldithiophosphate (ZDDP), or combination of IL and ZDDP. Nanoindentation was conducted at room and elevated temperatures. While there seems little correlation between the tribofilm hardness and tribological behavior, a higher modulus generally leads to better friction and wear performance. Interestingly, a lower P/S-2 ratio tends to reduce friction and improve wear protection, which is in an opposite trend as reported for bulk materials. This is likely attributable to the dynamic, self-healing characteristics of tribofilms. (C) 2016 Elsevier B.V. All rights reserved. C1 [Landauer, Alexander K.; Barnhill, William C.; Qu, Jun] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. [Landauer, Alexander K.] Brown Univ, Sch Engn, Providence, RI 02912 USA. RP Qu, J (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. EM qujn@ornl.gov OI Qu, Jun/0000-0001-9466-3179 FU Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, US Department of Energy (DOE); DOE Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships program; DOE Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Higher Education Research Experience (HERE) program; U.S. Department of Energy [DE-AC05-00OR22725] FX The authors thank A.E. Marquez Rossy from ORNL and Dr. S. Wang, Y. Meng, and D. Wu from University of Tennessee for training with nanoindentation, Dr. H. Luo from ORNL for synthesizing ILs, and Dr. B. L. Papke from Shell for providing the base oil and ZDDP. This research was sponsored by the Vehicle Technologies Office, Office of Energy Efficiency and Renewable Energy, US Department of Energy (DOE). This work was supported in part by the DOE Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships program (Landauer) and Higher Education Research Experience (HERE) program (Barnhill).; This manuscript has been authored by UT-Battelle, LLC, under Contract no. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 40 TC 2 Z9 2 U1 10 U2 22 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0043-1648 EI 1873-2577 J9 WEAR JI Wear PD MAY 15 PY 2016 VL 354-355 BP 78 EP 82 DI 10.1016/j.wear.2016.03.003 PG 5 WC Engineering, Mechanical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA DJ8ZX UT WOS:000374504600008 ER PT J AU Yuan, R Beyerlein, IJ Zhou, CZ AF Yuan, Rui Beyerlein, Irene J. Zhou, Caizhi TI Statistical dislocation activation from grain boundaries and its role in the plastic anisotropy of nanotwinned copper SO ACTA MATERIALIA LA English DT Article DE Crystal plasticity; Texture; Size effects; Strength; Interface ID ORIENTED NANOSCALE TWINS; STRAIN-RATE SENSITIVITY; CENTERED-CUBIC METALS; NANO-SCALE TWINS; NANOCRYSTALLINE METALS; CRYSTAL PLASTICITY; DEFORMATION MECHANISMS; TENSILE PROPERTIES; TEXTURE EVOLUTION; GROWTH TWINS AB In this work, we explore the microstructural properties that give rise to the plastic anisotropy observed in columnar-grained, nano-twinned Cu. A statistical model for randomly varying source lengths within the grain boundaries of the nanostructure is developed. The model is used to calculate a corresponding critical resolved shear stress for emitting dislocations within a twin lamella on slip systems lying either parallel or inclined from its twin boundary. By incorporating this model into a 3D crystal plasticity finite element model, we can link texture and slip patterns within the twin lamella to anisotropy in the plastic deformation behavior. The model achieves good agreement with flow stress strain evolution and yield data collected over many studies. We show that reducing twin thickness can increase plastic anisotropy as a result of the increase in mean stress to emit dislocations. It is also found that finer twins can lower strain hardening as a consequence of a lower statistical variation in the emission stress. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Yuan, Rui; Zhou, Caizhi] Missouri Univ Sci & Technol, Dept Mat Sci & Engn, Rolla, MO 65409 USA. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zhou, CZ (reprint author), Missouri Univ Sci & Technol, Dept Mat Sci & Engn, Rolla, MO 65409 USA. EM zhouc@mst.edu FU University of Missouri Research Board; MRC at Missouri University of Science and Technology; Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program [LDRD 20140348ER] FX RY and CZ gratefully acknowledge financial support from The University of Missouri Research Board and MRC at Missouri University of Science and Technology. IJB gratefully acknowledges support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) Program through project number LDRD 20140348ER. NR 56 TC 0 Z9 0 U1 15 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 8 EP 18 DI 10.1016/j.actamat.2016.02.064 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400002 ER PT J AU Jiao, ZB Luan, JH Miller, MK Yu, CY Liu, Y Liu, CT AF Jiao, Z. B. Luan, J. H. Miller, M. K. Yu, C. Y. Liu, Y. Liu, C. T. TI Precipitate transformation from NiAl-type to Ni2AlMn-type and its influence on the mechanical properties of high-strength steels SO ACTA MATERIALIA LA English DT Article DE Precipitation; Phase transformation; Precipitation strengthening; Atom probe tomography; Mechanical property ID LOW-CARBON STEEL; FIM-ATOM PROBE; FERRITIC STEELS; FE-CU; INTERMETALLIC COMPOUND; PCT COPPER; AL ALLOYS; MICROSTRUCTURE; METALS; MICROSCOPY AB The precipitate transformation from NiAl-type to Ni2AlMn-type and its influence on the mechanical properties of the Fe-5Ni-1Al-xMn (x = 0, 1, 3, and 5 wt.%) alloys were studied thoroughly through a combination of three-dimensional atom probe tomography (APT), first-principles calculations and mechanical tests. APT reveals the precipitation of NiAl-type nanoparticles in the 0-3Mn alloys and the co-precipitation of fine NiAl-type and coarse Ni2AlMn-type nanoparticles in the 5Mn alloy, in which the Ni2AlMn-type nanoparticles are formed as a result of the coarsening of the NiAl-type ones. The first principles calculations indicate that the Ni2AlMn-type nanoparticles are energetically more favorable than the NiAl-type ones, but their nucleation and growth kinetics are relatively slow, resulting in the initial precipitation of the NiAl-type nanoparticles and the later precipitate transformation from NiAl-type to Ni2AlMn-type. A quantitative analysis of the strengthening mechanism reveals that although the Ni2AlMn-type nanoparticles have a higher strengthening efficiency than the NiAl-type ones, they make a minor contribution to the total strengthening effects due mainly to their small number density. In addition, the Ni2AlMn-type nanoparticles with a composition consistent with that of the Heusler phase are likely to promote the brittle cleavage and intergranular fracture of the 5Mn alloy, resulting in a significant decrease of the alloy ductility. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Jiao, Z. B.; Luan, J. H.; Liu, C. T.] City Univ Hong Kong, Coll Sci & Engn, Dept Mech & Biomed Engn, Ctr Adv Struct Mat, Hong Kong, Hong Kong, Peoples R China. [Miller, M. K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Yu, C. Y.] Shenzhen Univ, Coll Phys Sci & Technol, Shenzhen 518060, Peoples R China. [Liu, Y.] Cent S Univ, Inst Powder Met, Changsha 410083, Peoples R China. RP Liu, CT (reprint author), City Univ Hong Kong, Coll Sci & Engn, Dept Mech & Biomed Engn, Ctr Adv Struct Mat, Hong Kong, Hong Kong, Peoples R China. EM chainliu@cityu.edu.hk FU City University of Hong Kong; General Research Fund from the Research Grant Council, Hong Kong [CityU 11205515] FX This research was supported by the internal funding from City University of Hong Kong (account CityU No. 9380060) and General Research Fund (account No. CityU 11205515) from the Research Grant Council, Hong Kong. Atom probe tomography (M.K.M.) was conducted at the Center for Nanophase Materials Sciences at Oak Ridge National Laboratory (ORNL), which is a DOE Office of Science User Facility located at Oak Ridge, Tennessee, USA. NR 48 TC 1 Z9 1 U1 11 U2 30 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 31 EP 43 DI 10.1016/j.actamat.2016.03.024 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400004 ER PT J AU Wen, J Sun, C Dholabhai, PP Xia, Y Tang, M Chen, D Yang, DY Li, YH Uberuaga, BP Wang, YQ AF Wen, J. Sun, C. Dholabhai, P. P. Xia, Y. Tang, M. Chen, D. Yang, D. Y. Li, Y. H. Uberuaga, B. P. Wang, Y. Q. TI Temperature dependence of the radiation tolerance of nanocrystalline pyrochlores A(2)Ti(2)O(7) (A = Gd, Ho and Lu) SO ACTA MATERIALIA LA English DT Article DE Nanocrystalline; Pyrochlores; Cation antisite defects; Critical amorphization fluence; Radiation damage ID HEAVY-ION IRRADIATION; WASTE FORM; NANOSTRUCTURED MATERIALS; GADOLINIUM ZIRCONATE; GRAIN-BOUNDARIES; COMPLEX OXIDES; NUCLEAR-WASTE; PLUTONIUM; DAMAGE; STABILITY AB A potentially enhanced radiation resistance of nanocrystalline materials, as a consequence of the high density of interfaces and surfaces, has attracted much attention both to understand the fundamental role of these defect sinks and to develop them for high-radiation environments. Here, irradiation response of nanocrystalline A(2)Ti(2)O(7) (A = Gd, Ho and Lu) pyrochlore powders with grain sizes of 20-30 nm was investigated by 1-MeV Kr2+ ion bombardment. In situ transmission electron microscopy (TEM) revealed that the critical amorphization fluence for each nanocrystalline compound at room temperature was greater than that for their coarse-grained counterparts, indicating an enhanced amorphization resistance. The effect of temperature on the irradiation response of one of these compounds, nanocrystalline Lu2Ti2O7, was further examined by performing ion irradiation at an elevated temperature range of 480 -600 K. The critical amorphization temperature (T-c) was found to be noticeably higher in nanocrystalline Lu2Ti2O7 (610 K) than its coarse -grained counterpart (480 K), revealing that nanocrystalline Lu2Ti2O7 is less resistant to amorphization compared to its coarse -grained phase under high temperatures. We interpret these results with the aid of atomistic simulations. Molecular statics calculations find that cation antisite defects are less energetically costly to form near surfaces than in the bulk, suggesting that the nanocrystalline form of these materials is generally less susceptible to amorphization than coarse grained counterparts at low temperatures where defect kinetics are negligible. In contrast, at high temperatures, the annealing efficiency of antisite defects by cation interstitials is significantly reduced due to the sink properties of the surfaces in the nanocrystalline pyrochlore, which contributes to the observed higher amorphization temperature in the nano -grained phase than in coarse -grained counterpart. Together, these results provide new insight into the behavior of nanocrystalline materials under irradiation. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Wen, J.; Xia, Y.; Yang, D. Y.; Li, Y. H.] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Gansu, Peoples R China. [Wen, J.; Sun, C.; Dholabhai, P. P.; Tang, M.; Chen, D.; Uberuaga, B. P.; Wang, Y. Q.] Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. RP Li, YH (reprint author), Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Gansu, Peoples R China.; Uberuaga, BP; Wang, YQ (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM liyuhong@lzu.edu.cn; blas@lanl.gov; yqwang@lanl.gov OI Wang, Yongqiang/0000-0002-2938-5640 FU National Natural Science Foundation of China [11175076, 11475076]; Fundamental Research Funds for the Central Universities of China (Lanzhou University) [lzujbky-2015-bt07]; US Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division [2013LANL8400]; Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000]; DOE Office of Nuclear Energy [DE-ACO2-06CH11357]; UChicago Argonne, LLC; China Scholarship Council; Center for Integrated Nanotechnologies FX This work was partially supported by the National Natural Science Foundation of China (11175076 and 11475076) and the Fundamental Research Funds for the Central Universities of China (Lanzhou University, lzujbky-2015-bt07). The funding for Los Alamos National Laboratory (LANL) staff was provided by the US Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division (2013LANL8400) and the Center for Integrated Nanotechnologies, a DOE user facility jointly operated by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000). The electron microscopy with in situ ion irradiation was accomplished at Argonne National Laboratory at the IVEM-Tandem Facility, a U.S. Department of Energy Facility funded by the DOE Office of Nuclear Energy, operated under Contract No. DE-ACO2-06CH11357 by UChicago Argonne, LLC. We thank IVEM staff members including Dr. Meimei Li, Dr. Mark Kirk, Pete Baldo and Ed Ryan for assistance in the irradiation experiments. Partial support was also provided to J. Wen by the China Scholarship Council, a nonprofit organization affiliated with Ministry of Education of the People's Republic of China. NR 46 TC 1 Z9 1 U1 9 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 175 EP 184 DI 10.1016/j.actamat.2016.03.025 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400018 ER PT J AU Shim, JH Voigt, HJL Wirth, BD AF Shim, Jae-Hyeok Voigt, Hyon-Jee Lee Wirth, Brian D. TI Temperature dependent dislocation bypass mechanism for coherent precipitates in Cu-Co alloys SO ACTA MATERIALIA LA English DT Article DE Precipitation strengthening; Dislocation glide; Critical resolved shear stress; Molecular dynamics simulation; Cu-Co alloy ID EMBEDDED-ATOM-METHOD; COPPER; METALS; COBALT AB Molecular dynamics simulations of dislocation interaction with coherent cobalt precipitates embedded in Cu-Co alloys reveal a temperature dependent bypass mechanism. Below 300 K, the trailing partial dislocation clearly bypasses the coherent, face centered cubic (FCC) cobalt precipitate by Orowan looping, caused by a reversible structural transformation as the leading partial locally converts the precipitate to the lower-energy hexagonal close packed (HCP) structure. The FCC versus HCP energy difference of cobalt is temperature dependent, and the dislocation bypass mechanism becomes pure shear above 300 K. Based on a combination of inertial effects due to phonon drag and this observed bypass mechanism, we develop a temperature dependent critical resolved shear stress (CRSS) model, which is in excellent agreement with long-standing measurements of the CRSS temperature dependence of Cu-Co alloys, and those obtained from MD simulation. The model explains both the CRSS increase at low temperatures and the existence of a peak value around 200 K. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Shim, Jae-Hyeok; Wirth, Brian D.] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37922 USA. [Shim, Jae-Hyeok] Korea Inst Sci & Technol, High Temp Energy Mat Res Ctr, Seoul 02792, South Korea. [Voigt, Hyon-Jee Lee] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Wirth, Brian D.] Oak Ridge Natl Lab, Nucl Sci & Engn Directorate, Oak Ridge, TN 37831 USA. RP Wirth, BD (reprint author), Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37922 USA. EM bdwirth@utk.edu FU NSF [NSF DMR 0244562, NSF DMR 0548259]; U.S. Department of Energy, Office of Fusion Energy Sciences [DOE-DE-SC0006661]; National Research Council of Science and Technology of Korea FX The authors acknowledge many helpful discussions with Professors Ian Robertson (University of Illinois at Urbana-Champaign) and David Rodney (Genie Physique et Mecanique des Materiaux) and financial support from the NSF under contracts NSF DMR 0244562, NSF DMR 0548259, and the U.S. Department of Energy, Office of Fusion Energy Sciences under grant DOE-DE-SC0006661. J.H.S. acknowledges the support from the Convergence Agenda Program (CAP) of the National Research Council of Science and Technology of Korea. NR 25 TC 0 Z9 0 U1 11 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 276 EP 282 DI 10.1016/j.actamat.2016.03.027 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400029 ER PT J AU Dunn, A Dingreville, R Martinez, E Capolungo, L AF Dunn, Aaron Dingreville, Remi Martinez, Enrique Capolungo, Laurent TI Identification of dominant damage accumulation processes at grain boundaries during irradiation in nanocrystalline alpha-Fe: A statistical study SO ACTA MATERIALIA LA English DT Article DE cluster dynamics; Grain boundary; Radiation damage; Sink efficiency ID KINETIC MONTE-CARLO; STOCHASTIC CLUSTER DYNAMICS; PRESSURE-VESSEL STEELS; MICROSTRUCTURAL EVOLUTION; DIFFUSION MECHANISMS; STRUCTURAL-MATERIALS; COMPUTER-SIMULATION; DEFECT PRODUCTION; BUBBLE FORMATION; DOSE DEPENDENCE AB Radiation defect accumulation in metals with high interface to volume ratios, such as nanocrystalline metals, is strongly dependent on the ability of these interfaces to act as unbiased sinks for defects. Multi-scale simulations of damage accumulation in such materials necessarily depend on parameters describing defect behaviors inside grain boundaries, such as migration and binding energies within grain boundaries as well as binding energies of defects to grain boundaries. In general, these behaviors are sensitive to the grain boundary structure, making atomic-scale quantification of such parameters challenging due to the large number of variables in the input space of such a problem. The goal of the present study is to identify which of these parameters most strongly influence defect accumulation and grain boundary sink efficiency in alpha-Fe during Frenkel pair implantation at room temperature and a dose rate of 10(-7) dpa. s(-1). Defect accumulation inside grains and in grain boundaries is simulated using spatially resolved stochastic cluster dynamics (SRSCD). Using this methodology, sensitivity studies investigating vacancy accumulation in grain boundaries, sink efficiency eta of grain boundaries, and vacancy cluster profiles inside grains are performed by varying model input parameters such as defect migration and binding energies inside grain boundaries. Principal component analysis of these model input parameters is then carried out to identify which defect behaviors are strongly correlated with changes in damage accumulation metrics when varying many parameters at once. In both of these analyses, single vacancy and self-interstitial diffusion inside grain boundaries, small vacancy cluster diffusion inside grain boundaries, and the binding energy of vacancies and self-interstitials to grain boundaries are shown to have the greatest impact on defect accumulation. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Dunn, Aaron; Dingreville, Remi] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Dunn, Aaron; Capolungo, Laurent] Georgia Inst Technol, George W Woodruff Sch Mech Engn, UMI 2958, Georgia Tech,CNRS, F-57070 Metz, France. [Martinez, Enrique] Los Alamos Natl Lab, Mat Sci & Technol Div, MST-8, Los Alamos, NM 87545 USA. RP Capolungo, L (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, UMI 2958, Georgia Tech,CNRS, F-57070 Metz, France. EM laurent.capolungo@me.gatech.edu FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; US Department of Energy's Nuclear Energy University Program [DE-NE0000678]; Sandia National Laboratories/Georgia Tech Excellence in Engineering Research Program; Lockheed Martin Corporation FX Supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000.; This work is also supported by the US Department of Energy's Nuclear Energy University Program (DE-NE0000678).; This work is also supported by the Sandia National Laboratories/Georgia Tech Excellence in Engineering Research Program. NR 70 TC 0 Z9 0 U1 5 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 306 EP 323 DI 10.1016/j.actamat.2016.03.026 PG 18 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400032 ER PT J AU Patra, A McDowell, DL AF Patra, Anirban McDowell, David L. TI Crystal plasticity investigation of the microstructural factors influencing dislocation channeling in a model irradiated bcc material SO ACTA MATERIALIA LA English DT Article DE Irradiation; bcc; Dislocation channel; Localization; Crystal plasticity ID AUSTENITIC STAINLESS-STEELS; LOCALIZED DEFORMATION; STRAIN LOCALIZATION; TENSILE PROPERTIES; NEUTRON-IRRADIATION; FLOW LOCALIZATION; MECHANICAL-PROPERTIES; DYNAMICS SIMULATIONS; DEFECT INTERACTIONS; GRAIN-BOUNDARIES AB A continuum crystal plasticity framework is used to study the effect of microstructure and mesoscopic factors on dislocation channeling and flow localization in an irradiated model bcc alloy. Simulated dislocation channeling characteristics are correlated to the dislocation and defect densities in the substructure, local Schmid factor, and stress triaxiality, in terms of their temporal and spatial evolution. A metric is introduced to assess the propensity for localization and is correlated to the grain-level Schmid factor. It is found that localization generally takes place in grains with a local Schmid factor in the range 0.42 or higher. Surface slip step heights are computed at free surfaces and compared to relevant experiments. Published by Elsevier Ltd on behalf of Acta Materialia Inc. C1 [Patra, Anirban] Los Alamos Natl Lab, Mat Sci & Technol Div, MS G755, Los Alamos, NM 87545 USA. [Patra, Anirban; McDowell, David L.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [McDowell, David L.] Georgia Inst Technol, Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. RP Patra, A (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, MS G755, Los Alamos, NM 87545 USA. EM apatra@lanl.gov NR 74 TC 0 Z9 0 U1 12 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD MAY 15 PY 2016 VL 110 BP 364 EP 376 DI 10.1016/j.actamat.2016.03.041 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DK3IN UT WOS:000374810400036 ER PT J AU Herring, SJ Batchelor, S Bieringer, PE Lingard, B Lorenzetti, DM Parker, ST Rodriguez, L Sohn, MD Steinhoff, D Wolski, M AF Herring, Steven J. Batchelor, Simon Bieringer, Paul E. Lingard, Bry Lorenzetti, David M. Parker, Simon T. Rodriguez, Luna Sohn, Michael D. Steinhoff, Dan Wolski, Matthew TI Providing pressure inputs to multizone building models SO BUILDING AND ENVIRONMENT LA English DT Article DE Multizone; Indoor models; Pressure inputs ID HIGHRISE RESIDENTIAL BUILDINGS; WIND-INDUCED PRESSURE; AIR-FLOW; SIMULATION; TRANSPORT; CFD AB A study to assess how the fidelity of wind pressure inputs and indoor model complexity affect the predicted air change rate for a study building is presented. The purpose of the work is to support the development of a combined indoor-outdoor hazard prediction tool, which links the CONTAM multizone building simulation tool with outdoor dispersion models. The study building, representing a large office block of a simple rectangular geometry under natural ventilation, was based on a real building used in the Joint Urban 2003 experiment. A total of 1600 indoor model flow simulations were made, driven by 100 meteorological conditions which provided a wide range of building surface pressures. These pressures were applied at four levels of resolution to four different building configurations with varying numbers of internal zones and indoor and outdoor flow paths. Analysis of the results suggests that surface pressures and flow paths across the envelope should be specified at a resolution consistent with the dimensions of the smallest volume of interest, to ensure that appropriate outputs are obtained. Crown Copyright (C) 2016 Published by Elsevier Ltd. All rights reserved. C1 [Herring, Steven J.; Batchelor, Simon; Lingard, Bry; Parker, Simon T.] Dstl, Salisbury SP4 0JQ, Wilts, England. [Rodriguez, Luna; Steinhoff, Dan] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Wolski, Matthew] Naval Surface Warfare Ctr, Dahlgren, VA 22448 USA. [Lorenzetti, David M.; Sohn, Michael D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Bieringer, Paul E.] Aeris, 1723 Madison Ct, Louisville, CO 80027 USA. RP Herring, SJ (reprint author), Dstl, Salisbury SP4 0JQ, Wilts, England. EM sjherring@dstl.gov.uk FU Defense Threat Reduction Agency; U.S. Department of Energy [DE-AC02- 05CH11231] FX The authors would like to acknowledge the support received from Mr R. Fry of the US Defense Threat Reduction Agency in conducting the work presented. Contributions from Lorenzetti and Sohn were supported in part by the Defense Threat Reduction Agency and performed under U.S. Department of Energy Contract number DE-AC02- 05CH11231. NR 33 TC 0 Z9 0 U1 3 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD MAY 15 PY 2016 VL 101 BP 32 EP 44 DI 10.1016/j.buildenv.2016.02.012 PG 13 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA DJ7AA UT WOS:000374363100004 ER PT J AU Matmon, A Elfassi, S Hidy, A Geller, Y Porat, N AF Matmon, A. Elfassi, S. Hidy, A. Geller, Y. Porat, N. CA ASTER Team TI Controls on aggradation and incision in the NE Negev, Israel, since the middle Pleistocene SO GEOMORPHOLOGY LA English DT Article DE Alluvial terraces; Aggradation; Incision; Negev desert ID DEAD-SEA; PLUVIAL EPISODES; EXPOSURE AGES; DESERT; RATES; EVOLUTION; EROSION; RIFT; LUMINESCENCE; ESCARPMENT AB We investigated the mid-Pleistocene to recent aggradation-incision pattern of two drainage systems (Nahal Peres and Nahal Tahmas) in the hyperarid north eastern Negev desert, southern Israel. Although these drainage systems drain into the tectonically active Dead Sea basin, lake level fluctuations cannot account for the aggradation-incision pattern as bedrock knickpoints disconnect the investigated parts of these drainage systems from base level influence. We applied geomorphic mapping, soil stratigraphy, optically stimulated luminescence (OSL) and costnogenic (in situ Be-10) exposure dating to reconstruct cycles of aggradation and incision of alluvial terraces and to study their temporal association with regional periods of humidity and aridity and global glacial interglacial cycles. The spatial and temporal relationships between the alluvial units suggest changes in the drainage system behavior since the middle Pleistocene, and show a pattern in which prolonged periods of sediment aggradation alternated with short periods of rapid and intense degradation through erosion and incision into sediment and bedrock. We obtain ages for several Pleistocene-Holocene periods of incision:similar to 1.1 Ma,similar to 300 ka, similar to 120 ka,similar to 20 ka,similar to 12 ka and similar to 2 ka. Although broadly synchronous, the Nahal Peres and Nahal Tahmas systems exhibit temporal differences in aggradation and incision. Hyperarid conditions have persisted in the region at least since the middle Pleistocene, as evidenced by gypsicsalic soils that ubiquitously cap the investigated alluvial terraces. This observation is consistent with other observations throughout the Negev indicating prolonged aridity. Thus, alternation between sediment aggradation and degradation cannot be correlated in a simple and straightforward way to climatic changes. We explain the temporal differences in aggradation and incision between Nahal Peres and Nahal Tahmas as resulting from the differences in stream gradient, basin hypsometry, and drainage basin area (which influences the amount of water passing through-the system). Regardless of humidity source (tropical plumes, Red Sea trough or Mediterranean fronts) and the frequency and intensity of rainfall in the region, our study shows that: 1) unlike other climatic proxies, such as speleothems, the evolution of alluvial terraces, which involves many stages (sediment generation, transport, deposition, and subsequent incision), results in a significant time gap between the actual ages of terraces and the timing of external triggers such as climatic fluctuations, and 2) such time-gaps may vary, even within nearby drainage systems, due to differences in drainage systems specific characteristics, and thus result in asynchronicity (or at least poor synchronicity) of alluvial terrace deposition and incision. (C) 2016 Elsevier B.V. All rights reserved. C1 [Matmon, A.; Elfassi, S.; Hidy, A.; Geller, Y.] Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. [Hidy, A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. [Porat, N.] Geol Survey Israel, 30 Malkhe Yisrael St, IL-95501 Jerusalem, Israel. [ASTER Team] Aix Marseille Univ, CNRS, UMR CNRS 6635, CEREGE, BP 80, F-13545 Aix En Provence 4, France. RP Matmon, A (reprint author), Hebrew Univ Jerusalem, Inst Earth Sci, IL-91904 Jerusalem, Israel. OI Bourles, Didier/0000-0001-5991-6126 NR 50 TC 0 Z9 0 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-555X EI 1872-695X J9 GEOMORPHOLOGY JI Geomorphology PD MAY 15 PY 2016 VL 261 BP 132 EP 146 DI 10.1016/j.geomorph.2016.02.020 PG 15 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA DK0TE UT WOS:000374624300010 ER PT J AU Hopf, J Kerisit, SN Angeli, F Charpentier, T Icenhower, JP McGrail, BP Windisch, CF Burton, SD Pierce, EM AF Hopf, J. Kerisit, S. N. Angeli, F. Charpentier, T. Icenhower, J. P. McGrail, B. P. Windisch, C. F. Burton, S. D. Pierce, E. M. TI Glass-water interaction: Effect of high-valence cations on glass structure and chemical durability SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID MONTE-CARLO SIMULATIONS; LIME BOROSILICATE GLASSES; NUCLEAR-WASTE GLASSES; RESOLUTION SI-29 NMR; LONG-TERM BEHAVIOR; X-RAY-ABSORPTION; DISSOLUTION KINETICS; SILICATE-GLASSES; ALUMINOBOROSILICATE GLASSES; EQUILIBRIUM CONDITIONS AB Borosilicate glass is a durable solid, but it dissolves when in contact with aqueous fluids. The dissolution mechanism, which involves a variety of sequential reactions that occur at the solid-fluid interface, has important implications for the corrosion resistance of industrial and nuclear waste glasses. In this study, spectroscopic measurements, dissolution experiments, and Monte Carlo simulations were performed to investigate the effect of high-valence cations (HVC) on the mechanisms of glass dissolution under dilute and near-saturated conditions. Raman and NMR spectroscopy were used to determine the structural changes that occur in glass, specifically network formers (e.g., Al, Si, and B), with the addition of the HVC element hafnium in the Na2O-Al2O3-B2O3-HfO2-SiO2 system (e.g., Na/[Al + B] = 1.0 and HfO2/SiO2 from 0.0 to 0.42). Spectroscopic measurements revealed that increasing hafnium content decreases N-4 (tetrahedral boron/total boron) and increases the amount of Si-O-Hf moieties in the glass. Results from flow-through experiments conducted under dilute and near-saturated conditions show a decrease of approximately 100x or more in the dissolution rate over the series from 0 to 20 mol% HfO2. Comparing the average steady-state rates obtained under dilute conditions to the rates obtained for near-saturated conditions reveals a divergence in the magnitude between the average steady state rates measured in these different conditions. The reason for this divergence was investigated more thoroughly using Monte Carlo simulations. Simulations indicate that the divergence in glass dissolution behavior under dilute and near-saturated conditions result from the stronger binding of Si sites that deposit on the surface from the influent when Hf is present in the glass. As a result, the residence time at the glass surface of these newly-formed Si sites is longer in the presence of Hf, which increases the density of anchor sites from which altered layers with higher Si densities can form. These results illustrate the importance of understanding solid-water/solid-fluid interactions by linking macroscopic reaction kinetics to nanometer scale interfacial processes. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Hopf, J.; Pierce, E. M.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN USA. [Kerisit, S. N.; Windisch, C. F.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Angeli, F.] CEA, DEN, Lab Etud Comportement Long Terme, Lyon, France. [Charpentier, T.] Univ Paris Saclay, CEA Saclay, CNRS, NIMBE,CEA, Paris, France. [Icenhower, J. P.] Sandia Natl Labs, Carlsbad Programs Grp, Livermore, CA 94550 USA. [McGrail, B. P.] Pacific NW Natl Lab, Energy Proc & Mat Div, Richland, WA 99352 USA. [Burton, S. D.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Pierce, EM (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN USA. EM pierceem@ornl.gov RI ANGELI, Frederic /B-7574-2011; Charpentier, Thibault/A-3557-2010; Pierce, Eric/G-1615-2011 OI Charpentier, Thibault/0000-0002-3034-1389; Pierce, Eric/0000-0002-4951-1931 FU Oak Ridge National Laboratory (ORNL) Laboratory Directed Research and Development Program; U.S. Department of Energy's (DOE) Environmental Management (EM) Tank Waste Management program; DOEs Office of Science and Technology under the Environmental Management Science Program [42400]; DOE EMs Office of River Protection; Washington River Protection Solutions; Areva; CEA; DOE's Office of Biological and Environmental Research; US DOE [DE-AC05-00OR22725, DE-AC05-76RL0-1830] FX This research was supported by the Oak Ridge National Laboratory (ORNL) Laboratory Directed Research and Development Program, U.S. Department of Energy's (DOE) Environmental Management (EM) Tank Waste Management program, DOEs Office of Science and Technology under the Environmental Management Science Program (proposal number 42400), and DOE EMs Office of River Protection, Immobilization of Low-Activity Waste Program funded through Washington River Protection Solutions. T. Charpentier and F. Angeli would like to acknowledge the financial support of Areva and CEA. The authors would like to thank David K. Shuh for his helpful discussions on the structure of hafnium in peralkaline glasses which was based on unpublished XAFS measurements. A portion of this research was performed in part with the Nuclear Magnetic Resonance Spectrometers and the Molecular Science Computing facilities in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. ORNL is operated by UT-Battelle, LLC and PNNL is operated by Battelle for the US DOE under Contract No.'s DE-AC05-00OR22725 and DE-AC05-76RL0-1830, respectively. NR 96 TC 2 Z9 2 U1 14 U2 41 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2016 VL 181 BP 54 EP 71 DI 10.1016/j.gca.2016.02.023 PG 18 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DI6OE UT WOS:000373618200004 ER PT J AU Zachara, JM Moran, JJ Resch, CT Lindemann, SR Felmy, AR Bowden, ME Cory, AB Fredrickson, JK AF Zachara, John M. Moran, James J. Resch, Charles T. Lindemann, Stephen R. Felmy, Andrew R. Bowden, Mark E. Cory, Alexandra B. Fredrickson, James K. TI Geo- and biogeochemical processes in a heliothermal hypersaline lake SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID PHOTOTROPHIC SULFUR BACTERIA; MINERAL SOLUBILITIES; MEROMICTIC LAKE; NA-K-MG-CA-H-CL-SO4-OH-HCO3-CO3-CO2-H2O SYSTEM; MICROBIAL COMMUNITIES; LOW-TEMPERATURES; GLYCINE BETAINE; NATURAL-WATERS; MAHONEY LAKE; MONO LAKE AB Water chemical variations were investigated over three annual hydrologic cycles in hypersaline, heliothermal, meromictic Hot Lake in north-central Washington State, USA. The lake contains diverse biota with dramatic zonation related to salinity and redox state. Water samples were collected at 10-cm depth intervals through the shallow lake (2.4 m) during 2012-2014, with comprehensive monitoring performed in 2013. Inorganic salt species, dissolved carbon forms (DOC, DIC), oxygen, sulfide, and methane were analyzed in lake water samples. Depth sonde measurements of pH and temperature were also performed to track their seasonal variations. A bathymetric survey of the lake was conducted to enable lake water volume and solute inventory calculations. Sediment cores were collected at low water and analyzed by X-ray diffraction to investigate sediment mineralogy. The primary dissolved salt in Hot Lake water was Mg2+-SO42- whereas sediments were dominated by gypsum (CaSO4 center dot 2H(2)O). Lake water concentrations increased with depth, reaching saturation with epsomite (MgSO4 center dot 7H(2)O) that was exposed at lake bottom. At maximum volume in spring, Hot Lake exhibited a relatively dilute mixolimnion; a lower saline metalimnion with stratified oxygenic and anoxygenic photosynthetic microbiological communities; and a stable, hypersaline monimolimnion, separated from above layers by a chemocline, containing high levels of sulfide and methane. The thickness of the mixolimnion regulates a heliothermal effect that creates temperatures in excess of 60 degrees C in the underlying metalimnion and monimolimnion. The mixolimnion was dynamic in volume and actively mixed. It displayed large pH variations, in-situ calcium carbonate precipitation, and large evaporative volume losses. The depletion of this layer by fall allowed deeper mixing into the metalimnion, more rapid heat exchange, and lower winter lake temperatures. Solubility calculations indicate seasonal biogenic and thermogenic aragonite precipitation in the mixolimnion and metalimnion, but the absence of calcareous sediments at depth suggests dissolution and recycling during winter months. Dissolved carbon concentrations [dissolved organic carbon (DOC) and dissolved inorganic carbon (DIC)] increased with depth, reaching similar to 0.04 mol/L at the metalimnion-monimolimnion boundary. DIC concentrations were seasonally variable in the mixolimnion and metalimnion, and were influenced by calcium carbonate precipitation. DOC concentrations mimicked those of conservative salts (e.g., Na+-Cl-) in the mixolimnion and metalimnion, but decreased in the monimolimnion where mass loss by anaerobic microbial processes is implied. Biogenic reduced solutes originating in monimolimnion (H2S and CH4) were biologically oxidized in the metalimnion as they were not observed in more shallow lake waters. Multi-year solute inventory calculations indicated that Hot Lake is a stable, albeit seasonally and annually dynamic feature, with inorganic solutes cycled between lake waters and sediments depending on annual recharge, temperature, and lake water dilution state. With its extreme geochemical and thermal regime, Hot Lake functions as analog of early earth and extraterrestrial life environments. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Zachara, John M.; Moran, James J.; Resch, Charles T.; Lindemann, Stephen R.; Felmy, Andrew R.; Bowden, Mark E.; Cory, Alexandra B.; Fredrickson, James K.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Felmy, Andrew R.] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. RP Zachara, JM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.zachara@pnnl.gov RI Lindemann, Steve/H-6088-2016; OI Lindemann, Steve/0000-0002-3788-5389; Moran, James/0000-0001-9081-9017 FU U.S. Department of Energy (DOE), Office of Biological and Environmental Research (BER) FX This research was supported by the U.S. Department of Energy (DOE), Office of Biological and Environmental Research (BER), as part of BER's Genomic Science Program (GSP). This contribution originates from the GSP Foundational Scientific Focus Area (FSFA) at the Pacific Northwest National Laboratory (PNNL). We thank Dr. Jim McKinley and Micah Miller for their assistance in electron microprobe analyses and interpretation, and Dr. Allan Konopka and three anonymous reviewers for their thorough review of the manuscript. The authors further acknowledge the U.S. Bureau of Land Management, Wenatchee Field Office, for authorizing a research permit and providing access to the Hot Lake Research Natural Area. PNNL is operated for the DOE by Battelle. NR 84 TC 1 Z9 1 U1 12 U2 35 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAY 15 PY 2016 VL 181 BP 144 EP 163 DI 10.1016/j.gca.2016.02.001 PG 20 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DI6OE UT WOS:000373618200009 ER PT J AU Reckinger, SJ Reckingera, J Vasilyev, OV AF Reckinger, Scott J. Livescu, Daniel Vasilyev, Oleg V. TI Comprehensive numerical methodology for direct numerical simulations of compressible Rayleigh-Taylor instability SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Rayleigh-Taylor instability; Compressible flow; Direct numerical simulations; Wavelet-based adaptive grid; Consistent initialization; Boundary conditions ID WAVELET-COLLOCATION METHOD; PARTIAL-DIFFERENTIAL EQUATIONS; BOUNDARY-CONDITIONS; SINGLE-MODE; 2ND-GENERATION WAVELETS; FLUID-DYNAMICS; FLOWS; ALGORITHM; PENALIZATION; DIFFUSION AB An investigation of compressible Rayleigh-Taylor instability (RTI) using Direct Numerical Simulations (DNS) requires efficient numerical methods, advanced boundary conditions, and consistent initialization in order to capture the wide range of scales and vortex dynamics present in the system, while reducing the computational impact associated with acoustic wave generation and the subsequent interaction with the flow. An advanced computational framework is presented that handles the challenges introduced by considering the compressive nature of RTI systems, which include sharp interfacial density gradients on strongly stratified background states, acoustic wave generation and removal at computational boundaries, and stratification dependent vorticity production. The foundation of the numerical methodology described here is the wavelet-based grid adaptivity of the Parallel Adaptive Wavelet Collocation Method (PAWCM) that maintains symmetry in single-mode RTI systems to extreme late-times. PAWCM is combined with a consistent initialization, which reduces the generation of acoustic disturbances, and effective boundary treatments, which prevent acoustic reflections. A dynamic time integration scheme that can handle highly nonlinear and potentially stiff systems, such as compressible RTI, completes the computational framework. The numerical methodology is used to simulate two-dimensional single-mode RTI to extreme late-times for a wide range of flow compressibility and variable density effects. The results show that flow compressibility acts to reduce the growth of RTI for low Atwood numbers, as predicted from linear stability analysis. (C) 2016 Elsevier Inc. All rights reserved. C1 [Reckinger, Scott J.; Vasilyev, Oleg V.] Univ Colorado, Dept Mech Engn, 427 UCB, Boulder, CO 80309 USA. [Reckinger, Scott J.] Montana State Univ, Civil Engn Dept, Bozeman, MT 59717 USA. [Livescu, Daniel] Los Alamos Natl Lab, CCS Computat Phys & Methods 2, POB 1663, Los Alamos, NM 87545 USA. RP Reckinger, SJ (reprint author), Univ Colorado, Dept Mech Engn, 427 UCB, Boulder, CO 80309 USA.; Reckinger, SJ (reprint author), Montana State Univ, Civil Engn Dept, Bozeman, MT 59717 USA. EM scott.reckinger@montana.edu; livescu@lanl.gov; oleg.vasilyev@colorado.edu RI Vasilyev, Oleg/H-5597-2016; OI Vasilyev, Oleg/0000-0003-0294-6097; Livescu, Daniel/0000-0003-2367-1547 FU LDRD program at Los Alamos National Laboratory [20070195ER, 20090058DR]; Los Alamos National Laboratory [57206-001-07] FX This work was made possible by funding from the LDRD program at Los Alamos National Laboratory through project numbers 20070195ER and 20090058DR. OVV and SJR were supported by Los Alamos National Laboratory, under subcontract No 57206-001-07. This support is gratefully acknowledged. Computational resources were provided by the LANL Institutional Computing (IC) Program. NR 50 TC 1 Z9 1 U1 1 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2016 VL 313 BP 181 EP 208 DI 10.1016/j.jcp.2015.11.002 PG 28 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DI6NG UT WOS:000373615500010 ER PT J AU Turinsky, PJ Kothe, DB AF Turinsky, Paul J. Kothe, Douglas B. TI Modeling and simulation challenges pursued by the Consortium for Advanced Simulation of Light Water Reactors (CASL) SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Modeling; Simulation; Core simulator; Multiphysics; Nuclear energy ID CODE AB The Consortium for the Advanced Simulation of Light Water Reactors (CASL), the first Energy Innovation Hub of the Department of Energy, was established in 2010 with the goal of providing modeling and simulation (M&S) capabilities that support and accelerate the improvement of nuclear energy's economic competitiveness and the reduction of spent nuclear fuel volume per unit energy, and all while assuring nuclear safety. To accomplish this requires advances in M&S capabilities in radiation transport, thermal-hydraulics, fuel performance and corrosion chemistry. To focus CASL's R&D, industry challenge problems have been defined, which equate with long standing issues of the nuclear power industry that M&S can assist in addressing. To date CASL has developed a multi-physics "core simulator" based upon pin-resolved radiation transport and subchannel (within fuel assembly) thermal-hydraulics, capitalizing on the capabilities of high performance computing. CASL's fuel performance M&S capability can also be optionally integrated into the core simulator, yielding a coupled multi-physics capability with untapped predictive potential. Material models have been developed to enhance predictive capabilities of fuel clad creep and growth, along with deeper understanding of zirconium alloy clad oxidation and hydrogen pickup. Understanding of corrosion chemistry (e.g., CRUD formation) has evolved at all scales: micro, meso and macro. CFD R&D has focused on improvement in closure models for subcooled boiling and bubbly flow, and the formulation of robust numerical solution algorithms. For multiphysics integration, several iterative acceleration methods have been assessed, illuminating areas where further research is needed. Finally, uncertainty quantification and data assimilation techniques, based upon sampling approaches, have been made more feasible for practicing nuclear engineers via R&D on dimensional reduction and biased sampling. Industry adoption of CASL's evolving M&S capabilities, which is in progress, will assist in addressing long-standing and future operational and safety challenges of the nuclear industry. (C) 2016 Elsevier Inc. All rights reserved. C1 [Turinsky, Paul J.] N Carolina State Univ, POB 7926, Raleigh, NC 27695 USA. [Kothe, Douglas B.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RP Turinsky, PJ (reprint author), N Carolina State Univ, POB 7926, Raleigh, NC 27695 USA. EM turinsky@ncsu.edu; kothe@ornl.gov FU Office of Nuclear Energy of the U.S. Department of Energy; Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modelingand Simulation of Nuclear Reactors under U.S. Department of Energy [DE-AC05-00OR22725] FX Members of the CASL team, whom the authors are most appreciative of, performed the work reported upon in this manuscript. The authors acknowledge the strong support and management provided by the Office of Nuclear Energy of the U.S. Department of Energy. This research was partially supported by the Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modelingand Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-00OR22725. NR 23 TC 1 Z9 1 U1 4 U2 17 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2016 VL 313 BP 367 EP 376 DI 10.1016/j.jcp.2016.02.043 PG 10 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DI6NG UT WOS:000373615500019 ER PT J AU Motheau, E Abraham, J AF Motheau, E. Abraham, J. TI A high-order numerical algorithm for DNS of low-Mach-number reactive flows with detailed chemistry and quasi-spectral accuracy SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE DNS; Low-Mach-number; Detailed chemistry; Turbulent reacting flow; High-order methods; Spectral accuracy; Operator splitting ID PRESSURE-CORRECTION METHOD; FINITE-DIFFERENCE SCHEMES; LARGE-EDDY SIMULATIONS; INCOMPRESSIBLE FLOWS; BOUNDARY-CONDITION; COMPRESSIBLE FLOW; STIFF CHEMISTRY; HEAT RELEASE; COMBUSTION; EQUATIONS AB A novel and efficient algorithm is presented in this paper to deal with DNS of turbulent reacting flows under the low-Mach-number assumption, with detailed chemistry and a quasi-spectral accuracy. The temporal integration of the equations relies on an operatingsplit strategy, where chemical reactions are solved implicitly with a stiff solver and the convection-diffusion operators are solved with a Runge-Kutta-Chebyshev method. The spatial discretisation is performed with high-order compact schemes, and a FFT based constant-coefficient spectral solver is employed to solve a variable-coefficient Poisson equation. The numerical implementation takes advantage of the 2DECOMP&FFT libraries developed by [1], which are based on a pencil decomposition method of the domain and are proven to be computationally very efficient. An enhanced pressure-correction method is proposed to speed up the achievement of machine precision accuracy. It is demonstrated that a second-order accuracy is reached in time, while the spatial accuracy ranges from fourth-order to sixth-order depending on the set of imposed boundary conditions. The software developed to implement the present algorithm is called HOLOMAC, and its numerical efficiency opens the way to deal with DNS of reacting flows to understand complex turbulent and chemical phenomena in flames. (C) 2016 Elsevier Inc. All rights reserved. C1 [Motheau, E.; Abraham, J.] Univ Adelaide, Sch Mech Engn, Adelaide, SA 5005, Australia. [Abraham, J.] Purdue Univ, Sch Mech Engn, 585 Purdue Mall, W Lafayette, IN 47907 USA. [Motheau, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, MS 50A-1148,1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Motheau, E (reprint author), Univ Adelaide, Sch Mech Engn, Adelaide, SA 5005, Australia.; Motheau, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, MS 50A-1148,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM emotheau@lbl.gov OI Motheau, Emmanuel/0000-0003-1968-1611 NR 58 TC 1 Z9 1 U1 1 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2016 VL 313 BP 430 EP 454 DI 10.1016/j.jcp.2016.02.059 PG 25 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DI6NG UT WOS:000373615500023 ER PT J AU D'Elia, M Ridzal, D Peterson, KJ Bochev, P Shashkov, M AF D'Elia, Marta Ridzal, Denis Peterson, Kara J. Bochev, Pavel Shashkov, Mikhail TI Optimization-based mesh correction with volume and convexity constraints SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Lagrangian motion; Incremental remap; Semi-Lagrangian transport; Departure volume correction; Volume fraction; Passive tracer transport ID GEOMETRIC CONSERVATION LAW; TRANSPORT PROBLEMS; FLOW COMPUTATIONS; SQP METHOD; ADVECTION; SCHEMES; ALGORITHMS; EFFICIENT AB We consider the problem of finding a mesh such that 1) it is the closest, with respect to a suitable metric, to a given source mesh having the same connectivity, and 2) the volumes of its cells match a set of prescribed positive values that are not necessarily equal to the cell volumes in the source mesh. This volume correction problem arises in important simulation contexts, such as satisfying a discrete geometric conservation law and solving transport equations by incremental remapping or similar semi-Lagrangian transport schemes. In this paper we formulate volume correction as a constrained optimization problem in which the distance to the source mesh defines an optimization objective, while the prescribed cell volumes, mesh validity and/or cell convexity specify the constraints. We solve this problem numerically using a sequential quadratic programming (SQP) method whose performance scales with the mesh size. To achieve scalable performance we develop a specialized multigrid-based preconditioner for optimality systems that arise in the application of the SQP method to the volume correction problem. Numerical examples illustrate the importance of volume correction, and showcase the accuracy, robustness and scalability of our approach. Published by Elsevier Inc. C1 [D'Elia, Marta; Ridzal, Denis; Peterson, Kara J.; Bochev, Pavel] Sandia Natl Labs, Ctr Comp Res, MS-1320, Albuquerque, NM 87185 USA. [Shashkov, Mikhail] Los Alamos Natl Lab, X Computat Phys, XCP 4, Los Alamos, NM 87545 USA. RP D'Elia, M (reprint author), Sandia Natl Labs, Ctr Comp Res, MS-1320, Albuquerque, NM 87185 USA. EM mdelia@sandia.gov; dridzal@sandia.gov; kjpeter@sandia.gov; pbbochev@sandia.gov; shashkov@lanl.gov FU US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research [14-017511]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program FX All the authors acknowledge the support of the US Department of Energy Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research 14-017511. The work of M. Shashkov was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. M. Shashkov also gratefully acknowledges the partial support of the US Department of Energy National Nuclear Security Administration Advanced Simulation and Computing (ASC) Program. NR 31 TC 0 Z9 0 U1 2 U2 2 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2016 VL 313 BP 455 EP 477 DI 10.1016/j.jcp.2016.02.050 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DI6NG UT WOS:000373615500024 ER PT J AU Starinshak, DP Owen, JM AF Starinshak, D. P. Owen, J. M. TI A multimaterial extension to subzonal reconstruction SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Remapping; ALE methods ID LAGRANGIAN-EULERIAN METHODS; TOTAL-ENERGY; ARBITRARY; REMAP; HYDRODYNAMICS AB We present a new algorithm for reconstructing material-dependent subzonal information based on staggered primary/dual-mesh remapping of material-dependent conserved quantities. The algorithm is appropriate in the context of geometric, intersection-based overlay remapping methods, with specific application to staggered, total energy conserving, multi-material Lagrangian hydrodynamics schemes that discretize material masses on subzonal mesh elements. Our new approach avoids direct remapping of material-dependent subzonal variables; instead, the spatial profile of each variable is reconstructed using a combination of material-dependent zone (primary mesh) information, material-independent node (dual mesh) information, and discrete interface-reconstructed material concentration information. Conservation and convergence properties of the new algorithm are established through several challenging multi-material remapping and hydrodynamics tests. (C) 2015 Published by Elsevier Inc. C1 [Starinshak, D. P.; Owen, J. M.] Lawrence Livermore Natl Lab, AX Div, M-S L-38,POB 808, Livermore, CA 94550 USA. RP Owen, JM (reprint author), Lawrence Livermore Natl Lab, AX Div, M-S L-38,POB 808, Livermore, CA 94550 USA. EM starinshak1@llnl.gov; mikeowen@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 17 TC 2 Z9 2 U1 2 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAY 15 PY 2016 VL 313 BP 594 EP 616 DI 10.1016/j.jcp.2015.11.056 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DI6NG UT WOS:000373615500030 ER PT J AU Kim, K Bolotnikov, AE Camarda, GS Hossain, A James, RB AF Kim, K. Bolotnikov, A. E. Camarda, G. S. Hossain, A. James, R. B. TI Overcoming Zn segregation in CdZnTe with the temperature gradient annealing SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Segregation; Bridgman technique; Cadmium compounds; Semiconducting II-VI materials ID BRIDGMAN-GROWN CDZNTE; DETECTOR APPLICATIONS; CADMIUM TELLURIDE; ZINC SEGREGATION; CDMNTE DETECTORS; CRYSTAL-GROWTH; LARGE-VOLUME; PERFORMANCE; CD1-XZNXTE; DIFFUSION AB The availability of large volume crystals with the same energy gap in melt-grown CdZnTe (CZT) is restricted due to the Zn segregation in CdTe hosts. We observed the migration of Zn in the solid phase along the positive temperature gradient direction both in situ and post-growth temperature gradient annealing (TGA) of CZT. Diffusivity of Zn obtained from the in situ TGA was approximately 10-5 cm2/s order and completely different mechanism with that of post-growth. The CZT ingots obtained through in situ TGA have uniform Zn and resistivity of 10(10) S2 cm orders. The CZT detectors fabricated from in situ TGA applied ingots exhibit 10% of energy resolution for 59.5 keV peak of Am-241. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kim, K.] Korea Univ, Dept Radiol Sci, Seoul 136713, South Korea. [Bolotnikov, A. E.; Camarda, G. S.; Hossain, A.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Kim, K (reprint author), Korea Univ, Dept Radiol Sci, Seoul 136713, South Korea. EM khkim1@korea.ac.kr FU National Research Foundation of Korea (NRF) Grant - Korea government (MSIP) [NRF-2015M2B2A9032788, NRF-2015M2A2A4A01045094]; U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development, DNN RD FX This work was supported by the National Research Foundation of Korea (NRF) Grant funded by the Korea government (MSIP) (NRF-2015M2B2A9032788 and NRF-2015M2A2A4A01045094) and the U.S. Department of Energy Office of Defense Nuclear Nonproliferation Research and Development, DNN R&D. NR 17 TC 0 Z9 0 U1 8 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD MAY 15 PY 2016 VL 442 BP 98 EP 101 DI 10.1016/j.jcrysgro.2016.02.038 PG 4 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA DI7KC UT WOS:000373677300015 ER PT J AU Wegner, S Heiger-Bernays, W Dix, D AF Wegner, Susanna Heiger-Bernays, Wendy Dix, David TI Spanning regulatory silos in the US EPA's Endocrine Disruptor Screening Program Letter to the Editor re: Evans et al. "Should the scope of human mixture risk assessment span legislative and regulatory silos for chemicals?" SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Letter DE Cumulative risk; High Throughput Screening; Endocrine Disruptor Screening Program ID ESTROGEN-RECEPTOR; MODEL C1 [Wegner, Susanna] ORISE, Oak Ridge, TN USA. [Heiger-Bernays, Wendy] US EPA, AAAS, Washington, DC 20460 USA. [Dix, David] US EPA, Off Sci Coordinat & Policy, Off Chem Safety & Pollut Prevent, Washington, DC 20460 USA. RP Dix, D (reprint author), US EPA, Off Sci Coordinat & Policy, Off Chem Safety & Pollut Prevent, Washington, DC 20460 USA. EM wegner.susanna@epa.gov; dix.david@epa.gov NR 9 TC 0 Z9 0 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD MAY 15 PY 2016 VL 553 BP 671 EP 672 DI 10.1016/j.scitotenv.2016.02.192 PG 2 WC Environmental Sciences SC Environmental Sciences & Ecology GA DI0XN UT WOS:000373220700068 PM 26972864 ER PT J AU Ortiz, CM Paulsen, VI AF Ortiz, Carlos M. Paulsen, Vern I. TI Quantum graph homomorphisms via operator systems SO LINEAR ALGEBRA AND ITS APPLICATIONS LA English DT Article DE Graph homomorphisms; Operator systems; Non-locality; Entangled games AB We explore the concept of a graph homomorphism through the lens of C*-algebras and operator systems. We start by studying the various notions of a quantum graph homomorphism and examine how they are related to each other. We then define and study a 0*-algebra that encodes all the information about these homomorphisms and establish a connection between computational complexity and the representation of these algebras. We use this 0*-algebra to define a new quantum chromatic number and establish some basic properties of this number. We then suggest a way of studying these quantum graph homomorphisms using certain completely positive maps and describe their structure. Finally, we use these completely positive maps to define the notion of a "quantum" core of a graph. Published by Elsevier Inc. C1 [Ortiz, Carlos M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Paulsen, Vern I.] Univ Waterloo, IQC, Waterloo, ON N2L 3G1, Canada. [Paulsen, Vern I.] Univ Waterloo, Dept Pure Math, Waterloo, ON N2L 3G1, Canada. RP Ortiz, CM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM carlos.ortiz@pnnl.gov; vpaulsen@uwaterloo.ca FU National Science Foundation [DMS-1101231] FX The authors wish to thank S. Severini and D. Stahlke for several valuable comments that led to improvements in the paper. This research was supported in part by National Science Foundation grant DMS-1101231. NR 18 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0024-3795 EI 1873-1856 J9 LINEAR ALGEBRA APPL JI Linear Alg. Appl. PD MAY 15 PY 2016 VL 497 BP 23 EP 43 DI 10.1016/j.laa.2016.02.019 PG 21 WC Mathematics, Applied; Mathematics SC Mathematics GA DH4LT UT WOS:000372758200002 ER PT J AU Kim, J Kyeong, JS Ham, MH Minor, AM Kim, DH Park, ES AF Kim, Jinwoo Kyeong, Joon Seok Ham, Moon-Ho Minor, Andrew M. Kim, Do Hyang Park, Eun Soo TI Development of Mo-Ni-Si-B metallic glass with high thermal stability and H versus E ratios SO MATERIALS & DESIGN LA English DT Article DE Molybdenum; Metallic glass; Glass-forming ability; H versus E ratio; Wear resistance ID FORMING ABILITY; AMORPHOUS-ALLOYS; MECHANICAL-PROPERTIES; SUPERCOOLED LIQUID; ELASTIC-MODULUS; THIN-FILMS; HARDNESS; BEHAVIOR; POWDERS; NANOINDENTATION AB We report a novel Mo-Ni-Si-B metallic glass which can be solidified into fully amorphous state by melt-spinning process, with high crystallization onset temperature of over 1100 K, extremely high Vickers hardness of 27.5 +/- 2.2 GPa and relatively low Young's modulus of 364.3 +/- 6.6 GPa. The dense cluster-packing model suggests that the addition of boron up to 10 at.% can occupy vacant cluster-interstices of (Mo, Ni)-Si cluster arrays, which results in a more efficiently dense-packed cluster structure, destabilizes the formation of nanocrystalline phases, and systematically increases the glass-forming ability (GFA) in Mo-Ni-Si-B alloys, The GFA parameters that do not directly rely on T-g, such as Delta T and epsilon parameter, show greater reliability to evaluate GFA for Mo-Ni-Si-B metallic glass exhibiting no clear T-g. The H/E and H-2/(2E) ratios of the newly developed Mo-Ni-Si-B metallic glass, which reflect wear resistance and resilience, exhibit the highest values among various hard ceramic materials as well as metallic glass-forming alloys developed up to now. These advantages of Mo-Ni-Si-B metallic glass can be used more widely to forma high temperature wear-resistant coating layer on various substrates. Furthermore, the same idea might be used to form a metallic glass-nitride nanocomposite coating layer by reactive deposition in N-2 ambient, with highly lubricative properly and high wear-resistance, especially at high temperature. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Kim, Jinwoo; Park, Eun Soo] Seoul Natl Univ, Dept Mat Sci & Engn, Res Inst Adv Mat, Seoul 08826, South Korea. [Kyeong, Joon Seok] Hyundai Mobis, R&D Div, Mat Res Team, Yongin 16891, Gyunggi Do, South Korea. [Ham, Moon-Ho] Gwangju Inst Sci & Technol, Sch Mat Sci & Engn, Gwangju 61005, South Korea. [Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Kim, Do Hyang] Yonsei Univ, Dept Mat Sci & Engn, Seoul 03722, South Korea. RP Park, ES (reprint author), Seoul Natl Univ, Dept Mat Sci & Engn, Res Inst Adv Mat, Seoul 08826, South Korea. EM espark@snu.ac.kr RI Park, Eun Soo/A-4443-2008; OI Kim, Jinwoo/0000-0002-5962-7452 FU National Research Foundation of Korea (NRF) - Korean Government (Ministry of Science, ICT and Future Planning) [2013M2A8A1042253]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Research Foundation of Korea (NRF) grant funded by the Korean Government (Ministry of Science, ICT and Future Planning) (No. 2013M2A8A1042253). The transmission electron microscopy experiments were supported by a user project at the National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Laboratory, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 57 TC 1 Z9 1 U1 7 U2 39 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0261-3069 EI 1873-4197 J9 MATER DESIGN JI Mater. Des. PD MAY 15 PY 2016 VL 98 BP 31 EP 40 DI 10.1016/j.matdes.2016.02.090 PG 10 WC Materials Science, Multidisciplinary SC Materials Science GA DI1RK UT WOS:000373273000004 ER PT J AU Zhang, GM Zhou, ZJ Mo, K Miao, YB Li, SF Liu, X Wang, M Park, JS Almer, J Stubbins, JF AF Zhang, Guangming Zhou, Zhangjian Mo, Kun Miao, Yinbin Li, Shaofu Liu, Xiang Wang, Man Park, Jun-Sang Almer, Jonathan Stubbins, James F. TI The comparison of microstructures and mechanical properties between 14Cr-Al and 14Cr-Ti ferritic ODS alloys SO MATERIALS & DESIGN LA English DT Article DE Synchrotron X-ray diffraction; Tensile deformation; Nanoscale particles; Microstructure ID ENERGY X-RAYS; TEMPERATURE-DEPENDENCE; MATERIALS CHALLENGES; MARTENSITIC STEEL; PRESSURIZED-WATER; TENSILE; NANOPARTICLES; DEFORMATION; DISLOCATION; SYNCHROTRON AB In this study, two kinds of 14Cr ODS alloys (14Cr-Al and 14Cr-Ti) were investigated to reveal the different effects between Al and Ti on the microstructures and mechanical properties of 14Cr ferritic ODS alloys. The microstructure information such as grains, minor phases of these two alloys has been investigated by high-energy X-ray diffraction and transmission electron microscopy (TEM). The in situ synchrotron X-ray diffraction tensile Lest was applied to investigate the mechanical properties of these two alloys. The lattice strains of different phases through the entire tensile deformation process in these two alloys were analyzed to calculate their elastic stresses. From the comparison of elastic stress, the strengthening capability of Y2Ti2O7 is better than TiN in 14Cr-Ti, and the strengthening capability of YAH is much better than YAM and AIN in 14Cr-Al ODS. The dislocation densities of 14Cr-Ti and 14Cr-Al ODS alloys during tensile deformation were also examined by modified Williamson-Hall analyses of peak broadening, respectively. The different increasing speed of dislocation density with plastic deformation reveals the better strengthening effect of Y-Ti-O particles in 14Cr-Ti ODS than that of Y-AI-O particles in 14Cr-Al ODS alloy. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Zhang, Guangming; Zhou, Zhangjian; Li, Shaofu; Wang, Man] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [Zhang, Guangming; Miao, Yinbin; Liu, Xiang; Stubbins, James F.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Mo, Kun; Miao, Yinbin] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Park, Jun-Sang; Almer, Jonathan] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zhou, ZJ (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Lab Special Ceram & Powder Met, Beijing 100083, Peoples R China. EM zhouzhj@mater.ustb.edu.cn RI Liu, Xiang/D-2005-2017; OI Liu, Xiang/0000-0002-2634-1888; Miao, Yinbin/0000-0002-3128-4275 FU National Magnetic Confinement Fusion Program of China [2015GB121006]; International SAMP;T Cooperation Program of China [2013DFG62090]; U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by National Magnetic Confinement Fusion Program of China under Grant No. 2015GB121006 and International S&T Cooperation Program of China (No.2013DFG62090). Argonne National Laboratory's work was supported under U.S. Department of Energy Contract No. DE-AC02-06CH11357. NR 37 TC 3 Z9 3 U1 12 U2 50 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0264-1275 EI 1873-4197 J9 MATER DESIGN JI Mater. Des. PD MAY 15 PY 2016 VL 98 BP 61 EP 67 DI 10.1016/j.matdes.2016.02.117 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA DI1RK UT WOS:000373273000007 ER PT J AU Liu, Y Zhang, BZ Kinsinger, CL Yang, Y Seifert, S Yan, YS Maupin, CM Liberatore, MW Herring, AM AF Liu, Ye Zhang, Bingzi Kinsinger, Corey L. Yang, Yuan Seifert, Soenke Yan, Yushan Maupin, C. Mark Liberatore, Matthew W. Herring, Andrew M. TI Anion exchange membranes composed of a poly(2,6-dimethyl-1, 4-phenylene oxide) random copolymer functionalized with a bulky phosphonium cation SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE Anion exchange membrane; Hansen solubility parameter; Morphology; Ionic conductivity; Water transport ID PROTON CONDUCTING MEMBRANES; FUEL-CELLS; TRANSPORT-PROPERTIES; SELF-DIFFUSION; SOLUBILITY PARAMETERS; WATER; HYDROXIDE; NAFION; MORPHOLOGY; IONOMER AB A random copolymer, tris(2,4,6-trimethoxyphenyl) phosphonium functionalized poly(2,6-dimethyl-1,4-phenylene oxide) (PPO-TPQP) was cast from three different solvents: dimethyl sulfoxide (DMSO), ethyl lactate, or a 41:59 vol% mixture of DMSO and ethyl lactate. Solvents were selected via analysis of the Hansen solubility parameters to vary the phase separation of the polymer in the films. An optimized mixture of DMSO and ethyl lactate chosen for film fabrication and this film was contrasted with films cast from the neat constituent solvents. Atomic force microscopy identified domains from nanometer to tens of nanometer sizes, while the light microscopy showed features on the order of micron. SAXS revealed a cation scattering peak with a d-spacing from 7 to 15 A. Trends in conductivity and water diffusion for the membranes vary depending on the solvent from which they are cast. The mixed solvent cast membrane shows a linear Arrhenius behavior indicating fully dissociated cationic/anionic groups, and has the highest bromide conductivity of 3 mS/cm at 95% RH, 90 degrees C. The ethyl lactate cast membrane shows a linear Arrhenius relation in conductivity, but a Vogel-Tamman-Fulcher behavior in its water self-diffusion. While water increases bromide dissociation, water and bromide transport in these films seems to be decoupled. This is particularly true for the film cast from ethyl lactate. (C) 2016 Elsevier B.V. All rights reserved. C1 [Liu, Ye; Kinsinger, Corey L.; Maupin, C. Mark; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Zhang, Bingzi; Yan, Yushan] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA. [Yang, Yuan] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Liberatore, Matthew W.] Univ Toledo, Dept Chem & Environm Engn, Toledo, OH 43606 USA. RP Herring, AM (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM aherring@mines.edu RI Liberatore, Matthew/B-6828-2008; OI Herring, Andrew/0000-0001-7318-5999 FU Army Research Office under the MURI Grant [W911NF-10-1-0520]; U. S. DOE [DE-AC02-06CH11357] FX The authors thank the Army Research Office for support of this research under the MURI Grant number #W911NF-10-1-0520. The Advanced Photon Source operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was support by the U. S. DOE under Contract No. DE-AC02-06CH11357. We also thank Dr. Steven Abbott for the HSP calculation on PPO-TPQP by using the HSPiP package. NR 47 TC 5 Z9 5 U1 27 U2 139 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 EI 1873-3123 J9 J MEMBRANE SCI JI J. Membr. Sci. PD MAY 15 PY 2016 VL 506 BP 50 EP 59 DI 10.1016/j.memsci.2016.01.042 PG 10 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA DE8HF UT WOS:000370875900006 ER PT J AU Zhen, L Ford, N Gale, DK Roesijadi, G Rorrer, GL AF Zhen, Le Ford, Nicole Gale, Debra K. Roesijadi, Guritno Rorrer, Gregory L. TI Photoluminescence detection of 2,4,6-trinitrotoluene (TNT) binding on diatom frustule biosilica functionalized with an anti-TNT monoclonal antibody fragment SO BIOSENSORS & BIOELECTRONICS LA English DT Article DE Antibody; Biosensor; Biosilica; Diatom; Photoluminescence; Trinitrotoluene ID SILICA NANOPARTICLES; OPTICAL BIOSENSORS; MARINE DIATOMS; EXPLOSIVES; SEAWATER; SENSORS; SURFACE AB A selective and label-free biosensor for detection of the explosive compound 2,4,6-trinitrotoluene (TNT) in aqueous solution was developed based on the principle of photoluminescence quenching of upon immunocomplex formation with antibody-functionalized diatom frustule biosilica. The diatom frustule is an intricately nanostructured, highly porous biogenic silica material derived from the shells of microscopic algae called diatoms. This material emits strong visible blue photoluminescence (PL) upon UV excitation. PL-active frustule biosilica was isolated from cultured cells of the marine diatom Pinnularia sp. and functionalized with a single chain variable fragment (scFv) derived from an anti-TNT monoclonal antibody. When TNT was bound to the anti-TNT scFv-functionalized diatom frustule biosilica, the PL emission from the biosilica was partially quenched due to the electrophilic nature of the nitro (-NO2) groups on the TNT molecule. The dose-response curve for immunocomplex formation of TNT on the scFv-functionalized diatom frustule biosilica had a half-saturation binding constant of 6.4 +/- 2.4. 10(-8) M and statistically-significant measured detection limit of 3.5.10(-8) M. The binding and detection were selective for TNT and TNB (trinitrobenzene) but not RDX (hexahydro-1,3,5-trinitro-1,3,5-triazine) or 2,6-DNT (2,6-dinitrotoluene). (C) 2016 Published by Elsevier B.V. C1 [Zhen, Le; Gale, Debra K.; Rorrer, Gregory L.] Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. [Ford, Nicole; Roesijadi, Guritno] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. [Roesijadi, Guritno] Oregon State Univ, Dept Microbiol, Corvallis, OR 97331 USA. RP Rorrer, GL (reprint author), Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. EM rorrergl@engr.orst.edu FU U.S. Department of Defense, Office of Naval Research, Synthetic Biology Program [N0001414IP20004, N000141210313] FX Support of this research was provided by U.S. Department of Defense, Office of Naval Research, Synthetic Biology Program, Award Numbers N0001414IP20004 (PNNL) and N000141210313 (OSU). Drs. Ellen Goldman and Igor Medintz, U.S. Naval Research Laboratory (NRL), Washington DC, kindly provided the plasmid containing the unmodified anti-TNT scFv, and the AF555-TNB standard. NR 28 TC 3 Z9 3 U1 5 U2 59 PU ELSEVIER ADVANCED TECHNOLOGY PI OXFORD PA OXFORD FULFILLMENT CENTRE THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0956-5663 EI 1873-4235 J9 BIOSENS BIOELECTRON JI Biosens. Bioelectron. PD MAY 15 PY 2016 VL 79 BP 742 EP 748 DI 10.1016/j.bios.2016.01.002 PG 7 WC Biophysics; Biotechnology & Applied Microbiology; Chemistry, Analytical; Electrochemistry; Nanoscience & Nanotechnology SC Biophysics; Biotechnology & Applied Microbiology; Chemistry; Electrochemistry; Science & Technology - Other Topics GA DE0IU UT WOS:000370309200102 ER PT J AU Wang, ZL Xiu, PY Huang, L Nie, ZH Zeng, JX Brown, DE Ren, Y Wang, YD AF Wang, Zilong Xiu, Pengyuan Huang, Lian Nie, Zhihua Zeng, Junxi Brown, Dennis E. Ren, Yang Wang, Yandong TI Observation of magnetic-field-induced transformation in MnCo0.78Fe0.22Ge alloys with colossal strain output and large magnetocaloric effect SO JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS LA English DT Article DE In-situ synchrotron high-energy X-ray diffraction; Magnetic field-induced phase transformation; Magnetocaloric effect ID ENTROPY CHANGE; TRANSITION; EXPANSION; MNCOGE AB The thermal, structural and magnetic properties were studied for the hexagonal MnCo0.78Fe0.22Ge alloys, which undergoes a first-order phase transformation from paramagnetic hexagonal phase into ferromagnetic orthorhombic martensite on cooling. Owing to the magnetostructural coupling, large magnetocaloric effect (Delta S-M= 10.97 J kg(-1) K-1) was obtained at 254 K. In-situ synchrotron high-energy X-ray diffraction experiments were conducted to reveal the detailed change in crystallographic structure of phases and the effect of applied magnetic field on phase transformation behaviors. An anomalously huge strain of 11.89% and volume expansion of 4.35% in unit-cell were obtained between martensite and parent phase across the transformation. Furthermore, the magnetic field-induced martensitic transformation was directly evidenced at 250 K, which eventually demonstrates the possibility to achieve magnetic-field-induced strain and large magnetocaloric effect simultaneously. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wang, Zilong; Wang, Yandong] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Wang, Zilong; Huang, Lian; Nie, Zhihua; Zeng, Junxi] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing 100081, Peoples R China. [Xiu, Pengyuan] Univ Michigan, Dept Mat Sci & Engn, Ann Arbor, MI 48109 USA. [Brown, Dennis E.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Ren, Yang] Argonne Natl Lab, XRay Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Wang, YD (reprint author), Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. EM ydwang@mail.neu.edu.cn RI wang, yandong/G-9404-2013; Nie, Zhihua/G-9459-2013 OI Nie, Zhihua/0000-0002-2533-933X FU National Basic Research Program of China (973 Program) [2012CB619405]; National Natural Science Foundation of China [50971031]; Fundamental Research Funds for the Central Universities [06111020]; U.S. Department of Energy, Office of Science, Office of Basic Energy Science [DE-AC02-06CH11357] FX This study was supported by the National Basic Research Program of China (973 Program) under Contract no. 2012CB619405, the National Natural Science Foundation of China (Grant no. 50971031) and the Fundamental Research Funds for the Central Universities (Grant no. 06111020). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, under Contract no. DE-AC02-06CH11357. NR 24 TC 2 Z9 2 U1 18 U2 81 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-8853 EI 1873-4766 J9 J MAGN MAGN MATER JI J. Magn. Magn. Mater. PD MAY 15 PY 2016 VL 406 BP 179 EP 183 DI 10.1016/j.jmmm.2015.12.083 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA DC4ZS UT WOS:000369230100026 ER PT J AU Cawkwell, MJ Luscher, DJ Addessio, FL Ramos, KJ AF Cawkwell, M. J. Luscher, D. J. Addessio, F. L. Ramos, K. J. TI Equations of state for the alpha and gamma polymorphs of cyclotrimethylene trinitramine SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID CRYSTAL-STRUCTURE; PENTAERYTHRITOL TETRANITRATE; DISPERSION CORRECTIONS; ENERGETIC MATERIALS; PHASE-DIAGRAM; OF-STATE; DFT-D; RDX; PRESSURE; HEXAHYDRO-1,3,5-TRINITRO-1,3,5-TRIAZINE AB Equations of state for the alpha and gamma polymorphs of the energetic molecular crystal cyclotrimethylene trinitramine (RDX) have been developed from their Helmholtz free energies. The ion motion contribution to the Helmholtz free energy is represented by Debye models with density-dependent Debye temperatures that are parameterized to vibrational densities of states computed from dispersion-corrected density functional theory. By separating the vibrational density of states into low frequency modes of mainly lattice phonon character and high frequency modes of intramolecular character we were able to significantly improve the description of the heat capacity at low temperatures and the thermal contribution to the pressure. The ion motion contribution to the Helmholtz free energy of the high pressure gamma polymorph was constructed from that of the a polymorph to reproduce the temperature-independent transformation pressure seen experimentally. The static lattice energies for both polymorphs were constructed to reproduce published isothermal compression data. The equations of state have been applied to the prediction of the path of the principal Hugoniot in the equilibrium phase diagram. Published by AIP Publishing. C1 [Cawkwell, M. J.; Luscher, D. J.; Addessio, F. L.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Ramos, K. J.] Los Alamos Natl Lab, Weap Expt Div, POB 1663, Los Alamos, NM 87545 USA. RP Cawkwell, MJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cawkwell@lanl.gov OI Cawkwell, Marc/0000-0002-8919-3368 NR 36 TC 2 Z9 2 U1 6 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 185106 DI 10.1063/1.4948673 PG 8 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500037 ER PT J AU Christensen, S Schmokel, MS Borup, KA Madsen, GKH McIntyre, GJ Capelli, SC Christensen, M Iversen, BB AF Christensen, Sebastian Schmokel, Mette Stokkebro Borup, Kasper Andersen Madsen, Georg K. H. McIntyre, Garry J. Capelli, Silvia C. Christensen, Mogens Iversen, Bo Brummerstedt TI "Glass-like" thermal conductivity gradually induced in thermoelectric Sr8Ga16Ge30 clathrate by off-centered guest atoms SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MAXIMUM-ENTROPY-METHOD; INELASTIC NEUTRON-SCATTERING; CRYSTAL-STRUCTURE; X-RAY; SINGLE-CRYSTAL; BA8GA16GE30; DIFFRACTION; VACANCIES; GE; BA8GA16SN30 AB The origin of the "glass-like" plateau in thermal conductivity of inorganic type I clathrates has been debated for more than a decade. Here, it is demonstrated that the low temperature thermal conductivity of Sr8Ga16Ge30 can be controlled by the synthesis method: A flux-grown sample has a "glass-like" plateau in thermal conductivity at low temperature, while a zone-melted sample instead has a crystalline peak. A combination of flux-growth and zone-melting produces an intermediate thermal conductivity. In a comprehensive study of three single crystal samples, it is shown by neutron diffraction that the transition from crystalline peak to "glass-like" plateau is related to an increase in Sr guest atom off-centering distance from 0.24 angstrom to 0.43 angstrom. By modifying ab initio calculated force constants for the guest atom to an isotropic model, we reproduce both measured heat capacity and inelastic neutron scattering data. The transition from peak to plateau in the thermal conductivity can be modeled by a combined increase of Rayleigh and disorder scattering. Measurement of heat capacity refutes simple models for tunneling of Sr between off-center sites. Furthermore, the electronic properties of the same samples are characterized by Hall carrier density, Seebeck coefficient, and resistivity. The present comprehensive analysis excludes tunneling and charge carrier scattering as dominant contributors to the "glass-like" plateau. The increased guest atom off-centering distance controlled by synthesis provides a possible microscopic mechanism for reducing the low temperature thermal conductivity of clathrates. Published by AIP Publishing. C1 [Christensen, Sebastian; Schmokel, Mette Stokkebro; Borup, Kasper Andersen; Christensen, Mogens; Iversen, Bo Brummerstedt] Aarhus Univ, Ctr Mat Crystallog, Dept Inorgan Chem, Langelandsgade 140, DK-8000 Aarhus C, Denmark. [Christensen, Sebastian; Schmokel, Mette Stokkebro; Borup, Kasper Andersen; Christensen, Mogens; Iversen, Bo Brummerstedt] Aarhus Univ, Ctr Mat Crystallog, iNANO, Langelandsgade 140, DK-8000 Aarhus C, Denmark. [Madsen, Georg K. H.] Ruhr Univ Bochum, ICAMS, Univ Str 150, Bochum, Germany. [McIntyre, Garry J.; Capelli, Silvia C.] Inst Laue Langevin, 71 Ave Martyrs,CS 20156, Grenoble 9, France. [Borup, Kasper Andersen] Natl Renewable Energy Lab, Mail Stop RSF200,15013 Denver West Pkwy, Golden, CO 80401 USA. [McIntyre, Garry J.] Australian Nucl Sci & Technol Org, New Illawarra Rd, Lucas Heights, NSW 2234, Australia. [Capelli, Silvia C.] Rutherford Appleton Lab, ISIS Neutron & Muon Source, Didcot OX11 0QX, Oxon, England. RP Christensen, M; Iversen, BB (reprint author), Aarhus Univ, Ctr Mat Crystallog, Dept Inorgan Chem, Langelandsgade 140, DK-8000 Aarhus C, Denmark.; Christensen, M; Iversen, BB (reprint author), Aarhus Univ, Ctr Mat Crystallog, iNANO, Langelandsgade 140, DK-8000 Aarhus C, Denmark. EM mch@chem.au.dkdk; bo@chem.au.dk NR 78 TC 1 Z9 1 U1 9 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 185102 DI 10.1063/1.4948334 PG 11 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500033 ER PT J AU Fioretti, AN Schwartz, CP Vinson, J Nordlund, D Prendergast, D Tamboli, AC Caskey, CM Tuomisto, F Linez, F Christensen, ST Toberer, ES Lany, S Zakutayev, A AF Fioretti, Angela N. Schwartz, Craig P. Vinson, John Nordlund, Dennis Prendergast, David Tamboli, Adele C. Caskey, Christopher M. Tuomisto, Filip Linez, Florence Christensen, Steven T. Toberer, Eric S. Lany, Stephan Zakutayev, Andriy TI Understanding and control of bipolar self-doping in copper nitride SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 28th International Conference on Defects in Semiconductors (ICDS) CY JUL 27-31, 2015 CL Espoo, FINLAND SP Aalto Univ Sch Sci, Helsinki Reg Transport, Agilent Technologies, Nokia ID THIN-FILMS; SEMICONDUCTORS; DEPOSITION; TIN AB Semiconductor materials that can be doped both n-type and p-type are desirable for diode-based applications and transistor technology. Copper nitride (Cu3N) is a metastable semiconductor with a solar-relevant bandgap that has been reported to exhibit bipolar doping behavior. However, deeper understanding and better control of the mechanism behind this behavior in Cu3N is currently lacking in the literature. In this work, we use combinatorial growth with a temperature gradient to demonstrate both conduction types of phase-pure, sputter-deposited Cu3N thin films. Room temperature Hall effect and Seebeck effect measurements show n-type Cu3N with 10(17) electrons/cm 3 for low growth temperature (approximate to 35 degrees C) and p-type with 10(15) holes/cm(3)-10(16) holes/cm(3) for elevated growth temperatures (50 degrees C-120 degrees C). Mobility for both types of Cu3N was approximate to 0.1 cm(2)/Vs-1 cm(2)/Vs. Additionally, temperature-dependent Hall effect measurements indicate that ionized defects are an important scattering mechanism in p-type films. By combining X-ray absorption spectroscopy and first-principles defect theory, we determined that V-Cu defects form preferentially in p-type Cu3N, while Cui defects form preferentially in n-type Cu3N, suggesting that Cu3N is a compensated semiconductor with conductivity type resulting from a balance between donor and acceptor defects. Based on these theoretical and experimental results, we propose a kinetic defect formation mechanism for bipolar doping in Cu3N that is also supported by positron annihilation experiments. Overall, the results of this work highlight the importance of kinetic processes in the defect physics of metastable materials and provide a framework that can be applied when considering the properties of such materials in general. Published by AIP Publishing. C1 [Fioretti, Angela N.; Tamboli, Adele C.; Caskey, Christopher M.; Christensen, Steven T.; Toberer, Eric S.; Lany, Stephan; Zakutayev, Andriy] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Fioretti, Angela N.; Tamboli, Adele C.; Caskey, Christopher M.; Toberer, Eric S.] Colorado Sch Mines, Golden, CO 80401 USA. [Schwartz, Craig P.; Nordlund, Dennis] SLAC Natl Accelerator Lab, Menlo Pk, CA 94720 USA. [Vinson, John] NIST, Gaithersburg, MD 20899 USA. [Prendergast, David] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tuomisto, Filip; Linez, Florence] Aalto Univ, Espoo 02150, Finland. RP Fioretti, AN; Zakutayev, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA.; Fioretti, AN (reprint author), Colorado Sch Mines, Golden, CO 80401 USA. EM afiorett@mines.edu; riy.zakutayev@nrel.gov RI Tuomisto, Filip/B-8189-2008; OI Tuomisto, Filip/0000-0002-6913-5654; Vinson, John/0000-0002-7619-7060; Fioretti, Angela/0000-0002-3271-9023 NR 35 TC 3 Z9 3 U1 11 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 181508 DI 10.1063/1.4948244 PG 10 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500010 ER PT J AU Grun, J Cranch, GA Lunsford, R Compton, S Walton, OR Weaver, J Dunlop, W Fournier, KB AF Grun, J. Cranch, G. A. Lunsford, R. Compton, S. Walton, O. R. Weaver, J. Dunlop, W. Fournier, K. B. TI Scaled experiments of explosions in cavities SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NUCLEAR-EXPLOSIONS; BLAST WAVES; PRESSURE; SHOCK AB Consequences of an explosion inside an air-filled cavity under the earth's surface are partly duplicated in a laboratory experiment on spatial scales 1000 smaller. The experiment measures shock pressures coupled into a block of material by an explosion inside a gas-filled cavity therein. The explosion is generated by suddenly heating a thin foil that is located near the cavity center with a short laser pulse, which turns the foil into expanding plasma, most of whose energy drives a blast wave in the cavity gas. Variables in the experiment are the cavity radius and explosion energy. Measurements and GEODYN code simulations show that shock pressures measured in the block exhibit a weak dependence on scaled cavity radius up to similar to 25 m/kt(1/3), above which they decrease rapidly. Possible mechanisms giving rise to this behavior are described. The applicability of this work to validating codes used to simulate full-scale cavity explosions is discussed. C1 [Grun, J.; Lunsford, R.; Weaver, J.] Naval Res Lab, Div Plasma Phys, Washington, DC 20375 USA. [Cranch, G. A.] Naval Res Lab, Opt Sci Div, Washington, DC 20375 USA. [Compton, S.] Lawrence Livermore Natl Lab, Def Technol Engn Div, Livermore, CA 94551 USA. [Walton, O. R.] Lawrence Livermore Natl Lab, Atmosphere Earth & Energy Div, Livermore, CA 94551 USA. [Dunlop, W.] Lawrence Livermore Natl Lab, Program N, Livermore, CA 94551 USA. [Fournier, K. B.] Lawrence Livermore Natl Lab, NIF User Off, Livermore, CA 94551 USA. [Lunsford, R.] Princeton Plasma Phys Lab, Plasma Sci & Technol, Princeton, NJ 08536 USA. RP Grun, J (reprint author), Naval Res Lab, Div Plasma Phys, Washington, DC 20375 USA. EM Jacob.Grun@NRL.NAVY.MIL OI Fournier, Kevin/0000-0002-1123-3788 NR 31 TC 0 Z9 0 U1 5 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 184903 DI 10.1063/1.4948952 PG 12 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500030 ER PT J AU Smith, BE Zhou, XZ Roder, PB Abramson, EH Pauzauskie, PJ AF Smith, Bennett E. Zhou, Xuezhe Roder, Paden B. Abramson, Evan H. Pauzauskie, Peter J. TI Recovery of hexagonal Si-IV nanowires from extreme GPa pressure SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PHOTONIC CRYSTALS; AMBIENT PRESSURE; SILICON; PHASES; LIGHT; GAP AB We use Raman spectroscopy in tandem with transmission electron microscopy and density functional theory simulations to show that extreme (GPa) pressure converts the phase of silicon nanowires from cubic (Si-I) to hexagonal (Si-IV) while preserving the nanowire's cylindrical morphology. In situ Raman scattering of the longitudinal transverse optical (LTO) mode demonstrates the high-pressure Si-I to Si-II phase transition near 9 GPa. Raman signal of the LTO phonon shows a decrease in intensity in the range of 9-14 GPa. Then, at 17 GPa, it is no longer detectable, indicating a second phase change (Si-II to Si-V) in the 14-17 GPa range. Recovery of exotic phases in individual silicon nanowires from diamond anvil cell experiments reaching 17 GPa is also shown. Raman measurements indicate Si-IV as the dominant phase in pressurized nanowires after decompression. Transmission electron microscopy and electron diffraction confirm crystalline Si-IV domains in individual nanowires. Computational electromagnetic simulations suggest that heating from the Raman laser probe is negligible and that near-hydrostatic pressure is the primary driving force for the formation of hexagonal silicon nanowires. Published by AIP Publishing. C1 [Smith, Bennett E.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Zhou, Xuezhe; Roder, Paden B.; Pauzauskie, Peter J.] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Abramson, Evan H.] Univ Washington, Dept Earth & Space Sci, Seattle, WA 98195 USA. [Pauzauskie, Peter J.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Pauzauskie, PJ (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.; Pauzauskie, PJ (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM peterpz@uw.edu OI abramson, evan/0000-0001-5278-0836 NR 33 TC 1 Z9 1 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 185902 DI 10.1063/1.4948576 PG 4 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500054 ER PT J AU Yu, KM Detert, DM Chen, GB Zhu, W Liu, CP Grankowska, S Hsu, L Dubon, OD Walukiewicz, W AF Yu, Kin Man Detert, D. M. Chen, Guibin Zhu, Wei Liu, Chaoping Grankowska, S. Hsu, L. Dubon, O. D. Walukiewicz, Wladek TI Defects and properties of cadmium oxide based transparent conductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article; Proceedings Paper CT 28th International Conference on Defects in Semiconductors (ICDS) CY JUL 27-31, 2015 CL Espoo, FINLAND SP Aalto Univ Sch Sci, Helsinki Reg Transport, Agilent Technologies, Nokia ID NATIVE DEFECTS; CDO; FILMS; SEMICONDUCTORS; CONDUCTIVITY; SCATTERING; TRANSPORT; MOBILITY; MOCVD AB Transparent conductors play an increasingly important role in a number of semiconductor technologies. This paper reports on the defects and properties of Cadmium Oxide, a transparent conducting oxide which can be potentially used for full spectrum photovoltaics. We carried out a systematic investigation on the effects of defects in CdO thin films undoped and intentionally doped with In and Ga under different deposition and annealing conditions. We found that at low growth temperatures (<200 degrees C), sputter deposition tends to trap both oxygen vacancies and compensating defects in the CdO film resulting in materials with high electron concentration of similar to 2 x 10(20)/cm(3) and mobility in the range of 40-100 cm(2)/Vs. Thermal annealing experiments in different ambients revealed that the dominating defects in sputtered CdO films are oxygen vacancies. Oxygen rich CdO films grown by sputtering with increasing O-2 partial pressure in the sputter gas mixture results in films with resistivity from similar to 4 x 10(-4) to >1 Omega cm due to incorporation of excess O in the form of O-related acceptor defects, likely to be O interstitials. Intentional doping with In and Ga donors leads to an increase of both the electron concentration and the mobility. With proper doping CdO films with electron concentration of more than 10(21) cm(-3) and electron mobility higher than 120 cm(2)/V s can be achieved. Thermal annealing of doped CdO films in N-2 ambient can further improve the electrical properties by removing native acceptors and improving film crystallinity. Furthermore, the unique doping behavior and electrical properties of CdO were explored via simulations based on the amphoteric defect model. A comparison of the calculations and experimental results show that the formation energy of native donors and acceptors at the Fermi stabilization energy is similar to 1 eV and that the mobility of sputtered deposited CdO is limited by a background acceptor concentration of similar to 5-6 x 10(20)/cm(3). The calculations offer an insight into understanding of the effects of defects on electrical properties of undoped and doped CdO and offer a potential to use similar methods to analyze doping and defect properties of other semiconductor materials. Published by AIP Publishing. C1 [Yu, Kin Man; Liu, Chaoping] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. [Yu, Kin Man; Detert, D. M.; Chen, Guibin; Zhu, Wei; Grankowska, S.; Dubon, O. D.; Walukiewicz, Wladek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Detert, D. M.; Dubon, O. D.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Chen, Guibin] Huaiyin Normal Univ, Dept Phys, Huaian 223300, Jiangsu, Peoples R China. [Chen, Guibin] Huaiyin Normal Univ, Jiangsu Key Lab Chem Low Dimens Mat, Huaian 223300, Jiangsu, Peoples R China. [Zhu, Wei] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Zhu, Wei] Univ Sci & Technol China, Ctr Phys Expt, Hefei 230026, Anhui, Peoples R China. [Grankowska, S.] Warsaw Univ, Inst Expt Phys IEP UW, Warsaw, Poland. [Hsu, L.] Univ Minnesota, Dept Postsecondary Teaching & Learning, Minneapolis, MN 55455 USA. RP Yu, KM (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China.; Yu, KM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM kinmanyu@cityu.edu.hk OI Yu, Kin Man/0000-0003-1350-9642 NR 31 TC 3 Z9 3 U1 11 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 14 PY 2016 VL 119 IS 18 AR 181501 DI 10.1063/1.4948236 PG 10 WC Physics, Applied SC Physics GA DO3YB UT WOS:000377717500003 ER PT J AU Alfonso, DR Kauffman, D Matranga, C AF Alfonso, Dominic R. Kauffman, Douglas Matranga, Christopher TI Active sites of ligand-protected Au-25 nanoparticle catalysts for CO2 electroreduction to CO SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ELECTROCATALYTIC ACTIVITY; OPTICAL-PROPERTIES; CRYSTAL-STRUCTURE; CARBON-DIOXIDE; NANOCLUSTERS; STABILITY; OXIDATION; CLUSTERS; WATER; REDUCTION AB Recent experimental studies have reported the electrochemical reduction of carbon dioxide (CO2) into CO at atomically precise negatively charged Au-25-nanoclusters. The studies showed CO2 conversion at remarkably low overpotentials, but the exact mechanisms and nature of the active sites remain unclear. We used first-principles density functional theory and continuum solvation models to examine the role of the cluster during electrochemical CO2 reduction and analyze the free energies of proposed intermediate species. Contrary to previous assumptions, our results show that the fully ligand protected cluster is not an active CO2 reduction catalyst because formation of the crucial carboxyl intermediate required very high electrochemical potentials. Instead, our calculations suggest that the reduction process likely occurs on a dethiolated gold site, and adsorbed carboxyl intermediate formation was significantly stabilized at dethiolated gold sites. These findings point to the crucial role of exposed metal sites during electrochemical CO2 reduction at gold nanocluster catalysts. C1 [Alfonso, Dominic R.; Kauffman, Douglas; Matranga, Christopher] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Alfonso, DR (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM alfonso@netl.doe.gov OI Kauffman, Douglas/0000-0002-7855-3428 FU United States Government FX This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of author(s) expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 42 TC 1 Z9 1 U1 26 U2 61 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2016 VL 144 IS 18 AR 184705 DI 10.1063/1.4948792 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WB UT WOS:000377711900035 PM 27179498 ER PT J AU Elkins, MH Williams, HL Neumark, DM AF Elkins, Madeline H. Williams, Holly L. Neumark, Daniel M. TI Isotope effect on hydrated electron relaxation dynamics studied with time-resolved liquid jet photoelectron spectroscopy SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID WATER-CLUSTER ANIONS; FEMTOSECOND SOLVATION DYNAMICS; QUANTUM DECOHERENCE; ULTRAFAST DYNAMICS; AQUEOUS-SOLUTIONS; EXCESS ELECTRONS; SIMULATION; SPECTRA; BULK; PHOTODETACHMENT AB The excited state relaxation dynamics of the solvated electron in H2O and D2O are investigated using time-resolved photoelectron spectroscopy in a liquid microjet. The data show that the initial excited state decays on a time scale of 75 +/- 12 fs in H2O and 102 +/- 8 fs in D2O, followed by slower relaxation on time scales of 400 +/- 70 fs and 390 +/- 70 fs that are isotopically invariant within the precision of our measurements. Based on the time evolution of the transient signals, the faster and slower time constants are assigned to p -> s internal conversion (IC) of the hydrated electron and relaxation on the ground electronic state, respectively. This assignment is consistent with the non-adiabatic mechanism for relaxation of the hydrated electron and yields an isotope effect of 1.4 +/- 0.2 for IC of the hydrated electron. Published by AIP Publishing. C1 [Elkins, Madeline H.; Williams, Holly L.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Elkins, Madeline H.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Neumark, DM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU National Science Foundation [CHE-1361412]; Air Force Office of Scientific Research [24086151-06]; UC Berkeley Center for Solvation Studies, CALSOLV; Ruhr Explores Solvation, RESOLV; Deutsche Forschungsgemeinschaft (DFG) [28 Mio. EUR] FX This work was funded by the National Science Foundation under the Grant No. CHE-1361412. Additional support is provided by the Air Force Office of Scientific Research under Grant No. 24086151-06 as part of the MURI topic "Time-Resolved Quantum Dynamics of Complex Systems." H.L.W. is supported through the UC Berkeley Center for Solvation Studies, CALSOLV, in collaboration with Ruhr Explores Solvation, RESOLV, and funded by 28 Mio. EUR by the Deutsche Forschungsgemeinschaft (DFG). The authors thank Benjamin Schwartz at UCLA for helpful discussions regarding isotope effects. The data presented here are available on request sent to dneumark@berkeley.edu. NR 72 TC 1 Z9 1 U1 4 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 14 PY 2016 VL 144 IS 18 AR 184503 DI 10.1063/1.4948546 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3WB UT WOS:000377711900028 PM 27179491 ER PT J AU Glenzer, SH Fletcher, LB Galtier, E Nagler, B Alonso-Mori, R Barbrel, B Brown, SB Chapman, DA Chen, Z Curry, CB Fiuza, F Gamboa, E Gauthier, M Gericke, DO Gleason, A Goede, S Granados, E Heimann, P Kim, J Kraus, D MacDonald, MJ Mackinnon, AJ Mishra, R Ravasio, A Roedel, C Sperling, P Schumaker, W Tsui, YY Vorberger, J Zastrau, U Fry, A White, WE Hasting, JB Lee, HJ AF Glenzer, S. H. Fletcher, L. B. Galtier, E. Nagler, B. Alonso-Mori, R. Barbrel, B. Brown, S. B. Chapman, D. A. Chen, Z. Curry, C. B. Fiuza, F. Gamboa, E. Gauthier, M. Gericke, D. O. Gleason, A. Goede, S. Granados, E. Heimann, P. Kim, J. Kraus, D. MacDonald, M. J. Mackinnon, A. J. Mishra, R. Ravasio, A. Roedel, C. Sperling, P. Schumaker, W. Tsui, Y. Y. Vorberger, J. Zastrau, U. Fry, A. White, W. E. Hasting, J. B. Lee, H. J. TI Matter under extreme conditions experiments at the Linac Coherent Light Source SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Review DE high-energy density physics; free electron x-ray laser; x-ray scattering; warm dense matter; dynamically compressed matter ID RAY THOMSON SCATTERING; FREE-ELECTRON LASER; EQUATION-OF-STATE; NATIONAL IGNITION FACILITY; WARM DENSE MATTER; X-RAYS; PLASMAS; ENERGY; ACCELERATION; CONDUCTIVITY AB The matter in extreme conditions end station at the Linac Coherent Light Source (LCLS) is a new tool enabling accurate pump-probe measurements for studying the physical properties of matter in the high-energy density (HED) physics regime. This instrument combines the world's brightest x-ray source, the LCLS x-ray beam, with high-power lasers consisting of two nanosecond Nd:glass laser beams and one short-pulse Ti:sapphire laser. These lasers produce short-lived states of matter with high pressures, high temperatures or high densities with properties that are important for applications in nuclear fusion research, laboratory astrophysics and the development of intense radiation sources. In the first experiments, we have performed highly accurate x-ray diffraction and x-ray Thomson scattering measurements on shock-compressed matter resolving the transition from compressed solid matter to a co-existence regime and into the warm dense matter state. These complex charged-particle systems are dominated by strong correlations and quantum effects. They exist in planetary interiors and laboratory experiments, e.g., during high-power laser interactions with solids or the compression phase of inertial confinement fusion implosions. Applying record peak brightness x-rays resolves the ionic interactions at atomic (Angstrom) scale lengths and measure the static structure factor, which is a key quantity for determining equation of state data and important transport coefficients. Simultaneously, spectrally resolved measurements of plasmon features provide dynamic structure factor information that yield temperature and density with unprecedented precision at micron-scale resolution in dynamic compression experiments. These studies have demonstrated our ability to measure fundamental thermodynamic properties that determine the state of matter in the HED physics regime. C1 [Glenzer, S. H.; Fletcher, L. B.; Galtier, E.; Nagler, B.; Alonso-Mori, R.; Brown, S. B.; Chen, Z.; Curry, C. B.; Fiuza, F.; Gamboa, E.; Gauthier, M.; Goede, S.; Granados, E.; Heimann, P.; Kim, J.; MacDonald, M. J.; Mackinnon, A. J.; Mishra, R.; Roedel, C.; Sperling, P.; Schumaker, W.; Fry, A.; White, W. E.; Hasting, J. B.; Lee, H. J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd,MS 19, Menlo Pk, CA 94025 USA. [Barbrel, B.] Univ Bordeaux, CNRS, CEA, Ctr Lasers Intenses & Applicat CELIA, F-33405 Talence, France. [Barbrel, B.; Kraus, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94709 USA. [Chapman, D. A.] AWE Plc, Reading RG7 4PR, Berks, England. [Gericke, D. O.] Univ Warwick, Dept Phys, Ctr Fus Space & Astrophys, Coventry CV4 7AL, W Midlands, England. [Gleason, A.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [MacDonald, M. J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Ravasio, A.] Ecole Polytech, LULI, F-91128 Palaiseau, France. [Tsui, Y. Y.] Univ Alberta, Dept Elect & Comp Engn, Edmonton, AB, Canada. [Vorberger, J.] Max Planck Inst Phys Komplexer Syst, Noethnitzer Str 38, D-01187 Dresden, Germany. [Zastrau, U.] European XFEL GmbH, Albert Einstein Ring 19, D-22761 Hamburg, Germany. RP Glenzer, SH (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd,MS 19, Menlo Pk, CA 94025 USA. EM glenzer@slac.stanford.edu RI gauthier, Maxence/K-2578-2014; OI gauthier, Maxence/0000-0001-6608-9325; MacDonald, Michael/0000-0002-6295-6978 FU DOE Office of Science, Fusion Energy Science under FWP [100182]; DOE Office of Science, Fusion Energy Science [SF00515]; Laboratory Directed Research and Development grant; Peter-Paul-Ewald Fellowship of the VolkswagenStiftung; Theodor-von-Lynen Fellowship of the Alexander-von-Humboldt foundation FX This work was supported by DOE Office of Science, Fusion Energy Science under FWP 100182. The experiments were performed at the Matter at Extreme Conditions (MEC) instrument of LCLS, supported by the DOE Office of Science, Fusion Energy Science under contract No. SF00515. This work was further supported by Laboratory Directed Research and Development grant, the Peter-Paul-Ewald Fellowship of the VolkswagenStiftung, and the Theodor-von-Lynen Fellowship of the Alexander-von-Humboldt foundation. NR 112 TC 7 Z9 7 U1 13 U2 31 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAY 14 PY 2016 VL 49 IS 9 AR 092001 DI 10.1088/0953-4075/49/9/092001 PG 26 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DK1TX UT WOS:000374698300001 ER PT J AU Bridges, CA Rios, O Allard, LF Meyer, HM Huq, A Jiang, Y Wang, JP Brady, MP AF Bridges, C. A. Rios, O. Allard, L. F. Meyer, H. M., III Huq, A. Jiang, Y. Wang, J. -P. Brady, M. P. TI The impact of carbon coating on the synthesis and properties of alpha"-Fe16N2 powders SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID LOW-TEMPERATURE NITRIDATION; ALPHA''-FE16N2 PHASE-FORMATION; CORE-SHELL ALPHA-FE/AL2O3; GIANT MAGNETIC-MOMENT; ELECTRONIC-STRUCTURE; SATURATION MAGNETIZATION; THERMAL-STABILITY; IRON NITRIDE; FE16N2; NANOPARTICLES AB This paper presents the preparation of carbon composite Fe16N2 powders, and the influence of a protective carbon coating on the yield and magnetic properties of Fe16N2. Nanoparticle precursors with and without carbon were reacted under ammonia gas flow to produce Fe16N2. Neutron and X-ray powder diffraction indicate that the powders contain typically 40-60% Fe16N2, with the remaining phases being unreacted iron, Fe4N or Fe3N. Transmission electron microscopy demonstrates that the carbon coating is effective at reducing the level of sintering of Fe nanoparticles during the reduction stage prior to ammonolysis. XPS results support the retention of a carbon coating on the surface after ammonolysis, and that there is Fe-C bonding present at the particle surface. In situ TEM was used to observe loss of ordering in the nitrogen sublattice of carbon composite Fe16N2 powders in the range of 168 degrees C to 200 degrees C. Magnetic susceptibility measurements show maximum values for saturation magnetization in the range of 232 emu g(-1), and for coercivity near 930 Oe, for different samples measured up to 2 T applied field at 300 K. C1 [Bridges, C. A.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Rios, O.; Allard, L. F.; Meyer, H. M., III; Brady, M. P.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Huq, A.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Jiang, Y.; Wang, J. -P.] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Wang, J. -P.] Univ Minnesota, Dept Phys, Minneapolis, MN 55455 USA. RP Bridges, CA (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM bridgesca@ornl.gov RI Huq, Ashfia/J-8772-2013; Brady, Michael/A-8122-2008; Rios, Orlando/E-6856-2017 OI Huq, Ashfia/0000-0002-8445-9649; Brady, Michael/0000-0003-1338-4747; Rios, Orlando/0000-0002-1814-7815 FU ARPA-E (Advanced Research Projects Agency-Energy) BCT Fe16N2 Magnet project [0472-1595]; Scientific User Facilities Division - U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division FX This work was supported by ARPA-E (Advanced Research Projects Agency-Energy) BCT Fe16N2 Magnet project under contract No. 0472-1595. We thank Andrew Payzant for useful discussions on the structure of alpha"-Fe16N2 and related phases. A portion of this research at ORNL's Spallation Neutron Source, as appropriate, was sponsored by the Scientific User Facilities Division supported by U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division. NR 52 TC 0 Z9 0 U1 11 U2 47 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAY 14 PY 2016 VL 18 IS 18 BP 13010 EP 13017 DI 10.1039/c6cp00737f PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL5PM UT WOS:000375689200069 PM 27109006 ER PT J AU Berto, S Chiavazza, E Canepa, P Prenesti, E Daniele, PG AF Berto, Silvia Chiavazza, Enrico Canepa, Pieremanuele Prenesti, Enrico Daniele, Pier Giuseppe TI Assessing the formation of weak sodium complexes with negatively charged ligands SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID IONIC-STRENGTH DEPENDENCE; MOLECULAR-WEIGHT LIGANDS; POLYFUNCTIONAL O-LIGANDS; ALKALI-METAL COMPLEXES; AQUEOUS-SOLUTION; FORMATION-CONSTANTS; DENSITY AB The stability of sodium complexes with poly-carboxylic and polyamino-carboxylic acids is investigated with ion-selective electrode-Na+ potentiometry, working at strictly constant ionic strength. It is observed that the formation constants of the Na+ complexes with monoligand stoichiometry (ML) increase with the number of charges on the ligand. For example, in poly-carboxylic acids this dependency is linear and is well captured by an experimental equation. A different behaviour is observed for the poly-amino carboxylic acids, which show higher complexation capabilities reaching a plateau of the binding energy past a specific ligand size. The experimental results are discussed qualitatively using ab initio calculations based on DFT B3LYP, and the principal electronic characteristics of the ligands under investigation are identified. As a result of the flexibility imparted by the long chains of polyaminocarboxylic ligands, both experimental and theoretical models demonstrate that nitrogen atoms in proximity of Na+ ions can participate in the metal coordination, thus providing further stabilization for the complexes. Moreover, by increasing the ligand size the stabilization gained in terms of DG reached a plateau for EDTA, in agreement with experimental observations. C1 [Berto, Silvia; Chiavazza, Enrico; Prenesti, Enrico; Daniele, Pier Giuseppe] Univ Turin, Dept Chem, Via P Giuria 7, I-10125 Turin, Italy. [Canepa, Pieremanuele] MIT, Dept Mat Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Canepa, Pieremanuele] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Berto, S (reprint author), Univ Turin, Dept Chem, Via P Giuria 7, I-10125 Turin, Italy. EM silvia.berto@unito.it; pcanepa@lbl.gov RI Canepa, Pieremanuele/O-2344-2013 OI Canepa, Pieremanuele/0000-0002-5168-9253 FU University of Torino FX We thank the University of Torino for financing part of the project. NR 25 TC 1 Z9 1 U1 1 U2 6 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAY 14 PY 2016 VL 18 IS 18 BP 13118 EP 13125 DI 10.1039/c6cp00192k PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL5PM UT WOS:000375689200080 PM 27113137 ER PT J AU Beiersdorfer, P Scofield, JH Brown, GV Chen, MH Hell, N Osterheld, AL Vogel, DA Wong, KL AF Beiersdorfer, P. Scofield, J. H. Brown, G. V. Chen, M. H. Hell, N. Osterheld, A. L. Vogel, D. A. Wong, K. L. TI Avoided level crossings in very highly charged ions SO PHYSICAL REVIEW A LA English DT Article ID X-RAY SPECTROMETER; ISOELECTRONIC SEQUENCE; ENERGY-LEVELS; TRANSITIONS; PROSPECTS; PROGRAM; PACKAGE; ATOMS; TRAP AB We report a systematic measurement of the (2p(1/2)(-1)3d(3/2))(J=1) and (2s(1/2)(-1)3p(1/2))(J=1) levels in 14 neonlike ions between Ba46+ and Pb72+ and document the effects of their avoided crossing near Z = 68. Strong mixing affects the oscillator strengths over a surprisingly wide range of atomic numbers and leads to the vanishing of one transition two atomic numbers below the crossing. The crossing voids the otherwise correct expectation that the (2p(1/2)(-1)3d(3/2))(J=1) level energy is only weakly affected by quantum electrodynamics (QED). For about 10 atomic numbers surrounding the crossing, its QED contributions are anomalously large, attaining almost equality to those affecting the (2s(1/2)(-1)3p(1/2))(J=1) level. As a result, the accuracy of energy level calculations appears compromised near the crossing. C1 [Beiersdorfer, P.; Scofield, J. H.; Brown, G. V.; Chen, M. H.; Hell, N.; Osterheld, A. L.; Vogel, D. A.; Wong, K. L.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hell, N.] Univ Erlangen Nurnberg, D-96049 Bamberg, Germany. [Hell, N.] Univ Erlangen Nurnberg, ECAP, D-96049 Bamberg, Germany. [Vogel, D. A.] Middle Georgia State Univ, Macon, GA 31206 USA. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM beiersdorfer1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; European Space Agency [4000114313115/NL/CB] FX We acknowledge many helpful discussions with R.W. Walling and thank M. Eckart and A. Hazi for their encouragement and support. We are grateful to Dr. Ulyana Safronova for making her numerical results available to us. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. N.H. acknowledges funding by the European Space Agency under Contract No. 4000114313115/NL/CB. NR 35 TC 0 Z9 0 U1 3 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 13 PY 2016 VL 93 IS 5 AR 051403 DI 10.1103/PhysRevA.93.051403 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DL9UX UT WOS:000375989700002 ER PT J AU Brown-Altvater, F Rangel, T Neaton, JB AF Brown-Altvater, Florian Rangel, Tonatiuh Neaton, Jeffrey B. TI Ab initio phonon dispersion in crystalline naphthalene using van der Waals density functionals SO PHYSICAL REVIEW B LA English DT Article ID LATTICE-VIBRATIONS; SINGLET FISSION; MOLECULAR SEMICONDUCTORS; ELECTRONIC-STRUCTURE; NEUTRON-DIFFRACTION; INFRARED-SPECTRA; FREQUENCIES; DYNAMICS; ANTHRACENE; PRESSURE AB Acene molecular crystals are of current interest in organic optoelectronics, both as active materials and for exploring and understanding new phenomena. Phonon scattering can be an important facilitator and dissipation mechanism in charge separation and carrier transport processes. Here, we carry out density functional theory (DFT) calculations of the structure and the full phonon dispersion of crystalline naphthalene, a well-characterized acene crystal for which detailed neutron-diffraction measurements, as well as infrared and Raman spectroscopy, are available. We evaluate the performance, relative to experiments, of DFTwithin the local density approximation (LDA); the generalized gradient approximation of Perdew, Burke, and Ernzerhof (PBE); and a recent van der Waals-corrected nonlocal correlation (vdW-DF-cx) functional. We find that the vdW-DF-cx functional accurately predicts lattice parameters of naphthalene within 1%. Intermolecular and intramolecular phonon frequencies across the Brillouin zone are reproduced within 7.8% and 1%, respectively. As expected, LDA (PBE) underestimates (overestimates) the lattice parameters and overestimates (underestimates) phonon frequencies, demonstrating their shortcomings for predictive calculations of weakly bound materials. If the unit cell is fixed to the experimental lattice parameters, PBE is shown to lead to improved phonon frequencies. Our study provides a detailed understanding of the phonon spectrum of naphthalene, and highlights the importance of including van der Waals dispersion interactions in predictive calculations of lattice parameters and phonon frequencies of molecular crystals and related organic materials. C1 [Brown-Altvater, Florian] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Brown-Altvater, Florian; Rangel, Tonatiuh; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Rangel, Tonatiuh; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Brown-Altvater, F (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Brown-Altvater, F; Neaton, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Neaton, JB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Neaton, JB (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. EM altvater@berkeley.edu; jbneaton@berkeley.edu FU US Department of Energy, Office of Basic Energy Sciences; US Department of Energy, Office of Advanced Scientific Computing Research; Chemical Sciences, Geosciences, and Biosciences Division in the Office of Basic Energy Sciences of the US Department of Energy; Office of Science of the US Department of Energy FX Part of this work is supported by the US Department of Energy, Office of Basic Energy Sciences and of Advanced Scientific Computing Research through the SciDAC Program on Excited State Phenomena, and by the Chemical Sciences, Geosciences, and Biosciences Division in the Office of Basic Energy Sciences of the US Department of Energy. Computational resources were provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy. Portions of this work took place at the Molecular Foundry, supported by the US Department of Energy, Office of Basic Energy Sciences. NR 87 TC 2 Z9 2 U1 8 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 13 PY 2016 VL 93 IS 19 AR 195206 DI 10.1103/PhysRevB.93.195206 PG 8 WC Physics, Condensed Matter SC Physics GA DL9WY UT WOS:000375995300005 ER PT J AU Regnier, D Dubray, N Schunck, N Verriere, M AF Regnier, D. Dubray, N. Schunck, N. Verriere, M. TI Fission fragment charge and mass distributions in Pu-239(n, f) in the adiabatic nuclear energy density functional theory SO PHYSICAL REVIEW C LA English DT Article ID GENERATOR-COORDINATE METHOD; GAUSSIAN OVERLAP APPROXIMATION; NEUTRON-INDUCED FISSION; HARTREE-FOCK THEORY; COLLECTIVE MOTION; SUPERHEAVY NUCLEI; SELF-CONSISTENT; R-PROCESS; SYSTEMS; NUCLEOSYNTHESIS AB Background: Accurate knowledge of fission fragment yields is an essential ingredient of numerous applications ranging from the formation of elements in the r process to fuel cycle optimization for nuclear energy. The need for a predictive theory applicable where no data are available, together with the variety of potential applications, is an incentive to develop a fully microscopic approach to fission dynamics. Purpose: In this work, we calculate the pre-neutron emission charge and mass distributions of the fission fragments formed in the neutron-induced fission of Pu-239 using a microscopic method based on nuclear density functional theory (DFT). Methods: Our theoretical framework is the nuclear energy density functional (EDF) method, where large-amplitude collective motion is treated adiabatically by using the time-dependent generator coordinate method (TDGCM) under the Gaussian overlap approximation (GOA). In practice, the TDGCM is implemented in two steps. First, a series of constrained EDF calculations map the configuration and potential-energy landscape of the fissioning system for a small set of collective variables (in this work, the axial quadrupole and octupole moments of the nucleus). Then, nuclear dynamics is modeled by propagating a collective wave packet on the potential-energy surface. Fission fragment distributions are extracted from the flux of the collective wave packet through the scission line. Results: We find that the main characteristics of the fission charge and mass distributions can be well reproduced by existing energy functionals even in two-dimensional collective spaces. Theory and experiment agree typically within two mass units for the position of the asymmetric peak. As expected, calculations are sensitive to the structure of the initial state and the prescription for the collective inertia. We emphasize that results are also sensitive to the continuity of the collective landscape near scission. Conclusions: Our analysis confirms that the adiabatic approximation provides an effective scheme to compute fission fragment yields. It also suggests that, at least in the framework of nuclear DFT, three-dimensional collective spaces may be a prerequisite to reach 10% accuracy in predicting pre-neutron emission fission fragment yields. C1 [Regnier, D.; Dubray, N.; Verriere, M.] CEA, DAM, DIF, F-91297 Arpajon, France. [Schunck, N.] LLNL, Nucl & Chem Sci Div, Livermore, CA 94551 USA. RP Regnier, D; Dubray, N (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France.; Schunck, N (reprint author), LLNL, Nucl & Chem Sci Div, Livermore, CA 94551 USA. EM david.regnier@cea.fr; noel.dubray@cea.fr; schunck1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Livermore Computing Resource Center at Lawrence Livermore National Laboratory; INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS) at Oak Ridge National Laboratory; INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS) at Oak Ridge National Laboratory (ORNL, USA) FX Part of this research was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Computational resources were provided through an INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences (NCCS) at Oak Ridge National Laboratory (ORNL, USA). Computing resources were also provided through an award by the Livermore Computing Resource Center at Lawrence Livermore National Laboratory. NR 65 TC 1 Z9 1 U1 5 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 13 PY 2016 VL 93 IS 5 AR 054611 DI 10.1103/PhysRevC.93.054611 PG 15 WC Physics, Nuclear SC Physics GA DL9YS UT WOS:000376000000002 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alex, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Andersb, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andreia, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arika, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, A Baasa, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Baia, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE BartosA, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Berlendis, S Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertram, IA Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohma, C Boisvert, V Bolda, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, K Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Broughton, JH De Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, B Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E BScher, D BScher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, M Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairoa, VM Cakira, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Calobaa, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Campoverde, A Canalea, V Canepaa, A Brete, MC Cantero, J Cantrilla, R Cao, T Garrido, MDMC Caprinib, I Caprinib, M Capuaa, M Caputo, R Carbone, RM Cardarellia, R Cardillo, F Carli, T Carlinoa, G Carminatia, L Caron, S Carquina, E Carrillo-Montoya, GD Carter, JR Carvalhoa, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Mirandaa, E Castelli, A Gimenez, VC Castroa, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V 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CA ATLAS Collaboration TI Measurements of W(+/-)Z production cross sections in pp collisions at root s=8 TeV with the ATLAS detector and limits on anomalous gauge boson self-couplings SO PHYSICAL REVIEW D LA English DT Article ID PROTON-PROTON COLLISIONS; HADRON COLLIDERS; WZ PRODUCTION; P(P)OVER-BAR COLLISIONS; ZZ PRODUCTION; HIGGS BOSONS; NNLO QCD; LHC; RECONSTRUCTION; ELECTRON AB This paper presents measurements of W(+/-)Z production in pp collisions at a center-of-mass energy of 8 TeV. The gauge bosons are reconstructed using their leptonic decay modes into electrons and muons. The data were collected in 2012 by the ATLAS experiment at the Large Hadron Collider and correspond to an integrated luminosity of 20.3 fb(-1). The measured inclusive cross section in the detector fiducial region is sigma W(+/-)Z -> l'nu ll = 35.1 +/- 0.9(stat) +/- 0.8(sys) +/- 0.8(lumi) fb, for one leptonic decay channel. In comparison, the next-to-leading-order Standard Model expectation is 30.0 +/- 2.1 fb. Cross sections for W(+)Z and W(-)Z production and their ratio are presented as well as differential cross sections for several kinematic observables. Limits on anomalous triple gauge boson couplings are derived from the transverse mass spectrum of the W(+/-)Z system. From the analysis of events with a W and a Z boson associated with two or more forward jets an upper limit at 95% confidence level on the W(+/-)Z scattering cross section of 0.63 fb, for each leptonic decay channel, is established, while the Standard Model prediction at next-to-leading order is 0.13 +/- 0.01 fb. Limits on anomalous quartic gauge boson couplings are also extracted. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, O.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. 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G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Brete, M. Cano; Guoe, J.; Lie, Q.; Yange, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Brete, M. Cano; Guoe, J.; Lie, Q.; Yange, H.] PKU CHEP, Beijing, Peoples R China. [Chenf, X.; Zhou, N.] Tsinghua Univ, Phys Dept, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairoa, V. M.; Capuaa, M.; Crosettia, G.; La Rotondaa, L.; Mastroberardinoa, A.; Policicchioa, A.; Salvatorea, D.; Scarfonea, V.; Schioppaa, M.; Susinnoa, G.; Tassia, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Cairoa, V. M.; Capuaa, M.; Crosettia, G.; La Rotondaa, L.; Mastroberardinoa, A.; Policicchioa, A.; Salvatorea, D.; Scarfonea, V.; Schioppaa, M.; Susinnoa, G.; Tassia, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bolda, T.; Dabrowskia, W.; Dyndala, M.; Gacha, G. P.; Grabowska-Bolda, I.; Kisielewskaa, D.; Kopernya, S.; Kowalskia, T. Z.; Mindura, B.; Przybyciena, M.; Zemlaa, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palkab, M.; Richter-Wasb, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; De Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, O.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, O.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, X.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; BScher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darboa, G.; Favaretoa, A.; Parodia, A. Ferretto; Gagliardia, G.; Gaudielloa, A.; Gemmea, C.; Guidoa, E.; Morettinia, P.; Osculatia, B.; Parodia, F.; Passaggioa, S.; Rossia, L. P.; Sanninoa, M.; Schiavia, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favaretoa, A.; Parodia, A. Ferretto; Gagliardia, G.; Gaudielloa, A.; Guidoa, E.; Osculatia, B.; Parodia, F.; Sanninoa, M.; Schiavia, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelavaa, J.; Tskhadadzea, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvilib, A.; Khubuab, J.; Mosidzeb, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; De Lima, D. E. Ferreira; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andreia, V.; Baasa, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geislera, M. P.; Hankea, P.; Jongmannsa, J.; Klugea, E-E.; Langa, V. S.; Meiera, K.; Theenhausena, H. Meyer Zu; Villara, I. Narrias; Sahinsoya, M.; Scharfa, V.; Schultz-Coulona, H-C.; Stamena, R.; Starovoitova, P.; Sucheka, S.; Wesselsa, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Andersb, C. F.; Giulinib, M.; Kolbb, M.; Lisovyib, M.; Radescub, V.; Schaetzelb, S.; Schoeningb, A.; Sosab, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Kretzc, M.; Kugelc, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chana, Y. L.; Castilloa, L. R. Flores; Lua, H.; Salvuccia, A.; Tsuia, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlandob, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofievc, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, O.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodinia, G.; Gorinia, E.; Longoa, L.; Primaveraa, M.; Spagnoloa, S.; Venturaa, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bachas, K.; Gorinia, E.; Longoa, L.; Spagnoloa, S.; Venturaa, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Bell, A. S.; Butterworth, M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; BScher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Sch, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, Y.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gaob, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Mm, J. Toth; Touchard, F.; Vacavant, L.; Wangd, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gaob, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Mm, J. Toth; Touchard, F.; Vacavant, L.; Wangd, C.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminatia, L.; Cavallia, D.; Costaa, G.; Fantia, M.; Giugnia, D.; Laria, T.; Lazzaronia, M.; Mandellia, L.; Manzonia, S.; Mazzaa, S. M.; Meronia, C.; Monzania, S.; Perinia, L.; Ragusaa, F.; Rattia, M. G.; Resconia, S.; Shojaiia, S.; Stabilea, A.; Tartarellia, G. F.; Troncona, C.; Turraa, R.; Pereza, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminatia, L.; Fantia, M.; Lazzaronia, M.; Manzonia, S.; Mazzaa, S. M.; Monzania, S.; Perinia, L.; Ragusaa, F.; Rattia, M. G.; Shojaiia, S.; Turraa, R.; Pereza, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F; Azuelos, G.; Dallaire, F.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, L.; Komar, A. A.; Mashinistov, R.; Mouraviev, V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canalea, V.; Carlinoa, G.; Cirottoa, F.; Conventia, F.; Della Pietra, M.; Doria, A.; Izzoa, V.; Merolaa, L.; Perrellaa, S.; Rossia, E.; Sancheza, A.; Sekhniaidzea, G.; Zurzoloa, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canalea, V.; Cirottoa, F.; Merolaa, L.; Perrellaa, S.; Rossia, E.; Sancheza, A.; Zurzoloa, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J-F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, CNRS, LAL,IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Contaa, C.; Dondero, P.; Ferraria, R.; Fraternalia, M.; Gaudioa, G.; Introzzia, G.; Lanzaa, A.; Livana, M.; Negria, A.; Poleselloa, G.; Rebuzzia, D. M.; Rimoldia, A.; Vercesia, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Contaa, C.; Dondero, P.; Fraternalia, M.; Introzzia, G.; Livana, M.; Negria, A.; Rebuzzia, D. M.; Rimoldia, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinnia, V.; Chiarellia, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannettia, P.; Leonea, S.; Rodaa, C.; Scuria, F.; Sotiropouloua, C. L.; Spallaa, M.; Volpia, G.; Whitea, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinnia, V.; Chiarellia, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannettia, P.; Leonea, S.; Rodaa, C.; Scuria, F.; Sotiropouloua, C. L.; Spallaa, M.; Volpia, G.; Whitea, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrilla, R.; Carvalhoa, J.; Castroa, N. F.; Muinoa, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Fiolhaisa, M. C. N.; Galhardoa, B.; Gomesa, A.; Gonaloa, R.; Jorgea, P. M.; Lopesa, L.; Maioa, A.; Maneiraa, J.; Seabraa, L. F. Oleiro; Onofrea, A.; Palmaa, A.; Pedroa, R.; Pinaa, J.; Santosa, H.; Saraivaa, J. G.; Silvaa, J.; Delgadoa, A. Tavares; Velosoa, F.; Woltersa, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muinoa, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Gomesa, A.; Jorgea, P. M.; Miguens, J. Machado; Maioa, A.; Maneiraa, J.; Palmaa, A.; Pedroa, R.; Pinaa, J.; Delgadoa, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalhoa, J.; Fiolhaisa, M. C. N.; Galhardoa, B.; Velosoa, F.; Woltersa, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomesa, A.; Maioa, A.; Pinaa, J.; Saraivaa, J. G.; Silvaa, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofrea, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Aloisio, A.; Chudoba, J.; Havranek, M.; Hejbal, J.; Kepka, O.; Kupco, A.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solovyev, V.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Baines, J. T.; Barnett, B. M.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Kirk, J.; Middleton, R. P.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapettia, G.; Corradia, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falcianoa, S.; Gentilea, S.; Giagua, S.; Gustavinoa, G.; Kunaa, M.; Lacavaa, F.; Lucia, C.; Luminaria, L.; Marzanoa, F.; Messinaa, A.; Nisatia, A.; Pasqualuccia, E.; Petroloa, E.; Pontecorvoa, L.; Rescignoa, M.; Rosatia, S.; Tehrania, F. Safai; Vanadiaa, M.; Varia, R.; Venezianoa, S.; Verduccia, M.; Zanelloa, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapettia, G.; Corradia, M.; Di Domenico, A.; Di Donato, C.; Gentilea, S.; Giagua, S.; Gustavinoa, G.; Kunaa, M.; Lacavaa, F.; Lucia, C.; Messinaa, A.; Vanadiaa, M.; Verduccia, M.; Zanelloa, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarellia, R.; Di Ciaccio, A.; Iuppaa, R.; Libertia, B.; Salamona, A.; Santonicoa, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppaa, R.; Salamona, A.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradinia, F.; Di Micco, B.; Farillaa, A.; Graziania, E.; Iodicea, M.; Orestanoa, D.; Pastorea, F.; Petruccia, F.; Puddua, D.; Salamannaa, G.; Sessaa, M.; Stanescua, C.; Taccinia, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradinia, F.; Di Micco, B.; Orestanoa, D.; Pastorea, F.; Petruccia, F.; Puddua, D.; Salamannaa, G.; Sessaa, M.; Taccinia, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaqa, A.; Hoummadaa, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlaneb, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimic, M.; Goujdamic, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrifd, M.; Tayalatid, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrifd, M.; Tayalatid, Y.] LPTPM, Oujda, Morocco. [El Mourslie, R. Cherkaoui; Fassie, F.; Haddade, N.; Idrissie, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Denysiuk, D.; Etienvre, A. I.; Formica, A.; Guyot, C.; Lanon, E.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Ouraou, A.; Peyaud, A.; Royon, C. R.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liao, H.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Liang, Z.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Bawa, H. S.; Black, J. E.; Garelli, N.; Kocian, M.; Malone, C.; Moss, J.; Nachman, B. P.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; BartosA, P.; Blazek, T.; Plazaka, L.; Sykoraa, I.; Tokara, S.; Zenisa, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladivab, E.; Strizenecb, P.; Urbanb, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Mirandaa, E.; Hamiltona, A.; Yacooba, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connellb, S. H.; Govenderb, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsuc, C.; Karc, D.; Garciac, B. R. Mellado; Ruanc, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bohma, C.; Clementa, C.; Jon-Anda, K.; Khandanyana, H.; Milsteada, D. A.; Shaikha, N. W.; Shcherbakovaa, A.; Sjolina, J.; Tylmada, M.; Ughettoa, M.; Santurioa, E. Valdes] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clementa, C.; Hellmana, S.; Jon-Anda, K.; Khandanyana, H.; Klimeka, P.; Lundberga, O.; Milsteada, D. A.; Pania, P.; Plucinskia, P.; Poettgena, R.; Shaikha, N. 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J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Bb, S. C. Lin; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Hh, L. Shi; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; Van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Hanawa, K.; Kanaya, N.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Mashimo, T.; Masubuchi, T.; Mori, T.; Morinaga, M.; Nakamura, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Hanawa, K.; Kanaya, N.; Kato, C.; Kazama, S.; Kobayashi, A.; Morinaga, M.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Canepaa, A.; Chekulaeva, S. V.; Jovicevica, J.; Koutsmana, A.; Orama, C. J.; Codinaa, E. Perez; Schneidera, B.; Schoutena, D.; Seustera, R.; Stelzer-Chiltona, O.; Tafirouta, R.; Triggera, I. 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P.; Pinamontia, M.; Serkina, L.; Shawa, K.; Truonga, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quaylea, W. B.; Serkina, L.; Shawa, K.; Truonga, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobala, M.; Giordania, M. P.; Miglioranzia, S.; Pinamontia, M.; Soualaha, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Ellert, M.; Ferrari, A.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Piqueras, D. Alvarez; Ferrer, A.; Fuster, J.; Garcia, C.; Higon-Rodriguez, E.; Quiles, A. Irles; Lacasta, C.; Rodriguez, D. 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[Jenni, P.] CERN, CH-1211 Geneva 23, Switzerland. [Khubuab, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.; Nagai, R.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Aa, B. Lib; Song, H. Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Bb, S. C. Lin] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Ee, M. Nessi] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamontia, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Hh, L. Shi; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Mm, J. Toth] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Oo, I. Yusuff] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. [Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] CNRS, IN2P3, Marseille, France. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Prokoshin, Fedor/E-2795-2012; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Monzani, Simone/D-6328-2017; Gladilin, Leonid/B-5226-2011; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Mitsou, Vasiliki/D-1967-2009; Lazzaroni, Massimo/N-3675-2015; Casado, Pilar/H-1484-2015; Guo, Jun/O-5202-2015; BESSON, NATHALIE/L-6250-2015; Warburton, Andreas/N-8028-2013; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Doyle, Anthony/C-5889-2009 OI Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Prokoshin, Fedor/0000-0001-6389-5399; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Monzani, Simone/0000-0002-0479-2207; Gladilin, Leonid/0000-0001-9422-8636; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Mitsou, Vasiliki/0000-0002-1533-8886; Lazzaroni, Massimo/0000-0002-4094-1273; Casado, Pilar/0000-0002-0394-5646; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Doyle, Anthony/0000-0001-6322-6195 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020 and Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales and Aristeia programmes - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 88 TC 4 Z9 4 U1 21 U2 58 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 13 PY 2016 VL 93 IS 9 AR 092004 DI 10.1103/PhysRevD.93.092004 PG 36 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM0AQ UT WOS:000376005200001 ER PT J AU Friddle, RW AF Friddle, Raymond W. TI Analytic descriptions of stochastic bistable systems under force ramp SO PHYSICAL REVIEW E LA English DT Article ID MECHANICAL FORCE; MOLECULES; BONDS; MODEL AB Solving the two-state master equation with time-dependent rates, the ubiquitous driven bistable system, is a long-standing problem that does not permit a complete solution for all driving rates. Here we show an accurate approximation to this problem by considering the system in the control parameter regime. The results are immediately applicable to a diverse range of bistable systems including single-molecule mechanics. C1 [Friddle, Raymond W.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Friddle, RW (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. FU Sandia Laboratory Directed Research and Development Program; U.S. Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX This work was supported by the Sandia Laboratory Directed Research and Development Program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a Lockheed-Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DEAC04-94AL85000. NR 14 TC 0 Z9 0 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 13 PY 2016 VL 93 IS 5 AR 052126 DI 10.1103/PhysRevE.93.052126 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DM0CH UT WOS:000376009700003 PM 27300849 ER PT J AU Kimball, DFJ Sushkov, AO Budker, D AF Kimball, Derek F. Jackson Sushkov, Alexander O. Budker, Dmitry TI Precessing Ferromagnetic Needle Magnetometer SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRIC-DIPOLE MOMENT; SPIN-WAVE EXCITATIONS; SINGLE-DOMAIN; MAGNETIZATION REVERSAL; SURFACE-RESISTANCE; FLUCTUATIONS; FIELDS; NOISE; SUPERCONDUCTORS; ENTANGLEMENT AB A ferromagnetic needle is predicted to precess about the magnetic field axis at a Larmor frequency Omega under conditions where its intrinsic spin dominates over its rotational angular momentum, Nh >> I Omega (I is the moment of inertia of the needle about the precession axis and N is the number of polarized spins in the needle). In this regime the needle behaves as a gyroscope with spin Nh maintained along the easy axis of the needle by the crystalline and shape anisotropy. A precessing ferromagnetic needle is a correlated system of N spins which can be used to measure magnetic fields for long times. In principle, by taking advantage of rapid averaging of quantum uncertainty, the sensitivity of a precessing needle magnetometer can far surpass that of magnetometers based on spin precession of atoms in the gas phase. Under conditions where noise from coupling to the environment is subdominant, the scaling with measurement time t of the quantum-and detection-limited magnetometric sensitivity is t(-3/2). The phenomenon of ferromagnetic needle precession may be of particular interest for precision measurements testing fundamental physics. C1 [Kimball, Derek F. Jackson] Calif State Univ East Bay, Dept Phys, Hayward, CA 94542 USA. [Sushkov, Alexander O.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Budker, Dmitry] Johannes Gutenberg Univ Mainz, Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Budker, Dmitry] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, Dmitry] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Kimball, DFJ (reprint author), Calif State Univ East Bay, Dept Phys, Hayward, CA 94542 USA. FU Heising-Simons Foundation; Simons Foundation; National Science Foundation [PHY-1307507]; Mainz Institute for Theoretical Physics (MITP) FX The authors are sincerely grateful to Eugene Commins, Max Zolotorev, Erwin Hahn, Marcis Auzinsh, Alex Zettl, Michael Crommie, Oleg Sushkov, Victor Flambaum, Mikhail Kozlov, John Clarke, Lutz Trahms, Kathryn A. Moler, Szymon Pustelny, Holger Muller, Jennie Guzman, Jason Singley, Erik Helgren, Nathan Leefer, Hunter Richards, Surjeet Rajendran, Amir Yacobi, Mikhail Lukin, and Asimina Arvanitaki for enlightening discussions. This work was supported by the Heising-Simons Foundation, the Simons Foundation, and the National Science Foundation under Grant No. PHY-1307507. The authors are grateful to the Mainz Institute for Theoretical Physics (MITP) for its hospitality and its partial support during the completion of this work. NR 89 TC 1 Z9 1 U1 7 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2016 VL 116 IS 19 AR 190801 DI 10.1103/PhysRevLett.116.190801 PG 7 WC Physics, Multidisciplinary SC Physics GA DM0EB UT WOS:000376014500002 PM 27232012 ER PT J AU Mou, DX Sapkota, A Kung, HH Krapivin, V Wu, Y Kreyssig, A Zhou, XJ Goldman, AI Blumberg, G Flint, R Kaminski, A AF Mou, Daixiang Sapkota, A. Kung, H-H Krapivin, Viktor Wu, Yun Kreyssig, A. Zhou, Xingjiang Goldman, A. I. Blumberg, G. Flint, Rebecca Kaminski, Adam TI Discovery of an Unconventional Charge Density Wave at the Surface of K0.9Mo6O17 SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRANSITION-METAL DICHALCOGENIDES; PURPLE BRONZE K0.9MO6O17; T-C; DEPENDENT SUPERCONDUCTIVITY; RAMAN-SCATTERING; ORDER; INSTABILITY; BI2SR2CACU2O8+DELTA; CONNECTION; POTASSIUM AB We use angle resolved photoemission spectroscopy, Raman spectroscopy, low energy electron diffraction, and x-ray scattering to reveal an unusual electronically mediated charge density wave (CDW) in K0.9Mo6O17. Not only does K0.9Mo6O17 lack signatures of electron-phonon coupling, but it also hosts an extraordinary surface CDW, with T-S_CDW = 220 K nearly twice that of the bulk CDW, T-B_CDW = 115 K. While the bulk CDW has a BCS-like gap of 12 meV, the surface gap is 10 times larger and well in the strong coupling regime. Strong coupling behavior combined with the absence of signatures of strong electron-phonon coupling indicates that the CDW is likely mediated by electronic interactions enhanced by low dimensionality. C1 [Mou, Daixiang; Sapkota, A.; Wu, Yun; Kreyssig, A.; Goldman, A. I.; Flint, Rebecca; Kaminski, Adam] US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. [Mou, Daixiang; Sapkota, A.; Wu, Yun; Kreyssig, A.; Goldman, A. I.; Flint, Rebecca; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Kung, H-H; Krapivin, Viktor; Blumberg, G.] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. [Zhou, Xingjiang] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Natl Lab Superconduct, Beijing 100190, Peoples R China. [Blumberg, G.] NICPB, EE-12618 Tallinn, Estonia. RP Mou, DX; Kaminski, A (reprint author), US DOE, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA.; Mou, DX; Kaminski, A (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM moudaixiang@gmail.com; kaminski@ameslab.gov RI Kung, Hsiang-Hsi/R-4949-2016; Flint, Rebecca/J-3628-2014 OI Kung, Hsiang-Hsi/0000-0002-2835-3196; FU Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; DOE Office of Science [DE-AC02-06CH11357]; National Science Foundation [NSF DMR-1104884]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0005463] FX We gratefully acknowledge discussion with Steve Kivelson, Patrick Lee, Mike Norman, and Mohit Randeria. Work at the Ames Laboratory was supported by the Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-07CH11358 (ARPES measurements). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357 (x-ray scattering measurements). Work at Rutgers was supported by the National Science Foundation under Grant No. NSF DMR-1104884 (Raman measurements). G. B. acknowledges support from the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-SC0005463 (interpretation of material behavior and reconciling information from various techniques). NR 65 TC 2 Z9 2 U1 12 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2016 VL 116 IS 19 AR 196401 DI 10.1103/PhysRevLett.116.196401 PG 6 WC Physics, Multidisciplinary SC Physics GA DM0EB UT WOS:000376014500004 PM 27232028 ER PT J AU Wang, QS Park, JT Feng, Y Shen, Y Hao, YQ Pan, BY Lynn, JW Ivanov, A Chi, SX Matsuda, M Cao, HB Birgeneau, RJ Efremov, DV Zhao, J AF Wang, Qisi Park, J. T. Feng, Yu Shen, Yao Hao, Yiqing Pan, Bingying Lynn, J. W. Ivanov, A. Chi, Songxue Matsuda, M. Cao, Huibo Birgeneau, R. J. Efremov, D. V. Zhao, Jun TI Transition from Sign-Reversed to Sign-Preserved Cooper-Pairing Symmetry in Sulfur-Doped Iron Selenide Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID UNCONVENTIONAL SUPERCONDUCTORS; KXFE2-YSE2; GAP AB An essential step toward elucidating the mechanism of superconductivity is to determine the sign or phase of the superconducting order parameter, as it is closely related to the pairing interaction. In conventional superconductors, the electron-phonon interaction induces attraction between electrons near the Fermi energy and results in a sign-preserved s-wave pairing. For high-temperature superconductors, including cuprates and iron-based superconductors, prevalent weak coupling theories suggest that the electron pairing is mediated by spin fluctuations which lead to repulsive interactions, and therefore that a sign-reversed pairing with an s(+/-) or d-wave symmetry is favored. Here, by using magnetic neutron scattering, a phase sensitive probe of the superconducting gap, we report the observation of a transition from the sign-reversed to sign-preserved Cooper-pairing symmetry with insignificant changes in T-c in the S-doped iron selenide superconductors KxFe2-y(Se1-zSz)(2). We show that a rather sharp magnetic resonant mode well below the superconducting gap (2 Delta) in the undoped sample (z = 0) is replaced by a broad hump structure above 2 Delta under 50% S doping. These results cannot be readily explained by simple spin fluctuation-exchange pairing theories and, therefore, multiple pairing channels are required to describe superconductivity in this system. Our findings may also yield a simple explanation for the sometimes contradictory data on the sign of the superconducting order parameter in iron-based materials. C1 [Wang, Qisi; Feng, Yu; Shen, Yao; Hao, Yiqing; Pan, Bingying; Zhao, Jun] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Wang, Qisi; Feng, Yu; Shen, Yao; Hao, Yiqing; Pan, Bingying; Zhao, Jun] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Park, J. T.] Tech Univ Munich, Heinz Maier Leibnitz Zentrum MLZ, D-85748 Garching, Germany. [Lynn, J. W.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Ivanov, A.] Inst Laue Langevin, 71 Ave Martyrs, F-38042 Grenoble 9, France. [Chi, Songxue; Matsuda, M.; Cao, Huibo] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Efremov, D. V.] IFW Dresden, Helmholtzstr 20, D-01069 Dresden, Germany. [Zhao, Jun] Fudan Univ, Collaborat Innovat Ctr Adv Microstruct, Shanghai 200433, Peoples R China. RP Zhao, J (reprint author), Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.; Zhao, J (reprint author), Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China.; Park, JT (reprint author), Tech Univ Munich, Heinz Maier Leibnitz Zentrum MLZ, D-85748 Garching, Germany.; Zhao, J (reprint author), Fudan Univ, Collaborat Innovat Ctr Adv Microstruct, Shanghai 200433, Peoples R China. EM jitae.park@frm2.tum.de; zhaoj@fudan.edu.cn RI Matsuda, Masaaki/A-6902-2016; Zhao, Jun/A-2492-2010; Park, Jitae/G-1358-2016; Chi, Songxue/A-6713-2013; Efremov, Dmitri/M-4393-2014 OI Matsuda, Masaaki/0000-0003-2209-9526; Zhao, Jun/0000-0002-0421-8934; Park, Jitae/0000-0001-6565-0192; Chi, Songxue/0000-0002-3851-9153; FU National Natural Science Foundation of China [11374059]; Ministry of Science and Technology of China [2015CB921302]; U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231, DE-AC03-76SF008] FX We thank D. L. Feng and X. H. Niu for helpful discussions. This work is supported by the National Natural Science Foundation of China (No. 11374059) and the Ministry of Science and Technology of China (973 project: 2015CB921302). Use of the high flux isotope reactor at the Oak Ridge National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division. The research at UC Berkeley is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contracts No. DE-AC02-05CH11231 and No. DE-AC03-76SF008. NR 43 TC 1 Z9 1 U1 20 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 13 PY 2016 VL 116 IS 19 AR 197004 DI 10.1103/PhysRevLett.116.197004 PG 5 WC Physics, Multidisciplinary SC Physics GA DM0EB UT WOS:000376014500006 PM 27232038 ER PT J AU Liu, X Hou, GL Wang, XF Wang, XB AF Liu, Xing Hou, Gao-Lei Wang, Xuefeng Wang, Xue-Bin TI Negative Ion Photoelectron Spectroscopy Reveals Remarkable Noninnocence of Ligands in Nickel Bis(dithiolene) Complexes [Ni(dddt)(2)](-) and [Ni(edo)(2)](-) SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CARBON-MONOXIDE DEHYDROGENASE; AB-INITIO PSEUDOPOTENTIALS; METAL-DITHIOLENE COMPLEXES; DENSITY-FUNCTIONAL THEORY; ELECTRONIC-STRUCTURE; GAS-PHASE; TOPOLOGICAL INSULATOR; REDUCTION POTENTIALS; TRANSITION-ELEMENTS; ACETYL-COENZYME AB [Ni(dddt)(2)](-) (dddt = 5,6-dihydro-1,4-dithiine-2,3-dithiolate) and [Ni(edo)(2)](-) (edo = 5,6-dihydro-1,4-dioxine-2,3-dithiolate) are two donor-type nickel bis(dithiolene) complexes, with the tendency of donating low binding energy electrons. These two structurally similar complexes differ only with respect to the outer atoms in the ligand framework where the former has four S atoms while the latter has four O atoms. Herein, we report a negative ion photoelectron spectroscopy (NIPES) study on these two complexes to probe the electronic structures of the anions and their corresponding neutrals. The NIPE spectra exhibit the adiabatic electron detachment energy (ADE) or, equivalently, the electron affinity (EA) of the neutral [Ni(L)(2)](0) to be relatively low for this type of complexes, 2.780 and 2.375 eV for L = dddt and edo, respectively. The 0.4 eV difference in ADEs shows a significant substitution effect for sulfur in dddt by oxygen in edo, i.e., noninnocence of the ligands, which has decreased the electronic stability of [Ni(edo)(2)](-) by lowering its electron binding energy by similar to 0.4 eV. The observed substitution effect on gas-phase EA values correlates well with the measured redox potentials for [Ni(dddt)(2)](-/0) and [Ni(edo)(2)](-/0) in solutions. The singlet-triplet splitting (Delta E-ST) of [Ni(dddt)(2)](0) and [Ni(edo)(2)](0) is also determined from the spectra to be 0.57 and 0.53 eV, respectively. Accompanying DFT calculations and molecular orbital (MO) composition analyses show significant ligand contributions to the redox MOs and allow the components of the orbitals involved in each electronic transition and spectral assignments to be identified. C1 [Liu, Xing] Southwest Univ, Coll Chem & Chem Engn, Chongqing 400715, Peoples R China. [Hou, Gao-Lei; Wang, Xue-Bin] Pacific NW Natl Lab, Phys Sci Div, POB 999,MS K8-88, Richland, WA 99352 USA. [Liu, Xing; Wang, Xuefeng] Tongji Univ, Dept Chem, Shanghai 200092, Peoples R China. RP Wang, XB (reprint author), Pacific NW Natl Lab, Phys Sci Div, POB 999,MS K8-88, Richland, WA 99352 USA.; Wang, XF (reprint author), Tongji Univ, Dept Chem, Shanghai 200092, Peoples R China. EM xfwang@tongji.edu.cn; xuebin.wang@pnnl.gov FU Fundamental Research Funds for the Central Universities [XDJK2016C030, SWU115072]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE's Office of Biological and Environmental Research; ministry of Science and Technology of China [2012YQ220113-7] FX This work was supported by Fundamental Research Funds for the Central Universities (Grant No. XDJK2016C030 and SWU115072) and by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. The experimental work was performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the DOE. The theoretical calculations were conducted on Rockscluster of Tongji University. X.-F.W is grateful for support from the ministry of Science and Technology of China (No. 2012YQ220113-7) NR 51 TC 0 Z9 0 U1 17 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2016 VL 120 IS 18 BP 2854 EP 2862 DI 10.1021/acs.jpca.6b02711 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL9NA UT WOS:000375968800009 PM 27099986 ER PT J AU Fedorov, DA Pruitt, SR Keipert, K Gordon, MS Varganov, SA AF Fedorov, Dmitry A. Pruitt, Spencer R. Keipert, Kristopher Gordon, Mark S. Varganov, Sergey A. TI Ab Initio Multiple Spawning Method for Intersystem Crossing Dynamics: Spin-Forbidden Transitions between 3B(1) and (1)A(1) States of GeH2 SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID QUANTUM MOLECULAR-DYNAMICS; ELECTRONIC-TRANSITIONS; KINETICS; PHOTOCHEMISTRY; VALIDATION; ETHYLENE; XANTHONE; PACKAGE; TRIPLET; MOLPRO AB Dynamics at intersystem crossings are fundamental to many processes in chemistry, physics, and biology. The ab initio multiple spawning (AIMS) method was originally developed to describe internal conversion dynamics at conical intersections where derivative coupling is responsible for nonadiabatic transitions between electronic states with the same spin multiplicity. Here, the applicability of the AIMS method is extended to intersystem crossing dynamics in which transitions between electronic states with different spin multiplicities are mediated by relativistic spin orbit coupling. In the direct AIMS dynamics, the nuclear wave function is expanded in the basis of frozen multidimensional Gaussians propagating on the coupled electronic potential energy surfaces calculated on the fly. The AIMS method for intersystem crossing is used to describe the nonadiabatic transitions between the B-3(1) and (1)A(1) states of GeH2. The potential energies and gradients were obtained at the CASSCF(6,6)/6-31G(d) level of theory. The spin orbit coupling matrix elements were calculated with the configuration interaction method using the two electron Breit Pauli Hamiltonian. The excited B-3(1) state lifetime and intersystem crossing rate constants were estimated by fitting the AIMS state population with the first-order kinetics equation for a reversible unimolecular reaction. The obtained rate constants are compared with the values predicted by the statistical nonadiabatic transition state theory with transition probabilities calculated using the Landau-Zener and weak coupling formulas. C1 [Fedorov, Dmitry A.; Varganov, Sergey A.] Univ Nevada, Dept Chem, 1664 North Virginia St, Reno, NV 89557 USA. [Pruitt, Spencer R.] Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Lemont, IL 60439 USA. [Keipert, Kristopher; Gordon, Mark S.] Iowa State Univ, Dept Chem, Ames Lab, Ames, IA 50010 USA. RP Varganov, SA (reprint author), Univ Nevada, Dept Chem, 1664 North Virginia St, Reno, NV 89557 USA. EM svarganov@unr.edu FU University of Nevada, Reno; Air Force Office of Scientific Research CoDesign grant, under AFOSR [FA9550-12-1-0476]; Office of Science, U.S. Department of Energy [DE-AC02-06CH113.57] FX D.A.F. and S.A.V. thank Profs. Benjamin Levine and Todd Martinez for fruitful discussions, and the University of Nevada, Reno, for financial support. M.S.G. and K.K. acknowledge support from an Air Force Office of Scientific Research CoDesign grant, under AFOSR Award No. FA9550-12-1-0476. S.R.P. was supported by the Office of Science, U.S. Department of Energy, under Contract DE-AC02-06CH113.57. NR 65 TC 4 Z9 4 U1 2 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 12 PY 2016 VL 120 IS 18 BP 2911 EP 2919 DI 10.1021/acs.jpca.6b01406 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL9NA UT WOS:000375968800016 PM 27064356 ER PT J AU Larsen, RE AF Larsen, Ross E. TI Simple Extrapolation Method To Predict the Electronic Structure of Conjugated Polymers from Calculations on Oligomers SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FIELD-EFFECT TRANSISTORS; LIGHT-EMITTING DEVICES; DENSITY-OF-STATES; ORGANIC PHOTOVOLTAICS; SOLAR-CELLS; THEORETICAL INVESTIGATIONS; RATIONAL DESIGN; COPOLYMERS; ENERGY; DONOR AB We introduce two simple tight-binding models, which we call fragment frontier orbital extrapolations (FFOE), to extrapolate important electronic properties to the polymer limit using electronic structure calculations on only a few small oligomers. In particular, we demonstrate by comparison to explicit density functional theory calculations that for long oligomers the energies of the highest occupied molecular orbital (HOMO), the lowest unoccupied molecular orbital (LUMO), and of the first electronic excited state are accurately described as a function of number of repeat units by a simple effective Hamiltonian parametrized from electronic structure calculations on monomers, dimers and, optionally, tetramers. For the alternating copolymer materials that currently comprise some of the most efficient polymer organic photovoltaic devices one can use these simple but rigorous models to extrapolate computed properties to the polymer limit based on calculations on a small number of low-molecular-weight oligomers. C1 [Larsen, Ross E.] Computat Sci Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Larsen, RE (reprint author), Computat Sci Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. EM ross.larsen@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory through the DOE SETP program; Department of Energy's Office of Energy Efficiency and Renewable Energy at the National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory through the DOE SETP program. The research was performed using resources sponsored by the Department of Energy's Office of Energy Efficiency and Renewable Energy, located at the National Renewable Energy Laboratory. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 57 TC 3 Z9 3 U1 0 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2016 VL 120 IS 18 BP 9650 EP 9660 DI 10.1021/acs.jpcc.6b02138 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL9NC UT WOS:000375969000013 ER PT J AU Mane, AU Allen, AJ Kanjolia, RK Elam, JW AF Mane, Anil U. Allen, Amy J. Kanjolia, Ravindra K. Elam, Jeffrey W. TI Indium Oxide Thin Films by Atomic Layer Deposition Using Trimethylindium and Ozone SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID QUARTZ-CRYSTAL MICROBALANCE; SENSITIZED SOLAR-CELLS; VAPOR-PHASE EPITAXY; OPTICAL-PROPERTIES; IN2O3 FILMS; CYCLOPENTADIENYL INDIUM; GAS SENSORS; INN GROWTH; WATER; TRANSISTORS AB We investigated the atomic layer deposition (ALD) of indium oxide (In2O3) thin films using alternating exposures of trimethylindium (TMIn) and a variety of oxygen sources: ozone (O-3), O-2, deionized H2O, and hydrogen peroxide (H2O2). We used in situ quartz crystal microbalance measurements to evaluate the effectiveness of the different oxygen sources and found that only O-3 yielded viable and sustained 111203 growth with TMIn. These measurements also provided details about the In2O3 growth mechanism and enabled us to verify that both the TMIn and O-3 surface reactions were self-limiting. In2O3 thin films were prepared and characterized using X-ray diffraction, ultraviolet visible spectrophotometry, spectroscopic ellipsometry, X-ray photoelectron spectroscopy, and scanning electron microscopy. The electrical transport properties of these layers were studied by Hall probe measurements. We found that, at deposition temperatures within the range of 100-200 degrees C, the In2O3 growth per cycle was nearly constant at 0.46 angstrom/cycle and the films were dense and pure. The film thickness was highly uniform (<0.3% variation) along the 45 cm length of our tubular ALD reactor. At higher growth temperatures the In2O3 growth per cycle increased due to thermal decomposition of the TMIn. The ALD In2O3 films showed resistivities as low as 3.2 x 10(-3) Omega cm, and carrier concentrations as large as 7.0 x 10(19) cm(-3). This TMIn/O-3 process for In2O3 ALD should be suitable for eventual scale-up in photovoltaics. C1 [Mane, Anil U.; Allen, Amy J.; Elam, Jeffrey W.] Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60439 USA. [Kanjolia, Ravindra K.] SAFC Hitech, 1429 Hilldale Ave, Haverhill, MA 01832 USA. RP Elam, JW (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60439 USA. EM jelam@anl.gov FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Solar Energy Technologies Office; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Solar Energy Technologies Office. We thank Dr. Qing Peng (Duke University) for performing the XPS measurements. Use of the Center for Nanoscale Materials, including resources in the Electron Microscopy Center, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 79 TC 2 Z9 2 U1 17 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 12 PY 2016 VL 120 IS 18 BP 9874 EP 9883 DI 10.1021/acs.jpcc.6b02657 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL9NC UT WOS:000375969000037 ER PT J AU Koch, A Maia, A Janssen, A Medema, RH AF Koch, A. Maia, A. Janssen, A. Medema, R. H. TI Molecular basis underlying resistance to Mps1/TTK inhibitors SO ONCOGENE LA English DT Article ID SPINDLE-ASSEMBLY CHECKPOINT; PROTEIN-KINASES; MITOTIC CHECKPOINT; MYELOID-LEUKEMIA; DRUG-RESISTANCE; AURORA KINASES; CANCER-THERAPY; BCR-ABL; CELLS; KINETOCHORES AB Mps1/TTK is a dual-specificity kinase, with an essential role in mitotic checkpoint signaling, which has emerged as a potential target in cancer therapy. Several Mps1/TTK small-molecule inhibitors have been described that exhibit promising activity in cell culture and xenograft models. Here, we investigated whether cancer cells can develop resistance to these drugs. To this end, we treated various cancer cell lines with sublethal concentrations of a potent Mps1/TTK inhibitor in order to isolate inhibitor-resistant monoclonal cell lines. We identified four point mutations in the catalytic domain of Mps1/TTK that gave rise to inhibitor resistance but retained wildtype catalytic activity. Interestingly, cross-resistance of the identified mutations to other Mps1/TTK inhibitors is limited. Our studies predict that Mps1/TTK inhibitor-resistant tumor cells can arise through the acquisition of mutations in the adenosine triphosphate-binding pocket of the kinase that prevent stable binding of the inhibitors. In addition, our results suggest that combinations of inhibitors could be used to prevent acquisition of drug resistance. Interestingly, cross-resistance seems nonspecific for inhibitor scaffolds, a notion that can be exploited in future drug design to evict possible resistance mutations during clinical treatment. C1 [Koch, A.; Maia, A.; Janssen, A.; Medema, R. H.] Netherlands Canc Inst, Div Cell Biol, Plesmanlaan 121, NL-1066 CX Amsterdam, Netherlands. [Janssen, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. RP Medema, RH (reprint author), Netherlands Canc Inst, Div Cell Biol, Plesmanlaan 121, NL-1066 CX Amsterdam, Netherlands. EM r.medema@nki.nl FU NWO Gravitation Program (Cancer Genomics Center, CGC.nl); EMBO long-term fellowship [ALTF-425-2013] FX We thank Geert Kops (UMC Utrecht, The Netherlands) Susanne Lens (UMC Utrecht, The Netherlands) and Anastassis Perrakis (NKI, Amsterdam, The Netherlands) for reagents. Roos Klop, Yoshitaka Hiruma and Mathijs Vleugel for technical help. Bram van den Broek (NKI, Amsterdam, The Netherlands) for providing the ImageJ analysis macro for mitotic index analysis. We thank our colleagues for support and helpful suggestions. The research was funded by the NWO Gravitation Program (Cancer Genomics Center, CGC.nl). AK was supported by an EMBO long-term fellowship (ALTF-425-2013). NR 43 TC 9 Z9 9 U1 2 U2 3 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0950-9232 EI 1476-5594 J9 ONCOGENE JI Oncogene PD MAY 12 PY 2016 VL 35 IS 19 BP 2518 EP 2528 DI 10.1038/onc.2015.319 PG 11 WC Biochemistry & Molecular Biology; Oncology; Cell Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Oncology; Cell Biology; Genetics & Heredity GA DM2GQ UT WOS:000376165500010 PM 26364596 ER PT J AU Rescigno, TN Trevisan, CS Orel, AE Slaughter, DS Adaniya, H Belkacem, A Weyland, M Dorn, A McCurdy, CW AF Rescigno, T. N. Trevisan, C. S. Orel, A. E. Slaughter, D. S. Adaniya, H. Belkacem, A. Weyland, Marvin Dorn, Alexander McCurdy, C. W. TI Dynamics of dissociative electron attachment to ammonia SO PHYSICAL REVIEW A LA English DT Article ID ABSOLUTE CROSS-SECTIONS; WAVE-FUNCTIONS; BASIS-SETS; NH3; SPECTROSCOPY; SCATTERING; EXCITATION; COLLISIONS; MOLECULES; IMPACT AB Ab initio theoretical studies and momentum-imaging experiments are combined to provide a consistent picture of the dynamics of dissociative electron attachment to ammonia through its 5.5- and 10.5-eV resonance channels. The present study clarifies the character and symmetry of the anion states involved and the dynamics that leads to the observed fragment-ion channels, their branching ratios, and angular distributions. C1 [Rescigno, T. N.; Slaughter, D. S.; Adaniya, H.; Belkacem, A.; McCurdy, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA. [Trevisan, C. S.] Calif Maritime Acad, Dept Sci & Math, Vallejo, CA 94590 USA. [Orel, A. E.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Weyland, Marvin] Phys Tech Bundesanstalt, D-38116 Braunschweig, Germany. [Weyland, Marvin; Dorn, Alexander] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [McCurdy, C. W.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. RP Rescigno, TN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA. FU USDOE by LBNL [DE-AC02-05CH11231]; U.S. DOE, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP) FX This work was performed under the auspices of the USDOE by LBNL under Contract No. DE-AC02-05CH11231 and was supported by the U.S. DOE, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. This work was also supported in part by the U.S. DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP). NR 39 TC 4 Z9 4 U1 4 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAY 12 PY 2016 VL 93 IS 5 AR 052704 DI 10.1103/PhysRevA.93.052704 PG 10 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DL9UV UT WOS:000375989400005 ER PT J AU Hayami, S Lin, SZ Batista, CD AF Hayami, Satoru Lin, Shi-Zeng Batista, Cristian D. TI Bubble and skyrmion crystals in frustrated magnets with easy-axis anisotropy SO PHYSICAL REVIEW B LA English DT Article ID RARE-EARTH METALS; NEUTRON-DIFFRACTION; PHASE; MODEL; ANTIFERROMAGNETISM; FERROMAGNETISM; LATTICE; STATES AB We clarify the conditions for the emergence of multiple-Qstructures out of lattice and easy-axis spin anisotropy in frustrated magnets. By considering magnets whose exchange interaction has multiple global minima in momentum space, we find that both types of anisotropy stabilize triple-Q orderings. Moderate anisotropy leads to a magnetic-field-induced skyrmion crystal, which evolves into a bubble crystal for increasing spatial and spin anisotropy. The bubble crystal exhibits a quasicontinuous (devil's staircase) temperature-dependent ordering wave vector, characteristic of the competition between frustrated exchange and strong easy-axis anisotropy. C1 [Hayami, Satoru; Lin, Shi-Zeng; Batista, Cristian D.] Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA. [Hayami, Satoru; Lin, Shi-Zeng; Batista, Cristian D.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. [Hayami, Satoru] Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. [Batista, Cristian D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Batista, Cristian D.] Oak Ridge Natl Lab, Shull Wollan Ctr, Oak Ridge, TN 37831 USA. RP Hayami, S (reprint author), Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA.; Hayami, S (reprint author), Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA.; Hayami, S (reprint author), Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016 OI Lin, Shi-Zeng/0000-0002-4368-5244; FU National Nuclear Security Administration of the US DOE at LANL [DE-AC52-06NA25396]; LANL LDRD-DR Program FX Computer resources for numerical calculations were supported by the Institutional Computing Program at LANL. This work was carried out under the auspices of the National Nuclear Security Administration of the US DOE at LANL under Contract No. DE-AC52-06NA25396 and was supported by the LANL LDRD-DR Program. NR 36 TC 5 Z9 5 U1 11 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2016 VL 93 IS 18 AR 184413 DI 10.1103/PhysRevB.93.184413 PG 8 WC Physics, Condensed Matter SC Physics GA DL9VZ UT WOS:000375992700005 ER PT J AU Zhao, LS Yelland, EA Bruin, JAN Sheikin, I Canfield, PC Fritsch, V Sakai, H Mackenzie, AP Hicks, CW AF Zhao, Lishan Yelland, Edward A. Bruin, Jan A. N. Sheikin, Ilya Canfield, Paul C. Fritsch, Veronika Sakai, Hideaki Mackenzie, Andrew P. Hicks, Clifford W. TI Field-temperature phase diagram and entropy landscape of CeAuSb2 SO PHYSICAL REVIEW B LA English DT Article ID PRESSURE-INDUCED SUPERCONDUCTIVITY; QUANTUM CRITICALITY; MAGNETIC-PROPERTIES; SINGLE-CRYSTALS; TRANSITION; CERU2SI2; GROWTH; CERH2SI2; ALLOYS AB We report a field-temperature phase diagram and an entropy map for the heavy-fermion compound CeAuSb2. CeAuSb2 orders antiferromagnetically below T-N = 6.6 K and has two metamagnetic transitions, at 2.8 and 5.6 T. The locations of the critical end points of the metamagnetic transitions, which may play a strong role in the putative quantum criticality of CeAuSb2 and related compounds, are identified. The entropy map reveals an apparent entropy balance with Fermi-liquid behavior, implying that above the Neel transition the Ce moments are incorporated into the Fermi liquid. High-field data showing that the magnetic behavior is remarkably anisotropic are also reported. C1 [Zhao, Lishan; Yelland, Edward A.; Bruin, Jan A. N.; Sakai, Hideaki; Mackenzie, Andrew P.] Univ St Andrews, SUPA, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Zhao, Lishan; Mackenzie, Andrew P.; Hicks, Clifford W.] Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany. [Yelland, Edward A.] Univ Edinburgh, Sch Phys & Astron, SUPA, Mayfield Rd, Edinburgh EH9 3JZ, Midlothian, Scotland. [Yelland, Edward A.] Univ Edinburgh, Ctr Sci Extreme Condit, Mayfield Rd, Edinburgh EH9 3JZ, Midlothian, Scotland. [Bruin, Jan A. N.] Max Planck Inst Solid State Res, Heisenbergstr 1, D-70569 Stuttgart, Germany. [Sheikin, Ilya] UJF, CNRS, LNCMI, EMFL, F-38042 Grenoble, France. [Canfield, Paul C.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Canfield, Paul C.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. [Fritsch, Veronika] Univ Augsburg, Inst Phys, Ctr Elect Correlat & Magnetism, Expt Phys 6, D-86135 Augsburg, Germany. [Fritsch, Veronika] Karlsruhe Inst Technol, Phys Inst, D-76131 Karlsruhe, Germany. [Sakai, Hideaki] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan. RP Mackenzie, AP (reprint author), Univ St Andrews, SUPA, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland.; Mackenzie, AP; Hicks, CW (reprint author), Max Planck Inst Chem Phys Solids, Nothnitzer Str 40, D-01187 Dresden, Germany. EM mackenzie@cpfs.mpg.de; hicks@cpfs.mpg.de RI Hicks, Clifford/N-9719-2015; Sakai, Hideaki/G-1008-2014; Fritsch, Veronika/P-1352-2016 OI Fritsch, Veronika/0000-0002-6620-4554 FU EPSRC [EP/1031014/1, EP/G03673X/1]; Max Planck Society; LNCMI-CNRS; Royal Society; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering through the Ames Laboratory; Deutsche Forschungsgemeinschaft through FOR Grant [960]; Canon Foundation; U.S. Department of Energy [DE-AC02-07CH11358] FX We acknowledge useful discussion with Manuel Brando and Christoph Geibel. We thank Hanoh Lee for advice on crystal growth. We thank the EPSRC (Grants No. EP/1031014/1 and No. EP/G03673X/1) and the Max Planck Society for financial support. We also acknowledge the support of the LNCMI-CNRS, member of the European Magnetic Field Laboratory (EMFL). E.A.Y. acknowledges support from the Royal Society. P.C.C. was supported, in part, by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering through the Ames Laboratory. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. V.F. acknowledges support by the Deutsche Forschungsgemeinschaft through FOR Grant No. 960. H.S. gratefully acknowledges fellowships from the Canon Foundation. NR 38 TC 0 Z9 0 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 12 PY 2016 VL 93 IS 19 AR 195124 DI 10.1103/PhysRevB.93.195124 PG 7 WC Physics, Condensed Matter SC Physics GA DL9WR UT WOS:000375994600002 ER PT J AU Abe, Y Abrahao, T Almazan, H Alt, C Appel, S Barriere, JC Baussan, E Bekman, I Bergevin, M Bezerra, TJC Bezrukov, L Blucher, E Brugiere, T Buck, C Busenitz, J Cabrera, A Camilleri, L Carr, R Cerrada, M Chauveau, E Chimenti, P Collin, AP Conover, E Conrad, JM Crespo-Anadon, JI Crum, K Cucoanes, AS Damon, E Dawson, JV De Kerret, H Dhooghe, J Dietrich, D Djurcic, Z dos Anjos, JC Dracos, M Etenko, A Fallot, M Felde, J Fernandes, SM Fischer, V Franco, D Franke, M Furuta, H Gil-Botella, I Giot, L Goger-Neff, M Gomez, H Gonzalez, LFG Goodenough, L Goodman, MC Haag, N Hara, T Haser, J Hellwig, D Hofmann, M Horton-Smith, GA Hourlier, A Ishitsuka, M Jochum, J Jollet, C Kaether, F Kalousis, LN Kamyshkov, Y Kaneda, M Kaplan, DM Kawasaki, T Kemp, E Kryn, D Kuze, M Lachenmaier, T Lane, CE Lasserre, T Letourneau, A Lhuillier, D Lima, HP Lindner, M Lopez-Castano, JM LoSecco, JM Lubsandorzhiev, B Lucht, S Maeda, J Mariani, C Maricic, J Martino, J Matsubara, T Mention, G Meregaglia, A Miletic, T Milincic, R Minotti, A Nagasaka, Y Navas-Nicolas, D Novella, P Oberauer, L Obolensky, M Onillon, A Osborn, A Palomares, C Pepe, IM Perasso, S Porta, A Pronost, G Reichenbacher, J Reinhold, B Rohling, M Roncin, R Rybolt, B Sakamoto, Y Santorelli, R Schilithz, AC Schonert, S Schoppmann, S Shaevitz, MH Sharankova, R Shrestha, D Sibille, V Sinev, V Skorokhvatov, M Smith, E Soiron, M Spitz, J Stahl, A Stancu, I Stokes, LFF Strait, M Suekane, F Sukhotin, S Sumiyoshi, T Sun, Y Svoboda, R Terao, K Tonazzo, A Thi, HHT Valdiviesso, G Vassilopoulos, N Veyssiere, C Vivier, M von Feilitzsch, F Wagner, S Walsh, N Watanabe, H Wiebusch, C Wurm, M Yang, G Yermia, F Zimmer, V AF Abe, Y. Abrahao, T. Almazan, H. Alt, C. Appel, S. Barriere, J. C. Baussan, E. Bekman, I. Bergevin, M. Bezerra, T. J. C. Bezrukov, L. Blucher, E. Brugiere, T. Buck, C. Busenitz, J. Cabrera, A. Camilleri, L. Carr, R. Cerrada, M. Chauveau, E. Chimenti, P. Collin, A. P. Conover, E. Conrad, J. M. Crespo-Anadon, J. I. Crum, K. Cucoanes, A. S. Damon, E. Dawson, J. V. De Kerret, H. Dhooghe, J. Dietrich, D. Djurcic, Z. dos Anjos, J. C. Dracos, M. Etenko, A. Fallot, M. Felde, J. Fernandes, S. M. Fischer, V. Franco, D. Franke, M. Furuta, H. Gil-Botella, I. Giot, L. Goeger-Neff, M. Gomez, H. Gonzalez, L. F. G. Goodenough, L. Goodman, M. C. Haag, N. Hara, T. Haser, J. Hellwig, D. Hofmann, M. Horton-Smith, G. A. Hourlier, A. Ishitsuka, M. Jochum, J. Jollet, C. Kaether, F. Kalousis, L. N. Kamyshkov, Y. Kaneda, M. Kaplan, D. M. Kawasaki, T. Kemp, E. Kryn, D. Kuze, M. Lachenmaier, T. Lane, C. E. Lasserre, T. Letourneau, A. Lhuillier, D. Lima, H. P., Jr. Lindner, M. Lopez-Castano, J. M. LoSecco, J. M. Lubsandorzhiev, B. Lucht, S. Maeda, J. Mariani, C. Maricic, J. Martino, J. Matsubara, T. Mention, G. Meregaglia, A. Miletic, T. Milincic, R. Minotti, A. Nagasaka, Y. Navas-Nicolas, D. Novella, P. Oberauer, L. Obolensky, M. Onillon, A. Osborn, A. Palomares, C. Pepe, I. M. Perasso, S. Porta, A. Pronost, G. Reichenbacher, J. Reinhold, B. Roehling, M. Roncin, R. Rybolt, B. Sakamoto, Y. Santorelli, R. Schilithz, A. C. Schoenert, S. Schoppmann, S. Shaevitz, M. H. Sharankova, R. Shrestha, D. Sibille, V. Sinev, V. Skorokhvatov, M. Smith, E. Soiron, M. Spitz, J. Stahl, A. Stancu, I. Stokes, L. F. F. Strait, M. Suekane, F. Sukhotin, S. Sumiyoshi, T. Sun, Y. Svoboda, R. Terao, K. Tonazzo, A. Thi, H. H. Trinh Valdiviesso, G. Vassilopoulos, N. Veyssiere, C. Vivier, M. von Feilitzsch, F. Wagner, S. Walsh, N. Watanabe, H. Wiebusch, C. Wurm, M. Yang, G. Yermia, F. Zimmer, V. CA Double Chooz Collaboration TI Muon capture on light isotopes measured with the Double Chooz detector SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR CAPTURE; ENERGY-LEVELS; BETA-DECAY; RATES; B-12; SPECTRUM; STATES; C-12; N-14 AB Using the Double Chooz detector, designed to measure the neutrino mixing angle theta(13), the products of mu(-) capture on C-12, C-13, N-14, and O-16 have been measured. Over a period of 489.5 days, 2.3 x 10(6) stopping cosmic mu(-) have been collected, of which 1.8 x 10(5) captured on carbon, nitrogen, or oxygen nuclei in the inner detector scintillator or acrylic vessels. The resulting isotopes were tagged using prompt neutron emission (when applicable), the subsequent beta decays, and, in some cases, beta-delayed neutrons. The most precise measurement of the rate of C-12(mu(-), nu)B-12 to date is reported: 6.57(-0.21)(+0.11) x 10(3) s(-1), or (17.35(-0.59)(+0.35))% of nuclear captures. By tagging excited states emitting gamma s, the ground state transition rate to B-12 has been determined to be 5.68(-0.23)(+0.14) x 10(3) s(-1). The heretofore unobserved reactions C-12(mu(-), nu alpha)Li-8, C-13(mu(-), nu n alpha)Li-8, and C-13(mu(-), nu n)B-12 are measured. Further, a population of beta n decays following stopping muons is identified with 5.5 sigma significance. Statistics limit our ability to identify these decays definitively. Assuming negligible production of He-8, the reaction C-13(mu(-), nu alpha)Li-9 is found to be present at the 2.7 sigma level. Limits are set on a variety of other processes. C1 [Alt, C.; Bekman, I.; Cabrera, A.; Hellwig, D.; Lucht, S.; Schoppmann, S.; Soiron, M.; Stahl, A.; Wiebusch, C.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Busenitz, J.; Fernandes, S. M.; Reichenbacher, J.; Stancu, I.; Sun, Y.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Djurcic, Z.; Goodenough, L.; Goodman, M. C.; Yang, G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Cabrera, A.; Dawson, J. V.; De Kerret, H.; Etenko, A.; Franco, D.; Gomez, H.; Hourlier, A.; Kryn, D.; Lasserre, T.; Obolensky, M.; Onillon, A.; Perasso, S.; Roncin, R.; Tonazzo, A.] Univ Paris Diderot, AstroParticule & Cosmol, CNRS IN2P3, CEA IRFU,Observ Paris,Sorbonne Paris Cite, F-75205 Paris 13, France. [Abrahao, T.; dos Anjos, J. C.; Lima, H. P., Jr.; Pepe, I. M.; Schilithz, A. C.; Valdiviesso, G.; Wagner, S.] Ctr Brasileiro Pesquisas Fis, BR-22290180 Rio De Janeiro, RJ, Brazil. [Blucher, E.; Conover, E.; Crum, K.; Strait, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cabrera, A.; Cerrada, M.; Crespo-Anadon, J. I.; Gil-Botella, I.; Lopez-Castano, J. M.; Navas-Nicolas, D.; Novella, P.; Palomares, C.; Santorelli, R.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain. [Camilleri, L.; Carr, R.; Shaevitz, M. H.] Columbia Univ, New York, NY 10027 USA. [Bergevin, M.; Dhooghe, J.; Felde, J.; Svoboda, R.; Walsh, N.] Univ Calif Davis, Davis, CA 95616 USA. [Damon, E.; Lane, C. E.; Maricic, J.; Miletic, T.; Milincic, R.; Smith, E.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Nagasaka, Y.; Novella, P.] Hiroshima Inst Technol, Hiroshima 7315193, Japan. [Kaplan, D. M.; Yang, G.] IIT, Dept Phys, Chicago, IL 60616 USA. [Bezrukov, L.; Lubsandorzhiev, B.; Sinev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Barriere, J. C.; Fischer, V.; Lasserre, T.; Letourneau, A.; Lhuillier, D.; Mention, G.; Sibille, V.; Veyssiere, C.; Vivier, M.] IRFU, Commissariat Energie Atom & Energies Alternat, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Horton-Smith, G. A.; Shrestha, D.] Kansas State Univ, Dept Phys, Manhattan, KS 66506 USA. [Kawasaki, T.] Kitasato Univ, Dept Phys, Sagamihara, Kanagawa 2520373, Japan. [Hara, T.] Kobe Univ, Dept Phys, Kobe, Hyogo 6578501, Japan. [Etenko, A.; Skorokhvatov, M.; Sukhotin, S.] NRC Kurchatov Inst, Moscow 123182, Russia. [Conrad, J. M.; Spitz, J.; Terao, K.] MIT, Cambridge, MA 02139 USA. [Almazan, H.; Buck, C.; Cabrera, A.; Collin, A. P.; Haser, J.; Kaether, F.; Lindner, M.; Reinhold, B.; Watanabe, H.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [LoSecco, J. M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Baussan, E.; Brugiere, T.; Cabrera, A.; Dracos, M.; Jollet, C.; Meregaglia, A.; Minotti, A.; Vassilopoulos, N.] Univ Strasbourg, IPHC, CNRS IN2P3, F-67037 Strasbourg, France. [Cucoanes, A. S.; Fallot, M.; Giot, L.; Martino, J.; Porta, A.; Pronost, G.; Yermia, F.] Univ Nantes, Ecole Mines Nantes, CNRS IN2P3, SUBATECH, F-44307 Nantes, France. [Kamyshkov, Y.; Osborn, A.; Rybolt, B.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Bezerra, T. J. C.; Chauveau, E.; Furuta, H.; Suekane, F.] Tohoku Univ, Res Ctr Neutrino Sci, Sendai, Miyagi 9808578, Japan. [Sakamoto, Y.] Tohoku Gakuin Univ, Sendai, Miyagi 9813193, Japan. [Abe, Y.; Ishitsuka, M.; Kaneda, M.; Kuze, M.; Sharankova, R.] Tokyo Inst Technol, Dept Phys, Tokyo 1528551, Japan. [Maeda, J.; Matsubara, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan. [Appel, S.; Cabrera, A.; Franke, M.; Goeger-Neff, M.; Haag, N.; Hofmann, M.; Oberauer, L.; Schoenert, S.; Thi, H. H. Trinh; von Feilitzsch, F.; Zimmer, V.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Dietrich, D.; Jochum, J.; Lachenmaier, T.; Roehling, M.; Stokes, L. F. F.; Wurm, M.] Univ Tubingen, Kepler Ctr Astro & Particle Phys, D-72076 Tubingen, Germany. [Chimenti, P.] Univ Fed ABC, UFABC, BR-09210580 Sao Paulo, Brazil. [Gonzalez, L. F. G.; Kemp, E.] Univ Estadual Campinas UNICAMP, BR-13083970 Campinas, SP, Brazil. [Kalousis, L. N.; Mariani, C.] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. [Cucoanes, A. S.] Horia Hulubei Natl Inst Phys & Nucl Engn, ELI NP, Bucharest 077125, Romania. [Felde, J.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Maeda, J.] Kobe Univ, Dept Phys, Kobe, Hyogo 6588501, Japan. [Maricic, J.; Milincic, R.; Reinhold, B.; Sun, Y.] Univ Hawaii Manoa, Dept Phys & Astron, Honolulu, HI 96822 USA. [Novella, P.] IFIC CSIC UV, Inst Fis Corpuscular, Paterna 46980, Spain. [Wurm, M.] Johannes Gutenberg Univ Mainz, Inst Phys & Excellence, Cluster PRISMA, D-55128 Mainz, Germany. RP Strait, M (reprint author), Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. EM strait@hep.uchicago.edu RI Kamyshkov, Yuri/J-7999-2016; Chimenti, Pietro/F-9898-2012; Stahl, Achim/E-8846-2011; Mariani, Camillo/J-6070-2015; Skorokhvatov, Mikhail/R-9735-2016; Wiebusch, Christopher/G-6490-2012; OI Kamyshkov, Yuri/0000-0002-3789-7152; Chimenti, Pietro/0000-0002-9755-5066; Stahl, Achim/0000-0002-8369-7506; Mariani, Camillo/0000-0003-3284-4681; Wiebusch, Christopher/0000-0002-6418-3008; Valdiviesso, Gustavo/0000-0002-0381-3619; Franco, Davide/0000-0001-5604-2531 FU CEA; CNRS/IN2P3; computer center CCIN2P3; LabEx UnivEarthS in France [ANR-11-IDEX-0005-02]; Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT); Japan Society for the Promotion of Science (JSPS); Department of Energy; National Science Foundation of the United States; U.S. Department of Energy through the Nuclear Science and Security Consortium [DE-NA0000979]; Ministerio de Economia y Competitividad (MINECO) of Spain; Max Planck Gesellschaft; Deutsche Forschungsgemeinschaft DFG; Transregional Collaborative Research Center [TR27]; excellence cluster "Origin and Structure of the Universe"; Maier-Leibnitz-Laboratorium Garching in Germany; Russian Academy of Science; Kurchatov Institute; RFBR (the Russian Foundation for Basic Research); Brazilian Ministry of Science, Technology and Innovation (MCTI); Financiadora de Estudos e Projetos (FINEP); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Sao Paulo Research Foundation (FAPESP); Brazilian Network for High Energy Physics (RENAFAE) in Brazil FX We thank the French electricity company EDF; the European fund FEDER; the Region de Champagne Ardenne; the Departement des Ardennes; and the Communaute de Communes Ardenne Rives de Meuse. We acknowledge the support of the CEA, CNRS/IN2P3, the computer center CCIN2P3, and LabEx UnivEarthS in France (ANR-11-IDEX-0005-02); the Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT) and the Japan Society for the Promotion of Science (JSPS); the Department of Energy and the National Science Foundation of the United States; U.S. Department of Energy Award No. DE-NA0000979 through the Nuclear Science and Security Consortium; the Ministerio de Economia y Competitividad (MINECO) of Spain; the Max Planck Gesellschaft, and the Deutsche Forschungsgemeinschaft DFG, the Transregional Collaborative Research Center TR27, the excellence cluster "Origin and Structure of the Universe", and the Maier-Leibnitz-Laboratorium Garching in Germany; the Russian Academy of Science, the Kurchatov Institute and RFBR (the Russian Foundation for Basic Research); the Brazilian Ministry of Science, Technology and Innovation (MCTI), the Financiadora de Estudos e Projetos (FINEP), the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), the Sao Paulo Research Foundation (FAPESP), and the Brazilian Network for High Energy Physics (RENAFAE) in Brazil. NR 45 TC 0 Z9 0 U1 4 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 12 PY 2016 VL 93 IS 5 AR 054608 DI 10.1103/PhysRevC.93.054608 PG 18 WC Physics, Nuclear SC Physics GA DL9YN UT WOS:000375999500003 ER PT J AU Ayangeakaa, AD Garg, U Petrache, CM Guo, S Zhao, PW Matta, JT Nayak, BK Patel, D Janssens, RVF Carpenter, MP Chiara, CJ Kondev, FG Lauritsen, T Seweryniak, D Zhu, S Ghugre, SS Palit, R AF Ayangeakaa, A. D. Garg, U. Petrache, C. M. Guo, S. Zhao, P. W. Matta, J. T. Nayak, B. K. Patel, D. Janssens, R. V. F. Carpenter, M. P. Chiara, C. J. Kondev, F. G. Lauritsen, T. Seweryniak, D. Zhu, S. Ghugre, S. S. Palit, R. TI In-beam spectroscopy of medium- and high-spin states in Ce-133 SO PHYSICAL REVIEW C LA English DT Article ID COINCIDENCE DATA SETS; ROTATIONAL BANDS; LIFETIME MEASUREMENTS; MAGNETIC ROTATION; COLLECTIVITY AB Medium and high-spin states in Ce-133 were investigated using the Cd-116(Ne-22, 5n) reaction and the Gammasphere array. The level scheme was extended up to an excitation energy of similar to 22.8 MeV and spin 93/2 (h) over bar. Eleven bands of quadrupole transitions and two new dipole bands are identified. The connections to low-lying states of the previously known, high-spin triaxial bands were firmly established, thus fixing the excitation energy and, in many cases, the spin parity of the levels. Based on comparisons with cranked Nilsson-Strutinsky calculations and tilted axis cranking covariant density functional theory, it is shown that all observed bands are characterized by pronounced triaxiality. Competing multiquasiparticle configurations are found to contribute to a rich variety of collective phenomena in this nucleus. C1 [Ayangeakaa, A. D.; Garg, U.; Matta, J. T.; Nayak, B. K.; Patel, D.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Petrache, C. M.; Guo, S.] Univ Paris Saclay, CNRS, IN2P3, Ctr Sci Nucl & Sci Mat, Bat 104-108, F-91405 Orsay, France. [Ayangeakaa, A. D.; Zhao, P. W.; Janssens, R. V. F.; Carpenter, M. P.; Chiara, C. J.; Lauritsen, T.; Seweryniak, D.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Chiara, C. J.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Ghugre, S. S.] UGC DAE Consortium Sci Res, Kolkata 700098, India. [Palit, R.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Palit, R.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Matta, J. T.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37830 USA. [Nayak, B. K.] Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. [Patel, D.] Univ Texas MD Anderson Canc Ctr, Houston, TX 77030 USA. [Chiara, C. J.] US Army Res Lab, Adelphi, MD 20783 USA. RP Ayangeakaa, AD (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA.; Ayangeakaa, AD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RI Zhao, Pengwei/F-9107-2010; Palit, Rudrajyoti/F-5185-2012 OI Zhao, Pengwei/0000-0001-8243-2381; FU U.S. National Science Foundation [PHY07-58100, PHY-0822648, PHY-1068192, PHY-1419765]; U.S. Department of Energy, Office of Nuclear Physics [DE-FG02-94ER40834, DE-AC02-06CH11357] FX C.M.P. expresses his gratitude to Prof. I. Ragnarsson for providing the CNS codes, for the training on how to use them, and for enlightening comments on the theoretical interpretation of the results. This work was supported in part by the U.S. National Science Foundation Grants No. PHY07-58100, No. PHY-0822648, No. PHY-1068192, and No. PHY-1419765, and the U.S. Department of Energy, Office of Nuclear Physics, under Grant No. DE-FG02-94ER40834 (UM) and Contract No. DE-AC02-06CH11357 (ANL). This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 30 TC 2 Z9 2 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 12 PY 2016 VL 93 IS 5 AR 054317 DI 10.1103/PhysRevC.93.054317 PG 19 WC Physics, Nuclear SC Physics GA DL9YN UT WOS:000375999500002 ER PT J AU Danczak, RE Yabusaki, SB Williams, KH Fang, YL Hobson, C Wilkins, MJ AF Danczak, Robert E. Yabusaki, Steven B. Williams, Kenneth H. Fang, Yilin Hobson, Chad Wilkins, Michael J. TI Snowmelt Induced Hydrologic Perturbations Drive Dynamic Microbiological and Geochemical Behaviors across a Shallow Riparian Aquifer SO FRONTIERS IN EARTH SCIENCE LA English DT Article DE aquifer; reactive transport modeling; fermentation; candidate phyla; Rifle ID URANIUM-CONTAMINATED AQUIFER; MICROBIAL COMMUNITY; GROUNDWATER; SEDIMENT; BIOREMEDIATION; SUBSURFACE; DIVERSITY; IMPACT; ORGANISMS; BACTERIA AB Shallow riparian aquifers represent hotspots of biogeochemical activity in the arid western US. While these environments provide extensive ecosystem services, little is known of how natural environmental perturbations influence subsurface microbial communities and associated biogeochemical processes. Over a 6-month period we tracked the annual snowmelt-driven incursion of groundwater into the vadose zone of an aquifer adjacent to the Colorado River, leading to increased dissolved oxygen (DO) concentrations in the normally suboxic saturated zone. Strong biogeochemical heterogeneity was measured across the site, with abiotic reactions between DO and sulfide minerals driving rapid DO consumption and mobilization of redox active species in reduced aquifer regions. Conversely, extensive DO increases were detected in less reduced sediments. 16S rRNA gene surveys tracked microbial community composition within the aquifer, revealing strong correlations between increases in putative oxygen-utilizing chemolithoautotrophs and heterotrophs and rising DO concentrations. The gradual return to suboxic aquifer conditions favored increasing abundances of 16S rRNA sequences matching members of the Microgenomates (OP11) and Parcubacteria (OD1) that have been strongly implicated in fermentative processes. Microbial community stability measurements indicated that deeper aquifer locations were relatively less affected by geochemical perturbations, while communities in shallower locations exhibited the greatest change. Reactive transport modeling of the geochemical and microbiological results supported field observations, suggesting that a predictive framework can be applied to develop a greater understanding of such environments. C1 [Danczak, Robert E.; Wilkins, Michael J.] Ohio State Univ, Dept Microbiol, 484 W 12th Ave, Columbus, OH 43210 USA. [Yabusaki, Steven B.; Fang, Yilin] Pacific Northwest Natl Lab, Hydrol Grp, Richland, WA 99352 USA. [Williams, Kenneth H.; Hobson, Chad] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Wilkins, Michael J.] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. RP Wilkins, MJ (reprint author), Ohio State Univ, Dept Microbiol, 484 W 12th Ave, Columbus, OH 43210 USA.; Wilkins, MJ (reprint author), Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. EM wilkins.231@osu.edu FU Genomes to Watershed Scientific Focus Area at Lawrence Berkeley National Laboratory; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DEAC02-05CH11231] FX This work was supported as part of the Genomes to Watershed Scientific Focus Area at Lawrence Berkeley National Laboratory, which is funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under Award Number DEAC02-05CH11231. NR 45 TC 2 Z9 2 U1 1 U2 1 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2296-6463 J9 FRONT EARTH SCI JI Front. Earth Sci. PD MAY 11 PY 2016 VL 4 AR UNSP 57 DI 10.3389/feart.2016.00057 PG 13 WC Geosciences, Multidisciplinary SC Geology GA EJ3VQ UT WOS:000393140700001 ER PT J AU Come, J Xie, Y Naguib, M Jesse, S Kalinin, SV Gogotsi, Y Kent, PRC Balke, N AF Come, Jeremy Xie, Yu Naguib, Michael Jesse, Stephen Kalinin, Sergei V. Gogotsi, Yury Kent, Paul R. C. Balke, Nina TI Nanoscale Elastic Changes in 2D Ti3C2Tx (MXene) Pseudocapacitive Electrodes SO ADVANCED ENERGY MATERIALS LA English DT Article ID TRANSITION-METAL CARBIDES; 2-DIMENSIONAL TITANIUM CARBIDE; FORCE ACOUSTIC MICROSCOPY; HIGH VOLUMETRIC CAPACITANCE; LITHIUM-ION BATTERIES; CATION INTERCALATION; ENERGY-STORAGE; GRAPHENE; SPECTROSCOPY; EXTRACTION AB Designing sustainable electrodes for next generation energy storage devices relies on the understanding of their fundamental properties at the nanoscale, including the comprehension of ions insertion into the electrode and their interactions with the active material. One consequence of ion storage is the change in the electrode volume resulting in mechanical strain and stress that can strongly affect the cycle life. Therefore, it is important to understand the changes of dimensions and mechanical properties occurring during electrochemical reactions. While the characterization of mechanical properties via macroscopic measurements is well documented, in situ characterization of their evolution has never been achieved at the nanoscale. It is reported here with in situ imaging, combined with density functional theory of the elastic changes of a 2D titanium carbide (Ti3C2Tx) based electrode in direction normal to the basal plane (electrode surface) during alkaline cation intercalation/extraction. 2D carbides, known as MXenes, are promising new materials for supercapacitors and various kinds of batteries, and understanding the coupling between their mechanical and electrochemical properties is therefore necessary. The results show a strong correlation between the cations content and the out-of-plane elastic modulus. This strategy enables identifying the preferential intercalation pathways within a single particle, which is important for understanding ionic transport in these materials. C1 [Come, Jeremy; Xie, Yu; Jesse, Stephen; Kalinin, Sergei V.; Kent, Paul R. C.; Balke, Nina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, POB 2008, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, POB 2008, Oak Ridge, TN 37831 USA. [Naguib, Michael] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Gogotsi, Yury] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. RP Xie, Y; Balke, N (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, POB 2008, Oak Ridge, TN 37831 USA. EM xiey@ornl.gov; balken@ornl.gov RI Kent, Paul/A-6756-2008; Balke, Nina/Q-2505-2015; Xie, Yu/E-5875-2011; OI Kent, Paul/0000-0001-5539-4017; Balke, Nina/0000-0001-5865-5892; Xie, Yu/0000-0002-7782-5428; Come, Jeremy/0000-0002-3335-0627; Naguib, Michael/0000-0002-4952-9023 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC0500OR22725] FX The experiments and sample preparation in this work were supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The facilities to perform the experiments were provided by the Center for Nanophase Materials Sciences, which is a DOE Office of Science user facility. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC0500OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 55 TC 5 Z9 5 U1 56 U2 103 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY 11 PY 2016 VL 6 IS 9 AR 1502290 DI 10.1002/aenm.201502290 PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DQ6HX UT WOS:000379306400012 ER PT J AU Yan, PF Zheng, JM Zheng, JX Wang, ZG Teng, GF Kuppan, S Xiao, J Chen, GY Pan, F Zhang, JG Wang, CM AF Yan, Pengfei Zheng, Jianming Zheng, Jiaxin Wang, Zhiguo Teng, Gaofeng Kuppan, Saravanan Xiao, Jie Chen, Guoying Pan, Feng Zhang, Ji-Guang Wang, Chong-Min TI Ni and Co Segregations on Selective Surface Facets and Rational Design of Layered Lithium Transition-Metal Oxide Cathodes SO ADVANCED ENERGY MATERIALS LA English DT Article ID LI-ION BATTERIES; LOW IRREVERSIBLE CAPACITY; CHEMICAL EVOLUTION; MANGANESE OXIDES; VOLTAGE FADE; HIGH-POWER; MN; ELECTRODES; NICKEL; BEHAVIOR AB The chemical processes occurring on the surface of cathode materials during battery cycling play a crucial role in determining battery's performance. However, the understanding of such surface chemistry is far from clear due to the complexity of redox chemistry during battery charge/discharge. Through intensive aberration corrected STEM investigation on ten layered oxide cathode materials, two important findings on the pristine oxides are reported. First, Ni and Co show strong plane selectivity when building up their respective surface segregation layers (SSLs). Specifically, Ni-SSL is exclusively developed on (200)(m) facet in Li-Mn-rich oxides (monoclinic C2/m symmetry) and on (012)(h) facet in Mn-Ni equally rich oxides (hexagonal R-3m symmetry), while Co-SSL has a strong preference to (20-2)(m) plane with minimal Co-SSL also developed on some other planes in Li-Mn-rich cathodes. Structurally, Ni-SSLs tend to form spinel-like lattice while Co-SSLs are in a rock-salt-like structure. Second, by increasing Ni concentration in these layered oxides, Ni and Co SSLs can be suppressed and even eliminated. The findings indicate that Ni and Co SSLs are tunable through controlling particle morphology and oxide composition, which opens up a new way for future rational design and synthesis of cathode materials. C1 [Yan, Pengfei; Wang, Chong-Min] Pacific Northwest Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA. [Zheng, Jiaxin; Xiao, Jie; Zhang, Ji-Guang] Pacific Northwest Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99352 USA. [Zheng, Jiaxin; Teng, Gaofeng; Pan, Feng] Peking Univ, Sch Adv Mat, Shenzhen Grad Sch, Shenzhen 518055, Peoples R China. [Wang, Zhiguo] Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. [Kuppan, Saravanan; Chen, Guoying] Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. RP Wang, CM (reprint author), Pacific Northwest Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA.; Zhang, JG (reprint author), Pacific Northwest Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99352 USA. EM Jiguang.zhang@pnnl.gov; Chongmin.wang@pnnl.gov RI Wang, Zhiguo/B-7132-2009; yan, pengfei/E-4784-2016; Zheng, Jianming/F-2517-2014; OI yan, pengfei/0000-0001-6387-7502; Zheng, Jianming/0000-0002-4928-8194; kuppan, saravanan/0000-0003-4976-4514 FU Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231, 6951379]; DOE's Office of Biological and Environmental Research; Battelle for the Department of Energy [DE-AC05-76RLO1830]; National Natural Science Foundation of China [11474047] FX P.Y. and J.Z. contributed equally to this work. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 6951379 under the Batteries for Advanced Battery Materials Research (BMR). The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the Department of Energy under Contract DE-AC05-76RLO1830. Z.W. was supported by the National Natural Science Foundation of China (Grant No. 11474047). NR 50 TC 5 Z9 5 U1 38 U2 56 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAY 11 PY 2016 VL 6 IS 9 AR 1502455 DI 10.1002/aenm.201502455 PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DQ6HX UT WOS:000379306400018 ER PT J AU Harris, J Bouchard, F Santamato, E Zurek, WH Boyd, RW Karimi, E AF Harris, Jeremie Bouchard, Frederic Santamato, Enrico Zurek, Wojciech H. Boyd, Robert W. Karimi, Ebrahim TI Quantum probabilities from quantum entanglement: experimentally unpackingthe Born rule SO NEW JOURNAL OF PHYSICS LA English DT Article DE Born probability rule; envariance; optical angular momentum ID ORBITAL ANGULAR-MOMENTUM; LIGHT AB The Born rule, a foundational axiom used to deduce probabilities of events from wavefunctions, is indispensable in the everyday practice of quantum physics. It is also key in the quest to reconcile the ostensibly inconsistent laws of the quantum and classical realms, as it confers physical significance to reduced density matrices, the essential tools of decoherence theory. Following Bohr's Copenhagen interpretation, textbooks postulate the Born rule outright. However, recent attempts to derive it from other quantum principles have been successful, holding promise for simplifying and clarifying the quantum foundational bedrock. A major family of derivations is based on envariance, a recently discovered symmetry of entangled quantum states. Here, we identify and experimentally test three premises central to these envariance-based derivations, thus demonstrating, in the microworld, the symmetries from which the Born rule is derived. Further, we demonstrate envariance in a purely local quantum system, showing its independence from relativistic causality. C1 [Harris, Jeremie; Bouchard, Frederic; Boyd, Robert W.; Karimi, Ebrahim] Univ Ottawa, Dept Phys, 25 Templeton, Ottawa, ON K1N 6N5, Canada. [Harris, Jeremie; Bouchard, Frederic; Boyd, Robert W.; Karimi, Ebrahim] Univ Ottawa, Max Planck Ctr Extreme & Quantum Photon, Ottawa, ON K1N 6N5, Canada. [Santamato, Enrico] Univ Naples Federico II, Dipartimento Fis, Via Cintia, I-80126 Naples, Italy. [Zurek, Wojciech H.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Boyd, Robert W.] Univ Rochester, Inst Opt, Rochester, NY 14627 USA. [Karimi, Ebrahim] Inst Adv Studies Basic Sci, Dept Phys, Zanjan 4513766731, Iran. RP Karimi, E (reprint author), Univ Ottawa, Dept Phys, 25 Templeton, Ottawa, ON K1N 6N5, Canada. EM ekarimi@uottawa.ca OI Bouchard, Frederic/0000-0003-4137-6250 FU Canada Excellence Research Chairs (CERC) Program; Vanier Canada Graduate Scholarships Program; Natural Sciences and Engineering Research Council's Canada Graduate Scholarships program; DoE under the Los Alamos LDRD program; Foundational Questions Institute [2015-144057]; Canada Research Chairs (CRC) program FX JH, FB, RWB and EK acknowledge the support of the Canada Excellence Research Chairs (CERC) Program. JH acknowledges the support of the Vanier Canada Graduate Scholarships Program. FB acknowledges the support of the Natural Sciences and Engineering Research Council's Canada Graduate Scholarships program. WHZ was supported by DoE under the Los Alamos LDRD program and, in part, by the Foundational Questions Institute Grant No. 2015-144057 on 'Physics of What Happens'. EK acknowledges the support of the Canada Research Chairs (CRC) program. The authors would like to thank Lorenzo Marrucci for the q-plate preparation, as well as Harjaspreet Mand, Alicia Sit, and Sarina Cotroneo for their assistance with the experiment. NR 21 TC 1 Z9 1 U1 2 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 11 PY 2016 VL 18 DI 10.1088/1367-2630/18/5/053013 PG 13 WC Physics, Multidisciplinary SC Physics GA DN6OT UT WOS:000377195500001 ER PT J AU Svahn, SL Varemo, L Gabrielsson, BG Peris, E Nookaew, I Grahnemo, L Sandberg, AS Asterholm, IW Jansson, JO Nielsen, J Johansson, ME AF Svahn, Sara L. Varemo, Leif Gabrielsson, Britt G. Peris, Eduard Nookaew, Intawat Grahnemo, Louise Sandberg, Ann-Sofie Asterholm, Ingrid Wernstedt Jansson, John-Olov Nielsen, Jens Johansson, Maria E. TI Six Tissue Transcriptomics Reveals Specific Immune Suppression in Spleen by Dietary Polyunsaturated Fatty Acids SO PLOS ONE LA English DT Article ID PROLIFERATOR-ACTIVATED RECEPTORS; ADIPOSE-TISSUE; INSULIN-RESISTANCE; METABOLIC SYNDROME; GENE-EXPRESSION; LIVER-DISEASE; OBESE MICE; INFLAMMATION; ATHEROSCLEROSIS; EICOSANOIDS AB Dietary polyunsaturated fatty acids (PUFA) are suggested to modulate immune function, but the effects of dietary fatty acids composition on gene expression patterns in immune organs have not been fully characterized. In the current study we investigated how dietary fatty acids composition affects the total transcriptome profile, and especially, immune related genes in two immune organs, spleen (SPL) and bone marrow cells (BMC). Four tissues with metabolic function, skeletal muscle (SKM), white adipose tissue (WAT), brown adipose tissue (BAT), and liver (LIV), were investigated as a comparison. Following 8 weeks on low fat diet (LFD), high fat diet (HFD) rich in saturated fatty acids (HFD-S), or HFD rich in PUFA (HFD-P), tissue transcriptomics were analyzed by microarray and metabolic health assessed by fasting blood glucose level, HOMA-IR index, oral glucose tolerance test as well as quantification of crown-like structures in WAT. HFD-P corrected the metabolic phenotype induced by HFD-S. Interestingly, SKM and BMC were relatively inert to the diets, whereas the two adipose tissues (WAT and BAT) were mainly affected by HFD per se (both HFD-S and HFD-P). In particular, WAT gene expression was driven closer to that of the immune organs SPL and BMC by HFDs. The LIV exhibited different responses to both of the HFDs. Surprisingly, the spleen showed a major response to HFD-P (82 genes differed from LFD, mostly immune genes), while it was not affected at all by HFD-S (0 genes differed from LFD). In conclusion, the quantity and composition of dietary fatty acids affected the transcriptome in distinct manners in different organs. Remarkably, dietary PUFA, but not saturated fat, prompted a specific regulation of immune related genes in the spleen, opening the possibility that PUFA can regulate immune function by influencing gene expression in this organ. C1 [Svahn, Sara L.; Peris, Eduard; Asterholm, Ingrid Wernstedt; Jansson, John-Olov; Johansson, Maria E.] Inst Neurosci & Physiol, Dept Physiol, Gothenburg, Sweden. [Varemo, Leif; Gabrielsson, Britt G.; Nookaew, Intawat; Sandberg, Ann-Sofie; Nielsen, Jens] Chalmers, Dept Biol & Biol Engn, S-41296 Gothenburg, Sweden. [Nookaew, Intawat] Oak Ridge Natl Lab, Comparat Genom Grp, Biosci Div, Oak Ridge, TN USA. [Grahnemo, Louise] Dept Rheumatol & Inflammat Res, Gothenburg, Sweden. [Nookaew, Intawat] Univ Arkansas Med Sci, Coll Med, Dept Biomed Informat, Little Rock, AR 72205 USA. RP Svahn, SL (reprint author), Inst Neurosci & Physiol, Dept Physiol, Gothenburg, Sweden. EM maria.e.johansson@neuro.gu.se OI /0000-0002-9681-3342 FU Swedish Research Council [K2013-54X-09894-19-3, 2012-1601, 2010-2667]; Swedish Society of Medicine; Sahlgrenska Center for Cardiovascular Metabolic Research (CMR) [A305:188]; Swedish Strategic Foundation; EC FP7 [Full4Health FP7-KBBE-2010-4-266408]; Knut and Alice Wallenberg Foundation; Magnus Bergvall Foundation; Langmanska Kulturfonden; Stiftelsen Gamla trotjanarinnor; OE och Edla Johanssons vetenskapliga Stiftelse; Lars Hiertas Foundation; Ake Wiberg Foundation; NovoNordisk Excellence Project Award; Diabetesfonden; Diabetes Wellness Research Foundation; Stiftelsen Tornspiran FX This work was supported by grants from the Swedish Research Council (K2013-54X-09894-19-3, 2012-1601 and 2010-2667), the Swedish Society of Medicine, the Sahlgrenska Center for Cardiovascular Metabolic Research (CMR, no. A305:188), which is supported by the Swedish Strategic Foundation, EC FP7 funding (Full4Health FP7-KBBE-2010-4-266408), the Knut and Alice Wallenberg Foundation, the Magnus Bergvall Foundation, Langmanska Kulturfonden, Stiftelsen Gamla trotjanarinnor, OE och Edla Johanssons vetenskapliga Stiftelse, the Lars Hiertas Foundation, the Ake Wiberg Foundation, NovoNordisk Excellence Project Award, Diabetesfonden, Diabetes Wellness Research Foundation and Stiftelsen Tornspiran. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 44 TC 1 Z9 1 U1 1 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 11 PY 2016 VL 11 IS 5 AR e0155099 DI 10.1371/journal.pone.0155099 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DM8CD UT WOS:000376587300089 PM 27166587 ER PT J AU Zhang, W Banerjee, D Liu, J Schaef, HT Crum, JV Fernandez, CA Kukkadapu, RK Nie, Z Nune, SK Motkuri, RK Chapman, KW Engelhard, MH Hayes, JC Silvers, KL Krishna, R McGrail, BP Liu, J Thallapally, PK AF Zhang, Wen Banerjee, Debasis Liu, Jian Schaef, Herbert T. Crum, Jarrod V. Fernandez, Carlos A. Kukkadapu, Ravi K. Nie, Zimin Nune, Satish K. Motkuri, Radha K. Chapman, Karena W. Engelhard, Mark H. Hayes, James C. Silvers, Kurt L. Krishna, Rajamani McGrail, B. Peter Liu, Jun Thallapally, Praveen K. TI Redox-Active Metal-Organic Composites for Highly Selective Oxygen Separation Applications SO ADVANCED MATERIALS LA English DT Article ID POROUS MATERIAL; SURFACE-AREA; FRAMEWORKS; GENERATION; MIXTURES; STORAGE AB A redox-active metal-organic composite material shows improved and selective O-2 adsorption over N-2 with respect to individual components (MIL-101 and ferrocene). The O-2 sensitivity of the composite material arises due to the formation of maghemite nanoparticles with the pore of the metal-organic framework material. C1 [Zhang, Wen; Banerjee, Debasis; Schaef, Herbert T.; Thallapally, Praveen K.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Liu, Jian; Crum, Jarrod V.; Fernandez, Carlos A.; Nie, Zimin; Nune, Satish K.; Motkuri, Radha K.; McGrail, B. Peter; Liu, Jun] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Kukkadapu, Ravi K.; Engelhard, Mark H.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Hayes, James C.; Silvers, Kurt L.] Pacific NW Natl Lab, Natl Secur Directorate, Richland, WA 99352 USA. [Krishna, Rajamani] Univ Amsterdam, Vant Hoff Inst Mol Sci, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. RP Thallapally, PK (reprint author), Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. EM Praveen.thallapally@pnnl.gov RI Krishna, Rajamani/A-1098-2012; Motkuri, Radha/F-1041-2014; OI Krishna, Rajamani/0000-0002-4784-8530; Motkuri, Radha/0000-0002-2079-4798; Engelhard, Mark/0000-0002-5543-0812; Thallapally, Praveen Kumar/0000-0001-7814-4467 FU DOE/BES/Division of Materials Sciences and Engineering [KC020105-FWP12152]; Department of Energy's Office of Biological and Environmental Research; U.S. Department of Energy [DE-AC05-76RL01830, DE-AC02-06CH11357] FX The authors would like to acknowledge the Office of Basic Energy Sciences (BES), U.S. Department of Energy (DOE), and DOE/BES/Division of Materials Sciences and Engineering (Award No. KC020105-FWP12152). A portion of this work (XPS and Mossbauer spectroscopy) was performed at Environmental Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for the U.S. Department of Energy by Battelle Memorial Institute under Contract No. DE-AC05-76RL01830. Work done at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Argonne National Laboratory, were supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 33 TC 3 Z9 3 U1 22 U2 50 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAY 11 PY 2016 VL 28 IS 18 BP 3572 EP + DI 10.1002/adma.201600259 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DM3MN UT WOS:000376250600020 PM 26953336 ER PT J AU Neupane, M Belopolski, I Hosen, MM Sanchez, DS Sankar, R Szlawska, M Xu, SY Dimitri, K Dhakal, N Maldonado, P Oppeneer, PM Kaczorowski, D Chou, FC Hasan, MZ Durakiewicz, T AF Neupane, Madhab Belopolski, Ilya Hosen, M. Mofazzel Sanchez, Daniel S. Sankar, Raman Szlawska, Maria Xu, Su-Yang Dimitri, Klauss Dhakal, Nagendra Maldonado, Pablo Oppeneer, Peter M. Kaczorowski, Dariusz Chou, Fangcheng Hasan, M. Zahid Durakiewicz, Tomasz TI Observation of topological nodal fermion semimetal phase in ZrSiS SO PHYSICAL REVIEW B LA English DT Article ID DIRAC SEMIMETALS; SURFACE; INSULATORS; ARCS AB Unveiling new topological phases of matter is one of the current objectives in condensed matter physics. Recent experimental discoveries of Dirac and Weyl semimetals prompt the search for other exotic phases of matter. Here we present a systematic angle-resolved photoemission spectroscopy study of ZrSiS, a prime topological nodal semimetal candidate. Our wider Brillouin zone (BZ) mapping shows multiple Fermi surface pockets such as the diamond-shaped Fermi surface, elliptical-shaped Fermi surface, and a small electron pocket encircling at the zone center (Gamma) point, the M point, and the X point of the BZ, respectively. We experimentally establish the spinless nodal fermion semimetal phase in ZrSiS, which is supported by our first-principles calculations. Our findings evidence that the ZrSiS-type of material family is a new platform on which to explore exotic states of quantum matter; these materials are expected to provide an avenue for engineering two-dimensional topological insulator systems. C1 [Neupane, Madhab; Hosen, M. Mofazzel; Dimitri, Klauss; Dhakal, Nagendra] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Sanchez, Daniel S.; Xu, Su-Yang; Hasan, M. Zahid] Princeton Univ, Joseph Henry Lab, Princeton, NJ 08544 USA. [Sanchez, Daniel S.; Xu, Su-Yang; Hasan, M. Zahid] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Sankar, Raman; Chou, Fangcheng] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Szlawska, Maria; Kaczorowski, Dariusz] Polish Acad Sci, Inst Low Temp & Struct Res, POB 937, PL-50950 Wroclaw, Poland. [Maldonado, Pablo; Oppeneer, Peter M.] Uppsala Univ, Dept Phys & Astron, POB 516, S-75120 Uppsala, Sweden. [Durakiewicz, Tomasz] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, POB 1663, Los Alamos, NM 87545 USA. RP Neupane, M (reprint author), Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. EM Madhab.Neupane@ucf.edu OI Maldonado, Pablo/0000-0002-8524-819X FU University of Central Florida; NSF IR/D program; NSF GRFP; National Science Centre (Poland) [2015/18/A/ST3/00057]; Emergent Phenomena in Quantum Systems Initiative of the Gordon and Betty Moore Foundation [GBMF4547]; National Science Foundation, Division of Materials Research [NSF-DMR-1507585, NSF-DMR-1006492]; Swedish Research Council (VR); K. and A. Wallenberg Foundation; Swedish National Infrastructure for computing (SNIC) FX M.N. is supported by the start-up fund from the University of Central Florida. T.D. is supported by the NSF IR/D program. I.B. acknowledges the support of the NSF GRFP. D.K. was supported by the National Science Centre (Poland) under Research Grant No. 2015/18/A/ST3/00057. Work at Princeton University is supported by the Emergent Phenomena in Quantum Systems Initiative of the Gordon and Betty Moore Foundation under Grant No. GBMF4547 (M.Z.H.) and by the National Science Foundation, Division of Materials Research, under Grants No. NSF-DMR-1507585 and No. NSF-DMR-1006492. P.M. and P.M.O. acknowledge support from the Swedish Research Council (VR), the K. and A. Wallenberg Foundation, and the Swedish National Infrastructure for computing (SNIC). We thank Plumb Nicholas Clark for beamline assistance at the SLS, PSI. We also thank Sung-Kwan Mo for beamline assistance at the LBNL. NR 40 TC 17 Z9 17 U1 21 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2016 VL 93 IS 20 AR 201104 DI 10.1103/PhysRevB.93.201104 PG 6 WC Physics, Condensed Matter SC Physics GA DL9XQ UT WOS:000375997100001 ER PT J AU She, JH Bishop, AR Balatsky, AV AF She, Jian-Huang Bishop, A. R. Balatsky, Alexander V. TI Strange metals from quantum geometric fluctuations of interfaces SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; TOPOLOGICAL INSULATORS; MOTT INSULATOR; CRITICAL-POINT; PHASE; ELECTRON; TRANSITIONS; CRITICALITY; EXPONENTS; BEHAVIOR AB Our current understanding of strongly correlated electron systems is based on a homogeneous framework. Here we take a step going beyond this paradigm by incorporating inhomogeneity from the beginning. Specifying to systems near the Mottmetal-insulator transition, we propose a real-space picture of itinerant electrons functioning in the fluctuating geometries bounded by interfaces between metallic and insulating regions. In 2+1 dimensions, the interfaces are closed bosonic strings, and we have a system of strings coupled to itinerant electrons. When the interface tension vanishes, the geometric fluctuations become critical, which gives rise to non-Fermi-liquid behavior for the itinerant electrons. In particular, the poles of the fermion Green's function can be converted to zeros, indicating the absence of propagating quasiparticles. Furthermore, the quantum geometric fluctuations mediate Cooper pairing among the itinerant electrons, indicating the intrinsic instability of electronic systems near the Mott transition. C1 [She, Jian-Huang] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Bishop, A. R.] Los Alamos Natl Lab, Directorate Sci Technol & Engn, POB 1663, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Los Alamos Natl Lab, Inst Mat Sci, POB 1663, Los Alamos, NM 87545 USA. [Balatsky, Alexander V.] Nord Inst Theoret Phys NORDITA, Ctr Quantum Mat, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. RP She, JH (reprint author), Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. FU U.S. Department of Energy (DOE) Basic Energy Sciences (BES) [E 304]; European Research Council [DM 32103]; KAW; Cornell Center for Materials Research; NSF MRSEC program [DMR-1120296] FX We are grateful to Steve Kivelson, Liam McAllister, Erich Mueller, Subir Sachdev, Yu-dai Tsai, and Jan Zaanen for useful discussions. Work at Los Alamos National Laboratory was supported by U.S. Department of Energy (DOE) Basic Energy Sciences (BES) E 304. Work at Nordita was supported by European Research Council Grant No. DM 32103 and KAW. Work at Cornell University was supported by the Cornell Center for Materials Research with funding from the NSF MRSEC program (Grant No. DMR-1120296). NR 76 TC 0 Z9 0 U1 6 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2016 VL 93 IS 19 AR 195122 DI 10.1103/PhysRevB.93.195122 PG 11 WC Physics, Condensed Matter SC Physics GA DL9WP UT WOS:000375994400003 ER PT J AU Sunku, SS Kong, T Ito, T Canfield, PC Shastry, BS Sengupta, P Panagopoulos, C AF Sunku, Sai Swaroop Kong, Tai Ito, Toshimitsu Canfield, Paul C. Shastry, B. Sriram Sengupta, Pinaki Panagopoulos, Christos TI Hysteretic magnetoresistance and unconventional anomalous Hall effect in the frustrated magnet TmB4 SO PHYSICAL REVIEW B LA English DT Article ID PHASE-DIAGRAM; FERROMAGNETICS; CHIRALITY; SYSTEM AB We study TmB4, a frustrated magnet on the Archimedean Shastry-Sutherland lattice, through magnetization and transport experiments. The lack of anisotropy in resistivity shows that TmB4 is an electronically three-dimensional system. The magnetoresistance (MR) is hysteretic at low temperature even though a corresponding hysteresis in magnetization is absent. The Hall resistivity shows unconventional anomalous Hall effect (AHE) and is linear above saturation despite a large MR. We propose that complex structures at magnetic domain walls may be responsible for the hysteretic MR and may also lead to the AHE. C1 [Sunku, Sai Swaroop; Sengupta, Pinaki; Panagopoulos, Christos] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link 637371, Singapore 639798, Singapore. [Kong, Tai; Canfield, Paul C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Kong, Tai; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ito, Toshimitsu] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058562, Japan. [Shastry, B. Sriram] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. RP Sunku, SS (reprint author), Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link 637371, Singapore 639798, Singapore. FU Ministry of Education, Singapore [MOE2011-T2-1-108]; National Research Foundation (NRF), NRF-Investigatorship [NRF-NRFI2015-04]; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [FG02-06ER46319] FX We thank Y. Ozaki for technical assistance in crystal alignment. S.S.S. thanks Tanmoy Das and Anjan Soumyanarayanan for helpful discussions. Work in Singapore was supported by Grant No. MOE2011-T2-1-108 from the Ministry of Education, Singapore and the National Research Foundation (NRF), NRF-Investigatorship (NRF-NRFI2015-04). Work at Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Work at UCSC was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. FG02-06ER46319. NR 38 TC 0 Z9 0 U1 11 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 11 PY 2016 VL 93 IS 17 AR 174408 DI 10.1103/PhysRevB.93.174408 PG 5 WC Physics, Condensed Matter SC Physics GA DL9VG UT WOS:000375990700002 ER PT J AU Gade, A Tostevin, JA Bader, V Baugher, T Bazin, D Berryman, JS Brown, BA Diget, CA Glasmacher, T Hartley, DJ Lunderberg, E Stroberg, SR Recchia, F Ratkiewicz, A Weisshaar, D Wimmer, K AF Gade, A. Tostevin, J. A. Bader, V. Baugher, T. Bazin, D. Berryman, J. S. Brown, B. A. Diget, C. Aa. Glasmacher, T. Hartley, D. J. Lunderberg, E. Stroberg, S. R. Recchia, F. Ratkiewicz, A. Weisshaar, D. Wimmer, K. TI Single-particle structure at N=29: The structure of Ar-47 and first spectroscopy of S-45 SO PHYSICAL REVIEW C LA English DT Article ID EXOTIC NUCLEI; ISOTOPES AB Comprehensive spectroscopy of the N = 29 nucleus Ar-47 is presented, based on two complementary direct reaction mechanisms: one-neutron pickup onto Ar-46 projectiles and one-proton removal from the 1-ground state of K-48. The results are compared with shell-model calculations that use the state-of-the-art SDPF-U and SDPF-MU effective interactions. Also, from the Be-9(Cl-46, S-45+gamma) X one-proton-removal reaction, we report the first gamma-ray transitions observed from S-45. By using comparisons with shell-model calculations, and from the observed intensities and energy sums, we propose a first tentative level scheme for S-45. C1 [Gade, A.; Bader, V.; Baugher, T.; Bazin, D.; Berryman, J. S.; Brown, B. A.; Diget, C. Aa.; Glasmacher, T.; Lunderberg, E.; Stroberg, S. R.; Recchia, F.; Ratkiewicz, A.; Weisshaar, D.; Wimmer, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Gade, A.; Bader, V.; Baugher, T.; Brown, B. A.; Glasmacher, T.; Lunderberg, E.; Stroberg, S. R.; Ratkiewicz, A.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Tostevin, J. A.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Hartley, D. J.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Diget, C. Aa.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Stroberg, S. R.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Ratkiewicz, A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Wimmer, K.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan. RP Gade, A (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA.; Gade, A (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. RI Diget, Christian Aaen/D-8063-2016; Gade, Alexandra/A-6850-2008 OI Diget, Christian Aaen/0000-0002-9778-8759; Gade, Alexandra/0000-0001-8825-0976 FU DOE, Office of Science; NSF [PHY-1102511, PHY-1404442, PHY-1203100]; DOE [DE-AC02-05CH11231]; Department of Energy National Nuclear Security Administration [DE-NA0000979]; US DOE, Office of Nuclear Physics [DEFG02-08ER41556]; Science and Technology Facilities Council (UK) [ST/J000051, ST/L005743] FX GRETINA was funded by the DOE, Office of Science. Operation of the array at NSCL was supported by the NSF under Cooperative Agreement No. PHY-1102511 (NSCL) and the DOE under Grant No. DE-AC02-05CH11231 (LBNL). We further acknowledge support from NSF Grant No. PHY-1404442 (NSCL), from the Department of Energy National Nuclear Security Administration under Award No. DE-NA0000979, and from the US DOE, Office of Nuclear Physics, under Contract No. DEFG02-08ER41556. D.H. acknowledges funding from NSF Grant No. PHY-1203100. J.A.T. acknowledges support of the Science and Technology Facilities Council (UK) Grants No. ST/J000051 and No. ST/L005743. NR 37 TC 1 Z9 1 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 11 PY 2016 VL 93 IS 5 AR 054315 DI 10.1103/PhysRevC.93.054315 PG 9 WC Physics, Nuclear SC Physics GA DL9YH UT WOS:000375998900001 ER PT J AU Dudek, JJ Edwards, RG Wilson, DJ AF Dudek, Jozef J. Edwards, Robert G. Wilson, David J. CA Hadron Spectrum Collaboration TI An a(0) resonance in strongly coupled pi eta, K(K)over-bar scattering from lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID CHANNEL ANALYSIS; FINITE-VOLUME; S-MATRIX; PHASE-SHIFTS; THRESHOLD; SYSTEMS; MESONS; ANNIHILATION; PARTICLES; STATES AB We present the first calculation of coupled-channel meson-meson scattering in the isospin = 1, G-parity negative sector, with channels pi eta, K (K) over bar and pi eta', in a first-principles approach to QCD. From the discrete spectrum of eigenstates in three volumes extracted from lattice QCD correlation functions we determine the energy dependence of the S-matrix, and find that the S-wave features a prominent cusplike structure in pi eta -> pi eta close to the K (K) over bar threshold coupled with a rapid turn-on of amplitudes leading to the K (K) over bar final state. This behavior is traced to an a(0)(980)-like resonance, strongly coupled to both pi eta and K (K) over bar, which is identified with a pole in the complex energy plane, appearing on only a single unphysical Riemann sheet. Consideration of D-wave scattering suggests a narrow tensor resonance at higher energy. C1 [Dudek, Jozef J.; Edwards, Robert G.] Jefferson Lab, Theory Ctr, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Dudek, Jozef J.; Wilson, David J.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Wilson, David J.] Univ Cambridge, Ctr Math Sci, Dept Appl Math & Theoret Phys, Wilberforce Rd, Cambridge CB3 0WA, England. RP Dudek, JJ; Edwards, RG (reprint author), Jefferson Lab, Theory Ctr, 12000 Jefferson Ave, Newport News, VA 23606 USA.; Dudek, JJ; Wilson, DJ (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Wilson, DJ (reprint author), Univ Cambridge, Ctr Math Sci, Dept Appl Math & Theoret Phys, Wilberforce Rd, Cambridge CB3 0WA, England. EM dudek@jlab.org; edwards@jlab.org; d.j.wilson@damtp.cam.ac.uk FU U.S. Department of Energy INCITE program at Oak Ridge National Lab; NSF Teragrid at the Texas Advanced Computer Center; Pittsburgh Supercomputer Center; Jefferson Lab; U.S. Department of Energy under Jefferson Science Associates, LLC [DE-AC05-06OR23177]; U.S. Department of Energy Early Career Award [DE-SC0006765]; Isaac Newton Trust/University of Cambridge Early Career Support Scheme [RG74916] FX We thank our colleagues within the Hadron Spectrum Collaboration and M. R. Pennington for fruitful discussions. CHROMA [91] and QUDA [92,93] were used to perform this work on clusters at Jefferson Laboratory under the USQCD Initiative and the LQCD ARRA project. Gauge configurations were generated using resources awarded from the U.S. Department of Energy INCITE program at Oak Ridge National Lab, the NSF Teragrid at the Texas Advanced Computer Center and the Pittsburgh Supercomputer Center, as well as at Jefferson Lab. R. G. E. and J. J. D. acknowledge support from U.S. Department of Energy Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates Jefferson Laboratory. J. J. D. acknowledges support from the U.S. Department of Energy Early Career Award Contract No. DE-SC0006765. D. J. W. received support from a grant from the Isaac Newton Trust/University of Cambridge Early Career Support Scheme [RG74916]. NR 92 TC 8 Z9 8 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 11 PY 2016 VL 93 IS 9 AR 094506 DI 10.1103/PhysRevD.93.094506 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL9ZF UT WOS:000376001400005 ER PT J AU Barajas-Solano, DA Tartakovsky, AM AF Barajas-Solano, David A. Tartakovsky, Alexandre M. TI Probabilistic density function method for nonlinear dynamical systems driven by colored noise SO PHYSICAL REVIEW E LA English DT Article ID ADVECTIVE-REACTIVE TRANSPORT; DIFFERENTIAL-EQUATIONS; PDF EQUATIONS; MEDIA AB We present a probability density function (PDF) method for a system of nonlinear stochastic ordinary differential equations driven by colored noise. The method provides an integrodifferential equation for the temporal evolution of the joint PDF of the system's state, which we close by means of a modified large-eddy-diffusivity (LED) closure. In contrast to the classical LED closure, the proposed closure accounts for advective transport of the PDF in the approximate temporal deconvolution of the integrodifferential equation. In addition, we introduce the generalized local linearization approximation for deriving a computable PDF equation in the form of a second-order partial differential equation. We demonstrate that the proposed closure and localization accurately describe the dynamics of the PDF in phase space for systems driven by noise with arbitrary autocorrelation time. We apply the proposed PDF method to analyze a set of Kramers equations driven by exponentially autocorrelated Gaussian colored noise to study nonlinear oscillators and the dynamics and stability of a power grid. Numerical experiments show the PDF method is accurate when the noise autocorrelation time is either much shorter or longer than the system's relaxation time, while the accuracy decreases as the ratio of the two time scales approaches unity. Similarly, the PDF method accuracy decreases with increasing standard deviation of the noise. C1 [Barajas-Solano, David A.; Tartakovsky, Alexandre M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Tartakovsky, AM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM alexandre.tartakovsky@pnnl.gov FU Applied Mathematics Program within the U.S. Department of Energy Office of Advanced Scientific Computing Research as part of the Multifaceted Mathematics for Complex Systems project; DOE [DE-AC05-76RL01830] FX The authors would like to thank P. Stinis (PNNL) and Professor D. M. Tartakovsky (University of California, San Diego) for their fruitful discussion and comments. This work was supported by the Applied Mathematics Program within the U.S. Department of Energy Office of Advanced Scientific Computing Research as part of the Multifaceted Mathematics for Complex Systems project. Pacific Northwest National Laboratory is operated by Battelle for the DOE under Contract DE-AC05-76RL01830. NR 30 TC 0 Z9 0 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 11 PY 2016 VL 93 IS 5 AR 052121 DI 10.1103/PhysRevE.93.052121 PG 13 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DM0BZ UT WOS:000376008900002 PM 27300844 ER PT J AU Frandsen, BA Brunelli, M Page, K Uemura, YJ Staunton, JB Billinge, SJL AF Frandsen, Benjamin A. Brunelli, Michela Page, Katharine Uemura, Yasutomo J. Staunton, Julie B. Billinge, Simon J. L. TI Verification of Anderson Superexchange in MnO via Magnetic Pair Distribution Function Analysis and ab initio Theory SO PHYSICAL REVIEW LETTERS LA English DT Article ID MANGANESE OXIDE; SPIN-WAVES; FIELDS AB We present a temperature-dependent atomic and magnetic pair distribution function (PDF) analysis of neutron total scattering measurements of antiferromagnetic MnO, an archetypal strongly correlated transition-metal oxide. The known antiferromagnetic ground-state structure fits the low-temperature data closely with refined parameters that agree with conventional techniques, confirming the reliability of the newly developed magnetic PDF method. The measurements performed in the paramagnetic phase reveal significant short-range magnetic correlations on a similar to 1 nm length scale that differ substantially from the low-temperature long-range spin arrangement. Ab initio calculations using a self-interaction-corrected local spin density approximation of density functional theory predict magnetic interactions dominated by Anderson superexchange and reproduce the measured short-range magnetic correlations to a high degree of accuracy. Further calculations simulating an additional contribution from a direct exchange interaction show much worse agreement with the data. The Anderson superexchange model for MnO is thus verified by experimentation and confirmed by ab initio theory. C1 [Frandsen, Benjamin A.; Uemura, Yasutomo J.] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Brunelli, Michela] European Synchrotron Radiat Facil, Swiss Norwegian Beamlines, F-38000 Grenoble, France. [Page, Katharine] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Staunton, Julie B.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Billinge, Simon J. L.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Billinge, Simon J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Billinge, SJL (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.; Billinge, SJL (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. EM sb2896@columbia.edu RI Page, Katharine/C-9726-2009 OI Page, Katharine/0000-0002-9071-3383 FU NSF via PIRE Program [OISE-0968226]; NSF via DMREF Program [DMR-1436095]; NSF GRFP Program [DGE-11-44155]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES) [DE-SC00112704]; EPSRC (UK) [EP/J006750/1]; DOE Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396] FX We thank Joan Siewenie for the technical assistance with the measurements performed on the NPDF instrument. B. A. F. and Y. J. U. acknowledge support from the NSF via PIRE Program No. OISE-0968226 and DMREF Program No. DMR-1436095, and B. A. F. by NSF GRFP Program No. DGE-11-44155. S. J. L. B. acknowledges support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DOE-BES) under Contract No. DE-SC00112704. J. B. S. acknowledges support from EPSRC (UK) Grant No. EP/J006750/1. Neutron scattering experiments were carried out on NPDF at the Lujan Center, funded by the DOE Office of Basic Energy Sciences. LANL is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. NR 31 TC 1 Z9 1 U1 7 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 11 PY 2016 VL 116 IS 19 AR 197204 DI 10.1103/PhysRevLett.116.197204 PG 5 WC Physics, Multidisciplinary SC Physics GA DM0CZ UT WOS:000376011700013 PM 27232042 ER PT J AU Rocco, N Lovato, A Benhar, O AF Rocco, Noemi Lovato, Alessandro Benhar, Omar TI Unified Description of Electron-Nucleus Scattering within the Spectral Function Formalism SO PHYSICAL REVIEW LETTERS LA English DT Article ID EXCHANGE CURRENTS; MESON-EXCHANGE; MATTER AB The formalism based on factorization and nuclear spectral functions has been generalized to treat transition matrix elements involving two-nucleon currents, whose contribution to the nuclear electromagnetic response in the transverse channel is known to be significant. We report the results of calculations of the inclusive electron-carbon cross section, showing that the inclusion of processes involving two-nucleon currents appreciably improves the agreement between theory and data in the dip region, between the quasielastic and Delta-production peaks. The relation to approaches based on the independent particle of the nucleus and the implications for the analysis of flux-integrated neutrino-nucleus cross sections are discussed. C1 [Rocco, Noemi; Benhar, Omar] Univ Roma La Sapienza, INFN, I-00185 Rome, Italy. [Rocco, Noemi; Benhar, Omar] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Lovato, Alessandro] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Benhar, Omar] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. RP Rocco, N (reprint author), Univ Roma La Sapienza, INFN, I-00185 Rome, Italy.; Rocco, N (reprint author), Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. FU INFN (Italy) under grant MANYBODY; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX This research is supported by INFN (Italy) under grant MANYBODY (N. R. and O. B.) and the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357 (A. L.). NR 37 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 11 PY 2016 VL 116 IS 19 AR 192501 DI 10.1103/PhysRevLett.116.192501 PG 5 WC Physics, Multidisciplinary SC Physics GA DM0CZ UT WOS:000376011700005 PM 27232018 ER PT J AU Bock, DC Pelliccione, CJ Zhang, W Wang, JJ Knehr, KW Wang, J Wang, F West, AC Marschilok, AC Takeuchi, KJ Takeuchi, ES AF Bock, David C. Pelliccione, Christopher J. Zhang, Wei Wang, Jiajun Knehr, K. W. Wang, Jun Wang, Feng West, Alan C. Marschilok, Amy C. Takeuchi, Kenneth J. Takeuchi, Esther S. TI Dispersion of Nanocrystalline Fe3O4 within Composite Electrodes: Insights on Battery-Related Electrochemistry SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE magnetite; composite; aggregate; EXAFS; lithium-ion battery; EIS; TXM ID LITHIUM-ION BATTERIES; X-RAY-ABSORPTION; CRYSTALLITE SIZE CONTROL; PARTICLE-SIZE; ANODE MATERIALS; FINE-STRUCTURE; IMPEDANCE SPECTROSCOPY; RECHARGEABLE BATTERIES; CATHODE MATERIAL; ENERGY-STORAGE AB Aggregation of nanosized materials in composite lithium-ion-battery electrodes can be a significant factor influencing electrochemical behavior. In this study, aggregation was controlled in magnetite, Fe3O4, composite electrodes via oleic acid capping and subsequent dispersion in a carbon black matrix. A heat treatment process was effective in the removal of the oleic acid capping agent while preserving a high degree of Fe3O4 dispersion. Electrochemical testing showed that Fe3O4 dispersion is initially beneficial in delivering a higher functional capacity, in agreement with continuum model simulations. However, increased capacity fade upon extended cycling was observed for the dispersed Fe3O4 composites relative to the aggregated Fe3O4 composites. X-ray absorption spectroscopy measurements of electrodes post cycling indicated that the dispersed Fe3O4 electrodes are more oxidized in the discharged state, consistent with reduced reversibility compared with the aggregated sample. Higher charge-transfer resistance for the dispersed sample after cycling suggests increased surface-film formation on the dispersed, high-surface-area nanocrystalline Fe3O4 compared to the aggregated materials. This study provides insight into the specific effects of aggregation on electrochemistry through a multiscale view of mechanisms for magnetite composite electrodes. C1 [Bock, David C.; Pelliccione, Christopher J.; Zhang, Wei; Wang, Jiajun; Wang, Jun; Wang, Feng; Takeuchi, Esther S.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Marschilok, Amy C.; Takeuchi, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Marschilok, Amy C.; Takeuchi, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Knehr, K. W.; West, Alan C.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. RP Takeuchi, ES (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA.; Marschilok, AC; Takeuchi, KJ; Takeuchi, ES (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Marschilok, AC; Takeuchi, KJ; Takeuchi, ES (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. EM amy.marschilok@stonybrook.edu; kenneth.takeuchi.1@stonybrook.edu; esther.takeuchi@stonybrook.edu RI Knehr, Kevin/R-4127-2016 OI Knehr, Kevin/0000-0001-5571-1537 FU Center for Mesoscale Transport Properties, an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences [DE-SC0012673]; U.S. DOE, Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704]; U.S. DOE, Office of Basic Energy Science [DE-AC02-98CH10886]; DOE Office of Science [DE-AC02-06CH11357]; National Synchrotron Light Source II, Brookhaven National Laboratory, under U.S. DOE [DE-SC0012704] FX This work was supported as part of the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, under Award DE-SC0012673. This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE, Office of Science Facility, at Brookhaven National Laboratory under Contract DE-SC0012704. The use of NSLS-I was supported by the U.S. DOE, Office of Basic Energy Science, under Contract DE-AC02-98CH10886. The authors acknowledge the Transmission Electron Microscopy Facility in the Central Microscopy Imaging Center (C-MIC) at Stony Brook University, Stony Brook, New York, for their contribution toward the TEM preparation and data collection. This research used resources of the APS, a U.S. DOE, Office of Science User Facility, operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. The use of APS Beamline 8BM is partially supported by the National Synchrotron Light Source II, Brookhaven National Laboratory, under U.S. DOE Contract DE-SC0012704. NR 75 TC 6 Z9 6 U1 20 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 11 PY 2016 VL 8 IS 18 BP 11418 EP 11430 DI 10.1021/acsami.6b01134 PG 13 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DL3GA UT WOS:000375521000028 PM 27096464 ER PT J AU He, MN Su, CC Peebles, C Feng, ZX Connell, JG Liao, C Wang, Y Shkrob, IA Zhang, ZC AF He, Meinan Su, Chi-Cheung Peebles, Cameron Feng, Zhenxing Connell, Justin G. Liao, Chen Wang, Yan Shkrob, Ilya A. Zhang, Zhengcheng TI Mechanistic Insight in the Function of Phosphite Additives for Protection of LiNi0.5Co0.2Mn0.3O2 Cathode in High Voltage Li-Ion Cells SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE fluorinated phosphite; electrolyte additives; surface passivation; solid electrolyte interphase; lithium-ion battery ID IRRADIATED TRIMETHYL PHOSPHITE; MANGANESE OXIDE CATHODE; TRIS(TRIMETHYLSILYL) PHOSPHITE; FLUORINATED ELECTROLYTES; ELECTROCHEMICAL PERFORMANCE; RECHARGEABLE BATTERIES; LITHIUM; CHEMISTRY; IDENTIFICATION; TRANSFORMATION AB Triethlylphosphite (TEP) and tris(2,2,2-trifluoroethyl) phosphite (TTFP) have been evaluated as electrolyte additives for high-voltage Li-ion battery cells using a Ni-rich layered cathode material LiNi0.5Co0.2Mn0.3O2 (NCM523) and the conventional carbonate electrolyte. The repeated charge/discharge cycling for cells containing 1 wt % of these additives was performed using an NCM523/graphite full cell operated at the voltage window from 3.0-4.6 V. During the initial charge process, these additives decompose on the cathode surface at a lower oxidation potential than the baseline electrolyte. Impedance spectroscopy and post-test analyses indicate the formation of protective coatings by both additives on the cathode surface that prevent oxidative breakdown of the electrolyte. However, only TTFP containing cells demonstrate the improved capacity retention and Coulombic efficiency. For TEP, the protective coating is also formed, but low Li+ ion mobility through the interphase layer results in inferior performance. These observations are rationalized through the inhibition of electrocatalytic centers present on the cathode surface and the formation of organophosphate deposits isolating the cathode surface from the electrolyte. The difference between the two phosphites clearly originates in the different properties of the resulting phosphate coatings, which may be in Li+ ion conductivity through such materials. C1 [He, Meinan; Su, Chi-Cheung; Peebles, Cameron; Feng, Zhenxing; Liao, Chen; Shkrob, Ilya A.; Zhang, Zhengcheng] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Su, Chi-Cheung; Feng, Zhenxing; Connell, Justin G.; Liao, Chen; Zhang, Zhengcheng] Argonne Natl Lab, Joint Ctr Energy Storage Res, 9700 S Cass Ave, Argonne, IL 60439 USA. [Connell, Justin G.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [He, Meinan; Wang, Yan] Worcester Polytech Inst, Dept Mech Engineer, 100 Inst Rd, Worcester, MA 01609 USA. RP Zhang, ZC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.; Zhang, ZC (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zzhang@anl.gov FU U.S. Department of Energy, Vehicle Technologies Office; U.S. Department of Energy by UChicago Argonne, LLC [DE-AC02-06CH11357] FX This research is supported by the U.S. Department of Energy, Vehicle Technologies Office. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC, under Contract No. DE-AC02-06CH11357. We would like to thank the Cell Analysis, Modeling, and Prototyping (CAMP) Facility of Argonne's Chemical Sciences and Engineering Division for providing the electrode materials. NR 50 TC 7 Z9 7 U1 41 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 11 PY 2016 VL 8 IS 18 BP 11450 EP 11458 DI 10.1021/acsami.6b01544 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DL3GA UT WOS:000375521000031 PM 27090502 ER PT J AU Quataert, E Fernandez, R Kasen, D Klion, H Paxton, B AF Quataert, Eliot Fernandez, Rodrigo Kasen, Daniel Klion, Hannah Paxton, Bill TI Super-Eddington stellar winds driven by near-surface energy deposition SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE stars: massive; stars: mass-loss; stars: winds; outflows ID CORE-COLLAPSE SUPERNOVAE; OPTICALLY THICK WINDS; WOLF-RAYET STARS; MASSIVE STARS; ASTROPHYSICS MESA; IA SUPERNOVAE; SN 2009IP; HYDRODYNAMIC INSTABILITIES; ETA-CARINAE; ERUPTIONS AB We develop analytic and numerical models of the properties of super-Eddington stellar winds, motivated by phases in stellar evolution when super-Eddington energy deposition (via, e.g., unstable fusion, wave heating, or a binary companion) heats a region near the stellar surface. This appears to occur in the giant eruptions of luminous blue variables (LBVs), Type IIn supernovae progenitors, classical novae, and X-ray bursts. We show that when the wind kinetic power exceeds Eddington, the photons are trapped and behave like a fluid. Convection does not play a significant role in the wind energy transport. The wind properties depend on the ratio of a characteristic speed in the problem v(crit) similar to(EG)(1/5) (where E is the heating rate) to the stellar escape speed near the heating region v(esc)(rh). For v(crit) greater than or similar to vesc(r(h)) the wind kinetic power at large radii E-w less than or similar to E For v(crit) less than or similar to v(esc)(r(h)), most of the energy is used to unbind the wind material and thus E-w less than or similar to E Multidimensional hydrodynamic simulations without radiation diffusion using FLASH and one-dimensional hydrodynamic simulations with radiation diffusion using MESA are in good agreement with the analytic predictions. The photon luminosity from the wind is itself super-Eddington but in many cases the photon luminosity is likely dominated by internal shocks in the wind. We discuss the application of our models to eruptive mass loss from massive stars and argue that the wind models described here can account for the broad properties of LBV outflows and the enhanced mass loss in the years prior to Type IIn core-collapse supernovae. C1 [Quataert, Eliot; Fernandez, Rodrigo; Kasen, Daniel; Klion, Hannah] Univ Calif Berkeley, Astron Dept, Berkeley, CA 94720 USA. [Quataert, Eliot; Fernandez, Rodrigo; Kasen, Daniel; Klion, Hannah] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Quataert, Eliot; Fernandez, Rodrigo; Kasen, Daniel; Klion, Hannah] Univ Calif Berkeley, Theoret Astrophys Ctr, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Nucl Sci Div, Berkeley, CA 94720 USA. [Paxton, Bill] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. RP Quataert, E (reprint author), Univ Calif Berkeley, Astron Dept, Berkeley, CA 94720 USA.; Quataert, E (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Quataert, E (reprint author), Univ Calif Berkeley, Theoret Astrophys Ctr, Berkeley, CA 94720 USA. EM eliot@astro.berkeley.edu FU NSF [AST-1205732, AST-1206097]; Simons Investigator award from the Simons Foundation; David and Lucile Packard Foundation; University of California Office of the President; Department of Energy Office of Nuclear Physics Early Career Award; Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics of the US Department of Energy [DE-AC02-05CH11231]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX We thank Lars Bildsten, Josiah Schwab, and Nathan Smith for useful conversations, and Nathan Smith and the referee for valuable comments on the paper. This work was supported in part by NSF grant AST-1205732. EQ was also supported by a Simons Investigator award from the Simons Foundation and the David and Lucile Packard Foundation. RF acknowledges support from the University of California Office of the President, and from NSF grant AST-1206097. DK is supported in part by a Department of Energy Office of Nuclear Physics Early Career Award, and by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the US Department of Energy under Contract No. DE-AC02-05CH11231. The software used in this work was in part developed by the DOE NNSA-ASC OASCR Flash Center at the University of Chicago. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. FLASH computations were performed at Carver and Hopper (repo2058). NR 55 TC 7 Z9 7 U1 0 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAY 11 PY 2016 VL 458 IS 2 BP 1214 EP 1233 DI 10.1093/mnras/stw365 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DJ9YO UT WOS:000374569600006 ER PT J AU Gor'kov, LP Kresin, VZ AF Gor'kov, Lev P. Kresin, Vladimir Z. TI Pressure and high-T-c superconductivity in sulfur hydrides SO SCIENTIFIC REPORTS LA English DT Article ID STRONG-COUPLED SUPERCONDUCTORS; TRANSITION-TEMPERATURE; LATTICE-VIBRATIONS; METAL; ELECTRONS; HYDROGEN; SYSTEM AB The paper discusses fundamentals of record-T-C superconductivity discovered under high pressure in sulfur hydride. The rapid increase of T-C with pressure in the vicinity of P-cr approximate to 123GPa is interpreted as the fingerprint of a first-order structural transition. Based on the cubic symmetry of the high-T-C phase, it is argued that the lower-T-C phase has a different periodicity, possibly related to an instability with a commensurate structural vector. In addition to the acoustic branches, the phonon spectrum of H3S contains hydrogen modes with much higher frequencies. Because of the complex spectrum, usual methods of calculating T-C are here inapplicable. A modified approach is formulated and shown to provide realistic values for T-C and to determine the relative contributions of optical and acoustic branches. The isotope effect ( change of T-C upon Deuterium for Hydrogen substitution) originates from high frequency phonons and differs in the two phases. The decrease of T-C following its maximum in the high-T-C phase is a sign of intermixing with pairing at hole-like pockets which arise in the energy spectrum of the cubic phase at the structural transition. On-pockets pairing leads to the appearance of a second gap and is remarkable for its non-adiabatic regime: hydrogen mode frequencies are comparable to the Fermi energy. C1 [Gor'kov, Lev P.] Florida State Univ, NHMFL, 1800 East Paul Dirac Dr, Tallahassee, FL 32310 USA. [Gor'kov, Lev P.] RAS, LD Landau Theoret Phys Inst, Chernogolovka 142432, Russia. [Kresin, Vladimir Z.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Gor'kov, LP (reprint author), Florida State Univ, NHMFL, 1800 East Paul Dirac Dr, Tallahassee, FL 32310 USA.; Gor'kov, LP (reprint author), RAS, LD Landau Theoret Phys Inst, Chernogolovka 142432, Russia. EM gorkov@magnet.fsu.edu FU National High Magnetic Field Laboratory through NSF Grant [DMR-1157490]; State of Florida; U.S. Department of Energy; Lawrence Berkeley National Laboratory; University of California at Berkeley FX The authors thank M.I. Eremets for clarification of a number of significant experimental details and providing us with more useful literature references and to M. Calandra for stimulating discussions and sharing some of his theoretical results before publication. The work of LPG is supported by the National High Magnetic Field Laboratory through NSF Grant No. DMR-1157490, the State of Florida and the U.S. Department of Energy. The work of VZK is supported by the Lawrence Berkeley National Laboratory, University of California at Berkeley, and the U.S. Department of Energy. NR 47 TC 6 Z9 6 U1 15 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 11 PY 2016 VL 6 AR 25608 DI 10.1038/srep25608 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL6OC UT WOS:000375757500001 PM 27167334 ER PT J AU Duxbury, PM Granlund, L Gujarathi, SR Juhas, P Billinge, SJL AF Duxbury, P. M. Granlund, L. Gujarathi, S. R. Juhas, P. Billinge, S. J. L. TI The unassigned distance geometry problem SO DISCRETE APPLIED MATHEMATICS LA English DT Article DE Nanostructure; Rigid cluster; Percolation; Unassigned distances; LIGA; TRIBOND ID MACROMOLECULAR STRUCTURE DETERMINATION; GENERIC RIGIDITY PERCOLATION; PAIR DISTRIBUTION-FUNCTIONS; AB-INITIO DETERMINATION; CONNECTIVITY PERCOLATION; GLOBAL RIGIDITY; 2 DIMENSIONS; PEBBLE GAME; ALGORITHM; GRAPHS AB Studies of distance geometry problems (DGP) have focused on cases where the vertices at the ends of all or most of the given distances are known or assigned, which we call assigned distance geometry problems (aDGPs). In this contribution we consider the unassigned distance geometry problem (uDGP) where the vertices associated with a given distance are unknown, so the graph structure has to be discovered. uDGPs arises when attempting to find the atomic structure of molecules and nanoparticles using X-ray or neutron diffraction data from non-crystalline materials. Rigidity theory provides a useful foundation for both aDGPs and uDGPs, though it is restricted to generic realizations of graphs, and key results are summarized. Conditions for unique realization are discussed for aDGP and uDGP cases, build-up algorithms for both cases are described and experimental results for uDGP are presented. (C) 2015 The Authors. Published by Elsevier B.V. C1 [Duxbury, P. M.; Granlund, L.; Gujarathi, S. R.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Juhas, P.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. [Billinge, S. J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Duxbury, PM (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM duxbury@pa.msu.edu OI Juhas, Pavol/0000-0001-8751-4458 FU MSU foundation; U.S. Department of Energy Office of Basic Energy Sciences (DOE-BES), as the Complex Modeling laboratory directed research and development grant at Brookhaven National Laboratory [DE-AC02-98CH10886] FX Support for work at Michigan State University by the MSU foundation is gratefully acknowledged. PMD would like to thank Carlile Lavor and Leo Liberti for interesting and motivating discussions and the referees for very constructive suggestions. He also thanks Bob Connelly for helpful and entertaining email correspondence. Work in the Billinge group was supported by the U.S. Department of Energy Office of Basic Energy Sciences (DOE-BES), as the Complex Modeling laboratory directed research and development grant at Brookhaven National Laboratory through Contract DE-AC02-98CH10886. NR 51 TC 1 Z9 1 U1 2 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0166-218X EI 1872-6771 J9 DISCRETE APPL MATH JI Discret Appl. Math. PD MAY 11 PY 2016 VL 204 BP 117 EP 132 DI 10.1016/j.dam.2015.10.029 PG 16 WC Mathematics, Applied SC Mathematics GA DJ6WQ UT WOS:000374354300010 ER PT J AU Wallace, DC De Lorenzi-Venneri, G Chisolm, ED AF Wallace, Duane C. De Lorenzi-Venneri, Giulia Chisolm, Eric D. TI Atomic motion from the mean square displacement in a monatomic liquid SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE liquid theory; Hamiltonian; atomic motion in liquids; statistical mechanics; dynamic response ID SUPERCOOLED LIQUIDS; SELF-DIFFUSION; DYNAMICS AB V-T theory is constructed in the many-body Hamiltonian formulation, and is being developed as a novel approach to liquid dynamics theory. In this theory the liquid atomic motion consists of two contributions, normal mode vibrations in a single representative potential energy valley, and transits, which carry the system across boundaries between valleys. The mean square displacement time correlation function (the MSD) is a direct measure of the atomic motion, and our goal is to determine if the V-T formalism can produce a physically sensible account of this motion. We employ molecular dynamics (MD) data for a system representing liquid Na, and find the motion evolves in three successive time intervals: on the first 'vibrational' interval, the vibrational motion alone gives a highly accurate account of the MD data; on the second 'crossover' interval, the vibrational MSD saturates to a constant while the transit motion builds up from zero; on the third 'random walk' interval, the transit motion produces a purely diffusive random walk of the vibrational equilibrium positions. This motional evolution agrees with, and adds refinement to, the MSD atomic motion as described by current liquid dynamics theories. C1 [Wallace, Duane C.; De Lorenzi-Venneri, Giulia] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chisolm, Eric D.] Descartes Labs, Los Alamos, NM 87544 USA. RP De Lorenzi-Venneri, G (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM gvenneri@lanl.gov FU Department of Energy [DE-AC52-06NA25396] FX We are pleased to thank B Clements, L Collins, J Kress and A Voter for helpful and encouraging discussions. This research is supported by the Department of Energy under Contract No. DE-AC52-06NA25396. NR 32 TC 1 Z9 1 U1 3 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 11 PY 2016 VL 28 IS 18 AR 185101 DI 10.1088/0953-8984/28/18/185101 PG 6 WC Physics, Condensed Matter SC Physics GA DJ7LX UT WOS:000374394000010 PM 27058024 ER PT J AU Akerib, DS Araujo, HM Bai, X Bailey, AJ Balajthy, J Beltrame, P Bernard, EP Bernstein, A Biesiadzinski, TP Boulton, EM Bradley, A Bramante, R Cahn, SB Carmona-Benitez, MC Chan, C Chapman, JJ Chiller, AA Chiller, C Currie, A Cutter, JE Davison, TJR de Viveiros, L Dobi, A Dobson, JEY Druszkiewicz, E Edwards, BN Faham, CH Fiorucci, S Gaitskell, RJ Gehmang, VM Ghag, C Gibson, KR Gilchriese, MGD Hall, CR Hanhardt, M Haselschwardt, SJ Herter, SA Hogan, DP Horn, M Huang, DQ Ignarra, CM Ihm, M Jacobsen, RG Ji, W Kazkaz, K Khaitang, D Knoche, R Larsen, NA Lee, C Lenardo, BG Lesko, KT Lindote, A Lopes, MI Mailing, DC Manalaysay, AG Mannino, RL Marzioni, MF McKinsey, DN Mei, DM Mock, J Moongweluwan, M Morad, JA Murphy, ASJ Nehrkorn, C Nelson, HN Neves, E O'Sullivan, K Oliver-Mallory, KC Ott, RA Palladino, KJ Pangilinan, M Pease, EK Phelps, P Reichhart, L Rhyne, C Shaw, S Shutt, TA Silva, C Skulski, W Solovovn, VN Sorensen, P Stephenson, S Sumner, TJ Szydagis, M Taylor, DJ Taylor, W Tennyson, BP Terman, PA Tiedt, DR To, WH Tripathi, M Tyrznikova, L Uvarov, S Verbus, JR Webb, RC White, JT Whitis, TJ Witherell, MS Wolfs, FLH Yin, J Young, SK Zhang, C AF Akerib, D. S. Araujo, H. M. Bai, X. Bailey, A. J. Balajthy, J. Beltrame, P. Bernard, E. P. Bernstein, A. Biesiadzinski, T. P. Boulton, E. M. Bradley, A. Bramante, R. Cahn, S. B. Carmona-Benitez, M. C. Chan, C. Chapman, J. J. Chiller, A. A. Chiller, C. Currie, A. Cutter, J. E. Davison, T. J. R. de Viveiros, L. Dobi, A. Dobson, J. E. Y. Druszkiewicz, E. Edwards, B. N. Faham, C. H. Fiorucci, S. Gaitskell, R. J. Gehmang, V. M. Ghag, C. Gibson, K. R. Gilchriese, M. G. D. Hall, C. R. Hanhardt, M. Haselschwardt, S. J. Herter, S. A. Hogan, D. P. Horn, M. Huang, D. Q. Ignarra, C. M. Ihm, M. Jacobsen, R. G. Ji, W. Kazkaz, K. Khaitang, D. Knoche, R. Larsen, N. A. Lee, C. Lenardo, B. G. Lesko, K. T. Lindote, A. Lopes, M. I. Mailing, D. C. Manalaysay, A. G. Mannino, R. L. Marzioni, M. F. McKinsey, D. N. Mei, D. -M. Mock, J. Moongweluwan, M. Morad, J. A. Murphy, A. St. J. Nehrkorn, C. Nelson, H. N. Neves, E. O'Sullivan, K. Oliver-Mallory, K. C. Ott, R. A. Palladino, K. J. Pangilinan, M. Pease, E. K. Phelps, P. Reichhart, L. Rhyne, C. Shaw, S. Shutt, T. A. Silva, C. Skulski, W. Solovovn, V. N. Sorensen, P. Stephenson, S. Sumner, T. J. Szydagis, M. Taylor, D. J. Taylor, W. Tennyson, B. P. Terman, P. A. Tiedt, D. R. To, W. H. Tripathi, M. Tyrznikova, L. Uvarov, S. Verbus, J. R. Webb, R. C. White, J. T. Whitis, T. J. Witherell, M. S. Wolfs, F. L. H. Yin, J. Young, S. K. Zhang, C. TI FPGA-based trigger system for the LUX dark matter experiment SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Trigger; Dark matter detectors; DSP; FPGA; DAQ; Baseline subtraction AB LUX is a two-phase (liquid/gas) xenon time projection chamber designed to detect nuclear recoils resulting from interactions with dark matter particles. Signals from the detector are processed with an FPGA-based digital trigger system that analyzes the incoming data in real-time, with just a few microsecond latency. The system enables first pass selection of events of interest based on their pulse shape characteristics and 3D localization of the interactions. It has been shown to be > 99% efficient in triggering on S2 signals induced by only few extracted liquid electrons. It is continuously and reliably operating since its full underground deployment in early 2013. This document is an overview of the systems capabilities, its inner workings, and its performance. (C) 2016 Elsevier B.V. All rights reserved. C1 [Akerib, D. S.; Biesiadzinski, T. P.; Bradley, A.; Bramante, R.; Gibson, K. R.; Ji, W.; Lee, C.; Phelps, P.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Case Western Reserve Univ, Dept Phys, 10900 Euclid Ave, Cleveland, OH 44106 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94205 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94309 USA. [Araujo, H. M.; Bailey, A. J.; Currie, A.; Sumner, T. J.] Univ London Imperial Coll Sci Technol & Med, High Energy Phys, Blackett Lab, London SW7 2BZ, England. [Bai, X.; Hanhardt, M.; Tiedt, D. R.] South Dakota Sch Mines & Technol, 501 East St Joseph St, Rapid City, SD 57701 USA. [Balajthy, J.; Hall, C. R.; Knoche, R.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beltrame, P.; Davison, T. J. R.; Marzioni, M. F.; Murphy, A. St. J.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh EH9 3FD, Midlothian, Scotland. [Bernard, E. P.; Boulton, E. M.; Cahn, S. B.; Edwards, B. N.; Herter, S. A.; Horn, M.; Larsen, N. A.; McKinsey, D. N.; O'Sullivan, K.; Pease, E. K.; Tennyson, B. P.; Tyrznikova, L.] Yale Univ, Dept Phys, 217 Prospect St, New Haven, CT 06511 USA. [Bernstein, A.; Kazkaz, K.; Lenardo, B. G.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. [Carmona-Benitez, M. C.; Haselschwardt, S. J.; Nehrkorn, C.; Nelson, H. N.; Witherell, M. S.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Chan, C.; Chapman, J. J.; Fiorucci, S.; Gaitskell, R. J.; Huang, D. Q.; Mailing, D. C.; Pangilinan, M.; Rhyne, C.; Taylor, W.; Verbus, J. R.] Brown Univ, Dept Phys, 182 Hope St, Providence, RI 02912 USA. [Chiller, A. A.; Chiller, C.; Mei, D. -M.; Zhang, C.] Univ S Dakota, Dept Phys, 414E Clark St, Vermillion, SD 57069 USA. [Cutter, J. E.; Lenardo, B. G.; Manalaysay, A. G.; Morad, J. A.; Ott, R. A.; Stephenson, S.; Tripathi, M.; Uvarov, S.] Univ Calif Davis, Dept Phys, 1 Shields Ave, Davis, CA 95616 USA. [de Viveiros, L.; Lindote, A.; Lopes, M. I.; Neves, E.; Silva, C.; Solovovn, V. N.] Univ Coimbra, Dept Phys, LIP Coimbra, Rua Larga, P-3004516 Coimbra, Portugal. [Dobi, A.; Faham, C. H.; Gehmang, V. M.; Gilchriese, M. G. D.; Lesko, K. T.; O'Sullivan, K.; Sorensen, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Dobson, J. E. Y.; Ghag, C.; Reichhart, L.; Shaw, S.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Druszkiewicz, E.; Khaitang, D.; Moongweluwan, M.; Skulski, W.; Wolfs, F. L. H.; Yin, J.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Hanhardt, M.; Taylor, D. J.] South Dakota Sci & Technol Author, Sanford Underground Res Facil, Lead, SD 57754 USA. [Herter, S. A.; Hogan, D. P.; Horn, M.; Ihm, M.; Jacobsen, R. G.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mannino, R. L.; Terman, P. A.; Webb, R. C.; White, J. T.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Mock, J.; Szydagis, M.; Young, S. K.] SUNY Albany, Dept Phys, 1400 Washington Ave, Albany, NY 12222 USA. RP Druszkiewicz, E (reprint author), Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. EM eyrk.druszkiewicz@rochester.edu OI Tvrznikova, Lucie/0000-0002-0394-7692 FU U.S. Department of Energy (DOE) [DE-FG02-08ER41549, DE-FG02-91ER40688, DE-FG02-95ER40917, DE-FG02-91ER40674, DE-NA0000979, DE-FG02-11ER41738, DE-SC0006605, DE-AC02-05CH11231, DE-AC52-07NA27344, DE-FG01-91ER40618]; U.S. National Science Foundation [PHYS-0750671, PHY-0801536, PHY-1004661, PHY-1102470, PHY-1003660, PHY-1312561, PHY-1347449]; Research Corporation grant [RA0350]; South Dakota Governor's Office Economic Development; Board of Regents for Center for Ultra-low Background Experiments in the Dakotas (CUBED); South Dakota School of Mines and Technology (SDSMT) [NSF: PHY-1242579, RES507395, DOE: DE-5C0014223]; Fundac ao para a Ciencia e a Tecnologia (FCT) [CERN/FP/123610/2011]; Imperial College and Brown University thank the UK Royal Society [IE120804]; Science & Technology Facilities Council [ST/K502042/1] FX This work was partially supported by the U.S. Department of Energy (DOE) under award numbers DE-FG02-08ER41549, DE-FG02-91ER40688, DE-FG02-95ER40917, DE-FG02-91ER40674, DE-NA0000979, DE-FG02-11ER41738, DE-SC0006605, DE-AC02-05CH11231, DE-AC52-07NA27344, and DE-FG01-91ER40618; the U.S. National Science Foundation under award numbers PHYS-0750671, PHY-0801536, PHY-1004661, PHY-1102470, PHY-1003660, PHY-1312561, PHY-1347449; the Research Corporation grant RA0350; the South Dakota Governor's Office Economic Development and the Board of Regents for Center for Ultra-low Background Experiments in the Dakotas (CUBED); and the South Dakota School of Mines and Technology (SDSMT) (NSF: PHY-1242579, Subaward: RES507395 and DOE: DE-5C0014223). LIP-Coimbra acknowledges funding from Fundac ao para a Ciencia e a Tecnologia (FCT) through the project-grant CERN/FP/123610/2011. Imperial College and Brown University thank the UK Royal Society for travel funds under the International Exchange Scheme (IE120804). The UK groups acknowledge institutional support from Imperial College London, University College London and Edinburgh University, and from the Science & Technology Facilities Council for PhD studentship ST/K502042/1 (AB). The University of Edinburgh is a charitable body, registered in Scotland, with registration number SC005336. NR 14 TC 1 Z9 1 U1 1 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2016 VL 818 BP 57 EP 67 DI 10.1016/j.nima.2016.02.017 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DG0PS UT WOS:000371768400010 ER PT J AU Upadhyay, J Im, D Peshl, J Basovic, M Popovic, S Valente-Feliciano, AM Phillips, L Vuskovic, L AF Upadhyay, J. Im, Do Peshl, J. Basovic, M. Popovic, S. Valente-Feliciano, A. -M. Phillips, L. Vuskovic, L. TI Apparatus and method for plasma processing of SRF cavities SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Plasma processing; Uniform plasma-surface interaction; Asymmetric plasma; SRF cavity AB An apparatus and a method are described for plasma etching of the inner surface of superconducting radio frequency (SRF) cavities. Accelerator SRF cavities are formed into a variable-diameter cylindrical structure made of bulk niobium, for resonant generation of the particle accelerating field. The etch rate non-uniformity due to depletion of the radicals has been overcome by the simultaneous movement of the gas flow inlet and the inner electrode. An effective shape of the inner electrode to reduce the plasma asymmetry for the coaxial cylindrical rf plasma reactor is determined and implemented in the cavity processing method. The processing was accomplished by moving axially the inner electrode and the gas flow inlet in a step-wise way to establish segmented plasma columns. The test structure was a pillbox cavity made of steel of similar dimension to the standard SRF cavity. This was adopted to experimentally verify the plasma surface reaction on cylindrical structures with variable diameter using the segmented plasma generation approach. The pill box cavity is filled with niobium ring- and disk-type samples and the etch rate of these samples was measured. (C) 2016 Elsevier B.V. All rights reserved. C1 [Upadhyay, J.; Im, Do; Peshl, J.; Popovic, S.; Vuskovic, L.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Upadhyay, J.; Im, Do; Peshl, J.; Basovic, M.; Popovic, S.; Vuskovic, L.] Old Dominion Univ, Ctr Accelerator Sci, Norfolk, VA 23529 USA. [Basovic, M.] Old Dominion Univ, Dept Mech Engn, Norfolk, VA 23529 USA. [Valente-Feliciano, A. -M.; Phillips, L.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Upadhyay, J (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Upadhyay, J (reprint author), Old Dominion Univ, Ctr Accelerator Sci, Norfolk, VA 23529 USA. EM jupad001@odu.edu FU Office of High Energy Physics, Office of Science, Department of Energy [DE-SC0007879]; JSA/DOE [DE-AC05-060R23177] FX This work is supported by the Office of High Energy Physics, Office of Science, Department of Energy under Grant no. DE-SC0007879. Thomas Jefferson National Accelerator Facility, Accelerator Division supports J. Upadhyay through a fellowship under JSA/DOE Contract no. DE-AC05-060R23177. NR 13 TC 0 Z9 0 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAY 11 PY 2016 VL 818 BP 76 EP 81 DI 10.1016/j.nima.2016.02.049 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DG0PS UT WOS:000371768400012 ER PT J AU Yang, K Cai, ZK Tyagi, M Feygenson, M Neuefeind, JC Moore, JS Zhang, Y AF Yang, Ke Cai, Zhikun Tyagi, Madhusudan Feygenson, Mikhail Neuefeind, Joerg C. Moore, Jeffrey S. Zhang, Yang TI Odd-Even Structural Sensitivity on Dynamics in Network-Forming Ionic Liquids SO CHEMISTRY OF MATERIALS LA English DT Article ID COLD NEUTRON SCATTERING; PHYSICAL-PROPERTIES; CATION SYMMETRY; ORGANIZATION; FABRICATION; ALTERNATION; CRYSTALS; POLYMER; BOTTOM; LENGTH AB As a compelling case of sensitive structure property-relationship, an odd even effect refers to the alternating trend of physical or chemical properties on odd/even number of repeating structural units. In crystalline or semicrystalline materials, such odd even effects emerge as manifestations of differences in the periodic packing patterns of molecules. Therefore, due to the lack of long-range order, such an odd-even phenomenon is not expected for dynamic properties in amorphous state. Herein, we report the discovery of a remarkable odd-even effect of dynamical properties in the liquid phase. In a class of glass forming diammonium citrate ionic liquids, using incoherent quasi-elastic neutron scattering measurements, we measured the dynamical properties including diffusion coefficient and rotational relaxation time. These directly measured molecular dynamics showed pronounced alternating trends with increased number of methylene (-CH2-) groups in the backbone. Meanwhile, the structure factor S(Q) showed no long-range periodic packing of molecules, while the pair distribution function G(r) revealed subtle differences in the local molecular morphology. The observed dynamical odd even phenomenon in liquids showed that profound dynamical changes originate from subtle local structural differences. C1 [Yang, Ke; Moore, Jeffrey S.; Zhang, Yang] Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. [Yang, Ke; Moore, Jeffrey S.; Zhang, Yang] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Cai, Zhikun; Zhang, Yang] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Moore, Jeffrey S.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Tyagi, Madhusudan] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Feygenson, Mikhail; Neuefeind, Joerg C.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Tyagi, Madhusudan] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Moore, JS; Zhang, Y (reprint author), Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA.; Moore, JS; Zhang, Y (reprint author), Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA.; Zhang, Y (reprint author), Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. EM jsmoore@illinois.edu; zhyang@illinois.edu RI Neuefeind, Joerg/D-9990-2015; Zhang, Yang/A-7975-2012; OI Neuefeind, Joerg/0000-0002-0563-1544; Zhang, Yang/0000-0002-7339-8342; Yang, Ke/0000-0002-0184-9124; Feygenson, Mikhail /0000-0002-0316-3265 FU ACS PRF [55642-DNI6]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-SC-0014804]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Y.Z. is supported by ACS PRF 55642-DNI6 and by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Award DE-SC-0014804. This work utilized facilities supported in part by the National Science Foundation under Agreement DMR-1508249. Part of the research conducted at ORNL's SNS and ANL's APS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 38 TC 1 Z9 1 U1 2 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2016 VL 28 IS 9 BP 3227 EP 3233 DI 10.1021/acs.chemmater.6b01429 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DL7HA UT WOS:000375810400039 ER PT J AU Qin, J de Pablo, JJ AF Qin, Jian de Pablo, Juan J. TI Ordering Transition in Salt-Doped Diblock Copolymers SO MACROMOLECULES LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; MINIMAL LATTICE MODEL; BLOCK-COPOLYMERS; PHASE-BEHAVIOR; MICROPHASE SEPARATION; POLYMER ELECTROLYTES; DISORDER TRANSITION; MELTS; BLENDS; DENSITY AB Lithium salt-doped block copolymers offer promise for applications as solid electrolytes in lithium ion batteries. Control of the conductivity and mechanical properties of these materials, for membrane applications relies critically on the ability to predict and manipulate their microphase separation temperature. Past attempts to predict the so-called "order-disorder transition temperature" of copolymer electrolytes have relied on approximate treatments of electrostatic interactions. In this work, we introduce a coarse-grained simulation model that treats Coulomb interactions explicitly, and we use it to investigate the ordering transition of charged block copolymers. The order-disorder transition temperature is determined from the ordering free energy, which we calculate with a high level of precision using a density-of-states approach. Our calculations allow us to discern a delicate competition between two physical effects: ion association, which raises the transition temperature, and solvent dilution, which lowers the transition temperature. In the intermediate salt concentration regime, our results predict that the order-disorder transition temperature increases with salt content, in agreement with available experimental data. C1 [Qin, Jian; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Qin, Jian; de Pablo, Juan J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Qin, Jian] Stanford Univ, Dept Chem Engn, Stanford, CA 93405 USA. RP de Pablo, JJ (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA.; de Pablo, JJ (reprint author), Argonne Natl Lab, Argonne, IL 60439 USA. EM depablo@uchicago.edu FU Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We acknowledge helpful discussions with Jens Glaser and David Morse for details regarding the choice of order parameter. This work was supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 46 TC 0 Z9 0 U1 2 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2016 VL 49 IS 9 BP 3630 EP 3638 DI 10.1021/acs.macromol.5b02643 PG 9 WC Polymer Science SC Polymer Science GA DL7GT UT WOS:000375809700045 ER PT J AU Orsini, L Gilbert, D Podicheti, R Jansen, M Brown, JB Solari, OS Spanier, KI Colbourne, JK Rush, D Decaestecker, E Asselman, J De Schamphelaere, KAC Ebert, D Haag, CR Kvist, J Laforsch, C Petrusek, A Beckerman, AP Little, TJ Chaturvedi, A Pfrender, ME De Meester, L Frilander, MJ AF Orsini, Luisa Gilbert, Donald Podicheti, Ram Jansen, Mieke Brown, James B. Solari, Omid Shams Spanier, Katina I. Colbourne, John K. Rush, Douglas Decaestecker, Ellen Asselman, Jana De Schamphelaere, Karel A. C. Ebert, Dieter Haag, Christoph R. Kvist, Jouni Laforsch, Christian Petrusek, Adam Beckerman, Andrew P. Little, Tom J. Chaturvedi, Anurag Pfrender, Michael E. De Meester, Luc Frilander, Mikko J. TI Daphnia magna transcriptome by RNA-Seq across 12 environmental stressors SO SCIENTIFIC DATA LA English DT Article ID FUNCTIONAL GENOMICS; ECOSYSTEMS DAPHNIA; WATERFLEA DAPHNIA; MODEL; MAP; ZOOPLANKTON; COMMUNITIES; ADAPTATION; EVOLUTION; RESPONSES AB The full exploration of gene-environment interactions requires model organisms with well-characterized ecological interactions in their natural environment, manipulability in the laboratory and genomic tools. The waterflea Daphnia magna is an established ecological and toxicological model species, central to the food webs of freshwater lentic habitats and sentinel for water quality. Its tractability and cyclic parthenogenetic life-cycle are ideal to investigate links between genes and the environment. Capitalizing on this unique model system, the STRESSFLEA consortium generated a comprehensive RNA-Seq data set by exposing two inbred genotypes of D. magna and a recombinant cross of these genotypes to a range of environmental perturbations. Gene models were constructed from the transcriptome data and mapped onto the draft genome of D. magna using EvidentialGene. The transcriptome data generated here, together with the available draft genome sequence of D. magna and a high-density genetic map will be a key asset for future investigations in environmental genomics. C1 [Orsini, Luisa; Colbourne, John K.] Univ Birmingham, Sch Biosci, Environm Genom Grp, Birmingham B15 2TT, W Midlands, England. [Gilbert, Donald] Indiana Univ, Dept Biol, 1001 E Third St, Bloomington, IN 47405 USA. [Podicheti, Ram] Indiana Univ, Sch Informat & Comp, 919 E Tenth St, Bloomington, IN 47408 USA. [Podicheti, Ram; Rush, Douglas] Indiana Univ, Sch Informat & Comp, Ctr Genom & Bioinformat, 1001 E Third St,919 E Tenth St, Bloomington, IN 47408 USA. [Jansen, Mieke; Spanier, Katina I.; Chaturvedi, Anurag; De Meester, Luc] Univ Leuven, Lab Aquat Ecol Evolut & Conservat, Ch Deberiotstr 32, B-3000 Leuven, Belgium. [Brown, James B.; Solari, Omid Shams] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Decaestecker, Ellen] Katholieke Univ Leuven, Interdisciplinary Res Facil Life Sci, Aquat Biol, Campus Kortrijk,E Sabbelaan 53, B-8500 Kortrijk, Belgium. [Asselman, Jana; De Schamphelaere, Karel A. C.] Univ Ghent, Lab Environm Toxicol & Aquat Ecol, GhEnToxLab, Ghent, Belgium. [Ebert, Dieter] Univ Basel, Zool Inst, Vesalgasse 1, CH-4051 Basel, Switzerland. [Haag, Christoph R.] Univ Montpellier, Univ Paul Valery Montpellier, EPHE, CEFE UMR 5175,CNRS, Campus CNRS 1919,Route Mende, F-34293 Montpellier 5, France. [Kvist, Jouni; Frilander, Mikko J.] Univ Helsinki, Inst Biotechnol, POB 56,Viikinkaari 9, Helsinki 00014, Finland. [Laforsch, Christian] Univ Bayreuth, Anim Ecol 1, D-95440 Bayreuth, Germany. [Laforsch, Christian] Univ Bayreuth, Bayreuth Ctr Ecol & Environm Res BayCEER, D-95440 Bayreuth, Germany. [Petrusek, Adam] Charles Univ Prague, Fac Sci, Dept Ecol, Vinicni 7, CZ-12844 Prague, Czech Republic. [Beckerman, Andrew P.] Univ Sheffield, Dept Anim & Plant Sci, Alfred Denny Bldg, Sheffield S10 2TN, S Yorkshire, England. [Little, Tom J.] Univ Edinburgh, Ashworth Labs, Inst Evolutionary Biol, Kings Bldg, Edinburgh EH9 3JT, Midlothian, Scotland. [Pfrender, Michael E.] Galvin Life Sci Ctr, Dept Biol Sci, Notre Dame, IN 46556 USA. [Pfrender, Michael E.] Galvin Life Sci Ctr, Environm Change Initiat, Notre Dame, IN 46556 USA. RP Orsini, L (reprint author), Univ Birmingham, Sch Biosci, Environm Genom Grp, Birmingham B15 2TT, W Midlands, England. EM l.orsini@bham.ac.uk RI Petrusek, Adam/A-3510-2008; Little, Tom/B-7890-2009; Frilander, Mikko/B-6660-2009; Ebert, Dieter/B-5502-2009; OI Petrusek, Adam/0000-0001-5150-4370; Little, Tom/0000-0002-8945-0416; Frilander, Mikko/0000-0002-1732-4808; Ebert, Dieter/0000-0003-2653-3772; Orsini, Luisa/0000-0002-1716-5624; Asselman, Jana/0000-0003-0185-6516; Kvist, Jouni/0000-0002-4089-8877 FU ESF EUROCORES Programme EuroEEFG [09-EEFG-FP-040]; FWO project STRESSFLEA-B [G061411N]; KU Leuven Research Fund [PF/2010/07]; NIH grant [R24-GM078274]; Academy of Finland [250444, 284601, 135291]; National Science Foundation [0640462]; FWO scholarship FX This research was financially supported by the ESF EUROCORES Programme EuroEEFG, Grant 09-EEFG-FP-040. The KU Leuven team was supported by FWO project STRESSFLEA-B (G061411N) and by the KU Leuven Research Fund (coordination grant and grant PF/2010/07). Kevin Pauwels helped with the exposure experiments; Veerle Lemaire, Aline Waterkeyn, Isabel Vanoverberghe and Nellie Konijnendijck provided material for exposures. The University of Notre Dame team was supported by NIH grant R24-GM078274 to MEP. The University of Helsinki Team was supported by Academy of Finland grants 250444, 284601 and 135291. Sayanty Roy, Kerry Regan, Jihyun Won and Jackie Lopez conducted the exposure experiments and RNA isolation for the recombinant genotype. Seanna McTaggart provided additional RNA-seq transcriptome clone data for the public D. magna gene set. Donald Gilbert has been supported by the National Science Foundation (grant No. 0640462 to DGG), including genomics computational resources via TeraGrid amd XSEDE. Jana Asselman is the recipient of a FWO scholarship. NR 49 TC 5 Z9 5 U1 17 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2052-4463 J9 SCI DATA JI Sci. Data PD MAY 10 PY 2016 VL 3 AR UNSP 160030 DI 10.1038/sdata.2016.30 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EF3HN UT WOS:000390215500001 PM 27164179 ER PT J AU Jenkins, RW Moore, CM Semelsberger, TA Chuck, CJ Gordon, JC Sutton, AD AF Jenkins, Rhodri W. Moore, Cameron M. Semelsberger, Troy A. Chuck, Christopher J. Gordon, John C. Sutton, Andrew D. TI The Effect of Functional Groups in Bio-Derived Fuel Candidates SO CHEMSUSCHEM LA English DT Article DE biofuel; biomass; fuels; renewable; review ID TAILOR-MADE FUELS; DIESEL COMBUSTION; FAST PYROLYSIS; CETANE NUMBER; METHYL-ESTER; N-ALKANES; BIOFUELS; BIOMASS; GASOLINE; ISOMERIZATION AB Interest in developing renewable fuels is continuing to grow and biomass represents a viable source of renewable carbon with which to replace fossil-based components in transportation fuels. During our own work, we noticed that chemists think in terms of functional groups whereas fuel engineers think in terms of physical fuel properties. In this Concept article, we discuss the effect of carbon and oxygen functional groups on potential fuel properties. This serves as a way of informing our own thinking and provides us with a basis with which to design and synthesize molecules from biomass that could provide useful transportation fuels. C1 [Jenkins, Rhodri W.; Moore, Cameron M.; Gordon, John C.; Sutton, Andrew D.] Los Alamos Natl Lab, Div Chem, MS K558, Los Alamos, NM 87544 USA. [Semelsberger, Troy A.] Los Alamos Natl Lab, Mat Phys Applicat Div, MS K793, Los Alamos, NM 87544 USA. [Chuck, Christopher J.] Univ Bath, Dept Chem Engn, Bath BA2 7AY, Avon, England. RP Sutton, AD (reprint author), Los Alamos Natl Lab, Div Chem, MS K558, Los Alamos, NM 87544 USA. EM adsutton@lanl.gov OI Sutton, Andrew/0000-0001-7984-1715 FU Los Alamos National Laboratory LDRD program [LDRD20160095ER]; Office of Energy Efficiency & Renewable Energy (EERE) Bioenergy Technology Office [WBS 2.3.1.103]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC5206A25396] FX We are grateful to the Los Alamos National Laboratory LDRD program (LDRD20160095ER) and the Office of Energy Efficiency & Renewable Energy (EERE) Bioenergy Technology Office (WBS 2.3.1.103) for financial support. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC5206A25396. NR 65 TC 3 Z9 3 U1 16 U2 23 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD MAY 10 PY 2016 VL 9 IS 9 BP 922 EP 931 DI 10.1002/cssc.201600159 PG 10 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DP6UO UT WOS:000378634800002 PM 27099975 ER PT J AU Oh, S Flynn, RA Floor, SN Purzner, J Martin, L Do, BT Schubert, S Vaka, D Morrissy, S Li, YS Kool, M Hovestadt, V Jones, DTW Northcott, PA Risch, T Warnatz, HJ Yaspo, ML Adams, CM Leib, RD Breese, M Marra, MA Malkin, D Lichter, P Doudna, JA Pfister, SM Taylor, MD Chang, HY Cho, YJ AF Oh, Sekyung Flynn, Ryan A. Floor, Stephen N. Purzner, James Martin, Lance Do, Brian T. Schubert, Simone Vaka, Dedeepya Morrissy, Sorana Li, Yisu Kool, Marcel Hovestadt, Volker Jones, David T. W. Northcott, Paul A. Risch, Thomas Warnatz, Hans-Joerg Yaspo, Marie-Laure Adams, Christopher M. Leib, Ryan D. Breese, Marcus Marra, Marco A. Malkin, David Lichter, Peter Doudna, Jennifer A. Pfister, Stefan M. Taylor, Michael D. Chang, Howard Y. Cho, Yoon-Jae TI Medulloblastoma-associated DDX3 variant selectively alters the translational response to stress SO ONCOTARGET LA English DT Article DE medulloblastoma; DDX3X; DDX3; RNA helicase; CLIP-seq ID RNA HELICASE DDX3; BOX PROTEIN DDX3; GRANULES; GENOME; CANCER; RESOLUTION; INHIBITION; EXPRESSION; ALIGNMENT; RIBOSOME AB DDX3X encodes a DEAD-box family RNA helicase (DDX3) commonly mutated in medulloblastoma, a highly aggressive cerebellar tumor affecting both children and adults. Despite being implicated in several facets of RNA metabolism, the nature and scope of DDX3's interactions with RNA remain unclear. Here, we show DDX3 collaborates extensively with the translation initiation machinery through direct binding to 5'UTRs of nearly all coding RNAs, specific sites on the 18S rRNA, and multiple components of the translation initiation complex. Impairment of translation initiation is also evident in primary medulloblastomas harboring mutations in DDX3X, further highlighting DDX3's role in this process. Arsenite-induced stress shifts DDX3 binding from the 5'UTR into the coding region of mRNAs concomitant with a general reduction of translation, and both the shift of DDX3 on mRNA and decreased translation are blunted by expression of a catalytically-impaired, medulloblastoma-associated DDX3(R534H) variant. Furthermore, despite the global repression of translation induced by arsenite, translation is preserved on select genes involved in chromatin organization in DDX3(R534H)-expressing cells. Thus, DDX3 interacts extensively with RNA and ribosomal machinery to help remodel the translation landscape in response to stress, while cancer-related DDX3 variants adapt this response to selectively preserve translation. C1 [Oh, Sekyung; Schubert, Simone; Vaka, Dedeepya; Cho, Yoon-Jae] Stanford Univ, Sch Med, Dept Neurol & Neurol Sci, Stanford, CA 94305 USA. [Oh, Sekyung; Cho, Yoon-Jae] Stanford Univ, Sch Med, Dept Neurosurg, Stanford, CA 94305 USA. [Flynn, Ryan A.; Chang, Howard Y.] Stanford Univ, Sch Med, Program Epithelial Biol, Stanford, CA 94305 USA. [Floor, Stephen N.; Martin, Lance; Do, Brian T.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Purzner, James] Stanford Univ, Sch Med, Dept Dev Biol, Stanford, CA 94305 USA. [Purzner, James] Univ Toronto, Dept Surg, Div Neurosurg, Toronto, ON M5S 1A1, Canada. [Morrissy, Sorana; Taylor, Michael D.] Hosp Sick Children, Dev & Stem Cell Biol Program, 555 Univ Ave, Toronto, ON M5G 1X8, Canada. [Morrissy, Sorana; Taylor, Michael D.] Hosp Sick Children, Dept Surg, Div Neurosurg, 555 Univ Ave, Toronto, ON M5G 1X8, Canada. [Morrissy, Sorana; Taylor, Michael D.] Hosp Sick Children, Labatt Brain Tumour Res Ctr, 555 Univ Ave, Toronto, ON M5G 1X8, Canada. [Li, Yisu; Marra, Marco A.; Taylor, Michael D.] BC Canc Agcy, Canadas Michael Smith Genome Sci Ctr, Vancouver, BC, Canada. [Kool, Marcel; Jones, David T. W.; Northcott, Paul A.; Pfister, Stefan M.] German Canc Res Ctr, Div Pediat Neurooncol, Heidelberg, Germany. [Hovestadt, Volker; Lichter, Peter] German Canc Res Ctr, Div Mol Genet, Heidelberg, Germany. [Risch, Thomas; Warnatz, Hans-Joerg; Yaspo, Marie-Laure] Max Planck Inst Mol Genet, Dept Vertebrate Genom, Ihnestr 73, D-14195 Berlin, Germany. [Adams, Christopher M.; Leib, Ryan D.] Stanford Univ, Vincent Coates Fdn Mass Spectrometry Lab, Stanford, CA 94305 USA. [Breese, Marcus] Stanford Univ, Sch Med, Canc Biol Program, Stanford, CA 94305 USA. [Malkin, David] Hosp Sick Children, Canc Genet Program, 555 Univ Ave, Toronto, ON M5G 1X8, Canada. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Taylor, Michael D.] Univ Toronto, Dept Lab Med & Pathobiol, Toronto, ON M5S 1A1, Canada. [Chang, Howard Y.] Stanford Univ, Sch Med, Howard Hughes Med Inst, Stanford, CA 94305 USA. [Cho, Yoon-Jae] Oregon Hlth & Sci Univ, Dept Pediat, Pape Family Pediat Res Inst, 3181 Sw Sam Jackson Pk Rd, Portland, OR 97201 USA. [Cho, Yoon-Jae] Oregon Hlth & Sci Univ, Knight Canc Inst, Portland, OR 97201 USA. RP Cho, YJ (reprint author), Stanford Univ, Sch Med, Dept Neurol & Neurol Sci, Stanford, CA 94305 USA.; Cho, YJ (reprint author), Stanford Univ, Sch Med, Dept Neurosurg, Stanford, CA 94305 USA.; Chang, HY (reprint author), Stanford Univ, Sch Med, Program Epithelial Biol, Stanford, CA 94305 USA.; Chang, HY (reprint author), Stanford Univ, Sch Med, Howard Hughes Med Inst, Stanford, CA 94305 USA.; Cho, YJ (reprint author), Oregon Hlth & Sci Univ, Dept Pediat, Pape Family Pediat Res Inst, 3181 Sw Sam Jackson Pk Rd, Portland, OR 97201 USA.; Cho, YJ (reprint author), Oregon Hlth & Sci Univ, Knight Canc Inst, Portland, OR 97201 USA. EM howchang@stanford.edu; chyo@ohsu.edu RI Vaka, Dedeepya/L-9041-2016; Marra, Marco/B-5987-2008; OI Do, Brian/0000-0003-4992-2623; Hovestadt, Volker/0000-0002-3480-6649 FU St. Baldrick's Foundation Scholar Award; Beirne Faculty Scholar Endowment; NIH [U01-CA176287]; Stanford Center for Children's Brain Tumors; Stanford University Mass Spectrometry Seed Grant; Center for RNA Systems Biology [5P50GM102706]; Genome Canada; Genome BC; Terry Fox Research Institute; Ontario Institute for Cancer Research; Pediatric Oncology Group Ontario; Family of Kathleen Lorette; Clark H. Smith Brain Tumour Centre; Montreal Children's Hospital Foundation; Hospital for Sick Children: Sonia and Arthur Labatt Brain Tumour Research Centre; Cancer Genetics Program; Garron Family Cancer Centre; German Cancer Aid [S.M.P.109252]; German Federal Ministry of Education and Research [01KU1201A, 0315416C, 01GS0883]; B.R.A.I.N. Child FX This work was supported by the St. Baldrick's Foundation Scholar Award (Y.-J.C.), Beirne Faculty Scholar Endowment (Y.-J.C.), NIH U01-CA176287 (Y-J.C.), Stanford Center for Children's Brain Tumors (Y.-J.C.), Stanford University Mass Spectrometry Seed Grant (Y.-J.C.), Center for RNA Systems Biology (J.A.D.; 5P50GM102706). S.N.F. is a Howard Hughes Medical Institute fellow of the Helen Hay Whitney Foundation. J.A.D. and H.Y.C. are investigators of the Howard Hughes Medical Institute. Human medulloblastoma data generated through the Medulloblastoma Advanced Genomics International Consortium (M.D.T., M.A.M., D.M.) was supported by Genome Canada, Genome BC, Terry Fox Research Institute, Ontario Institute for Cancer Research, Pediatric Oncology Group Ontario, Funds from 'The Family of Kathleen Lorette' and the Clark H. Smith Brain Tumour Centre, Montreal Children's Hospital Foundation, Hospital for Sick Children: Sonia and Arthur Labatt Brain Tumour Research Centre, Chief of Research Fund, Cancer Genetics Program, Garron Family Cancer Centre, and B.R.A.I.N. Child. Human medulloblastoma data generated from the PedBrain Tumor Project/International Cancer Genome Consortium was funded by German Cancer Aid (S.M.P.109252) and the German Federal Ministry of Education and Research (grants#01KU1201A, MedSys#0315416C and NGFNplus#01GS0883). We are grateful for R. Reed (Harvard University) for DDX3X cDNA, and V. Raman (Johns Hopkins University) for anti DDX3 mAb, and members of the Chang and Cho laboratories for reagents, helpful suggestions and critical reading of the manuscript. NR 43 TC 1 Z9 1 U1 0 U2 1 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1949-2553 J9 ONCOTARGET JI Oncotarget PD MAY 10 PY 2016 VL 7 IS 19 BP 28169 EP 28182 DI 10.18632/oncotarget.8612 PG 14 WC Oncology; Cell Biology SC Oncology; Cell Biology GA DO4HF UT WOS:000377741700097 PM 27058758 ER PT J AU Cao, RG Chen, JZ Han, KS Xu, W Mei, DH Bhattacharya, P Engelhard, MH Mueller, KT Liu, J Zhang, JG AF Cao, Ruiguo Chen, Junzheng Han, Kee Sung Xu, Wu Mei, Donghai Bhattacharya, Priyanka Engelhard, Mark H. Mueller, Karl T. Liu, Jun Zhang, Ji-Guang TI Effect of the Anion Activity on the Stability of Li Metal Anodes in Lithium-Sulfur Batteries SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID SALT ELECTROLYTE; GRAPHENE OXIDE; PERFORMANCE; DISCHARGE AB With the significant progress made in the development of cathodes in lithium-sulfur (Li-S) batteries, the stability of Li metal anodes becomes a more urgent challenge in these batteries. Here the systematic investigation of the stability of the anode/electrolyte interface in Li-S batteries with concentrated electrolytes containing various lithium salts is reported. It is found that Li-S batteries using LiTFSI-based electrolytes are more stable than those using LiFSI-based electrolytes. The decreased stability is because the N-S bond in the FSI-anion is fairly weak and the scission of this bond leads to the formation of lithium sulfate (LiSOx) in the presence of polysulfide species. In contrast, in the LiTFSI-based electrolyte, the lithium metal anode tends to react with polysulfide to form lithium sulfide (LiSx), which is more reversible than LiSOx formed in the LiFSI-based electrolyte. This fundamental difference in the bond strength of the salt anions in the presence of polysulfide species leads to a large difference in the stability of the anode-electrolyte interface and performance of the Li-S batteries with electrolytes composed of these salts. Therefore, anion selection is one of the key parameters in the search for new electrolytes for stable operation of Li-S batteries. C1 [Cao, Ruiguo; Chen, Junzheng; Xu, Wu; Bhattacharya, Priyanka; Liu, Jun; Zhang, Ji-Guang] Energy & Environm Directorate, Pacific NW Natl Lab, Richland, WA 99354 USA. [Han, Kee Sung; Engelhard, Mark H.] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99354 USA. [Mei, Donghai; Mueller, Karl T.] Phys & Computat Sci Directorate, Pacific NW Natl Lab, Richland, WA 99354 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. RP Zhang, JG (reprint author), Energy & Environm Directorate, Pacific NW Natl Lab, Richland, WA 99354 USA. EM jiguang.zhang@pnnl.gov RI Mei, Donghai/A-2115-2012; Mei, Donghai/D-3251-2011; Cao, Ruiguo/O-7354-2016; OI Mei, Donghai/0000-0002-0286-4182; Xu, Wu/0000-0002-2685-8684 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; DOE's Office of Biological and Environmental Research FX This work was supported by the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The microscopic images and spectroscopic measurements were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory-a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). NR 29 TC 8 Z9 8 U1 68 U2 128 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 10 PY 2016 VL 26 IS 18 BP 3059 EP 3066 DI 10.1002/adfm.201505074 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO2EC UT WOS:000377591500009 ER PT J AU Halim, J Kota, S Lukatskaya, MR Naguib, M Zhao, MQ Moon, EJ Pitock, J Nanda, J May, SJ Gogotsi, Y Barsoum, MW AF Halim, Joseph Kota, Sankalp Lukatskaya, Maria R. Naguib, Michael Zhao, Meng-Qiang Moon, Eun Ju Pitock, Jeremy Nanda, Jagjit May, Steven J. Gogotsi, Yury Barsoum, Michel W. TI Synthesis and Characterization of 2D Molybdenum Carbide (MXene) SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID 2-DIMENSIONAL TITANIUM CARBIDE; HIGH VOLUMETRIC CAPACITANCE; TRANSITION-METAL CARBIDES; LITHIUM-ION BATTERIES; X-RAY PHOTOELECTRON; NANOLAMINATED CARBIDE; CATION INTERCALATION; ENERGY-STORAGE; THIN-FILMS; LI AB Large scale synthesis and delamination of 2D Mo2CTx (where T is a surface termination group) has been achieved by selectively etching gallium from the recently discovered nanolaminated, ternary transition metal carbide Mo2Ga2C. Different synthesis and delamination routes result in different flake morphologies. The resistivity of free-standing Mo2CTx films increases by an order of magnitude as the temperature is reduced from 300 to 10 K, suggesting semiconductor-like behavior of this MXene, in contrast to Ti3C2Tx which exhibits metallic behavior. At 10 K, the magnetoresistance is positive. Additionally, changes in electronic transport are observed upon annealing of the films. When 2 mu m thick films are tested as electrodes in supercapacitors, capacitances as high as 700 F cm(-3) in a 1 M sulfuric acid electrolyte and high capacity retention for at least 10,000 cycles at 10 A g(-1) are obtained. Free-standing Mo2CTx films, with approximate to 8 wt% carbon nanotubes, perform well when tested as an electrode material for Li-ions, especially at high rates. At 20 and 131 C cycling rates, stable reversible capacities of 250 and 76 mAh g(-1), respectively, are achieved for over 1000 cycles. C1 [Halim, Joseph; Kota, Sankalp; Lukatskaya, Maria R.; Zhao, Meng-Qiang; Moon, Eun Ju; Pitock, Jeremy; May, Steven J.; Gogotsi, Yury; Barsoum, Michel W.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Halim, Joseph; Lukatskaya, Maria R.; Zhao, Meng-Qiang; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Halim, Joseph] Linkoping Univ, Dept Phys Chem & Biol IFM, Thin Film Phys Div, SE-58183 Linkoping, Sweden. [Naguib, Michael; Nanda, Jagjit] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37381 USA. RP Gogotsi, Y; Barsoum, MW (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA.; Gogotsi, Y (reprint author), Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. EM gogotsi@drexel.edu; barsoumw@drexel.edu RI May, Steven/D-8563-2011; OI May, Steven/0000-0002-8097-1549; Naguib, Michael/0000-0002-4952-9023; Kota, Sankalp/0000-0003-3775-3279 FU Swedish Research Council [621-2012-4430]; Swedish Foundation for Strategic Research through the Synergy Grant FUNCASE Functional Carbides for Advanced Surface Engineering; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Army Research Office [W911NF-15-1-0133] FX S.K., M.R.L., and M.N. contributed equally to this work. The authors acknowledge the support from the Swedish Research Council (Project Grant No. 621-2012-4430), the Swedish Foundation for Strategic Research through the Synergy Grant FUNCASE Functional Carbides for Advanced Surface Engineering (M.W.B. and J.H.). M.N. and J.N. were supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. E.J.M and S.J.M. acknowledge support from the U.S. Army Research Office (grant number W911NF-15-1-0133). The authors also acknowledge Dr. Chunfeng Hu for his help regarding the synthesis of Mo2Ga2C powders. NR 56 TC 29 Z9 29 U1 138 U2 235 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 10 PY 2016 VL 26 IS 18 BP 3118 EP 3127 DI 10.1002/adfm.201505328 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO2EC UT WOS:000377591500015 ER PT J AU Finkbeiner, DP Schlafly, EF Schlegel, DJ Padmanabhan, N Juric, M Burgett, WS Chambers, KC Denneau, L Draper, PW Flewelling, H Hodapp, KW Kaiser, N Magnier, EA Metcalfe, N Morgan, JS Price, PA Stubbs, CW Tonry, JL AF Finkbeiner, Douglas P. Schlafly, Edward F. Schlegel, David J. Padmanabhan, Nikhil Juric, Mario Burgett, William S. Chambers, Kenneth C. Denneau, Larry Draper, Peter W. Flewelling, Heather Hodapp, Klaus W. Kaiser, Nick Magnier, E. A. Metcalfe, N. Morgan, Jeffrey S. Price, Paul A. Stubbs, Christopher W. Tonry, John L. TI HYPERCALIBRATION: A PAN-STARRS1-BASED RECALIBRATION OF THE SLOAN DIGITAL SKY SURVEY PHOTOMETRY SO ASTROPHYSICAL JOURNAL LA English DT Article DE methods: data analysis; surveys; techniques: photometric ID DATA RELEASE; SDSS-III; CALIBRATION; EXTINCTION; TELESCOPE; MONITOR AB We present a recalibration of the Sloan Digital Sky Survey (SDSS) photometry with new flat fields and zero points derived from Pan-STARRS1. Using point-spread function (PSF) photometry of 60 million stars with 16 < r < 20, we derive a model of amplifier gain and flat-field corrections with per-run rms residuals of 3 millimagnitudes (mmag) in griz bands and 15 mmag in u band. The new photometric zero points are adjusted to leave the median in the Galactic north unchanged for compatibility with previous SDSS work. We also identify transient nonphotometric periods in SDSS ("contrails") based on photometric deviations co-temporal in SDSS bands. The recalibrated stellar PSF photometry of SDSS and PS1 has an rms difference of {9, 7, 7, 8} mmag in griz, respectively, when averaged over 15' regions. C1 [Finkbeiner, Douglas P.] Harvard Smithsonian Ctr Astrophys, Inst Theory & Computat, 60 Garden St,MS-51, Cambridge, MA 02138 USA. [Finkbeiner, Douglas P.; Stubbs, Christopher W.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Schlafly, Edward F.] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Schlegel, David J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Padmanabhan, Nikhil] Yale Univ, Dept Phys, 260 Whitney Ave, New Haven, CT 06520 USA. [Juric, Mario] LSST Corp, 933 N Cherry Ave, Tucson, AZ 85721 USA. [Burgett, William S.; Chambers, Kenneth C.; Denneau, Larry; Flewelling, Heather; Hodapp, Klaus W.; Kaiser, Nick; Magnier, E. A.; Morgan, Jeffrey S.; Tonry, John L.] Univ Hawaii Manoa, Inst Astron, Honolulu, HI 96822 USA. [Draper, Peter W.; Metcalfe, N.] Univ Durham, Dept Phys, South Rd, Durham DH1 3LE, England. [Price, Paul A.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. RP Finkbeiner, DP (reprint author), Harvard Smithsonian Ctr Astrophys, Inst Theory & Computat, 60 Garden St,MS-51, Cambridge, MA 02138 USA.; Finkbeiner, DP (reprint author), Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. OI Chambers, Kenneth /0000-0001-6965-7789 FU NASA [NNX10AD69G]; German Research Foundation (DFG) [Sonderforschungsbereich SFB 881]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; National Aeronautics and Space Administration [NNX08AR22G]; National Science Foundation [AST-1238877] FX We acknowledge helpful conversations with Michael Blanton. DPF and EFS have been partially supported by NASA grant NNX10AD69G. EFS acknowledges funding by Sonderforschungsbereich SFB 881 "The Milky Way System" (subproject A3) of the German Research Foundation (DFG). This research made use of the NASA Astrophysics Data System (ADS) and the IDL Astronomy User's Library at Goddard.16; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; The Pan-STARRS1 Surveys (PS1) have been made possible through contributions of the Institute for Astronomy, the University of Hawaii, the Pan-STARRS Project Office, the Max-Planck Society and its participating institutes, the Max Planck Institute for Astronomy, Heidelberg and the Max Planck Institute for Extraterrestrial Physics, Garching, The Johns Hopkins University, Durham University, the University of Edinburgh, Queens University Belfast, the Harvard-Smithsonian Center for Astrophysics, the Las Cumbres Observatory Global Telescope Network Incorporated, the National Central University of Taiwan, the Space Telescope Science Institute, the National Aeronautics and Space Administration under Grant No. NNX08AR22G issued through the Planetary Science Division of the NASA Science Mission Directorate, the National Science Foundation under Grant No. AST-1238877, and the University of Maryland. NR 30 TC 7 Z9 7 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2016 VL 822 IS 2 AR 66 DI 10.3847/0004-637X/822/2/66 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN6RZ UT WOS:000377204900009 ER PT J AU Harding, JP Fryer, CL Mendel, S AF Harding, J. Patrick Fryer, Chris L. Mendel, Susan TI EXPLAINING TEV COSMIC-RAY ANISOTROPIES WITH NON-DIFFUSIVE COSMIC-RAY PROPAGATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE astroparticle physics; cosmic rays; ISM: kinematics and dynamics; magnetic fields; turbulence ID AIR-SHOWER ARRAY; MILAGRO HOT-SPOTS; ENERGETIC PARTICLES; ARRIVAL DIRECTIONS; MAGNETIC-FIELD; DIFFUSION; TURBULENCE; TRANSPORT; ICECUBE; IBEX AB Constraining the behavior of cosmic ray data observed at Earth requires a precise understanding of how the cosmic rays propagate in the interstellar medium. The interstellar medium is not homogeneous; although turbulent magnetic fields dominate over large scales, small coherent regions of magnetic field exist on scales relevant to particle propagation in the nearby Galaxy. Guided propagation through a coherent field is significantly different from random particle diffusion and could be the explanation of spatial anisotropies in the observed cosmic rays. We present a Monte Carlo code to propagate cosmic particle through realistic magnetic field structures. We discuss the details of the model as well as some preliminary studies which indicate that coherent magnetic structures are important effects in local cosmic-ray propagation, increasing the flux of cosmic rays by over two orders of magnitude at anisotropic locations on the sky. The features induced by coherent magnetic structure could be the cause of the observed TeV cosmic-ray anisotropy. C1 [Harding, J. Patrick] Los Alamos Natl Lab, P-23, Los Alamos, NM 87545 USA. [Fryer, Chris L.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [Mendel, Susan] Los Alamos Natl Lab, ISR 2, Los Alamos, NM 87545 USA. RP Harding, JP (reprint author), Los Alamos Natl Lab, P-23, Los Alamos, NM 87545 USA. EM jpharding@lanl.gov; fryer@lanl.gov; smendel@lanl.gov OI Mendel, Susan/0000-0002-1294-6747 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory through an IGPPS grant [DE-AC52-06NA25396] FX We thank Brenda Dingus and Fan Guo for useful discussions. Work at LANL was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under contract no. DE-AC52-06NA25396 through an IGPPS grant. NR 52 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2016 VL 822 IS 2 AR 102 DI 10.3847/0004-637X/822/2/102 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN6RZ UT WOS:000377204900045 ER PT J AU Paparo, M Benko, JM Hareter, M Guzik, JA AF Paparo, M. Benko, J. M. Hareter, M. Guzik, J. A. TI UNEXPECTED SERIES OF REGULAR FREQUENCY SPACING OF delta SCUTI STARS IN THE NON-ASYMPTOTIC REGIME. I. THE METHODOLOGY SO ASTROPHYSICAL JOURNAL LA English DT Article DE space vehicles; stars: oscillations; stars: variables: delta Scuti; techniques: photometric ID RAPIDLY ROTATING STARS; COROT-FIELDS IRA01; FG-VIRGINIS; ASTEROSEISMIC MEASUREMENT; MULTIOBJECT SPECTROSCOPY; CENTRIFUGAL-DISTORTION; ACOUSTIC-OSCILLATIONS; MODE-IDENTIFICATIONS; POLYTROPIC STARS; ECHELLE DIAGRAMS AB A sequence search method was developed to search the regular frequency spacing in delta Scuti stars through visual inspection and an algorithmic search. We searched for sequences of quasi-equally spaced frequencies, containing at least four members per sequence, in 90 delta Scuti stars observed by CoRoT. We found an unexpectedly large number of independent series of regular frequenct spacing in 77 delta Scuti stars (from one to eight sequences) in the non-asymptotic regime. We introduce the sequence search method presenting the sequences and echelle diagram of CoRoT 102675756 and the structure of the algorithmic search. Four sequences (echelle ridges) were found in the 5-21 d(-1) region where the pairs of the sequences are shifted (between 0.5 and 0.59 d(-1)) by twice the value of the estimated rotational splitting frequency (0.269 d(-1)). The general conclusions for the whole sample are also presented in this paper. The statistics of the spacings derived by the sequence search method, by FT (Fourier transform of the frequencies), and the statistics of the shifts are also compared. In many stars more than one almost equally valid spacing appeared. The model frequencies of FG Vir and their rotationally split components were used to formulate the possible explanation that one spacing is the large separation while the other is the sum of the large separation and the rotational frequency. In CoRoT 102675756, the two spacings (2.249 and 1.977 d(-1)) are in better agreement with the sum of a possible 1.710 d(-1) large separation and two or one times, respectively, the value of the rotational frequency. C1 [Paparo, M.; Benko, J. M.; Hareter, M.] MTA CSFK, Konkoly Observ, Konkoly Thege Miklos Ut 15-17, H-1121 Budapest, Hungary. [Guzik, J. A.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Paparo, M (reprint author), MTA CSFK, Konkoly Observ, Konkoly Thege Miklos Ut 15-17, H-1121 Budapest, Hungary. EM paparo@konkoly.hu FU grant ESA PECS [4000103541/11/NL/KLM] FX This work was supported by grant ESA PECS No 4000103541/11/NL/KLM. NR 54 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2016 VL 822 IS 2 AR 100 DI 10.3847/0004-637X/822/2/100 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN6RZ UT WOS:000377204900043 ER PT J AU Ruiz-Velasco, AE Felli, D Migenes, V Wiggins, BK AF Ruiz-Velasco, A. E. Felli, D. Migenes, V. Wiggins, B. K. TI VLBA SURVEYS OF OH MASERS IN STAR-FORMING REGIONS. I. SATELLITE LINES SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: star formation; instrumentation: interferometers; ISM: molecules; masers ID YOUNG STELLAR OBJECTS; TRIGONOMETRIC PARALLAXES; OUTFLOW COLLIMATION; MAGNETIC-FIELD; 1720 MHZ; EMISSION; EVOLUTION; FLARE; W75N; IONIZATION AB Using the Very Long Baseline Array we performed a high-resolution OH maser survey in Galactic star-forming regions (SFRs). We observed all the ground state spectral lines: the main lines at 1665 and 1667 MHz and the satellite lines at 1612 and 1720 MHz. Due to the exceptionality of finding satellite lines in SFRs, we will focus our discussion on those lines. In our sample of 41 OH maser sources, five (12%) showed the 1612 MHz line and ten (24%) showed the 1720 MHz line, with only one source showing both lines. We find that 1720 MHz emission is correlated with the presence of H II regions, suggesting that this emission could be used to diagnose or trace high-mass star formation. We include an analysis of the possible mechanisms that could be causing this correlation as well as assessing the possible relationships between lines in our sample. In particular, the presence of magnetic fields seems to play an important role as we found Zeeman splitting in four of our sources (W75 N, W3(OH), W51 and NGC 7538). Our results have implications for current understanding of the formation of high-mass stars as well as on the masing processes present in SFRs. C1 [Ruiz-Velasco, A. E.] Lowell Observ, 1400 W Mars Hill Rd, Flagstaff, AZ 86001 USA. [Felli, D.; Migenes, V.; Wiggins, B. K.] Brigham Young Univ, Dept Phys & Astron, ESC, Provo, UT 84602 USA. [Migenes, V.] Texas So Univ, Dept Phys, 3100 Clebourne Ave, Houston, TX 77004 USA. [Wiggins, B. K.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Ruiz-Velasco, AE (reprint author), Lowell Observ, 1400 W Mars Hill Rd, Flagstaff, AZ 86001 USA. EM alma@lowell.edu FU CONACYT; Lowell Observatory; BYU ORCA grant FX A.R-V. acknowledges the support of CONACYT and Lowell Observatory. D.F. would like to acknowledge a BYU ORCA grant in helping fund the research project. This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France, and NASA's Astrophysics Data System. NR 41 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAY 10 PY 2016 VL 822 IS 2 AR 101 DI 10.3847/0004-637X/822/2/101 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN6RZ UT WOS:000377204900044 ER PT J AU Rameau, J Nielsen, EL De Rosa, RJ Blunt, SC Patience, J Doyon, R Graham, JR Lafreniere, D Macintosh, B Marchis, F Bailey, V Chilcote, JK Duchene, G Esposito, TM Hung, LW Konopacky, QM Maire, J Marois, C Metchev, S Perrin, MD Pueyo, L Rajan, A Savransky, D Wang, JJ Ward-Duong, K Wolff, SG Ammons, SM Hibon, P Ingraham, P Kalas, P Morzinski, KM Oppenheimer, R Rantakyearo, FT Thomas, S AF Rameau, Julien Nielsen, Eric L. De Rosa, Robert J. Blunt, Sarah C. Patience, Jenny Doyon, Rene Graham, James R. Lafreniere, David Macintosh, Bruce Marchis, Franck Bailey, Vanessa Chilcote, Jeffrey K. Duchene, Gaspard Esposito, Thomas M. Hung, Li-Wei Konopacky, Quinn M. Maire, Jerome Marois, Christian Metchev, Stanimir Perrin, Marshall D. Pueyo, Laurent Rajan, Abhijith Savransky, Dmitry Wang, Jason J. Ward-Duong, Kimberly Wolff, Schuyler G. Ammons, S. Mark Hibon, Pascale Ingraham, Patrick Kalas, Paul Morzinski, Katie M. Oppenheimer, Rebecca Rantakyearo, Fredrik T. Thomas, Sandrine TI CONSTRAINTS ON THE ARCHITECTURE OF THE HD 95086 PLANETARY SYSTEM WITH THE GEMINI PLANET IMAGER SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE astrometry; planet-disk interactions; planetary systems; stars: individual (HD 95086) ID BETA-PICTORIS B; HR 8799; GIANT PLANET; DEBRIS DISK; ORBITAL PARAMETERS; MASS COMPANION; 1ST LIGHT; EXOPLANET; STARS; CONFIRMATION AB We present astrometric monitoring of the young exoplanet HD 95086 b obtained with the Gemini Planet Imager between 2013 and 2016. A small but significant position angle change is detected at constant separation; the orbital motion is confirmed with literature measurements. Efficient Monte Carlo techniques place preliminary constraints on the orbital parameters of HD 95086 b. With 68% confidence, a semimajor axis of 61.7(-8.4)(+20.7) au and an inclination of. 153.0(+9.7)(-13.5) are favored, with eccentricity less than 0.21. Under the assumption of a coplanar planet-disk system, the periastron of HD 95086 b is beyond 51 au with 68% confidence. Therefore, HD 95086 b cannot carve the entire gap inferred from the measured infrared excess in the SED of HD 95086. We use our sensitivity to additional planets to discuss specific scenarios presented in the literature to explain the geometry of the debris belts. We suggest that either two planets on moderately eccentric orbits or three to four planets with inhomogeneous masses and orbital properties are possible. The sensitivity to additional planetary companions within the observations presented in this study can be used to help further constrain future dynamical simulations of the planet-disk system. C1 [Rameau, Julien; Doyon, Rene; Lafreniere, David] Univ Montreal, Dept Phys, Inst Rech Exoplanetes, CP 6128, Montreal, PQ H3C 3J7, Canada. [Nielsen, Eric L.; Blunt, Sarah C.; Marchis, Franck; Kalas, Paul] Carl Sagan Ctr, SETI Inst, 189 Bernardo Ave, Mountain View, CA 94043 USA. [Nielsen, Eric L.; Macintosh, Bruce; Bailey, Vanessa] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [De Rosa, Robert J.; Graham, James R.; Duchene, Gaspard; Esposito, Thomas M.; Wang, Jason J.; Kalas, Paul] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Blunt, Sarah C.] Brown Univ, Dept Phys, Providence, RI 02912 USA. [Patience, Jenny; Rajan, Abhijith; Ward-Duong, Kimberly] Arizona State Univ, Sch Earth & Space Explorat, POB 871404, Tempe, AZ 85287 USA. [Chilcote, Jeffrey K.; Maire, Jerome] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Duchene, Gaspard] Univ Grenoble Alpes, CNRS, Inst Planetol & Astrophys Grenoble, F-38000 Grenoble, France. [Hung, Li-Wei; Konopacky, Quinn M.] Univ Calif Los Angeles, Dept Phys & Astron, 430 Portola Plaza, Los Angeles, CA 90095 USA. [Marois, Christian] Univ Victoria, Dept Phys & Astron, 3800 Finnerty Rd, Victoria, BC V8P 5C2, Canada. [Marois, Christian] Natl Res Council Canada Herzberg, 5071 West Saanich Rd, Victoria, BC V9E 2E7, Canada. [Metchev, Stanimir] Univ Western Ontario, Dept Phys & Astron, Ctr Planetary Sci & Explorat, London, ON N6A 3K7, Canada. [Metchev, Stanimir] SUNY Stony Brook, Dept Phys & Astron, 100 Nicolls Rd, Stony Brook, NY 11790 USA. [Perrin, Marshall D.; Pueyo, Laurent; Wolff, Schuyler G.] Space Telescope Sci Inst, 3700 San Martin Dr, Baltimore, MD 21218 USA. [Savransky, Dmitry] Cornell Univ, Sibley Sch Mech & Aerosp Engn, Ithaca, NY 14853 USA. [Wolff, Schuyler G.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Ammons, S. Mark] Lawrence Livermore Natl Lab, L-210,7000 East Ave, Livermore, CA 94550 USA. [Hibon, Pascale] European So Observ, Alonso Cordova 3107,Casilla 19001, Santiago, Chile. [Ingraham, Patrick] Large Synopt Survey Telescope, 950 N Cherry Ave, Tucson, AZ 85719 USA. [Morzinski, Katie M.] Univ Arizona, Steward Observ, 933 N Cherry Ave, Tucson, AZ 85721 USA. [Oppenheimer, Rebecca] Amer Museum Nat Hist, New York, NY 10024 USA. [Rantakyearo, Fredrik T.] Gemini Observ, Casilla 603, La Serena, Chile. RP Rameau, J (reprint author), Univ Montreal, Dept Phys, Inst Rech Exoplanetes, CP 6128, Montreal, PQ H3C 3J7, Canada. RI Savransky, Dmitry/M-1298-2014; OI Savransky, Dmitry/0000-0002-8711-7206; Nielsen, Eric/0000-0001-6975-9056; Perrin, Marshall/0000-0002-3191-8151; Bailey, Vanessa/0000-0002-5407-2806 FU Fonds de Recherche du Quebec; NSF [AST-1518332, AST-1411868, AST-141378]; NASA [NNX15AD95G/NEXSS, NNX15AC89G, NNX14AJ80G]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Kate Y. L. Su for interesting discussions about the debris system and Virginie Faramaz for her fruitful advices on handling chaotic zones. Based on observations obtained at the Gemini Observatory, which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the National Science Foundation (NSF) on behalf of the Gemini partnership: the NSF (United States), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia, Tecnologia e Inovacao (Brazil) and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina). J.R., R.D., and D.L. acknowledge support from the Fonds de Recherche du Quebec. Supported by NSF grants AST-1518332 (R.J.D.R., J.R.G., J.J.W., T.M.E., P.K.), AST-1411868 (B.M., A.R., K.W.D.), and AST-141378 (G.D.). Supported by NASA grants NNX15AD95G/NEXSS and NNX15AC89G (R.J.D.R., J.R.G., P.K., J.J.W., T.M.E.), and NNX14AJ80G (E.L.N., S.C.B., B.M., F.M., M.P.). Portions of this work were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 (S.M.A.). NR 44 TC 1 Z9 1 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD MAY 10 PY 2016 VL 822 IS 2 AR L29 DI 10.3847/2041-8205/822/2/L29 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DM2JQ UT WOS:000376173300009 ER PT J AU Ferru, G Reinhart, B Bera, MK de la Cruz, MO Qiao, B Ellis, RJ AF Ferru, Geoffroy Reinhart, Benjamin Bera, Mrinal K. de la Cruz, Monica Olvera Qiao, Baofu Ellis, Ross J. TI The Lanthanide Contraction beyond Coordination Chemistry SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE atomistic simulation; coordination; lanthanide contraction; mesoscale interactions; small-angle X-ray scattering ID PARTICLE MESH EWALD; AQUEOUS-SOLUTIONS; SOLVENT-EXTRACTION; SURFACE-ADHESION; HARD-SPHERES; N-DODECANE; HYDRATION; DYNAMICS; PHASE; IONS AB The lanthanide contraction is conceptualized traditionally through coordination chemistry. Here we break this mold in a structural study of lanthanide ions dissolved in an amphiphilic liquid. The lanthanide contraction perturbs the weak interactions between molecular aggregates that drive mesoscale assembly and emergent behavior. The weak interactions correlate with lanthanide ion transport properties, suggesting new strategies for rare-earth separation that exploit forces outside of the coordination sphere. C1 [Ellis, Ross J.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Ferru, Geoffroy; Bera, Mrinal K.; Qiao, Baofu] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Reinhart, Benjamin] Argonne Natl Lab, Xray Sci Div, APS, 9700 S Cass Ave, Argonne, IL 60439 USA. [de la Cruz, Monica Olvera] Northwestern Univ, Dept Mat Sci, Evanston, IL 60208 USA. [de la Cruz, Monica Olvera] Northwestern Univ, Dept Engn, Evanston, IL 60208 USA. [de la Cruz, Monica Olvera] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Ellis, RJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Qiao, B (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM qiaobf@gmail.com; ellisrj1@ornl.gov RI ellis, ross/J-1981-2016 OI ellis, ross/0000-0001-7691-5205 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences [DE-AC02-06CH11357]; US Department of Energy [DE-FG02-08ER46539] FX This work and the use of the Advanced Photon Source are supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, under Contract DE-AC02-06CH11357. B. Q. gratefully acknowledges the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. M. O. d. l. C would like to thank the US Department of Energy grant DE-FG02-08ER46539 for financial support. NR 31 TC 4 Z9 4 U1 15 U2 29 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAY 10 PY 2016 VL 22 IS 20 BP 6899 EP 6904 DI 10.1002/chem.201601032 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DL8CI UT WOS:000375866600027 PM 27060294 ER PT J AU Alemayehu, AB Vazquez-Lima, H Gagnon, KJ Ghosh, A AF Alemayehu, Abraham B. Vazquez-Lima, Hugo Gagnon, Kevin J. Ghosh, Abhik TI Tungsten Biscorroles: New Chiral Sandwich Compounds SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE chirality; density functional calculations; metalation; sandwich complexes; tungsten ID TRANSITION-METAL CORROLES; 8-COORDINATE COMPLEXES; ELECTRONIC ABSORPTION; OXIDATIVE METALATION; CORRELATION-ENERGY; NONINNOCENT; CHEMISTRY; TEMPERATURE; INNOCENT; SYSTEMS AB The oxidative metalation method, involving the interaction of free-base meso-triarylcorroles and W(CO)(6) in refluxing decalin, led to a set of three tungsten(VI) biscorroles, the first homoleptic sandwich compounds involving corroles. Single-crystal X-ray structures of two of the complexes revealed square-antiprismatic coordination and strongly domed corroles with long W-N distances of 2.15-2.22 angstrom and a substantial displacement of approximate to 1.17 angstrom of the metal relative to the mean N-4 planes of the ligands. The structures correspond to approximate C-2 symmetry and are thus chiral. DFT calculations strongly indicate that the enantiomers are configurationally stable and hence amenable to chiral resolution. Their other notable properties include a strongly blueshifted Soret band at (357 +/- 2)nm, a relatively intense W(dz2 ) near-IR feature at (781 +/- 3)nm, and a low electrochemical HOMO-LUMO gap of approximately 1.3V. The results obtained herein suggest that metallobiscorroles may emerge as a new class of inherently chiral chromophores with novel optical and electrochemical properties. C1 [Alemayehu, Abraham B.; Vazquez-Lima, Hugo; Ghosh, Abhik] UiT Arctic Univ Norway, Dept Chem, N-9037 Tromso, Norway. [Gagnon, Kevin J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Ghosh, A (reprint author), UiT Arctic Univ Norway, Dept Chem, N-9037 Tromso, Norway. EM abhik.ghosh@uit.no RI Ghosh, Abhik/G-8164-2016; OI Ghosh, Abhik/0000-0003-1161-6364; Alemayehu, Abraham/0000-0003-0166-8937 FU FRINATEK project of the Research Council of Norway [231086]; Advanced Light Source, Berkeley, California; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by FRINATEK project 231086 of the Research Council of Norway (AG) and the Advanced Light Source, Berkeley, California (CMB, KJG). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 69 TC 4 Z9 4 U1 2 U2 5 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAY 10 PY 2016 VL 22 IS 20 BP 6914 EP 6920 DI 10.1002/chem.201504848 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DL8CI UT WOS:000375866600029 PM 27059004 ER PT J AU Bylund, OB Maltoni, F Tsinikos, I Vryonidou, E Zhang, C AF Bylund, Olga Bessidskaia Maltoni, Fabio Tsinikos, Ioannis Vryonidou, Eleni Zhang, Cen TI Probing top quark neutral couplings in the Standard Model Effective Field Theory at NLO in QCD SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Effective field theories AB Top quark pair production in association with a Z-boson or a photon at the LHC directly probes neutral top-quark couplings. We present predictions for these two processes in the Standard Model (SM) Effective Field Theory (EFT) at next-to-leading order (NLO) in QCD. We include the full set of CP-even dimension-six operators that enter the top-quark interactions with the SM gauge bosons. For comparison, we also present predictions in the SMEFT for top loop-induced HZ production at the LHC and for t (t) over bar production at the ILC at NLO in QCD. Results for total cross sections and differential distributions are obtained and uncertainties coming from missing higher orders in the strong coupling and in the EFT expansions are discussed. NLO results matched to the parton shower are available, allowing for event generation to be directly employed in an experimental analyses. Our framework provides a solid basis for the interpretation of current and future measurements in the SMEFT, with improved accuracy and precision. C1 [Bylund, Olga Bessidskaia] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Bylund, Olga Bessidskaia] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Maltoni, Fabio; Tsinikos, Ioannis; Vryonidou, Eleni] Catholic Univ Louvain, Ctr Cosmol Particle Phys & Phenomenol CP3, B-1348 Louvain, Belgium. [Zhang, Cen] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Bylund, OB (reprint author), Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden.; Bylund, OB (reprint author), Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden.; Maltoni, F; Tsinikos, I; Vryonidou, E (reprint author), Catholic Univ Louvain, Ctr Cosmol Particle Phys & Phenomenol CP3, B-1348 Louvain, Belgium.; Zhang, C (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM olga.bylund@cern.ch; fabio.maltoni@uclouvain.be; ioannis.tsinikos@uclouvain.be; eleni.vryonidou@uclouvain.be; cenzhang@bnl.gov FU ERC [291377]; European Union as part of the FP7 Marie Curie Initial Training Network MCnetITN [PITN-GA-2012-315877]; United States Department of Energy [DE-SC0012704] FX We acknowledge illuminating discussions with Christophe Grojean, Alex Pomarol, Francesco Riva on the SMEFT and its range of validity. We would like to thank Raoul Rontsch and Markus Schulze for discussions and helpful checks. C.Z. would like to thank Valentin Hirschi and Hua-Sheng Shao for valuable discussions about gauge anomaly. This work has been performed in the framework of the ERC Grant No. 291377 "LHCTheory" and has been supported in part by the European Union as part of the FP7 Marie Curie Initial Training Network MCnetITN (PITN-GA-2012-315877). C.Z. is supported by the United States Department of Energy under Grant Contracts DE-SC0012704. NR 56 TC 8 Z9 8 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 10 PY 2016 IS 5 AR 052 DI 10.1007/JHEP05(2016)052 PG 39 WC Physics, Particles & Fields SC Physics GA DM1LY UT WOS:000376108000001 ER PT J AU Raimondi, F Hupin, G Navratil, P Quaglioni, S AF Raimondi, Francesco Hupin, Guillaume Navratil, Petr Quaglioni, Sofia TI Deuteron-induced nucleon transfer reactions within an ab initio framework: First application to p-shell nuclei SO PHYSICAL REVIEW C LA English DT Article ID CROSS-SECTION; PRIMORDIAL NUCLEOSYNTHESIS; ELASTIC-SCATTERING; LI-7(D,P)LI-8; LI-7; MODEL; BE-7 AB Background: Low-energy transfer reactions in which a proton is stripped from a deuteron projectile and dropped into a target play a crucial role in the formation of nuclei in both primordial and stellar nucleosynthesis, as well as in the study of exotic nuclei using radioactive beam facilities and inverse kinematics. Ab initio approaches have been successfully applied to describe the H-3(d,n)He-4 and He-3(d,p)He-4 fusion processes. Purpose: An ab initio treatment of transfer reactions would also be desirable for heavier targets. In this work, we extend the ab initio description of ( d, p) reactions to processes with light p-shell nuclei. As a first application, we study the elastic scattering of deuterium on Li-7 and the Li-7(d,p)Li-8 transfer reaction based on a two-body Hamiltonian. Methods: We use the no-core shell model to compute the wave functions of the nuclei involved in the reaction, and describe the dynamics between targets and projectiles with the help of microscopic-cluster states in the spirit of the resonating group method. Results: The shapes of the excitation functions for deuterons impinging on Li-7 are qualitatively reproduced up to the deuteron breakup energy. The interplay between d-Li-7 and p-Li-8 particle-decay channels determines some features of the Be-9 spectrum above the d + Li-7 threshold. Our prediction for the parity of the 17.298 MeV resonance is at odds with the experimental assignment. Conclusions: Deuteron stripping reactions with p-shell targets can now be computed ab initio, but calculations are very demanding. A quantitative description of the Li-7(d,p)Li-8 reaction will require further work to include the effect of three-nucleon forces and additional decay channels and to improve the convergence rate of our calculations. C1 [Raimondi, Francesco; Navratil, Petr] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Hupin, Guillaume; Quaglioni, Sofia] Lawrence Livermore Natl Lab, POB 808,L-414, Livermore, CA 94551 USA. [Hupin, Guillaume] Univ Paris 11, CNRS, IN2P3, Inst Phys Nucl, F-91406 Orsay, France. [Raimondi, Francesco] Univ Surrey, Fac Engn & Phys Sci, Dept Phys, Guildford GU2 7XH, Surrey, England. [Hupin, Guillaume] CEA, DAM, DIF, F-91297 Arpajon, France. RP Raimondi, F; Navratil, P (reprint author), TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada.; Hupin, G; Quaglioni, S (reprint author), Lawrence Livermore Natl Lab, POB 808,L-414, Livermore, CA 94551 USA.; Hupin, G (reprint author), Univ Paris 11, CNRS, IN2P3, Inst Phys Nucl, F-91406 Orsay, France.; Raimondi, F (reprint author), Univ Surrey, Fac Engn & Phys Sci, Dept Phys, Guildford GU2 7XH, Surrey, England.; Hupin, G (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM f.raimondi@surrey.ac.uk; hupin@ipno.in2p3.fr; navratil@triumf.ca; quaglioni1@llnl.gov FU National Research Council of Canada; NSERC [401945-2011]; LLNL [DE- AC52-07NA27344]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [SCW1158] FX F.R. would like to acknowledge fruitful discussions with Jeremy Dohet-Eraly. TRIUMF receives federal funding via a contribution agreement with the National Research Council of Canada. This work was supported in part by NSERC under Grant No. 401945-2011, by LLNL under Contract DE- AC52-07NA27344, and by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Work Proposal Number SCW1158. Computing support came from the LLNL institutional Computing Grand Challenge Program and from an INCITE Award on the Titan supercomputer of the Oak Ridge Leadership Computing Facility (OLCF) at ORNL. NR 52 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 10 PY 2016 VL 93 IS 5 AR 054606 DI 10.1103/PhysRevC.93.054606 PG 14 WC Physics, Nuclear SC Physics GA DL9YB UT WOS:000375998200003 ER PT J AU Agrawal, P Chacko, Z Fortes, ECFS Kilic, C AF Agrawal, Prateek Chacko, Zackaria Fortes, Elaine C. F. S. Kilic, Can TI Skew-flavored dark matter SO PHYSICAL REVIEW D LA English DT Article ID DYNAMICAL SUPERSYMMETRY BREAKING; STANDARD MODEL; VIOLATION; COLLISIONS; SEARCH; SCALAR AB We explore a novel flavor structure in the interactions of dark matter with the Standard Model. We consider theories in which both the dark matter candidate, and the particles that mediate its interactions with the Standard Model fields, carry flavor quantum numbers. The interactions are skewed in flavor space, so that a dark matter particle does not directly couple to the Standard Model matter fields of the same flavor, but only to the other two flavors. This framework respects minimal flavor violation and is, therefore, naturally consistent with flavor constraints. We study the phenomenology of a benchmark model in which dark matter couples to right-handed charged leptons. In large regions of parameter space, the dark matter can emerge as a thermal relic, while remaining consistent with the constraints from direct and indirect detection. The collider signatures of this scenario include events with multiple leptons and missing energy. These events exhibit a characteristic flavor pattern that may allow this class of models to be distinguished from other theories of dark matter. C1 [Agrawal, Prateek] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Agrawal, Prateek] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Chacko, Zackaria] Univ Maryland, Dept Phys, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. [Fortes, Elaine C. F. S.] Univ Estadual Paulista, Inst Fis Teor, Rua Dr Bento Teobaldo Ferraz 271, BR-01140070 Sao Paulo, SP, Brazil. [Kilic, Can] Univ Texas Austin, Dept Phys, Theory Grp, Austin, TX 78712 USA. [Kilic, Can] Univ Texas Austin, Texas Cosmol Ctr, Austin, TX 78712 USA. RP Agrawal, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.; Agrawal, P (reprint author), Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. FU United States Department of Energy [De-AC02-07CH11359]; National Science Foundation (NSF) [PHY-1315155]; FAPESP [14/05505-6, 11/21945-8]; National Science Foundation [PHY-1315983, PHY-1316033]; NSF [PHY-0855591, PHY-1216270, PHY-1066293] FX Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. Z. C. is supported by the National Science Foundation (NSF) under Grant No. PHY-1315155. E. C. F. S. F. thanks the University of Maryland and NASA Goddard Space Flight Center for the hospitality while this work was being completed and FAPESP for full support under Contracts No. 14/05505-6 and No. 11/21945-8. The research of C. K. is supported by the National Science Foundation under Grants No. PHY-1315983 and No. PHY-1316033. The work of P. A. was supported in part by NSF Grants No. PHY-0855591 and No. PHY-1216270. P. A. would also like to thank the Aspen Center for Physics, which is supported by NSF Grant No. PHY-1066293. NR 61 TC 1 Z9 1 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 10 PY 2016 VL 93 IS 10 AR 103510 DI 10.1103/PhysRevD.93.103510 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM0AX UT WOS:000376005900003 ER PT J AU Banik, N Sikivie, P AF Banik, Nilanjan Sikivie, Pierre TI Evolution of velocity dispersion along cold collisionless flows SO PHYSICAL REVIEW D LA English DT Article ID DARK-MATTER; COSMIC AXIONS; SECONDARY INFALL; MILKY-WAY; SAGITTARIUS; UNIVERSE; SEARCH; HALO AB The infall of cold dark matter onto a galaxy produces cold collisionless flows and caustics in its halo. If a signal is found in the cavity detector of dark matter axions, the flows will be readily apparent as peaks in the energy spectrum of photons from axion conversion, allowing the densities, velocity vectors and velocity dispersions of the flows to be determined. We discuss the evolution of velocity dispersion along cold collisionless flows in one and two dimensions. A technique is presented for obtaining the leading behavior of the velocity dispersion near caustics. The results are used to derive an upper limit on the energy dispersion of the big flow from the sharpness of its nearby caustic and a prediction for the dispersions in its velocity components. C1 [Banik, Nilanjan; Sikivie, Pierre] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Banik, Nilanjan] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Banik, N (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA.; Banik, N (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy at the University of Florida [DE-FG02-97ER41209]; National Science Foundation at the Aspen Center for Physics [PHYS-1066293]; U.S. Department of Energy [DE-AC02-07CH11359]; Fermilab Graduate Student Research Program in Theoretical Physics FX This work was supported in part by the U.S. Department of Energy under Grant No. DE-FG02-97ER41209 at the University of Florida and the National Science Foundation under Grant No. PHYS-1066293 at the Aspen Center for Physics. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. N.B. is supported by the Fermilab Graduate Student Research Program in Theoretical Physics. NR 24 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 10 PY 2016 VL 93 IS 10 AR 103509 DI 10.1103/PhysRevD.93.103509 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DM0AX UT WOS:000376005900002 ER PT J AU Berlin, A Robertson, DS Solon, MP Zurek, KM AF Berlin, Asher Robertson, Denis S. Solon, Mikhail P. Zurek, Kathryn M. TI Bino variations: Effective field theory methods for dark matter direct detection SO PHYSICAL REVIEW D LA English DT Article ID NEUTRALINO-NUCLEON SCATTERING; LIGHT; PHENOMENOLOGY; PARTICLES AB We apply effective field theory methods to compute bino-nucleon scattering, in the case where tree-level interactions are suppressed and the leading contribution is at loop order via heavy flavor squarks or sleptons. We find that leading log corrections to fixed-order calculations can increase the bino mass reach of direct detection experiments by a factor of 2 in some models. These effects are particularly large for the bino-sbottom coannihilation region, where bino dark matter as heavy as 5-10 TeV may be detected by near future experiments. For the case of stop-and selectron-loop mediated scattering, an experiment reaching the neutrino background will probe thermal binos as heavy as 500 and 300 GeV, respectively. We present three key examples that illustrate in detail the framework for determining weak scale coefficients, and for mapping onto a low-energy theory at hadronic scales, through a sequence of effective theories and renormalization group evolution. For the case of a squark degenerate with the bino, we extend the framework to include a squark degree of freedom at low energies using heavy particle effective theory, thus accounting for large logarithms through a "heavy-light current." Benchmark predictions for scattering cross sections are evaluated, including complete leading order matching onto quark and gluon operators, and a systematic treatment of perturbative and hadronic uncertainties. C1 [Berlin, Asher] Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. [Robertson, Denis S.; Solon, Mikhail P.; Zurek, Kathryn M.] Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94709 USA. [Robertson, Denis S.; Solon, Mikhail P.; Zurek, Kathryn M.] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94709 USA. [Robertson, Denis S.] Univ Sao Paulo, Inst Fis, R Matao 187, BR-05508900 Sao Paulo, Sao, Brazil. RP Berlin, A (reprint author), Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. FU Kavli Institute for Cosmological Physics at the University of Chicago [NSF PHY-1125897]; DoE [DE-AC02-05CH11231]; Sao Paulo Research Foundation (FAPESP) FX We thank Richard Hill and Jason Kumar for valuable discussions. A. B. is supported by the Kavli Institute for Cosmological Physics at the University of Chicago through Grant No. NSF PHY-1125897. D. R., M. S., and K. Z. are supported by the DoE under Contract No. DE-AC02-05CH11231. D. R. is supported by the Sao Paulo Research Foundation (FAPESP). NR 63 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 10 PY 2016 VL 93 IS 9 AR 095008 DI 10.1103/PhysRevD.93.095008 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL9ZC UT WOS:000376001100006 ER PT J AU Sa, N Kinnibrugh, TL Wang, H Gautam, GS Chapman, KW Vaughey, JT Key, B Fister, TT Freeland, JW Proffit, DL Chupas, PJ Ceder, G Bareno, JG Bloom, ID Burrell, AK AF Sa, Niya Kinnibrugh, Tiffany L. Wang, Hao Gautam, Gopalakrishnan Sai Chapman, Karena W. Vaughey, John T. Key, Baris Fister, Timothy T. Freeland, John W. Proffit, Danielle L. Chupas, Peter J. Ceder, Gerbrand Bareno, Javier G. Bloom, Ira D. Burrell, Anthony K. TI Structural Evolution of Reversible Mg Insertion into a Bilayer Structure of V2O5 center dot nH(2)O Xerogel Material SO CHEMISTRY OF MATERIALS LA English DT Article ID X-RAY-ABSORPTION; RECHARGEABLE MAGNESIUM BATTERIES; VANADIUM PENTOXIDE GELS; CENTER-DOT H2O; V2O5 XEROGEL; MOLECULAR-DYNAMICS; CRYSTAL-STRUCTURES; SPECTROSCOPY; INTERCALATION; DEPOSITION AB Functional multivalent intercalation cathodes represent one of the largest hurdles in the development of Mg batteries. While there are many reports of Mg cathodes, many times the evidence of intercalation chemistry is only circumstantial. In this work, direct evidence of Mg intercalation into a bilayer structure of V2O5 center dot nH(2)O xerogel is confirmed, and the nature of the Mg intercalated species is reported. The interlayer spacing of V2O5 center dot nH(2)O contracts upon Mg intercalation and expands for Mg deintercalation due to the strong electrostatic interaction between the divalent cation and the cathode. A combination of NMR, pair distribution function (PDF) analysis, and X-ray absorption near edge spectroscopy (XANES) confirmed reversible Mg insertion into the V2O5 center dot nH(2)O material, and structural evolution of Mg intercalation leads to the formation of multiple new phases. Structures of V2O5 center dot nH(2)O with Mg intercalation were further supported by the first principle simulations. A solvent cointercalated Mg in V2O5 center dot nH(2)O is observed for the first time, and the Mg-25 magic angle spinning nuclear magnetic resonance (MAS NMR) spectroscopy was used to elucidate the structure obtained upon electrochemical cycling. Specifically, existence of a well-defined Mg-O environment is revealed for the Mg intercalated structures. Information reported here reveals the fundamental Mg ion intercalation mechanism in a bilayer structure of V2O5 center dot nH(2)O material and provides insightful design metrics for future Mg cathodes. C1 [Sa, Niya; Wang, Hao; Vaughey, John T.; Key, Baris; Fister, Timothy T.; Proffit, Danielle L.; Burrell, Anthony K.] Argonne Natl Lab, Adv Photon Source, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. [Sa, Niya; Wang, Hao; Vaughey, John T.; Key, Baris; Proffit, Danielle L.; Bareno, Javier G.; Bloom, Ira D.; Burrell, Anthony K.] Argonne Natl Lab, Adv Photon Source, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Kinnibrugh, Tiffany L.; Chapman, Karena W.; Freeland, John W.; Chupas, Peter J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Lemont, IL 60439 USA. [Gautam, Gopalakrishnan Sai; Ceder, Gerbrand] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Sa, N; Burrell, AK (reprint author), Argonne Natl Lab, Adv Photon Source, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA.; Sa, N; Burrell, AK (reprint author), Argonne Natl Lab, Adv Photon Source, Chem Sci & Engn Div, Lemont, IL 60439 USA. EM saniyabnu@gmail.com; burrell@anl.gov RI SA, NIYA/E-8521-2017 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; DOE Office of Science [DE-AC02-06CH11357]; BES DOE [EDCBEE] FX This work was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. This research used resources at the Advanced Photon Source (beamline 20-BM-B, 4-ID-C, and 11-ID-B), the U.S. Department of Energy (DOE) Office of Science User Facilities operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The Materials Project (BES DOE Grant No. EDCBEE) is acknowledged for the simulation support. Premkumar Senguttuvan and Christopher Johnson were acknowledged for providing a chemically synthesized MgV2O5 sample. Andrew S. Lipton is acknowledged for high field NMR access at Environmental Molecular Sciences Laboratory at Pacific Northwest National Laboratory. NR 50 TC 8 Z9 8 U1 29 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2016 VL 28 IS 9 BP 2962 EP 2969 DI 10.1021/acs.chemmater.6b00026 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DL7HA UT WOS:000375810400012 ER PT J AU Li, MR Hodges, JP Retuerto, M Deng, Z Stephens, PW Croft, MC Deng, XY Kotliar, G Sanchez-Benitez, J Walker, D Greenblatt, M AF Li, Man-Rong Hodges, Jason P. Retuerto, Maria Deng, Zheng Stephens, Peter W. Croft, Mark C. Deng, Xiaoyu Kotliar, Gabriel Sanchez-Benitez, Javier Walker, David Greenblatt, Martha TI Mn2MnReO6: Synthesis and Magnetic Structure Determination of a New Transition-Metal-Only Double Perovskite Canted Antiferromagnet SO CHEMISTRY OF MATERIALS LA English DT Article ID HIGH-PRESSURE SYNTHESIS; FERRIMAGNET MN2FEREO6; WEAK FERROMAGNETISM; MAGNETORESISTANCE; TEMPERATURE; CRYSTAL; OXIDE; POLAR; ILMENITE; PHASE AB Transition-metal-only double perovskite oxides (A(2)BB'O-6) are of great interest due to their strong and unusual magnetic interactions; only one compound, Mn2FeReO6, was reported in this category to date. Herein, we report the second transition-metal-only double perovskite, Mn2MnReO6, prepared at high pressure and temperature. Mn2MnReO6 crystallizes in a monoclinic P2(1)/n structure, as established by synchrotron Xray and powder neutron diffraction (PND) methods, with eight-coordinated A sites and rock-salt arrangement of the B and B'-site MnO6 and ReO6. Both the structural analysis and the X-ray absorption near edge spectroscopy results indicate mixed valence states of the B/B'-site in mn(2)(2+)Mn(2+/3+)Re(5+/6+)O(6). The magnetic and PND studies evidence an antiferromagnetic (AFM) transition at similar to 110 K and a transition from a simple AFM to canted AFM with net ferromagnetic component at similar to 50 K. The observed Efros Shklovskii variable-range-hopping semiconducting behavior is attributed to the three (A-site Mn2+, B-site Mn2+/3+, and B'-site Re5+/6+) interpenetrating canted AFM lattices. Theoretical calculations demonstrate that the almost fully polarized Mn states in Mn2MnReO6 are driven away from the Fermi level by static on-site interactions and open a small gap, which is responsible for the insulating state in such a d-electron-rich system. These results provide insight of the electronic origin of the physical properties of Mn2MnReO6 with local electronic structure similar to that of Mn2FeReO6. C1 [Li, Man-Rong; Retuerto, Maria; Deng, Zheng; Greenblatt, Martha] Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. [Croft, Mark C.; Deng, Xiaoyu; Kotliar, Gabriel] Rutgers State Univ, Dept Phys & Astron, 610 Taylor Rd, Piscataway, NJ 08854 USA. [Hodges, Jason P.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Stephens, Peter W.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Sanchez-Benitez, Javier] Univ Complutense Madrid, Fac Ciencias Quim, Dept Quim Fis 1, E-28040 Madrid, Spain. [Walker, David] Columbia Univ, Lamont Doherty Earth Observ, 61 Route 9W, Palisades, NY 10964 USA. RP Greenblatt, M (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. EM martha@rutchem.rutgers.edu RI Sanchez-Benitez, Javier/B-2366-2012; Deng, Xiaoyu/F-2322-2015; Retuerto, Maria/D-6425-2014 OI Sanchez-Benitez, Javier/0000-0002-3108-6594; Deng, Xiaoyu/0000-0001-7802-0966; Retuerto, Maria/0000-0001-7564-3500 FU NSF-DMREF project [DMR-1435918]; Spanish projects [MAT2013-41099-R, RyC-2010-06276]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; DOE BES [DE-AC02-98CH10886]; [NSF-DMR-1507252] FX This work was supported by the NSF-DMR-1507252 grant. X.D. and G.K. are supported by the NSF-DMREF project DMR-1435918. J.S.-B. is supported by the Spanish projects MAT2013-41099-R and RyC-2010-06276. A portion of this research at ORNL's Spoliation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Use of the NSLS, Brookhaven National Laboratory was supported by the DOE BES (DE-AC02-98CH10886). We would like to thank Ms. J. Hanley at LDEO in Columbia University for making the high pressure assemblies. NR 57 TC 1 Z9 1 U1 16 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAY 10 PY 2016 VL 28 IS 9 BP 3148 EP 3158 DI 10.1021/acs.chemmater.6b00755 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DL7HA UT WOS:000375810400031 ER PT J AU Zeno, WF Rystov, A Sasaki, DY Rishud, SH Longo, ML AF Zeno, Wade F. Rystov, Alice Sasaki, Darryl Y. Rishud, Subhash H. Longo, Marjorie L. TI Crowding-Induced Mixing Behavior of Lipid Bilayers: Examination of Mixing Energy, Phase, Packing Geometry, and Reversibility SO LANGMUIR LA English DT Article ID MEMBRANE SCAFFOLD PROTEINS; MONTE-CARLO-SIMULATION; SUPPORTED BILAYERS; NANOLIPOPROTEIN PARTICLES; TAGGED PROTEINS; CURVATURE; NANODISCS; MIXTURES; VESICLES; SILICA AB In an effort to develop a general thermodynamic model from first-principles to describe the mixing behavior of lipid membranes, we examined lipid mixing induced by targeted binding of small (Green Fluorescent Protein (GFP)) and large (nanolipoprotein particles (NLPs)) structures to specific phases of phase-separated lipid bilayers. Phases were targeted by incorporation of phase-partitioning iminodiacetic acid (IDA)-functionalized lipids into ternary lipid mixtures consisting of DPPC, DOPC, and cholesterol. GFP and NLPs, containing histidine tags, bound the IDA portion of these lipids via a metal, Cu2+, chelating mechanism. In giant unilamellar vesicles (GUVs), GFP and NLPs bound to the L-o domains of bilayers containing DPIDA, and bound to the L-d region of bilayers containing DOIDA. At sufficiently large concentrations of DPIDA or DOIDA, lipid mixing was induced by bound GFP and NLPs. The validity of the thermodynamic model was confirmed when it was found that the statistical mixing distribution as a function of crowding, energy for smaller GFP and larger NLPs collapsed to the same trend line for each GUV composition. Moreover, results of this analysis show that the free energy of mixing for a ternary lipid bilayer consisting of DOPC, DPPC, and cholesterol varied from 7.9 X 10(-22) to 1.5 X 10(-20) J/lipid at the compositions observed, decreasing as the relative cholesterol concentration was increased. It was discovered that there appears to be a maximum packing density, and associated maximum crowding pressure, of the NLPs, suggestive of circular packing. A similarity in mixing induced by NLP1 and NLP3 despite large difference in projected areas was analytically consistent with monovalent (one histidine tag) versus divalent (two histidine tags) surface interactions, respectively. In addition to GUVs, binding and induced mixing behavior of NLPs was also observed on planar, supported lipid multibilayers. The mixing process was reversible, with L-o domains reappearing after addition of EDTA for NLP removal. C1 [Zeno, Wade F.; Rystov, Alice; Longo, Marjorie L.] Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. [Rishud, Subhash H.] Univ Calif Davis, Det Mat Sci & Engn, Davis, CA 95616 USA. [Sasaki, Darryl Y.] Sandia Natl Labs, POB 969, Livermore, CA 94551 USA. RP Longo, ML (reprint author), Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. EM mllongo@ucdavis.edu FU National Science Foundation [DMR-1500275]; NIGMS-NIH [T32-GM008799]; Blacutt-Underwood Endowed Chair funds; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [KC0203010]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX M.L.L., S.H.R, and W.F.Z. acknowledge partial support from the National Science Foundation under award number DMR-1500275. W.F.Z. was partially supported by Grant Number T32-GM008799 from NIGMS-NIH. S.H.R. also acknowledges partial support derived from his Blacutt-Underwood Endowed Chair funds. D.Y.S. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under award number KC0203010. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 46 TC 1 Z9 1 U1 7 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 10 PY 2016 VL 32 IS 18 BP 4688 EP 4697 DI 10.1021/acs.langmuir.6b00831 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DL7GN UT WOS:000375809100034 PM 27096947 ER PT J AU Gu, XD Gunkel, I Hexemer, A Russell, TP AF Gu, Xiaodan Gunkel, Ilja Hexemer, Alexander Russell, Thomas P. TI Controlling Domain Spacing and Grain Size in Cylindrical Block Copolymer Thin Films by Means of Thermal and Solvent Vapor Annealing SO MACROMOLECULES LA English DT Article ID DIBLOCK COPOLYMERS; PHASE-BEHAVIOR; DIFFUSION; LITHOGRAPHY; PATTERNS; ORDER; OPTIMIZATION; TEMPLATES; MESOSCALE; POLYMERS AB Red-time grazing-incidence small-angle X-ray scattering (GISAXS) experiments were used to study the self assembly of cylinder-forming block copolymers (BCPs) in thin films during thermal annealing and solvent vapor annealing. BCP thin films were annealed-in near-neutral solvent vapor for solvent vapor annealing and on a hot plate under an inert gas atmosphere for thermal annealing. The initially ordered films were heated or swollen to induce an order disorder transition (ODT) and then cooled or the solvent was removed, respectively. The,domain spacings of BCPs as determined from in situ GISAXS measurements during solvent removal. and cooling were analyzed with respect to the polymer concentration and the reciprocal temperature., Close to the ODT the domain spacing was found to be nearly identical for thermal and solvent vapor annealing. At lower solvent concentrations phi and lower temperatures T, the domain spacing was found to increase for both thermal and solvent vapor annealing until structural reorganization in the film was limited by the slow kinetics at solvent concentrations and temperatures close to the glass transition. In this regime, the domain spacing in solvent annealed films was found to be higher than that in, thermally annealed films, which is likely due to a significantly smaller diffusion coefficient in the case of thermal annealing. On the basis of an ex situ scanning electron microscopy characterization of annealed block copolymer thin films, we show that the grain size of the cylindrical: microdomains can be strongly increased by annealing films dose to the ODT. Well below phi(ODT) and T-ODT, the formation of large grains is kinetically limited. In thermally annealed films the grain size was found to smaller than that for the solvent annealed films, which was attributed to a smaller diffusion-coefficient in the absence of solvent. C1 [Gu, Xiaodan; Gunkel, Ilja; Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. [Gunkel, Ilja; Hexemer, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Gu, Xiaodan] Stanford Univ, Dept Chem Engn, 443 Via Ortega, Stanford, CA 94305 USA. [Gunkel, Ilja] Adolphe Merkle Inst, Chemin Verdiers 4, CH-1700 Fribourg, Switzerland. RP Russell, TP (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA.; Russell, TP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM russell@mail.pse.umass.edu OI Gunkel, Ilja/0000-0001-5738-5309 FU U.S. Department of Energy BES [BES-DE-FG02-96ER45612]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; ALS Doctoral Fellowship program; ALS Postdoctoral Fellowship program; DOE Early Career Research Program grant FX This work was supported by the U.S. Department of Energy BES under Contract BES-DE-FG02-96ER45612. Beamline 7.3.3 of the Advanced Light Source is supported by the Director of the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. X. Gu acknowledges an ALS Doctoral Fellowship program for providing partial financial support. I.G. acknowledges the support by the ALS Postdoctoral Fellowship program. A.H. was supported by a DOE Early Career Research Program grant. The authors also gratefully acknowledge the assistance of E. Schaible with GISAXS measurements. NR 45 TC 6 Z9 6 U1 27 U2 61 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2016 VL 49 IS 9 BP 3373 EP 3381 DI 10.1021/acs.macromol.6b00429 PG 9 WC Polymer Science SC Polymer Science GA DL7GT UT WOS:000375809700018 ER PT J AU Ogawa, H Takenaka, M Miyazaki, T Fujiwara, A Lee, B Shimokita, K Nishibori, E Takata, M AF Ogawa, Hiroki Takenaka, Mikihito Miyazaki, Tsukasa Fujiwara, Akihiko Lee, Byeongdu Shimokita, Keisuke Nishibori, Eiji Takata, Masaki TI Direct Observation on Spin-Coating Process of PS-b-P2VP Thin Films SO MACROMOLECULES LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; X-RAY-SCATTERING; BLOCK-COPOLYMER; SOLVENT EVAPORATION; PHASE-BEHAVIOR; SMALL-ANGLE; SELECTIVE SOLVENT; MEMBRANES; MICRODOMAINS; ORIENTATION AB We studied the structural development of symmetric poly(styrene-b-2-vinylpyridine) (PS-b-P2VP)block copolymers during spin-coating using in situ grazing incidence small-angle X-ray scattering (GISAXS) measurements. During the spin-coating process, after the formation of the micelles in dilute solution,, the selective solvent-induced two kinds of the morphological transition. First, the disordered spherical micelles were transformed into a BCC lattice of spheres, of which the (110) plane was oriented perpendicularly to the subtrate surface. Second, further evaporation induced a transition from spheres on the BCC lattice into cylindrical structures. The orientation of the cylinders perpendicular to the substrate surface was induced by solvent convection perpendicular to the substrate, which occurs during rapid solvent evaporation. After this transition, vitrification of PS and P2VP prevented any further transition from cylinders to the more thermodynamically stable lamellar structures, as are generally observed as the bulk equilibrium state. C1 [Ogawa, Hiroki] Kyoto Univ, Inst Chem Res, Uji, Kyoto 6110011, Japan. [Ogawa, Hiroki; Fujiwara, Akihiko; Takata, Masaki] Japan Synchrotron Radiat Res Inst, 1-1-1 Kouto, Sayo, Hyogo 6795198, Japan. [Takenaka, Mikihito] Kyoto Univ, Grad Sch Engn, Dept Polymer Chem, Kyoto 6158510, Japan. [Miyazaki, Tsukasa; Shimokita, Keisuke] Nitto Denko Corp, 1-1-2 Shimohozumi, Ibaraki, Osaka 5678680, Japan. [Lee, Byeongdu] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Nishibori, Eiji] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba Res Ctr Interdisciplinary Mat Sci, 1-1-1 Tennodai, Tsukuba, Ibaraki 3058571, Japan. [Ogawa, Hiroki; Takenaka, Mikihito; Nishibori, Eiji; Takata, Masaki] RIKEN SPring 8 Ctr, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. RP Ogawa, H (reprint author), Kyoto Univ, Inst Chem Res, Uji, Kyoto 6110011, Japan.; Ogawa, H (reprint author), Japan Synchrotron Radiat Res Inst, 1-1-1 Kouto, Sayo, Hyogo 6795198, Japan.; Ogawa, H (reprint author), RIKEN SPring 8 Ctr, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. EM ogawa@scl.kyoto-u.ac.jp RI Fujiwara, Akihiko/F-3031-2015 OI Fujiwara, Akihiko/0000-0002-1319-388X FU Ministry of Education, Science, Sports, and Culture of Japan [25790095]; MEXT [22108530]; Photon and Quantum Basic Research Coordinated Development Program by MEXT, Japan; U.S. DOE [DE-AC02-06CH11357] FX This work was supported by a Grant-in-aid from the Ministry of Education, Science, Sports, and Culture of Japan (No. 25790095), and a Grant-in-aid for Scientific Research on Innovative Areas ("Coordination Programming", Area 2107, Grant No. 22108530) from MEXT, Photon and Quantum Basic Research Coordinated Development Program by MEXT, Japan. SR GISAXS measurements were carried out at the first hutch of the Consortium of Advanced Softmaterial Beamline (FSBL) with the proposal No. 2013A1871 and 2013B7264. BL12ID-B at Advanced Photon Source was supported by the U.S. DOE under Contract DE-AC02-06CH11357. We would like to thank Professor Toshiji Kanaya (KEK) and Atsushi Takahara (Kyushu University) for helpful discussions. NR 36 TC 2 Z9 2 U1 19 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2016 VL 49 IS 9 BP 3471 EP 3477 DI 10.1021/acs.macromol.6b00049 PG 7 WC Polymer Science SC Polymer Science GA DL7GT UT WOS:000375809700028 ER PT J AU Morgan, B Dadmun, MD AF Morgan, Brian Dadmun, Mark D. TI Illumination of Conjugated Polymer in Solution Alters Its Conformation and Thermodynamics SO MACROMOLECULES LA English DT Article ID SOLUTION VISCOSITY CHANGE; PHOTORESPONSIVE POLYMERS; THIN-FILMS; MORPHOLOGY CONTROL; OPTICAL-PROPERTIES; CHARGE-TRANSPORT; ENERGY-TRANSFER; LIGHT; POLY(3-HEXYLTHIOPHENE); CHAIN AB The importance of chain structure in conjugated polymer-based material active layers and its relation to device efficiencies in OPVs, organic field transistors, OLEDs, and other devices has been well established. However, the influence that the absorbance of the light inherent to these devices might have on the conjugated polymer structure is not well understood. Herein, we employ small angle neutron scattering to investigate structural change's occurring in solutions of poly(3-hexylthiophene-2,5-diyl) with exposure to white light. Results indicate significant decrease in both Kuhn length (b) and radius of gyration (R-g) of the polymer upon illumination, coupled with a drop in the second virial coefficient (A(2)). We explain this phenomenon through a chain collapse model, proposing that the interaction of light with the polymer backbone alters its thermodynamic interactions with and solubility in the surrounding solvent. The presence of such an effect, which we observe in several conjugated polymers, introduces the possibility of a powerful, nondestructive, and tunable method for controlling polymer conformation in solution. This in turn opens a path to develop a broad range of new light-responsive materials, in that a variety of conjugated polymers could be used as the stimuli-responsive material. Additional implications include the identification of the importance of illumination in the reproducible fabrication of organic electronic active layers from conjugated polymer inks. C1 [Morgan, Brian; Dadmun, Mark D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Dadmun, Mark D.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Dadmun, MD (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Dadmun, MD (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM dad@utk.edu FU National Science Foundation [DMR-1409034, DMR-0944772]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The authors gratefully acknowledge the National Science Foundation (DMR-1409034) for support of this project. We also acknowledge the support of the National Institute of Standards and Technology, U.S. Department of Commerce, in providing the SANS facilities used in this work, where these facilities are supported in part by the National Science Foundation under Agreement DMR-0944772. A portion of this research was also completed at ORNL's High Flux Isotope Reactor, which was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 44 TC 2 Z9 2 U1 8 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2016 VL 49 IS 9 BP 3490 EP 3496 DI 10.1021/acs.macromol.6b00527 PG 7 WC Polymer Science SC Polymer Science GA DL7GT UT WOS:000375809700030 ER PT J AU Chintapalli, M Timachova, K Olson, KR Mecham, SJ Devaux, D DeSimone, JM Balsara, NP AF Chintapalli, Mahati Timachova, Ksenia Olson, Kevin R. Mecham, Sue J. Devaux, Didier DeSimone, Joseph M. Balsara, Nitash P. TI Relationship between Conductivity, Ion Diffusion, and Transference Number in Perfluoropolyether Electrolytes SO MACROMOLECULES LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; NUCLEAR-MAGNETIC-RESONANCE; RECHARGEABLE LI BATTERIES; STEADY-STATE CURRENT; POLYMER ELECTROLYTES; TRANSPORT-PROPERTIES; SALT; WEIGHT; LIQUID; PEO AB Connecting continuum-scale ion transport properties such as conductivity and cation transference number to microscopic transport properties such as ion dissociation and ion self-diffusivities is an unresolved challenge in characterizing polymer electrolytes. Better understanding of the relationship between microscopic and continuum scale transport properties would enable the rational design of improved electrolytes for applications such as lithium batteries. We present measurements of continuum and microscopic ion transport properties of nonflammable liquid electrolytes consisting of binary mixtures of lithium bis(trifluoromethanesulfonyl)imide (LiTFSI) and perfluoropolyethers (PFPE) with different end groups: diol, dimethyl carbonate, ethoxy-diol, and ethoxy-dimethyl carbonate. The continuum properties, conductivity and cation transference number, were measured by ac impedance spectroscopy and potentiostatic polarization, respectively. The ion self-diffusivities were measured by pulsed field gradient nuclear magnetic resonance spectroscopy (PFG-NMR), and a microscopic cation transference number was calculated from these measurements. The measured ion self-diffusivities did not reflect the measured conductivities; in some cases, samples with high diffusivities exhibited low conductivity. We introduce a nondimensional parameter, beta, that combines microscopic diffusivities and conductivity. We show that beta is a sensitive function of end-group chemistry. In the ethoxylated electrolytes, beta is close to unity, the value expected for electrolytes that obey the Nernst-Einstein equation. In these cases, the microscopic and continuum transference numbers are in reasonable agreement. PFPE electrolytes devoid of ethoxy groups exhibit values of beta that are significantly lower than unity. In these cases, there is significant deviation between microscopic and continuum transference numbers. We propose that this may be due to electrostatic coupling of the cation and anion or contributions to the NMR signal from neutral ion pairs. C1 [Chintapalli, Mahati] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Timachova, Ksenia; Balsara, Nitash P.] Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA. [Chintapalli, Mahati; Timachova, Ksenia; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Devaux, Didier; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Olson, Kevin R.; Mecham, Sue J.; DeSimone, Joseph M.] Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA. [DeSimone, Joseph M.] N Carolina State Univ, Dept Biomol & Chem Engn, Raleigh, NC 27695 USA. RP Balsara, NP (reprint author), Univ Calif Berkeley, Dept Biomol & Chem Engn, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.; DeSimone, JM (reprint author), Univ N Carolina, Dept Chem, CB 3290, Chapel Hill, NC 27599 USA.; DeSimone, JM (reprint author), N Carolina State Univ, Dept Biomol & Chem Engn, Raleigh, NC 27695 USA. EM desimone@unc.edu; nbalsara@berkeley.edu FU Center for Mesoscale Transport Properties, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012673] FX This work was supported as part of the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award #DE-SC0012673. The authors thank Dr. Christopher Canlas for guidance with NMR experiments. NR 50 TC 5 Z9 5 U1 36 U2 83 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAY 10 PY 2016 VL 49 IS 9 BP 3508 EP 3515 DI 10.1021/acs.macromol.6b00412 PG 8 WC Polymer Science SC Polymer Science GA DL7GT UT WOS:000375809700032 ER PT J AU Bie, BX Huang, JY Su, B Lu, L Fan, D E, JC Sun, T Fezzaa, K Qi, ML Luo, SN AF Bie, B. X. Huang, J. Y. Su, B. Lu, L. Fan, D. E, J. C. Sun, T. Fezzaa, K. Qi, M. L. Luo, S. N. TI Dynamic tensile deformation and damage of B4C-reinforced Al composites: Time-resolved imaging with synchrotron x-rays SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Metal-matrix composites (MMCs); Fracture; Fractography; Radiography ID METAL-MATRIX COMPOSITES; PARTICLE-REINFORCED ALUMINUM; SINGLE-CRYSTAL MULTILAYERS; MECHANICAL-PROPERTIES; BEHAVIOR; MICRODIFFRACTION; SIZE; MICROSTRUCTURE; FABRICATION; PLASTICITY AB Dynamic tensile experiments are conducted on 15% and 30% in weight percentage B4C/Al composites with a split Hopkinson tension bar, along with high-speed synchrotron x-ray digital image correlation (XDIC) to map strain fields at mu m and mu s scales. As manifested by bulk-scale stress-strain curves, a higher particle content leads to a higher yield strength but lower ductility. Strain field mapping by XDIC demonstrates that tension deformation and tensile fracture, as opposed to shear and shear failure, dominate deformation and failure of the composites. The fractographs of recovered samples show consistent features. The particle-matrix interfaces are nucleation sites for strain localizations, and their propagation and coalescence are diffused by the Al matrix. The reduced spacing between strain localization sites with increasing particle content, facilitates their coalescence and leads to decreased ductility. Designing a particle-reinforced, metallic-matrix composite with balanced strength and ductility should consider optimizing the inter-particle distance as a key parameter. (C) 2016 Elsevier B.V. All rights reserved. C1 [Bie, B. X.; Qi, M. L.] Wuhan Univ Technol, Sch Sci, Wuhan 430070, Hubei, Peoples R China. [Bie, B. X.; Huang, J. Y.; Luo, S. N.] Southwest Jiaotong Univ, Minist Educ, Key Lab Adv Technol Mat, Chengdu 610031, Sichuan, Peoples R China. [Bie, B. X.; Huang, J. Y.; Lu, L.; Fan, D.; E, J. C.; Luo, S. N.] Peac Inst Multiscale Sci, Chengdu 610207, Sichuan, Peoples R China. [Huang, J. Y.; Lu, L.] Univ Sci & Technol China, Dept Modern Mech, CAS Key Lab Mat Behav & Design, Hefei 230027, Anhui, Peoples R China. [Su, B.] China Acad Engn Phys, Inst Mat, Mianyang 621900, Sichuan, Peoples R China. [Sun, T.; Fezzaa, K.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Qi, ML (reprint author), Wuhan Univ Technol, Sch Sci, Wuhan 430070, Hubei, Peoples R China.; Luo, SN (reprint author), Peac Inst Multiscale Sci, Chengdu 610207, Sichuan, Peoples R China. EM emmy_qi@163.cn; sluo@pims.ac.cn RI Luo, Sheng-Nian /D-2257-2010; OI Luo, Sheng-Nian /0000-0002-7538-0541; E, Juncheng/0000-0001-6061-5734 FU 973 Project [2014CB845904]; NSAF [U1330111]; National Natural Science Foundation of China [11172221, 11472253]; US DOE [DE-AC02-06CH11357] FX This work was partially supported by the 973 Project (2014CB845904), NSAF (No. U1330111) and National Natural Science Foundation of China (11172221 and 11472253). Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract no. DE-AC02-06CH11357. NR 39 TC 2 Z9 2 U1 12 U2 31 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAY 10 PY 2016 VL 664 BP 86 EP 93 DI 10.1016/j.msea.2016.03.124 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DL7KN UT WOS:000375819700010 ER PT J AU Ye, R Hurlburt, TJ Sabyrov, K Alayoglu, S Somorjai, GA AF Ye, Rong Hurlburt, Tyler J. Sabyrov, Kairat Alayoglu, Selim Somorjai, Gabor A. TI Molecular catalysis science: Perspective on unifying the fields of catalysis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE catalysis; surface chemistry; nanocatalyst synthesis; in situ characterization; real-time dynamics ID RAY PHOTOELECTRON-SPECTROSCOPY; MESOPOROUS SILICA; ABSORPTION SPECTROSCOPY; NANOPARTICLE CATALYSTS; HETEROGENEOUS CATALYST; PYRROLE HYDROGENATION; SHAPE CONTROL; SURFACE; GOLD; SIZE AB Colloidal chemistry is used to control the size, shape, morphology, and composition of metal nanoparticles. Model catalysts as such are applied to catalytic transformations in the three types of catalysts: heterogeneous, homogeneous, and enzymatic. Real-time dynamics of oxidation state, coordination, and bonding of nanoparticle catalysts are put under the microscope using surface techniques such as sum-frequency generation vibrational spectroscopy and ambient pressure X-ray photoelectron spectroscopy under catalytically relevant conditions. It was demonstrated that catalytic behavior and trends are strongly tied to oxidation state, the coordination number and crystallographic orientation of metal sites, and bonding and orientation of surface adsorbates. It was also found that catalytic performance can be tuned by carefully designing and fabricating catalysts from the bottom up. Homogeneous and heterogeneous catalysts, and likely enzymes, behave similarly at the molecular level. Unifying the fields of catalysis is the key to achieving the goal of 100% selectivity in catalysis. C1 [Ye, Rong; Hurlburt, Tyler J.; Sabyrov, Kairat; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ye, Rong; Hurlburt, Tyler J.; Sabyrov, Kairat; Alayoglu, Selim; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Somorjai, GA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu OI Ye, Rong/0000-0002-4171-5964 FU Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the US Department of Energy [De-AC02-05CH11231] FX The work shown in this perspective article was supported by the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the US Department of Energy under Contract De-AC02-05CH11231. NR 63 TC 4 Z9 4 U1 44 U2 75 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 10 PY 2016 VL 113 IS 19 BP 5159 EP 5166 DI 10.1073/pnas.1601766113 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL2QA UT WOS:000375478800034 PM 27114536 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertolia, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connellb, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A 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CA ATLAS Collaboration TI Measurement of the dependence of transverse energy production at large pseudorapidity on the hard-scattering kinematics of proton-proton collisions at root s=2.76 TeV with ATLAS SO PHYSICS LETTERS B LA English DT Article ID ROOT-S-NN=2.76 TEV; LEAD COLLISIONS; JET PRODUCTION; DETECTOR; CENTRALITY; COLLIDER; EVENTS; PLUS AB The relationship between jet production in the central region and the underlying-event activity in a pseudorapidity-separated region is studied in 4.0 pb(-1) of root s = 2.76 TeV pp collision data recorded with the ATLAS detector at the LHC. The underlying event is characterised through measurements of the average value of the sum of the transverse energy at large pseudorapidity downstream of one of the protons, which are reported here as a function of hard-scattering kinematic variables. The hard scattering is characterised by the average transverse momentum and pseudorapidity of the two highest transverse momentum jets in the event. The dijet kinematics are used to estimate, on an event-by-event basis, the scaled longitudinal momenta of the hard-scattered partons in the target and projectile beam-protons moving toward and away from the region measuring transverse energy, respectively. Transverse energy production at large pseudorapidity is observed to decrease with a linear dependence on the longitudinal momentum fraction in the target proton and to depend only weakly on that in the projectile proton. The results are compared to the predictions of various Monte Carlo event generators, which qualitatively reproduce the trends observed in data but generally underpredict the overall level of transverse energy at forward pseudorapidity. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, A.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Stanek, R. W.; Van Gemmeren, R.; Vaniachine, A.; Wang, R.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, POB 19059, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; St Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, GR-15773 Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Juste Rozas, A.; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pacheco Pages, A.; Padilla Aranda, C.; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Barcelona Inst Sci & Technol, Inst Fis Altes Energies, Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Rosendahl, P. L.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W. -M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W. -M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Invalidenstr 110, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Gach, G. P.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Gabrielli, A.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, R.; Stillings, J. A.; Tannoury, N.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarrod, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Damazio, D. Oliveira; Paige, F.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariua, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Wuhan, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Lab Nazl Frascati, INFN, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewskaa, D.; Kopernya, S.; Kowalskia, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. 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Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Barreiro Guimaraes da Costa, J.; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Langa, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villara, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, Inst Tech Informat, ZITI, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Univ Innsbruck, Inst Astro & Teilchenphysik, A-6020 Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. 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E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. 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D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, G.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, R.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, R.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Victoria, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; True, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, Lansing, MI USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazzaa, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazzaa, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van Der Deijl, Rc.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van Der Deijl, Rc.; van der Geer, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, R.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, R.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris 11, LAL, CNRS,IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livana, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livana, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Reichert, J.; Stahlman, I.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov', D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrument & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, R.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, R.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, R.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, NRC KI, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Particle Phys Dept, Rutherford Appleton Lab, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminaria, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferroa, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferroa, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, DSM IRFU Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladivab, E.; Strizenec, P.; Urban, I.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connellb, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertolia, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Kamenshchikov, A.; Khandanyana, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertolia, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyana, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, Re.; Strandberg, S.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silveri, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. 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RI Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; Chiarelli, Giorgio/E-8953-2012; Casado, Pilar/H-1484-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; Gladilin, Leonid/B-5226-2011; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Mashinistov, Ruslan/M-8356-2015; White, Ryan/E-2979-2015; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; OI Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Chiarelli, Giorgio/0000-0001-9851-4816; Casado, Pilar/0000-0002-0394-5646; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Gladilin, Leonid/0000-0001-9422-8636; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Brooks, William/0000-0001-6161-3570; Vykydal, Zdenek/0000-0003-2329-0672; Mashinistov, Ruslan/0000-0001-7925-4676; White, Ryan/0000-0003-3589-5900; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, FP7, European Union; Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 37 TC 3 Z9 3 U1 18 U2 84 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 10 EP 28 DI 10.1016/j.physletb.2016.02.056 PG 19 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200003 ER PT J AU Yin, Y Liao, JF AF Yin, Yi Liao, Jinfeng TI Hydrodynamics with chiral anomaly and charge separation in relativistic heavy ion collisions SO PHYSICS LETTERS B LA English DT Article ID MAGNETIC-FIELD; ODD BUBBLES; FLUCTUATIONS; VIOLATION; EVENT; QCD AB Matter with chiral fermions is microscopically described by theory with quantum anomaly and macroscopically described (at low energy) by anomalous hydrodynamics. For such systems in the presence of external magnetic field and chirality imbalance, a charge current is generated along the magnetic field direction - a phenomenon known as the Chiral Magnetic Effect (CME). The quark-gluon plasma created in relativistic heavy ion collisions provides an (approximate) example, for which the CME predicts a charge separation perpendicular to the collisional reaction plane. Charge correlation measurements designed for the search of such signal have been done at RHIC and the LHC for which the interpretations, however, remain unclear due to contamination by background effects that are collective flow driven, theoretically poorly constrained, and experimentally hard to separate. Using anomalous (and viscous) hydrodynamic simulations, we make a first attempt at quantifying contributions to observed charge correlations from both CME and background effects in one and same framework. The implications for the search of CME are discussed. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Yin, Yi] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Liao, Jinfeng] Indiana Univ, Dept Phys, 2401 N Milo B Sampson Lane, Bloomington, IN 47408 USA. [Liao, Jinfeng] Indiana Univ, Ctr Explorat Energy & Matter, 2401 N Milo B Sampson Lane, Bloomington, IN 47408 USA. [Liao, Jinfeng] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Bldg 510A, Upton, NY 11973 USA. RP Yin, Y (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM yyin@bnl.gov; liaoji@indiana.edu FU DOE grant [DE-AC02-98CH10886]; National Science Foundation [PHY-1352368]; RIKEN BNL Research Center FX We thank A. Bzdak, Y. Hirono, D. Kharzeev, V. Koch, S. Schlichting, C. Shen for discussions and communications. We are particularly grateful to U. Heinz, P. Huovinen, H. Song and C. Shen who made simulation results of "VISH" available to the public. This work is supported in part by DOE grant No. DE-AC02-98CH10886 (Y.Y.) and by the National Science Foundation Grant No. PHY-1352368 (J.L.). J.L. is also grateful to the RIKEN BNL Research Center for partial support. NR 51 TC 4 Z9 4 U1 5 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. 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Winklmeier, F. Winston, O. J. Winter, B. T. Wittgen, M. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. YauWong, K. H. Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the charge asymmetry in highly boosted top-quark pair production in root s=8 TeV pp collision data collected by the ATLAS experiment SO PHYSICS LETTERS B LA English DT Article ID HADRON COLLIDERS; JET SUBSTRUCTURE; RESUMMATION; LHC AB In the pp -> t (t) over bar process the angular distributions of top and anti-top quarks are expected to present a subtle difference, which could be enhanced by processes not included in the Standard Model. This Letter presents a measurement of the charge asymmetry in events where the top-quark pair is produced with a large invariant mass. The analysis is performed on 20.3 fb(-1) of pp collision data at root s=8 TeV collected by the ATLAS experiment at the LHC, using reconstruction techniques specifically designed for the decay topology of highly boosted top quarks. The charge asymmetry in a fiducial region with large invariant mass of the top-quark pair (m(t (t) over bar) > 0.75 TeV) and an absolute rapidity difference of the top and anti-top quark candidates within -2 vertical bar y(t)vertical bar - vertical bar y(<(t) over bar)vertical bar < 2is measured to be 4.2 +/- 3.2%, in agreement with the Standard Model prediction at next-to-leading order. A differential measurement in three <(t)over bar> mass bins is also presented. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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B.] Univ Fed Sao Joao del Rei, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarrod, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescub, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Bossio Sola, J. D.; Marceca, G.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sanchez, C. A. Solans; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Tremblet, L.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastrandrea, P.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; Ristic, B.; Schram, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoya, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, A.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borisov, A.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Lefebvre, M.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Departamento Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. 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A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Alviggi, M. G.; Beddall, A.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; McFadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Aloisio, A.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, CNRS, Univ Paris Saclay, IN2P3,LAL, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr, Inst High Energy Phys Protvino, NRC KI, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrania, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescua, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [ElKacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univ, F-91191 Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silversteina, S. B.; Sjolin, J.; Tylmad, M.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Aloisio, A.; Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, D.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, C.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; McGoldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Acharya, B. S.; Barisonzi, M.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Alberich, L. Cerda; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Alberich, L. Cerda; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, A.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Alberich, L. Cerda; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. 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RI messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; White, Ryan/E-2979-2015; Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Lazzaroni, Massimo/N-3675-2015; Mashinistov, Ruslan/M-8356-2015; Gladilin, Leonid/B-5226-2011 OI Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; White, Ryan/0000-0003-3589-5900; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Di Domenico, Antonio/0000-0001-8078-2759; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Brooks, William/0000-0001-6161-3570; Vykydal, Zdenek/0000-0003-2329-0672; Lazzaroni, Massimo/0000-0002-4094-1273; Mashinistov, Ruslan/0000-0001-7925-4676; Gladilin, Leonid/0000-0001-9422-8636 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE , United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, FP7, European Union; Horizon 2020 and Marie SklodowskaCurie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie SklodowskaCurie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 83 TC 5 Z9 5 U1 17 U2 62 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 52 EP 71 DI 10.1016/j.physletb.2016.02.055 PG 20 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200008 ER PT J AU Loher, B Savran, D Aumann, T Beller, J Bhike, M Cooper, N Derya, V Duchene, M Endres, J Hennig, A Humby, P Isaak, J Kelley, JH Knorzer, M Pietralla, N Ponomarev, VY Romig, C Scheck, M Scheit, H Silva, J Tonchev, AP Tornow, W Wamers, F Weller, H Werner, V Zilges, A AF Loeher, B. Savran, D. Aumann, T. Beller, J. Bhike, M. Cooper, N. Derya, V. Duchene, M. Endres, J. Hennig, A. Humby, P. Isaak, J. Kelley, J. H. Knoerzer, M. Pietralla, N. Ponomarev, V. Yu. Romig, C. Scheck, M. Scheit, H. Silva, J. Tonchev, A. P. Tornow, W. Wamers, F. Weller, H. Werner, V. Zilges, A. TI The decay pattern of the Pygmy Dipole Resonance of Ce-140 SO PHYSICS LETTERS B LA English DT Article DE gamma-ray spectroscopy; Ce-140; Pygmy Dipole Resonance; Nuclear resonance fluorescence; Coincidence measurement; Quasi-particle phonon model ID GAMMA-RAY SPECTROSCOPY; INELASTIC-SCATTERING; NUCLEI; STATES; STRENGTH; ENERGY; EXCITATION; PARTICLE; SN-124; MODES AB The decay properties of the Pygmy Dipole Resonance (PDR) have been investigated in the semi-magic N=82 nucleus Ce-140 using a novel combination of nuclear resonance fluorescence and gamma-gamma coincidence techniques. Branching ratios for transitions to low-lying excited states are determined in a direct and model-independent way both for individual excited states and for excitation energy intervals. Comparison of the experimental results to microscopic calculations in the quasi-particle phonon model exhibits an excellent agreement, supporting the observation that the Pygmy Dipole Resonance couples to the ground state as well as to low-lying excited states. A 10% mixing of the PDR and the [2(1)(+) x PDR] is extracted. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Loeher, B.; Savran, D.; Isaak, J.; Silva, J.; Wamers, F.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Planckstr 1, D-64291 Darmstadt, Germany. [Loeher, B.; Savran, D.; Isaak, J.; Silva, J.; Wamers, F.] GSI Helmholtzzentrum Schwerionenforsch, Div Res, Planckstr 1, D-64291 Darmstadt, Germany. [Bhike, M.; Tornow, W.; Weller, H.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Bhike, M.; Tornow, W.; Weller, H.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Loeher, B.; Savran, D.; Isaak, J.; Silva, J.; Wamers, F.] Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. [Tonchev, A. P.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. [Kelley, J. H.] N Carolina State Univ, Dept Phys, Raleigh, NC 27607 USA. [Aumann, T.; Wamers, F.] GSI Helmholtzzentrum Schwerionenforsch, Planckstr 1, D-64291 Darmstadt, Germany. [Derya, V.; Endres, J.; Hennig, A.; Zilges, A.] Univ Cologne, Inst Kernphys, Zulpicher tr 77, D-50937 Cologne, Germany. [Loeher, B.; Aumann, T.; Beller, J.; Duchene, M.; Knoerzer, M.; Pietralla, N.; Ponomarev, V. Yu.; Romig, C.; Scheit, H.; Werner, V.] Tech Univ Darmstadt, Inst Kernphys, Schlossgartenstr 9, D-64289 Darmstadt, Germany. [Cooper, N.; Humby, P.; Werner, V.] Yale Univ, WNSL, POB 208120, New Haven, CT 06520 USA. [Scheck, M.] Univ West Scotland, Paisley PA1 2BE, Renfrew, Scotland. [Scheck, M.] Scottish Univ Phys Alliance, SUPA, Glasgow G12 8QQ, Lanark, Scotland. RP Loher, B (reprint author), GSI Helmholtzzentrum Schwerionenforsch, Planckstr 1, D-64291 Darmstadt, Germany. EM b.loeher@gsi.de RI Aumann, Thomas/B-1455-2012; Werner, Volker/C-1181-2017 OI Werner, Volker/0000-0003-4001-0150 FU Alliance Program of the Helmholtz Association [HA216/EMMI]; DFG [SFB 1245, ZI510/7-1]; U.S. DOE [DE-FG02-91ER-40609, DE-FG02-97ER-41033] FX The work described in this article is supported by the Alliance Program of the Helmholtz Association (HA216/EMMI), the DFG (SFB 1245 and ZI510/7-1) and U.S. DOE grants No. DE-FG02-91ER-40609 and No. DE-FG02-97ER-41033. NR 57 TC 1 Z9 1 U1 4 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 72 EP 76 DI 10.1016/j.physletb.2016.02.042 PG 5 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200009 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schobeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, R Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, R Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-Conde, A Reis, T Seva, T Thomas, L Velde, V Vanlaer, R Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Fagot, A Garcia, G Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, R Komm, M Lemaitre, V Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TDR Molina, J Herrera, CM Pol, ME Teles, RR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DDJ Martins, CDO De Souza, SF Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santaolalla, J 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Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Kaplan, S. Lath, A. Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Suarez, I. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, R. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Measurement of the ratio B(B-s(0) -> J/psi f(0)(980))/B(B-s(0) -> J/psi phi(1020)) in pp collisions at root s=7 TeV SO PHYSICS LETTERS B LA English DT Article ID VIOLATING PHASE PHI(S); (B)OVER-BAR(S)(0); DECAY AB A measurement of the ratio of the branching fractions of the B-s(0) meson to J/psi f(0)(980) and to J/psi phi(1020) is presented. The J/psi, f(0)(980), and phi(1020) are observed through their decays to mu(+)mu(-), pi(+)pi(-), and K+K-, respectively. The f(0) and the phi are identified by requiring |M-pi+(pi)- - 974 MeV| < 50 MeV and |M-K+(K)- - 1020 MeV| < 10 MeV. The analysis is based on a data sample of pp collisions at a centre-of-mass energy of 7 TeV, collected by the CMS experiment at the LHC, corresponding to an integrated luminosity of 5.3fb(-1). The measured ratio is B(B-s(0) -> J/psi f(0)) B(f(0) ->pi(+)pi(-))/B(B-s(0) -> J/psi phi) B(phi -> K+K-)= 0.140 +/- 0.008 (stat) +/- 0.023 (syst), where the first uncertainty is statistical and the second is systematic. (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; CMS Collaboration] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, R.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, R.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Federico 2, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Carlin, R.; Checchia, R.; Dall'Osso, M.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, R.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, R.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, R.; Simonetto, F.; Tosi, M.; Zotto, R.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, R.; Vitulo, R.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, R.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, R.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, R.; Squillacioti, R.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, R.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, R.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, R.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Moon, D. 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A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, R.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Covarelli, R.; Bargassa, R.; Beira Da Cruz E Silva, C.; Faccioli, R.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Vischia, R.] Lab Instrumentactio & Fis Expt Particulas, Lisbon, Portugal. [Finger, M., Jr.; Tsamalaidze, Z.; Gavrilenko, M.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Laney, A.; Malakhov, A.; Matveev, V.; Mitsyn, V. V.; Moisenz, R.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, R.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, R.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, R.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, R.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudou, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Sharma, A.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, R.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, R.; Casasso, S.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, R.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, R.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, R.; Hegeman, J.; Innocente, V.; Janot, R.; Kousouris, K.; Krajczar, K.; Lecoq, R.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, R.; Silva, R.; Simon, M.; Sphicas, R.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, R.; Ronga, F. J.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kanga, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Buchmann, M. A.; Baber, M.; Bainbridge, R.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, R.; Davies, G.; Della Negra, M.; Dunne, R.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, R.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, R.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, R.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, R.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; George, P. Geffert C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, R.; Merkel, R.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, R.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -R; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Xiao, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.] SUNY Coll Buffalo, Buffalo, NY 14222 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.; Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Verzetti, M.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, R.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Manganote, E. J. Tonelli] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, D-03044 Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Gulmini, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, R.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ & Quot, Moscow, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kanga, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Lokhtin, Igor/D-7004-2012; Varela, Joao/K-4829-2016; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Chinellato, Jose Augusto/I-7972-2012; Manganote, Edmilson/K-8251-2013; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Dubinin, Mikhail/I-3942-2016; Tinoco Mendes, Andre David/D-4314-2011 OI Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Varela, Joao/0000-0003-2613-3146; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699 FU BMWFW (Austria); FWF (Austria); Fonds De La Recherche Scientifique - FNRS (Belgium); Fonds De La Recherche Scientifique - FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); Fonds De La Recherche Scientifique - FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 29 TC 0 Z9 0 U1 17 U2 62 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 84 EP 102 DI 10.1016/j.physletb.2016.02.047 PG 19 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200011 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, R Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, R Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, R Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H 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Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, R D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, R Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K De Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, R De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ 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CA ATLAS Collaboration TI Evidence for single top-quark production in the s-channel in proton-proton collisions at root s=8 TeV with the ATLAS detector using the Matrix Element Method SO PHYSICS LETTERS B LA English DT Article ID HADRON COLLIDERS; PARTON DISTRIBUTIONS; LIKELIHOOD METHOD; MISSING MOMENTUM; CROSS-SECTION; LHC; RECONSTRUCTION; ALGORITHM; EVENTS; SEARCH AB This Letter presents evidence for single top-quark production in the s-channel using proton-proton collisions at a centre-of-mass energy of 8 TeV with the ATLAS detector at the CERN Large Hadron Collider. The analysis is performed on events containing one isolated electron or muon, large missing transverse momentum and exactly two b-tagged jets in the final state. The analysed data set corresponds to an integrated luminosity of 20.3 fb(-1). The signal is extracted using a maximum-likelihood fit of a discriminant which is based on the matrix element method and optimized in order to separate single-top-quark s-channel events from the main background contributions, which are top-quark pair production and W boson production in association with heavy-flavour jets. The measurement leads to an observed signal significance of 3.2 standard deviations and a measured cross-section of sigma s = 4.8 +/- 0.8(stat.)(-1.3)(+1.6)(syst.) pb, which is consistent with the Standard Model expectation. The expected significance for the analysis is 3.9 standard deviations. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. 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R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, R.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, R.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero Y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincterq, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, R.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, R.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Wuhan, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Du, Y.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pinge, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, R. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcy, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobe, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, R.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Alonso, A.; Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, E.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefal, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Samme, D.; Schillo, C.; Schumacher, M.; Sommer, R.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, E.; Iacobucci, G.; Katre, A.; Mermod, R.; Muenstermann, D.; Nackenhorst, O.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, A. S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenze, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, R.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, R.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, La Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, R.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, R.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, R.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwel, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Pre, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolod, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolod, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, R.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, R.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snider, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, R.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, R.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter's, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacours, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ride, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacours, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ride, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, R.; Krasny, M. W.; Lacours, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ride, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, D.; Tapprogge, S.; Urrejola, R.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Nagai, Y.; Nagy, E.; Pralavorio, R.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. 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A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Perez, S. Fernandez; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. 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A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ, MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, R.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Leggerl, F.; Lorenz, J.; Loesel, P. J.; Maierl, T.; Mann, A.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscherl, F.; Ruschke, A.; Sandersm, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryuninl, A. E.; Kluth, S.; Kortner, O.; Kortnerml, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Lot, D. Salihagic; Sandstroemml, R.; Schacht, R.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchil, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchil, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, R.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, R.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, R.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deij, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, O.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, R.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, R.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, R.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deij, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, O.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignottiiii, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, R.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, R.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, R.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, R.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, R.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, R.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, R.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinnia, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, R.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinnia, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, R.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, R.; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, R.; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, P-1200 Lisbon, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, P-1200 Lisbon, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, J.; Kupco, A.; Kus, V.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, R.; Staroba, R.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, R.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykyda, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, R.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, R.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, R.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, R.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tynde, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, R.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gauzzi, R.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Di Micco, B.; Farina, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwegler, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, R.; Johansson, R.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q. -S.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, R.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, R.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, U.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soifer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, O.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, O.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, 7-3-1 Hongo, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, R.; Liblong, A.; Orr, R. S.; Polifla, R.; Rudolph, M. S.; Savard, R.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, R.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacinob, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. 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[Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Guo, Jun/O-5202-2015; Gladilin, Leonid/B-5226-2011; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Nechaeva, Polina/N-1148-2015; Fedin, Oleg/H-6753-2016; Mashinistov, Ruslan/M-8356-2015; White, Ryan/E-2979-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; OI Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Guo, Jun/0000-0001-8125-9433; Gladilin, Leonid/0000-0001-9422-8636; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; White, Ryan/0000-0003-3589-5900; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Prokofiev, Kirill/0000-0002-2177-6401 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE; NSF; United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales; Aristeia programmes - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 77 TC 3 Z9 3 U1 20 U2 56 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 228 EP 246 DI 10.1016/j.physletb.2016.03.017 PG 19 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200035 ER PT J AU Tichai, A Langhammer, J Binder, S Roth, R AF Tichai, Alexander Langhammer, Joachim Binder, Sven Roth, Robert TI Hartree-Fock many-body perturbation theory for nuclear ground-states SO PHYSICS LETTERS B LA English DT Article ID OPEN-SHELL SYSTEMS; ANHARMONIC-OSCILLATOR; BORN SERIES; EXTENSION AB We investigate the order-by-order convergence behavior of many-body perturbation theory (MBPT) as a simple and efficient tool to approximate the ground-state energy of closed-shell nuclei. To address the convergence properties directly, we explore perturbative corrections up to 30th order and highlight the role of the partitioning for convergence. The use of a simple Hartree-Fock solution for the unperturbed basis leads to a convergent MBPT series for soft interactions, in contrast to the divergent MBPT series obtained with a harmonic oscillator basis. For larger model spaces and heavier nuclei, where a direct high-order MBPT calculation is not feasible, we perform third-order calculations and compare to advanced ab initio coupled-cluster results for the same interactions and model spaces. We demonstrate that third-order MBPT provides ground-state energies for nuclei up into the tin isotopic chain in excellent agreement with the best available coupled-cluster calculations at a fraction of the computational cost. (C) 2016 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Tichai, Alexander; Langhammer, Joachim; Roth, Robert] Tech Univ Darmstadt, Inst Kernphys, Petersenstr 30, D-64289 Darmstadt, Germany. [Binder, Sven] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Binder, Sven] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Tichai, A (reprint author), Tech Univ Darmstadt, Inst Kernphys, Petersenstr 30, D-64289 Darmstadt, Germany. EM alexander.tichai@physik.tu-darmstadt.de; robert.roth@physik.tu-darmstadt.de RI Roth, Robert/B-6502-2008 FU DFG [SFB 1245]; Helmholtz International Center for FAIR; BMBF [05P15RDFN1]; Alexander-von-Humboldt Foundation; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-96ER40963, DE-SC0008499, DEAC05-00OR22725]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work is supported by the DFG through grant SFB 1245, the Helmholtz International Center for FAIR, and the BMBF through contract 05P15RDFN1. S. Binder gratefully acknowledges the financial support of the Alexander-von-Humboldt Foundation (Feodor-Lynen scholarship). This material is based upon work supported in part by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Award Numbers DE-FG02-96ER40963, DE-SC0008499, and under Contract No. DEAC05-00OR22725. Numerical calculations have been performed at the computing center of the TU Darmstadt (lichtenberg), at the LOEWE-CSC Frankfurt, and at the National Energy Research Scientific Computing Center supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 3 Z9 3 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD MAY 10 PY 2016 VL 756 BP 283 EP 288 DI 10.1016/j.physletb.2016.03.029 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VS UT WOS:000373569200043 ER PT J AU Wang, HL Niu, GD Zhou, M Wang, X Park, JH Bao, SX Chi, MF Cai, ZS Xia, YN AF Wang, Helan Niu, Guangda Zhou, Ming Wang, Xue Park, Jinho Bao, Shixiong Chi, Miaofang Cai, Zaisheng Xia, Younan TI Scalable Synthesis of Palladium Icosahedra in Plug Reactors for the Production of Oxygen Reduction Reaction Catalysts SO CHEMCATCHEM LA English DT Article DE nanostructures; oxygen reduction; palladium; crystal growth ID NOBLE-METAL NANOCRYSTALS; FORMIC-ACID OXIDATION; COLLOIDAL NANOCRYSTALS; POLYOL SYNTHESIS; SILVER NANOPARTICLES; ENHANCED ACTIVITY; DROPLET REACTORS; CONTROLLED SIZES; FACETS; SHAPE AB We have synthesized Pd icosahedra with uniform, controllable sizes in plug reactors separated by air. The oxygen contained in the air segments not only contributed to the generation of a reductant from diethylene glycol in situ, but also oxidized elemental Pd back to the ionic form by oxidative etching and thus slowed down the reduction kinetics. Compared to droplet reactors involving silicone oil or fluorocarbon, the use of air as a carrier phase could reduce the production cost by avoiding additional procedures for the separation of products from the oil. The average diameters of the Pd icosahedra could be readily controlled in the range of 12-20 nm. The Pd icosahedra were further employed as seeds for the production of Pd@Pt2-3L core-shell icosahedra, which could serve as a catalyst toward the oxygen reduction reaction with greatly enhanced activity. We believe that the plug reactors could be extended to other types of noble-metal nanocrystals for their scale-up production. C1 [Wang, Helan; Niu, Guangda; Zhou, Ming; Wang, Xue; Bao, Shixiong; Xia, Younan] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. [Wang, Helan; Niu, Guangda; Zhou, Ming; Wang, Xue; Bao, Shixiong; Xia, Younan] Emory Univ, Atlanta, GA 30332 USA. [Wang, Helan; Cai, Zaisheng] Donghua Univ, Coll Chem Chem Engn & Biotechnol, Key Lab Sci & Technol Ecotext, Minist Educ, Shanghai 201620, Peoples R China. [Park, Jinho; Xia, Younan] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Xia, YN (reprint author), Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA.; Xia, YN (reprint author), Emory Univ, Atlanta, GA 30332 USA.; Xia, YN (reprint author), Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. EM younan.xia@bme.gatech.edu RI Chi, Miaofang/Q-2489-2015; Xia, Younan/E-8499-2011; OI Chi, Miaofang/0000-0003-0764-1567; Wang, Xue/0000-0002-6298-1858 FU Georgia Institute of Technology; National Science Foundation [CHE-1505441]; China Scholarship Council FX This work was supported in part by startup funds from the Georgia Institute of Technology and a grant from the National Science Foundation (CHE-1505441). As visiting Ph.D. students, H.W., G.N., X.W., and M.Z. were also partially supported by the China Scholarship Council. High-Resolution imaging was completed at the Center for Nanophase Materials Science, which is a DOE Office of Science User Facility. NR 40 TC 2 Z9 2 U1 12 U2 25 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1867-3880 EI 1867-3899 J9 CHEMCATCHEM JI ChemCatChem PD MAY 9 PY 2016 VL 8 IS 9 BP 1658 EP 1664 DI 10.1002/cctc.201600060 PG 7 WC Chemistry, Physical SC Chemistry GA DQ9KJ UT WOS:000379528500008 ER PT J AU Collins, L Belianinov, A Proksch, R Zuo, TT Zhang, Y Liaw, PK Kalinin, SV Jesse, S AF Collins, Liam Belianinov, Alex Proksch, Roger Zuo, Tingting Zhang, Yong Liaw, Peter K. Kalinin, Sergei V. Jesse, Stephen TI G-mode magnetic force microscopy: Separating magnetic and electrostatic interactions using big data analytics SO APPLIED PHYSICS LETTERS LA English DT Article ID YTTRIUM-IRON-GARNET; HIGH-ENTROPY ALLOYS; FILMS; MODULATION; INTERFACE; IMAGES AB In this work, we develop a full information capture approach for Magnetic Force Microscopy (MFM), referred to as generalized mode (G-Mode) MFM. G-Mode MFM acquires and stores the full data stream from the photodetector, captured at sampling rates approaching the intrinsic photodiode limit. The data can be subsequently compressed, denoised, and analyzed, without information loss. Here, G-Mode MFM is implemented and compared to the traditional heterodyne-based MFM on model systems, including domain structures in ferromagnetic Yttrium Iron Garnet and the electronically and magnetically inhomogeneous high entropy alloy, CoFeMnNiSn. We investigate the use of information theory to mine the G-Mode MFM data and demonstrate its usefulness for extracting information which may be hidden in traditional MFM modes, including signatures of nonlinearities and mode-coupling phenomena. Finally, we demonstrate detection and separation of magnetic and electrostatic tip-sample interactions from a single G-Mode image, by analyzing the entire frequency response of the cantilever. G-Mode MFM is immediately implementable on any atomic force microscopy platform and as such is expected to be a useful technique for probing spatiotemporal cantilever dynamics and mapping material properties, as well as their mutual interactions. Published by AIP Publishing. C1 [Collins, Liam; Belianinov, Alex; Kalinin, Sergei V.; Jesse, Stephen] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Collins, Liam; Belianinov, Alex; Kalinin, Sergei V.; Jesse, Stephen] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Proksch, Roger] Asylum Res, Santa Barbara, CA 93117 USA. [Zuo, Tingting; Zhang, Yong] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Zuo, Tingting; Liaw, Peter K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Collins, L (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Collins, L (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. RI ZHANG, Yong/B-7928-2009; OI ZHANG, Yong/0000-0002-6355-9923; Belianinov, Alex/0000-0002-3975-4112 FU U.S. Army Research Office Project [W911NF-13-1-0438]; National Science Foundation [CMMI-1100080] FX This research (for L.C., A.B., S.V.K., S.J.) was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. P.K.L. would like to acknowledge the DOE, Office of Fossil Energy, National Energy Technology Laboratory (DE-FE-0008855, DE-FE-0024054, and DE-FE-0011194). P.K.L. appreciates the support of the U.S. Army Research Office Project (W911NF-13-1-0438) and the support for the National Science Foundation (CMMI-1100080). NR 42 TC 3 Z9 3 U1 17 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 9 PY 2016 VL 108 IS 19 AR 193103 DI 10.1063/1.4948601 PG 5 WC Physics, Applied SC Physics GA DN4HA UT WOS:000377023500043 ER PT J AU Jing, C Gold, SH Fischer, R Gai, W AF Jing, C. Gold, S. H. Fischer, Richard Gai, W. TI Complete multipactor suppression in an X-band dielectric-loaded accelerating structure SO APPLIED PHYSICS LETTERS LA English DT Article AB Multipactor is a major issue limiting the gradient of rf-driven Dielectric-Loaded Accelerating (DLA) structures. Theoretical models have predicted that an axial magnetic field applied to DLA structures may completely block the multipactor discharge. However, previous attempts to demonstrate this magnetic field effect in an X-band traveling-wave DLA structure were inconclusive, due to the axial variation of the applied magnetic field, and showed only partial suppression of the multipactor loading [Jing et al., Appl. Phys. Lett. 103, 213503 (2013)]. The present experiment has been performed under improved conditions with a uniform axial magnetic field extending along the length of an X-band standing-wave DLA structure. Multipactor loading began to be continuously reduced starting from 3.5 kG applied magnetic field and was completely suppressed at similar to 8 kG. Dependence of multipactor suppression on the rf gradient inside the DLA structure was also measured. Published by AIP Publishing. C1 [Jing, C.] Euclid Techlabs LLC, 5900 Harper Rd, Solon, OH 44139 USA. [Jing, C.; Gai, W.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Gold, S. H.; Fischer, Richard] Naval Res Lab, Div Plasma Phys, Washington, DC 20375 USA. RP Jing, C (reprint author), Euclid Techlabs LLC, 5900 Harper Rd, Solon, OH 44139 USA.; Jing, C (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. FU DoE SBIR Grant [DE-SC0006303] FX This work is supported by the DoE SBIR Grant No. DE-SC0006303. We thank the Argonne Wakefield Accelerator group for supplying the solenoid and power supply used in the experiment. NR 14 TC 0 Z9 0 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 9 PY 2016 VL 108 IS 19 AR 193501 DI 10.1063/1.4949334 PG 4 WC Physics, Applied SC Physics GA DN4HA UT WOS:000377023500054 ER PT J AU Williams, TJ Taylor, AE Christianson, AD Hahn, SE Fishman, RS Parker, DS McGuire, MA Sales, BC Lumsden, MD AF Williams, T. J. Taylor, A. E. Christianson, A. D. Hahn, S. E. Fishman, R. S. Parker, D. S. McGuire, M. A. Sales, B. C. Lumsden, M. D. TI Extended magnetic exchange interactions in the high-temperature ferromagnet MnBi SO APPLIED PHYSICS LETTERS LA English DT Article ID MANGANESE BISMUTHIDE; PHASE; FILMS; FIELD AB The high-temperature ferromagnet MnBi continues to receive attention as a candidate to replace rare-earth-containing permanent magnets in applications above room temperature. This is due to a high Curie temperature, large magnetic moments, and a coercivity that increases with temperature. The synthesis of MnBi also allows for crystals that are free of interstitial Mn, enabling more direct access to the key interactions underlying the physical properties of binary Mn-based ferromagnets. In this work, we use inelastic neutron scattering to measure the spin waves of MnBi in order to characterize the magnetic exchange at low temperature. Consistent with the spin reorientation that occurs below 140 K, we do not observe a spin gap in this system above our experimental resolution. A Heisenberg model was fit to the spin wave data in order to characterize the long-range nature of the exchange. It was found that interactions up to sixth nearest neighbor are required to fully parametrize the spin waves. Surprisingly, the nearest-neighbor term is antiferromagnetic, and the realization of a ferromagnetic ground state relies on the more numerous ferromagnetic terms beyond nearest neighbor, suggesting that the ferromagnetic ground state arises as a consequence of the long-ranged interactions in the system. Published by AIP Publishing. C1 [Williams, T. J.; Taylor, A. E.; Christianson, A. D.; Lumsden, M. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Christianson, A. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA. [Hahn, S. E.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Fishman, R. S.; Parker, D. S.; McGuire, M. A.; Sales, B. C.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Phys Sci Directorate, Oak Ridge, TN 37831 USA. RP Williams, TJ (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM williamstj@ornl.gov RI McGuire, Michael/B-5453-2009; BL18, ARCS/A-3000-2012; Lumsden, Mark/F-5366-2012; OI McGuire, Michael/0000-0003-1762-9406; Lumsden, Mark/0000-0002-5472-9660; Taylor, Alice/0000-0002-3036-3019 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Wigner Fellowship program at Oak Ridge National Laboratory; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program; Critical Materials Institute, an Energy Innovation Hub; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX We acknowledge instrument support from D. A. Abernathy and J. Niedziela. This research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. T.J.W. acknowledges the support from the Wigner Fellowship program at Oak Ridge National Laboratory. M.A.M. acknowledges the support from U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program. B.C.S. and D.S.P. were supported by the Critical Materials Institute, an Energy Innovation Hub, funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. R.S.F. was supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 31 TC 7 Z9 7 U1 19 U2 42 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 9 PY 2016 VL 108 IS 19 AR 192403 DI 10.1063/1.4948933 PG 4 WC Physics, Applied SC Physics GA DN4HA UT WOS:000377023500031 ER PT J AU Dobrescu, BA Fox, PJ AF Dobrescu, Bogdan A. Fox, Patrick J. TI Signals of a 2 TeV W' boson and a heavier Z' boson SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Gauge Symmetry ID LEFT-RIGHT SYMMETRY; ELECTROWEAK INTERACTIONS; MAJORANA NEUTRINOS; ATLAS DETECTOR; B-L; DISTRIBUTIONS; COLLISIONS; VIOLATION; SEARCH; MODEL AB We construct an SU(2)(L) x SU(2)(R) x U(l)(B-L) model with a Higgs sector that consists of a bidoublet and a doublet, and with a right-handed neutrino sector that includes one Dirac fermion and one Majorana fermion. This model explains the Run 1 CMS and ATLAS excess events in the e(+)e(-) jj, jj, Wh(0) and WZ channels in terms of a W' boson of mass near 1.9 TeV and of coupling gR in the 0.4-0.5 range, with the lower half preferred by limits on t (b) over bar resonances and Run 2 results. The production cross section of this W' boson at the 13 TeV LHC is in the 700-900 fb range, allowing sensitivity in more than 17 final states. We determine that the Z' boson has a mass in the 3.4-4.5 TeV range and several decay channels that can be probed in Run 2 of the LHC, including cascade decays via heavy Higgs bosons. C1 [Dobrescu, Bogdan A.; Fox, Patrick J.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. RP Dobrescu, BA; Fox, PJ (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM bdob@fnal.gov; pjfox@fnal.gov NR 63 TC 5 Z9 5 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 9 PY 2016 IS 5 AR 047 DI 10.1007/JHEP05(2016)047 PG 24 WC Physics, Particles & Fields SC Physics GA DM1LT UT WOS:000376107500005 ER PT J AU Weimer, MS Hu, B Kraft, SJ Gordon, RG Segre, CU Hock, AS AF Weimer, Matthew S. Hu, Bo Kraft, Steven J. Gordon, Roy G. Segre, Carlo U. Hock, Adam S. TI Synthetic and Spectroscopic Study of the Mechanism of Atomic Layer Deposition of Tin Dioxide SO ORGANOMETALLICS LA English DT Article ID 4B METAL ALKYLS; OXIDATIVE ADDITION; THIN-FILMS; COMPLEXES; SN; AMIDES; GE; STANNYLENES; REACTIVITY; PHNC(ME)CHC(ME)NPH AB This study details the surface reaction chemistry relevant to the vapor deposition mechanism of SnO2 thin films by atomic layer deposition. The mechanism was elucidated by combining different spectroscopic studies. Initial nucleation of cyclic N-2,N-3-di-tert-butylbutane-2,3-diamidotin-(II) (1) consists of surface SiOH protonation of ligands as shown by diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS). This SiO2-surface-bound stannylene was further characterized by X-ray absorption (XAS) and resonance Raman spectroscopy. XAS, DRIFTS, and Raman spectroscopy were then used to follow the further reaction of the surface-bound stannylene with different oxygen sources and a second equivalent of 1. It was observed that water does not oxidize the initial surface-bound tin site, and a well-defined, three-coordinate tin(II) species, with two surface oxygen bonds and one coordinated water molecule, was characterized. Treatment of the surface stannylene with protic oxidants such as H2O2 or tBuOOH fully oxidizes tin to 4+, and coordination of additional oxygen ligands is observed. When a second equivalent of 1 is added to surface-bound Sn4+, the resulting surface tin is also found to be in the 4+ oxidation state, contrary to the nonoxidative nucleation step. As such, surface peroxide species provide a probable growth mechanism of SnO2 through oxidation, while nucleation occurs through protic ligand exchange. C1 [Weimer, Matthew S.; Hu, Bo; Hock, Adam S.] IIT, Dept Chem, 3101 South Dearborn St, Chicago, IL 60616 USA. [Segre, Carlo U.] IIT, Dept Phys, 3101 South Dearborn St, Chicago, IL 60616 USA. [Segre, Carlo U.; Hock, Adam S.] IIT, Ctr Synchrotron Radiat Res & Instrumentat, 3101 South Dearborn St, Chicago, IL 60616 USA. [Gordon, Roy G.] Harvard Univ, Dept Chem & Chem Biol, 12 Oxford St, Cambridge, MA 02138 USA. [Hu, Bo; Kraft, Steven J.; Hock, Adam S.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. RP Hock, AS (reprint author), IIT, Dept Chem, 3101 South Dearborn St, Chicago, IL 60616 USA.; Hock, AS (reprint author), IIT, Ctr Synchrotron Radiat Res & Instrumentat, 3101 South Dearborn St, Chicago, IL 60616 USA.; Hock, AS (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Argonne, IL 60439 USA. EM ahock@iit.edu RI Segre, Carlo/B-1548-2009; Hock, Adam/D-7660-2012; BM, MRCAT/G-7576-2011 OI Segre, Carlo/0000-0001-7664-1574; Hock, Adam/0000-0003-1440-1473; FU Department of Education GAANN Fellowship [P200A090137]; Department of Energy [DE-AC02-06CH11357]; Department of Energy; Illinois Institute of Technology; MRCAT member institutions; DOE Office of Science [DE-AC02-06CH11357] FX M.S.W. acknowledges support by the Department of Education GAANN Fellowship under Grant No. P200A090137. B.H. is thankful for a Starr Fieldhouse Fellowship. S.J.K. acknowledges the Department of Energy Contract No. DE-AC02-06CH11357. A.S.H. would like to thank the Department of Energy and the Illinois Institute of Technology for funding and startup support. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The authors also thank Dr. Jeff Miller for assistance with XAS data analysis and Dr. Aditya Unni for donation of tert-butyl hydroperoxide. NR 47 TC 0 Z9 0 U1 3 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAY 9 PY 2016 VL 35 IS 9 BP 1202 EP 1208 DI 10.1021/acs.organomet.5b01004 PG 7 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA DL8JC UT WOS:000375887300005 ER PT J AU Dau, PD Rios, D Gong, Y Michelini, MC Marcalo, J Shuh, DK Mogannam, M Van Stipdonk, MJ Corcovilos, TA Martens, JK Berden, G Oomens, J Redlich, B Gibson, JK AF Dau, Phuong D. Rios, Daniel Gong, Yu Michelini, Maria C. Marcalo, Joaquim Shuh, David K. Mogannam, Mejdi Van Stipdonk, Michael J. Corcovilos, Theodore A. Martens, Jonathan K. Berden, Giel Oomens, Jos Redlich, Britta Gibson, John K. TI Synthesis and Hydrolysis of Uranyl, Neptunyl, and Plutonyl Gas Phase Complexes Exhibiting Discrete Actinide-Carbon Bonds SO ORGANOMETALLICS LA English DT Article ID QUADRUPOLE ION-TRAP; EQUATORIAL COORDINATION; INFRARED-SPECTROSCOPY; ORGANOMETALLIC IONS; OF-PLANE; REACTIVITY; DECARBOXYLATION; CHEMISTRY; CATIONS; HYDRATION AB Gas-phase organoactinyl complexes possessing discrete An-C bonds (An = U, Np, Pu) were synthesized in a quadrupole ion trap by endothermic decarboxylation of [AnO(2)(O2C-R)(3)](-) anion complexes in which a formally AnO(2)(2+) actinyl core is coordinated by three carboxylate ligands, with R = CH3 (methyl), CH3CC (1-propynyl), C6H5 (phenyl), C6F5 (pentafluorophenyl). Decarboxylation and competing ligand loss were studied computationally by density functional theory complementing experiment. Although decarboxylation was computed to be the energetically most favorable process in all cases, reduction from An(VI) to An(V) via neutral ligand loss was often prevalent, particularly for An = Np, Pu, presumably resulting from barriers associated with decarboxylation. Comparative hydrolysis rates of the An-C bonds were experimentally determined, and the chemical properties of these bonds were analyzed by the quantum theory of atoms in molecules. The measured hydrolysis rates differed by up to 3 orders of magnitude: the fastest was for [(CH3CC)UO2(O2C-CCCH3)(2)](-) and the slowest for [(C6F5)PuO2(O2C-C6F5)(2)](-). There is a general correlation between hydrolysis exothermicity and hydrolysis rate. Prototypical hydrolysis reaction pathways computed for R = CH3 (An = U, Np) reveal a mechanism in which an outer-sphere water becomes inner-sphere concomitant with transfer of an H atom to yield an OH ligand and CH4, with a net energy release of 170 kJ mol(-1) and a transition state barrier of 45 kJ mol(-1) for An = U. Infrared multiphoton dissociation spectra of selected complexes were acquired to confirm the predicted structures by agreement between the computed and observed vibrational frequencies. The experiment and theory results provide an evaluation of the comparative propensities for formation of the organoactinyls as a function of actinide and carboxylate and an assessment of the nature and stability toward hydrolysis of the primarily ionic An-C bonds. C1 [Dau, Phuong D.; Rios, Daniel; Gong, Yu; Shuh, David K.; Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Michelini, Maria C.] Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. [Marcalo, Joaquim] Univ Lisbon, Inst Super Tecn, Ctr Ciencias & Tecnol Nucl, P-2695066 Bobadela Lrs, Portugal. [Mogannam, Mejdi] Skyline Coll, San Bruno, CA 94066 USA. [Van Stipdonk, Michael J.] Duquesne Univ, Dept Chem & Biochem, Pittsburgh, PA 15282 USA. [Corcovilos, Theodore A.] Duquesne Univ, Dept Phys, Pittsburgh, PA 15282 USA. [Martens, Jonathan K.; Berden, Giel; Oomens, Jos; Redlich, Britta] Radboud Univ Nijmegen, Inst Mol & Mat, FELIX Lab, Toernooiveld 7c, NL-6525 ED Nijmegen, Netherlands. [Oomens, Jos] Univ Amsterdam, vant Hoff Inst Mol Sci, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. RP Gibson, JK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA.; Michelini, MC (reprint author), Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. EM mc.michelini@unical.it; jkgibson@lbl.gov RI Marcalo, Joaquim/J-5476-2013; Berden, Giel/F-9690-2015; OI Marcalo, Joaquim/0000-0001-7580-057X; Corcovilos, Theodore/0000-0001-5716-1188 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, Heavy Element Chemistry program, at LBNL [DE-AC02-05CH11231]; Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS), under the Science Undergraduate Laboratory Internship (SULI) program; Universita della Calabria, Italy; Fundacao para a Ciencia e a Tecnologia [UID/Multi/04349/2013]; Bayer School of Natural and Environmental Sciences; Duquesne University; Netherlands Organisation for Scientific Research (NWO) [724.011.002]; Stichting Physica; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, Heavy Element Chemistry program, at LBNL under Contract No. DE-AC02-05CH11231 (P.D.D., D.R, Y.G., D.K.S., J.K.G.) and by the Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS), under the Science Undergraduate Laboratory Internship (SULI) program (M.M.), by the Universita della Calabria, Italy (M.C.M.), by the Fundacao para a Ciencia e a Tecnologia through project UID/Multi/04349/2013 (J.M.), by start-up funds from the Bayer School of Natural and Environmental Sciences and Duquesne University (M.J.V.S., T.A.C.), and by The Netherlands Organisation for Scientific Research (NWO) under vici-grant no. 724.011.002 and the Stichting Physica (J.O.). This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 67 TC 4 Z9 4 U1 24 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAY 9 PY 2016 VL 35 IS 9 BP 1228 EP 1240 DI 10.1021/acs.organomet.6b00079 PG 13 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA DL8JC UT WOS:000375887300008 ER PT J AU Jeffries, JR Stillwell, RL Weir, ST Vohra, YK Butch, NP AF Jeffries, Jason R. Stillwell, Ryan L. Weir, Samuel T. Vohra, Yogesh K. Butch, Nicholas P. TI Emergent ferromagnetism and T-linear scattering in USb2 at high pressure SO PHYSICAL REVIEW B LA English DT Article ID RAY CIRCULAR-DICHROISM; UBI2; TEMPERATURE; PNICTIDES; ELECTRON; UAS2; UP2 AB The material USb2 is a correlated, moderately heavy-electron compound within the uranium dipnictide (UX2) series. It is antiferromagnetic with a relatively high transition temperature T-N = 204 K and a large U-U separation. While the uranium atoms in the lighter dipnictides are considered to be localized, those of USb2 exhibit hybridization and itineracy, promoting uncertainty as to the continuity of the magnetic order within the UX2. We have explored the evolution of the magnetic order by employing magnetotransport measurements as a function of pressure and temperature. We find that the TN in USb2 is enhanced, moving towards that of its smaller sibling UAs2. But, long before reaching a TN as high as UAs2, the antiferromagnetism of USb2 is abruptly destroyed in favor of another magnetic ground state. We identify this pressure-induced ground state as being ferromagnetic based on the appearance of a strong anomalous Hall effect in the transverse resistance in magnetic field. With pressure, this emergent ferromagnetic state is suppressed and ultimately destroyed in favor of a non-Fermi-liquid ground state. C1 [Jeffries, Jason R.; Stillwell, Ryan L.; Weir, Samuel T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Vohra, Yogesh K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35924 USA. [Butch, Nicholas P.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. RP Jeffries, JR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU LDRD at Lawrence Livermore National Laboratory [14-ERD-041]; US Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; DOE-NNSA [DE-NA0002014] FX We thank G. Lander, P. Soderlind, and J. Paglione for valuable comments and discussion. We are very grateful to S. K. McCall and J. R. I. Lee for their assistance with maintaining/operating the cryostat. This work was supported by LDRD (Tracking Code 14-ERD-041) at Lawrence Livermore National Laboratory. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the US Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. Y.K.V. acknowledges support from DOE-NNSA Grant No. DE-NA0002014. NR 39 TC 2 Z9 2 U1 4 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 9 PY 2016 VL 93 IS 18 AR 184406 DI 10.1103/PhysRevB.93.184406 PG 7 WC Physics, Condensed Matter SC Physics GA DL9VN UT WOS:000375991500004 ER PT J AU Sagert, I Fann, GI Fattoyev, FJ Postnikov, S Horowitz, CJ AF Sagert, I. Fann, G. I. Fattoyev, F. J. Postnikov, S. Horowitz, C. J. TI Quantum simulations of nuclei and nuclear pasta with the multiresolution adaptive numerical environment for scientific simulations SO PHYSICAL REVIEW C LA English DT Article ID NEUTRON-STAR CRUSTS; HARTREE-FOCK; MULTIWAVELET BASES; MATTER; CHEMISTRY; DENSITY; MECHANISMS; LIMITS; SHAPE; TDHF AB Background: Neutron star and supernova matter at densities just below the nuclear matter saturation density is expected to form a lattice of exotic shapes. These so-called nuclear pasta phases are caused by Coulomb frustration. Their elastic and transport properties are believed to play an important role for thermal and magnetic field evolution, rotation, and oscillation of neutron stars. Furthermore, they can impact neutrino opacities in core-collapse supernovae. Purpose: In this work, we present proof-of-principle three-dimensional (3D) Skyrme Hartree-Fock (SHF) simulations of nuclear pasta with the Multi-resolution ADaptive Numerical Environment for Scientific Simulations (MADNESS). Methods: We perform benchmark studies of O-16, Pb-208, and U-238 nuclear ground states and calculate binding energies via 3D SHF simulations. Results are compared with experimentally measured binding energies as well as with theoretically predicted values from an established SHF code. The nuclear pasta simulation is initialized in the so-called waffle geometry as obtained by the Indiana University Molecular Dynamics (IUMD) code. The size of the unit cell is 24 fm with an average density of about rho = 0.05fm(-3), proton fraction of Y-p = 0.3, and temperature of T = 0 MeV. Results: Our calculations reproduce the binding energies and shapes of light and heavy nuclei with different geometries. For the pasta simulation, we find that the final geometry is very similar to the initial waffle state. We compare calculations with and without spin-orbit forces. We find that while subtle differences are present, the pasta phase remains in the waffle geometry. Conclusions: Within the MADNESS framework, we can successfully perform calculations of inhomogeneous nuclear matter. By using pasta configurations from IUMD it is possible to explore different geometries and test the impact of self-consistent calculations on the latter. C1 [Sagert, I.; Fattoyev, F. J.; Postnikov, S.; Horowitz, C. J.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47405 USA. [Sagert, I.; Fattoyev, F. J.; Postnikov, S.; Horowitz, C. J.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Fann, G. I.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Sagert, I (reprint author), Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47405 USA.; Sagert, I (reprint author), Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. FU Lilly Endowment, Inc.; Indiana METACyt Initiative; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; DOE [DE-FG02-87ER40365, DE-SC0008808] FX The authors thank M. Caplan for providing data from simulations with the Indiana University Molecular Dynamics (IUMD) code and Bastian Schuetrumpf for his assistance with the Molecular Dynamics simulation initialization for the Sky3D code. This work was supported in part by the Lilly Endowment, Inc., through its support for the Indiana University Pervasive Technology Institute and in part by the Indiana METACyt Initiative. The Indiana METACyt Initiative at IU is also supported in part by the Lilly Endowment, Inc. This research used resources of the Oak Ridge Leadership Computing Facility at ORNL, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. This work was also supported by DOE Grants No. DE-FG02-87ER40365 (Indiana University) and No. DE-SC0008808 (NUCLEI SciDAC Collaboration). NR 59 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 9 PY 2016 VL 93 IS 5 AR 055801 DI 10.1103/PhysRevC.93.055801 PG 17 WC Physics, Nuclear SC Physics GA DL9XX UT WOS:000375997800005 ER PT J AU Offermann, DT Welch, DR Rose, DV Thoma, C Clark, RE Mostrom, CB Schmidt, AEW Link, AJ AF Offermann, Dustin T. Welch, Dale R. Rose, Dave V. Thoma, Carsten Clark, Robert E. Mostrom, Chris B. Schmidt, Andrea E. W. Link, Anthony J. TI Transition from Beam-Target to Thermonuclear Fusion in High-Current Deuterium Z-Pinch Simulations SO PHYSICAL REVIEW LETTERS LA English DT Article ID PLASMA-FOCUS AB Fusion yields from dense, Z-pinch plasmas are known to scale with the drive current, which is favorable for many potential applications. Decades of experimental studies, however, show an unexplained drop in yield for currents above a few mega-ampere (MA). In this work, simulations of DD Z-Pinch plasmas have been performed in 1D and 2D for a constant pinch time and initial radius using the code LSP, and observations of a shift in scaling are presented. The results show that yields below 3 MA are enhanced relative to pure thermonuclear scaling by beamlike particles accelerated in the Rayleigh-Taylor induced electric fields, while yields above 3 MA are reduced because of energy lost by the instability and the inability of the beamlike ions to enter the pinch region. C1 [Offermann, Dustin T.; Welch, Dale R.; Rose, Dave V.; Thoma, Carsten; Clark, Robert E.; Mostrom, Chris B.] Voss Sci LLC, Albuquerque, NM 87108 USA. [Schmidt, Andrea E. W.; Link, Anthony J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Offermann, DT (reprint author), Voss Sci LLC, Albuquerque, NM 87108 USA. EM dustino@vosssci.com OI Offermann, Dustin/0000-0002-6033-4905 FU Defense Advanced Research Projects Agency (DARPA) FX The authors would like to acknowledge Dr. Radu Presura and Peggy Voss of Voss Scientific for their comments. Thanks are also given to Dr. Nicki Bennett of National Security Technologies (NSTec) for her review. This research was developed with funding from the Defense Advanced Research Projects Agency (DARPA). The views, opinions, and/or findings contained in this article are those of the authors and should not be interpreted as representing the official views or policies of the Department of Defense or the U.S. Government. NR 23 TC 1 Z9 1 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 9 PY 2016 VL 116 IS 19 AR 195001 DI 10.1103/PhysRevLett.116.195001 PG 5 WC Physics, Multidisciplinary SC Physics GA DM0CW UT WOS:000376011400004 PM 27232025 ER PT J AU Verbanis, E Martin, A Rosset, D Lim, CCW Thew, RT Zbinden, H AF Verbanis, E. Martin, A. Rosset, D. Lim, C. C. W. Thew, R. T. Zbinden, H. TI Resource-Efficient Measurement-Device-Independent Entanglement Witness SO PHYSICAL REVIEW LETTERS LA English DT Article ID ATOMIC ENSEMBLES; QUANTUM AB Imperfections in experimental measurement schemes can lead to falsely identifying, or over estimating, entanglement in a quantum system. A recent solution to this is to define schemes that are robust to measurement imperfections-measurement-device-independent entanglement witness (MDI-EW). This approach can be adapted to witness all entangled qubit states for a wide range of physical systems and does not depend on detection efficiencies or classical communication between devices. Here we extend the theory to remove the necessity of prior knowledge about the two-qubit states to be witnessed. Moreover, we tested this model via a novel experimental implementation for MDI-EW that significantly reduces the experimental complexity. By applying it to a bipartite Werner state, we demonstrate the robustness of this approach against noise by witnessing entanglement down to an entangled state fraction close to 0.4. C1 [Verbanis, E.; Martin, A.; Rosset, D.; Lim, C. C. W.; Thew, R. T.; Zbinden, H.] Univ Geneva, Grp Appl Phys, CH-1211 Geneva, Switzerland. [Lim, C. C. W.] Oak Ridge Natl Lab, Computat Sci & Engn Div, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. RP Thew, RT (reprint author), Univ Geneva, Grp Appl Phys, CH-1211 Geneva, Switzerland. EM robert.thew@unige.ch RI Thew, Robert/B-2407-2009; OI Thew, Robert/0000-0003-0188-6053; Lim, Charles Ci Wen/0000-0002-2332-4126 FU Swiss National Sciences Foundation [200021-159592]; Oak Ridge National Laboratory directed research and development program FX The authors would like to thank Natalia Bruno, Flavien Hirsch, Nicolas Brunner, and Nicolas Gisin for discussions. This work was supported by the Swiss National Sciences Foundation Project No. 200021-159592. C. C. W. Lim acknowledges support from the Oak Ridge National Laboratory directed research and development program. NR 31 TC 2 Z9 2 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 9 PY 2016 VL 116 IS 19 AR 190501 DI 10.1103/PhysRevLett.116.190501 PG 5 WC Physics, Multidisciplinary SC Physics GA DM0CW UT WOS:000376011400001 PM 27232009 ER PT J AU Hurley, JH AF Hurley, James H. TI Editorial Overview: Molecular Mechanisms of Autophagy-Part A SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Editorial Material C1 [Hurley, James H.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Hurley, James H.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Hurley, James H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. RP Hurley, JH (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Hurley, JH (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Hurley, JH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. EM jimhurley@berkeley.edu NR 8 TC 0 Z9 0 U1 1 U2 1 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD MAY 8 PY 2016 VL 428 IS 9 BP 1657 EP 1658 PN A PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DM9OG UT WOS:000376695000001 PM 27037195 ER PT J AU Langan, PS Close, DW Coates, L Rocha, RC Ghosh, K Kiss, C Waldo, G Freyer, J Kovalevsky, A Bradbury, ARM AF Langan, Patricia S. Close, Devin W. Coates, Leighton Rocha, Reginaldo C. Ghosh, Koushik Kiss, Csaba Waldo, Geoff Freyer, James Kovalevsky, Andrey Bradbury, Andrew R. M. TI Evolution and characterization of a new reversibly photoswitching chromogenic protein, Dathail SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE chromoprotein; photoswitchable; pcFRET; neutron crystallography; ensemble refinement ID GREEN FLUORESCENT PROTEIN; CHROMOPHORE ISOMERIZATION; NEUTRON CRYSTALLOGRAPHY; PROTON-TRANSFER; NMR SYSTEM; GFP; DRONPA; PHOTOACTIVATION; CHROMOPROTEINS; CHEMISTRY AB We report the engineering of a new reversibly switching chromogenic protein, Dathail. Dathail was evolved from the extremely thermostable fluorescent proteins thermal green protein (TGP) and eCGP123 using directed evolution and ratiometric sorting. Dathail has two spectrally distinct chromogenic states with low quantum yields, corresponding to absorbance in a ground state with a maximum at 389 nm, and a photo-induced metastable state with a maximum at 497 nm. In contrast to all previously described photoswitchable proteins, both spectral states of Dathail are non-fluorescent. The photo-induced chromogenic state of Dathail has a lifetime of similar to 50 min at 293 K and pH 7.5 as measured by UV-Vis spectrophotometry, returning to the ground state through thermal relaxation. X-ray crystallography provided structural insights supporting a change in conformation and coordination in the chromophore pocket as being responsible for Dathail's photoswitching. Neutron crystallography, carried out for the first time on a protein from the green fluorescent protein family, showed a distribution of hydrogen atoms revealing protonation of the chromophore 4-hydroxybenzyl group in the ground state. The neutron structure also supports the hypothesis that the photo-induced proton transfer from the chromophore occurs through water-mediated proton relay into the bulk solvent. Beyond its spectroscopic curiosity, Dathail has several characteristics that are improvements for applications, including low background fluorescence, large spectral separation, rapid switching time, and the ability to switch many times. Therefore, Dathail is likely to be extremely useful in the quickly developing fields of imaging and biosensors, including photochromic Forster resonance energy transfer, high-resolution microscopy, and live tracking within the cell. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Langan, Patricia S.; Close, Devin W.; Kiss, Csaba; Waldo, Geoff; Bradbury, Andrew R. M.] Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. [Close, Devin W.; Rocha, Reginaldo C.; Ghosh, Koushik] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. [Close, Devin W.] ARUP Labs Inst Clin & Expt Pathol, Salt Lake City, UT USA. [Coates, Leighton; Kovalevsky, Andrey] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Freyer, James] Univ New Mexico, Ctr Biomed Engn, Albuquerque, NM 87131 USA. [Langan, Patricia S.] Univ New Mexico, Nanosci & Microsyst Engn, Albuquerque, NM 87131 USA. RP Bradbury, ARM (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. EM amb@lanl.gov OI Coates, Leighton/0000-0003-2342-049X; Kovalevsky, Andrey/0000-0003-4459-9142; Bradbury, Andrew/0000-0002-5567-8172; Langan, Patricia/0000-0002-1097-5958 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Biological and Environmental Research FX This research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The Office of Biological and Environmental Research supported research at Oak Ridge National Laboratory's Center for Structural Molecular Biology, using facilities supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 56 TC 2 Z9 2 U1 7 U2 18 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD MAY 8 PY 2016 VL 428 IS 9 BP 1776 EP 1789 DI 10.1016/j.jmb.2016.02.029 PN A PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DM9OG UT WOS:000376695000009 PM 27000644 ER PT J AU Luo, CT Wang, YJ Ge, WW Li, JF Viehland, D Delaire, O Li, XB Luo, HS AF Luo, Chengtao Wang, Yaojin Ge, Wenwei Li, Jiefang Viehland, Dwight Delaire, Olivier Li, Xiaobin Luo, Haosu TI Hierarchical domain structure of lead-free piezoelectric (Na-1/2 Bi-1/2)TiO3-(K-1/2 Bi-1/2)TiO3 single crystals SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FREE PIEZOCERAMICS; SOLID-SOLUTION; CERAMICS; SYSTEMS; BOUNDARY; STRAIN; GROWTH; PHASE AB We report a unique hierarchical domain structure in single crystals of (Na1/2Bi1/2)TiO3-xat. % (K1/2Bi1/2)TiO3 for x = 5 and 8 by transmission electron microscopy (TEM). A high density of polar nano-domains with a lamellar morphology was found, which were self-assembled into a quadrant-like configuration, which then assembled into conventional ferroelectric macro-domains. Studies by high resolution TEM revealed that the polar lamellar regions contained a coexistence of in-phase and anti-phase oxygen octahedral tilt regions of a few nanometers in size. Domain frustration over multiple length scales may play an important role in the stabilization of the hierarchy, and in reducing the piezoelectric response of this Pb-free piezoelectric solid solution. Published by AIP Publishing. C1 [Luo, Chengtao; Wang, Yaojin; Ge, Wenwei; Li, Jiefang; Viehland, Dwight] Virginia Tech, Mat Sci & Engn, Blacksburg, VA 24061 USA. [Delaire, Olivier] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Li, Xiaobin; Luo, Haosu] Chinese Acad Sci, Shanghai Inst Ceram, 215 Chengbei Rd, Shanghai 201800, Peoples R China. RP Luo, CT (reprint author), Virginia Tech, Mat Sci & Engn, Blacksburg, VA 24061 USA. EM lchentao@vt.edu RI Wang, Yaojin/F-3748-2012 OI Wang, Yaojin/0000-0003-2561-1855 FU ONRL-GO; Office of Naval Research [N00014-13-1-0049]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX Authors C.L., D.V., and O.D. would like to thank the ONRL-GO program for support of this work, and Y.W. and J.F.L. would like to thank the Office of Naval Research for support of this work (N00014-13-1-0049). The authors also thank Dr. C. Winkler for useful discussion and the Nanoscale Characterization and Fabrication Laboratory in Virginia Tech for the instrumentation support and training. O.D. acknowledges funding from the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. DOE. NR 46 TC 0 Z9 0 U1 20 U2 27 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAY 7 PY 2016 VL 119 IS 17 AR 174102 DI 10.1063/1.4948478 PG 6 WC Physics, Applied SC Physics GA DO3XS UT WOS:000377716500012 ER PT J AU Aschaffenburg, DJ Williams, MRC Schmuttenmaer, CA AF Aschaffenburg, Daniel J. Williams, Michael R. C. Schmuttenmaer, Charles A. TI Terahertz spectroscopic polarimetry of generalized anisotropic media composed of Archimedean spiral arrays: Experiments and simulations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID OPTICAL-ACTIVITY; DOMAIN; METAMATERIALS; RESONATORS AB Terahertz time-domain spectroscopic polarimetry has been used to measure the polarization state of all spectral components in a broadband THz pulse upon transmission through generalized anisotropic media consisting of two-dimensional arrays of lithographically defined Archimedean spirals. The technique allows a full determination of the frequency-dependent, complex-valued transmission matrix and eigenpolarizations of the spiral arrays. Measurements were made on a series of spiral array orientations. The frequency-dependent transmission matrix elements as well as the eigenpolarizations were determined, and the eigenpolarizations were found be to elliptically corotating, as expected from their symmetry. Numerical simulations are in quantitative agreement with measured spectra. Published by AIP Publishing. C1 [Aschaffenburg, Daniel J.; Williams, Michael R. C.; Schmuttenmaer, Charles A.] Yale Univ, Dept Chem, 225 Prospect St,POB 208107, New Haven, CT 06520 USA. [Aschaffenburg, Daniel J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Williams, Michael R. C.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. RP Schmuttenmaer, CA (reprint author), Yale Univ, Dept Chem, 225 Prospect St,POB 208107, New Haven, CT 06520 USA. EM charles.schmuttenmaer@yale.edu FU National Science Foundation [CHE- 1465085] FX We acknowledge the National Science Foundation ( Grant No. CHE- 1465085) for partial support of this work. The authors thank Mikhael Guy, Daniel F. Santavicca, and Daniel E. Prober for technical assistance and helpful discussions. This work was supported in part by the facilities and staff of the Yale University Faculty of Arts and Sciences Science Research Software Core. NR 48 TC 0 Z9 0 U1 2 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174705 DI 10.1063/1.4947469 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300031 PM 27155645 ER PT J AU de Oliveira, TE Netz, PA Kremer, K Junghans, C Mukherji, D AF de Oliveira, Tiago E. Netz, Paulo A. Kremer, Kurt Junghans, Christoph Mukherji, Debashish TI C-IBI: Targeting cumulative coordination within an iterative protocol to derive coarse-grained models of (multi-component) complex fluids SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS; POLYMER MELTS; AQUEOUS UREA; FORCE-FIELD; SIMULATION; POTENTIALS; WATER; TRANSFERABILITY AB We present a coarse-graining strategy that we test for aqueous mixtures. The method uses pair-wise cumulative coordination as a target function within an iterative Boltzmann inversion (IBI) like protocol. We name this method coordination iterative Boltzmann inversion (C-IBI). While the underlying coarse-grained model is still structure based and, thus, preserves pair-wise solution structure, our method also reproduces solvation thermodynamics of binary and/or ternary mixtures. Additionally, we observe much faster convergence within C-IBI compared to IBI. To validate the robustness, we apply C-IBI to study test cases of solvation thermodynamics of aqueous urea and a triglycine solvation in aqueous urea. Published by AIP Publishing. C1 [de Oliveira, Tiago E.; Netz, Paulo A.; Kremer, Kurt; Mukherji, Debashish] Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany. [de Oliveira, Tiago E.; Netz, Paulo A.] Univ Fed Rio Grande do Sul, Porto Alegre, RS, Brazil. [Junghans, Christoph] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, POB 1663, Los Alamos, NM 87545 USA. RP Mukherji, D (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany.; Junghans, C (reprint author), Los Alamos Natl Lab, Comp Computat & Stat Sci Div, POB 1663, Los Alamos, NM 87545 USA. EM junghans@lanl.gov; mukherji@mpip-mainz.mpg.de RI Junghans, Christoph/G-4238-2010; Kremer, Kurt/G-5652-2011; MPIP, Theory/I-9884-2014 OI Junghans, Christoph/0000-0003-0925-1458; FU CNPq from Brazilian Government; CAPES from Brazilian Government; LANL; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396] FX We thank Christine Peter and Nico van der Vegt for stimulating discussions. T. E. O. and P. A. N. acknowledges financial support from CNPq and CAPES from Brazilian Government and hospitality at the Max-Planck Institut fur Polymerforschung, where this work was performed and generous allocation of computational facilities at the supercomputing center of CESUP-UFRGS. C. J. thanks LANL for a Director's fellowship. Assigned: LA-UR-15-28326. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract No. DE-AC52-06NA25396. We thank Robinson Cortes-Huerto, Tanja Kling, Tristan Bereau, and Torsten Stuhn for critical reading of the manuscript. Simulation snapshots in this manuscript are rendered using VMD.41 NR 41 TC 1 Z9 1 U1 2 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174106 DI 10.1063/1.4947253 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300010 PM 27155624 ER PT J AU Kulakhmetov, M Gallis, M Alexeenko, A AF Kulakhmetov, Marat Gallis, Michael Alexeenko, Alina TI Ab initio-informed maximum entropy modeling of rovibrational relaxation and state-specific dissociation with application to the O-2 + O system SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CLASSICAL TRAJECTORY CALCULATIONS; DIRECT SIMULATION; THERMOCHEMICAL NONEQUILIBRIUM; VIBRATION-DISSOCIATION; SHOCK-WAVES; ENERGY; NITROGEN; COLLISIONS; SURFACE; OZONE AB Quasi-classical trajectory (QCT) calculations are used to study state-specific ro-vibrational energy exchange and dissociation in the O-2 + O system. Atom-diatom collisions with energy between 0.1 and 20 eV are calculated with a double many body expansion potential energy surface by Varandas and Pais [Mol. Phys. 65, 843 (1988)]. Inelastic collisions favor mono-quantum vibrational transitions at translational energies above 1.3 eV although multi-quantum transitions are also important. Post-collision vibrational favoring decreases first exponentially and then linearly as Delta v increases. Vibrationally elastic collisions (Delta v = 0) favor small Delta J transitions while vibrationally inelastic collisions have equilibrium post-collision rotational distributions. Dissociation exhibits both vibrational and rotational favoring. New vibrational-translational (VT), vibrational-rotational-translational (VRT) energy exchange, and dissociation models are developed based on QCT observations and maximum entropy considerations. Full set of parameters for state-to-state modeling of oxygen is presented. The VT energy exchange model describes 22 000 state-to-state vibrational cross sections using 11 parameters and reproduces vibrational relaxation rates within 30% in the 2500-20 000 K temperature range. The VRT model captures 80 x 10(6) state-to-state ro-vibrational cross sections using 19 parameters and reproduces vibrational relaxation rates within 60% in the 5000-15 000 K temperature range. The developed dissociation model reproduces state-specific and equilibrium dissociation rates within 25% using just 48 parameters. The maximum entropy framework makes it feasible to upscale ab initio simulation to full nonequilibrium flow calculations. Published by AIP Publishing. C1 [Kulakhmetov, Marat; Alexeenko, Alina] Purdue Univ, Aeronaut & Astronaut, W Lafayette, IN 47907 USA. [Gallis, Michael] Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. RP Kulakhmetov, M; Alexeenko, A (reprint author), Purdue Univ, Aeronaut & Astronaut, W Lafayette, IN 47907 USA.; Gallis, M (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM mkulakhm@purdue.edu; magalli@sandia.gov; alexeenk@purdue.edu OI Gallis, Michael/0000-0002-4985-6956; Alexeenko, Alina/0000-0003-2123-9064 FU Sandia National Laboratory through the Sandia Excellence in Science and Engineering Research Fellowship FX This work has been supported by Sandia National Laboratory through the Sandia Excellence in Science and Engineering Research Fellowship. In particular, we would like to acknowledge Dr. Dan Rader at Sandia. We would also like to thank Professor Antonio Varandas at University of Coimbra for providing an O3 potential energy surface. NR 50 TC 4 Z9 4 U1 2 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174302 DI 10.1063/1.4947590 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300021 PM 27155635 ER PT J AU Leiding, J Coe, JD AF Leiding, Jeff Coe, Joshua D. TI Reactive Monte Carlo sampling with an ab initio potential SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CHEMICAL-REACTION EQUILIBRIA; DENSITY-FUNCTIONAL THEORY; TOTAL-ENERGY CALCULATIONS; REACTION ENSEMBLE METHOD; VAPOR-LIQUID INTERFACES; WAVE BASIS-SET; PHASE-EQUILIBRIA; 1ST PRINCIPLES; MOLECULAR-DYNAMICS; CARBON MICROPORES AB We present the first application of reactive Monte Carlo in a first-principles context. The algorithm samples in a modified NVT ensemble in which the volume, temperature, and total number of atoms of a given type are held fixed, but molecular composition is allowed to evolve through stochastic variation of chemical connectivity. We discuss general features of the method, as well as techniques needed to enhance the efficiency of Boltzmann sampling. Finally, we compare the results of simulation of NH3 to those of ab initio molecular dynamics (AIMD). We find that there are regions of state space for which RxMC sampling is much more efficient than AIMD due to the "rare-event" character of chemical reactions. Published by AIP Publishing. C1 [Leiding, Jeff; Coe, Joshua D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Leiding, J; Coe, JD (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jal@lanl.gov; jcoe@lanl.gov FU Advanced Simulation and Computing (ASC) program; NNSA of the U.S. DOE [DE-AC52-06NA25396] FX We thank the Advanced Simulation and Computing (ASC) program for funding. LANL is operated by Los Alamos National Security, LLC, for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. This manuscript is designated LA-UR-16-21006. NR 86 TC 0 Z9 0 U1 1 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174109 DI 10.1063/1.4948303 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300013 PM 27155627 ER PT J AU Mann, GW Lee, K Cococcioni, M Smit, B Neaton, JB AF Mann, Gregory W. Lee, Kyuho Cococcioni, Matteo Smit, Berend Neaton, Jeffrey B. TI First-principles Hubbard U approach for small molecule binding in metal-organic frameworks SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; IRON(II) COORDINATION SITES; CARBON-DIOXIDE; ELECTRONIC-STRUCTURE; CO2 ADSORPTION; LDA+U METHOD; CAPTURE; INSULATORS; SPECTRA; ENERGY AB We apply first-principles approaches with Hubbard U corrections for calculation of small molecule binding energetics to open-shell transition metal atoms in metal-organic frameworks (MOFs). Using density functional theory with van derWaals dispersion-corrected functionals, we determine Hubbard U values ab initio through an established linear response procedure for M-MOF-74, for a number of different metal centers (M = Ti, V, Cr, Mn, Fe, Co, Ni, and Cu). While our ab initio U values differ from those used in previous work, we show that they result in lattice parameters and electronic contributions to CO2-MOF binding energies that lead to excellent agreement with experiments and previous results, yielding lattice parameters within 3%. In addition, U-dependent calculations for an example system, Co-MOF-74, suggest that the CO2 binding energy grows monotonically with the value of Hubbard U, with the binding energy shifting 4 kJ/mol (or 0.041 eV) over the range of U = 0-5.4 eV. These results provide insight into an approximate but computationally efficient means for calculation of small molecule binding energies to open-shell transition metal atoms in MOFs and suggest that the approach can be predictive with good accuracy, independent of the cations used and the availability of experimental data. Published by AIP Publishing. C1 [Mann, Gregory W.; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mann, Gregory W.] Mesosphere Inc, San Francisco, CA 94105 USA. [Lee, Kyuho; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Lee, Kyuho; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Lee, Kyuho] Synopsys Inc, Mountain View, CA 94043 USA. [Cococcioni, Matteo] Ecole Polytech Fed Lausanne, Theory & Simulat Mat THEOS, Lausanne, Switzerland. [Smit, Berend] Valais Ecole Polytech Fed Lausanne EPFL, Lab Mol Simulat, Inst Sci & Ingn Chim, Rue Ind 17, CH-1951 Sion, Switzerland. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Mann, GW; Smit, B (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Mann, GW (reprint author), Mesosphere Inc, San Francisco, CA 94105 USA.; Lee, K; Smit, B (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Lee, K; Neaton, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Lee, K (reprint author), Synopsys Inc, Mountain View, CA 94043 USA.; Cococcioni, M (reprint author), Ecole Polytech Fed Lausanne, Theory & Simulat Mat THEOS, Lausanne, Switzerland.; Smit, B (reprint author), Valais Ecole Polytech Fed Lausanne EPFL, Lab Mol Simulat, Inst Sci & Ingn Chim, Rue Ind 17, CH-1951 Sion, Switzerland.; Neaton, JB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Neaton, JB (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. EM gmann@berkeley.edu; kyuholee@lbl.gov; matteo.cococcioni@epfl.ch; Berend-Smit@berkeley.edu; jbneaton@lbl.gov RI Smit, Berend/B-7580-2009 OI Smit, Berend/0000-0003-4653-8562 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Center of Competence in Research (NCCR) Materials' Revolution: Computational Design and Discovery of Novel Materials (MARVEL) of the Swiss National Science Foundation (SNSF) FX Funding for this work was provided by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the DOE, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001015. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B. S. is partially supported by the National Center of Competence in Research (NCCR) Materials' Revolution: Computational Design and Discovery of Novel Materials (MARVEL) of the Swiss National Science Foundation (SNSF). NR 58 TC 1 Z9 1 U1 15 U2 49 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174104 DI 10.1063/1.4947240 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300008 PM 27155622 ER PT J AU Santana, JA Krogel, JT Kent, PRC Reboredo, FA AF Santana, Juan A. Krogel, Jaron T. Kent, Paul R. C. Reboredo, Fernando A. TI Cohesive energy and structural parameters of binary oxides of groups IIA and IIIB from diffusion quantum Monte Carlo SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; COUPLED-CLUSTER METHOD; CRYSTAL-STRUCTURE; HIGH-PRESSURE; TRANSITION; PSEUDOPOTENTIALS; SYSTEMS; SIMULATIONS; SOLIDS; ATOMS AB We have applied the diffusion quantum Monte Carlo (DMC) method to calculate the cohesive energy and the structural parameters of the binary oxides CaO, SrO, BaO, Sc2O3, Y2O3, and La2O3. The aim of our calculations is to systematically quantify the accuracy of the DMC method to study this type of metal oxides. The DMC results were compared with local, semi-local, and hybrid Density Functional Theory (DFT) approximations as well as with experimental measurements. The DMC method yields cohesive energies for these oxides with a mean absolute deviation from experimental measurements of 0.18(2) eV, while with local, semi-local, and hybrid DFT approximations, the deviation is 3.06, 0.94, and 1.23 eV, respectively. For lattice constants, the mean absolute deviations in DMC, local, semi-local, and hybrid DFT approximations are 0.017(1), 0.07, 0.05, and 0.04 angstrom, respectively. DMC is a highly accurate method, outperforming the DFT approximations in describing the cohesive energies and structural parameters of these binary oxides. Published by AIP Publishing. C1 [Santana, Juan A.; Krogel, Jaron T.; Reboredo, Fernando A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Santana, Juan A.] Univ Puerto Rico, Dept Chem, POB 372230, Cayey, PR 00737 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Reboredo, FA (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM reboredofa@ornl.gov RI Kent, Paul/A-6756-2008; OI Kent, Paul/0000-0001-5539-4017; Santana, Juan A./0000-0003-2349-6312; Krogel, Jaron/0000-0002-1859-181X FU Materials Sciences & Engineering Division of the Office of Basic Energy Sciences, U.S. Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX The work was supported by the Materials Sciences & Engineering Division of the Office of Basic Energy Sciences, U.S. Department of Energy. Paul R. C. Kent was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Computational resources were provided by the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 72 TC 1 Z9 1 U1 3 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAY 7 PY 2016 VL 144 IS 17 AR 174707 DI 10.1063/1.4947569 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DO3VV UT WOS:000377711300033 PM 27155647 ER PT J AU Allendorf, MD AF Allendorf, Mark D. TI A framework for success SO NATURE ENERGY LA English DT Editorial Material ID OXYGEN REDUCTION AB Oxygen reduction at the cathode of fuel cells typically requires a platinum-based material to catalyse the reaction, but lower-cost, more stable catalysts are sought. Now, an intrinsically conductive metal-organic framework based on cheaper elements is shown to be a durable, structurally well-defined catalyst for this reaction. C1 [Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Allendorf, MD (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM mdallen@sandia.gov NR 7 TC 1 Z9 1 U1 5 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2058-7546 J9 NAT ENERGY JI Nat. Energy PD MAY 6 PY 2016 VL 1 AR 16058 DI 10.1038/NENERGY.2016.58 PG 2 WC Energy & Fuels; Materials Science, Multidisciplinary SC Energy & Fuels; Materials Science GA EK7TB UT WOS:000394127000002 ER PT J AU Stern, PC Janda, KB Brown, MA Steg, L Vine, EL Lutzenhiser, L AF Stern, Paul C. Janda, Kathryn B. Brown, Marilyn A. Steg, Linda Vine, Edward L. Lutzenhiser, Loren TI Opportunities and insights for reducing fossil fuel consumption by households and organizations SO NATURE ENERGY LA English DT Review ID ENERGY EFFICIENCY; BUILDING COMMUNITIES; SOCIAL-INFLUENCE; RESEARCH AGENDA; CONSERVATION; INCENTIVES; BARRIERS; MARKET AB Realizing the ambitious commitments of the 2015 Paris Climate Conference (COP21) will require new ways of meeting human needs previously met by burning fossil fuels. Technological developments will be critical, but so will accelerated adoption of promising low-emission technologies and practices. National commitments will be more achievable if interventions take into account key psychological, social, cultural and organizational factors that influence energy choices, along with factors of an infrastructural, technical and economic nature. Broader engagement of social and behavioural science is needed to identify promising opportunities for reducing fossil fuel consumption. Here we discuss opportunities for change in households and organizations, primarily at short and intermediate timescales, and identify opportunities that have been underused in much of energy policy. Based on this survey, we suggest design principles for interventions by governments and other organizations, and identify areas of emphasis for future social science and interdisciplinary research. C1 [Stern, Paul C.] Natl Acad Sci, 500 Fifth St NW, Washington, DC 20001 USA. [Stern, Paul C.] Natl Acad Engn, 500 Fifth St NW, Washington, DC 20001 USA. [Stern, Paul C.] Natl Acad Med, 500 Fifth St NW, Washington, DC 20001 USA. [Stern, Paul C.] Norwegian Univ Sci & Technol, Hgsk Ringen 1, N-7491 Trondheim, Norway. [Stern, Paul C.] Social & Environm Res Inst, POB 1487, Northampton, MA 01060 USA. [Janda, Kathryn B.] Univ Oxford, Environm Change Inst, South Parks Rd, Oxford OX1 3QY, England. [Brown, Marilyn A.] Georgia Inst Technol, Sch Publ Policy, 685 Cherry St, Atlanta, GA 30332 USA. [Steg, Linda] Univ Groningen, Fac Social & Behav Sci, Grote Kruisstr 2-1, NL-9712 TS Groningen, Netherlands. [Vine, Edward L.] Lawrence Berkeley Natl Lab, Bldg 90-2128, Berkeley, CA 94720 USA. [Lutzenhiser, Loren] Portland State Univ, Toulan Sch Urban Studies & Planning, Portland, OR 97207 USA. RP Stern, PC (reprint author), Natl Acad Sci, 500 Fifth St NW, Washington, DC 20001 USA.; Stern, PC (reprint author), Natl Acad Engn, 500 Fifth St NW, Washington, DC 20001 USA.; Stern, PC (reprint author), Natl Acad Med, 500 Fifth St NW, Washington, DC 20001 USA.; Stern, PC (reprint author), Norwegian Univ Sci & Technol, Hgsk Ringen 1, N-7491 Trondheim, Norway.; Stern, PC (reprint author), Social & Environm Res Inst, POB 1487, Northampton, MA 01060 USA. EM pstern@nas.edu RI Steg, Linda/H-6878-2014 OI Steg, Linda/0000-0002-8375-9607 FU UK Engineering and Physical Sciences Research Council grant [EP/L024557/1] FX The views expressed in this paper are those of the authors and not of the US National Academies of Sciences, Engineering, and Medicine, nor of the UK Engineering and Physical Sciences Research Council. Portions of this work have been supported by UK Engineering and Physical Sciences Research Council grant EP/L024557/1. NR 90 TC 5 Z9 5 U1 4 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2058-7546 J9 NAT ENERGY JI Nat. Energy PD MAY 6 PY 2016 VL 1 AR 16043 DI 10.1038/NENERGY.2016.43 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary SC Energy & Fuels; Materials Science GA EK7RU UT WOS:000394123700001 ER PT J AU Li, H Bi, XX Bai, Y Yuan, YF Shahbazian-Yassar, R Wu, C Wu, F Lu, J Amine, K AF Li, Hui Bi, Xuanxuan Bai, Ying Yuan, Yifei Shahbazian-Yassar, Reza Wu, Chuan Wu, Feng Lu, Jun Amine, Khalil TI High-Rate, Durable Sodium-Ion Battery Cathode Enabled by Carbon-Coated Micro-Sized Na3V2(PO4)(3) Particles with Interconnected Vertical Nanowalls SO ADVANCED MATERIALS INTERFACES LA English DT Article ID ELECTROCHEMICAL PERFORMANCE; ENERGY-STORAGE; ELECTRODE MATERIAL; RATE CAPABILITY; NATI2(PO4)(3); NANOFIBERS; NANOSHEETS; FRAMEWORK; MATRIX; ANODE AB Na-ion batteries have been regarded as promising alternatives for Li-ion batteries due to the extensive sodium reserves in the world. Na3V2(PO4)(3) has been proved to be a good candidate of the cathode materials in Na-ion batteries but the intrinsic low electrical conductivity and sluggish kinetics handicapped its application. Here, 3D hierarchical Na3V2(PO4)(3) particles are synthesized by a facile hydrothermal method, constructed by carbon-coated 2D Na3V2(PO4)(3) nanowalls. Superior cell performance of high rate capability and cycle stability are observed in the well-defined structure. As the cathode in Na-ion batteries, it delivers a high capacity almost reaching the theoretical one and exhibits high capacity retention. The enhanced rate capability and cycle performance can be attributed to the improved electrical conductivity from the interconnected carbon layer and the shortened ion diffusion length and high specific surface area from the nanowalls. C1 [Li, Hui; Bai, Ying; Wu, Chuan; Wu, Feng] Beijing Inst Technol, Sch Mat Sci & Engn, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. [Bi, Xuanxuan; Yuan, Yifei; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. [Wu, Chuan; Wu, Feng] Collaborat Innovat Ctr Elect Vehicles Beijing, Beijing 100081, Peoples R China. [Yuan, Yifei; Shahbazian-Yassar, Reza] Michigan Technol Univ, Dept Mat Sci & Engn, 1400 Townsend Dr, Houghton, MI 49931 USA. RP Bai, Y (reprint author), Beijing Inst Technol, Sch Mat Sci & Engn, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. EM membrane@bit.edu.cn; junlu@anl.gov RI wu, chuan/A-1447-2009 FU National Key Program for Basic Research of China [2015CB251100]; Program for New Century Excellent Talents in University [NCET-12-0047]; U.S. Department of Energy under Vehicle Technologies Office, Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE) [DE-AC0206CH11357]; State Scholarship Fund of the China Scholarship Council [201406035025]; National Science Foundation [CMMI-1200383]; Argonne National Laboratory [4F31422] FX H.L. and X.B. contributed equally to this work. This research was supported by the National Key Program for Basic Research of China through Grant 2015CB251100 and the Program for New Century Excellent Talents in University through Grant NCET-12-0047. This work was also supported by the U.S. Department of Energy under Contract DE-AC0206CH11357 from the Vehicle Technologies Office, Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE). Y.B. acknowledges the support from the State Scholarship Fund (Grant No. 201406035025) of the China Scholarship Council. R.S. acknowledges financial support from the National Science Foundation (Award No. CMMI-1200383). Partial funding from Argonne National Laboratory for Y.Y. under subcontract No. 4F31422 is acknowledged. NR 50 TC 5 Z9 5 U1 27 U2 60 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD MAY 6 PY 2016 VL 3 IS 9 AR 1500740 DI 10.1002/admi.201500740 PG 8 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DQ0JN UT WOS:000378885300006 ER PT J AU Xin, JW Mark, A Afrasiabi, C Tsueng, G Juchler, M Gopal, N Stupp, GS Putman, TE Ainscough, BJ Griffith, OL Torkamani, A Whetzel, PL Mungall, CJ Mooney, SD Su, AI Wu, CL AF Xin, Jiwen Mark, Adam Afrasiabi, Cyrus Tsueng, Ginger Juchler, Moritz Gopal, Nikhil Stupp, Gregory S. Putman, Timothy E. Ainscough, Benjamin J. Griffith, Obi L. Torkamani, Ali Whetzel, Patricia L. Mungall, Christopher J. Mooney, Sean D. Su, Andrew I. Wu, Chunlei TI High-performance web services for querying gene and variant annotation SO GENOME BIOLOGY LA English DT Article DE Annotation; Gene; Variant; API; Cloud; Repository; Database ID CENTERED INFORMATION; SEQUENCING DATA; DATABASE; GENOME; UPDATE; NCBI; MUTATIONS; PHENOTYPE; DISCOVERY; KNOWLEDGE AB Efficient tools for data management and integration are essential for many aspects of high-throughput biology. In particular, annotations of genes and human genetic variants are commonly used but highly fragmented across many resources. Here, we describe MyGene. info and MyVariant. info, high-performance web services for querying gene and variant annotation information. These web services are currently accessed more than three million times permonth. They also demonstrate a generalizable cloud-based model for organizing and querying biological annotation information. MyGene. info and MyVariant. info are provided as high-performance web services, accessible at http://mygene.info and http://myvariant.info. Both are offered free of charge to the research community. C1 [Xin, Jiwen; Mark, Adam; Afrasiabi, Cyrus; Tsueng, Ginger; Stupp, Gregory S.; Putman, Timothy E.; Su, Andrew I.; Wu, Chunlei] Scripps Res Inst, Dept Mol & Expt Med, 10550 North Torrey Pines Rd, La Jolla, CA 92037 USA. [Mark, Adam] Avera Canc Inst, 11099 N Torrey Pines Rd, La Jolla, CA 92037 USA. [Juchler, Moritz; Gopal, Nikhil; Mooney, Sean D.] Univ Washington, Dept Biomed Informat & Med Educ, Box SLU BIME 358047, Seattle, WA 98195 USA. [Ainscough, Benjamin J.; Griffith, Obi L.] Washington Univ, Sch Med, McDonnell Genome Inst, 4444 Forest Pk Ave, St Louis, MO 63108 USA. [Torkamani, Ali] Scripps Res Inst, Dept Integrat Struct & Computat Biol, 10550 North Torrey Pines Rd, La Jolla, CA 92037 USA. [Torkamani, Ali; Su, Andrew I.] Scripps Res Inst, Scripps Translat Sci Inst, 10550 N Torrey Pines Rd, La Jolla, CA 92037 USA. [Whetzel, Patricia L.] Univ Calif San Diego, Ctr Res Biol Syst, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Mungall, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Su, AI; Wu, CL (reprint author), Scripps Res Inst, Dept Mol & Expt Med, 10550 North Torrey Pines Rd, La Jolla, CA 92037 USA.; Su, AI (reprint author), Scripps Res Inst, Scripps Translat Sci Inst, 10550 N Torrey Pines Rd, La Jolla, CA 92037 USA. EM asu@scripps.edu; cwu@scripps.edu OI Stupp, Gregory/0000-0002-0644-7212; Ainscough, Benjamin/0000-0001-8340-514X; Putman, Timothy/0000-0002-4291-0737 FU US National Institute of Health [U01HG008473, GM083924, U54GM114833, U01HG006476, K22CA188163]; Scripps Translational Science Institute; NIH-NCATS Clinical and Translational Science Award (CTSA) [5 UL1 TR001114] FX This work was supported by the US National Institute of Health ( grants U01HG008473 to CW, GM083924 and U54GM114833 to AIS, U01HG006476 to AT, and K22CA188163 to OLG). This work was also supported by the Scripps Translational Science Institute with an NIH-NCATS Clinical and Translational Science Award (CTSA; 5 UL1 TR001114). NR 42 TC 5 Z9 5 U1 3 U2 6 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1465-6906 EI 1474-760X J9 GENOME BIOL JI Genome Biol. PD MAY 6 PY 2016 VL 17 AR 91 DI 10.1186/s13059-016-0953-9 PG 7 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA DL9KY UT WOS:000375962700001 PM 27154141 ER PT J AU Pereira, JH Heins, RA Gall, DL McAndrew, RP Deng, K Holland, KC Donohue, TJ Noguera, DR Simmons, BA Sale, KL Ralph, J Adams, PD AF Pereira, Jose Henrique Heins, Richard A. Gall, Daniel L. McAndrew, Ryan P. Deng, Kai Holland, Keefe C. Donohue, Timothy J. Noguera, Daniel R. Simmons, Blake A. Sale, Kenneth L. Ralph, John Adams, Paul D. TI Structural and Biochemical Characterization of the Early and Late Enzymes in the Lignin beta-Aryl Ether Cleavage Pathway from Sphingobium sp.SYK-6 SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID SHORT-CHAIN DEHYDROGENASES/REDUCTASES; SP STRAIN SYK-6; ALCOHOL-DEHYDROGENASE; STRUCTURE REFINEMENT; DEGRADATION; BACTERIA; PHENIX; TRANSFERASES; SPECIFICITY; PROTEINS AB There has been great progress in the development of technology for the conversion of lignocellulosic biomass to sugars and subsequent fermentation to fuels. However, plant lignin remains an untapped source of materials for production of fuels or high value chemicals. Biological cleavage of lignin has been well characterized in fungi, in which enzymes that create free radical intermediates are used to degrade this material. In contrast, a catabolic pathway for the stereospecific cleavage of beta-aryl ether units that are found in lignin has been identified in Sphingobium sp.SYK-6 bacteria. beta-Aryl ether units are typically abundant in lignin, corresponding to 50-70% of all of the intermonomer linkages. Consequently, a comprehensive understanding of enzymatic beta-aryl ether (beta-ether) cleavage is important for future efforts to biologically process lignin and its breakdown products. The crystal structures and biochemical characterization of the NAD-dependent dehydrogenases (LigD, LigO, and LigL) and the glutathione-dependent lyase LigG provide new insights into the early and late enzymes in the beta-ether degradation pathway. We present detailed information on the cofactor and substrate binding sites and on the catalytic mechanisms of these enzymes, comparing them with other known members of their respective families. Information on the Lig enzymes provides new insight into their catalysis mechanisms and can inform future strategies for using aromatic oligomers derived from plant lignin as a source of valuable aromatic compounds for biofuels and other bioproducts. C1 [Pereira, Jose Henrique; Heins, Richard A.; McAndrew, Ryan P.; Deng, Kai; Holland, Keefe C.; Simmons, Blake A.; Sale, Kenneth L.; Adams, Paul D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Pereira, Jose Henrique; McAndrew, Ryan P.; Adams, Paul D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Heins, Richard A.; Deng, Kai; Holland, Keefe C.; Simmons, Blake A.; Sale, Kenneth L.] Sandia Natl Labs, Biol & Engn Sci Ctr, Livermore, CA 94551 USA. [Gall, Daniel L.; Donohue, Timothy J.; Noguera, Daniel R.; Ralph, John] Univ Wisconsin, US Dept, Energy Great Lakes Bioenergy Res Ctr, Wisconsin Energy Inst, Madison, WI 53726 USA. [Gall, Daniel L.; Noguera, Daniel R.] Univ Wisconsin, Dept Civil & Environm Engn, Madison, WI 53706 USA. [Donohue, Timothy J.; Ralph, John] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Adams, Paul D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Adams, PD (reprint author), Joint BioEnergy Inst, Emeryville, CA 94608 USA.; Adams, PD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA.; Adams, PD (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM pdadams@lbl.gov FU NIGMS, National Institutes of Health; Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231] FX We are grateful to the staff of the Berkeley Center for Structural Biology at the Advanced Light Source of Lawrence Berkeley National Laboratory. The Berkeley Center for Structural Biology is supported in part by NIGMS, National Institutes of Health. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under Contract DE-AC02-05CH11231. NR 36 TC 0 Z9 0 U1 9 U2 25 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAY 6 PY 2016 VL 291 IS 19 BP 10228 EP + DI 10.1074/jbc.M115.700427 PG 26 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DL4KB UT WOS:000375602800031 PM 26940872 ER PT J AU Hansen, RH Timm, AC Timm, CM Bible, AN Morrell-Falvey, JL Pelletier, DA Simpson, ML Doktycz, MJ Retterer, ST AF Hansen, Ryan H. Timm, Andrea C. Timm, Collin M. Bible, Amber N. Morrell-Falvey, Jennifer L. Pelletier, Dale A. Simpson, Michael L. Doktycz, Mitchel J. Retterer, Scott T. TI Stochastic Assembly of Bacteria in Microwell Arrays Reveals the Importance of Confinement in Community Development SO PLOS ONE LA English DT Article ID MICROBIAL COMMUNITIES; VI SECRETION; LIFT-OFF; MICROFLUIDICS; BIOFILMS; CULTURE; SYSTEM; GROWTH; FLOW AB The structure and function of microbial communities is deeply influenced by the physical and chemical architecture of the local microenvironment and the abundance of its community members. The complexity of this natural parameter space has made characterization of the key drivers of community development difficult. In order to facilitate these characterizations, we have developed a microwell platform designed to screen microbial growth and interactions across a wide variety of physical and initial conditions. Assembly of microbial communities into microwells was achieved using a novel biofabrication method that exploits well feature sizes for control of innoculum levels. Wells with incrementally smaller size features created populations with increasingly larger variations in inoculum levels. This allowed for reproducible growth measurement in large (20 mu m diameter) wells, and screening for favorable growth conditions in small (5, 10 mu m diameter) wells. We demonstrate the utility of this approach for screening and discovery using 5 mu m wells to assemble P. aeruginosa colonies across a broad distribution of innoculum levels, and identify those conditions that promote the highest probability of survivial and growth under spatial confinement. Multi-member community assembly was also characterized to demonstrate the broad potential of this platform for studying the role of member abundance on microbial competition, mutualism and community succession. C1 [Hansen, Ryan H.] Kansas State Univ, Manhattan, KS 66506 USA. [Hansen, Ryan H.; Morrell-Falvey, Jennifer L.; Simpson, Michael L.; Doktycz, Mitchel J.; Retterer, Scott T.] Univ Tennessee, Knoxville, TN USA. [Timm, Andrea C.; Timm, Collin M.; Bible, Amber N.; Morrell-Falvey, Jennifer L.; Pelletier, Dale A.; Simpson, Michael L.; Doktycz, Mitchel J.; Retterer, Scott T.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Retterer, ST (reprint author), Univ Tennessee, Knoxville, TN USA.; Retterer, ST (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA. EM rettererst@ornl.gov RI Morrell-Falvey, Jennifer/A-6615-2011; Doktycz, Mitchel/A-7499-2011; Simpson, Michael/A-8410-2011 OI Morrell-Falvey, Jennifer/0000-0002-9362-7528; Doktycz, Mitchel/0000-0003-4856-8343; Simpson, Michael/0000-0002-3933-3457 FU Genomic Science Program; U.S. Department of Energy; Office of Science; Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area; ORNL Laboratory Directed Research and Development FX This work was supported in part by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov) as well as ORNL Laboratory Directed Research and Development. Microwell arrays were fabricated and characterized at the Center for Nanophase Materials Sciences User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors would also like to thank the J. Mougous Laboratory (University of Washington, Seattle, WA) for the supply of P. aeruginosa strains used in these studies and Dr. B. Tseng Laboratory (University of Washington, Seattle, WA) for the supply of plasmids used to express GFP and mCherry in E. coli. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 42 TC 4 Z9 4 U1 12 U2 31 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 6 PY 2016 VL 11 IS 5 AR e0155080 DI 10.1371/journal.pone.0155080 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL5KX UT WOS:000375677000066 PM 27152511 ER PT J AU Olesen, SW Vora, S Techtmann, SM Fortney, JL Bastidas-Oyanedel, JR Rodriguez, J Hazen, TC Alm, EJ AF Olesen, Scott W. Vora, Suhani Techtmann, Stephen M. Fortney, Julian L. Bastidas-Oyanedel, Juan R. Rodriguez, Jorge Hazen, Terry C. Alm, Eric J. TI A Novel Analysis Method for Paired-Sample Microbial Ecology Experiments SO PLOS ONE LA English DT Article ID HORIZON OIL-SPILL; SPECIES-ABUNDANCE; MULTIVARIATE ANALYSES; GEN. NOV.; COMMUNITIES; SEQUENCES; FRAMEWORK; BACTERIA; DATABASE AB Many microbial ecology experiments use sequencing data to measure a community's response to an experimental treatment. In a common experimental design, two units, one control and one experimental, are sampled before and after the treatment is applied to the experimental unit. The four resulting samples contain information about the dynamics of organisms that respond to the treatment, but there are no analytical methods designed to extract exactly this type of information from this configuration of samples. Here we present an analytical method specifically designed to visualize and generate hypotheses about microbial community dynamics in experiments that have paired samples and few or no replicates. The method is based on the Poisson lognormal distribution, long studied in macroecology, which we found accurately models the abundance distribution of taxa counts from 16S rRNA surveys. To demonstrate the method's validity and potential, we analyzed an experiment that measured the effect of crude oil on ocean microbial communities in microcosm. Our method identified known oil degraders as well as two clades, Maricurvus and Rhodobacteraceae, that responded to amendment with oil but do not include known oil degraders. Our approach is sensitive to organisms that increased in abundance only in the experimental unit but less sensitive to organisms that increased in both control and experimental units, thus mitigating the role of "bottle effects". C1 [Olesen, Scott W.; Vora, Suhani; Alm, Eric J.] MIT, Dept Biol Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Techtmann, Stephen M.; Fortney, Julian L.; Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Fortney, Julian L.; Hazen, Terry C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bastidas-Oyanedel, Juan R.; Rodriguez, Jorge] Masdar Inst Sci & Technol, Inst Ctr Water & Environm iWater, Abu Dhabi, U Arab Emirates. RP Alm, EJ (reprint author), MIT, Dept Biol Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM ejalm@mit.edu RI Hazen, Terry/C-1076-2012; OI Hazen, Terry/0000-0002-2536-9993; Rodriguez, Jorge/0000-0002-5936-9676 FU BP Exploration/MIT Energy Initiative [6926835]; National Science Foundation [0821391, 1122374] FX This material is based upon work supported by BP Exploration/MIT Energy Initiative (mitei.mit.edu) under Grant No. 6926835, the National Science Foundation (nsf.gov) under Grant No. 0821391, and the National Science Foundation Graduate Research Fellowship (nsfgrfp.org) under Grant No. 1122374. NR 44 TC 1 Z9 1 U1 2 U2 13 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 6 PY 2016 VL 11 IS 5 AR e0154804 DI 10.1371/journal.pone.0154804 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL5KX UT WOS:000375677000038 PM 27152415 ER PT J AU Xue, K Xie, JP Zhou, AF Liu, FF Li, DJ Wu, LY Deng, Y He, ZL Van Nostrand, JD Luo, YQ Zhou, JZ AF Xue, Kai Xie, Jianping Zhou, Aifen Liu, Feifei Li, Dejun Wu, Liyou Deng, Ye He, Zhili Van Nostrand, Joy D. Luo, Yiqi Zhou, Jizhong TI Warming Alters Expressions of Microbial Functional Genes Important to Ecosystem Functioning SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE RNA; functional gene expression; global climate change; warming; GeoChip ID MICROARRAY-BASED ANALYSIS; NET PRIMARY PRODUCTIVITY; NITROGEN-USE EFFICIENCY; MOUNTAIN FOREST SOIL; 16S RIBOSOMAL-RNA; TALLGRASS PRAIRIE; COMMUNITY STRUCTURE; SULFATE ASSIMILATION; BACTERIAL COMMUNITY; ORGANIC-CARBON AB Soil microbial communities play critical roles in ecosystem functioning and are likely altered by climate warming. However, so far, little is known about effects of warming on microbial functional gene expressions. Here, we applied functional gene array (GeoChip 3.0) to analyze cDNA reversely transcribed from total RNA to assess expressed functional genes in active soil microbial communities after nine years of experimental warming in a tallgrass prairie. Our results showed that warming significantly altered the community wide gene expressions. Specifically, expressed genes for degrading more recalcitrant carbon were stimulated by warming, likely linked to the plant community shift toward more C-4 species under warming and to decrease the long-term soil carbon stability. In addition, warming changed expressed genes in labile C degradation and N cycling in different directions (increase and decrease), possibly reflecting the dynamics of labile C and available N pools during sampling. However, the average abundances of expressed genes in phosphorus and sulfur cycling were all increased by warming, implying a stable trend of accelerated P and S processes which might be a mechanism to sustain higher plant growth. Furthermore, the expressed gene composition was closely related to both dynamic (e.g., soil moisture) and stable environmental attributes (e.g., C-4 leaf C or N content), indicating that RNA analyses could also capture certain stable trends in the long-term treatment. Overall, this study revealed the importance of elucidating functional gene expressions of soil microbial community in enhancing our understanding of ecosystem responses to warming. C1 [Xue, Kai; Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Xue, Kai; Xie, Jianping; Zhou, Aifen; Liu, Feifei; Wu, Liyou; Deng, Ye; He, Zhili; Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Xue, Kai; Xie, Jianping; Zhou, Aifen; Liu, Feifei; Li, Dejun; Wu, Liyou; Deng, Ye; He, Zhili; Van Nostrand, Joy D.; Luo, Yiqi; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Xie, Jianping] Cent S Univ, Sch Mineral Proc & Bioengn, Changsha, Hunan, Peoples R China. [Deng, Ye] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Environm Biotechnol, Beijing, Peoples R China. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Zhou, JZ (reprint author), Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China.; Zhou, JZ (reprint author), Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM jzhou@ou.edu OI ?, ?/0000-0002-7584-0632 FU United States Department of Energy, Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program [DE-SC0004601]; Oklahoma Bioenergy Center (OBC) FX This work was supported by the United States Department of Energy, Biological Systems Research on the Role of Microbial Communities in Carbon Cycling Program (DE-SC0004601), and Oklahoma Bioenergy Center (OBC). NR 78 TC 1 Z9 1 U1 15 U2 42 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAY 6 PY 2016 VL 7 AR 668 DI 10.3389/fmicb.2016.00668 PG 13 WC Microbiology SC Microbiology GA DL1OD UT WOS:000375400700002 PM 27199978 ER PT J AU Malone, MW Yoder, J Hunter, JF Espy, MA Dickman, LT Nelson, RO Vogel, SC Sandin, HJ Sevanto, S AF Malone, Michael W. Yoder, Jacob Hunter, James F. Espy, Michelle A. Dickman, Lee T. Nelson, Ron O. Vogel, Sven C. Sandin, Henrik J. Sevanto, Sanna TI In vivo Observation of Tree Drought Response with Low-Field NMR and Neutron Imaging SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE water; NMR; tree; health; flow; neutron imaging; drought; hydraulics ID STEM DIAMETER VARIATIONS; DISTANCE WATER TRANSPORT; SCOTS PINE; SAP FLOW; XYLEM; CAVITATION; MRI; EMBOLISM; PHLOEM; LEAVES AB Using a simple low-field NMR system, we monitored water content in a living tree in a greenhouse over 2 months. By continuously running the system, we observed changes in tree water content on a scale of half an hour. The data showed a diurnal change in water content consistent both with previous NMR and biological observations. Neutron imaging experiments show that our NMR signal is primarily due to water being rapidly transported through the plant, and not to other sources of hydrogen, such as water in cytoplasm, or water in cell walls. After accounting for the role of temperature in the observed NMR signal, we demonstrate a change in the diurnal signal behavior due to simulated drought conditions for the tree. These results illustrate the utility of our system to perform noninvasive measurements of tree water content outside of a temperature controlled environment. C1 [Malone, Michael W.; Yoder, Jacob; Hunter, James F.; Espy, Michelle A.; Dickman, Lee T.; Nelson, Ron O.; Vogel, Sven C.; Sandin, Henrik J.; Sevanto, Sanna] Los Alamos Natl Lab, Los Alamos, NM USA. RP Malone, MW (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM mwmalone@lanl.gov OI Vogel, Sven C./0000-0003-2049-0361 FU Los Alamos National Laboratory LDRD program [20130442ER] FX Leaf area measurements were performed by Elizabeth Stockton. This project was supported by the Los Alamos National Laboratory LDRD program via Grant No. 20130442ER. NR 35 TC 0 Z9 0 U1 9 U2 18 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAY 6 PY 2016 VL 7 AR 564 DI 10.3389/fpls.2016.00564 PG 9 WC Plant Sciences SC Plant Sciences GA DL0SJ UT WOS:000375342600001 PM 27200037 ER PT J AU Vagov, A Shanenko, AA Milosevic, MV Axt, VM Vinokur, VM Aguiar, JA Peeters, FM AF Vagov, A. Shanenko, A. A. Milosevic, M. V. Axt, V. M. Vinokur, V. M. Albino Aguiar, J. Peeters, F. M. TI Superconductivity between standard types: Multiband versus single-band materials SO PHYSICAL REVIEW B LA English DT Article ID GINZBURG-LANDAU EQUATIONS; INTERMEDIATE-MIXED STATE; CHERN-SIMONS VORTICES; FLUX LINE PROFILES; II SUPERCONDUCTORS; 1ST-ORDER TRANSITIONS; VORTEX; PARAMETERS; BEHAVIOR; T=TC AB In the nearest vicinity of the critical temperature, types I and II of conventional single-band superconductors interchange at the Ginzburg-Landau parameter kappa = 1/root 2. At lower temperatures this point unfolds into a narrow but finite interval of kappa's, shaping an intertype (transitional) domain in the (kappa, T) plane. In the present work, based on the extended Ginzburg-Landau formalism, we show that the same picture of the two standard types with the transitional domain in between applies also to multiband superconductors. However, the intertype domain notably widens in the presence of multiple bands and can become extremely large when the system has a significant disparity between the band parameters. It is concluded that many multiband superconductors, such as recently discovered borides and iron-based materials, can belong to the intertype regime. C1 [Vagov, A.; Axt, V. M.] Univ Bayreuth, Inst Theoret Phys 3, POB 101251, D-95440 Bayreuth, Germany. [Shanenko, A. A.; Albino Aguiar, J.] Univ Fed Pernambuco, Dept Fis, Av Jorn Anibal Fernandes S-N, BR-50740901 Recife, PE, Brazil. [Milosevic, M. V.; Peeters, F. M.] Univ Antwerp, Dept Fys, Groenenborgerlaan 171, B-2020 Antwerp, Belgium. [Vinokur, V. M.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Vagov, A (reprint author), Univ Bayreuth, Inst Theoret Phys 3, POB 101251, D-95440 Bayreuth, Germany. RI Milosevic, Milorad/H-9393-2012 FU Brazilian agency CNPq [307552/2012-8, 141911/2012-3]; Brazilian agency FACEPE [APQ-0589-1.05/08]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX This work was supported by Brazilian agencies CNPq (Grants No. 307552/2012-8 and No. 141911/2012-3) and FACEPE (Grant No. APQ-0589-1.05/08) as well as by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 63 TC 5 Z9 5 U1 8 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 6 PY 2016 VL 93 IS 17 AR 174503 DI 10.1103/PhysRevB.93.174503 PG 15 WC Physics, Condensed Matter SC Physics GA DL3IM UT WOS:000375527500001 ER PT J AU Boyken, SE Chen, ZB Groves, B Langan, RA Oberdorfer, G Ford, A Gilmore, JM Xu, CF DiMaio, F Pereira, JH Sankaran, B Seelig, G Zwart, PH Baker, D AF Boyken, Scott E. Chen, Zibo Groves, Benjamin Langan, Robert A. Oberdorfer, Gustav Ford, Alex Gilmore, Jason M. Xu, Chunfu DiMaio, Frank Pereira, Jose Henrique Sankaran, Banumathi Seelig, Georg Zwart, Peter H. Baker, David TI De novo design of protein homo-oligomers with modular hydrogen-bond network-mediated specificity SO SCIENCE LA English DT Article ID BURIED POLAR RESIDUES; ATOMIC-LEVEL ACCURACY; BZIP-BINDING PEPTIDES; TRIMERIC COILED-COIL; GCN4 LEUCINE-ZIPPER; COMPUTATIONAL DESIGN; ELECTROSTATIC INTERACTIONS; STRUCTURAL SPECIFICITY; DNA NANOTECHNOLOGY; CRYSTAL-STRUCTURE AB In nature, structural specificity in DNA and proteins is encoded differently: In DNA, specificity arises from modular hydrogen bonds in the core of the double helix, whereas in proteins, specificity arises largely from buried hydrophobic packing complemented by irregular peripheral polar interactions. Here, we describe a general approach for designing a wide range of protein homo-oligomers with specificity determined by modular arrays of central hydrogen-bond networks. We use the approach to design dimers, trimers, and tetramers consisting of two concentric rings of helices, including previously not seen triangular, square, and supercoiled topologies. X-ray crystallography confirms that the structures overall, and the hydrogen-bond networks in particular, are nearly identical to the design models, and the networks confer interaction specificity in vivo. The ability to design extensive hydrogen-bond networks with atomic accuracy enables the programming of protein interaction specificity for a broad range of synthetic biology applications; more generally, our results demonstrate that, even with the tremendous diversity observed in nature, there are fundamentally new modes of interaction to be discovered in proteins. C1 [Boyken, Scott E.; Chen, Zibo; Langan, Robert A.; Oberdorfer, Gustav; Ford, Alex; Gilmore, Jason M.; Xu, Chunfu; DiMaio, Frank; Baker, David] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [Boyken, Scott E.; Chen, Zibo; Langan, Robert A.; Oberdorfer, Gustav; Ford, Alex; Gilmore, Jason M.; Xu, Chunfu; DiMaio, Frank; Baker, David] Univ Washington, Inst Prot Design, Seattle, WA 98195 USA. [Boyken, Scott E.; Baker, David] Univ Washington, Howard Hughes Med Inst, Seattle, WA 98195 USA. [Chen, Zibo] Univ Washington, Grad Program Biol Phys Struct & Design, Seattle, WA 98195 USA. [Groves, Benjamin; Seelig, Georg] Univ Washington, Dept Elect Engn, Seattle, WA 98195 USA. [Oberdorfer, Gustav] Univ Washington, Dept Comp Sci & Engn, Seattle, WA 98195 USA. [Pereira, Jose Henrique] Graz Univ, Inst Mol Biosci, Humboldtstr 50-3, A-8010 Graz, Austria. [Pereira, Jose Henrique] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Sankaran, Banumathi; Zwart, Peter H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. [Seelig, Georg] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Mol Biophys & Integrated Bioimaging, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Zwart, Peter H.] Univ Washington, Dept Comp Sci & Engn, Seattle, WA 98195 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Adv Math Energy Res Applicat, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Baker, D (reprint author), Univ Washington, Dept Biochem, Seattle, WA 98195 USA. EM dabaker@u.washington.edu FU Howard Hughes Medical Institute; U.S. Department of Energy; European Research Area (ERA)-NET BioOrigami consortium; NSF [MCB-1445201]; Lawrence Berkeley National Laboratory, Berkeley, California Department of Energy [DE-AC02-05CH11231]; National Institute of General Medical Sciences (NIH); Marie Curie International Outgoing Fellowship [332094]; Washington Research Foundation Innovation Postdoctoral Fellowships FX We thank L. Carter for assistance with SEC-MALS and protein production and Rosetta@Home volunteers for contributing computing resources to enable rigorous testing of designs by ab initio structure prediction, F. Seeger for guidance with SAXS data analysis, and M. Bick and P. Lu for assistance with crystallographic refinement. This work was supported by the Howard Hughes Medical Institute, the U.S. Department of Energy, the European Research Area (ERA)-NET BioOrigami consortium, and NSF (MCB-1445201). Design calculations were facilitated though the use of advanced computational, storage, and networking infrastructure provided by the Hyak supercomputer system at the University of Washington. X-ray crystallography and SAXS data were collected at the Advanced Light Source (Lawrence Berkeley National Laboratory, Berkeley, California Department of Energy, contract no. DE-AC02-05CH11231); SAXS data were collected through the SIBYLS mail-in SAXS program under the aforementioned contract number, and we thank K. Burnett and G. Hura. The Berkeley Center for Structural Biology is supported in part by the National Institute of General Medical Sciences (NIH), and the Howard Hughes Medical Institute. G.O. is a Marie Curie International Outgoing Fellowship fellow (332094 ASR-CompEnzDes FP7-People-2012-IOF). B.G and J.M.G. are supported by Washington Research Foundation Innovation Postdoctoral Fellowships. Coordinates and structure files have been deposited to the Protein Data Bank with accession codes: 5J0J (2L6HC3_6), 5J0I (2L6HC3_12), 5J0H (2L6HC3_13), 5IZS (5L6HC3_1), 5J73 (2L4HC2_9), 5J2L (2L4HC2_11), 5J0L (3L6HC2_2), 5J0K (2L4HC2_23), 5J10 (2L4HC2_24). S.E.B., Z.C., and D.B. designed the research and S.E.B. and D.B. wrote the manuscript S.E.B. developed the HBNet method and wrote the program code. D.B. wrote the parametric backbone generation code with help from C.X. and G.O. A.F. wrote the loop closure program code. S.E.B., Z.C., R.A.L., and D.B. carried out design calculations. S.E.B. and Z.C. purified and biophysically characterized the designed proteins. B.G. performed yeast two-hybrid assays. J.M.G. performed mass spectrometry. J.H.P. crystallized the designed proteins. B.S. NR 60 TC 14 Z9 14 U1 21 U2 64 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 6 PY 2016 VL 352 IS 6286 BP 680 EP 687 DI 10.1126/science.aad8865 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1UC UT WOS:000375417100031 PM 27151862 ER PT J AU Pande, K Hutchison, CDM Groenhof, G Aquila, A Robinson, JS Tenboer, J Basu, S Boutet, S DePonte, DP Liang, MN White, TA Zatsepin, NA Yefanov, O Morozov, D Oberthuer, D Gati, C Subramanian, G James, D Zhao, Y Koralek, J Brayshaw, J Kupitz, C Conrad, C Roy-Chowdhury, S Coe, JD Metz, M Xavier, PL Grant, TD Koglin, JE Ketawala, G Fromme, R Srajer, V Henning, R Spence, JCH Ourmazd, A Schwander, P Weierstall, U Frank, M Fromme, P Barty, A Chapman, HN Moffat, K van Thor, JJ Schmidt, M AF Pande, Kanupriya Hutchison, Christopher D. M. Groenhof, Gerrit Aquila, Andy Robinson, Josef S. Tenboer, Jason Basu, Shibom Boutet, Sebastien DePonte, Daniel P. Liang, Mengning White, Thomas A. Zatsepin, Nadia A. Yefanov, Oleksandr Morozov, Dmitry Oberthuer, Dominik Gati, Cornelius Subramanian, Ganesh James, Daniel Zhao, Yun Koralek, Jake Brayshaw, Jennifer Kupitz, Christopher Conrad, Chelsie Roy-Chowdhury, Shatabdi Coe, Jesse D. Metz, Markus Xavier, Paulraj Lourdu Grant, Thomas D. Koglin, Jason E. Ketawala, Gihan Fromme, Raimund Srajer, Vukica Henning, Robert Spence, John C. H. Ourmazd, Abbas Schwander, Peter Weierstall, Uwe Frank, Matthias Fromme, Petra Barty, Anton Chapman, Henry N. Moffat, Keith van Thor, Jasper J. Schmidt, Marius TI Femtosecond structural dynamics drives the trans/cis isomerization in photoactive yellow protein SO SCIENCE LA English DT Article ID X-RAY-DIFFRACTION; FREE-ELECTRON LASER; TIME; SPECTROSCOPY; CHROMOPHORE; MYOGLOBIN; CRYSTALLOGRAPHY; PHOTOCYCLE; EXCITATION; PULSES AB A variety of organisms have evolved mechanisms to detect and respond to light, in which the response is mediated by protein structural changes after photon absorption. The initial step is often the photoisomerization of a conjugated chromophore. Isomerization occurs on ultrafast time scales and is substantially influenced by the chromophore environment. Here we identify structural changes associated with the earliest steps in the trans-to-cis isomerization of the chromophore in photoactive yellow protein. Femtosecond hard x-ray pulses emitted by the Linac Coherent Light Source were used to conduct time-resolved serial femtosecond crystallography on photoactive yellow protein microcrystals over a time range from 100 femtoseconds to 3 picoseconds to determine the structural dynamics of the photoisomerization reaction. C1 [Pande, Kanupriya; Tenboer, Jason; Brayshaw, Jennifer; Kupitz, Christopher; Ourmazd, Abbas; Schwander, Peter; Schmidt, Marius] Univ Wisconsin, Dept Phys, Milwaukee, WI 53211 USA. [Pande, Kanupriya; Yefanov, Oleksandr; Oberthuer, Dominik; Gati, Cornelius; Metz, Markus; Xavier, Paulraj Lourdu; Barty, Anton; Chapman, Henry N.] DESY, Ctr Free Electron Laser Sci, Notkestr 85, D-22607 Hamburg, Germany. [Hutchison, Christopher D. M.; van Thor, Jasper J.] Univ London Imperial Coll Sci Technol & Med, Dept Life Sci, Fac Nat Sci, London SW7 2AZ, England. [Groenhof, Gerrit] Univ Jyvaskyla, Nanosci Ctr, POB 35, Jyvaskyla 40014, Finland. [Groenhof, Gerrit] Univ Jyvaskyla, Dept Chem, POB 35, Jyvaskyla 40014, Finland. [Aquila, Andy; Robinson, Josef S.; Boutet, Sebastien; DePonte, Daniel P.; Liang, Mengning; Koralek, Jake] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Sand Hill Rd, Menlo Pk, CA 94025 USA. [Basu, Shibom; Conrad, Chelsie; Roy-Chowdhury, Shatabdi; Coe, Jesse D.; Ketawala, Gihan; Fromme, Raimund; Fromme, Petra] Arizona State Univ, Sch Mol Sci, Tempe, AZ 85287 USA. [Basu, Shibom; Conrad, Chelsie; Roy-Chowdhury, Shatabdi; Coe, Jesse D.; Ketawala, Gihan; Fromme, Raimund; Fromme, Petra] Arizona State Univ, Biodesign Ctr Appl Struct Discovery, Tempe, AZ 85287 USA. [Zatsepin, Nadia A.; Subramanian, Ganesh; James, Daniel; Zhao, Yun; Spence, John C. H.; Weierstall, Uwe] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Xavier, Paulraj Lourdu] Max Planck Inst Struct & Dynam Matter, IMPRS UFAST, Luruper Chaussee 149, D-22761 Hamburg, Germany. [Grant, Thomas D.] SUNY Buffalo, Hauptman Woodward Inst, 700 Ellicott St, Buffalo, NY 14203 USA. [Srajer, Vukica; Henning, Robert; Moffat, Keith] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. [Frank, Matthias] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Chapman, Henry N.] Univ Hamburg, Ctr Ultrafast Imaging, Luruper Chaussee 149, D-22761 Hamburg, Germany. [Moffat, Keith] Univ Chicago, Dept Biochem & Mol Biol, 920 E 58Th St, Chicago, IL 60637 USA. [Moffat, Keith] Univ Chicago, Inst Biophys Dynam, Chicago, IL 60637 USA. RP Schmidt, M (reprint author), Univ Wisconsin, Dept Phys, Milwaukee, WI 53211 USA. EM m-schmidt@uwm.edu RI Fromme, Raimund/C-8885-2012; Chapman, Henry/G-2153-2010; OI Fromme, Raimund/0000-0003-4835-1080; Chapman, Henry/0000-0002-4655-1743; Groenhof, Gerrit/0000-0001-8148-5334; James, Daniel/0000-0002-8348-6661 FU NSF Science and Technology Center BioXFEL [NSF-1231306]; NIH [R01GM095583, R01EY024363, R24GM111072, P41GM103393, P41RR001209]; Helmholtz Association Virtual Institute Dynamic Pathways; Federal Ministry of Education and Research, Germany (BMBF) [05K14CHA]; Engineering and Physical Sciences Research Council [EP/M000192/1]; Academy of Finland; BMBF project [05K13GUK]; European Union [FP7-PEOPLE-2011-ITN NanoMem]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; LLNL Lab-Directed Research and Development Project [012-ERD-031]; PIER Helmholtz Graduate School; [NSF-0952643]; [NSF-1158138] FX This work is supported by the NSF Science and Technology Center BioXFEL (grant NSF-1231306); by NIH grants R01GM095583 (P.F.), R01EY024363 (K.M.), and R24GM111072 (V.S., R.H., and K.M.); Helmholtz Association Virtual Institute Dynamic Pathways (H.C.); and grant NSF-0952643 (M.S.). K.P. is partly supported by grant NSF-1158138 (to D. Saldin and M.S.) and Federal Ministry of Education and Research, Germany (BMBF) grant 05K14CHA (to H.C.). J.J.v.T. acknowledges support from the Engineering and Physical Sciences Research Council via grant agreement EP/M000192/1. G.G. and D.M. are supported by the Academy of Finland, D.O. by BMBF project 05K13GUK, and M.M. by the European Union through grant FP7-PEOPLE-2011-ITN NanoMem. Use of the LCLS, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-76SF00515. Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under contract DE-AC52-07NA27344, and M.F. was supported by LLNL Lab-Directed Research and Development Project 012-ERD-031. C.G. thanks the PIER Helmholtz Graduate School for financial support. Parts of the sample injector used at LCLS for this research were funded by NIH grant P41GM103393, formerly P41RR001209. We thank the Moscow State University supercomputing center and the Finnish IT Center for Science (CSC-IT) Center for Science, Finland, for computing resources. We thank M. Hunter for valuable discussions, T. Graen for help with the computer simulations, and C. Li for assistance with injectors. The PYPref, PYPfast, PYPslow, PYP3ps, and PYP200ns structures are deposited in the Protein Data Bank together with their respective weighted difference structure factor amplitudes under accession codes 5HD3, 5HDC, 5HDD, 5HDS, and 5HD5, respectively. M.S. prepared the proposal with input from J.J.vT., K.M., V.S., J.C.H.S., H.N.C., A.O., and P.F.; A.A., S.B., M.L., J.S.R., and J.E.K. operated the CXI instrument, including the time tool and the femtosecond laser; and K.P., A.B., J.T., S.B., T.A.W., N.Z., O.Y., and T.D.G. analyzed the SFX data. C.D.M.H and J.J.vT. set up the FROG at the CXI instrument; G.G. and D.M. performed QM/MM calculations; J.T., J.B., D.O., P.L.X., C.G., C.K., and M.S. prepared protein and grew nano-and microcrystals; D.DeP., C.K., C.C., S.R.-C., J.D.C., M.M., G.K., and U.W. provided and operated the injector system; M.F., R.F., M.S., J.T., P.F., D.O., and C.G. wrote the electronic log; M.F., M.S, J.T., J.S.R., J.J.vT., and K.M. discussed femtosecond laser excitation; J.T., M.S, V.S, R.H, C. D.M.H., and J.J.vT. performed preliminary ultrafast experiments on crystals; M.S. calculated and analyzed the difference maps; and M.S., K.P., K.M., G.G., P.F., and J.J.vT. wrote the manuscript, with improvements from all authors. NR 47 TC 23 Z9 23 U1 45 U2 89 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 6 PY 2016 VL 352 IS 6286 BP 725 EP 729 DI 10.1126/science.aad5081 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1UC UT WOS:000375417100042 PM 27151871 ER PT J AU Viswanathan, V Pande, V Abraham, KM Luntz, AC McCloskey, BD Addison, D AF Viswanathan, Venkatasubramanian Pande, Vikram Abraham, K. M. Luntz, Alan C. McCloskey, Bryan D. Addison, Dan TI Comment on "Cycling Li-O-2 batteries via LiOH formation and decomposition" SO SCIENCE LA English DT Editorial Material AB Based on a simple thermodynamic analysis, we show that iodide-mediated electrochemical decomposition of lithium hydroxide (LiOH) likely occurs through a different mechanism than that proposed by Liu et al. (Research Article, 30 October 2015, p. 530). The mismatch in thermodynamic potentials for iodide/triiodide (I-/I-3(-)) redox and O-2 evolution from LiOH implies a different active iodine/oxygen electrochemistry on battery charge. It is therefore possible that the system described in Liu et al. may not form the basis for a rechargeable lithium-oxygen (Li-O-2) battery. C1 [Viswanathan, Venkatasubramanian; Pande, Vikram] Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. [Abraham, K. M.] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. [Luntz, Alan C.] SLAC Natl Accelerator Lab, SUNCAT, Menlo Pk, CA 94025 USA. [McCloskey, Bryan D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [McCloskey, Bryan D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Berkeley, CA 94720 USA. [Addison, Dan] Liox Power Inc, 129 North Hill Ave,Suite 103, Pasadena, CA 91106 USA. RP Viswanathan, V (reprint author), Carnegie Mellon Univ, Dept Mech Engn, Pittsburgh, PA 15213 USA. EM venkvis@cmu.edu NR 7 TC 5 Z9 5 U1 21 U2 51 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAY 6 PY 2016 VL 352 IS 6286 DI 10.1126/science.aad8689 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1UC UT WOS:000375417100026 ER PT J AU Kim, DO Song, KM Choi, Y Min, BC Kim, JS Choi, JW Lee, DR AF Kim, Dong-Ok Song, Kyung Mee Choi, Yongseong Min, Byoung-Chul Kim, Jae-Sung Choi, Jun Woo Lee, Dong Ryeol TI Asymmetric magnetic proximity effect in a Pd/Co/Pd trilayer system SO SCIENTIFIC REPORTS LA English DT Article ID CHIRAL SPIN TORQUE; DOMAIN-WALLS; CIRCULAR-DICHROISM; LAYERED STRUCTURES; EFFECTIVE-FIELD; MULTILAYERS; ANISOTROPY; FERROMAGNETISM; FILMS; SEMICONDUCTORS AB In spintronic devices consisting of ferromagnetic/nonmagnetic systems, the ferromagnet-induced magnetic moment in the adjacent nonmagnetic material significantly influences the spin transport properties. In this study, such magnetic proximity effect in a Pd/Co/Pd trilayer system is investigated by x-ray magnetic circular dichroism and x-ray resonant magnetic reflectivity, which enables magnetic characterizations with element and depth resolution. We observe that the total Pd magnetic moments induced at the top Co/Pd interface are significantly larger than the Pd moments at the bottom Pd/Co interface, whereas transmission electron microscopy and reflectivity analysis indicate the two interfaces are nearly identical structurally. Such asymmetry in magnetic proximity effects could be important for understanding spin transport characteristics in ferromagnetic/nonmagnetic systems and its potential application to spin devices. C1 [Kim, Dong-Ok; Lee, Dong Ryeol] Soongsil Univ, Dept Phys, Seoul 06978, South Korea. [Kim, Dong-Ok; Song, Kyung Mee; Min, Byoung-Chul; Choi, Jun Woo] Korea Inst Sci & Technol, Ctr Spintron, Seoul 02792, South Korea. [Song, Kyung Mee; Kim, Jae-Sung] Sookmyung Womens Univ, Dept Phys, Seoul 04130, South Korea. [Choi, Yongseong; Lee, Dong Ryeol] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Lee, DR (reprint author), Soongsil Univ, Dept Phys, Seoul 06978, South Korea.; Choi, JW (reprint author), Korea Inst Sci & Technol, Ctr Spintron, Seoul 02792, South Korea.; Lee, DR (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM junwoo@kist.re.kr; drlee@ssu.ac.kr OI Min, Byoung-Chul/0000-0001-8215-3286 FU KIST Institutional Program [2E26380]; Pioneer Research Center Program [2011-0027905]; NRF - Korean Government (MSIP) [2010-0004614, 2013R1A1A2011326, 2014K2A1A2048433, 2013R1A2000245]; U.S. Department of Energy, Office of Science [DEAC02-06CH11357]; NRF - Korean Government (MOE) [2010-0004614, 2013R1A1A2011326, 2014K2A1A2048433, 2013R1A2000245] FX This work was supported by the KIST Institutional Program (2E26380), the Pioneer Research Center Program (2011-0027905), and NRF grants 2010-0004614, 2013R1A1A2011326, 2014K2A1A2048433, and 2013R1A2000245 funded by the Korean Government (MSIP and MOE). Work at the Advanced Photon Source is supported by the U.S. Department of Energy, Office of Science under Grant No. DEAC02-06CH11357. NR 55 TC 1 Z9 1 U1 4 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 6 PY 2016 VL 6 AR 25391 DI 10.1038/srep25391 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1WS UT WOS:000375424300001 PM 27151368 ER PT J AU Sharma, A Gilbert, JA Lal, R AF Sharma, Anukriti Gilbert, Jack A. Lal, Rup TI (Meta) genomic insights into the pathogenome of Cellulosimicrobium cellulans SO SCIENTIFIC REPORTS LA English DT Article ID MYCOBACTERIUM-TUBERCULOSIS; MAXIMUM-LIKELIHOOD; CLPP PROTEASE; DRUG TARGET; SEQUENCE; ISLANDS; BACTERIAL; GENE; VIRULENCE; ALIGNMENT AB Despite having serious clinical manifestations, Cellulosimicrobium cellulans remain under-reported with only three genome sequences available at the time of writing. Genome sequences of C. cellulans LMG16121, C. cellulans J36 and Cellulosimicrobium sp. strain MM were used to determine distribution of pathogenicity islands (PAIs) across C. cellulans, which revealed 49 potential marker genes with known association to human infections, e.g. Fic and VbhA toxin-antitoxin system. Oligonucleotide composition-based analysis of orthologous proteins (n = 791) across three genomes revealed significant negative correlation (P < 0.05) between frequency of optimal codons (F-opt) and gene G+C content, highlighting the G+C-biased gene conversion (gBGC) effect across Cellulosimicrobium strains. Bayesian molecular-clock analysis performed on three virulent PAI proteins (Fic; D-alanyl- D-alanine-carboxypeptidase; transposase) dated the divergence event at 300 million years ago from the most common recent ancestor. Synteny-based annotation of hypothetical proteins highlighted gene transfers from non-pathogenic bacteria as a key factor in the evolution of PAIs. Additonally, deciphering the metagenomic islands using strain MM's genome with environmental data from the site of isolation (hot-spring biofilm) revealed (an) aerobic respiration as population segregation factor across the in situ cohorts. Using reference genomes and metagenomic data, our results highlight the emergence and evolution of PAIs in the genus Cellulosimicrobium. C1 [Sharma, Anukriti; Lal, Rup] Univ Delhi, Dept Zool, Delhi 110007, India. [Gilbert, Jack A.] Argonne Natl Lab, Biosci Div BIO, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Surg, 5841 S Maryland Ave, Chicago, IL 60637 USA. [Gilbert, Jack A.] Marine Biol Lab, Woods Hole, MA 02543 USA. RP Lal, R (reprint author), Univ Delhi, Dept Zool, Delhi 110007, India. EM ruplal@gmail.com FU Department of Biotechnology (DBT); National Bureau of Agriculturally Important Microorganisms (NBAIM) FX The authors acknowledge funds from Department of Biotechnology (DBT) and National Bureau of Agriculturally Important Microorganisms (NBAIM). AS gratefully acknowledge National Bureau of Agriculturally Important Microorganisms (NBAIM) for providing research fellowship. This paper was partly written during the visit by R.L. under DST-DAAD project to Germany (Helmholtz Zentrum fur Umweltzforschung-UFZ, Leipzig). NR 63 TC 4 Z9 4 U1 2 U2 7 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 6 PY 2016 VL 6 AR 25527 DI 10.1038/srep25527 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1VB UT WOS:000375419600003 PM 27151933 ER PT J AU Zhuang, HLL Zhang, LP Xu, HX Kent, PRC Ganesh, P Cooper, VR AF Zhuang, Houlong L. Zhang, Lipeng Xu, Haixuan Kent, P. R. C. Ganesh, P. Cooper, Valentino R. TI Tunable one-dimensional electron gas carrier densities at nanostructured oxide interfaces SO SCIENTIFIC REPORTS LA English DT Article ID AUGMENTED-WAVE METHOD; HIGH-MOBILITY; INDUCED POLARIZATION; HETEROSTRUCTURES; CONDUCTIVITY; SURFACE; CREATION; SRTIO3 AB The emergence of two-dimensional metallic states at the LaAlO3/SrTiO3 (LAO/STO) heterostructure interface is known to occur at a critical thickness of four LAO layers. This insulator to-metal transition can be explained through the "polar catastrophe" mechanism arising from the divergence of the electrostatic potential at the LAO surface. Here, we demonstrate that nanostructuring can be effective in reducing or eliminating this critical thickness. Employing a modified "polar catastrophe" model, we demonstrate that the nanowire heterostructure electrostatic potential diverges more rapidly as a function of layer thickness than in a regular heterostructure. Our first-principles calculations indicate that for nanowire heterostructures a robust one-dimensional electron gas (1DEG) can be induced, consistent with recent experimental observations of 1D conductivity at LAO/STO steps. Similar to LAO/STO 2DEGs, we predict that the 1D charge density decays laterally within a few unit cells away from the nanowire; thus providing a mechanism for tuning the carrier dimensionality between 1D and 2D conductivity. Our work provides insight into the creation and manipulation of charge density at an oxide heterostructure interface and therefore may be beneficial for future nanoelectronic devices and for the engineering of novel quantum phases. C1 [Zhuang, Houlong L.; Kent, P. R. C.; Ganesh, P.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Zhang, Lipeng; Xu, Haixuan] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Kent, P. R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Cooper, Valentino R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Zhuang, HLL; Ganesh, P (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA.; Cooper, VR (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM zhuanghl@ornl.gov; ganeshp@ornl.gov; coopervr@ornl.gov RI Zhuang, Houlong/D-8801-2014; Kent, Paul/A-6756-2008; Cooper, Valentino /A-2070-2012 OI Zhuang, Houlong/0000-0002-3845-4601; Kent, Paul/0000-0001-5539-4017; Cooper, Valentino /0000-0001-6714-4410 FU Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; UT/ORNL Joint Institute of Advanced Materials (JIAM) FX The authors thank A. Ron and Y. Dagan for helpful discussions and feedback. This research was sponsored by the Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy, and (HX, LZ) The University of Tennessee (UT) Science Alliance Joint Directed Research and Development Program (JDRD) and UT/ORNL Joint Institute of Advanced Materials (JIAM). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 0 Z9 0 U1 8 U2 23 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 6 PY 2016 VL 6 AR 25452 DI 10.1038/srep25452 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1UQ UT WOS:000375418500002 PM 27151049 ER PT J AU Vasudevan, RK Tselev, A Baddorf, AP Kalinin, SV AF Vasudevan, Rama K. Tselev, Alexander Baddorf, Arthur P. Kalinin, Sergei V. TI The Ehrlich-Schwoebel barrier on an oxide surface: a combined Monte-Carlo and in situ scanning tunneling microscopy approach (vol 45, 455705, 2015) SO NANOTECHNOLOGY LA English DT Correction C1 [Vasudevan, Rama K.; Tselev, Alexander; Baddorf, Arthur P.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Vasudevan, Rama K.; Tselev, Alexander; Baddorf, Arthur P.; Kalinin, Sergei V.] Oak Ridge Natl Lab, ORNL Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. RP Vasudevan, RK (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Vasudevan, RK (reprint author), Oak Ridge Natl Lab, ORNL Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. RI Baddorf, Arthur/I-1308-2016 OI Baddorf, Arthur/0000-0001-7023-2382 NR 1 TC 0 Z9 0 U1 3 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAY 6 PY 2016 VL 27 IS 18 AR 189501 DI 10.1088/0957-4484/27/18/189501 PG 2 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DH5AU UT WOS:000372798100024 ER PT J AU Moon, AF Krahn, JM Lu, X Cuneo, MJ Pedersen, LC AF Moon, Andrea F. Krahn, Juno M. Lu, Xun Cuneo, Matthew J. Pedersen, Lars C. TI Structural characterization of the virulence factor Sda1 nuclease from Streptococcus pyogenes SO NUCLEIC ACIDS RESEARCH LA English DT Article ID GROUP-A STREPTOCOCCUS; NEUTROPHIL EXTRACELLULAR TRAPS; ACTIVE-SITE; M1T1 CLONE; CHEMICAL RESCUE; PNEUMONIAE; DNASE; ENDA; SUPERANTIGENS; INFECTIONS AB Infection by Group A Streptococcus pyogenes (GAS) is a leading cause of severe invasive disease in humans, including streptococcal toxic shock syndrome and necrotizing fasciitis. GAS infections lead to nearly 163,000 annual deaths worldwide. Hypervirulent strains of S. pyogenes have evolved a plethora of virulence factors that aid in disease-by promoting bacterial adhesion to host cells, subsequent invasion of deeper tissues and blocking the immune system's attempts to eradicate the infection. Expression and secretion of the extracellular nuclease Sda1 is advantageous for promoting bacterial dissemination throughout the host organism, and evasion of the host's innate immune response. Here we present two crystal structures of Sda1, as well as biochemical studies to address key structural features and surface residues involved in DNA binding and catalysis. In the active site, Asn211 is observed to directly chelate a hydrated divalent metal ion and Arg124, on the putative substrate binding loop, likely stabilizes the transition state during phosphodiester bond cleavage. These structures provide a foundation for rational drug design of small molecule inhibitors to be used in prevention of invasive streptococcal disease. C1 [Moon, Andrea F.; Krahn, Juno M.; Pedersen, Lars C.] NIEHS, Genome Integr & Struct Biol Lab, NIH, POB 12233, Res Triangle Pk, NC 27709 USA. [Lu, Xun; Cuneo, Matthew J.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Moon, AF (reprint author), NIEHS, Genome Integr & Struct Biol Lab, NIH, POB 12233, Res Triangle Pk, NC 27709 USA. EM moon@niehs.nih.gov FU Division of Intramural Research of the National Institute of Environmental Health Sciences; National Institutes of Health [1ZIA ES102645-03]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Office of Biological and Environmental Research FX Division of Intramural Research of the National Institute of Environmental Health Sciences; National Institutes of Health Grant 1ZIA ES102645-03 (to L.C.P.); US Department of Energy, Office of Science, Office of Basic Energy Sciences Contract W-31-109-Eng-38. The research at the Spallation Neutron Source at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Office of Biological and Environmental Research supported the research at Oak Ridge National Laboratory's Center for Structural Molecular Biology (CSMB) using facilities supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 35 TC 0 Z9 0 U1 10 U2 12 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD MAY 5 PY 2016 VL 44 IS 8 BP 3946 EP 3957 DI 10.1093/nar/gkw143 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DM5KX UT WOS:000376389000045 PM 26969731 ER PT J AU Mankos, M Persson, HHJ N'Diaye, AT Shadman, K Schmid, AK Davis, RW AF Mankos, Marian Persson, Henrik H. J. N'Diaye, Alpha T. Shadman, Khashayar Schmid, Andreas K. Davis, Ronald W. TI Nucleotide-Specific Contrast for DNA Sequencing by Electron Spectroscopy SO PLOS ONE LA English DT Article ID MOLECULE; GOLD; ELASTICITY; MODELS AB DNA sequencing by imaging in an electron microscope is an approach that holds promise to deliver long reads with low error rates and without the need for amplification. Earlier work using transmission electron microscopes, which use high electron energies on the order of 100 keV, has shown that low contrast and radiation damage necessitates the use of heavy atom labeling of individual nucleotides, which increases the read error rates. Other prior work using scattering electrons with much lower energy has shown to suppress beam damage on DNA. Here we explore possibilities to increase contrast by employing two methods, X-ray photoelectron and Auger electron spectroscopy. Using bulk DNA samples with monomers of each base, both methods are shown to provide contrast mechanisms that can distinguish individual nucleotides without labels. Both spectroscopic techniques can be readily implemented in a low energy electron microscope, which may enable label-free DNA sequencing by direct imaging. C1 [Mankos, Marian; Shadman, Khashayar] Electron Opt Inc, 1000 Elwell Court 110, Palo Alto, CA 94303 USA. [Persson, Henrik H. J.; Davis, Ronald W.] Stanford Univ, Stanford Genome Technol Ctr, Sch Med, 855 Calif Ave, Palo Alto, CA 94304 USA. [N'Diaye, Alpha T.; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, NCEM, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Mankos, M (reprint author), Electron Opt Inc, 1000 Elwell Court 110, Palo Alto, CA 94303 USA. EM marian@electronoptica.com FU National Human Genome Research Institute (NHGRI) [R43HG006303]; US National Institutes of Health [HG000205]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX This project was supported by grant number R43HG006303 from the National Human Genome Research Institute (NHGRI). HP and RD were supported in part by US National Institutes of Health grant HG000205. Portions of this work were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; This project was supported by Grant Number R43HG006303 from the National Human Genome Research Institute (NHGRI). H. H. J. Persson and R. W. Davis were supported in part by US National Institutes of Health grant HG000205. Portions of this work were performed at the Molecular Foundry, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The content is solely the responsibility of the authors and does not necessarily represent the official views of the NHGRI or the National Institutes of Health. The authors would also like to thank T.H.P. Chang for his continuous support and numerous suggestions leading to this paper. NR 24 TC 0 Z9 0 U1 5 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 5 PY 2016 VL 11 IS 5 AR e0154707 DI 10.1371/journal.pone.0154707 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL5KV UT WOS:000375676800050 PM 27149617 ER PT J AU Stewart-Jones, GBE Soto, C Lemmin, T Chuang, GY Druz, A Kong, R Thomas, PV Wagh, K Zhou, TQ Behrens, AJ Bylund, T Choi, CW Davison, JR Georgiev, IS Joyce, MG Do Kwon, Y Pancera, M Taft, J Yang, YP Zhang, BS Shivatare, SS Shivatare, VS Lee, CCD Wu, CY Bewley, CA Burton, DR Koff, WC Connors, M Crispin, M Baxa, U Korber, BT Wong, CH Mascola, JR Kwong, PD AF Stewart-Jones, Guillaume B. E. Soto, Cinque Lemmin, Thomas Chuang, Gwo-Yu Druz, Aliaksandr Kong, Rui Thomas, Paul V. Wagh, Kshitij Zhou, Tongqing Behrens, Anna-Janina Bylund, Tatsiana Choi, Chang W. Davison, Jack R. Georgiev, Ivelin S. Joyce, M. Gordon Do Kwon, Young Pancera, Marie Taft, Justin Yang, Yongping Zhang, Baoshan Shivatare, Sachin S. Shivatare, Vidya S. Lee, Chang-Chun D. Wu, Chung-Yi Bewley, Carole A. Burton, Dennis R. Koff, Wayne C. Connors, Mark Crispin, Max Baxa, Ulrich Korber, Bette T. Wong, Chi-Huey Mascola, John R. Kwong, Peter D. TI Trimeric HIV-1-Env Structures Define Glycan Shields from Clades A, B, and G SO CELL LA English DT Article ID BROADLY NEUTRALIZING ANTIBODIES; CRYO-EM STRUCTURE; HIV-ANTIBODIES; ENVELOPE TRIMER; CRYSTAL-STRUCTURE; VACCINE DESIGN; ENV; GLYCOPROTEIN; RECOGNITION; POTENT AB The HIV-1-envelope (Env) trimer is covered by a glycan shield of similar to 90 N-linked oligosaccharides, which comprises roughly half its mass and is a key component of HIV evasion from humoral immunity. To understand how antibodies can overcome the barriers imposed by the glycan shield, we crystallized fully glycosylated Env trimers from clades A, B, and G, visualizing the shield at 3.4-3.7 angstrom resolution. These structures reveal the HIV-1-glycan shield to comprise a network of interlocking oligosaccharides, substantially ordered by glycan crowding, that encase the protein component of Env and enable HIV-1 to avoid most antibody-mediated neutralization. The revealed features delineate a taxonomy of N-linked glycan-glycan interactions. Crowded and dispersed glycans are differently ordered, conserved, processed, and recognized by antibody. The structures, along with glycan-array binding and molecular dynamics, reveal a diversity in oligosaccharide affinity and a requirement for accommodating glycans among known broadly neutralizing antibodies that target the glycan-shielded trimer. C1 [Stewart-Jones, Guillaume B. E.; Soto, Cinque; Lemmin, Thomas; Chuang, Gwo-Yu; Druz, Aliaksandr; Kong, Rui; Thomas, Paul V.; Zhou, Tongqing; Bylund, Tatsiana; Choi, Chang W.; Georgiev, Ivelin S.; Joyce, M. Gordon; Do Kwon, Young; Pancera, Marie; Taft, Justin; Yang, Yongping; Zhang, Baoshan; Mascola, John R.; Kwong, Peter D.] NIAID, Vaccine Res Ctr, NIH, 9000 Rockville Pike, Bethesda, MD 20892 USA. [Lemmin, Thomas] Univ Calif San Francisco, Dept Pharmaceut Chem, San Francisco, CA 94143 USA. [Wagh, Kshitij; Korber, Bette T.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, POB 1663, Los Alamos, NM 87544 USA. [Behrens, Anna-Janina; Crispin, Max] Univ Oxford, Dept Biochem, Oxford Glycobiol Inst, S Parks Rd, Oxford OX1 3QU, England. [Davison, Jack R.; Bewley, Carole A.] NIDDK, Bioorgan Chem Lab, NIH, Bethesda, MD 20892 USA. [Shivatare, Sachin S.; Shivatare, Vidya S.; Lee, Chang-Chun D.; Wu, Chung-Yi; Wong, Chi-Huey] Acad Sinica, Genom Res Ctr, 128 Acad Rd,Sect 2, Taipei 115, Taiwan. [Burton, Dennis R.] Scripps Res Inst, Dept Immunol & Microbial Sci, Int AIDS Vaccine Initiat Neutralizing Antibody Ct, Ctr HIV AIDS Vaccine Immunol & Immunogen Discover, La Jolla, CA 92037 USA. [Burton, Dennis R.] Ragon Inst Massachusetts Gen Hosp Massachusetts I, Boston, MA 02142 USA. [Koff, Wayne C.] Int AIDS Vaccine Initiat, New York, NY 10038 USA. [Connors, Mark] NIAID, HIV Specif Immun Sect, Immunoregulat Lab, NIH, 9000 Rockville Pike, Bethesda, MD 20892 USA. [Baxa, Ulrich] Leidos Biomed Res Inc, Frederick Natl Lab Canc Res, Canc Res Technol Program, Electron Microscopy Lab, Ft Detrick, MD 21702 USA. [Wong, Chi-Huey] Scripps Res Inst, Dept Chem, La Jolla, CA 92037 USA. RP Kwong, PD (reprint author), NIAID, Vaccine Res Ctr, NIH, 9000 Rockville Pike, Bethesda, MD 20892 USA. EM pdkwong@nih.gov RI Kwon, Young Do/A-6957-2010; Zhou, Tongqing/A-6880-2010; OI Zhou, Tongqing/0000-0002-3935-4637; Korber, Bette/0000-0002-2026-5757; Davison, Jack/0000-0002-6803-304X FU Intramural Research Program of the Vaccine Research Center; National Institute of Allergy and Infectious Diseases; National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health (NIH); International AIDS Vaccine Initiative's (IAVI's) Neutralizing Antibody Consortium; Bill & Melinda Gates Foundation; Ministry of Foreign Affairs of Denmark; Irish Aid; Ministry of Finance of Japan; Ministry of Foreign Affairs of the Netherlands; Norwegian Agency for Development Cooperation; UK Department for International Development; United States Agency for International Development (USAID); International AIDS Vaccine Initiative Neutralizing Antibody Center CAVD grant; Scripps Center For HIV/AIDS Vaccine Immunology-Immunogen Discovery (CHAVI-ID) grant [1UM1AI100663]; Duke CHAVI-ID grant [UM1 AI100645]; Swiss National Foundation of Science Fellowship [148914]; Academia Sinica; Ministry of Science and Technology [MOST 104-0210-01-09-02, 103-2321-B-001-004]; NIH [R01 AI072155]; US Department of Energy, Basic Energy Sciences, Office of Science [W-31-109-Eng-38]; [HHSN261200800001E] FX We thank R. O'Connor for NMR support, J. Stuckey for assistance with graphics, and members of the Structural Biology Section and Structural Bioinformatics Core, Vaccine Research Center for discussions and comments on the manuscript. We thank Acellera for assistance with molecular dynamics simulations. Support for this work was provided by the Intramural Research Program of the Vaccine Research Center, National Institute of Allergy and Infectious Diseases and the National Institute of Diabetes and Digestive and Kidney Diseases, National Institutes of Health (NIH), and from the International AIDS Vaccine Initiative's (IAVI's) Neutralizing Antibody Consortium. IAVI's work is made possible by support from many donors, including the Bill & Melinda Gates Foundation; the Ministry of Foreign Affairs of Denmark; Irish Aid; the Ministry of Finance of Japan; the Ministry of Foreign Affairs of the Netherlands; the Norwegian Agency for Development Cooperation; the UK Department for International Development; and the United States Agency for International Development (USAID). The contents of this manuscript do not necessarily reflect the views of USAID or the US Government. The full list of IAVI donors is available at http://www.iavi.org. A.-J.B. and M. Crispin were supported by the International AIDS Vaccine Initiative Neutralizing Antibody Center CAVD grant (Glycan characterization and Outer Domain glycoform design) and the Scripps Center For HIV/AIDS Vaccine Immunology-Immunogen Discovery (CHAVI-ID) grant 1UM1AI100663. K.W. and B.K. were supported by the Duke CHAVI-ID grant UM1 AI100645. T.L. was supported by the Swiss National Foundation of Science Fellowship 148914. V.S.S., C.-C.D.L., C.-Y.W., and C.-H.W. were supported by Academia Sinica and Ministry of Science and Technology grants MOST 104-0210-01-09-02 and 103-2321-B-001-004. C.-H.W. was supported by NIH grant R01 AI072155. The Frederick National Laboratory for Cancer Research, National Institutes of Health, is supported under contract HHSN261200800001E. Use of sector 22 (Southeast Region Collaborative Access team) at the Advanced Photon Source was supported by the US Department of Energy, Basic Energy Sciences, Office of Science, under contract number W-31-109-Eng-38. NR 46 TC 37 Z9 37 U1 12 U2 20 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD MAY 5 PY 2016 VL 165 IS 4 BP 813 EP 826 DI 10.1016/j.cell.2016.04.010 PG 14 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DL7DN UT WOS:000375800300011 PM 27114034 ER PT J AU Upshur, MA Chase, HM Strick, BF Ebben, CJ Fu, L Wang, HF Thomson, RJ Geiger, FM AF Upshur, Mary Alice Chase, Hilary M. Strick, Benjamin F. Ebben, Carlena J. Fu, Li Wang, Hongfei Thomson, Regan J. Geiger, Franz M. TI Vibrational Mode Assignment of alpha-Pinene by Isotope Editing: One Down, Seventy-One To Go SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SUM-FREQUENCY GENERATION; SECONDARY ORGANIC AEROSOL; HETEROGENEOUS CATALYSIS; SURFACE SCIENCE; ENVIRONMENTAL INTERFACES; HIGH-PRESSURES; SPECTROSCOPY; ORIENTATION; PARTICLES; CHEMISTRY AB This study aims to reliably assign the vibrational sum frequency generation (SFG) spectrum of alpha-pinene at the vapor/solid interface using a method involving deuteration of various methyl groups. The synthesis of five deuterated isotopologues of alpha-pinene is presented to determine the impact that removing contributions from methyl group C-H oscillators has on its SFG response. 0.6 cm(-1) resolution SFG spectra of these isotopologues show varying degrees of differences in the C-H stretching region when compared to the SFG response of unlabeled alpha-pinene. The largest spectral changes were observed for the isotopologue containing a fully deuterated vinyl methyl group. Noticeable losses in signal intensities allow us to reliably assign the 2860 cm(-1) peak to the vinyl methyl symmetric stretch. Furthermore, upon removing the vinyl methyl group entirely by synthesizing apopinene, the steric influence of the unlabeled C9H14 fragment on the SFG response of alpha-pinene SFG can be readily observed. The work presented here brings us one step closer to understanding the vibrational spectroscopy of alpha-pinene. C1 [Upshur, Mary Alice; Chase, Hilary M.; Strick, Benjamin F.; Ebben, Carlena J.; Thomson, Regan J.; Geiger, Franz M.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Fu, Li; Wang, Hongfei] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. [Ebben, Carlena J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Thomson, RJ; Geiger, FM (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM r-thomson@northwestern.edu; geigerf@chem.northwestem.edu RI Wang, Hongfei/B-1263-2010 OI Wang, Hongfei/0000-0001-8238-1641 FU Initiative for Sustainability and Energy at Northwestern (ISEN); National Science Foundation [CHE 1212692]; National Aeronautics and Space Administration Earth and Space (NASA ESS) Fellowship; National Science Foundation (NSF) Graduate Research Fellowship (NSF-GRFP); NSF-GRFP; U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER) [47891] FX We gratefully acknowledge support from the Initiative for Sustainability and Energy at Northwestern (ISEN) and the National Science Foundation (CHE 1212692 to R.J.T. and F.M.G.). M.A.U. gratefully acknowledges support from a National Aeronautics and Space Administration Earth and Space (NASA ESS) Fellowship and a National Science Foundation (NSF) Graduate Research Fellowship (NSF-GRFP). H.M.C. acknowledges support from the NSF-GRFP. Part of this work was conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at the Pacific Northwest National Laboratory and sponsored by the U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER) under user Grant No. 47891. NR 57 TC 3 Z9 3 U1 9 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 5 PY 2016 VL 120 IS 17 BP 2684 EP 2690 DI 10.1021/acs.jpca.6b01995 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL4TX UT WOS:000375631500009 PM 27063197 ER PT J AU Lindquist, BA Takeshita, TY Dunning, TH AF Lindquist, Beth A. Takeshita, Tyler Y. Dunning, Thom H., Jr. TI Insights into the Electronic Structure of Ozone and Sulfur Dioxide from Generalized Valence Bond Theory: Addition of Hydrogen Atoms SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CORRELATED MOLECULAR CALCULATIONS; POTENTIAL-ENERGY SURFACE; GAUSSIAN-BASIS SETS; TRIOXIDE HOOOH; 1,3-DIPOLAR CYCLOADDITION; COUPLED-CLUSTER; WAVE-FUNCTIONS; REACTIVITY; MECHANISMS; CHEMISTRY AB Ozone (O-3) and sulfur dioxide (SO2) are valence isoelectronic species, yet their properties and reactivities differ dramatically. In particular, O-3 is highly reactive, whereas SO2 is chemically relatively stable. In this paper, we investigate serial addition of hydrogen atoms to both the terminal atoms of O-3 and SO2 and to the central atom of these species. It is well-known that the terminal atoms of O-3 are much more amenable to bond formation than those of SO2. We show that the differences in the electronic structure of the pi systems in the parent triatomic species account for the differences in the addition of hydrogen atoms to the terminal atoms of O-3 and SO2. Further, we find that the pi system in SO2, which is a recoupled pair bond dyad, facilitates the addition of hydrogen atoms to the sulfur atom, resulting in stable HSO2 and H2SO2 species. C1 [Lindquist, Beth A.; Takeshita, Tyler Y.; Dunning, Thom H., Jr.] Univ Illinois, Dept Chem, 600 S Mathews Ave, Urbana, IL 61801 USA. [Lindquist, Beth A.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Takeshita, Tyler Y.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Dunning, Thom H., Jr.] Univ Washington, Pacific NW Natl Lab, Northwest Inst Adv Comp, Seattle, WA 98195 USA. [Dunning, Thom H., Jr.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. RP Dunning, TH (reprint author), Univ Washington, Pacific NW Natl Lab, Northwest Inst Adv Comp, Seattle, WA 98195 USA.; Dunning, TH (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM thdjr@illinois.edu FU Distinguished Chair for Research Excellence in Chemistry; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; National Science Foundation Graduate Research Fellowship FX This work was supported by funds from the Distinguished Chair for Research Excellence in Chemistry and the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign. One of the authors (B.A.L.) is the grateful recipient of a National Science Foundation Graduate Research Fellowship. NR 45 TC 0 Z9 0 U1 9 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAY 5 PY 2016 VL 120 IS 17 BP 2720 EP 2726 DI 10.1021/acs.jpca.6b02014 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL4TX UT WOS:000375631500013 PM 27070292 ER PT J AU Pang, ZQ Duerrbeck, S Kha, C Bertel, E Somorjai, GA Salmeron, M AF Pang, Zongqiang Duerrbeck, Stefan Kha, Calvin Bertel, Erminald Somorjai, Gabor A. Salmeron, Miquel TI Adsorption and Reactions of Water on Oxygen-Precovered Cu(110) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; SURFACE; DISSOCIATION; H2O; CHEMISORPTION; CO AB Using scanning tunneling microscopy we studied the adsorption and reactions of water on a Cu(110) surface partially covered with oxygen in the O(2 X 1) phase formed by Cu-O chains. The experiments were carried out from low (77 K) to higher temperatures to sequentially open reaction channels that require increased activation energy. At 77 K, water adsorbs at the edges and on top of the Cu-O chains. Heating to 155 K caused water molecules to react with the oxygen atoms in the chains to produce OH. These hydroxyl groups form elongated H-bonded structures mixed with excess unreacted water molecules. The Cu atoms freed in the reaction form small clusters at the location of the initial Cu-O chains. Heating to 180 K leads to a second reaction that desorbs all excess water (i.e., water not H-bonded with OH), leaving H2O-OH zigzag chains along [110] directions. At the low oxygen coverage studied here (<0.12 ML) the extent of the partial water dissociation reaction is stoichiometrically determined by the amount of preadsorbed oxygen (H2O + O -> 2OH). A third annealing to 280 K resulted in desorption of all water and hydroxyl species and the reappearance of Cu-O chains. After heating to 280 K, the oxygen coverage returns to nearly the same value as that of the initially surface. C1 [Pang, Zongqiang; Duerrbeck, Stefan; Kha, Calvin; Somorjai, Gabor A.; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Pang, Zongqiang] Nanjing Univ Posts & Telecommun, Coll Automat, Nanjing 210023, Jiangsu, Peoples R China. [Duerrbeck, Stefan; Bertel, Erminald] Univ Innsbruck, Inst Phys Chem, A-6020 Innsbruck, Austria. [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Salmeron, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov OI Bertel, Erminald/0000-0002-9006-8222 FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231, FWP KC3101]; Jiangsu Province Natural Science Fund [BK20140862]; University of Innsbruck FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures Program (FWP KC3101). Z.P. was supported by the Jiangsu Province Natural Science Fund under Grant No. BK20140862. S.D. acknowledges support by the University of Innsbruck. NR 22 TC 3 Z9 3 U1 6 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 5 PY 2016 VL 120 IS 17 BP 9218 EP 9222 DI 10.1021/acs.jpcc.6b00769 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL4TV UT WOS:000375631100024 ER PT J AU Kestell, J Walker, J Bai, Y Boscoboinik, JA Garvey, M Tysoe, WT AF Kestell, John Walker, Joshua Bai, Yun Boscoboinik, J. Anibal Garvey, Michael Tysoe, Wilfred T. TI Adsorption and Oligomerization of 1,3-Phenylene Diisocyanide on Au(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; 1,4-PHENYLENE DIISOCYANIDE; BASIS-SET; GOLD; ISOCYANIDES; ADATOMS; SURFACE; SPECTROSCOPY; PALLADIUM AB The adsorption and self-assembly of 1,3-phenylene diisocyanide (1,3-PDI) are studied on Au(111) using reflection adsorption infrared spectroscopy (RAIRS), scanning tunneling microscopy (STM), and temperature-programmed desorption (TPD) supplemented by density functional theory (DFT) calculations and the results compared with the structures formed from 1,4-PDI where it assembled to form (Au PDI) oligomer chains that incorporate gold adatoms. The infrared spectra display a single isocyanide feature consistent with the isocyanide binding to gold adatoms, while DFT calculations confirm that isocyanide binding to gold adatoms is more energetically favorable than binding to the surface. STM images show that 1,3-PDI forms zigzag chains containing hairpin bends that cause the chains to double back on each other, consistent with the 120 angle between the isocyanide groups. Hexagonal structural motifs are also observed that are proposed to be due to the self-assembly of three isocyanides as well as small structures that are assigned to 1,3-PDI dimers. The results suggest that the formation of gold-containing oligomers from isocyanide-containing molecules is a general phenomenon. C1 [Kestell, John; Walker, Joshua; Bai, Yun; Boscoboinik, J. Anibal; Garvey, Michael; Tysoe, Wilfred T.] Univ Wisconsin, Dept Chem & Biochem, Milwaukee, WI 53211 USA. [Kestell, John; Walker, Joshua; Bai, Yun; Boscoboinik, J. Anibal; Garvey, Michael; Tysoe, Wilfred T.] Univ Wisconsin, Surface Studies Lab, Milwaukee, WI 53211 USA. [Kestell, John; Boscoboinik, J. Anibal] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Garvey, Michael] Univ Illinois, Appl Res Inst, Champaign, IL 61820 USA. RP Tysoe, WT (reprint author), Univ Wisconsin, Dept Chem & Biochem, Milwaukee, WI 53211 USA.; Tysoe, WT (reprint author), Univ Wisconsin, Surface Studies Lab, Milwaukee, WI 53211 USA. EM wtt@uwm.edu NR 34 TC 0 Z9 0 U1 6 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 5 PY 2016 VL 120 IS 17 BP 9270 EP 9275 DI 10.1021/acs.jpcc.6b01613 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL4TV UT WOS:000375631100031 ER PT J AU Neeway, JJ Kerisit, SN Liu, J Zhang, JD Zhu, ZH Riley, BJ Ryan, JV AF Neeway, James Joseph Kerisit, Sebastien N. Liu, Jia Zhang, Jiandong Zhu, Zihua Riley, Brian Joseph Ryan, Joseph Vincent TI Ion-Exchange Interdiffusion Model with Potential Application to Long-Term Nuclear Waste Glass Performance SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MONTE-CARLO SIMULATIONS; BOROSILICATE GLASS; NA2O-AL2O3-SIO2 GLASS; SURFACE-LAYERS; GRAAL MODEL; CORROSION; WATER; DISSOLUTION; DIFFUSION; MECHANISMS AB Ion exchange and interdiffusion are critical processes in glass applications. In the field of aqueous glass corrosion, it is difficult to conclusively deconvolute the process of ion exchange from other processes, principally dissolution of the glass matrix, due to the formation of alteration layers, Therefore, we have developed a method to isolate alkali diffusion that involves contacting glass coupons with a solution of (LiCl)-Li-6 dissolved in functionally inert dimethyl sulfoxide. We employ the method at temperatures ranging from 25 to 150 degrees C with various glass compositions. Glass compositions include simulant nuclear waste glasses, such as SON68 and the ISG, glasses in which the nature of the alkali element was varied, and glasses that contained more than one alkali element. An interdiffusion model based on Fick's second law was developed and applied to all experiments to extract diffusion coefficients. The model expands established models of interdiffusion to the case where multiple types of alkali sites are present in the glass. Activation energies for alkali ion diffusion were calculated. The interdiffusion model derived from laboratory experiments is expected to be useful for modeling glass corrosion in a geological repository when silicon concentrations are high. C1 [Neeway, James Joseph; Riley, Brian Joseph; Ryan, Joseph Vincent] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Kerisit, Sebastien N.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Liu, Jia; Zhang, Jiandong; Zhu, Zihua] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Neeway, JJ (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM james.neeway@pnnl.gov RI Zhu, Zihua/K-7652-2012; OI Neeway, Jim/0000-0001-7046-8408; Riley, Brian/0000-0002-7745-6730 FU U.S. Department of Energy (DOE) through the Office of Nuclear Energy; DOE [DE-AC06-76RLO 1830]; U.S. Department of Energy's Office of Biological and Environmental Research FX These studies were supported by the U.S. Department of Energy (DOE) through the Office of Nuclear Energy. We would like to thank Dr. Stephane Gin of the CEA for useful discussions and for supplying the CJ-6 glass. We also thank Dr. Peter Rieke (PNNL) for his help in improving the manuscript, Jodi Mayer (PNNL) and Carmen Rodriguez (PNNL) for help in glass fabrication, and Clyde Chamberlin (PNNL) for help in sample preparation. Pacific Northwest National Laboratory is operated for the DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. The research described in this paper was performed in part in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory in Richland, WA. NR 51 TC 2 Z9 2 U1 5 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAY 5 PY 2016 VL 120 IS 17 BP 9374 EP 9384 DI 10.1021/acs.jpcc.6b03681 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL4TV UT WOS:000375631100044 ER PT J AU Weatherup, RS Eren, B Hao, YB Bluhm, H Salmeron, MB AF Weatherup, Robert S. Eren, Baran Hao, Yibo Bluhm, Hendrik Salmeron, Miquel B. TI Graphene Membranes for Atmospheric Pressure Photoelectron Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID HEXAGONAL BORON-NITRIDE; ELECTRON-MICROSCOPY; IN-SITU; POLYCRYSTALLINE CU; LIQUID CELLS; HIGH-QUALITY; INTERFACES; CVD; OXYGEN; CATALYSTS AB Atmospheric pressure X-ray photoelectron spectroscopy (XPS) is demonstrated using single-layer graphene membranes as photoelectron-transparent barriers that sustain pressure differences in excess of 6 orders of magnitude. The graphene serves as a support for catalyst nanoparticles under atmospheric pressure reaction conditions (up to 1.5 bar), where XPS allows the oxidation state of Cu nanoparticles and gas phase species to be simultaneously probed. We thereby observe that the Cu2+ oxidation state is stable in O-2 (1 bar) but is spontaneously reduced under vacuum. We further demonstrate the detection of various gas-phase species (Ar, CO, CO2, N-2, O-2) in the pressure range 10-1500 mbar including species with low photoionization cross sections (He, H-2). Pressure-dependent changes in the apparent binding energies of gas-phase species are observed, attributable to changes in work function of the metal-coated grids supporting the graphene. We expect atmospheric pressure XPS based on this graphene membrane approach to be a valuable tool for studying nanoparticle catalysis. C1 [Weatherup, Robert S.; Eren, Baran; Hao, Yibo; Salmeron, Miquel B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Salmeron, Miquel B.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, MB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Salmeron, MB (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov RI Eren, Baran/A-9644-2013; Weatherup, Robert/O-5725-2016 OI Weatherup, Robert/0000-0002-3993-9045 FU St. John's College, Cambridge; Marie Sklodowska-Curie Individual Fellowship (Global) under grant ARTIST from the European Union [656870]; Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX We are grateful to Ed Wong of the Molecular Foundry for his assistance in fabricating the gas cell. RSW acknowledges a Research Fellowship from St. John's College, Cambridge and a Marie Sklodowska-Curie Individual Fellowship (Global) under grant ARTIST (no. 656870) from the European Union's Horizon 2020 research and innovation programme. This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) under Contract DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program and through work performed at the Advanced Light Source and Molecular Foundry user facilities of the DOE Office of Basic Energy Sciences. HB acknowledges support by the Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences of the U.S. Department of Energy (DOE) under Contract DE-AC02-05CH11231. NR 37 TC 5 Z9 5 U1 19 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2016 VL 7 IS 9 BP 1622 EP 1627 DI 10.1021/acs.jpclett.6b00640 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DL4WM UT WOS:000375638500004 PM 27082434 ER PT J AU Cantu, DC Lee, J Lee, MS Heldebrant, DJ Koech, PK Freeman, CJ Rousseau, R Glezakou, VA AF Cantu, David C. Lee, Juntaek Lee, Mal-Soon Heldebrant, David J. Koech, Phillip K. Freeman, Charles J. Rousseau, Roger Glezakou, Vassiliki-Alexandra TI Dynamic Acid/Base Equilibrium in Single Component Switchable Ionic Liquids and Consequences on Viscosity SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CO2 CAPTURE; MOLECULAR-DYNAMICS; CARBON-DIOXIDE; REACTION-MECHANISM; AQUEOUS-SOLUTIONS; SOLVENT SYNTHESIS; ORGANIC LIQUIDS; KINETICS; ABSORPTION; SIMULATION AB The deployment of transformational nonaqueous CO2-capture solvent systems is encumbered by high viscosities even at intermediate uptakes. Using single-molecule CO2 binding organic liquids as a prototypical example, we present key molecular features that control bulk viscosity. Fast CO2-uptake kinetics arise from close proximity of the alcohol and amine sites involved in CO2 binding in a concerted fashion, resulting in a Zwitterion containing both an alkyl-carbonate and a protonated amine. The population of internal hydrogen bonds between the two functional groups determines the solution viscosity. Unlike the ion pair interactions in ionic liquids, these observations are novel and specific to a hydrogen-bonding network that can be controlled by chemically tuning single molecule CO2 capture solvents. We present a molecular design strategy to reduce viscosity by shifting the proton transfer equilibrium toward a neutral acid/amine species, as opposed to the ubiquitously accepted zwitterionic state. The molecular design concepts proposed here are readily extensible to other CO2 capture technologies. C1 [Cantu, David C.; Lee, Mal-Soon; Rousseau, Roger; Glezakou, Vassiliki-Alexandra] Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99352 USA. [Lee, Juntaek; Heldebrant, David J.; Koech, Phillip K.; Freeman, Charles J.] Pacific NW Natl Lab, Energy Proc & Mat Div, Richland, WA 99352 USA. RP Glezakou, VA (reprint author), Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99352 USA. EM Vanda.Glezakou@pnnl.gov RI Rousseau, Roger/C-3703-2014; OI Koech, Phillip/0000-0003-2996-0593; Lee, Mal-Soon/0000-0001-6851-177X FU U.S. Department of Energy's Office of Fossil Energy [FWP-65872] FX The authors wish to dedicate this paper to Prof. M. Parrinello on the occasion of this 70th birthday. May his creativity, unstoppable innovation, and limitless enthusiasm continue to inspire many more generations of scientists. We gratefully acknowledge the U.S. Department of Energy's Office of Fossil Energy for funding through award FWP-65872. Computational resources were provided through a NERSC User Proposal. PNNL is proudly operated by Battelle for the U.S. Department of Energy. The authors wish to thank Mr. T. Brouns for his constant support of this work, as well as the editor Prof. B. Mennucci and the reviewers for their insightful comments and criticisms. NR 49 TC 3 Z9 3 U1 18 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2016 VL 7 IS 9 BP 1646 EP 1652 DI 10.1021/acs.jpclett.6b00395 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DL4WM UT WOS:000375638500008 PM 27019342 ER PT J AU Simpson, MJ Doughty, B Yang, B Xiao, K Ma, YZ AF Simpson, Mary Jane Doughty, Benjamin Yang, Bin Xiao, Kai Ma, Ying-Zhong TI Imaging Electronic Trap States in Perovskite Thin Films with Combined Fluorescence and Femtosecond Transient Absorption Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SOLAR-CELLS; CARRIER DYNAMICS; CHARGE-CARRIERS; HALIDE PEROVSKITES; RECOMBINATION; CH3NH3PBI3; PLANAR; SEPARATION; EFFICIENCY; TRANSPORT AB Charge carrier trapping degrades the performance of organometallic halide perovskite solar cells. To characterize the locations of electronic trap states in a heterogeneous photoactive layer, a spatially resolved approach is essential. Here, we report a comparative study on methylammonium lead tri-iodide perovskite thin films subject to different thermal annealing times using a combined photoluminescence (PL) and femtosecond transient absorption microscopy (TAM) approach to spatially map trap states. This approach coregisters the initially populated electronic excited states with the regions that recombine radiatively. Although the TAM images are relatively homogeneous for both samples, the corresponding PL images are highly structured. The remarkable variation in the PL intensities as compared to transient absorption signal amplitude suggests spatially dependent PL quantum efficiency, indicative of trapping events. Detailed analysis enables identification of two trapping regimes: a densely packed trapping region and a sparse trapping area that appear as unique spatial features in scaled PL maps. C1 [Simpson, Mary Jane; Doughty, Benjamin; Ma, Ying-Zhong] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Yang, Bin; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Ma, YZ (reprint author), Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. EM may1@ornl.gov RI Yang, Bin/P-8529-2014; Ma, Yingzhong/L-6261-2016; Doughty, Benjamin /M-5704-2016 OI Yang, Bin/0000-0002-5667-9126; Ma, Yingzhong/0000-0002-8154-1006; Doughty, Benjamin /0000-0001-6429-9329 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX Work by M.J.S., B.D., and Y.-Z.M. was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Perovskite sample preparation and SEM characterization by B.Y. and K.X. were conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 39 TC 3 Z9 3 U1 13 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAY 5 PY 2016 VL 7 IS 9 BP 1725 EP 1731 DI 10.1021/acs.jpclett.6b00715 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DL4WM UT WOS:000375638500022 PM 27103096 ER PT J AU Kim, TH Puggioni, D Yuan, Y Xie, L Zhou, H Campbell, N Ryan, PJ Choi, Y Kim, JW Patzner, JR Ryu, S Podkaminer, JP Irwin, J Ma, Y Fennie, CJ Rzchowski, MS Pan, XQ Gopalan, V Rondinelli, JM Eom, CB AF Kim, T. H. Puggioni, D. Yuan, Y. Xie, L. Zhou, H. Campbell, N. Ryan, P. J. Choi, Y. Kim, J-W Patzner, J. R. Ryu, S. Podkaminer, J. P. Irwin, J. Ma, Y. Fennie, C. J. Rzchowski, M. S. Pan, X. Q. Gopalan, V. Rondinelli, J. M. Eom, C. B. TI Polar metals by geometric design SO NATURE LA English DT Article ID AUGMENTED-WAVE METHOD; IMPROPER FERROELECTRICITY; PEROVSKITE NICKELATE; THIN-FILMS; SUPERLATTICES; TRANSITION; OXIDES; ROUTE AB Gauss's law dictates that the net electric field inside a conductor in electrostatic equilibrium is zero by effective charge screening; free carriers within a metal eliminate internal dipoles that may arise owing to asymmetric charge distributions(1). Quantum physics supports this view(2), demonstrating that delocalized electrons make a static macroscopic polarization, an ill-defined quantity in metals(3)-it is exceedingly unusual to find a polar metal that exhibits long-range ordered dipoles owing to cooperative atomic displacements aligned from dipolar interactions as in insulating phases(4). Here we describe the quantum mechanical design and experimental realization of room-temperature polar metals in thin-film ANiO(3) perovskite nickelates using a strategy based on atomic-scale control of inversion-preserving (centric) displacements(5). We predict with ab initio calculations that cooperative polar A cation displacements are geometrically stabilized with a non-equilibrium amplitude and tilt pattern of the corner-connected NiO6 octahedra-the structural signatures of perovskites-owing to geometric constraints imposed by the underlying substrate. Heteroepitaxial thin-films grown on LaAlO3 (111) substrates fulfil the design principles. We achieve both a conducting polar monoclinic oxide that is inaccessible in compositionally identical films grown on (001) substrates, and observe a hidden, previously unreported(6-10), non-equilibrium structure in thin-film geometries. We expect that the geometric stabilization approach will provide novel avenues for realizing new multifunctional materials with unusual coexisting properties. C1 [Kim, T. H.; Patzner, J. R.; Ryu, S.; Podkaminer, J. P.; Ma, Y.; Eom, C. B.] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Puggioni, D.; Rondinelli, J. M.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Yuan, Y.; Gopalan, V.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Yuan, Y.; Gopalan, V.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Xie, L.; Pan, X. Q.] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA. [Xie, L.; Pan, X. Q.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Xie, L.] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Xie, L.] Nanjing Univ, Coll Engn & Appl Sci, Nanjing 210093, Jiangsu, Peoples R China. [Zhou, H.; Ryan, P. J.; Choi, Y.; Kim, J-W] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Campbell, N.; Irwin, J.; Rzchowski, M. S.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Fennie, C. J.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. RP Eom, CB (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM ceom@wisc.edu RI Rondinelli, James/A-2071-2009; Zhou, Hai/B-7331-2009; OI Rondinelli, James/0000-0003-0508-2175; Irwin, Julian/0000-0002-4845-7558 FU National Science Foundation (NSF) under Designing Materials to Revolutionize and Engineer our Future grant [DMR-1234096]; US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) [DE-FG02-06ER46327]; DOE-BES [DE-SC0012375, DE-AC-02-06CH11357]; Army Research Office [W911NF-15-1-0017]; NSF XSEDE [ACI-1053575]; [DMR-1056441] FX This work was supported by the National Science Foundation (NSF) under Designing Materials to Revolutionize and Engineer our Future grant number DMR-1234096. Transport measurement at the University of Wisconsin-Madison was supported by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), under award number DE-FG02-06ER46327. The work at Pennsylvania State University was supported by the DOE-BES, under award number DE-SC0012375 (Y.Y., V.G.). The work at Northwestern University was supported by the Army Research Office under award numbers W911NF-15-1-0017 (J.M.R.) and DOE-BES DE-SC0012375 (D.P.). The work at the Argonne National Laboratory is supported by the DOE-BES under contract number DE-AC-02-06CH11357 (H.Z., P.J.R., Y.C., J.W.K.). The computational work made use of the Haise and Kilrain clusters at the Navy DoD Supercomputing Resource Center under the High Performance Computing Modernization Program initiative of the US Department of Defense and NSF XSEDE (ACI-1053575). The work at Cornell University was funded by DMR-1056441 (C.J.F.). NR 40 TC 13 Z9 13 U1 38 U2 91 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 5 PY 2016 VL 533 IS 7601 BP 68 EP + DI 10.1038/nature17628 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL2OE UT WOS:000375473900040 PM 27096369 ER PT J AU Qiu, JZ Sheedlo, MJ Yu, KW Tan, YH Nakayasu, ES Das, C Liu, XY Luo, ZQ AF Qiu, Jiazhang Sheedlo, Michael J. Yu, Kaiwen Tan, Yunhao Nakayasu, Ernesto S. Das, Chittaranjan Liu, Xiaoyun Luo, Zhao-Qing TI Ubiquitination independent of E1 and E2 enzymes by bacterial effectors SO NATURE LA English DT Article ID LEGIONELLA-PNEUMOPHILA; ENDOPLASMIC-RETICULUM; SUBSTRATE RECOGNITION; STRUCTURAL BASIS; CELL BIOLOGY; PROTEIN; SYSTEM; FAMILY; PHAGOSOME; REPLICATION AB Signalling by ubiquitination regulates virtually every cellular process in eukaryotes. Covalent attachment of ubiquitin to a substrate is catalysed by the E1, E2 and E3 three-enzyme cascade(1), which links the carboxy terminus of ubiquitin to the e-amino group of, in most cases, a lysine of the substrate via an isopeptide bond. Given the essential roles of ubiquitination in the regulation of the immune system, it is not surprising that the ubiquitination network is a common target for diverse infectious agents(2). For example, many bacterial pathogens exploit ubiquitin signalling using virulence factors that function as E3 ligases, deubiquitinases3 or as enzymes that directly attack ubiquitin(4). The bacterial pathogen Legionella pneumophila utilizes approximately 300 effectors that modulate diverse host processes to create a permissive niche for its replication in phagocytes(5). Here we demonstrate that members of the SidE effector family of L. pneumophila ubiquitinate multiple Rab small GTPases associated with the endoplasmic reticulum. Moreover, we show that these proteins are capable of catalysing ubiquitination without the need for the E1 and E2 enzymes. A putative mono-ADP-ribosyltransferase motif critical for the ubiquitination activity is also essential for the role of the SidE family in intracellular bacterial replication in a protozoan host. The E1/E2-independent ubiquitination catalysed by these enzymes is energized by nicotinamide adenine dinucleotide, which activates ubiquitin by the formation of ADP-ribosylated ubiquitin. These results establish that ubiquitination can be catalysed by a single enzyme, the activity of which does not require ATP. C1 [Qiu, Jiazhang; Tan, Yunhao; Luo, Zhao-Qing] Purdue Univ, Purdue Inst Inflammat Immunol & Infect Dis, W Lafayette, IN 47907 USA. [Qiu, Jiazhang; Tan, Yunhao; Luo, Zhao-Qing] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. [Sheedlo, Michael J.; Das, Chittaranjan] Purdue Univ, Dept Chem, 560 Oval Dr, W Lafayette, IN 47907 USA. [Yu, Kaiwen; Liu, Xiaoyun] Peking Univ, Inst Analyt Chem, Coll Chem & Mol Engn, Beijing 100871, Peoples R China. [Yu, Kaiwen; Liu, Xiaoyun] Peking Univ, Synthet & Funct Biomol Ctr, Coll Chem & Mol Engn, Beijing 100871, Peoples R China. [Nakayasu, Ernesto S.] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Tan, Yunhao] Harvard Univ, Sch Med, Div Gastroenterol, Boston Childrens Hosp, Boston, MA 02115 USA. RP Luo, ZQ (reprint author), Purdue Univ, Purdue Inst Inflammat Immunol & Infect Dis, W Lafayette, IN 47907 USA.; Luo, ZQ (reprint author), Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. EM luoz@purdue.edu RI Tan, Yunhao/K-7442-2016 OI Tan, Yunhao/0000-0002-5516-4980 FU National Institutes of Health [R56AI103168, K02AI085403, R21AI105714, 2R01GM103401]; National Natural Science Foundation of China [21305006, 21475005] FX We thank P. Hollenbeck (Purdue University) for critical reading of the manuscript. J. Barbieri (Medical College of Wisconsin) for plasmids. This work was supported by National Institutes of Health grants R56AI103168, K02AI085403 and R21AI105714 (Z.-Q.L.), 2R01GM103401 (C.D.) and National Natural Science Foundation of China grants 21305006 and 21475005 (X.L.). NR 40 TC 16 Z9 16 U1 8 U2 18 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAY 5 PY 2016 VL 533 IS 7601 BP 120 EP + DI 10.1038/nature17657 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL2OE UT WOS:000375473900051 PM 27049943 ER PT J AU Shintani, E Blum, T Izubuchi, T Soni, A AF Shintani, Eigo Blum, Thomas Izubuchi, Taku Soni, Amarjit CA RBC Collaborations UKQCD Collaborations TI Neutron and proton electric dipole moments from N-f=2+1 domain-wall fermion lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID STRONG CP-VIOLATION; CHIRAL PERTURBATION-THEORY; KOBAYASHI-MASKAWA MODEL; EFFECTIVE-FIELD THEORY; STANDARD MODEL; FORM-FACTOR; NUCLEON; VACUUM AB We present a lattice calculation of the neutron and proton electric dipole moments (EDMs) with N-f = 2 + 1 flavors of domain-wall fermions. The neutron and proton EDM form factors are extracted from three-point functions at the next-to-leading order in the theta vacuum of QCD. In this computation, we use pion masses of 0.33 and 0.42 GeV and 2.7 fm(3) lattices with Iwasaki gauge action, and a 0.17 GeV pion and a 4.6 fm(3) lattice with I-DSDR gauge action, all generated by the RBC and UKQCD collaborations. The all-mode averaging technique enables an efficient and high statistics calculation. Chiral behavior of lattice EDMs is discussed in the context of baryon chiral perturbation theory. In addition, we also show numerical evidence on the relationship of three-and two-point correlation functions with the local topological charge distribution. C1 [Shintani, Eigo] RIKEN, Adv Inst Computat Sci, Kobe, Hyogo 6500047, Japan. [Shintani, Eigo; Blum, Thomas; Izubuchi, Taku] Brookhaven Natl Lab, RIKEN, Res Ctr, Upton, NY 11973 USA. [Blum, Thomas] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Izubuchi, Taku; Soni, Amarjit] Brookhaven Natl Lab, High Energy Theory Grp, Upton, NY 11973 USA. RP Shintani, E (reprint author), RIKEN, Adv Inst Computat Sci, Kobe, Hyogo 6500047, Japan.; Shintani, E (reprint author), Brookhaven Natl Lab, RIKEN, Res Ctr, Upton, NY 11973 USA. EM shintani@riken.jp FU Japanese Ministry of Education [22540301, 23105714, 23105715]; U.S. Department of Energy [DE-AC02-98CH10886, DE-FG02-13ER41989]; INT; Program "Intersections of BSM Phenomenology and QCD for New Physics Searches" [INT-15-3] FX We thank members of RIKEN-BNL-Columbia (RBC) and the UKQCD Collaboration for sharing USQCD resources for part of our calculation. E. S. thanks F.-K. Guo and U.-G. Meissner, E. Mereghetti, J. de Vries, U. van Kolck, and M. J. Ramsey-Musolf for useful discussions on chiral perturbation theory, and also G. Schierholz and A. Shindler for discussion and comments. Numerical calculations were performed using the RICC at RIKEN and the Ds cluster at FNAL. This work was supported by the Japanese Ministry of Education through Grants-in-Aid No. 22540301 (T. I.), No. 23105714 (E. S.), No. 23105715 (T. I.) and through U.S. Department of Energy Grants No. DE-AC02-98CH10886 (T. I. and A. S.) and No. DE-FG02-13ER41989 (T.B.). We are grateful to BNL, the RIKEN BNL Research Center, the RIKEN Advanced Center for Computing and Communication, and USQCD for providing resources necessary for completion of this work. For their support, we also thank the INT and organizers of Program INT-15-3, "Intersections of BSM Phenomenology and QCD for New Physics Searches," 14 September-23 October, 2015. NR 67 TC 4 Z9 4 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 5 PY 2016 VL 93 IS 9 AR 094503 DI 10.1103/PhysRevD.93.094503 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL5CT UT WOS:000375655600001 ER PT J AU Rai, DK Beaucage, G Ratkanthwar, K Beaucage, P Ramachandran, R Hadjichristidis, N AF Rai, Durgesh K. Beaucage, Gregory Ratkanthwar, Kedar Beaucage, Peter Ramachandran, Ramnath Hadjichristidis, Nikos TI Quantification of interaction and topological parameters of polyisoprene star polymers under good solvent conditions SO PHYSICAL REVIEW E LA English DT Article ID SMALL-ANGLE SCATTERING; BRANCHED POLYMERS; NEUTRON-SCATTERING; THERMODYNAMIC PROPERTIES; ANIONIC-POLYMERIZATION; SEMIDILUTE SOLUTIONS; SHAPED POLYMERS; POLYETHYLENE; BEHAVIOR; DILUTE AB Mass fractal scaling, reflected in the mass fractal dimension d(f), is independently impacted by topology, reflected in the connectivity dimension c, and by tortuosity, reflected in the minimum dimension d(min). The mass fractal dimension is related to these other dimensions by d(f) = cd(min). Branched fractal structures have a higher mass fractal dimension compared to linear structures due to a higher c, and extended structures have a lower dimension compared to convoluted self-avoiding and Gaussian walks due to a lower d(min). It is found, in this work, that macromolecules in thermodynamic equilibrium display a fixed mass fractal dimension d(f) under good solvent conditions, regardless of chain topology. These equilibrium structures accommodate changes in chain topology such as branching c by a decrease in chain tortuosity d(min). Symmetric star polymers are used to understand the structure of complex macromolecular topologies. A recently published hybrid Unified scattering function accounts for interarm correlations in symmetric star polymers along with polymer-solvent interaction for chains of arbitrary scaling dimension. Dilute solutions of linear, three-arm and six-arm polyisoprene stars are studied under good solvent conditions in deuterated p-xylene. Reduced chain tortuosity can be viewed as steric straightening of the arms. Steric effects for star topologies are quantified, and it is found that steric straightening of arms is more significant for lower-molecular-weight arms. The observation of constant d(f) is explained through a modification of Flory-Krigbaum theory for branched polymers. C1 [Rai, Durgesh K.] Oak Ridge Natl Lab, Biol & Soft Matter Div, POB 2008,MS 6454, Oak Ridge, TN 37831 USA. [Beaucage, Gregory] Univ Cincinnati, Mat Sci & Engn, 492 Rhodes Hall, Cincinnati, OH 45221 USA. [Ratkanthwar, Kedar] Univ Athens, Dept Chem, Athens 15771, Greece. [Ratkanthwar, Kedar; Hadjichristidis, Nikos] KAUST, Div Phys Sci & Engn, Catalysis Ctr, Thuwal, Saudi Arabia. [Beaucage, Peter] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Ramachandran, Ramnath] Procter & Gamble, 1 P&G Plaza, Cincinnati, OH 45202 USA. RP Rai, DK (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, POB 2008,MS 6454, Oak Ridge, TN 37831 USA.; Beaucage, G (reprint author), Univ Cincinnati, Mat Sci & Engn, 492 Rhodes Hall, Cincinnati, OH 45221 USA. EM raidk@ornl.gov; beaucag@uc.edu OI Ratkanthwar, Kedar/0000-0002-6324-696X; Rai, Durgesh/0000-0001-7257-7210 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (USA); National Institute of Standards and Technology (USA), U.S. Department of Commerce; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX R.K. and N.H. thank Dr. Ema Zagar, National Institute of Chemistry Slovenia, for the SEC-MALS characterization of the star PIs. The research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (USA). We acknowledge the support of the National Institute of Standards and Technology (USA), U.S. Department of Commerce, in providing the neutron research facilities used in this work. D.K.R. is supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory. NR 48 TC 0 Z9 0 U1 3 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAY 5 PY 2016 VL 93 IS 5 AR 052501 DI 10.1103/PhysRevE.93.052501 PG 11 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DL5FG UT WOS:000375662100007 PM 27300939 ER PT J AU Hinderer, T Taracchini, A Foucart, F Buonanno, A Steinhoff, J Duez, M Kidder, LE Pfeiffer, HP Scheel, MA Szilagyi, B Hotokezaka, K Kyutoku, K Shibata, M Carpenter, CW AF Hinderer, Tanja Taracchini, Andrea Foucart, Francois Buonanno, Alessandra Steinhoff, Jan Duez, Matthew Kidder, Lawrence E. Pfeiffer, Harald P. Scheel, Mark A. Szilagyi, Bela Hotokezaka, Kenta Kyutoku, Koutarou Shibata, Masaru Carpenter, Cory W. TI Effects of Neutron-Star Dynamic Tides on Gravitational Waveforms within the Effective-One-Body Approach SO PHYSICAL REVIEW LETTERS LA English DT Article ID EQUATION-OF-STATE; COALESCING BINARIES AB Extracting the unique information on ultradense nuclear matter from the gravitational waves emitted by merging neutron-star binaries requires robust theoretical models of the signal. We develop a novel effective-one-body waveform model that includes, for the first time, dynamic (instead of only adiabatic) tides of the neutron star as well as the merger signal for neutron-star-black-hole binaries. We demonstrate the importance of the dynamic tides by comparing our model against new numerical-relativity simulations of nonspinning neutron-star-black-hole binaries spanning more than 24 gravitational-wave cycles, and to other existing numerical simulations for double neutron-star systems. Furthermore, we derive an effective description that makes explicit the dependence of matter effects on two key parameters: tidal deformability and fundamental oscillation frequency. C1 [Hinderer, Tanja] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Hinderer, Tanja; Taracchini, Andrea; Buonanno, Alessandra; Steinhoff, Jan] Albert Einstein Inst, Max Planck Inst Gravitat Phys, Muhlenberg 1, D-14476 Potsdam, Germany. [Foucart, Francois] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Steinhoff, Jan] Univ Lisbon, Inst Super Tecn, Ctr Multidisciplinar Astrofis, Dept Fis, Ave Rovisco Pais 1, P-1049001 Lisbon, Portugal. [Duez, Matthew; Carpenter, Cory W.] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Kidder, Lawrence E.] Cornell Univ, Cornell Ctr Astrophys & Planetary Sci, Ithaca, NY 14853 USA. [Pfeiffer, Harald P.] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [Scheel, Mark A.; Szilagyi, Bela] CALTECH, Theoret Astrophys 350 17, Pasadena, CA 91125 USA. [Szilagyi, Bela] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Hotokezaka, Kenta] Hebrew Univ Jerusalem, Racah Inst Phys, IL-91904 Jerusalem, Israel. [Kyutoku, Koutarou] RIKEN, Res Grp, Interdisciplinary Theoret Sci iTHES, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Shibata, Masaru] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. RP Hinderer, T (reprint author), Univ Maryland, Dept Phys, College Pk, MD 20742 USA.; Hinderer, T (reprint author), Albert Einstein Inst, Max Planck Inst Gravitat Phys, Muhlenberg 1, D-14476 Potsdam, Germany. FU NSF [PHY-1208881, PHY-1402916, PHY-1404569, AST-1333520, PHY-0960291, ACI-1053575]; NASA [NNX12AN10G, NAS8-03060]; NASA through Einstein Postdoctoral Fellowship - Chandra X-ray Center [PF4-150122]; Japanese MEXT [24244028]; NSERC Canada; NSF at Cornell [PHY-1306125, AST-1333129]; Sherman Fairchild Foundation; Canada Foundation for Innovation (CFI); NanoQuebec; RMGA; Fonds de recherche du Quebec-Nature et Technologie (FRQ-NT) FX We thank Kostas Kokkotas and Cole Miller for useful discussions. A. B. and T. H. acknowledge support from NSF Grant No. PHY-1208881. A. B. also acknowledges partial support from NASA Grant No. NNX12AN10G. T. H. thanks the Max Planck Institut fur Gravitationsphysik for hospitality. Support for this work was provided by NASA through Einstein Postdoctoral Fellowship Grant No. PF4-150122 (F. F.) awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under Contract No. NAS8-03060. M. D. acknowledges support from NSF Grant No. PHY-1402916. M. S. was supported by Grant-in-Aid for Scientific Research 24244028 of the Japanese MEXT. H. P. gratefully acknowledge support from the NSERC Canada. L. K. acknowledges support from NSF Grants No. PHY-1306125 and No. AST-1333129 at Cornell, while the authors at Caltech acknowledge support from NSF Grants No. PHY-1404569 and No. AST-1333520. Authors at both Cornell and Caltech also thank the Sherman Fairchild Foundation for their support. Computations were performed on the supercomputer Briaree from the Universite de Montreal, managed by Calcul Quebec and Compute Canada. The operation of these supercomputers is funded by the Canada Foundation for Innovation (CFI), NanoQuebec, RMGA, and the Fonds de recherche du Quebec-Nature et Technologie (FRQ-NT). Computations were also performed on the Zwicky cluster at Caltech, supported by the Sherman Fairchild Foundation and by NSF Award No. PHY-0960291. This work also used the Extreme Science and Engineering Discovery Environment (XSEDE) through allocation No. TGPHY990007N, supported by NSF Grant No. ACI-1053575. NR 58 TC 13 Z9 13 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2016 VL 116 IS 18 AR 181101 DI 10.1103/PhysRevLett.116.181101 PG 6 WC Physics, Multidisciplinary SC Physics GA DL5HZ UT WOS:000375669300002 PM 27203312 ER PT J AU Jung, SW Shin, WJ Kim, J Moreschini, L Yeom, HW Rotenberg, E Bostwick, A Kim, KS AF Jung, Sung Won Shin, Woo Jong Kim, Jimin Moreschini, Luca Yeom, Han Woong Rotenberg, Eli Bostwick, Aaron Kim, Keun Su TI Sublattice Interference as the Origin of sigma Band Kinks in Graphene SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANGLE-RESOLVED PHOTOEMISSION; BILAYER GRAPHENE; SUPERCONDUCTORS; GRAPHITE; ENERGY AB Kinks near the Fermi level observed in angle-resolved photoemission spectroscopy (ARPES) have been widely accepted to represent electronic coupling to collective excitations, but kinks at higher energies have eluded a unified description. We identify the mechanism leading to such kink features by means of ARPES and tight-binding band calculations on sigma bands of graphene, where anomalous kinks at energies as high as similar to 4 eV were reported recently [Phys. Rev. Lett. 111, 216806 (2013)]. We found that two s bands show a strong intensity modulation with abruptly vanishing intensity near the kink features, which is due to sublattice interference. The interference induced local singularity in the matrix element is a critical factor that gives rise to apparent kink features, as confirmed by our spectral simulations without involving any coupling to collective excitations. C1 [Jung, Sung Won; Shin, Woo Jong; Kim, Jimin; Moreschini, Luca; Yeom, Han Woong; Kim, Keun Su] Inst for Basic Sci Korea, Ctr Artificial Low Dimens Elect Syst, Pohang 37673, South Korea. [Jung, Sung Won; Shin, Woo Jong; Kim, Jimin; Yeom, Han Woong; Kim, Keun Su] Pohang Univ Sci & Technol, Dept Phys, Pohang 37673, South Korea. [Moreschini, Luca; Rotenberg, Eli; Bostwick, Aaron] EO Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kim, KS (reprint author), Inst for Basic Sci Korea, Ctr Artificial Low Dimens Elect Syst, Pohang 37673, South Korea.; Kim, KS (reprint author), Pohang Univ Sci & Technol, Dept Phys, Pohang 37673, South Korea. EM keunsukim@postech.edu RI Rotenberg, Eli/B-3700-2009 OI Rotenberg, Eli/0000-0002-3979-8844 FU U.S. Department of Energy, Office of Sciences [DE-AC02-05CH11231]; [IBS-R014-D1] FX This work was supported by IBS-R014-D1. The ALS was supported by the U.S. Department of Energy, Office of Sciences, under Contract No. DE-AC02-05CH11231. We thank J. Denlinger and Y. K. Kim for help with experiments, and S.-H. Jhi, S.-H. Lee, and D. Cho for valuable discussions. NR 40 TC 5 Z9 5 U1 8 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2016 VL 116 IS 18 AR 186802 DI 10.1103/PhysRevLett.116.186802 PG 5 WC Physics, Multidisciplinary SC Physics GA DL5HZ UT WOS:000375669300015 PM 27203340 ER PT J AU Lin, SZ Hayami, S Batista, CD AF Lin, Shi-Zeng Hayami, Satoru Batista, Cristian D. TI Magnetic Vortex Induced by Nonmagnetic Impurity in Frustrated Magnets SO PHYSICAL REVIEW LETTERS LA English DT Article ID STATES; CHAINS AB We study the effect of a nonmagnetic impurity inserted in a two-dimensional frustrated ferromagnet above its saturation magnetic field Hsai for arbitrary spin S. We demonstrate that the ground state includes a magnetic vortex that is nucleated around the 'impurity over a finite range of magnetic field H-sat <= H <= H-sat(1). Upon approaching the quantum critical point at H = Hat, the radius of the magnetic vortex diverges as the magnetic correlation length: H-sat. These results are derived both for the lattice and in the continuum limit. C1 [Lin, Shi-Zeng; Hayami, Satoru; Batista, Cristian D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Lin, Shi-Zeng; Hayami, Satoru; Batista, Cristian D.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. [Hayami, Satoru] Hokkaido Univ, Dept Phys, Sapporo, Hokkaido 0600810, Japan. [Batista, Cristian D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Batista, Cristian D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Batista, Cristian D.] Oak Ridge Natl Lab, Shull Wollan Ctr, Oak Ridge, TN 37831 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Lin, SZ (reprint author), Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016 OI Lin, Shi-Zeng/0000-0002-4368-5244; FU NNSA of the US DOE at LANL [DE-AC52-06NA25396]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX We thank Y. Kamiya, I. R. Fisher, H. Zhou, A. T. Hrsitov, and E. D. Bauer for useful discussions. Computer resources for numerical calculations were supported by the Institutional Computing Program at LANL. This work was carried out under the auspices of the NNSA of the US DOE at LANL under Contract No. DE-AC52-06NA25396, and was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 28 TC 2 Z9 2 U1 4 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2016 VL 116 IS 18 AR 187202 DI 10.1103/PhysRevLett.116.187202 PG 5 WC Physics, Multidisciplinary SC Physics GA DL5HZ UT WOS:000375669300016 PM 27203342 ER PT J AU Zhang, Z Yan, LX Du, YC Zhou, Z Su, XL Zheng, LM Wang, D Tian, QL Wang, W Shi, JR Chen, HB Huang, WH Gai, W Tang, CX AF Zhang, Zhen Yan, Lixin Du, Yingchao Zhou, Zheng Su, Xiaolu Zheng, Lianmin Wang, Dong Tian, Qili Wang, Wei Shi, Jiaru Chen, Huaibi Huang, Wenhui Gai, Wei Tang, Chuanxiang TI Tunable High-Intensity Electron Bunch Train Production Based on Nonlinear Longitudinal Space Charge Oscillation SO PHYSICAL REVIEW LETTERS LA English DT Article ID PLASMA WAKEFIELD ACCELERATOR; TERAHERTZ; GENERATION; BEAM; TECHNOLOGY; RADIATION AB High-intensity trains of electron bunches with tunable picosecond spacing are produced and measured experimentally with the goal of generating terahertz (THz) radiation. By imposing an initial density modulation on a relativistic electron beam and controlling the charge density over the beam propagation, density spikes of several-hundred-ampere peak current in the temporal profile, which are several times higher than the initial amplitudes, have been observed for the first time. We also demonstrate that the periodic spacing of the bunch train can be varied continuously either by tuning launching phase of a radiofrequency gun or by tuning the compression of a downstream magnetic chicane. Narrow-band coherent THz radiation from the bunch train was also measured with mu J-level energies and tunable central frequency of the spectrum in the range of similar to 0.5 to 1.6 THz. Our results pave the way towards generating mJ-level narrow-band coherent THz radiation and driving high-gradient wakefield-based acceleration. C1 [Zhang, Zhen; Yan, Lixin; Du, Yingchao; Zhou, Zheng; Su, Xiaolu; Zheng, Lianmin; Wang, Dong; Tian, Qili; Wang, Wei; Shi, Jiaru; Chen, Huaibi; Huang, Wenhui; Gai, Wei; Tang, Chuanxiang] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Gai, Wei] Argonne Natl Lab, Lemont, IL 60439 USA. RP Tang, CX (reprint author), Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. EM tang.xuh@tsinghua.edu.cn FU National Natural Science Foundation of China (NSFC) [11475097, 11375097, 11435015]; National Key Scientific Instrument and Equipment Development Project of China [2013YQ12034504] FX The authors want to thank R. K. Li from SLAC for many helpful discussions and suggestions on the experiment. This work was supported by the National Natural Science Foundation of China (NSFC Grants No. 11475097, No. 11375097, and No. 11435015) and the National Key Scientific Instrument and Equipment Development Project of China (Grant No. 2013YQ12034504). NR 35 TC 5 Z9 5 U1 13 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 5 PY 2016 VL 116 IS 18 AR 184801 DI 10.1103/PhysRevLett.116.184801 PG 5 WC Physics, Multidisciplinary SC Physics GA DL5HZ UT WOS:000375669300008 PM 27203327 ER PT J AU Sulmonetti, TP Pang, SH Claure, MT Lee, S Cullen, DA Agrawal, PK Jones, CW AF Sulmonetti, Taylor P. Pang, Simon H. Claure, Micaela Taborga Lee, Sungsik Cullen, David A. Agrawal, Pradeep K. Jones, Christopher W. TI Vapor phase hydrogenation of furfural over nickel mixed metal oxide catalysts derived from layered double hydroxides SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Biomass; Furfural; Hydrogenation; Layered double hydroxide; Mixed metal oxide; Cobalt ID FISCHER-TROPSCH SYNTHESIS; RAY PHOTOELECTRON-SPECTROSCOPY; IN-SITU; SELECTIVE HYDROGENATION; ABSORPTION-SPECTROSCOPY; SUPPORTED CATALYSTS; COBALT CATALYSTS; MILD CONDITIONS; ANIONIC CLAYS; AL CATALYSTS AB The hydrogenation of furfural is investigated over various reduced nickel mixed metal oxides derived from layered double hydroxides (LDHs) containing Ni-Mg-Al and Ni-Co-Al. Upon reduction, relatively large Ni(0) domains develop in the Ni-Mg-Al catalysts, whereas in the Ni-Co-Al catalysts smaller metal particles of Ni(0) and Co(0), potentially as alloys, are formed, as evidenced by XAS, XPS, STEM and EELS. All the reduced Ni catalysts display similar selectivities towards major hydrogenation products (furfuryl alcohol and tetrahydrofurfuryl alcohol), though the side products varied with the catalyst composition. The 1.1Ni-0.8Co-Al catalyst showed the greatest activity per titrated site when compared to the other catalysts, with promising activity compared to related catalysts in the literature. The use of base metal catalysts for hydrogenation of furanic compounds may be a promising alternative to the well-studied precious metal catalysts for making biomass-derived chemicals if catalyst selectivity can be improved in future work by alloying or tuning metal-oxide support interactions (C) 2016 Elsevier B.V. All rights reserved. C1 [Sulmonetti, Taylor P.; Pang, Simon H.; Claure, Micaela Taborga; Agrawal, Pradeep K.; Jones, Christopher W.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Lee, Sungsik] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. [Cullen, David A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Jones, CW (reprint author), Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. EM cjones@chbe.gatech.edu RI Cullen, David/A-2918-2015; OI Cullen, David/0000-0002-2593-7866; Pang, Simon/0000-0003-2913-1648 FU Catalysis Center for Energy Innovation, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science [DE-SC0001004]; DOE Office of Science [DE-AC02-06CH11357] FX This work was supported as part of the Catalysis Center for Energy Innovation, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science under grant DE-SC0001004. STEM analysis was performed through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is a Department of Energy, Office of Science, User Facility.; This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 67 TC 5 Z9 5 U1 36 U2 73 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD MAY 5 PY 2016 VL 517 BP 187 EP 195 DI 10.1016/j.apcata.2016.03.005 PG 9 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA DK8FH UT WOS:000375162100021 ER PT J AU Kumar, N Roy, A Wang, Z L'Abbate, EM Haynes, D Shekhawat, D Spivey, JJ AF Kumar, Nitin Roy, Amitava Wang, Zi L'Abbate, Enrico Mario Haynes, Daniel Shekhawat, Dushyant Spivey, J. J. TI Bi-reforming of methane on Ni-based pyrochlore catalyst SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Reforming; Dry-reforming; Bi-reforming; Pyrochlore; Syngas; Methane activation ID PARTIAL OXIDATION; SUPPORTED CATALYSTS; SYNGAS PRODUCTION; CARBON-DIOXIDE; STEAM; BEHAVIOR; PHASES; NICKEL; OXIDE; GAS AB A Ni-based pyrochlore catalyst was synthesized using the modified Pechini method. In this method, 1 wt% Ni was doped into the La2Zr2O7 Pyrochlore structure. The catalyst was characterized by H-2-TPR, TPO, XRD, and EXAFS, and tested for its methane reforming activity under bi-reforming reaction conditions; i.e., in the presence of CO2 and steam: 3CH(4) + CO2 + 2H(2)O reversible arrow 4CO + 8H(2) Repeated TPR/TPO cycles showed that the two consecutive TPR spectra do not change, showing that the catalyst is stable at high temperatures, and that the nickel oxidation/reduction process is reversible. The catalyst showed constant activity with time at all temperatures in the range of 700-950 degrees C over a cumulative period of 170 h. After this series of bi-reforming tests, TPO of the spent catalyst was carried out, which showed detectable but unquantifiable carbon deposition. The presence of steam in bi-reforming greatly limits carbon deposition compared to directly related dry-reforming tests on this same catalyst. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kumar, Nitin; Roy, Amitava; Wang, Zi; Spivey, J. J.] Louisiana State Univ, Baton Rouge, LA 70803 USA. [L'Abbate, Enrico Mario] KTH Royal Inst Technol, Stockholm, Sweden. [Haynes, Daniel; Shekhawat, Dushyant] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Spivey, JJ (reprint author), Louisiana State Univ, Baton Rouge, LA 70803 USA. EM jjspivey@lsu.edu FU Climate Change and Emissions Management Corporation (CCEMC), Canada FX We acknowledge financial support from Climate Change and Emissions Management Corporation (CCEMC), Canada. Dr. Arun Raju at UC, Riverside is gratefully acknowledged for bi-reforming process development. NR 35 TC 3 Z9 3 U1 18 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD MAY 5 PY 2016 VL 517 BP 211 EP 216 DI 10.1016/j.apcata.2016.03.016 PG 6 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA DK8FH UT WOS:000375162100023 ER PT J AU Samolyuk, GD Beland, LK Stocks, GM Stoller, RE AF Samolyuk, G. D. Beland, L. K. Stocks, G. M. Stoller, R. E. TI Electron-phonon coupling in Ni-based binary alloys with application to displacement cascade modeling SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE density functional theory; cascades; electron phonon coupling; nickel-based binary alloys; coherent potential approximation ID COHERENT-POTENTIAL-APPROXIMATION; HIGH-ENTROPY ALLOYS; CU-NI; TRANSITION-TEMPERATURE; MOLECULAR-DYNAMICS; METALS; ENERGY; PHASE; ENHANCEMENT; EQUATIONS AB Energy transfer between lattice atoms and electrons is an important channel of energy dissipation during displacement cascade evolution in irradiated materials. On the assumption of small atomic displacements, the intensity of this transfer is controlled by the strength of electron-phonon (el-ph) coupling. The el-ph coupling in concentrated Ni-based alloys was calculated using electronic structure results obtained within the coherent potential approximation. It was found that Ni0.5Fe0.5, Ni0.5Co0.5 and Ni0.5Pd0.5 are ordered ferromagnetically, whereas Ni0.5Cr0.5 is nonmagnetic. Since the magnetism in these alloys has a Stoner-type origin, the magnetic ordering is accompanied by a decrease of electronic density of states at the Fermi level, which in turn reduces the el-ph coupling. Thus, the el-ph coupling values for all alloys are approximately 50% smaller in the magnetic state than for the same alloy in a nonmagnetic state. As the temperature increases, the calculated coupling initially increases. After passing the Curie temperature, the coupling decreases. The rate of decrease is controlled by the shape of the density of states above the Fermi level. Introducing a two-temperature model based on these parameters in 10 keV molecular dynamics cascade simulation increases defect production by 10-20% in the alloys under consideration. C1 [Samolyuk, G. D.; Beland, L. K.; Stocks, G. M.; Stoller, R. E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Samolyuk, GD (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM samolyukgd@ornl.gov RI Stocks, George Malcollm/Q-1251-2016 OI Stocks, George Malcollm/0000-0002-9013-260X FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Fonds Quebecois de recherche Nature et Technologies; Office of Science of the US Department of Energy FX GDS would like to thank Dr A Caro and A A Correa for useful discussions. This work was supported as part of the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. LKB acknowledges additional support from a fellowship awarded by the Fonds Quebecois de recherche Nature et Technologies. Authors used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy. NR 56 TC 5 Z9 5 U1 4 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAY 5 PY 2016 VL 28 IS 17 AR 175501 DI 10.1088/0953-8984/28/17/175501 PG 11 WC Physics, Condensed Matter SC Physics GA DJ7LO UT WOS:000374393100007 PM 27033732 ER PT J AU Luo, YK Rosa, PFS Bauer, ED Thompson, JD AF Luo, Yongkang Rosa, P. F. S. Bauer, E. D. Thompson, J. D. TI Vortexlike excitations in the heavy-fermion superconductor CeIrIn5 SO PHYSICAL REVIEW B LA English DT Article ID ZERO-TEMPERATURE LIMIT; PRESSURE; THERMOELECTRICITY; CERHIN5; CECOIN5; NQR AB We report a systematic study of temperature- and field-dependent charge (rho) and entropy (S) transport in the heavy-fermion superconductor CeIrIn5. Its large positive thermopower S-xx is typical of Ce-based Kondo lattice systems, and strong electronic correlations play an important role in enhancing the Nernst signal S-xy. By separating the off-diagonal Peltier coefficient alpha(xy) from S-xy, we find that alpha(xy) becomes positive and greatly enhanced at temperatures well above the bulk T-c. Compared with the nonmagnetic analog LaIrIn5, these results suggest vortexlike excitations in a precursor state to unconventional superconductivity in CeIrIn5. This study sheds light on the similarity of heavy-fermion and cuprate superconductors and on the possibility of states not characterized by the amplitude of an order parameter. C1 [Luo, Yongkang; Rosa, P. F. S.; Bauer, E. D.; Thompson, J. D.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Luo, YK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM ykluo@lanl.gov OI Bauer, Eric/0000-0003-0017-1937; Ferrari Silveira Rosa, Priscila/0000-0002-3437-548X FU U.S. Department of Energy, Division of Materials Sciences and Engineering; Director's Postdoctoral Fellowship - Los Alamos LDRD program FX We thank Shizeng Lin for insightful conversations. Work at Los Alamos was performed under the auspices of the U.S. Department of Energy, Division of Materials Sciences and Engineering. P.F.S.R. acknowledges support through a Director's Postdoctoral Fellowship that is funded by the Los Alamos LDRD program. NR 45 TC 0 Z9 0 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 5 PY 2016 VL 93 IS 20 AR 201102 DI 10.1103/PhysRevB.93.201102 PG 5 WC Physics, Condensed Matter SC Physics GA DL3NM UT WOS:000375540500002 ER PT J AU Zhang, WL Yin, ZP Ignatov, A Bukowski, Z Karpinski, J Sefat, AS Ding, H Richard, P Blumberg, G AF Zhang, W. -L. Yin, Z. P. Ignatov, A. Bukowski, Z. Karpinski, Janusz Sefat, Athena S. Ding, H. Richard, P. Blumberg, G. TI Raman scattering study of spin-density-wave-induced anisotropic electronic properties in AFe(2)As(2) (A = Ca, Eu) SO PHYSICAL REVIEW B LA English DT Article ID DETWINNED BA(FE1-XCOX)(2)AS-2; CHARGE DYNAMICS; IRON PNICTIDES; SUPERCONDUCTORS; TRANSITION AB We present a polarization-resolved and temperature-dependent Raman scattering study of AFe(2)As(2) (A = Ca, Eu). In the spin-density-wave phase, spectral weight redistribution is observed in the fully symmetric and nonsymmetric scattering channels at different energies. An anisotropic Raman response is observed in the fully symmetric channel in spontaneously detwinned CaFe2As2 samples. We calculate the orbital-resolved electronic structures using a combination of density functional theory and dynamical mean field theory. We identify the electronic transitions corresponding to these two spectral features and find that the anisotropic Raman response originates from the lifted degeneracy of the d(xz/yz) orbitals in the broken-symmetry phase. C1 [Zhang, W. -L.; Ding, H.; Richard, P.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Zhang, W. -L.; Ding, H.; Richard, P.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Zhang, W. -L.; Yin, Z. P.; Ignatov, A.; Blumberg, G.] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. [Bukowski, Z.; Karpinski, Janusz] ETH, Solid State Phys Lab, CH-8093 Zurich, Switzerland. [Bukowski, Z.] Polish Acad Sci, Inst Low Temp & Struct Res, POB 1410, PL-50422 Wroclaw, Poland. [Sefat, Athena S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Ding, H.; Richard, P.] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. [Blumberg, G.] NICPB, Akad Tee 23, EE-12618 Tallinn, Estonia. RP Zhang, WL (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.; Zhang, WL (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.; Zhang, WL; Blumberg, G (reprint author), Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA.; Blumberg, G (reprint author), NICPB, Akad Tee 23, EE-12618 Tallinn, Estonia. EM wlzhang@iphy.ac.cn; girsh@physics.rutgers.edu RI Richard, Pierre/F-7652-2010; Sefat, Athena/R-5457-2016 OI Richard, Pierre/0000-0003-0544-4551; Sefat, Athena/0000-0002-5596-3504 FU ICAM (NSF-IMI) [DMR-0844115]; NSF [DMR-1104884, DMR130814]; MoST [2011CBA001001, 2015CB921301]; National Natural Science Foundation of China of China [11274362]; NCN, Poland [2011/01/B/ST5/06937]; U.S. Department of Energy, BES and Division of Materials Sciences and Engineering [DE-SC0005463] FX W.-L.Z. acknowledges ICAM (NSF-IMI Grant No. DMR-0844115) and NSF (Grant No. DMR-1104884). P.R. and H.D. acknowledge MoST (Grants No. 2011CBA001001 and No. 2015CB921301) and National Natural Science Foundation of China (Grant No. 11274362) of China. Z.P.Y. acknowledges NSF Grant No. DMR130814. Z.B. acknowledges the NCN, Poland (Grant No. 2011/01/B/ST5/06937). A.S.S. and G.B. acknowledge the U.S. Department of Energy, BES, and Division of Materials Sciences and Engineering under Awards to ORNL and Grant No. DE-SC0005463 correspondingly. NR 33 TC 2 Z9 2 U1 6 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 5 PY 2016 VL 93 IS 20 AR 205106 DI 10.1103/PhysRevB.93.205106 PG 7 WC Physics, Condensed Matter SC Physics GA DL3NM UT WOS:000375540500003 ER PT J AU Jiang, YF Al Mehedi, M Fu, EG Wang, YQ Allard, LF Wang, JP AF Jiang, Yanfeng Al Mehedi, Md Fu, Engang Wang, Yongqiang Allard, Lawrence F. Wang, Jian-Ping TI Synthesis of Fe16N2 compound Free-Standing Foils with 20 MGOe Magnetic Energy Product by Nitrogen Ion-Implantation SO SCIENTIFIC REPORTS LA English DT Article ID IRON NITRIDES; GRAIN-SIZE; FILMS; THICKNESS; SILICON AB Rare-earth-free magnets are highly demanded by clean and renewable energy industries because of the supply constraints and environmental issues. A promising permanent magnet should possess high remanent magnetic flux density (B-r), large coercivity (H-c) and hence large maximum magnetic energy product ((BH)(max)). Fe16N2 has been emerging as one of promising candidates because of the redundancy of Fe and N on the earth, its large magnetocrystalline anisotropy (Ku > 1.0 x 10(7) erg/cc), and large saturation magnetization (4 pi Ms > 2.4 T). However, there is no report on the formation of Fe16N2 magnet with high Br and large Hc in bulk format before. In this paper, we successfully synthesize freestanding Fe16N2 foils with a coercivity of up to 1910 Oe and a magnetic energy product of up to 20 MGOe at room temperature. Nitrogen ion implantation is used as an alternative nitriding approach with the benefit of tunable implantation energy and fluence. An integrated synthesis technique is developed, including a direct foil-substrate bonding step, an ion implantation step and a two-step post-annealing process. With the tunable capability of the ion implantation fluence and energy, a microstructure with grain size 25-30 nm is constructed on the FeN foil sample with the implantation fluence of 5 x 10(17)/cm(2). C1 [Jiang, Yanfeng; Wang, Jian-Ping] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Al Mehedi, Md; Wang, Jian-Ping] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. [Fu, Engang; Wang, Yongqiang] Los Alamos Natl Lab, Ion Beam Mat Lab, POB 1663, Los Alamos, NM 87545 USA. [Allard, Lawrence F.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Wang, JP (reprint author), Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA.; Wang, JP (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA. EM jpwang@umn.edu FU ARPA-E (Advanced Research Projects Agency-Energy) BCT Fe16N2 Magnet project [0472-1595]; NSF through the NSF Minnesota MRSEC program [DMR-0819885]; Center for Integrated Nanotechnologies (CINT), a DOE nanoscience; Sandia National Laboratories FX This work was supported in part by ARPA-E (Advanced Research Projects Agency-Energy) BCT Fe16N2 Magnet project under contract No. 0472-1595. Parts of this work were carried out in using the Characterization Facility, which receives partial support from NSF through the NSF Minnesota MRSEC program under Award Number DMR-0819885. Ion implantation was supported by Center for Integrated Nanotechnologies (CINT), a DOE nanoscience user facility jointly operated by Los Alamos and Sandia National Laboratories. NR 30 TC 4 Z9 4 U1 7 U2 43 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 5 PY 2016 VL 6 AR 25436 DI 10.1038/srep25436 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL3ND UT WOS:000375539600002 PM 27145983 ER PT J AU Merwin, A Phillips, WC Williamson, MA Willit, JL Motsegood, PN Chidambaram, D AF Merwin, Augustus Phillips, William C. Williamson, Mark A. Willit, James L. Motsegood, Perry N. Chidambaram, Dev TI Presence of Li Clusters in Molten LiCl-Li SO SCIENTIFIC REPORTS LA English DT Article ID ELECTROCHEMICAL REDUCTION; ELECTROLYTIC REDUCTION; IONIZATION ENERGIES; LITHIUM-CHLORIDE; METAL-CLUSTERS; SALT-SOLUTIONS; ELECTRONIC-STRUCTURE; MASS-SPECTROMETRY; LICL-LI2O; MOLECULES AB Molten mixtures of lithium chloride and metallic lithium are of significant interest in various metal oxide reduction processes. These solutions have been reported to exhibit seemingly anomalous physical characteristics that lack a comprehensive explanation. In the current work, the physical chemistry of molten solutions of lithium chloride and metallic lithium, with and without lithium oxide, was investigated using in situ Raman spectroscopy. The Raman spectra obtained from these solutions were in agreement with the previously reported spectrum of the lithium cluster, Li-8. This observation is indicative of a nanofluid type colloidal suspension of Li-8 in a molten salt matrix. It is suggested that the formation and suspension of lithium clusters in lithium chloride is the cause of various phenomena exhibited by these solutions that were previously unexplainable. C1 [Merwin, Augustus; Phillips, William C.; Chidambaram, Dev] Univ Nevada, Mat Sci & Engn, 1664 N Virginia St Reno,MS0388, Reno, NV 89557 USA. [Williamson, Mark A.; Willit, James L.; Motsegood, Perry N.] Argonne Natl Lab, Nucl Engn Div, Nucl Chem Engn Dept, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Chidambaram, D (reprint author), Univ Nevada, Mat Sci & Engn, 1664 N Virginia St Reno,MS0388, Reno, NV 89557 USA. EM dcc@unr.edu FU Department of Energy (DOE) [DE-NE0008262]; US Nuclear Regulatory Commission (NRC) [NRCHQ-11-G-38-0039, NRC-38-10-949, NRC-HQ-13-G-38-0027] FX This work was performed under the auspices of the Department of Energy (DOE) through grant DE-NE0008262, and the US Nuclear Regulatory Commission (NRC) under contracts NRCHQ-11-G-38-0039, NRC-38-10-949 and NRC-HQ-13-G-38-0027. Mr. Kenny Osborne serves as the program manager for the DOE awards and Ms. Nancy Hebron-Isreal serves as the grants program officer for the NRC awards. NR 53 TC 1 Z9 1 U1 4 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 5 PY 2016 VL 6 AR 25435 DI 10.1038/srep25435 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL3ND UT WOS:000375539600001 PM 27145895 ER PT J AU Zhang, J Nguyen, MC Balasubramanian, B Das, B Sellmyer, DJ Zeng, Z Ho, KM Wang, CZ AF Zhang, Jie Manh Cuong Nguyen Balasubramanian, Balamurugan Das, Bhaskar Sellmyer, David J. Zeng, Zhi Ho, Kai-Ming Wang, Cai-Zhuang TI Crystal structure and magnetic properties of new Fe3Co3X2 (X = Ti, Nb) intermetallic compounds SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article DE rare-earth free magnetic materials; magnetocrystalline anisotropy energy; genetic algorithm: first-principles calculations; x-ray diffraction ID AUGMENTED-WAVE METHOD; FECO AB The structure and magnetic properties of new magnetic Fe3Co3X2 (X = Ti, Nb) compounds are studied by genetic algorithm, first-principles density functional theory (DFT) calculations, and experiments. The atomic structure of a hexagonal structure with P-6m2 symmetry is determined. The simulated x-ray diffraction (XRD) spectra of the P-6m2 structures agree well with experimental XRD data for both Fe3Co3Ti2 and Fe3Co3Nb2. The magnetic properties of these structures as well as the effect of the disorder of Fe and Co on their magnetic properties are also investigated. The magnetocrystalline anisotropy energy is found to be very sensitive to the occupancy disorder between Fe and Co. C1 [Zhang, Jie; Zeng, Zhi] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China. [Zhang, Jie; Manh Cuong Nguyen; Ho, Kai-Ming; Wang, Cai-Zhuang] Iowa State Univ, Dept Phys & Astron, Ames Lab, US DOE, Ames, IA 50011 USA. [Balasubramanian, Balamurugan; Das, Bhaskar] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Balasubramanian, Balamurugan; Das, Bhaskar] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. RP Wang, CZ (reprint author), Iowa State Univ, Dept Phys & Astron, Ames Lab, US DOE, Ames, IA 50011 USA. EM wangcz@ameslab.gov RI Nguyen, Manh Cuong/G-2783-2015 OI Nguyen, Manh Cuong/0000-0001-8027-9029 FU National Science Foundation (NSF), Division of Materials Research (DMR) under Award DMREF: SusChEM [1436383]; NSF, DMR under Award DMREF: SusChEM [1436385]; National Science Foundation of China [11504381, U1230202]; National Science Foundation [NNCI: 1542182]; Nebraska Research Initiative FX Theoretical research by KMH and CZW was supported by the National Science Foundation (NSF), Division of Materials Research (DMR) under Award DMREF: SusChEM 1436383. Experimental work by BB, BD, and DJS was supported by NSF, DMR under Award DMREF: SusChEM 1436385. J Zhang and Z Zeng were supported by the National Science Foundation of China under Grant Nos. 11504381 and U1230202 (NSAF). Research at Nebraska was performed in part at the Nebraska Nanoscale Facility, Nebraska Center for Materials and Nanoscience, which is supported by the National Science Foundation under Award NNCI: 1542182, and the Nebraska Research Initiative. NR 19 TC 0 Z9 0 U1 10 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 EI 1361-6463 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD MAY 5 PY 2016 VL 49 IS 17 AR 175002 DI 10.1088/0022-3727/49/17/175002 PG 5 WC Physics, Applied SC Physics GA DJ4AA UT WOS:000374146600002 ER PT J AU Dagle, VL Dagle, R Kovarik, L Genc, A Wang, YG Bowden, M Wan, HY Flake, M Glezakou, VA King, DL Rousseau, R AF Dagle, Vanessa Lebarbier Dagle, Robert Kovarik, Libor Genc, Arda Wang, Yang-Gang Bowden, Mark Wan, Haiying Flake, Matthew Glezakou, Vassiliki-Alexandra King, David L. Rousseau, Roger TI Steam reforming of hydrocarbons from biomass-derived syngas over MgAl2O4-supported transition metals and bimetallic IrNi catalysts SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Biomass; Tar; Steam reforming; Gasification; Syngas; Ir; Rh; Ni; Bimetallic catalyst; Noble metals ID GASIFICATION; METHANE; TEMPERATURE; CONVERSION; REMOVAL; TARS; RH AB This study presents an investigation into the steam reforming of hydrocarbons from biomass gasifier derived syngas over MgAl2O4-supported transition metals (Ni, Rh, Ir, Ru, Pt, and Pd) and novel bimetallic IrNi catalysts. Using a model syngas consisting of H-2, CO, CO2, CH4, C2H4, and H2O, Ir and Rh catalysts were found to be the most stable catalysts (at 850 degrees C,1 bar, 114,000 h(-1)). When benzene and naphthalene are added to the feed (as a tar simulant) stability is affected by both tar concentration and type of tar. Catalytic deactivation, caused primarily by coking can be minimized by operating at a high reaction temperature (e.g., 850 degrees C). In addition, promoting Ni catalyst with Ir significantly enhances stability. By using bimetallic formulations of it and Ni (0.5-5.0% Ir, 15%Ni), nickel sintering during the reaction is reduced. Surprisingly, IrNi catalysts also offer more stability than catalysts with Ir particles alone. In agreement with theoretical calculations, small Ir degrees clusters (similar to 2-3 atoms) supported on large Ni degrees particles (>= 5 nm) present more resistance to coking than either small Ir degrees clusters or Ni degrees particles alone. Hence, superior stability of the bimetallic catalysts results from both resistance to coking and a decrease in nickel sintering. Minimal loss of activity of 12% for TOS = 80 h is demonstrated for a bimetallic catalyst with optimal concentrations of 2.5% Ir and 15% Ni. Both monometallic Ir and Ni catalysts suffer substantial loss of activity (i.e., >= 40% loss, TOS = 80 h) under comparable conditions. Published by Elsevier B.V. C1 [Dagle, Vanessa Lebarbier; Dagle, Robert; Wang, Yang-Gang; Wan, Haiying; Flake, Matthew; Glezakou, Vassiliki-Alexandra; King, David L.; Rousseau, Roger] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Kovarik, Libor; Bowden, Mark] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Genc, Arda] FEI Co, 5350 NE Dawson Creek Dr, Hillsboro, OR 97124 USA. RP Dagle, R; Rousseau, R (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. EM vanessa.dagle@pnnl.gov; Robert.Dagle@pnnl.gov; Roger.Rousseau@pnnl.gov RI Rousseau, Roger/C-3703-2014; Kovarik, Libor/L-7139-2016 FU United States Department of Energy (DOE)'s Bioenergy Technologies Office (BETO); Department of Energy's Office of Biological and Environmental Research; BETO FX This work was financially supported by the United States Department of Energy (DOE)'s Bioenergy Technologies Office (BETO) and performed at the Pacific Northwest National Laboratory (PNNL). PNNL is a multi-program national laboratory operated for DOE by Battelle Memorial Institute. Computing time and advanced catalyst characterization use was granted by a user proposal at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL). EMSL is a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. The authors would like to thank Cary Counts of PNNL for help with technical editing of this manuscript. Finally, the authors would also like to thank and dedicate this paper to Mark Gerber who recently retired from PNNL. Mark had a long history of leading BETO-funded PNNL activities in the area of gasification, syngas cleanup, and syngas conversion. Mark was also instrumental in integrating experimental and theoretical catalysis activities pertaining to mixed alcohol synthesis in addition to syngas cleanup research. NR 30 TC 7 Z9 7 U1 10 U2 101 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD MAY 5 PY 2016 VL 184 BP 142 EP 152 DI 10.1016/j.apcatb.2015.11.022 PG 11 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA DC4QO UT WOS:000369205600015 ER PT J AU Chien, YT Vitev, I AF Chien, Yang-Ting Vitev, Ivan TI Towards the understanding of jet shapes and cross sections in heavy ion collisions using soft-collinear effective theory SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadronic Colliders; Jets ID QUARK-GLUON PLASMA; RADIATIVE ENERGY-LOSS; ELECTRON-POSITRON ANNIHILATION; QUANTUM-CHROMODYNAMICS; HADRON-COLLISIONS; E(+)E(-) ANNIHILATION; NUCLEAR MODIFICATION; E&E ANNIHILATION; QCD; ORDER AB We calculate the jet shape and the jet cross section in heavy ion collisions using soft-collinear effective theory (SCET) and its extension with Glauber gluon interactions in the medium (SCETG). We use the previously developed framework to systematically resum the jet shape at next-to-leading logarithmic accuracy, and we consistently include the medium modification by incorporating the leading order medium-induced splitting functions. The calculation provides, for the first time, a quantitative understanding of the jet shape modification measurement in lead-lead collisions at root(NN)-N-S = 2.76 TeV at the LHC. The inclusive jet suppression is also calculated within the same framework beyond the traditional concept of parton energy loss, and the dependence on the centrality, the jet radius and the jet kinematics is examined. In the end we present predictions for the anticipated jet shape and cross section measurements in lead-lead collisions at root(NN)-N-s approximate to 5.1 TeV at the LHC. C1 [Chien, Yang-Ting; Vitev, Ivan] Los Alamos Natl Lab, Div Theoret, T-2, Los Alamos, NM 87545 USA. RP Chien, YT (reprint author), Los Alamos Natl Lab, Div Theoret, T-2, Los Alamos, NM 87545 USA. EM ytchien@lanl.gov; ivitev@lanl.gov FU US Department of Energy, Office of Science [DE-AC52-06NA25396]; DOE Early Career Program FX Y.-T. C. would like to thank Doga Can Gulhan, Christopher Lee, Yen-Jie Lee, Emanuele Mereghetti, Daniel Pablos and Gregory Soyez for helpful discussions, and to Yen-Jie Lee for very useful comments on the manuscript. We would also like to thank the anonymous referee for many useful suggestions. This work is supported by the US Department of Energy, Office of Science under Contract Nos. DE-AC52-06NA25396 and by the DOE Early Career Program. NR 140 TC 0 Z9 0 U1 2 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 4 PY 2016 IS 5 AR 023 DI 10.1007/JHEP05(2016)023 PG 30 WC Physics, Particles & Fields SC Physics GA EH4LF UT WOS:000391742000001 ER PT J AU Warburton, RE Iddir, H Curtiss, LA Greeley, J AF Warburton, Robert E. Iddir, Hakim Curtiss, Larry A. Greeley, Jeffrey TI Thermodynamic Stability of Low- and High-Index Spinel LiMn2O4 Surface Terminations SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE LiMn2O4; LMO; DFT; surface thermodynamics; Li-ion batteries; reducible oxides ID RECHARGEABLE LITHIUM BATTERIES; ULTRASONIC SPRAY-PYROLYSIS; DENSITY-FUNCTIONAL THEORY; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; ELECTROCHEMICAL PERFORMANCES; MOLECULAR-DYNAMICS; STRUCTURAL-CHANGES; MANGANESE OXIDE; ION BATTERY AB Density functional theory calculations are performed within the generalized gradient approximation (GGA-FU) to determine stable terminations of both low- and high-index spinel LiMn2O4 (LMO) surfaces. A grand canonical thermodynamic approach is employed, permitting a direct comparison of off-stoichiometric surfaces with previously reported stoichiometric surface terminations at various environmental conditions. Within this formalism, we have identified trends in the structure of the low-index surfaces as a function of the Li and O chemical potentials. The results suggest that, under a range of chemical potentials for which bulk LMO is stable, Li/O and Li-rich (111) surface terminations are favored, neither of which adopts an inverse spinel structure in the subsurface region. This thermodynamic analysis is extended to identify stable structures for certain high-index surfaces, including (311), (331), (511), and (531), which constitute simple models for steps or defects that may be present on real LMO particles. The low- and high-index results are combined to determine the relative stability of each surface facet under a range of environmental conditions. The relative surface energies are further employed to predict LMO particle shapes through a Wulff construction approach, which suggests that LMO particles will adopt either an octahedron or a truncated octahedron shape at conditions in which LMO is thermodynamically stable. These results are in agreement with the experimental observations of LMO particle shapes. C1 [Warburton, Robert E.; Greeley, Jeffrey] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Iddir, Hakim; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Greeley, J (reprint author), Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. EM jgreeley@purdue.edu FU Center for Electrochemical Energy Science, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This research was supported as part of the Center for Electrochemical Energy Science, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. Some calculations were performed at the National Energy Research Scientific Computing Center. NR 60 TC 4 Z9 4 U1 21 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAY 4 PY 2016 VL 8 IS 17 BP 11108 EP 11121 DI 10.1021/acsami.6b01069 PG 14 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DL3FX UT WOS:000375520700055 PM 27031889 ER PT J AU Costa, THF Vega-Sanchez, ME Milagres, AMF Scheller, HV Ferraz, A AF Costa, Thales H. F. Vega-Sanchez, Miguel E. Milagres, Adriane M. F. Scheller, Henrik V. Ferraz, Andre TI Tissue-specific distribution of hemicelluloses in six different sugarcane hybrids as related to cell wall recalcitrance SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Recalcitrance; Mixed-linkage glucans; Immunofluorescence; Sugarcane ID MIXED-LINKAGE GLUCAN; BIOMASS RECALCITRANCE; CHEMICAL-COMPOSITION; ENZYMATIC-HYDROLYSIS; MONOCLONAL-ANTIBODIES; CELLULOSE; POLYSACCHARIDES; DEGRADABILITY; INTERNODES; LIGNIN AB Background: Grasses are lignocellulosic materials useful to supply the billion-tons annual requirement for renewable resources that aim to produce transportation fuels and a variety of chemicals. However, the polysaccharides contained in grass cell walls are built in a recalcitrant composite. Deconstruction of these cell walls is still a challenge for the energy-efficient and economically viable transformation of lignocellulosic materials. The varied tissue-specific distribution of cell wall components adds complexity to the origins of cell wall recalcitrance in grasses. This complexity usually led to empirically developed pretreatment processes to overcome recalcitrance. A further complication is that efficient pretreatment procedures generally treat the less recalcitrant tissues more than necessary, which results in the generation of undesirable biomass degradation products. Results: Six different sugarcane hybrids were used as model grasses to evaluate the tissue-specific distribution of hemicelluloses and the role of these components in cell wall recalcitrance. Acetylated glucuronoarabinoxylan (GAX) occurs in all tissues. Mixed-linkage glucan (MLG) was relevant in the innermost regions of the sugarcane internodes (up to 15.4 % w/w), especially in the low-lignin content hybrids. Immunofluorescence microscopy showed that xylans predominated in vascular bundles, whereas MLG occurred mostly in the parenchyma cell walls from the pith region of the hybrids with low-lignin content. Evaluation of the digestibility of sugarcane polysaccharides by commercial enzymes indicated that the cell wall recalcitrance varied considerably along the internode regions and in the sugarcane hybrids. Pith regions of the hybrids with high MLG and low-lignin contents reached up to 85 % cellulose conversion after 72 h of hydrolysis, without any pretreatment. Conclusions: The collective characteristics of the internode regions were related to the varied recalcitrance found in the samples. Components such as lignin and GAX were critical for the increased recalcitrance, but low cellulose crystallinity index, high MLG contents, and highly substituted GAX contributed to the generation of a less recalcitrant material. C1 [Costa, Thales H. F.; Milagres, Adriane M. F.; Ferraz, Andre] Univ Sao Paulo, Escola Engn Lorena, Dept Biotecnol, BR-12602810 Lorena, SP, Brazil. [Vega-Sanchez, Miguel E.; Scheller, Henrik V.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Vega-Sanchez, Miguel E.] Monsanto Co, 800N Lindbergh Blvd, St Louis, MO 63141 USA. RP Ferraz, A (reprint author), Univ Sao Paulo, Escola Engn Lorena, Dept Biotecnol, BR-12602810 Lorena, SP, Brazil. EM aferraz@debiq.eel.usp.br RI Ferraz, Andre/A-6484-2009; FAPESP, BIOEN/H-6149-2012; Scheller, Henrik/A-8106-2008 OI Scheller, Henrik/0000-0002-6702-3560 FU Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP) [08/56256-5, 11/50535-2, 14/06923-6]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX The work was supported by Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), Contract numbers 08/56256-5; 11/50535-2; 14/06923-6 and by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. NR 44 TC 1 Z9 1 U1 3 U2 8 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 4 PY 2016 VL 9 AR 99 DI 10.1186/s13068-016-0513-2 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DL8PM UT WOS:000375903900001 PM 27148403 ER PT J AU Shao, XJ Zhou, JL Olson, DG Lynd, LR AF Shao, Xiongjun Zhou, Jilai Olson, Daniel G. Lynd, Lee R. TI A markerless gene deletion and integration system for Thermoanaerobacter ethanolicus SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Thermoanaerobacter ethanolicus; Gene deletion; Gene integration; Marker removal; Clean knockout; tdk; FUDR; Natural competence ID THERMUS-THERMOPHILUS; SELECTION MARKER; THYMIDINE; CELLULOSE; JW200 AB Background: Thermoanaerobacter ethanolicus produces a considerable amount of ethanol from a range of carbohydrates and is an attractive candidate for applications in bioconversion processes. A genetic system with reusable selective markers would be useful for deleting acid production pathways as well as other genetic modifications. Results: The thymidine kinase (tdk) gene was deleted from T. ethanolicus JW200 to allow it to be used as a selectable marker, resulting in strain X20. Deletion of the tdk gene reduced growth rate by 20 %; however, this could be reversed by reintroducing the tdk gene (strain X20C). The tdk and high-temperature kanamycin (htk) markers were tested by using them to delete lactate dehydrogenase (ldh). During positive selection of ldh knockouts in strain X20 on kanamycin agar plates, six out of seven picked colonies were verified transformants. Deletion of ldh reduced lactic acid production by 90 %. The tdk and 5-fluoro-2'-deoxyuridine (FUDR) combination worked reliably as demonstrated by successful tdk removal in all 21 colonies tested. Conclusion: A gene deletion and integration system with reusable markers has been developed for Thermoanaerobacter ethanolicus JW200 with positive selection on kanamycin and negative selection on FUDR. Gene deletion was demonstrated by ldh gene deletion and gene integration was demonstrated by re-integration of the tdk gene. Transformation via a natural competence protocol could use DNA PCR products amplified directly from Gibson Assembly mixture for efficient genetic modification. C1 [Shao, Xiongjun; Zhou, Jilai; Olson, Daniel G.; Lynd, Lee R.] Dartmouth Coll, Thayer Sch Engn, 14 Engn Dr, Hanover, NH 03755 USA. [Shao, Xiongjun; Zhou, Jilai; Olson, Daniel G.; Lynd, Lee R.] Oak Ridge Natl Lab, DOE BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Lynd, LR (reprint author), Dartmouth Coll, Thayer Sch Engn, 14 Engn Dr, Hanover, NH 03755 USA.; Lynd, LR (reprint author), Oak Ridge Natl Lab, DOE BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. EM lee.lynd@dartmouth.edu FU BioEnergy Science Center (BESC); U.S. Department of Energy (DOE) Research Center - Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory; Department of Energy [DE-AC05-00OR22725] FX The authors were supported by the BioEnergy Science Center (BESC), a U.S. Department of Energy (DOE) Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science, Oak Ridge National Laboratory. Oak Ridge National Laboratory is managed by University of Tennessee UT-Battelle LLC for the Department of Energy under Contract No. DE-AC05-00OR22725. NR 20 TC 3 Z9 3 U1 2 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAY 4 PY 2016 VL 9 AR 100 DI 10.1186/s13068-016-0514-1 PG 8 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DL8PM UT WOS:000375903900002 PM 27152121 ER PT J AU Yang, KR Matula, AJ Kwon, G Hong, JY Sheehan, SW Thomsen, JM Brudvig, GW Crabtree, RH Tiede, DM Chen, LX Batista, VS AF Yang, Ke R. Matula, Adam J. Kwon, Gihan Hong, Jiyun Sheehan, Stafford W. Thomsen, Julianne M. Brudvig, Gary W. Crabtree, Robert H. Tiede, David M. Chen, Lin X. Batista, Victor S. TI Solution Structures of Highly Active Molecular Ir Water-Oxidation Catalysts from Density Functional Theory Combined with High-Energy X-ray Scattering and EXAFS Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ORGANOMETALLIC IRIDIUM COMPLEXES; ABSORPTION FINE-STRUCTURE; AMMONIUM-NITRATE; DOMAIN-STRUCTURE; TRANSFORMATION; PRECATALYST; DEGRADATION; DIMER AB The solution structures of highly active Ir water-oxidation catalysts are elucidated by combining density functional theory, high-energy X-ray scattering (HEXS), and extended X-ray absorption fine structure (EXAFS) spectroscopy. We find that the catalysts are Jr dimers with mono-mu-O cores and terminal anionic ligands, generated in situ through partial oxidation of a common catalyst precursor. The proposed structures are supported by H-1 and O-17 NMR, EPR, resonance Raman and UV-vis spectra, electrophoresis, etc. Our findings are particularly valuable to understand the mechanism of water oxidation by highly reactive Ir catalysts. Importantly, our DFT-EXAFS-HEXS methodology provides a new in situ technique for characterization of active species in catalytic systems. C1 [Yang, Ke R.; Matula, Adam J.; Sheehan, Stafford W.; Thomsen, Julianne M.; Brudvig, Gary W.; Crabtree, Robert H.; Batista, Victor S.] Yale Univ, Yale Energy Sci Inst, New Haven, CT 06520 USA. [Yang, Ke R.; Matula, Adam J.; Sheehan, Stafford W.; Thomsen, Julianne M.; Brudvig, Gary W.; Crabtree, Robert H.; Batista, Victor S.] Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. [Kwon, Gihan; Tiede, David M.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hong, Jiyun; Chen, Lin X.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Sheehan, Stafford W.] Catalyt Innovat LLC, 70 Crandall Rd,POB 356, Adamsville, RI 02801 USA. RP Batista, VS (reprint author), Yale Univ, Yale Energy Sci Inst, New Haven, CT 06520 USA.; Batista, VS (reprint author), Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. EM victor.batista@yale.edu OI Sheehan, Stafford/0000-0003-0432-9260 FU Argonne-Northwestern Solar Energy Research (ANSER) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (US DOE-OS-BES) [DE-SC0001059]; US DOE-OS-BES [DE-AC02-06CH11357] FX This work was supported as part of the Argonne-Northwestern Solar Energy Research (ANSER) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (US DOE-OS-BES) under award no. DE-SC0001059. X-ray measurements were carried out at the Advanced Photon Source, operated by Argonne National Laboratory for the US DOE-OS-BES under contract no. DE-AC02-06CH11357. D.M.T. acknowledges DOE BES program support for the model-based calculation of PDF data under this Laboratory Contract. We thank the National Energy Research Scientific Computing Center (NERSC) and Yale High Performance Computation Center for generous computer time allocations. NR 41 TC 9 Z9 9 U1 20 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2016 VL 138 IS 17 BP 5511 EP 5514 DI 10.1021/jacs.6b01750 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DL3GB UT WOS:000375521100010 PM 27087202 ER PT J AU Zhou, YY Yang, MJ Pang, SP Zhu, K Padture, NP AF Zhou, Yuanyuan Yang, Mengjin Pang, Shuping Zhu, Kai Padture, Nitin P. TI Exceptional Morphology-Preserving Evolution of Formamidinium Lead Triiodide Perovskite Thin Films via Organic-Cation Displacement SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PERFORMANCE SOLAR-CELLS; INORGANIC PEROVSKITES; TRIHALIDE; IODIDE; CRYSTALLIZATION; DEPOSITION AB Here we demonstrate a radically different chemical route for the creation of HC(NH2)(2)PbI3 (FAPbI(3)) perovskite thin films. This approach entails a simple exposure of as-synthesized CH3NH3PbI3 (MAPbI(3)) perovskite thin films to HC(=NH)NH2 (formamidine or FA) gas at 150 degrees C, which leads to rapid displacement of the MA cations by FA(+) cations in the perovskite structure. The resultant FAPbI(3) perovskite thin films preserve the microstructural morphology of the original MAPbI(3) thin films exceptionally well. Importantly, the myriad processing innovations that have led to the creation of high quality MAPbI(3) perovskite thin films are directly adaptable to FAPbI(3) through this simple, rapid chemical-conversion route. Accordingly, we show that efficiencies of perovskite solar cells fabricated with FAPbI(3) thin films created using this route can reach similar to 18%. C1 [Zhou, Yuanyuan; Padture, Nitin P.] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Yang, Mengjin; Zhu, Kai] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. [Pang, Shuping] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266101, Peoples R China. RP Padture, NP (reprint author), Brown Univ, Sch Engn, Providence, RI 02912 USA.; Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM kai.zhu@nrel.gov; nitin_padture@brown.edu RI Zhou, Yuanyuan/G-2173-2011; Padture, Nitin/A-9746-2009; OI Zhou, Yuanyuan/0000-0002-8364-4295; Padture, Nitin/0000-0001-6622-8559; Yang, Mengjin/0000-0003-2019-4298 FU National Science Foundation [DMR-1305913, OIA-1538893]; Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990]; Youth Innovation Promotion Association of CAS [2015167] FX Y.Z. and N.P.P acknowledge the support from the National Science Foundation (DMR-1305913, OIA-1538893) for the work performed at Brown University and at NREL. M.Y. and K.Z. acknowledge the support from the Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990) for the work performed at NREL (DE-AC36-08-GO28308). S.P. thanks the Youth Innovation Promotion Association of CAS (2015167) for additional financial support. NR 30 TC 21 Z9 21 U1 39 U2 113 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2016 VL 138 IS 17 BP 5535 EP 5538 DI 10.1021/jacs.6b02787 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DL3GB UT WOS:000375521100016 PM 27088448 ER PT J AU Reed, DA Xiao, DJ Gonzalez, MI Darago, LE Herm, ZR Grandjean, F Long, JR AF Reed, Douglas A. Xiao, Dianne J. Gonzalez, Miguel I. Darago, Lucy E. Herm, Zoey R. Grandjean, Fernande Long, Jeffrey R. TI Reversible CO Scavenging via Adsorbate-Dependent Spin State Transitions in an Iron(II) Triazolate Metal-Organic Framework SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBON-DIOXIDE CAPTURE; COORDINATIVELY UNSATURATED SITES; HYDROGEN STORAGE; ROOM-TEMPERATURE; SINGLE-CRYSTAL; ADSORPTION PROPERTIES; SMALL MOLECULES; CROSSOVER; MONOXIDE; COMPLEXES AB A new metal-organic framework, Fe-BTTri (Fe-3[(Fe4Cl)(3)(BTTri)(8)](2)center dot 18CH(3)OH, H(3)BTTri = 1,3,5-tris(1H-1,2,3-triazol-5-yObenzene)), is found to be highly selective in the adsorption of CO over a variety of other gas molecules, making it extremely effective, for example, in the removal of trace CO from mixtures with H-2, N-2, and CH4. This framework not only displays significant CO adsorption capacity at very low pressures (1.45 mmol/g at just 100 mu bar), but, importantly, also exhibits readily reversible CO binding. Fe-BTTri utilizes a unique spin state change mechanism to bind CO in which the coordinatively unsaturated, high-spin Fe-II centers of the framework convert to octahedral, low-spin Fe-II centers upon CO coordination. Desorption of CO converts the Fe-II sites back to a high-spin ground state; enabling the facile regeneration and recyclability of the material. This spin state change is supported by characterization via infrared spectroscopy, single crystal X-ray analysis, Mossbauer spectroscopy, and magnetic susceptibility measurements. Importantly, the spin state change is selective for CO and is not observed in the presence of other gases, such as H-2, N-2, CO2, CH4, or other hydrocarbons, resulting in unprecedentedly high selectivities for CO adsorption for use in CO/H-2, CO/N-2, and CO/CH4 separations and in preferential CO adsorption over typical strongly adsorbing gases like CO2 and ethylene. While adsorbate-induced spin state transitions are well-known in molecular chemistry, particularly for CO, to our knowledge this is the first time such behavior has been observed in a porous material suitable for use in a gas separation process. Potentially, this effect can be extended to selective separations involving other pi-acids. C1 [Reed, Douglas A.; Xiao, Dianne J.; Gonzalez, Miguel I.; Darago, Lucy E.; Herm, Zoey R.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Grandjean, Fernande] Univ Missouri, Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu OI Darago, Lucy/0000-0001-7515-5558; Gonzalez, Miguel/0000-0003-4250-9035 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; [DE-AC02-05CH11231]; [DE-AC02-06CH11357] FX This research was supported through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001015. Single-crystal X-ray diffraction experiments were performed at Beamline 11.3.1 at the Advanced Light Source, a DoE Office of Science User Facility operated by Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. Powder X-ray diffraction data were collected at Beamline 17-BM at the Advanced Photon Source, a DoE Office of Science User Facility, operated by Argonne National Laboratory under Contract DE-AC02-06CH11357. We thank Dr. B. K. Keitz, Dr. J. A. Mason, Dr. E. D. Bloch, and P. C. Bunting for helpful discussions, and we thank the NSF for providing graduate fellowship support for D.A.R, D.J.X., and L.E.D. NR 78 TC 6 Z9 6 U1 23 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAY 4 PY 2016 VL 138 IS 17 BP 5594 EP 5602 DI 10.1021/jacs.6b00248 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DL3GB UT WOS:000375521100025 PM 27097297 ER PT J AU Rhee, M Light, YK Meagher, RJ Singh, AK AF Rhee, Minsoung Light, Yooli K. Meagher, Robert J. Singh, Anup K. TI Digital Droplet Multiple Displacement Amplification (ddMDA) for Whole Genome Sequencing of Limited DNA Samples SO PLOS ONE LA English DT Article ID ROLLING-CIRCLE AMPLIFICATION; MICROFLUIDIC SYSTEMS; POLYMERASE CLONING; SINGLE CELLS; FIDELITY AB Multiple displacement amplification (MDA) is a widely used technique for amplification of DNA from samples containing limited amounts of DNA (e.g., uncultivable microbes or clinical samples) before whole genome sequencing. Despite its advantages of high yield and fidelity, it suffers from high amplification bias and non-specific amplification when amplifying sub-nanogram of template DNA. Here, we present a microfluidic digital droplet MDA (ddMDA) technique where partitioning of the template DNA into thousands of sub-nanoliter droplets, each containing a small number of DNA fragments, greatly reduces the competition among DNA fragments for primers and polymerase thereby greatly reducing amplification bias. Consequently, the ddMDA approach enabled a more uniform coverage of amplification over the entire length of the genome, with significantly lower bias and non-specific amplification than conventional MDA. For a sample containing 0.1 pg/mu L of E. coli DNA (equivalent of similar to 3/1000 of an E. coli genome per droplet), ddMDA achieves a 65-fold increase in coverage in de novo assembly, and more than 20-fold increase in specificity (percentage of reads mapping to E. coli) compared to the conventional tube MDA. ddMDA offers a powerful method useful for many applications including medical diagnostics, forensics, and environmental microbiology. C1 [Rhee, Minsoung; Light, Yooli K.; Meagher, Robert J.; Singh, Anup K.] Sandia Natl Labs, Biotechnol & Bioengn Dept, Livermore, CA USA. [Rhee, Minsoung] Illumina Inc, 5200 Illumina Way, San Diego, CA USA. RP Meagher, RJ; Singh, AK (reprint author), Sandia Natl Labs, Biotechnol & Bioengn Dept, Livermore, CA USA. EM rmeaghe@sandia.gov; aksingh@sandia.gov FU NIDCR [R01 DE020891]; ENIGMA, a LBNL Scientific Focus Area Program - U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research; US DOE's Nuclear Security Administration [DE-AC04-94AL85000] FX Financial support for the work was provided by the grants: R01 DE020891, funded by the NIDCR and ENIGMA, a LBNL Scientific Focus Area Program supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for US DOE's Nuclear Security Administration under contract DE-AC04-94AL85000. The funder provided support in the form of salaries for authors MR, YKL, RJM, and AKS, but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the 'author contributions' section. NR 42 TC 3 Z9 3 U1 13 U2 28 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAY 4 PY 2016 VL 11 IS 5 AR e0153699 DI 10.1371/journal.pone.0153699 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL5KR UT WOS:000375676400024 PM 27144304 ER PT J AU Loiudice, A Lobaccaro, P Kamali, EA Thao, T Huang, BH Ager, JW Buonsanti, R AF Loiudice, Anna Lobaccaro, Peter Kamali, Esmail A. Thao, Timothy Huang, Brandon H. Ager, Joel W. Buonsanti, Raffaella TI Tailoring Copper Nanocrystals towards C-2 Products in Electrochemical CO2 Reduction SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE colloidal chemistry; electrochemical CO2 reduction; nanocrystals; nanocubes; selectivity ID ACTIVE EDGE SITES; CARBON-DIOXIDE; STRUCTURE SENSITIVITY; ELECTRODES; ETHYLENE; ELECTROREDUCTION; NANOPARTICLES; SELECTIVITY; SURFACES; MOS2 AB Favoring the CO2 reduction reaction (CO2RR) over the hydrogen evolution reaction and controlling the selectivity towards multicarbon products are currently major scientific challenges in sustainable energy research. It is known that the morphology of the catalyst can modulate catalytic activity and selectivity, yet this remains a relatively underexplored area in electrochemical CO2 reduction. Here, we exploit the material tunability afforded by colloidal chemistry to establish unambiguous structure/property relations between Cu nanocrystals and their behavior as electrocatalysts for CO2 reduction. Our study reveals a non-monotonic size-dependence of the selectivity in cube-shaped copper nanocrystals. Among 24nm, 44nm and 63nm cubes tested, the cubes with 44nm edge length exhibited the highest selectivity towards CO2RR (80%) and faradaic efficiency for ethylene (41%). Statistical analysis of the surface atom density suggests the key role played by edge sites in CO2RR. C1 [Loiudice, Anna; Kamali, Esmail A.; Buonsanti, Raffaella] Ecole Polytech Fed Lausanne, Dept Chem Sci & Engn, CH-1950 Sion, Switzerland. [Lobaccaro, Peter; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Lobaccaro, Peter; Huang, Brandon H.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Thao, Timothy; Ager, Joel W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Buonsanti, R (reprint author), Ecole Polytech Fed Lausanne, Dept Chem Sci & Engn, CH-1950 Sion, Switzerland. EM raffaella.buonsanti@epfl.ch FU Berkeley Lab, Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231]; Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub through the Office of Science of the U.S. Department of Energy [DE-SC0004993]; California Energy Commission [500-11-023]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; California Energy Corps program FX We thank Tracy Mattox, at the Molecular Foundry, for elemental analysis of the samples by ICP-AES and Dr. Kendra Kuhl and Dr. Etosha Cave for helpful discussions. The synthetic development and material integration was supported by Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Electrochemical measuraments and product analysis were supported by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. Faradaic efficiency measurements were supported by the California Energy Commission under agreement 500-11-023. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B. H. acknowledges the California Energy Corps program for finalncial support. NR 29 TC 13 Z9 13 U1 68 U2 151 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY 4 PY 2016 VL 55 IS 19 BP 5789 EP 5792 DI 10.1002/anie.201601582 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DK7PP UT WOS:000375118500022 PM 27059162 ER PT J AU Jiang, XY Chen, WY Hartwig, JF AF Jiang, Xingyu Chen, Wenyong Hartwig, John F. TI Iridium-Catalyzed Diastereoselective and Enantioselective Allylic Substitutions with Acyclic -Alkoxy Ketones SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE alkylation; asymmetric catalysis; diastereoselectivity; iridium; ketones ID CARBON QUATERNARY STEREOCENTERS; ASYMMETRIC-SYNTHESIS; ALPHA-ALLYLATION; BUILDING-BLOCKS; ALKYLATION; REGIO; AMINO; CONSTRUCTION; ENANTIO; 5H-OXAZOL-4-ONES AB The asymmetric alkylation of acyclic ketones is a longstanding challenge in organic synthesis. Reported herein are diastereoselective and enantioselective allylic substitutions with acyclic -alkoxy ketones catalyzed by a metallacyclic iridium complex to form products with contiguous stereogenic centers derived from the nucleophile and electrophile. These reactions occur between allyl methyl carbonates and unstabilized copper(I) enolates generated insitu from acyclic -alkoxy ketones. The resulting products can be readily converted into enantioenriched tertiary alcohols and tetrahydrofuran derivatives without erosion of enantiomeric purity. C1 [Jiang, Xingyu; Chen, Wenyong; Hartwig, John F.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Jiang, Xingyu; Chen, Wenyong; Hartwig, John F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Hartwig, JF (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Hartwig, JF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jhartwig@berkeley.edu OI jiang, xingyu/0000-0002-4170-3736 FU Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231]; NIH-NIGMS [GM-55382] FX Financial support provided by the Director, Office of Science, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231 and the NIH-NIGMS (GM-55382). NR 48 TC 9 Z9 9 U1 10 U2 27 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAY 4 PY 2016 VL 55 IS 19 BP 5819 EP 5823 DI 10.1002/anie.201600235 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DK7PP UT WOS:000375118500028 PM 27038004 ER PT J AU Ding, JJ Lapa, P Jain, S Khaire, T Lendinez, S Zhang, W Jungfleisch, MB Posada, CM Yefremenko, VG Pearson, JE Hoffmann, A Novosad, V AF Ding, Junjia Lapa, Pavel Jain, Shikha Khaire, Trupti Lendinez, Sergi Zhang, Wei Jungfleisch, Matthias B. Posada, Christian M. Yefremenko, Volodymyr G. Pearson, John E. Hoffmann, Axel Novosad, Valentine TI Spin Vortex Resonance in Non-planar Ferromagnetic Dots SO SCIENTIFIC REPORTS LA English DT Article ID MAGNETIC VORTEX; DISKS; STATE AB In planar structures, the vortex resonance frequency changes little as a function of an in-plane magnetic field as long as the vortex state persists. Altering the topography of the element leads to a vastly different dynamic response that arises due to the local vortex core confinement effect. In this work, we studied the magnetic excitations in non-planar ferromagnetic dots using a broadband microwave spectroscopy technique. Two distinct regimes of vortex gyration were detected depending on the vortex core position. The experimental results are in qualitative agreement with micromagnetic simulations. C1 [Ding, Junjia; Lapa, Pavel; Jain, Shikha; Khaire, Trupti; Lendinez, Sergi; Zhang, Wei; Jungfleisch, Matthias B.; Posada, Christian M.; Yefremenko, Volodymyr G.; Pearson, John E.; Hoffmann, Axel; Novosad, Valentine] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lapa, Pavel] Texas A&M Univ, College Stn, TX 77843 USA. [Jain, Shikha] HGST, 3403 Yerba Buena Rd, San Jose, CA 95135 USA. [Yefremenko, Volodymyr G.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RP Novosad, V (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM novosad@anl.gov RI Jungfleisch, Matthias Benjamin/G-1069-2015; Novosad, V /J-4843-2015; DING, Junjia/K-2277-2013 OI Jungfleisch, Matthias Benjamin/0000-0001-8204-3677; DING, Junjia/0000-0002-9917-9156 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award # DE-AC02-06CH11357. NR 22 TC 0 Z9 0 U1 0 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 4 PY 2016 VL 6 AR 25196 DI 10.1038/srep25196 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1PH UT WOS:000375403700001 PM 27143405 ER PT J AU Qiu, YH Vlassiouk, I Chen, YF Siwy, ZS AF Qiu, Yinghua Vlassiouk, Ivan Chen, Yunfei Siwy, Zuzanna S. TI Direction Dependence of Resistive-Pulse Amplitude in Conically Shaped Mesopores SO ANALYTICAL CHEMISTRY LA English DT Article ID IONIC CURRENT RECTIFICATION; NANOFLUIDIC DIODE; SINGLE NANOCHANNELS; NANOPORE MEMBRANES; CHARGED-PARTICLES; GLASS NANOPORES; SURFACE-CHARGE; PORES; TRANSPORT; NANOCAPILLARIES AB Conically shaped pores such as glass pipets as well as asymmetric pores in polymers became an important analytics tool used for the detection of molecules, viruses, and particles. Electrokinetic or pressure driven passage of single particles through a single pore causes a transient change of the transmembrane current, called a resistive-pulse, whose amplitude is the measure of the particle volume. The shape of the pulse reflects the pore topography, and in a conical pore, resistive pulses have a shape of a tick point Passage of particles in both directions was reported to produce pulses of the same amplitude and shapes that are mirror images of each other. In this manuscript we identify conditions at which the amplitude of resistive-pulses in a conical mesopore is direction dependent. Neutral particles entering the pore from the larger entrance of a conical pore, called the base, block the current to a larger extent than the particles traveling in the opposite direction. Negatively charged particles on the other hand size larger when being transported in the direction from tip to base. The findings are explained via voltage-regulated ionic concentrations in the pore such that for one voltage polarity a weak depletion zone is formed, which increases the current blockage caused by a particle. For the opposite polarity, an enhancement of ionic concentrations was predicted. The findings reported here are of crucial importance for the resistive-pulse technique, which relates the current blockage with the size of the passing object. C1 [Qiu, Yinghua; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Qiu, Yinghua; Chen, Yunfei] Southeast Univ, Sch Mech Engn, Nanjing 211189, Jiangsu, Peoples R China. [Qiu, Yinghua; Chen, Yunfei] Southeast Univ, Jiangsu Key Lab Design & Mfg Micronano Biomed Ins, Nanjing 211189, Jiangsu, Peoples R China. [Vlassiouk, Ivan] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Siwy, Zuzanna S.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Siwy, Zuzanna S.] Univ Calif Irvine, Dept Biomed Engn, Irvine, CA 92697 USA. RP Siwy, ZS (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA.; Siwy, ZS (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.; Siwy, ZS (reprint author), Univ Calif Irvine, Dept Biomed Engn, Irvine, CA 92697 USA. EM zsiwy@uci.edu RI Vlassiouk, Ivan/F-9587-2010; Qiu, Yinghua/N-6497-2014 OI Vlassiouk, Ivan/0000-0002-5494-0386; Qiu, Yinghua/0000-0003-2489-0784 FU National Science Foundation [CHE 1306058]; Scientific Research Foundation of Graduate School of Southeast University [YBPY 1504]; China Scholarship Council [CSC 201406090034] FX Irradiation with swift heavy ions was performed at the GSI Helmholtzzentrum fur Schwerionenforschung GmbH, Darmstadt, Germany. We thank Chih-Yuan Lin at the Taiwan University for his advice in the Comsol modeling and Timothy Plett and Preston Hinkle at the University of California, Irvine, for helpful discussions. This research was supported by the National Science Foundation (Grant CHE 1306058). Y.Q, acknowledges financial support from the Scientific Research Foundation of Graduate School of Southeast University (Grant YBPY 1504) and the China Scholarship Council (Grant CSC 201406090034). NR 57 TC 6 Z9 7 U1 19 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD MAY 3 PY 2016 VL 88 IS 9 BP 4917 EP 4925 DI 10.1021/acs.analchem.6b00796 PG 9 WC Chemistry, Analytical SC Chemistry GA DR0ZV UT WOS:000379636600046 PM 27049655 ER PT J AU Pudasaini, PR Noh, JH Wong, AT Ovchinnikova, OS Haglund, AV Dai, S Ward, TZ Mandrus, D Rack, PD AF Pudasaini, Pushpa Raj Noh, Joo Hyon Wong, Anthony T. Ovchinnikova, Olga S. Haglund, Amanda V. Dai, Sheng Ward, Thomas Zac Mandrus, David Rack, Philip D. TI Ionic Liquid Activation of Amorphous Metal-Oxide Semiconductors for Flexible Transparent Electronic Devices SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID THIN-FILM TRANSISTORS; FIELD-EFFECT TRANSISTORS; HIGH-PERFORMANCE; LOW-TEMPERATURE; SPRAY-PYROLYSIS; SOL-GEL; PHOTOCHEMICAL ACTIVATION; ZINC-OXIDE; ZNO; MOBILITY AB Amorphous metal-oxide semiconductors offer the high carrier mobilities and excellent large-area uniformity required for high performance, transparent, flexible electronic devices; however, a critical bottleneck to their widespread implementation is the need to activate these materials at high temperatures which are not compatible with flexible polymer substrates. The highly controllable activation of amorphous indium gallium zinc oxide semiconductor channels using ionic liquid gating at room temperature is reported. Activation is controlled by electric field-induced oxygen migration across the ionic liquid-semiconductor interface. In addition to activation of unannealed devices, it is shown that threshold voltages of a transistor can be linearly tuned between the enhancement and depletion modes. Finally, the first ever example of transparent flexible thin film metal oxide transistor on a polyamide substrate created using this simple technique is demonstrated. This study demonstrates the potential of field-induced activation as a promising alternative to traditional postdeposition thermal annealing which opens the door to wide scale implementation into flexible electronic applications. C1 [Pudasaini, Pushpa Raj; Noh, Joo Hyon; Wong, Anthony T.; Haglund, Amanda V.; Mandrus, David; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37931 USA. [Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37931 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Ward, Thomas Zac; Mandrus, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Rack, PD (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.; Rack, PD (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM prack@utk.edu RI Dai, Sheng/K-8411-2015; OI Dai, Sheng/0000-0002-8046-3931; Haglund, Amanda/0000-0003-3973-9577; Ward, Thomas/0000-0002-1027-9186 FU Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4416]; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. DOE [DE-SC0002136] FX P.R.P. and J.H.N. contributed equally to this work. P.R.P. and D.M. acknowledge funding by the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant No. GBMF4416. T.Z.W. and S.D. acknowledge support by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. O.O. acknowledges support by Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. A.T.W. acknowledges U.S. DOE Grant No. DE-SC0002136. P.D.R. acknowledges his contribution (a-IGZO/IL concept and project management) and all the authors acknowledge that the device synthesis was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 46 TC 2 Z9 2 U1 26 U2 47 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAY 3 PY 2016 VL 26 IS 17 BP 2820 EP 2825 DI 10.1002/adfm.201505274 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO2CR UT WOS:000377587800004 ER PT J AU Schimmel, DH Tsvelik, AM Yevtushenko, OM AF Schimmel, D. H. Tsvelik, A. M. Yevtushenko, O. M. TI Low energy properties of the Kondo chain in the RKKY regime SO NEW JOURNAL OF PHYSICS LA English DT Article DE helical symmetry; ideal protected transport; Kondo chain; RKKY ID LATTICE MODEL; QUANTUM WIRES; CLEAVED EDGE; OVERGROWTH; IMPURITIES; TRANSPORT; METALS; PHASE AB We study the Kondo chain in the regime of high spin concentration where the low energy physics is dominated by the Ruderman-Kittel-Kasuya-Yosida interaction. As has been recently shown (Tsvelik and Yevtushenko 2015 Phys. Rev. Lett. 115 216402), this model has two phases with drastically different transport properties depending on the anisotropy of the exchange interaction. In particular, the helical symmetry of the fermions is spontaneously broken when the anisotropy is of the easy plane type. This leads to a parametrical suppression of the localization effects. In the present paper we substantially extend the previous theory, in particular, by analyzing a competition of forward-and backward-scattering, including into the theory short range electron interactions and calculating spin correlation functions. We discuss applicability of our theory and possible experiments which could support the theoretical findings. C1 [Schimmel, D. H.; Yevtushenko, O. M.] Univ Munich, Arnold Sommerfeld Ctr, D-80333 Munich, Germany. [Schimmel, D. H.; Yevtushenko, O. M.] Univ Munich, Ctr Nanosci, D-80333 Munich, Germany. [Tsvelik, A. M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA. [Yevtushenko, O. M.] Univ Erlangen Nurnberg, Inst Theoret Phys, Staudtstr 7, D-91058 Erlangen, Germany. RP Tsvelik, AM (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA. EM tsvelik@gmail.com FU US Department of Energy (DOE), Division of Materials Science [DE-AC02-98CH10886]; DFG [SFB TR-12]; Cluster of Excellence, Nanosystems Initiative Munich; DFG through the Excellence Cluster Nanosystems Initiative Munich [SFB/TR 12, SFB 631] FX AMT acknowledges the hospitality of Ludwig Maximilians University where part of this work was done. AMT was supported by the US Department of Energy (DOE), Division of Materials Science, under Contract No. DE-AC02-98CH10886. OMYe acknowledges support from the DFG through SFB TR-12, and the Cluster of Excellence, Nanosystems Initiative Munich. DHS is supported through by the DFG through the Excellence Cluster Nanosystems Initiative Munich, SFB/TR 12 and SFB 631. We are grateful to Vladimir Yudson and Igor Yurkevich for useful discussions. NR 43 TC 0 Z9 0 U1 4 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAY 3 PY 2016 VL 18 AR 053004 DI 10.1088/1367-2630/18/5/053004 PG 23 WC Physics, Multidisciplinary SC Physics GA DN6MT UT WOS:000377189800002 ER PT J AU Teeguarden, JG Tan, YM Edwards, SW Leonard, JA Anderson, KA Corley, RA Kile, ML Simonich, SM Stone, D Tanguay, RL Waters, KM Harper, SL Williams, DE AF Teeguarden, Justin G. Tan, Yu-Mei Edwards, Stephen W. Leonard, Jeremy A. Anderson, Kim A. Corley, Richard A. Kile, Molly L. Simonich, Staci M. Stone, David Tanguay, Robert L. Waters, Katrina M. Harper, Stacey L. Williams, David E. TI Completing the Link between Exposure Science and Toxicology for Improved Environmental Health Decision Making: The Aggregate Exposure Pathway Framework SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID ADVERSE OUTCOME PATHWAYS; PERSONAL CARE PRODUCTS; CONSUMER EXPOSURE; RISK ASSESSMENTS; MODEL; DOSIMETRY; CHEMICALS; PESTICIDES; EMISSIONS; IMPACT C1 [Teeguarden, Justin G.; Corley, Richard A.; Waters, Katrina M.] Pacific NW Natl Lab, Hlth Effects & Exposure Sci, Richland, WA 99352 USA. [Teeguarden, Justin G.; Anderson, Kim A.; Corley, Richard A.; Simonich, Staci M.; Stone, David; Tanguay, Robert L.; Waters, Katrina M.; Harper, Stacey L.; Williams, David E.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 93771 USA. [Kile, Molly L.] Oregon State Univ, Sch Biol & Populat Hlth Sci, Corvallis, OR 93771 USA. [Tan, Yu-Mei] US EPA, Natl Exposure Res Lab, Durham, NC 27709 USA. [Edwards, Stephen W.] US EPA, Natl Hlth & Environm Effects Res Lab, Durham, NC 27709 USA. [Leonard, Jeremy A.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Harper, Stacey L.] Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. RP Teeguarden, JG (reprint author), Pacific NW Natl Lab, Hlth Effects & Exposure Sci, Richland, WA 99352 USA.; Teeguarden, JG (reprint author), Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 93771 USA. EM justin.teeg-uarden@pnl.gov FU National Institute of Environmental Health Sciences [P42ES016465]; Laboratory Directed Research and Development program at the Pacific Northwest National Laboratory (PNNL); DOE [DE-AC05-76RLO 1830] FX This work (J.G.T.) was supported by P42ES016465 (Oregon State University-PNNL) by the National Institute of Environmental Health Sciences and the Laboratory Directed Research and Development program at the Pacific Northwest National Laboratory (PNNL) and is a contribution of the Global Forensic Chemical Exposure Assessment for the Environmental Exposome project. PNNL is a multiprogram national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RLO 1830. The U.S. Environmental Protection Agency has provided administrative review and has approved for publication. NR 38 TC 8 Z9 8 U1 11 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAY 3 PY 2016 VL 50 IS 9 BP 4579 EP 4586 DI 10.1021/acs.est.5b05311 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DL3GE UT WOS:000375521400001 PM 26759916 ER PT J AU Freytsis, M Knapen, S Robinson, DJ Tsai, Y AF Freytsis, Marat Knapen, Simon Robinson, Dean J. Tsai, Yuhsin TI Gamma-rays from dark showers with twin Higgs models SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Global Symmetries ID EMISSION; SEARCH; MATTER AB We consider a twin WIMP scenario whose twin sector contains a full dark copy of the SM hadrons, where the lightest twin particles are twin pions. By analogy to the standard WIMP paradigm, the dark matter (DM) freezes out through twin electroweak interactions, and annihilates into a dark shower of light twin hadrons. These are either stable or decay predominantly to standard model (SM) photons. We show that this 'hadrosymmetric' scenario can be consistent with all applicable astrophysical, cosmological and collider constraints. In order to decay the twin hadrons before the big-bang nucleosynthesis epoch, an additional portal between the SM and twin sector is required. In most cases we find this additional mediator is within reach of either the LHC or future intensity frontier experiments. Furthermore, we conduct simulations of the dark shower and consequent photon spectra. We find that fits of these spectra to the claimed galactic center gamma-ray excess seen by Fermi-LAT non-trivially coincide with regions of parameter space that both successfully generate the observed DM abundance and exhibit minimal fine-tuning. C1 [Freytsis, Marat] Univ Oregon, Inst Theoret Sci, Eugene, OR 97403 USA. [Knapen, Simon; Robinson, Dean J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Knapen, Simon; Robinson, Dean J.] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tsai, Yuhsin] Univ Maryland, Dept Phys, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. RP Freytsis, M (reprint author), Univ Oregon, Inst Theoret Sci, Eugene, OR 97403 USA.; Knapen, S; Robinson, DJ (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Knapen, S; Robinson, DJ (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Tsai, Y (reprint author), Univ Maryland, Dept Phys, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. EM freytsis@uoregon.edu; smknapen@lbl.gov; djrobinson@berkeley.edu; yhtsai@umd.edu OI Tsai, Yuhsin/0000-0001-7847-225X FU National Science Foundation (NSF) [PHY-1066293]; U.S. Department of Energy (DOE) [DE-SC0011640]; Office of High Energy Physics of the DOE [DE-AC02-05CH11231]; NSF [PHY-1002399, PHY-1315155]; Maryland Center for Fundamental Physics FX The authors thank Zackaria Chacko, David Curtin, Nathaniel Craig, Marco Farina, Andrey Katz, Eric Kuflik, John March-Russell, Michele Papucci, Tracy Slatyer, Matt Strassler, Wei Xue and Yue Zhao for helpful discussions. MF, SK and YT are grateful to the Galileo Galilei Institute for Theoretical Physics for hospitality during the preparation of part of this work. This work was prepared in part at the Aspen Center for Physics, which is supported by National Science Foundation (NSF) grant PHY-1066293. This work was supported in part by: the U.S. Department of Energy (DOE) under contract DE-SC0011640 (MF); the Office of High Energy Physics of the DOE under contract DE-AC02-05CH11231 (SK); the NSF under grant No. PHY-1002399 (DR); and the NSF under grant No. PHY-1315155 and the Maryland Center for Fundamental Physics (YT). NR 101 TC 2 Z9 2 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAY 3 PY 2016 IS 5 AR 018 DI 10.1007/JHEP05(2016)018 PG 36 WC Physics, Particles & Fields SC Physics GA DL5LL UT WOS:000375678400006 ER PT J AU Junghans, A Watkins, EB Majewski, J Miranker, A Stroe, I AF Junghans, Ann Watkins, Erik B. Majewski, Jaroslaw Miranker, Andrew Stroe, Izabela TI Influence of the Human and Rat Islet Amyloid Polypeptides on Structure of Phospholipid Bilayers: Neutron Reflectometry and Fluorescence Microscopy Studies SO LANGMUIR LA English DT Article ID TYPE-2 DIABETES-MELLITUS; PANCREATIC BETA-CELLS; LIPID-BILAYERS; HUMAN AMYLIN; MEMBRANE DISRUPTION; A-BETA; MECHANISM; INSULIN; INTERFACES; IAPP AB Neutron reflectivity (NR) and fluorescent microscopy (FM) were used to study the interactions of human (hIAPP) and rat (rIAPP) islet amyloid polypeptides with several formulations of supported model lipid bilayers at the solid-liquid interface. Aggregation and deposition of islet amyloid polypeptide is correlated with the pathology of many diseases, including Alzheimer's, Parkinson, and type II diabetes (T2DM). A central component of T2DM pathology is the deposition of fibrils in the endocrine pancreas, which is toxic to the insulin secreting beta-cells. The molecular mechanism by which the cell death occurs is not yet understood, but existing evidence points toward interactions of LAPP oligomers with cellular membranes in a manner leading to loss of their integrity. Our NR and FM results showed that the human sequence variant, hIAPP, had little or no effect on bilayers composed of saturated-acyl chains like zwitterionic DPPC, anionic DPPG, and mixed 80:20 mol % DPPC:DPPG bilayers. In marked contrast, the bilayer structure and stability of anionic unsaturated DOPG were sensitive to protein interaction, and the bilayer was partly solubilized by hIAPP under the conditions used here. The rIAPP, which is considered less toxic, had no perturbing effects on any of the above membrane formulations. Understanding the conditions that result in membrane disruption by hIAPP can be crucial in developing counter strategies to fight T2DM and also physicochemically similar neurodegenerative diseases such as Alzheimer's. C1 [Junghans, Ann] Los Alamos Natl Lab, MST Manuel Lujan Jr Neutron Scattering Ctr 7, Los Alamos, NM 87545 USA. [Watkins, Erik B.] Los Alamos Natl Lab, MPA Manuel Lujan Jr Neutron Scattering Ctr 11, Los Alamos, NM 87545 USA. [Majewski, Jaroslaw] Los Alamos Natl Lab, MPA CINT Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Majewski, Jaroslaw] Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. [Miranker, Andrew] Yale Univ, Dept Mol Biophys & Biochem, New Haven, CT 06520 USA. [Stroe, Izabela] Worcester Polytech Inst, Worcester, MA 01609 USA. RP Majewski, J (reprint author), Los Alamos Natl Lab, MPA CINT Manuel Lujan Jr Neutron Scattering Ctr, Los Alamos, NM 87545 USA.; Majewski, J (reprint author), Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. EM jarek@lanl.gov OI Junghans, Sylvia Ann/0000-0001-7061-4663 FU DOE Office of Basic Energy Sciences and Los Alamos National Laboratory under DOE [DE-AC52-06NA25396]; Kalenian Award FX This work benefited from the use of the Lujan Neutron Scattering Center at LANSCE funded by the DOE Office of Basic Energy Sciences and Los Alamos National Laboratory under DOE Contract DE-AC52-06NA25396. I.S. gratefully acknowledges the Kalenian Award for support. We are grateful to Dr. Alex Lacerda (LANL) for encouragement and support for the neutron scattering experiments. We also thank John Bacik for assistance with peptide visualization. NR 66 TC 2 Z9 2 U1 7 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAY 3 PY 2016 VL 32 IS 17 BP 4382 EP 4391 DI 10.1021/acs.langmuir.6b00825 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DL3FY UT WOS:000375520800028 PM 27065348 ER PT J AU Lappi, T Mantysaari, H AF Lappi, T. Mantysaari, H. TI Next-to-leading order Balitsky-Kovchegov equation with resummation SO PHYSICAL REVIEW D LA English DT Article ID COLOR GLASS CONDENSATE; NONLINEAR GLUON EVOLUTION; SMALL-X; BFKL EQUATION; HERA DATA; RENORMALIZATION-GROUP; QCD ANALYSIS; COLLISIONS; JIMWLK; APPROXIMATION AB We solve the Balitsky-Kovchegov evolution equation at next-to-leading order accuracy including a resummation of large single and double transverse momentum logarithms to all orders. We numerically determine an optimal value for the constant under the large transverse momentum logarithm that enables including a maximal amount of the full NLO result in the resummation. When this value is used, the contribution from the alpha(2)(s) terms without large logarithms is found to be small at large saturation scales and at small dipoles. Close to initial conditions relevant for phenomenological applications, these fixed-order corrections are shown to be numerically important. C1 [Lappi, T.] Univ Jyvaskyla, Dept Phys, POB 35, Univ Jyvaskyla 40014, Finland. [Lappi, T.] Helsinki Inst Phys, POB 64, Univ Helsinki 00014, Finland. [Mantysaari, H.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Lappi, T (reprint author), Univ Jyvaskyla, Dept Phys, POB 35, Univ Jyvaskyla 40014, Finland.; Lappi, T (reprint author), Helsinki Inst Phys, POB 64, Univ Helsinki 00014, Finland. FU Academy of Finland [267321, 273464]; DOE [DE-SC0012704] FX We thank D. Triantofyllopoulos and R. Paatelainen for discussions. This work has been supported by the Academy of Finland, Projects No. 267321 and No. 273464, and by computing resources from CSC-IT Center for Science in Espoo, Finland. H. M. is supported under DOE Contract No. DE-SC0012704. NR 54 TC 8 Z9 8 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAY 3 PY 2016 VL 93 IS 9 AR 094004 DI 10.1103/PhysRevD.93.094004 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DL5CN UT WOS:000375655000006 ER PT J AU Pierleoni, C Morales, MA Rillo, G Holzmann, M Ceperley, DM AF Pierleoni, Carlo Morales, Miguel A. Rillo, Giovanni Holzmann, Markus Ceperley, David M. TI Liquid-liquid phase transition in hydrogen by coupled electron-ion Monte Carlo simulations SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE high pressure; phase transitions; quantum Monte Carlo; hydrogen metallization; molecular dissociation ID DENSE SOLID HYDROGEN; GPA 1.4 MBAR; FLUID HYDROGEN; MOLECULAR DISSOCIATION; HIGH-PRESSURE; HOT; METALLIZATION; PLASMA; CONDUCTIVITY; COMPRESSION AB The phase diagram of high-pressure hydrogen is of great interest for fundamental research, planetary physics, and energy applications. A first-order phase transition in the fluid phase between a molecular insulating fluid and a monoatomic metallic fluid has been predicted. The existence and precise location of the transition line is relevant for planetary models. Recent experiments reported contrasting results about the location of the transition. Theoretical results based on density functional theory are also very scattered. We report highly accurate coupled electron-ion Monte Carlo calculations of this transition, finding results that lie between the two experimental predictions, close to that measured in diamond anvil cell experiments but at 25-30 GPa higher pressure. The transition along an isotherm is signaled by a discontinuity in the specific volume, a sudden dissociation of the molecules, a jump in electrical conductivity, and loss of electron localization. C1 [Pierleoni, Carlo] Univ Aquila, Dept Phys & Chem Sci, Via Vetoio 10, I-67010 Laquila, Italy. [Morales, Miguel A.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Rillo, Giovanni] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Holzmann, Markus] CNRS, Lab Phys & Modelisat Milieux Condenses, F-38000 Grenoble, France. [Holzmann, Markus] Univ Grenoble Alpes, F-38000 Grenoble, France. [Ceperley, David M.] Univ Illinois, Dept Phys, Champaign, IL 61801 USA. RP Pierleoni, C (reprint author), Univ Aquila, Dept Phys & Chem Sci, Via Vetoio 10, I-67010 Laquila, Italy.; Ceperley, DM (reprint author), Univ Illinois, Dept Phys, Champaign, IL 61801 USA. EM carlo.pierleoni@aquila.infn.it; ceperley@uiuc.edu RI Pierleoni, Carlo/D-5519-2016 OI Pierleoni, Carlo/0000-0001-9188-3846 FU Italian Institute of Technology under the SEED project [259 SIMBEDD]; Predictive Theory and Modeling for Materials and Chemical Science program by the US Department of Energy (DOE) Office of Science, Basic Energy Sciences; US DOE by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE [NA DE-NA0001789]; Fondation NanoSciences (Grenoble); PRACE [2011050781, 2013091918]; National Science Foundation [OCI 07-25070]; State of Illinois FX We would like to dedicate this work to Peri who has been so important for this collaboration. She will always remain in our hearts. M.H. and C.P. thank the Theory Group at ILL Grenoble for hospitality. C.P. was partially supported by the Italian Institute of Technology under the SEED project 259 SIMBEDD. M.A.M. was supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the US Department of Energy (DOE) Office of Science, Basic Energy Sciences. This work was performed in part under the auspices of the US DOE by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. D.M.C. was supported by DOE Grant NA DE-NA0001789 and by the Fondation NanoSciences (Grenoble). Computer time was provided by PRACE Projects 2011050781 and 2013091918 and by an allocation of the Blue Waters sustained-petascale computing project, supported by the National Science Foundation (Award OCI 07-25070) and the State of Illinois. NR 39 TC 5 Z9 5 U1 5 U2 10 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAY 3 PY 2016 VL 113 IS 18 BP 4953 EP 4957 DI 10.1073/pnas.1603853113 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL1MH UT WOS:000375395700030 PM 27099295 ER PT J AU Stojanoski, V Adamski, CJ Hu, LY Mehta, SC Sankaran, B Zwart, P Prasad, BVV Palzkill, T AF Stojanoski, Vlatko Adamski, Carolyn J. Hu, Liya Mehta, Shrenik C. Sankaran, Banumathi Zwart, Peter Prasad, B. V. Venkataram Palzkill, Timothy TI Removal of the Side Chain at the Active-Site Serine by a Glycine Substitution Increases the Stability of a Wide Range of Serine beta-Lactamases by Relieving Steric Strain SO BIOCHEMISTRY LA English DT Article ID CLASS-A; PROTEIN STABILITY; CRYSTALLOGRAPHIC STRUCTURE; ANTIBIOTIC-RESISTANCE; POLYPEPTIDE BACKBONE; FUNCTION TRADEOFFS; CRYSTAL-STRUCTURE; STRUCTURAL BASES; ALPHA-HELIX; ENZYME AB Serine beta-lactamases are bacterial enzymes Mat hydrolyze beta-lactam antibiotics. They utilize an active-site serine residue as a nucleophile, forming an aryl enzyme intermediate during hydrolysis. In this study, thermal denaturation experiments as well as X-ray crystallography were performed to test the effect of substitution of the catalytic serine with glycine on protein stability in serine beta-lactamases. Six different enzymes comprising representatives from each of the three classes of serine beta-lactamases were examined, including TEM-1, CTX-M-14, and KPC-2 of class A, P99 of class C, and OXA-48 and OXA-163 of class D. For each enzyme, the wild type and a serine-to-glycine mutant were evaluated for stability. The glycine mutants all exhibited enhanced thermostability compared to that of the wild type. In contrast,, alanine substitutions of the catalytic serine in TEM-1, OXA-48, and OXA-163 did not alter stability, suggesting removal of the C beta atom is key to the stability increase associated with the glycine mutants. The X-ray crystal structures of P99 S64G, OXA-48 S70G and S70A, and OXA-163 S70G suggest that removal of the side chain of the catalytic serine releases steric strain to improve enzyme stability. Additionally, analysis of the torsion angles at the nucleophile position indicates that the glycine mutants exhibit improved distance and angular parameters of the intrahelical hydrogen bond network compared to those of the wild-type enzymes, which is also consistent with increased stability. The increased stability of the mutants indicates that the enzyme pays a price in stability for the presence of a side chain at the catalytic serine position but that the cost is necessary in that removal of the serine drastically impairs function. These findings support the stability function hypothesis, which states that active-site residues are optimized for substrate binding and catalysis but that the requirements for catalysis are often not consistent with the requirements for optimal stability. C1 [Stojanoski, Vlatko; Adamski, Carolyn J.; Hu, Liya; Prasad, B. V. Venkataram; Palzkill, Timothy] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, One Baylor Plaza, Houston, TX 77030 USA. [Mehta, Shrenik C.; Palzkill, Timothy] Baylor Coll Med, Dept Pharmacol, One Baylor Plaza, Houston, TX 77030 USA. [Sankaran, Banumathi; Zwart, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol Mol Biophys & Integrated, Adv Light Source, Berkeley, CA 94720 USA. RP Palzkill, T (reprint author), Baylor Coll Med, Dept Pharmacol, One Baylor Plaza, Houston, TX 77030 USA. EM timothyp@bcm.edu FU National Institutes of Health [AI32956]; Robert Welch Grant [Q1279]; National Institute of Allergy and Infectious Diseases [T32 AI55449]; National Institutes of Health; Howard Hughes Medical Institute; Office of Science, and Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH1123]; National Institute of General Medical Sciences FX This work was supported by National Institutes of Health Grant AI32956 to T.P. and Robert Welch Grant Q1279 to B.V.V.P. V.S. is supported by Training grant T32 AI55449 from the National Institute of Allergy and Infectious Diseases. The Berkeley Center for Structural Biology is supported by the National Institutes of Health, National Institute of General Medical Sciences, and the Howard Hughes Medical Institute. The Advanced Light Source is supported by the Director, Office of Science, and Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH1123. NR 71 TC 0 Z9 0 U1 1 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAY 3 PY 2016 VL 55 IS 17 BP 2479 EP 2490 DI 10.1021/acs.biochem.6b00056 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DL3FV UT WOS:000375520500006 PM 27073009 ER PT J AU Choi, YY Tong, S Ducharme, S Roelofs, A Hong, S AF Choi, Yoon-Young Tong, Sheng Ducharme, Stephen Roelofs, Andreas Hong, Seungbum TI Charge collection kinetics on ferroelectric polymer surface using charge gradient microscopy SO SCIENTIFIC REPORTS LA English DT Article ID FIELD-EFFECT TRANSISTOR; TRIBOELECTRIC NANOGENERATORS; ENERGY; POLARIZATION; PIEZORESPONSE; GENERATOR; SENSORS; FILMS AB A charge gradient microscopy (CGM) probe was used to collect surface screening charges on poly(vinylidene fluoride-trifluoroethylene) [P(VDF-TrFE)] thin films. These charges are naturally formed on unscreened ferroelectric domains in ambient condition. The CGM data were used to map the local electric current originating from the collected surface charges on the poled ferroelectric domains in the P(VDF-TrFE) thin films. Both the direction and amount of the collected current were controlled by changing the polarity and area of the poled domains. The endurance of charge collection by rubbing the CGM tip on the polymer film was limited to 20 scan cycles, after which the current reduced to almost zero. This degradation was attributed to the increase of the chemical bonding strength between the external screening charges and the polarization charges. Once this degradation mechanism is mitigated, the CGM technique can be applied to efficient energy harvesting devices using polymer ferroelectrics. C1 [Choi, Yoon-Young; Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Tong, Sheng; Roelofs, Andreas] Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA. [Ducharme, Stephen] Univ Nebraska, Dept Phys & Astron, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. RP Hong, S (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. EM hong@anl.gov RI Tong, Sheng/A-2129-2011; Hong, Seungbum/B-7708-2009; Ducharme, Stephen/A-1909-2009 OI Tong, Sheng/0000-0003-0355-7368; Hong, Seungbum/0000-0002-2667-1983; Ducharme, Stephen/0000-0003-0936-7995 FU Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 32 TC 2 Z9 2 U1 4 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAY 3 PY 2016 VL 6 AR 25087 DI 10.1038/srep25087 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK9YZ UT WOS:000375289600001 PM 27138943 ER PT J AU Kim, JJ Lorenz, R Arold, ST Reger, AS Sankaran, B Casteel, DE Herberg, FW Kim, C AF Kim, Jeong Joo Lorenz, Robin Arold, Stefan T. Reger, Albert S. Sankaran, Banumathi Casteel, Darren E. Herberg, Friedrich W. Kim, Choel TI Crystal Structure of PKG I:cGMP Complex Reveals a cGMP-Mediated Dimeric Interface that Facilitates cGMP-Induced Activation SO STRUCTURE LA English DT Article ID DEPENDENT PROTEIN-KINASE; CAMP BINDING; I-BETA; SELECTIVE ACTIVATION; HOLOENZYME; DOMAIN; REFINEMENT; MODEL AB Cyclic guanosine monophosphate (cGMP)-dependent protein kinase (PKG) is a key regulator of smooth muscle and vascular tone and represents an important drug target for treating hypertensive diseases and erectile dysfunction. Despite its importance, its activation mechanism is not fully understood. To understand the activation mechanism, we determined a 2.5 angstrom crystal structure of the PKG I regulatory (R) domain bound with cGMP, which represents the activated state. Although we used a monomeric domain for crystallization, the structure reveals that two R domains form a symmetric dimer where the cGMP bound at high-affinity pockets provide critical dimeric contacts. Small-angle X-ray scattering and mutagenesis support this dimer model, suggesting that the dimer interface modulates kinase activation. Finally, structural comparison with the homologous cyclic AMP-dependent protein kinase reveals that PKG is drastically different from protein kinase A in its active conformation, suggesting a novel activation mechanism for PKG. C1 [Kim, Jeong Joo; Reger, Albert S.; Kim, Choel] Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA. [Kim, Jeong Joo; Lorenz, Robin; Herberg, Friedrich W.] Univ Kassel, Dept Biochem, D-34132 Kassel, Hesse, Germany. [Arold, Stefan T.] KAUST, Computat Biosci Res Ctr, Div Biol & Environm Sci & Engn, Thuwal 239556900, Saudi Arabia. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. [Casteel, Darren E.] Univ Calif San Diego, Dept Med, La Jolla, CA 92093 USA. [Kim, Choel] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Reger, Albert S.] Patheon Biol STL, St Louis, MO 63134 USA. RP Kim, C (reprint author), Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA.; Kim, C (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. EM ckim@bcm.edu RI Herberg, Friedrich/B-5572-2015 OI Herberg, Friedrich/0000-0001-7117-7653 FU NIH [R01 GM090161, R21 HL111953]; NCI [Y1-CO-1020]; NIGMS [Y1-GM-1104]; CCP4; STFC in the UK; King Abdullah University of Science and Technology (KAUST); Federal Ministry of Education and Research Project NO PAIN [FKZ 0316177F]; European Union (EU) FP7 collaborative project AFFINOMICS [241481]; National Institute of General Medical Sciences; Howard Hughes Medical Institute; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; US DOE program Integrated Diffraction Analysis Technologies (IDAT); NIH project MINOS [R01 GM105404] FX We thank Dr. Gilbert Y. Huang (M.D. Anderson Cancer Center) and the members of Kim's laboratory for critical reading of the manuscript and E. Franz (University of Kassel) for technical support. We specially thank R. Sanishvili, M. Becker, and C. Ogata (GM/CA@APS) for their kind assistance with data collection during the APS-CCP4 summer school in 2012. C.K. was funded by the NIH grants R01 GM090161 and R21 HL111953. The CCP4 school was funded partly by the NCI (Y1-CO-1020), the NIGMS (Y1-GM-1104), a grant from CCP4, and the STFC in the UK. Research by S.T.A. reported in this publication was supported by funding from King Abdullah University of Science and Technology (KAUST). F.W.H. was supported by the Federal Ministry of Education and Research Project NO PAIN (FKZ 0316177F) and the European Union (EU) FP7 collaborative project AFFINOMICS (contract no. 241481). The Berkeley Center for Structural Biology is supported in part by the NIH, the National Institute of General Medical Sciences, and the Howard Hughes Medical Institute. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. The SIBYLS beamline (ALS) is supported in part by US DOE program Integrated Diffraction Analysis Technologies (IDAT) and the NIH project MINOS (R01 GM105404). NR 39 TC 0 Z9 0 U1 0 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD MAY 3 PY 2016 VL 24 IS 5 BP 710 EP 720 DI 10.1016/j.str.2016.03.009 PG 11 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA DL1VG UT WOS:000375420100007 PM 27066748 ER PT J AU Matulef, K Annen, AW Nix, JC Valiyaveetil, FI AF Matulef, Kimberly Annen, Alvin W. Nix, Jay C. Valiyaveetil, Francis I. TI Individual Ion Binding Sites in the K+ Channel Play Distinct Roles in C-type Inactivation and in Recovery from Inactivation SO STRUCTURE LA English DT Article ID NUCLEOTIDE-GATED CHANNELS; SELECTIVITY FILTER; POTASSIUM CHANNELS; SLOW INACTIVATION; STRUCTURAL BASIS; KCSA; ACTIVATION; CONDUCTION; PORE; CONFORMATION AB The selectivity filter of K+ channels contains four ion binding sites (S1-S4) and serves dual functions of discriminating K+ from Na+ and acting as a gate during C-type inactivation. C-type inactivation is modulated by ion binding to the selectivity filter sites, but the underlying mechanism is not known. Here we evaluate how the ion binding sites in the selectivity filter of the KcsA channel participate in C-type inactivation and in recovery from inactivation. We use unnatural amide-to-ester substitutions in the protein backbone to manipulate the S1-S3 sites and a side-chain substitution to perturb the S4 site. We develop an improved semisynthetic approach for generating these amide-to-ester substitutions in the selectivity filter. Our combined electrophysiological and X-ray crystallographic analysis of the selectivity filter mutants show that the ion binding sites play specific roles during inactivation and provide insights into the structural changes at the selectivity filter during C-type inactivation. C1 [Matulef, Kimberly; Annen, Alvin W.; Valiyaveetil, Francis I.] Oregon Hlth & Sci Univ, Dept Physiol & Pharmacol, Program Chem Biol, 3181 Southwest Sam Jackson Pk Rd, Portland, OR 97239 USA. [Nix, Jay C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biol Consortium, Berkeley, CA 94720 USA. RP Valiyaveetil, FI (reprint author), Oregon Hlth & Sci Univ, Dept Physiol & Pharmacol, Program Chem Biol, 3181 Southwest Sam Jackson Pk Rd, Portland, OR 97239 USA. EM valiyave@ohsu.edu FU Office of Science, Office of Basic Energy Sciences, Materials Sciences Division, US Department of Energy at Lawrence Berkeley National Laboratory [DE-AC03-76SF00098]; NIH [GM087546] FX We thank Dr. R. MacKinnon for providing the Fab-expressing hybridoma cells, Daniel Cawley for monoclonal antibody production, and Dr. Michael Chapman and members of the Chapman group for answering our queries on X-ray crystallography. Part of this research was performed at the Advanced Light Source, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences Division, US Department of Energy, under contract no. DE-AC03-76SF00098, at Lawrence Berkeley National Laboratory. This research was supported by a grant from the NIH (GM087546) to F.I.V. NR 60 TC 2 Z9 2 U1 3 U2 8 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD MAY 3 PY 2016 VL 24 IS 5 BP 750 EP 761 DI 10.1016/j.str.2016.02.021 PG 12 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA DL1VG UT WOS:000375420100011 PM 27150040 ER PT J AU Harding, RN Hara, CA Hall, SB Vitalis, EA Thomas, CB Jones, AD Day, JA Tur-Rojas, VR Jorgensen, T Herchert, E Yoder, R Wheeler, EK Farquar, GR AF Harding, Ruth N. Hara, Christine A. Hall, Sara B. Vitalis, Elizabeth A. Thomas, Cynthia B. Jones, A. Daniel Day, James A. Tur-Rojas, Vicente R. Jorgensen, Trond Herchert, Edwin Yoder, Richard Wheeler, Elizabeth K. Farquar, George R. TI Unique DNA-barcoded aerosol test particles for studying aerosol transport SO AEROSOL SCIENCE AND TECHNOLOGY LA English DT Article DE Tiina Reponen ID BIOLOGICAL THREAT AGENTS; SIMULANT; TRACKING AB Data are presented for the first use of novel DNA-barcoded aerosol test particles that have been developed to track the fate of airborne contaminants in populated environments. Until DNATrax (DNA Tagged Reagents for Aerosol eXperiments) particles were developed, there was no way to rapidly validate air transport models with realistic particles in the respirable range of 1-10m in diameter. The DNATrax particles, developed at Lawrence Livermore National Laboratory (LLNL) and tested with the assistance of the Pentagon Force Protection Agency, are the first safe and effective materials for aerosol transport studies that are identified by DNA molecules. The use of unique synthetic DNA barcodes overcomes the challenges of discerning the test material from pre-existing environmental or background contaminants (either naturally occurring or previously released). The DNATrax particle properties are demonstrated to have appropriate size range (approximately 1-4.5m in diameter) to accurately simulate bacterial spore transport. Here, we describe details of the first field test of the DNATrax aerosol test particles in a large indoor facility.Copyright (c) 2016 American Association for Aerosol Research C1 [Harding, Ruth N.; Hara, Christine A.; Hall, Sara B.; Vitalis, Elizabeth A.; Thomas, Cynthia B.; Wheeler, Elizabeth K.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Jones, A. Daniel] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Jones, A. Daniel] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Day, James A.; Tur-Rojas, Vicente R.] Pentagon Force Protect Agcy, Arlington, VA USA. [Jorgensen, Trond; Herchert, Edwin; Yoder, Richard] Parsons Corp, Arlington, VA USA. [Farquar, George R.] SkyeSciences LLC, 2324 Second St, Livermore, CA 94550 USA. RP Farquar, GR (reprint author), SkyeSciences LLC, 2324 Second St, Livermore, CA 94550 USA. EM george@skyesciences.com OI Jones, A. Daniel/0000-0002-7408-6690 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Defense Threat Reduction Agency [DTRA10027-4691]; Lawrence Livermore National Laboratory Lawrence Scholar Program FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and was supported by the Defense Threat Reduction Agency (contract DTRA10027-4691) and the Lawrence Livermore National Laboratory Lawrence Scholar Program. LLNL release number: LLNL-JRNL-669940. NR 16 TC 0 Z9 0 U1 6 U2 10 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0278-6826 EI 1521-7388 J9 AEROSOL SCI TECH JI Aerosol Sci. Technol. PD MAY 3 PY 2016 VL 50 IS 5 BP 429 EP 435 DI 10.1080/02786826.2016.1162903 PG 7 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DJ1FB UT WOS:000373947600002 ER PT J AU Lucachick, G Curran, S Storey, J Prikhodko, V Northrop, WF AF Lucachick, Glenn Curran, Scott Storey, John Prikhodko, Vitaly Northrop, William F. TI Volatility characterization of nanoparticles from single and dual-fuel low temperature combustion in compression ignition engines SO AEROSOL SCIENCE AND TECHNOLOGY LA English DT Article DE Matti Maricq ID CORRELATION GAS-CHROMATOGRAPHY; VAPOR-PRESSURES; VAPORIZATION ENTHALPIES; CONDENSATIONAL GROWTH; PARTICULATE MATTER; DIESEL COMBUSTION; T=298.15 K; N-ALKANES; MODELS AB This work explores the volatility of particles produced from two diesel low temperature combustion (LTC) modes proposed for high-efficiency compression ignition engines. It also explores mechanisms of particulate formation and growth upon dilution in the near-tailpipe environment. The number distribution of exhaust particles from low- and mid-load dual-fuel reactivity controlled compression ignition (RCCI) and single-fuel premixed charge compression ignition (PPCI) modes were experimentally studied over a gradient of dilution temperature. Particle volatility of select particle diameters was investigated using volatility tandem differential mobility analysis (V-TDMA). Evaporation rates for exhaust particles were compared with V-TDMA results for candidate pure n-alkanes to identify species with similar volatility characteristics. The results show that LTC particles are mostly comprised of material with volatility similar to engine oil alkanes. V-TDMA results were used as inputs to an aerosol condensation and evaporation model to support the finding that smaller particles in the distribution are comprised of lower volatility material than large particles under primary dilution conditions. Although our results show that saturation levels are high enough to drive condensation of alkanes onto existing particles under the dilution conditions investigated, they are not high enough to allow homogeneous nucleation of these same compounds in the primary exhaust plume. Therefore, we conclude that observed particles from LTC operation must grow from low concentrations of highly nonvolatile compounds present in the exhaust.Copyright (c) 2016 American Association for Aerosol Research C1 [Lucachick, Glenn; Northrop, William F.] Univ Minnesota, Dept Mech Engn, 111 Church St SE, Minneapolis, MN 55455 USA. [Curran, Scott; Storey, John; Prikhodko, Vitaly] Fuels Engines & Emiss Res Ctr, Oak Ridge Natl Lab, Knoxville, TN USA. RP Northrop, WF (reprint author), Univ Minnesota, Dept Mech Engn, 111 Church St SE, Minneapolis, MN 55455 USA. EM wnorthro@umn.edu FU Oak Ridge National Laboratory Fuels, Engines, and Emissions Research Center; University of Minnesota FX Funding the accommodations of G. Lucachick was provided by Oak Ridge National Laboratory Fuels, Engines, and Emissions Research Center. Funding of the University of Minnesota portion of this work was provided by a research gift from General Motors. NR 34 TC 0 Z9 0 U1 5 U2 12 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0278-6826 EI 1521-7388 J9 AEROSOL SCI TECH JI Aerosol Sci. Technol. PD MAY 3 PY 2016 VL 50 IS 5 BP 436 EP 447 DI 10.1080/02786826.2016.1163320 PG 12 WC Engineering, Chemical; Engineering, Mechanical; Environmental Sciences; Meteorology & Atmospheric Sciences SC Engineering; Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DJ1FB UT WOS:000373947600003 ER PT J AU Chi, H Tan, GJ Kanatzidis, MG Li, Q Uher, C AF Chi, Hang Tan, Gangjian Kanatzidis, Mercouri G. Li, Qiang Uher, Ctirad TI A low-temperature study of manganese-induced ferromagnetism and valence band convergence in tin telluride SO APPLIED PHYSICS LETTERS LA English DT Article ID HIGH THERMOELECTRIC PERFORMANCE; TOPOLOGICAL CRYSTALLINE INSULATOR; THERMAL-CONDUCTIVITY; LATTICE-DYNAMICS; DIRAC-FERMION; SNTE; SEMICONDUCTOR; EFFICIENCY; SNSE; PBTE AB SnTe is renowned for its promise in advancing energy-related technologies based on thermoelectricity and for its topological crystalline insulator character. Here, we demonstrate that each Mn atom introduces similar to 4 mu(B) (Bohr magneton) of magnetic moment to Sn1-xMnxTe. The Curie temperature T-C reaches similar to 14K for x = 0.12, as observed in the field dependent hysteresis of magnetization and the anomalous Hall effect. In accordance with a modified two-band electronic Kane model, the light L-valence-band and the heavy Sigma-valence-band gradually converge in energy with increasing Mn concentration, leading to a decreasing ordinary Hall coefficient R-H and a favorably enhanced Seebeck coefficient S at the same time. With the thermal conductivity kappa lowered chiefly via point defects associated with the incorporation of Mn, the strategy of Mn doping also bodes well for efficient thermoelectric applications at elevated temperatures. Published by AIP Publishing. C1 [Chi, Hang; Uher, Ctirad] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Chi, Hang; Li, Qiang] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Tan, Gangjian; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. RP Chi, H (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA.; Chi, H (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM chihang@bnl.gov RI Chi, Hang/F-1537-2011; OI Chi, Hang/0000-0002-1299-1150; Tan, Gangjian/0000-0002-9087-4048 FU Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001054]; U.S. Department of Energy, Office of Basic Energy Science, Materials Sciences and Engineering Division [DE-SC00112704] FX The work was supported by the Revolutionary Materials for Solid State Energy Conversion, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001054. A part of transport property measurements was performed by H.C. and Q.L. at Brookhaven National Laboratory, which was supported by the U.S. Department of Energy, Office of Basic Energy Science, Materials Sciences and Engineering Division, under Contract No. DE-SC00112704. NR 60 TC 0 Z9 0 U1 20 U2 35 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2016 VL 108 IS 18 AR 182101 DI 10.1063/1.4948523 PG 5 WC Physics, Applied SC Physics GA DN4GY UT WOS:000377023300018 ER PT J AU Merz, TA Noad, H Xu, R Inoue, H Liu, W Hikita, Y Vailionis, A Moler, KA Hwang, HY AF Merz, T. A. Noad, H. Xu, R. Inoue, H. Liu, W. Hikita, Y. Vailionis, A. Moler, K. A. Hwang, H. Y. TI Depth resolved domain mapping in tetragonal SrTiO3 by micro-Laue diffraction SO APPLIED PHYSICS LETTERS LA English DT Article ID STRUCTURAL PHASE-TRANSITION; X-RAY MICRODIFFRACTION; STRONTIUM-TITANATE; THIN-FILMS; LOW-TEMPERATURE; LAALO3/SRTIO3; BIREFRINGENCE; TOPOGRAPHY; BATIO3; STRAIN AB We present depth resolved X-ray micro-Laue diffraction experiments on the low temperature domain structure of SrTiO3. At 80K, monochromatic X-ray diffraction shows an elongated out-of-plane unit cell axis within a matrix of in-plane oriented tetragonal unit cells. Full deviatoric strain mappings from white beam diffraction show a dominance of two tetragonal domain orientations (x- and z-axes) over a large area of sample surface. This information sets an upper bound on domain wall widths and offers a method for studying 3D domain structure at low temperatures. Published by AIP Publishing. C1 [Merz, T. A.; Noad, H.; Inoue, H.; Hikita, Y.; Vailionis, A.; Moler, K. A.; Hwang, H. Y.] Stanford Univ, Geballe Lab Adv Mat, Dept Appl Phys, Stanford, CA 94305 USA. [Noad, H.; Hikita, Y.; Vailionis, A.; Moler, K. A.; Hwang, H. Y.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Xu, R.; Liu, W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Merz, TA (reprint author), Stanford Univ, Geballe Lab Adv Mat, Dept Appl Phys, Stanford, CA 94305 USA. EM tmerz@stanford.edu RI Merz, Tyler/B-2582-2012; Vailionis, Arturas/C-5202-2008; Hikita, Yasuyuki/F-5600-2011 OI Vailionis, Arturas/0000-0001-5878-1864; Hikita, Yasuyuki/0000-0002-7748-8329 FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515]; National Science Foundation Graduate Research Fellowship [DGE-114747]; NSERC of Canada; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX The authors would like to acknowledge support from the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-76SF00515. T.A.M. also acknowledges support from the National Science Foundation Graduate Research Fellowship under Grant No. DGE-114747. H.N. acknowledges support from the NSERC of Canada through a PGS-D. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 41 TC 2 Z9 2 U1 11 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2016 VL 108 IS 18 AR 182901 DI 10.1063/1.4948351 PG 4 WC Physics, Applied SC Physics GA DN4GY UT WOS:000377023300026 ER PT J AU Wickenbrock, A Leefer, N Blanchard, JW Budker, D AF Wickenbrock, Arne Leefer, Nathan Blanchard, John W. Budker, Dmitry TI Eddy current imaging with an atomic radio-frequency magnetometer SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETIC INDUCTION TOMOGRAPHY; SENSORS; SYSTEM; VAPOR; LASER AB We use a radio-frequency Rb-85 alkali-vapor cell magnetometer based on a paraffin-coated cell with long spin-coherence time and a small, low-inductance driving coil to create highly resolved conductivity maps of different objects. We resolve sub-mm features in conductive objects, we characterize the frequency response of our technique, and by operating at frequencies up to 250 kHz we are able to discriminate between differently conductive materials based on the induced response. The method is suited to cover a wide range of driving frequencies and can potentially be used for detecting non-metallic objects with low DC conductivity. Published by AIP Publishing. C1 [Wickenbrock, Arne; Budker, Dmitry] Johannes Gutenberg Univ Mainz, D-55128 Mainz, Germany. [Leefer, Nathan; Blanchard, John W.; Budker, Dmitry] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Budker, Dmitry] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Budker, Dmitry] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Wickenbrock, A (reprint author), Johannes Gutenberg Univ Mainz, D-55128 Mainz, Germany. EM wickenbr@uni-mainz.de OI Blanchard, John/0000-0002-1621-6637 FU DFG through DIP program [FO 703/2-1]; Marie Curie International Incoming Fellowship within European Community; Helmholtz Postdoc Programme FX We acknowledge the support by the DFG through the DIP program (FO 703/2-1). N.L. was supported by a Marie Curie International Incoming Fellowship within the 7th European Community Framework Programme. J.W.B acknowledges support from the Helmholtz Postdoc Programme. NR 26 TC 3 Z9 3 U1 9 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2016 VL 108 IS 18 AR 183507 DI 10.1063/1.4948534 PG 4 WC Physics, Applied SC Physics GA DN4GY UT WOS:000377023300046 ER PT J AU Zhou, ZY Grocke, G Yanguas-Gil, A Wang, XJ Gao, Y Sun, NX Howe, B Chen, X AF Zhou, Ziyao Grocke, Garrett Yanguas-Gil, Angel Wang, Xinjun Gao, Yuan Sun, Nianxiang Howe, Brandon Chen, Xing TI CoFe2/Al2O3/PMNPT multiferroic heterostructures by atomic layer deposition SO APPLIED PHYSICS LETTERS LA English DT Article ID FILMS; NANOPARTICLES; NANOWIRES; METALS AB Multiferroic materials and applications allow electric bias control of magnetism or magnetic bias control of polarization, enabling fast, compact, energy-efficient devices in RF/microwave communication systems such as filters, shifters, and antennas; electronics devices such as inductors and capacitors; and other magnetic material related applications including sensors and memories. In this manuscript, we utilize atomic layer deposition technology to grow magnetic CoFe metallic thin films onto PMNPT, with a similar to 110 Oe electric field induced ferromagnetic resonance field shift in the CoFe/Al2O3/PMNPT multiferroic heterostructure. Our work demonstrates an atomic layer deposition fabricated multiferroic heterostructure with significant tunability and shows that the unique thin film growth mechanism will benefit integrated multiferroic application in near future. Published by AIP Publishing. C1 [Zhou, Ziyao; Grocke, Garrett; Yanguas-Gil, Angel; Chen, Xing] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60517 USA. [Wang, Xinjun; Gao, Yuan; Sun, Nianxiang] Northeastern Univ, Elect & Comp Engn, Boston, MA 02115 USA. [Howe, Brandon] Air Force Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. RP Chen, X (reprint author), Argonne Natl Lab, Div Energy Syst, Lemont, IL 60517 USA. EM xchen@anl.gov RI Sun, Nian Xiang/F-9590-2010; Gao, Yuan/E-4277-2016; OI Sun, Nian Xiang/0000-0002-3120-0094; Gao, Yuan/0000-0002-2444-1180; Chen, Xing/0000-0002-8076-657X FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; [DE-AC02-06CH11357] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. Use of the TEM at the Center for Nanoscale Materials at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under the same contract. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. The funding source for the work reported here did not have a role in study design, data collection, analysis, data interpretation, writing, or in the decision to publish. NR 27 TC 1 Z9 1 U1 20 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAY 2 PY 2016 VL 108 IS 18 AR 182907 DI 10.1063/1.4948977 PG 4 WC Physics, Applied SC Physics GA DN4GY UT WOS:000377023300032 ER PT J AU Barrios, LA Bartual-Murgui, C Peyrecave-Lleixa, E Le Guennic, B Teat, SJ Roubeau, O Aromi, G AF Barrios, Leoni A. Bartual-Murgui, Carlos Peyrecave-Lleixa, Eugenia Le Guennic, Boris Teat, Simon J. Roubeau, Olivier Aromi, Guillem TI Homoleptic versus Heteroleptic Formation of Mononuclear Fe(II) Complexes with Tris-Imine Ligands SO INORGANIC CHEMISTRY LA English DT Article ID SPIN-CROSSOVER COMPOUNDS; CRYSTAL-STRUCTURE; IRON(II); STATE; TRANSFORMATION; PACKING AB We show a marked tendency of Fe(II) to form heteroleptic [Fe(L)(L')](ClO4)(2) complexes from pairs of chelating tris-imine 3bpp, tpy, or 2bbp ligands. New synthetic avenues for spin crossover research become thus available, here illustrated with three new heteroleptic compounds with differing magnetic behaviors: [Fe(H(4)L1)(Cl-tpy)](ClO4)(2)center dot C3H6O (1), [Fe(H2L3)(Me3bpp)](ClO4)(2)center dot C3H6O (2), [Fe(H(4)L1)(2bbp)](ClO4)(2)center dot 3C(3)H(6)O (3). Structural studies demonstrate that 1 is in the low-spin (LS) state up to 350 K, while complexes 2 and 3 are, by contrast, in the high-spin (HS) state down to 2 K, as corroborated through magnetic susceptibility measurements. Upon exposure to the atmosphere, the latter exhibits the release of three molecules of acetone per complex, turning into the solvent-free analogue [Fe(H(4)L1)(2bbp)](ClO4)(2) (3a), through a single-crystal-to-single-crystal transformation. This guest extrusion process is accompanied by a spin switch, from HS to LS. C1 [Barrios, Leoni A.; Bartual-Murgui, Carlos; Peyrecave-Lleixa, Eugenia; Aromi, Guillem] Univ Barcelona, Dept Quim Inorgan, Diagonal 645, Barcelona 08028, Spain. [Bartual-Murgui, Carlos; Roubeau, Olivier] CSIC, ICMA, Plaza San Francisco S-N, E-50009 Zaragoza, Spain. [Bartual-Murgui, Carlos; Roubeau, Olivier] Univ Zaragoza, Plaza San Francisco S-N, E-50009 Zaragoza, Spain. [Le Guennic, Boris] Univ Rennes 1, CNRS, Inst Sci Chim Rennes, UMR 6226, 263 Ave Gen Leclerc, F-35042 Rennes, France. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Aromi, G (reprint author), Univ Barcelona, Dept Quim Inorgan, Diagonal 645, Barcelona 08028, Spain.; Roubeau, O (reprint author), CSIC, ICMA, Plaza San Francisco S-N, E-50009 Zaragoza, Spain.; Roubeau, O (reprint author), Univ Zaragoza, Plaza San Francisco S-N, E-50009 Zaragoza, Spain. EM roubeau@unizar.es; guillem.aromi@qi.ub.es RI Roubeau, Olivier/A-6839-2010; Aromi, Guillem/I-2483-2015; BARRIOS MORENO, LEONI ALEJANDRA/E-5413-2017 OI Roubeau, Olivier/0000-0003-2095-5843; Aromi, Guillem/0000-0002-0997-9484; BARRIOS MORENO, LEONI ALEJANDRA/0000-0001-7075-9950 FU Generalitat de Catalunya; ERC for Starting Grant [258060]; MINECO [MAT2014-53961-R, CTQ2012-32247]; CEI Iberus; ERC [StG 258060]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; GENCI-IDRIS [2014-80649] FX The authors thank the Generalitat de Catalunya for the prize ICREA Academia 2008 and 2013 and the ERC for Starting Grant 258060 (GA), MINECO through MAT2014-53961-R (O.R) and CTQ2012-32247 (GA), the CEI Iberus (C.B.M.), the ERC (StG 258060) for a Predoctoral Fellowship (E.P.L.), and a Postdoctoral contract (LAB.). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy, contract no. DE-AC02-05CH11231 (SJ.T.). Computations were performed (B.L.G.) using HPC resources from GENCI-CINES and GENCI-IDRIS (Grant 2014-80649), which are acknowledged. NR 31 TC 2 Z9 2 U1 7 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 2 PY 2016 VL 55 IS 9 BP 4110 EP 4116 DI 10.1021/acs.inorgchem.5b02058 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DL3FN UT WOS:000375519700006 PM 27074060 ER PT J AU Retuerto, M Skiadopoulou, S Li, MR Abakumov, AM Croft, M Ignatov, A Sarkar, T Abbett, BM Pokorny, J Savinov, M Nuzhnyy, D Prokleska, J Abeykoon, M Stephens, PW Hodges, JP Vanek, P Fennie, CJ Rabe, KM Kamba, S Greenblatt, M AF Retuerto, Maria Skiadopoulou, Stella Li, Man-Rong Abakumov, Artem M. Croft, Mark Ignatov, Alexander Sarkar, Tapati Abbett, Brian M. Pokorny, Jan Savinov, Maxim Nuzhnyy, Dmitry Prokleska, Jan Abeykoon, Milinda Stephens, Peter W. Hodges, Jason P. Vanek, Premysl Fennie, Craig J. Rabe, Karin M. Kamba, Stanislav Greenblatt, Martha TI Pb2MnTeO6 Double Perovskite: An Antipolar Anti-ferromagnet SO INORGANIC CHEMISTRY LA English DT Article ID NEUTRON POWDER DIFFRACTION; MAGNETIC-STRUCTURE; ROOM-TEMPERATURE; PHASE-TRANSITION; FERROELECTRICS; REFINEMENT; NUCLEAR; PBZRO3; PAIR; SR AB Pb2MnTeO6, a new double perovskite, was synthesized. Its crystal structure was determined by synchrotron X-ray and powder neutron diffraction. Pb2MnTeO6 is monoclinic (I2/m) at room temperature with a regular arrangement of all the cations in their polyhedra. However, when the temperature is lowered to similar to 120 K it undergoes a phase transition from I2/m to C2/c structure. This transition is accompanied by a displacement of the Pb atoms from the center of their polyhedra due to the 6s2 lone-pair electrons, together with a surprising off-centering of Mn2+ (d5) magnetic cations. This strong first-order phase transition is also evidenced by specific heat, dielectric, Raman, and infrared spectroscopy measurements. The magnetic characterizations indicate an anti-ferromagnetic (AFM) order below TN approximate to 20 K; analysis of powder neutron diffraction data confirms the magnetic structure with propagation vector k = (0 1 0) and collinear AFM spins. The observed jump in dielectric permittivity near similar to 150 K implies possible anti-ferroelectric behavior; however, the absence of switching suggests that Pb2MnTeO6 can only be antipolar. First-principle calculations confirmed that the crystal and magnetic structures determined are locally stable and that anti-ferroelectric switching is unlikely to be observed in Pb2MnTeO6. C1 [Retuerto, Maria; Li, Man-Rong; Sarkar, Tapati; Greenblatt, Martha] Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. [Skiadopoulou, Stella; Pokorny, Jan; Savinov, Maxim; Nuzhnyy, Dmitry; Vanek, Premysl] Acad Sci Czech Republic, Inst Phys, Na Slovance 2, Prague 18221 8, Czech Republic. [Abakumov, Artem M.] Univ Antwerp, EMAT, Groenenborgerlaan 171, B-2020 Antwerp, Belgium. [Abakumov, Artem M.] Moscow MV Lomonosov State Univ, Dept Chem, Moscow 119991, Russia. [Croft, Mark; Ignatov, Alexander; Rabe, Karin M.] Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. [Abbett, Brian M.; Fennie, Craig J.] Cornell Univ, Dept Appl & Engn Phys, Ithaca, NY 14853 USA. [Prokleska, Jan] Charles Univ Prague, Fac Math & Phys, Dept Condensed Matter Phys, Ke Karlovu 5, CR-12116 Prague, Czech Republic. [Abeykoon, Milinda] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Stephens, Peter W.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Hodges, Jason P.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Retuerto, Maria] CSIC, Inst Catalisis & Petr Quim, Grp Energia & Quim Sostenibles EQS, C Marie Curie 2,L10, Madrid 28049, Spain. [Sarkar, Tapati] Uppsala Univ, Dept Engn Sci, Box 534, SE-75121 Uppsala, Sweden. RP Greenblatt, M (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. EM martha@rutchem.rutgers.ed RI Kamba, Stanislav/G-5332-2014; Retuerto, Maria/D-6425-2014; Prokleska, Jan/B-8814-2017; Vanek, Premysl/G-6211-2014; Pokorny, Jan/F-4569-2011; Skiadopoulou, Stella/C-8855-2016 OI Kamba, Stanislav/0000-0003-4699-869X; Retuerto, Maria/0000-0001-7564-3500; Prokleska, Jan/0000-0003-3246-5112; Vanek, Premysl/0000-0002-7607-3033; Pokorny, Jan/0000-0002-2614-1667; Skiadopoulou, Stella/0000-0001-8871-7302 FU Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; UT-Battelle, LLC.; DOE BES [DE-AC02-98CH10886]; Russian Science Foundation [14-13-00680]; Army Research Office [W911NF-10-1-0345]; Office of Naval Research [N00014-12-1-1040]; Czech Science Foundation [15-08389S]; EU; program of Czech Research Infrastructures [LM2011025]; [NSF-DMR-0966829]; [ARO-DOD-VV911NF-12-1-0172] FX This work was supported by the NSF-DMR-0966829, the ARO-DOD-VV911NF-12-1-0172 grants. Thanks to F. O. Saouma and J. I. Jang for the second harmonic generation measurements. Use of the Spallation Neutron Source is supported by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy (DOE), under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the DOE BES (DE-AC02-98CH10886). A.M.A. is grateful to the Russian Science Foundation for the financial support (Grant No. 14-13-00680). B.M.A. and C.J.F. were supported by the Army Research Office under Grant No. W911NF-10-1-0345. The work of K.M.R. was supported by the Office of Naval Research N00014-12-1-1040. The work in Prague (J.P., M.S., D.N., P.V., and S.K.) was supported by the Czech Science Foundation Project No. 15-08389S. S.S. was supported by EU funding under the 7th Framework Programme (Project NOTEDEV). Heat capacity studies in external magnetic field were performed in MLTL (see: http://mltl.eu), which is supported within the program of Czech Research Infrastructures (Project No. LM2011025). NR 48 TC 1 Z9 1 U1 11 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 2 PY 2016 VL 55 IS 9 BP 4320 EP 4329 DI 10.1021/acs.inorgchem.6b00054 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DL3FN UT WOS:000375519700027 PM 27058393 ER PT J AU Cary, SK Ferrier, MG Baumbach, RE Silver, MA Pacheco, JL Kozimor, SA La Pierre, HS Stein, BW Arico, AA Gray, DL Albrecht-Schmitt, TE AF Cary, Samantha K. Ferrier, Maryline G. Baumbach, Ryan E. Silver, Mark A. Pacheco, Juan Lezama Kozimor, Stosh A. La Pierre, Henry S. Stein, Benjamin W. Arico, Alexandra A. Gray, Danielle L. Albrecht-Schmitt, Thomas E. TI Monomers, Dimers, and Helices: Complexities of Cerium and Plutonium Phenanthrolinecarboxylates SO INORGANIC CHEMISTRY LA English DT Article ID DENSITY-FUNCTIONAL THEORY; 1,10-PHENANTHROLINE-2,9-DICARBOXYLIC ACID; SEQUESTERING AGENTS; COORDINATION; COMPLEXATION; ACTINIDES; METAL; SPECTROSCOPY; NEPTUNIUM; OXIDATION AB The reaction of Ce-III or Pu-III with 1,10-phenanthroline-2,9-dicarboxylic acid (PDAH(2)) results in the formation of new f-element coordination complexes. In the case of cerium, Ce(PDA)(H2O)(2)Cl center dot H2O (1) or [Ce(PDAH)(PDA)](2)[Ce(PDAH)(PDA)] (2) was isolated depending on the Ce/ligand ratio in the reaction. The structure of 2 is composed of two distinct substructures that are constructed from the same monomer. This monomer is composed of a CeIII cation bound by one PDA(2-) dianionic ligand and one PDAH monoanionic ligand, both of which are tetradentate. Bridging by the carboxylate moieties leads to either [Ce(PDAH)(PDA)](2) dimers or [Ce(PDAH)(PDA)](1 infinity) helical chains. For plutonium, Pu(PDA)(2) (3) was the only product isolated regardless of the Pu/ligand ratio employed in the reaction. During the reaction of plutonium with PDAH(2), Pu-III is oxidized to Pu-IV, generating 3. This assignment is consistent with structural metrics and the optical absorption spectrum. Ambiguity in the assignment of the oxidation state of cerium in 1 and 2 from UV-vis-near-IR spectra invoked the use of Ce L-3,L-2-edge X-ray absorption near-edge spectroscopy, magnetic susceptibility, and heat capacity measurements. These experiments support the assignment of Ce-III in both compounds. The bond distances and coordination numbers are also consistent with these assignments. 3 contains 8-coordinate Pu-IV, whereas the cerium centers in 1 and 2 are 9- and/or 10-coordinate, which correlates with the increased size of Ce-III versus Pu-IV. Taken together, these data provide an example of a system where the differences in the redox behavior between these f elements creates more complex chemistry with cerium than with plutonium. C1 [Cary, Samantha K.; Silver, Mark A.; Arico, Alexandra A.; Albrecht-Schmitt, Thomas E.] Florida State Univ, Dept Chem & Biochem, 95 Chieftan Way, Tallahassee, FL 32306 USA. [Ferrier, Maryline G.; Kozimor, Stosh A.; La Pierre, Henry S.; Stein, Benjamin W.] Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. [Baumbach, Ryan E.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Gray, Danielle L.] Univ Illinois, Dept Chem, George L Clark Xray Facil, 505 S Mathews Ave, Urbana, IL 61801 USA. [Gray, Danielle L.] Univ Illinois, Mat Lab 3M, 505 S Mathews Ave, Urbana, IL 61801 USA. [Pacheco, Juan Lezama] Stanford Univ, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA. RP Albrecht-Schmitt, TE (reprint author), Florida State Univ, Dept Chem & Biochem, 95 Chieftan Way, Tallahassee, FL 32306 USA. EM albrecht-schmitt@chem.fsu.edu OI Gray, Danielle/0000-0003-0059-2096 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program [DE-FG02-13ER16414]; Heavy Element Chemistry Program at the LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Glenn T. Seaborg Institute; LANL Director's Postdoctoral Fellowship; National Nuclear Security Administration of U.S. Department of Energy [DE-AC52-06NA25396] FX This research was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Heavy Elements Chemistry Program, under Award DE-FG02-13ER16414. Synchrotron studies were supported under the Heavy Element Chemistry Program at the LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy (Kozimor, Lezama, Trujillo). We are grateful for postdoctoral and graduate fellowships from the Glenn T. Seaborg Institute (Ferrier, Stein) and the LANL Director's Postdoctoral Fellowship (La Pierre). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy (Contract DE-AC52-06NA25396). The synchrotron studies were carried out at the SSRL, a Directorate of the SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. NR 32 TC 1 Z9 1 U1 9 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 2 PY 2016 VL 55 IS 9 BP 4373 EP 4380 DI 10.1021/acs.inorgchem.6b00077 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DL3FN UT WOS:000375519700033 PM 27070401 ER PT J AU Duan, LL Manbeck, GF Kowalczyk, M Szalda, DJ Muckerman, JT Himeda, Y Fujita, E AF Duan, Lele Manbeck, Gerald F. Kowalczyk, Marta Szalda, David J. Muckerman, James T. Himeda, Yuichiro Fujita, Etsuko TI Noninnocent Proton-Responsive Ligand Facilitates Reductive Deprotonation and Hinders CO2 Reduction Catalysis in [Ru(tpy)(6DHBP)(NCCH3)](2+) (6DHBP=6,6 '-(OH)(2)bpy) SO INORGANIC CHEMISTRY LA English DT Article ID MOLECULAR-ORBITAL METHODS; GAUSSIAN-TYPE BASIS; CARBON-DIOXIDE; WATER-OXIDATION; ELECTROCHEMICAL REDUCTION; AQUEOUS-MEDIA; PHOTOCATALYTIC REDUCTION; MECHANISTIC INSIGHT; ORGANIC-MOLECULES; RUTHENIUM COMPLEX AB Ruthenium complexes with proton-responsive ligands [Ru(tpy)(nDHBP)(NCCH3)](CF3SO3)(2) (tpy = 2,2':6',2 ''-terpyridine; nDHBP = n,n'-dihydroxy-2,2'-bipyridine, n = 4 or 6) were examined for reductive chemistry and as catalysts for CO2 reduction. Electrochemical reduction of [Ru(tpy)(nDHBP)(NCCH3)](2+) generates deprotonated species through interligand electron transfer in which the initially formed tpy radical anion reacts with a proton source to produce singly and doubly deprotonated complexes that are identical to those obtained by base titration. A third reduction (i.e., reduction of [Ru(tpy)(nDHBP2H(+))](0)) triggers catalysis of CO2 reduction; however, the catalytic efficiency is strikingly lower than that of unsubstituted [Ru(tpy)(bpy)(NCCH3)](2+) (bpy = 2,2'-bipyridine). Cyclic voltammetry, bulk electrolysis, and spectroelectrochemical infrared experiments suggest the reactivity of CO2 at both the Ru center and the deprotonated quinone-type ligand. The Ru carbonyl formed by the intermediacy of a metallocarboxylic acid is stable against reduction, and mass spectrometry analysis of this product indicates the presence of two carbonates formed by the reaction of DHBP-2H(+) with CO2. C1 [Duan, Lele; Manbeck, Gerald F.; Kowalczyk, Marta; Szalda, David J.; Muckerman, James T.; Fujita, Etsuko] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Szalda, David J.] CUNY Bernard M Baruch Coll, Dept Nat Sci, 17 Lexington Ave, New York, NY 10010 USA. [Himeda, Yuichiro] Natl Inst Adv Ind Sci & Technol, Tsukuba Cent 5-1,1-1-1 Higashi, Tsukuba, Ibaraki 3058565, Japan. RP Muckerman, JT; Fujita, E (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM muckerma@bnl.gov; fujita@bnl.gov OI /0000-0003-1662-5817 FU U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences [DE-SC00112704]; Japan Science and Technology Agency (JST), ACT-C FX The work carried out at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences, under contract DE-SC00112704. Y.H. thanks the Japan Science and Technology Agency (JST), ACT-C, for financial support. NR 91 TC 2 Z9 2 U1 21 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAY 2 PY 2016 VL 55 IS 9 BP 4582 EP 4594 DI 10.1021/acs.inorgchem.6b00398 PG 13 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DL3FN UT WOS:000375519700055 PM 27077460 ER PT J AU Wang, ZM Garnsworthy, AB Andreoiu, C Ball, GC Bender, PC Bildstein, V Cross, DS Demand, G Dunlop, R Evitts, LJ Garrett, PE Hackman, G Hadinia, B Ketelhut, S Krucken, R Leach, KG Laffoley, AT Miller, D Moukaddam, M Pore, J Radich, AJ Rajabali, MM Svensson, CE Tan, A Tardiff, E Unsworth, C Voss, A Voss, P AF Wang, Z. M. Garnsworthy, A. B. Andreoiu, C. Ball, G. C. Bender, P. C. Bildstein, V. Cross, D. S. Demand, G. Dunlop, R. Evitts, L. J. Garrett, P. E. Hackman, G. Hadinia, B. Ketelhut, S. Krucken, R. Leach, K. G. Laffoley, A. T. Miller, D. Moukaddam, M. Pore, J. Radich, A. J. Rajabali, M. M. Svensson, C. E. Tan, A. Tardiff, E. Unsworth, C. Voss, A. Voss, P. TI Observation of a large beta-delayed neutron emission component in Rb-102 decay and identification of excited states in Sr-102 SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR PROPERTIES; R-PROCESS; NUCLEOSYNTHESIS; PROBABILITIES; LIMITS AB The beta decay and beta-delayed neutron emission of Rb-102 have been studied using the 8 pi spectrometer at TRIUMF-ISAC. The level scheme of Sr-102 has been expanded from results of a gamma-gamma coincidence analysis, including the identification of the (4+) member of the ground-state band. The beta-delayed neutron branching ratio of (102)Rbwas found to be significantly larger than previously reported. This larger value has the potential to modify the results of r-process calculations and motivates further measurements as well as refinements of theoretical models. C1 [Wang, Z. M.; Garnsworthy, A. B.; Ball, G. C.; Bender, P. C.; Evitts, L. J.; Hackman, G.; Ketelhut, S.; Krucken, R.; Miller, D.; Moukaddam, M.; Rajabali, M. M.; Tardiff, E.; Unsworth, C.; Voss, A.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Wang, Z. M.; Andreoiu, C.; Cross, D. S.; Pore, J.; Voss, P.] Simon Fraser Univ, Dept Chem, Burnaby, BC V5A 1S6, Canada. [Bildstein, V.; Demand, G.; Dunlop, R.; Garrett, P. E.; Hadinia, B.; Leach, K. G.; Laffoley, A. T.; Radich, A. J.; Svensson, C. E.; Tan, A.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Krucken, R.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Voss, A.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Bender, P. C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Leach, K. G.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Miller, D.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Rajabali, M. M.] Tennessee Technol Univ, Dept Phys, Cookeville, TN 38505 USA. [Tardiff, E.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Unsworth, C.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England. [Voss, A.] Univ Jyvaskyla, FI-40014 Jyvaskyla, Finland. [Voss, P.] Concordia Coll, Dept Phys, Moorhead, MN 56562 USA. RP Garnsworthy, AB (reprint author), TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. EM garns@triumf.ca RI Kruecken, Reiner/A-1640-2013 OI Kruecken, Reiner/0000-0002-2755-8042 FU Natural Sciences and Engineering Research Council of Canada; National Research Council Canada; Canada Research Chairs program FX The authors would like to thank the targets, beam delivery, and operations personnel at TRIUMF-ISAC for providing the radioactive beam. This work was supported in part by the Natural Sciences and Engineering Research Council of Canada. TRIUMF receives federal funding via a contribution agreement through the National Research Council Canada. C.E.S. acknowledges support from the Canada Research Chairs program. NR 27 TC 0 Z9 0 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAY 2 PY 2016 VL 93 IS 5 AR 054301 DI 10.1103/PhysRevC.93.054301 PG 6 WC Physics, Nuclear SC Physics GA DL5AL UT WOS:000375649000003 ER PT J AU Vlcek, V Eisenberg, HR Steinle-Neumann, G Neuhauser, D Rabani, E Baer, R AF Vlcek, Vojtech Eisenberg, Helen R. Steinle-Neumann, Gerd Neuhauser, Daniel Rabani, Eran Baer, Roi TI Spontaneous Charge Carrier Localization in Extended One-Dimensional Systems SO PHYSICAL REVIEW LETTERS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; METAL-INSULATOR-TRANSITION; CONJUGATED POLYMERS; CORRELATION-ENERGY; POLYACETYLENE; EXCITATIONS; OLIGOMERS; DISORDER; IMPACT; REORGANIZATION AB Charge carrier localization in extended atomic systems has been described previously as being driven by disorder, point defects, or distortions of the ionic lattice. Here we show for the first time by means of first-principles computations that charge carriers can spontaneously localize due to a purely electronic effect in otherwise perfectly ordered structures. Optimally tuned range-separated density functional theory and many-body perturbation calculations within the GW approximation reveal that in trans-polyacetylene and polythiophene the hole density localizes on a length scale of several nanometers. This is due to exchange-induced translational symmetry breaking of the charge density. Ionization potentials, optical absorption peaks, excitonic binding energies, and the optimally tuned range parameter itself all become independent of polymer length as it exceeds the critical localization length. Moreover, we find that lattice disorder and the formation of a polaron result from the charge localization in contrast to the traditional view that lattice distortions precede charge localization. Our results can explain experimental findings that polarons in conjugated polymers form instantaneously after exposure to ultrafast light pulses. C1 [Vlcek, Vojtech; Eisenberg, Helen R.; Baer, Roi] Hebrew Univ Jerusalem, Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel. [Vlcek, Vojtech; Steinle-Neumann, Gerd] Univ Bayreuth, Bayer Geoinst, D-95440 Bayreuth, Germany. [Neuhauser, Daniel] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Rabani, Eran] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Berkeley, CA 94720 USA. [Rabani, Eran] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Rabani, Eran] Tel Aviv Univ, Sackler Ctr Computat Mol & Mat Sci, IL-69978 Tel Aviv, Israel. RP Vlcek, V (reprint author), Hebrew Univ Jerusalem, Inst Chem, Fritz Haber Ctr Mol Dynam, IL-91904 Jerusalem, Israel.; Vlcek, V (reprint author), Univ Bayreuth, Bayer Geoinst, D-95440 Bayreuth, Germany. FU Israel-USA Binational Science Foundation [201250]; Minerva Stiftung of the Max Planck Society; NSF [CHE-1112500, CHE-1465064]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Professor Ulrike Salzner and Professor Leeor Kronik for illuminating discussions on polymers and localization in large systems. R. B. and D. N. are supported by The Israel-USA Binational Science Foundation (Grant No. 201250). V. V. is supported by Minerva Stiftung of the Max Planck Society, R. B. gratefully acknowledges support for his sabbatical visit by the Pitzer Center and the Kavli Institute of the University of California, Berkeley. D. N. and E. R. acknowledge support by the NSF, Grants No. CHE-1112500 and No. CHE-1465064, respectively. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and at the Leibniz Supercomputing Center of the Bavarian Academy of Sciences and the Humanities. NR 65 TC 3 Z9 3 U1 4 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAY 2 PY 2016 VL 116 IS 18 AR 186401 DI 10.1103/PhysRevLett.116.186401 PG 6 WC Physics, Multidisciplinary SC Physics GA DL5HF UT WOS:000375667300012 PM 27203334 ER PT J AU Shanavas, KV Satpathy, S AF Shanavas, K. V. Satpathy, S. TI Electronic structure and the origin of the Dzyaloshinskii-Moriya interaction in MnSi SO PHYSICAL REVIEW B LA English DT Article ID WEAK FERROMAGNETISM; BAND-STRUCTURE; SUPEREXCHANGE; CRYSTALS AB The metallic helimagnet MnSi has been found to exhibit skyrmionic spin textures when subjected to magnetic fields at low temperatures. The Dzyaloshinskii-Moriya (DM) interaction plays a key role in stabilizing the skyrmion state. With the help of first-principles calculations, crystal field theory, and a tight-binding model we study the electronic structure and the origin of the DM interaction in the B20 phase of MnSi. The strength of the (D) over right arrow parameter is determined by the magnitude of the spin-orbit interaction and the degree of orbital mixing, induced by the symmetry-breaking distortions in the B20 phase. Our calculations suggest strong coupling between Mn-d and Si-p states, which is consistent with a mixed valence ground state vertical bar d(7-x)p(2+x)> configuration. Consistent with previous calculations, we find that DFT+U leads to the experimental magnetic moment of 0.4 mu(B), which redistributes electrons between the majority and minority spin channels. We derive the magnetic interaction parameters J and (D) over right arrow for Mn-Si-Mn superexchange paths using Moriya's theory assuming the interaction to be mediated by e(g) electrons near the Fermi level. Using parameters from our calculations, we get reasonable agreement with the observations. C1 [Shanavas, K. V.; Satpathy, S.] Univ Missouri, Dept Phys, Columbia, MO 65211 USA. [Shanavas, K. V.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Shanavas, KV (reprint author), Univ Missouri, Dept Phys, Columbia, MO 65211 USA.; Shanavas, KV (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM kavungalvees@ornl.gov FU US Department of Energy [DE-FG02-00ER45818]; Critical Materials Institute, an Energy Innovation Hub - US Department of Energy, Energy Efficiency and Renewable Energy, Advanced Manufacturing Office FX We would like to thank Zoran Popovic for stimulating discussions. The work at MU was supported by the US Department of Energy through Grant No. DE-FG02-00ER45818, and the work at ORNL was supported by the Critical Materials Institute, an Energy Innovation Hub funded by the US Department of Energy, Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. NR 38 TC 1 Z9 1 U1 11 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAY 2 PY 2016 VL 93 IS 19 AR 195101 DI 10.1103/PhysRevB.93.195101 PG 8 WC Physics, Condensed Matter SC Physics GA DL3JN UT WOS:000375530200001 ER PT J AU Zhang, PF Lu, HF Yang, SZ Zhan, WC Zhu, WS Jiang, XG Huang, CL Dai, S AF Zhang, Pengfei Lu, Hanfeng Yang, Shize Zhan, Wangcheng Zhu, Wenshuai Jiang, Xueguang Huang, Caili Dai, Sheng TI Realizing Selective and Aerobic Oxidation by Porous Transition-Metal-Salt@Ceria Catalyst SO CHEMISTRYSELECT LA English DT Article DE Mesoporous Materials; Ionic Liquids; Oxidation; Ceria Catalyst; Template Synthesis ID OXIDE CATALYSTS; LOW-TEMPERATURE; SULFIDE OXIDATION; MOLECULAR-OXYGEN; GOLD CLUSTERS; CO OXIDATION; NANOPARTICLES; COMBUSTION; NITRIDE; SYSTEM AB In the past decades, ceria-based materials have been well developed as catalysts for complete oxidation; however, only a very few studies have involved ceria-promoted selective oxidations. Herein, porous transition-metal-salt-doped ceria (TMS@CeO2) materials (up to 455 m(2)/g) were fabricated by a simple, general co-assembly strategy with ionic liquids as recyclable templates. The TMS@CeO2 catalyst was found to be active in the selective oxidation of sulfides to sulfoxides/sulfones by molecular oxygen. It is interesting that the TMS doping significantly increases the catalytic performance of the original ceria catalyst and, surprisingly, the TMS@CeO2 catalyst showed much higher activity than a transition metal-doped cerium oxide solid solution. The TMS and CeO2 are supposed to synergistically activate O-2 at the interface. It is believed that the abundant ceria-based materials will provide more efficient catalysts for controlled oxidation in the near future. C1 [Zhang, Pengfei; Zhan, Wangcheng; Zhu, Wenshuai; Dai, Sheng] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37830 USA. [Jiang, Xueguang; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Yang, Shize] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA. [Huang, Caili] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN USA. [Lu, Hanfeng] Zhejiang Univ Technol, Inst Catalyt React Engn, Coll Chem Engn, Hangzhou 310014, Peoples R China. RP Dai, S (reprint author), Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37830 USA.; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM dais@ornl.gov OI Yang, Shize/0000-0002-0421-006X FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geo-sciences, and Biosciences Division; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX P.F.Z. and S.D. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geo-sciences, and Biosciences Division. The electron microscopy at ORNL was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and performed in part as a user project at the ORNL Center for Nanophase Materials Sciences, which is a DOE Office of the Science User Facility. NR 41 TC 0 Z9 0 U1 0 U2 0 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2365-6549 J9 CHEMISTRYSELECT JI ChemistrySelect PD MAY 1 PY 2016 VL 1 IS 6 BP 1179 EP 1183 DI 10.1002/slct.201600351 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA EM6CY UT WOS:000395401600012 ER PT J AU Brown, RA Borst, M AF Brown, Robert A. Borst, Michael TI Evaluating the Accuracy of Common Runoff Estimation Methods for New Impervious Hot-Mix Asphalt SO JOURNAL OF SUSTAINABLE WATER IN THE BUILT ENVIRONMENT LA English DT Article DE Runoff; Hot-mix asphalt; Stormwater; Small storm hydrology method; Simple method; SCS-curve number method ID CURVE NUMBERS; CONCRETE AB Accurately predicting runoff volume from impervious surfaces for water quality design events is an important step to meet water quality and infiltration design targets for green infrastructure stormwater control measures. The objectives of this research were to quantify abstraction from a recently paved impervious hot-mix asphalt (HMA) parking lot surface and evaluate the accuracy in modeling runoff volume from small events using the following runoff estimation methods: the Soil Conservation Service Curve Number (SCS-CN) method, the Simple Method (SM), and the Small Storm Hydrology Method (SSHM). A 4,000 m(2) (0.4-ha) parking lot in Edison, New Jersey, was designed with impervious HMA driving lanes evenly draining onto parking lanes constructed with permeable pavement. Ten lined permeable pavement sections that capture all infiltrating water and route it to collection tanks were included in this study. Using a water balance approach on an event basis, the measured infiltrate volume was compared to the rainfall volume across the drainage area to determine the rainfall retained by the HMA surface and in the permeable pavement strata and underlying aggregate. Only events with an antecedent dry period (ADP) less than 24 h (N = 16) were used in this analysis because it minimized evaporation and additional storage in the permeable pavement profile. It was assumed that the rainfall retention depth for these events was completely abstracted in the HMA surface. In comparing measured retention in the HMA surface to the three runoff estimation methods, the SCS-CN method overpredicted abstraction in half of the test sections, and the SM and SSHM underpredicted abstraction in 8 of the 10 test sections. While evaporation from the permeable pavement profile from the events analyzed was small, it was not zero, so the measured rainfall retention depth had a small positive bias. After correcting for this bias, the results shifted closer to the predictions using the SM and SSHM and farther from the predictions using the SCS-CN method. The average and interquartile range (IQR) of the corrected depression storage depth in the HMA surface for the 10 test sections were 2.0 mm and 0.9-3.0 mm, respectively. For a 25.4-mm water quality design event, the predicted abstraction depth by the SM was within the IQR, the SSHM prediction was 0.1 mm below the IQR, and the SCS-CN prediction exceeded the IQR by 2.3 mm. The runoff predicted by the SCS-CN method for this example water quality event was about 15% less than the average and about 10% less than the IQR bound. (C) 2015 American Society of Civil Engineers. C1 [Brown, Robert A.] US EPA, Oak Ridge Inst Sci & Educ, 2890 Woodbridge Ave,MS 104, Edison, NJ 08837 USA. [Borst, Michael] US EPA, 2890 Woodbridge Ave,MS 104, Edison, NJ 08837 USA. RP Brown, RA (reprint author), US EPA, Oak Ridge Inst Sci & Educ, 2890 Woodbridge Ave,MS 104, Edison, NJ 08837 USA. EM rob.brown.rab@gmail.com; borst.mike@epa.gov FU U.S. Department of Energy; U.S. Environmental Protection Agency FX This project was supported in part by an appointment to the Research Participation Program at the National Risk Management Research Laboratory administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. Department of Energy and U.S. Environmental Protection Agency. The parking lot was constructed as a cooperative project with EPA's Office of Administration and Resources Management and Region 2. The authors would like to thank Ms. Lisa Cherry for organizing and analyzing the water level data; PARS Environmental, Inc. for conducting depth-to-volume measurements and providing on-site support; and Johnson, Mirmiran, and Thompson, Inc. for conducting the high-definition survey and assisting with interpretation of the output. NR 23 TC 0 Z9 0 U1 0 U2 1 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 2379-6111 J9 J SUSTAIN WATER BUIL JI J. Sustain. Water Built Environ. PD MAY PY 2016 VL 2 IS 2 AR 04015010 DI 10.1061/JSWBAY.0000806 PG 7 WC Water Resources SC Water Resources GA EJ1BT UT WOS:000392945900002 ER PT J AU Armengaud, E Arnaud, Q Augier, C Benoit, A Berge, L Bergmann, T Billard, J Blumer, J de Boissiere, T Bres, G Broniatowski, A Brudanin, V Camus, P Cazes, A Chapellier, M Charlieux, F Dumoulin, L Eitel, K Filosofov, D Foerster, N Fourches, N Garde, G Gascon, J Gerbier, G Giuliani, A Grollier, M Gros, M Hehn, L Herve, S Heuermann, G Humbert, V De Jesus, M Jin, Y Jokisch, S Juillard, A Kefelian, C Kleifges, M Kozlov, V Kraus, H Kudryavtsev, VA Le-Sueur, H Lin, J Mancuso, M Marnieros, S Menshikov, A Navick, XF Nones, C Olivieri, E Pari, P Paul, B Piro, MC Poda, DV Queguiner, E Robinson, M Rodenas, H Rozov, S Sanglard, V Schmidt, B Scorza, S Siebenborn, B Tcherniakhovski, D Vagneron, L Weber, M Yakushev, E Zhang, X AF Armengaud, E. Arnaud, Q. Augier, C. Benoit, A. Berge, L. Bergmann, T. Billard, J. Bluemer, J. de Boissiere, T. Bres, G. Broniatowski, A. Brudanin, V. Camus, P. Cazes, A. Chapellier, M. Charlieux, F. Dumoulin, L. Eitel, K. Filosofov, D. Foerster, N. Fourches, N. Garde, G. Gascon, J. Gerbier, G. Giuliani, A. Grollier, M. Gros, M. Hehn, L. Herve, S. Heuermann, G. Humbert, V. De Jesus, M. Jin, Y. Jokisch, S. Juillard, A. Kefelian, C. Kleifges, M. Kozlov, V. Kraus, H. Kudryavtsev, V. A. Le-Sueur, H. Lin, J. Mancuso, M. Marnieros, S. Menshikov, A. Navick, X. -F. Nones, C. Olivieri, E. Pari, P. Paul, B. Piro, M. -C. Poda, D. V. Queguiner, E. Robinson, M. Rodenas, H. Rozov, S. Sanglard, V. Schmidt, B. Scorza, S. Siebenborn, B. Tcherniakhovski, D. Vagneron, L. Weber, M. Yakushev, E. Zhang, X. CA Edelweiss Collaboration TI Constraints on low-mass WIMPs from the EDELWEISS-III dark matter search SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter detectors; dark matter experiments ID GERMANIUM DETECTORS; CANDIDATES; PROSPECTS AB We present the results of a search for elastic scattering from galactic dark matter in the form of Weakly Interacting Massive Particles (WIMPs) in the 4-30 GeV/c(2) mass range. We make use of a 582 kg-day fiducial exposure from an array of 800 g Germanium bolometers equipped with a set of interleaved electrodes with full surface coverage. We searched specifically for similar to 2.5-20 keV nuclear recoils inside the detector fiducial volume. As an illustration the number of observed events in the search for 5 (resp. 20) GeV/c(2) WIMPs are 9 (resp. 4), compared to an expected background of 6.1 (resp. 1.4). A 90% CL limit of 4.3 x 10(-4)0 cm(2) (resp. 9.4 x 10(-44) cm(2)) is set on the spin-independent WIMP-nucleon scattering cross-section for 5 (resp. 20) GeV/c(2) WIMPs. This result represents a 41-fold improvement with respect to the previous EDELWEISS-II low-mass WIMP search for 7 GeV/c(2) WIMPs. The derived constraint is in tension with hints of WIMP signals from some recent experiments, thus confirming results obtained with different detection techniques. C1 [Armengaud, E.; de Boissiere, T.; Fourches, N.; Gros, M.; Herve, S.; Navick, X. -F.; Nones, C.; Paul, B.] CEA Saclay, DSM, IRFU, F-91191 Gif Sur Yvette, France. [Arnaud, Q.; Augier, C.; Benoit, A.; Billard, J.; Cazes, A.; Gascon, J.; De Jesus, M.; Juillard, A.; Kefelian, C.; Queguiner, E.; Sanglard, V.; Vagneron, L.] UCBL, CNRS, IN2P3, Inst Phys Nucl Lyon, 4 Rue Enrico Fermi, F-69622 Villeurbanne, France. [Armengaud, E.; Arnaud, Q.] Queens Univ, Kingston, ON K7L 3N6, Canada. [Piro, M. -C.] Rensselaer Polytech Inst, Troy, NY USA. [Piro, M. -C.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Benoit, A.; Bres, G.; Camus, P.; Garde, G.; Grollier, M.; Rodenas, H.] UJF, CNRS, Inst Neel, 25 Rue Martyrs,BP 166, F-38042 Grenoble, France. [Berge, L.; Broniatowski, A.; Chapellier, M.; Dumoulin, L.; Giuliani, A.; Humbert, V.; Le-Sueur, H.; Mancuso, M.; Marnieros, S.; Olivieri, E.; Piro, M. -C.] Univ Paris Saclay, Univ Paris 11, CSNSM, CNRS IN2P3, F-91405 Orsay, France. [Bergmann, T.; Kleifges, M.; Menshikov, A.; Tcherniakhovski, D.; Weber, M.] Karlsruhe Inst Technol, Inst Prozessdatenverarbeitung & Elekt, Postfach 3640, D-76021 Karlsruhe, Germany. [Bluemer, J.; Foerster, N.; Heuermann, G.; Kefelian, C.; Scorza, S.] Karlsruhe Inst Technol, Inst Expt Kernphys, Gaedestr 1, D-76128 Karlsruhe, Germany. [Bluemer, J.; Eitel, K.; Hehn, L.; Jokisch, S.; Kozlov, V.; Schmidt, B.; Siebenborn, B.] Karlsruhe Inst Technol, Inst Kernphys, Postfach 3640, D-76021 Karlsruhe, Germany. [Brudanin, V.; Filosofov, D.; Rozov, S.; Yakushev, E.] JINR, Lab Nucl Problems, Joliot Curie 6, Dubna 141980, Moscow Region, Russia. [Jin, Y.] CNRS, Route Nozay, Lab Photon & Nanostruct, F-91460 Marcoussis, France. [Kraus, H.; Lin, J.; Zhang, X.] Univ Oxford, Dept Phys, Keble Rd, Oxford OX1 3RH, England. [Kudryavtsev, V. A.; Robinson, M.] Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England. [Pari, P.] CEA Saclay, IRAMIS, DSM, F-91191 Gif Sur Yvette, France. RP Armengaud, E (reprint author), CEA Saclay, DSM, IRFU, F-91191 Gif Sur Yvette, France. EM eric.armengaud@cea.fr RI Kozlov, Valentin/B-8884-2008; OI Kozlov, Valentin/0000-0002-8770-3619; Lin, Junsong/0000-0002-9970-8150; Kudryavtsev, Vitaly/0000-0002-7018-5827 FU German ministry of science and education (BMBF Verbundforschung ATP Proj.) [05A14VKA]; Helmholtz Alliance for Astroparticle Phyics (HAP); French Agence Nationale pour la Recherche (ANR); LabEx Lyon Institute of Origins of the Universite de Lyon within the program "Investissements d'Avenir" [ANR-11-IDEX-00007, ANR-10-LABX-0066]; P2IO LabEx [ANR-10-LABX-0038, ANR-11-IDEX-0003-01]; Science and Technology Facilities Council (U.K); Russian Foundation for Basic Research [15-02-03561] FX The help of the technical staff of the Laboratoire Souterrain de Modane and the participant laboratories is gratefully acknowledged. The EDELWEISS project is supported in part by the German ministry of science and education (BMBF Verbundforschung ATP Proj.-Nr. 05A14VKA), by the Helmholtz Alliance for Astroparticle Phyics (HAP), by the French Agence Nationale pour la Recherche (ANR) and the LabEx Lyon Institute of Origins (ANR-10-LABX-0066) of the Universite de Lyon within the program "Investissements d'Avenir" (ANR-11-IDEX-00007), by the P2IO LabEx (ANR-10-LABX-0038) in the framework "Investissements d'Avenir" (ANR-11-IDEX-0003-01) managed by the ANR (France), by Science and Technology Facilities Council (U.K.), and the Russian Foundation for Basic Research (grant No. 15-02-03561). NR 45 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAY PY 2016 IS 5 AR 019 DI 10.1088/1475-7516/2016/05/019 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DO8NY UT WOS:000378041500020 ER PT J AU Bertoni, B Hooper, D Linden, T AF Bertoni, Bridget Hooper, Dan Linden, Tim TI Is the gamma-ray source 3FGL J2212.5+0703 a dark matter subhalo? SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter theory; gamma ray experiments ID 2ND SOURCE CATALOG; ALL-SKY SURVEY; MILKY-WAY; FERMI-LAT; X-RAY; ANNIHILATION SIGNAL; GALAXY CANDIDATES; ENERGY SURVEY; SEARCH; DISCOVERY AB In a previous paper, we pointed out that the gamma-ray source 3FGL J2212.5+ 0703 shows evidence of being spatially extended. If a gamma-ray source without detectable emission at other wavelengths were unambiguously determined to be spatially extended, it could not be explained by known astrophysics, and would constitute a smoking gun for dark matter particles annihilating in a nearby subhalo. With this prospect in mind, we scrutinize the gamma-ray emission from this source, finding that it prefers a spatially extended profile over that of a single point-like source with 5.10-statistical significance. We also use a large sample of active galactic nuclei and other known gamma-rays sources as a control group, confirming, as expected, that statistically significant extension is rare among such objects. We argue that the most likely (non-dark matter) explanation for this apparent extension is a pair of bright gamma-ray sources that serendipitously lie very close to each other, and estimate that there is a chance probability of similar to 2% that such a pair would exist somewhere on the sky. In the case of 3FGL J2212.5+0703, we test an alternative model that includes a second gamma-ray point source at the position of the radio source BZQ J2212+0646, and find that the addition of this source alongside a point source at the position of 3FGL J2212.5+0703 yields a fit of comparable quality to that obtained for a single extended source. If 3FGL J2212.5+0703 is a dark matter subhalo, it would imply that dark matter particles have a mass of similar to 18-33 GeV and an annihilation cross section on the order of sigma v similar to 10(-26) cm(3)/s (for the representative case of annihilations to bb), similar to the values required to generate the Galactic Center gamma-ray excess. C1 [Bertoni, Bridget] Univ Washington, Inst Nucl Theory, Box 351550, Seattle, WA 98195 USA. [Bertoni, Bridget] Stanford Univ, Stanford Inst Theoret Phys, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. [Bertoni, Bridget] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94305 USA. [Bertoni, Bridget] Univ Washington, Dept Phys, Box 351560, Seattle, WA 98195 USA. [Hooper, Dan] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Linden, Tim] Ohio State Univ, CCAPP, 191 West Woodruff Ave, Columbus, OH 43210 USA. [Linden, Tim] Univ Chicago, Kavli Inst Cosmol Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. RP Bertoni, B (reprint author), Univ Washington, Inst Nucl Theory, Box 351550, Seattle, WA 98195 USA.; Bertoni, B (reprint author), Stanford Univ, Stanford Inst Theoret Phys, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA.; Bertoni, B (reprint author), Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94305 USA.; Bertoni, B (reprint author), Univ Washington, Dept Phys, Box 351560, Seattle, WA 98195 USA. EM bbertoni@stanford.edu; dhooper@fnal.gov; linden.70@osu.edu FU US Department of Energy Office of Science Graduate Student Research (SCGSR) Program [DE-AC05-06OR23100]; US Department of Energy [DE-FG02-00ER41132, DE-SC0011637, DE-SC0012012, DE-FG02-13ER41958, DE-AC02-07CH11359]; National Aeronautics and Space Administration through Einstein Postdoctoral Fellowship [PF3-140110]; University of Chicago Research Computing Center; Ohio Supercomputer Center FX We would like to thank Alex Drlica-Wagner, Keith Bechtol, Frank Schninzel, Elizabeth Ferrara, Fernando Camilo, Paul Ray and Eric Charles for valuable discussions. BB is supported by the US Department of Energy Office of Science Graduate Student Research (SCGSR) Program under Contrast No. DE-AC05-06OR23100 and the US Department of Energy under Contract Nos. DE-FG02-00ER41132, DE-SC0011637, and DE-SC0012012. DH is supported by the US Department of Energy under contract DE-FG02-13ER41958. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the US Department of Energy. TL is supported by the National Aeronautics and Space Administration through Einstein Postdoctoral Fellowship Award No. PF3-140110. We acknowledge the University of Chicago Research Computing Center and the Ohio Supercomputer Center for providing support for this work. NR 83 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAY PY 2016 IS 5 AR 049 DI 10.1088/1475-7516/2016/05/049 PG 24 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DO8NY UT WOS:000378041500050 ER PT J AU Foreman, S Perrier, H Senatore, L AF Foreman, Simon Perrier, Hideki Senatore, Leonardo TI Precision comparison of the power spectrum in the EFTofLSS with simulations SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE cosmological perturbation theory; power spectrum; cosmic web; cosmological simulations ID COSMOLOGICAL PERTURBATION-THEORY; UNIVERSE; EMULATION; MODELS AB We study the prediction of the dark matter power spectrum at two-loop order in the Effective Field Theory of Large Scale Structures (EFTofLSS) using high precision numerical simulations. In our universe, short distance non-linear fluctuations, not under perturbative control, affect long distance fluctuations through an effective stress tensor that needs to be parametrized in terms of counterterms that are functions of the long distance fluctuating fields. We find that at two-loop order it is necessary to include three counterterms: a linear term in the overdensity, delta, a quadratic term, delta(2), and a higher derivative term, partial derivative(2)delta. After the inclusion of these three terms, the EFTofLSS at two-loop order matches simulation data up to k similar or equal to 0.34 h Mpc(-1) at redshift z = 0, up to k similar or equal to 0.55 h Mpc(-1) at z = 1, and up to k similar or equal to 1.1 hMpc(-1) at z = 2. At these wavenumbers, the cosmic variance of the simulation is at least as small as 10(-3), providing for the first time a high precision comparison between theory and data. The actual reach of the theory is affected by theoretical uncertainties associated to not having included higher order terms in perturbation theory, for which we provide an estimate, and by potentially overfitting the data, which we also try to address. Since in the EFTofLSS the coupling constants associated with the counterterms are unknown functions of time, we show how a simple parametrization gives a sensible description of their time-dependence. Overall, the k-reach of the EFTofLSS is much larger than previous analytical techniques, showing that the amount of cosmological information amenable to high-precision analytical control might be much larger than previously believed. C1 [Foreman, Simon; Senatore, Leonardo] Stanford Univ, Stanford Inst Theoret Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA. [Foreman, Simon; Senatore, Leonardo] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA. [Foreman, Simon; Senatore, Leonardo] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Foreman, Simon; Senatore, Leonardo] SLAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Foreman, Simon; Senatore, Leonardo] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA. [Perrier, Hideki] Univ Geneva, Dept Theoret Phys, 24 Quai E Ansermet, CH-1211 Geneva 4, Switzerland. [Perrier, Hideki] CAP, 24 Quai E Ansermet, CH-1211 Geneva 4, Switzerland. RP Foreman, S (reprint author), Stanford Univ, Stanford Inst Theoret Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA.; Foreman, S (reprint author), Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA.; Foreman, S (reprint author), Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Foreman, S (reprint author), SLAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Foreman, S (reprint author), Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA. EM sfore@stanford.edu; senatore@stanford.edu; hideki.perrier@unige.ch FU Natural Sciences and Engineering Research Council of Canada; Swiss National Science Foundation (SNSF) [200021140236]; DOE [DE-FG02-12ER41854]; NSF [PHY-1068380] FX We thank Risa Wechsler and Sam Skillman for providing the power spectrum measurements from the Dark Sky simulation. A few days earlier than our paper was submitted, ref. [15, 16] appeared, which have some overlap with our paper. Indeed, we had communicated with the authors and had mutually exchanged drafts prior to the respective submissions. Indeed we wish to thank Tobias Baldauf and Matias Zaldarriaga for discussions. S.F. is partially supported by the Natural Sciences and Engineering Research Council of Canada. H.P. is supported by the Swiss National Science Foundation (SNSF), project "The non-Gaussian Universe" (project number: 200021140236). L.S. is supported by DOE Early Career Award DE-FG02-12ER41854 and by NSF grant PHY-1068380. NR 46 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAY PY 2016 IS 5 AR 027 DI 10.1088/1475-7516/2016/05/027 PG 40 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DO8NY UT WOS:000378041500028 ER PT J AU Sunayama, T Padmanabhan, N Heitmann, K Habib, S Rangel, E AF Sunayama, Tomomi Padmanabhan, Nikhil Heitmann, Katrin Habib, Salman Rangel, Esteban TI Efficient construction of mock catalogs for baryon acoustic oscillation surveys SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE cosmological simulations; baryon acoustic oscillations; galaxy clusters; red-shift surveys ID SDSS-III; SPECTROSCOPIC SURVEY; COSMOLOGICAL SIMULATIONS; GALAXY CATALOGS; HALO; UNIVERSE; RELEASE; SCALE; PREDICTIONS; SAMPLE AB Precision measurements of the large scale structure of the Universe require large numbers of high fidelity mock catalogs to accurately assess, and account for. the presence of systematic effects. We introduce and test a scheme for generating mock catalogs rapidly using suitably derated N-body simulations. Our aim is to reproduce the large scale structure and the gross properties of dark matter halos with high accuracy, while sacrificing the details of the halo's internal structure. By adjusting global and local time-steps in an N-body code. we demonstrate that we recover halo masses to better than 0.5% and the power spectrum to better than 1% both in real and redshift space for k = 1hMpc(-1), while requiring a factor of 4 less CPU time. We also calibrate the redshift spacing of outputs required to generate simulated light cones. We find that outputs separated by Delta z = 0.05 allow us to interpolate particle positions and velocities to reproduce the real and redshift space power spectra to better than 1% (out to k = 1hMpc(-1)). We apply these ideas to generate a suite of simulations spanning a range of cosmologies, motivated by the Baryon Oscillation Spectroscopic Survey (BOSS) but broadly applicable to future large scale structure surveys including eBOSS and DESI. As an initial demonstration of the utility of such simulations. we calibrate the shift in the baryonic acoustic oscillation peak position as a function of galaxy bias with higher precision than has been possible so far. This paper also serves to document the simulations, which we make publicly available. C1 [Sunayama, Tomomi; Padmanabhan, Nikhil] Yale Univ, Dept Phys, 260 Whitney Ave, New Haven, CT 06511 USA. [Heitmann, Katrin; Habib, Salman; Rangel, Esteban] Argonne Natl Lab, High Energy Phys & Math Div, 9700 S Cass Ave, Lemont, IL 60439 USA. [Heitmann, Katrin; Habib, Salman; Rangel, Esteban] Argonne Natl Lab, Div Comp Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. [Rangel, Esteban] Northwestern Univ, Dept Elect Engn & Comp Sci, 2145 Sheridan Rd, Evanston, IL 60620 USA. RP Sunayama, T (reprint author), Yale Univ, Dept Phys, 260 Whitney Ave, New Haven, CT 06511 USA. EM tomomi.sunayama@yale.edu; nikhil.padmanabhan@yale.edu; heitmann@anl.gov; habib@anl.gov; steverangel@u.northwestern.edu FU DOE [DE-SC0008080]; U.S. Department of Energy [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX NP and TS acknowledge support from the DOE Early Career Grant DE-SC0008080. This work was supported in part by the facilities and staff of the Yale University Faculty of Arts and Sciences High Performance Computing Center. TS would like to thank Andrew Szymkowiak for useful discussions. SH, KH, and ER record their indebtedness to other HACC team members - Hal Finkel, Nicholas Frontiere, Vitali Morozov, Adrian Pope - for their assistance and contributions. The work of SH, KH, and ER at Argonne National Laboratory work was supported under the U.S. Department of Energy contract DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD MAY PY 2016 IS 5 AR 051 DI 10.1088/1475-7516/2016/05/051 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DO8NY UT WOS:000378041500052 ER PT J AU Sun, K Liu, HL Gan, H AF Sun, Ke Liu, Helen Gan, Hong TI Cathode Loading Effect on Sulfur Utilization in Lithium-Sulfur Battery SO JOURNAL OF ELECTROCHEMICAL ENERGY CONVERSION AND STORAGE LA English DT Article DE lithium-sulfur battery; sulfur utilization; sulfur loading; activation ID LI-S BATTERIES; ENERGY DENSITY; CHEMISTRY AB The lithium-sulfur (Li-S) battery is under intensive research in recent years due to its potential to provide higher energy density and lower cost than the current state-of-the-art lithium-ion battery technology. To meet cost target for transportation application, high-sulfur loading up to 8 mAh cm(-2) is predicted by modeling. In this work, we have investigated the sulfur loading effect on the galvanostatic charge/discharge cycling performance of Li-S cells with theoretical sulfur loading ranging from 0.5 to 7.5 mAh cm(-2). We found that the low sulfur utilization of electrodes with sulfur loading of > 3.0 mAh cm(-2) is due to their inability to deliver capacities at the voltage plateau of 2.1 V, which corresponds to the conversion of soluble Li2S4 to insoluble Li2S2/Li2S. This electrochemical conversion process recovers to deliver the expected sulfur utilization after several activation cycles for electrodes with sulfur loading up to 4.5 mAh cm(-2). For electrodes with 7.0 mAh cm(-2) loading, no sulfur utilization recovery was observed for 100 cycles. The root cause of this phenomenon is elucidated by SEM/EDS and EIS investigation. Carboninter-layer cell design and low-rate discharge activation are demonstrated to be effective mitigation methods. C1 [Sun, Ke; Gan, Hong] Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. [Liu, Helen] SUNY Stony Brook, Dept Mat Sci & Chem Engn, Stony Brook, NY 11790 USA. RP Gan, H (reprint author), Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. EM hgan@bnl.gov FU U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy under the Advanced Battery Materials Research (BMR) program [DE-SC0012704]; DOE, Office of Basic Energy Sciences [DE-SC0012704]; DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI) FX This work was supported by the U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy under the Advanced Battery Materials Research (BMR) program Contract No. DE-SC0012704. Part of this work has been carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the DOE, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. Helen Liu was supported by the DOE, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships Program (SULI). NR 25 TC 0 Z9 0 U1 10 U2 10 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 2381-6872 EI 2381-6910 J9 J ELECTROCHEM ENERGY JI J. Electrochem. Energy Convers. Storage PD MAY PY 2016 VL 13 IS 2 AR UNSP 021002 DI 10.1115/1.4034738 PG 9 WC Electrochemistry; Energy & Fuels SC Electrochemistry; Energy & Fuels GA EF2ZI UT WOS:000390193700002 ER PT J AU Weker, JN Huang, XJ Toney, MF AF Weker, Johanna Nelson Huang, Xiaojing Toney, Michael F. TI In situ X-ray-based imaging of nano materials SO CURRENT OPINION IN CHEMICAL ENGINEERING LA English DT Article ID SCAN PTYCHOGRAPHY; NANOSCALE; NANOTOMOGRAPHY; MICROSCOPY; NANOPARTICLES; LITHIATION; TOMOGRAPHY; NANOWIRES; DYNAMICS; ANODES AB Functional nanomaterials are heterogeneous and understanding their behavior during synthesis and operation requires high resolution diagnostic imaging tools that can be used in situ. Over the past decade, huge progress has been made in the development of X-ray based imaging, including full field and scanning microscopy and their analogs in coherent diffractive imaging. Currently, spatial resolution of about 10 nm and time resolution of sub-seconds are achievable. For catalysis, X-ray imaging allows tracking of particle chemistry under reaction conditions. In energy storage, in situ X-ray imaging of electrode particles is providing important insight into degradation processes. Recently, both spatial and temporal resolutions are improving to a few nm and milliseconds and these developments will open up unprecedented opportunities. C1 [Weker, Johanna Nelson; Toney, Michael F.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Huang, Xiaojing] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Toney, MF (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM mftoney@slac.stanford.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515, DE-SC0012704]; Department of Energy, Laboratory Direct Research and Development [DE-AC02-76SF00515] FX Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. JNW was partly supported by the Department of Energy, Laboratory Direct Research and Development funding, under contract DE-AC02-76SF00515. Work at the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science, under Contract No. DE-SC0012704. NR 36 TC 0 Z9 0 U1 4 U2 4 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 2211-3398 J9 CURR OPIN CHEM ENG JI Curr. Opin. Chem. Eng. PD MAY PY 2016 VL 12 BP 14 EP 21 DI 10.1016/j.coche.2016.01.006 PG 8 WC Biotechnology & Applied Microbiology; Engineering, Chemical SC Biotechnology & Applied Microbiology; Engineering GA ED0DK UT WOS:000388513000005 ER PT J AU Frei, H AF Frei, Heinz TI Water oxidation investigated by rapid-scan FT-IR spectroscopy SO CURRENT OPINION IN CHEMICAL ENGINEERING LA English DT Article ID OXYGEN EVOLUTION REACTION; IN-SITU FORMATION; COBALT OXIDE; EVOLVING CATALYST; NEUTRAL PH; CO3O4; PHOSPHATE; EFFICIENT; ELECTROCATALYSTS; STATE AB Oxidation of water provides the electrons and protons needed for the generation of fuels in any solar fuel system. In order to guide catalyst performance improvement, knowledge of the detailed mechanism of the four-electron oxidation of water to oxygen at the elementary step level is required. This has proved especially challenging for robust, Earth abundant metal oxide catalysts. Electrokinetic methods and ex situ or in situ steady state spectroscopy have revealed some insights into rate limiting steps or structural phase transformations of the catalyst under applied potential. Recent observation of surface reaction intermediates with rapid-scan FT-IR spectroscopy under reaction conditions with temporal resolution of milliseconds has allowed to establish the molecular structure and kinetic relevancy of transient species, and to identify their role in the catalytic cycle. C1 [Frei, Heinz] Univ Calif Berkeley, Mol Biophys Div, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Frei, H (reprint author), Univ Calif Berkeley, Mol Biophys Div, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM hmfrei@lbl.gov FU U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical, Geological and Biosciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 40 TC 0 Z9 0 U1 5 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 2211-3398 J9 CURR OPIN CHEM ENG JI Curr. Opin. Chem. Eng. PD MAY PY 2016 VL 12 BP 91 EP 97 DI 10.1016/j.coche.2016.04.001 PG 7 WC Biotechnology & Applied Microbiology; Engineering, Chemical SC Biotechnology & Applied Microbiology; Engineering GA ED0DK UT WOS:000388513000013 ER PT J AU Starrfield, S Iliadis, C Hix, WR AF Starrfield, S. Iliadis, C. Hix, W. R. TI X The Thermonuclear Runaway and the Classical Nova Outburst SO PUBLICATIONS OF THE ASTRONOMICAL SOCIETY OF THE PACIFIC LA English DT Review DE (stars:) novae; cataclysmic variables; stars: interiors; stars: evolution ID ACCRETING WHITE-DWARFS; HYDROGEN SHELL FLASHES; STELLAR ASTROPHYSICS MESA; POSSESSING ANGULAR-MOMENTUM; ROSSELAND OPACITY TABLES; NUCLEAR-REACTION RATES; LARGE-MAGELLANIC-CLOUD; REACTION-RATE LIBRARY; SUPERNOVA SN 2011FE; IA SUPERNOVAE AB Nova explosions occur on the white dwarf component of a cataclysmic variable binary stellar system that is accreting matter lost by its companion. When sufficient material has been accreted by the white dwarf, a thermonuclear runaway occurs and ejects material in what is observed as a classical nova explosion. We describe both the recent advances in our understanding of the progress of the outburst and outline some of the puzzles that are still outstanding. We report on the effects of improving both the nuclear reaction rate library and including a modern nuclear reaction network in our one-dimensional, fully implicit, hydrodynamic computer code. In addition, there has been progress in observational studies of supernovae Ia with implications about the progenitors, and we discuss that in this review. C1 [Starrfield, S.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Iliadis, C.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA. [Hix, W. R.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Hix, W. R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Starrfield, S (reprint author), Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. EM starrfield@asu.edu; iliadis@unc.edu; raph@ornl.gov FU NASA; NSF; DoE; U.S. Department of Energy [DE-AC05-00OR22725, DE-FG0297ER41041] FX We are extremely grateful to the referee for a detailed and careful reading of the original manuscript that has improved the presentation. We are also grateful to a number of collaborators who over the years have helped us to better understand the nova outburst. We have benefited from discussions with A. Beardmore, M. Bode, A. Champagne, M. Darnley, J. Drake, A. Evans, R.D. Gehrz, P.H. Hauschildt, M. Hernanz, R. Hounsell, J. Jose, S. Kafka, J. Krautter, T. Liimits, J.-U. Ness, J. Osborne, K. Page, D. Prialnik, F. Sarina, G. Schwarz, H. Schatz, A. Shafter, G. Shaviv, S.N. Shore, E.M. Sion, W.M. Sparks, P. Szkody, J. Truran, K. Vanlandingham, R.M. Wagner, M. Wiescher, P. Woudt, and C.E. Woodward. S. S. acknowledges partial support from NASA and NSF grants to ASU. W.R.H. acknowledges partial support from DoE and NSF. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. C.I. acknowledges partial support by the U.S. Department of Energy under contract No. DE-FG0297ER41041. NR 181 TC 2 Z9 2 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-6280 EI 1538-3873 J9 PUBL ASTRON SOC PAC JI Publ. Astron. Soc. Pac. PD MAY PY 2016 VL 128 IS 963 AR 051001 DI 10.1088/1538-3873/128/963/051001 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA EB1JX UT WOS:000387108400001 ER PT J AU Choi, KS Barker, E Cheng, G Sun, X Forsmark, J Li, M AF Choi, Kyoo Sil Barker, Erin Cheng, Guang Sun, Xin Forsmark, Joy Li, Mei TI Predicting Stress vs. Strain Behaviors of Thin-Walled High Pressure Die Cast Magnesium Alloy with Actual Pore Distribution SO SAE INTERNATIONAL JOURNAL OF MATERIALS AND MANUFACTURING LA English DT Article ID MICROSTRUCTURE; DUCTILITY AB In this paper, a three-dimensional (3D) microstructure-based finite element modeling method (i.e., extrinsic modeling method) is developed, which can be used in examining the effects of porosity on the ductility/fracture of Mg castings. For this purpose, AM60 Mg tensile samples were generated under high-pressure die-casting in a specially-designed mold. Before the tensile test, the samples were CT-scanned to obtain the pore distributions within the samples. 3D microstructure-based finite element models were then developed based on the obtained actual pore distributions of the gauge area. The input properties for the matrix material were determined by fitting the simulation result to the experimental result of a selected sample, and then used for all the other samples' simulation. The results show that the ductility and fracture locations predicted from simulations agree well with the experimental results. This indicates that the developed 3D extrinsic modeling method may be used to examine the influence of various aspects of pore sizes/distributions as well as intrinsic properties (i.e., matrix properties) on the ductility/fracture of Mg castings. C1 [Choi, Kyoo Sil; Barker, Erin; Cheng, Guang; Sun, Xin] Pacific Northwest Natl Lab, K7-90,PO 999, Richland, WA 99352 USA. [Forsmark, Joy; Li, Mei] Ford Motor Co, Dearborn, MI 48121 USA. RP Choi, KS (reprint author), Pacific Northwest Natl Lab, K7-90,PO 999, Richland, WA 99352 USA. EM kyoosil.choi@pnnl.gov OI Cheng, Guang /0000-0002-6860-4420 NR 9 TC 0 Z9 0 U1 0 U2 0 PU SAE INT PI WARRENDALE PA 400 COMMONWEALTH DR, WARRENDALE, PA 15096 USA SN 1946-3979 EI 1946-3987 J9 SAE INT J MATER MANU JI SAE Int. J. Mater. Manuf. PD MAY PY 2016 VL 9 IS 2 BP 361 EP 367 DI 10.4271/2016-01-0290 PG 7 WC Transportation Science & Technology SC Transportation GA EA2TS UT WOS:000386448300018 ER PT J AU Chaturvedi, P Rodriguez, SD Vlassiouk, I Hansen, IA Smirnov, SN AF Chaturvedi, Pavan Rodriguez, Stacy D. Vlassiouk, Ivan Hansen, Immo A. Smirnov, Sergei N. TI Simple and Versatile Detection of Viruses Using Anodized Alumina Membranes SO ACS SENSORS LA English DT Article DE AAO; biosensor; virus sensor; MS2; ionic conductance; volume exclusion effect ID SOLID-STATE NANOPORE; IONIC CONDUCTANCE; DENGUE VIRUS; DNA; NANOCHANNELS; BIOSENSORS; RECOGNITION; SELECTIVITY; DIFFUSION; CHANNELS AB A simple sensor for viral particles based on ionic conductivity through anodized alumina membranes was demonstrated using MS2 bacteriophage as an example. A facile two-point measuring scheme is geared toward realization using a computer's sound card input/output capabilities suitable for a fast and inexpensive point of care testing. The lowest detection concentration down to similar to 7 pfu/mL and a large dynamic range up to similar to 2000 pfu/mL were obtained due to physical optimization that included proper length and diameter for the pores, removing the oxide layer at the electrode, as well as the chemical optimization of covalent binding of antibodies to the pore's walls. C1 [Chaturvedi, Pavan; Smirnov, Sergei N.] New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA. [Chaturvedi, Pavan] New Mexico State Univ, Dept Phys, Las Cruces, NM 88003 USA. [Rodriguez, Stacy D.; Hansen, Immo A.] New Mexico State Univ, Dept Biol, Las Cruces, NM 88003 USA. [Vlassiouk, Ivan] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Smirnov, SN (reprint author), New Mexico State Univ, Dept Chem & Biochem, Las Cruces, NM 88003 USA. EM snsm@nmsu.edu RI Vlassiouk, Ivan/F-9587-2010 OI Vlassiouk, Ivan/0000-0002-5494-0386 FU National Institute of Health [R15-EB-016401-01] FX This work was partially supported by grant from the National Institute of Health (R15-EB-016401-01). The authors are grateful to Dr. P. Cook for help with SEM and Dr. C. Bruce for lending some equipment. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 37 TC 1 Z9 1 U1 9 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2379-3694 J9 ACS SENSORS JI ACS Sens. PD MAY PY 2016 VL 1 IS 5 BP 488 EP 492 DI 10.1021/acssensors.6b00003 PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Chemistry; Science & Technology - Other Topics GA DY9OV UT WOS:000385464600004 ER PT J AU Yang, C Trikantzopoulos, E Nguyen, MD Jacobs, CB Wang, Y Mahjouri-Samani, M Ivanov, IN Venton, BJ AF Yang, Cheng Trikantzopoulos, Elefterios Nguyen, Michael D. Jacobs, Christopher B. Wang, Ying Mahjouri-Samani, Masoud Ivanov, Ilia N. Venton, B. Jill TI Laser Treated Carbon Nanotube Yarn Microelectrodes for Rapid and Sensitive Detection of Dopamine in Vivo SO ACS SENSORS LA English DT Article DE dopamine; fast-scan cyclic voltammetry; in vivo; CNT yarn; laser treatment; ascorbic acid ID SCAN CYCLIC VOLTAMMETRY; FIBER MICROELECTRODES; MICRODISK ELECTRODES; ENHANCED DETECTION; NEUROTRANSMITTERS; NANOELECTRODES; ACTIVATION; ADENOSINE; RELEASE; ARRAYS AB Carbon nanotube yarn microelectrodes (CNTYMEs) exhibit rapid and selective detection of dopamine with fast-scan cyclic voltammetry (FSCV); however, the sensitivity limits their application in vivo. In this study, we introduce laser treatment as a simple, reliable, and efficient approach to improve the sensitivity of CNTYMEs by threefold while maintaining high temporal resolution. The effect of laser treatment on the microelectrode surface was characterized by scanning electron microscopy, Raman spectroscopy, energy dispersion spectroscopy, and laser scanning confocal microscopy. Laser treatment increases the surface area and oxygen containing functional groups on the surface, which provides more adsorption sites for dopamine than at unmodified CNTYMEs. Moreover, similar to unmodified CNTYMEs, the dopamine signal at laser treated CNTYMEs is not dependent on scan repetition frequency, unlike the current at carbon fiber microelectrodes (CFMEs) which decreases with increasing scan repetition frequency. This frequency independence is caused by the significantly larger surface roughness which would trap dopamine-o-quinone and amplify the dopamine signal. CNTYMEs were applied as an in vivo sensor with FSCV for the first time, and laser treated CNTYMEs maintained high dopamine sensitivity compared to CFMEs with an increased scan repetition frequency of 50 Hz, which is 5-fold faster than the conventional frequency. CNTYMEs with laser treatment are advantageous because of their easy fabrication, high reproducibility, fast electron transfer kinetics, high sensitivity, and rapid in vivo measurement of dopamine and could be a potential alternative to CFMEs in the future. C1 [Yang, Cheng; Trikantzopoulos, Elefterios; Nguyen, Michael D.; Wang, Ying; Venton, B. Jill] Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. [Jacobs, Christopher B.; Mahjouri-Samani, Masoud; Ivanov, Ilia N.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Venton, BJ (reprint author), Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. EM jventon@virginia.edu OI Jacobs, Christopher/0000-0001-7906-6368; ivanov, ilia/0000-0002-6726-2502 FU NIH [R21 DA037584]; DOE Office of Science User Facility [CNMS2014-083]; ORNL-UVA Travel Award (University of Virginia) FX This research was supported by NIH Grant R21 DA037584. Laser treatment and physical characterization on the CNT yarn microelectrodes were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility (User Grant CNMS2014-083). Travel aid to Oak Ridge National Laboratory was supported by ORNL-UVA Travel Award (University of Virginia). NR 45 TC 2 Z9 2 U1 8 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2379-3694 J9 ACS SENSORS JI ACS Sens. PD MAY PY 2016 VL 1 IS 5 BP 508 EP 515 DI 10.1021/acssensors.6b00021 PG 8 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Chemistry; Science & Technology - Other Topics GA DY9OV UT WOS:000385464600008 PM 27430021 ER PT J AU Weiss, CJ Aldridge, DF Knox, HA Schramm, KA Bartel, LC AF Weiss, Chester J. Aldridge, David F. Knox, Hunter A. Schramm, Kimberly A. Bartel, Lewis C. TI The direct-current response of electrically conducting fractures excited by a grounded current source SO GEOPHYSICS LA English DT Article ID BOREHOLE-TO-SURFACE; RESISTIVITY MEASUREMENTS; INVERSION; FIELD; MICROEARTHQUAKES; SENSITIVITY; SYSTEMS AB Hydraulic fracture stimulation of low permeability reservoir rocks is an established and cross-cutting technology for enhancing hydrocarbon production in sedimentary formations and increasing heat exchange in crystalline geothermal systems. Whereas the primary measure of success is the ability to keep the newly generated fractures sufficiently open, long-term reservoir management requires a knowledge of the spatial extent, morphology, and distribution of the fractures - knowledge primarily informed by microseismic and ground deformation monitoring. To minimize the uncertainty associated with interpreting such data, we investigate through numerical simulation the usefulness of direct-current (DC) resistivity data for characterizing subsurface fractures with elevated electrical conductivity by considering a geophysical experiment consisting of a grounded current source deployed in a steel cased borehole. In doing so, the casing efficiently energizes the fractures with steady current. Finite element simulations of this experiment for a horizontal well intersecting a small set of vertical fractures indicate that the fractures manifest electrically in (at least) two ways: (1) a local perturbation in electric potential proximal to the fracture set, with limited farfield expression and (2) an overall reduction in the electric potential along the borehole casing due to enhanced current flow through the fractures into the surrounding formation. The change in casing potential results in a measurable effect that can be observed far from fractures themselves. Under these conditions, our results suggest that farfield, time-lapse measurements of DC potentials can be interpreted by simple, linear inversion for a Coulomb charge distribution along the borehole path, including a local charge perturbation due to the fractures. This approach offers an inexpensive method for detecting and monitoring the time-evolution of electrically conducting fractures while ultimately providing an estimate of their effective conductivity - the latter providing an important measure independent of seismic methods on fracture shape, size, and hydraulic connectivity. C1 [Weiss, Chester J.; Aldridge, David F.; Knox, Hunter A.; Schramm, Kimberly A.] Sandia Natl Labs, Dept Geophys, POB 5800, Albuquerque, NM 87185 USA. [Bartel, Lewis C.] CARBO Ceram Inc, Houston, TX USA. RP Weiss, CJ (reprint author), Sandia Natl Labs, Dept Geophys, POB 5800, Albuquerque, NM 87185 USA. EM cjweiss@sandia.gov; dfaldri@sandia.gov; haknox@sandia.gov; kschramm@gmail.com; lewisbartel@comcast.net FU CARBO Ceramics, Inc., under CRADA [SC11/01780.00]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank A. Rinehart for helpful discussions on finite-element meshing with CUBIT (Hanks et al., 2014). The constructive comments by three anonymous reviewers are greatly appreciated and led to the additional benchmarking work included in Appendix A. Funding for this work was provided by CARBO Ceramics, Inc., under CRADA agreement SC11/01780.00. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 39 TC 0 Z9 0 U1 8 U2 8 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD MAY-JUN PY 2016 VL 81 IS 3 BP E201 EP E210 DI 10.1190/GEO2015-0262.1 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DY3IL UT WOS:000384984900015 ER PT J AU Conlon, BP Rowe, SE Gandt, AB Nuxoll, AS Donegan, NP Zalis, EA Clair, G Adkins, JN Cheung, AL Lewis, K AF Conlon, Brian P. Rowe, Sarah E. Gandt, Autumn Brown Nuxoll, Austin S. Donegan, Niles P. Zalis, Eliza A. Clair, Geremy Adkins, Joshua N. Cheung, Ambrose L. Lewis, Kim TI Persister formation in Staphylococcus aureus is associated with ATP depletion SO NATURE MICROBIOLOGY LA English DT Article ID BACTERIAL PERSISTENCE; ESCHERICHIA-COLI; CELLS; TOLERANCE; HIPA; ANTIBIOTICS; INFECTIONS; EXPRESSION; BIOFILMS; SYSTEM AB Persisters are dormant phenotypic variants of bacterial cells that are tolerant to killing by antibiotics(1). Persisters are associated with chronic infections and antibiotic treatment failure(1-3). In Escherichia coli, toxin-antitoxin modules have been linked to persister formation(4-6). The mechanism of persister formation in Gram-positive bacteria is unknown. Staphylococcus aureus is a major human pathogen, responsible for a variety of chronic and relapsing infections such as osteomyelitis, endocarditis and infections of implanted devices. Deleting toxinantitoxin modules in S. aureus did not affect the level of persisters. Here, we show that S. aureus persisters are produced due to a stochastic entrance into the stationary phase accompanied by a drop in intracellular adenosine triphosphate. Cells expressing stationary-state markers are present throughout the growth phase, and increase in frequency with cell density. Cell sorting revealed that the expression of stationary markers is associated with a 100-1,000-fold increase in the likelihood of survival to antibiotic challenge. The adenosine triphosphate level of the cell is predictive of bactericidal antibiotic efficacy and explains bacterial tolerance to antibiotics. C1 [Conlon, Brian P.; Rowe, Sarah E.; Gandt, Autumn Brown; Nuxoll, Austin S.; Zalis, Eliza A.; Lewis, Kim] Northeastern Univ, Dept Biol, Antimicrobial Discovery Ctr, Boston, MA 02115 USA. [Rowe, Sarah E.] Synlogic, Cambridge, MA 02139 USA. [Donegan, Niles P.; Cheung, Ambrose L.] Geisel Sch Med Dartmouth, Dept Microbiol & Immunol, Hanover, NH 03755 USA. [Clair, Geremy; Adkins, Joshua N.] Pacific Northwest Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Lewis, K (reprint author), Northeastern Univ, Dept Biol, Antimicrobial Discovery Ctr, Boston, MA 02115 USA. EM k.lewis@neu.edu OI Donegan, Niles/0000-0002-8328-2044; Conlon, Brian/0000-0002-2155-8375 FU National Institutes of Health [R01AI110578]; Charles A. King fellowship FX The authors thank C. Wolz for the gift of the HG001, HG001 rshsyn and triple mutant rshsyn, relP, relQ strains. The authors thank R. Lee and M. LaFleur for critical discussions. This work was supported by National Institutes of Health grant no. R01AI110578 to K.L. and by a Charles A. King fellowship to B.C. NR 40 TC 16 Z9 16 U1 11 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND EI 2058-5276 J9 NAT MICROBIOL JI NAT. MICROBIOL PD MAY PY 2016 VL 1 IS 5 AR 16051 DI 10.1038/NMICROBIOL.2016.51 PG 7 WC Microbiology SC Microbiology GA DW4IA UT WOS:000383605200011 PM 27572649 ER PT J AU Jansson, JK Baker, ES AF Jansson, Janet K. Baker, Erin S. TI A multi-omic future for microbiome studies SO NATURE MICROBIOLOGY LA English DT Editorial Material ID PERMAFROST; REVEALS; DISEASE AB Integration of multiple 'omics' technologies will allow researchers to gain a more complete picture of the constituents and functions of microbial communities and provide far richer information for predictive modelling of community phenotypes. C1 [Jansson, Janet K.; Baker, Erin S.] Pacific Northwest Natl Lab, Earth & Biol Sci Div, 902 Battelle Blvd, Richland, WA 99352 USA. RP Jansson, JK; Baker, ES (reprint author), Pacific Northwest Natl Lab, Earth & Biol Sci Div, 902 Battelle Blvd, Richland, WA 99352 USA. EM janet.jansson@pnnl.gov; erin.baker@pnnl.gov NR 15 TC 3 Z9 3 U1 8 U2 8 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND EI 2058-5276 J9 NAT MICROBIOL JI NAT. MICROBIOL PD MAY PY 2016 VL 1 IS 5 AR 16049 DI 10.1038/NMICROBIOL.2016.49 PG 3 WC Microbiology SC Microbiology GA DW4IA UT WOS:000383605200010 PM 27572648 ER PT J AU Boys, CA Robinson, W Miller, B Pflugrath, B Baumgartner, LJ Navarro, A Brown, R Deng, Z AF Boys, C. A. Robinson, W. Miller, B. Pflugrath, B. Baumgartner, L. J. Navarro, A. Brown, R. Deng, Z. TI A piecewise regression approach for determining biologically relevant hydraulic thresholds for the protection of fishes at river infrastructure SO JOURNAL OF FISH BIOLOGY LA English DT Article DE barotrauma; downstream fish passage; hydropower; Murray cod; physoclistous; silver perch ID HYDRO-TURBINE PASSAGE; HYDROTURBINE PASSAGE; JUVENILE; BAROTRAUMA; MANAGEMENT; MORTALITY; SURVIVAL; CHALLENGES; AUSTRALIA; MIGRATION AB A piecewise regression approach was used to objectively quantify barotrauma injury thresholds in two physoclistous species, Murray cod Maccullochella peelii and silver perch Bidyanus bidyanus, following simulated infrastructure passage in a barometric chamber. The probability of injuries such as swimbladder rupture, exophthalmia and haemorrhage, and emphysema in various organs increased as the ratio between the lowest exposure pressure and the acclimation pressure (ratio of pressure change, R-(NE:A)) reduced. The relationship was typically non-linear and piecewise regression was able to quantify thresholds in R-(NE:A) that once exceeded resulted in a substantial increase in barotrauma injury. Thresholds differed among injury types and between species but by applying a multispecies precautionary principle, the maintenance of exposure pressures at river infrastructure above 70% of acclimation pressure (R-(NE:A) of 0.7) should protect downstream migrating juveniles of these two physoclistous species sufficiently. These findings have important implications for determining the risk posed by current infrastructures and informing the design and operation of new ones. (C) 2016 The Fisheries Society of the British Isles C1 [Boys, C. A.; Pflugrath, B.] Port Stephens Fisheries Inst, New South Wales Dept Primary Ind, Taylors Beach Rd, Taylors Beach, NSW 2316, Australia. [Robinson, W.; Baumgartner, L. J.; Navarro, A.] Charles Sturt Univ, Elizabeth Mitchell Dr, Thurgoona, NSW 2640, Australia. [Miller, B.; Pflugrath, B.] Univ New South Wales, Water Res Lab, 110 King St Manly Vale, Sydney, NSW 2093, Australia. [Brown, R.; Deng, Z.] Pacific Northwest Natl Lab, Richland, WA 99352 USA. RP Boys, CA (reprint author), Port Stephens Fisheries Inst, New South Wales Dept Primary Ind, Taylors Beach Rd, Taylors Beach, NSW 2316, Australia. EM craig.boys@dpi.nsw.gov.au RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU New South Wales Department of Primary Industries (NSW DPI); Waratah Power through Australian Renewable Energy Agency (ARENA) Emerging Renewables Programme; Australian Centre for International Agricultural Research (ACIAR); Animal Care and Ethics Authority [ACEC 12/05] FX This project was funded in part by New South Wales Department of Primary Industries (NSW DPI), Waratah Power through a grant provided by the Australian Renewable Energy Agency (ARENA) Emerging Renewables Programme and the Australian Centre for International Agricultural Research (ACIAR). NSW DPI staff who assisted with the experiments included T. Fowler and S. Chilcott. All animal experimentation undertaken in this project was approved under Animal Care and Ethics Authority (ACEC 12/05). NR 46 TC 1 Z9 1 U1 1 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-1112 EI 1095-8649 J9 J FISH BIOL JI J. Fish Biol. PD MAY PY 2016 VL 88 IS 5 BP 1677 EP 1692 DI 10.1111/jfb.12910 PG 16 WC Fisheries; Marine & Freshwater Biology SC Fisheries; Marine & Freshwater Biology GA DX3UL UT WOS:000384300800001 PM 26991929 ER PT J AU Wang, ST Iskandarani, M Srinivasan, A Thacker, WC Winokur, J Knio, OM AF Wang, Shitao Iskandarani, Mohamed Srinivasan, Ashwanth Thacker, W. Carlisle Winokur, Justin Knio, Omar M. TI Propagation of uncertainty and sensitivity analysis in an integral oil-gas plume model SO JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS LA English DT Article ID DEEP-WATER-HORIZON; POLYNOMIAL CHAOS; BUBBLE PLUMES; NUMERICAL SIMULATIONS; DISPERSANT INJECTION; DROPLET BREAKUP; SUBSEA OIL; MEAN FLOW; BLOWOUT; SPILL AB Polynomial Chaos expansions are used to analyze uncertainties in an integral oil-gas plume model simulating the Deepwater Horizon oil spill. The study focuses on six uncertain input parameters-two entrainment parameters, the gas to oil ratio, two parameters associated with the droplet-size distribution, and the flow rate-that impact the model's estimates of the plume's trap and peel heights, and of its various gas fluxes. The ranges of the uncertain inputs were determined by experimental data. Ensemble calculations were performed to construct polynomial chaos-based surrogates that describe the variations in the outputs due to variations in the uncertain inputs. The surrogates were then used to estimate reliably the statistics of the model outputs, and to perform an analysis of variance. Two experiments were performed to study the impacts of high and low flow rate uncertainties. The analysis shows that in the former case the flow rate is the largest contributor to output uncertainties, whereas in the latter case, with the uncertainty range constrained by aposteriori analyses, the flow rate's contribution becomes negligible. The trap and peel heights uncertainties are then mainly due to uncertainties in the 95% percentile of the droplet size and in the entrainment parameters. C1 [Wang, Shitao; Iskandarani, Mohamed] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, 4600 Rickenbacker Causeway, Miami, FL 33149 USA. [Srinivasan, Ashwanth] Tendral LLC, Miami, FL USA. [Winokur, Justin] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Knio, Omar M.] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27706 USA. [Knio, Omar M.] King Abdullah Univ Sci & Technol, Div Comp Elect & Math Sci & Engn, Thuwal, Saudi Arabia. RP Wang, ST (reprint author), Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, 4600 Rickenbacker Causeway, Miami, FL 33149 USA. EM swang@rsmas.miami.edu FU BP/The Gulf of Mexico Research Initiative; Office of Naval Research [N00014-101-0498]; U.S. Department of Energy (DOE), Office of Science, Office of Advanced Scientific Computing Research [DE-SC0008789] FX We thank the two anonymous reviewers for their constructive suggestions which improve this manuscript. This work was made possible in part by a grant from BP/The Gulf of Mexico Research Initiative, and by the Office of Naval Research, Award N00014-101-0498. J. Winokur and O. M. Knio were also supported in part by the U.S. Department of Energy (DOE), Office of Science, Office of Advanced Scientific Computing Research, under Award DE-SC0008789. This research was conducted in collaboration with and using the resources of the University of Miami Center for Computational Science. The model data are publicly available in the Gulf of Mexico Research Initiative Information and Data Cooperative (GRIIDC) repository (https://data.gulfresearchinitiative.org/data/R4.x265.252:0002/). NR 56 TC 1 Z9 1 U1 4 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9275 EI 2169-9291 J9 J GEOPHYS RES-OCEANS JI J. Geophys. Res.-Oceans PD MAY PY 2016 VL 121 IS 5 BP 3488 EP 3501 DI 10.1002/2015JC011365 PG 14 WC Oceanography SC Oceanography GA DW2IQ UT WOS:000383466500040 ER PT J AU Suzuki, N Fox-Kemper, B Hamlington, PE Van Roekel, LP AF Suzuki, Nobuhiro Fox-Kemper, Baylor Hamlington, Peter E. Van Roekel, Luke P. TI Surface waves affect frontogenesis SO JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS LA English DT Article ID LARGE-EDDY SIMULATION; MIXED-LAYER; BOUNDARY-LAYER; LANGMUIR CIRCULATIONS; OCEAN FRONTS; VERTICAL CIRCULATION; ENERGY-TRANSFER; VORTEX-FORCE; TURBULENCE; MODEL AB This paper provides a detailed analysis of momentum, angular momentum, vorticity, and energy budgets of a submesoscale front undergoing frontogenesis driven by an upper-ocean, submesoscale eddy field in a Large Eddy Simulation (LES). The LES solves the wave-averaged, or Craik-Leibovich, equations in order to account for the Stokes forces that result from interactions between nonbreaking surface waves and currents, and resolves both submesoscale eddies and boundary layer turbulence down to 4.9 m x 4.9 m x 1.25 m grid scales. It is found that submesoscale frontogenesis differs from traditional frontogenesis theory due to four effects: Stokes forces, momentum and kinetic energy transfer from submesoscale eddies to frontal secondary circulations, resolved turbulent stresses, and unbalanced torque. In the energy, momentum, angular momentum, and vorticity budgets for the frontal overturning circulation, the Stokes shear force is a leading-order contributor, typically either the second or third largest source of frontal overturning. These effects violate hydrostatic and thermal wind balances during submesoscale frontogenesis. The effect of the Stokes shear force becomes stronger with increasing alignment of the front and Stokes shear and with a nondimensional scaling. The Stokes shear force and momentum transfer from submesoscale eddies significantly energize the frontal secondary circulation along with the buoyancy. C1 [Suzuki, Nobuhiro; Fox-Kemper, Baylor] Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA. [Hamlington, Peter E.] Univ Colorado, Dept Mech Engn, Boulder, CO 80309 USA. [Van Roekel, Luke P.] Los Alamos Natl Lab, Theoret Div, Climate Ocean & Sea Ice Modeling, Los Alamos, NM USA. RP Suzuki, N (reprint author), Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA. EM nobuhiro_suzuki@brown.edu RI Fox-Kemper, Baylor/A-1159-2007 OI Fox-Kemper, Baylor/0000-0002-2871-2048 FU Brown University; Rhode Island Science & Technology Advisory Council; Gulf of Mexico Research Initiative; NSF [1258907, 1258995] FX The authors would like to acknowledge fruitful conversations with Eric D'Asaro, Sean Haney, and James McWilliams. This work would not be possible without the use of the NCAR LES code written by Peter Sullivan and collaborators. N.S. is supported by Brown University and a grant from the Rhode Island Science & Technology Advisory Council. B.F.-K.'s contribution was made possible in part by a grant from The Gulf of Mexico Research Initiative and in part by NSF 1258907. P.E.H was supported in part by NSF 1258995. The data analyzed in this paper are available from the authors upon request (nobuhiro_suzuki@brown.edu). NR 65 TC 0 Z9 0 U1 11 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9275 EI 2169-9291 J9 J GEOPHYS RES-OCEANS JI J. Geophys. Res.-Oceans PD MAY PY 2016 VL 121 IS 5 BP 3597 EP 3624 DI 10.1002/2015JC011563 PG 28 WC Oceanography SC Oceanography GA DW2IQ UT WOS:000383466500047 ER PT J AU Tourassi, G Yoon, HJ Xu, SH Han, XS AF Tourassi, Georgia Yoon, Hong-Jun Xu, Songhua Han, Xuesong TI The utility of web mining for epidemiological research: studying the association between parity and cancer risk SO JOURNAL OF THE AMERICAN MEDICAL INFORMATICS ASSOCIATION LA English DT Article DE digital epidemiology; web mining; cancer risk; parity ID ORAL-CONTRACEPTIVE USE; REPRODUCTIVE FACTORS; OVARIAN-CANCER; BREAST-CANCER; COLORECTAL-CANCER; POSTMENOPAUSAL WOMEN; SEARCH BEHAVIOR; UNITED-STATES; SOCIAL MEDIA; WHITE WOMEN AB Background The World Wide Web has emerged as a powerful data source for epidemiological studies related to infectious disease surveillance. However, its potential for cancer-related epidemiological discoveries is largely unexplored. Methods Using advanced web crawling and tailored information extraction procedures, the authors automatically collected and analyzed the text content of 79 394 online obituary articles published between 1998 and 2014. The collected data included 51 911 cancer (27 330 breast; 9470 lung; 6496 pancreatic; 6342 ovarian; 2273 colon) and 27 483 non-cancer cases. With the derived information, the authors replicated a case-control study design to investigate the association between parity (i.e., childbearing) and cancer risk. Age-adjusted odds ratios (ORs) with 95% confidence intervals (CIs) were calculated for each cancer type and compared to those reported in large-scale epidemiological studies. Results Parity was found to be associated with a significantly reduced risk of breast cancer (OR = 0.78, 95% CI, 0.75-0.82), pancreatic cancer (OR = 0.78, 95% CI, 0.72-0.83), colon cancer (OR = 0.67, 95% CI, 0.60-0.74), and ovarian cancer (OR = 0.58, 95% CI, 0.54-0.62). Marginal association was found for lung cancer risk (OR = 0.87, 95% CI, 0.81-0.92). The linear trend between increased parity and reduced cancer risk was dramatically more pronounced for breast and ovarian cancer than the other cancers included in the analysis. Conclusion This large web-mining study on parity and cancer risk produced findings very similar to those reported with traditional observational studies. It may be used as a promising strategy to generate study hypotheses for guiding and prioritizing future epidemiological studies. C1 [Tourassi, Georgia; Yoon, Hong-Jun] Oak Ridge Natl Lab, Hlth Data Sci Inst, Biomed Sci & Engn Ctr, Oak Ridge, TN 37831 USA. [Xu, Songhua] New Jersey Inst Technol, Dept Informat Syst, Newark, NJ 07102 USA. [Han, Xuesong] Amer Canc Soc, Surveillance & Hlth Serv Res, Atlanta, GA 30303 USA. RP Tourassi, G (reprint author), Oak Ridge Natl Lab, POB 2008 MS6085, Oak Ridge, TN 37831 USA. EM tourassig@ornl.gov FU National Cancer Institute at the National Institutes of Health [1R01-CA170508] FX This work was supported by the National Cancer Institute at the National Institutes of Health (Grant No. 1R01-CA170508). NR 56 TC 0 Z9 0 U1 7 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1067-5027 EI 1527-974X J9 J AM MED INFORM ASSN JI J. Am. Med. Inf. Assoc. PD MAY PY 2016 VL 23 IS 3 BP 588 EP 595 DI 10.1093/jamia/ocv141 PG 8 WC Computer Science, Information Systems; Computer Science, Interdisciplinary Applications; Health Care Sciences & Services; Information Science & Library Science; Medical Informatics SC Computer Science; Health Care Sciences & Services; Information Science & Library Science; Medical Informatics GA DW6SP UT WOS:000383781800022 PM 26615183 ER PT J AU Antonopoulos, DA Chang, EB AF Antonopoulos, Dionysios A. Chang, Eugene B. TI Transplanting a Microbial Organ: the Good, the Bad, and the Unknown SO MBIO LA English DT Editorial Material AB Fecal microbiota transplantation (FMT) has received increased attention as a therapy for correcting intestinal dysbiosis and restoring a state of health in patients suffering from either recalcitrant infection by Clostridium difficile or more complex disease states, such as inflammatory bowel disease (IBD). The "gut microbial organ" from the donor that is used in these transplants may serve to transfer genetic material between donor and recipient via virus-like particles, specifically bacteriophages, that infect the bacterial component of the microbiota. The recently published study by Chehoud et al. provides evidence for not only the transfer of bacteriophages during F MT but also the transfer of multiple populations of bacteriophages to recipients from the donor microbiota used (C. Chehoud et al., mBio 7:e00322-16, 2016, http://dx.doi.org/10.1128/mBio.00322-16). While the clinical significance of these findings remains unclear, nothing short of a diligent and persistent effort is needed to define the intended and unintended consequences of FMT. C1 [Antonopoulos, Dionysios A.; Chang, Eugene B.] Univ Chicago, Dept Med, 5841 S Maryland Ave, Chicago, IL 60637 USA. [Antonopoulos, Dionysios A.] Argonne Natl Lab, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Chang, EB (reprint author), Univ Chicago, Dept Med, 5841 S Maryland Ave, Chicago, IL 60637 USA. EM echang@medicine.bsd.uchicago.edu NR 12 TC 2 Z9 2 U1 4 U2 4 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2016 VL 7 IS 3 AR e00572-16 DI 10.1128/mBio.00572-16 PG 2 WC Microbiology SC Microbiology GA DW1YP UT WOS:000383440300036 ER PT J AU Blaser, MJ Cardon, ZG Cho, MK Dangl, JL Donohue, TJ Green, JL Knight, R Maxon, ME Northen, TR Pollard, KS Brodie, EL AF Blaser, Martin J. Cardon, Zoe G. Cho, Mildred K. Dangl, Jeffrey L. Donohue, Timothy J. Green, Jessica L. Knight, Rob Maxon, Mary E. Northen, Trent R. Pollard, Katherine S. Brodie, Eoin L. TI Toward a Predictive Understanding of Earth's Microbiomes to Address 21st Century Challenges SO MBIO LA English DT Editorial Material ID GUT MICROBIOME; DARK-MATTER; INTESTINAL MICROBIOTA; NITROGEN-FIXATION; PERMAFROST THAW; ORGANIC-MATTER; CLIMATE-CHANGE; INSECT PEST; BACTERIAL; HEALTH AB Microorganisms have shaped our planet and its inhabitants for over 3.5 billion years. Humankind has had a profound influence on the biosphere, manifested as global climate and land use changes, and extensive urbanization in response to a growing population. The challenges we face to supply food, energy, and clean water while maintaining and improving the health of our population and ecosystems are significant. Given the extensive influence of microorganisms across our biosphere, we propose that a coordinated, cross-disciplinary effort is required to understand, predict, and harness microbiome function. From the parallelization of gene function testing to precision manipulation of genes, communities, and model ecosystems and development of novel analytical and simulation approaches, we outline strategies to move microbiome research into an era of causality. These efforts will improve prediction of ecosystem response and enable the development of new, responsible, microbiome-based solutions to significant challenges of our time. C1 [Blaser, Martin J.] NYU, Sch Med, Dept Microbiol, New York, NY 10016 USA. [Blaser, Martin J.] NYU, Sch Med, Dept Med, New York, NY USA. [Cardon, Zoe G.] Marine Biol Lab, Ctr Ecosyst, Woods Hole, MA 02543 USA. [Cho, Mildred K.] Stanford Univ, Stanford Ctr Biomed Eth, Palo Alto, CA 94304 USA. [Dangl, Jeffrey L.] Univ N Carolina, Dept Biol, Chapel Hill, NC USA. [Dangl, Jeffrey L.] Univ N Carolina, Howard Hughes Med Inst, Chapel Hill, NC USA. [Donohue, Timothy J.] Univ Wisconsin, Dept Bacteriol, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. [Donohue, Timothy J.] Univ Wisconsin, Wisconsin Energy Inst, Madison, WI USA. [Green, Jessica L.] Univ Oregon, Biol & Built Environm Ctr, Eugene, OR 97403 USA. [Green, Jessica L.] Univ Oregon, Dept Biol, Inst Ecol & Evolut, Eugene, OR 97403 USA. [Knight, Rob] Univ Calif San Diego, Dept Pediat, La Jolla, CA 92093 USA. [Knight, Rob] Univ Calif San Diego, Dept Comp Sci & Engn, La Jolla, CA 92093 USA. [Knight, Rob] Univ Calif San Diego, Ctr Microbiome Innovat, La Jolla, CA 92093 USA. [Maxon, Mary E.; Northen, Trent R.] Lawrence Berkeley Natl Lab, Biosci, Berkeley, CA USA. [Pollard, Katherine S.] Univ Calif San Francisco, Gladstone Inst, Div Biostat, San Francisco, CA 94143 USA. [Pollard, Katherine S.] Univ Calif San Francisco, Inst Human Genet, Inst Computat Hlth Sci, San Francisco, CA 94143 USA. [Brodie, Eoin L.] Lawrence Berkeley Natl Lab, Earth & Environm Sci, Berkeley, CA 94720 USA. [Brodie, Eoin L.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Brodie, EL (reprint author), Lawrence Berkeley Natl Lab, Earth & Environm Sci, Berkeley, CA 94720 USA.; Brodie, EL (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. EM ELBrodie@lbl.gov RI Brodie, Eoin/A-7853-2008; OI Brodie, Eoin/0000-0002-8453-8435; Donohue, Timothy/0000-0001-8738-2467; Cardon, Zoe/0000-0001-8725-7842; Northen, Trent/0000-0001-8404-3259 NR 184 TC 6 Z9 6 U1 21 U2 21 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2016 VL 7 IS 3 AR e00714-16 DI 10.1128/mBio.00714-16 PG 16 WC Microbiology SC Microbiology GA DW1YP UT WOS:000383440300055 ER PT J AU Smith, KN Mailliard, RB Piazza, PA Fischer, W Korber, BT Fecek, RJ Ratner, D Gupta, P Mullins, JI Rinaldo, CR AF Smith, Kellie N. Mailliard, Robbie B. Piazza, Paolo A. Fischer, Will Korber, Bette T. Fecek, Ronald J. Ratner, Deena Gupta, Phalguni Mullins, James I. Rinaldo, Charles R. TI Effective Cytotoxic T Lymphocyte Targeting of Persistent HIV-1 during Antiretroviral Therapy Requires Priming of Naive CD8(+) T Cells (vol 7, e00473-16, 2016) SO MBIO LA English DT Correction C1 [Smith, Kellie N.] Univ Pittsburgh, Dept Microbiol & Mol Genet, Pittsburgh, PA USA. [Smith, Kellie N.; Mailliard, Robbie B.; Piazza, Paolo A.; Fecek, Ronald J.; Ratner, Deena; Gupta, Phalguni; Rinaldo, Charles R.] Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15260 USA. [Fischer, Will; Korber, Bette T.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. [Mullins, James I.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Rinaldo, Charles R.] Univ Pittsburgh, Sch Med, Dept Pathol, Pittsburgh, PA 15260 USA. [Smith, Kellie N.] Johns Hopkins Univ, Sch Med, Baltimore, MD USA. RP Rinaldo, CR (reprint author), Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15260 USA.; Rinaldo, CR (reprint author), Univ Pittsburgh, Sch Med, Dept Pathol, Pittsburgh, PA 15260 USA. EM rinaldo@pitt.edu NR 1 TC 0 Z9 0 U1 0 U2 0 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2016 VL 7 IS 3 AR e01012-16 DI 10.1128/mBio.01012-16 PG 1 WC Microbiology SC Microbiology GA DW1YP UT WOS:000383440300024 ER PT J AU Smith, KN Mailliard, RB Piazza, PA Fischer, W Korber, BT Fecek, RJ Ratner, D Gupta, P Mullins, JI Rinaldo, CR AF Smith, Kellie N. Mailliard, Robbie B. Piazza, Paolo A. Fischer, Will Korber, Bette T. Fecek, Ronald J. Ratner, Deena Gupta, Phalguni Mullins, James I. Rinaldo, Charles R. TI Effective Cytotoxic T Lymphocyte Targeting of Persistent HIV-1 during Antiretroviral Therapy Requires Priming of Naive CD8(+) T Cells SO MBIO LA English DT Article ID IMMUNODEFICIENCY-VIRUS TYPE-1; MULTICENTER AIDS COHORT; DENDRITIC CELLS; VIRAL LOAD; IN-VITRO; VARIANT EPITOPES; INFECTION; RESPONSES; ESCAPE; CD4(+) AB Curing HIV-1 infection will require elimination of persistent cellular reservoirs that harbor latent virus in the face of combination antiretroviral therapy (cART). Proposed immunotherapeutic strategies to cure HIV-1 infection include enhancing lysis of these infected cells by cytotoxic T lymphocytes (CTL). A major challenge in this strategy is overcoming viral immune escape variants that have evaded host immune control. Here we report that naive CD8(+) T cells from chronic HIV-1-infected participants on long-term cART can be primed by dendritic cells (DC). These DC must be mature, produce high levels of interleukin 12p70 (IL-12p70), be responsive to CD40 ligand (CD40L), and be loaded with inactivated, autologous HIV-1. These DC-primed CD8(+) T cell responders produced high levels of gamma interferon (IFN-gamma) in response to a broad range of both conserved and variable regions of Gag and effectively killed CD4(+) T cell targets that were either infected with the autologous latent reservoir-associated virus or loaded with autologous Gag peptides. In contrast, HIV-1-specific memory CD8(+) T cells stimulated with autologous HIV-1-loaded DC produced IFN-gamma in response to a narrow range of conserved and variable Gag peptides compared to the primed T cells and most notably, displayed significantly lower cytolytic function. Our findings highlight the need to selectively induce new HIV-1-specific CTL from naive precursors while avoiding activation of existing, dysfunctional memory T cells in potential curative immunotherapeutic strategies for HIV-1 infection. IMPORTANCE Current immunotherapeutic approaches aim to enhance antiviral immunity against the HIV-1 reservoir; however, it has yet to be shown whether T cells from persons on cART can recognize and eliminate virus-infected cells. We show that in persons on cART a personalized medicine approach using their dendritic cells to stimulate their naive T cells induces potent effector CTL in vitro that recognize and eradicate HIV-1-infected CD4(+) T cells. Additionally, we show that the same stimulation of existing memory T cells results in cytokine secretion but limited effector function. Our study demonstrates that the naive T cell repertoire can recognize persistent HIV-1 during cART and supports immunotherapy strategies for an HIV-1 cure that targets naive T cells, rather than existing, dysfunctional, memory T cells. C1 [Smith, Kellie N.] Univ Pittsburgh, Dept Microbiol & Mol Genet, Pittsburgh, PA USA. [Smith, Kellie N.; Mailliard, Robbie B.; Piazza, Paolo A.; Fecek, Ronald J.; Ratner, Deena; Gupta, Phalguni; Rinaldo, Charles R.] Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15260 USA. [Fischer, Will; Korber, Bette T.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. [Mullins, James I.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Rinaldo, Charles R.] Univ Pittsburgh, Dept Pathol, Sch Med, Pittsburgh, PA 15260 USA. [Smith, Kellie N.] Johns Hopkins Univ, Sch Med, Dept Oncol, Baltimore, MD 21205 USA. RP Rinaldo, CR (reprint author), Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15260 USA.; Rinaldo, CR (reprint author), Univ Pittsburgh, Dept Pathol, Sch Med, Pittsburgh, PA 15260 USA. EM rinaldo@pitt.edu OI Mailliard, Robbie/0000-0001-5501-503X FU HHS \ National Institutes of Health (NIH) [R37-AI-41870, U01-AI-35041, T32-AI065380] FX This work was funded by HHS vertical bar National Institutes of Health (NIH) (R37-AI-41870, U01-AI-35041, and T32-AI065380). NR 87 TC 2 Z9 2 U1 3 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2016 VL 7 IS 3 AR e00473-16 DI 10.1128/mBio.00473-16 PG 17 WC Microbiology SC Microbiology GA DW1YP UT WOS:000383440300023 ER PT J AU Stuart, RK Mayali, X Boaro, AA Zemla, A Everroad, RC Nilson, D Weber, PK Lipton, M Bebout, BM Pett-Ridge, J Thelen, MP AF Stuart, Rhona K. Mayali, Xavier Boaro, Amy A. Zemla, Adam Everroad, R. Craig Nilson, Daniel Weber, Peter K. Lipton, Mary Bebout, Brad M. Pett-Ridge, Jennifer Thelen, Michael P. TI Light Regimes Shape Utilization of Extracellular Organic C and N in a Cyanobacterial Biofilm SO MBIO LA English DT Article ID SUBTROPICAL NORTH PACIFIC; MARINE SYNECHOCOCCUS; MICROBIAL MAT; ALKALINE-PHOSPHATASE; CARBON; BACTERIA; ACID; PROCHLOROCOCCUS; PROTEOME; ANABAENA AB Although it is becoming clear that many microbial primary producers can also play a role as organic consumers, we know very little about the metabolic regulation of photoautotroph organic matter consumption. Cyanobacteria in phototrophic biofilms can reuse extracellular organic carbon, but the metabolic drivers of extracellular processes are surprisingly complex. We investigated the metabolic foundations of organic matter reuse by comparing exoproteome composition and incorporation of C-13-labeled and N-15-labeled cyanobacterial extracellular organic matter (EOM) in a unicyanobacterial biofilm incubated using different light regimes. In the light and the dark, cyanobacterial direct organic C assimilation accounted for 32% and 43%, respectively, of all organic C assimilation in the community. Under photosynthesis conditions, we measured increased excretion of extracellular polymeric substances (EPS) and proteins involved in micronutrient transport, suggesting that requirements for micronutrients may drive EOM assimilation during daylight hours. This interpretation was supported by photosynthesis inhibition experiments, in which cyanobacteria incorporated N-rich EOM-derived material. In contrast, under dark, C-starved conditions, cyanobacteria incorporated C-rich EOM-derived organic matter, decreased excretion of EPS, and showed an increased abundance of degradative exoproteins, demonstrating the use of the extracellular domain for C storage. Sequence-structure modeling of one of these exoproteins predicted a specific hydrolytic activity that was subsequently detected, confirming increased EOM degradation in the dark. Associated heterotrophic bacteria increased in abundance and upregulated transport proteins under dark relative to light conditions. Taken together, our results indicate that biofilm cyanobacteria are successful competitors for organic C and N and that cyanobacterial nutrient and energy requirements control the use of EOM. IMPORTANCE Cyanobacteria are globally distributed primary producers, and the fate of their fixed C influences microbial biogeochemical cycling. This fate is complicated by cyanobacterial degradation and assimilation of organic matter, but because cyanobacteria are assumed to be poor competitors for organic matter consumption, regulation of this process is not well tested. In mats and biofilms, this is especially relevant because cyanobacteria produce an extensive organic extracellular matrix, providing the community with a rich source of nutrients. Light is a well-known regulator of cyanobacterial metabolism, so we characterized the effects of light availability on the incorporation of organic matter. Using stable isotope tracing at the single-cell level, we quantified photoautotroph assimilation under different metabolic conditions and integrated the results with proteomics to elucidate metabolic status. We found that cyanobacteria effectively compete for organic matter in the light and the dark and that nutrient requirements and community interactions contribute to cycling of extracellular organic matter. C1 [Stuart, Rhona K.; Mayali, Xavier; Zemla, Adam; Nilson, Daniel; Weber, Peter K.; Pett-Ridge, Jennifer; Thelen, Michael P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Boaro, Amy A.; Lipton, Mary] Pacific Northwest Natl Lab, Richland, WA USA. [Everroad, R. Craig; Bebout, Brad M.] NASA, Exobiol Branch, Ames Res Ctr, Moffett Field, CA USA. RP Thelen, MP (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM mthelen@llnl.gov RI Thelen, Michael/G-2032-2014; Lipton, Mary/H-3913-2012; OI Thelen, Michael/0000-0002-2479-5480; Stuart, Rhona/0000-0001-5916-9693 FU U.S. Department of Energy (DOE); DOE Genomic Science Program [SCW1039]; DOE [DE-AC52-07NA27344] FX This work, including the efforts of Rhona K Stuart, Xavier Mayali, Amy Boaro, Adam Zemla, Craig Everroad, Daniel Nilson, Peter K Weber, Mary Lipton, Brad M Bebout, Jennifer Pett-Ridge, and Michael P. Thelen, was funded by U.S. Department of Energy (DOE).; Funding was provided by the DOE Genomic Science Program under contract SCW1039. Work at Lawrence Livermore National Laboratory was performed under the auspices of DOE contract DE-AC52-07NA27344. The funders had no role in study design, data collection and interpretation, or the decision to submit the work for publication. NR 70 TC 1 Z9 1 U1 15 U2 15 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD MAY-JUN PY 2016 VL 7 IS 3 AR e00650-16 DI 10.1128/mBio.00650-16 PG 14 WC Microbiology SC Microbiology GA DW1YP UT WOS:000383440300045 ER PT J AU Krishnan, V Das, T AF Krishnan, Venkat Das, Trishna TI Slow dynamics model of compressed air energy storage and battery storage technologies for automatic generation control SO ENERGY SYSTEMS-OPTIMIZATION MODELING SIMULATION AND ECONOMIC ASPECTS LA English DT Article DE Compressed air energy storage; Battery; Automatic generation control; Frequency response; Control performance standard; State space representation ID POWER-SYSTEMS; FREQUENCY; PERFORMANCE; MARKET AB Increasing variable generation penetration and the consequent increase in short-term variability makes energy storage technologies look attractive, especially in the ancillary market for providing frequency regulation services. This paper presents slow dynamics model for compressed air energy storage and battery storage technologies that can be used in automatic generation control studies to assess the system frequency response and quantify the benefits from storage technologies in providing regulation service. The paper also represents the slow dynamics model of the power system integrated with storage technologies in a complete state space form. The storage technologies have been integrated to the IEEE 24 bus system with single area, and a comparative study of various solution strategies including transmission enhancement and combustion turbine have been performed in terms of generation cycling and frequency response performance metrics. C1 [Krishnan, Venkat; Das, Trishna] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50014 USA. [Krishnan, Venkat] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Krishnan, V (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50014 USA.; Krishnan, V (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM venky83krish@gmail.com NR 27 TC 0 Z9 0 U1 3 U2 3 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1868-3967 EI 1868-3975 J9 ENERGY SYST JI Energy Syst. PD MAY PY 2016 VL 7 IS 2 BP 271 EP 295 DI 10.1007/s12667-015-0157-5 PG 25 WC Energy & Fuels SC Energy & Fuels GA DU4MH UT WOS:000382186200004 ER PT J AU Krishnan, V Ho, J Hobbs, BF Liu, AL McCalley, JD Shahidehpour, M Zheng, QPP AF Krishnan, Venkat Ho, Jonathan Hobbs, Benjamin F. Liu, Andrew L. McCalley, James D. Shahidehpour, Mohammad Zheng, Qipeng P. TI Co-optimization of electricity transmission and generation resources for planning and policy analysis: review of concepts and modeling approaches SO ENERGY SYSTEMS-OPTIMIZATION MODELING SIMULATION AND ECONOMIC ASPECTS LA English DT Review DE Co-optimization; Transmission expansion planning; Generation expansion planning; Model fidelity; Energy storage; Demand response; Integrated network uncertainty; Long-term planning; AC and DC power flow ID ENERGY-STORAGE; EXPANSION; TECHNOLOGIES; INVESTMENT; ECONOMICS; MARKETS; SYSTEMS; US; COORDINATION; FLEXIBILITY AB The recognition of transmission's interaction with other resources has motivated the development of co-optimization methods to optimize transmission investment while simultaneously considering tradeoffs with investments in electricity supply, demand, and storage resources. For a given set of constraints, co-optimized planning models provide solutions that have lower costs than solutions obtained from decoupled optimization (transmission-only, generation-only, or iterations between them). This paper describes co-optimization and provides an overview of approaches to co-optimizing transmission options, supply-side resources, demand-side resources, and natural gas pipelines. In particular, the paper provides an up-to-date assessment of the present and potential capabilities of existing co-optimization tools, and it discusses needs and challenges for developing advanced co-optimization models. C1 [Krishnan, Venkat; McCalley, James D.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Krishnan, Venkat] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ho, Jonathan; Hobbs, Benjamin F.] Johns Hopkins Univ, Dept Geog & Environm Engn, Baltimore, MD 21218 USA. [Liu, Andrew L.] Purdue Univ, Sch Ind Engn, W Lafayette, IN 47907 USA. [Shahidehpour, Mohammad] IIT, Elect & Comp Engn Dept, Chicago, IL 60616 USA. [Zheng, Qipeng P.] Univ Cent Florida, Dept Ind Engn & Management Syst, Orlando, FL 32816 USA. RP Krishnan, V (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA.; Krishnan, V (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM venky83krish@gmail.com NR 76 TC 1 Z9 1 U1 1 U2 1 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1868-3967 EI 1868-3975 J9 ENERGY SYST JI Energy Syst. PD MAY PY 2016 VL 7 IS 2 BP 297 EP 332 DI 10.1007/s12667-015-0158-4 PG 36 WC Energy & Fuels SC Energy & Fuels GA DU4MH UT WOS:000382186200005 ER PT J AU Rubel, O Loring, B Vay, JL Grote, DP Lehe, R Bulanov, S Vincenti, H Bethel, EW AF Rubel, Oliver Loring, Burlen Vay, Jean-Luc Grote, David P. Lehe, Remi Bulanov, Stepan Vincenti, Henri Bethel, E. Wes TI WarpIV: In Situ Visualization and Analysis of Ion Accelerator Simulations SO IEEE COMPUTER GRAPHICS AND APPLICATIONS LA English DT Article C1 [Rubel, Oliver; Loring, Burlen; Vay, Jean-Luc; Lehe, Remi; Vincenti, Henri; Bethel, E. Wes] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Grote, David P.] Lawrence Berkeley Natl Lab, Div Phys, Phys & Life Sci Directorate, Berkeley, CA 94720 USA. [Bulanov, Stepan] Lawrence Berkeley Natl Lab, BELLA Ctr, Berkeley, CA 94720 USA. RP Rubel, O; Loring, B; Vay, JL; Lehe, R; Vincenti, H; Bethel, EW (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Grote, DP (reprint author), Lawrence Berkeley Natl Lab, Div Phys, Phys & Life Sci Directorate, Berkeley, CA 94720 USA.; Bulanov, S (reprint author), Lawrence Berkeley Natl Lab, BELLA Ctr, Berkeley, CA 94720 USA. EM oruebel@lbl.gov; bloring@lbl.gov; jlvay@lbl.gov; grote1@llnl.gov; rlehe@lbl.gov; sbulanov@lbl.gov; hvincenti@lbl.gov; ewbethel@lbl.gov FU Office of Science, Office of Advanced Scientific Computing Research, of the US Department of Energy (DoE) as part of the SciDAC Institute for Scalable Data Management Analysis and Visualization (SDAV) [DE-AC02-05CH11231]; Office of Science of the US DoE [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Advanced Scientific Computing Research, of the US Department of Energy (DoE) under contract DE-AC02-05CH11231 as part of the SciDAC Institute for Scalable Data Management Analysis and Visualization (SDAV). This research used resources of the National Energy Research Scientific Computing Center, a DoE Office of Science User Facility supported by the Office of Science of the US DoE under contract DE-AC02-05CH11231. Oliver Rubel and Burlen Loring contributed equally to this work. NR 13 TC 0 Z9 0 U1 2 U2 2 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1716 EI 1558-1756 J9 IEEE COMPUT GRAPH JI IEEE Comput. Graph. Appl. PD MAY-JUN PY 2016 VL 36 IS 3 BP 22 EP 35 PG 14 WC Computer Science, Software Engineering SC Computer Science GA DU4FV UT WOS:000382169100006 PM 28113157 ER PT J AU Moreland, K Sewell, C Usher, W Lo, LT Meredith, J Pugmire, D Kress, J Schroots, H Ma, KL Childs, H Larsen, M Chen, CM Maynard, R Geveci, B AF Moreland, Kenneth Sewell, Christopher Usher, William Lo, Li-ta Meredith, Jeremy Pugmire, David Kress, James Schroots, Hendrik Ma, Kwan-Liu Childs, Hank Larsen, Matthew Chen, Chun-Ming Maynard, Robert Geveci, Berk TI VTK-m: Accelerating the Visualization Toolkit for Massively Threaded Architectures SO IEEE COMPUTER GRAPHICS AND APPLICATIONS LA English DT Article ID SOFTWARE C1 [Moreland, Kenneth] Sandia Natl Labs, Livermore, CA 94550 USA. [Sewell, Christopher] Los Alamos Natl Lab, Comp & Computat Sci Div, Los Alamos, NM 87545 USA. [Usher, William] Univ Utah, Sci Comp & Imaging Inst, Salt Lake City, UT 84112 USA. [Lo, Li-ta] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Meredith, Jeremy; Pugmire, David] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Kress, James] Univ Oregon, Comp Sci, Eugene, OR 97403 USA. [Schroots, Hendrik] Intel Corp, Santa Clara, CA 95051 USA. [Ma, Kwan-Liu] Univ Calif Davis, Comp Sci, Davis, CA 95616 USA. [Childs, Hank] Univ Oregon, Eugene, OR 97403 USA. [Larsen, Matthew] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Chen, Chun-Ming] Ohio State Univ, Dept Comp Sci & Engn, Columbus, OH 43210 USA. [Maynard, Robert] Kitware, Clifton Pk, NY 12065 USA. [Geveci, Berk] Kitware, Sci Comp, Clifton Pk, NY 12065 USA. RP Moreland, K (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA.; Sewell, C (reprint author), Los Alamos Natl Lab, Comp & Computat Sci Div, Los Alamos, NM 87545 USA.; Usher, W (reprint author), Univ Utah, Sci Comp & Imaging Inst, Salt Lake City, UT 84112 USA.; Lo, LT (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.; Meredith, J; Pugmire, D (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.; Kress, J (reprint author), Univ Oregon, Comp Sci, Eugene, OR 97403 USA.; Schroots, H (reprint author), Intel Corp, Santa Clara, CA 95051 USA.; Ma, KL (reprint author), Univ Calif Davis, Comp Sci, Davis, CA 95616 USA.; Childs, H (reprint author), Univ Oregon, Eugene, OR 97403 USA.; Larsen, M (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.; Chen, CM (reprint author), Ohio State Univ, Dept Comp Sci & Engn, Columbus, OH 43210 USA.; Maynard, R (reprint author), Kitware, Clifton Pk, NY 12065 USA.; Geveci, B (reprint author), Kitware, Sci Comp, Clifton Pk, NY 12065 USA. EM kmorel@sandia.gov; csewell@lanl.gov; will@sci.utah.edu; ollie@lanl.gov; jsmeredith@ornl.gov; pugmire@ornl.gov; jkress@cs.uoregon.edu; hschroot@ucdavis.edu; ma@cs.ucdavis.edu; hank@uoregon.edu; larsen30@llnl.gov; chen.1701@osu.edu; robert.maynard@kitware.com; berk.geveci@kitware.com OI Kress, James/0000-0002-9706-6182 FU US Department of Energy (DoE), Office of Science, Office of Advanced Scientific Computing Research [14-017566, 12-015215]; US DoE's National Nuclear Security Administration [DE-AC04-94AL85000, SAND 2016-1719 J]; US DoE [DE-AC05-00OR22725]; DoE FX We thank Kewei Lu from the Ohio State University for valuable contributions to the VTK-m isosurface implementation. This material is based on work supported by the US Department of Energy (DoE), Office of Science, Office of Advanced Scientific Computing Research, under award numbers 14-017566 and 12-015215. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia, a wholly owned subsidiary of Lockheed Martin, for the US DoE's National Nuclear Security Administration under contract DE-AC04-94AL85000, SAND 2016-1719 J. The original manuscript was authored by UT-Battelle LLC under contract DE-AC05-00OR22725 with the US DoE. The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. The DoE will provide public access to these results of federally sponsored research in accordance with the DoE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 16 TC 0 Z9 0 U1 0 U2 0 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1716 EI 1558-1756 J9 IEEE COMPUT GRAPH JI IEEE Comput. Graph. Appl. PD MAY-JUN PY 2016 VL 36 IS 3 BP 48 EP 58 PG 11 WC Computer Science, Software Engineering SC Computer Science GA DU4FV UT WOS:000382169100008 PM 28113158 ER PT J AU Mahurin, SM Surwade, SP Crespo, M Dai, S AF Mahurin, Shannon M. Surwade, Sumedh P. Crespo, Marcos Dai, Sheng TI Probing the interaction of ionic liquids with graphene using surface-enhanced Raman spectroscopy SO JOURNAL OF RAMAN SPECTROSCOPY LA English DT Article DE room-temperature ionic liquids; graphene; energy storage; interfacial interactions; surface enhanced Raman spectroscopy ID TEMPERATURE; ELECTRODES; INTERFACE; CAPACITANCE; CHALLENGES; SCATTERING; GRAPHITE; INSIGHTS AB We report an in situ measurement of the interaction of an imidazolium-based room temperature ionic liquid with both pure silver and a graphene-over-silver electrode under an applied electrochemical potential. At a negative applied potential, overall signal intensity increased indicating enhanced ionic liquid concentration at both silver and graphene electrodes. Vibrational modes associated with the imidazolium ring exhibited greater intensity enhancements and larger peak shifts compared with the anion indicating that the cation adsorbs with the ring and alkyl chain parallel to the electrode surface for both silver and graphene. In contrast to the silver, the surface enhanced Raman spectra of the ionic liquid near graphene showed shifts in the cation peaks even at no applied potential because of the strong p-p interaction between the ionic liquid and the graphene. Furthermore, the intensity of the graphene peak decreased in the presence of ionic liquid possibly due to the interaction between the ionic liquid and graphene. These results illustrate the effectiveness of surface-enhanced Raman spectroscopy to investigate electrolyte interactions with graphene at the liquid/electrode interface. Copyright (C) 2015 John Wiley & Sons, Ltd. C1 [Mahurin, Shannon M.; Surwade, Sumedh P.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Crespo, Marcos] Univ Puerto Rico Piedras, Dept Chem, San Juan, PR USA. RP Mahurin, SM; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM mahurinsm@ornl.gov; dais@ornl.gov FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 33 TC 0 Z9 0 U1 9 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0377-0486 EI 1097-4555 J9 J RAMAN SPECTROSC JI J. Raman Spectrosc. PD MAY PY 2016 VL 47 IS 5 BP 585 EP 590 DI 10.1002/jrs.4858 PG 6 WC Spectroscopy SC Spectroscopy GA DS1QG UT WOS:000380370400010 ER PT J AU Greene, AC Sasaki, DY Bachand, GD AF Greene, Adrienne C. Sasaki, Darryl Y. Bachand, George D. TI Forming Giant-sized Polymersomes Using Gel-assisted Rehydration SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Bioengineering; Issue 111; Polymersome; gel; vesicle; rehydration; polymer; membrane ID VESICLES; COPOLYMERS AB Polymer vesicles, or polymersomes, are being widely explored as synthetic analogs of lipid vesicles based on their stability, robustness, barrier properties, chemical versatility and tunable physical characteristics. Typical methods used to prepare giant-sized (> 4 mu m) vesicles, however, are both time and labor intensive, yielding low numbers of intact polymersomes. Here, we present for the first time the use of gel-assisted rehydration for the rapid and high-yielding formation of giant (> 4 mu m) polymer vesicles (polymersomes). Using this method, polymersomes can be formed from a wide array of rehydration solutions including several different physiologically-compatible buffers and full cell culture media, making them readily useful for biomimicry studies. This technique is also capable of reliably producing polymersomes from different polymer compositions with far better yields and much less difficulty than traditional methods. Polymersome size is readily tunable by altering temperature during rehydration or adding membrane fluidizers to the polymer membrane, generating giant-sized polymersomes (> 100 mu m). C1 [Greene, Adrienne C.; Bachand, George D.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Livermore, CA 94550 USA. [Sasaki, Darryl Y.] Sandia Natl Labs, Biol & Engn Sci, Livermore, CA 94550 USA. RP Greene, AC (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, Livermore, CA 94550 USA. EM acgreen@sandia.gov OI Bachand, George/0000-0002-3169-9980 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE); BES-MSE; U.S. Department of Energy (DOE) Office of Science [RA2015A0004] FX We would like to gratefully acknowledge Dr. Ian M. Henderson, Andrew Gomez and Dr. Walter F. Paxton for their technical expertise, advice and help in this work. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE). ACG, DYS and GDB were supported by BES-MSE. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science (user project number RA2015A0004, PI: ACG). NR 13 TC 0 Z9 0 U1 2 U2 2 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD MAY PY 2016 IS 111 AR e54051 DI 10.3791/54051 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS0BJ UT WOS:000380259900078 ER PT J AU Gould, B Greco, A AF Gould, Benjamin Greco, Aaron TI Investigating the Process of White Etching Crack Initiation in Bearing Steel SO TRIBOLOGY LETTERS LA English DT Article DE White etching cracks; Wind turbine gearbox bearings; Microstructural alterations; Bearing failures ID ROLLING-CONTACT FATIGUE; MICROSTRUCTURAL CHANGES; WEC FORMATION; HYDROGEN; AREA; TRANSFORMATIONS; MARTENSITE; INCLUSIONS; BEHAVIOR; LIFE AB White etching cracks (WECs) have been identified as a dominant mode of premature failure within wind turbine gearbox bearings. Though WECs have been reported in the field for over a decade, the conditions leading to WECs and the process by which this failure culminates are both highly debated. In previously published work, the generation of WECs on a benchtop scale was linked to sliding at the surface of the test sample, and it was also postulated that the generation of WECs was dependent on the cumulative energy that had been applied to the sample over the entirety of the test. In this paper, a three-ring-on-roller benchtop test rig is used to systematically alter the cumulative energy that a sample experiences through changes in normal load, sliding, and run-time, in an attempt to correlate cumulative energy with the formation of WECs. It was determined that, in the current test setup, the presence of WECs can be predicted by this energy criterion. The authors then used this information to study the process by which WECs initiate. It was found that, under the current testing conditions, the formation of a dark etching microstructure precedes the formation of a crack, and a crack precedes the formation of white etching microstructure. C1 [Gould, Benjamin; Greco, Aaron] Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA. [Gould, Benjamin] Univ Delaware, Dept Mech Engn, Newark, DE 19716 USA. RP Gould, B (reprint author), Argonne Natl Lab, Div Energy Syst, Lemont, IL 60439 USA.; Gould, B (reprint author), Univ Delaware, Dept Mech Engn, Newark, DE 19716 USA. EM Bengould@udel.edu OI Gould, Benjamin/0000-0002-4363-6602; Greco, Aaron/0000-0002-2189-0888 FU US Department of Energy Office of Energy Efficiency and Renewable Energy; US Department of Energy Wind and Water Power Technology Office [DE-AC02-06CH11357]; DOE; US Department of Energy Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work is supported by the US Department of Energy Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technology Office under Contract No. DE-AC02-06CH11357. The authors are grateful to DOE Project Managers Mr. Michael Derby and Mr. Nick Johnson for their support and encouragement. The authors would also like to acknowledge the assistance provided by our colleagues at Argonne National Laboratory's Tribology Section, especially Dr. Maria De La Cinta Lorenzo Martin for her assistance with electron microscopy and Dr. Oyelayo Ajayi for his helpful discussion on metallurgy. As well as Dr. David L. Burris of the University of Delaware's department of Mechanical Engineering for serving as an advisor over the course of this work. The authors would also like to thank Dr. Mihails Scepanskis for many useful conversations pertaining to WEC generation and PCS Instruments for providing samples for the MPR testing. Use of the Center for Nanoscale Materials an Office of Science user facility was supported by the US Department of Energy Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 43 TC 1 Z9 1 U1 9 U2 9 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1023-8883 EI 1573-2711 J9 TRIBOL LETT JI Tribol. Lett. PD MAY PY 2016 VL 62 IS 2 AR 26 DI 10.1007/s11249-016-0673-z PG 14 WC Engineering, Chemical; Engineering, Mechanical SC Engineering GA DS1FH UT WOS:000380340700011 ER PT J AU Polyzos, A Holt, A Brown, C Cosme, C Wipf, P Gomez-Marin, A Castro, MR Ayala-Pena, S McMurray, CT AF Polyzos, Aris Holt, Amy Brown, Christopher Cosme, Celica Wipf, Peter Gomez-Marin, Alex Castro, Mariadel R. Ayala-Pena, Sylvette McMurray, Cynthia T. TI Mitochondrial targeting of XJB-5-131 attenuates or improves pathophysiology in HdhQ150 animals with well-developed disease phenotypes SO HUMAN MOLECULAR GENETICS LA English DT Article ID HUNTINGTONS-DISEASE; OXIDATIVE STRESS; TRANSGENIC MICE; MOUSE MODEL; DNA-DAMAGE; PARKINSONS-DISEASE; COENZYME-Q; ABNORMALITIES; ANTIOXIDANTS; MECHANISMS AB Oxidative damage to mitochondria (MT) is a major mechanism for aging and neurodegeneration. We have developed a novel synthetic antioxidant, XJB-5-131, which directly targets MT, the primary site and primary target of oxidative damage. XJB-5-131 prevents the onset of motor decline in an HdhQ(150/150) mouse model for Huntington's disease (HD) if treatment starts early. Here, we report that XJB-5-131 attenuates or reverses disease progression if treatment occurs after disease onset. In animals with well-developed pathology, XJB-5-131 promotes weight gain, prevents neuronal death, reduces oxidative damage in neurons, suppresses the decline of motor performance or improves it, and reduces a graying phenotype in treated HdhQ(150/150) animals relative to matched littermate controls. XJB-5-131 holds promise as a clinical candidate for the treatment of HD. C1 [Polyzos, Aris; Holt, Amy; McMurray, Cynthia T.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Brown, Christopher; Cosme, Celica] Univ Calif Berkeley, Mol Cellular Biol Program, Berkeley, CA 94720 USA. [Wipf, Peter] Univ Pittsburgh, Dept Chem, 219 Parkman Ave, Pittsburgh, PA 15260 USA. [Gomez-Marin, Alex] CSIC, Inst Neurociencias, Sant Joan dAlacant, Spain. [Gomez-Marin, Alex] Univ Miguel Hernandez, Sant Joan dAlacant, Spain. [Castro, Mariadel R.; Ayala-Pena, Sylvette] Univ Puerto Rico, Dept Pharmacol & Toxicol, POB 365067, San Juan, PR 00936 USA. RP McMurray, CT (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ctmcmurray@lbl.gov OI Gomez Marin, Alejandro/0000-0003-2764-2583 FU National Institutes of Health [ES020766-01, NS060115, CA092584, SC1NS095380, GM061838]; University of Puerto Rico Infrastructural [MD007600, AG04337601]; Portuguese Foundation for Science and Technology [SFRH/BPD/97544/2013] FX This work was supported by National Institutes of Health (grants ES020766-01, NS060115, CA092584 to C.T.M.; SC1NS095380 to S.A.P.; GM061838) and the University of Puerto Rico Infrastructural (grant MD007600 to S.A.P.; AG04337601 to P.W.) and Portuguese Foundation for Science and Technology (grant no SFRH/BPD/97544/2013 to A.G.-M.). NR 53 TC 3 Z9 3 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0964-6906 EI 1460-2083 J9 HUM MOL GENET JI Hum. Mol. Genet. PD MAY 1 PY 2016 VL 25 IS 9 BP 1792 EP 1802 DI 10.1093/hmg/ddw051 PG 11 WC Biochemistry & Molecular Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Genetics & Heredity GA DR9WX UT WOS:000380247900010 PM 26908614 ER PT J AU Weilhammer, DR Dunkle, AD Blanchette, C Boone, T Gilmore, S Corzett, M Fischer, N Lehmann, D Lychak, C Hoeprich, P Driks, A Rasley, A AF Weilhammer, Dina R. Dunkle, Alexis D. Blanchette, Craig Boone, Tyler Gilmore, Sean Corzett, Michele Fischer, Nicholas Lehmann, Doerte Lychak, Cheri Hoeprich, Paul Driks, Adam Rasley, Amy TI Use of biologic nanolipoprotein particles containing monophosphoryl lipid A as a novel intranasal vaccine platform for Bacillus anthracis SO JOURNAL OF IMMUNOLOGY LA English DT Meeting Abstract CT Annual Meeting of the American-Association-of-Immunologists (AAI) CY MAY 13-17, 2016 CL Seattle, WA SP Amer Assoc Immunologists C1 [Weilhammer, Dina R.; Gilmore, Sean; Corzett, Michele; Fischer, Nicholas; Lychak, Cheri; Hoeprich, Paul; Rasley, Amy] Lawrence Livermore Natl Lab, Livermore, CA USA. [Dunkle, Alexis D.; Blanchette, Craig] Genentech Inc, San Francisco, CA 94080 USA. [Boone, Tyler; Lehmann, Doerte; Driks, Adam] Loyola Univ Chicago, Chicago, IL USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU AMER ASSOC IMMUNOLOGISTS PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814 USA SN 0022-1767 EI 1550-6606 J9 J IMMUNOL JI J. Immunol. PD MAY 1 PY 2016 VL 196 SU 1 PG 2 WC Immunology SC Immunology GA DS0LX UT WOS:000380288302214 ER PT J AU Su, CC He, MN Redfern, P Curtiss, LA Liao, C Zhang, L Burrell, AK Zhang, ZC AF Su, Chi-Cheung He, Meinan Redfern, Paul Curtiss, Larry A. Liao, Chen Zhang, Lu Burrell, Anthony K. Zhang, Zhengcheng TI Alkyl Substitution Effect on Oxidation Stability of Sulfone-Based Electrolytes SO CHEMELECTROCHEM LA English DT Article DE alkyl substitution; high-voltage lithium-ion batteries; oxidation stability; quantum chemistry; sulfone-based electrolytes ID LITHIUM-ION BATTERIES; FLUORINATED ELECTROLYTES; RECHARGEABLE BATTERIES; ANODIC STABILITY; CHEMISTRY; CARBONATE; CATHODE; LINI0.5MN1.5O4; DINITRILE; PERFORMANCES AB Organic sulfone compounds have been widely used as high-voltage electrolytes for lithium-ion batteries for decades. However, owing to the complexity of the synthesis of new sulfones, only a few commercially available sulfones have been studied. In this paper, we report the synthesis of new sulfone compounds with various substituent groups and the impact of the substituent group on the oxidation stability of sulfones. Electrochemical floating tests using a 5 V LiNi0.5Mn1.5O4 spinel cathode and density functional theory calculations showed that the cyclopentyl-substituted sulfone McPS suffered from oxidation instability, starting from 4.9 V versus Li+/Li, as observed by the large leakage currents. On the other hand, the isopropyl-substituted sulfone MiPS and tetramethylene substituted sulfone TMS showed much improved oxidation stability under identical testing conditions. The substitution structure of the sulfone plays a significant role in the determination of its oxidative stability and should first be considered for the development of new sulfone-based electrolytes for high-voltage, high-energy lithium-ion batteries. C1 [Su, Chi-Cheung; He, Meinan; Liao, Chen; Zhang, Lu; Burrell, Anthony K.; Zhang, Zhengcheng] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Redfern, Paul; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zhang, ZC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zzhang@anl.gov FU U.S. Department of Energy, Vehicle Technologies Office; U.S. Department of Energy by UChicago Argonne, LLC [DE-AC02-06CH11357] FX This research is supported by the U.S. Department of Energy, Vehicle Technologies Office. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC, under contract DE-AC02-06CH11357. We would like to thank the Cell Analysis, Modeling, and Prototyping (CAMP) Facility of Argonne's Chemical Sciences and Engineering Division for providing the electrode materials. NR 42 TC 2 Z9 2 U1 6 U2 8 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2196-0216 J9 CHEMELECTROCHEM JI ChemElectroChem PD MAY PY 2016 VL 3 IS 5 BP 790 EP 797 DI 10.1002/celc.201500550 PG 8 WC Electrochemistry SC Electrochemistry GA DR6BG UT WOS:000379985500018 ER PT J AU Wilfong, WC Gray, ML Kail, BW Howard, BH AF Wilfong, Walter Christopher Gray, McMahan L. Kail, Brian W. Howard, Bret H. TI Pelletization of Immobilized Amine Carbon Dioxide Sorbents with Fly Ash and Poly(vinyl chloride) SO ENERGY TECHNOLOGY LA English DT Article DE amines; carbon dioxide capture; fly ash; pelletspoly(vinyl chloride) ID POSTCOMBUSTION CO2 CAPTURE; SILICA-SUPPORTED AMINE; COMPOSITE FILMS; ADSORBED CO2; CHEMICAL-MODIFICATION; IR SPECTROSCOPY; FLUIDIZED-BED; ADSORPTION; POLYETHYLENEIMINE; STABILITY AB A combination of coal fly ash (FA) and a polymer binder, namely, poly(vinyl chloride) (PVC), was used to pelletize immobilized amine CO2 sorbents. The pelletization of mixtures of FA and 50 wt% tetraethylenepentamine (TEPA) or ethylenimine oligomer mixture (M-w = 423)/silica (EI423-S) with PVC created a rigid PVC/FA/sorbent network. The strength of the network was attributed, in part, to the hydrogen bonding of PVC with the hydroxy and amine groups of the FA and sorbent (infrared spectroscopy). Increasing the PVC molecular weight or FA content enhanced the pellet strength and reduced CO2 capture. The optimum pellet, FA/EI423-S (20/80)_PVC62 [10 wt% PVC62 (M-w = 62 000), 17 wt% FA], captured 1.33 mmol(CO2) g(-1) and exhibited a crush strength of 1.42 MPa. The reaction between PVC and amines produced ammonium ions (-NH3+/-NH2+), which reduced the CO2 captured by the pellet during stability testing. This issue was partially resolved by replacing PVC62 with p-phenylenediamine- modified PVC62, which also enhanced the pellet CO2 capture to 1.5 mmol(CO2) g(-1). C1 [Wilfong, Walter Christopher] Natl Energy Technol Lab, ORISE, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Gray, McMahan L.; Howard, Bret H.] US DOE, Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Kail, Brian W.] Natl Energy Technol Lab, AECOM, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. RP Wilfong, WC (reprint author), Natl Energy Technol Lab, ORISE, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM Walter.Wilfong@netl.doe.gov FU Department of Energy, National Energy Technology Laboratory, an agency of the United States Government; AECOM; U.S. Department of Energy; National Energy Technology Laboratory's under RES [DE-FE0004000] FX This project was funded by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with AECOM. This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. Neither the United States Government nor any agency thereof, nor any of their employees, nor AECOM, nor Oak Ridge, nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by tradename, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. A portion of this technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES contract DE-FE0004000. A portion of this data in another form was discussed in a poster presentation at the International Pittsburgh Coal Conference on Oct. 7, 2015. We thank Vyacheslav Romanov and Lei Hong for usage of the IR. We also thank Thiago Fernandes De Aquino for providing the fly ash composition. NR 47 TC 2 Z9 2 U1 7 U2 10 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2194-4288 EI 2194-4296 J9 ENERGY TECHNOL-GER JI Energy Technol. PD MAY PY 2016 VL 4 IS 5 BP 610 EP 619 DI 10.1002/ente.201500419 PG 10 WC Energy & Fuels SC Energy & Fuels GA DR5UZ UT WOS:000379969200007 ER PT J AU Mitrofanov, O Khromova, I Siday, T Thompson, RJ Ponomarev, AN Brener, I Reno, JL AF Mitrofanov, Oleg Khromova, Irina Siday, Thomas Thompson, Robert J. Ponomarev, Andrey N. Brener, Igal Reno, John L. TI Near-Field Spectroscopy and Imaging of Subwavelength Plasmonic Terahertz Resonators SO IEEE TRANSACTIONS ON TERAHERTZ SCIENCE AND TECHNOLOGY LA English DT Article DE Antennas; aperture; carbon fibers; graphite; near-field microscopy; plasmons; resonators; terahertz (THz) ID FREQUENCY-RANGE; WAVES; PROBE; SURFACE; RESOLUTION; APERTURES; GRAPHENE; METAMATERIAL; MICROSCOPE; RESONANCES AB We present the temporal evolution of the terahertz (THz) field leading to the excitation of plasmonic resonances in carbon microfibers. The field evolution is mapped in space and time for the 3/2 wavelength resonance using a subwavelength aperture THz near-field probe with an embedded THz photoconductive detector. The excitation of surface waves at the fiber tips leads to the formation of a standing wave along the fiber. Local THz time-domain spectroscopy at one of the standing wave crests shows a clear third-order resonance peak at 1.65 THz, well described by the Lorentz model. This application of the subwavelength aperture THz near-field microscopy for mode mapping and local spectroscopy demonstrates the potential of near-field methods for studies of subwavelength plasmonic THz resonators. C1 [Mitrofanov, Oleg; Khromova, Irina; Siday, Thomas; Thompson, Robert J.] UCL, Elect & Elect Engn Dept, London WC1E 7JE, England. [Khromova, Irina] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Khromova, Irina] ITMO Univ, Int Res Ctr Nanophoton & Metamat, St Petersburg 199034, Russia. [Ponomarev, Andrey N.] St Petersburg Polytech Univ, St Petersburg 199034, Russia. [Brener, Igal; Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Mitrofanov, O (reprint author), UCL, Elect & Elect Engn Dept, London WC1E 7JE, England. EM o.mitrofanov@ucl.ac.uk; i.khromova@ucl.ac.uk; tom.siday.15@ucl.ac.uk; robert.j.thompson@ucl.ac.uk; 9293522@gmail.com; ibrener@sandia.gov; jlreno@sandia.gov RI Mitrofanov, Oleg/C-1938-2008; Khromova, Irina/C-7587-2011 OI Mitrofanov, Oleg/0000-0003-3510-2675; Khromova, Irina/0000-0002-9977-3411 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The work was performed at UCL and, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 51 TC 2 Z9 2 U1 19 U2 25 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-342X J9 IEEE T THZ SCI TECHN JI IEEE Trans. Terahertz Sci. Technol. PD MAY PY 2016 VL 6 IS 3 BP 382 EP 388 DI 10.1109/TTHZ.2016.2549367 PG 7 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA DR2RS UT WOS:000379752200005 ER PT J AU Le Deit, L Mangold, N Forni, O Cousin, A Lasue, J Schroder, S Wiens, RC Sumner, D Fabre, C Stack, KM Anderson, RB Blaney, D Clegg, S Dromart, G Fisk, M Gasnault, O Grotzinger, JP Gupta, S Lanza, N Le Mouelic, S Maurice, S McLennan, SM Meslin, PY Nachon, M Newsom, H Payre, V Rapin, W Rice, M Sautter, V Treiman, AH AF Le Deit, L. Mangold, N. Forni, O. Cousin, A. Lasue, J. Schroder, S. Wiens, R. C. Sumner, D. Fabre, C. Stack, K. M. Anderson, R. B. Blaney, D. Clegg, S. Dromart, G. Fisk, M. Gasnault, O. Grotzinger, J. P. Gupta, S. Lanza, N. Le Mouelic, S. Maurice, S. McLennan, S. M. Meslin, P. -Y. Nachon, M. Newsom, H. Payre, V. Rapin, W. Rice, M. Sautter, V. Treiman, A. H. TI The potassic sedimentary rocks in Gale Crater, Mars, as seen by ChemCam on board Curiosity SO JOURNAL OF GEOPHYSICAL RESEARCH-PLANETS LA English DT Article ID IN-SITU; INSTRUMENT SUITE; K-FELDSPAR; ORIGIN; ROVER; SANDSTONE; EVOLUTION; ROCKNEST; OLIVINE; OUTCROP AB The Mars Science Laboratory rover Curiosity encountered potassium-rich clastic sedimentary rocks at two sites in Gale Crater, the waypoints Cooperstown and Kimberley. These rocks include several distinct meters thick sedimentary outcrops ranging from fine sandstone to conglomerate, interpreted to record an ancient fluvial or fluvio-deltaic depositional system. From ChemCam Laser-Induced Breakdown Spectroscopy (LIBS) chemical analyses, this suite of sedimentary rocks has an overall mean K2O abundance that is more than 5 times higher than that of the average Martian crust. The combined analysis of ChemCam data with stratigraphic and geographic locations reveals that the mean K2O abundance increases upward through the stratigraphic section. Chemical analyses across each unit can be represented as mixtures of several distinct chemical components, i.e., mineral phases, including K-bearing minerals, mafic silicates, Fe-oxides, and Fe-hydroxide/oxyhydroxides. Possible K-bearing minerals include alkali feldspar (including anorthoclase and sanidine) and K-bearing phyllosilicate such as illite. Mixtures of different source rocks, including a potassium-rich rock located on the rim and walls of Gale Crater, are the likely origin of observed chemical variations within each unit. Physical sorting may have also played a role in the enrichment in K in the Kimberley formation. The occurrence of these potassic sedimentary rocks provides additional evidence for the chemical diversity of the crust exposed at Gale Crater. C1 [Le Deit, L.; Mangold, N.; Le Mouelic, S.; Nachon, M.] Univ Nantes, UMR CNRS 6112, LPG Nantes, Lab Planetol & Geodynam, Nantes, France. [Forni, O.; Cousin, A.; Lasue, J.; Schroder, S.; Gasnault, O.; Maurice, S.; Meslin, P. -Y.; Rapin, W.] Inst Rech Astrophys & Planetol, Toulouse, France. [Schroder, S.] German Aerosp Ctr DLR, Inst Opt Sensorsyst, Berlin, Germany. [Wiens, R. C.; Clegg, S.; Lanza, N.] Los Alamos Natl Lab, Los Alamos, NM USA. [Sumner, D.] Univ Calif Davis, Earth & Planetary Sci, Davis, CA 95616 USA. [Fabre, C.; Payre, V.] Univ Lorraine, GeoRessources, Nancy, France. [Stack, K. M.; Blaney, D.] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Anderson, R. B.] US Geol Survey, Astrogeol Sci Ctr, Flagstaff, AZ 86001 USA. [Dromart, G.] ENS Lyon, Lab Geol Lyon, Terre Planetes Environm, Lyon, France. [Fisk, M.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. [Grotzinger, J. P.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Gupta, S.] Imperial Coll London, London, England. [McLennan, S. M.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Newsom, H.] Univ New Mexico, Inst Meteorit, Albuquerque, NM 87131 USA. [Rice, M.] Western Washington Univ, Geol Dept, Bellingham, WA 98225 USA. [Sautter, V.] Museum Hist Nat, LMCM, Paris, France. [Treiman, A. H.] Lunar & Planetary Inst, 3303 NASA Rd 1, Houston, TX 77058 USA. RP Le Deit, L (reprint author), Univ Nantes, UMR CNRS 6112, LPG Nantes, Lab Planetol & Geodynam, Nantes, France. EM Laetitia.Ledeit@univ-nantes.fr RI Gasnault, Olivier/F-4327-2010; OI Gasnault, Olivier/0000-0002-6979-9012; Clegg, Sam/0000-0002-0338-0948 FU Centre National d'Etudes Spatiales (CNES), France; NASA Mars Program Office FX This work is supported by the Centre National d'Etudes Spatiales (CNES), France, and by the NASA Mars Program Office. We gratefully thank the Curiosity rover operation team at Jet Propulsion Laboratory for the success of this mission. We also thank Jeff Taylor, our anonymous reviewer, and associate editor for their very thoughtful and thorough comments that greatly improved the manuscript. Imaging and chemical data presented here are available in the NASA Planetary Data System (PDS) http://pds-geosciences.wustl.edu/missions/msl. NR 59 TC 6 Z9 6 U1 9 U2 15 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9097 EI 2169-9100 J9 J GEOPHYS RES-PLANET JI J. Geophys. Res.-Planets PD MAY PY 2016 VL 121 IS 5 BP 784 EP 804 DI 10.1002/2015JE004987 PG 21 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DR5FB UT WOS:000379927600004 ER PT J AU Allegrini, F Ebert, RW Funsten, HO AF Allegrini, F. Ebert, R. W. Funsten, H. O. TI Carbon foils for space plasma instrumentation SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Review DE carbon foil; plasma instrument; time of flight; ENA imager ID SECONDARY-ELECTRON EMISSION; LOW-ENERGY IONS; EQUILIBRIUM CHARGE-DISTRIBUTIONS; CLEAN METAL-SURFACE; MOVING HEAVY-IONS; HYDROGEN-IONS; THIN FOILS; ANGULAR-DISTRIBUTIONS; STATE DISTRIBUTIONS; IMAGE MISSION AB Carbon foils have been successfully used for several decades in space plasma instruments to detect ions and neutral atoms. These instruments take advantage of two properties of the particle-foil interaction: charge conversion of neutral atoms and/or secondary electron emission. This interaction also creates several adverse effects for the projectile exiting the foil, such as angular scattering and energy straggling, which usually act to reduce the sensitivity and overall performance of an instrument. The magnitude of these effects mainly varies with the incident angle, energy, and mass of the incoming projectile and the foil thickness. In this paper, we describe these effects and the properties of the interaction. We also summarize results from recent studies with graphene foils, which can be made thinner than carbon foils due to their superior strength. Graphene foils may soon replace carbon foils in space plasma instruments and open new opportunities for space research in the future. C1 [Allegrini, F.; Ebert, R. W.] Southwest Res Inst, Space Sci & Engn Div, San Antonio, TX 78238 USA. [Allegrini, F.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Funsten, H. O.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Allegrini, F (reprint author), Southwest Res Inst, Space Sci & Engn Div, San Antonio, TX 78238 USA.; Allegrini, F (reprint author), Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. EM fallegrini@swri.edu FU Southwest Research Institute internal research and development; NASA [NNX13AG23G] FX The authors would like to thank Peter Bedworth, Chip Beebe, Kent Coulter, Dave Cronk, Mark Ferris, Stephen Fuselier, Guy Grubbs, Mike Gruntman, Ron Harper, Roberto Livi, Dave McComas, Georgios Nicolaou, Jim Raines, Ben Rodriguez, Steve Sinton, Ken Smith, Karlheinz Trattner, Phil Valek, Scott Weidner, Paul Wilson, Jiachen Xue, Dave Young, Qingkai Yu, and Vicky Zorbas Poenitzsch. The authors would like to thank SPIE, AIP Publishing LLC, and Elsevier for permission to reuse the figures in Figure 10. This work was supported by Southwest Research Institute internal research and development and by NASA grant NNX13AG23G. NR 102 TC 4 Z9 4 U1 5 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 3931 EP 3950 DI 10.1002/2016JA022570 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500005 ER PT J AU Burke, WJ Erickson, PJ Yang, J Foster, J Wygant, J Reeves, G Kletzing, C AF Burke, W. J. Erickson, P. J. Yang, J. Foster, J. Wygant, J. Reeves, G. Kletzing, C. TI O+ ion conic and plasma sheet dynamics observed by Van Allen Probe satellites during the 1 June 2013 magnetic storm SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE oxygen ion conics; plasma sheet dynamics ID IONOSPHERIC ACCELERATION MECHANISM; ADVANCED COMPOSITION EXPLORER; PARALLEL ELECTRIC-FIELDS; RING CURRENT; INNER MAGNETOSPHERE; GEOMAGNETIC STORMS; ENERGIZATION; SUBSTORMS; SECTOR; PRECIPITATION AB The Van Allen Probe satellites were near apogee in the late evening local time sector during the 1 June 2013 magnetic storm's main phase. About an hour after crossing the ring current's nose structure into the plasma sheet, the satellites encountered a quasiperiodic sequence of 0.08-3keV O+ ions. Pitch angle distributions of this population consistently peaked nearly antiparallel to the local magnetic field. We interpret this population as O+ conics originating in the northern ionosphere. Sequences began as fairly steady state conic fluxes with energies in the 80 to 100eV range. Over about a half hour buildup phase, O+ energies peaked near 1keV. During subsequent release phases lasting 20min, O+ energies returned to low-energy starting points. We argue these observations reflect repeated formations and dissolutions of downward, magnetically aligned electric fields (epsilon(||)) layers trapping O+ conics between mirror points within heating layers below and electrostatic barriers above. Nearly identical variations were observed at the locations of both satellites during 9 of these 13 conic cycles. Phase differences between cycles were observed at both spacecraft during the remaining events. Most buildup to release phase transitions coincided with AL index minima. However, in situ magnetometer measurements indicate only weak dipolarizations of tail-like magnetic fields. The lack of field-aligned reflected O+ and tail-like magnetic fields suggest that both ionospheres may be active. However, Southern Hemisphere origin conics cannot be observed since they would be isotropized and accelerated during neutral sheet crossings. C1 [Burke, W. J.] Boston Coll, Inst Sci Res, Chestnut Hill, MA 02167 USA. [Erickson, P. J.; Foster, J.] MIT, Haystack Observ, Westford, MA 01886 USA. [Yang, J.] Univ Massachusetts Lowell, Ctr Atmospher Res, Lowell, MA USA. [Wygant, J.] Univ Minnesota, Dept Phys & Astron, Minneapolis, MN 55455 USA. [Reeves, G.] Los Alamos Natl Lab, Los Alamos, NM USA. [Kletzing, C.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. RP Erickson, PJ (reprint author), MIT, Haystack Observ, Westford, MA 01886 USA. EM pje@haystack.mit.edu OI Reeves, Geoffrey/0000-0002-7985-8098 FU Van Allen Probes subaward from the University of Minnesota; NASA [NAS5-01072] FX The authors wish to express our profound gratitude to Herbert Funsten of the Los Alamos National Laboratory for making HOPE data available to the public via the National Space Science Data Center CDAWeb site (cdaw.gsfc.nasa.gov/). We are also indebted to Paul Song of the University of Massachusetts, Lowell (UML) for suggesting that we concentrate on Van Allen Probes data, as well as to J.-C. Zhang of the University of New Hampshire and M. A. Noah of UML who provided initial assistance in accessing Van Allen Probes measurements. Work at MIT Haystack Observatory was supported by a Van Allen Probes subaward from the University of Minnesota to the Massachusetts Institute of Technology. Van Allen Probes Mission Operations and Data Analysis (MO&DA) services are supported by NASA Prime contract NAS5-01072 to Johns Hopkins University Applied Physics Laboratory (JHU/APL). NR 55 TC 1 Z9 1 U1 1 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 4072 EP 4091 DI 10.1002/2015JA021795 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500014 ER PT J AU Ma, Q Li, W Thorne, RM Nishimura, Y Zhang, XJ Reeves, GD Kletzing, CA Kurth, WS Hospodarsky, GB Henderson, MG Spence, HE Baker, DN Blake, JB Fennell, JF Angelopoulos, V AF Ma, Q. Li, W. Thorne, R. M. Nishimura, Y. Zhang, X. -J. Reeves, G. D. Kletzing, C. A. Kurth, W. S. Hospodarsky, G. B. Henderson, M. G. Spence, H. E. Baker, D. N. Blake, J. B. Fennell, J. F. Angelopoulos, V. TI Simulation of energy-dependent electron diffusion processes in the Earth's outer radiation belt SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE energy-dependent diffusion; radiation belt simulation; electron acceleration and loss; radial diffusion ID VAN ALLEN PROBES; QUASI-LINEAR DIFFUSION; PITCH-ANGLE; RELATIVISTIC ELECTRONS; GEOMAGNETIC STORMS; EMIC WAVES; RESONANT SCATTERING; PLASMASPHERIC HISS; MAGNETIC STORM; ION-CYCLOTRON AB The radial and local diffusion processes induced by various plasma waves govern the highly energetic electron dynamics in the Earth's radiation belts, causing distinct characteristics in electron distributions at various energies. In this study, we present our simulation results of the energetic electron evolution during a geomagnetic storm using the University of California, Los Angeles 3-D diffusion code. Following the plasma sheet electron injections, the electrons at different energy bands detected by the Magnetic Electron Ion Spectrometer (MagEIS) and Relativistic Electron Proton Telescope (REPT) instruments on board the Van Allen Probes exhibit a rapid enhancement followed by a slow diffusive movement in differential energy fluxes, and the radial extent to which electrons can penetrate into depends on energy with closer penetration toward the Earth at lower energies than higher energies. We incorporate radial diffusion, local acceleration, and loss processes due to whistler mode wave observations to perform a 3-D diffusion simulation. Our simulation results demonstrate that chorus waves cause electron flux increase by more than 1 order of magnitude during the first 18h, and the subsequent radial extents of the energetic electrons during the storm recovery phase are determined by the coupled radial diffusion and the pitch angle scattering by EMIC waves and plasmaspheric hiss. The radial diffusion caused by ULF waves and local plasma wave scattering are energy dependent, which lead to the observed electron flux variations with energy dependences. This study suggests that plasma wave distributions in the inner magnetosphere are crucial for the energy-dependent intrusions of several hundred keV to several MeV electrons. C1 [Ma, Q.; Li, W.; Thorne, R. M.; Nishimura, Y.; Zhang, X. -J.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. [Zhang, X. -J.; Angelopoulos, V.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys Earth Planetary & S, Los Angeles, CA USA. [Reeves, G. D.; Henderson, M. G.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Baker, D. N.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO USA. [Blake, J. B.; Fennell, J. F.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. RP Ma, Q (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. EM qianlima@atmos.ucla.edu RI Henderson, Michael/A-3948-2011; OI Henderson, Michael/0000-0003-4975-9029; Ma, Qianli/0000-0001-5452-4756; Reeves, Geoffrey/0000-0002-7985-8098 FU RBSP-ECT; JHU/APL under NASA [967399, 921647, NAS5-01072]; AFOSR [FA9550-15-1-0158]; NASA [NNX15AI96G, NNX15AF61G, NNX11AR64G, NNX13AI61G, NNX14AI18G]; NSF AGS [1405054, 1451911] FX This work was supported by RBSP-ECT and EMFISIS funding provided by JHU/APL contract 967399 and 921647 under NASA's prime contract NAS5-01072. The analysis at UCLA was supported by AFOSR award FA9550-15-1-0158, NASA grants NNX15AI96G, NNX15AF61G, NNX11AR64G, NNX13AI61G, and NNX14AI18G, and the NSF grant AGS 1405054 and 1451911. We acknowledge the Van Allen Probes data from the EMFISIS instrument obtained from http://emfisis.physics.uiowa.edu/Flight/, data from the MagEIS and REPT instruments obtained from http://www.rbsp-ect.lanl.gov/data_pub/, the THEMIS data obtained from http://themis.ssl.berkeley.edu/data/themis/, and the TEC data obtained from http://www.openmadrigal.org/. We thank the World Data Center for Geomagnetism, Kyoto, for providing Kp and Dst indices (http://wdc.kugi.kyoto-u.ac.jp/kp/index.html). NR 73 TC 3 Z9 3 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 4217 EP 4231 DI 10.1002/2016JA022507 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500025 ER PT J AU McComas, DJ Elliott, HA Weidner, S Valek, P Zirnstein, EJ Bagenal, F Delamere, PA Ebert, RW Funsten, HO Horanyi, M McNutt, RL Moser, C Schwadron, NA Strobel, DF Young, LA Ennico, K Olkin, CB Stern, SA Weaver, HA AF McComas, D. J. Elliott, H. A. Weidner, S. Valek, P. Zirnstein, E. J. Bagenal, F. Delamere, P. A. Ebert, R. W. Funsten, H. O. Horanyi, M. McNutt, R. L. Moser, C. Schwadron, N. A. Strobel, D. F. Young, L. A. Ennico, K. Olkin, C. B. Stern, S. A. Weaver, H. A. TI Pluto's interaction with the solar wind SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE Plutopause; Pluto; heavy ion tail; bow shock; solar wind interaction; pickup ions ID CARBON FOILS; KUIPER-BELT; ATMOSPHERE; IRRADIATION; MODELS; HORIZONS; SURFACE; ESCAPE; PLASMA; IONS AB This study provides the first observations of Plutogenic ions and their unique interaction with the solar wind. We find 20% solar wind slowing that maps to a point only 4.5 R-P upstream of Pluto and a bow shock most likely produced by comet-like mass loading. The Pluto obstacle is a region of dense heavy ions bounded by a Plutopause where the solar wind is largely excluded and which extends back >100 R-P into a heavy ion tail. The upstream standoff distance is at only 2.5 R-P. The heavy ion tail contains considerable structure, may still be partially threaded by the interplanetary magnetic field (IMF), and is surrounded by a light ion sheath. The heavy ions (presumably CH4+) have average speed, density, and temperature of 90kms(-1), 0.009cm(-3), and 7x10(5)K, with significant variability, slightly increasing speed/temperature with distance, and are N-S asymmetric. Density and temperature are roughly anticorrelated yielding a pressure 2x10(-2)pPa, roughly in balance with the interstellar pickup ions at 33AU. We set an upper bound of <30nT surface field at Pluto and argue that the obstacle is largely produced by atmospheric thermal pressure like Venus and Mars; we also show that the loss rate down the tail (5x10(23)s(-1)) is only 1% of the expected total CH4 loss rate from Pluto. Finally, we observe a burst of heavy ions upstream from the bow shock as they are becoming picked up and tentatively identify an IMF outward sector at the time of the NH flyby. C1 [McComas, D. J.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08544 USA. [McComas, D. J.; Elliott, H. A.; Weidner, S.; Valek, P.; Zirnstein, E. J.; Ebert, R. W.; Moser, C.] Southwest Res Inst, San Antonio, TX 78238 USA. [McComas, D. J.; Weidner, S.; Valek, P.; Moser, C.] Univ Texas San Antonio, Phys Astron, San Antonio, TX 78249 USA. [Bagenal, F.; Horanyi, M.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO USA. [Delamere, P. A.] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA. [Funsten, H. O.] Los Alamos Natl Lab, Los Alamos, NM USA. [McNutt, R. L.; Weaver, H. A.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. [Schwadron, N. A.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Strobel, D. F.] Johns Hopkins Univ, Earth & Planetary Sci, Baltimore, MD USA. [Young, L. A.; Olkin, C. B.; Stern, S. A.] Southwest Res Inst, Boulder, CO USA. [Ennico, K.] NASA, Ames Res Ctr, Div Space Sci, Moffett Field, CA 94035 USA. RP McComas, DJ (reprint author), Princeton Univ, Plasma Phys Lab, Princeton, NJ 08544 USA.; McComas, DJ (reprint author), Southwest Res Inst, San Antonio, TX 78238 USA.; McComas, DJ (reprint author), Univ Texas San Antonio, Phys Astron, San Antonio, TX 78249 USA. EM dmccomas@princeton.edu OI Valek, Philip/0000-0002-2318-8750 NR 41 TC 6 Z9 6 U1 2 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 4232 EP 4246 DI 10.1002/2016JA022599 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500026 ER PT J AU Zhou, QH Xiao, FL Yang, C Liu, S He, YH Wygant, JR Baker, DN Spence, HE Reeves, GD Funsten, HO AF Zhou, Qinghua Xiao, Fuliang Yang, Chang Liu, Si He, Yihua Wygant, J. R. Baker, D. N. Spence, H. E. Reeves, G. D. Funsten, H. O. TI Evolution of chorus emissions into plasmaspheric hiss observed by Van Allen Probes SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE plasmaspheric hiss; chorus waves; RBSP results ID MAGNETOSONIC WAVES; RADIAL DIFFUSION; ELECTRON-DENSITY; WHISTLER-MODE; MAGNETOSPHERE; ORIGIN AB The two classes of whistler mode waves (chorus and hiss) play different roles in the dynamics of radiation belt energetic electrons. Chorus can efficiently accelerate energetic electrons, and hiss is responsible for the loss of energetic electrons. Previous studies have proposed that chorus is the source of plasmaspheric hiss, but this still requires an observational confirmation because the previously observed chorus and hiss emissions were not in the same frequency range in the same time. Here we report simultaneous observations form Van Allen Probes that chorus and hiss emissions occurred in the same range approximate to 300-1500Hz with the peak wave power density about 10(-5)nT(2)/Hz during a weak storm on 3 July 2014. Chorus emissions propagate in a broad region outside the plasmapause. Meanwhile, hiss emissions are confined inside the plasmasphere, with a higher intensity and a broader area at a lower frequency. A sum of bi-Maxwellian distribution is used to model the observed anisotropic electron distributions and to evaluate the instability of waves. A three-dimensional ray tracing simulation shows that a portion of chorus emission outside the plasmasphere can propagate into the plasmasphere and evolve into plasmaspheric hiss. Moreover, hiss waves below 1kHz are more intense and propagate over a broader area than those above 1kHz, consistent with the observation. The current results can explain distributions of the observed hiss emission and provide a further support for the mechanism of evolution of chorus into hiss emissions. C1 [Zhou, Qinghua; Xiao, Fuliang; Yang, Chang; Liu, Si; He, Yihua] Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha, Hunan, Peoples R China. [Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN USA. [Baker, D. N.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Funsten, H. O.] Los Alamos Natl Lab, ISR Div, Los Alamos, NM USA. RP Xiao, FL (reprint author), Changsha Univ Sci & Technol, Sch Phys & Elect Sci, Changsha, Hunan, Peoples R China. EM flxiao@126.com RI Xiao, Fuliang/B-9245-2011; OI Xiao, Fuliang/0000-0003-1487-6620; Reeves, Geoffrey/0000-0002-7985-8098 FU National Natural Science Foundation of China [41531072, 41274165, 41404130]; JHU/APL under NASA [921647, 967399, NAS5-01072] FX This work is supported by the National Natural Science Foundation of China grants 41531072, 41274165, and 41404130. All the Van Allen Probes data are publicly available at https://emfisis.physics.uiowa.edu/data/index by the EMFISIS suite and at http://www.rbsp-ect.lanl.gov/data_pub/ by the HOPE and MagEIS instruments. The OMNI data are obtained from http://omniweb.gsfc.nasa.gov/form/dx1.html. This work was also supported from JHU/APL contract 921647 and 967399 under NASA Prime contract NAS5-01072. NR 64 TC 1 Z9 1 U1 2 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 4518 EP 4529 DI 10.1002/2016JA022366 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500046 ER PT J AU Rout, D Chakrabarty, D Sekar, R Reeves, GD Ruohoniemi, JM Pant, TK Veenadhari, B Shiokawa, K AF Rout, Diptiranjan Chakrabarty, D. Sekar, R. Reeves, G. D. Ruohoniemi, J. M. Pant, Tarun K. Veenadhari, B. Shiokawa, K. TI An evidence for prompt electric field disturbance driven by changes in the solar wind density under northward IMF B-z condition SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE prompt penetration; solar wind density; equatorial ionosphere ID GEOMAGNETIC SUDDEN COMMENCEMENTS; DYNAMIC PRESSURE ENHANCEMENTS; MAGNETOSPHERIC SUBSTORMS; ALIGNED CURRENTS; LOW LATITUDES; PENETRATION; RESPONSES; EVENT; IONOSPHERE; SIMULATION AB Before the onset of a geomagnetic storm on 22 January 2012 (Ap = 24), an enhancement in solar wind number density from 10/cm(3) to 22/cm(3) during 0440-0510UT under northward interplanetary magnetic field (IMF B-z) condition is shown to have enhanced the high-latitude ionospheric convection and also caused variations in the geomagnetic field globally. Conspicuous changes in X are observed not only at longitudinally separated low-latitude stations over Indian (prenoon), South American (midnight), Japanese (afternoon), Pacific (afternoon) and African (morning) sectors but also at latitudinally separated stations located over high and middle latitudes. The latitudinal variation of the amplitude of the X during 0440-0510UT is shown to be consistent with the characteristics of prompt penetration electric field disturbances. Most importantly, the density pulse event caused enhancements in the equatorial electrojet strength and the peak height of the F layer (h(m)F(2)) over the Indian dip equatorial sector. Further, the concomitant enhancements in electrojet current and F layer movement over the dip equator observed during this space weather event suggest a common driver of prompt electric field disturbance at this time. Such simultaneous variations are found to be absent during magnetically quiet days. In absence of significant change in solar wind velocity and magnetospheric substorm activity, these observations point toward perceptible prompt electric field disturbance over the dip equator driven by the overcompression of the magnetosphere by solar wind density enhancement. C1 [Rout, Diptiranjan; Chakrabarty, D.; Sekar, R.] Phys Res Lab, Ahmadabad, Gujarat, India. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Ruohoniemi, J. M.] Virginia Polytech Inst & State Univ, Bradley Dept Elect & Comp Engn, Blacksburg, VA 24061 USA. [Pant, Tarun K.] VSSC, Space Phys Lab, Thiruvananthapuram, Kerala, India. [Veenadhari, B.] Indian Inst Geomagnetism, Navi Mumbai, India. [Shiokawa, K.] Nagoya Univ, ISEE, Nagoya, Aichi, Japan. RP Rout, D (reprint author), Phys Res Lab, Ahmadabad, Gujarat, India. EM diptir@prl.res.in OI Reeves, Geoffrey/0000-0002-7985-8098 FU JSPS; B. Asia-Africa Science Platforms; JSPS KAKENHI [16H06286, 15H05815] FX Magnetic data from the three Indian stations (TIR, ABG, and JPR) are provided by Indian Institute of Geomagnetism, India. Data from the one Japanese station (KTB) is provided by the Solar Terrestrial Environment Laboratory, Japan, and this station is part of 210 MM chain (http://stdb2.stelab.nagoya-u.ac.jp/mm210/). This work of K.S. is supported by the JSPS Core-to-Core Program, B. Asia-Africa Science Platforms, and JSPS KAKENHI grants 16H06286 and 15H05815. All the other representative magnetic data used in this work are taken from SuperMAG network (http://supermag.jhuapl.edu). The authors are grateful to the PIs of the magnetic observatories and the National institutes that support the observatories based on which the present study is carried out. SuperDARN data are available from the Virginia Tech SuperDARN website (http://vt.superdarn.org/). SuperDARN is a collection of radars funded by national scientific funding agencies of Australia, Canada, China, France, Japan, South Africa, United Kingdom and United States of America. The geosynchronous particle injection data are provided by Los Alamos National Laboratory, USA. The geomagnetic indices and solar wind data are obtained from NASA GSFC CDAWeb (http://cdaweb.gsfc.nasa.gov/). We thank the reviewers for the insightful comments. NR 38 TC 0 Z9 0 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD MAY PY 2016 VL 121 IS 5 BP 4800 EP 4810 DI 10.1002/2016JA022475 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR6QD UT WOS:000380025500066 ER PT J AU Chantel, J Manthilake, G Andrault, D Novella, D Yu, T Wang, YB AF Chantel, Julien Manthilake, Geeth Andrault, Denis Novella, Davide Yu, Tony Wang, Yanbin TI Experimental evidence supports mantle partial melting in the asthenosphere SO SCIENCE ADVANCES LA English DT Article ID LOW-VELOCITY ZONE; ELECTRICAL-CONDUCTIVITY; POLYCRYSTALLINE OLIVINE; SHEAR ATTENUATION; WAVE ATTENUATION; SEISMIC EVIDENCE; BASALTIC MELT; PLATE FLEXURE; TRAVEL-TIMES; MODEL AB The low-velocity zone (LVZ) is a persistent seismic feature in a broad range of geological contexts. It coincides in depth with the asthenosphere, a mantle region of lowered viscosity that may be essential to enabling plate motions. The LVZ has been proposed to originate from either partial melting or a change in the rheological properties of solid mantle minerals. The two scenarios imply drastically distinct physical and geochemical states, leading to fundamentally different conclusions on the dynamics of plate tectonics. We report in situ ultrasonic velocity measurements on a series of partially molten samples, composed of mixtures of olivine plus 0.1 to 4.0 volume % of basalt, under conditions relevant to the LVZ. Our measurements provide direct compressional (VP) and shear (V-S) wave velocities and constrain attenuation as a function of melt fraction. Mantle partial melting appears to be a viable origin for the LVZ, for melt fractions as low as similar to 0.2%. In contrast, the presence of volatile elements appears necessary to explaining the extremely high V-P/V-S values observed in some local areas. The presence of melt in LVZ could play a major role in the dynamics of plate tectonics, favoring the decoupling of the plate relative to the asthenosphere. C1 [Chantel, Julien; Manthilake, Geeth; Andrault, Denis; Novella, Davide] Univ Clermont Ferrand, Inst Rech Dev, CNRS UMR 6524, Lab Magmas & Volcans, F-63178 Clermont Ferrand, France. [Yu, Tony; Wang, Yanbin] Univ Chicago, Ctr Adv Radiat Source, Chicago, IL 60637 USA. [Chantel, Julien] Case Western Reserve Univ, Dept Earth Environm & Planetary Sci, Cleveland, OH 44106 USA. [Novella, Davide] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Chantel, J (reprint author), Univ Clermont Ferrand, Inst Rech Dev, CNRS UMR 6524, Lab Magmas & Volcans, F-63178 Clermont Ferrand, France.; Chantel, J (reprint author), Case Western Reserve Univ, Dept Earth Environm & Planetary Sci, Cleveland, OH 44106 USA. EM julien.chantel@case.edu RI ANDRAULT, Denis/N-8843-2016 OI ANDRAULT, Denis/0000-0002-9921-4572 NR 71 TC 3 Z9 3 U1 14 U2 24 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 2375-2548 J9 SCI ADV JI Sci. Adv. PD MAY PY 2016 VL 2 IS 5 AR UNSP e1600246 DI 10.1126/sciadv.1600246 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR7IK UT WOS:000380073000034 PM 27386548 ER PT J AU Manthilake, G Bolfan-Casanova, N Novella, D Mookherjee, M Andrault, D AF Manthilake, Geeth Bolfan-Casanova, Nathalie Novella, Davide Mookherjee, Mainak Andrault, Denis TI Dehydration of chlorite explains anomalously high electrical conductivity in the mantle wedges SO SCIENCE ADVANCES LA English DT Article ID SUBDUCTION ZONE; SOUTHWESTERN JAPAN; FLUID; GPA; MAGNETITE; CRUST; TEMPERATURES; RESISTIVITY; PRESSURES; STABILITY AB Mantle wedge regions in subduction zone settings show anomalously high electrical conductivity (similar to 1 S/m) that has often been attributed to the presence of aqueous fluids released by slab dehydration. Laboratory-based measurements of the electrical conductivity of hydrous phases and aqueous fluids are significantly lower and cannot readily explain the geophysically observed anomalously high electrical conductivity. The released aqueous fluid also rehydrates the mantle wedge and stabilizes a suite of hydrous phases, including serpentine and chlorite. In this present study, we have measured the electrical conductivity of a natural chlorite at pressures and temperatures relevant for the subduction zone setting. In our experiment, we observe two distinct conductivity enhancements when chlorite is heated to temperatures beyond its thermodynamic stability field. The initial increase in electrical conductivity to similar to 3 x 10(-3) S/m can be attributed to chlorite dehydration and the release of aqueous fluids. This is followed by a unique, subsequent enhancement of electrical conductivity of up to 7 x 10(-1) S/m. This is related to the growth of an interconnected network of a highly conductive and chemically impure magnetite mineral phase. Thus, the dehydration of chlorite and associated processes are likely to be crucial in explaining the anomalously high electrical conductivity observed in mantle wedges. Chlorite dehydration in the mantle wedge provides an additional source of aqueous fluid above the slab and could also be responsible for the fixed depth (120 +/- 40 km) of melting at the top of the subducting slab beneath the subduction-related volcanic arc front. C1 [Manthilake, Geeth; Bolfan-Casanova, Nathalie; Novella, Davide; Andrault, Denis] Univ Clermont Ferrand, CNRS, Inst Rech Dev, Lab Magmas & Volcans,UMR 6524, F-63178 Clermont Ferrand, France. [Mookherjee, Mainak] Florida State Univ, Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Novella, Davide] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Manthilake, G (reprint author), Univ Clermont Ferrand, CNRS, Inst Rech Dev, Lab Magmas & Volcans,UMR 6524, F-63178 Clermont Ferrand, France. EM g.manthilake@opgc.univ-bpclermont.fr RI ANDRAULT, Denis/N-8843-2016; Mookherjee, Mainak/F-7949-2010 OI ANDRAULT, Denis/0000-0002-9921-4572; Mookherjee, Mainak/0000-0002-0605-5964 NR 39 TC 0 Z9 0 U1 5 U2 7 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 2375-2548 J9 SCI ADV JI Sci. Adv. PD MAY PY 2016 VL 2 IS 5 AR e1501631 DI 10.1126/sciadv.1501631 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR7IK UT WOS:000380073000012 PM 27386526 ER PT J AU Hogue, S Marland, E Andres, RJ Marland, G Woodard, D AF Hogue, Susannah Marland, Eric Andres, Robert J. Marland, Gregg Woodard, Dawn TI Uncertainty in gridded CO2 emissions estimates SO EARTHS FUTURE LA English DT Article DE U; S; CO2 emissions; gridded emissions; large point sources; CO2 proxy data ID CARBON-DIOXIDE EMISSIONS; FOSSIL-FUEL COMBUSTION AB We are interested in the spatial distribution of fossil-fuel-related emissions of CO2 for both geochemical and geopolitical reasons, but it is important to understand the uncertainty that exists in spatially explicit emissions estimates. Working from one of the widely used gridded data sets of CO2 emissions, we examine the elements of uncertainty, focusing on gridded data for the United States at the scale of 1 degrees latitude by 1 degrees longitude. Uncertainty is introduced in the magnitude of total United States emissions, the magnitude and location of large point sources, the magnitude and distribution of non-point sources, and from the use of proxy data to characterize emissions. For the United States, we develop estimates of the contribution of each component of uncertainty. At 1 degrees resolution, in most grid cells, the largest contribution to uncertainty comes from how well the distribution of the proxy (in this case population density) represents the distribution of emissions. In other grid cells, the magnitude and location of large point sources make the major contribution to uncertainty. Uncertainty in population density can be important where a large gradient in population density occurs near a grid cell boundary. Uncertainty is strongly scale-dependent with uncertainty increasing as grid size decreases. Uncertainty for our data set with 1 degrees grid cells for the United States is typically on the order of 150%, but this is perhaps not excessive in a data set where emissions per grid cell vary over 8 orders of magnitude. C1 [Hogue, Susannah; Marland, Eric] Appalachian State Univ, Dept Math Sci, Boone, NC 28608 USA. [Marland, Eric; Marland, Gregg] Appalachian State Univ, Res Inst Environm Energy & Econ, Boone, NC 28608 USA. [Andres, Robert J.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Woodard, Dawn] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA USA. RP Marland, E (reprint author), Appalachian State Univ, Dept Math Sci, Boone, NC 28608 USA.; Marland, E (reprint author), Appalachian State Univ, Res Inst Environm Energy & Econ, Boone, NC 28608 USA. EM marlandes@appstate.edu FU NASA CMS grant [NNH11ZDA001N-CMS] FX This work could not have been done without the help of many people. We offer special thanks to Appalachian State CMS team members G. Buckingham, M. Branham, and M. Hutchins for valuable input and feedback. We are grateful to Charles Robison for help with the graphics and to Jeff Quick for helping in the application of his data. Two anonymous reviewers have contributed importantly to the clarity and completeness of our discussion. Portions of this work were supported by NASA CMS grant NNH11ZDA001N-CMS. Data for all of the maps shown in this article are available at https://libres.uncg.edu/ir/asu/listing.aspx?id=19166. NR 18 TC 1 Z9 1 U1 4 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2328-4277 J9 EARTHS FUTURE JI Earth Future PD MAY PY 2016 VL 4 IS 5 BP 225 EP 239 DI 10.1002/2015EF000343 PG 15 WC Environmental Sciences; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Geology; Meteorology & Atmospheric Sciences GA DR1LP UT WOS:000379667300007 ER PT J AU Ahmed, T Azad, AK Chellappa, R Higginbotham-Duque, A Dattelbaum, DM Zhu, JX Moore, D Graf, MJ AF Ahmed, Towfiq Azad, Abul K. Chellappa, Raja Higginbotham-Duque, Amanda Dattelbaum, Dana M. Zhu, Jian-Xin Moore, David Graf, Matthias J. TI Vibrational signatures in the THz spectrum of 1,3-DNB: A first-principles and experimental study SO EPL LA English DT Article ID CRYSTALLOGRAPHY OPEN DATABASE; OPEN-ACCESS COLLECTION; ULTRASOFT PSEUDOPOTENTIALS; MOLECULAR-CRYSTALS; AB-INITIO; EXPLOSIVES; SPECTROSCOPY AB Understanding the fundamental processes of light-matter interaction is important for detection of explosives and other energetic materials, which are active in the infrared and terahertz (THz) region. We report a comprehensive study on electronic and vibrational lattice properties of structurally similar 1,3-dinitrobenzene (1,3-DNB) crystals through first-principles electronic structure calculations and THz spectroscopy measurements on polycrystalline samples. Starting from reported x-ray crystal structures, we use density-functional theory (DFT) with periodic boundary conditions to optimize the structures and perform linear response calculations of the vibrational properties at zero phonon momentum. The theoretically identified normal modes agree qualitatively with those obtained experimentally in a frequency range up to 2.5THz and quantitatively at much higher frequencies. The latter frequencies are set by intra-molecular forces. Our results suggest that van der Waals dispersion forces need to be included to improve the agreement between theory and experiment in the THz region, which is dominated by intermolecular modes and sensitive to details in the DFT calculation. An improved comparison is needed to assess and distinguish between intra-and intermolecular vibrational modes characteristic of energetic materials. Copyright (C) EPLA, 2016 C1 [Ahmed, Towfiq; Zhu, Jian-Xin; Graf, Matthias J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Azad, Abul K.; Zhu, Jian-Xin] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Chellappa, Raja] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Higginbotham-Duque, Amanda; Dattelbaum, Dana M.; Moore, David] Los Alamos Natl Lab, Shock & Detonat Phys, Los Alamos, NM 87545 USA. [Graf, Matthias J.] US DOE, Off Sci, Washington, DC 20585 USA. RP Ahmed, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM atowfiq@lanl.gov; aazad@lanl.gov OI Azad, Abul/0000-0002-7784-7432; Duque, Amanda/0000-0002-2023-1389 FU U.S. DOE through the LDRD Program [DE-AC52-06NA25396]; NERSC, a U.S. DOE Office of Basic Energy Sciences [DE-AC02-05CH11231] FX We thank XIAODONG WEN for helpful discussions regarding the DFT calculations and crystallographic databases. This work was supported by the U.S. DOE under Contract No. DE-AC52-06NA25396 through the LDRD Program. We gratefully acknowledge computing allocations by NERSC, a U.S. DOE Office of Basic Energy Sciences user facility, under Contract No. DE-AC02-05CH11231. NR 23 TC 0 Z9 0 U1 5 U2 6 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD MAY PY 2016 VL 114 IS 3 AR 37010 DI 10.1209/0295-5075/114/37010 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9HY UT WOS:000379522200026 ER PT J AU Chern, GW Mellado, P AF Chern, Gia-Wei Mellado, Paula TI Magnetic monopole polarons in artificial spin ices SO EPL LA English DT Article ID CHARGE; DYNAMICS; LATTICE AB Emergent quasiparticles that arise from the fractionalization of the microscopic degrees of freedom have been one of the central themes in modern condensed-matter physics. The notion of magnetic monopoles, freely moving quasiparticles fragmented from local dipole excitations, has enjoyed much success in understanding the thermodynamic, static, and transport properties of the so-called spin-ice materials. The artificial version of spin ice, where a lattice of nanoscale magnetic dipoles is sculpted out of a ferromagnetic film, provides a unique opportunity to study these unusual quasiparticles in a material-by-design approach. Here we show that the elementary excitations in the ice phase of a nano-magnetic array arranged in the pentagonal lattice are composite objects comprised of the emergent monopole and a surrounding cloud of opposite uncompensated magnetic charges. Copyright (C) EPLA, 2016 C1 [Chern, Gia-Wei] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA. [Chern, Gia-Wei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chern, Gia-Wei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Mellado, Paula] Univ Adolfo Ibanez, Dept Sci & Engn, Santiago, Chile. RP Chern, GW (reprint author), Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA.; Chern, GW (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Chern, GW (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. FU LANL Oppenheimer Fellowship; Fondecyt [11121397]; Conicyt [79112004] FX We gratefully acknowledge insightful discussions with J. CUMINGS, C. NISOLI, P. SCHIFFER, and O. TCHERNYSHYOV. G-WC acknowledges the support of the LANL Oppenheimer Fellowship. PM acknowledges the support from Fondecyt project No 11121397, and Conicyt, project No 79112004. NR 35 TC 1 Z9 1 U1 5 U2 9 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD MAY PY 2016 VL 114 IS 3 AR 37004 DI 10.1209/0295-5075/114/37004 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9HY UT WOS:000379522200020 ER PT J AU Colgan, J Faenov, AY Pikuz, SA Tubman, E Butler, NMH Abdallah, J Dance, RJ Pikuz, TA Skobelev, IY Alkhimova, MA Booth, N Green, J Gregory, C Andreev, A Lotzsch, R Uschmann, I Zhidkov, A Kodama, R McKenna, P Woolsey, N AF Colgan, J. Faenov, A. Ya. Pikuz, S. A. Tubman, E. Butler, N. M. H. Abdallah, J., Jr. Dance, R. J. Pikuz, T. A. Skobelev, I. Yu. Alkhimova, M. A. Booth, N. Green, J. Gregory, C. Andreev, A. Loetzsch, R. Uschmann, I. Zhidkov, A. Kodama, R. McKenna, P. Woolsey, N. TI Evidence of high-n hollow-ion emission from Si ions pumped by ultraintense x-rays from relativistic laser plasma SO EPL LA English DT Article ID FEMTOSECOND LASER; ATOMS; SPECTRA; IONIZATION; OPACITY; PULSES AB We report on the first observation of high-n hollow ions (ions having no electrons in the K or L shells) produced in Si targets via pumping by ultra-intense x-ray radiation produced in intense laser-plasma interactions reaching the radiation dominant kinetics regime (RDKR). The existence of these new types of hollow ions in high-energy density plasma has been found via observation of highly resolved x-ray emission spectra of silicon plasma. This has been confirmed by plasma kinetics calculations, underscoring the ability of powerful radiation sources to fully strip electrons from the innermost shells of light atoms. Hollow-ions spectral diagnostics provide a unique opportunity to characterize powerful x-ray radiation of laboratory and astrophysical plasmas. With the use of this technique we provide evidence for the existence of the RDKR via observation of asymmetry in the observed radiation of hollow ions from the front and rear sides of the target. Copyright (C) EPLA, 2016 C1 [Colgan, J.; Abdallah, J., Jr.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Faenov, A. Ya.; Kodama, R.] Osaka Univ, Inst Acad Initiat, Suita, Osaka 5650871, Japan. [Faenov, A. Ya.; Pikuz, S. A.; Pikuz, T. A.; Skobelev, I. Yu.; Alkhimova, M. A.] Russian Acad Sci, Joint Inst High Temp, Moscow 125412, Russia. [Pikuz, S. A.; Skobelev, I. Yu.; Alkhimova, M. A.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Tubman, E.; Woolsey, N.] Univ York, Dept Phys, York Plasma Inst, York YO10 5DD, N Yorkshire, England. [Butler, N. M. H.; Dance, R. J.; McKenna, P.] Univ Strathclyde, Dept Phys, SUPA, Glasgow G4 ONG, Lanark, Scotland. [Pikuz, T. A.; Zhidkov, A.; Kodama, R.] PPC Osaka Univ, 2-1 Yamadaoka, Suita, Osaka 5650871, Japan. [Pikuz, T. A.; Zhidkov, A.; Kodama, R.] JST, CREST, 2-1 Yamadaoka, Suita, Osaka 5650871, Japan. [Booth, N.; Green, J.; Gregory, C.] STFC Rutherford Appleton Lab Didcot, Cent Laser Facil, Didcot OX11 0QX, Oxon, England. [Andreev, A.] Max Born Inst Berlin 12489, Max Born Str 2a, Berlin, Germany. [Andreev, A.] ELI ALPS, H-6720 Szeged, Hungary. [Loetzsch, R.; Uschmann, I.] Univ Jena, Inst Opt & Quantenelekt, Max Wien Pl 1, D-07743 Jena, Germany. RP Colgan, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI McKenna, Paul/B-9764-2009; Kodama, Ryosuke/G-2627-2016 OI McKenna, Paul/0000-0001-8061-7091; FU Science and Technology Facilities Council; Engineering and Physical Science Research Council of the United Kingdom [EP/J003832/1]; NNSA of the U.S. DOE [DE-AC5206NA25396]; Russian Foundation for Basic Research [15-32-21121, 14-22-02089] FX We thank the Vulcan technical and target preparation teams at the Central Laser Facility for their support during the experiments. The research leading to these results has received funding from the Science and Technology Facilities Council, and the Engineering and Physical Science Research Council (Grant No. EP/J003832/1) of the United Kingdom. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC5206NA25396. The work is supported by Russian Foundation for Basic Research via grants No. 15-32-21121 and No. 14-22-02089. NR 36 TC 2 Z9 2 U1 1 U2 4 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD MAY PY 2016 VL 114 IS 3 AR 35001 DI 10.1209/0295-5075/114/35001 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9HY UT WOS:000379522200012 ER PT J AU Nass, K Meinhart, A Barends, TRM Foucar, L Gorel, A Aquila, A Botha, S Doak, RB Koglin, J Liang, MN Shoeman, RL Williams, G Boutet, S Schlichting, I AF Nass, Karol Meinhart, Anton Barends, Thomas R. M. Foucar, Lutz Gorel, Alexander Aquila, Andrew Botha, Sabine Doak, R. Bruce Koglin, Jason Liang, Mengning Shoeman, Robert L. Williams, Garth Boutet, Sebastien Schlichting, Ilme TI Protein structure determination by single-wavelength anomalous diffraction phasing of X-ray free-electron laser data SO IUCRJ LA English DT Article DE serial femtosecond crystallography; SFX; X-ray free-electron lasers; XFELs; SAD phasing; single wavelength anomalous diffraction ID SERIAL FEMTOSECOND CRYSTALLOGRAPHY; CRYSTAL-STRUCTURE; MACROMOLECULAR CRYSTALLOGRAPHY; NATIVE-SAD; RESOLUTION; SULFUR; NANOCRYSTALLOGRAPHY; REFINEMENT; INSTRUMENT; MODEL AB Serial femtosecond crystallography (SFX) at X-ray free-electron lasers (XFELs) offers unprecedented possibilities for macromolecular structure determination of systems that are prone to radiation damage. However, phasing XFEL data de novo is complicated by the inherent inaccuracy of SFX data, and only a few successful examples, mostly based on exceedingly strong anomalous or isomorphous difference signals, have been reported. Here, it is shown that SFX data from thaumatin microcrystals can be successfully phased using only the weak anomalous scattering from the endogenous S atoms. Moreover, a step-by-step investigation is presented of the particular problems of SAD phasing of SFX data, analysing data from a derivative with a strong anomalous signal as well as the weak signal from endogenous S atoms. C1 [Nass, Karol; Meinhart, Anton; Barends, Thomas R. M.; Foucar, Lutz; Gorel, Alexander; Botha, Sabine; Doak, R. Bruce; Shoeman, Robert L.; Schlichting, Ilme] Max Planck Inst Med Res, Dept Biomol Mech, Jahnstr 29, D-69120 Heidelberg, Germany. [Aquila, Andrew] European XFEL GmbH, Albert Einstein Ring 19, D-22761 Hamburg, Germany. [Aquila, Andrew; Koglin, Jason; Liang, Mengning; Williams, Garth; Boutet, Sebastien] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA USA. [Botha, Sabine] Univ Hamburg, Dept Chem, Martin Luther King Pl 6, D-20146 Hamburg, Germany. [Williams, Garth] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Schlichting, I (reprint author), Max Planck Inst Med Res, Dept Biomol Mech, Jahnstr 29, D-69120 Heidelberg, Germany. EM ilme.schlichting@mpimf-heidelberg.mpg.de FU US Department of Energy, Office of Science and Office of Basic Energy Sciences [DE-AC02-76SF00515]; LCLS Ultrafast Science Instruments (LUSI) project - US Department of Energy, Office of Basic Energy Sciences; Max Planck Society; Center for Modelling and Simulation in the Biosciences (BIOMS), Heidelberg FX Use of the Linac Coherent Light Source (LCLS), SLAC National Accelerator Laboratory is supported by the US Department of Energy, Office of Science and Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The CXI instrument was funded by the LCLS Ultrafast Science Instruments (LUSI) project funded by the US Department of Energy, Office of Basic Energy Sciences. We acknowledge support from the Max Planck Society and from the Center for Modelling and Simulation in the Biosciences (BIOMS), Heidelberg to KN. We are indebted to S. Pesch and R. van Gessel (Bracco Imaging Konstanz and Singen, Germany) for the kind gift of the sample of gadoteridol used for the derivatization of lysozyme microcrystals. We thank Beatrice Latz for preparing GDVN nozzles and Chris Roome and Frank Koeck for excellent computing support. We also thank Dr Tobias Weinert of the Paul Scherrer Institute in Villigen, Switzerland for the collection of the thaumatin synchrotron reference data set. NR 52 TC 6 Z9 6 U1 4 U2 4 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2052-2525 J9 IUCRJ JI IUCrJ PD MAY PY 2016 VL 3 BP 180 EP 191 DI 10.1107/S2052252516002980 PN 3 PG 12 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA DR0KZ UT WOS:000379597700004 PM 27158504 ER PT J AU Elliott, J Hoemmen, M Mueller, F AF Elliott, J. Hoemmen, M. Mueller, F. TI Exploiting data representation for fault tolerance SO JOURNAL OF COMPUTATIONAL SCIENCE LA English DT Article DE Algorithm-based fault tolerance; Resilient algorithms; Numerical methods ID SUPERCOMPUTER; GMRES AB Incorrect computer hardware behavior may corrupt intermediate computations in numerical algorithms, possibly resulting in incorrect answers. Prior work models misbehaving hardware by randomly flipping bits in memory. We start by accepting this premise, and present an analytic model for the error introduced by a bit flip in an IEEE 754 floating-point number. We then relate this finding to the linear algebra concepts of normalization and matrix equilibration. In particular, we present a case study illustrating that normalizing both vector inputs of a dot product minimizes the probability of a single bit flip causing a large error in the dot product's result. Furthermore, the absolute error is either less than one or very large, which allows detection of large errors. Then, we apply this to the GMRES iterative solver. We count all possible errors that can be introduced through faults in arithmetic in the computationally intensive orthogonalization phase of GMRES, and show that when the matrix is equilibrated, the absolute error is bounded above by one. (C) 2016 Elsevier B.V. All rights reserved. C1 [Elliott, J.; Mueller, F.] North Carolina State Univ, Dept Comp Sci, Raleigh, NC 27695 USA. [Elliott, J.; Hoemmen, M.] Sandia Natl Labs, Ctr Res Comp, POB 5800, Albuquerque, NM 87185 USA. RP Elliott, J (reprint author), North Carolina State Univ, Dept Comp Sci, Raleigh, NC 27695 USA. EM jjellio3@ncsu.edu; mhoemme@sandia.gov; mueller@cs.ncsu.edu FU NSF [1058779, 0958311]; U.S. Department of Energy Office of Science, Advanced Scientific Computing Research; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported in part by grants from NSF (awards 1058779 and 0958311) and the U.S. Department of Energy Office of Science, Advanced Scientific Computing Research, under Program Manager Dr. Karen Pao.; Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 28 TC 1 Z9 1 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-7503 J9 J COMPUT SCI-NETH JI J. Comput. Sci. PD MAY PY 2016 VL 14 SI SI BP 51 EP 60 DI 10.1016/j.jocs.2015.12.002 PG 10 WC Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA DQ9WM UT WOS:000379560000006 ER PT J AU Hseuh, HC Hetzel, C Leng, SW Wilson, K Xu, HJ Zigrosser, D AF Hseuh, Hsiao-Chaun Hetzel, Charles Leng, Shuwei Wilson, King Xu, Huijuan Zigrosser, Douglas TI National Synchrotron Light Source II storage ring vacuum systems SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article AB The National Synchrotron Light Source II, completed in 2014, is a 3-GeV synchrotron radiation (SR) facility at Brookhaven National Laboratory and has been in steady operation since. With a design electron current of 500 mA and subnanometer radians horizontal emittance, this 792-m circumference storage ring is providing the highest flux and brightness x-ray beam for SR users. The majority of the storage ring vacuum chambers are made of extruded aluminium. Chamber sections are interconnected using low-impedance radiofrequency shielded bellows. SR from the bending magnets is intercepted by water-cooled compact photon absorbers resided in the storage ring chambers. This paper presents the design of the storage ring vacuum system, the fabrication of vacuum chambers and other hardware, the installation, the commissioning, and the continuing beam conditioning of the vacuum systems. (C) 2016 American Vacuum Society. C1 [Hseuh, Hsiao-Chaun; Hetzel, Charles; Leng, Shuwei; Wilson, King; Xu, Huijuan; Zigrosser, Douglas] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Hseuh, HC (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM hseuh@bnl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC00112704] FX Work at National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC00112704. The authors thank many colleagues at NSLS-II and in Brookhaven for their guidance and support during design and construction of the vacuum systems. The authors also thank many colleagues at other accelerator facilities for their valuable assistance in the design and fabrication of NSLS-II vacuum systems, in particular, Joe Gagliano and George Goeppner of APS, Gao-Yu Hsiung and Che-Kai Chan of National Synchrotron Radiation Research Center in Taiwan, and Marcelo Ferreira of European Spallation Source in Sweden, to name a few. NR 12 TC 0 Z9 0 U1 0 U2 0 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAY PY 2016 VL 34 IS 3 AR 031603 DI 10.1116/1.4945406 PG 7 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DR3GZ UT WOS:000379792200032 ER PT J AU Weiland, C Rumaiz, AK Pianetta, P Woicik, JC AF Weiland, Conan Rumaiz, Abdul K. Pianetta, Piero Woicik, Joseph C. TI Recent applications of hard x-ray photoelectron spectroscopy SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Review ID ANGULAR-DISTRIBUTION PARAMETERS; AUGER-ELECTRON-SPECTROSCOPY; RANGE 100-5000 EV; STANDING WAVES; PHOTOEMISSION-SPECTROSCOPY; VALENCE-BAND; OXIDE INTERFACES; KINETIC-ENERGY; HETEROJUNCTION DISCONTINUITIES; SEMICONDUCTOR HETEROJUNCTIONS AB Recent applications of hard x-ray photoelectron spectroscopy (HAXPES) demonstrate its many capabilities in addition to several of its limitations. Examples are given, including measurement of buried interfaces and materials under in situ or in operando conditions, as well as measurements under x-ray standing-wave and resonant excitation. Physical considerations that differentiate HAXPES from photoemission measurements utilizing soft x-ray and ultraviolet photon sources are also presented. C1 [Weiland, Conan; Woicik, Joseph C.] NIST, Gaithersburg, MD 20899 USA. [Rumaiz, Abdul K.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Pianetta, Piero] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Woicik, JC (reprint author), NIST, Gaithersburg, MD 20899 USA. EM Joseph.Woicik@NIST.gov NR 160 TC 1 Z9 1 U1 16 U2 21 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD MAY PY 2016 VL 34 IS 3 AR 030801 DI 10.1116/1.4946046 PG 21 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA DR3GZ UT WOS:000379792200001 ER PT J AU Yang, JC Kuo, CY Liu, HJ Ding, HC Duan, CG Lin, HJ Hu, Z Pi, TW Tjeng, LH Chen, CT Arenholz, E He, Q Chu, YH AF Yang, Jan-Chi Kuo, Chang-Yang Liu, Heng-Jui Ding, Hang-Chen Duan, Chun-Gang Lin, Hong-Ji Hu, Zhiwei Pi, Tun-Wen Tjeng, Liu Hao Chen, Chien-Te Arenholz, Elke He, Qing Chu, Ying-Hao TI Electrically enhanced magnetization in highly strained BiFeO3 films SO NPG ASIA MATERIALS LA English DT Article ID ROOM-TEMPERATURE; THIN-FILMS; MULTIFERROICS; FERROMAGNETISM; FIELD AB The control of magnetism via an electric field has attracted substantial attention because of potential applications in magnetoelectronics, spintronics and high-frequency devices. In this study, we demonstrate a new approach to enhance and control the magnetization of multiferroic thin film by an electric stimulus. First, to reduce the strength of the antiferromagnetic superexchange interaction in BiFeO3, we applied strain engineering to stabilize a highly strained phase. Second, the direction of the ferroelectric polarization was controlled by an electric field to enhance the Dzyaloshinskii-Moriya interaction in the highly strained BiFeO3 phase. Because of the magnetoelectric coupling in BiFeO3, a strong correlation between the modulated ferroelectricity and enhanced magnetization was observed. The tunability of this strong correlation by an electric field provides an intriguing route to control ferromagnetism in a single-phase multiferroic. C1 [Yang, Jan-Chi; Kuo, Chang-Yang; Hu, Zhiwei; Tjeng, Liu Hao] Max Planck Inst Chem Phys Solids, Dresden, Germany. [Liu, Heng-Jui; Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Room 709,Engn Bldg VI,1001 Univ Rd, Hsinchu 30010, Taiwan. [Ding, Hang-Chen; Duan, Chun-Gang] E China Normal Univ, Key Lab Polar Mat & Devices, Minist Educ, Shanghai, Peoples R China. [Lin, Hong-Ji; Pi, Tun-Wen; Chen, Chien-Te] Natl Synchrotron Radiat Res, Hsinchu, Taiwan. [Arenholz, Elke] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA USA. [He, Qing] Univ Durham, Dept Phys, Room 235,Rochester Bldg,Sci Site,South Rd, Durham DH1 3LE, England. [Chu, Ying-Hao] Acad Sinica, Inst Phys, Taipei, Taiwan. RP Chu, YH (reprint author), Natl Chiao Tung Univ, Dept Mat Sci & Engn, Room 709,Engn Bldg VI,1001 Univ Rd, Hsinchu 30010, Taiwan.; He, Q (reprint author), Univ Durham, Dept Phys, Room 235,Rochester Bldg,Sci Site,South Rd, Durham DH1 3LE, England. EM qing.he@durham.ac.uk; yhc@nctu.edu.tw RI Duan, Chun-Gang/D-2755-2013; He, Qing/E-3202-2010; Ying-Hao, Chu/A-4204-2008 OI Ying-Hao, Chu/0000-0002-3435-9084 FU Ministry of Science and Technology, R.O.C. [MOST 103-2119-M-009-003-MY3]; Center for Interdisciplinary Science of National Chiao Tung University, Ministry of Education [MOE-ATU 101W961]; National Key Project for Basic Research of China [2014CB921104, 2013CB922301]; NSFC [61125403] FX We acknowledge the insightful suggestions from Prof R Ramesh. This work was supported by the Ministry of Science and Technology, R.O.C. (MOST 103-2119-M-009-003-MY3), and the Center for Interdisciplinary Science of National Chiao Tung University, Ministry of Education (MOE-ATU 101W961). CGD is supported by the National Key Project for Basic Research of China (Grants No. 2014CB921104 and 2013CB922301) and the NSFC under Grant No. 61125403. NR 37 TC 0 Z9 0 U1 16 U2 26 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1884-4049 EI 1884-4057 J9 NPG ASIA MATER JI NPG Asia Mater. PD MAY PY 2016 VL 8 AR e269 DI 10.1038/am.2016.55 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA DR2UM UT WOS:000379759400002 ER PT J AU Horn, PJ Liu, JJ Cocuron, JC McGlew, K Thrower, NA Larson, M Lu, CF Alonso, AP Ohlrogge, J AF Horn, Patrick J. Liu, Jinjie Cocuron, Jean-Christophe McGlew, Kathleen Thrower, Nicholas A. Larson, Matt Lu, Chaofu Alonso, Ana P. Ohlrogge, John TI Identification of multiple lipid genes with modifications in expression and sequence associated with the evolution of hydroxy fatty acid accumulation in Physaria fendleri SO PLANT JOURNAL LA English DT Article DE Physaria fendleri; Camelina sativa; hydroxy fatty acids; oilseeds; evolution; transcriptomics; metabolic engineering; RNA-Seq ID RNA-SEQ DATA; RICINUS-COMMUNIS L; SEED-OIL; ACYL-COA; TRIACYLGLYCEROL SYNTHESIS; MICROSOMAL PREPARATIONS; TRANSGENIC ARABIDOPSIS; LESQUERELLA-FENDLERI; CAMELINA-SATIVA; DIACYLGLYCEROL ACYLTRANSFERASE AB Two Brassicaceae species, Physaria fendleri and Camelina sativa, are genetically very closely related to each other and to Arabidopsis thaliana. Physaria fendleri seeds contain over 50% hydroxy fatty acids (HFAs), while Camelina sativa and Arabidopsis do not accumulate HFAs. To better understand how plants evolved new biochemical pathways with the capacity to accumulate high levels of unusual fatty acids, transcript expression and protein sequences of developing seeds of Physaria fendleri, wild-type Camelina sativa, and Camelina sativa expressing a castor bean (Ricinus communis) hydroxylase were analyzed. A number of potential evolutionary adaptations within lipid metabolism that probably enhance HFA production and accumulation in Physaria fendleri, and, in their absence, limit accumulation in transgenic tissues were revealed. These adaptations occurred in at least 20 genes within several lipid pathways from the onset of fatty acid synthesis and its regulation to the assembly of triacylglycerols. Lipid genes of Physaria fendleri appear to have co-evolved through modulation of transcriptional abundances and alterations within protein sequences. Only a handful of genes showed evidence for sequence adaptation through gene duplication. Collectively, these evolutionary changes probably occurred to minimize deleterious effects of high HFA amounts and/or to enhance accumulation for physiological advantage. These results shed light on the evolution of pathways for novel fatty acid production in seeds, help explain some of the current limitations to accumulation of HFAs in transgenic plants, and may provide improved strategies for future engineering of their production. Significance Statement Comparison of protein sequences and transcript expression from developing seeds of Physaria fendleri that accumulate high amounts of hydroxy FAs, to Camelina sativa, a closely related plant that does not accumulate hydroxy FAs revealed multiple genes, many of which have not been previously considered, that likely co-evolved to enable hydroxy FA accumulation in Physaria. These genes provide new strategies to improve the ability of transgenic commodity crops to accumulate these and other value-added oils. C1 [Horn, Patrick J.; Liu, Jinjie; McGlew, Kathleen; Ohlrogge, John] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Liu, Jinjie; Thrower, Nicholas A.; Larson, Matt; Ohlrogge, John] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Cocuron, Jean-Christophe; Alonso, Ana P.] Ohio State Univ, Dept Mol Genet, Columbus, OH 43210 USA. [Lu, Chaofu] Montana State Univ, Dept Plant Sci & Plant Pathol, Bozeman, MT 59717 USA. RP Horn, PJ (reprint author), Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. EM hornp@msu.edu OI Lu, Chaofu/0000-0001-6901-7490 FU US National Science Foundation [DBI-0701919, DBI-1339385]; Department of Energy/Great Lakes Bioenergy Research Center [DE-FC02-07ER64494] FX We thank Phillip Bates (Department of Chemistry and Biochemistry, University of Southern Mississippi, Hattiesburg, MS) and Henrik Tjellstrom (Department of Plant Biology, Michigan State University) for helpful discussions and comments on the manuscript, and Curtis Wilkerson (Department of Biochemistry and Molecular Biology, Michigan State University) for advice on RNA-Seq analysis. This work was supported in part by the US National Science Foundation (grants DBI-0701919 and DBI-1339385) and by the Department of Energy/Great Lakes Bioenergy Research Center Cooperative Agreement (DE-FC02-07ER64494). NR 133 TC 2 Z9 2 U1 11 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0960-7412 EI 1365-313X J9 PLANT J JI Plant J. PD MAY PY 2016 VL 86 IS 4 BP 322 EP 348 DI 10.1111/tpj.13163 PG 27 WC Plant Sciences SC Plant Sciences GA DR0LG UT WOS:000379598400004 PM 26991237 ER PT J AU Leung, MCK Kapraun, DF Williams, AJ Knudsen, TB AF Leung, M. C. K. Kapraun, D. F. Williams, A. J. Knudsen, T. B. TI An Evaluation of ToxCast Angiogenic Disruptors for Effects on Mitochondrial Bioactivity Profiles SO BIRTH DEFECTS RESEARCH PART A-CLINICAL AND MOLECULAR TERATOLOGY LA English DT Meeting Abstract C1 [Leung, M. C. K.; Kapraun, D. F.; Williams, A. J.; Knudsen, T. B.] US EPA, Res Triangle Pk, NC 27711 USA. [Leung, M. C. K.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. NR 0 TC 0 Z9 0 U1 2 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1542-0752 EI 1542-0760 J9 BIRTH DEFECTS RES A JI Birth Defects Res. Part A-Clin. Mol. Teratol. PD MAY PY 2016 VL 106 IS 5 SI SI MA 10 BP 389 EP 389 PG 1 WC Developmental Biology; Toxicology SC Developmental Biology; Toxicology GA DQ2HT UT WOS:000379024100079 ER PT J AU Neal-Kluever, AP Aungst, J Wu, Y Liu, J Shackelford, M Ogungbesan, A Gu, Y Jacobs, K AF Neal-Kluever, A. P. Aungst, J. Wu, Y. Liu, J. Shackelford, M. Ogungbesan, A. Gu, Y. Jacobs, K. TI Regulatory Research to Support Food-Contact Infant Safety Assessment at US Food and Drug Administration SO BIRTH DEFECTS RESEARCH PART A-CLINICAL AND MOLECULAR TERATOLOGY LA English DT Meeting Abstract C1 [Neal-Kluever, A. P.; Aungst, J.; Wu, Y.; Shackelford, M.; Ogungbesan, A.; Gu, Y.; Jacobs, K.] US FDA, CFSAN, OFAS, DFCN, College Pk, MD USA. [Liu, J.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1542-0752 EI 1542-0760 J9 BIRTH DEFECTS RES A JI Birth Defects Res. Part A-Clin. Mol. Teratol. PD MAY PY 2016 VL 106 IS 5 SI SI MA P1 BP 404 EP 404 PG 1 WC Developmental Biology; Toxicology SC Developmental Biology; Toxicology GA DQ2HT UT WOS:000379024100105 ER PT J AU Narotsky, MG Manley, AL Ola, O AF Narotsky, M. G. Manley, A. L. Ola, O. TI Assessment of Iodoform Effects on Pregnancy Maintenance and Eye Malformations in a Developmental Toxicity Screen with F344 Rats SO BIRTH DEFECTS RESEARCH PART A-CLINICAL AND MOLECULAR TERATOLOGY LA English DT Meeting Abstract C1 [Narotsky, M. G.] US EPA, Res Triangle Pk, NC 27711 USA. [Manley, A. L.] ORISE, Oak Ridge, TN USA. [Ola, O.] Student Serv Contractor, Raleigh, NC USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1542-0752 EI 1542-0760 J9 BIRTH DEFECTS RES A JI Birth Defects Res. Part A-Clin. Mol. Teratol. PD MAY PY 2016 VL 106 IS 5 SI SI MA P31 BP 418 EP 418 PG 1 WC Developmental Biology; Toxicology SC Developmental Biology; Toxicology GA DQ2HT UT WOS:000379024100135 ER PT J AU Fernandez-de-Una, L McDowell, NG Canellas, I Gea-Izquierdo, G AF Fernandez-de-Una, Laura McDowell, Nate G. Canellas, Isabel Gea-Izquierdo, Guillermo TI Disentangling the effect of competition, CO2 and climate on intrinsic water-use efficiency and tree growth SO JOURNAL OF ECOLOGY LA English DT Article DE basal area increments; carbon isotopes; global change; Pinus sylvestris; plant-climate interactions; Quercus faginea; Quercus pyrenaica; tree rings ID CARBON-ISOTOPE DISCRIMINATION; PINUS-PONDEROSA TREES; SPRUCE PICEA-ABIES; GAS-EXCHANGE; MEDITERRANEAN REGION; RING DELTA-C-13; STABLE-ISOTOPES; ATMOSPHERIC CO2; FOREST TREES; SCOTS PINE AB 1. Climate change scenarios forecast rising temperatures for the Mediterranean region, which could enhance the vulnerability to drought stress in forest ecosystems. The long-term effects of climate forcing on tree performance can be, however, modulated by other environmental factors, such as competition and rising atmospheric CO2 concentrations. 2. We assessed the concomitant effect of competition, climate and CO2 concentrations on the treering delta C-13-derived intrinsic water-use efficiency (iWUE) and basal area increments (BAI) of species with different drought tolerance: two Mediterranean deciduous species (Quercus faginea Lam. and Quercus pyrenaica Willd.) and one conifer (Pinus sylvestris L.). Additionally, given that competition may be managed to mitigate the effect of increasing drought stress, we further examined the influence of this variable on iWUE and growth using data compiled from the literature, providing the first review on the response of iWUE to competition. 3. Competition had no significant effect on iWUE in any of the three species studied, whereas, as expected, growth rates were significantly higher under low-competition levels. This was consistent with the literature review, which showed that shifts in iWUE with competition changes are rare; supporting the hypothesis that leaf-level gas exchange tends to be a homeostatic trait. In the long term, the three species exhibited a significant increasing trend in iWUE due to the combined effect of increased CO2 concentration, climate and age. Growth, however, was mostly affected by competition and climate and in most cases was not enhanced as a result of the increase in iWUE. 4. Synthesis. Regardless of their functional response to drought, trees respond to reduced competition through the structural shifts such as increased radial growth rather than leaf-level gas exchange adjustments. CO2 and climate are, therefore, the main drivers of iWUE variability, rather than competition. Thus, if temperature-induced drought becomes limiting, reducing competition for resources may not offset the detrimental effect of increasing drought stress on tree physiology and growth decline may occur without a CO2 fertilization effect. C1 [Fernandez-de-Una, Laura; Canellas, Isabel; Gea-Izquierdo, Guillermo] IINIA CIFOR, Ctra La Coruna Km 7-5, Madrid 28040, Spain. [McDowell, Nate G.] Los Alamos Natl Lab, Div Earth & Environm Sci, MS J495, Los Alamos, NM 87545 USA. RP Fernandez-de-Una, L (reprint author), IINIA CIFOR, Ctra La Coruna Km 7-5, Madrid 28040, Spain. EM fernandez.laura@inia.es RI Ca�ellas, Isabel/B-7658-2008; OI Ca�ellas, Isabel/0000-0002-9716-7776; Fernandez de Una, Laura/0000-0001-8136-2545 FU Spanish Ministry of Economy and Competitiveness [AGL2013 46028R, AGL2010-21153-C02]; Madrid Regional Government [S2013/MAE-2760]; REGEN-FOR; EUFORINO; Department of Energy, Office of Science FX The authors would like to thank the funding from the Spanish Ministry of Economy and Competitiveness for the projects AGL2013 46028R and AGL2010-21153-C02 and the associated PhD scholarship for L.F.U., the Madrid Regional Government for the projects S2013/MAE-2760 and REGEN-FOR, as well as funding from EUFORINO and the Department of Energy, Office of Science, to N.G.M. The authors also thank AEMET and the University of Cantabria for the data provided for this work (Spain02 dataset, http:// www.meteo.unican.es/datasets/spain02), as well as the Penalara Natural Park Research and Management Centre for their climate data. Finally, we would like to thank A. Bachiller, E. Garriga, G. Perkins, Z. R Vance and E. Viscasillas for their field and laboratory assistance. NR 76 TC 3 Z9 3 U1 30 U2 42 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-0477 EI 1365-2745 J9 J ECOL JI J. Ecol. PD MAY PY 2016 VL 104 IS 3 BP 678 EP 690 DI 10.1111/1365-2745.12544 PG 13 WC Plant Sciences; Ecology SC Plant Sciences; Environmental Sciences & Ecology GA DQ2EO UT WOS:000379014900007 ER PT J AU Price, DN Kusewitt, DF Lino, CA McBride, AA Muttil, P AF Price, Dominique N. Kusewitt, Donna F. Lino, Christopher A. McBride, Amber A. Muttil, Pavan TI Oral Tolerance to Environmental Mycobacteria Interferes with Intradermal, but Not Pulmonary, Immunization against Tuberculosis SO PLOS PATHOGENS LA English DT Article ID BOVIS BCG VACCINATION; BACILLE CALMETTE-GUERIN; REGULATORY T-CELLS; IMMUNE-RESPONSES; NONTUBERCULOUS MYCOBACTERIA; ATYPICAL MYCOBACTERIA; PROTECTIVE IMMUNITY; GAMMA RESPONSE; MUCOSAL; INFECTION AB Bacille Calmette-Guerin (BCG) is currently the only approved vaccine against tuberculosis (TB) and is administered in over 150 countries worldwide. Despite its widespread use, the vaccine has a variable protective efficacy of 0-80%, with the lowest efficacy rates in tropical regions where TB is most prevalent. This variability is partially due to ubiquitous environmental mycobacteria (EM) found in soil and water sources, with high EM prevalence coinciding with areas of poor vaccine efficacy. In an effort to elucidate the mechanisms underlying EM interference with BCG vaccine efficacy, we exposed mice chronically to Mycobacterium avium(M. avium), a specific EM, by two different routes, the oral and intradermal route, to mimic human exposure. After intradermal BCG immunization in mice exposed to oral M. avium, we saw a significant decrease in the pro-inflammatory cytokine IFN-gamma, and an increase in T regulatory cells and the immunosuppressive cytokine IL-10 compared to naive BCG-vaccinated animals. To circumvent the immunosuppressive effect of oral M. avium exposure, we vaccinated mice by the pulmonary route with BCG. Inhaled BCG immunization rescued IFN-gamma levels and increased CD4 and CD8 T cell recruitment into airways in M. avium-presensitized mice. In contrast, intradermal BCG vaccination was ineffective at T cell recruitment into the airway. Pulmonary BCG vaccination proved protective against Mtb infection regardless of previous oral M. avium exposure, compared to intradermal BCG immunization. In conclusion, our data indicate that vaccination against TB by the pulmonary route increases BCG vaccine efficacy by avoiding the immunosuppressive interference generated by chronic oral exposure to EM. This has implications in TB-burdened countries where drug resistance is on the rise and health care options are limited due to economic considerations. A successful vaccine against TB is necessary in these areas as it is both effective and economical. C1 [Price, Dominique N.; McBride, Amber A.; Muttil, Pavan] Univ New Mexico, Coll Pharm, Dept Pharmaceut Sci, Albuquerque, NM 87131 USA. [Price, Dominique N.] Univ New Mexico, Biomed Sci Grad Program, Albuquerque, NM 87131 USA. Univ New Mexico, Dept Pathol, Albuquerque, NM 87131 USA. [Lino, Christopher A.] Univ New Mexico, Dept Mol Genet & Microbiol, Albuquerque, NM 87131 USA. [Lino, Christopher A.; McBride, Amber A.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Muttil, P (reprint author), Univ New Mexico, Coll Pharm, Dept Pharmaceut Sci, Albuquerque, NM 87131 USA. EM pmuttil@salud.unm.edu FU Discovery Program of the Bill & Melinda Gates Foundation [OPP1061393]; National Institute of Allergy and Infectious Diseases [A1007538] FX This study was funded by the Discovery Program of the Bill & Melinda Gates Foundation (Grand Challenges Explorations Grant Number: OPP1061393) and National Institute of Allergy and Infectious Diseases (T32 Training grant No: A1007538; P.I. - Dr. Michelle Ozbun). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 51 TC 2 Z9 2 U1 4 U2 5 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7366 EI 1553-7374 J9 PLOS PATHOG JI PLoS Pathog. PD MAY PY 2016 VL 12 IS 5 AR e1005614 DI 10.1371/journal.ppat.1005614 PG 21 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA DQ6VV UT WOS:000379344500022 PM 27153120 ER PT J AU Cao, HN Tan, KM Wang, FB Bigelow, L Yennamalli, RM Jedrzejczak, R Babnigg, G Bingman, CA Joachimiak, A Kharel, MK Singh, S Thorson, JS Phillips, GN AF Cao, Hongnan Tan, Kemin Wang, Fengbin Bigelow, Lance Yennamalli, Ragothaman M. Jedrzejczak, Robert Babnigg, Gyorgy Bingman, Craig A. Joachimiak, Andrzej Kharel, Madan K. Singh, Shanteri Thorson, Jon S. Phillips, George N., Jr. TI Structural dynamics of a methionine gamma-lyase for calicheamicin biosynthesis: Rotation of the conserved tyrosine stacking with pyridoxal phosphate SO STRUCTURAL DYNAMICS LA English DT Article ID POLYKETIDE SYNTHASE CALE8; DOUBLE-STRANDED DNA; CITROBACTER-FREUNDII; CRYSTALLINE STATE; WEB SERVER; PROTEIN; BIOLOGY; CRYSTALLOGRAPHY; SPECIFICITY; VALIDATION AB CalE6 from Micromonospora echinospora is a (pyridoxal 5' phosphate) PLP-dependent methionine gamma-lyase involved in the biosynthesis of calicheamicins. We report the crystal structure of a CalE6 2-(N-morpholino)ethanesulfonic acid complex showing ligand-induced rotation of Tyr100, which stacks with PLP, resembling the corresponding tyrosine rotation of true catalytic intermediates of CalE6 homologs. Elastic network modeling and crystallographic ensemble refinement reveal mobility of the N-terminal loop, which involves both tetrameric assembly and PLP binding. Modeling and comparative structural analysis of PLP-dependent enzymes involved in Cys/Met metabolism shine light on the functional implications of the intrinsic dynamic properties of CalE6 in catalysis and holoenzyme maturation. (C) 2016 Author(s). C1 [Cao, Hongnan; Wang, Fengbin; Yennamalli, Ragothaman M.; Phillips, George N., Jr.] Rice Univ, Biosci Rice, 6100 Main St, Houston, TX 77005 USA. [Tan, Kemin; Bigelow, Lance; Jedrzejczak, Robert; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Midwest Ctr Struct Genom, Bldg 446 Rm A104,970 South Cass Ave, Argonne, IL 60439 USA. [Bingman, Craig A.] Univ Wisconsin, Dept Biochem, Madison, WI 53706 USA. [Kharel, Madan K.; Singh, Shanteri; Thorson, Jon S.] Univ Kentucky, Coll Pharm, Dept Pharmaceut Sci, Lexington, KY 40536 USA. [Yennamalli, Ragothaman M.] Jaypee Univ Informat Technol, Dept Biotechnol & Bioinformat, Waknaghat 173234, Himachal Prades, India. [Singh, Shanteri] Univ Oklahoma, Dept Chem & Biochem, Norman, OK 73019 USA. RP Phillips, GN (reprint author), Rice Univ, Biosci Rice, 6100 Main St, Houston, TX 77005 USA. EM georgep@rice.edu RI Thorson, Jon/L-3696-2013 OI Thorson, Jon/0000-0002-7148-0721 FU National Institutes of Health [CA84374, U01GM098248, GM094585]; National Center for Advancing Translational Sciences [UL1TR000117]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX This work was supported by the National Institutes of Health Grant Nos. CA84374 (J.S.T.), U01GM098248 (G.N.P.), and GM094585 (A.J.) and the National Center for Advancing Translational Sciences (UL1TR000117). Results shown in this report are derived from work performed at 19-ID beamline of Argonne National Laboratory, Structural Biology Center at the Advanced Photon Source. Argonne is operated by UChicago Argonne, LLC, for the U.S. Department of Energy, Office of Biological and Environmental Research under Contract No. DE-AC02-06CH11357. NR 60 TC 0 Z9 0 U1 5 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD MAY PY 2016 VL 3 IS 3 AR 034702 DI 10.1063/1.4948539 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ4MJ UT WOS:000379177700008 PM 27191010 ER PT J AU Szoke, A Hajdu, J AF Szoke, Abraham Hajdu, Janos TI Energy utilization in fluctuating biological energy converters SO STRUCTURAL DYNAMICS LA English DT Article ID BACTERIAL FLAGELLAR MOTOR; HAND-OVER-HAND; PURPLE BACTERIA; KINESIN; MOLECULES; MECHANISM; RESOLUTION; EVOLUTION; MEMBRANES; SYNTHASE AB We have argued previously [Szoke et al., FEBS Lett. 553, 18-20 (2003); Curr. Chem. Biol. 1, 53-57 (2007)] that energy utilization and evolution are emergent properties based on a small number of established laws of physics and chemistry. The relevant laws constitute a framework for biology on a level intermediate between quantum chemistry and cell biology. There are legitimate questions whether these concepts are valid at the mesoscopic level. Such systems fluctuate appreciably, so it is not clear what their efficiency is. Advances in fluctuation theorems allow the description of such systems on a molecular level. We attempt to clarify this topic and bridge the biochemical and physical descriptions of mesoscopic systems. (C) 2016 Author(s). C1 [Szoke, Abraham] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Hajdu, Janos] Uppsala Univ, Dept Cell & Mol Biol, Box 596, S-75124 Uppsala, Sweden. RP Szoke, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. FU U. S. Department of Energy by the University of California, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Swedish Research Council STINT; Swedish Research Council SSF; Swedish Research Council VR; European Research Council FX This work was supported by the U. S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. It was also supported by the Swedish Research Councils STINT, SSF, VR, and the European Research Council. NR 58 TC 0 Z9 0 U1 3 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD MAY PY 2016 VL 3 IS 3 AR 034701 DI 10.1063/1.4945792 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ4MJ UT WOS:000379177700007 PM 27191009 ER EF