FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Hodge, CD Ismail, IH Edwards, RA Hura, GL Xiao, AT Tainer, JA Hendzel, MJ Glover, JNM AF Hodge, Curtis D. Ismail, Ismail H. Edwards, Ross A. Hura, Greg L. Xiao, Andrew T. Tainer, John A. Hendzel, Michael J. Glover, J. N. Mark TI RNF8 E3 Ubiquitin Ligase Stimulates Ubc13 E2 Conjugating Activity That Is Essential for DNA Double Strand Break Signaling and BRCA1 Tumor Suppressor Recruitment SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID X-RAY-SCATTERING; DAMAGE RESPONSE; CRYSTAL-STRUCTURE; STRUCTURAL BASIS; BINDING DOMAINS; REPAIR PROTEINS; COMPLEX; MDC1; SAXS; UBIQUITYLATION AB DNA double strand break (DSB) responses depend on the sequential actions of the E3 ubiquitin ligases RNF8 and RNF168 plus E2 ubiquitin-conjugating enzyme Ubc13 to specifically generate histone Lys-63-linked ubiquitin chains in DSB signaling. Here, we defined the activated RNF8-Ubc13 similar to ubiquitin complex by x-ray crystallography and its functional solution conformations by x-ray scattering, as tested by separation-offunction mutations imaged in cells by immunofluorescence. The collective results show that the RING E3 RNF8 targets E2 Ubc13 to DSB sites and plays a critical role in damage signaling by stimulating polyubiquitination through modulating conformations of ubiquitin covalently linked to the Ubc13 active site. Structure-guided separation-of-function mutations show that the RNF8 E2 stimulating activity is essential for DSB signaling in mammalian cells and is necessary for down stream recruitment of 53BP1 and BRCA1. Chromatin-targeted RNF168 rescues 53BP1 recruitment involved in non-homologous end joining but not BRCA1 recruitment for homologous recombination. These findings suggest an allosteric approach to targeting the ubiquitin-docking cleft at the E2-E3 interface for possible interventions in cancer and chronic inflammation, and moreover, they establish an independent RNF8 role in BRCA1 recruitment. C1 [Hodge, Curtis D.; Edwards, Ross A.; Xiao, Andrew T.; Glover, J. N. Mark] Univ Alberta, Dept Biochem, Edmonton, AB T6G 2H7, Canada. [Ismail, Ismail H.; Hendzel, Michael J.] Univ Alberta, Dept Oncol, Edmonton, AB T6G 1Z2, Canada. [Hura, Greg L.; Tainer, John A.] Lawrence Berkeley Natl Lab, Berkeley, CA 94704 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, Houston, TX 77030 USA. [Ismail, Ismail H.] Cairo Univ, Fac Sci, Dept Biophys, Giza 12613, Egypt. RP Glover, JNM (reprint author), Univ Alberta, Fac Med & Dent, Dept Biochem, Edmonton, AB T6G 2H7, Canada. EM mark.glover@ualberta.ca OI Ismail, Ismail Hassan/0000-0002-5526-6063; Hodge, Curtis/0000-0002-7528-4058 FU Integrated Diffraction Analysis Technologies Program (Department of Energy/Biological and Environmental Research); National Institutes of Health MINOS Grant [GM105404] FX We thank S. Classen at the Advanced Light Source (SIBYLS) for crystallographic data collections and support. We also thank the Cellular Imaging Facility at the Cross Cancer Institute for the use of microscopes. We thank X. Yu, Division of Molecular Medicine and Genetics, University of Michigan Medical School, Ann Arbor, MI, for the gift of the RNF8 knock-out MEFs. SAXS data collection and analysis at SIBYLS BL12.3.1 at the Advanced Light Source were supported by the Integrated Diffraction Analysis Technologies Program (Department of Energy/Biological and Environmental Research) and by National Institutes of Health MINOS Grant GM105404. NR 64 TC 1 Z9 1 U1 5 U2 8 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD APR 29 PY 2016 VL 291 IS 18 BP 9396 EP 9410 DI 10.1074/jbc.M116.715698 PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DL4JY UT WOS:000375602300002 PM 26903517 ER PT J AU Marlow, JJ Skennerton, CT Li, Z Chourey, K Hettich, RL Pan, C Orphan, VJ AF Marlow, Jeffrey J. Skennerton, Connor T. Li, Zhou Chourey, Karuna Hettich, Robert L. Pan, Chongle Orphan, Victoria J. TI Proteomic Stable Isotope Probing Reveals Biosynthesis Dynamics of Slow Growing Methane Based Microbial Communities SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE proteomics; stable isotope probing; methane seeps; anaerobic oxidation of methane; environmental microbiology ID SULFATE-REDUCING BACTERIA; COENZYME-M REDUCTASE; MEDIATING ANAEROBIC OXIDATION; MULTIPLE SEQUENCE ALIGNMENT; CASCADIA CONVERGENT MARGIN; COLD SEEP SEDIMENTS; METHANOTROPHIC ARCHAEA; MASS-SPECTROMETRY; MEMBRANE-PROTEINS; MARINE-SEDIMENTS AB Marine methane seep habitats represent an important control on the global flux of methane. Nucleotide-based meta-omics studies outline community-wide metabolic potential, but expression patterns of environmentally relevant proteins are poorly characterized. Proteomic stable isotope probing (proteomic SIP) provides additional information by characterizing phylogenetically specific, functionally relevant activity in mixed microbial communities, offering enhanced detection through system-wide product integration. Here we applied proteomic SIP to (NH4+)-N-15 and CH4 amended seep sediment microcosms in an attempt to track protein synthesis of slow-growing, low-energy microbial systems. Across all samples, 3495 unique proteins were identified, 11% of which were N-15-labeled. Consistent with the dominant anaerobic oxidation of methane (AOM) activity commonly observed in anoxic seep sediments, proteins associated with sulfate reduction and reverse methanogenesis-including the ANME-2 associated methylenetetrahydromethanopterin reductase (Mer) were all observed to be actively synthesized (N-15-enriched). Conversely, proteins affiliated with putative aerobic sulfur-oxidizing epsilon- and gammaproteobacteria showed a marked decrease over time in our anoxic sediment incubations. The abundance and phylogenetic range of N-15-enriched methyl-coenzyme M reductase (Mcr) orthologs, many of which exhibited novel post-translational modifications, suggests that seep sediments provide niches for multiple organisms performing analogous metabolisms. In addition, 26 proteins of unknown function were consistently detected and actively expressed under conditions supporting AOM, suggesting that they play important roles in methane seep ecosystems. Stable isotope probing in environmental proteomics experiments provides a mechanism to determine protein durability and evaluate lineage-specific responses in complex microbial communities placed under environmentally relevant conditions. Our work here demonstrates the active synthesis of a metabolically specific minority of enzymes, revealing the surprising longevity of most proteins over the course of an extended incubation experiment in an established, slow-growing, methane-impacted environmental system. C1 [Marlow, Jeffrey J.; Skennerton, Connor T.; Orphan, Victoria J.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Li, Zhou; Chourey, Karuna; Hettich, Robert L.; Pan, Chongle] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. RP Marlow, JJ; Orphan, VJ (reprint author), CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. EM marlow@fas.harvard.edu; vorphan@gps.caltech.edu RI Hettich, Robert/N-1458-2016; Li, Zhou/L-7976-2015; OI Hettich, Robert/0000-0001-7708-786X; , /0000-0002-9216-3813; Orphan, Victoria/0000-0002-5374-6178; Skennerton, Connor/0000-0003-1320-4873 FU US Department of Energy, Office of Science, Office of Biological Environmental Research [DE-SC0004949, DE-SC0010574]; Life Underground NASA Astrobiology Institute [NNA13AA92A]; National Energy Technology Laboratory Methane Hydrate Research Fellowship - National Research Council of the National Academies FX This work was supported by the US Department of Energy, Office of Science, Office of Biological Environmental Research, under award numbers DE-SC0004949 and DE-SC0010574, and the Life Underground NASA Astrobiology Institute (NNA13AA92A) (to VO). JM was supported by a National Energy Technology Laboratory Methane Hydrate Research Fellowship funded by the National Research Council of the National Academies. The funders had no role in study design, data collection and interpretation, or the manuscript preparation and submission process. NR 123 TC 1 Z9 1 U1 14 U2 33 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 29 PY 2016 VL 7 AR 563 DI 10.3389/fmicb.2016.00563 PG 21 WC Microbiology SC Microbiology GA DL1IW UT WOS:000375386800001 PM 27199908 ER PT J AU Curtis, JA Tokumoto, T Hatke, AT Cherian, JG Reno, JL McGill, SA Karaiskaj, D Hilton, DJ AF Curtis, Jeremy A. Tokumoto, Takahisa Hatke, A. T. Cherian, Judy G. Reno, John L. McGill, Stephen A. Karaiskaj, Denis Hilton, David J. TI Cyclotron decay time of a two-dimensional electron gas from 0.4 to 100 K SO PHYSICAL REVIEW B LA English DT Article ID HIGH-MOBILITY; DOMAIN SPECTROSCOPY; RESONANCE LINEWIDTH; GAAS-ALXGA1-XAS HETEROSTRUCTURES; TERAHERTZ SPECTROSCOPY; MATERIAL PARAMETERS; PHONON-SCATTERING; CARRIER DENSITY; HETEROJUNCTIONS; QUANTUM AB We have studied the cyclotron decay time of a Landau-quantized two-dimensional electron gas as a function of temperature (0.4-100 K) at a fixed magnetic field (+/- 1.25 T) using terahertz time-domain spectroscopy in a gallium arsenide quantum well with a mobility of mu(dc) = 3.6 x 10(6) cm(2) V-1 s(-1) and a carrier concentration of n(s) = 2 x 10(11) cm(-2). We find a cyclotron decay time that is limited by superradiant decay of the cyclotron ensemble and a temperature dependence that may result from both dissipative processes as well as a decrease in n(s) below 1.5K. Shubnikov-de Haas characterization determines a quantum lifetime, tau(q) = 1.1 ps, which is significantly faster than the corresponding dephasing time, tau(s) = 66.4 ps, in our cyclotron data. This is consistent with small-angle scattering as the dominant contribution in this sample, where scattering angles below theta <= 13 degrees. do not efficiently contribute to dephasing. Above 50 K, the cyclotron oscillations show a strong reduction in both the oscillation amplitude and lifetime that result from polar optical phonon scattering. C1 [Curtis, Jeremy A.; Tokumoto, Takahisa; Hilton, David J.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Hatke, A. T.; Cherian, Judy G.; McGill, Stephen A.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 30301 USA. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Karaiskaj, Denis] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. RP Hilton, DJ (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. EM dhilton@uab.edu FU National Science Foundation [DMR-1056827, DMR-1409473, DMR-1157490]; U.S. Department of Education GAANN Fellowship [P200A090143]; state of Florida; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported by the National Science Foundation under Grants No. DMR-1056827 (J.A.C., T.T., and D.J.H.) and No. DMR-1409473 (D.K.). J.A.C. also acknowledges support from the U.S. Department of Education GAANN Fellowship (P200A090143). A.T.H. acknowledges L.W. Engel for support and use of equipment for the SdHO measurements. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490 and the state of Florida. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences, user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 51 TC 2 Z9 2 U1 4 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 29 PY 2016 VL 93 IS 15 AR 155437 DI 10.1103/PhysRevB.93.155437 PG 8 WC Physics, Condensed Matter SC Physics GA DK8UA UT WOS:000375202600004 ER PT J AU Kung, YF Chen, CC Wang, Y Huang, EW Nowadnick, EA Moritz, B Scalettar, RT Johnston, S Devereaux, TP AF Kung, Y. F. Chen, C-C. Wang, Yao Huang, E. W. Nowadnick, E. A. Moritz, B. Scalettar, R. T. Johnston, S. Devereaux, T. P. TI Characterizing the three-orbital Hubbard model with determinant quantum Monte Carlo SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; HIGH-TC SUPERCONDUCTORS; COPPER-OXIDE SUPERCONDUCTORS; MATRIX RENORMALIZATION-GROUP; CHARGE-TRANSFER; ELECTRONIC-STRUCTURE; FERMION SYSTEMS; PRODUCT STATES; CUO2 PLANE; LA2CUO4 AB We characterize the three-orbital Hubbard model using state-of-the-art determinant quantum Monte Carlo (DQMC) simulations with parameters relevant to the cuprate high-temperature superconductors. The simulations find that doped holes preferentially reside on oxygen orbitals and that the (pi, pi) antiferromagnetic ordering vector dominates in the vicinity of the undoped system, as known from experiments. The orbitally-resolved spectral functions agree well with photoemission spectroscopy studies and enable identification of orbital content in the bands. A comparison of DQMC results with exact diagonalization and cluster perturbation theory studies elucidates how these different numerical techniques complement one another to produce a more complete understanding of the model and the cuprates. Interestingly, our DQMC simulations predict a charge-transfer gap that is significantly smaller than the direct (optical) gap measured in experiment. Most likely, it corresponds to the indirect gap that has recently been suggested to be on the order of 0.8 eV, and demonstrates the subtlety in identifying charge gaps. C1 [Kung, Y. F.; Huang, E. W.; Nowadnick, E. A.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Kung, Y. F.; Wang, Yao; Huang, E. W.; Nowadnick, E. A.; Moritz, B.; Devereaux, T. P.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Stanford, CA 94305 USA. [Kung, Y. F.; Wang, Yao; Huang, E. W.; Nowadnick, E. A.; Moritz, B.; Devereaux, T. P.] Stanford Univ, Stanford, CA 94305 USA. [Chen, C-C.] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. [Chen, C-C.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Wang, Yao] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Nowadnick, E. A.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Moritz, B.] Univ N Dakota, Dept Phys & Astrophys, Grand Forks, ND 58202 USA. [Scalettar, R. T.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Johnston, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Devereaux, T. P.] Stanford Univ, Geballe Lab Adv Mat, Stanford, CA 94305 USA. RP Kung, YF (reprint author), Stanford Univ, Dept Phys, Stanford, CA 94305 USA. RI Moritz, Brian/D-7505-2015; Johnston, Steven/J-7777-2016 OI Moritz, Brian/0000-0002-3747-8484; FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under SLAC National Accelerator Laboratory (SLAC), Stanford Institute for Materials and Energy Sciences [DE-AC02-76SF00515]; Department of Defense (DOD) through the National Defense Science and Engineering Graduate Fellowship (NDSEG) Program; National Science Foundation (NSF) [1147470]; Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory (ANL); US Department of Energy (DOE) [DE-AC02-06CH11357]; DOE [Er-046169]; University of Tennessee Science Alliance JDRD program; Oak Ridge National Laboratory; Stewardship Science Academic Alliances (SSAA) program of the National Nuclear Security Administration (NNSA); U.S. DOE [DE-AC02-05CH11231] FX This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-76SF00515, SLAC National Accelerator Laboratory (SLAC), Stanford Institute for Materials and Energy Sciences. Y.F.K. was supported by the Department of Defense (DOD) through the National Defense Science and Engineering Graduate Fellowship (NDSEG) Program and by the National Science Foundation (NSF) Graduate Research Fellowship under Grant No. 1147470. C.C.C. is supported by the Aneesur Rahman Postdoctoral Fellowship at Argonne National Laboratory (ANL), operated by the US Department of Energy (DOE) Contract No. DE-AC02-06CH11357. Y.W. was supported by the Stanford Graduate Fellows in Science and Engineering. E.A.N. also acknowledges support from DOE Er-046169. S.J. is funded by the University of Tennessee Science Alliance JDRD program; a collaboration with Oak Ridge National Laboratory. R.T.S. was supported by the Stewardship Science Academic Alliances (SSAA) program of the National Nuclear Security Administration (NNSA). The computational work was partially performed at the National Energy Research Scientific Computing Center (NERSC), supported by the U.S. DOE under Contract No. DE-AC02-05CH11231. NR 72 TC 2 Z9 2 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 29 PY 2016 VL 93 IS 15 AR 155166 DI 10.1103/PhysRevB.93.155166 PG 14 WC Physics, Condensed Matter SC Physics GA DK8UA UT WOS:000375202600001 ER PT J AU Zapf, VS Ueland, BG Laver, M Lonsky, M Pohlit, M Muller, J Lancaster, T Moller, JS Blundell, SJ Singleton, J Mira, J Yanez-Vilar, S Senaris-Rodriguez, MA AF Zapf, Vivien S. Ueland, B. G. Laver, Mark Lonsky, Martin Pohlit, Merlin Mueller, Jens Lancaster, Tom Moeller, Johannes S. Blundell, Stephen J. Singleton, John Mira, Jorge Yanez-Vilar, Susana Antonia Senaris-Rodriguez, Maria TI Magnetization dynamics and frustration in the multiferroic double perovskite Lu2MnCoO6 SO PHYSICAL REVIEW B LA English DT Article AB We investigate the magnetic ordering and the magnetization dynamics (from kHz to THz time scales) of the double perovskite Lu2MnCoO6 using elastic neutron diffraction, muon spin relaxation, and micro-Hall magnetization measurements. This compound is known to be a type II multiferroic with the interesting feature that a ferromagneticlike magnetization hysteresis loop couples to an equally hysteretic electric polarization in the bulk of the material despite a zero-field magnetic ordering of the type up arrow up arrow down arrow down arrow along Co-Mn spin chains. Here we explore the unusual dynamics of this compound and find extremely strong fluctuations, consistent with the axial next-nearest-neighbor Ising (ANNNI) model for frustrated spin chains. We identify three temperature scales in Lu2MnCoO6 corresponding to the onset of highly fluctuating long-range order below T-N = 50 +/- 3 K identified from neutron scattering, the onset of magnetic and electric hysteresis, with change in kHz magnetic and electric dynamics below a 30 K temperature scale, and partial freezing of similar to MHz spin fluctuations in the muon spin relaxation data below 12 +/- 3 K. Our results provide a framework for understanding the multiferroic behavior of this compound and its hysteresis and dynamics. C1 [Zapf, Vivien S.; Singleton, John] Los Alamos Natl Lab, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. [Ueland, B. G.] Iowa State Univ, US DOE, Ames Lab, Ames, IA USA. [Ueland, B. G.] Iowa State Univ, Dept Phys, Ames, IA USA. [Laver, Mark] Univ Birmingham, Sch Met & Mat, Edgbaston B15 2TT, W Midlands, England. [Lonsky, Martin; Pohlit, Merlin; Mueller, Jens] Goethe Univ Frankfurt, Inst Phys, D-60438 Frankfurt M, Germany. [Lancaster, Tom] Univ Durham, Dept Phys, South Rd, Durham DH1 3LE, England. [Moeller, Johannes S.; Blundell, Stephen J.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Mira, Jorge] Univ Santiago de Compostela, Dept Fis Aplicada, E-15782 Santiago De Compostela, Spain. [Yanez-Vilar, Susana; Antonia Senaris-Rodriguez, Maria] Dept Quim Fundamental U Coruna, La Coruna 15071, Spain. [Moeller, Johannes S.] ETH, Solid State Phys Lab, CH-8093 Zurich, Switzerland. RP Zapf, VS (reprint author), Los Alamos Natl Lab, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. RI Senaris-Rodriguez, M./L-1400-2014; Ueland, Benjamin/B-2312-2008; Mira, Jorge/F-9077-2016; OI Senaris-Rodriguez, M./0000-0002-0117-6855; Ueland, Benjamin/0000-0001-9784-6595; Mira, Jorge/0000-0002-6024-6294; Yanez, Susana/0000-0002-0314-8567 FU Laboratory-Directed Research and Development program (LDRD); U.S. National Science Foundation [DMR-1157490]; State of Florida; U.S. Department of Energy; EPSRC (UK); Ministerio de Economa y Competitividad (MINECO) (Spain); EU [FEDER MAT2010-21342-C02]; Department of Energy, Basic Energy Sciences, Division of Materials Sciences Engineering [DE-AC02-07CH11358] FX Work at LANL was supported by the Laboratory-Directed Research and Development program (LDRD). The NHMFL Pulsed-Field Facility is funded by the U.S. National Science Foundation through Cooperative Grant No. DMR-1157490, the State of Florida, and the U.S. Department of Energy. mu SR measurements were carried out at S mu S, Paul Scherrer Institut, Switzerland and we are grateful to Alex Amato for technical assistance. That work is supported by EPSRC (UK). The Spanish authors are grateful for financial support from Ministerio de Economa y Competitividad (MINECO) (Spain) and EU under projects FEDER MAT2010-21342-C02. Work at the Ames Laboratory was supported by the Department of Energy, Basic Energy Sciences, Division of Materials Sciences & Engineering, under Contract No. DE-AC02-07CH11358. NR 24 TC 3 Z9 3 U1 12 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 29 PY 2016 VL 93 IS 13 AR 134431 DI 10.1103/PhysRevB.93.134431 PG 7 WC Physics, Condensed Matter SC Physics GA DK8TI UT WOS:000375200800003 ER PT J AU Gori, S Kim, IW Shah, NR Zurek, KM AF Gori, Stefania Kim, Ian-Woo Shah, Nausheen R. Zurek, Kathryn M. TI Closing the wedge: Search strategies for extended Higgs sectors with heavy flavor final states SO PHYSICAL REVIEW D LA English DT Article ID LHC; COLLISIONS; BOSONS; QUARKS; MODEL; TEV AB We consider search strategies for an extended Higgs sector at the high-luminosity LHC14 utilizing multitop final states. In the framework of a two Higgs doublet model, the purely top final states (t (t) over bar, 4t) are important channels for heavy Higgs bosons with masses in the wedge above 2m(t) and at low values of tan beta, while a 2b2t final state is most relevant at moderate values of tan beta. We find, in the t (t) over barH channel, with H -> t (t) over bar, that both single and three lepton final states can provide statistically significant constraints at low values of tan beta for m(A) as high as similar to 750 GeV. When systematics on the t (t) over bar background are taken into account, however, the three lepton final state is more powerful, though the precise constraint depends fairly sensitively on lepton fake rates. We also find that neither 2b2t nor t (t) over bar final states provide constraints on additional heavy Higgs bosons with couplings to tops smaller than the top Yukawa due to expected systematic uncertainties in the t (t) over bar background. C1 [Gori, Stefania] Perimeter Inst Theoret Phys, 31 Caroline St North, Waterloo, ON N2L 2Y5, Canada. [Gori, Stefania] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Kim, Ian-Woo] CERN TH PH Div, CH-1211 Meyrin, Switzerland. [Kim, Ian-Woo] UpHere, San Francisco, CA 94122 USA. [Shah, Nausheen R.] Wayne State Univ, Dept Phys & Astron, Detroit, MI 48201 USA. [Zurek, Kathryn M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Zurek, Kathryn M.] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. RP Gori, S (reprint author), Perimeter Inst Theoret Phys, 31 Caroline St North, Waterloo, ON N2L 2Y5, Canada.; Gori, S (reprint author), Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. FU National Science Foundation [PHYS-1066293]; [DE-AC02-05CH11231] FX We thank Marco Farina, Yuri Gershtein, Moira Gresham, Ben Hooberman, Fabio Maltoni, Michele Papucci, Brian Shuve and Carlos Wagner for the useful conversations. K. Z. is supported by Contract No. DE-AC02-05CH11231. N. R. S. acknowledges the hospitality of the Aspen Center for Physics, which is supported by the National Science Foundation under Grant No. PHYS-1066293. NR 60 TC 13 Z9 13 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 29 PY 2016 VL 93 IS 7 AR 075038 DI 10.1103/PhysRevD.93.075038 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK8VD UT WOS:000375205500003 ER PT J AU Shahar, A Schauble, EA Caracas, R Gleason, AE Reagan, MM Xiao, Y Shu, J Mao, W AF Shahar, A. Schauble, E. A. Caracas, R. Gleason, A. E. Reagan, M. M. Xiao, Y. Shu, J. Mao, W. TI Pressure-dependent isotopic composition of iron alloys SO SCIENCE LA English DT Article ID FRACTIONATION FACTORS; LATTICE-PARAMETER; EARTHS CORE; HYDROGEN; MANTLE; CALIBRATION; ACCRETION; MINERALS; CARBON; WATER AB Our current understanding of Earth's core formation is limited by the fact that this profound event is far removed from us physically and temporally. The composition of the iron metal in the core was a result of the conditions of its formation, which has important implications for our planet's geochemical evolution and physical history. We present experimental and theoretical evidence for the effect of pressure on iron isotopic composition, which we found to vary according to the alloy tested (FeO, FeHx, or Fe3C versus pure Fe). These results suggest that hydrogen or carbon is not the major light-element component in the core. The pressure dependence of iron isotopic composition provides an independent constraint on Earth's core composition. C1 [Shahar, A.; Shu, J.] Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. [Schauble, E. A.] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA 90095 USA. [Caracas, R.] Univ Lyon 1, CNRS, Ecole Normale Super Lyon, Lab Geol Lyon,UMR 5276, F-69364 Lyon 07, France. [Gleason, A. E.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Reagan, M. M.; Mao, W.] Stanford Univ, Dept Geol Sci, Stanford, CA 94305 USA. [Xiao, Y.] Carnegie Inst Sci, HPCAT, Argonne, IL USA. RP Shahar, A (reprint author), Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. EM ashahar@carnegiescience.edu RI Schauble, Edwin/E-7812-2012 FU Stanford University Blaustein Fellowship; NSF [EAR1321858, EAR1464008, EAR1530306]; CNRS PICS grant [x2015106368] FX Supported by a Stanford University Blaustein Fellowship during which this project developed, and NSF grant EAR1321858 (A.S.); NSF grant EAR1464008 (A.S. and W.M.); NSF grant EAR1530306 (E.A.S.), and CNRS PICS grant Carmelts and eDARI/CINES grant x2015106368 for computational resources (R.C.). The complete data tables for this study can be found on www.gl.ciw.edu/static/users/ashahar/shahar_nrixs/. We thank four anonymous reviewers for providing very helpful comments and suggestions. NR 31 TC 9 Z9 9 U1 10 U2 27 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD APR 29 PY 2016 VL 352 IS 6285 BP 580 EP 582 DI 10.1126/science.aad9945 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK5ZA UT WOS:000374998600043 PM 27126042 ER PT J AU Jiang, Z Li, P Van Nostrand, JD Zhang, P Zhou, JZ Wang, YH Dai, XY Zhang, R Jiang, DW Wang, YX AF Jiang, Zhou Li, Ping Van Nostrand, Joy D. Zhang, Ping Zhou, Jizhong Wang, Yanhong Dai, Xinyue Zhang, Rui Jiang, Dawei Wang, Yanxin TI Microbial communities and arsenic biogeochemistry at the outflow of an alkaline sulfide-rich hot spring SO SCIENTIFIC REPORTS LA English DT Article ID YELLOWSTONE-NATIONAL-PARK; YUNNAN PROVINCE; GEN. NOV.; HYPERTHERMOPHILIC ARCHAEUM; CHEMOLITHOTROPHIC GROWTH; GEOTHERMAL WATERS; OXIDASE GENES; CHINA; TENGCHONG; BACTERIUM AB Alkaline sulfide-rich hot springs provide a unique environment for microbial community and arsenic (As) biogeochemistry. In this study, a representative alkaline sulfide-rich hot spring, Zimeiquan in the Tengchong geothermal area, was chosen to study arsenic geochemistry and microbial community using Illumina MiSeq sequencing. Over 0.26 million 16S rRNA sequence reads were obtained from 5-paired parallel water and sediment samples along the hot spring's outflow channel. High ratios of As(V)/As-Sum (total combined arsenate and arsenite concentrations) (0.59-0.78), coupled with high sulfide (up to 5.87 mg/L), were present in the hot spring's pools, which suggested As(III) oxidation occurred. Along the outflow channel, As-Sum increased from 5.45 to 13.86 mu mol/L, and the combined sulfide and sulfate concentrations increased from 292.02 to 364.28 mu mol/L. These increases were primarily attributed to thioarsenic transformation. Temperature, sulfide, As and dissolved oxygen significantly shaped the microbial communities between not only the pools and downstream samples, but also water and sediment samples. Results implied that the upstream Thermocrinis was responsible for the transformation of thioarsenic to As(III) and the downstream Thermus contributed to derived As(III) oxidation. This study improves our understanding of microbially-mediated As transformation in alkaline sulfide-rich hot springs. C1 [Jiang, Zhou; Li, Ping; Wang, Yanhong; Dai, Xinyue; Zhang, Rui; Jiang, Dawei; Wang, Yanxin] China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China. [Jiang, Zhou; Dai, Xinyue; Wang, Yanxin] China Univ Geosci, Sch Environm Studies, Wuhan 430074, Peoples R China. [Van Nostrand, Joy D.; Zhang, Ping; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Van Nostrand, Joy D.; Zhang, Ping; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China. RP Li, P; Wang, YX (reprint author), China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China.; Wang, YX (reprint author), China Univ Geosci, Sch Environm Studies, Wuhan 430074, Peoples R China. EM pli@cug.edu.cn; yx.wang@cug.edu.cn FU National Natural Science Foundation of China [41120124003, 41521001, 41372348]; Fundamental Research Funds for the Central Universities [CUG140505]; State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences [GBL11505] FX This research was financially supported by National Natural Science Foundation of China (Grant No. 41120124003, 41521001, 41372348), the Fundamental Research Funds for the Central Universities (No. CUG140505) and State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences (No. GBL11505). NR 52 TC 0 Z9 0 U1 12 U2 24 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 29 PY 2016 VL 6 AR 25262 DI 10.1038/srep25262 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK8NW UT WOS:000375184600001 PM 27126380 ER PT J AU Isaac, RS Jiang, FG Doudna, JA Lim, WA Narlikar, GJ Almeida, R AF Isaac, R. Stefan Jiang, Fuguo Doudna, Jennifer A. Lim, Wendell A. Narlikar, Geeta J. Almeida, Ricardo TI Nucleosome breathing and remodeling constrain CRISPR-Cas9 function SO ELIFE LA English DT Article ID DNA TARGET SITES; HISTONE OCTAMER; GENE-REGULATION; HUMAN GENOME; IN-VITRO; CHROMATIN; CAS9; ENDONUCLEASE; MECHANISM; INTERROGATION AB The CRISPR-Cas9 bacterial surveillance system has become a versatile tool for genome editing and gene regulation in eukaryotic cells, yet how CRISPR-Cas9 contends with the barriers presented by eukaryotic chromatin is poorly understood. Here we investigate how the smallest unit of chromatin, a nucleosome, constrains the activity of the CRISPR-Cas9 system. We find that nucleosomes assembled on native DNA sequences are permissive to Cas9 action. However, the accessibility of nucleosomal DNA to Cas9 is variable over several orders of magnitude depending on dynamic properties of the DNA sequence and the distance of the PAM site from the nucleosome dyad. We further find that chromatin remodeling enzymes stimulate Cas9 activity on nucleosomal templates. Our findings imply that the spontaneous breathing of nucleosomal DNA together with the action of chromatin remodelers allow Cas9 to effectively act on chromatin in vivo. C1 [Isaac, R. Stefan; Narlikar, Geeta J.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94143 USA. [Isaac, R. Stefan] Univ Calif San Francisco, Tetrad Grad Program, San Francisco, CA 94143 USA. [Jiang, Fuguo] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Jiang, Fuguo; Doudna, Jennifer A.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA. [Lim, Wendell A.] Univ Calif San Francisco, Howard Hughes Med Inst, Dept Cellular & Mol Pharmacol, San Francisco, CA USA. [Lim, Wendell A.; Almeida, Ricardo] Univ Calif San Francisco, Ctr Syst & Synthet Biol, San Francisco, CA 94143 USA. [Lim, Wendell A.; Almeida, Ricardo] Univ Calif San Francisco, Calif Inst Quantitat Biosci, San Francisco, CA 94143 USA. [Almeida, Ricardo] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94143 USA. RP Narlikar, GJ (reprint author), Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94143 USA.; Lim, WA (reprint author), Univ Calif San Francisco, Howard Hughes Med Inst, Dept Cellular & Mol Pharmacol, San Francisco, CA USA.; Lim, WA (reprint author), Univ Calif San Francisco, Ctr Syst & Synthet Biol, San Francisco, CA 94143 USA.; Lim, WA (reprint author), Univ Calif San Francisco, Calif Inst Quantitat Biosci, San Francisco, CA 94143 USA. EM Wendell.Lim@ucsf.edu; Geeta.Narlikar@ucsf.edu FU Merck Fellow of the Damon Runyon Cancer Research Foundation [DRG-2201-14]; National Science Foundation [1244557]; National Institutes of Health [R01 DA036858, P50 GM081879, R01 GM073767]; Howard Hughes Medical Institute FX Merck Fellow of the Damon Runyon Cancer Research Foundation DRG-2201-14 Fuguo Jiang; National Science Foundation 1244557 Jennifer A Doudna; National Institutes of Health R01 DA036858 Wendell A Lim; National Institutes of Health P50 GM081879 Wendell A Lim; National Institutes of Health R01 GM073767 Geeta J Narlikar; Howard Hughes Medical Institute Jennifer A Doudna Wendell A Lim; The funders had no role in study design, data collection and interpretation, or the decision to submit the work for publication NR 50 TC 13 Z9 13 U1 7 U2 7 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD APR 28 PY 2016 VL 5 AR e13450 DI 10.7554/eLife.13450 PG 14 WC Biology SC Life Sciences & Biomedicine - Other Topics GA EB5YG UT WOS:000387456200001 ER PT J AU Peers, F Bellouin, N Waquet, F Ducos, F Goloub, P Mollard, J Myhre, G Skeie, RB Takemura, T Tanre, D Thieuleux, F Zhang, K AF Peers, F. Bellouin, N. Waquet, F. Ducos, F. Goloub, P. Mollard, J. Myhre, G. Skeie, R. B. Takemura, T. Tanre, D. Thieuleux, F. Zhang, K. TI Comparison of aerosol optical properties above clouds between POLDER and AeroCom models over the South East Atlantic Ocean during the fire season SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID BLACK CARBON; POLARIZATION MEASUREMENTS; LIGHT-ABSORPTION; DUST AEROSOLS; GOCART MODEL; GLOBAL-MODEL; SAFARI 2000; A-TRAIN; SATELLITE; SENSITIVITY AB Aerosol properties above clouds have been retrieved over the South East Atlantic Ocean during the fire season 2006 using satellite observations from POLDER (Polarization and Directionality of Earth Reflectances). From June to October, POLDER has observed a mean Above-Cloud Aerosol Optical Thickness (ACAOT) of 0.28 and a mean Above-Clouds Single Scattering Albedo (ACSSA) of 0.87 at 550 nm. These results have been used to evaluate the simulation of aerosols above clouds in five Aerosol Comparisons between Observations and Models (Goddard Chemistry Aerosol Radiation and Transport (GOCART), Hadley Centre Global Environmental Model 3 (HadGEM3), European Centre Hamburg Model 5-Hamburg Aerosol Module 2 (ECHAM5-HAM2), Oslo-Chemical Transport Model 2 (OsloCTM2), and Spectral Radiation-Transport Model for Aerosol Species (SPRINTARS)). Most models do not reproduce the observed large aerosol load episodes. The comparison highlights the importance of the injection height and the vertical transport parameterizations to simulate the large ACAOT observed by POLDER. Furthermore, POLDER ACSSA is best reproduced by models with a high imaginary part of black carbon refractive index, in accordance with recent recommendations. C1 [Peers, F.; Waquet, F.; Ducos, F.; Goloub, P.; Tanre, D.; Thieuleux, F.] Univ Lille 1, Opt Atmospher Lab, F-59655 Villeneuve Dascq, France. [Peers, F.] Univ Exeter, Coll Engn Math & Phys Sci, Exeter, Devon, England. [Bellouin, N.; Mollard, J.] Univ Reading, Dept Meteorol, Reading, Berks, England. [Myhre, G.; Skeie, R. B.] Ctr Int Climate & Environm Res Oslo, Oslo, Norway. [Takemura, T.] Kyushu Univ, Res Inst Appl Mech, Fukuoka 812, Japan. [Zhang, K.] Max Planck Inst Meteorol, Bundesstr 55, D-20146 Hamburg, Germany. [Zhang, K.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Peers, F (reprint author), Univ Lille 1, Opt Atmospher Lab, F-59655 Villeneuve Dascq, France.; Peers, F (reprint author), Univ Exeter, Coll Engn Math & Phys Sci, Exeter, Devon, England. EM f.peers@exeter.ac.uk RI Takemura, Toshihiko/C-2822-2009; Zhang, Kai/F-8415-2010; Kyushu, RIAM/F-4018-2015; Skeie, Ragnhild/K-1173-2015; Myhre, Gunnar/A-3598-2008 OI Takemura, Toshihiko/0000-0002-2859-6067; Zhang, Kai/0000-0003-0457-6368; Skeie, Ragnhild/0000-0003-1246-4446; Myhre, Gunnar/0000-0002-4309-476X FU French National Research Agency (ANR) [ANR-11-LABX-0005-01]; Regional Council Nord-Pas de Calais; European Funds for Regional Economic Development; Programme National de Teledetection Spatiale (PNTS) [PNTS-2013-10]; DOE [DE-AC06-76RLO 1830] FX The Chemical and Physical Properties of the Atmosphere project is funded by the French National Research Agency (ANR) through the Programme d'Investissement d'Avenir under contract ANR-11-LABX-0005-01 and by the Regional Council Nord-Pas de Calais and the European Funds for Regional Economic Development. This work was supported by the Programme National de Teledetection Spatiale (PNTS, http://www.insu.cnrs.fr/ pnts), grant PNTS-2013-10. The authors are grateful to the CNES, NASA, and the ICARE data and services center. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. Authors are grateful to the Editor and the anonymous reviewer whose insightful comments helped improve the manuscript. The AeroCom database can be accessed by following the instructions on http://aerocom.met.no/data.html. POLDER products are available through the ICARE data and service center (http://www.icare.univ-lille1.fr/) and, for the data set used in this analysis, upon request to Fanny Peers (f.peers@exeter.ac.uk) or Fabien Waquet (fabien.waquet@univ-lille1.fr). The AERONET data are accessible via the web interface http://aeronet.gsfc.nasa.gov/. NR 49 TC 0 Z9 0 U1 2 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. 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Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Reis, T Seva, T Velde, CV Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Wang, M Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A 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Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sinthuprasith, T. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for massive WH resonances decaying into the l nu b(b)over-bar final state at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PROTON-PROTON COLLISIONS; ATLAS DETECTOR; CROSS-SECTION; PP COLLISIONS; HIGGS-BOSON; LHC; WZ AB A search for a massive resonance W'decaying into a W and a Higgs boson in the l nu b (b) over bar (l = e, mu) final state is presented. Results are based on data corresponding to an integrated luminosity of 19.7 fb(-1) of proton-proton collisions at root s = 8 TeV, collected using the CMS detector at the LHC. For a high-mass (greater than or similar to 1 TeV) resonance, the two bottom quarks coming from the Higgs boson decay are reconstructed as a single jet, which can be tagged by placing requirements on its substructure and flavour. Exclusion limits at 95 % confidence level are set on the production cross section of a narrow resonance decaying into WH, as a function of its mass. In the context of a little Higgs model, a lower limit on the W' mass of 1.4 TeV is set. In a heavy vector triplet model that mimics the properties of composite Higgs models, a lower limit on the W' mass of 1.5 TeV is set. In the context of this model, the results are combined with related searches to obtain a lower limit on the W' mass of 1.8 TeV, the most restrictive to date for decays to a pair of standard model bosons. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. 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[Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. 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M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.; Agapitos, A.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] Inst Nucl & Particle Phys, NCSR Demokritos, Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens 11528, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. 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[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, R.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, R.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, I-56100 Pisa, Italy. [Donato, S.; Fedi, G.; Grippo, M. T.; Lomtadze, T.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Migliore, E.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Solano, A.; Staiano, A.] INFN, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. 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[Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Matveev, V.; Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Kalinin, A.; Konstantinov, D.; Sobol, A.; Tourtchanovitch, L.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Thyssen, F.; Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Thyssen, F.; Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Gonzalez Caballero, I.; Palencia Cortezon, E.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Viliani, L.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Med, Dept Phys, Bangkok 10330, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Polatoz, A.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Ball, F.; Clement, E.; Cussans, D.; Heath, G. P.; Lucas, C.; Newbold, D. M.; Poll, A.; Smith, D.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. 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G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Finger, M.; Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Hempel, M.; Karacheban, O.; Lobanov, A.; Mankel, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Giassi, A.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. [De La Cruz, B.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale Super Pisa, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Zanetti, M.] Univ Rome, Fac Engn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. Erzincan Univ, Erzincan, Turkey. [Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Lokhtin, Igor/D-7004-2012; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Da Silveira, Gustavo Gil/N-7279-2014; Della Ricca, Giuseppe/B-6826-2013; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010 OI Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science - European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 73 TC 1 Z9 1 U1 19 U2 33 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 28 PY 2016 VL 76 IS 5 AR 237 DI 10.1140/epjc/s10052-016-4067-z PG 26 WC Physics, Particles & Fields SC Physics GA DM9JA UT WOS:000376680500001 PM 28280427 ER PT J AU Jain, A Hautier, G Ong, SP Persson, K AF Jain, Anubhav Hautier, Geoffroy Ong, Shyue Ping Persson, Kristin TI New opportunities for materials informatics: Resources and data mining techniques for uncovering hidden relationships SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID ARTIFICIAL NEURAL-NETWORKS; CRYSTAL-STRUCTURE DATABASE; DENSITY-FUNCTIONAL THEORY; TRANSPARENT CONDUCTING OXIDES; STRUCTURE MAPS; DESIGN; PRINCIPLES; ALGORITHMS; CATHODES; INFRASTRUCTURE AB Data mining has revolutionized sectors as diverse as pharmaceutical drug discovery, finance, medicine, and marketing, and has the potential to similarly advance materials science. In this paper, we describe advances in simulation-based materials databases, open-source software tools, and machine learning algorithms that are converging to create new opportunities for materials informatics. We discuss the data mining techniques of exploratory data analysis, clustering, linear models, kernel ridge regression, tree-based regression, and recommendation engines. We present these techniques in the context of several materials application areas, including compound prediction, Li-ion battery design, piezoelectric materials, photocatalysts, and thermoelectric materials. Finally, we demonstrate how new data and tools are making it easier and more accessible than ever to perform data mining through a new analysis that learns trends in the valence and conduction band character of compounds in the Materials Project database using data on over 2500 compounds. C1 [Jain, Anubhav; Persson, Kristin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy & Environm Technol Div, Berkeley, CA 94720 USA. [Hautier, Geoffroy] Catholic Univ Louvain, Inst Condensed Matter & Nanosci IMCN, B-1348 Louvain La Neuve, Belgium. [Ong, Shyue Ping] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Persson, Kristin] Univ Calif Berkeley, Mat Sci & Engn, Berkeley, CA 94720 USA. RP Jain, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy & Environm Technol Div, Berkeley, CA 94720 USA. EM ajain@lbl.edu FU U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Department [DE-AC02-05CH11231]; European Union Marie Curie Career Integration (CIG) grant [HT4TCOs PCIG11-GA-2012-321988] FX This work was intellectually led by the Materials Project (DOE Basic Energy Sciences Grant No. EDC-BEE). Work at the Lawrence Berkeley National Laboratory was supported by the U.S. Department of Energy Office of Science, Office of Basic Energy Sciences Department under Contract No. DE-AC02-05CH11231. GH acknowledges financial support from the European Union Marie Curie Career Integration (CIG) grant HT4TCOs PCIG11-GA-2012-321988. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility. NR 128 TC 4 Z9 4 U1 25 U2 60 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 28 PY 2016 VL 31 IS 8 BP 977 EP 994 DI 10.1557/jmr.2016.80 PG 18 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LK UT WOS:000376178000001 ER PT J AU Mohanty, G Wehrs, J Boyce, BL Taylor, A Hasegawa, M Philippe, L Michler, J AF Mohanty, Gaurav Wehrs, Juri Boyce, Brad L. Taylor, Aidan Hasegawa, Madoka Philippe, Laetitia Michler, Johann TI Room temperature stress relaxation in nanocrystalline Ni measured by micropillar compression and miniature tension SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID STRAIN-RATE SENSITIVITY; ULTRAFINE-GRAINED ALUMINUM; ACTIVATION VOLUME; NANOINDENTATION CREEP; PLASTIC-DEFORMATION; SINGLE-CRYSTALS; NICKEL; METALS; BEHAVIOR; FCC AB In this study, we report a micropillar stress relaxation technique employing a stable displacement-controlled, in-situ scanning electron microscope indenter, and unusually large micropillars to precisely measure stress relaxation in electroplated nanocrystalline Ni thin films. The observed stress relaxation is significant under constant displacement: even well below the 0.2% offset yield strength, the stresses relax by; similar to 4% within a minute; in the work hardening regime, stress relaxes by; similar to 9% in 1 min. A logarithmic fit of the relaxation curves is consistent with an Arrhenius thermal activation of plasticity and suggests an activation volume in the vicinity of; similar to 10 b(3). The apparent and effective activation volumes diverge at lower strains, particularly in the "elastic" regime. These measurements are compared to similar measurements performed on free-standing thin film tensile coupons. Both methods yield similar results, thereby validating the applicability of pillar compression to capture time-dependent plasticity. To our knowledge, these are the first micropillar stress relaxation experiments on metals ever reported. C1 [Mohanty, Gaurav; Wehrs, Juri; Taylor, Aidan; Hasegawa, Madoka; Philippe, Laetitia; Michler, Johann] Empa Swiss Fed Labs Mat Sci & Technol, Lab Mech Mat & Nanostruct, CH-3602 Thun, Switzerland. [Boyce, Brad L.] Sandia Natl Labs, Mat Sci & Engn Ctr, POB 5800, Albuquerque, NM 87185 USA. RP Mohanty, G (reprint author), Empa Swiss Fed Labs Mat Sci & Technol, Lab Mech Mat & Nanostruct, CH-3602 Thun, Switzerland. EM Gaurav.Mohanty@empa.ch OI Philippe, laetitia/0000-0003-0928-4487; Mohanty, Gaurav/0000-0002-0816-307X FU Strength-ABLE, an EURAMET joint research project - European Community [EMPIR 14IND03, 217257]; EMPA Postdoc program - FP7: Marie Curie Actions; United States Department of Energy, office of Basic Energy Science (BES) FX Funding by Strength-ABLE (EMPIR 14IND03), an EURAMET joint research project funded by the European Community's Seventh Framework Programme, ERA-NET Plus, under Grant Agreement No. 217257 is gratefully acknowledged. Gaurav Mohanty, Aidan Taylor and Madoka Hasegawa would like to acknowledge funding from EMPA Postdoc program cofunded by FP7: Marie Curie Actions. BLB was funded by The United States Department of Energy, office of Basic Energy Science (BES). NR 41 TC 2 Z9 2 U1 10 U2 19 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 28 PY 2016 VL 31 IS 8 BP 1085 EP 1095 DI 10.1557/jmr.2016.101 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LK UT WOS:000376178000012 ER PT J AU Jacobsen, MK Velisavljevic, N AF Jacobsen, M. K. Velisavljevic, N. TI High pressure elasticity and thermal properties of depleted uranium SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ALPHA-URANIUM; DEGREES K; PHASE-TRANSITION; 1ST PRINCIPLES; TEMPERATURE; MODULI; CONSTANTS; ANVIL; STATE; GPA AB Studies of the phase diagram of uranium have revealed a wealth of high pressure and temperature phases. Under ambient conditions the crystal structure is well defined up to 100 gigapascals (GPa), but very little information on thermal conduction or elasticity is available over this same range. This work has applied ultrasonic interferometry to determine the elasticity, mechanical, and thermal properties of depleted uranium to 4.5 GPa. Results show general strengthening with applied load, including an overall increase in acoustic thermal conductivity. Further implications are discussed within. This work presents the first high pressure studies of the elasticity and thermal properties of depleted uranium metal and the first real-world application of a previously developed containment system for making such measurements. (C) 2016 Author(s). C1 [Jacobsen, M. K.; Velisavljevic, N.] Los Alamos Natl Lab, Shock & Detonat Phys M 9, POB 1663, Los Alamos, NM 87544 USA. RP Jacobsen, MK; Velisavljevic, N (reprint author), Los Alamos Natl Lab, Shock & Detonat Phys M 9, POB 1663, Los Alamos, NM 87544 USA. EM mjacobsen@lanl.gov; nenad@lanl.gov FU DOE-NNSA [DE-AC52-06NA25396, DE-NA0001974]; LANL Science Campaign 1; LANL Science Campaign 2; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357]; NSF; U.S. DOE [DE-AC02-06CH11357]; U.S. Department of Energy through the LANL/LDRD Program; G.T. Seaborg Institute FX Los Alamos National Laboratory (LANL) is operated by LANS, LLC, for the DOE-NNSA under Contract No. DE-AC52-06NA25396. The authors acknowledge funding support from LANL Science Campaigns 1 and 2. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. M.K.J. gratefully acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program and the G.T. Seaborg Institute for this work. The authors also thank Dr. Baosheng Li for the use of his pulse-echo overlap software for determination of transit times. NR 44 TC 0 Z9 0 U1 6 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 28 PY 2016 VL 119 IS 16 AR 165904 DI 10.1063/1.4948300 PG 6 WC Physics, Applied SC Physics GA DL8ZD UT WOS:000375929900049 ER PT J AU Lischner, J Nemsak, S Conti, G Gloskovskii, A Palsson, GK Schneider, CM Drube, W Louie, SG Fadley, C AF Lischner, Johannes Nemsak, Slavomir Conti, Giuseppina Gloskovskii, Andrei Palsson, Gunnar Karl Schneider, Claus M. Drube, Wolfgang Louie, Steven G. Fadley, Charles TI Accurate determination of the valence band edge in hard x-ray photoemission spectra using GW theory SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; PRECISE DETERMINATION; QUASI-PARTICLE; DIAMOND; TIO2 AB We introduce a new method for determining accurate values of the valence-band maximum in x-ray photoemission spectra. Specifically, we align the sharpest peak in the valence-band region of the experimental spectrum with the corresponding feature of a theoretical valence-band density of states curve from ab initio GW theory calculations. This method is particularly useful for soft and hard x-ray photoemission studies of materials with a mixture of valence-band characters, where strong matrix element effects can render standard methods for extracting the valence-band maximum unreliable. We apply our method to hydrogen-terminated boron-doped diamond, which is a promising substrate material for novel solar cell devices. By carrying out photoemission experiments with variable light polarizations, we verify the accuracy of our analysis and the general validity of the method. Published by AIP Publishing. C1 [Lischner, Johannes; Nemsak, Slavomir; Conti, Giuseppina; Palsson, Gunnar Karl; Louie, Steven G.; Fadley, Charles] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Thomas Young Ctr Theory & Simulat Mat, London SW7 2AZ, England. [Nemsak, Slavomir; Conti, Giuseppina; Palsson, Gunnar Karl; Fadley, Charles] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Nemsak, Slavomir; Schneider, Claus M.] Forschungszentrum Julich, Peter Gruenberg Inst 6, D-52425 Julich, Germany. [Gloskovskii, Andrei; Drube, Wolfgang] Deutsch Elektronen Synchrotron DESY, Photon Sci, Notkestr 85, D-22607 Hamburg, Germany. [Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Palsson, Gunnar Karl] Uppsala Univ, Dept Phys & Astron, SE-75120 Uppsala, Sweden. RP Lischner, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Lischner, J (reprint author), Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England.; Lischner, J (reprint author), Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England.; Lischner, J (reprint author), Univ London Imperial Coll Sci Technol & Med, Thomas Young Ctr Theory & Simulat Mat, London SW7 2AZ, England. EM jlischner597@gmail.com RI Hloskovsky, Andrei/A-3009-2012; Schneider, Claus/H-7453-2012 OI Schneider, Claus/0000-0002-3920-6255 FU SciDAC Program on Excited State Phenomena (methods and software developments) and Theory Program - U.S. Department of Energy, the Office of Basic Energy Sciences and of Advanced Scientific Computing Research at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; NSF [DMR15-1508412]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering via the LBNL Materials Sciences Division, Magnetic Materials Program [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering via the Department of Physics, University of California Davis [DE-SC0014697]; International Union for Vacuum Science, Technique and Applications; Swedish Research Council; MURI grant of the Army Research Office [W911-NF-09-1-0398]; German Federal Ministry of Education and Research (BMBF) [05KS7UM1, 05K10UMA]; Universitat Mainz; Universitat Wurzburg [05KS7WW3, 05K10WW1, 05K13WW1] FX This work was supported by the SciDAC Program on Excited State Phenomena (methods and software developments) and Theory Program (GW calculations) funded by the U.S. Department of Energy, the Office of Basic Energy Sciences and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory, and by NSF Grant No. DMR15-1508412 (theoretical analysis). Computational resources have been provided by the DOE at NERSC. G.K.P. and C.S.F. acknowledge salary support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-05CH11231, via the LBNL Materials Sciences Division, Magnetic Materials Program, and Grant No. DE-SC0014697, via the Department of Physics, University of California Davis. G.K.P. also acknowledges the International Union for Vacuum Science, Technique and Applications and the Swedish Research Council for financial support as well as partial salary support and travel support from a MURI grant of the Army Research Office (Grant No. W911-NF-09-1-0398). Funding for the photoemission instrument at beamline P09 (DESY) by the German Federal Ministry of Education and Research (BMBF) under contracts 05KS7UM1 and 05K10UMA with Universitat Mainz; 05KS7WW3, 05K10WW1, and 05K13WW1 with Universitat Wurzburg was gratefully acknowledged. NR 30 TC 0 Z9 0 U1 6 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 28 PY 2016 VL 119 IS 16 AR 165703 DI 10.1063/1.4947594 PG 7 WC Physics, Applied SC Physics GA DL8ZD UT WOS:000375929900044 ER PT J AU Samanta, A Morales, MA Schwegler, E AF Samanta, Amit Morales, Miguel A. Schwegler, Eric TI Exploring the free energy surface using ab initio molecular dynamics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RARE EVENT SIMULATIONS; WAVE BASIS-SET; MECHANICAL ATTRITION; CANONICAL ENSEMBLE; MULTISCALE METHODS; STRING METHOD; EQUILIBRIUM; PREDICTION; EFFICIENCY; ALGORITHM AB Efficient exploration of configuration space and identification of metastable structures in condensed phase systems are challenging from both computational and algorithmic perspectives. In this regard, schemes that utilize a set of pre-defined order parameters to sample the relevant parts of the configuration space [L. Maragliano and E. Vanden-Eijnden, Chem. Phys. Lett. 426, 168 (2006); J. B. Abrams and M. E. Tuckerman, J. Phys. Chem. B 112, 15742 (2008)] have proved useful. Here, we demonstrate how these order-parameter aided temperature accelerated sampling schemes can be used within the Born-Oppenheimer and the Car-Parrinello frameworks of ab initio molecular dynamics to efficiently and systematically explore free energy surfaces, and search for metastable states and reaction pathways. We have used these methods to identify the metastable structures and reaction pathways in SiO2 and Ti. In addition, we have used the string method [W. E, W. Ren, and E. Vanden-Eijnden, Phys. Rev. B 66, 052301 (2002); L. Maragliano et al., J. Chem. Phys. 125, 024106 (2006)] within the density functional theory to study the melting pathways in the high pressure cotunnite phase of SiO2 and the hexagonal closed packed to face centered cubic phase transition in Ti. Published by AIP Publishing. C1 [Samanta, Amit; Morales, Miguel A.; Schwegler, Eric] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Samanta, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM samanta1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX The authors are grateful to Liang Qi and Qian Yu for motivating us to study the stability of FCC phase in bulk Ti and to Sebastian Hamel for motivating us to study the cotunnite phase of SiO2. A.S. wishes to thank Professor Weinan E, Professor Mark Tuckerman, Professor Giovanni Ciccotti, Professor Eric Vanden-Eijnden, and Professor Sara Bonella for their comments. In addition, we want to thank Alfredo Correa and Xavier Andrade-Valencia for their help in improving the manuscript. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 61 TC 1 Z9 1 U1 9 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 28 PY 2016 VL 144 IS 16 AR 164101 DI 10.1063/1.4945653 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL6YK UT WOS:000375785800008 PM 27131525 ER PT J AU Xu, YT Dibble, CJ Petrik, NG Smith, RS Joly, AG Tonkyn, RG Kay, BD Kimmel, GA AF Xu, Yuntao Dibble, Collin J. Petrik, Nikolay G. Smith, R. Scott Joly, Alan G. Tonkyn, Russell G. Kay, Bruce D. Kimmel, Greg A. TI A nanosecond pulsed laser heating system for studying liquid and supercooled liquid films in ultrahigh vacuum SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID AMORPHOUS SOLID WATER; NEAR-AMBIENT CONDITIONS; NO-MANS-LAND; GLASSY WATER; 150 K; PHOTOELECTRON-SPECTROSCOPY; THERMAL TRANSPORT; INFRARED-SPECTRA; NUCLEATION RATES; METAL-SURFACES AB A pulsed laser heating system has been developed that enables investigations of the dynamics and kinetics of nanoscale liquid films and liquid/solid interfaces on the nanosecond time scale in ultrahigh vacuum (UHV). Details of the design, implementation, and characterization of a nanosecond pulsed laser system for transiently heating nanoscale films are described. Nanosecond pulses from a Nd: YAG laser are used to rapidly heat thin films of adsorbed water or other volatile materials on a clean, well-characterized Pt(111) crystal in UHV. Heating rates of similar to 10(10) K/s for temperature increases of similar to 100-200 K are obtained. Subsequent rapid cooling (similar to 5 x 10(9) K/s) quenches the film, permitting insitu, post-heating analysis using a variety of surface science techniques. Lateral variations in the laser pulse energy are similar to +/- 2.7% leading to a temperature uncertainty of similar to +/- 4.4 K for a temperature jump of 200 K. Initial experiments with the apparatus demonstrate that crystalline ice films initially held at 90 K can be rapidly transformed into liquid water films with T > 273 K. No discernable recrystallization occurs during the rapid cooling back to cryogenic temperatures. In contrast, amorphous solid water films heated below the melting point rapidly crystallize. The nanosecond pulsed laser heating system can prepare nanoscale liquid and supercooled liquid films that persist for nanoseconds per heat pulse in an UHV environment, enabling experimental studies of a wide range of phenomena in liquids and at liquid/solid interfaces. Published by AIP Publishing. C1 [Xu, Yuntao; Dibble, Collin J.; Petrik, Nikolay G.; Smith, R. Scott; Joly, Alan G.; Tonkyn, Russell G.; Kay, Bruce D.; Kimmel, Greg A.] Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. RP Kay, BD; Kimmel, GA (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. EM bruce.kay@pnnl.gov; gregory.kimmel@pnnl.gov RI Smith, Scott/G-2310-2015; Petrik, Nikolay/G-3267-2015; Xu, Yuntao/G-1896-2015; OI Smith, Scott/0000-0002-7145-1963; Petrik, Nikolay/0000-0001-7129-0752; Kimmel, Greg/0000-0003-4447-2440 FU US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. The research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 78 TC 1 Z9 1 U1 10 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 28 PY 2016 VL 144 IS 16 AR 164201 DI 10.1063/1.4947304 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL6YK UT WOS:000375785800026 PM 27131543 ER PT J AU Chenard, E Sutrisno, A Zhu, LY Assary, RS Kowalski, JA Barton, JL Bertke, JA Gray, DL Brushett, FR Curtiss, LA Moore, JS AF Chenard, Etienne Sutrisno, Andre Zhu, Lingyang Assary, Rajeev S. Kowalski, Jeffrey A. Barton, John L. Bertke, Jeffery A. Gray, Danielle L. Brushett, Fikile R. Curtiss, Larry A. Moore, Jeffrey S. TI Synthesis of Pyridine- and Pyrazine-BF3 Complexes and Their Characterization in Solution and Solid State SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID BORON-TRIFLUORIDE COMPLEXES; BASE-INDUCED DEPROTONATION; DENSITY-FUNCTIONAL THEORY; ELECTRIC-FIELD GRADIENT; LEWIS-ACID COMPLEXES; B-11 MAS NMR; N-OXIDES; ELECTROPHILIC REACTION; ELECTROLYTE ADDITIVES; CHEMICAL-SHIFTS AB Following the discovery of the redox-active 1,4-bis-BF3-quinoxaline complex, we undertook a structure activity study with the objective to understand the active nature of the quinoxaline complex. Through systematic synthesis and characterization, we have compared complexes prepared from pyridine and pyrazine derivatives, as hetero-cyclic core analogues. This paper reports the structural requirements that give rise to the electrochemical features of the 1,4-bis-BF3-quinoxaline adduct. Using solution and solid-state NMR spectroscopy, the role of aromatic ring fusion and nitrogen incorporation in bonding and electronics was elucidated. We establish the boron atom location and its interaction with its environment from 1D and 2D solution NMR, X-ray diffraction analysis, and B-11 solid-state NMR experiments. Crystallographic analysis of single crystals helped to correlate the boron geometry with B-11 quadrupolar coupling constant (C-Q) and asymmetry parameter (eta(Q)), extracted from B-11 solid-state NMR spectra. Additionally, computations based on density functional theory were performed to predict electrochemical behavior of the BF3-heteroaromatic complexes. We then experimentally measured electrochemical potential using cyclic voltammetry and found that the redox potentials and C-Q values are similarly affected by electronic changes in the complexes. C1 [Chenard, Etienne; Assary, Rajeev S.; Kowalski, Jeffrey A.; Barton, John L.; Brushett, Fikile R.; Curtiss, Larry A.; Moore, Jeffrey S.] Univ Illinois, Joint Ctr Energy Storage Res, Urbana, IL 61801 USA. [Chenard, Etienne; Moore, Jeffrey S.] Univ Illinois, Sch Chem Sci, Urbana, IL 61801 USA. [Sutrisno, Andre; Zhu, Lingyang] Univ Illinois, Sch Chem Sci, NMR EPR Lab, Urbana, IL 61801 USA. [Bertke, Jeffery A.; Gray, Danielle L.] Univ Illinois, Sch Chem Sci, GL Clark Xray Facil, Urbana, IL 61801 USA. [Moore, Jeffrey S.] Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. [Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kowalski, Jeffrey A.; Barton, John L.; Brushett, Fikile R.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. RP Moore, JS (reprint author), Univ Illinois, Joint Ctr Energy Storage Res, Urbana, IL 61801 USA.; Moore, JS (reprint author), Univ Illinois, Sch Chem Sci, Urbana, IL 61801 USA.; Moore, JS (reprint author), Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. EM jsmoore@illinois.edu OI Gray, Danielle/0000-0003-0059-2096 FU Joint Center for Energy Storage Research, an Energy Innovative Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovative Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The authors also thank Professor Charles Diesendruck for providing the 1,4-bis-BF3-quinoxaline complex, in addition to all the inspiring discussions. NR 44 TC 2 Z9 2 U1 7 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 28 PY 2016 VL 120 IS 16 BP 8461 EP 8471 DI 10.1021/acs.jpcc.6b00858 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL3GH UT WOS:000375521700006 ER PT J AU Weinhardt, L Fuchs, O Fischer, A Weigand, M Meyer, F Benkert, A Blum, M Bar, M Pookpanratana, S Denlinger, J Heske, C Umbach, E AF Weinhardt, Lothar Fuchs, Oliver Fischer, Andre Weigand, Markus Meyer, Frank Benkert, Andreas Blum, Monika Baer, Marcus Pookpanratana, Sujitra Denlinger, Jonathan Heske, Clemens Umbach, Eberhard TI Site- and Symmetry-Resolved Resonant X-ray Emission Study of a Highly Ordered PTCDA Thin Film SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LARGE AROMATIC-MOLECULES; CHARGE-TRANSFER DYNAMICS; SURFACE CHEMICAL-BOND; ELECTRONIC-STRUCTURE; 3,4,9,10-PERYLENETETRACARBOXYLICACID-DIANHYDRIDE PTCDA; PHOTOEMISSION-SPECTROSCOPY; ABSORPTION-SPECTRA; DENSITY; ADSORBATES; CU(110) AB The complex electronic structure of ordered 3,4,9,10-perylene tetracarboxylic acid dianhydride (PTCDA) multilayers on Ag(111) is investigated by angle-dependent resonant X-ray emission spectroscopy at the carbon K edge. Beam damage effects were characterized and special care was taken to avoid their influence on the spectra. Appropriate selection of excitation energies and detection geometries allow us to record element-, atom-, and symmetry-specific X-ray emission spectra by making use of dipole selection rules. This specificity, especially the ability to distinguish between sigma and pi orbitals, gives unprecedented experimental insights into the electronic structure of this large organic molecule. The experimental results are compared with calculated spectra of the isolated molecule, as derived from density functional theory. This allows a detailed discussion of the spectra and separation of the contributions from nonequivalent carbon atoms. C1 [Weinhardt, Lothar; Benkert, Andreas; Heske, Clemens; Umbach, Eberhard] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat IPS, Hermann V Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Weinhardt, Lothar; Heske, Clemens] Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem ITCP, Engesserstr 18-20, D-76128 Karlsruhe, Germany. [Weinhardt, Lothar; Heske, Clemens] Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, Hermann V Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Weinhardt, Lothar; Blum, Monika; Pookpanratana, Sujitra; Heske, Clemens] Univ Nevada, Dept Chem & Biochem, Las Vegas UNLV, Las Vegas, NV 89154 USA. [Fuchs, Oliver; Fischer, Andre; Weigand, Markus; Meyer, Frank; Benkert, Andreas; Umbach, Eberhard] Univ Wurzburg, Expt Phys 7, D-97074 Wurzburg, Germany. [Blum, Monika; Denlinger, Jonathan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Baer, Marcus] Helmholtz Zentrum Berlin Mat & Energie GmbH, Renewable Energy, Hahn Meitner Pl 1, D-14109 Berlin, Germany. [Baer, Marcus] Brandenburg Tech Univ Cottbus Senftenberg, Inst Phys & Chem, Pl Deutsch Einheit 1, D-03046 Cottbus, Germany. RP Weinhardt, L; Heske, C (reprint author), Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat IPS, Hermann V Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany.; Weinhardt, L; Heske, C (reprint author), Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem ITCP, Engesserstr 18-20, D-76128 Karlsruhe, Germany.; Weinhardt, L; Heske, C (reprint author), Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, Hermann V Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany.; Weinhardt, L; Heske, C (reprint author), Univ Nevada, Dept Chem & Biochem, Las Vegas UNLV, Las Vegas, NV 89154 USA. EM lothar.weinhardt@kit.edu; heske@unlv.nevada.edu FU German BMBF [05 KS4WWA/6, 05 KS4VHA/4]; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Impuls- and Vernetzungsfonds of the Helmholtz Association [VH-NG-423] FX We are grateful to Rudiger Szargan and his research group (Physikalische Chemie II, Universitat Leipzig) for providing and preparing the ROSA endstation for our experiment. Further, we thank Moritz Sokolowski and his group (Institut fur Physikalische and Theoretische Chemie, Universitat Bonn) for supplying the highly purified PTCDA powder, Achim Scholl and Stefan Krause for fruitful discussions, and the ALS and BESSY staff for technical support. This work was funded by the German BMBF (projects No. 05 KS4WWA/6 and 05 KS4VHA/4). The ALS is supported by the Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.B. acknowledges support by the Impuls- and Vernetzungsfonds of the Helmholtz Association (VH-NG-423). NR 57 TC 0 Z9 0 U1 5 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 28 PY 2016 VL 120 IS 16 BP 8607 EP 8615 DI 10.1021/acs.jpcc.5b12422 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL3GH UT WOS:000375521700021 ER PT J AU Dyatkin, B Zhang, Y Mamontov, E Kolesnikov, AI Cheng, YQ Meyer, HM Cummings, PT Gogotsi, Y AF Dyatkin, Boris Zhang, Yu Mamontov, Eugene Kolesnikov, Alexander I. Cheng, Yongqiang Meyer, Harry M., III Cummings, Peter T. Gogotsi, Yury TI Influence of Surface Oxidation on Ion Dynamics and Capacitance in Porous and Nonporous Carbon Electrodes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBIDE-DERIVED CARBONS; DOUBLE-LAYER; FORCE-FIELD; PORE-SIZE; THERMAL-STABILITY; SLIT PORES; LIQUID; SUPERCAPACITORS; SIMULATION; NANOTUBES AB We investigate the influence of surface chemistry and ion confinement on capacitance and electrosorption dynamics of room-temperature ionic liquids (RTILs) in supercapacitors. Using air oxidation and vacuum annealing, we produced defunctionalized and oxygen-rich surfaces of carbide-derived carbons (CDCs) and graphene nanoplatelets (GNPs). While oxidized surfaces of porous CDCs improve capacitance and rate handling abilities of ions, defunctionalized nonporous GNPs improve charge storage densities on planar electrodes. Quasi elastic neutron scattering (QENS) and inelastic neutron scattering (INS) probed the structure, dynamics, and orientation of RTIL ions confined in divergently functionalized pores. Oxidized, ionophilic surfaces draw ions closer to pore surfaces and enhance potential-driven ion transport during electrosorption. Molecular dynamics (MD) simulations corroborated experimental data and demonstrated the significance of surface functional groups on ion orientations, accumulation densities, and capacitance. C1 [Dyatkin, Boris; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Dyatkin, Boris; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Zhang, Yu; Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. [Mamontov, Eugene; Kolesnikov, Alexander I.; Cheng, Yongqiang] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Meyer, Harry M., III] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Gogotsi, Y (reprint author), Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA.; Gogotsi, Y (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. EM gogotsi@drexel.edu RI Mamontov, Eugene/Q-1003-2015; OI Mamontov, Eugene/0000-0002-5684-2675; Dyatkin, Boris/0000-0001-7537-2181 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; DOE Office of Science Graduate Student Research Program (SCGSR) FX The authors (B.D., E.M., Y.Z., P.T.C., and Y.G.) were supported by the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. B.D. was also supported by the DOE Office of Science Graduate Student Research Program (SCGSR). INS and QENS measurements (at ORNL) were made available through the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The authors thank Luke Daemen (ORNL) for assistance with INS measurements. The authors also thank Guang Feng (HUST) and Hsiu-Wen Wang (ORNL) for helpful discussions. NR 66 TC 1 Z9 1 U1 8 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 28 PY 2016 VL 120 IS 16 BP 8730 EP 8741 DI 10.1021/acs.jpcc.6b01204 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL3GH UT WOS:000375521700033 ER PT J AU Reddy, UV Bowers, GM Loganathan, N Bowden, M Yazaydin, AO Kirkpatrick, RJ AF Reddy, U. Venkateswara Bowers, Geoffrey M. Loganathan, Narasimhan Bowden, Mark Yazaydin, A. Ozgur Kirkpatrick, R. James TI Water Structure and Dynamics in Smectites: X-ray Diffraction and H-2 NMR Spectroscopy of Mg-, Ca-, Sr-, Na-, Cs-, and Pb-Hectorite SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID QUADRUPOLE COUPLING-CONSTANTS; NUCLEAR-MAGNETIC-RESONANCE; MOLECULAR-DYNAMICS; CLAY-MINERALS; INTERLAYER STRUCTURE; FLUORHECTORITE CLAY; INTERCALATED WATER; MONTE-CARLO; H2O; MONTMORILLONITE AB Variable-temperature X-ray diffraction and H-2 NMR spectroscopy of the smectite mineral, hectorite, containing interlayer Na+, K+, Cs+, Mg2+,Ca2+ Sr2+, and Pb2+ equilibrated at 43% relative humidity (RH) and mixed with (H2O)-H-2 to form a paste provide a comprehensive picture of the structural environments and dynamics of interlayer (H2O)-H-2 and the relationships of these properties to interlayer hydration state, the hydration energy and polarizability of the cation, temperature, and the formation of ice-lh in the interparticle pores. The variation in basal spacing shown by the XRD data correlates well with the H-2 NMR behavior, and the XRD data show show for the first time in hectorites that crystallizationof interpraticle ice-lh causes a decrease in the interlayer spacing, likely due to removal of interlayer (H2O)-H-2. The variation of the H-2 NMR behavior of all the samples with decreasing temperature reflects decreasing frequencies of motion for the rotation of the (H2O)-H-2 molecules around their dipoles, reorientation of the (H2O)-H-2 molecules, and exchange of the (H2O)-H-2 molecules between interlayer sites coordinated to and not coordinated to the cations. C1 [Reddy, U. Venkateswara; Loganathan, Narasimhan; Yazaydin, A. Ozgur] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Kirkpatrick, R. James] Michigan State Univ, Coll Nat Sci, E Lansing, MI 48824 USA. [Bowers, Geoffrey M.] Alfred Univ, Coll Liberal Arts & Sci, Div Chem, 1 Saxon Dr, Alfred, NY 14802 USA. [Bowden, Mark] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Yazaydin, A. Ozgur] UCL, Dept Chem Engn, London WC1E 7JE, England. RP Reddy, UV (reprint author), Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. EM uddigiri@msu.edu OI Bowers, Geoffrey/0000-0003-4876-9305 FU U.S. Department of Energy, Office of Basic Energy Science [DE-FG02-10ER16128, DE-FG02-08ER15929]; Office of Biological and Environmental Research at Pacific Northwest National Laboratory FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Science through grants DE-FG02-10ER16128 (Bowers, P.I.) and DE-FG02-08ER15929 (Kirkpatrick, P.I.). A portion of the research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 50 TC 3 Z9 3 U1 7 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 28 PY 2016 VL 120 IS 16 BP 8863 EP 8876 DI 10.1021/acs.jpcc.6b03431 PG 14 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DL3GH UT WOS:000375521700046 ER PT J AU Glaeser, RM AF Glaeser, Robert M. TI Cryo-EM: Protein complexes in focus SO ELIFE LA English DT Editorial Material ID TRANSMISSION ELECTRON-MICROSCOPY; PHASE-CONTRAST AB A new advance in electron microscopy can reveal highly-detailed structures of protein complexes. C1 [Glaeser, Robert M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. RP Glaeser, RM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. EM rmglaeser@lbl.gov NR 12 TC 3 Z9 3 U1 6 U2 10 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD APR 28 PY 2016 VL 5 AR e16156 DI 10.7554/eLife.16156 PG 3 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DK7SP UT WOS:000375126300001 ER PT J AU Badamchi-Zadeh, A McKay, PF Korber, BT Barinaga, G Walters, AA Nunes, A Gomes, JP Follmann, F Tregoning, JS Shattock, RJ AF Badamchi-Zadeh, Alexander McKay, Paul F. Korber, Bette T. Barinaga, Guillermo Walters, Adam A. Nunes, Alexandra Gomes, Joao Paulo Follmann, Frank Tregoning, John S. Shattock, Robin J. TI A Multi-Component Prime-Boost Vaccination Regimen with a Consensus MOMP Antigen Enghances Chlamydia trachomatis Clearance SO FRONTIERS IN IMMUNOLOGY LA English DT Article DE Chlamydia trachomatis; consensus; mosaic; prime-boost regimens; adenovirus-vector vaccines; MVA-vector vaccines; DNA vaccines ID OUTER-MEMBRANE PROTEIN; CD4(+) T-CELLS; GENITAL-TRACT INFECTION; HIGH-RISK WOMEN; IMMUNE-RESPONSES; SEROVAR DISTRIBUTION; PROTECTIVE IMMUNITY; MOUSE MODEL; MURIDARUM INFECTION; GAMMA-INTERFERON AB Background: A vaccine for Chlamydia trachomatis is of urgent medical need. We explored bioinformatic approaches to generate an immunogen against C. trachomatis that would induce cross-serovar T-cell responses as (i) CD4(+) T cells have been shown in animal models and human studies to be important in chlamydial protection and (ii) antibody responses may be restrictive and serovar specific. Methods: A consensus antigen based on over 1,500 major outer membrane protein (MOMP) sequences provided high epitope coverage against the most prevalent C. trachomatis strains in silico. Having designed the T-cell immunogen, we assessed it for immunogenicity in prime-boost regimens. This consensus MOMP transgene was delivered using plasmid DNA, Human Adenovirus 5 (HuAd5) or modified vaccinia Ankara (MVA) vectors with or without MF59 (R) adjuvanted recombinant MOMP protein. Results: Different regimens induced distinct immune profiles. The DNA-HuAd5-MVA-Protein vaccine regimen induced a cellular response with a Th1-biased serum antibody response, alongside high serum and vaginal MOMP-specific antibodies. This regimen significantly enhanced clearance against intravaginal C. trachomatis serovar D infection in both BALB/c and B6C3F1 mouse strains. This enhanced clearance was shown to be CD4(+) T-cell dependent. Future studies will need to confirm the specificity and precise mechanisms of protection. Conclusion: A C. trachomatis vaccine needs to induce a robust cellular response with broad cross-serovar coverage and a heterologous prime-boost regimen may be an approach to achieve this. C1 [Badamchi-Zadeh, Alexander; McKay, Paul F.; Barinaga, Guillermo; Walters, Adam A.; Tregoning, John S.; Shattock, Robin J.] Univ London Imperial Coll Sci Technol & Med, Mucosal Infect & Immun Grp, London, England. [Korber, Bette T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Nunes, Alexandra; Gomes, Joao Paulo] Natl Inst Hlth, Dept Infect Dis, Lisbon, Portugal. [Follmann, Frank] Statens Serum Inst, Dept Infect Dis Immunol, Chlamydia Vaccine Res, DK-2300 Copenhagen, Denmark. [Badamchi-Zadeh, Alexander] Harvard Univ, Sch Med, Ctr Virol & Vaccine Res, Boston, MA USA. [Walters, Adam A.] Univ Oxford, Jenner Inst, Oxford, England. RP Shattock, RJ (reprint author), Univ London Imperial Coll Sci Technol & Med, Mucosal Infect & Immun Grp, London, England. EM r.shattock@imperial.ac.uk FU Wellcome Trust; European Community's European 7th Framework Program ADITEC [HEALTH-F4-2011-18 280873] FX AB was funded by the Wellcome Trust. RS was supported by the European Community's European 7th Framework Program ADITEC (HEALTH-F4-2011-18 280873). NR 57 TC 3 Z9 3 U1 0 U2 1 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-3224 J9 FRONT IMMUNOL JI Front. Immunol. PD APR 28 PY 2016 VL 7 AR 162 DI 10.3389/fimmu.2016.00162 PG 11 WC Immunology SC Immunology GA DK5ID UT WOS:000374952700001 PM 27199987 ER PT J AU Wuddineh, WA Mazarei, M Zhang, JY Turner, GB Sykes, RW Decker, SR Davis, MF Udvardi, MK Stewart, CN AF Wuddineh, Wegi A. Mazarei, Mitra Zhang, Ji-Yi Turner, Geoffrey B. Sykes, Robert W. Decker, Stephen R. Davis, Mark F. Udvardi, Michael K. Stewart, C. Neal, Jr. TI Identification and Overexpression of a Knotted1-Like Transcription Factorin Switchgrass (Panicum virgatum L.) for Lignocellulosic Feedstock Improvement SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE gene regulation; lignin; gibberellin; cell walls; cellulose; hemicellulose; sugar release; biofuel ID SECONDARY WALL BIOSYNTHESIS; MAIZE HOMEOBOX GENE; CELL-WALL; LIGNIN BIOSYNTHESIS; HIGH-THROUGHPUT; KNOX GENES; GIBBERELLIN METABOLISM; BIOMASS ACCUMULATION; FUNCTIONAL-ANALYSIS; TRANSGENIC TOBACCO AB High biomass production and wide adaptation has made switchgrass (Panicum virgatum L.) an important candidate lignocellulosic bioenergy crop. One major limitation of this and other lignocellulosic feedstocks is the recalcitrance of complex carbohydrates to hydrolysis for conversion to biofuels. Lignin is the major contributor to recalcitrance as it limits the accessibility of cell wall carbohydrates to enzymatic breakdown into fermentable sugars. Therefore, genetic manipulation of the lignin biosynthesis pathway is one strategy to reduce recalcitrance. Here, we identified a switchgrass Knotted1 transcription factor, PvKN1, with the aim of genetically engineering switchgrass for reduced biomass recalcitrance for biofuel production. Gene expression of the endogenous PvKN1 gene was observed to be highest in young inflorescences and stems. Ectopic overexpression of PvKN1 in switchgrass altered growth, especially in early developmental stages. Transgenic lines had reduced expression of most lignin biosynthetic genes accompanied by a reduction in lignin content suggesting the involvement of PvKN1 in the broad regulation of the lignin biosynthesis pathway. Moreover, the reduced expression of the Gibberellin 20-oxidase (GA20ox) gene in tandem with the increased expression of Gibberellin 2-oxidase (GA2ox) genes in transgenic PvKN1 lines suggest that PvKN1 may exert regulatory effects via modulation of GA signaling. Furthermore, overexpression of PvKN1 altered the expression of cellulose and hemicellulose biosynthetic genes and increased sugar release efficiency in transgenic lines. Our results demonstrated that switchgrass PvKN1 is a putative ortholog of maize KN1 that is linked to plant lignification and cell wall and development traits as a major regulatory gene. Therefore, targeted overexpression of PvKN1 in bioenergy feedstocks may provide one feasible strategy for reducing biomass recalcitrance and simultaneously improving plant growth characteristics. C1 [Wuddineh, Wegi A.; Mazarei, Mitra; Stewart, C. Neal, Jr.] Univ Tennessee, Dept Plant Sci, Knoxville, TN USA. [Wuddineh, Wegi A.; Mazarei, Mitra; Zhang, Ji-Yi; Turner, Geoffrey B.; Sykes, Robert W.; Decker, Stephen R.; Davis, Mark F.; Udvardi, Michael K.; Stewart, C. Neal, Jr.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA. [Zhang, Ji-Yi; Udvardi, Michael K.] Samuel Roberts Noble Fdn Inc, Div Plant Biol, Ardmore, OK USA. [Turner, Geoffrey B.; Sykes, Robert W.; Decker, Stephen R.; Davis, Mark F.] Natl Renewable Energy Lab, Golden, CO USA. [Zhang, Ji-Yi] Bayer AG, R&D Trait Res, Crop Sci Div, 2 TW Alexander Dr, Res Triangle Pk, NC USA. RP Stewart, CN (reprint author), Univ Tennessee, Dept Plant Sci, Knoxville, TN USA.; Stewart, CN (reprint author), Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA. EM nealstewart@utk.edu OI davis, mark/0000-0003-4541-9852 FU BioEnergy Science Center [DE-PS02-06ER64304]; Office of Biological and Environmental Research in the DOE Office of Science; Tennessee Agricultural Experiment Station FX This work was supported by funding from the BioEnergy Science Center (DE-PS02-06ER64304). The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. We also thank Tennessee Agricultural Experiment Station for providing partial financial support for WW. We also thank DOE-JGI for the prepublication access to the switchgrass genome. NR 85 TC 0 Z9 0 U1 10 U2 22 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD APR 28 PY 2016 VL 7 AR 520 DI 10.3389/fpls.2016.00520 PG 15 WC Plant Sciences SC Plant Sciences GA DK5AC UT WOS:000374930800001 PM 27200006 ER PT J AU Kruiswijk, F Hasenfuss, SC Sivapatham, R Baar, MP Putavet, D Naipal, KAT van den Broek, NJF Kruit, W van der Spek, PJ van Gent, DC Brenkman, AB Campisi, J Burgering, BMT Hoeijmakers, JHJ de Keizer, PLJ AF Kruiswijk, F. Hasenfuss, S. C. Sivapatham, R. Baar, M. P. Putavet, D. Naipal, K. A. T. van den Broek, N. J. F. Kruit, W. van der Spek, P. J. van Gent, D. C. Brenkman, A. B. Campisi, J. Burgering, B. M. T. Hoeijmakers, J. H. J. de Keizer, P. L. J. TI Targeted inhibition of metastatic melanoma through interference with Pin1-FOXM1 signaling SO ONCOGENE LA English DT Article ID MEK INHIBITION; TRANSCRIPTION FACTORS; MELANOCYTIC LESIONS; TUMOR PROGRESSION; IMPROVED SURVIVAL; MITOTIC PROGRAM; BRAF; FOXM1; EXPRESSION; GENE AB Melanoma is the most lethal form of skin cancer and successful treatment of metastatic melanoma remains challenging. BRAF/MEK inhibitors only show a temporary benefit due to rapid occurrence of resistance, whereas immunotherapy is mainly effective in selected subsets of patients. Thus, there is a need to identify new targets to improve treatment of metastatic melanoma. To this extent, we searched for markers that are elevated in melanoma and are under regulation of potentially druggable enzymes. Here, we show that the pro-proliferative transcription factor FOXM1 is elevated and activated in malignant melanoma. FOXM1 activity correlated with expression of the enzyme Pin1, which we found to be indicative of a poor prognosis. In functional experiments, Pin1 proved to be a main regulator of FOXM1 activity through MEK-dependent physical regulation during the cell cycle. The Pin1-FOXM1 interaction was enhanced by BRAF(V600E), the driver oncogene in the majority of melanomas, and in extrapolation of the correlation data, interference with\Pin1 in BRAF(V600E)-driven metastatic melanoma cells impaired both FOXM1 activity and cell survival. Importantly, cell-permeable Pin1-FOXM1-blocking peptides repressed the proliferation of melanoma cells in freshly isolated human metastatic melanoma ex vivo and in three-dimensional-cultured patient-derived melanoids. When combined with the BRAF(V600) Einhibitor PLX4032 a robust repression in melanoid viability was obtained, establishing preclinical value of patient-derived melanoids for prognostic use of drug sensitivity and further underscoring the beneficial effect of Pin1-FOXM1 inhibitory peptides as anti-melanoma drugs. These proof-of-concept results provide a starting point for development of therapeutic Pin1-FOXM1 inhibitors to target metastatic melanoma. C1 [Kruiswijk, F.; Hasenfuss, S. C.; van den Broek, N. J. F.; Brenkman, A. B.; Burgering, B. M. T.; de Keizer, P. L. J.] Univ Med Ctr, Ctr Mol Med, Mol Canc Res, Utrecht, Netherlands. [Sivapatham, R.; Campisi, J.; de Keizer, P. L. J.] Buck Inst Res Aging, Novato, CA USA. [Baar, M. P.; Putavet, D.; Naipal, K. A. T.; van Gent, D. C.; Hoeijmakers, J. H. J.; de Keizer, P. L. J.] Erasmus Med Ctr Rotterdam, Dept Genet, Wytemaweg 80,POB 2040, NL-3000 CA Rotterdam, Netherlands. [Kruit, W.] Erasmus Med Ctr Rotterdam, Dept Med Oncol, Rotterdam, Netherlands. [van der Spek, P. J.] Erasmus Med Ctr Rotterdam, Dept Bioinformat, Rotterdam, Netherlands. [Brenkman, A. B.] Univ Med Ctr, Dept Metab & Endocrine Dis, Utrecht, Netherlands. [Campisi, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP de Keizer, PLJ (reprint author), Erasmus Med Ctr Rotterdam, Dept Genet, Wytemaweg 80,POB 2040, NL-3000 CA Rotterdam, Netherlands. EM p.dekeizer@erasmusmc.nl FU NIH [R37-AG009909]; NIH/NIA [AG-17242-02]; KNAW; ERC; FP7 framework [HEALTH-F2-2010-259893]; Dutch Cancer Society [Buit-4649]; EMCR [2014-7141]; Erasmus Medical Center Rotterdam: EMC fellowship; CGC FX We would like to gratefully acknowledge Dr Richard Marais for material from BRAFV600E-inducible mice, Dr Hugo Snippert and Dr Rene Overmeer for advice on organoid culture and Dr Jamila Laoukili and Dr Rene Medema for general advice on FOXM1 signaling. This work has been supported by grants from the NIH: R37-AG009909 (JC), CGC (BB), NIH/NIA: AG-17242-02 (JC/JH), KNAW (JH), ERC (JH), FP7 framework HEALTH-F2-2010-259893 (JH), the Dutch Cancer Society: Buit-4649 (PDK), EMCR 2014-7141 (PDK) and the Erasmus Medical Center Rotterdam: 2013 EMC fellowship (PDK). NR 47 TC 4 Z9 4 U1 4 U2 7 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0950-9232 EI 1476-5594 J9 ONCOGENE JI Oncogene PD APR 28 PY 2016 VL 35 IS 17 BP 2166 EP 2177 DI 10.1038/onc.2015.282 PG 12 WC Biochemistry & Molecular Biology; Oncology; Cell Biology; Genetics & Heredity SC Biochemistry & Molecular Biology; Oncology; Cell Biology; Genetics & Heredity GA DK5UK UT WOS:000374986000003 PM 26279295 ER PT J AU Malliakas, CD Leung, K Pupek, KZ Shkrob, IA Abraham, DP AF Malliakas, Christos D. Leung, Kevin Pupek, Krzysztof Z. Shkrob, Ilya A. Abraham, Daniel P. TI Spontaneous aggregation of lithium ion coordination polymers in fluorinated electrolytes for high-voltage batteries SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS; FLUOROETHYLENE CARBONATE; PROPYLENE CARBONATE; SOLVATE STRUCTURES; CHEMISTRY; GRAPHITE; LIPF6 AB Fluorinated carbonates are pursued as liquid electrolyte solvents for high-voltage Li-ion batteries. Here we report aggregation of [Li+(FEC)(3)](n) polymer species in fluoroethylene carbonate containing electrolytes and scrutinize the causes for this behavior. C1 [Malliakas, Christos D.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Malliakas, Christos D.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Leung, Kevin] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Pupek, Krzysztof Z.] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Pupek, Krzysztof Z.] Argonne Natl Lab, Mat Engn Res Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. [Shkrob, Ilya A.; Abraham, Daniel P.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Shkrob, IA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM Shkrob@anl.gov FU US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC02-06CH11357]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This work was supported by the US-DOE Office of Science, Division of Chemical Sciences, Geosciences and Biosciences under contracts No. DE-AC02-06CH11357 to Argonne. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne''). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract DE-AC02-06CH11357. NR 29 TC 5 Z9 5 U1 12 U2 35 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 28 PY 2016 VL 18 IS 16 BP 10846 EP 10849 DI 10.1039/c6cp01157h PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK3AD UT WOS:000374786300020 PM 27040896 ER PT J AU Parkes, MV Greathouse, JA Hart, DB Sava Gallis, DF Nenoff, TM AF Parkes, Marie V. Greathouse, Jeffery A. Hart, David B. Sava Gallis, Dorina F. Nenoff, Tina M. TI Ab initio molecular dynamics determination of competitive O-2 vs. N-2 adsorption at open metal sites of M-2(dobdc) SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID HIGHLY SELECTIVE ADSORPTION; IRON(II) COORDINATION SITES; ORGANIC FRAMEWORK MATERIALS; WAALS DENSITY FUNCTIONALS; HYDROGEN STORAGE; GAS-ADSORPTION; RATIONAL DESIGN; CO2 ADSORPTION; SEPARATION; WATER AB The separation of oxygen from nitrogen using metal-organic frameworks (MOFs) is of great interest for potential pressure-swing adsorption processes for the generation of purified O-2 on industrial scales. This study uses ab initio molecular dynamics (AIMD) simulations to examine for the first time the pure-gas and competitive gas adsorption of O-2 and N-2 in the M-2(dobdc) (M = Cr, Mn, Fe) MOF series with coordinatively unsaturated metal centers. Effects of metal, temperature, and gas composition are explored. This unique application of AIMD allows us to study in detail the adsorption/desorption processes and to visualize the process of multiple guests competitively binding to coordinatively unsaturated metal sites of a MOF. C1 [Parkes, Marie V.; Greathouse, Jeffery A.; Hart, David B.] Sandia Natl Labs, Geochem Dept, POB 5800, Albuquerque, NM 87185 USA. [Sava Gallis, Dorina F.] Sandia Natl Labs, Nanoscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. [Nenoff, Tina M.] Sandia Natl Labs, Phys Chem & Nano Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. RP Nenoff, TM (reprint author), Sandia Natl Labs, Phys Chem & Nano Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM tmnenof@sandia.gov RI Sava Gallis, Dorina/D-2827-2015 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia's Laboratory Directed Research and Development program FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This research was funded by Sandia's Laboratory Directed Research and Development program. NR 90 TC 2 Z9 2 U1 7 U2 17 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 28 PY 2016 VL 18 IS 16 BP 11528 EP 11538 DI 10.1039/c6cp00768f PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK3AD UT WOS:000374786300096 PM 27063148 ER PT J AU Checchin, M Martinello, M Romanenko, A Grassellino, A Sergatskov, DA Posen, S Melnychuk, O Zasadzinski, JF AF Checchin, M. Martinello, M. Romanenko, A. Grassellino, A. Sergatskov, D. A. Posen, S. Melnychuk, O. Zasadzinski, J. F. TI Quench-Induced Degradation of the Quality Factor in Superconducting Resonators SO PHYSICAL REVIEW APPLIED LA English DT Article ID RADIOFREQUENCY CAVITIES AB Quench of superconducting radio-frequency cavities frequently leads to the lowered quality factor Q(0), which had been attributed to the additional trapped magnetic flux. Here we demonstrate that the origin of this magnetic flux is purely extrinsic to the cavity by showing no extra dissipation (unchanged Q(0)) after quenching in zero magnetic field, which allows us to rule out intrinsic mechanisms of flux trapping such as generation of thermal currents or trapping of the rf field. We also show the clear relation of dissipation introduced by quenching to the orientation of the applied magnetic field and the possibility to fully recover the quality factor by requenching in the compensated field. We discover that for larger values of the ambient field, the Q-factor degradation may become irreversible by this technique, likely due to the outward flux migration beyond the normal zone opening during quench. Our findings are of special practical importance for accelerators based on low- and medium-beta accelerating structures residing close to focusing magnets, as well as for all high-Q cavity-based accelerators. C1 [Checchin, M.; Martinello, M.; Romanenko, A.; Grassellino, A.; Sergatskov, D. A.; Posen, S.; Melnychuk, O.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Checchin, M.; Martinello, M.; Zasadzinski, J. F.] IIT, Dept Phys, Chicago, IL 60616 USA. RP Checchin, M (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.; Checchin, M (reprint author), IIT, Dept Phys, Chicago, IL 60616 USA. EM checchin@fnal.gov FU United States Department of Energy [DE-AC02-07CH11359]; DOE HEP Early Career Grant; DOE NP Early Career Grant FX Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. The work is supported by the DOE HEP Early Career Grant of A. Grassellino, and DOE NP Early Career Grant of A. Romanenko. NR 26 TC 1 Z9 1 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD APR 28 PY 2016 VL 5 IS 4 AR 044019 DI 10.1103/PhysRevApplied.5.044019 PG 11 WC Physics, Applied SC Physics GA DK5NK UT WOS:000374966400003 ER PT J AU Morozovska, AN Ievlev, AV Obukhovskii, VV Fomichov, Y Varenyk, OV Shur, VY Kalinin, SV Eliseev, EA AF Morozovska, Anna N. Ievlev, Anton V. Obukhovskii, Vyacheslav V. Fomichov, Yevhen Varenyk, Oleksandr V. Shur, Vladimir Ya. Kalinin, Sergei V. Eliseev, Eugene A. TI Self-consistent theory of nanodomain formation on nonpolar surfaces of ferroelectrics SO PHYSICAL REVIEW B LA English DT Article ID ATOMIC-FORCE MICROSCOPE; LITHIUM-NIOBATE; DOMAIN-WALLS; POLARIZATION REVERSAL; PB(ZR,TI)O-3; DIFFRACTION; MECHANISM; DYNAMICS; MOTION; LINBO3 AB We propose a self-consistent theoretical approach capable of describing the features of the anisotropic nanodomain formation induced by a strongly inhomogeneous electric field of a charged scanning probe microscopy tip on nonpolar cuts of ferroelectrics. We obtained that a threshold field, previously regarded as an isotropic parameter, is an anisotropic function that is specified from the polar properties and lattice pinning anisotropy of a given ferroelectric in a self-consistent way. The proposed method for the calculation of the anisotropic threshold field is not material specific, thus the field should be anisotropic in all ferroelectrics with the spontaneous polarization anisotropy along the main crystallographic directions. The most evident examples are uniaxial ferroelectrics, layered ferroelectric perovskites, and low-symmetry incommensurate ferroelectrics. Obtained results quantitatively describe the differences at several times in the nanodomain length experimentally observed on X and Y cuts of LiNbO3 and can give insight into the anisotropic dynamics of nanoscale polarization reversal in strongly inhomogeneous electric fields. C1 [Morozovska, Anna N.; Varenyk, Oleksandr V.] Natl Acad Sci Ukraine, Inst Phys, 46 Pr Nauky, UA-03028 Kiev, Ukraine. [Ievlev, Anton V.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Ievlev, Anton V.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Obukhovskii, Vyacheslav V.] Taras Shevchenko Kyiv Natl Univ, Radiophys Fac 4g, UA-03022 Kiev, Ukraine. [Fomichov, Yevhen; Eliseev, Eugene A.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, 3 Krjijanovskogo, UA-03142 Kiev, Ukraine. [Shur, Vladimir Ya.] Ural Fed Univ, Inst Nat Sci, 51 Lenin Ave, Ekaterinburg 620000, Russia. RP Morozovska, AN (reprint author), Natl Acad Sci Ukraine, Inst Phys, 46 Pr Nauky, UA-03028 Kiev, Ukraine.; Eliseev, EA (reprint author), Natl Acad Sci Ukraine, Inst Problems Mat Sci, 3 Krjijanovskogo, UA-03142 Kiev, Ukraine. EM anna.n.morozovska@gmail.com; eugene.a.eliseev@gmail.com RI Ievlev, Anton/H-3678-2012 OI Ievlev, Anton/0000-0003-3645-0508 FU National Academy of Sciences of Ukraine [35-02-15]; RFBR [14-02-90447 Ukr-a]; DOE Office of the Science [CNMS2016-061] FX E.A.E. and A.N.M. acknowledge the National Academy of Sciences of Ukraine (Grant No. 35-02-15). V.Y.S. acknowledges RFBR (Grant No. 14-02-90447 Ukr-a). A portion of this research (A.V.I, S.V.K.) was conducted at the Center for Nanophase Materials Sciences (Project No. CNMS2016-061), which is a DOE Office of the Science User Facility. A.N.M. formulated and elaborated the theoretical model, derived the corresponding analytical expressions, and wrote the initial text of the paper with illustrations. A.I. performed the corresponding numerical simulations of the domain shapes and sizes in COMSOL, the numerical results processing and smoothing jointly with O.V.V. Y.M.F. performed the fitting of the COMSOL results by interpolation functions. E.A.E. densely worked on the improvement of the anisotropic threshold field model and correlation with experiment of the obtained theoretical results. A.N.M., A.V.I., V.V.O, V.Y.S., S.V.K. and E.A.E. worked on the physical interpretation of the obtained theoretical results, improvement of the paper text, discussion, and conclusions. NR 54 TC 0 Z9 0 U1 5 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 28 PY 2016 VL 93 IS 16 AR 165439 DI 10.1103/PhysRevB.93.165439 PG 10 WC Physics, Condensed Matter SC Physics GA DK5IE UT WOS:000374952800007 ER PT J AU Randeria, MT Feldman, BE Drozdov, IK Yazdani, A AF Randeria, Mallika T. Feldman, Benjamin E. Drozdov, Ilya K. Yazdani, Ali TI Scanning Josephson spectroscopy on the atomic scale SO PHYSICAL REVIEW B LA English DT Article ID C SUPERCONDUCTOR BI2SR2CACU2O8+DELTA; LOCAL ELECTRONIC-STRUCTURE; MAGNETIC-IMPURITIES; SPATIAL VARIATIONS; ORDER-PARAMETER; ENERGY GAPS; JUNCTIONS; SINGLE; STM AB The Josephson effect provides a direct method to probe the strength of the pairing interaction in superconductors. By measuring the phase fluctuating Josephson current between a superconducting tip of a scanning tunneling microscope and a BCS superconductor with isolated magnetic adatoms on its surface, we demonstrate that the spatial variation of the pairing order parameter can be characterized on the atomic scale. This system provides an example where the local pairing potential suppression is not directly reflected in the spectra measured via quasiparticle tunneling. Spectroscopy with such superconducting tips also shows signatures of previously unexplored Andreev processes through individual impurity-bound Shiba states. The atomic resolution achieved here establishes scanning Josephson spectroscopy as a promising technique for the study of novel superconducting phases. C1 [Yazdani, Ali] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Drozdov, Ilya K.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Yazdani, A (reprint author), Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. EM yazdani@princeton.edu FU Gordon and Betty Moore Foundation as part of EPiQS initiative [GBMF4530]; DOE-BES; NSF-MRSEC programs through the Princeton Center for Complex Materials [DMR-1420541]; NSF; [NSF-DMR-1104612]; [ARO-W911NF-1-0262]; [ONR-N00014-14-1-0330]; [ONR-N00014-13-10661]; [N6601-11-1-4110]; [ARO-W911NF-1-0606] FX We would like to thank J. Li, B. Jack, and F. Pientka for valuable discussions. This work has been supported by the Gordon and Betty Moore Foundation as part of EPiQS initiative (GBMF4530) and DOE-BES. This project was also made possible using the facilities at Princeton Nanoscale Microscopy Laboratory supported by Grants No. NSF-DMR-1104612, No. ARO-W911NF-1-0262, No. ONR-N00014-14-1-0330, No. ONR-N00014-13-10661, DARPA-SPWAR Meso program N6601-11-1-4110, LPS and ARO-W911NF-1-0606, and NSF-MRSEC programs through the Princeton Center for Complex Materials DMR-1420541. M.T.R. acknowledges support from the NSF Graduate Research Fellowship Program. NR 43 TC 1 Z9 1 U1 8 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 28 PY 2016 VL 93 IS 16 AR 161115 DI 10.1103/PhysRevB.93.161115 PG 5 WC Physics, Condensed Matter SC Physics GA DK5IE UT WOS:000374952800002 ER PT J AU Wang, JC Ye, F Chi, SX Fernandez-Baca, JA Cao, HB Tian, W Gooch, M Poudel, N Wang, YQ Lorenz, B Chu, CW AF Wang, Jinchen Ye, Feng Chi, Songxue Fernandez-Baca, Jaime A. Cao, Huibo Tian, Wei Gooch, M. Poudel, N. Wang, Yaqi Lorenz, Bernd Chu, C. W. TI Pressure effects on magnetic ground states in cobalt-doped multiferroic Mn1-xCoxWO4 SO PHYSICAL REVIEW B LA English DT Article ID POLARIZATION; MNWO4; FERROELECTRICITY AB Using ambient pressure x-ray and high pressure neutron diffraction, we studied the pressure effect on structural and magnetic properties of multiferroic Mn1-xCoxWO4 single crystals (x = 0, 0.05, 0.135, and 0.17) and compared it with the effects of doping. Both Co doping and pressure stretch the Mn-Mn chain along the c direction. At high doping level (x = 0.135 and 0.17), pressure and Co doping drive the system in a similar way and induce a spin-flop transition for the x = 0.135 compound. In contrast, magnetic ground states at lower doping level (x = 0 and 0.05) are robust against pressure but experience a pronounced change upon Co substitution. As Co introduces both chemical pressure and magnetic anisotropy into the frustrated magnetic system, our results suggest the magnetic anisotropy is the main driving force for the Co induced phase transitions at low doping level, and chemical pressure plays a more significant role at higher Co concentrations. C1 [Wang, Jinchen] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Wang, Jinchen; Ye, Feng] Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. [Wang, Jinchen; Ye, Feng; Chi, Songxue; Fernandez-Baca, Jaime A.; Cao, Huibo; Tian, Wei] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Fernandez-Baca, Jaime A.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Gooch, M.; Poudel, N.; Wang, Yaqi; Lorenz, Bernd; Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Gooch, M.; Poudel, N.; Wang, Yaqi; Lorenz, Bernd; Chu, C. W.] Univ Houston, TCSUH, Houston, TX 77204 USA. [Chu, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Ye, F (reprint author), Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA.; Ye, F (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM yef1@ornl.gov RI Ye, Feng/B-3210-2010; SNS, Corelli/O-8443-2015; Fernandez-Baca, Jaime/C-3984-2014; Chi, Songxue/A-6713-2013; Tian, Wei/C-8604-2013 OI Ye, Feng/0000-0001-7477-4648; SNS, Corelli/0000-0001-5563-3292; Fernandez-Baca, Jaime/0000-0001-9080-5096; Chi, Songxue/0000-0002-3851-9153; Tian, Wei/0000-0001-7735-3187 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; T.L.L. Temple Foundation; John J. and Rebecca Moores Endowment; State of Texas through TCSUH; US Air Force Office of Scientific Research [FA9550-09-1-0656]; China Scholarship Council FX Research at ORNL's HFIR and SNS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Work at Houston is supported in part by the T.L.L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through TCSUH, the US Air Force Office of Scientific Research, Award No. FA9550-09-1-0656. J.C.W. acknowledges support from China Scholarship Council. NR 49 TC 0 Z9 0 U1 9 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 28 PY 2016 VL 93 IS 15 AR 155164 DI 10.1103/PhysRevB.93.155164 PG 5 WC Physics, Condensed Matter SC Physics GA DK5GT UT WOS:000374949000002 ER PT J AU Kovarik, K Kusina, A Jezo, T Clark, DB Keppel, C Lyonnet, F Morfin, JG Olness, FI Owens, JF Schienbein, I Yu, JY AF Kovarik, K. Kusina, A. Jezo, T. Clark, D. B. Keppel, C. Lyonnet, F. Morfin, J. G. Olness, F. I. Owens, J. F. Schienbein, I. Yu, J. Y. TI nCTEQ15: Global analysis of nuclear parton distributions with uncertainties in the CTEQ framework SO PHYSICAL REVIEW D LA English DT Article ID INELASTIC MUON SCATTERING; STRUCTURE-FUNCTION RATIOS; TO-LEADING-ORDER; FRAGMENTATION FUNCTIONS; ELECTRON-SCATTERING; DIMUON PRODUCTION; CROSS-SECTIONS; HEAVY QUARKS; IRON TARGETS; DEUTERIUM AB We present the new nCTEQ15 set of nuclear parton distribution functions (PDFs) with uncertainties. This fit extends the CTEQ proton PDFs to include the nuclear dependence using data on nuclei all the way up to Pb-208. The uncertainties are determined using the Hessian method with an optimal rescaling of the eigenvectors to accurately represent the uncertainties for the chosen tolerance criteria. In addition to the deep inelastic scattering and Drell-Yan processes, we also include inclusive pion production data from the Relativistic Heavy Ion Collider to help constrain the nuclear gluon PDF. Furthermore, we investigate the correlation of the data sets with specific nuclear PDF flavor components and asses the impact of individual experiments. We also provide comparisons of the nCTEQ15 set with recent fits from other groups. C1 [Kovarik, K.] Univ Munster, Inst Theoret Phys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. [Kusina, A.; Schienbein, I.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, 53 Ave Martyrs, F-38026 Grenoble, France. [Jezo, T.] Univ Milano Bicocca, Piazza Sci 3, I-20126 Milan, Italy. [Jezo, T.] Ist Nazl Fis Nucl, Sez Milano Bicocca, Piazza Sci 3, I-20126 Milan, Italy. [Clark, D. B.; Lyonnet, F.; Olness, F. I.; Yu, J. Y.] So Methodist Univ, Dallas, TX 75275 USA. [Keppel, C.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Morfin, J. G.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Owens, J. F.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. RP Kovarik, K (reprint author), Univ Munster, Inst Theoret Phys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. FU DOE [DE-FG02-13ER41942]; Research Executive Agency of the European Union [PITN-GA-2010-264564]; U.S. Department of Energy [DE-FG02-13ER41996]; Projet International de Cooperation Scientifique [PICS05854]; Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy FX The authors would like to thank J. Gao for proposing the use of Delta chieff2 as an alternative to the correlation cosine and for other useful discussions. Furthermore, we would like to thank M. Botje, E. Godat, S. Kumano, P. Nadolsky, and V. Radescu for valuable discussions. We acknowledge the hospitality of CERN, DESY, and Fermilab where a portion of this work was performed. The work of J. F. O. was supported by the DOE under Grant No. DE-FG02-13ER41942. T. J. was partly supported by the Research Executive Agency of the European Union under Grant No. PITN-GA-2010-264564 (LHCPhenoNet). This work was also partially supported by the U.S. Department of Energy under Grant No. DE-FG02-13ER41996 and by Projet International de Cooperation Scientifique PICS05854 between France, and the U.S. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 85 TC 7 Z9 7 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 28 PY 2016 VL 93 IS 8 AR 085037 DI 10.1103/PhysRevD.93.085037 PG 34 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK5LF UT WOS:000374960700007 ER PT J AU Mace, M Schlichting, S Venugopalan, R AF Mace, Mark Schlichting, Soeren Venugopalan, Raju TI Off-equilibrium sphaleron transitions in the glasma SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; ENERGY NUCLEAR COLLISIONS; NUMBER NON-CONSERVATION; WEINBERG-SALAM THEORY; CHERN-SIMONS NUMBER; TOPOLOGICAL CHARGE; GAUGE-THEORIES; REAL-TIME; LATTICE; VIOLATION AB We perform the first, to our knowledge, classical-statistical real time lattice simulations of topological transitions in the nonequilibrium glasma of weakly coupled but highly occupied gauge fields created immediately after the collision of ultrarelativistic nuclei. Simplifying our description by employing SU(2) gauge fields, and neglecting their longitudinal expansion, we find that the rate of topological transitions is initially strongly enhanced relative to the thermal sphaleron transition rate and decays with time during the thermalization process. Qualitative features of the time dependence of this nonequilibrium transition rate can be understood when expressed in terms of the magnetic screening length, which we also extract nonperturbatively. A detailed investigation of autocorrelation functions of the Chern-Simons number (N-CS) reveals non-Markovian features of the evolution distinct from previous simulations of non-Abelian plasmas in thermal equilibrium. C1 [Mace, Mark] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11973 USA. [Mace, Mark; Schlichting, Soeren; Venugopalan, Raju] Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. [Venugopalan, Raju] Heidelberg Univ, Inst Theoret Phys, Philosophenweg 16, D-69120 Heidelberg, Germany. RP Mace, M (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11973 USA.; Mace, M (reprint author), Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. FU DOE [DE-SC0012704]; Office of Science of U.S. Department of Energy [DEAC02-05CH11231]; Excellence Initiative of Heidelberg University; Brookhaven Science Associates FX We would like to thank Peter Arnold, Jurgen Berges, Dima Kharzeev, Guy D. Moore, Alexander Rothkopf, and Sayantan Sharma for helpful discussions. S. S. and R. V. are supported under DOE Contract No. DE-SC0012704. This research used the resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DEAC02-05CH11231. M. M., S. S., and R. V. would like to thank the Institut fur Theoretische Physik at the Universitat Heidelberg for hospitality during the latter portion of this work. R. V. would like to thank the Excellence Initiative of Heidelberg University for their support. S. S. gratefully acknowledges a Goldhaber Distinguished Fellowship from Brookhaven Science Associates. NR 90 TC 5 Z9 5 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 28 PY 2016 VL 93 IS 7 AR 074036 DI 10.1103/PhysRevD.93.074036 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK5KH UT WOS:000374958300001 ER PT J AU Zablocki, A Dodelson, S AF Zablocki, Alan Dodelson, Scott TI Extreme data compression for the CMB SO PHYSICAL REVIEW D LA English DT Article ID MICROWAVE BACKGROUND DATA; PROBE WMAP OBSERVATIONS; PARAMETER-ESTIMATION; POWER SPECTRUM; GALAXY SPECTRA; DATA SETS; LIKELIHOOD AB We apply the Karhunen-Loeve methods to cosmic microwave background (CMB) data sets, and show that we can recover the input cosmology and obtain the marginalized likelihoods in. cold dark matter cosmologies in under a minute, much faster than Markov chain Monte Carlo methods. This is achieved by forming a linear combination of the power spectra at each multipole l, and solving a system of simultaneous equations such that the Fisher matrix is locally unchanged. Instead of carrying out a full likelihood evaluation over the whole parameter space, we need evaluate the likelihood only for the parameter of interest, with the data compression effectively marginalizing over all other parameters. The weighting vectors contain insight about the physical effects of the parameters on the CMB anisotropy power spectrum Cl. The shape and amplitude of these vectors give an intuitive feel for the physics of the CMB, the sensitivity of the observed spectrum to cosmological parameters, and the relative sensitivity of different experiments to cosmological parameters. We test this method on exact theory Cl as well as on a Wilkinson Microwave Anisotropy Probe (WMAP)-like CMB data set generated from a random realization of a fiducial cosmology, comparing the compression results to those from a full likelihood analysis using CosmoMC. After showing that the method works, we apply it to the temperature power spectrum from the WMAP seven-year data release, and discuss the successes and limitations of our method as applied to a real data set. C1 [Zablocki, Alan; Dodelson, Scott] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Zablocki, Alan; Dodelson, Scott] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Dodelson, Scott] Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. RP Zablocki, A (reprint author), Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Zablocki, A (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. FU Fermilab; Kavli Institute for Cosmological Physics; University of Chicago; KICP; Brinson Foundation; U.S. Department of Energy [DE-FG02-13ER41958, DE-FG02-95ER40896] FX The authors would like to thank the anonymous referee for the valuable comments on the manuscript. A. Z. would like to thank Wayne Hu for the useful discussions. This work was completed in part with resources provided by the University of Chicago Research Computing Center as well as the Joint Fermilab-KICP Supercomputing Cluster, supported by grants from Fermilab, the Kavli Institute for Cosmological Physics, and the University of Chicago. A. Z. acknowledges support from KICP, the Brinson Foundation and U.S. Department of Energy Contract No. DE-FG02-13ER41958. The work of S. D. is supported by the U.S. Department of Energy, including Grant No. DE-FG02-95ER40896. NR 25 TC 0 Z9 0 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 28 PY 2016 VL 93 IS 8 AR 083525 DI 10.1103/PhysRevD.93.083525 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK5LF UT WOS:000374960700003 ER PT J AU Ji, FH Shi, T Ye, M Wan, WS Liu, Z Wang, JJ Xu, T Qiao, S AF Ji, Fuhao Shi, Tan Ye, Mao Wan, Weishi Liu, Zhen Wang, Jiajia Xu, Tao Qiao, Shan TI Multichannel Exchange-Scattering Spin Polarimetry SO PHYSICAL REVIEW LETTERS LA English DT Article ID POLARIZATION ANALYZER; REFLECTION; ELECTRONS AB Electron spin plays important roles in determining the physical and chemical properties of matter. However, measurements of electron spin are of poor quality, impeding the development of material sciences, because the spin polarimeter has a low efficiency. Here, we show an imaging-type exchange-scattering spin polarimeter with 6786 channels and an 8.5 x 10(-3) single channel efficiency. As a demonstration, the fine spin structure of the electronic states in bismuth (111) is investigated, for which strong Rashba-type spin splitting behavior is seen in both the bulk and surface states. This improvement paves the way to study novel spin related phenomena with unprecedented accuracy. C1 [Ye, Mao; Qiao, Shan] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, 865 Changning Rd, Shanghai 200050, Peoples R China. [Ji, Fuhao; Shi, Tan; Liu, Zhen] Fudan Univ, Adv Mat Lab, Dept Phys, 2005 Songhu Rd, Shanghai 200438, Peoples R China. [Ji, Fuhao; Shi, Tan; Liu, Zhen] Fudan Univ, Surface Phys Lab, Natl Key Lab, 2005 Songhu Rd, Shanghai 200438, Peoples R China. [Wan, Weishi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Wang, Jiajia; Xu, Tao; Qiao, Shan] ShanghaiTech Univ, Sch Phys Sci & Technol, 319 Yueyang Rd, Shanghai 200031, Peoples R China. RP Qiao, S (reprint author), Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, 865 Changning Rd, Shanghai 200050, Peoples R China.; Qiao, S (reprint author), ShanghaiTech Univ, Sch Phys Sci & Technol, 319 Yueyang Rd, Shanghai 200031, Peoples R China. EM qiaoshan@mail.sim.ac.cn FU National Natural Science Foundation of China [10979021, 11027401, 11174054, 11304338, 11227902]; Ministry of Science and Technology of China [2011CB921800]; Chinese Academy of Sciences [XDB04010100]; Helmholtz Association through the Virtual Institute for Topological Insulators FX We wish to express our gratitude to J. Kirschner of the Max Planck Institute of Microstructure Physics for enlightening discussions on the Stoner excitation. We also gratefully acknowledge T. Okuda of Hiroshima University for discussions on the preparation of the ferromagnetic targets. This work was supported by the National Natural Science Foundation of China (Grants No. 10979021, No. 11027401, No. 11174054, No. 11304338, and No. 11227902), the Ministry of Science and Technology of China (National Basic Research Program Grant No. 2011CB921800), the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No. XDB04010100), and the Helmholtz Association through the Virtual Institute for Topological Insulators. NR 27 TC 3 Z9 3 U1 9 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 28 PY 2016 VL 116 IS 17 AR 177601 DI 10.1103/PhysRevLett.116.177601 PG 5 WC Physics, Multidisciplinary SC Physics GA DK5MW UT WOS:000374965000012 PM 27176539 ER PT J AU Zou, L Zhao, HH Zhang, HB AF Zou, Ling Zhao, Haihua Zhang, Hongbin TI Solving phase appearance/disappearance two-phase flow problems with high resolution staggered grid and fully implicit schemes by the Jacobian-free Newton-Krylov Method SO COMPUTERS & FLUIDS LA English DT Article DE Two-Phase Flow; Jacobian-free Newton-Krylov method; High-resolution spatial discretization; scheme; Phase disappearing; Implicit ID MODEL; IMPLEMENTATION AB The phase appearance/disappearance issue presents serious numerical challenges in two-phase flow simulations. Although many existing nuclear reactor safety analysis codes use different kinds of treatments for the phase appearance/disappearance problem, there are no fully consensual solutions. In this paper, a high-resolution spatial discretization scheme on staggered grid mesh and fully implicit time integration methods was used in two-phase flow simulations. Numerical treatments of the momentum equations were introduced for the disappearing phase without the need to use a cut-off value on void fraction. A discretized nonlinear system was solved using the Jacobian-free Newton Krylov (JFNK) method, which does not require expensive and error-prone derivation and implementation of analytical Jacobian matrix. These methods were tested with several two-phase flow problems with phase appearance/disappearance phenomena considered, such as a linear advection problem, an oscillating manometer problem, and a sedimentation problem. The combined methods demonstrated extremely robust and stable behaviors in solving the one-dimensional two-phase flow problems with phase appearance/disappearance. High resolution spatial discretization and second-order fully implicit method also demonstrated their capabilities in significantly reducing numerical errors. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Zou, Ling; Zhao, Haihua; Zhang, Hongbin] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. RP Zou, L (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM ling.zou@inl.gov OI Zou, Ling/0000-0003-0664-0474 FU U.S. Department of Energy, under Department of Energy Idaho Operations Office [DE-AC07-051D14517] FX This work is supported by the U.S. Department of Energy, under Department of Energy Idaho Operations Office Contract DE-AC07-051D14517. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 30 TC 2 Z9 2 U1 0 U2 0 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD APR 28 PY 2016 VL 129 BP 179 EP 188 DI 10.1016/j.compfluid.2016.02.008 PG 10 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA DK0OW UT WOS:000374613100013 ER PT J AU Haley, CAL AF Haley, Charlotte A. L. TI Glitches in time SO NATURE LA English DT Editorial Material C1 [Haley, Charlotte A. L.] Argonne Natl Lab, Math & Comp Sci Div, Lemont, IL 60439 USA. RP Haley, CAL (reprint author), Argonne Natl Lab, Math & Comp Sci Div, Lemont, IL 60439 USA. EM haley@anl.gov NR 10 TC 0 Z9 0 U1 4 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD APR 28 PY 2016 VL 532 IS 7600 BP 450 EP 451 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK3KQ UT WOS:000374815900035 PM 27121837 ER PT J AU Ye, CX Zhou, XL Pu, D Stutz, J Festa, J Spolaor, M Tsai, C Cantrell, C Mauldin, RL Campos, T Weinheimer, A Hornbrook, RS Apel, EC Guenther, A Kaser, L Yuan, B Karl, T Haggerty, J Hall, S Ullmann, K Smith, JN Ortega, J Knote, C AF Ye, Chunxiang Zhou, Xianliang Pu, Dennis Stutz, Jochen Festa, James Spolaor, Max Tsai, Catalina Cantrell, Christopher Mauldin, Roy L., III Campos, Teresa Weinheimer, Andrew Hornbrook, Rebecca S. Apel, Eric C. Guenther, Alex Kaser, Lisa Yuan, Bin Karl, Thomas Haggerty, Julie Hall, Samuel Ullmann, Kirk Smith, James N. Ortega, John Knote, Christoph TI Rapid cycling of reactive nitrogen in the marine boundary layer SO NATURE LA English DT Article ID VOLATILE ORGANIC-COMPOUNDS; MASTER CHEMICAL MECHANISM; NITRIC-ACID PHOTOLYSIS; MCM V3 PART; TROPOSPHERIC DEGRADATION; PHOTOCHEMICAL PRODUCTION; FOREST CANOPY; AIR-QUALITY; DUST STORM; GAS-PHASE AB Nitrogen oxides are essential for the formation of secondary atmospheric aerosols and of atmospheric oxidants such as ozone and the hydroxyl radical, which controls the self-cleansing capacity of the atmosphere(1). Nitric acid, a major oxidation product of nitrogen oxides, has traditionally been considered to be a permanent sink of nitrogen oxides(1). However, model studies predict higher ratios of nitric acid to nitrogen oxides in the troposphere than are observed(2,3). A 'renoxification' process that recycles nitric acid into nitrogen oxides has been proposed to reconcile observations with model studies(2-4), but the mechanisms responsible for this process remain uncertain(5-9). Here we present data from an aircraft measurement campaign over the North Atlantic Ocean and find evidence for rapid recycling of nitric acid to nitrous acid and nitrogen oxides in the clean marine boundary layer via particulate nitrate photolysis. Laboratory experiments further demonstrate the photolysis of particulate nitrate collected on filters at a rate more than two orders of magnitude greater than that of gaseous nitric acid, with nitrous acid as the main product. Box model calculations based on the Master Chemical Mechanism(10,11) suggest that particulate nitrate photolysis mainly sustains the observed levels of nitrous acid and nitrogen oxides at midday under typical marine boundary layer conditions. Given that oceans account for more than 70 per cent of Earth's surface, we propose that particulate nitrate photolysis could be a substantial tropospheric nitrogen oxide source. Recycling of nitrogen oxides in remote oceanic regions with minimal direct nitrogen oxide emissions could increase the formation of tropospheric oxidants and secondary atmospheric aerosols on a global scale. C1 [Ye, Chunxiang; Zhou, Xianliang] New York State Dept Hlth, Wadsworth Ctr, Albany, NY USA. [Zhou, Xianliang; Pu, Dennis] SUNY Albany, Dept Environm Hlth Sci, Albany, NY 12222 USA. [Stutz, Jochen; Festa, James; Spolaor, Max; Tsai, Catalina] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90024 USA. [Cantrell, Christopher; Mauldin, Roy L., III] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Mauldin, Roy L., III] Univ Helsinki, Dept Phys, Helsinki, Finland. [Campos, Teresa; Weinheimer, Andrew; Hornbrook, Rebecca S.; Apel, Eric C.; Kaser, Lisa; Haggerty, Julie; Hall, Samuel; Ullmann, Kirk; Smith, James N.; Ortega, John; Knote, Christoph] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Guenther, Alex] Pacific NW Natl Lab, Richland, WA 99352 USA. [Yuan, Bin] NOAA, Earth Syst Res Lab, Div Chem Sci, Boulder, CO USA. [Yuan, Bin] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Karl, Thomas] Univ Innsbruck, Inst Meteorol & Geophys, A-6020 Innsbruck, Austria. [Smith, James N.] Univ Eastern Finland, Kuopio, Finland. [Knote, Christoph] Univ Munich, Inst Meteorol, Marchioninistr 15, D-81377 Munich, Germany. RP Zhou, XL (reprint author), New York State Dept Hlth, Wadsworth Ctr, Albany, NY USA.; Zhou, XL (reprint author), SUNY Albany, Dept Environm Hlth Sci, Albany, NY 12222 USA. EM xianliang.zhou@health.ny.gov RI Smith, James/C-5614-2008; Karl, Thomas/D-1891-2009; Yuan, Bin/A-1223-2012; Knote, Christoph/A-9809-2010; Manager, CSD Publications/B-2789-2015 OI Smith, James/0000-0003-4677-8224; Karl, Thomas/0000-0003-2869-9426; Yuan, Bin/0000-0003-3041-0329; Knote, Christoph/0000-0001-9105-9179; FU National Science Foundation (NSF) [AGS-1216166, AGS-1215712, AGS-1216743]; National Science Foundation FX This research is funded by National Science Foundation (NSF) grants (AGS-1216166, AGS-1215712, and AGS-1216743). We would like to acknowledge operational, technical and scientific support provided by NCAR's Earth Observing Laboratory, sponsored by the National Science Foundation. Any opinions, findings, conclusions or recommendations expressed in this paper are those of the authors and do not necessarily reflect the views of NSF. NR 51 TC 5 Z9 5 U1 33 U2 94 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD APR 28 PY 2016 VL 532 IS 7600 BP 489 EP 491 DI 10.1038/nature17195 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK3KQ UT WOS:000374815900044 PM 27064904 ER PT J AU McCoy, VE Saupe, EE Lamsdell, JC Tarhan, LG McMahon, S Lidgard, S Mayer, P Whalen, CD Soriano, C Finney, L Vogt, S Clark, EG Anderson, RP Petermann, H Locatelli, ER Briggs, DEG AF McCoy, Victoria E. Saupe, Erin E. Lamsdell, James C. Tarhan, Lidya G. McMahon, Sean Lidgard, Scott Mayer, Paul Whalen, Christopher D. Soriano, Carmen Finney, Lydia Vogt, Stefan Clark, Elizabeth G. Anderson, Ross P. Petermann, Holger Locatelli, Emma R. Briggs, Derek E. G. TI The 'Tully monster' is a vertebrate SO NATURE LA English DT Article ID FOSSIL; ILLINOIS AB Problematic fossils, extinct taxa of enigmatic morphology that cannot be assigned to a known major group, were once a major issue in palaeontology. A long-favoured solution to the 'problem of the problematica'(1), particularly the 'weird wonders'(2) of the Cambrian Burgess Shale, was to consider them representatives of extinct phyla. A combination of new evidence and modern approaches to phylogenetic analysis has now resolved the affinities of most of these forms. Perhaps the most notable exception is Tullimonstrum gregarium(3), popularly known as the Tully monster, a large soft-bodied organism from the late Carboniferous Mazon Creek biota (approximately 309-307 million years ago) of Illinois, USA, which was designated the official state fossil of Illinois in 1989. Its phylogenetic position has remained uncertain and it has been compared with nemerteans(4,5), polychaetes(4), gastropods(4), conodonts(6), and the stem arthropod Opabinia(4). Here we review the morphology of Tullimonstrum based on an analysis of more than 1,200 specimens. We find that the anterior proboscis ends in a buccal apparatus containing teeth, the eyes project laterally on a long rigid bar, and the elongate segmented body bears a caudal fin with dorsal and ventral lobes(3-6). We describe new evidence for a notochord, cartilaginous arcualia, gill pouches, articulations within the proboscis, and multiple tooth rows adjacent to the mouth. This combination of characters, supported by phylogenetic analysis, identifies Tullimonstrum as a vertebrate, and places it on the stem lineage to lampreys (Petromyzontida). In addition to increasing the known morphological disparity of extinct lampreys(7-9), a chordate affinity for T. gregarium resolves the nature of a soft-bodied fossil which has been debated for more than 50 years. C1 [McCoy, Victoria E.; Saupe, Erin E.; Lamsdell, James C.; Tarhan, Lidya G.; McMahon, Sean; Whalen, Christopher D.; Clark, Elizabeth G.; Anderson, Ross P.; Petermann, Holger; Locatelli, Emma R.; Briggs, Derek E. G.] Yale Univ, Dept Geol & Geophys, 210 Whitney Ave, New Haven, CT 06511 USA. [Lamsdell, James C.] Amer Museum Nat Hist, Cent Pk West & 79th St, New York, NY 10024 USA. [Lidgard, Scott; Mayer, Paul] Field Museum Nat Hist, 1400 S Lake Shore Dr, Chicago, IL 60605 USA. [Soriano, Carmen; Finney, Lydia; Vogt, Stefan] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Briggs, Derek E. G.] Yale Peabody Museum Nat Hist, 170 Whitney Ave, New Haven, CT 06511 USA. RP McCoy, VE (reprint author), Yale Univ, Dept Geol & Geophys, 210 Whitney Ave, New Haven, CT 06511 USA. EM victoria.mccoy@yale.edu RI Vogt, Stefan/J-7937-2013; OI Vogt, Stefan/0000-0002-8034-5513; McMahon, Sean/0000-0001-8589-2041; Lamsdell, James/0000-0002-1045-9574 FU US Department of Energy Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; Field Museum visiting scholarship; NASA Astrobiology Institute Foundations of Complex Life, Evolution, Preservation and Detection on Earth and Beyond [NNA13AA90A] FX We thank affiliates of the Field Museum of Natural History: J. Voight and J. Wittry for discussion; P. Heck for help with scanning electron microscopy and energy-dispersive spectroscopy; and N. Karpus for specimen photography. This research used resources of the Advanced Photon Source, a US Department of Energy Office of Science User Facility operated for the US Department of Energy Office of Science by Argonne National Laboratory under contract number DE-AC02-06CH11357. The Field Museum of Natural History, the Sedgwick Museum in Cambridge, UK, and C. Eaton at the University of Wisconsin-Madison Geology Museum provided access to specimens. Access to the software TNT for phylogenetic analysis was provided by the Willi Hennig Society. Funding was provided by a Field Museum visiting scholarship to V.E.M. and by the NASA Astrobiology Institute (NNA13AA90A) Foundations of Complex Life, Evolution, Preservation and Detection on Earth and Beyond. NR 28 TC 6 Z9 8 U1 15 U2 26 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD APR 28 PY 2016 VL 532 IS 7600 BP 496 EP + DI 10.1038/nature16992 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK3KQ UT WOS:000374815900046 PM 26982721 ER PT J AU Beyerlein, IJ Hunter, A AF Beyerlein, I. J. Hunter, A. TI d Understanding dislocation mechanics at the mesoscale using phase field dislocation dynamics SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Review DE dislocations; grain boundaries; interfaces; metals; crystals ID STACKING-FAULT ENERGIES; BCC TRANSITION-METALS; NANOCRYSTALLINE AL; SINGLE-CRYSTALS; DEFORMATION-MECHANISM; SCREW DISLOCATIONS; CUBIC METALS; STRAIN-RATE; SIMULATION; NUCLEATION AB In this paper, we discuss the formulation, recent developments and findings obtained from a mesoscale mechanics technique called phase field dislocation dynamics (PFDD). We begin by presenting recent advancements made in modelling face-centred cubic materials, such as integration with atomic-scale simulations to account for partial dislocations. We discuss calculations that help in understanding grain size effects on transitions from full to partial dislocation-mediated slip behaviour and deformation twinning. Finally, we present recent extensions of the PFDD framework to alternative crystal structures, such as body-centred cubic metals, and two-phase materials, including free surfaces, voids and bi-metallic crystals. With several examples we demonstrate that the PFDD model is a powerful and versatile method that can bridge the length and time scales between atomistic and continuum-scale methods, providing a much needed understanding of deformation mechanisms in the mesoscale regime. C1 [Beyerlein, I. J.] Los Alamos Natl Lab, Div Theoret, POB 1663 MS B261, Los Alamos, NM 87545 USA. [Hunter, A.] Los Alamos Natl Lab, X Computat Phys Div, POB 1663 MS T086, Los Alamos, NM 87545 USA. RP Beyerlein, IJ (reprint author), Los Alamos Natl Lab, Div Theoret, POB 1663 MS B261, Los Alamos, NM 87545 USA. EM irene@lanl.gov OI Hunter, Abigail/0000-0002-0443-4020 FU National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract no. DE-AC52-06NA25396. NR 68 TC 0 Z9 0 U1 5 U2 25 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-503X EI 1471-2962 J9 PHILOS T R SOC A JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci. PD APR 28 PY 2016 VL 374 IS 2066 AR 20150166 DI 10.1098/rsta.2015.0166 PG 27 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1OG UT WOS:000372553900001 ER PT J AU Boldon, L Sabharwall, P Rabiti, C Bragg-Sitton, SM Liu, L AF Boldon, Lauren Sabharwall, Piyush Rabiti, Cristian Bragg-Sitton, Shannon M. Liu, Li TI Thermodynamic exergy analysis for small modular reactor in nuclear hybrid energy system SO EPJ NUCLEAR SCIENCES & TECHNOLOGIES LA English DT Article ID COST AB Small modular reactors (SMRs) provide a unique opportunity for future nuclear development with reduced financial risks, allowing the United States to meet growing energy demands through safe, reliable, clean air electricity generation while reducing greenhouse gas emissions and the reliance on unstable fossil fuel prices. A nuclear power plant is comprised of several complex subsystems which utilize materials from other subsystems and their surroundings. The economic utility of resources, or thermoeconomics, is extremely difficult to analyze, particularly when trying to optimize resources and costs among individual subsystems and determine prices for products. Economics and thermodynamics cannot provide this information individually. Thermoeconomics, however, provides a method of coupling the quality of energy available based on exergy and the value of this available energy "exergetic costs". For an SMR exergy analysis, both the physical and economic environments must be considered. The physical environment incorporates the energy, raw materials, and reference environment, where the reference environment refers to natural resources available without limit and without cost, such as air input to a boiler. The economic environment includes market influences and prices in addition to installation, operation, and maintenance costs required for production to occur. The exergetic cost or the required exergy for production may be determined by analyzing the physical environment alone. However, to optimize the system economics, this environment must be coupled with the economic environment. A balance exists between enhancing systems to improve efficiency and optimizing costs. Prior research into SMR thermodynamics has not detailed methods on improving exergetic costs for an SMR coupled with storage technologies and renewable energy such as wind or solar in a hybrid energy system. This process requires balancing technological efficiencies and economics to demonstrate financially competitive systems. This paper aims to explore the use of exergy analysis methods to estimate and optimize SMR resources and costs for individual subsystems, based on thermodynamic principles - resource utilization and efficiency. The paper will present background information on exergy theory; identify the core subsystems in an SMR plant coupled with storage systems in support of renewable energy and hydrogen production; perform a thermodynamic exergy analysis; determine the cost allocation among these subsystems; and calculate unit exergetic costs, unit exergoeconomic costs, and first and second law efficiencies. Exergetic and exergoeconomic costs ultimately determine how individual subsystems contribute to overall profitability and how efficiencies and consumption may be optimized to improve profitability, making SMRs more competitive with other generation technologies. C1 [Boldon, Lauren; Sabharwall, Piyush; Liu, Li] Rensselaer Polytech Inst, 110 8th St,JEC 5046, Troy, NY 12180 USA. [Sabharwall, Piyush; Rabiti, Cristian; Bragg-Sitton, Shannon M.] Idaho Natl Lab, POB 1625, Idaho Falls, ID USA. RP Boldon, L (reprint author), Rensselaer Polytech Inst, 110 8th St,JEC 5046, Troy, NY 12180 USA. EM boldol@rpi.edu NR 14 TC 0 Z9 0 U1 3 U2 3 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 2491-9292 J9 EPJ NUCL SCI TECHNOL JI EPJ Nucl. Sci. Technol. PD APR 27 PY 2016 VL 2 AR UNSP 23 DI 10.1051/epjn/2016011 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DY0RX UT WOS:000384805000001 ER PT J AU Shingler, T Crosbie, E Ortega, A Shiraiwa, M Zuend, A Beyersdorf, A Ziemba, L Anderson, B Thornhill, L Perring, AE Schwarz, JP Campazano-Jost, P Day, DA Jimenez, JL Hair, JW Mikoviny, T Wisthaler, A Sorooshian, A AF Shingler, Taylor Crosbie, Ewan Ortega, Amber Shiraiwa, Manabu Zuend, Andreas Beyersdorf, Andreas Ziemba, Luke Anderson, Bruce Thornhill, Lee Perring, Anne E. Schwarz, Joshua P. Campazano-Jost, Pedro Day, Douglas A. Jimenez, Jose L. Hair, Johnathan W. Mikoviny, Tomas Wisthaler, Armin Sorooshian, Armin TI Airborne characterization of subsaturated aerosol hygroscopicity and dry refractive index from the surface to 6.5km during the SEAC(4)RS campaign SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID ORGANIC-INORGANIC AEROSOLS; SINGLE-SCATTERING ALBEDO; LIQUID-LIQUID EQUILIBRIA; OPTICAL-PROPERTIES; AMMONIUM-SULFATE; LIGHT-SCATTERING; ACTIVITY-COEFFICIENTS; RADIATIVE PROPERTIES; CHEMICAL-COMPOSITION; THERMODYNAMIC MODEL AB In situ aerosol particle measurements were conducted during 21 NASA DC-8 flights in the Studies of Emissions and Atmospheric Composition, Clouds, and Climate Coupling by Regional Surveys field campaign over the United States, Canada, Pacific Ocean, and Gulf of Mexico. For the first time, this study reports rapid, size-resolved hygroscopic growth and real refractive index (RI at 532 nm) data between the surface and upper troposphere in a variety of air masses including wildfires, agricultural fires, biogenic, marine, and urban outflow. The Differential Aerosol Sizing and Hygroscopicity Spectrometer Probe (DASH-SP) quantified size-resolved diameter growth factors (GF = D-p,D-wet/D-p,D-dry) that are used to infer the hygroscopicity parameter kappa. Thermokinetic simulations were conducted to estimate the impact of partial particle volatilization within the DASH-SP across a range of sampling conditions. Analyses of GF and RI data as a function of air mass origin, dry size, and altitude are reported, in addition to kappa values for the inorganic and organic fractions of aerosol. Average RI values are found to be fairly constant (1.52-1.54) for all air mass categories. An algorithm is used to compare size-resolved DASH-SP GF with bulk scattering f(RH=80%) data obtained from a pair of nephelometers, and the results show that the two can only be reconciled if GF is assumed to decrease with increasing dry size above 400 nm (i.e., beyond the upper bound of DASH-SP measurements). Individual case studies illustrate variations of hygroscopicity as a function of dry size, environmental conditions, altitude, and composition. C1 [Shingler, Taylor; Ortega, Amber; Sorooshian, Armin] Univ Arizona, Dept Chem & Environm Engn, Tucson, AZ USA. [Crosbie, Ewan; Beyersdorf, Andreas; Ziemba, Luke; Anderson, Bruce; Thornhill, Lee; Hair, Johnathan W.] NASA, Langley Res Ctr, Chem & Dynam Branch, Hampton, VA 23665 USA. [Crosbie, Ewan] Oak Ridge Associated Univ, Oak Ridge, TN USA. [Shiraiwa, Manabu] Max Planck Inst Chem, Multiphase Chem Dept, Mainz, Germany. [Zuend, Andreas] McGill Univ, Dept Atmospher & Ocean Sci, Montreal, PQ, Canada. [Thornhill, Lee] Sci Syst & Applicat Inc, Hampton, VA USA. [Perring, Anne E.; Schwarz, Joshua P.] NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO USA. [Perring, Anne E.; Campazano-Jost, Pedro; Day, Douglas A.; Jimenez, Jose L.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Campazano-Jost, Pedro; Day, Douglas A.; Jimenez, Jose L.] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Mikoviny, Tomas; Wisthaler, Armin] Univ Oslo, Dept Chem, Oslo, Norway. [Wisthaler, Armin] Univ Innsbruck, Inst Ion Phys & Appl Phys, A-6020 Innsbruck, Austria. [Sorooshian, Armin] Univ Arizona, Dept Atmospher Sci, Tucson, AZ USA. RP Sorooshian, A (reprint author), Univ Arizona, Dept Chem & Environm Engn, Tucson, AZ USA.; Sorooshian, A (reprint author), Univ Arizona, Dept Atmospher Sci, Tucson, AZ USA. EM armin@email.arizona.edu RI Perring, Anne/G-4597-2013; Jimenez, Jose/A-5294-2008; schwarz, joshua/G-4556-2013; Manager, CSD Publications/B-2789-2015 OI Perring, Anne/0000-0003-2231-7503; Jimenez, Jose/0000-0001-6203-1847; schwarz, joshua/0000-0002-9123-2223; FU NASA [NNX12AC10G, NNX14AP75G, NNX12AC03G, NNX15AT96G]; ONR [N00014-10-1-0811]; NASA Earth and Space Science Fellowship [NNX14AK79H]; Visiting Scientist Program at the National Institute of Aerospace FX All data and results are available from the corresponding author (armin@email.arizona.edu). This research was funded by NASA grants NNX12AC10G and NNX14AP75G. The development of the DASH-SP instrument was funded by ONR grant N00014-10-1-0811. T.S. acknowledges support from a NASA Earth and Space Science Fellowship (NNX14AK79H). P.C.J., D.A.D., and J.L.J. were supported by NASA grants NNX12AC03G and NNX15AT96G. PTR-MS measurements during SEAC4RS were supported by the Austrian Federal Ministry for Transport, Innovation and Technology (bmvit) through the Austrian Space Applications Programme of the Austrian Research Promotion Agency (FFG). A.W. and T.M. received support from the Visiting Scientist Program at the National Institute of Aerospace. NR 98 TC 5 Z9 5 U1 8 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD APR 27 PY 2016 VL 121 IS 8 BP 4188 EP 4210 DI 10.1002/2015JD024498 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DP2KU UT WOS:000378318100028 ER PT J AU Bela, MM Barth, MC Toon, OB Fried, A Homeyer, CR Morrison, H Cummings, KA Li, YY Pickering, KE Allen, DJ Yang, Q Wennberg, PO Crounse, JD St Clair, JM Teng, AP O'Sullivan, D Huey, LG Chen, DX Liu, XX Blake, DR Blake, NJ Apel, EC Hornbrook, RS Flocke, F Campos, T Diskin, G AF Bela, Megan M. Barth, Mary C. Toon, Owen B. Fried, Alan Homeyer, Cameron R. Morrison, Hugh Cummings, Kristin A. Li, Yunyao Pickering, Kenneth E. Allen, Dale J. Yang, Qing Wennberg, Paul O. Crounse, John D. St Clair, Jason M. Teng, Alex P. O'Sullivan, Daniel Huey, L. Gregory Chen, Dexian Liu, Xiaoxi Blake, Donald R. Blake, Nicola J. Apel, Eric C. Hornbrook, Rebecca S. Flocke, Frank Campos, Teresa Diskin, Glenn TI Wet scavenging of soluble gases in DC3 deep convective storms using WRF-Chem simulations and aircraft observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID IONIZATION MASS-SPECTROMETRY; UPPER TROPOSPHERE; HYDROGEN-PEROXIDE; TRACE GASES; RADAR OBSERVATIONS; MODEL PERFORMANCE; MOIST CONVECTION; CENTRAL VIRGINIA; HIGH-SENSITIVITY; SULFUR-DIOXIDE AB We examine wet scavenging of soluble trace gases in storms observed during the Deep Convective Clouds and Chemistry (DC3) field campaign. We conduct high-resolution simulations with the Weather Research and Forecasting model with Chemistry (WRF-Chem) of a severe storm in Oklahoma. The model represents well the storm location, size, and structure as compared with Next Generation Weather Radar reflectivity, and simulated CO transport is consistent with aircraft observations. Scavenging efficiencies (SEs) between inflow and outflow of soluble species are calculated from aircraft measurements and model simulations. Using a simple wet scavenging scheme, we simulate the SE of each soluble species within the error bars of the observations. The simulated SEs of all species except nitric acid (HNO3) are highly sensitive to the values specified for the fractions retained in ice when cloud water freezes. To reproduce the observations, we must assume zero ice retention for formaldehyde (CH2O) and hydrogen peroxide (H2O2) and complete retention for methyl hydrogen peroxide (CH3OOH) and sulfur dioxide (SO2), likely to compensate for the lack of aqueous chemistry in the model. We then compare scavenging efficiencies among storms that formed in Alabama and northeast Colorado and the Oklahoma storm. Significant differences in SEs are seen among storms and species. More scavenging of HNO3 and less removal of CH3OOH are seen in storms with higher maximum flash rates, an indication of more graupel mass. Graupel is associated with mixed-phase scavenging and lightning production of nitrogen oxides (NOx), processes that may explain the observed differences in HNO3 and CH3OOH scavenging. C1 [Bela, Megan M.; Toon, Owen B.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Bela, Megan M.; Toon, Owen B.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Barth, Mary C.; Morrison, Hugh; Apel, Eric C.; Hornbrook, Rebecca S.; Flocke, Frank; Campos, Teresa] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Fried, Alan] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Homeyer, Cameron R.] Univ Oklahoma, Sch Meteorol, Norman, OK 73019 USA. [Cummings, Kristin A.; Li, Yunyao; Pickering, Kenneth E.; Allen, Dale J.] Univ Maryland, Dept Atmospher & Ocean Sci, College Pk, MD 20742 USA. [Pickering, Kenneth E.; St Clair, Jason M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Yang, Qing] Pacific NW Natl Lab, Richland, WA 99352 USA. [Wennberg, Paul O.; Crounse, John D.; St Clair, Jason M.; Teng, Alex P.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Wennberg, Paul O.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [St Clair, Jason M.] Univ Maryland Baltimore Cty, Joint Ctr Earth Syst Technol, Baltimore, MD 21228 USA. [O'Sullivan, Daniel] US Naval Acad, Annapolis, MD 21402 USA. [Huey, L. Gregory; Chen, Dexian; Liu, Xiaoxi] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Blake, Donald R.; Blake, Nicola J.] Univ Calif Irvine, Dept Chem, Irvine, CA 92717 USA. [Diskin, Glenn] NASA, Langley Res Ctr, Hampton, VA 23665 USA. RP Bela, MM (reprint author), Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA.; Bela, MM (reprint author), Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. EM megan.bela@colorado.edu RI Allen, Dale/F-7168-2010; Crounse, John/C-3700-2014; Pickering, Kenneth/E-6274-2012; Homeyer, Cameron/D-5034-2013 OI Allen, Dale/0000-0003-3305-9669; Crounse, John/0000-0001-5443-729X; Homeyer, Cameron/0000-0002-4883-6670 FU National Science Foundation; NSF [AGS-1261559, AGS-1522910, 1063479, 1522551, ATM1063467]; NASA [ACCDAMNNX14AR56G, NNX12AMO8G, NNX12AC06G, NNX14AP46G-ACCDAM, NNX12AB77G, NNX12AB76G]; Office of Science of the U.S. Department of Energy as part of the Atmospheric System Research Program (ASR) FX We express our appreciation to the following researchers for the aircraft observations: T. Ryerson and the NOAA NOyO3 team; Andrew Weinheimer; Mark Zondlo, Josh DiGangi, and Anthony O'Brien for the VCSEL hygrometer water vapor measurements on the GV; and P. Lawson and S. Woods from SPEC Inc. We also thank A. Weinheimer and M. Zondlo for their helpful feedback on this manuscript. M. M. Bela and O.B. Toon were supported by NASA ACCDAMNNX14AR56G. The National Center for Atmospheric Research is sponsored by the National Science Foundation. A. Fried was supported by NSF and NASA under grants AGS-1261559 and NNX12AMO8G, respectively. C. Homeyer was funded by NSF grant AGS-1522910. The University of Maryland co-authors were supported under NSF grants 1063479 and 1522551. Q. Yang was supported by the Office of Science of the U.S. Department of Energy as part of the Atmospheric System Research Program (ASR). P.O. Wennberg, J.D. Crounse, A. P. Teng, and J.M. St. Clair thank NASA for supporting their contribution to this study (NNX12AC06G and NNX14AP46G-ACCDAM). D. O'Sullivan thanks NSF for support from grant ATM1063467. L.G. Huey, D. Chen, and X. Liu were funded by NASA grant NNX12AB77G. DC3 measurements by N. Blake and D. Blake were supported by NASA award NNX12AB76G. We would like to thank Earth Networks for providing the ENTLN lightning data for research purposes. The data used in this study can be downloaded from the following websites: 1 s data merges from the NASA Langley DC3 Merged Aircraft Dataset Archive (http://www-air.larc.nasa.gov/cgi-bin/ArcView/dc3); NEXRAD data for individual radars from the National Climatic Data Center (NCDC; http://has.ncdc.noaa.gov/pls/plhas/has.dsselect); NSSL-MGAUS sounding data (http://data.eol.ucar.edu/codiac/dss/id=353.105); NCEP Stage IV precipitation analysis (http://www.emc.ncep.noaa.gov/mmb/ylin/pcpanl/stage4/); and NAM-ANL (http://nomads.ncdc.noaa.gov/data/namanl/). The WRF-Chem code and land surface data are available for download from NCAR/MMM (http://www.mmm.ucar.edu/wrf/users/download/get_sources_wps_geog.html). WRF-Chem model output is available upon request to M. M. Bela (megan.bela@colorado.edu). NR 104 TC 4 Z9 4 U1 5 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD APR 27 PY 2016 VL 121 IS 8 BP 4233 EP 4257 DI 10.1002/2015JD024623 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DP2KU UT WOS:000378318100030 ER PT J AU Jaffe, A Lin, Y Beavers, CM Voss, J Mao, WL Karunadasa, HI AF Jaffe, Adam Lin, Yu Beavers, Christine M. Voss, Johannes Mao, Wendy L. Karunadasa, Hemamala I. TI High-Pressure Single-Crystal Structures of 3D Lead-Halide Hybrid Perovskites and Pressure Effects on their Electronic and Optical Properties SO ACS CENTRAL SCIENCE LA English DT Article ID LIGHT-EMITTING-DIODES; PHASE-TRANSITIONS; CHEMICAL PRESSURE; SOLAR-CELLS; SEMICONDUCTORS; SUPERCONDUCTIVITY; DIFFRACTION; CROSSOVER; OCTAHEDRA; BROMIDE AB We report the first high-pressure single-crystal structures of hybrid perovskites. The crystalline semiconductors (MA)PbX3 (MA = CH3NH3+, X = Br- or I-) afford us the rare opportunity of understanding how compression modulates their structures and thereby their optoelectronic properties. Using atomic coordinates obtained from high-pressure single-crystal X-ray diffraction we track the perovskites' precise structural evolution upon compression. These structural changes correlate well with pressure-dependent single-crystal photoluminescence (PL) spectra and high-pressure bandgaps derived from density functional theory. We further observe dramatic piezochromism where the solids become lighter in color and then transition to opaque black with compression. Indeed, electronic conductivity measurements of (MA)PbI3 obtained within a diamond-anvil cell show that the material's resistivity decreases by 3 orders of magnitude between 0 and 51 GPa. The activation energy for conduction at 51 GPa is only 13.2(3) meV, suggesting that the perovskite is approaching a metallic state. Furthermore, the pressure response of mixed-halide perovskites shows new luminescent states that emerge at elevated pressures. We recently reported that the perovskites (MA) Pb(BrxI(1-x))(3) (0.2 < x < 1) reversibly form light-induced trap states, which pin their PL to a low energy. This may explain the low voltages obtained from solar cells employing these absorbers. Our high-pressure PL data indicate that compression can mitigate this PL redshift and may afford higher steady-state voltages from these absorbers. These studies show that pressure can significantly alter the transport and thermodynamic properties of these technologically important semiconductors. C1 [Jaffe, Adam; Lin, Yu; Karunadasa, Hemamala I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Lin, Yu; Mao, Wendy L.] Stanford Univ, Dept Geol Sci, Stanford, CA 94305 USA. [Lin, Yu; Mao, Wendy L.] SLAC Natl Accelerator Lab, Photon Sci, Menlo Pk, CA 94025 USA. [Lin, Yu; Mao, Wendy L.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Beavers, Christine M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Voss, Johannes] SLAC Natl Accelerator Lab, SUNCAT Ctr Interface Sci & Catalysis, Menlo Pk, CA 94025 USA. RP Karunadasa, HI (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94305 USA.; Mao, WL (reprint author), Stanford Univ, Dept Geol Sci, Stanford, CA 94305 USA.; Mao, WL (reprint author), SLAC Natl Accelerator Lab, Photon Sci, Menlo Pk, CA 94025 USA.; Mao, WL (reprint author), SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. EM wmao@stanford.edu; hemamala@stanford.edu NR 45 TC 19 Z9 19 U1 14 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD APR 27 PY 2016 VL 2 IS 4 BP 201 EP 209 DI 10.1021/acscentsci.6b00055 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DO5LR UT WOS:000377825100006 PM 27163050 ER PT J AU Demir, S Brune, NK Van Humbeck, JF Mason, JA Plakhova, TV Wang, SA Tian, GX Minasian, SG Tyliszczak, T Yaita, T Kobayashi, T Kalmykov, SN Shiwaku, H Shuh, DK Long, JR AF Demir, Selvan Brune, Nicholas K. Van Humbeck, Jeffrey F. Mason, Jarad A. Plakhova, Tatiana V. Wang, Shuao Tian, Guoxin Minasian, Stefan G. Tyliszczak, Tolek Yaita, Tsuyoshi Kobayashi, Tohru Kalmykov, Stepan N. Shiwaku, Hideaki Shuh, David K. Long, Jeffrey R. TI Extraction of Lanthanide and Actinide Ions from Aqueous Mixtures Using a Carboxylic Acid-Functionalized Porous Aromatic Framework SO ACS CENTRAL SCIENCE LA English DT Article ID METAL-ORGANIC FRAMEWORKS; X-RAY MICROSCOPY; CARBON-DIOXIDE CAPTURE; CRYSTAL-STRUCTURE; NITRIC-ACID; ABSORPTION-SPECTROSCOPY; MOLECULAR SIMULATIONS; MICROBIAL BIOFILMS; POLYMER NETWORKS; TRUEX PROCESS AB Porous aromatic frameworks (PAFs) incorporating a high concentration of acid functional groups possess characteristics that are promising for use in separating lanthanide and actinide metal ions, as required in the treatment of radioactive waste. These materials have been shown to be indefinitely stable to concentrated acids and bases, potentially allowing for multiple adsorption/stripping cycles. Additionally, the PAFs combine exceptional features from MOFs and inorganic/activated carbons giving rise to tunable pore surfaces and maximum chemical stability. Herein, we present a study of the adsorption of selected metal ions, Sr2+, Fe3+, Nd3+, and Am3+, from aqueous solutions employing a carbon-based porous aromatic framework, BPP-7 (Berkeley Porous Polymer-7). This material displays high metal loading capacities together with excellent adsorption selectivity for neodymium over strontium based on Langmuir adsorption isotherms and ideal adsorbed solution theory (IAST) calculations. Based in part upon X-ray absorption spectroscopy studies, the stronger adsorption of neodymium is attributed to multiple metal ion and binding site interactions resulting from the densely functionalized and highly interpenetrated structure of BPP-7. Recyclability and combustibility experiments demonstrate that multiple adsorption/stripping cycles can be completed with minimal degradation of the polymer adsorption capacity. C1 [Demir, Selvan; Brune, Nicholas K.; Van Humbeck, Jeffrey F.; Mason, Jarad A.; Wang, Shuao; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Demir, Selvan; Brune, Nicholas K.; Plakhova, Tatiana V.; Wang, Shuao; Tian, Guoxin; Minasian, Stefan G.; Shuh, David K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Plakhova, Tatiana V.; Kalmykov, Stepan N.] Moscow MV Lomonosov State Univ, Dept Chem, Moscow 11991, Russia. [Yaita, Tsuyoshi; Kobayashi, Tohru; Shiwaku, Hideaki] Japan Atom Energy Agcy, Actinide Chem Grp, Energy & Environm Sci Div, Quantum Beam Sci Ctr, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. [Tian, Guoxin] China Inst Atom Energy, Dept Radiochem, Beijing 102413, Peoples R China. [Van Humbeck, Jeffrey F.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Wang, Shuao] Soochow Univ, Sch Radiat Med & Protect, Suzhou 215123, Jiangsu, Peoples R China. [Wang, Shuao] Soochow Univ, Sch Radiol & Interdisciplinary Sci RAD X, Suzhou 215123, Jiangsu, Peoples R China. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Long, JR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu NR 77 TC 3 Z9 3 U1 23 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD APR 27 PY 2016 VL 2 IS 4 BP 253 EP 265 DI 10.1021/acscentsci.6b00066 PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA DO5LR UT WOS:000377825100012 PM 27163056 ER PT J AU Brumm, PJ Land, ML Mead, DA AF Brumm, Phillip J. Land, Miriam L. Mead, David A. TI Complete genome sequences of Geobacillus sp WCH70, a thermophilic strain isolated from wood compost SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Geobacillus sp WCH70; Wood compost; Thermophile; Transposons; Restriction-modification ID SP-NOV.; RNA GENES; ACCURACY; BACTERIA; DATABASE; REVEALS; SYSTEM; TOOL AB Geobacillus sp. WCH70 was one of several thermophilic organisms isolated from hot composts in the Middleton, WI area. Comparison of 16 S rRNA sequences showed the strain may be a new species, and is most closely related to G. galactosidasius and G. toebii. The genome was sequenced, assembled, and annotated by the DOE Joint Genome Institute and deposited at the NCBI in December 2009 (CP001638). The genome of Geobacillus species WCH70 consists of one circular chromosome of 3,893,306 bp with an average G + C content of 43 %, and two circular plasmids of 33,899 and 10,287 bp with an average G + C content of 40 %. Among sequenced organisms, Geobacillus sp. WCH70 shares highest Average Nucleotide Identity (86 %) with G. thermoglucosidasius strains, as well as similar genome organization. Geobacillus sp. WCH70 appears to be a highly adaptable organism, with an exceptionally high 125 annotated transposons in the genome. The organism also possesses four predicted restriction-modification systems not found in other Geobacillus species. C1 [Brumm, Phillip J.] C5 6 Technol LLC, Fitchburg, WI USA. [Brumm, Phillip J.; Mead, David A.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Land, Miriam L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Mead, David A.] Lucigen Corp, Middleton, WI USA. RP Brumm, PJ (reprint author), C5 6 Technol LLC, Fitchburg, WI USA.; Brumm, PJ (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI USA. EM pbrumm@c56technologies.com RI Land, Miriam/A-6200-2011 OI Land, Miriam/0000-0001-7102-0031 FU DOE Great Lakes Bioenergy Research Center (DOE Office of Science) [BER DE-FC02-07ER64494]; US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; University of California, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of California, Los Alamos National Laboratory [DE-AC02-06NA25396] FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494). Sequencing work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231, Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344, and Los Alamos National Laboratory under contract No. DE-AC02-06NA25396. NR 42 TC 0 Z9 0 U1 5 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD APR 27 PY 2016 VL 11 AR 33 DI 10.1186/s40793-016-0153-y PG 8 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DO7HE UT WOS:000377952400001 PM 27123157 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A 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CA ATLAS Collaboration TI Observation of Long-Range Elliptic Azimuthal Anisotropies in root s=13 and 2.76 TeV pp Collisions with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID PROTON-PROTON COLLISIONS; ANGULAR-CORRELATIONS; FLOW; MULTIPLICITY; DEPENDENCE; ENERGY; SIDE AB ATLAS has measured two-particle correlations as a function of the relative azimuthal angle, Delta phi, and pseudorapidity, Delta eta, in root s = 13 and 2.76 TeV pp collisions at the LHC using charged particles measured in the pseudorapidity interval vertical bar eta vertical bar < 2.5. The correlation functions evaluated in different intervals of measured charged-particle multiplicity show a multiplicity-dependent enhancement at Delta phi similar to 0 that extends over a wide range of Delta eta, which has been referred to as the "ridge." Per-trigger-particle yields, Y(Delta phi) are measured over 2 < vertical bar Delta eta vertical bar < 5. For both collision energies, the Y(Delta phi) distribution in all multiplicity intervals is found to be consistent with a linear combination of the per-trigger-particle yields measured in collisions with less than 2 phi reconstructed tracks, and a constant combinatoric contribution modulated by cos (2 Delta phi). The fitted Fourier coefficient, nu(2,2), exhibits factorization, suggesting that the ridge results from per-event cos (2 phi) modulation of the single-particle distribution with Fourier coefficients nu(2). The nu(2) values are presented as a function of multiplicity and transverse momentum. They are found to be approximately constant as a function of multiplicity and to have a p(T) dependence similar to that measured in p + Pb and Pb + Pb collisions. The nu(2) values in the 13 and 2.76 TeV data are consistent within uncertainties. 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R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Du, Y.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Li, Y.; Zhang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Phys Dept, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Phys Dept, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Phys Dept, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Aloisio, A.; Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, High Energy Phys Inst, GE-380086 Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; De Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subat & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Serre, T.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gabizon, O.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gabizon, O.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huesing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Aloisio, A.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Savard, P.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Di Donato, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Vergata, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.; Haddad, N.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energie Al, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, IMB, CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez De la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. 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RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Jung, David/Q-4068-2016; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Gladilin, Leonid/B-5226-2011; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015 OI Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Jung, David/0000-0001-8631-610X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Pina, Joao /0000-0001-8959-5044; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Gerbaudo, Davide/0000-0002-4463-0878; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Leverhulme Trust, United Kingdom; Royal Society, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 45 TC 13 Z9 13 U1 22 U2 50 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. 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CA CMS Collaboration TI Measurement of Long-Range Near-Side Two-Particle Angular Correlations in pp Collisions at root s=13 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRANSVERSE-MOMENTUM DEPENDENCE; PLUS PB COLLISIONS; ROOT-S(NN)=5.02 TEV; CHARGED-PARTICLES; ATLAS DETECTOR; FLOW; LHC AB Results on two-particle angular correlations for charged particles produced in pp collisions at a center-of- mass energy of 13 TeV are presented. The data were taken with the CMS detector at the LHC and correspond to an integrated luminosity of about 270 nb(-1). The correlations are studied over a broad range of pseudorapidity (vertical bar eta vertical bar < 2.4) and over the full azimuth (phi) as a function of charged particle multiplicity and transverse momentum (p(T)). In high-multiplicity events, a long-range (vertical bar Delta eta vertical bar > 2.0), near-side (Delta phi approximate to 0) structure emerges in the two-particle Delta eta-Delta phi correlation functions. The magnitude of the correlation exhibits a pronounced maximum in the range 1.0 < p(T) < 2.0 GeV/c and an approximately linear increase with the charged particle multiplicity, with an overall correlation strength similar to that found in earlier pp data at root s = 7 TeV. The present measurement extends the study of near-side long-range correlations up to charged particle multiplicities N-ch similar to 180, a region so far unexplored in pp collisions. The observed longrange correlations are compared to those seen in pp, pPb, and PbPb collisions at lower collision energies. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; El-khateeb, E.; Elkafrawy, T.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Ero, J.; Flechl, M.; Friedl, M.; Fruhwirth, R.; Ghete, V. M.; Hartl, C.; Hormann, N.; Hrubec, J.; Jeitler, M.; Knunz, V.; Konig, A.; Krammer, M.; Kratschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schofbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Van de Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Brun, H.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Fasanella, G.; Favart, L.; Grebenyuk, A.; Karapostoli, G.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Marinov, A.; Pernie, L.; Randle-conde, A.; Seva, T.; Vander Velde, C.; Vanlaer, P.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Musich, M.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. 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[Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Davignon, O.; Filipovic, N.; de Cassagnac, R. Granier; Jo, M.; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. 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[Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Guth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Mukherjee, S.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Campbell, A.; Costanza, F.; Pardos, C. 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S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Scharf, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baur, S.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Schroeder, M.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. 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[Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Trento, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Trento, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, Novara, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Novara, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Casarsa, M.; Cossutti, F.; Gobbo, B.; La Licata, C.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Da Cruz E Silva, C. Beirao; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.; Afanasiev, S.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Ershov, A.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Lukina, O.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schoenenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Gecit, F. H.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozcan, M.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. 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[Borras, K.; Rolandi, G.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Gallo, E.; Sphicas, P.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.; Starodumov, A.; Nikitenko, A.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.; Amsler, C.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.; Cerci, S.; Tali, B.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.; Kangal, E. E.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.; Onengut, G.] Wigner Res Ctr Phys, Budapest, Hungary. [Choudhury, S.; Ozdemir, K.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.; Ozturk, S.; Topakli, H.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.; Isildak, B.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Invest Cient & Tecn, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.; Milenovic, P.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Matveev, V.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Di Marco, E.] Univ Rome, Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. Vinca Inst Nucl Sci, Belgrade, Serbia. Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Lokhtin, Igor/D-7004-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011 OI Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 45 TC 9 Z9 9 U1 19 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 27 PY 2016 VL 116 IS 17 AR 172302 DI 10.1103/PhysRevLett.116.172302 PG 19 WC Physics, Multidisciplinary SC Physics GA DK5MQ UT WOS:000374964400005 PM 27176516 ER PT J AU Butler, KS Durfee, PN Theron, C Ashley, CE Carnes, EC Brinker, CJ AF Butler, Kimberly S. Durfee, Paul N. Theron, Christophe Ashley, Carlee E. Carnes, Eric C. Brinker, C. Jeffrey TI Protocells: Modular Mesoporous Silica Nanoparticle-Supported Lipid Bilayers for Drug Delivery SO SMALL LA English DT Review DE mesoporous silica; supported lipid bilayers; protocells; nanoparticles; targeted delivery; drug delivery ID IN-VIVO BIODISTRIBUTION; CANCER-CELLS; MAGNETIC-RESONANCE; TARGETED DELIVERY; HEMOLYTIC-ACTIVITY; ANTICANCER DRUGS; LIPOSOMES; SIZE; NANOCARRIERS; MEMBRANE AB Mesoporous silica nanoparticle-supported lipid bilayers, termed protocells,' represent a potentially transformative class of therapeutic and theranostic delivery vehicle. The field of targeted drug delivery poses considerable challenges that cannot be addressed with a single magic bullet'. Consequently, the protocell has been designed as a modular platform composed of interchangeable biocompatible components. The mesoporous silica core has variable size and shape to direct biodistribution and a controlled pore size and surface chemistry to accommodate diverse cargo. The encapsulating supported lipid bilayer can be modified with targeting and trafficking ligands as well as polyethylene glycol (PEG) to effect selective binding, endosomal escape of cargo, drug efflux prevention, and potent therapeutic delivery, while maintaining in vivo colloidal stability. This review describes the individual components of the platform, including the mesoporous silica nanoparticle core and supported lipid bilayer, their assembly (by multiple techniques) into a protocell, and the combined, often synergistic, performance of the protocell based on in vitro and in vivo studies, including the assessment of biocompatibility and toxicity. In closing, the many emerging variations of the protocell theme and the future directions for protocell research are commented on. C1 [Butler, Kimberly S.; Theron, Christophe; Brinker, C. Jeffrey] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Durfee, Paul N.; Brinker, C. Jeffrey] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Ashley, Carlee E.] Sandia Natl Labs, Bioenergy & Def Technol Dept, Livermore, CA 94551 USA. [Carnes, Eric C.] Sandia Natl Labs, Nanobiol Dept, Livermore, CA 94551 USA. [Brinker, C. Jeffrey] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87185 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA.; Brinker, CJ (reprint author), Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov FU NIH National Cancer Institute (NCI) Alliance [UO1 CA151792-01]; Lymphoma and Leukemia Society (LLS) Specialized Center of Research (SCOR) [7010-14]; Oncothyreon, Inc.; New Mexico Cancer Nanoscience and Microsystems Training Center (CNTC); George D. Montoya Research Scholarship; Edmund J. & Thelma W. Evans Charitable Trust Scholarship; Charlotte and William Kraft Graduate Fellowship; U.S. Department of Energy (DOE), Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering; Sandia National Laboratories' Laboratory Directed Research and Development (LDRD) program; Air Force Office of Scientific Research [FA 9550-1-14-066]; National Science Foundation; 21 Environment Protection Agency; University of California's Center for Environmental Implications of Nanotechnology; Defense Threat Reduction Agency grant DTRA JSTO-CBD NATV FX K. S. Butler and P. N. Durfee contributed equally to this work. This work was supported by NIH National Cancer Institute (NCI) Alliance Grant UO1 CA151792-01, the Lymphoma and Leukemia Society (LLS) Specialized Center of Research (SCOR) Award 7010-14, and Oncothyreon, Inc. P.N.D. was funded by a fellowship from the New Mexico Cancer Nanoscience and Microsystems Training Center (CNTC) and by the George D. Montoya Research Scholarship, Edmund J. & Thelma W. Evans Charitable Trust Scholarship, and the Charlotte and William Kraft Graduate Fellowship. C.J.B acknowledges additional support from U.S. Department of Energy (DOE), Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering for supporting research on mesoporous silica materials. CJB also acknowledges support from Sandia National Laboratories' Laboratory Directed Research and Development (LDRD) program, the Air Force Office of Scientific Research grant FA 9550-1-14-066, National Science Foundation, 21 Environment Protection Agency, and University of California's Center for Environmental Implications of Nanotechnology. CJB, CEA and ECC acknowledge support from the Defense Threat Reduction Agency grant DTRA JSTO-CBD NATV. NR 73 TC 7 Z9 7 U1 51 U2 114 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD APR 27 PY 2016 VL 12 IS 16 SI SI BP 2173 EP 2185 DI 10.1002/smll.201502119 PG 13 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DK1YX UT WOS:000374712700006 PM 26780591 ER PT J AU Bae, YJ Cho, ES Qu, F Sun, DT Williams, TE Urban, JJ Queen, WL AF Bae, Youn Jue Cho, Eun Seon Qu, Fen Sun, Daniel T. Williams, Teresa E. Urban, Jeffrey J. Queen, Wendy L. TI Transparent Metal-Organic Framework/Polymer Mixed Matrix Membranes as Water Vapor Barriers SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE metal-organic framework; postsynthetic modification; water vapor transmission rate; mixed-matrix membrane gas barrier; encapsulant ID ZR-FUMARATE MOF; MODULATED SYNTHESIS; GAS-SEPARATION; CRYSTALS; COATINGS; POROSITY; FILMS; OXIDE AB Preventing the permeation of reactive molecules into electronic devices or photovoltaic modules is of great importance to ensure their life span and reliability. This work is focused on the formation of highly functioning barrier films based on nanocrystals (NCs) of a water-scavenging metal organic framework (MOP) and a hydrophobic cyclic olefin copolymer (COC) to overcome the current limitations. Water vapor transmission rates (WVTR) of the films reveal a 10-fold enhancement in the WVTR compared to the substrate while maintaining outstanding transparency over most of the visible and solar spectrum, a necessary condition for integration with optoelectronic devices. C1 [Bae, Youn Jue] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Williams, Teresa E.] Univ Calif Berkeley, Grad Grp Appl Sci & Technol, Berkeley, CA 94720 USA. [Bae, Youn Jue; Cho, Eun Seon; Qu, Fen; Williams, Teresa E.; Urban, Jeffrey J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA. [Queen, Wendy L.] EPFL, Inst Sci & Ingn Chim, CH-1051 Sion, Switzerland. RP Urban, JJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA.; Queen, WL (reprint author), EPFL, Inst Sci & Ingn Chim, CH-1051 Sion, Switzerland. EM jjurban@lbl.gov; wendy.queen@epfl.ch RI Cho, Eun Seon/D-2658-2017 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Swiss National Science Foundation [PYAPP2_160581]; Center for Gas Separations Relevant to Clean Energy Technologies; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Department of Energy (DOE) through the Bay Area Photovoltaic Consortium (BAPVC) [DE-EE0004946]; U.S. Department of Energy (Office of Science, Office of Basic Energy Sciences, and Energy Efficiency and Renewable Energy, Solar Energy Technology Program) [DE-AC36-08GO28308]; Government of India, through the Department of Science and Technology [DE-AC36-08GO28308]; Berkeley Lab; Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Work at the Molecular Foundry and the ALS was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. W. Q acknowledges support from the Swiss National Science Foundation under grant number PYAPP2_160581. Y. B. acknowledges support provided by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001015. The formation of the mixed-matrix membranes is based upon work supported by the Department of Energy (DOE) through the Bay Area Photovoltaic Consortium (BAPVC) under Award Number DE-EE0004946 and also in part under the US-India Partnership to Advance Clean Energy-Research (PACE-R) for the Solar Energy Research Institute for India and the United States (SERIIUS), funded jointly by the U.S. Department of Energy (Office of Science, Office of Basic Energy Sciences, and Energy Efficiency and Renewable Energy, Solar Energy Technology Program, under Subcontract DE-AC36-08GO28308 to the National Renewable Energy Laboratory, Golden, Colorado) and the Government of India, through the Department of Science and Technology under Subcontract IUSSTF/JCERDC-SERIIUS/2012 dated 22nd Nov. 2012. The authors greatly thank Dupont Teijin Films for providing the PET substrate. The authors thank Christine Beavers of the Advanced Light Source for her assistance in obtaining powder x-ray diffraction data on BL 12.2.2. D.S. acknowledges support by Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 30 TC 4 Z9 4 U1 25 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 27 PY 2016 VL 8 IS 16 BP 10098 EP 10103 DI 10.1021/acsami.6b01299 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DK9IW UT WOS:000375245100005 PM 27071544 ER PT J AU Zheng, D Yang, XQ Qu, DY AF Zheng, Dong Yang, Xiao-Qing Qu, Deyang TI Stability of the Solid Electrolyte Interface on the Li Electrode in Li-S Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE SEI stability; lithium-sulfur battery; HPLC; polysulfide identification; Li sulfur reaction ID LITHIUM-SULFUR BATTERIES; ELECTROCHEMICAL REDUCTION; LIQUID ELECTROLYTES; POLYSULFIDES; DISCHARGE; CATHODES AB By means of high performance liquid chromatography-mass spectroscopy, the concentration of sulfur and polysulfides was determined in nonaqueous electrolytes. The stability of sulfur and Li in eight electrolytes was studied quantitatively. It was found that sulfur reacted with Li in most of the commonly used electrolytes for lithium-sulfur batteries. The reaction products between sulfur and Li were qualitatively identified. In some cases, the solid electrolyte interface on the Li can successfully prevent the interaction between S and Li; however, it was found that the solid electrolyte interface was damaged by polysulfide ions. C1 [Zheng, Dong; Qu, Deyang] Univ Wisconsin, Coll Engn & Appl Sci, Dept Mech Engn, Milwaukee, WI 53211 USA. [Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Qu, DY (reprint author), Univ Wisconsin, Coll Engn & Appl Sci, Dept Mech Engn, Milwaukee, WI 53211 USA. EM qud@uwm.edu RI Zheng, Dong/J-9975-2015 OI Zheng, Dong/0000-0002-5824-3270 FU Office of Vehicle Technologies, under the program of Vehicle Technology Program [DE-SC0012704] FX The authors from UWM and BNL are indebted to the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under the program of Vehicle Technology Program, under Contract DE-SC0012704. NR 18 TC 2 Z9 2 U1 24 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 27 PY 2016 VL 8 IS 16 BP 10360 EP 10366 DI 10.1021/acsami.6b02242 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DK9IW UT WOS:000375245100034 PM 27045986 ER PT J AU Kim, J Kim, J Jo, S Kang, J Jo, JW Lee, M Moon, J Yang, L Kim, MG Kim, YH Park, SK AF Kim, Jaehyun Kim, Jaekyun Jo, Sangho Kang, Jingu Jo, Jeong-Wan Lee, Myungwon Moon, Juhyuk Yang, Lin Kim, Myung-Gil Kim, Yong-Hoon Park, Sung Kyu TI Ultrahigh Detective Heterogeneous Photosensor Arrays with In-Pixel Signal Boosting Capability for Large-Area and Skin-Compatible Electronics SO ADVANCED MATERIALS LA English DT Article ID HIGH-PERFORMANCE; PHOTODETECTORS; FILMS; TRANSISTORS; SENSOR; PHOTOTRANSISTORS; NANOCOMPOSITES; TRANSPARENT; PHOTODIODES; PRESSURE AB An ultra-thin and large-area skin-compatible heterogeneous organic/metal-oxide photosensor array is demonstrated which is capable of sensing and boosting signals with high detectivity and signal-to-noise ratio. For the realization of ultra-flexible and high-sensitive heterogeneous photosensor arrays on a polyimide substrate having organic sensor arrays and metal-oxide boosting circuitry, solution-processing and room-temperature alternating photochemical conversion routes are applied. C1 [Kim, Jaehyun; Kim, Jaekyun; Jo, Sangho; Kang, Jingu; Jo, Jeong-Wan; Park, Sung Kyu] Chung Ang Univ, Sch Elect & Elect Engn, Seoul 156756, South Korea. [Kim, Jaehyun] Hanbat Natl Univ, Dept Appl Mat Engn, Daejeon, South Korea. [Lee, Myungwon] LG Elect, Mat & Devices Adv Res Inst, Seoul, South Korea. [Moon, Juhyuk] SUNY Stony Brook, Dept Mech Engn, Civil Engn Program, Stony Brook, NY USA. [Yang, Lin] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Kim, Myung-Gil] Chung Ang Univ, Dept Chem, Seoul 156756, South Korea. [Kim, Yong-Hoon] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea. [Kim, Yong-Hoon] Sungkyunkwan Univ, SKKU Adv Inst Nanotechnol SAINT, Suwon 440746, South Korea. RP Park, SK (reprint author), Chung Ang Univ, Sch Elect & Elect Engn, Seoul 156756, South Korea.; Kim, YH (reprint author), Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea.; Kim, YH (reprint author), Sungkyunkwan Univ, SKKU Adv Inst Nanotechnol SAINT, Suwon 440746, South Korea. EM yhkim76@skku.edu; skpark@cau.ac.kr RI park, sung kyu/H-5338-2011; OI Moon, Juhyuk/0000-0002-7049-892X FU National Research Foundation of Korea (NRF) - Korea government (MSIP) [NRF-2013R1A2A2A01006404]; Chung-Ang University FX J.K. and J.K. contributed equally to this work. This research was partially supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIP) (Grant No. NRF-2013R1A2A2A01006404) and by the Chung-Ang University Research Scholarship Grants in 2015. NR 41 TC 2 Z9 2 U1 28 U2 47 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 27 PY 2016 VL 28 IS 16 BP 3078 EP 3086 DI 10.1002/adma.201505149 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DK0BM UT WOS:000374577400004 PM 26928606 ER PT J AU Poole, ZL Ohodnicki, PR AF Poole, Zsolt L. Ohodnicki, Paul R. TI Thermal Emissivity-Based Chemical Spectroscopy through Evanescent Tunneling SO ADVANCED MATERIALS LA English DT Article ID SELECTIVE EMITTER; OPTICAL-FIBERS; RADIATION; SENSORS; ENERGY; TEMPERATURES; SURFACE AB A new spectroscopic technique is presented, with which environmental-chemistry-induced thermal emissivity changes of thin films are extracted with high isolation through evanescent tunneling. With this method the hydrogen-induced emissivity changes of films of TiO2, Pd-TiO2, and Au-TiO2, with properties of high conductivity, hydrogen chemisorption, and plasmonic activity, are characterized in the UV-vis and NIR wavelength ranges, at 1073 K. C1 [Poole, Zsolt L.; Ohodnicki, Paul R.] Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. RP Poole, ZL (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM Zsolt.Poole@NETL.DOE.GOV FU U.S. DOE Advanced Research/Crosscutting Technologies program at the National Energy Technology Laboratory; U.S. Department of Energy; agency of the United States Government FX The authors acknowledge Thomas D. Brown for assistance and support with instrumentation and Dr. Michael Carpenter for useful discussion. This work was funded by the U.S. DOE Advanced Research/Crosscutting Technologies program at the National Energy Technology Laboratory. This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, expresses or implies, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 35 TC 0 Z9 0 U1 9 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 27 PY 2016 VL 28 IS 16 BP 3111 EP 3114 DI 10.1002/adma.201505758 PG 4 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DK0BM UT WOS:000374577400008 PM 26901747 ER PT J AU Hofmann, S Heinz, S Mann, R Maurer, J Munzenberg, G Antalic, S Barth, W Dahl, L Eberhardt, K Grzywacz, R Hamilton, JH Henderson, RA Kenneally, JM Kindler, B Kojouharov, I Lang, R Lommel, B Miernik, K Miller, D Moody, KJ Morita, K Nishio, K Popeko, AG Roberto, JB Runke, J Rykaczewski, KP Scheidenberger, C Shaughnessy, DA Stoyer, MA Thorle-Pospiech, P Tinschert, K Trautmann, N Uusitalo, J Yeremin, AV AF Hofmann, S. Heinz, S. Mann, R. Maurer, J. Muenzenberg, G. Antalic, S. Barth, W. Dahl, L. Eberhardt, K. Grzywacz, R. Hamilton, J. H. Henderson, R. A. Kenneally, J. M. Kindler, B. Kojouharov, I. Lang, R. Lommel, B. Miernik, K. Miller, D. Moody, K. J. Morita, K. Nishio, K. Popeko, A. G. Roberto, J. B. Runke, J. Rykaczewski, K. P. Scheidenberger, C. Shaughnessy, D. A. Stoyer, M. A. Thoerle-Pospiech, P. Tinschert, K. Trautmann, N. Uusitalo, J. Yeremin, A. V. TI Remarks on the fission barriers of super-heavy nuclei SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID HEAVIEST NUCLEI; MASSES; DEFORMATIONS; STABILITY; ELEMENTS; FUSION; MODEL AB Shell-correction energies of super-heavy nuclei are approximated by using Q(alpha) values of measured decay chains. Five decay chains were analyzed, which start at the isotopes (285)Fl, (294)118, (291)Lv, (292)Lv and (293)Lv. The data are compared with predictions of macroscopic-microscopic models. Fission barriers are estimated that can be used to eliminate uncertainties in partial fission half-lives and in calculations of evaporation-residue cross-sections. In that calculations, fission probability of the compound nucleus is a major factor contributing to the total cross-section. The data also provide constraints on the cross-sections of capture and quasi-fission in the entrance channel of the fusion reaction. Arguments are presented that fusion reactions for synthesis of isotopes of elements 118 and 120 may have higher cross-sections than assumed so far. C1 [Hofmann, S.; Heinz, S.; Mann, R.; Maurer, J.; Muenzenberg, G.; Barth, W.; Dahl, L.; Kindler, B.; Kojouharov, I.; Lang, R.; Lommel, B.; Runke, J.; Scheidenberger, C.; Tinschert, K.] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. [Hofmann, S.] Univ Frankfurt, Inst Phys, D-60438 Frankfurt, Germany. [Antalic, S.] Comenius Univ, Dept Nucl Phys & Biophys, Bratislava 84248, Slovakia. [Eberhardt, K.; Thoerle-Pospiech, P.; Trautmann, N.] Univ Mainz, D-55128 Mainz, Germany. [Grzywacz, R.; Miernik, K.; Roberto, J. B.; Rykaczewski, K. P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Grzywacz, R.; Miller, D.] Univ Tennessee, Knoxville, TN 37996 USA. [Hamilton, J. H.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Henderson, R. A.; Kenneally, J. M.; Moody, K. J.; Shaughnessy, D. A.; Stoyer, M. A.] Univ Calif Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Miernik, K.] Univ Warsaw, Warsaw, Poland. [Morita, K.] RIKEN, Nishina Ctr Accelerator Based Sci, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Nishio, K.] Japan Atom Energy Agcy, Tokai, Ibaraki 3191195, Japan. [Popeko, A. G.; Yeremin, A. V.] Joint Inst Nucl Res, Dubna 141980, Russia. [Uusitalo, J.] Univ Jyvaskyla, Dept Phys, SF-40351 Jyvaskyla, Finland. RP Hofmann, S (reprint author), GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany.; Hofmann, S (reprint author), Univ Frankfurt, Inst Phys, D-60438 Frankfurt, Germany. EM S.Hofmann@gsi.de OI Roberto, James/0000-0002-4234-0252; Miller, David/0000-0002-0426-974X FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Slovak grant agency VEGA [1/0576/13]; Slovak Research and Development Agency [APVV-0105-10] FX We gratefully acknowledge stimulating discussions with Walter Greiner, Peter Moller and Adam Sobiczewski, who also supplied us with results of calculations prior to publication. Delightful discussions with Gurgen G. Adamian and Nikolai V. Antonenko are gratefully acknowledged. The work at LLNL was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. SA acknowledges support from the Slovak grant agency VEGA (contract No. 1/0576/13) and the Slovak Research and Development Agency (contract No. APVV-0105-10). NR 56 TC 4 Z9 4 U1 7 U2 12 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD APR 27 PY 2016 VL 52 IS 4 AR 116 DI 10.1140/epja/i2016-16116-0 PG 12 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DK5TQ UT WOS:000374983900001 ER PT J AU Aoun, B Pellegrini, E Trapp, M Natali, F Cantu, L Brocca, P Gerelli, Y Deme, B Koza, MM Johnson, M Peters, J AF Aoun, Bachir Pellegrini, Eric Trapp, Marcus Natali, Francesca Cantu, Laura Brocca, Paola Gerelli, Yuri Deme, Bruno Koza, Michael Marek Johnson, Mark Peters, Judith TI Direct comparison of elastic incoherent neutron scattering experiments with molecular dynamics simulations of DMPC phase transitions SO EUROPEAN PHYSICAL JOURNAL E LA English DT Article ID LIPID-BILAYERS; X-RAY; DIMYRISTOYLPHOSPHATIDYLCHOLINE BILAYERS; PHOSPHOLIPID-MEMBRANES; COMPUTER-SIMULATIONS; CHAIN-LENGTH; PRESSURE; TEMPERATURE; PROTEIN; GEL AB Neutron scattering techniques have been employed to investigate 1,2-dimyristoyl-sn -glycero-3-phosphocholine (DMPC) membranes in the form of multilamellar vesicles (MLVs) and deposited, stacked multilamellar-bilayers (MLBs), covering transitions from the gel to the liquid phase. Neutron diffraction was used to characterise the samples in terms of transition temperatures, whereas elastic incoherent neutron scattering (EINS) demonstrates that the dynamics on the sub-macromolecular length-scale and pico- to nano-second time-scale are correlated with the structural transitions through a discontinuity in the observed elastic intensities and the derived mean square displacements. Molecular dynamics simulations have been performed in parallel focussing on the length-, time- and temperature-scales of the neutron experiments. They correctly reproduce the structural features of the main gel-liquid phase transition. Particular emphasis is placed on the dynamical amplitudes derived from experiment and simulations. Two methods are used to analyse the experimental data and mean square displacements. They agree within a factor of 2 irrespective of the probed time-scale, i.e. the instrument utilized. Mean square displacements computed from simulations show a comparable level of agreement with the experimental values, albeit, the best match with the two methods varies for the two instruments. Consequently, experiments and simulations together give a consistent picture of the structural and dynamical aspects of the main lipid transition and provide a basis for future, theoretical modelling of dynamics and phase behaviour in membranes. The need for more detailed analytical models is pointed out by the remaining variation of the dynamical amplitudes derived in two different ways from experiments on the one hand and simulations on the other. C1 [Aoun, Bachir; Pellegrini, Eric; Natali, Francesca; Gerelli, Yuri; Deme, Bruno; Koza, Michael Marek; Johnson, Mark; Peters, Judith] Inst Laue Langevin, 71 Ave Martyrs,CS 20156, F-38042 Grenoble 9, France. [Trapp, Marcus] Heidelberg Univ, Angew Phys Chem, Neuenheimer Feld 253, D-69120 Heidelberg, Germany. [Trapp, Marcus] Helmholtz Zentrum Berlin Mat & Energie, Lise Meitner Campus,Hahn Meitner Pl 1, D-14109 Berlin, Germany. [Natali, Francesca] Inst Laue Langevin, CNR IOM OGG, 71 Ave Martyrs,CS 20156, F-38042 Grenoble 9, France. [Cantu, Laura; Brocca, Paola] Univ Milan, Via F Lli Cervi 93, I-20090 Segrate, Italy. [Peters, Judith] Univ Grenoble Alpes, LiPhy, UFR PhITEM, 71 Ave Martyrs,CS 10090, F-38044 Grenoble, France. [Aoun, Bachir] Argonne Natl Lab, 9700 South Cass Ave,Build 433 E095, Lemont, IL USA. RP Peters, J (reprint author), Inst Laue Langevin, 71 Ave Martyrs,CS 20156, F-38042 Grenoble 9, France.; Peters, J (reprint author), Univ Grenoble Alpes, LiPhy, UFR PhITEM, 71 Ave Martyrs,CS 10090, F-38044 Grenoble, France. EM peters@ill.fr RI Trapp, Marcus/F-9448-2010; OI Trapp, Marcus/0000-0002-5648-9584; Peters, Judith/0000-0001-5151-7710 NR 55 TC 0 Z9 0 U1 10 U2 27 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1292-8941 EI 1292-895X J9 EUR PHYS J E JI Eur. Phys. J. E PD APR 27 PY 2016 VL 39 IS 4 AR 48 DI 10.1140/epje/i2016-16048-y PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA DK5UC UT WOS:000374985200001 PM 27112937 ER PT J AU Whyatt, GA Freeman, CJ Zwoster, A Heldebrant, DJ AF Whyatt, Greg A. Freeman, Charles J. Zwoster, Andy Heldebrant, David J. TI Measuring Nitrous Oxide Mass Transfer into Non-Aqueous CO2BOL CO2 Capture Solvents SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CARBON-DIOXIDE; IONIC LIQUIDS; GREEN CHEMISTRY; ABSORPTION RATE; SOLUBILITY; WATER; N2O; ALKANOLAMINES; PIPERAZINE; PRESSURES AB This paper investigates CO2 absorption behavior in CO2BOL solvents by decoupling the physical and chemical effects using N2O as a nonreactive mimic. Absorption measurements were performed using a wetted-wall contactor. Testing was performed using a "first generation" CO2-binding organic liquid (CO2BOL), composed of an independent base and alcohol. Measurements were made with N2O at a lean (0.06 mol CO2/mol BOL) and rich (0.26 mol CO2/mol BOL) loading, each at three temperatures (35, 45, and 55 degrees C). Liquid-film mass transfer coefficients (kg') were calculated by subtracting the gas film resistance-determined from a correlation from literature-from the overall mass transfer measurement. The resulting kg' values for N2O in CO(2)BOLs were found to be higher than that of 5 M aqueous MEA under comparable conditions, which is supported by published measurements of Henrys coefficients for N2O in various solvents. These results suggest that the physical solubility contribution for CO2 absorption in CO(2)BOLs is greater than that of aqueous amines, an effect that may pertain to other nonaqueous solvents. C1 [Whyatt, Greg A.; Freeman, Charles J.; Zwoster, Andy; Heldebrant, David J.] Pacific NW Natl Lab, Richland, WA 99325 USA. RP Heldebrant, DJ (reprint author), Pacific NW Natl Lab, Richland, WA 99325 USA. EM david.heldebrant@pnnl.gov FU Department of Energy's Office of Fossil Energy's Carbon Capture Simulation Initiative (CCSI) FX Funding for this work was provided by the Department of Energy's Office of Fossil Energy's Carbon Capture Simulation Initiative (CCSI). NR 39 TC 1 Z9 1 U1 9 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 27 PY 2016 VL 55 IS 16 BP 4720 EP 4725 DI 10.1021/acs.iecr.6b00390 PG 6 WC Engineering, Chemical SC Engineering GA DK9IU UT WOS:000375244900034 ER PT J AU Aussignargues, C Pandelia, ME Sutter, M Plegaria, JS Zarzycki, J Turmo, A Huang, JC Ducat, DC Hegg, EL Gibney, BR Kerfeld, CA AF Aussignargues, Clement Pandelia, Maria-Eirini Sutter, Markus Plegaria, Jefferson S. Zarzycki, Jan Turmo, Aiko Huang, Jingcheng Ducat, Daniel C. Hegg, Eric L. Gibney, Brian R. Kerfeld, Cheryl A. TI Structure and Function of a Bacterial Microcompartment Shell Protein Engineered to Bind a [4Fe-4S] Cluster SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IRON-SULFUR CLUSTERS; DE-NOVO DESIGN; CARBOXYSOME SHELL; CRYSTAL-STRUCTURES; FERREDOXIN; CONSTRUCTION; SITE; IDENTIFICATION; RESOLUTION; ORGANELLES AB Bacterial microcompartments (BMCs) are self-assembling organelles composed of a selectively permeable protein shell and encapsulated enzymes. They are considered promising templates for the engineering of designed bionanoreactors for biotechnology. In particular, encapsulation of oxidoreductive reactions requiring electron transfer between the lumen of the BMC and the cytosol relies on the ability to conduct electrons across the shell. We determined the crystal structure of a component protein of a synthetic BMC shell, which informed the rational design of a [4Fe-4S] cluster-binding site in its pore. We also solved the structure of the [4Fe-4S] cluster-bound, engineered protein to 1.8 A resolution, providing the first structure of a BMC shell protein containing a metal center. The [4Fe-45] cluster was characterized by optical and EPR spectroscopies; it has a reduction potential of -370 mV vs the standard hydrogen electrode (SHE) and is stable through redox cycling. This remarkable stability may be attributable to the hydrogen-bonding network provided by the main chain of the protein scaffold. The properties of the [4Fe-4S] cluster resemble those in low-potential bacterial ferredoxins, while its ligation to three cysteine residues is reminiscent of enzymes such as aconitase and radical S-adenosymethionine (SAM) enzymes. This engineered shell protein provides the foundation for conferring electron-transfer functionality to BMC shells. C1 [Aussignargues, Clement; Sutter, Markus; Plegaria, Jefferson S.; Zarzycki, Jan; Turmo, Aiko; Huang, Jingcheng; Ducat, Daniel C.; Kerfeld, Cheryl A.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Huang, Jingcheng; Ducat, Daniel C.; Hegg, Eric L.; Kerfeld, Cheryl A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Pandelia, Maria-Eirini] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Sutter, Markus; Kerfeld, Cheryl A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys Biochem, Berkeley, CA 94720 USA. [Gibney, Brian R.] CUNY Brooklyn Coll, Dept Chem, Brooklyn, NY 11210 USA. [Gibney, Brian R.] CUNY, Grad Ctr, PhD Programs Chem & Biochem, New York, NY 10016 USA. [Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Kerfeld, Cheryl A.] Berkeley Synthet Biol Inst, Berkeley, CA 94720 USA. Max Planck Inst Terr Microbiol, D-35043 Marburg, Germany. [Pandelia, Maria-Eirini] Brandeis Univ, Dept Biochem, Waltham, MA 02453 USA. RP Kerfeld, CA (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys Biochem, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Berkeley Synthet Biol Inst, Berkeley, CA 94720 USA. EM ckerfeld@lbl.gov FU Office of Science of the U.S. Department of Energy [DE-FG02-91ER20021]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; EU FP7 project PEPDIODE [GA 256672] FX This work was supported by the Office of Science of the U.S. Department of Energy DE-FG02-91ER20021 and with infrastructure support from MSU AgBio Research. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under contract no. DE-AC02-76SF00515. B.R.G. acknowledges support from EU FP7 project PEPDIODE (GA 256672). The authors would like to thank Dr. Jonathan Lassila and Susan Bernstein for the construction of the plasmid carrying hoch_5812, Prof. John McCracken for the preliminary EPR experiments, and all members of the Kerfeld Lab for helpful discussions. NR 57 TC 6 Z9 6 U1 9 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 27 PY 2016 VL 138 IS 16 BP 5262 EP 5270 DI 10.1021/jacs.5b11734 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DK9IS UT WOS:000375244700021 PM 26704697 ER PT J AU Glavic, A Dixit, H Cooper, VR Aczel, AA AF Glavic, Artur Dixit, Hemant Cooper, Valentino R. Aczel, Adam A. TI Constructing a magnetic handle for antiferromagnetic manganites SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; FERROELECTRIC POLARIZATION; EXCHANGE-ANISOTROPY; ELECTRON-GAS; BASIS-SET; SUPERLATTICES; SCATTERING; NEUTRONS; MULTIFERROICS AB An intrinsic property of antiferromagnetic materials is the compensation of the magnetic moments from the individual atoms that prohibits the direct interaction of the spin lattice with an external magnetic field. To overcome this limitation we have created artificial spin structures by heteroepitaxy between two bulk antiferromagnets SrMnO3 and NdMnO3. Here, we demonstrate that charge transfer at the interface results in the creation of thin ferromagnetic layers adjacent to A-type antiferromagnetism in thick NdMnO3 layers. A novel interference based neutron diffraction technique and polarized neutron reflectometry are used to confirm the presence of ferromagnetism in the SrMnO3 layers and to probe the relative alignment of antiferromagnetic spins induced by the coupling at the ferro-to antiferromagnet interface. A density functional theory analysis of the driving forces for the exchange reveals strong ferromagnetic interfacial coupling through quantifiable short range charge transfer. These results confirm a layer-by-layer control of magnetic arrangements that constitutes a promising step on a path towards isothermal magnetic control of antiferromagnetic arrangements as would be necessary in spin-based heterostructures like multiferroic devices. C1 [Glavic, Artur] Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. [Dixit, Hemant; Cooper, Valentino R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008,MS6114, Oak Ridge, TN 37831 USA. [Dixit, Hemant] GLOBALFOUNDRIES Engn Private Ltd, 9th Floor,N1 Bldg,Manyata Embassy Business Pk, Bangalore 560045, Karnataka, India. [Aczel, Adam A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, POB 2008,MS6475, Oak Ridge, TN 37831 USA. RP Glavic, A (reprint author), Paul Scherrer Inst, Lab Neutron Scattering & Imaging, CH-5232 Villigen, Switzerland. EM artur.glavic@psi.ch RI Cooper, Valentino /A-2070-2012; Glavic, Artur/B-3453-2015 OI Cooper, Valentino /0000-0001-6714-4410; Glavic, Artur/0000-0003-4951-235X FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We want to thank Satoshi Okamoto for useful discussion related to the analysis of the theoretical results and the late Michael Biegalski for his support during the PLD growth. A portion of this research at ORNL's High Flux Isotope Reactor and Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Sample preparation and characterization for this research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. H.D. and V.R.C were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (V.R.C). This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 0 Z9 0 U1 8 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 27 PY 2016 VL 93 IS 14 AR 140413 DI 10.1103/PhysRevB.93.140413 PG 6 WC Physics, Condensed Matter SC Physics GA DK5FL UT WOS:000374945100001 ER PT J AU Staar, P Jiang, M Hahner, R Schulthess, TC Maier, TA AF Staar, P. Jiang, M. Hahner, R. Schulthess, T. C. Maier, T. A. TI Interlaced coarse-graining for the dynamic cluster approximation SO PHYSICAL REVIEW B LA English DT Article ID ELECTRON-SYSTEMS; MONTE-CARLO AB The dynamical cluster approximation (DCA) and its DCA(+) extension use coarse-graining of the momentum space to reduce the complexity of quantum many-body problems, thereby mapping the bulk lattice to a cluster embedded in a dynamical mean-field host. Here, we introduce a new form of an interlaced coarse-graining and compare it with the traditional coarse-graining. While it gives a more localized self-energy for a given cluster size, we show that it leads to more controlled results with weaker cluster shape and smoother cluster size dependence, which converge to the results obtained from the standard coarse-graining with increasing cluster size. Most importantly, the new coarse-graining reduces the severity of the fermionic sign problem of the underlying quantum Monte Carlo cluster solver and thus allows for calculations on larger clusters. This enables the treatment of correlations longer ranged than those accessible with the standard coarse-graining and thus can allow for the evaluation of the exact infinite cluster size result via finite size scaling. As a demonstration, we study the hole-doped two-dimensional Hubbard model and show that the interlaced coarse-graining in combination with the extended DCA(+) algorithm permits the determination of the superconducting T-c on cluster sizes for which the results can be fit with a Kosterlitz-Thouless scaling law. C1 [Staar, P.] IBM Res Zurich, CH-8803 Ruschlikon, Switzerland. [Jiang, M.; Hahner, R.; Schulthess, T. C.] ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. [Maier, T. A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Maier, T. A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Staar, P (reprint author), IBM Res Zurich, CH-8803 Ruschlikon, Switzerland. RI Maier, Thomas/F-6759-2012 OI Maier, Thomas/0000-0002-1424-9996 FU Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program; MARVEL NCCR; DOE Office of Science User Facility [DE-AC05-00OR22725] FX We would like to thank Richard Scalettar for useful comments. Part of this research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research received generous support from the MARVEL NCCR and used resources of the Swiss National Supercomputing Center, as well as the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC05-00OR22725. NR 14 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 27 PY 2016 VL 93 IS 16 AR 165144 DI 10.1103/PhysRevB.93.165144 PG 6 WC Physics, Condensed Matter SC Physics GA DK5HY UT WOS:000374952200004 ER PT J AU Orrigo, SEA Rubio, B Fujita, Y Gelletly, W Agramunt, J Algora, A Ascher, P Bilgier, B Blank, B Caceres, L Cakirli, RB Ganioglu, E Gerbaux, M Giovinazzo, J Grevy, S Kamalou, O Kozer, HC Kucuk, L Kurtukian-Nieto, T Molina, F Popescu, L Rogers, AM Susoy, G Stodel, C Suzuki, T Tamii, A Thomas, JC AF Orrigo, S. E. A. Rubio, B. Fujita, Y. Gelletly, W. Agramunt, J. Algora, A. Ascher, P. Bilgier, B. Blank, B. Caceres, L. Cakirli, R. B. Ganioglu, E. Gerbaux, M. Giovinazzo, J. Grevy, S. Kamalou, O. Kozer, H. C. Kucuk, L. Kurtukian-Nieto, T. Molina, F. Popescu, L. Rogers, A. M. Susoy, G. Stodel, C. Suzuki, T. Tamii, A. Thomas, J. C. TI beta decay of the exotic T-z =-2 nuclei Fe-48, Ni-52, and Zn-56 SO PHYSICAL REVIEW C LA English DT Article ID RADIOACTIVE BEAM PRODUCTION; PROTON-RICH NUCLEI; 1ST OBSERVATION; SPECTROMETER; REGION; STATES; ARRAY AB The results of a study of the beta decays of three proton-rich nuclei with T-z = -2, namely Fe-48, Ni-52, and Zn-56, produced in an experiment carried out at GANIL, are reported. In all three cases we have extracted the half-lives and the total beta-delayed proton emission branching ratios. We have measured the individual beta-delayed protons and beta-delayed. rays and the branching ratios of the corresponding levels. Decay schemes have been determined for the three nuclei, and new energy levels are identified in the daughter nuclei. Competition between beta-delayed protons and. rays is observed in the de-excitation of the T = 2 isobaric analog states in all three cases. Absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. In addition, we discuss in detail the data analysis taking as a test case Zn-56, where the exotic beta-delayed gamma-proton decay has been observed. C1 [Orrigo, S. E. A.; Rubio, B.; Gelletly, W.; Agramunt, J.; Algora, A.; Molina, F.] Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain. [Fujita, Y.] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan. [Fujita, Y.; Suzuki, T.; Tamii, A.] Osaka Univ, Res Ctr Nucl Phys, Osaka 5670047, Japan. [Gelletly, W.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Algora, A.] Hungarian Acad Sci, Inst Nucl Res, H-4026 Debrecen, Hungary. [Ascher, P.; Blank, B.; Gerbaux, M.; Giovinazzo, J.; Grevy, S.; Kurtukian-Nieto, T.] Univ Bordeaux, CNRS, IN2P3, Ctr Etud Nucl Bordeaux Gradignan, F-33175 Gradignan, France. [Bilgier, B.; Cakirli, R. B.; Ganioglu, E.; Kozer, H. C.; Kucuk, L.; Susoy, G.] Istanbul Univ, Dept Phys, TR-34134 Istanbul, Turkey. [Caceres, L.; Kamalou, O.; Stodel, C.; Thomas, J. C.] CEA, DSM, CNRS, Grand Accelerateur Natl Ions Lourds,IN2P3, BP 55027, F-14076 Caen 5, France. [Molina, F.] Comis Chilena Energia Nucl, Casilla 188-D, Santiago, Chile. [Popescu, L.] CEN SCK, Boeretang 200, B-2400 Mol, Belgium. [Rogers, A. M.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Orrigo, SEA (reprint author), Univ Valencia, CSIC, Inst Fis Corpuscular, E-46071 Valencia, Spain. EM sonja.orrigo@ific.uv.es RI Popescu, Lucia/F-9964-2011; Molina, Francisco/D-5319-2014 OI Popescu, Lucia/0000-0003-1678-4260; Molina, Francisco/0000-0002-9459-1336 FU Spanish MICINN [FPA2008-06419-C02-01, FPA2011-24553]; Centro de Excelencia Severo Ochoa del IFIC Grant [SEV-2014-0398]; CPAN Consolider-Ingenio Programme [CSD2007-00042]; Junta para la Ampliacion de Estudios Programme (CSIC JAE-Doc contract) - FSE; ENSAR Project [262010]; MEXT, Japan [18540270, 22540310]; Japan-Spain coll. program of JSPS; CSIC; UK Science and Technology Facilities Council (STFC) [ST/F012012/1]; Region of Aquitaine; International Post Doctoral Research Fellowship Programme [TUBITAK 2219]; Alexander von Humboldt foundation; Max-Planck-Partner Group FX This work was supported by the Spanish MICINN Grants No. FPA2008-06419-C02-01, No. FPA2011-24553; Centro de Excelencia Severo Ochoa del IFIC Grant No. SEV-2014-0398; CPAN Consolider-Ingenio 2010 Programme Grant No. CSD2007-00042; Junta para la Ampliacion de Estudios Programme (CSIC JAE-Doc contract) cofinanced by FSE; ENSAR Project No. 262010; MEXT, Japan Grants No. 18540270 and No. 22540310; Japan-Spain coll. program of JSPS and CSIC; UK Science and Technology Facilities Council (STFC) Grant No. ST/F012012/1; Region of Aquitaine. E.G. acknowledges support by TUBITAK 2219 International Post Doctoral Research Fellowship Programme. R.B.C. acknowledges support by the Alexander von Humboldt foundation and the Max-Planck-Partner Group. We acknowledge the EXOGAM collaboration for the use of their clover detectors. We thank Professor I. Hamamoto and Dr. J. L. Tain for useful discussions. NR 43 TC 5 Z9 6 U1 10 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 27 PY 2016 VL 93 IS 4 AR 044336 DI 10.1103/PhysRevC.93.044336 PG 18 WC Physics, Nuclear SC Physics GA DK5JF UT WOS:000374955500002 ER PT J AU Ranea-Sandoval, IF Han, S Orsaria, MG Contrera, GA Weber, F Alford, MG AF Ranea-Sandoval, Ignacio F. Han, Sophia Orsaria, Milva G. Contrera, Gustavo A. Weber, Fridolin Alford, Mark G. TI Constant-sound-speed parametrization for Nambu-Jona-Lasinio models of quark matter in hybrid stars SO PHYSICAL REVIEW C LA English DT Article ID DYSON-SCHWINGER EQUATIONS; PHASE-TRANSITIONS; NEUTRON-STARS; COMPACT STARS; NJL-MODEL; EQUILIBRIUM-CONFIGURATIONS; GENERAL-RELATIVITY; FINITE-TEMPERATURE; NUCLEAR-MATTER; STELLAR CORES AB The discovery of pulsars as heavy as 2 solar masses has led astrophysicists to rethink the core compositions of neutron stars, ruling out many models for the nuclear equations of state (EoS). We explore the hybrid stars that occur when hadronic matter is treated in a relativistic mean-field approximation and quark matter is modeled by three-flavor local and nonlocal Nambu-Jona-Lasinio (NJL) models with repulsive vector interactions. The NJL models typically yield equations of state that feature a first-order transition to quark matter. Assuming that the quark-hadron surface tension is high enough to disfavor mixed phases and restricting to EoSs that allow stars to reach 2 solar masses, we find that the appearance of the quark-matter core either destabilizes the star immediately (this is typical for nonlocal NJL models) or leads to a very short hybrid star branch in the mass-radius relation (this is typical for local NJL models). Using the constant-sound-speed parametrization we can see that the reason for the near absence of hybrid stars is that the transition pressure is fairly high and the transition is strongly first order. C1 [Ranea-Sandoval, Ignacio F.; Orsaria, Milva G.; Contrera, Gustavo A.] Univ Nacl La Plata, Fac Ciencias Astron & Geofis, Grp Gravitac Astrofis & Cosmol, Paseo Bosque S-N, RA-1900 La Plata, Buenos Aires, Argentina. [Ranea-Sandoval, Ignacio F.; Orsaria, Milva G.] Consejo Nacl Invest Cient & Tecn, Godoy Cruz 2290, RA-1425 Buenos Aires, DF, Argentina. [Han, Sophia] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Han, Sophia] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Han, Sophia; Alford, Mark G.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Contrera, Gustavo A.] Fac Ciencias Exactas, CONICET, UNLP, IFLP, La Plata, Buenos Aires, Argentina. [Weber, Fridolin] San Diego State Univ, Dept Phys, 5500 Campanile Dr, San Diego, CA 92182 USA. [Weber, Fridolin] Univ Calif San Diego, Ctr Astrophys & Space Sci, La Jolla, CA 92093 USA. RP Ranea-Sandoval, IF; Orsaria, MG; Contrera, GA (reprint author), Univ Nacl La Plata, Fac Ciencias Astron & Geofis, Grp Gravitac Astrofis & Cosmol, Paseo Bosque S-N, RA-1900 La Plata, Buenos Aires, Argentina.; Ranea-Sandoval, IF; Orsaria, MG (reprint author), Consejo Nacl Invest Cient & Tecn, Godoy Cruz 2290, RA-1425 Buenos Aires, DF, Argentina.; Han, S (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.; Han, S (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA.; Han, S; Alford, MG (reprint author), Washington Univ, Dept Phys, St Louis, MO 63130 USA.; Contrera, GA (reprint author), Fac Ciencias Exactas, CONICET, UNLP, IFLP, La Plata, Buenos Aires, Argentina.; Weber, F (reprint author), San Diego State Univ, Dept Phys, 5500 Campanile Dr, San Diego, CA 92182 USA.; Weber, F (reprint author), Univ Calif San Diego, Ctr Astrophys & Space Sci, La Jolla, CA 92093 USA. EM iranea@fcaglp.unlp.edu.ar; jhan@physics.wustl.edu; morsaria@fcaglp.unlp.edu.ar; contrera@fisica.unlp.edu.ar; fweber@mail.sdsu.edu; alford@wuphys.wustl.edu FU U.S. National Science Foundation [PHY-1411708]; UNLP (Argentina) [11/G119, 11/X718]; CONICET (Argentina); U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-05ER41375]; DOE Topical Collaboration Neutrinos and Nucleosynthesis in Hot and Dense Matter [DE-SC0004955] FX F.W. is supported by the U.S. National Science Foundation under Grant No. PHY-1411708. I.F.R.-S., G.A.C., and M.G.O. acknowledge financial support by UNLP (Argentina), Projects No. 11/G119 and No. 11/X718 (G.A.C.) and by CONICET (Argentina). M.G.A. and S.H. are supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Award No. DE-FG02-05ER41375, and by the DOE Topical Collaboration Neutrinos and Nucleosynthesis in Hot and Dense Matter Contract No. DE-SC0004955. NR 79 TC 4 Z9 4 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 27 PY 2016 VL 93 IS 4 AR 045812 DI 10.1103/PhysRevC.93.045812 PG 12 WC Physics, Nuclear SC Physics GA DK5JF UT WOS:000374955500004 ER PT J AU Mannige, RV Whitelam, S AF Mannige, Ranjan V. Whitelam, Stephen TI Predicting the outcome of the growth of binary solids far from equilibrium SO PHYSICAL REVIEW E LA English DT Article ID KINETIC ISING-MODEL; MAGNETIC EDEN MODEL; NUCLEATION; TRANSITION; NUMBER; SIZE AB The growth of multicomponent structures in simulations and experiments often results in kinetically trapped, nonequilibrium objects. In such cases we have no general theoretical framework for predicting the outcome of the growth process. Here we use computer simulations to study the growth of two-component structures within a simple lattice model. We show that kinetic trapping happens for many choices of growth rate and intercomponent interaction energies, and that qualitatively distinct kinds of kinetic trapping are found in different regions of parameter space. In a region in which the low-energy structure is an "antiferromagnet" or "checkerboard," we show that the grown nonequilibrium structure displays a component-type stoichiometry that is different from the equilibrium one but is insensitive to growth rate and solution conditions. This robust nonequilibrium stoichiometry can be predicted via a mapping to the jammed random tiling of dimers studied by Flory, a finding that suggests a way of making defined nonequilibrium structures in experiment. C1 [Mannige, Ranjan V.; Whitelam, Stephen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Mannige, RV; Whitelam, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM rvmannige@lbl.gov; swhitelam@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of U.S. Department of Energy [DE-AC02-05CH11231] FX This work was done at the Molecular Foundry at Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 25 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 27 PY 2016 VL 93 IS 4 AR 042136 DI 10.1103/PhysRevE.93.042136 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DK5MB UT WOS:000374962900002 PM 27176283 ER PT J AU Davern, SM McKnight, TE Standaert, RF Morrell-Falvey, JL Shpak, ED Kalluri, UC Jelenska, J Greenberg, JT Mirzadeh, S AF Davern, Sandra M. McKnight, Timothy E. Standaert, Robert F. Morrell-Falvey, Jennifer L. Shpak, Elena D. Kalluri, Udaya C. Jelenska, Joanna Greenberg, Jean T. Mirzadeh, Saed TI Carbon Nanofiber Arrays: A Novel Tool for Microdelivery of Biomolecules to Plants SO PLOS ONE LA English DT Article ID POST-PHLOEM TRANSPORT; FLUORESCENT TRACERS; MOVEMENT PROTEIN; LUCIFER YELLOW; MOSAIC-VIRUS; MINOR VEINS; SIEVE TUBE; TRANSIENT TRANSFORMATION; SYMPLASTIC TRANSPORT; HYDRODYNAMIC RADII AB Effective methods for delivering bioprobes into the cells of intact plants are essential for investigating diverse biological processes. Increasing research on trees, such as Populus spp., for bioenergy applications is driving the need for techniques that work well with tree species. This report introduces vertically aligned carbon nanofiber (VACNF) arrays as a new tool for microdelivery of labeled molecules to Populus leaf tissue and whole plants. We demonstrated that VACNFs penetrate the leaf surface to deliver sub-microliter quantities of solution containing fluorescent or radiolabeled molecules into Populus leaf cells. Importantly, VACNFs proved to be gentler than abrasion with carborundum, a common way to introduce material into leaves. Unlike carborundum, VACNFs did not disrupt cell or tissue integrity, nor did they induce production of hydrogen peroxide, a typical wound response. We show that femtomole to picomole quantities of labeled molecules (fluorescent dyes, small proteins and dextran), ranging from 0.5-500 kDa, can be introduced by VACNFs, and we demonstrate the use of the approach to track delivered probes from their site of introduction on the leaf to distal plant regions. VACNF arrays thus offer an attractive microdelivery method for the introduction of biomolecules and other probes into trees and potentially other types of plants. C1 [Davern, Sandra M.; Standaert, Robert F.; Morrell-Falvey, Jennifer L.; Kalluri, Udaya C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [McKnight, Timothy E.] Oak Ridge Natl Lab, Elect & Elect Syst Res Div, Oak Ridge, TN USA. [Standaert, Robert F.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. [Mirzadeh, Saed] Oak Ridge Natl Lab, Nucl Secur & Isotope Technol Div, Oak Ridge, TN USA. [Standaert, Robert F.; Morrell-Falvey, Jennifer L.; Shpak, Elena D.] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN USA. [Jelenska, Joanna; Greenberg, Jean T.] Univ Chicago, Dept Mol Genet & Cell Biol, 920 E 58Th St, Chicago, IL 60637 USA. RP Standaert, RF (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA.; Standaert, RF (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA.; Standaert, RF (reprint author), Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN USA. EM standaertrf@ornl.gov RI Morrell-Falvey, Jennifer/A-6615-2011; OI Morrell-Falvey, Jennifer/0000-0002-9362-7528; Standaert, Robert/0000-0002-5684-1322; KALLURI, UDAYA/0000-0002-5963-8370 FU U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [ERKP-417]; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research, ERKP-417, http://science.energy.gov/ber/. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; We thank Dr. David Weston and Dr. Abhijit Karve for the CmPP16-1 DNA. We acknowledge Dr. Tim Tschaplinski and Dr. Mitch Doktycz for critical review of the manuscript. We thank Trish Lankford for technical assistance, and Zackary Moore for assistance with plant growth and maintenance. Nanofiber arrays were produced at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. We thank Dale Hensley and the CNMS for assistance with the production of nanofiber arrays. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 70 TC 0 Z9 0 U1 5 U2 10 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 27 PY 2016 VL 11 IS 4 AR e0153621 DI 10.1371/journal.pone.0153621 PG 25 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK5QZ UT WOS:000374976200031 PM 27119338 ER PT J AU Maiti, A Small, W Lewicki, JP Weisgraber, TH Duoss, EB Chinn, SC Pearson, MA Spadaccini, CM Maxwell, RS Wilson, TS AF Maiti, A. Small, W. Lewicki, J. P. Weisgraber, T. H. Duoss, E. B. Chinn, S. C. Pearson, M. A. Spadaccini, C. M. Maxwell, R. S. Wilson, T. S. TI 3D printed cellular solid outperforms traditional stochastic foam in long-term mechanical response SO SCIENTIFIC REPORTS LA English DT Article ID TIME-TEMPERATURE SUPERPOSITION; COMPOSITE-MATERIALS; NEGATIVE-STIFFNESS; METALS; RUBBER AB 3D printing of polymeric foams by direct-ink-write is a recent technological breakthrough that enables the creation of versatile compressible solids with programmable microstructure, customizable shapes, and tunable mechanical response including negative elastic modulus. However, in many applications the success of these 3D printed materials as a viable replacement for traditional stochastic foams critically depends on their mechanical performance and micro-architectural stability while deployed under long-term mechanical strain. To predict the long-term performance of the two types of foams we employed multi-year-long accelerated aging studies under compressive strain followed by a time-temperature- superposition analysis using a minimum-arc-length-based algorithm. The resulting master curves predict superior long-term performance of the 3D printed foam in terms of two different metrics, i.e., compression set and load retention. To gain deeper understanding, we imaged the microstructure of both foams using X-ray computed tomography, and performed finite-element analysis of the mechanical response within these microstructures. This indicates a wider stress variation in the stochastic foam with points of more extreme local stress as compared to the 3D printed material, which might explain the latter's improved long-term stability and mechanical performance. C1 [Maiti, A.; Small, W.; Lewicki, J. P.; Weisgraber, T. H.; Duoss, E. B.; Chinn, S. C.; Pearson, M. A.; Spadaccini, C. M.; Maxwell, R. S.; Wilson, T. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Maiti, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM maiti2@llnl.gov FU US. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We would like to sincerely thank Dr. Jim Schneider of National Security Campus, MO (formerly Kansas City Plant) for giving us access to the results of their load retention study on the stochastic foam material. This work was performed under the auspices of the US. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 30 TC 2 Z9 2 U1 19 U2 44 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 27 PY 2016 VL 6 AR 24871 DI 10.1038/srep24871 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK4QY UT WOS:000374905200001 PM 27117858 ER PT J AU Zarzycki, P Gilbert, B AF Zarzycki, Piotr Gilbert, Benjamin TI Long-Range Interactions Restrict Water Transport in Pyrophyllite Interlayers SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; CLAY-MINERALS; MONTMORILLONITE; DIFFUSION; HYSTERESIS; NANOPORES AB Water diffusion within smectite clay interlayers is reduced by confinement and hence is highly determined by the interlayer spacings that are adopted during swelling. However, a molecular understanding of the short-and long-range forces governing interlayer water structure and dynamics is lacking. Using molecular dynamics simulations of water intercalated between pyrophyllite (smectite prototype) layers we provide a detailed picture of the variation of interlayered water mobility accompanying smectite expansion. Subtle changes in hydrogen bond network structure cause significant changes in water mobility that is greater for stable hydration states and reduced for intermediate separations. By studying pyrophyllite with and without external water we reveal that long-range electrostatic forces apply a restraining effect upon interlayer water mobility. Our findings are relevant for broad range of confining nanostructures with walls thin enough to permit long-range interactions that could affect the mobility of confined solvent molecules and solute species. C1 [Zarzycki, Piotr] Polish Acad Sci, Inst Phys Chem, Warsaw, Poland. [Gilbert, Benjamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zarzycki, P (reprint author), Polish Acad Sci, Inst Phys Chem, Warsaw, Poland.; Gilbert, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM zarzycki.piotrek@gmail.com; bgilbert@lbl.gov RI Gilbert, Benjamin/E-3182-2010 FU Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, of the US. Department of Energy [DE-AC02-05CH11231]; Polish National Science Center [UMO-2011/03/B/ST5/02693] FX We thank Dr. Ian Bourg for valuable discussions about this work. B.G. was supported by the Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division, of the US. Department of Energy under Contract No. DE-AC02-05CH11231. P.Z. was supported by Polish National Science Center (grant UMO-2011/03/B/ST5/02693). NR 26 TC 0 Z9 0 U1 9 U2 26 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 27 PY 2016 VL 6 AR 25278 DI 10.1038/srep25278 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK4AH UT WOS:000374858100001 PM 27118164 ER PT J AU Dordevic, SV Foster, GM Wolf, MS Stojilovic, N Lei, H Petrovic, C Chen, Z Li, ZQ Tung, LC AF Dordevic, S. V. Foster, G. M. Wolf, M. S. Stojilovic, N. Lei, H. Petrovic, C. Chen, Z. Li, Z. Q. Tung, L. C. TI Fano q-reversal in topological insulator Bi2Se3 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE Bi2Se3; topological insulators; optical spectroscopy; magneto; optical spectroscopy ID CONDUCTION-BAND; SINGLE-CRYSTALS; RESONANCE; PHASE AB We studied the magneto-optical response of a canonical topological insulator Bi2Se3 with the goal of addressing a controversial issue of electron-phonon coupling. Magnetic-field induced modifications of reflectance are very pronounced in the infrared part of the spectrum, indicating strong electron-phonon coupling. This coupling causes an asymmetric line-shape of the 60 cm(-1) phonon mode, and is analyzed within the Fano formalism. The analysis reveals that the Fano asymmetry parameter (q) changes sign when the cyclotron resonance is degenerate with the phonon mode. To the best of our knowledge this is the first example of magnetic field driven q-reversal. C1 [Dordevic, S. V.; Foster, G. M.; Wolf, M. S.] Univ Akron, Dept Phys, Akron, OH 44325 USA. [Stojilovic, N.] Univ Wisconsin, Dept Phys & Astron, Oshkosh, WI 54901 USA. [Lei, H.; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Chen, Z.; Li, Z. Q.; Tung, L. C.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Tung, L. C.] Univ N Dakota, Dept Phys & Astron, Grand Forks, ND 58202 USA. [Lei, H.] Renmin Univ, Dept Phys, Beijing 100872, Peoples R China. RP Dordevic, SV (reprint author), Univ Akron, Dept Phys, Akron, OH 44325 USA. EM dsasa@uakron.edu RI Chen, Zhiguo/B-9192-2015 OI Chen, Zhiguo/0000-0002-8242-4784 FU University of Akron FRG; UW Oshkosh grant [FDM262]; US DOE [DE-SC00112704]; NSF [DMR-0654118]; State of Florida; DOE FX The authors thank A B Kuzmenko for useful discussions. SVD acknowledges the support from The University of Akron FRG. NS was supported with UW Oshkosh FDM262 grant. Work at Brookhaven is supported by the US DOE under Contract No. DE-SC00112704 (HL and CP). Magneto-optical measurements were carried out at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-0654118, by the State of Florida, and by the DOE. NR 35 TC 0 Z9 0 U1 3 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 27 PY 2016 VL 28 IS 16 AR 165602 DI 10.1088/0953-8984/28/16/165602 PG 5 WC Physics, Condensed Matter SC Physics GA DI4GB UT WOS:000373457300007 PM 27001951 ER PT J AU Gordon, RT Vannette, MD Strychalska, J Klimczuk, T Cava, RJ Prozorov, R AF Gordon, R. T. Vannette, M. D. Strychalska, J. Klimczuk, T. Cava, R. J. Prozorov, R. TI Superconductivity and itinerant ferromagnetism of Y9Co7 probed by ac susceptibility SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE itinerant ferromagnetism; superconductivity; tunnel diode resonator ID MAGNETIC SUPERCONDUCTOR; WEAK FERROMAGNETS; FIELD; TEMPERATURE AB The ac magnetic susceptibility of a single crystal sample of the compound Y9Co7 has been measured in applied dc fields ranging from 0-6.7 kOe by utilizing a tunnel diode resonator circuit. In agreement with previous measurements on this material, a superconducting transition has been observed to occur at T-SC approximate to 2.5 K. A broad maximum has been observed in the zero field susceptibility measurements from 2.5 K < T < 8 K and its behavior with applied dc magnetic fields is consistent with that of the itinerant ferromagnet ZrZn2, which supports previous claims of itinerant ferromagnetism in this compound. The susceptibility has also been measured as a function of applied magnetic field and the results indicate that the actual Curie temperature for this system is higher than that suggested by previous reports based on Arrott plots constructed from dc magnetization. C1 [Gordon, R. T.] Western Illinois Univ, Dept Phys, Macomb, IL 61455 USA. [Vannette, M. D.] Saginaw Valley State Univ, Dept Phys, University Ctr, MI 48710 USA. [Strychalska, J.; Klimczuk, T.] Gdansk Univ Technol, Fac Appl Phys, Narutowicza 11-12, PL-80233 Gdansk, Poland. [Cava, R. J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Gordon, R. T.; Vannette, M. D.; Prozorov, R.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Gordon, R. T.; Vannette, M. D.; Prozorov, R.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Prozorov, R (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA.; Prozorov, R (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM prozorov@ameslab.gov FU National Science Centre (Poland) [DEC-2012/07/E/ST3/00584] FX The research performed at Gdansk University of Technology was financially supported by National Science Centre (Poland) grant (DEC-2012/07/E/ST3/00584). NR 20 TC 0 Z9 0 U1 10 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 27 PY 2016 VL 28 IS 16 AR 166006 DI 10.1088/0953-8984/28/16/166006 PG 5 WC Physics, Condensed Matter SC Physics GA DI4GB UT WOS:000373457300018 PM 27022686 ER PT J AU Pilania, G Balachandran, PV Kim, C Lookman, T AF Pilania, Ghanshyam Balachandran, Prasanna V. Kim, Chiho Lookman, Turab TI Finding New Perovskite Halides via Machine Learning SO FRONTIERS IN MATERIALS LA English DT Article DE perovskites; informatics; support vector machines; formability; materials discovery ID AB-INITIO CALCULATIONS; POLYMER DIELECTRICS; FORMABILITY; DESIGN; CHEMISTRY; STABILITY; SOLIDS AB Advanced materials with improved properties have the potential to fuel future technological advancements. However, identification and discovery of these optimal materials for a specific application is a non-trivial task, because of the vastness of the chemical search space with enormous compositional and configurational degrees of freedom. Materials informatics provides an efficient approach toward rational design of new materials, via learning from known data to make decisions on new and previously unexplored compounds in an accelerated manner. Here, we demonstrate the power and utility of such statistical learning (or machine learning, henceforth referred to as ML) via building a support vector machine (SVM) based classifier that uses elemental features (or descriptors) to predict the formability of a given ABX(3) halide composition (where A and B represent monovalent and divalent cations, respectively, and X is F, Cl, Br, or I anion) in the perovskite crystal structure. The classification model is built by learning from a dataset of 185 experimentally known ABX(3) compounds. After exploring a wide range of features, we identify ionic radii, tolerance factor, and octahedral factor to be the most important factors for the classification, suggesting that steric and geometric packing effects govern the stability of these halides. The trained and validated models then predict, with a high degree of confidence, several novel ABX(3) compositions with perovskite crystal structure. C1 [Pilania, Ghanshyam] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM USA. [Balachandran, Prasanna V.; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Kim, Chiho] Univ Connecticut, Inst Mat Sci, Dept Mat Sci & Engn, Storrs, CT USA. RP Pilania, G (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM USA. EM gpilania@lanl.gov FU Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD); (U.S.) Department of Energy [DE-AC52-06NA25396] FX GP, PB and TL acknowledge support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the (U.S.) Department of Energy under contract DE-AC52-06NA25396. NR 39 TC 0 Z9 0 U1 3 U2 3 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2296-8016 J9 FRONT MATER JI Front. Mater. PD APR 26 PY 2016 VL 3 AR UNSP 19 DI 10.3389/fmats.2016.00019 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA EK0TP UT WOS:000393640300001 ER PT J AU Ma, J Wang, LW AF Ma, Jie Wang, Lin-Wang TI Using Wannier functions to improve solid band gap predictions in density functional theory SO SCIENTIFIC REPORTS LA English DT Article ID ANGLE-RESOLVED PHOTOEMISSION; DERIVATIVE DISCONTINUITIES; ELECTRON-AFFINITY; ORBITAL ENERGIES; INSULATORS; EXCHANGE AB Enforcing a straight-line condition of the total energy upon removal/addition of fractional electrons on eigen states has been successfully applied to atoms and molecules for calculating ionization potentials and electron affinities, but fails for solids due to the extended nature of the eigen orbitals. Here we have extended the straight-line condition to the removal/addition of fractional electrons on Wannier functions constructed within the occupied/unoccupied subspaces. It removes the self-interaction energies of those Wannier functions, and yields accurate band gaps for solids compared to experiments. It does not have any adjustable parameters and the computational cost is at the DFT level. This method can also work for molecules, providing eigen energies in good agreement with experimental ionization potentials and electron affinities. Our approach can be viewed as an alternative approach of the standard LDA+U procedure. C1 [Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wang, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM lwwang@lbl.gov FU Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub through the Office of Science of the U.S. Department of Energy [DESC0004993]; Theory of Materials Project at the LBNL by the Basic Energy Science, Material Science and Engineering, Office of Science of the U.S. Department of Energy [KC2301, DE-AC02-05CH11231] FX J.M is supported by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award No. DESC0004993. L.-W.W is supported through the Theory of Materials Project (KC2301) at the LBNL by the Basic Energy Science, Material Science and Engineering, Office of Science of the U.S. Department of Energy under Contracts No. DE-AC02-05CH11231. Computations are performed using resources of the National Energy Research Scientific Computing Center (NERSC) at the LBNL. NR 54 TC 2 Z9 2 U1 11 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 26 PY 2016 VL 6 AR 24924 DI 10.1038/srep24924 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK2PZ UT WOS:000374758200001 PM 27114185 ER PT J AU Rouet-Leduc, B Barros, K Lookman, T Humphreys, CJ AF Rouet-Leduc, Bertrand Barros, Kipton Lookman, Turab Humphreys, Colin J. TI Optimisation of GaN LEDs and the reduction of efficiency droop using active machine learning SO SCIENTIFIC REPORTS LA English DT Article ID QUANTUM-WELLS; PREDICTION AB A fundamental challenge in the design of LEDs is to maximise electro-luminescence efficiency at high current densities. We simulate GaN-based LED structures that delay the onset of efficiency droop by spreading carrier concentrations evenly across the active region. Statistical analysis and machine learning effectively guide the selection of the next LED structure to be examined based upon its expected efficiency as well as model uncertainty. This active learning strategy rapidly constructs a model that predicts Poisson-Schrodinger simulations of devices, and that simultaneously produces structures with higher simulated efficiencies. C1 [Rouet-Leduc, Bertrand; Humphreys, Colin J.] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Rouet-Leduc, Bertrand; Barros, Kipton; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Rouet-Leduc, B (reprint author), Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England.; Rouet-Leduc, B; Barros, K (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM br346@cam.ac.uk; kbarros@lanl.gov OI Barros, Kipton/0000-0002-1333-5972 FU Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR on Materials Informatics [20140013DR]; EPSRC [EP/I012591/1] FX B.R.-L., K.B. and T.L. acknowledge funding support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR (#20140013DR) on Materials Informatics. B.R.-L. and C.J.H. acknowledge funding support from the EPSRC Programme Grant "Lighting the Future" (#EP/I012591/1). NR 38 TC 1 Z9 1 U1 6 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 26 PY 2016 VL 6 AR 24862 DI 10.1038/srep24862 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK2PQ UT WOS:000374757300002 PM 27113018 ER PT J AU Vu, AD Coraux, J Chen, G N'Diaye, AT Schmid, AK Rougemaille, N AF Vu, A. D. Coraux, J. Chen, G. N'Diaye, A. T. Schmid, A. K. Rougemaille, N. TI Unconventional magnetisation texture in graphene/cobalt hybrids SO SCIENTIFIC REPORTS LA English DT Article ID ENERGY-ELECTRON MICROSCOPY; SENSITIZED SOLAR-CELLS; EPITAXIAL GRAPHENE; REORIENTATION TRANSITIONS; FERROMAGNETIC-FILMS; SUSPENDED GRAPHENE; ROOM-TEMPERATURE; SPIN TRANSPORT; ANISOTROPY; SPINTRONICS AB Magnetic domain structure and spin-dependent reflectivity measurements on cobalt thin films intercalated at the graphene/Ir(111)interface are investigated using spin-polarised low-energy electron microscopy. We find that graphene-covered cobalt films have surprising magnetic properties. Vectorial imaging of magnetic domains reveals an unusually gradual thickness-dependent spin reorientation transition, in which magnetisation rotates from out-of-the-film plane to the in-plane direction by less than 10 degrees per cobalt monolayer. During this transition, cobalt films have a meandering spin texture, characterised by a complex, three-dimensional, wavy magnetisation pattern. In addition, spectroscopy measurements suggest that the electronic band structure of the unoccupied states is essentially spin-independent already a few electron-Volts above the vacuum level. These properties strikingly differ from those of pristine cobalt films and could open new prospects in surface magnetism. C1 [Vu, A. D.; Coraux, J.; Rougemaille, N.] CNRS, Inst NEEL, F-38000 Grenoble, France. [Vu, A. D.; Coraux, J.; Rougemaille, N.] Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France. [Chen, G.; Schmid, A. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, NCEM, Berkeley, CA 94720 USA. [N'Diaye, A. T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Rougemaille, N (reprint author), CNRS, Inst NEEL, F-38000 Grenoble, France.; Rougemaille, N (reprint author), Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France. EM nicolas.rougemaille@neel.cnrs.fr RI Coraux, Johann/A-7897-2008; Chen, Gong/H-3074-2015 FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; French National Research Agency [ANR-12-BS-1000-401-NANOCELLS] FX Experiments were performed at the Molecular Foundry, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank the French National Research Agency for financial support via the ANR-12-BS-1000-401-NANOCELLS contract. The authors also thank W. Weber for fruitful discussions. NR 70 TC 2 Z9 2 U1 11 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 26 PY 2016 VL 6 AR 24783 DI 10.1038/srep24783 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK2PE UT WOS:000374756100002 PM 27114039 ER PT J AU Marangoni, MN Martynowycz, MW Kuzmenko, I Braun, D Polak, PE Weinberg, G Rubinstein, I Gidalevitz, D Feinstein, DL AF Marangoni, M. Natalia Martynowycz, Michael W. Kuzmenko, Ivan Braun, David Polak, Paul E. Weinberg, Guy Rubinstein, Israel Gidalevitz, David Feinstein, Douglas L. TI Membrane Cholesterol Modulates Superwarfarin Toxicity SO BIOPHYSICAL JOURNAL LA English DT Article ID WARFARIN; BRODIFACOUM; RESISTANCE; MUTATIONS; PHARMACOKINETICS; ANTICOAGULANTS; RODENTICIDE; MONOLAYERS; MECHANISM; WATER AB Superwarfarins are modified analogs of warfarin with additional lipophilic aromatic rings, up to 100-fold greater potency, and longer biological half-lives. We hypothesized that increased hydrophobicity allowed interactions with amphiphilic membranes and modulation of biological responses. We find that superwarfarins brodifacoum and difenacoum increase lactate production and cell death in neuroblastoma cells. In contrast, neither causes changes in glioma cells that have higher cholesterol content. After choleterol depletion, lactate production was increased and cell viability was reduced. Drug-membrane interactions were examined by surface X-ray scattering using Langmuir monolayers of dipalmitoylphosphatidylcholine and/or cholesterol. Specular X-ray reflectivity data revealed that superwarfarins, but not warfarin, intercalate between dipalmitoylphosphatidylcholine molecules, whereas grazing incidence X-ray diffraction demonstrated changes in lateral crystalline order of the film. Neither agent showed significant interactions with monolayers containing > 20% cholesterol. These findings demonstrate an affinity of superwarfarins to biomembranes and suggest that cellular responses to these agents are regulated by cholesterol content. C1 [Marangoni, M. Natalia; Braun, David; Polak, Paul E.; Weinberg, Guy; Feinstein, Douglas L.] Univ Illinois, Dept Anesthesiol, Chicago, IL USA. [Martynowycz, Michael W.; Gidalevitz, David] IIT, Dept Phys, Chicago, IL 60616 USA. [Martynowycz, Michael W.; Gidalevitz, David] IIT, Ctr Mol Study Condensed Soft Matter, Chicago, IL 60616 USA. [Martynowycz, Michael W.; Kuzmenko, Ivan] Argonne Natl Lab, Xray Sci Div, Lemont, IL USA. [Weinberg, Guy; Rubinstein, Israel; Feinstein, Douglas L.] Jesse Brown VA Med Ctr, Chicago, IL USA. [Rubinstein, Israel] Univ Illinois, Dept Med, Chicago, IL USA. RP Feinstein, DL (reprint author), Univ Illinois, Dept Anesthesiol, Chicago, IL USA. EM dlfeins@uic.edu FU National Institutes of Health [5U01NS083457]; Veterans Affairs Research Career Scientist Award; Veterans Affairs Merit grant; DARPA [W911NF-09-1-378]; Argonne National Laboratory's X-ray Science Division, Inelastic X-ray Nuclear Resonant Scattering group; U.S. Department of Energy [W-31-109-Eng-38] FX This work was supported by National Institutes of Health grant 5U01NS083457 to D.L.F., Veterans Affairs Research Career Scientist Award to D.L.F., Veterans Affairs Merit grant to G.W. and I.R., and DARPA grant W911NF-09-1-378 to D.G.M.W.M. was supported by Argonne National Laboratory's X-ray Science Division, Inelastic X-ray Nuclear Resonant Scattering group. Use of the Advanced Photon Source was supported by the U.S. Department of Energy under contract W-31-109-Eng-38 (I.K.). NR 41 TC 1 Z9 1 U1 6 U2 6 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD APR 26 PY 2016 VL 110 IS 8 BP 1777 EP 1788 DI 10.1016/j.bpj.2016.03.004 PG 12 WC Biophysics SC Biophysics GA DK4AV UT WOS:000374859600012 PM 27119638 ER PT J AU Chen, IMA Markowitz, VM Palaniappan, K Szeto, E Chu, K Huang, JH Ratner, A Pillay, M Hadjithomas, M Huntemann, M Mikhailova, N Ovchinnikova, G Ivanova, NN Kyrpides, NC AF Chen, I-Min A. Markowitz, Victor M. Palaniappan, Krishna Szeto, Ernest Chu, Ken Huang, Jinghua Ratner, Anna Pillay, Manoj Hadjithomas, Michalis Huntemann, Marcel Mikhailova, Natalia Ovchinnikova, Galina Ivanova, Natalia N. Kyrpides, Nikos C. TI Supporting community annotation and user collaboration in the integrated microbial genomes (IMG) system SO BMC GENOMICS LA English DT Article DE Gene annotation; Functional curation; Manual curation; IMG; Metagenomics; Microbial genomics ID PROKARYOTIC GENOMES; SEQUENCE AB Background: The exponential growth of genomic data from next generation technologies renders traditional manual expert curation effort unsustainable. Many genomic systems have included community annotation tools to address the problem. Most of these systems adopted a "Wiki-based" approach to take advantage of existing wiki technologies, but encountered obstacles in issues such as usability, authorship recognition, information reliability and incentive for community participation. Results: Here, we present a different approach, relying on tightly integrated method rather than "Wiki-based" method, to support community annotation and user collaboration in the Integrated Microbial Genomes (IMG) system. The IMG approach allows users to use existing IMG data warehouse and analysis tools to add gene, pathway and biosynthetic cluster annotations, to analyze/reorganize contigs, genes and functions using workspace datasets, and to share private user annotations and workspace datasets with collaborators. We show that the annotation effort using IMG can be part of the research process to overcome the user incentive and authorship recognition problems thus fostering collaboration among domain experts. The usability and reliability issues are addressed by the integration of curated information and analysis tools in IMG, together with DOE Joint Genome Institute (JGI) expert review. Conclusion: By incorporating annotation operations into IMG, we provide an integrated environment for users to perform deeper and extended data analysis and annotation in a single system that can lead to publications and community knowledge sharing as shown in the case studies. C1 [Chen, I-Min A.; Markowitz, Victor M.; Palaniappan, Krishna; Szeto, Ernest; Chu, Ken; Huang, Jinghua; Ratner, Anna; Pillay, Manoj] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Biosci Comp, Berkeley, CA 94720 USA. [Hadjithomas, Michalis; Huntemann, Marcel; Mikhailova, Natalia; Ovchinnikova, Galina; Ivanova, Natalia N.; Kyrpides, Nikos C.] DOE Joint Genome Inst, Prokaryot Super Program, Walnut Creek, CA USA. RP Chen, IMA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Biosci Comp, Berkeley, CA 94720 USA. EM imachen@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 FU U.S. Department of Energy [DE-AC02-05CH11231]; University of California FX Director, Office of Science, Office of Biological and Environmental Research, Life Sciences Division, U.S. Department of Energy (Contract No. DE-AC02-05CH11231); Office of Science of the U.S. Department of Energy (Contract No. DE-AC02-05CH11231, resources of the National Energy Research Scientific Computing Center). Funding for open access charge: University of California. NR 31 TC 6 Z9 6 U1 5 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD APR 26 PY 2016 VL 17 AR 307 DI 10.1186/s12864-016-2629-y PG 16 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA DK5EB UT WOS:000374941400001 PM 27118214 ER PT J AU Carino, EV Staszak-Jirkovsky, J Assary, RS Curtiss, LA Markovic, NM Brushett, FR AF Carino, Emily V. Staszak-Jirkovsky, Jakub Assary, Rajeev S. Curtiss, Larry A. Markovic, Nenad M. Brushett, Fikile R. TI Tuning the Stability of Organic Active Materials for Nonaqueous Redox Flow Batteries via Reversible, Electrochemically Mediated Li+ Coordination SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; DENSITY-FUNCTIONAL THEORY; SOLVATION FREE-ENERGIES; OXIDATION POTENTIALS; PROPYLENE CARBONATE; SHUTTLE ADDITIVES; DECOMPOSITION REACTIONS; OVERCHARGE PERFORMANCE; HYDROGEN ELECTRODE; STORAGE AB We describe an electrochemically mediated interaction between Li+ and a promising active material for nonaqueous redox flow batteries (RFBs), 1,2,3,4-tetrahydro-6,7-dimethoxy-1,1,4,4-tetramethylnaphthalene (TDT), and the impact of this structural interaction on material stability during voltammetric cycling. TDT could be an advantageous organic positive electrolyte material for nonaqueous RFBs due to its high oxidation potential, 4.21 V vs Li/Li+, and solubility of at least 1.0 M in select electrolytes. Although results from voltammetry suggest TDT displays Nernstian reversibility in many nonaqueous electrolyte solutions, bulk electrolysis reveals significant degradation in all electrolytes studied, the extent of which depends on the electrolyte solution composition. Results of subtractively normalized in situ Fourier transform infrared spectroscopy (SNIFTIRS) confirm that TDT undergoes reversible structural changes during cyclic voltammetry in propylene carbonate and 1,2-dimethoxyethane solutions containing Li+ electrolytes, but irreversible degradation occurs when tetrabutylammonium (TBA(+)) replaces Li+ as the electrolyte cation in these solutions. By combining the results from SNIFTIRS experiments with calculations from density functional theory, solution-phase active species structure and potential-dependent interactions can be determined. We find that Li+ coordinates to the Lewis basic methoxy groups of neutral TDT and, upon electrochemical oxidation, this complex dissociates into the radical cation TDT and Lit The improved cycling stability in the presence of Li+ relative to TBA(+) suggests that the structural interaction reported herein may be advantageous to the design of energy storage materials based on organic molecules. C1 [Carino, Emily V.; Staszak-Jirkovsky, Jakub; Assary, Rajeev S.; Curtiss, Larry A.; Markovic, Nenad M.; Brushett, Fikile R.] MIT, Joint Ctr Energy Storage Res, Cambridge, MA 02139 USA. [Carino, Emily V.; Brushett, Fikile R.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. [Staszak-Jirkovsky, Jakub; Assary, Rajeev S.; Curtiss, Larry A.; Markovic, Nenad M.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Staszak-Jirkovsky, Jakub] Machavert Pharmaceut LLC, Aurora, CO 80045 USA. RP Brushett, FR (reprint author), MIT, Joint Ctr Energy Storage Res, Cambridge, MA 02139 USA.; Brushett, FR (reprint author), MIT, Dept Chem Engn, Cambridge, MA 02139 USA. EM brushett@mit.edu FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences by Argonne National Laboratory's Materials Engineering Research Facility [ANL RS-21]; DOE-EERE Office of Vehicle Technologies. Argonne, a U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX The authors thank Bostjan Genorio, Ilya Shkrob, Lu Zhang, Steve Harris, and Jack Vaughey for insightful conversations. We thank Raja Selvakumar for assistance with the bulk electrolysis measurements. This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. TDT (available under the name "ANL RS-21") was generously provided by Argonne National Laboratory's Materials Engineering Research Facility and was funded by DOE-EERE Office of Vehicle Technologies. Argonne, a U.S. Department of Energy Office of Science Laboratory, is operated under Contract No. DE-AC02-06CH11357. NR 49 TC 1 Z9 1 U1 17 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 26 PY 2016 VL 28 IS 8 BP 2529 EP 2539 DI 10.1021/acs.chemmater.5b04053 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DK9IQ UT WOS:000375244500009 ER PT J AU Raja, SN Luong, AJ Zhang, WC Lin, LW Ritchie, RO Alivisatos, AP AF Raja, Shilpa N. Luong, Andrew J. Zhang, Wencong Lin, Liwei Ritchie, Robert O. Alivisatos, A. Paul TI Cavitation-Induced Stiffness Reductions in Quantum Dot-Polymer Nanocomposites SO CHEMISTRY OF MATERIALS LA English DT Article ID DYNAMIC-MECHANICAL PROPERTIES; RUBBER-TOUGHENED NYLON-6; YOUNGS MODULUS; THERMOPLASTIC POLYMERS; MATRIX COMPOSITES; NANOPARTICLE SIZE; FILLED COMPOSITES; FIBERS; NANOCRYSTALS; DEFORMATION AB The elastic stiffness of two polymer nano composite systems is investigated. The nanoscale fillers comprise cadmium selenide (CdSe, similar to 4 nm) and cadmium selenide/cadmium sulfide (CdSe/CdS, similar to 13 nm) quantum dots (QDs). The QDs are embedded within an electrospun structural block copolymer, poly(styrene-ethylene-butylene-styrene) (SEBS). Tensile testing shows a monotonic decrease in the tensile Young's modulus with increasing partially phase separated QD concentration; this is to be compared to corresponding nanocomposites reinforced with nanorod (NR) and tetrapod (TP)-SEBS nanocomposites which show a monotonic increase with particle loading. While most studies to date emphasize the increase in Young's modulus in polymer nanocomposites at higher reinforcement loadings, few focus on the tunability of the modulus from reductions in stiffness. The present work reveals up to an similar to 80% reduction in tensile Young's modulus with the addition of 5 vol % of QDs to electrospun SEBS. In this study, we sought mechanistic insight into this reduction in composite stiffness using a 2D lattice spring model. Simulation results reveal that the stiffness decrease with the addition of QD reinforcements is likely due to cavitation in the polymer in the vicinity of the QD aggregates arising from polymer debonding under tension. We anticipate that this study, performed with a commonly used structural rubber, may find use in designing polymer-matrix nanocomposite fibers with specific Young's moduli for applications requiring a tunable lower stiffness material. C1 [Raja, Shilpa N.; Ritchie, Robert O.; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Raja, Shilpa N.; Ritchie, Robert O.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Luong, Andrew J.; Zhang, Wencong] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. [Lin, Liwei; Ritchie, Robert O.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ritchie, RO; Alivisatos, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA.; Ritchie, RO; Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Ritchie, RO (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. EM roritchie@lbl.gov; apalivisatos@lbl.gov RI Ritchie, Robert/A-8066-2008 OI Ritchie, Robert/0000-0002-0501-6998 FU "Self-Assembly of Organic/Inorganic Nanocomposite Materials" program, Office of Science, the Office of Basic Energy Sciences (BES), Materials Sciences and Engineering (MSE) Division of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; NSF [ECCS-0901864] FX This work was supported by the "Self-Assembly of Organic/Inorganic Nanocomposite Materials" program, Office of Science, the Office of Basic Energy Sciences (BES), Materials Sciences and Engineering (MSE) Division of the U.S. Department of Energy (DOE), under Contract No. DE-AC02-05CH11231. The electrospinning work, performed by L.L., was supported by NSF Grant ECCS-0901864. NR 70 TC 4 Z9 4 U1 14 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 26 PY 2016 VL 28 IS 8 BP 2540 EP 2549 DI 10.1021/acs.chemmater.5b04165 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DK9IQ UT WOS:000375244500010 ER PT J AU Fauvell, TJ Zheng, TY Jackson, NE Ratner, MA Yu, LP Chen, LX AF Fauvell, Thomas J. Zheng, Tianyue Jackson, Nicholas E. Ratner, Mark A. Yu, Luping Chen, Lin X. TI Photophysical and Morphological Implications of Single-Strand Conjugated Polymer Folding in Solution SO CHEMISTRY OF MATERIALS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; CHARGE SEPARATION; ENERGY-TRANSFER; OLIGOMERS; PERFORMANCE; PTB7; AGGREGATION; COPOLYMER; DYNAMICS; FILM AB Organic semiconductors have garnered substantial interest in optoelectronics, but their device performances exhibit strong dependencies on material crystallinity and packing. In an effort to understand the interactions dictating the morphological and photophysical properties of a high-performing photovoltaic polymer, PTB7, a series of short oligomers and low molecular weight polymers of PTB7 were synthesized. Chain-length dependent optical studies of these oligomers demonstrate that PTB7's low-energy visible absorption is largely due to self-aggregation-induced ordering, rather than in chain charge transfer, as previously thought. By examining molecular weight and concentration dependent optical properties, supplemented by molecular dynamics simulations, we attribute polymeric PTB7's unique midgap fluorescence and concentration independent absorption spectrum to an interplay between low molecular weight unaggregated strands and high-molecular weight self-aggregated (folded) strands. Specifically, we propose that the onset of PTB7 self-folding occurs between 7 and 13 repeat units, but the aggregates characteristic of polymeric PTB7 only develop at lengths of similar to 30 repeat units. Atomistic molecular dynamics simulations of PTB7 corroborate these conclusions, and a simple relation is proposed which quantifies the free-energy of conjugated polymer folding. This study provides detailed guidance in the design of intra- and interchain contributions to the photophysical and morphological properties of polymeric semiconductors. C1 [Fauvell, Thomas J.; Jackson, Nicholas E.; Ratner, Mark A.; Chen, Lin X.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Fauvell, Thomas J.; Jackson, Nicholas E.; Ratner, Mark A.; Chen, Lin X.] Northwestern Univ, Argonne Northwestern Solar Energy Res ANSER Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Fauvell, Thomas J.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zheng, Tianyue; Yu, Luping] Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA. [Zheng, Tianyue; Yu, Luping] Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. RP Chen, LX (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Chen, LX (reprint author), Northwestern Univ, Argonne Northwestern Solar Energy Res ANSER Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Chen, LX (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.; Yu, LP (reprint author), Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA.; Yu, LP (reprint author), Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. EM lupingyu@uchicago.edu; l-chen@northwestern.edu RI Zheng, Tianyue/P-2674-2016 FU ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; Division of Chemical Sciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-06CH11357] FX This research was supported through the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-SC0001059, and the lab equipment was supported through the Division of Chemical Sciences, Office of Basic Energy Sciences, the U.S. Department of Energy, under Contract DE-AC02-06CH11357. NR 48 TC 5 Z9 5 U1 13 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 26 PY 2016 VL 28 IS 8 BP 2814 EP 2822 DI 10.1021/acs.chemmater.6b00734 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DK9IQ UT WOS:000375244500039 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorima, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovia, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairoa, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colomboc, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V 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Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Probing lepton flavour violation via neutrinoless tau -> 3 mu decays with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SEARCH AB This article presents the sensitivity of the ATLAS experiment to the lepton-flavour-violating decays of tau -> 3 mu. A method utilising the production of t leptons via W -> tau nu decays is used. This method is applied to the sample of 20.3 fb(-1) of pp collision data at a centre-of-mass energy of 8 TeV collected by the ATLAS experiment at the LHC in 2012. 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[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairoa, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Cairoa, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Stanecka, E.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Benhar Noccioli, E.; De Mendizabal, J. Bilbao; Calace, N.; Coccaro, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristie, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Zu Theenhausen, H. Meyer; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colomboc, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pokfulam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipeic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandie, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipeic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandie, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, E.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, E.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, E.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Kopke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, E.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandellia, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ, MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundisa, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Delgado, A. Tavares; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, CNRS, IN2P3, Univ Paris Saclay,LAL, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, P.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovia, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovia, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorima, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorima, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, P-1200 Lisbon, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, P-1200 Lisbon, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Donati, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Pires, S.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacooba, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Acharya, B. S.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, C.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Teuscher, R. J.; Trischuk, W.; Veloso, F.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramosb, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, G.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Sandstroem, R.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, E.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachgrp Phys, Fachbereich Fak Mathemat & Nat Wissensch C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, E.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Rec & Estud Avancats, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Scuola Int Super Studi Avanzati, SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Kukla, Romain/P-9760-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014 OI Kukla, Romain/0000-0002-1140-2465; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Prokofiev, Kirill/0000-0002-2177-6401; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 27 TC 0 Z9 0 U1 19 U2 46 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 26 PY 2016 VL 76 IS 5 AR 232 DI 10.1140/epjc/s10052-016-4041-9 PG 25 WC Physics, Particles & Fields SC Physics GA DK5WH UT WOS:000374991300004 ER PT J AU Homyak, PD Liu, Y Harris, JD Liu, F Carter, KR Russell, TP Coughlin, EB AF Homyak, Patrick D. Liu, Yao Harris, Jared D. Liu, Feng Carter, Kenneth R. Russell, Thomas P. Coughlin, E. Bryan TI Systematic Fluorination of P3HT: Synthesis of P(3HT-co-3H4FT)s by Direct Arylation Polymerization, Characterization, and Device Performance in OPVs SO MACROMOLECULES LA English DT Article ID ORGANIC SOLAR-CELLS; OPEN-CIRCUIT VOLTAGE; CONJUGATED POLYMERS; BACKBONE FLUORINATION; ELECTRONIC-PROPERTIES; SIDE-CHAINS; POLY(3-HEXYLTHIOPHENE); COPOLYMERS; POLYCONDENSATION; SELENOPHENE AB We present a strategy for tuning physical properties of P3HT-based copolymers by incorporating a fluorinated thiophene repeat unit. The synthesis and characterization of a series of fluorinated polythiophene P(3HT-co-3H4FT) materials are described, where the percentage of fluorinated repeat units in the polymer backbone is systematically varied from 0 to 100%. These P(3HT-co-3H4FT)s (P0, P25, P50, P75, and P100) were synthesized via direct arylation polymerization (DArP) methods. By varying the feed ratio of the two monomers, the percent of fluorinated repeat units (3H4FT) could be precisely controlled. As fluorination is increased, there is a strong effect on the electronic properties of the polymers, evidenced by a 0.4 eV drop in the E-HOMO level for P100 when compared to P0. GIWAXS and TEM were used to determine the crystallinity and morphology. TEM analysis of thin film polymer/PCBM bulk-heterojunction blends indicates that increased fluorination does not result in stronger phase separation. Organic photovoltaic devices were fabricated to evaluate changes in device performance as a result of fluorination. C1 [Homyak, Patrick D.; Liu, Yao; Harris, Jared D.; Carter, Kenneth R.; Russell, Thomas P.; Coughlin, E. Bryan] Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. [Liu, Feng; Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Coughlin, EB (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. EM Coughlin@mail.pse.umass.edu RI Liu, Feng/J-4361-2014 OI Liu, Feng/0000-0002-5572-8512 FU Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001087]; U.S. Office of Naval Research [N00014-15-1-2244]; Center for UMass/Industry Research on Polymers (CUMIRP) through Cluster E: Polymers for Renewable Energy; National Science Foundation [GRFP-1451512]; DOE, Office of Science, and Office of Basic Energy Sciences FX This work is supported as part of Polymer-Based Materials for Harvesting Solar Energy (PHaSE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0001087. Support was also provided by the U.S. Office of Naval Research under contract N00014-15-1-2244, and by the Center for UMass/Industry Research on Polymers (CUMIRP) through Cluster E: Polymers for Renewable Energy. UPS experiments were performed in the UMass Center for Electronic Materials and Devices with the support of V. Duzhko. Mass spectral data for all materials were obtained at the University of Massachusetts Mass Spectrometry Center. J.D.H. acknowledges support from the National Science Foundation Graduate Research Fellowship Program (GRFP-1451512). The authors also acknowledge A. Hexemer and E. Schaible for support in ALS beamline 7.3.3. Portions of this research were performed at the Advanced Light Source, Lawrence Berkeley National Laboratory (LBNL), which is supported by the DOE, Office of Science, and Office of Basic Energy Sciences. NR 46 TC 8 Z9 8 U1 15 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 26 PY 2016 VL 49 IS 8 BP 3028 EP 3037 DI 10.1021/acs.macromol.6b00386 PG 10 WC Polymer Science SC Polymer Science GA DK9IR UT WOS:000375244600015 ER PT J AU Sun, J Jiang, X Siegmund, A Connolly, MD Downing, KH Balsara, NP Zuckermann, RN AF Sun, Jing Jiang, Xi Siegmund, Aaron Connolly, Michael D. Downing, Kenneth H. Balsara, Nitash P. Zuckermann, Ronald N. TI Morphology and Proton Transport in Humidified Phosphonated Peptoid Block Copolymers SO MACROMOLECULES LA English DT Article ID FUEL-CELL MEMBRANES; ANGLE X-RAY; PHASE-BEHAVIOR; MICROPHASE SEPARATION; POLYMER ELECTROLYTES; CONDUCTING POLYMERS; VARYING SELECTIVITY; DIBLOCK COPOLYMERS; NAFION MEMBRANES; ACID AB Polymers that conduct protons in the hydrated state are of crucial importance in a wide variety of clean energy applications such as hydrogen fuel cells and artificial photosynthesis. Phosphonated and sulfonated polymers are known to conduct protons at low water content. In this paper, we report on the synthesis phosphonated peptoid diblock copolymers, poly-N-(2-ethyl)hexylglycine-block-poly-N-phosphonomethylglycine (pNeh-b-pNpm), with volume fractions of pNpm (phi(Npm)) values ranging from 0.13 to 0.44 and dispersity (D) <= 1.0003. The morphologies of the dry block copolypeptoids were determined by transmission electron microscopy and in both the dry and hydrated states by synchrotron small-angle X-ray scattering. Dry samples with phi(Npm) > 0.13 exhibited a lamellar morphology. Upon hydration, the lowest molecular weight sample transitioned to a hexagonally packed cylinder morphology, while the others maintained their dry morphologies. Water uptake of all of the ordered samples was 8.1 +/- 1.1 water molecules per phosphonate group. In spite of this, the proton conductivity of the ordered pNeh-b-pNpm copolymers ranged from 0.002 to 0.008 S/cm. We demonstrate that proton conductivity is maximized in high molecular weight, symmetric pNeh-b-pNpm copolymers. C1 [Sun, Jing; Connolly, Michael D.; Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Jiang, Xi; Connolly, Michael D.; Balsara, Nitash P.; Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Downing, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Sun, Jing] Qingdao Univ Sci & Technol, Sch Polymer Sci & Engn, Qingdao 266042, Peoples R China. [Siegmund, Aaron] Amgen Inc, Dept Med Chem, One Amgen Ctr Dr, Thousand Oaks, CA 91320 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Zuckermann, RN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Balsara, NP; Zuckermann, RN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.; Balsara, NP (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM nbalsara@berkeley.edu; rnzuckermann@lbl.gov FU Soft Matter Electron Microscopy Program - Office of Science, Office of Basic Energy Science, U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Science, U.S. Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [51503115]; Taishan Scholars Program; NIH [GM51487] FX Funding for this work was provided by the Soft Matter Electron Microscopy Program, supported by the Office of Science, Office of Basic Energy Science, U.S. Department of Energy, under Contract DE-AC02-05CH11231. The work was carried out at the Molecular Foundry and the Advanced Light Source at the Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Science, U.S. Department of Energy, under Contract DE-AC02-05CH11231. J.S. acknowledges grants from the National Natural Science Foundation of China (No. 51503115) and Taishan Scholars Program. Cryo-EM facilities are supported by NIH Grant GM51487. NR 56 TC 1 Z9 1 U1 15 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 26 PY 2016 VL 49 IS 8 BP 3083 EP 3090 DI 10.1021/acs.macromol.6b00353 PG 8 WC Polymer Science SC Polymer Science GA DK9IR UT WOS:000375244600020 PM 27134312 ER PT J AU Mineart, KP Lee, B Spontak, RJ AF Mineart, Kenneth P. Lee, Byeongdu Spontak, Richard J. TI A Solvent-Vapor Approach toward the Control of Block lonomer Morphologies SO MACROMOLECULES LA English DT Article ID ABC TRIBLOCK COPOLYMERS; DILUTION APPROXIMATION; SULFONATED POLYSTYRENE; PENTABLOCK COPOLYMERS; MEMBRANE APPLICATIONS; TRANSPORT-PROPERTIES; PHYSICAL-PROPERTIES; PHASE-BEHAVIOR; LINEAR ABCBA; THIN-FILMS AB Sulfonated block ionomers possess advantageous properties for a wide range of diverse applications such as desalination membranes, fuel cells, electroactive media, and photovoltaic devices. Unfortunately, their inherently high incompatibilities and glass transition temperatures effectively prevent the use of thermal annealing, routinely employed to refine the morphologies of nonionic block copolymers. An alternative approach is therefore required to promote morphological equilibration in block ionomers. The present study explores the morphological characteristics of midblock-sulfonated pentablock ionomers (SBIs) differing in their degree of sulfonation (DOS) and cast from solution followed by solvent-vapor annealing (SVA). Transmission electron microscopy confirms that films deposited from different solvent systems form nonequilibrium morphologies due to solvent-regulated self-assembly and drying. A series of SVA tests performed with solvents varying in polarity reveals that exposing cast films to tetrahydrofuran (THF) vapor for at least 2 h constitutes the most effective SVA protocol, yielding the anticipated equilibrium morphology. That is, three SBI grades subjected to THF-SVA self-assemble into well-ordered lamellae wherein the increase in DOS is accompanied by an increase in lamellar periodicity, as measured by small-angle X-ray scattering. C1 [Mineart, Kenneth P.; Spontak, Richard J.] N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA. [Spontak, Richard J.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Mineart, Kenneth P.] Natl Inst Stand & Technol, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. RP Spontak, RJ (reprint author), N Carolina State Univ, Dept Chem & Biomol Engn, Raleigh, NC 27695 USA.; Spontak, RJ (reprint author), N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27695 USA. EM Rich_Spontak@ncsu.edu OI Mineart, Kenneth/0000-0003-2374-4670 FU Nonwovens Institute at North Carolina State University; MANN+HUMMEL GmbH; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported by the Nonwovens Institute at North Carolina State University and MANN+HUMMEL GmbH. In addition, this research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. NR 63 TC 6 Z9 6 U1 15 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 26 PY 2016 VL 49 IS 8 BP 3126 EP 3137 DI 10.1021/acs.macromol.6b00134 PG 12 WC Polymer Science SC Polymer Science GA DK9IR UT WOS:000375244600025 ER PT J AU Xing, KY Chatterjee, S Saito, T Gainaru, C Sokolov, AP AF Xing, Kunyue Chatterjee, Sabornie Saito, Tomonori Gainaru, Catalin Sokolov, Alexei P. TI Impact of Hydrogen Bonding on Dynamics of Hydroxyl-Terminated Polydimethylsiloxane SO MACROMOLECULES LA English DT Article ID X-RAY-DIFFRACTION; SUPRAMOLECULAR POLYMERS; POLY(PROPYLENE GLYCOL); MOLECULAR-DYNAMICS; N-METHYLACETAMIDE; BONDED COMPLEXES; LIQUID METHANOL; GLASS FORMERS; ETHANOL; RELAXATION AB Dielectric spectroscopy, rheology, and differential scanning calorimetry were employed to study the effect of chain-end hydrogen bonding on the dynamics of hydroxyl terminated polydimethylsiloxane. We demonstrate that hydrogen bonding has a strong influence on both segmental and slower dynamics in the systems with low molecular weights. In particular, the decrease in the chain length leads to an increase of the glass transition temperature, viscosity, and fragility index, at variance with the usual behavior of nonassociating polymers. The supramolecular association of hydroxyl terminated chains leads to the emergence in dielectric and mechanical relaxation spectra of the so-called Debye process traditionally observed in monohydroxy alcohols. Our analysis suggests that the hydroxyl-terminated PDMS oligomers may associate in brush-like or chain-like structures, depending on the size of their covalent chains. The effective length of the linear-associated chains was estimated from the rheological measurements. C1 [Xing, Kunyue; Chatterjee, Sabornie; Gainaru, Catalin; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Gainaru, Catalin] Tech Univ Dortmund, Fak Phys, D-44221 Dortmund, Germany. [Saito, Tomonori; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Gainaru, C (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Gainaru, C (reprint author), Tech Univ Dortmund, Fak Phys, D-44221 Dortmund, Germany. EM catalin.gainaru@uni-dortmund.de RI Saito, Tomonori/M-1735-2016 OI Saito, Tomonori/0000-0002-4536-7530 FU NSF Polymer program [DMR-1408811] FX This work was supported by NSF Polymer program (Grant DMR-1408811). NR 68 TC 3 Z9 3 U1 18 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 26 PY 2016 VL 49 IS 8 BP 3138 EP 3147 DI 10.1021/acs.macromol.6b00262 PG 10 WC Polymer Science SC Polymer Science GA DK9IR UT WOS:000375244600026 ER PT J AU Michler, T San Marchi, C Berreth, K Naumann, J Mishra, RK Kubic, RC AF Michler, Thorsten San Marchi, Christopher Berreth, Karl Naumann, Jorg Mishra, Raj K. Kubic, Robert C. TI Microstructure, deformation mechanisms and influence of hydrogen on tensile properties of the Co based super alloy DIN 2.4711/UNS N30003 SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Hydrogen embrittlement; Microstructure; Deformation mechanism; Elgiloy; 2.4711; N30003 ID AUSTENITIC STAINLESS-STEELS; ENVIRONMENT EMBRITTLEMENT; LOW-TEMPERATURES; MARTENSITIC-TRANSFORMATION; STRENGTHENING MECHANISMS; DIFFUSION; FRACTURE; COBALT; CRACK; DISLOCATIONS AB The Co-based alloy 2.4711 investigated in this study consists of an austenitic martix with epsilon-martensite from both strain hardening and aging. Upon deformation, the microstructure shows strain-induced gamma -> epsilon transformation. Mechanical twinning could not be verified in this study using EBSD. Tensile testing in hydrogen gas and with H-precharged specimens revealed negligible embrittlement for the specimens tested in H-2 gas, whereas severe embrittlement was found for the H-precharged specimen. This was interpreted and explained by hydrogen transport during the two test configurations. It appears that the epsilon-martensite in alloy 2.4711, unlike strain-induced martensite in type 304 austenitic stainless steels, does not enhance hydrogen ingress over long distances during tensile testing in gaseous hydrogen. Limiting hydrogen transport during testing in gaseous hydrogen precludes observation of intrinsic hydrogen effects, while saturation of hydrogen by H-precharging illuminates intrinsic hydrogen sensitivity. (C) 2016 Elsevier B.V. All rights reserved. C1 [Michler, Thorsten] Adam Opel AG, Russelsheim, Germany. [San Marchi, Christopher] Sandia Natl Labs, Livermore, CA USA. [Berreth, Karl] Mat Prufanstalt Univ Stuttgart, Stuttgart, Germany. [Naumann, Jorg] BMW AG, Munich, Germany. [Mishra, Raj K.; Kubic, Robert C.] Gen Motors Res & Dev, Warren, MI USA. RP Michler, T (reprint author), Adam Opel AG, Russelsheim, Germany. EM thorsten.dr.michler@de.opel.com NR 38 TC 0 Z9 0 U1 4 U2 11 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD APR 26 PY 2016 VL 662 BP 36 EP 45 DI 10.1016/j.msea.2016.03.041 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DK8GD UT WOS:000375164300005 ER PT J AU Pelliciari, J Huang, YB Das, T Dantz, M Bisogni, V Velasco, PO Strocov, VN Xing, LY Wang, XC Jin, CQ Schmitt, T AF Pelliciari, Jonathan Huang, Yaobo Das, Tanmoy Dantz, Marcus Bisogni, Valentina Velasco, Paul Olalde Strocov, Vladimir N. Xing, Lingyi Wang, Xiancheng Jin, Changqing Schmitt, Thorsten TI Intralayer doping effects on the high-energy magnetic correlations in NaFeAs SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-SCATTERING; HIGH-TEMPERATURE SUPERCONDUCTIVITY; SPIN EXCITATIONS; IRON PNICTIDES; PHONON RELAXATION; CHALCOGENIDES; METALS AB We have used resonant inelastic x-ray scattering (RIXS) and dynamical susceptibility calculations to study the magnetic excitations in NaFe1-x Co-x As (x = 0, 0.03, and 0.08). Despite a relatively low ordered magnetic moment, collective magnetic modes are observed in parent compounds (x = 0) and persist in optimally (x = 0.03) and overdoped (x = 0.08) samples. Their magnetic bandwidths are unaffected by doping within the range investigated. High-energy magnetic excitations in iron pnictides are robust against doping and present irrespectively of the ordered magnetic moment. Nevertheless, Co doping slightly reduces the overall magnetic spectral weight, differently from previous studies on hole-doped BaFe2As2, where it was observed constant. Finally, we demonstrate that the doping evolution of magnetic modes is different for the dopants being inside or outside the Fe-As layer. C1 [Pelliciari, Jonathan; Huang, Yaobo; Dantz, Marcus; Bisogni, Valentina; Velasco, Paul Olalde; Strocov, Vladimir N.; Schmitt, Thorsten] Paul Scherrer Inst, Dept Synchrotron Radiat & Nanotechnol, CH-5232 Villigen, Switzerland. [Huang, Yaobo; Xing, Lingyi; Wang, Xiancheng; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, POB 603, Beijing 100190, Peoples R China. [Das, Tanmoy] Indian Inst Sci, Dept Phys, Bangalore 560012, Karnataka, India. [Bisogni, Valentina] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Jin, Changqing] Collaborat Innovat Ctr Quantum Matters, Beijing, Peoples R China. RP Pelliciari, J; Schmitt, T (reprint author), Paul Scherrer Inst, Dept Synchrotron Radiat & Nanotechnol, CH-5232 Villigen, Switzerland. EM jonathan.pelliciari@psi.ch; thorsten.schmitt@psi.ch RI Schmitt, Thorsten/A-7025-2010 FU Dysenos AG by Kabelwerke Brugg AG Holding; Fachhochschule Nordwestschweiz; Paul Scherrer Institut; Swiss National Science Foundation through Sinergia network Mott Physics Beyond Heisenberg (MPBH) model; D-A-CH program (SNSF Research) [200021L 141325]; European Community's Seventh Framework Programme [290605]; PSI-FELLOW; NSF; MOST FX J.P. and T.S. acknowledge financial support through the Dysenos AG by Kabelwerke Brugg AG Holding, Fachhochschule Nordwestschweiz, and the Paul Scherrer Institut. Experiments have been performed at the ADRESS beamline of the Swiss Light Source at Paul Scherrer Institut. Part of this research has been funded by the Swiss National Science Foundation through the Sinergia network Mott Physics Beyond the Heisenberg (MPBH) model and the D-A-CH program (SNSF Research Grant No. 200021L 141325). The research leading to these results has received funding from the European Community's Seventh Framework Programme (FP7/2007-2013) under Grant Agreement No. 290605 (COFUND: PSI-FELLOW). The work at IOP-CAS is supported by NSF and MOST through research projects. NR 45 TC 2 Z9 2 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 26 PY 2016 VL 93 IS 13 AR 134515 DI 10.1103/PhysRevB.93.134515 PG 9 WC Physics, Condensed Matter SC Physics GA DK5DO UT WOS:000374940100001 ER PT J AU Iatrakis, I Kharzeev, DE AF Iatrakis, Ioannis Kharzeev, Dmitri E. TI Holographic entropy and real-time dynamics of quarkonium dissociation in non-Abelian plasma SO PHYSICAL REVIEW D LA English DT Article ID DE-SITTER SUPERGRAVITY; N GAUGE-THEORY; FINITE-TEMPERATURE; STRINGS; QCD AB The peak of the heavy quark pair entropy at the deconfinement transition, observed in lattice QCD, suggests that the transition is effectively driven by the increase of the entropy of bound states. The growth of the entropy with the interquark distance leads to the emergent entropic force that induces dissociation of quarkonium states. Since the quark-gluon plasma around the transition point is a strongly coupled system, we use the gauge-gravity duality to study the entropy of heavy quarkonium and the real-time dynamics of its dissociation. In particular, we employ the improved holographic QCD model as a dual description of large N-c Yang-Mills theory. Studying the dynamics of the fundamental string between the quarks placed on the boundary, we find that the entropy peaks at the transition point. We also study the real-time dynamics of the system by considering the holographic string falling in the black hole horizon where it equilibrates. In the vicinity of the deconfinement transition, the dissociation time is found to be less than a fermi, suggesting that the entropic destruction is the dominant dissociation mechanism in this temperature region. C1 [Iatrakis, Ioannis; Kharzeev, Dmitri E.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kharzeev, Dmitri E.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Kharzeev, Dmitri E.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Iatrakis, Ioannis] Univ Utrecht, Inst Theoret Phys, Leuvenlaan 4, NL-3584 CE Utrecht, Netherlands. RP Iatrakis, I; Kharzeev, DE (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA.; Kharzeev, DE (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Kharzeev, DE (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; Iatrakis, I (reprint author), Univ Utrecht, Inst Theoret Phys, Leuvenlaan 4, NL-3584 CE Utrecht, Netherlands. EM ioannis.iatrakis@stonybrook.edu; dmitri.kharzeev@stonybrook.edu FU U.S. Department of Energy [DE-FG-88ER40388, DE-SC0012704]; Dutch Ministry of Education, Culture and Science FX We thank Koji Hashimoto for useful discussions. This work was supported in part by the U.S. Department of Energy under Contracts No. DE-FG-88ER40388 and No. DE-SC0012704. This work is also part of the D-ITP consortium, a program of the Netherlands Organisation for Scientific Research that is funded by the Dutch Ministry of Education, Culture and Science. NR 30 TC 3 Z9 3 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 26 PY 2016 VL 93 IS 8 AR 086009 DI 10.1103/PhysRevD.93.086009 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK5KU UT WOS:000374959600003 ER PT J AU Rousseaux, C Baton, SD Benisti, D Gremillet, L Loupias, B Philippe, F Tassin, V Amiranoff, F Kline, JL Montgomery, DS Afeyan, BB AF Rousseaux, C. Baton, S. D. Benisti, D. Gremillet, L. Loupias, B. Philippe, F. Tassin, V. Amiranoff, F. Kline, J. L. Montgomery, D. S. Afeyan, B. B. TI Experimental investigation of stimulated Raman and Brillouin scattering instabilities driven by two successive collinear picosecond laser pulses SO PHYSICAL REVIEW E LA English DT Article AB Backward stimulated Raman and Brillouin scattering (SRS and SBS) are experimentally investigated by using two successive 1-mu m, 1.5-ps FWHM laser pulses. The collinear pulses, separated by 3 or 6 ps and of moderate laser intensities (similar to 2 x 10(16) Wcm(-2)), are fired into a preionized He plasma of density similar to 2.5 - 6 x 10(19) cm(-3). The electron plasma waves and ion acoustic waves, respectively driven by SRS and SBS, are analyzed through space-and time-resolved Thomson scattering. Depending on the laser and plasma parameters, we observe the effect of the first pulse on the time-resolved SRS and SBS signals of the second pulse. The measurements are found to qualitatively agree with the results of a large-scale particle-in-cell simulation. C1 [Rousseaux, C.; Benisti, D.; Gremillet, L.; Loupias, B.; Philippe, F.; Tassin, V.] CEA, DAM, DIF, F-91297 Arpajon, France. [Baton, S. D.; Amiranoff, F.] Univ Paris 06, Sorbonne Univ, Univ Paris Saclay, LULI CNRS,Ecole Polytech,CEA, F-91128 Palaiseau, France. [Kline, J. L.; Montgomery, D. S.] Los Alamos Natl Lab, Div Phys, P-24, Los Alamos, NM 87545 USA. [Afeyan, B. B.] Polymath Res Inc, 827 Bonde Court, Pleasanton, CA 94566 USA. RP Rousseaux, C (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. NR 18 TC 2 Z9 2 U1 7 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 26 PY 2016 VL 93 IS 4 AR 043209 DI 10.1103/PhysRevE.93.043209 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DK5LY UT WOS:000374962600006 PM 27176420 ER PT J AU Shioda, K Cosmas, L Audi, A Gregoricus, N Vinje, J Parashar, UD Montgomery, JM Feikin, DR Breiman, RF Hall, AJ AF Shioda, Kayoko Cosmas, Leonard Audi, Allan Gregoricus, Nicole Vinje, Jan Parashar, Umesh D. Montgomery, Joel M. Feikin, Daniel R. Breiman, Robert F. Hall, Aron J. TI Population-Based Incidence Rates of Diarrheal Disease Associated with Norovirus, Sapovirus, and Astrovirus in Kenya SO PLOS ONE LA English DT Article ID INFECTIOUS INTESTINAL DISEASE; HOSPITAL-BASED SURVEILLANCE; REVERSE TRANSCRIPTION-PCR; HUMAN ROTAVIRUS VACCINE; UNITED-STATES; YOUNG-CHILDREN; GASTROENTERITIS; BURDEN; COMMUNITY; ASSAY AB Background Diarrheal diseases remain a major cause of mortality in Africa and worldwide. While the burden of rotavirus is well described, population-based rates of disease caused by norovirus, sapovirus, and astrovirus are lacking, particularly in developing countries. Methods Data on diarrhea cases were collected through a population-based surveillance platform including healthcare encounters and household visits in Kenya. We analyzed data from June 2007 to October 2008 in Lwak, a rural site in western Kenya, and from October 2006 to February 2009 in Kibera, an urban slum. Stool specimens from diarrhea cases of all ages who visited study clinics were tested for norovirus, sapovirus, and astrovirus by RT-PCR. Results Of 334 stool specimens from Lwak and 524 from Kibera, 85 (25%) and 159 (30%) were positive for norovirus, 13 (4%) and 31 (6%) for sapovirus, and 28 (8%) and 18 (3%) for astrovirus, respectively. Among norovirus-positive specimens, genogroup II predominated in both sites, detected in 74 (87%) in Lwak and 140 (88%) in Kibera. The adjusted community incidence per 100,000 person-years was the highest for norovirus (Lwak: 9,635; Kibera: 4,116), followed by astrovirus (Lwak: 3,051; Kibera: 440) and sapovirus (Lwak: 1,445; Kibera: 879). For all viruses, the adjusted incidence was higher among children aged <5 years (norovirus: 22,225 in Lwak and 17,511 in Kibera; sapovirus: 5,556 in Lwak and 4,378 in Kibera; astrovirus: 11,113 in Lwak and 2,814 in Kibera) compared to cases aged >= 5 years. Conclusion Although limited by a lack of controls, this is the first study to estimate the outpatient and community incidence rates of norovirus, sapovirus, and astrovirus across the age spectrum in Kenya, suggesting a substantial disease burden imposed by these viruses. By applying adjusted rates, we estimate approximately 2.8-3.3 million, 0.45-0.54 million, and 0.77-0.95 million people become ill with norovirus, sapovirus, and astrovirus, respectively, every year in Kenya. C1 [Shioda, Kayoko; Gregoricus, Nicole; Vinje, Jan; Parashar, Umesh D.; Feikin, Daniel R.; Hall, Aron J.] Ctr Dis Control & Prevent, Div Viral Dis, Natl Ctr Immunizat & Resp Dis, Atlanta, GA USA. [Shioda, Kayoko] Oak Ridge Inst Sci & Technol, Oak Ridge, TN USA. [Cosmas, Leonard; Montgomery, Joel M.; Feikin, Daniel R.; Breiman, Robert F.] Ctr Dis Control & Prevent, Div Global Hlth Protect, Ctr Global Hlth, Nairobi, Kenya. [Audi, Allan] Kenya Govt Med Res Ctr, Ctr Global Hlth Res, Nairobi, Kenya. [Breiman, Robert F.] Emory Univ, Emory Global Hlth Inst, Atlanta, GA 30322 USA. RP Shioda, K (reprint author), Ctr Dis Control & Prevent, Div Viral Dis, Natl Ctr Immunizat & Resp Dis, Atlanta, GA USA.; Shioda, K (reprint author), Oak Ridge Inst Sci & Technol, Oak Ridge, TN USA. EM yji4@cdc.gov NR 34 TC 1 Z9 1 U1 1 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 26 PY 2016 VL 11 IS 4 AR e0145943 DI 10.1371/journal.pone.0145943 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK5QB UT WOS:000374973600004 PM 27116458 ER PT J AU Timm, CM Pelletier, DA Jawdy, SS Gunter, LE Henning, JA Engle, N Aufrecht, J Gee, E Nookaew, I Yang, ZM Lu, TY Tschaplinski, TJ Doktycz, MJ Tuskan, GA Weston, DJ AF Timm, Collin M. Pelletier, Dale A. Jawdy, Sara S. Gunter, Lee E. Henning, Jeremiah A. Engle, Nancy Aufrecht, Jayde Gee, Emily Nookaew, Intawat Yang, Zamin Lu, Tse-Yuan Tschaplinski, Timothy J. Doktycz, Mitchel J. Tuskan, Gerald A. Weston, David J. TI Two Poplar-Associated Bacterial Isolates Induce Additive Favorable Responses in a Constructed Plant-Microbiome System SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE Burkholderia; Pseudomonas; Populus deltoides; microbiome; plant -microbe interactions ID POPULUS-DELTOIDES; GENOME SEQUENCES; ROOT MICROBIOME; COLANIC ACID; ARABIDOPSIS; RHIZOSPHERE; ENDOSPHERE; METABOLISM; NETWORKS; REVEALS AB The biological function of the plant-microbiome system is the result of contributions from the host plant and microbiome members. The Populus root microbiome is a diverse community that has high abundance of beta- and gamma-Proteobacteria, both classes which include multiple plant-growth promoting representatives. To understand the contribution of individual microbiome members in a community, we studied the function of a simplified community consisting of Pseudomonas and Burkholderia bacterial strains isolated from Populus hosts and inoculated on axenic Populus cutting in controlled laboratory conditions. Both strains increased lateral root formation and root hair production in Arabidopsis plate assays and are predicted to encode for different functions related to growth and plant growth promotion in Populus hosts. Inoculation individually, with either bacterial isolate, increased root growth relative to uninoculated controls, and while root area was increased in mixed inoculation, the interaction term was insignificant indicating additive effects of root phenotype. Complementary data including photosynthetic efficiency, whole-transcriptome gene expression and GC-MS metabolite expression data in individual and mixed inoculated treatments indicate that the effects of these bacterial strains are unique and additive. These results suggest that the function of a microbiome community may be predicted from the additive functions of the individual members. C1 [Timm, Collin M.; Pelletier, Dale A.; Jawdy, Sara S.; Gunter, Lee E.; Engle, Nancy; Aufrecht, Jayde; Gee, Emily; Nookaew, Intawat; Yang, Zamin; Lu, Tse-Yuan; Tschaplinski, Timothy J.; Doktycz, Mitchel J.; Tuskan, Gerald A.; Weston, David J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Henning, Jeremiah A.] Univ Tennessee, Dept Ecol & Evolutionary Biol, Knoxville, TN USA. [Aufrecht, Jayde] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN USA. RP Timm, CM (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. EM timmcm@ornl.gov RI Doktycz, Mitchel/A-7499-2011; Gunter, Lee/L-3480-2016; Tuskan, Gerald/A-6225-2011; OI Doktycz, Mitchel/0000-0003-4856-8343; Gunter, Lee/0000-0003-1211-7532; Tuskan, Gerald/0000-0003-0106-1289; Tschaplinski, Timothy/0000-0002-9540-6622; Engle, Nancy/0000-0003-0290-7987 FU U.S. DOE Office of Biological and Environmental Research, Genomic Science Program under Plant Feedstock Genomics [DE-SC001043]; Plant-Microbe Interfaces Scientific Focus Area at Oak Ridge National Laboratory FX This research was funded by the U.S. DOE Office of Biological and Environmental Research, Genomic Science Program under Plant Feedstock Genomics projects: DE-SC001043 (50%) and the Plant-Microbe Interfaces Scientific Focus Area (50%) at Oak Ridge National Laboratory. NR 60 TC 3 Z9 3 U1 12 U2 26 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD APR 26 PY 2016 VL 7 AR 497 DI 10.3389/fpls.2016.00497 PG 10 WC Plant Sciences SC Plant Sciences GA DK2GB UT WOS:000374731500001 PM 27200001 ER PT J AU Johnston, ER Rodriguez-R, LM Luo, CW Yuan, MM Wu, LY He, ZL Schuur, EAG Luo, YQ Tiedje, JM Zhou, JZ Konstantinidis, KT AF Johnston, Eric R. Rodriguez-R, Luis M. Luo, Chengwei Yuan, Mengting M. Wu, Liyou He, Zhili Schuur, Edward A. G. Luo, Yiqi Tiedje, James M. Zhou, Jizhong Konstantinidis, Konstantinos T. TI Metagenomics Reveals Pervasive Bacterial Populations and Reduced Community Diversity across the Alaska Tundra Ecosystem SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE tundra; soil microbiology; metagenomics; ecosystem ecology; environmental science; permafrost; climate change; microbial diversity ID RNA GENE DATABASE; SP-NOV; MICROBIAL COMMUNITIES; PERMAFROST THAW; HIGH-THROUGHPUT; ACTIVE LAYER; SOIL; SEQUENCES; CLIMATE; THERMODESULFOVIBRIO AB How soil microbial communities contrast with respect to taxonomic and functional composition within and between ecosystems remains an unresolved question that is central to predicting how global anthropogenic change will affect soil functioning and services. In particular, it remains unclear how small-scale observations of soil communities based on the typical volume sampled (1-2 g) are generalizable to ecosystem-scale responses and processes. This is especially relevant for remote, northern latitude soils, which are challenging to sample and are also thought to be more vulnerable to climate change compared to temperate soils. Here, we employed well-replicated shotgun metagenome and 16S rRNA gene amplicon sequencing to characterize community composition and metabolic potential in Alaskan tundra soils, combining our own datasets with those publically available from distant tundra and temperate grassland and agriculture habitats. We found that the abundance of many taxa and metabolic functions differed substantially between tundra soil metagenomes relative to those from temperate soils, and that a high degree of OTU-sharing exists between tundra locations. Tundra soils were an order of magnitude less complex than their temperate counterparts, allowing for near-complete coverage of microbial community richness (similar to 92% breadth) by sequencing, and the recovery of 27 high-quality, almost complete (>80% completeness) population bins. These population bins, collectively, made up to similar to 10% of the metagenomic datasets, and represented diverse taxonomic groups and metabolic lifestyles tuned toward sulfur cycling, hydrogen metabolism, methanotrophy, and organic matter oxidation. Several population bins, including members of Acidobacteria, Actinobacteria, and Proteobacteria, were also present in geographically distant (similar to 100-530 km apart) tundra habitats (full genome representation and up to 99.6% genome-derived average nucleotide identity). Collectively, our results revealed that Alaska tundra microbial communities are less diverse and more homogenous across spatial scales than previously anticipated, and provided DNA sequences of abundant populations and genes that would be relevant for future studies of the effects of environmental change on tundra ecosystems. C1 [Johnston, Eric R.; Konstantinidis, Konstantinos T.] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. [Rodriguez-R, Luis M.; Luo, Chengwei; Konstantinidis, Konstantinos T.] Georgia Inst Technol, Ctr Bioinformat & Computat Genom, Atlanta, GA 30332 USA. [Rodriguez-R, Luis M.; Konstantinidis, Konstantinos T.] Georgia Inst Technol, Sch Biol, Atlanta, GA 30332 USA. [Yuan, Mengting M.; Wu, Liyou; He, Zhili; Luo, Yiqi; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Genom, Norman, OK 73019 USA. [Schuur, Edward A. G.] No Arizona Univ, Dept Biol Sci, Box 5640, Flagstaff, AZ 86011 USA. [Tiedje, James M.] Michigan State Univ, Ctr Microbial Ecol, E Lansing, MI 48824 USA. [Zhou, Jizhong] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China. RP Konstantinidis, KT (reprint author), Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA.; Konstantinidis, KT (reprint author), Georgia Inst Technol, Ctr Bioinformat & Computat Genom, Atlanta, GA 30332 USA.; Konstantinidis, KT (reprint author), Georgia Inst Technol, Sch Biol, Atlanta, GA 30332 USA.; Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Genom, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA.; Zhou, JZ (reprint author), Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing, Peoples R China. EM jzhou@ou.edu; kostas@ce.gatech.edu OI Rodriguez-R, Luis M/0000-0001-7603-3093 FU U.S. Department of Energy [DE-SC0004601] FX This research was supported by the U.S. Department of Energy (award DE-SC0004601). NR 73 TC 2 Z9 2 U1 13 U2 15 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 25 PY 2016 VL 7 AR 579 DI 10.3389/fmicb.2016.00579 PG 16 WC Microbiology SC Microbiology GA ED2IV UT WOS:000388668200001 PM 27199914 ER PT J AU Terzic, B Reeves, C Krafft, GA AF Terzic, Balsa Reeves, Cody Krafft, Geoffrey A. TI Combining harmonic generation and laser chirping to achieve high spectral density in Compton sources SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID FREE-ELECTRON LASER AB Recently various laser-chirping schemes have been investigated with the goal of reducing or eliminating ponderomotive line broadening in Compton or Thomson scattering occurring at high laser intensities. As a next level of detail in the spectrum calculations, we have calculated the line smoothing and broadening expected due to incident beam energy spread within a one-dimensional plane wave model for the incident laser pulse, both for compensated (chirped) and unchirped cases. The scattered compensated distributions are treatable analytically within three models for the envelope of the incident laser pulses: Gaussian, Lorentzian, or hyperbolic secant. We use the new results to demonstrate that the laser chirping in Compton sources at high laser intensities: (i) enables the use of higher order harmonics, thereby reducing the required electron beam energies; and (ii) increases the photon yield in a small frequency band beyond that possible with the fundamental without chirping. This combination of chirping and higher harmonics can lead to substantial savings in the design, construction and operational costs of the new Compton sources. This is of particular importance to the widely popular laser-plasma accelerator based Compton sources, as the improvement in their beam quality enters the regime where chirping is most effective. C1 [Terzic, Balsa; Krafft, Geoffrey A.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Terzic, Balsa; Krafft, Geoffrey A.] Old Dominion Univ, Ctr Accelerator Sci, Norfolk, VA 23529 USA. [Reeves, Cody] Northwestern Univ, Dept Engn Sci & Appl Math, Evanston, IL 60208 USA. [Reeves, Cody; Krafft, Geoffrey A.] Jefferson Lab, Newport News, VA 23606 USA. RP Terzic, B (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Terzic, B (reprint author), Old Dominion Univ, Ctr Accelerator Sci, Norfolk, VA 23529 USA. EM bterzic@odu.edu FU U.S. Department of Energy (DOE) [DE-AC05-06OR23177]; U.S. Department of Energy, Science Undergraduate Laboratory Internship (SULI) program FX This paper is authored by Jefferson Science Associates, LLC under U.S. Department of Energy (DOE) Contract No. DE-AC05-06OR23177. The U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce this manuscript for U.S. Government purposes. C. R. acknowledges the support from the U.S. Department of Energy, Science Undergraduate Laboratory Internship (SULI) program. NR 21 TC 1 Z9 1 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD APR 25 PY 2016 VL 19 IS 4 AR 044403 DI 10.1103/PhysRevAccelBeams.19.044403 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6XL UT WOS:000379349500003 ER PT J AU Desautels, RD Shueh, C Lin, KW Freeland, JW van Lierop, J AF Desautels, R. D. Shueh, C. Lin, K. -W. Freeland, J. W. van Lierop, J. TI Dynamical freezing, magnetic ordering, and the magnetocaloric effect in nanostructured Fe/Cu thin films SO APPLIED PHYSICS LETTERS LA English DT Article AB Dynamical freezing of Fe nanocrystallites in a Cu matrix with magnetic ordering of an FeCu interfacial phase provides a unique window into the magnetocaloric effect. The FeCu alloy altered the Fe nanocrystallite surface atoms, and with a magnetic ordering temperature comparable to the dynamical freezing temperature of the nanocrystallites enabled Fe surface atoms to contribute to the overall magnetization. Tuning the amount of interfacial alloy resulted in the control of the magnetic ordering temperature and the magnetocaloric properties. Published by AIP Publishing. C1 [Desautels, R. D.; van Lierop, J.] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada. [Shueh, C.; Lin, K. -W.] Natl Chung Hsing Univ, Dept Mat Sci & Engn, Taichung 402, Taiwan. [Freeland, J. W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Desautels, RD (reprint author), Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada. OI Desautels, Ryan/0000-0001-5359-3565 FU NSERC (Canada); CFI (Canada); NSCT (Taiwan); U.S. DOE [DE-AC02-06CH11357] FX This work was supported by grants from NSERC and CFI (Canada) and NSCT (Taiwan). Use of the Advanced Photon Source at Argonne National Laboratories was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 20 TC 1 Z9 1 U1 5 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 25 PY 2016 VL 108 IS 17 AR 172410 DI 10.1063/1.4948347 PG 5 WC Physics, Applied SC Physics GA DL7UW UT WOS:000375846600031 ER PT J AU Li, LL Yang, YD Liu, ZC Jesse, S Kalinin, SV Vasudevan, RK AF Li, Linglong Yang, Yaodong Liu, Zhengchun Jesse, Stephen Kalinin, Sergei V. Vasudevan, Rama K. TI Correlation between piezoresponse nonlinearity and hysteresis in ferroelectric crystals at the nanoscale SO APPLIED PHYSICS LETTERS LA English DT Article ID THIN-FILMS; POLYCRYSTALLINE FERROELECTRICS; CERAMICS; POLARIZATION; DYNAMICS; BEHAVIOR; ORIGINS AB The nonlinear response of a ferroic to external fields has been studied for decades, garnering interest for both understanding fundamental physics, as well as technological applications such as memory devices. Yet, the behavior of ferroelectrics at mesoscopic regimes remains poorly understood, and the scale limits of theories developed for macroscopic regimes are not well tested experimentally. Here, we test the link between piezo-nonlinearity and local piezoelectric strain hysteresis, via AC-field dependent measurements in conjunction with hysteresis measurements with varying voltage windows on (K, Na) NbO3 crystals with band-excitation piezoelectric force microscopy. The correlation coefficient between nonlinearity amplitude and the amplitude during hysteresis loop acquisition shows a clear decrease with increasing AC bias. Further, correlation of polynomial fitting terms from the nonlinear measurements with the hysteresis loop area reveals that the largest correlations are reserved for the quadratic terms, which is expected for irreversible domain wall motion contributions that impact both piezoelectric behavior as well as minor loop formation. This study suggests applicability at local length scales of fundamental principles of Rayleigh behavior, with associated implications for future nanoscale ferroic devices. Published by AIP Publishing. C1 [Li, Linglong; Jesse, Stephen; Kalinin, Sergei V.; Vasudevan, Rama K.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Li, Linglong; Jesse, Stephen; Kalinin, Sergei V.; Vasudevan, Rama K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Li, Linglong; Yang, Yaodong] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Multidisciplinary Mat Res Ctr, Xian 710049, Shaanxi, Peoples R China. [Liu, Zhengchun] Univ Autonoma Barcelona, Comp Architecture & Operating Syst, E-08193 Barcelona, Spain. RP Kalinin, SV; Vasudevan, RK (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA.; Kalinin, SV; Vasudevan, RK (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM sergei2@ornl.gov; rvv@ornl.gov RI li, linglong/F-5756-2013; Yang, Yaodong/B-4000-2009; OI Yang, Yaodong/0000-0002-1707-0633; Vasudevan, Rama/0000-0003-4692-8579 FU Division of Materials Sciences and Engineering, BES, DOE; Chinese Scholarship Council; Ministry of Science and Technology of China through a 973-Project [2012CB619401]; MOE [IRT13034]; Center for Nanophase Materials Sciences FX This research was sponsored by the Division of Materials Sciences and Engineering, BES, DOE (R.K.V. and S.V.K.). Research was conducted at the Center for Nanophase Materials Sciences, which also provided support (S.J.) and is a DOE Office of Science User Facility. L.L. acknowledges financial support from Chinese Scholarship Council. Supports from the Ministry of Science and Technology of China through a 973-Project (Grant No. 2012CB619401) and MOE innovation team (Grant No. IRT13034) are also acknowledged. NR 22 TC 0 Z9 0 U1 6 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 25 PY 2016 VL 108 IS 17 AR 172905 DI 10.1063/1.4947533 PG 5 WC Physics, Applied SC Physics GA DL7UW UT WOS:000375846600042 ER PT J AU Maynard, B Long, Q Schiff, EA Yang, MJ Zhu, K Kottokkaran, R Abbas, H Dalal, VL AF Maynard, Brian Long, Qi Schiff, Eric A. Yang, Mengjin Zhu, Kai Kottokkaran, Ranjith Abbas, Hisham Dalal, Vikram L. TI Electron and hole drift mobility measurements on methylammonium lead iodide perovskite solar cells SO APPLIED PHYSICS LETTERS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITE; AMORPHOUS-SILICON; THIN-FILMS; TRANSPORT; PERFORMANCE; EFFICIENCY; DIFFUSION; CRYSTALS AB We report nanosecond domain time-of-flight measurements of electron and hole photocarriers in methylammonium lead iodide perovskite solar cells. The mobilities ranged from 0.06 to 1.4 cm(2)/Vs at room temperature, but there is little systematic difference between the two carriers. We also find that the drift mobilities are dispersive (time-dependent). The dispersion parameters are in the range of 0.4-0.7, and they imply that terahertz domain mobilities will be much larger than nanosecond domain mobilities. The temperature-dependences of the dispersion parameters are consistent with confinement of electron and hole transport to fractal-like spatial networks within nanoseconds of their photogeneration. Published by AIP Publishing. C1 [Maynard, Brian; Long, Qi; Schiff, Eric A.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Yang, Mengjin; Zhu, Kai] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Kottokkaran, Ranjith; Abbas, Hisham; Dalal, Vikram L.] Iowa State Univ, Ames, IA 50011 USA. RP Maynard, B (reprint author), Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. RI Kottokkaran, Ranjith/B-8415-2017; OI Kottokkaran, Ranjith/0000-0001-5542-2719; Schiff, Eric/0000-0002-4104-7038; Yang, Mengjin/0000-0003-2019-4298 FU National Science Foundation [CBET-1336147, CBET-1336134] FX This research was partly supported by the National Science Foundation (CBET-1336147 and CBET-1336134). NR 33 TC 6 Z9 6 U1 15 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 25 PY 2016 VL 108 IS 17 AR 173505 DI 10.1063/1.4948344 PG 4 WC Physics, Applied SC Physics GA DL7UW UT WOS:000375846600051 ER PT J AU Tran, CD Chen, JH Keum, JK Naskar, AK AF Tran, Chau D. Chen, Jihua Keum, Jong K. Naskar, Amit K. TI A New Class of Renewable Thermoplastics with Extraordinary Performance from Nanostructured Lignin-Elastomers SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID RUBBER COMPOSITES; VALORIZATION; POLYMERS; CARBON; FILLER; IMPACT AB A new class of thermoplastic elastomers has been created by introducing nanoscale-dispersed lignin (a biomass-derived phenolic oligomer) into nitrile rubber. Temperature-induced controlled miscibility between the lignin and the rubber during high shear melt-phase synthesis allows tuning the material's morphology and performance. The sustainable product has unprecedented yield stress (15-45 MPa), strain hardens at large deformation, and has outstanding recyclability. The multiphase polymers developed from an equal-mass mixture of a melt-stable lignin fraction and nitrile rubber with optimal acrylonitrile content, using the method described here, show 5-100 nm lignin lamellae with a high-modulus rubbery interphase. Molded or printed elastomeric products prepared from the lignin-nitrile material offer an additional revenue stream to pulping mills and biorefineries. C1 [Tran, Chau D.; Naskar, Amit K.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Carbon & Composites Grp, Oak Ridge, TN 37831 USA. [Chen, Jihua; Keum, Jong K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Keum, Jong K.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Naskar, AK (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Carbon & Composites Grp, Oak Ridge, TN 37831 USA. EM naskarak@ornl.gov RI Chen, Jihua/F-1417-2011; Keum, Jong/N-4412-2015 OI Chen, Jihua/0000-0001-6879-5936; Keum, Jong/0000-0002-5529-1373 FU Technology Innovation Program of Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX Research was sponsored by the Technology Innovation Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. TEM (J.C. and C.D.T.) and SAXS (J.K.K.) experiments were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Mr. Tony Bova assisted with Soxhlet extraction. C.D.T. conducted the experiment and collected and analyzed the data with input from A.K.N. J.C. and C.D.T. ran the TEM experiments. J.K.K. collected and analyzed SAXS data. A.K.N conceived the concept, directed the research, analyzed the data, and wrote the paper with input from all authors. This paper was authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this paper, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 35 TC 6 Z9 6 U1 22 U2 38 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD APR 25 PY 2016 VL 26 IS 16 BP 2677 EP 2685 DI 10.1002/adfm.201504990 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DK7SF UT WOS:000375125300009 ER PT J AU Peng, Q Pavlik, JW Silvernail, NJ Alp, EE Hu, MY Zhao, JY Sage, JT Scheidt, WR AF Peng, Qian Pavlik, Jeffrey W. Silvernail, Nathan J. Alp, E. Ercan Hu, Michael Y. Zhao, Jiyong Sage, J. Timothy Scheidt, W. Robert TI 3D Motions of Iron in Six-Coordinate {FeNO}(7) Hemes by Nuclear Resonance Vibration Spectroscopy SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE iron; nitric oxide; nuclear resonance vibrational spectroscopy (NRVS); porphyrinoids; vibrational spectra ID NITRIC-OXIDE SYNTHASE; SYNCHROTRON-RADIATION; BIOLOGICAL-SYSTEMS; LIGAND VIBRATIONS; GUANYLYL CYCLASE; SINGLE-CRYSTAL; NO ACTIVATION; COMPLEXES; DYNAMICS; PORPHYRINS AB The vibrational spectrum of a six-coordinate nitrosyl iron porphyrinate, monoclinic [Fe(TpFPP)(1-MeIm)(NO)] (TpFPP = tetra-para-fluorophenylporphyrin; 1-MeIm=1-methylimidazole), has been studied by oriented single-crystal nuclear resonance vibrational spectroscopy (NRVS). The crystal was oriented to give spectra perpendicular to the porphyrin plane and two in-plane spectra perpendicular or parallel to the projection of the FeNO plane. These enable assignment of the FeNO bending and stretching modes. The measurements reveal that the two in-plane spectra have substantial differences that result from the strongly bonded axial NO ligand. The direction of the in-plane iron motion is found to be largely parallel and perpendicular to the projection of the bent FeNO on the porphyrin plane. The out-of-plane Fe-N-O stretching and bending modes are strongly mixed with each other, as well as with porphyrin ligand modes. The stretch is mixed with v(50) as was also observed for dioxygen complexes. The frequency of the assigned stretching mode of eight Fe-X-O (X= N, C, and O) complexes is correlated with the Fe XO bond lengths. The nature of highest frequency band at 560 cm(-1) has also been examined in two additional new derivatives. Previously assigned as the Fe NO stretch (by resonance Raman), it is better described as the bend, as the motion of the central nitrogen atom of the FeNO group is very large. There is significant mixing of this mode. The results emphasize the importance of mode mixing; the extent of mixing must be related to the peripheral phenyl substituents. C1 [Peng, Qian; Pavlik, Jeffrey W.; Silvernail, Nathan J.; Scheidt, W. Robert] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Alp, E. Ercan; Hu, Michael Y.; Zhao, Jiyong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sage, J. Timothy] Northeastern Univ, Dept Phys, 120 Forsyth St, Boston, MA 02115 USA. [Sage, J. Timothy] Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, 120 Forsyth St, Boston, MA 02115 USA. RP Scheidt, WR (reprint author), Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA.; Sage, JT (reprint author), Northeastern Univ, Dept Phys, 120 Forsyth St, Boston, MA 02115 USA.; Sage, JT (reprint author), Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, 120 Forsyth St, Boston, MA 02115 USA. EM jtsage@neu.edu; scheidt.1@nd.edu RI Peng, Qian/N-7093-2013; OI Peng, Qian/0000-0002-1218-5976; Scheidt, W. Robert/0000-0002-6643-2995 FU National Institutes of Health [GM-38401]; National Science Foundation [CHE-1026369]; U.S. DOE [DE-AC02-06CH11357] FX We thank the National Institutes of Health for support of this research under Grant GM-38401 to WRS and the National Science Foundation under CHE-1026369 to JTS. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. We thank Dr. Allen G. Oliver for assistance with crystal alignments. We are grateful for the loan of an Oxford cryocooler from BioCARS. NR 82 TC 1 Z9 1 U1 4 U2 13 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD APR 25 PY 2016 VL 22 IS 18 BP 6323 EP 6332 DI 10.1002/chem.201505155 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DK1SC UT WOS:000374693300026 PM 26999733 ER PT J AU Wood, HM Parkinson, DY Griswold, CE Gillespie, RG Elias, DO AF Wood, Hannah M. Parkinson, Dilworth Y. Griswold, Charles E. Gillespie, Rosemary G. Elias, Damian O. TI Repeated Evolution of Power-Amplified Predatory Strikes in Trap-Jaw Spiders SO CURRENT BIOLOGY LA English DT Article ID SUPERFAMILY PALPIMANOIDEA; ANT ODONTOMACHUS; MANDIBLE STRIKE; BIOMECHANICS; PHYLOGENY; ARANEAE AB Small animals possess intriguing morphological and behavioral traits that allow them to capture prey, including innovative structural mechanisms that produce ballistic movements by amplifying power [1-6]. Power amplification occurs when an organism produces a relatively high power output by releasing slowly stored energy almost instantaneously, resulting in movements that surpass the maximal power output of muscles [7]. For example, trap-jaw, power -amplified mechanisms have been described for several ant genera [5, 8], which have evolved some of the fastest known movements in the animal kingdom [6]. However, power -amplified predatory strikes were not previously known in one of the largest animal classes, the arachnids. Mecysmaucheniidae spiders, which occur only in New Zealand and southern South America, are tiny, cryptic, ground-dwelling spiders that rely on hunting rather than web-building to capture prey [9]. Analysis of high-speed video revealed that power -amplified mechanisms occur in some mecysmaucheniid species, with the fastest species being two orders of magnitude faster than the slowest species. Molecular phylogenetic analysis revealed that power-amplified cheliceral strikes have evolved four times independently within the family. Furthermore, we identified morphological innovations that directly relate to cheliceral function: a highly modified carapace in which the cheliceral muscles are oriented horizontally; modification of a cheliceral sclerite to have muscle attachments; and, in the power-amplified species, a thicker clypeus and clypeal apodemes. These structural innovations may have set the stage for the parallel evolution of ballistic predatory strikes. C1 [Wood, Hannah M.] Natl Museum Nat Hist, Smithsonian Inst, Dept Entomol, Washington, DC 20013 USA. [Wood, Hannah M.; Griswold, Charles E.] Calif Acad Sci, Entomol Dept, San Francisco, CA 94118 USA. [Wood, Hannah M.; Gillespie, Rosemary G.; Elias, Damian O.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Parkinson, Dilworth Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Wood, HM (reprint author), Natl Museum Nat Hist, Smithsonian Inst, Dept Entomol, Washington, DC 20013 USA.; Wood, HM (reprint author), Calif Acad Sci, Entomol Dept, San Francisco, CA 94118 USA.; Wood, HM (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. EM woodh@si.edu FU NSF [1202873, DDIG 0909800, DEB-0613775, DEB-0072713, EAR-0228699]; NSF EAPSI New Zealand grant; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX Funding for this project came from NSF Postdoctoral Fellowship 1202873, NSF DDIG 0909800, and an NSF EAPSI New Zealand grant to H.M.W. Additional funding came from the following NSF grants: DEB-0613775 to R.G.G. and C.E.G., DEB-0072713 to C.E.G., and EAR-0228699. Support for fieldwork came from the Lindsay Expedition, Exline-Frizzell Funds at California Academy of Sciences, and the Schlinger Foundation. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 19 TC 0 Z9 0 U1 8 U2 10 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0960-9822 EI 1879-0445 J9 CURR BIOL JI Curr. Biol. PD APR 25 PY 2016 VL 26 IS 8 BP 1057 EP 1061 DI 10.1016/j.cub.2016.02.029 PG 5 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DL0RG UT WOS:000375339700024 PM 27068421 ER PT J AU Liberman-Martin, AL Levine, DS Liu, WJ Bergman, RG Tilley, TD AF Liberman-Martin, Allegra L. Levine, Daniel S. Liu, Wenjun Bergman, Robert G. Tilley, T. Don TI Biaryl Reductive Elimination Is Dramatically Accelerated by Remote Lewis Acid Binding to a 2,2 '-Bipyrimidyl-Platinum Complex: Evidence for a Bidentate Ligand Dissociation Mechanism SO ORGANOMETALLICS LA English DT Article ID SPECTROSCOPIC CHARACTERISTICS; PLATINUM COMPLEXES; CRYSTAL-STRUCTURE; ALKYNE COMPLEXES; ELECTRON-POOR; REACTIVITY; ACTIVATION; OXIDATION; CATALYSTS; NICKEL AB The silicon and zinc Lewis. acids Si(cat)(2) (cat = catecholato), Si(cat(F))(2) (cat(F) = tetrafluorocatecholato), and Zn(C6F5)(2) bind to the remote ligand site of a 2,2'-bipyrimidyl-platinum diaryl complex. This platinum complex provides a platform to systematically evaluate electronic and reactivity differences triggered by Lewis acid binding. The electron density of the bipyrimidine ligand is substantially depleted upon Lewis acid binding, as evidenced by UV-vis spectroscopy and cyclic voltammetry. Biaryl reductive elimination studies allowed quantification of the effect of Lewis acid binding on reactivity, and Lewis acid binding accelerated reductive elimination rates by up to 8 orders of magnitude. Kinetics experiments in combination with DFT studies support an unusual mechanism featuring complete dissociation of the Lewis acid coordinated bidentate bipyrimidine ligand prior to reductive elimination. C1 [Liberman-Martin, Allegra L.; Levine, Daniel S.; Bergman, Robert G.; Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Liu, Wenjun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Bergman, RG; Tilley, TD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM rbergman@berkeley.edu; tdtilley@berkeley.edu OI Levine, Daniel S/0000-0001-8921-3659; Liberman-Martin, Allegra/0000-0002-8447-905X FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-0841786, CHE-0840505]; National Institutes of Health [S10-RR027172]; Berkeley College of Chemstry NMR facility [SRR023679A]; NSF Graduate Research Fellowship; Office of Science of the U.S. Department of Energy [DE-SC0004993] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy, under contract no. DE-AC02-05CH11231 (T.D.T.) and the National Science Foundation under award no. CHE-0841786 (RG.B.). We also acknowledge the National Institutes of Health for funding of the ChexRay X-ray crystallographic facility (College of Chemistry, University of California, Berkeley) under grant number S10-RR027172, the Berkeley College of Chemstry NMR facility under grant SRR023679A, and the National Science Foundation for funding the Molecular Graphics and Computation Facility under grant number CHE-0840505. D.S.L. would like to acknowledge support of an NSF Graduate Research Fellowship. Electrochemical measurements were performed at the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under award number DE-SC0004993 (W.L.). The authors thank Mark C. Lipke for useful discussions on silicon Lewis acids, Michael I. Lipschutz and Micah S. Ziegler for assistance with X-ray diffraction, and Teera Chantarojsiri for assistance with UV vis spectroscopy. NR 45 TC 5 Z9 5 U1 10 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD APR 25 PY 2016 VL 35 IS 8 BP 1064 EP 1069 DI 10.1021/acs.organomet.5b01003 PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA DK6GP UT WOS:000375021000003 ER PT J AU Dicks, OA Shluger, AL Sushko, PV Littlewood, PB AF Dicks, Oliver A. Shluger, Alexander L. Sushko, Peter V. Littlewood, Peter B. TI Spectroscopic properties of oxygen vacancies in LaAlO3 SO PHYSICAL REVIEW B LA English DT Article ID SPACE GAUSSIAN PSEUDOPOTENTIALS; EFFECTIVE CORE POTENTIALS; DENSITY-FUNCTIONAL THEORY; MOLECULAR CALCULATIONS; PHASE-TRANSITION; BASIS-SETS; AB-INITIO; INTERFACES; PEROVSKITES; FILMS AB Oxygen vacancies in LaAlO3 (LAO) play an important role in the formation of the two-dimensional electron gas observed at the LaAlO3/SrTiO3 interface and affect the performance of MOSFETs using LAO as a gate dielectric. However, their spectroscopic properties are still poorly understood, which hampers their experimental identification. Here we predict the absorption spectra and ESR parameters of oxygen vacancies in LAO using periodic and embedded cluster methods and density functional theory (DFT). The structure, charge distribution, and spectroscopic properties of the neutral (V-O(0)) and charged (V-O(+) and V-O(2+)) oxygen vacancies in cubic and rhombohedral LaAlO3 are investigated. The highest intensity optical transitions [calculated using time-dependent DFT (TDDFT)], from the oxygen vacancy states to the conduction-band states have onsets at 3.5 and 4.2 eV for V-O(0) and 3.6 eV for V-O(+) in rhombohedral LAO and 3.3 and 4.0 eV for V-O(0) and 3.4 eV for V-O(+) in cubic LAO, respectively. Also reported are the isotropic g value (2.004026) and hyperfine coupling constants of V-O(0), which are compared to the experimental data obtained using electron spin resonance (ESR) spectroscopy, and accurately predict both the position and the width (3 mT) of its ESR signature. These results may further facilitate the experimental identification of oxygen vacancies in LAO and help to establish their role at the LAO/STO interfaces and in nanodevices using LAO. C1 [Dicks, Oliver A.; Shluger, Alexander L.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Sushko, Peter V.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Littlewood, Peter B.] Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60439 USA. RP Dicks, OA (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. EM oliver.dicks.11@ucl.ac.uk RI Littlewood, Peter/B-7746-2008; Sushko, Peter/F-5171-2013 OI Sushko, Peter/0000-0001-7338-4146 FU Argonne National Laboratory; Royal Society; EPSRC [EP/L000202]; Office of Science and Technology through EPSRC's High End Computing Programme FX O.A.D. thanks Argonne National Laboratory for the financial support. P.V.S. thanks the Royal Society, which supported preliminary work on this project, and the Laboratory Directed Research and Development program at PNNL, a multiprogram national laboratory operated by Battelle for the US Department of Energy. We would like to thank Dr. Matthew Watkins for useful discussions. Via our membership of the UK's HPC Materials Chemistry Consortium, which is funded by EPSRC (EP/L000202), this work made use of the facilities of HECToR and ARCHER, the UK's national high-performance computing service, which is funded by the Office of Science and Technology through EPSRC's High End Computing Programme. NR 58 TC 0 Z9 0 U1 13 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 13 AR 134114 DI 10.1103/PhysRevB.93.134114 PG 10 WC Physics, Condensed Matter SC Physics GA DK5DA UT WOS:000374938700001 ER PT J AU Farmer, B Bhat, VS Balk, A Teipel, E Smith, N Unguris, J Keavney, DJ Hastings, JT De Long, LE AF Farmer, B. Bhat, V. S. Balk, A. Teipel, E. Smith, N. Unguris, J. Keavney, D. J. Hastings, J. T. De Long, L. E. TI Direct imaging of coexisting ordered and frustrated sublattices in artificial ferromagnetic quasicrystals SO PHYSICAL REVIEW B LA English DT Article ID SPIN ICE; FILMS AB We have used scanning electron microscopy with polarization analysis and photoemission electron microscopy to image the two-dimensional magnetization of permalloy films patterned into Penrose P2 tilings (P2T). The interplay of exchange interactions in asymmetrically coordinated vertices and short-range dipole interactions among connected film segments stabilize magnetically ordered, spatially distinct sublattices that coexist with frustrated sublattices at room temperature. Numerical simulations that include long-range dipole interactions between sublattices agree with images of as-grown P2T samples and predict a magnetically ordered ground state for a two-dimensional quasicrystal lattice of classical Ising spins. C1 [Farmer, B.; Bhat, V. S.; Teipel, E.; Smith, N.; De Long, L. E.] Univ Kentucky, Dept Phys & Astron, 505 Rose St, Lexington, KY 40506 USA. [Balk, A.; Unguris, J.] NIST, Ctr Nanoscale Sci & Technol, 100 Bur Dr, Gaithersburg, MD 20899 USA. [Balk, A.] Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA. [Keavney, D. J.] Argonne Natl Lab, Adv Photon Source 431 E007, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hastings, J. T.] Univ Kentucky, Dept Elect & Comp Engn, 453F Paul Anderson Tower, Lexington, KY 40506 USA. RP De Long, LE (reprint author), Univ Kentucky, Dept Phys & Astron, 505 Rose St, Lexington, KY 40506 USA. EM delong@pa.uky.edu FU U.S. DoE [DE-FG02-97ER45653]; U.S. NSF [DMR-1506979]; UK Center for Advanced Materials; UK Center for Computational Sciences; UK Center for Nanoscale Science and Engineering; University of Maryland [70NANB10H193]; National Institute of Standards and Technology Center for Nanoscale Science and Technology through the University of Maryland [70NANB10H193]; Research at the Advanced Photon Source, a U.S. Department of Energy Office of Science User Facility [DE-AC02-06CH11357] FX Research at University of Kentucky was supported by U.S. DoE Grant DE-FG02-97ER45653, U.S. NSF Grant DMR-1506979, the UK Center for Advanced Materials, the UK Center for Computational Sciences, and the UK Center for Nanoscale Science and Engineering. AB acknowledges support of this research under the Cooperative Research Agreement between the University of Maryland and National Institute of Standards and Technology Center for Nanoscale Science and Technology, Award 70NANB10H193, through the University of Maryland. Research at the Advanced Photon Source, a U.S. Department of Energy Office of Science User Facility operated by Argonne National Laboratory, was supported under Contract No. DE-AC02-06CH11357. J. P. Straley, K. Ross, and F. Guo contributed helpful criticism. NR 45 TC 4 Z9 4 U1 6 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 13 AR 134428 DI 10.1103/PhysRevB.93.134428 PG 11 WC Physics, Condensed Matter SC Physics GA DK5DA UT WOS:000374938700005 ER PT J AU Shatnawi, M Bozin, ES Mitchell, JF Billinge, SJL AF Shatnawi, Mouath Bozin, Emil S. Mitchell, J. F. Billinge, Simon J. L. TI Nonpercolative nature of the metal-insulator transition and persistence of local Jahn-Teller distortions in the rhombohedral regime of La1-xCaxMnO3 SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC PHASE-SEPARATION; MIXED-VALENT MANGANITES; COLOSSAL MAGNETORESISTANCE; CHARGE LOCALIZATION; NEUTRON-DIFFRACTION; FERROMAGNETIC PHASE; MAGNETIC PHASE; TRANSPORT; LA0.7CA0.3MNO3; PEROVSKITES AB Evolution of the average and local crystal structure of Ca-doped LaMnO3 has been studied across the metal to insulator (MI) and the orthorhombic to rhombohedral (OR) structural phase transitions over a broad temperature range for two Ca concentrations (x = 0.18,0.22). Combined Rietveld and high real space resolution atomic pair distribution function (PDF) analysis of neutron total scattering data was carried out with aims of exploring the possibility of nanoscale phase separation (PS) in relation to MI transition, and charting the evolution of local Jahn-Teller (JT) distortion of MnO6 octahedra across the OR transition at T-S similar to 720 K. The study utilized explicit two-phase PDF structural modeling, revealing that away from T-MI there is no evidence for nanoscale phase coexistence. The local JT distortions disappear abruptly upon crossing into the metallic regime both with doping and temperature, with only a small temperature-independent signature of quenched disorder being observable at low temperature as compared to CaMnO3. The results hence do not support the percolative scenario for the MI transition in La1-xCaxMnO3 based on PS, and question its ubiquity in the manganites. In contrast to LaMnO3 that exhibits long-range orbital correlations and sizable octahedral distortions at low temperature, the doped samples with compositions straddling the MI boundary exhibit correlations (in the insulating regime) limited to only similar to 1 nm with observably smaller distortions. In the x = 0.22 sample local JT distortions are found to persist across the OR transition and deep into the R phase (up to similar to 1050 K), where they are crystallographically prohibited. Their magnitude and subnanometer spatial extent remain unchanged. C1 [Shatnawi, Mouath] Hashemite Univ, Dept Phys, Zarqa 13115, Jordan. [Bozin, Emil S.; Billinge, Simon J. L.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. [Mitchell, J. F.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Billinge, Simon J. L.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Bozin, ES (reprint author), Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. EM bozin@bnl.gov FU U.S. DOE, Office of Science, Office of Basic Energy Sciences (DOE-BES) [DE-SC00112704]; U.S. Department of Energy Office of Science, Basic Energy Sciences; Materials Science and Engineering Division; [DE-AC52-06NA25396] FX Work at Brookhaven National Laboratory was supported by U.S. DOE, Office of Science, Office of Basic Energy Sciences (DOE-BES) under Contract DE-SC00112704. Work in the Materials Science Division of Argonne National Laboratory (sample preparation and characterization) was sponsored by the U.S. Department of Energy Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Neutron PDF experiments were carried out on NPDF at LANSCE, funded by DOE BES; Los Alamos National Laboratory is operated by Los Alamos National Security LLC under Contract No. DE-AC52-06NA25396. E.S.B. gratefully acknowledges T.E. Proffen and J. Siewenie for assistance with the NPDF measurements. NR 59 TC 0 Z9 0 U1 12 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 16 AR 165138 DI 10.1103/PhysRevB.93.165138 PG 10 WC Physics, Condensed Matter SC Physics GA DK5HF UT WOS:000374950300010 ER PT J AU Xiao, S Yoon, Y Lee, YH Bird, JP Ochiai, Y Aoki, N Reno, JL Fransson, J AF Xiao, S. Yoon, Y. Lee, Y. -H. Bird, J. P. Ochiai, Y. Aoki, N. Reno, J. L. Fransson, J. TI Detecting weak coupling in mesoscopic systems with a nonequilibrium Fano resonance SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM POINT CONTACTS; PLASMONIC NANOCAVITIES; METAMATERIALS AB A critical aspect of quantum mechanics is the nonlocal nature of the wave function, a characteristic that may yield unexpected coupling of nominally isolated systems. The capacity to detect this coupling can be vital in many situations, especially those in which its strength is weak. In this work, we address this problem in the context of mesoscopic physics, by implementing an electron-wave realization of a Fano interferometer using pairs of coupled quantum point contacts (QPCs). Within this scheme, the discrete level required for a Fano resonance is provided by pinching off one of the QPCs, thereby inducing the formation of a quasibound state at the center of its self-consistent potential barrier. Using this system, we demonstrate a form of nonequilibrium Fano resonance (NEFR), in which nonlinear electrical biasing of the interferometer gives rise to pronounced distortions of its Fano resonance. Our experimental results are captured well by a quantitative theoretical model, which considers a system in which a standard two-path Fano interferometer is coupled to an additional, intruder, continuum. According to this theory, the observed distortions in the Fano resonance arise only in the presence of coupling to the intruder, indicating that the NEFR provides a sensitive means to infer the presence of weak coupling between mesoscopic systems. C1 [Xiao, S.; Yoon, Y.; Lee, Y. -H.; Bird, J. P.] Univ Buffalo, State Univ New York, Dept Elect Engn, Buffalo, NY 14260 USA. [Bird, J. P.; Ochiai, Y.; Aoki, N.] Chiba Univ, Grad Sch Adv Integrat Sci, Inage Ku, 1-33 Yayoi Cho, Chiba 2638522, Japan. [Reno, J. L.] Sandia Natl Labs, CINT, Dept 1131, MS 1303, Albuquerque, NM 87185 USA. [Fransson, J.] Uppsala Univ, Dept Phys & Astron, Box 516, SE-75121 Uppsala, Sweden. RP Bird, JP (reprint author), Univ Buffalo, State Univ New York, Dept Elect Engn, Buffalo, NY 14260 USA.; Bird, JP (reprint author), Chiba Univ, Grad Sch Adv Integrat Sci, Inage Ku, 1-33 Yayoi Cho, Chiba 2638522, Japan.; Fransson, J (reprint author), Uppsala Univ, Dept Phys & Astron, Box 516, SE-75121 Uppsala, Sweden. EM jbird@buffalo.edu; jonas.fransson@physics.uu.se FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-04ER46180]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Swedish Research Council FX The experimental research in the group of JPB at Buffalo was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-FG02-04ER46180. Epitaxial growth of the high-quality 2DEG layers was performed by JLR at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. JF acknowledges support from the Swedish Research Council. NR 54 TC 1 Z9 1 U1 4 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 16 AR 165435 DI 10.1103/PhysRevB.93.165435 PG 12 WC Physics, Condensed Matter SC Physics GA DK5HF UT WOS:000374950300017 ER PT J AU Yuan, SJ Butrouna, K Terzic, J Zheng, H Aswartham, S DeLong, LE Ye, F Schlottmann, P Cao, G AF Yuan, S. J. Butrouna, K. Terzic, J. Zheng, H. Aswartham, S. DeLong, L. E. Ye, Feng Schlottmann, P. Cao, G. TI Ground-state tuning of metal-insulator transition by compositional variations in BaIr1-xRuxO3 (0 <= x <= 1) SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-WAVE FORMATION; WEAK FERROMAGNETISM; BAIRO3; SR2IRO4 AB Hexagonal BaIrO3 is a magnetic insulator driven by the spin-orbit interaction (SOI), whereas BaRuO3 is an enhanced paramagnetic metal. Our investigation of structural, magnetic, transport, and thermal properties reveals that substitution of Ru4+ (4d(4)) ions for Ir4+ (5d(5)) ions in BaIrO3 reduces the magnitudes of the SOI and a monoclinic structural distortion and rebalances the competition between the SOI and the lattice degrees of freedom to render an evolution from a magnetic insulting state to a robust metallic state. The central findings of this paper are as follows: (1) light Ru doping (0 < x <= 0.15) prompts simultaneous, precipitous drops in both the magnetic ordering temperature T-N and the electrical resistivity, and (2) heavier Ru doping (0.41 <= x <= 0.9) induces a robust metallic state without any long-range magnetic order. All results suggest a critical role of the lattice degrees of freedom in determining the ground state in the heavy transition-metal oxides. C1 [Yuan, S. J.; Butrouna, K.; Terzic, J.; Zheng, H.; Aswartham, S.; DeLong, L. E.; Cao, G.] Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. [Ye, Feng] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Schlottmann, P.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. RP Yuan, SJ (reprint author), Univ Kentucky, Dept Phys & Astron, Ctr Adv Mat, Lexington, KY 40506 USA. EM sjyuan.shu@gmail.com; cao@uky.edu RI Ye, Feng/B-3210-2010 OI Ye, Feng/0000-0001-7477-4648 FU National Science Foundation [DMR-1265162]; Department of Energy (BES) [DE-FG02-98ER45707, DE-FG02-97ER45653] FX This work was supported by the National Science Foundation via Grant No. DMR-1265162 (G.C.) and Department of Energy (BES) through Grants No. DE-FG02-98ER45707 (P.S.) and No. DE-FG02-97ER45653 (L.E.D.). NR 22 TC 0 Z9 0 U1 8 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 16 AR 165136 DI 10.1103/PhysRevB.93.165136 PG 5 WC Physics, Condensed Matter SC Physics GA DK5HF UT WOS:000374950300008 ER PT J AU Zhao, ZY Calder, S Aczel, AA McGuire, MA Sales, BC Mandrus, DG Chen, G Trivedi, N Zhou, HD Yan, JQ AF Zhao, Z. Y. Calder, S. Aczel, A. A. McGuire, M. A. Sales, B. C. Mandrus, D. G. Chen, G. Trivedi, N. Zhou, H. D. Yan, J. -Q. TI Fragile singlet ground-state magnetism in the pyrochlore osmates R2Os2O7 (R=Y and Ho) SO PHYSICAL REVIEW B LA English DT Article ID R=RARE EARTH; SPIN AB The singlet ground-state magnetism in pyrochlore osmates Y2Os2O7 and Ho2Os2O7 is studied by dc and ac susceptibility, specific heat, and neutron powder diffraction measurements. Despite the expected nonmagnetic singlet in the strong spin-orbit coupling (SOC) limit for Os4+ (5d(4)), Y2Os2O7 exhibits a spin-glass ground state below 4 K with weak magnetism, suggesting possible proximity to a quantum phase transition between the nonmagnetic state in the strong SOC limit and a magnetic state in the strong superexchange limit. Ho2Os2O7 has the same structural distortion as in Y2Os2O7; however, the Os sublattice in Ho2Os2O7 shows long-range magnetic ordering below 36 K. The sharp difference of the magnetic ground state between Y2Os2O7 and Ho2Os2O7 signals that the singlet ground-statemagnetism in R2Os2O7 is fragile and can be disturbed by the weak 4f-5d interactions. C1 [Zhao, Z. Y.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Zhao, Z. Y.; McGuire, M. A.; Sales, B. C.; Mandrus, D. G.; Yan, J. -Q.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Calder, S.; Aczel, A. A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Mandrus, D. G.; Yan, J. -Q.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Chen, G.] Fudan Univ, Dept Phys, Collaborat Innovat Ctr Adv Microstruct, Shanghai 200433, Peoples R China. [Chen, G.] Fudan Univ, Ctr Field Theory & Particle Phys, Shanghai 200433, Peoples R China. [Trivedi, N.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. RP Yan, JQ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.; Yan, JQ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM yanj@ornl.gov RI McGuire, Michael/B-5453-2009; Zhou, Haidong/O-4373-2016 OI McGuire, Michael/0000-0003-1762-9406; FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; NSF MRSEC [DMR-1420451]; Scientific User Facilities Division, Office of Basic Energy Sciences; US Department of Energy; Gordon and Betty Moore Foundations EPiQS Initiative [GBMF4416]; [NSF-DMR-1350002] FX Work at ORNL was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Z.Y.Z. and N.T. acknowledge the CEM, and NSF MRSEC, under Grant No. DMR-1420451. Research conducted at ORNL's HFIR was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, and US Department of Energy. H.D.Z. acknowledges support from NSF-DMR-1350002. D.G.M. acknowledges support from the Gordon and Betty Moore Foundations EPiQS Initiative through Grant No. GBMF4416. NR 27 TC 3 Z9 3 U1 6 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 25 PY 2016 VL 93 IS 13 AR 134426 DI 10.1103/PhysRevB.93.134426 PG 6 WC Physics, Condensed Matter SC Physics GA DK5DA UT WOS:000374938700003 ER PT J AU Alduino, C Alfonso, K Artusa, DR Avignone, FT Azzolini, O Banks, TI Bari, G Beeman, JW Bellini, F Bersani, A Biassoni, M Brofferio, C Bucci, C Caminata, A Canonica, L Cao, XG Capelli, S Cappelli, L Carbone, L Cardani, L Carniti, P Casali, N Cassina, L Chiesa, D Chott, N Clemenza, M Copello, S Cosmelli, C Cremonesi, O Creswick, RJ Cushman, JS Dafinei, I Dally, A Davis, CJ Dell'Oro, S Deninno, MM Di Domizio, S Di Vacri, ML Drobizhev, A Fang, DQ Faverzani, M Fernandes, G Ferri, E Ferroni, F Fiorini, E Freedman, SJ Fujikawa, BK Giachero, A Gironi, L Giuliani, A Gladstone, L Gorla, P Gotti, C Gutierrez, TD Haller, EE Han, K Hansen, E Heeger, KM Hennings-Yeomans, R Hickerson, KP Huang, HZ Kadel, R Keppel, G Kolomensky, YG Lim, KE Liu, X Ma, YG Maino, M Marini, L Martinez, M Maruyama, RH Mei, Y Moggi, N Morganti, S Mosteiro, PJ Nones, C Norman, EB Nucciotti, A O'Donnell, T Orio, F Ouellet, JL Pagliarone, CE Pallavicini, M Palmieri, V Pattavina, L Pavan, M Pessina, G Pettinacci, V Piperno, G Pirro, S Pozzi, S Previtali, E Rosenfeld, C Rusconi, C Sala, E Sangiorgio, S Santone, D Scielzo, ND Singh, V Sisti, M Smith, AR Taffarello, L Tenconi, M Terranova, F Tomei, C Trentalange, S Ventura, G Vignati, M Wagaarachchi, SL Wang, BS Wang, HW Wilson, J Winslow, LA Wise, T Woodcraft, A Zanotti, L Zhang, GQ Zhu, BX Zimmermann, S Zucchelli, S AF Alduino, C. Alfonso, K. Artusa, D. R. Avignone, F. T., III Azzolini, O. Banks, T. I. Bari, G. Beeman, J. W. Bellini, F. Bersani, A. Biassoni, M. Brofferio, C. Bucci, C. Caminata, A. Canonica, L. Cao, X. G. Capelli, S. Cappelli, L. Carbone, L. Cardani, L. Carniti, P. Casali, N. Cassina, L. Chiesa, D. Chott, N. Clemenza, M. Copello, S. Cosmelli, C. Cremonesi, O. Creswick, R. J. Cushman, J. S. Dafinei, I. Dally, A. Davis, C. J. Dell'Oro, S. Deninno, M. M. Di Domizio, S. Di Vacri, M. L. Drobizhev, A. Fang, D. Q. Faverzani, M. Fernandes, G. Ferri, E. Ferroni, F. Fiorini, E. Freedman, S. J. Fujikawa, B. K. Giachero, A. Gironi, L. Giuliani, A. Gladstone, L. Gorla, P. Gotti, C. Gutierrez, T. D. Haller, E. E. Han, K. Hansen, E. Heeger, K. M. Hennings-Yeomans, R. Hickerson, K. P. Huang, H. Z. Kadel, R. Keppel, G. Kolomensky, Yu. G. Lim, K. E. Liu, X. Ma, Y. G. Maino, M. Marini, L. Martinez, M. Maruyama, R. H. Mei, Y. Moggi, N. Morganti, S. Mosteiro, P. J. Nones, C. Norman, E. B. Nucciotti, A. O'Donnell, T. Orio, F. Ouellet, J. L. Pagliarone, C. E. Pallavicini, M. Palmieri, V. Pattavina, L. Pavan, M. Pessina, G. Pettinacci, V. Piperno, G. Pirro, S. Pozzi, S. Previtali, E. Rosenfeld, C. Rusconi, C. Sala, E. Sangiorgio, S. Santone, D. Scielzo, N. D. Singh, V. Sisti, M. Smith, A. R. Taffarello, L. Tenconi, M. Terranova, F. Tomei, C. Trentalange, S. Ventura, G. Vignati, M. Wagaarachchi, S. L. Wang, B. S. Wang, H. W. Wilson, J. Winslow, L. A. Wise, T. Woodcraft, A. Zanotti, L. Zhang, G. Q. Zhu, B. X. Zimmermann, S. Zucchelli, S. CA CUORE Collaboration TI Analysis techniques for the evaluation of the neutrinoless double-beta decay lifetime in Te-130 with the CUORE-0 detector SO PHYSICAL REVIEW C LA English DT Article ID MAJORANA NEUTRINOS; RARE DECAYS; CONTAMINATION; PERFORMANCE; PRINCIPLES; VALIDATION; LIMITS AB We describe in detail the methods used to obtain the lower bound on the lifetime of neutrinoless double-beta (0 nu beta beta) decay in Te-130 and the associated limit on the effective Majorana mass of the neutrino using the CUORE-0 detector. CUORE-0 is a bolometric detector array located at the Laboratori Nazionali del Gran Sasso that was designed to validate the background reduction techniques developed for CUORE, a next-generation experiment scheduled to come online in 2016. CUORE-0 is also a competitive 0 nu beta beta decay search in its own right and functions as a platform to further develop the analysis tools and procedures to be used in CUORE. These include data collection, event selection and processing, as well as an evaluation of signal efficiency. In particular, we describe the amplitude evaluation, thermal gain stabilization, energy calibration methods, and the analysis event selection used to create our final 0 nu beta beta search spectrum. We define our high level analysis procedures, with emphasis on the new insights gained and challenges encountered. We outline in detail our fitting methods near the hypothesized 0 nu beta beta decay peak and catalog the main sources of systematic uncertainty. Finally, we derive the 0 nu beta beta decay half-life limits previously reported for CUORE-0, T-1/2(0 nu) > 2.7 x 10(24) yr, and in combination with the Cuoricino limit, T-1/2(0 nu) > 4.0 x 10(24) yr. C1 [Alduino, C.; Artusa, D. R.; Avignone, F. T., III; Chott, N.; Creswick, R. J.; Rosenfeld, C.; Wilson, J.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Alfonso, K.; Hansen, E.; Hickerson, K. P.; Huang, H. Z.; Liu, X.; Trentalange, S.; Zhu, B. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Artusa, D. R.; Bucci, C.; Canonica, L.; Cappelli, L.; Dell'Oro, S.; Di Vacri, M. L.; Gorla, P.; Pagliarone, C. E.; Pattavina, L.; Pirro, S.; Santone, D.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. [Azzolini, O.; Keppel, G.; Palmieri, V.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Padova, Italy. [Banks, T. I.; Drobizhev, A.; Freedman, S. J.; Hennings-Yeomans, R.; Kolomensky, Yu. G.; O'Donnell, T.; Ouellet, J. L.; Singh, V.; Wagaarachchi, S. L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Banks, T. I.; Drobizhev, A.; Freedman, S. J.; Fujikawa, B. K.; Han, K.; Hennings-Yeomans, R.; Mei, Y.; O'Donnell, T.; Ouellet, J. L.; Smith, A. R.; Wagaarachchi, S. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Bari, G.; Deninno, M. M.; Moggi, N.; Zucchelli, S.] Ist Nazl Fis Nucl, Sez Bologna, I-40127 Bologna, Italy. [Beeman, J. W.; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Casali, N.; Cosmelli, C.; Ferroni, F.; Martinez, M.; Piperno, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Bellini, F.; Cardani, L.; Casali, N.; Cosmelli, C.; Dafinei, I.; Ferroni, F.; Martinez, M.; Morganti, S.; Mosteiro, P. J.; Orio, F.; Pettinacci, V.; Piperno, G.; Tomei, C.; Vignati, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bersani, A.; Caminata, A.; Cappelli, L.; Copello, S.; Di Domizio, S.; Fernandes, G.; Marini, L.; Pallavicini, M.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carniti, P.; Cassina, L.; Chiesa, D.; Clemenza, M.; Faverzani, M.; Ferri, E.; Fiorini, E.; Gironi, L.; Gotti, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Pozzi, S.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carbone, L.; Carniti, P.; Cassina, L.; Chiesa, D.; Clemenza, M.; Cremonesi, O.; Faverzani, M.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Pessina, G.; Pozzi, S.; Previtali, E.; Rusconi, C.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Cao, X. G.; Fang, D. Q.; Ma, Y. G.; Wang, H. W.; Zhang, G. Q.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Cappelli, L.; Pagliarone, C. E.] Univ Cassino & Lazio Meridionale, Dipartimento Ingn Civile & Meccan, I-03043 Cassino, Italy. [Copello, S.; Di Domizio, S.; Fernandes, G.; Marini, L.; Pallavicini, M.] Univ Genoa, Dipartimento Fis, Via Dodecaneso 33, I-16146 Genoa, Italy. [Cushman, J. S.; Davis, C. J.; Han, K.; Heeger, K. M.; Lim, K. E.; Maruyama, R. H.; Wise, T.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Dally, A.; Wise, T.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Dell'Oro, S.] Ist Nazl Fis Nucl, Gran Sasso Sci Inst, I-67100 Laquila, Italy. [Di Vacri, M. L.; Santone, D.] Univ Aquila, Dipartimento Sci Fis & Chim, I-67100 Laquila, Italy. [Giuliani, A.; Tenconi, M.] Ctr Spectrometrie Nucl & Spectrometrie Masse, F-91405 Orsay, France. [Gladstone, L.; Hansen, E.; Ouellet, J. L.; Winslow, L. A.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Gutierrez, T. D.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Kadel, R.; Kolomensky, Yu. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Martinez, M.] Univ Zaragoza, Lab Fis Nucl & Astroparticulas, E-50009 Zaragoza, Spain. [Moggi, N.] Univ Bologna, Alma Mater Studiorum, Dipartimento Sci Qualita Vita, I-47921 Bologna, Italy. [Nones, C.] CEA Saclay, Serv Phys Particules, F-91191 Gif Sur Yvette, France. [Norman, E. B.; Sangiorgio, S.; Scielzo, N. D.; Wang, B. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Norman, E. B.; Wang, B. S.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Taffarello, L.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Ventura, G.] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy. [Ventura, G.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Woodcraft, A.] Univ Edinburgh, Inst Astron, SUPA, Blackford Hill, Edinburgh EH9 3HJ, Midlothian, Scotland. [Zimmermann, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Zucchelli, S.] Univ Bologna, Alma Mater Studiorum, Dipartimento Fis & Astron, I-40127 Bologna, Italy. [Cardani, L.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. RP Alduino, C (reprint author), Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. EM cuore-spokesperson@lngs.infn.it RI Han, Ke/D-3697-2017; Chiesa, Davide/H-7240-2014; Di Domizio, Sergio/L-6378-2014; Vignati, Marco/H-1684-2013; Giachero, Andrea/I-1081-2013; Ferri, Elena/L-8531-2014; Ma, Yu-Gang/M-8122-2013; Casali, Nicola/C-9475-2017; Maruyama, Reina/A-1064-2013; Martinez, Maria/K-4827-2012; Gironi, Luca/P-2860-2016; Pattavina, Luca/I-7498-2015; capelli, silvia/G-5168-2012; Bellini, Fabio/D-1055-2009 OI Han, Ke/0000-0002-1609-7367; Chiesa, Davide/0000-0003-1978-1727; Di Domizio, Sergio/0000-0003-2863-5895; Vignati, Marco/0000-0002-8945-1128; Giachero, Andrea/0000-0003-0493-695X; Ferri, Elena/0000-0003-1425-3669; Ma, Yu-Gang/0000-0002-0233-9900; Casali, Nicola/0000-0003-3669-8247; Maruyama, Reina/0000-0003-2794-512X; Martinez, Maria/0000-0002-9043-4691; Gironi, Luca/0000-0003-2019-0967; Pattavina, Luca/0000-0003-4192-849X; capelli, silvia/0000-0002-0300-2752; Bellini, Fabio/0000-0002-2936-660X FU Istituto Nazionale di Fisica Nucleare (INFN); National Science Foundation [NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, NSF-PHY-0902171, NSF-PHY-0969852, NSF-PHY-1307204, NSF-PHY-1314881, NSF-PHY-1401832, NSF-PHY-1404205]; Alfred P. Sloan Foundation; University of Wisconsin Foundation; Yale University; US Department of Energy (DOE) Office of Science [DE-AC02-05CH11231, DE-AC52-07NA27344, DE-SC0012654]; DOE Office of Science, Office of Nuclear Physics [DE-FG02-08ER41551, DE-FG03-00ER41138] FX The CUORE Collaboration thanks the directors and staff of the Laboratori Nazionali del Gran Sasso and the technical staff of our laboratories. This work was supported by the Istituto Nazionale di Fisica Nucleare (INFN); the National Science Foundation under Grant Nos. NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, NSF-PHY-0902171, NSF-PHY-0969852, NSF-PHY-1307204, NSF-PHY-1314881, NSF-PHY-1401832, and NSF-PHY-1404205; the Alfred P. Sloan Foundation; the University of Wisconsin Foundation; and Yale University. This material is also based upon work supported by the US Department of Energy (DOE) Office of Science under Contract Nos. DE-AC02-05CH11231, DE-AC52-07NA27344, and DE-SC0012654; and by the DOE Office of Science, Office of Nuclear Physics under Contract Nos. DE-FG02-08ER41551 and DE-FG03-00ER41138. This research used resources of the National Energy Research Scientific Computing Center (NERSC). NR 43 TC 6 Z9 6 U1 12 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 25 PY 2016 VL 93 IS 4 AR 045503 DI 10.1103/PhysRevC.93.045503 PG 17 WC Physics, Nuclear SC Physics GA DK5IR UT WOS:000374954100014 ER PT J AU Binder, S Ekstrom, A Hagen, G Papenbrock, T Wendt, KA AF Binder, S. Ekstrom, A. Hagen, G. Papenbrock, T. Wendt, K. A. TI Effective field theory in the harmonic oscillator basis SO PHYSICAL REVIEW C LA English DT Article ID QUANTUM-MECHANICAL PROBLEMS; CORE-SHELL-MODEL; MATRIX-ELEMENTS; NUCLEAR-FORCES; FRAMEWORK AB We develop interactions from chiral effective field theory (EFT) that are tailored to the harmonic oscillator basis. As a consequence, ultraviolet convergence with respect to the model space is implemented by construction and infrared convergence can be achieved by enlarging the model space for the kinetic energy. In oscillator EFT, matrix elements of EFTs formulated for continuous momenta are evaluated at the discrete momenta that stem from the diagonalization of the kinetic energy in the finite oscillator space. By fitting to realistic phase shifts and deuteron data we construct an effective interaction from chiral EFT at next-to-leading order. Many-body coupled-cluster calculations of nuclei up to Sn-132 converge fast for the ground-state energies and radii in feasible model spaces. C1 [Binder, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Binder, S (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-96ER40963, DE-SC0008499]; ORNL [DEAC05-00OR22725]; Alexander-von-Humboldt Foundation FX We are grateful to R. J. Furnstahl and S. Konig for helpful discussions and comments on the manuscript. We also thank J. Rotureau for helpful discussions. This material is based upon work supported in part by the US Department of Energy, Office of Science, Office of Nuclear Physics, under Awards No. DE-FG02-96ER40963 (University of Tennessee) and No. DE-SC0008499 (SciDAC-3 NUCLEI Collaboration), Field Work Proposal No. ERKBP57 at Oak Ridge National Laboratory (ORNL), and Contract No. DEAC05-00OR22725 (ORNL). S.B. gratefully acknowledges the financial support from the Alexander-von-Humboldt Foundation (Feodor-Lynen fellowship). NR 70 TC 1 Z9 1 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 25 PY 2016 VL 93 IS 4 AR 044332 DI 10.1103/PhysRevC.93.044332 PG 14 WC Physics, Nuclear SC Physics GA DK5IR UT WOS:000374954100006 ER PT J AU Moreland, JS Soltz, RA AF Moreland, J. Scott Soltz, Ron A. TI Hydrodynamic simulations of relativistic heavy-ion collisions with different lattice quantum chromodynamics calculations of the equation of state SO PHYSICAL REVIEW C LA English DT Article ID ENERGY AB Hydrodynamic calculations of ultrarelativistic heavy-ion collisions are performed using the iEBE-VISHNU 2+1-dimensional code with fluctuating initial conditions and three different parametrizations of the lattice QCD equations of state: continuum extrapolations for stout and HISQ/tree actions, as well as the s95p-v1 parametrization based upon calculations using the p4 action. All parametrizations are matched to a hadron resonance gas equation of state at T = 155 MeV, at which point the calculations are continued using the UrQMD hadronic cascade. Simulations of root sNN = 200 GeV Au+Au collisions in three centrality classes are used to quantify anisotropic flow developed in the hydrodynamic phase of the collision as well as particle spectra and pion Hanbury-Brown-Twiss (HBT) radii after hadronic rescattering, which are compared with experimental data. Experimental observables for the stout and HISQ/tree equations of state are observed to differ by less than a few percent for all observables, while the s95p-v1 equation of state generates spectra and flow coefficients which differ by similar to 10-20%. Calculations in which the HISQ/tree equation of state is sampled from the published error distribution are also observed to differ by less than a few percent. C1 [Moreland, J. Scott] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Soltz, Ron A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Moreland, JS (reprint author), Duke Univ, Dept Phys, Durham, NC 27708 USA. FU U.S. Department of Energy NNSA Stockpile Stewardship Graduate Fellowship [DE-FC52-08NA28752]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We wish to thank Jonah Bernard, Ulrich Heinz, and Christopher Plumberg for many helpful discussions. This work was performed with support from the U.S. Department of Energy NNSA Stockpile Stewardship Graduate Fellowship under Grant no. DE-FC52-08NA28752 and from Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 36 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 25 PY 2016 VL 93 IS 4 AR 044913 DI 10.1103/PhysRevC.93.044913 PG 10 WC Physics, Nuclear SC Physics GA DK5IR UT WOS:000374954100011 ER PT J AU Odell, D Papenbrock, T Platter, L AF Odell, D. Papenbrock, T. Platter, L. TI Infrared extrapolations of quadrupole moments and transitions SO PHYSICAL REVIEW C LA English DT Article ID CORE-SHELL-MODEL AB We study the convergence of bound-state quadrupole moments in finite harmonic oscillator spaces. We derive an expression for the infrared extrapolation for the quadrupole moment of a nucleus and benchmark our results using different model interactions for the deuteron. We find good agreement between the analytically derived and numerically obtained convergence behavior. We also derive an extrapolation formula for electric quadrupole transitions and find good agreement with the numerical calculation of a simple system. C1 [Odell, D.; Papenbrock, T.; Platter, L.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Papenbrock, T.; Platter, L.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Odell, D (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Platter, Lucas/N-3887-2013; OI Platter, Lucas/0000-0001-6632-8250; Papenbrock, Thomas/0000-0001-8733-2849 FU US Department of Energy, Office of Science, Office of Nuclear Physics [DEFG02-96ER40963, DE-AC05-00OR22725]; National Science Foundation [PHY-1516077]; US-Israel Binational Science Foundation [2012212] FX We thank A. Ekstrom for providing us with matrix elements. This work was supported in parts by the US Department of Energy, Office of Science, Office of Nuclear Physics under Grant No. DEFG02-96ER40963 (University of Tennessee) and Contract No. DE-AC05-00OR22725 (Oak Ridge National Laboratory), the National Science Foundation under Grant No. PHY-1516077, and by the US-Israel Binational Science Foundation under Grant No. 2012212. NR 18 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 25 PY 2016 VL 93 IS 4 AR 044331 DI 10.1103/PhysRevC.93.044331 PG 7 WC Physics, Nuclear SC Physics GA DK5IR UT WOS:000374954100005 ER PT J AU Albright, CH Feger, RP Kephart, TW AF Albright, Carl H. Feger, Robert P. Kephart, Thomas W. TI Unification of gauge, family, and flavor symmetries illustrated in gauged SU(12) models SO PHYSICAL REVIEW D LA English DT Article ID GRAND UNIFICATION; UNIFIED MODEL AB To explain quark and lepton masses and mixing angles, one has to extend the standard model, and the usual practice is to put the quarks and leptons into irreducible representations of discrete groups. We argue that discrete flavor symmetries (and their concomitant problems) can be avoided if we extend the gauge group. In the framework of SU(12) we give explicit examples of models having varying degrees of predictability obtained by scanning over groups and representations and identifying cases with operators contributing to mass and mixing matrices that need little fine-tuning of prefactors. Fitting with quark and lepton masses run to the GUT scale and known mixing angles allows us to make predictions for the neutrino masses and hierarchy, the octant of the atmospheric mixing angle, leptonic CP violation, Majorana phases, and the effective mass observed in neutrinoless double beta decay. C1 [Albright, Carl H.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Albright, Carl H.] Fermilab Natl Accelerator Lab, Theoret Phys, Batavia, IL 60510 USA. [Feger, Robert P.] Univ Wurzburg, Inst Theoret Phys & Astrophys, D-97074 Wurzburg, Germany. [Kephart, Thomas W.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. RP Albright, CH (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.; Albright, CH (reprint author), Fermilab Natl Accelerator Lab, Theoret Phys, Batavia, IL 60510 USA.; Feger, RP (reprint author), Univ Wurzburg, Inst Theoret Phys & Astrophys, D-97074 Wurzburg, Germany.; Kephart, TW (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. EM albright@fnal.gov; robert.feger@gmail.com; thomas.w.kephart@vanderbilt.edu OI Albright, Carl/0000-0002-2252-6359 FU Postdoc Programme of the German Academic Exchange Sevice (DAAD); Bundesministerium fur Bildung und Forschung (BMBF) [05H12WWE]; U.S. Department of Energy [DE-FG05-85ER40226, DE-AC02-07CH11359] FX One of us (C.H.A.) thanks the Fermilab Theoretical Division for its kind hospitality where his research was carried out. The work of R.P.F. was supported by a fellowship within the Postdoc Programme of the German Academic Exchange Sevice (DAAD) and the Bundesministerium fur Bildung und Forschung (BMBF) under Contract No. 05H12WWE. The work of T.W.K. was supported by U.S. Department of Energy Grant No. DE-FG05-85ER40226. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 27 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 25 PY 2016 VL 93 IS 7 AR 075032 DI 10.1103/PhysRevD.93.075032 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DK5JV UT WOS:000374957100003 ER PT J AU Tolstykh, EI Degteva, MO Bougrov, NG Napier, BA AF Tolstykh, Evgenia I. Degteva, Marina O. Bougrov, Nikolay G. Napier, Bruce A. TI Body Potassium Content and Radiation Dose from K-40 for the Urals Population (Russia) SO PLOS ONE LA English DT Article ID SKELETAL-MUSCLE MASS; AGE; SARCOPENIA; ETHNICITY; CHILDREN; SPAN; LIFE AB Long-term whole-body monitoring of radionuclides in residents of the Urals Region has been performed at the Urals Research Center for Radiation Medicine (URCRM, Chelyabinsk). Quantification of K-40 was achieved by measuring the K-40 photopeak with four phoswich detectors in whole body counter SICH-9.1M. The current study presents the results of K-40 measurements in 3,651 women and 1,961 t-test; U-test men aged 11-90; measurements were performed in 2006-2014. The residents belonged to two ethnic groups, Turkic (Tatar, Bashkir) and Slavs (mainly Russian). The levels of K-40-body contents depend upon gender, age, and body mass. Significant ethnic-differences were not found in K-40-body contents and K-40 concentrations in terms of Bq per kg of body weight (in groups homogenous by age and gender). Both K-40-body contents and concentrations were significantly higher in men than in women in all age-groups; the difference was about 25%. The measured K-40-body content in men of 20-50 years was about 4200 Bq (134 g of K) and about 3000 Bq (95 g of K) in women. By the age of 80 these values decreased to 3200 Bq (102 g of K) in men and 2500 Bq (80 g of K) in women. Annual dose rates were maximal in the age group of 20-30 years-0.16 mGy/y for men and 0.13 mGy/y for women. Further, the dose-rates decreased with age and in the groups of 60-80 years were 0.13 mGy/y for men and 0.10 mGy/y for women. Within groups homogeneous by age and gender, individual dose rates are described by a normal statistical distribution. The coefficient of variation ranges from 9 to 14%, and on the average is 12.5%. Doses from naturally occurring K-40 accumulated over 70 years were found to be 9.9 mGy for men and 8.3 mGy for women; over 90 years - 12.5 and 10.4 mGy. C1 [Tolstykh, Evgenia I.; Degteva, Marina O.; Bougrov, Nikolay G.] Urals Res Ctr Radiat Med, Biophys Lab, Chelyabinsk, Russia. [Napier, Bruce A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Tolstykh, EI (reprint author), Urals Res Ctr Radiat Med, Biophys Lab, Chelyabinsk, Russia. EM evgnia@urcrm.ru FU U.S. Department of Energy's, Office of International Health Programs; Federal Medical-Biological Agency [27.504.14.9] FX The research was funded by the U.S. Department of Energy's, Office of International Health Programs (http://www.energy.gov/ehss/russian-health-studies-program-active-projec ts, Barret N. Fountos, Program Manager, to BN, MO); and by Federal Medical-Biological Agency (contract 27.504.14.9 http://fcp.economy.gov.ru/cgi-bin/cis/fcp.cgi/Fcp/ViewFcp/View/2012/368/ , to ET, NB). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 27 TC 0 Z9 0 U1 0 U2 2 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 25 PY 2016 VL 11 IS 4 AR e0154266 DI 10.1371/journal.pone.0154266 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK5OX UT WOS:000374970600054 PM 27111330 ER PT J AU Valdes-Lopez, O Batek, J Gomez-Hernandez, N Nguyen, CT Isidra-Arellano, MC Zhang, N Joshi, T Xu, D Hixson, KK Weitz, KK Aldrich, JT Pasa-Tolic, L Stacey, G AF Valdes-Lopez, Oswaldo Batek, Josef Gomez-Hernandez, Nicolas Nguyen, Cuong T. Isidra-Arellano, Mariel C. Zhang, Ning Joshi, Trupti Xu, Dong Hixson, Kim K. Weitz, Karl K. Aldrich, Joshua T. Pasa-Tolic, Ljiljana Stacey, Gary TI Soybean Roots Grown under Heat Stress Show Global Changes in Their Transcriptional and Proteomic Profiles SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE soybean; root hairs; heat stress; gene module; transcriptomics; proteomics ID TANDEM MASS-SPECTRA; MOLECULAR-MECHANISMS; ARABIDOPSIS-THALIANA; EXPRESSION ANALYSIS; ABIOTIC STRESS; CLIMATE-CHANGE; RNA-SEQ; RESPONSES; PLANTS; THERMOTOLERANCE AB Heat stress is likely to be a key factor in the negative impact of climate change on crop production. Heat stress significantly influences the functions of roots, which provide support, water, and nutrients to other plant organs. Likewise, roots play an important role in the establishment of symbiotic associations with different microorganisms. Despite the physiological relevance of roots, few studies have examined their response to heat stress. In this study, we performed genome-wide transcriptomic and proteomic analyses on isolated root hairs, which are a single, epidermal cell type, and compared their response to stripped roots. On average, we identified 1849 and 3091 genes differentially regulated in root hairs and stripped roots, respectively, in response to heat stress. Our gene regulatory module analysis identified 10 key modules that might control the majority of the transcriptional response to heat stress. We also conducted proteomic analysis on membrane fractions isolated from root hairs and compared these responses to stripped roots. These experiments identified a variety of proteins whose expression changed within 3 h of application of heat stress. Most of these proteins were predicted to play a significant role in thermo-tolerance, as well as in chromatin remodeling and post-transcriptional regulation. The data presented represent an in-depth analysis of the heat stress response of a single cell type in soybean. C1 [Valdes-Lopez, Oswaldo; Batek, Josef; Gomez-Hernandez, Nicolas; Nguyen, Cuong T.; Stacey, Gary] Univ Missouri, CS Bond Life Sci Ctr, Natl Ctr Soybean Biotechnol, Div Pant Sci & Biochem, Columbia, MO USA. [Valdes-Lopez, Oswaldo; Isidra-Arellano, Mariel C.] Univ Nacl Autonoma Mexico, FES Iztacala, Lab Genom Func Leguminosas, Mexico City 04510, DF, Mexico. [Zhang, Ning; Joshi, Trupti; Xu, Dong] Univ Missouri, Inst Informat, CS Bond Life Sci Ctr, Columbia, MO USA. [Joshi, Trupti; Xu, Dong] Univ Missouri, Dept Comp Sci, Columbia, MO USA. [Joshi, Trupti] Univ Missouri, Sch Med, Dept Mol Microbiol & Immunol, Columbia, MO 65212 USA. [Joshi, Trupti] Univ Missouri, Sch Med, Res Off, Columbia, MO USA. [Hixson, Kim K.; Weitz, Karl K.; Aldrich, Joshua T.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Stacey, G (reprint author), Univ Missouri, CS Bond Life Sci Ctr, Natl Ctr Soybean Biotechnol, Div Pant Sci & Biochem, Columbia, MO USA. EM staceyg@missouri.edu FU Biological and Environmental Research Division, Department of Energy, Office of Science [DE-SC0004898]; United Soybean Board; U.S. Department of Energy [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research; CONACyT [219759, 252260]; PAPIIT-UNAIVI [IA203815]; PAPCA-FES Iztacala [FESI-DIP-PAPCA-2014-3] FX Research was funded by a grant from the Biological and Environmental Research Division, Department of Energy, Office of Science (Grant DE-SC0004898 to GS, DX, LP), as well as funding to GS from the United Soybean Board. A portion of this research was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi-program national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The work was performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. OVL research is founded by a CONACyT (CONACyT# 219759 and 252260), PAPIIT-UNAIVI (PAPIIT# IA203815), and PAPCA-FES Iztacala (FESI-DIP-PAPCA-2014-3) grant. NR 53 TC 1 Z9 1 U1 5 U2 22 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD APR 25 PY 2016 VL 7 AR 517 DI 10.3389/fpls.2016.00517 PG 12 WC Plant Sciences SC Plant Sciences GA DK0UO UT WOS:000374627900001 PM 27200004 ER PT J AU Velaga, SC Levine, JS Warzinski, RP Anderson, BJ AF Velaga, Srinath C. Levine, Jonathan S. Warzinski, Robert P. Anderson, Brian J. TI A thermodynamic model to predict the aqueous solubility of hydrocarbon mixtures at two-phase hydrate-liquid water equilibrium SO FLUID PHASE EQUILIBRIA LA English DT Article DE Gas hydrates; Aqueous solubility of hydrocarbon mixtures; Hydrate cage occupancy; Hydrate-liquid water two-phase thermodynamic equilibrium; Deep sea hydrates ID AB-INITIO METHODS; PHASE-EQUILIBRIA; GAS HYDRATE; METHANE HYDRATE; CARBON-DIOXIDE; ACTIVITY-COEFFICIENTS; POTENTIAL-ENERGY; OIL-SPILL; SYSTEM; PROPANE AB Understanding the fate and transport of hydrocarbons and hydrocarbon mixtures in the deep sea and underlying sediments requires accurate determination of the two-phase hydrate (H)-liquid water (L-W) thermodynamic equilibrium in the absence of a free gas phase. In addition to controlling hydrate formation directly from the aqueous phase, the H-L-w equilibrium provides the aqueous solubility of dissolving hydrate. The aqueous solubility of hydrocarbon mixture at H-L-w equilibrium was calculated based on the van der Waals and Platteeuw statistical thermodynamic model and the Holder model. Langmuir constants were calculated from cell potential parameters obtained from ab initio intermolecular potentials and thus the model contains no fitting parameters. The model accurately predicts pure methane, ethane, and propane experimental H-L-w equilibrium solubility data, including new data provided here for methane. We present hydrocarbon solubilities in water and seawater at H-L-w equilibrium at deep sea conditions for both methane and a thermogenic mixture based on the methane-ethane-propane ratio from the 2010 Macondo oil spill. We also present model predictions of the proportion of occupied large and small cages at H-L-w equilibrium for both systems, as well as hydrocarbon ratios in the hydrate phase for the thermogenic mixture. (C) 2015 Elsevier B.V. All rights reserved. C1 [Velaga, Srinath C.; Anderson, Brian J.] W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. [Velaga, Srinath C.; Levine, Jonathan S.; Warzinski, Robert P.; Anderson, Brian J.] Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. RP Anderson, BJ (reprint author), W Virginia Univ, Dept Chem Engn, Morgantown, WV 26506 USA. EM SVelaga@mix.wvu.edu; Jonathan.Levine@netl.doe.gov; Robert.Warzinski@netl.doe.gov; Brian.Anderson@mail.wvu.edu FU Department of Energy Complementary Research Program of Energy policy Act [999]; Department of Interior, Bureau of Safety and Environmental Enforcement [M11PG00053]; Oak Ridge Institute for Science and Education Postgraduate Research Program at NETL FX This work was supported by the Department of Energy Complementary Research Program under Section 999 of the Energy policy Act of 2005 and by the Department of Interior, Bureau of Safety and Environmental Enforcement under Interagency Agreement M11PG00053. Support for Jonathan Levine came through the Oak Ridge Institute for Science and Education Postgraduate Research Program at NETL. The authors would like to thank Jason Guinan and the NETL Multimedia team for assistance with the figures. NR 64 TC 0 Z9 0 U1 5 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-3812 EI 1879-0224 J9 FLUID PHASE EQUILIBR JI Fluid Phase Equilib. PD APR 25 PY 2016 VL 414 BP 75 EP 87 DI 10.1016/j.fluid.2015.12.049 PG 13 WC Thermodynamics; Chemistry, Physical; Engineering, Chemical SC Thermodynamics; Chemistry; Engineering GA DH3KP UT WOS:000372686200009 ER PT J AU Thieberger, P Altinbas, Z Carlson, C Chasman, C Costanzo, M Degen, C Drees, KA Fischer, W Gassner, D Gu, X Hamdi, K Hock, J Marusic, A Miller, T Minty, M Montag, C Luo, Y Pikin, AI White, SM AF Thieberger, P. Altinbas, Z. Carlson, C. Chasman, C. Costanzo, M. Degen, C. Drees, K. A. Fischer, W. Gassner, D. Gu, X. Hamdi, K. Hock, J. Marusic, A. Miller, T. Minty, M. Montag, C. Luo, Y. Pikin, A. I. White, S. M. TI High energy Coulomb-scattered electrons for relativistic particle beam diagnostics SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID PROBE AB A new system used for monitoring energetic Coulomb-scattered electrons as the main diagnostic for accurately aligning the electron and ion beams in the new Relativistic Heavy Ion Collider (RHIC) electron lenses is described in detail. The theory of electron scattering from relativistic ions is developed and applied to the design and implementation of the system used to achieve and maintain the alignment. Commissioning with gold and He-3 beams is then described as well as the successful utilization of the new system during the 2015 RHIC polarized proton run. Systematic errors of the new method are then estimated. Finally, some possible future applications of Coulomb-scattered electrons for beam diagnostics are briefly discussed. C1 [Thieberger, P.; Altinbas, Z.; Carlson, C.; Chasman, C.; Costanzo, M.; Degen, C.; Drees, K. A.; Fischer, W.; Gassner, D.; Gu, X.; Hamdi, K.; Hock, J.; Marusic, A.; Miller, T.; Minty, M.; Montag, C.; Luo, Y.; Pikin, A. I.] Brookhaven Natl Lab, Upton, NY 11973 USA. [White, S. M.] European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. RP Thieberger, P (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM PT@BNL.GOV FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. Department of Energy FX We are grateful to the RHIC operations crew for their expert assistance in the development, testing and implementation of this new system. We would like to thank the referees for many valuable suggestions. In particular, the idea of modulating the electron beam, described in Sec. VII A, could lead to an important sensitivity improvement and the possibility mentioned in Sec. VI of displacing both beams simultaneously to better evaluate a systematic error may be implemented in the future. This work was supported by Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 41 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD APR 22 PY 2016 VL 19 IS 4 AR 041002 DI 10.1103/PhysRevAccelBeams.19.041002 PG 13 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6XK UT WOS:000379349400001 ER PT J AU van Deurzen, H Frederix, R Hirschi, V Luisoni, G Mastrolia, P Ossola, G AF van Deurzen, Hans Frederix, Rikkert Hirschi, Valentin Luisoni, Gionata Mastrolia, Pierpaolo Ossola, Giovanni TI Spin polarisation of t(t)over-bar gamma gamma production at NLO plus PS with GOSAM interfaced to MADGRAPH5_AMC@NLO SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID QUARK PAIR PRODUCTION; ONE-LOOP CALCULATIONS; QCD CORRECTIONS; HELICITY AMPLITUDES; FEYNMAN DIAGRAMS; CHARGE ASYMMETRY; PERTURBATIVE QCD; ISOLATED PHOTONS; ROOT-S=7 TEV; 2 JETS AB We present an interface between the multipurpose Monte Carlo tool MadGraph5_aMC@NLO and the automated amplitude generator GOSAM. As a first application of this novel framework, we compute the NLO corrections to pp -> t (t) over barH and pp -> t (t) over bar gamma gamma matched to a parton shower. In the phenomenological analyses of these processes, we focus our attention on observables which are sensitive to the polarisation of the top quarks. C1 [van Deurzen, Hans; Luisoni, Gionata; Mastrolia, Pierpaolo] Max Planck Inst Phys & Astrophys, Fohringer Ring 6, D-80805 Munich, Germany. [Frederix, Rikkert] Tech Univ Munich, Phys Dept T31, James Franck Str 1, D-85748 Garching, Germany. [Hirschi, Valentin] Natl Accelerator Lab, SLAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Mastrolia, Pierpaolo] Univ Padua, Dipartimento Fis & Astron, Via Marzolo 8, I-35131 Padua, Italy. [Mastrolia, Pierpaolo] Ist Nazl Fis Nucl, Sez Padova, Via Marzolo 8, I-35131 Padua, Italy. [Ossola, Giovanni] CUNY, New York City Coll Technol, 300 Jay St, Brooklyn, NY 11201 USA. [Ossola, Giovanni] CUNY, Grad Sch, 365 Fifth Ave, New York, NY 10016 USA. [Ossola, Giovanni] CUNY, Univ Ctr, 365 Fifth Ave, New York, NY 10016 USA. RP van Deurzen, H; Luisoni, G; Mastrolia, P (reprint author), Max Planck Inst Phys & Astrophys, Fohringer Ring 6, D-80805 Munich, Germany.; Frederix, R (reprint author), Tech Univ Munich, Phys Dept T31, James Franck Str 1, D-85748 Garching, Germany.; Hirschi, V (reprint author), Natl Accelerator Lab, SLAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Mastrolia, P (reprint author), Univ Padua, Dipartimento Fis & Astron, Via Marzolo 8, I-35131 Padua, Italy.; Mastrolia, P (reprint author), Ist Nazl Fis Nucl, Sez Padova, Via Marzolo 8, I-35131 Padua, Italy.; Ossola, G (reprint author), CUNY, New York City Coll Technol, 300 Jay St, Brooklyn, NY 11201 USA.; Ossola, G (reprint author), CUNY, Grad Sch, 365 Fifth Ave, New York, NY 10016 USA.; Ossola, G (reprint author), CUNY, Univ Ctr, 365 Fifth Ave, New York, NY 10016 USA. EM hdeurzen@mpp.mpg.de; rikkert.frederix@tum.de; vahirsch@slac.stanford.edu; luisonig@mpp.mpg.de; pierpaolo.mastrolia@cern.ch; gossola@citytech.cuny.edu FU Alexander von Humboldt Foundation; NSF [PHY-1068550, PHY-1417354]; Swiss National Fund for Science (SNSF) [P300P2_161050] FX We thank German Rodrigo and Jan Winter for valuable discussions. The work of H.v.D., R.F., G.L. and P.M. is supported by the Alexander von Humboldt Foundation, in the framework of the Sofja Kovaleskaja Award Projects "Advanced Mathematical Methods for Particle Physics" (H.v.D., G.L. and P.M.) and "Event Simulation for the Large Hadron Collider at High Precision" (R.F.), endowed by the German Federal Ministry of Education and Research. The work of G.O. is supported in part by the NSF under Grants PHY-1068550 and PHY-1417354. V.H. is supported by the Swiss National Fund for Science (SNSF) under grant number P300P2_161050. This research made use of the CTP computational cluster of the New York City College of Technology. We thank the CP3 IT team for their constant support and the availability of the cluster hosted by the Universite Catholique de Louvain. NR 111 TC 0 Z9 0 U1 4 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 22 PY 2016 VL 76 IS 4 AR 221 DI 10.1140/epjc/s10052-016-4048-2 PG 17 WC Physics, Particles & Fields SC Physics GA DK0AK UT WOS:000374574500001 ER PT J AU Freysoldt, C Lange, B Neugebauer, J Yan, QM Lyons, JL Janotti, A Van de Walle, CG AF Freysoldt, Christoph Lange, Bjoern Neugebauer, Joerg Yan, Qimin Lyons, John L. Janotti, Anderson Van de Walle, Chris G. TI Electron and chemical reservoir corrections for point-defect formation energies SO PHYSICAL REVIEW B LA English DT Article ID AB-INITIO CALCULATIONS; AUGMENTED-WAVE METHOD; GALLIUM NITRIDE; 1ST-PRINCIPLES CALCULATIONS; SEMICONDUCTORS; IMPURITIES; GAN AB Point-defect formation energies calculated within the framework of density functional theory often depend on the choice of the exchange and correlation (xc) functional. We show that variations between the local density approximation (LDA), generalized gradient approximation (GGA), and hybrid functionals mainly arise from differences in the position of the bulk valence-band maximum, as well as in the reference energies for the chemical potential obtained with distinct xc functionals. We demonstrate for point defects relevant for p-type GaN that these differences can be accounted for by corrections, reducing the maximum disagreement between the different functionals from more than 2 eV to below 0.2 eV. Our correction scheme should be useful for performing high-throughput calculations in cases where full hybrid functional calculations are prohibitively expensive. C1 [Freysoldt, Christoph; Lange, Bjoern; Neugebauer, Joerg] Max Planck Inst Eisenforsch GmbH, Max Planck Str 1, D-40237 Dusseldorf, Germany. [Yan, Qimin; Lyons, John L.; Janotti, Anderson; Van de Walle, Chris G.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Lange, Bjoern] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. [Yan, Qimin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Lyons, John L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Janotti, Anderson] Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA. RP Freysoldt, C (reprint author), Max Planck Inst Eisenforsch GmbH, Max Planck Str 1, D-40237 Dusseldorf, Germany. FU Bundesministerium fur Bildung und Forschung [03X0512G]; UCSB Solid State Lighting and Energy Center; National Science Foundation (NSF) [DMR-1434854]; Center for Low Energy Systems Technology (LEAST), SRC STARnet Centers; MARCO; DARPA; NSF [ACI-1053575] FX This work was supported by the Bundesministerium fur Bildung und Forschung (03X0512G, VEKTRA), by the UCSB Solid State Lighting and Energy Center, by the National Science Foundation (NSF) (DMR-1434854), and by the Center for Low Energy Systems Technology (LEAST), one of the six SRC STARnet Centers, sponsored by MARCO and DARPA. Computational resources were provided by the Center for Scientific Computing at the CNSI and MRL (an NSF MRSEC, DMR-1121053) (NSF CNS-0960316) and by the Extreme Science and Engineering Discovery Environment (XSEDE), supported by NSF (ACI-1053575). NR 49 TC 3 Z9 3 U1 13 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 22 PY 2016 VL 93 IS 16 AR 165206 DI 10.1103/PhysRevB.93.165206 PG 9 WC Physics, Condensed Matter SC Physics GA DJ9MV UT WOS:000374538500006 ER PT J AU Wang, Y Linscheid, A Berlijn, T Johnston, S AF Wang, Y. Linscheid, A. Berlijn, T. Johnston, S. TI Ab initio study of cross-interface electron-phonon couplings in FeSe thin films on SrTiO3 and BaTiO3 SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; SINGLE-LAYER FESE; FUNCTIONAL PERTURBATION-THEORY; NONADIABATIC SUPERCONDUCTIVITY; VERTEX CORRECTIONS; ORIGIN; MODE AB We study the electron-phonon coupling strength near the interface of monolayer and bilayer FeSe thin films on SrTiO3, BaTiO3, and oxygen-vacant SrTiO3 substrates, using ab initio methods. The calculated total electron-phonon coupling strength lambda = 0.2-0.3 cannot account for the high T-c similar to 70 K observed in these systems through the conventional phonon-mediated pairing mechanism. In all of these systems, however, we find that the coupling constant of a polar oxygen branch peaks at q = 0 with negligible coupling elsewhere, while the energy of this mode coincides with the offset energy of the replica bands measured recently by angle-resolved photoemission spectroscopy experiments. But the integrated coupling strength for this mode from our current calculations is still too small to produce the observed high T-c, even through the more efficient pairing mechanism provided by the forward scattering. We arrive at the same qualitative conclusion when considering a checkerboard antiferromagnetic configuration in the Fe layer. In light of the experimental observations of the replica band feature and the relatively high T-c of FeSe monolayers on polar substrates, our results point towards a cooperative role for the electron-phonon interaction, where the cross-interface interaction acts in conjunction with a purely electronic interaction. We also discuss a few scenarios where the coupling strength obtained here may be enhanced. C1 [Wang, Y.; Johnston, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Linscheid, A.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Berlijn, T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Berlijn, T.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Wang, Y (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RI Johnston, Steven/J-7777-2016 FU University of Tennessee's Science Alliance Joint Directed Research and Development (JDRD) program; University of Tennessee's Office of Research and Engagement's Organized Research Unit program; Oak Ridge National Laboratory; [DE-FG02-05ER46236] FX We thank A. Kemper for useful discussions. S.J. and Y.W. are partially funded by the University of Tennessee's Science Alliance Joint Directed Research and Development (JDRD) program, a collaboration with Oak Ridge National Laboratory. S.J. acknowledges additional support from the University of Tennessee's Office of Research and Engagement's Organized Research Unit program. A.L. was supported by Grant No. DE-FG02-05ER46236. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is a Department of Energy (DOE) Office of Science User Facility. This research used computational resources supported by the University of Tennessee and Oak Ridge National Laboratory's Joint Institute for Computational Sciences and resources of the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility. NR 59 TC 5 Z9 5 U1 13 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 22 PY 2016 VL 93 IS 13 AR 134513 DI 10.1103/PhysRevB.93.134513 PG 9 WC Physics, Condensed Matter SC Physics GA DJ9JK UT WOS:000374529600004 ER PT J AU Wysocki, AL Birol, T AF Wysocki, Aleksander L. Birol, Turan TI Magnetically induced phonon splitting in ACr(2)O(4) spinels from first principles SO PHYSICAL REVIEW B LA English DT Article ID INSULATORS; ELECTRONS; ORDER AB We study the magnetically-induced phonon splitting in cubic ACr(2)O(4) (A = Mg, Zn, Cd) spinels from first principles and demonstrate that the sign of the splitting, which is experimentally observed to be opposite in CdCr2O4 compared to ZnCr2O4 and MgCr2O4, is determined solely by the particular magnetic ordering pattern observed in these compounds. We further show that this interaction between magnetism and phonon frequencies can be fully described by the previously proposed spin-phonon coupling model [C. J. Fennie and K. M. Rabe, Phys. Rev. Lett. 96, 205505 (2006)] that includes only the nearest neighbor exchange. Using this model with materials specific parameters calculated from first principles, we provide additional insights into the physics of spin-phonon coupling in this intriguing family of compounds. C1 [Wysocki, Aleksander L.] US DOE, Ames Lab, Ames, IA 50011 USA. [Birol, Turan] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. RP Wysocki, AL (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. RI Birol, Turan/D-1948-2012 OI Birol, Turan/0000-0001-5174-3320 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358]; Rutgers Center for Materials Theory FX We acknowledge fruitful discussions with Craig J. Fennie and Karin Rabe. Work at Ames Lab was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. T.B. was supported by the Rutgers Center for Materials Theory. NR 35 TC 0 Z9 0 U1 3 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 22 PY 2016 VL 93 IS 13 AR 134425 DI 10.1103/PhysRevB.93.134425 PG 6 WC Physics, Condensed Matter SC Physics GA DJ9JK UT WOS:000374529600003 ER PT J AU Alshudifat, MF Grzywacz, R Madurga, M Gross, CJ Rykaczewski, KP Batchelder, JC Bingham, C Borzov, IN Brewer, NT Cartegni, L Fijalkowska, A Hamilton, JH Hwang, JK Ilyushkin, SV Jost, C Karny, M Korgul, A Krolas, W Liu, SH Mazzocchi, C Mendez, AJ Miernik, K Miller, D Padgett, SW Paulauskas, SV Ramayya, AV Stracener, DW Surman, R Winger, JA Wolinska-Cichocka, M Zganjar, EF AF Alshudifat, M. F. Grzywacz, R. Madurga, M. Gross, C. J. Rykaczewski, K. P. Batchelder, J. C. Bingham, C. Borzov, I. N. Brewer, N. T. Cartegni, L. Fijalkowska, A. Hamilton, J. H. Hwang, J. K. Ilyushkin, S. V. Jost, C. Karny, M. Korgul, A. Krolas, W. Liu, S. H. Mazzocchi, C. Mendez, A. J., II Miernik, K. Miller, D. Padgett, S. W. Paulauskas, S. V. Ramayya, A. V. Stracener, D. W. Surman, R. Winger, J. A. Wolinska-Cichocka, M. Zganjar, E. F. TI Reexamining Gamow-Teller decays near Ni-78 SO PHYSICAL REVIEW C LA English DT Article AB Decays of neutron-rich nuclei Zn-82,Zn-83 and Ga-82,Ga-83 produced in proton-induced fission of U-238 were studied at the Holifield Radioactive Ion Beam Facility using on-line mass separation and beta-gamma spectroscopy techniques. New gamma-ray transitions were identified and level schemes, which include states at high excitation energies in the range between 3-7 MeV were constructed. These high-energy levels were identified to be populated through allowed Gamow-Teller beta transitions, and their structure was interpreted with new shell-model calculations. A beta-delayed neutron branching ratio of 69 +/- 7% was deduced for Zn-82 and revised beta-decay half-life values of Zn-82 [155(17)(20) ms] and Zn-83 [122(28) ms] were determined. C1 [Alshudifat, M. F.] AL al Bayt Univ, Dept Phys, Mafraq 25113, Jordan. [Alshudifat, M. F.; Grzywacz, R.; Madurga, M.; Bingham, C.; Cartegni, L.; Fijalkowska, A.; Jost, C.; Miller, D.; Padgett, S. W.; Paulauskas, S. V.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Grzywacz, R.; Gross, C. J.; Rykaczewski, K. P.; Mendez, A. J., II; Miernik, K.; Stracener, D. W.; Wolinska-Cichocka, M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37830 USA. [Grzywacz, R.; Bingham, C.] Joint Inst Nucl Phys & Applicat, Oak Ridge, TN 37831 USA. [Batchelder, J. C.; Karny, M.; Liu, S. H.; Wolinska-Cichocka, M.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Bingham, C.; Korgul, A.; Krolas, W.; Mazzocchi, C.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Borzov, I. N.] Joint Inst Nucl Res, Dubna 141980, Russia. [Brewer, N. T.; Hamilton, J. H.; Hwang, J. K.; Ramayya, A. V.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Fijalkowska, A.; Karny, M.; Korgul, A.; Mazzocchi, C.; Miernik, K.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Ilyushkin, S. V.; Winger, J. A.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Krolas, W.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Surman, R.] Union Coll, Dept Phys, Schenectady, NY 12308 USA. [Wolinska-Cichocka, M.] Univ Warsaw, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Zganjar, E. F.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. RP Alshudifat, MF (reprint author), AL al Bayt Univ, Dept Phys, Mafraq 25113, Jordan.; Alshudifat, MF (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM mohmd7shudif@gmail.com FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics; US DOE [DE-AC05-00OR22725, DE-FG02-96ER40983, DE-AC05-06OR23100, DE-FG05-88ER40407]; National Nuclear Security Administration [DEFC03-03NA00143]; Stewardship Science Academic Alliance program through DOE [DE-FG52-08NA28552]; National Science Centre of the Polish Ministry of Science and Higher Education [2011/01/B/ST2/02476]; U.S. Department of Energy [DE-AC05-00OR22725] FX We wish to acknowledge the Holifield Radioactive Ion Beam Facility (HRIBF) staff for their assistance with the experiments and providing excellent quality neutron-rich radioactive beams. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics and this research used resources of the Holifield Radioactive Ion Beam Facility of Oak Ridge National Laboratory, which was a DOE Office of Science User Facility. This is supported in part by US DOE grants DE-AC05-00OR22725 (ORNL), DE-FG02-96ER40983 (UTK), DE-AC05-06OR23100 (ORAU), and DE-FG05-88ER40407 (Vanderbilt); in part by the National Nuclear Security Administration Grant No. DEFC03-03NA00143 and under the Stewardship Science Academic Alliance program through DOE Cooperative Agreement No. DE-FG52-08NA28552 (UTK); in part by the National Science Centre of the Polish Ministry of Science and Higher Education, Grant No. 2011/01/B/ST2/02476. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 41 TC 6 Z9 6 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 22 PY 2016 VL 93 IS 4 AR 044325 DI 10.1103/PhysRevC.93.044325 PG 14 WC Physics, Nuclear SC Physics GA DJ9PX UT WOS:000374546500002 ER PT J AU Jha, PK Mrejen, M Kim, J Wu, CH Wang, Y Rostovtsev, YV Zhang, X AF Jha, Pankaj K. Mrejen, Michael Kim, Jeongmin Wu, Chihhui Wang, Yuan Rostovtsev, Yuri V. Zhang, Xiang TI Coherence-Driven Topological Transition in Quantum Metamaterials SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTROMAGNETICALLY INDUCED TRANSPARENCY; HYPERBOLIC METAMATERIALS; NEGATIVE REFRACTION; OPTICAL HYPERLENS; LATTICES; ATOMS; WAVE AB We introduce and theoretically demonstrate a quantum metamaterial made of dense ultracold neutral atoms loaded into an inherently defect-free artificial crystal of light, immune to well-known critical challenges inevitable in conventional solid-state platforms. We demonstrate an all-optical control, on ultrafast time scales, over the photonic topological transition of the isofrequency contour from an open to closed topology at the same frequency. This atomic lattice quantum metamaterial enables a dynamic manipulation of the decay rate branching ratio of a probe quantum emitter by more than an order of magnitude. Our proposal may lead to practically lossless, tunable, and topologically reconfigurable quantum metamaterials, for single or few-photon-level applications as varied as quantum sensing, quantum information processing, and quantum simulations using metamaterials. C1 [Jha, Pankaj K.; Mrejen, Michael; Kim, Jeongmin; Wu, Chihhui; Wang, Yuan; Zhang, Xiang] Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, 3112 Etcheverry Hall, Berkeley, CA 94720 USA. [Rostovtsev, Yuri V.] Univ N Texas, Ctr Nonlinear Sci, Denton, TX 76203 USA. [Rostovtsev, Yuri V.] Univ N Texas, Dept Phys, Denton, TX 76203 USA. [Zhang, Xiang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Zhang, Xiang] King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. RP Zhang, X (reprint author), Univ Calif Berkeley, NSF Nanoscale Sci & Engn Ctr NSEC, 3112 Etcheverry Hall, Berkeley, CA 94720 USA.; Zhang, X (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Zhang, X (reprint author), King Abdulaziz Univ, Dept Phys, Jeddah 21589, Saudi Arabia. EM xiang@berkeley.edu RI Wang, Yuan/F-7211-2011 FU Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research (AFOSR MURI) [FA9550-12-1-0488]; Gordon and Betty Moore Foundation FX The authors acknowledge funding support from the Multidisciplinary University Research Initiative from the Air Force Office of Scientific Research (AFOSR MURI Award No. FA9550-12-1-0488) and the Gordon and Betty Moore Foundation. NR 56 TC 5 Z9 5 U1 21 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 22 PY 2016 VL 116 IS 16 AR 165502 DI 10.1103/PhysRevLett.116.165502 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ9VE UT WOS:000374560300008 PM 27152810 ER PT J AU Kolesnikov, AI Reiter, GF Choudhury, N Prisk, TR Mamontov, E Podlesnyak, A Ehlers, G Seel, AG Wesolowski, DJ Anovitz, LM AF Kolesnikov, Alexander I. Reiter, George F. Choudhury, Narayani Prisk, Timothy R. Mamontov, Eugene Podlesnyak, Andrey Ehlers, George Seel, Andrew G. Wesolowski, David J. Anovitz, Lawrence M. TI Quantum Tunneling of Water in Beryl: A New State of the Water Molecule SO PHYSICAL REVIEW LETTERS LA English DT Article ID INELASTIC NEUTRON-SCATTERING; ALKALI-POOR BERYL; DYNAMICS; ICE; VISUALIZATION; AL4BE6SI12O36; SPECTROSCOPY; INSIGHTS; LATTICE; POINT AB Using neutron scattering and ab initio simulations, we document the discovery of a new "quantum tunneling state" of the water molecule confined in 5 angstrom channels in the mineral beryl, characterized by extended proton and electron delocalization. We observed a number of peaks in the inelastic neutron scattering spectra that were uniquely assigned to water quantum tunneling. In addition, the water proton momentum distribution was measured with deep inelastic neutron scattering, which directly revealed coherent delocalization of the protons in the ground state. C1 [Kolesnikov, Alexander I.; Mamontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Reiter, George F.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Choudhury, Narayani] Lake Washington Inst Technol, Div Math & Sci, Kirkland, WA 98034 USA. [Choudhury, Narayani] Univ Washington, Sch Sci Technol Engn & Math, Bothell, WA 98011 USA. [Prisk, Timothy R.; Wesolowski, David J.; Anovitz, Lawrence M.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Podlesnyak, Andrey; Ehlers, George] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Seel, Andrew G.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Seel, Andrew G.] Univ Oxford, Dept Inorgan Chem, S Parks Rd, Oxford OX1 3QR, England. RP Kolesnikov, AI (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM kolesnikovai@ornl.gov RI Mamontov, Eugene/Q-1003-2015; Podlesnyak, Andrey/A-5593-2013; Anovitz, Lawrence/P-3144-2016; Ehlers, Georg/B-5412-2008; OI Mamontov, Eugene/0000-0002-5684-2675; Podlesnyak, Andrey/0000-0001-9366-6319; Anovitz, Lawrence/0000-0002-2609-8750; Ehlers, Georg/0000-0003-3513-508X; Prisk, Timothy/0000-0002-7943-5175 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; University of Washington (DOE/UW) [4000127504, 6400012674, 66-1283]; U.S. Department of Energy [DE-AC05-00OR22725] FX This material is primarily based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. The neutron scattering experiments at Oak Ridge National Laboratory's Spallation Neutron Source were sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The STFC Rutherford Appleton Laboratory is thanked for access to neutron beam facilities. Some of the beryl crystals used in our experiments were cut by Bradley S. Wilson of Coast-to-Coast Rarestones, International. N. C. also gratefully acknowledges research support from the University of Washington (DOE/UW Grants No. 4000127504, No. 6400012674; No. 66-1283).; This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. NR 52 TC 9 Z9 9 U1 15 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 22 PY 2016 VL 116 IS 16 AR 167802 DI 10.1103/PhysRevLett.116.167802 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ9VE UT WOS:000374560300012 PM 27152824 ER PT J AU Kim, YJ Savukov, I AF Kim, Young Jin Savukov, Igor TI Ultra-sensitive Magnetic Microscopy with an Optically Pumped Magnetometer SO SCIENTIFIC REPORTS LA English DT Article ID ATOMIC MAGNETOMETER; SENSORS; TISSUE AB Optically pumped magnetometers (OPMs) based on lasers and alkali-metal vapor cells are currently the most sensitive non-cryogenic magnetic field sensors. Many applications in neuroscience and other fields require high-resolution, high-sensitivity magnetic microscopic measurements. In order to meet this demand we combined a cm-size spin-exchange relaxation-free (SERF) OPM and flux guides (FGs) to realize an ultra-sensitive FG-OPM magnetic microscope. The FGs serve to transmit the target magnetic flux to the OPM thus improving both the resolution and sensitivity to small magnetic objects. We investigated the performance of the FG-OPM device using experimental and numerical methods, and demonstrated that an optimized device can achieve a unique combination of high resolution (80 mu m) and high sensitivity (8.1pT/root Hz). In addition, we also performed numerical calculations of the magnetic field distribution in the FGs to estimate the magnetic noise originating from the domain fluctuations in the material of the FGs. We anticipate many applications of the FG-OPM device such as the detection of micro-biological magnetic fields; the detection of magnetic nano-particles; and non-destructive testing. From our theoretical estimate, an FG-OPM could detect the magnetic field of a single neuron, which would be an important milestone in neuroscience. C1 [Kim, Young Jin; Savukov, Igor] Univ Calif Los Alamos Natl Lab, P-21,POB 1663,MS D454, Los Alamos, NM 87545 USA. RP Kim, YJ (reprint author), Univ Calif Los Alamos Natl Lab, P-21,POB 1663,MS D454, Los Alamos, NM 87545 USA. EM youngjin@lanl.gov OI Savukov, Igor/0000-0003-4190-5335 FU U.S. DOE through the LANL/LDRD program FX We acknowledge this work was supported by the U.S. DOE through the LANL/LDRD program. The authors thank Michelle Espy, John George, and Michael Malone for very helpful discussions. NR 19 TC 4 Z9 4 U1 9 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 22 PY 2016 VL 6 AR 24773 DI 10.1038/srep24773 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DK0FK UT WOS:000374587800001 PM 27103463 ER PT J AU Youngblut, MD Tsai, CL Clark, IC Carlson, HK Maglaqui, AP Gau-Pan, PS Redford, SA Wong, A Tainer, JA Coates, JD AF Youngblut, Matthew D. Tsai, Chi-Lin Clark, Iain C. Carlson, Hans K. Maglaqui, Adrian P. Gau-Pan, Phonchien S. Redford, Steven A. Wong, Alan Tainer, John A. Coates, John D. TI Perchlorate Reductase Is Distinguished by Active Site Aromatic Gate Residues SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID PERIPLASMIC NITRATE REDUCTASE; CRYSTAL-STRUCTURE; MOLYBDENUM; SEQUENCE; PROTEIN; SYSTEM; MARS; DEHYDROGENASE; COORDINATION; PREDICTION AB Perchlorate is an important ion on both Earth and Mars. Perchlorate reductase (PcrAB), a specialized member of the dimethylsulfoxide reductase superfamily, catalyzes the first step of microbial perchlorate respiration, but little is known about the biochemistry, specificity, structure, and mechanism of PcrAB. Here we characterize the biophysics and phylogeny of this enzyme and report the 1.86-angstrom resolution PcrAB complex crystal structure. Biochemical analysis revealed a relatively high perchlorate affinity (K-m = 6 mu M) and a characteristic substrate inhibition compared with the highly similar respiratory nitrate reductase NarGHI, which has a relatively much lower affinity for perchlorate (K-m = 1.1 mM) and no substrate inhibition. Structural analysis of oxidized and reduced PcrAB with and without the substrate analog SeO32- bound to the active site identified key residues in the positively charged and funnel-shaped substrate access tunnel that gated substrate entrance and product release while trapping transiently produced chlorate. The structures suggest gating was associated with shifts of a Phe residue between open and closed conformations plus an Asp residue carboxylate shift between monodentate and bidentate coordination to the active site molybdenum atom. Taken together, structural and mutational analyses of gate residues suggest key roles of these gate residues for substrate entrance and product release. Our combined results provide the first detailed structural insight into the mechanism of biological perchlorate reduction, a critical component of the chlorine redox cycle on Earth. C1 [Youngblut, Matthew D.; Clark, Iain C.; Carlson, Hans K.; Maglaqui, Adrian P.; Gau-Pan, Phonchien S.; Redford, Steven A.; Wong, Alan; Coates, John D.] Univ Calif Berkeley, Energy Biosci Inst, 271 Koshland Hall, Berkeley, CA 94720 USA. [Coates, John D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, 271 Koshland Hall, Berkeley, CA 94720 USA. [Tsai, Chi-Lin; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, Houston, TX 77030 USA. RP Coates, JD (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, 271 Koshland Hall, Berkeley, CA 94720 USA. EM jdcoates@berkeley.edu OI Tsai, Chi-Lin/0000-0002-0365-2405 FU Energy Biosciences Institute, University of California, Berkeley; National Institute of Health Project MINOS (Macromolecular INsights Optimized by Scattering) [R01GM105404]; Robert A. Welch Distinguished Chair in Chemistry FX The work on perchlorate and chlorate respiration in the laboratory of J. D. C. was supported by the Energy Biosciences Institute, University of California, Berkeley, and structural studies were supported by National Institute of Health Project MINOS (Macromolecular INsights Optimized by Scattering) Grant R01GM105404. The authors declare that they have no conflicts of interest with the contents of this article. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health.; Supported by a Robert A. Welch Distinguished Chair in Chemistry. NR 52 TC 3 Z9 3 U1 11 U2 22 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD APR 22 PY 2016 VL 291 IS 17 BP 9190 EP 9202 DI 10.1074/jbc.M116.714618 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DK3WV UT WOS:000374849000030 PM 26940877 ER PT J AU Chien, YT Emerman, A Kang, ZB Ovanesyan, G Vitev, I AF Chien, Yang-Ting Emerman, Alexander Kang, Zhong-Bo Ovanesyan, Grigory Vitev, Ivan TI Jet quenching from QCD evolution SO PHYSICAL REVIEW D LA English DT Article ID PB-PB COLLISIONS; CHARGED-PARTICLE PRODUCTION; COLLINEAR EFFECTIVE THEORY; LARGE TRANSVERSE-MOMENTUM; ABELIAN ENERGY-LOSS; ROOT-S(NN)=2.76 TEV; INCLUSIVE JET; QUANTUM CHROMODYNAMICS; CENTRALITY DEPENDENCE; INELASTIC-SCATTERING AB Recent advances in soft-collinear effective theory with Glauber gluons have led to the development of a new method that gives a unified description of inclusive hadron production in reactions with nucleons and heavy nuclei. We show how this approach, based on the generalization of the DGLAP evolution equations to include final-state medium-induced parton shower corrections for large Q(2) processes, can be combined with initial-state effects for applications to jet quenching phenomenology. We demonstrate that the traditional parton energy loss calculations can be regarded as a special soft-gluon emission limit of the general QCD evolution framework. We present phenomenological comparison of the SCETG-based results on the suppression of inclusive charged hadron and neutral pion production in root s(NN) = 2.76 TeV lead-lead collisions at the Large Hadron Collider to experimental data. We also show theoretical predictions for the upcoming root s(NN) similar or equal to 5.1 TeV Pb + Pb run at the LHC. C1 [Chien, Yang-Ting; Kang, Zhong-Bo; Vitev, Ivan] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Emerman, Alexander] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Ovanesyan, Grigory] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. RP Chien, YT; Kang, ZB; Vitev, I (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Emerman, A (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA.; Ovanesyan, G (reprint author), Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. EM ytchien@lanl.gov; aze2001@columbia.edu; zkang@lanl.gov; ovanesyan@umass.edu; ivitev@lanl.gov RI Kang, Zhongbo/P-3645-2014 FU U.S. Department of Energy, Office of Science [DE-AC52-06NA25396, DE-SC0011095]; DOE Early Career Program; LDRD program at Los Alamos National Laboratory FX This work is supported by the U.S. Department of Energy, Office of Science under Contracts No. DE-AC52-06NA25396 and No. DE-SC0011095, by the DOE Early Career Program, as well as in part by the LDRD program at Los Alamos National Laboratory. NR 98 TC 0 Z9 0 U1 4 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 22 PY 2016 VL 93 IS 7 AR 074030 DI 10.1103/PhysRevD.93.074030 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QQ UT WOS:000374548400001 ER PT J AU Brown, KA Harris, DF Wilker, MB Rasmussen, A Khadka, N Hamby, H Keable, S Dukovic, G Peters, JW Seefeldt, LC King, PW AF Brown, Katherine A. Harris, Derek F. Wilker, Molly B. Rasmussen, Andrew Khadka, Nimesh Hamby, Hayden Keable, Stephen Dukovic, Gordana Peters, John W. Seefeldt, Lance C. King, Paul W. TI Light-driven dinitrogen reduction catalyzed by a CdS:nitrogenase MoFe protein biohybrid SO SCIENCE LA English DT Article ID MOLYBDENUM-IRON PROTEIN; SEMICONDUCTOR CLUSTERS; NITROGENASE; ATP; INTERMEDIATE; ACETYLENE; OXIDATION; AMMONIA; WATER; H-2 AB The splitting of dinitrogen (N-2) and reduction to ammonia (NH3) is a kinetically complex and energetically challenging multistep reaction. In the Haber-Bosch process, N-2 reduction is accomplished at high temperature and pressure, whereas N-2 fixation by the enzyme nitrogenase occurs under ambient conditions using chemical energy from adenosine 5'-triphosphate (ATP) hydrolysis. We show that cadmium sulfide (CdS) nanocrystals can be used to photosensitize the nitrogenase molybdenum-iron (MoFe) protein, where light harvesting replaces ATP hydrolysis to drive the enzymatic reduction of N-2 into NH3. The turnover rate was 75 per minute, 63% of the ATP-coupled reaction rate for the nitrogenase complex under optimal conditions. Inhibitors of nitrogenase (i.e., acetylene, carbon monoxide, and dihydrogen) suppressed N-2 reduction. The CdS: MoFe protein biohybrids provide a photochemical model for achieving light-driven N-2 reduction to NH3. C1 [Brown, Katherine A.; King, Paul W.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Harris, Derek F.; Rasmussen, Andrew; Khadka, Nimesh; Seefeldt, Lance C.] Utah State Univ, Dept Chem & Biochem, Logan, UT 84322 USA. [Wilker, Molly B.; Hamby, Hayden; Dukovic, Gordana] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Keable, Stephen; Peters, John W.] Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA. [Wilker, Molly B.] Luther Coll, Dept Chem, Decorah, IA 52101 USA. RP King, PW (reprint author), Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. EM paul.king@nrel.gov RI King, Paul/D-9979-2011; OI King, Paul/0000-0001-5039-654X; Peters, John/0000-0001-9117-9568 FU Laboratory Directed Research and Development Program seed project; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0010334]; U.S. Department of Energy, Office of Science [DE-SC0012518] FX K.A.B. and P.W.K. were supported by a Laboratory Directed Research and Development Program seed project at the National Renewable Energy Laboratory for CdS:MoFe protein photochemical H2 production experiments, and by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; and the U.S. Department of Energy under Contract no. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory for CdS:MoFe protein biohybrid N2 reduction experiments. M.B.W., H.H., and G.D. conducted nanocrystal synthesis and ligand exchange under support by U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-SC0010334. D.F.H., A.R., N.K., S.K., L.C.S., and J.W.P. were supported for nitrogenase purification and product quantification as part of the Biological and Electron Transfer and Catalysis (BETCy) EFRC, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science (DE-SC0012518). The authors thank W. Tumas and R. Greene for thoughtful advice and many helpful discussions, and B. Hoffman for helpful discussions and constructive reading of the manuscript. Data are available in the supplementary materials. K.A.B. preformed photochemical experiments, including colorimetric NH3 measurements; N.K., A.R., D.F.H., and S.K. preformed nitrogenase and MoFe protein purifications, physiological nitrogenase assays, and fluorometric NH3 measurements; M.B.W. and H.H. performed CdS nanocrystal synthesis, ligand exchange, and transmission electron microscopy imaging; K.A.B, L.C.S., G.D., J.W.P., and P.W.K. conceived and designed the study. All authors contributed to the writing of the manuscript. NR 21 TC 19 Z9 20 U1 50 U2 121 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD APR 22 PY 2016 VL 352 IS 6284 BP 448 EP 450 DI 10.1126/science.aaf2091 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ8RH UT WOS:000374479700044 PM 27102481 ER PT J AU Zeng, LS Zhang, J Sarovar, M AF Zeng, Lishan Zhang, Jun Sarovar, Mohan TI Schedule path optimization for adiabatic quantum computing and optimization SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE quantum annealing; adiabatic quantum computing; convex optimization ID COMPUTATION; QUBITS AB Adiabatic quantum computing and optimization have garnered much attention recently as possible models for achieving a quantum advantage over classical approaches to optimization and other special purpose computations. Both techniques are probabilistic in nature and the minimum gap between the ground state and first excited state of the system during evolution is a major factor in determining the success probability. In this work we investigate a strategy for increasing the minimum gap and success probability by introducing intermediate Hamiltonians that modify the evolution path between initial and final Hamiltonians. We focus on an optimization problem relevant to recent hardware implementations and present numerical evidence for the existence of a purely local intermediate Hamiltonian that achieve the optimum performance in terms of pushing the minimum gap to one of the end points of the evolution. As a part of this study we develop a convex optimization formulation of the search for optimal adiabatic schedules that makes this computation more tractable, and which may be of independent interest. We further study the effectiveness of random intermediate Hamiltonians on the minimum gap and success probability, and empirically find that random Hamiltonians have a significant probability of increasing the success probability, but only by a modest amount. C1 [Zeng, Lishan; Zhang, Jun] Shanghai Jiao Tong Univ, Joint Inst UMich SJTU, Shanghai 200240, Peoples R China. [Zeng, Lishan; Zhang, Jun] Shanghai Jiao Tong Univ, Key Lab Syst Control & Informat Proc MOE, Shanghai 200240, Peoples R China. [Sarovar, Mohan] Sandia Natl Labs, Digital & Quantum Informat Syst, Livermore, CA 94550 USA. RP Zhang, J (reprint author), Shanghai Jiao Tong Univ, Joint Inst UMich SJTU, Shanghai 200240, Peoples R China.; Zhang, J (reprint author), Shanghai Jiao Tong Univ, Key Lab Syst Control & Informat Proc MOE, Shanghai 200240, Peoples R China.; Sarovar, M (reprint author), Sandia Natl Labs, Digital & Quantum Informat Syst, Livermore, CA 94550 USA. EM zhangjun12@sjtu.edu.cn; mnsarov@sandia.gov FU Laboratory Directed Research and Development program; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF China [61174086, 61533012]; State Key Laboratory of Precision Spectroscopy, ECNU, China FX MS would like to thank Kevin Young, Constantin Brif, and Eddie Farhi for useful discussions. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. JZ acknowledges financial support from NSF China under Grant No. 61174086 and 61533012, and State Key Laboratory of Precision Spectroscopy, ECNU, China. NR 45 TC 0 Z9 0 U1 2 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD APR 22 PY 2016 VL 49 IS 16 AR 165305 DI 10.1088/1751-8113/49/16/165305 PG 20 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA DG6LJ UT WOS:000372195600017 ER PT J AU Gur, S Danielson, T Xiong, QG Hin, C Pannala, S Frantziskonis, G Savara, A Daw, CS AF Gur, Sourav Danielson, Thomas Xiong, Qingang Hin, Celine Pannala, Sreekanth Frantziskonis, George Savara, Aditya Daw, C. Stuart TI Wavelet-based surrogate time series for multiscale simulation of heterogeneous catalysis SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Wavelet based transformation; Random surrogates; Kinetic Monte Carlo; Temporal upscaling; Multiscale modeling of catalysis ID STOCHASTIC SIMULATION; DIFFUSION PROBLEMS; DYNAMICAL-SYSTEMS; EQUATIONS; FRAMEWORK; SCALES AB We propose a wavelet-based scheme that encodes the essential dynamics of discrete microscale surface reactions in a form that can be coupled with continuum macroscale flow simulations with high computational efficiency. This makes it possible to simulate the dynamic behavior of reactor-scale heterogeneous catalysis without requiring detailed concurrent simulations at both the surface and continuum scales using different models. Our scheme is based on the application of wavelet-based surrogate time series that encodes the essential temporal and/or spatial fine-scale dynamics at the catalyst surface. The encoded dynamics are then used to generate statistically equivalent, randomized surrogate time series, which can be linked to the continuum scale simulation. We illustrate an application of this approach using two different kinetic Monte Carlo simulations with different characteristic behaviors typical for heterogeneous chemical reactions. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Gur, Sourav; Frantziskonis, George] Univ Arizona, Dept Civil Engn & Engn Mech, Tucson, AZ 85721 USA. [Danielson, Thomas; Xiong, Qingang; Savara, Aditya; Daw, C. Stuart] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hin, Celine] Virginia Polytech Inst & State Univ, 635 Prices Ford Rd, Blacksburg, VA 24060 USA. [Pannala, Sreekanth] SABIC, Sugar Land, TX 77478 USA. RP Frantziskonis, G (reprint author), Univ Arizona, Dept Civil Engn & Engn Mech, Tucson, AZ 85721 USA. EM frantzis@email.arizona.edu RI Savara, Aditya (Ashi)/A-8831-2010 OI Savara, Aditya (Ashi)/0000-0002-1937-2571 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX Research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. NR 40 TC 2 Z9 2 U1 7 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD APR 22 PY 2016 VL 144 BP 165 EP 175 DI 10.1016/j.ces.2016.01.037 PG 11 WC Engineering, Chemical SC Engineering GA DF6NO UT WOS:000371472700017 ER PT J AU Crawford, NC Sprague, MA Stickel, JJ AF Crawford, Nathan C. Sprague, Michael A. Stickel, Jonathan J. TI Mixing behavior of a model cellulosic biomass slurry during settling and resuspension SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Biomass; Cellulose; Resuspension; Settling Mixing; Rheology ID HIGH SOLIDS CONCENTRATIONS; VISCOUS RESUSPENSION; ETHANOL-PRODUCTION; DENSE SUSPENSIONS; YIELD-STRESS; SHEAR; FLOW; RHEOLOGY; VANE; COUETTE AB Thorough mixing during biochemical deconstruction of biomass is crucial for achieving maximum process yields and economic success. However, due to the complex morphology and surface chemistry of biomass particles, biomass mixing is challenging and currently it is not well understood. This study investigates the bulk rheology of negatively buoyant, non-Brownian a-cellulose particles during settling and resuspension. The torque signal of a vane mixer across two distinct experimental setups (vane-in-cup and vane-in-beaker) was used to understand how mixing conditions affect the distribution of biomass particles. During experimentation, a bifurcated torque response as a function of vane speed was observed, indicating that the slurry transitions from a "settling-dominant" regime to a "suspension dominant" regime. The torque response of well-characterized fluids (i.e., DI water) were then used to empirically identify when sufficient mixing turbulence was established in each experimental setup. The predicted critical mixing speeds were in agreement with measured values, suggesting that secondary flows are required in order to keep the cellulose particles fully suspended. In addition, a simple scaling relationship was developed to model the entire torque signal of the slurry throughout settling and resuspension. Qualitative and semi-quantitative agreement between the model and experimental results was observed. Published by Elsevier Ltd. C1 [Crawford, Nathan C.; Stickel, Jonathan J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. [Sprague, Michael A.] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. RP Crawford, NC (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. EM nathan.crawford@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory (NREL); Office of the Biomass Program FX This work was funded by the U.S. Department of Energy under Contract no. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory (NREL) and through the Office of the Biomass Program. The authors thank Prof. Matthew Liberatore (Colorado School of Mines) for the use of his laboratory to collect the rheological data presented here. The authors also thank Jessica Olstad (NREL) who performed the laser diffraction particle size measurements. The U.S. Government and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 57 TC 0 Z9 0 U1 4 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD APR 22 PY 2016 VL 144 BP 310 EP 320 DI 10.1016/j.ces.2016.01.028 PG 11 WC Engineering, Chemical SC Engineering GA DF6NO UT WOS:000371472700031 ER PT J AU Lin, MW Kravchenko, II Fowlkes, J Li, XF Puretzky, AA Rouleau, CM Geohegan, DB Xiao, K AF Lin, Ming-Wei Kravchenko, Ivan I. Fowlkes, Jason Li, Xufan Puretzky, Alexander A. Rouleau, Christopher M. Geohegan, David B. Xiao, Kai TI Thickness-dependent charge transport in few-layer MoS2 field-effect transistors SO NANOTECHNOLOGY LA English DT Article DE MoS2; field-effect transistor; metal insulator transition ID TRANSITION-METAL DICHALCOGENIDES; CHEMICAL-VAPOR-DEPOSITION; IOFFE-REGEL CRITERION; MONOLAYER MOS2; BILAYER MOS2; MOLYBDENUM-DISULFIDE; MOBILITY; OPTOELECTRONICS; SCATTERING; INSULATOR AB Molybdenum disulfide (MoS2) is currently under intensive study because of its exceptional optical and electrical properties in few-layer form. However, how charge transport mechanisms vary with the number of layers in MoS2 flakes remains unclear. Here, exfoliated flakes of MoS2 with various thicknesses were successfully fabricated into field-effect transistors (FETs) to measure the thickness and temperature dependences of electrical mobility. For these MoS2 FETs, measurements at both 295 K and 77 K revealed the maximum mobility for layer thicknesses between 5 layers (similar to 3.6 nm) and 10 layers (similar to 7 nm), with similar to 70 cm(2) V-1 s(-1) measured for 5 layer devices at 295 K. Temperature-dependent mobility measurements revealed that the mobility rises with increasing temperature to a maximum. This maximum occurs at increasing temperature with increasing layer thickness, possibly due to strong Coulomb scattering from charge impurities or weakened electron-phonon interactions for thicker devices. Temperature-dependent conductivity measurements for different gate voltages revealed a metal-to-insulator transition for devices thinner than 10 layers, which may enable new memory and switching applications. This study advances the understanding of fundamental charge transport mechanisms in few-layer MoS2, and indicates the promise of few-layer transition metal dichalcogenides as candidates for potential optoelectronic applications. C1 [Lin, Ming-Wei; Kravchenko, Ivan I.; Fowlkes, Jason; Li, Xufan; Puretzky, Alexander A.; Rouleau, Christopher M.; Geohegan, David B.; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Xiao, K (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM xiaok@ornl.gov RI Kravchenko, Ivan/K-3022-2015; Li, Xufan/A-8292-2013; Geohegan, David/D-3599-2013 OI Kravchenko, Ivan/0000-0003-4999-5822; Li, Xufan/0000-0001-9814-0383; Geohegan, David/0000-0003-0273-3139 FU Laboratory Directed Research and Development award from Oak Ridge National Laboratory FX This research was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. MWL acknowledges support provided by a Laboratory Directed Research and Development award from Oak Ridge National Laboratory for device fabrication and characterization. NR 47 TC 4 Z9 4 U1 9 U2 74 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD APR 22 PY 2016 VL 27 IS 16 AR 165203 DI 10.1088/0957-4484/27/16/165203 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DG0RU UT WOS:000371774100005 PM 26963583 ER PT J AU Hamidian, MH Edkins, SD Joo, SH Kostin, A Eisaki, H Uchida, S Lawler, MJ Kim, EA Mackenzie, AP Fujita, K Lee, J Davis, JCS AF Hamidian, M. H. Edkins, S. D. Joo, Sang Hyun Kostin, A. Eisaki, H. Uchida, S. Lawler, M. J. Kim, E. -A. Mackenzie, A. P. . Fujita, K. Lee, Jinho Davis, J. C. Seamus TI Detection of a Cooper-pair density wave in Bi2Sr2CaCu2O8+x SO NATURE LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; ELECTROMAGNETIC ENVIRONMENT; CUPRATE SUPERCONDUCTORS; JOSEPHSON-JUNCTIONS; CHARGE ORDER; SYMMETRY AB The quantum condensate of Cooper pairs forming a superconductor was originally conceived as being translationally invariant. In theory, however, pairs can exist with finite momentum Q, thus generating a state with a spatially modulated Cooper-pair density(1,2). Such a state has been created in ultracold Li-6 gas(3) but never observed directly in any superconductor. It is now widely hypothesized that the pseudogap phase(4) of the copper oxide superconductors contains such a 'pair density wave' state(5-21). Here we report the use of nanometre-resolution scanned Josephson tunnelling microscopy(22-24) to image Cooper pair tunnelling from a d-wave superconducting microscope tip to the condensate of the superconductor Bi2Sr2CaCu2O8+x. We demonstrate condensate visualization capabilities directly by using the Cooper-pair density variations surrounding zinc impurity atoms(25) and at the Bi2Sr2CaCu2O8+x crystal supermodulation(26). Then, by using Fourier analysis of scanned Josephson tunnelling images, we discover the direct signature of a Cooper-pair density modulation at wavevectors Q(P) approximate to (0.25, 0)2 pi/a(0) and (0, 0.25)2 pi/a(0) in Bi2Sr2CaCu2O8+x. The amplitude of these modulations is about five per cent of the background condensate density and their form factor exhibits primarily s or s' symmetry. This phenomenology is consistent with Ginzburg-Landau theory(5,13,14) when a charge density wave(5,27) with d-symmetry form factor(28-30) and wavevector Q(C) = Q(P) coexists with a d-symmetry superconductor; it is also predicted by several contemporary microscopic theories for the pseudogap phase(18-21). C1 [Hamidian, M. H.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Edkins, S. D.; Kostin, A.; Lawler, M. J.; Kim, E. -A.; Davis, J. C. Seamus] Cornell Univ, Dept Phys, Lab Atom & Solid State Phys, Ithaca, NY 14853 USA. [Edkins, S. D.; Mackenzie, A. P. .; Davis, J. C. Seamus] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Joo, Sang Hyun; Lee, Jinho] Seoul Natl Univ, Inst Appl Phys, Dept Phys & Astron, Seoul 151747, South Korea. [Joo, Sang Hyun; Lee, Jinho] Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151742, South Korea. [Eisaki, H.; Uchida, S.] Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. [Uchida, S.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130011, Japan. [Lawler, M. J.] SUNY Binghamton, Dept Phys, Binghamton, NY 13902 USA. [Mackenzie, A. P. .] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Fujita, K.; Davis, J. C. Seamus] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Davis, J. C. Seamus] Cornell Univ, Cornell Nanoscale Sci, Kavli Inst, Ithaca, NY 14853 USA. RP Davis, JCS (reprint author), Cornell Univ, Dept Phys, Lab Atom & Solid State Phys, Ithaca, NY 14853 USA.; Davis, JCS (reprint author), Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland.; Lee, J (reprint author), Seoul Natl Univ, Inst Appl Phys, Dept Phys & Astron, Seoul 151747, South Korea.; Lee, J (reprint author), Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151742, South Korea.; Davis, JCS (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.; Davis, JCS (reprint author), Cornell Univ, Cornell Nanoscale Sci, Kavli Inst, Ithaca, NY 14853 USA. EM jinholee@snu.ac.kr; jcseamusdavis@gmail.com NR 44 TC 18 Z9 18 U1 21 U2 25 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD APR 21 PY 2016 VL 532 IS 7599 BP 343 EP + DI 10.1038/nature17411 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DZ9WR UT WOS:000386232400001 PM 27074504 ER PT J AU Menasche, DB Lind, J Li, SF Kenesei, P Bingert, JF Lienert, U Suter, RM AF Menasche, David B. Lind, Jonathan Li, Shiu Fai Kenesei, Peter Bingert, John F. Lienert, Ulrich Suter, Robert M. TI Shock induced damage in copper: A before and after, three-dimensional study SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ENERGY DIFFRACTION MICROSCOPY; ADVANCED PHOTON SOURCE; X-RAY-DIFFRACTION; POLYCRYSTALLINE COPPER; PLASTIC-DEFORMATION; GRAIN-BOUNDARIES; TWIN NUCLEATION; DYNAMIC DAMAGE; STRAIN-RATE; ORIENTATION AB We report on the microstructural features associated with the formation of incipient spall and damage in a fully recrystallized, high purity copper sample. Before and after ballistic shock loading, approximately 0.8 mm(3) of the sample's crystal lattice orientation field is mapped using non-destructive near-field High Energy Diffraction Microscopy. Absorption contrast tomography is used to image voids after loading. This non-destructive interrogation of damage initiation allows for novel characterization of spall points vis-a-vis microstructural features and a fully 3D examination of microstructural topology and its influence on incipient damage. The spalled region is registered with and mapped back onto the pre-shock orientation field. As expected, the great majority of voids occur at grain boundaries and higher order microstructural features; however, we find no statistical preference for particular grain boundary types. The damaged region contains a large volume of Sigma-3 (60 degrees < 111 >) connected domains with a large area fraction of incoherent R-3 boundaries. Published by AIP Publishing. C1 [Menasche, David B.; Suter, Robert M.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Lind, Jonathan] Lawrence Livermore Natl Lab LLNL, Mat Engn Div, Livermore, CA 94550 USA. [Li, Shiu Fai] LLNL, Computat Engn Div, Livermore, CA 94550 USA. [Kenesei, Peter] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Bingert, John F.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. [Lienert, Ulrich] DESY, Hamburg, Germany. RP Menasche, DB (reprint author), Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. EM davidmenasche@cmu.edu RI Suter, Robert/P-2541-2014 OI Suter, Robert/0000-0002-0651-0437 FU LANL's Laboratory-Directed Research and Development-Directed Research (LDRD-DR) [20140114DR]; Joint DoD/DOE Munitions Program; National Nuclear Security Administration's Science Campaign 2; U.S. DOE [DEAC02-06CH11357] FX The authors would like to thank many individuals for their assistance: C. M. Hefferan and R. Pokharel (CMU) for assisting with HEDM measurements at APS, S. Maddali (CMU) for boundary smoothing code. M. Prijatelj (CMU) for image artifact removal, R. Randolph (LANL) for micro machining, M. F. Lopez (LANL) for heat treating, G. T. Gray III (LANL) for providing material, M. Tucker (LANL) for APS assistance, D. Martinez (LANL) for experimentation, A. D. Rollett (CMU), R. A. Lebensohn (LANL), and C. A. Bronkhorst (LANL) for useful discussions, and E. K. Cerreta and C. A. Bronkhorst whose collaborations helped secure APS beamtime. Work at CMU was supported by LANL's Laboratory-Directed Research and Development-Directed Research (LDRD-DR Project No. 20140114DR "Mesoscale Materials Science of Ductile Damage in 4 Dimensions"). J.F.B. acknowledges the support of the Joint DoD/DOE Munitions Program and the National Nuclear Security Administration's Science Campaign 2. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DEAC02-06CH11357. NR 47 TC 1 Z9 1 U1 6 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 21 PY 2016 VL 119 IS 15 AR 154902 DI 10.1063/1.4947270 PG 7 WC Physics, Applied SC Physics GA DQ1WS UT WOS:000378991800030 ER PT J AU Sarikurt, S Ozden, A Kandemir, A Sevik, C Kinaci, A Haskins, JB Cagin, T AF Sarikurt, S. Ozden, A. Kandemir, A. Sevik, C. Kinaci, A. Haskins, J. B. Cagin, T. TI Tailoring thermal conductivity of silicon/germanium nanowires utilizing core-shell architecture SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NANOSCALE ELECTRONIC DEVICES; SILICON NANOWIRES; THERMOELECTRIC FIGURE; CARBON NANOTUBES; TRANSPORT-COEFFICIENTS; SIMULATION; GERMANIUM; GE; SI; HETEROSTRUCTURES AB Low-dimensional nanostructured materials show large variations in their thermal transport properties. In this work, we investigate the influence of the core-shell architecture on nanowire (1D) thermal conductivity and evaluate its validity as a strategy to achieve a better thermoelectric performance. To obtain the thermal conductivity values, equilibrium molecular dynamics simulations are conducted for core-shell nanowires of silicon and germanium. To explore the parameter space, we have calculated thermal conductivity values of the Si-core/Ge-shell and Ge-core/Si-shell nanowires having different cross-sectional sizes and core contents at several temperatures. Our results indicate that (1) increasing the cross-sectional area of pristine Si and pristine Ge nanowires increases the thermal conductivity, (2) increasing the Ge core size in the Ge-core/Si-shell structure results in a decrease in the thermal conductivity at 300 K, (3) the thermal conductivity of the Sicore/Ge-shell nanowires demonstrates a minima at a specific core size, (4) no significant variation in the thermal conductivity is observed in nanowires for temperatures larger than 300 K, and (5) the predicted thermal conductivity within the frame of applied geometrical constraints is found to be around 10 W/(mK) for the Si and Ge core-shell architecture with a smooth interface. The value is still higher than the amorphous limit (1 W/(mK)). This represents a significant reduction in thermal conductivity with respect to their bulk crystalline and pristine nanowire forms. Furthermore, we observed additional suppression of thermal conductivity through the introduction of interface roughness to Si/Ge core-shell nanowires. Published by AIP Publishing. C1 [Sarikurt, S.; Kinaci, A.; Cagin, T.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sarikurt, S.] Dokuz Eylul Univ, Fac Sci, Dept Phys, TR-35390 Izmir, Turkey. [Ozden, A.; Kandemir, A.] Anadolu Univ, Fac Engn, Dept Mat Sci & Engn, TR-26555 Eskisehir, Turkey. [Sevik, C.] Anadolu Univ, Fac Engn, Dept Mech Engn, TR-26555 Eskisehir, Turkey. [Kinaci, A.] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60439 USA. [Haskins, J. B.] NASA, AMA Inc, Ames Res Ctr, Moffett Field, CA 94035 USA. [Haskins, J. B.; Cagin, T.] Texas A&M Univ, Artie McFerrin Dept Chem Engn, College Stn, TX 77843 USA. RP Cagin, T (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA.; Cagin, T (reprint author), Texas A&M Univ, Artie McFerrin Dept Chem Engn, College Stn, TX 77843 USA. EM sevil.sarikurt@deu.edu.tr; csevik@anadolu.edu.tr; tcagin@tamu.edu RI Kandemir, Ali/A-4034-2017 OI Kandemir, Ali/0000-0001-9813-6421 FU International Institute of Materials for Energy Conversion (IIMEC) at Texas AM University; NSF International Materials Institute [DMR 0844082]; Scientific and Technological Research Council of Turkey (TUBITAK-BIDEB) [2219]; Scientific and Technological Research Council of Turkey [TUBITAK-113F096]; Anadolu University [BAP-140717335]; Turkish Academy of Sciences (TUBA-GEBIP) FX We acknowledge support from the International Institute of Materials for Energy Conversion (IIMEC) at Texas A&M University, an NSF International Materials Institute (DMR 0844082). All of the computations were carried out at the facilities of Laboratory of Computational Engineering of Nanomaterials, Chemical Engineering Cluster, Supercomputing Center of Texas A&M University, and also Eskisehir Anadolu University. S. Sarikurt was supported by Scientific and Technological Research Council of Turkey (TUBITAK-BIDEB) 2219 International Postdoctoral Research Scholarship Program and IIMEC during this study at Texas A&M University, C. Sevik acknowledges the support from Scientific and Technological Research Council of Turkey (TUBITAK-113F096), Anadolu University (BAP-140717335), and Turkish Academy of Sciences (TUBA-GEBIP) to this project. NR 52 TC 1 Z9 1 U1 7 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 21 PY 2016 VL 119 IS 15 AR 155101 DI 10.1063/1.4946835 PG 9 WC Physics, Applied SC Physics GA DQ1WS UT WOS:000378991800031 ER PT J AU Tadaki, D Ma, T Zhang, JY Iino, S Hirano-Iwata, A Kimura, Y Rosenberg, RA Niwano, M AF Tadaki, Daisuke Ma, Teng Zhang, Jinyu Iino, Shohei Hirano-Iwata, Ayumi Kimura, Yasuo Rosenberg, Richard A. Niwano, Michio TI Fabrication and characterization of p(+)-i-p(+) type organic thin film transistors with electrodes of highly doped polymer SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LIGHT-EMITTING-DIODES; FIELD-EFFECT MOBILITY; CONDUCTING-POLYMER; VOLTAGE; DEVICES; P3HT; EFFICIENCY; INTERFACE; STABILITY; BARRIER AB Organic thin film transistors (OTFTs) have been explored because of their advantageous features such as light-weight, flexible, and large-area. For more practical application of organic electronic devices, it is very important to realize OTFTs that are composed only of organic materials. In this paper, we have fabricated p(+)-i-p(+) type of OTFTs in which an intrinsic (i) regioregular poly (3-hexylthiophene) (P3HT) layer is used as the active layer and highly doped p-type (p(+)) P3HT is used as the source and drain electrodes. The 2,3,5,6-tetrafluoro-7,7,8,8-tetracyanoquinodimethane (F-4-TCNQ) was used as the p-type dopant. A fabricating method of p(+)-i-p(+) OTFTs has been developed by using SiO2 and aluminum films as capping layers for micro-scaled patterning of the p(+)-P3HT electrodes. The characteristics of the OTFTs were examined using the photoelectron spectroscopy and electrical measurements. We demonstrated that the fabricated p(+)-i-p(+) OTFTs work with carrier injection through a built-in potential at p(+)/i interfaces. We found that the p(+)-i-p(+) OTFTs exhibit better FET characteristics than the conventional P3HT-OTFT with metal (Au) electrodes, indicating that the influence of a carrier injection barrier at the interface between the electrode and the active layer was suppressed by replacing the metal electrodes with p(+)-P3HT layers. Published by AIP Publishing. C1 [Tadaki, Daisuke; Hirano-Iwata, Ayumi] Tohoku Univ, Grad Sch Biomed Engn, Sendai, Miyagi 9808579, Japan. [Tadaki, Daisuke; Ma, Teng; Zhang, Jinyu; Iino, Shohei; Niwano, Michio] Tohoku Univ, Elect Commun Res Inst, Lab Nanoelect & Spintron, Sendai, Miyagi 9808577, Japan. [Tadaki, Daisuke; Ma, Teng; Hirano-Iwata, Ayumi; Kimura, Yasuo; Niwano, Michio] Japan Sci & Technol Agcy, CREST, Kawaguchi, Saitama 3320012, Japan. [Kimura, Yasuo] Tokyo Univ Technol, Hachioji, Tokyo 1920982, Japan. [Rosenberg, Richard A.] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Niwano, M (reprint author), Tohoku Univ, Elect Commun Res Inst, Lab Nanoelect & Spintron, Sendai, Miyagi 9808577, Japan.; Niwano, M (reprint author), Japan Sci & Technol Agcy, CREST, Kawaguchi, Saitama 3320012, Japan. EM niwano@riec.tohoku.ac.jp FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; CREST program (Development of Atomic or Molecular Two-Dimensional Functional Films and Creation of Fundamental Technologies for Their Applications) of Japan Science and Technology Agency (JST) FX We would like to thank Scienta Omicron for the loan of the Argus electron energy analyzer. This work has been performed at the Laboratory for Nanoelectronics and Spintronics, Research Institute of Electrical Communication, Tohoku University, and partly at Advanced Photon Source, Argonne National Laboratory. The work performed at the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. This work was supported in part by CREST program (Development of Atomic or Molecular Two-Dimensional Functional Films and Creation of Fundamental Technologies for Their Applications) of Japan Science and Technology Agency (JST). NR 35 TC 1 Z9 1 U1 7 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 21 PY 2016 VL 119 IS 15 AR 154503 DI 10.1063/1.4946888 PG 8 WC Physics, Applied SC Physics GA DQ1WS UT WOS:000378991800024 ER PT J AU Johnson, RC Garza, JC MacFarlane, RB Grimes, CB Phillis, CC Koch, PL Weber, PK Carr, MH AF Johnson, Rachel C. Garza, John Carlos MacFarlane, R. Bruce Grimes, Churchill B. Phillis, Corey C. Koch, Paul L. Weber, Peter K. Carr, Mark H. TI Isotopes and genes reveal freshwater origins of Chinook salmon Oncorhynchus tshawytscha aggregations in California's coastal ocean SO MARINE ECOLOGY PROGRESS SERIES LA English DT Article DE Winter-run Chinook salmon; Schooling; Otolith microchemistry; Strontium; Navigation ID WIRE TAG RECOVERIES; LA-MC-ICPMS; PACIFIC SALMON; STOCK IDENTIFICATION; POPULATION-STRUCTURE; MICROSATELLITE DNA; CENTRAL VALLEY; OTOLITH MICROCHEMISTRY; SPATIAL-DISTRIBUTION; ATLANTIC SALMON AB The ability of salmon to navigate from the ocean back to their river of origin to spawn acts to reinforce local adaptation and maintenance of unique and heritable traits among salmon populations. Here, the extent to which Chinook salmon Oncorhynchus tshawytscha from the same freshwater breeding groups associate together in the ocean at regional and smaller-scale aggregations prior to homeward migration is evaluated. Natural variation in salmon otolith daily growth bands, strontium isotopes (Sr-87/Sr-86), and microsatellite DNA were used as intrinsic tags to link the distributions of fish caught in the ocean with their freshwater origins. Adults were caught from vessels by hook and line in small aggregations (7-18 ind.) at the same geographic location (1-24 km of coastline) and time (4-36 h) from 3 ocean regions along central California, USA. Salmon caught together in aggregations were from the same genetic group, and to a lesser extent, of the same natal origin (individual rivers or hatcheries). However, at regional scales, adult salmon mixed. Central Valley winter-run Chinook salmon caught together in the ocean varied in the duration of freshwater rearing for up to 2-3 mo prior to seaward migration, suggesting associations within the group were not established in freshwater or maintained over the lifetime of the fish. Our findings are consistent with coarser information indicating stocks are distributed differently in time and space, but larger sample sizes are required to evaluate the consistency of patterns at smaller spatial scales. This study uncovers freshwater associations prior to homeward migration, a principle and undocumented prerequisite of the collective navigation hypothesis. C1 [Johnson, Rachel C.; Garza, John Carlos; MacFarlane, R. Bruce; Grimes, Churchill B.] NOAA, Fisheries Ecol Div, Southwest Fisheries Sci Ctr, Natl Marine Fisheries Serv, 110 Shaffer Rd, Santa Cruz, CA 95060 USA. [Johnson, Rachel C.; Carr, Mark H.] Univ Calif Santa Cruz, Dept Ecol & Evolutionary Biol, 110 Shaffer Rd, Santa Cruz, CA 95060 USA. [Garza, John Carlos] Univ Calif Santa Cruz, Dept Ocean Sci, 1156 High St, Santa Cruz, CA 95060 USA. [MacFarlane, R. Bruce; Grimes, Churchill B.] Univ Calif Santa Cruz, Inst Marine Sci, 110 Shaffer Rd, Santa Cruz, CA 95060 USA. [Phillis, Corey C.] Univ Calif Berkeley, Dept Earth & Planetary Sci, 307 McCone Hall, Berkeley, CA 94720 USA. [Koch, Paul L.] Univ Calif Santa Cruz, Dept Earth & Planetary Sci, 1156 High St, Santa Cruz, CA 95060 USA. [Weber, Peter K.] Lawrence Livermore Natl Lab, Glenn T Seaborg Inst, 7000 East Ave, Livermore, CA 94550 USA. [Phillis, Corey C.] Metropolitan Water Dist Southern Calif, 1121 L St Suite 900, Sacramento, CA 95814 USA. RP Johnson, RC (reprint author), NOAA, Fisheries Ecol Div, Southwest Fisheries Sci Ctr, Natl Marine Fisheries Serv, 110 Shaffer Rd, Santa Cruz, CA 95060 USA.; Johnson, RC (reprint author), Univ Calif Santa Cruz, Dept Ecol & Evolutionary Biol, 110 Shaffer Rd, Santa Cruz, CA 95060 USA. EM rachel.johnson@noaa.gov FU NOAA Fisheries through the Student Careers' Experience Program; University of California's Coastal Environmental Quality Initiative; Partnership for Interdisciplinary Studies of Coastal Oceans (PISCO); Gordon and Betty Moore Foundation; David and Lucile Packard Foundation; Myers Oceanographic Trust FX We thank W. Satterthwaite and S. Lindley for discussions and significant improvements to the manuscript, F. Ramos and D. Tollstrup for assistance with Sr isotopic measurements, E. Anderson and A. Clemento for assistance with genetic analyses, and P. Raimondi and C. Syms for statistical advice. Special thanks to M. Kilgour, A. Nickels, S. Reins, and A. Bachar for tissue collection and preparation. This project would not have been possible without the fishing skills of P. Parravano, J. Hie, R. Block, J. Estes, S. Berkeley, J. Figurski, S. Sogard and the crew and patrons of the 'New Captain Pete', 'The Outer Limits', and 'Dave's Albacore'. A. Smith provided GIS assistance for Fig. 1, and G. Whitman provided editorial assistance. We thank the programs that funded this work: NOAA Fisheries through the Student Careers' Experience Program, University of California's Coastal Environmental Quality Initiative, and the Partnership for Interdisciplinary Studies of Coastal Oceans (PISCO), which is funded primarily by the Gordon and Betty Moore Foundation, the David and Lucile Packard Foundation, and the Myers Oceanographic Trust. NR 86 TC 0 Z9 0 U1 5 U2 6 PU INTER-RESEARCH PI OLDENDORF LUHE PA NORDBUNTE 23, D-21385 OLDENDORF LUHE, GERMANY SN 0171-8630 EI 1616-1599 J9 MAR ECOL PROG SER JI Mar. Ecol.-Prog. Ser. PD APR 21 PY 2016 VL 548 BP 181 EP 196 DI 10.3354/meps11623 PG 16 WC Ecology; Marine & Freshwater Biology; Oceanography SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Oceanography GA DM5GF UT WOS:000376375000013 ER PT J AU Bjorgaard, JA Velizhanin, KA Tretiak, S AF Bjorgaard, J. A. Velizhanin, K. A. Tretiak, S. TI Nonequilibrium solvent effects in Born-Oppenheimer molecular dynamics for ground and excited electronic states SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID POLARIZABLE CONTINUUM MODEL; DENSITY-FUNCTIONAL THEORY; DEPENDENT STOKES SHIFT; CONJUGATED MOLECULES; DIELECTRIC FRICTION; POLAR-SOLVENTS; SOLVATION; ENERGY; SIMULATIONS; EXCITATIONS AB The effects of solvent on molecular processes such as excited state relaxation and photochemical reaction often occurs in a nonequilibrium regime. Dynamic processes such as these can be simulated using excited state molecular dynamics. In this work, we describe methods of simulating nonequilibrium solvent effects in excited state molecular dynamics using linear-response time-dependent density functional theory and apparent surface charge methods. These developments include a propagation method for solvent degrees of freedom and analytical energy gradients for the calculation of forces. Molecular dynamics of acetaldehyde in water or acetonitrile are demonstrated where the solute-solvent system is out of equilibrium due to photoexcitation and emission. Published by AIP Publishing. C1 [Bjorgaard, J. A.] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Velizhanin, K. A.; Tretiak, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Tretiak, S.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Bjorgaard, JA (reprint author), Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.; Tretiak, S (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Tretiak, S (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. EM jbjorgaard@lanl.gov; serg@lanl.gov RI Velizhanin, Kirill/C-4835-2008; Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Bjorgaard, Josiah/0000-0003-3679-2487 FU U.S. Department of Energy; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Center for Nonlinear Studies (CNLS) at LANL; Center for Integrated Nanotechnology (CINT) at LANL FX We acknowledge support of the U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. We also acknowledge support of the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnology (CINT) at LANL. We also acknowledge the LANL Institutional Computing (IC) Program for providing computational resources. NR 50 TC 0 Z9 0 U1 3 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 21 PY 2016 VL 144 IS 15 AR 154104 DI 10.1063/1.4946009 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL6YM UT WOS:000375786000010 PM 27389206 ER PT J AU Griffin, PJ Wang, YY Holt, AP Sokolov, AP AF Griffin, Philip J. Wang, Yangyang Holt, Adam P. Sokolov, Alexei P. TI Communication: Influence of nanophase segregation on ion transport in room temperature ionic liquids SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ORIENTATIONAL DYNAMICS; SUPERCOOLED LIQUIDS; MOLECULAR-DYNAMICS; NANOSTRUCTURE; AGGREGATION; RELAXATION; CATION AB We report measurements of the ionic conductivity, shear viscosity, and structural dynamics in a homologous series of quaternary ammonium ionic liquids (ILs) and a prototypical imidazolium-based IL over a wide range of temperatures down to the glass transition. We find that the ionic conductivity of these materials generally decreases, while the shear viscosity correspondingly increases, with increasing volume fraction of aliphatic side groups. Upon crossing an aliphatic volume fraction of similar to 0.40, we observe a sharp, order-of-magnitude decrease in ionic conductivity and enhancement of viscosity, which coincides with the presence of long-lived, nanometer-sized alkyl aggregates. These strong changes in dynamics are not mirrored in the ionicity of these ILs, which decreases nearly linearly with aliphatic volume fraction. Our results demonstrate that nanophase segregation in neat ILs strongly reduces ionic conductivity primarily due to an aggregation-induced suppression of dynamics. Published by AIP Publishing. C1 [Griffin, Philip J.] Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. [Wang, Yangyang] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Holt, Adam P.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Griffin, PJ (reprint author), Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA.; Sokolov, AP (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Sokolov, AP (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM pgrif@seas.upenn.edu; sokolov@utk.edu RI Wang, Yangyang/A-5925-2010 OI Wang, Yangyang/0000-0001-7042-9804 FU NSF chemistry [CHE-1213444] FX The authors thank NSF chemistry for financial support of this work through Grant No. CHE-1213444. We thank J. Sangoro and V. Novikov for helpful discussions. NR 42 TC 0 Z9 0 U1 10 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 21 PY 2016 VL 144 IS 15 AR 151104 DI 10.1063/1.4947552 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL6YM UT WOS:000375786000006 PM 27389202 ER PT J AU Tolokh, IS Drozdetski, AV Pollack, L Baker, NA Onufriev, AV AF Tolokh, Igor S. Drozdetski, Aleksander V. Pollack, Lois Baker, Nathan A. Onufriev, Alexey V. TI Multi-shell model of ion-induced nucleic acid condensation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID X-RAY-SCATTERING; POISSON-BOLTZMANN EQUATION; HELIX-HELIX INTERACTIONS; MONTE-CARLO-SIMULATION; DOUBLE-STRANDED DNA; MULTIVALENT CATIONS; B-DNA; ELECTROSTATIC CORRELATIONS; POLYELECTROLYTE SOLUTIONS; COUNTERION CONDENSATION AB We present a semi-quantitative model of condensation of short nucleic acid (NA) duplexes induced by trivalent cobalt(III) hexammine (CoHex) ions. The model is based on partitioning of bound counterion distribution around single NA duplex into "external" and "internal" ion binding shells distinguished by the proximity to duplex helical axis. In the aggregated phase the shells overlap, which leads to significantly increased attraction of CoHex ions in these overlaps with the neighboring duplexes. The duplex aggregation free energy is decomposed into attractive and repulsive components in such a way that they can be represented by simple analytical expressions with parameters derived from molecular dynamic simulations and numerical solutions of Poisson equation. The attractive term depends on the fractions of bound ions in the overlapping shells and affinity of CoHex to the "external" shell of nearly neutralized duplex. The repulsive components of the free energy are duplex configurational entropy loss upon the aggregation and the electrostatic repulsion of the duplexes that remains after neutralization by bound CoHex ions. The estimates of the aggregation free energy are consistent with the experimental range of NA duplex condensation propensities, including the unusually poor condensation of RNA structures and subtle sequence effects upon DNA condensation. The model predicts that, in contrast to DNA, RNA duplexes may condense into tighter packed aggregates with a higher degree of duplex neutralization. An appreciable CoHex mediated RNA-RNA attraction requires closer inter-duplex separation to engage CoHex ions (bound mostly in the "internal" shell of RNA) into short-range attractive interactions. The model also predicts that longer NA fragments will condense more readily than shorter ones. The ability of this model to explain experimentally observed trends in NA condensation lends support to proposed NA condensation picture based on the multivalent "ion binding shells." (C) 2016 AIP Publishing LLC. C1 [Tolokh, Igor S.; Onufriev, Alexey V.] Virginia Tech, Dept Comp Sci, Blacksburg, VA 24061 USA. [Drozdetski, Aleksander V.; Onufriev, Alexey V.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Pollack, Lois] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Baker, Nathan A.] Pacific NW Natl Lab, Adv Comp Math & Data Div, Richland, WA 99352 USA. [Baker, Nathan A.] Brown Univ, Div Appl Math, Providence, RI 02912 USA. RP Tolokh, IS (reprint author), Virginia Tech, Dept Comp Sci, Blacksburg, VA 24061 USA. FU National Institutes of Health (NIH) [R01 GM099450] FX This work was supported by the National Institutes of Health (NIH) Grant No. R01 GM099450. NR 86 TC 1 Z9 1 U1 5 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 21 PY 2016 VL 144 IS 15 AR 155101 DI 10.1063/1.4945382 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DL6YM UT WOS:000375786000045 PM 27389241 ER PT J AU Bedoor, S Wuosmaa, AH Albers, M Alcorta, M Almaraz-Calderon, S Back, BB Bertone, PF Deibel, CM Hoffman, CR Lighthall, JC Marley, ST Mcneel, DG Pardo, RC Rehm, KE Schiffer, JP Shetty, DV AF Bedoor, S. Wuosmaa, A. H. Albers, M. Alcorta, M. Almaraz-Calderon, Sergio Back, B. B. Bertone, P. F. Deibel, C. M. Hoffman, C. R. Lighthall, J. C. Marley, S. T. Mcneel, D. G. Pardo, R. C. Rehm, K. E. Schiffer, J. P. Shetty, D. V. TI Structure of C-14 and B-14 from the C-14,C-15(d,He-3)B-13,B-14 reactions SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; 1P SHELL; STATE; BEAMS; HE-3 AB We have studied the C-14,C-15(d,He-3)B-13,B-14 proton-removing reactions in inverse kinematics. The (d,He-3) reaction probes the proton occupation of the target ground state, and also provides spectroscopic information about the final states in B-13,B-14. The experiments were performed using C-14,C-15 beams from the ATLAS accelerator at Argonne National Laboratory. The reaction products were analyzed with the HELIOS device. Angular distributions were obtained for transitions from both reactions. The C-14-beam data reveal transitions to excited states in B-13 that suggest configurations with protons outside the pi(0p(3/2)) orbital, and some possibility of proton cross-shell 0p-1s0d excitations, in the C-14 ground state. The C-15-beam data confirm the existence of a broad 2(-) excited state in B-14. The experimental data are compared to the results of shell-model calculations. C1 [Bedoor, S.; Wuosmaa, A. H.; Lighthall, J. C.; Marley, S. T.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Bedoor, S.; Wuosmaa, A. H.; Mcneel, D. G.] Univ Connecticut, Dept Phys, Storrs, CT 06268 USA. [Albers, M.; Alcorta, M.; Almaraz-Calderon, Sergio; Back, B. B.; Bertone, P. F.; Hoffman, C. R.; Marley, S. T.; Pardo, R. C.; Rehm, K. E.; Schiffer, J. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Deibel, C. M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Shetty, D. V.] Grand Valley State Univ, Dept Phys, Allendale, MI 49401 USA. [Bedoor, S.] Texas A&M Univ, College Stn, TX 77843 USA. [Alcorta, M.; Lighthall, J. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Almaraz-Calderon, Sergio] Florida State Univ, Tallahassee, FL 32306 USA. [Bertone, P. F.] Marshall Space Flight Ctr, Huntsville, AL 35811 USA. [Marley, S. T.] Louisiana State Univ, Baton Rouge, LA 70803 USA. RP Wuosmaa, AH (reprint author), Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA.; Wuosmaa, AH (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06268 USA. EM alan.wuosmaa@uconn.edu FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG02-04ER41320, DE-SC0014552, DE-AC02-06CH11357]; U.S. National Science Foundation [PHY-1068217] FX The authors would like to acknowledge the hard work of the support and operations staff of the ATLAS facility, and thank B. A. Brown for his assistance with the shell-model calculations. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Grants No. DE-FG02-04ER41320, No. DE-SC0014552, and No. DE-AC02-06CH11357, and the U.S. National Science Foundation under Grant No. PHY-1068217. This research used resources of the Argonne National Laboratory ATLAS Accelerator Facility, which is a DOE Office of Science User Facility. NR 32 TC 0 Z9 0 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 21 PY 2016 VL 93 IS 4 AR 044323 DI 10.1103/PhysRevC.93.044323 PG 11 WC Physics, Nuclear SC Physics GA DJ9PW UT WOS:000374546400004 ER PT J AU Binder, S Calci, A Epelbaum, E Furnstahl, RJ Golak, J Hebeler, K Kamada, H Krebs, H Langhammer, J Liebig, S Maris, P Meissner, UG Minossi, D Nogga, A Potter, H Roth, R Skibinski, R Topolnicki, K Vary, JP Witala, H AF Binder, S. Calci, A. Epelbaum, E. Furnstahl, R. J. Golak, J. Hebeler, K. Kamada, H. Krebs, H. Langhammer, J. Liebig, S. Maris, P. Meissner, Ulf-G. Minossi, D. Nogga, A. Potter, H. Roth, R. Skibinski, R. Topolnicki, K. Vary, J. P. Witala, H. CA LENPIC Collaboration TI Few-nucleon systems with state-of-the-art chiral nucleon-nucleon forces SO PHYSICAL REVIEW C LA English DT Article ID TO-LEADING ORDER; CORE-SHELL-MODEL; ATOMS AB We apply improved nucleon-nucleon potentials up to fifth order in chiral effective field theory, along with a new analysis of the theoretical truncation errors to study nucleon-deuteron (Nd) scattering and selected low-energy observables in H-3, He-4, and Li-6. Calculations beyond second order differ from experiment well outside the range of quantified uncertainties, providing truly unambiguous evidence for missing three-nucleon forces within the employed framework. The sizes of the required three-nucleon-force contributions agree well with expectations based on Weinberg's power counting. We identify the energy range in elastic Nd scattering best suited to study three-nucleon-force effects and estimate the achievable accuracy of theoretical predictions for various observables. C1 [Binder, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Binder, S.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Calci, A.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Epelbaum, E.; Krebs, H.] Ruhr Univ Bochum, Inst Theoret Phys 2, D-44780 Bochum, Germany. [Furnstahl, R. J.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Golak, J.; Skibinski, R.; Topolnicki, K.; Witala, H.] Jagiellonian Univ, M Smoluchowski Inst Phys, PL-30348 Krakow, Poland. [Hebeler, K.; Langhammer, J.; Roth, R.] Tech Univ Darmstadt, Inst Kernphys, Petersenstr 30, D-64289 Darmstadt, Germany. [Hebeler, K.] GSI Helmholtzzentrum Schwerionenforsch GmbH, ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Kamada, H.] Kyushu Inst Technol, Dept Phys, Fac Engn, Kitakyushu, Fukuoka 8048550, Japan. [Liebig, S.; Meissner, Ulf-G.; Minossi, D.; Nogga, A.] Forschungszentrum Julich, Inst Kernphys, Inst Adv Simulat, Julich Ctr Hadron Phys, D-52425 Julich, Germany. [Liebig, S.; Meissner, Ulf-G.; Minossi, D.; Nogga, A.] Forschungszentrum Julich, JARA High Performance Comp, D-52425 Julich, Germany. [Maris, P.; Potter, H.; Vary, J. P.] Iowa State Univ Sci & Technol, Dept Phys & Astron, Ames, IA 50011 USA. [Meissner, Ulf-G.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Meissner, Ulf-G.] Univ Bonn, Bethe Ctr Theoret Phys, D-53115 Bonn, Germany. RP Binder, S (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.; Binder, S (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RI Roth, Robert/B-6502-2008 FU AvH Foundation; BMBF [05P15RDFN1, 05P2015 - NUSTAR R D]; DFG [SFB 634, SFB/TR 16]; NSFC [CRC 110]; ERC [259218 NUCLEAREFT, 307986 STRONGINT]; EU (HadronPhysics3) [283286]; HIC for FAIR; Polish National Science Center [DEC-2013/10/M/ST2/00420]; US DOE [DESC0008485, DE-FG-02-87ER40371, DE-SC0006758, DE-SC0008533, DE-AC05-00OR22725]; US NSF [PHY-0904782, PHY-1306250]; Chinese Academy of Sciences (CAS) President's International Fellowship Initiative (PIFI) [2015VMA076] FX This work was performed by the LENPIC collaboration with support from AvH Foundation; BMBF (Contracts No. 05P15RDFN1 and No. 05P2015 - NUSTAR R & D); DFG and NSFC (CRC 110); DFG (SFB 634, SFB/TR 16); ERC projects 259218 NUCLEAREFT and 307986 STRONGINT; EU (HadronPhysics3, Grant 283286); HIC for FAIR; Polish National Science Center DEC-2013/10/M/ST2/00420; US DOE DESC0008485, DE-FG-02-87ER40371, DE-SC0006758, DE-SC0008533, DE-AC05-00OR22725; US NSF PHY-0904782, PHY-1306250. Supercomputer usage included JSC-Julich; PAS0680-Ohio SC; Edison-NERSC. The work of U.G.M. was supported in part by the Chinese Academy of Sciences (CAS) President's International Fellowship Initiative (PIFI) Grant No. 2015VMA076. NR 29 TC 17 Z9 17 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 21 PY 2016 VL 93 IS 4 AR 044002 DI 10.1103/PhysRevC.93.044002 PG 6 WC Physics, Nuclear SC Physics GA DJ9PW UT WOS:000374546400002 ER PT J AU Buckner, MQ Wu, CY Henderson, RA Bucher, B Chyzh, A Bredeweg, TA Baramsai, B Couture, A Jandel, M Mosby, S O'Donnell, JM Ullmann, JL AF Buckner, M. Q. Wu, C. Y. Henderson, R. A. Bucher, B. Chyzh, A. Bredeweg, T. A. Baramsai, B. Couture, A. Jandel, M. Mosby, S. O'Donnell, J. M. Ullmann, J. L. CA DANCE Collaboration TI Absolute measurement of the Pu-242 neutron-capture cross section SO PHYSICAL REVIEW C LA English DT Article ID INDUCED FISSION; NUCLEAR-DATA; NP-237; AM-241; U-235 AB The absolute neutron-capture cross section of Pu-242 was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the Pu-242(n,gamma) cross section was made over the incident neutron energy range from thermal to approximate to 6 keV, and the absolute scale of the (n,gamma) cross section was set according to the known Pu-239(n, f) resonance at E-n,E-R = 7.83 eV. This was accomplished by adding a small quantity of Pu-239 to the Pu-242 sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to approximate to 40 keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII. 1; the Pu-242(n,gamma) cross section at the E-n,E-R = 2.68 eV resonance is within 2.4% of the evaluated value. However, discrepancies exist at higher energies; our data are approximate to 30% lower than the evaluated data at E-n approximate to 1 keV and are approximately 2 sigma away from the previous measurement at E-n approximate to 20 keV. C1 [Buckner, M. Q.; Wu, C. Y.; Henderson, R. A.; Bucher, B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Chyzh, A.] N Carolina State Univ, Raleigh, NC 27695 USA. [Bredeweg, T. A.; Baramsai, B.; Couture, A.; Jandel, M.; Mosby, S.; O'Donnell, J. M.; Ullmann, J. L.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. RP Buckner, MQ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM buckner4@llnl.gov FU US Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; Los Alamos National Security, LLC [DE-AC52-06NA25396]; US DOE/NNSA Office of Defense Nuclear Nonproliferation Research and Development FX This measurement was performed under the auspices of the US Department of Energy by Lawrence Livermore National Security, LLC under Contract No. DE-AC52-07NA27344 and by Los Alamos National Security, LLC under Contract No. DE-AC52-06NA25396. Additional funding was provided by the US DOE/NNSA Office of Defense Nuclear Nonproliferation Research and Development. The isotopes used in the measurement were obtained from Oak Ridge National Laboratory. NR 44 TC 1 Z9 1 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 21 PY 2016 VL 93 IS 4 AR 044613 DI 10.1103/PhysRevC.93.044613 PG 7 WC Physics, Nuclear SC Physics GA DJ9PW UT WOS:000374546400006 ER PT J AU Gupta, YK Garg, U Hoffman, J Matta, J Rao, PVM Patel, D Peach, T Yoshida, K Itoh, M Fujiwara, M Hara, K Hashimoto, H Nakanishi, K Yosoi, M Sakaguchi, H Terashima, S Kishi, S Murakami, T Uchida, M Yasuda, Y Akimune, H Kawabata, T Harakeh, MN AF Gupta, Y. K. Garg, U. Hoffman, J. Matta, J. Rao, P. V. Madhusudhana Patel, D. Peach, T. Yoshida, K. Itoh, M. Fujiwara, M. Hara, K. Hashimoto, H. Nakanishi, K. Yosoi, M. Sakaguchi, H. Terashima, S. Kishi, S. Murakami, T. Uchida, M. Yasuda, Y. Akimune, H. Kawabata, T. Harakeh, M. N. TI Deformation effects on isoscalar giant resonances in Mg-24 SO PHYSICAL REVIEW C LA English DT Article ID INELASTIC ALPHA-SCATTERING; COUPLED-CHANNELS CALCULATIONS; MONOPOLE RESONANCE; DIPOLE RESONANCE; STRENGTH; CA-40; EXCITATION; STATE; NUCLEI; ENERGY AB Strength distributions for isoscalar giant resonances with multipolarity L <= 2 have been determined in Mg-24 from "instrumental background-free" inelastic scattering of 386-MeV alpha particles at extreme forward angles, including 0 degrees. The isoscalar E0, E1, and E2 strengths are observed to be 57 +/- 7%, 111.1(-7.2)(+10.9)%, and 148.6 +/- 7.3%, respectively, of their energy-weighted sum rules in the excitation energy range of 6 to 35 MeV. The isoscalar giant monopole (ISGMR) and quadrupole (ISGQR) resonances exhibit a prominent K splitting which is consistent with microscopic theory for a prolate-deformed ground state of Mg-24. For the ISGQR it is due to splitting of the three K components, whereas for the ISGMR it is due to its coupling to the K = 0 component of the ISGQR. Deformation effects on the isoscalar giant dipole resonance are less pronounced, however. C1 [Gupta, Y. K.; Garg, U.; Hoffman, J.; Matta, J.; Rao, P. V. Madhusudhana; Patel, D.; Peach, T.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Yoshida, K.] Niigata Univ, Grad Sch Sci & Technol, Niigata 9502181, Japan. [Yoshida, K.] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan. [Itoh, M.; Fujiwara, M.; Hara, K.; Hashimoto, H.; Nakanishi, K.; Yosoi, M.] Osaka Univ, Nucl Phys Res Ctr, Osaka 5670047, Japan. [Sakaguchi, H.; Terashima, S.; Kishi, S.; Murakami, T.; Uchida, M.; Yasuda, Y.; Kawabata, T.] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Akimune, H.] Konan Univ, Dept Phys, Kobe, Hyogo 6588501, Japan. [Kawabata, T.] Univ Tokyo, Ctr Nucl Study, Wako, Saitama 3510198, Japan. [Harakeh, M. N.] Univ Groningen, KVI CART, NL-9747 AA Groningen, Netherlands. [Gupta, Y. K.] Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. [Hoffman, J.] Volcano Corp, San Diego, CA 92130 USA. [Matta, J.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37380 USA. [Rao, P. V. Madhusudhana] Andhra Univ, Dept Nucl Phys, Visakhapatnam 530030, Andhra Pradesh, India. [Patel, D.] Univ Texas MD Anderson Canc Ctr, Houston, TX 77030 USA. [Itoh, M.] Tohoku Univ, Ctr Cyclotron & Radioisotope, Sendai, Miyagi 9808578, Japan. [Uchida, M.] Tokyo Inst Technol, Dept Phys, Tokyo 1528850, Japan. RP Gupta, YK (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. RI Yoshida, Kenichi/J-8056-2013 OI Yoshida, Kenichi/0000-0002-4224-1668 FU US National Science Foundation [INT-9910015, PHY04-57120, PHY-1419765]; JSPS KAKENHI [23740223, 25287065] FX The authors acknowledge the efforts of the staff of the RCNP Ring Cyclotron Facility in providing a high-quality, halo-free a beam required for the measurements reported in this paper, and are grateful to Prof. G. Colo for many discussions about the theoretical aspects of this work. This work has been supported in part by the US National Science Foundation (Grants No. INT-9910015, No. PHY04-57120, and No. PHY-1419765), and by the JSPS KAKENHI (Grants No. 23740223 and No. 25287065). The numerical calculations were performed on SR16000 at the Yukawa Institute for Theoretical Physics, Kyoto University. NR 42 TC 1 Z9 1 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 21 PY 2016 VL 93 IS 4 AR 044324 DI 10.1103/PhysRevC.93.044324 PG 7 WC Physics, Nuclear SC Physics GA DJ9PW UT WOS:000374546400005 ER PT J AU Larsen, AC Guttormsen, M Schwengner, R Bleuel, DL Goriely, S Harissopulos, S Garrote, FLB Byun, Y Eriksen, TK Giacoppo, F Gorgen, A Hagen, TW Klintefjord, M Renstrom, T Rose, SJ Sahin, E Siem, S Tornyi, TG Tveten, GM Voinov, AV Wiedeking, M AF Larsen, A. C. Guttormsen, M. Schwengner, R. Bleuel, D. L. Goriely, S. Harissopulos, S. Garrote, F. L. Bello Byun, Y. Eriksen, T. K. Giacoppo, F. Gorgen, A. Hagen, T. W. Klintefjord, M. Renstrom, T. Rose, S. J. Sahin, E. Siem, S. Tornyi, T. G. Tveten, G. M. Voinov, A. V. Wiedeking, M. TI Experimentally constrained (p,gamma)Y-89 and (n,gamma)Y-89 reaction rates relevant to p-process nucleosynthesis SO PHYSICAL REVIEW C LA English DT Article ID PHOTONEUTRON CROSS-SECTIONS; MODEL-CALCULATIONS; STRENGTH FUNCTION; LEVEL DENSITY; ASTROPHYSICS; ELEMENTS; SPECTRA; LIBRARY; NUCLEI; SYSTEM AB The nuclear level density and the gamma-ray strength function have been extracted for Y-89 by using the Oslo method on Y-89(p,p gamma')Y-89 coincidence data. The gamma-ray strength function displays a low-energy enhancement consistent with previous observations in this mass region (Mo93-98). Shell-model calculations support the conclusion that the observed enhancement is due to strong, low-energy M1 transitions at high excitation energies. The data were further used as input for calculations of the Sr-88(p,gamma)Y-89 and Y-88(n,gamma)Y-89 cross sections with the TALYS reaction code. Comparison with cross-section data, where available, as well as with values from the BRUSLIB library, shows a satisfying agreement. C1 [Larsen, A. C.; Guttormsen, M.; Garrote, F. L. Bello; Eriksen, T. K.; Giacoppo, F.; Gorgen, A.; Hagen, T. W.; Klintefjord, M.; Renstrom, T.; Rose, S. J.; Sahin, E.; Siem, S.; Tornyi, T. G.; Tveten, G. M.] Univ Oslo, Dept Phys, POB 1048, N-0316 Oslo, Norway. [Schwengner, R.] Helmholtz Zentrum Dresden Rossendorf, D-01328 Dresden, Germany. [Bleuel, D. L.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Goriely, S.] Univ Libre Bruxelles, Inst Astron & Astrophys, Brussels, Belgium. [Harissopulos, S.] NCSR Demokritos, Inst Nucl & Particle Phys, Athens, Greece. [Byun, Y.; Voinov, A. V.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Wiedeking, M.] IThemba LABS, POB 722, ZA-7129 Somerset West, South Africa. RP Larsen, AC; Guttormsen, M (reprint author), Univ Oslo, Dept Phys, POB 1048, N-0316 Oslo, Norway.; Schwengner, R (reprint author), Helmholtz Zentrum Dresden Rossendorf, D-01328 Dresden, Germany. EM a.c.larsen@fys.uio.no; magne.guttormsen@fys.uio.no; r.schwengner@hzdr.de RI Harissopulos, Sotirios/G-9541-2011; Larsen, Ann-Cecilie/C-8742-2014 OI Harissopulos, Sotirios/0000-0003-4022-7595; Larsen, Ann-Cecilie/0000-0002-2188-3709 FU Research Council of Norway (NFR) [205528, 637686]; NFR [210007]; National Research Foundation of South Africa [92789] FX The authors wish to thank J. C. Muller, E. A. Olsen, A. Semchenkov, and J. Wikne at the Oslo Cyclotron Laboratory for providing excellent experimental conditions. This work was financed in part by the Research Council of Norway (NFR), Project Grant No. 205528, and through the ERC-STG-2014 under Grant Agreement No. 637686. S.G. is an FNRS research associate. S. S. acknowledges financial support from the NFR under Project Grant No. 210007. M.W. acknowledges support by the National Research Foundation of South Africa under Grant No. 92789. NR 62 TC 1 Z9 1 U1 4 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 21 PY 2016 VL 93 IS 4 AR 045810 DI 10.1103/PhysRevC.93.045810 PG 13 WC Physics, Nuclear SC Physics GA DJ9PW UT WOS:000374546400010 ER PT J AU An, FP Balantekin, AB Band, HR Bishai, M Blyth, S Cao, D Cao, GF Cao, J Cen, WR Chan, YL Chang, JF Chang, LC Chang, Y Chen, HS Chen, QY Chen, SM Chen, YX Chen, Y Cheng, JH Cheng, JH Cheng, J Cheng, YP Cheng, ZK Cherwinka, JJ Chu, MC Chukanov, A Cummings, JP de Arcos, J Deng, ZY Ding, XF Ding, YY Diwan, MV Dolgareva, M Dove, J Dwyer, DA Edwards, WR Gill, R Gonchar, M Gong, GH Gong, H Grassi, M Gu, WQ Guan, MY Guo, L Guo, RP Guo, XH Guo, Z Hackenburg, RW Han, R Hans, S He, M Heeger, KM Heng, YK Higuera, A Hor, YK Hsiung, YB Hu, BZ Hu, T Hu, W Huang, EC Huang, HX Huang, XT Huber, P Huo, W Hussain, G Jaffe, DE Jaffke, P Jen, KL Jetter, S Ji, XP Ji, XL Jiao, JB Johnson, RA Joshi, J Kang, L Kettell, SH Kohn, S Kramer, M Kwan, KK Kwok, MW Kwok, T Langford, TJ Lau, K Lebanowski, L Lee, J Lee, JHC Lei, RT Leitner, R Leung, JKC Li, C Li, DJ Li, F Li, GS Li, QJ Li, S Li, SC Li, WD Li, XN Li, YF Li, ZB Liang, H Lin, CJ Lin, GL Lin, S Lin, SK Lin, YC Ling, JJ Link, JM Littenberg, L Littlejohn, BR Liu, DW Liu, JJ Liu, JL Liu, JC Loh, CW Lu, C Lu, HQ Lu, JS Luk, KB Lv, Z Ma, QM Ma, XY Ma, XB Ma, YQ Malyshkin, Y Caicedo, DAM McDonald, KT McKeown, RD Mitchell, I Mooney, M Nakajima, Y Napolitano, J Naumov, D Naumova, E Ngai, HY Ning, Z Ochoa-Ricoux, JP Olshevskiy, A Pan, HR Park, J Patton, S Pec, V Peng, JC Pinsky, L Pun, CSJ Qi, FZ Qi, M Qian, X Raper, N Ren, J Rosero, R Roskovec, B Ruan, XC Steiner, H Sun, GX Sun, JL Tang, W Taychenachev, D Konstantin, T Tsang, KV Tull, CE Viaux, N Viren, B Vorobel, V Wang, CH Wang, M Wang, NY Wang, RG Wang, W Wang, WW Wang, X Wang, YF Wang, Z Wang, Z Wang, ZM Wei, HY Wen, LJ Whisnant, K White, CG Whitehead, L Wise, T Wong, HLH Wong, SCF Worcester, E Wu, CH Wu, Q Xia, DM Xia, JK Xing, ZZ Xu, JY Xu, JL Xu, J Xu, Y Xue, T Yan, J Yang, CG Yang, H Yang, L Yang, MS Yang, MT Ye, M Ye, Z Yeh, M Young, BL Yu, GY Yu, ZY Zhan, L Zhang, C Zhang, HH Zhang, JW Zhang, QM Zhang, XT Zhang, YM Zhang, YX Zhang, YM Zhang, ZJ Zhang, ZY Zhang, ZP Zhao, J Zhao, QW Zhao, YF Zhao, YB Zhong, WL Zhou, L Zhou, N Zhuang, HL Zou, JH AF An, F. P. Balantekin, A. B. Band, H. R. Bishai, M. Blyth, S. Cao, D. Cao, G. F. Cao, J. Cen, W. R. Chan, Y. L. Chang, J. F. Chang, L. C. Chang, Y. Chen, H. S. Chen, Q. Y. Chen, S. M. Chen, Y. X. Chen, Y. Cheng, J. H. Cheng, J. -H. Cheng, J. Cheng, Y. P. Cheng, Z. K. Cherwinka, J. J. Chu, M. C. Chukanov, A. Cummings, J. P. de Arcos, J. Deng, Z. Y. Ding, X. F. Ding, Y. Y. Diwan, M. V. Dolgareva, M. Dove, J. Dwyer, D. A. Edwards, W. R. Gill, R. Gonchar, M. Gong, G. H. Gong, H. Grassi, M. Gu, W. Q. Guan, M. Y. Guo, L. Guo, R. P. Guo, X. H. Guo, Z. Hackenburg, R. W. Han, R. Hans, S. He, M. Heeger, K. M. Heng, Y. K. Higuera, A. Hor, Y. K. Hsiung, Y. B. Hu, B. Z. Hu, T. Hu, W. Huang, E. C. Huang, H. X. Huang, X. T. Huber, P. Huo, W. Hussain, G. Jaffe, D. E. Jaffke, P. Jen, K. L. Jetter, S. Ji, X. P. Ji, X. L. Jiao, J. B. Johnson, R. A. Joshi, J. Kang, L. Kettell, S. H. Kohn, S. Kramer, M. Kwan, K. K. Kwok, M. W. Kwok, T. Langford, T. J. Lau, K. Lebanowski, L. Lee, J. Lee, J. H. C. Lei, R. T. Leitner, R. Leung, J. K. C. Li, C. Li, D. J. Li, F. Li, G. S. Li, Q. J. Li, S. Li, S. C. Li, W. D. Li, X. N. Li, Y. F. Li, Z. B. Liang, H. Lin, C. J. Lin, G. L. Lin, S. Lin, S. K. Lin, Y. -C. Ling, J. J. Link, J. M. Littenberg, L. Littlejohn, B. R. Liu, D. W. Liu, J. J. Liu, J. L. Liu, J. C. Loh, C. W. Lu, C. Lu, H. Q. Lu, J. S. Luk, K. B. Lv, Z. Ma, Q. M. Ma, X. Y. Ma, X. B. Ma, Y. Q. Malyshkin, Y. Caicedo, D. A. Martinez McDonald, K. T. McKeown, R. D. Mitchell, I. Mooney, M. Nakajima, Y. Napolitano, J. Naumov, D. Naumova, E. Ngai, H. Y. Ning, Z. Ochoa-Ricoux, J. P. Olshevskiy, A. Pan, H. -R. Park, J. Patton, S. Pec, V. Peng, J. C. Pinsky, L. Pun, C. S. J. Qi, F. Z. Qi, M. Qian, X. Raper, N. Ren, J. Rosero, R. Roskovec, B. Ruan, X. C. Steiner, H. Sun, G. X. Sun, J. L. Tang, W. Taychenachev, D. Konstantin, T. Tsang, K. V. Tull, C. E. Viaux, N. Viren, B. Vorobel, V. Wang, C. H. Wang, M. Wang, N. Y. Wang, R. G. Wang, W. Wang, W. W. Wang, X. Wang, Y. F. Wang, Z. Wang, Z. Wang, Z. M. Wei, H. Y. Wen, L. J. Whisnant, K. White, C. G. Whitehead, L. Wise, T. Wong, H. L. H. Wong, S. C. F. Worcester, E. Wu, C. -H. Wu, Q. Xia, D. M. Xia, J. K. Xing, Z. Z. Xu, J. Y. Xu, J. L. Xu, J. Xu, Y. Xue, T. Yan, J. Yang, C. G. Yang, H. Yang, L. Yang, M. S. Yang, M. T. Ye, M. Ye, Z. Yeh, M. Young, B. L. Yu, G. Y. Yu, Z. Y. Zhan, L. Zhang, C. Zhang, H. H. Zhang, J. W. Zhang, Q. M. Zhang, X. T. Zhang, Y. M. Zhang, Y. X. Zhang, Y. M. Zhang, Z. J. Zhang, Z. Y. Zhang, Z. P. Zhao, J. Zhao, Q. W. Zhao, Y. F. Zhao, Y. B. Zhong, W. L. Zhou, L. Zhou, N. Zhuang, H. L. Zou, J. H. CA Daya Bay Collaboration TI New measurement of theta(13) via neutron capture on hydrogen at Daya Bay SO PHYSICAL REVIEW D LA English DT Article ID ANTINEUTRINO DETECTORS; LIQUID-SCINTILLATOR; SYSTEM; SENSITIVITY; SEARCH AB This article reports an improved independent measurement of neutrino mixing angle theta(13) at the Daya Bay Reactor Neutrino Experiment. Electron antineutrinos were identified by inverse beta-decays with the emitted neutron captured by hydrogen, yielding a data set with principally distinct uncertainties from that with neutrons captured by gadolinium. With the final two of eight antineutrino detectors installed, this study used 621 days of data including the previously reported 217-day data set with six detectors. The dominant statistical uncertainty was reduced by 49%. Intensive studies of the cosmogenic muon-induced Li-9 and fast neutron backgrounds and the neutron-capture energy selection efficiency, resulted in a reduction of the systematic uncertainty by 26%. The deficit in the detected number of antineutrinos at the far detectors relative to the expected number based on the near detectors yielded sin(2)2 theta(13) = 0.071 +/- 0.011 in the three-neutrino-oscillation framework. The combination of this result with the gadolinium-capture result is also reported. C1 [An, F. P.] E China Univ Sci & Technol, Inst Modern Phys, Shanghai 200237, Peoples R China. [Balantekin, A. B.; Cherwinka, J. J.; Wise, T.] Univ Wisconsin, Madison, WI 53706 USA. [Band, H. R.; Heeger, K. M.; Langford, T. J.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Bishai, M.; Diwan, M. V.; Gill, R.; Hackenburg, R. W.; Hans, S.; Jaffe, D. E.; Joshi, J.; Kettell, S. H.; Littenberg, L.; Mooney, M.; Qian, X.; Rosero, R.; Tang, W.; Viren, B.; Worcester, E.; Yeh, M.; Zhang, C.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Blyth, S.; Hsiung, Y. B.; Hu, B. Z.; Lin, Y. -C.; Pan, H. -R.] Natl Taiwan Univ, Dept Phys, Taipei, Taiwan. [Blyth, S.; Chang, Y.; Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Cao, D.; Loh, C. W.; Qi, M.; Wang, W. W.; Yang, H.; Yu, G. Y.] Nanjing Univ, Nanjing 210008, Jiangsu, Peoples R China. [Cao, G. F.; Cao, J.; Cen, W. R.; Chang, J. F.; Chen, H. S.; Cheng, Y. P.; Deng, Z. Y.; Ding, X. F.; Ding, Y. Y.; Grassi, M.; Guan, M. Y.; Guo, R. P.; He, M.; Heng, Y. K.; Hu, T.; Hu, W.; Jetter, S.; Ji, X. L.; Li, F.; Li, Q. J.; Li, W. D.; Li, X. N.; Li, Y. F.; Liu, J. C.; Lu, H. Q.; Lu, J. S.; Ma, Q. M.; Ma, X. Y.; Ma, Y. Q.; Ning, Z.; Qi, F. Z.; Sun, G. X.; Wang, R. G.; Wang, Y. F.; Wang, Z.; Wang, Z. M.; Wen, L. J.; Xia, D. M.; Xia, J. K.; Xing, Z. Z.; Xu, J. L.; Yang, C. G.; Yang, M. S.; Ye, M.; Yu, Z. Y.; Zhan, L.; Zhang, J. W.; Zhang, X. T.; Zhang, Z. Y.; Zhao, J.; Zhao, Q. W.; Zhao, Y. B.; Zhong, W. L.; Zhou, L.; Zhuang, H. L.; Zou, J. H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Chan, Y. L.; Chu, M. C.; Kwan, K. K.; Kwok, M. W.; Xu, J. Y.] Chinese Univ Hong Kong, Hong Kong, Hong Kong, Peoples R China. [Chang, L. C.; Cheng, J. H.; Cheng, J. -H.; Jen, K. L.; Lin, G. L.; Wu, C. -H.] Natl Chiao Tung Univ, Inst Phys, Hsinchu, Taiwan. [Chen, Q. Y.; Cheng, J.; Huang, X. T.; Jiao, J. B.; Li, C.; Wang, M.; Wu, Q.; Yang, M. T.] Shandong Univ, Jinan 250100, Peoples R China. [Chen, S. M.; Gong, G. H.; Gong, H.; Guo, L.; Guo, Z.; Hussain, G.; Ji, X. P.; Lebanowski, L.; Wang, Z.; Wei, H. Y.; Xue, T.; Zhang, Y. M.] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Chen, Y. X.; Han, R.; Ma, X. B.; Zhao, Y. F.] North China Elect Power Univ, Beijing, Peoples R China. [Chen, Y.] Shenzhen Univ, Shenzhen, Peoples R China. [Cheng, Z. K.; Li, Z. B.; Ling, J. J.; Wang, W.; Wong, S. C. F.; Xu, Y.; Zhang, H. H.; Zhang, Y. M.] Sun Yat Sen Zhongshan Univ, Guangzhou, Guangdong, Peoples R China. [Chukanov, A.; Dolgareva, M.; Gonchar, M.; Naumov, D.; Naumova, E.; Olshevskiy, A.; Taychenachev, D.; Konstantin, T.] Joint Inst Nucl Res, Dubna, Moscow Region, Russia. [Cummings, J. P.] Siena Coll, New York, NY 12211 USA. [de Arcos, J.; Littlejohn, B. R.; Caicedo, D. A. Martinez; White, C. G.] IIT, Dept Phys, Chicago, IL 60616 USA. [Dove, J.; Huang, E. C.; Peng, J. C.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Dwyer, D. A.; Edwards, W. R.; Kramer, M.; Lee, J.; Lin, C. J.; Luk, K. B.; Nakajima, Y.; Patton, S.; Steiner, H.; Tsang, K. V.; Tull, C. E.; Wong, H. L. H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Gu, W. Q.; Li, G. S.; Liu, J. L.] Shanghai Jiao Tong Univ, Shanghai Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Guo, X. H.; Wang, N. Y.; Xu, J.] Beijing Normal Univ, Beijing 100875, Peoples R China. [Higuera, A.; Lau, K.; Lin, S. K.; Liu, D. W.; Mitchell, I.; Pinsky, L.; Whitehead, L.; Ye, Z.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Hor, Y. K.; Huber, P.; Jaffke, P.; Li, S. C.; Link, J. M.; Park, J.] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA 24061 USA. [Huang, H. X.; Ren, J.; Ruan, X. C.] China Inst Atom Energy, Beijing, Peoples R China. [Huo, W.; Li, D. J.; Liang, H.; Zhang, Z. P.; Zhou, N.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Kang, L.; Lei, R. T.; Li, S.; Lin, S.; Yang, L.; Zhang, Z. J.] Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China. [Johnson, R. A.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Kang, L.; Lei, R. T.; Li, S.; Lin, S.; Yang, L.; Zhang, Z. J.] Dongguan Univ Technol, Dongguan, Peoples R China. [Kohn, S.; Kramer, M.; Luk, K. B.; Steiner, H.; Wong, H. L. H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kwok, T.; Lee, J. H. C.; Leung, J. K. C.; Li, S. C.; Liu, J. J.; Ngai, H. Y.; Pun, C. S. J.] Univ Hong Kong, Dept Phys, Pokfulam, Hong Kong, Peoples R China. [Leitner, R.; Pec, V.; Roskovec, B.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Lu, C.; McDonald, K. T.] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. [Lv, Z.; Yan, J.; Zhang, Q. M.] Xi An Jiao Tong Univ, Xian 710049, Peoples R China. [Malyshkin, Y.; Ochoa-Ricoux, J. P.; Viaux, N.] Pontificia Univ Catolica Chile, Inst Fis, Alameda 340, Santiago, Chile. [McKeown, R. D.] CALTECH, Pasadena, CA 91125 USA. [McKeown, R. D.; Wang, W.] Coll William & Mary, Williamsburg, VA 23187 USA. [Napolitano, J.] Temple Univ, Coll Sci & Technol, Dept Phys, Philadelphia, PA 19122 USA. [Raper, N.] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Sun, J. L.; Zhang, Y. X.] China Gen Nucl Power Grp, Shenzhen, Peoples R China. [Wang, X.] Natl Univ Def Technol, Coll Elect Sci & Engn, Changsha, Hunan, Peoples R China. [Whisnant, K.; Young, B. L.] Iowa State Univ, Ames, IA 50011 USA. [Xia, D. M.] Chongqing Univ, Chongqing 630044, Peoples R China. RP An, FP (reprint author), E China Univ Sci & Technol, Inst Modern Phys, Shanghai 200237, Peoples R China. RI Link, Jonathan/L-2560-2013; Ling, Jiajie/I-9173-2014; Wei, Hanyu/D-7291-2017; OI Link, Jonathan/0000-0002-1514-0650; Ling, Jiajie/0000-0003-2982-0670; Wei, Hanyu/0000-0003-1973-4912; HSIUNG, YEE/0000-0003-4801-1238; Lebanowski, Logan/0000-0002-8255-6613; Qian, Xin/0000-0002-7903-7935; Zhang, Chao/0000-0003-2298-6272; Grassi, Marco/0000-0003-2422-6736; Ochoa-Ricoux, Juan Pedro/0000-0001-7376-5555 FU Ministry of Science and Technology of China; United States Department of Energy; Chinese Academy of Sciences; CAS Center for Excellence in Particle Physics; National Natural Science Foundation of China; Guangdong provincial government; Shenzhen municipal government; China General Nuclear Power Group; Key Laboratory of Particle & Radiation Imaging (Tsinghua University), Ministry of Education; Key Laboratory of Particle Physics and Particle Irradiation (Shandong University), Ministry of Education; Research Grants Council of the Hong Kong Special Administrative Region of China; MOST fund from Taiwan; U.S. National Science Foundation; Ministry of Education, Youth and Sports of the Czech Republic; Joint Institute of Nuclear Research in Dubna, Russia; NSFC-RFBR joint research program; National Commission for Scientific and Technological Research of Chile; Tsinghua University Initiative Scientific Research Program FX The Daya Bay Experiment is supported in part by the Ministry of Science and Technology of China, the United States Department of Energy, the Chinese Academy of Sciences, the CAS Center for Excellence in Particle Physics, the National Natural Science Foundation of China, the Guangdong provincial government, the Shenzhen municipal government, the China General Nuclear Power Group, the Key Laboratory of Particle & Radiation Imaging (Tsinghua University), Ministry of Education, the Key Laboratory of Particle Physics and Particle Irradiation (Shandong University), Ministry of Education, the Research Grants Council of the Hong Kong Special Administrative Region of China, the MOST fund support from Taiwan, the U.S. National Science Foundation, the Ministry of Education, Youth and Sports of the Czech Republic, the Joint Institute of Nuclear Research in Dubna, Russia, the NSFC-RFBR joint research program, the National Commission for Scientific and Technological Research of Chile, and the Tsinghua University Initiative Scientific Research Program. We acknowledge Yellow River Engineering Consulting Co., Ltd. and China Railway 15th Bureau Group Co., Ltd. for building the underground laboratory. We are grateful for the ongoing cooperation from the China Guangdong Nuclear Power Group and China Light & Power Company. NR 65 TC 5 Z9 5 U1 18 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 21 PY 2016 VL 93 IS 7 AR 072011 DI 10.1103/PhysRevD.93.072011 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QP UT WOS:000374548300002 ER PT J AU Grohs, E Fuller, GM Kishimoto, CT Paris, MW Vlasenko, A AF Grohs, E. Fuller, G. M. Kishimoto, C. T. Paris, M. W. Vlasenko, A. TI Neutrino energy transport in weak decoupling and big bang nucleosynthesis SO PHYSICAL REVIEW D LA English DT Article ID EARLY UNIVERSE; PRIMORDIAL NUCLEOSYNTHESIS; HIGH-TEMPERATURES; NONEQUILIBRIUM CORRECTIONS; MASSLESS NEUTRINOS; DEUTERIUM; ELEMENTS; SPECTRA; OSCILLATIONS; SUPERNOVAE AB We calculate the evolution of the early universe through the epochs of weak decoupling, weak freeze-out and big bang nucleosynthesis (BBN) by simultaneously coupling a full strong, electromagnetic, and weak nuclear reaction network with a multienergy group Boltzmann neutrino energy transport scheme. The modular structure of our code provides the ability to dissect the relative contributions of each process responsible for evolving the dynamics of the early universe in the absence of neutrino flavor oscillations. Such an approach allows a detailed accounting of the evolution of the nu(e), (nu) over bar (e), nu(mu), (nu) over bar (mu), nu(tau), (nu) over bar (tau) energy distribution functions alongside and self-consistently with the nuclear reactions and entropy/heat generation and flow between the neutrino and photon/electron/positron/baryon plasma components. This calculation reveals nonlinear feedback in the time evolution of neutrino distribution functions and plasma thermodynamic conditions (e.g., electron-positron pair densities), with implications for the phasing between scale factor and plasma temperature; the neutron-to-proton ratio; light-element abundance histories; and the cosmological parameter N-eff. We find that our approach of following the time development of neutrino spectral distortions and concomitant entropy production and extraction from the plasma results in changes in the computed value of the BBN deuterium yield. For example, for particular implementations of quantum corrections in plasma thermodynamics, our calculations show a 0.4% increase in deuterium. These changes are potentially significant in the context of anticipated improvements in observational and nuclear physics uncertainties. C1 [Grohs, E.; Fuller, G. M.; Kishimoto, C. T.; Vlasenko, A.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Grohs, E.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Kishimoto, C. T.] Univ San Diego, Dept Phys & Biophys, San Diego, CA 92110 USA. [Paris, M. W.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Vlasenko, A.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. RP Grohs, E (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA.; Grohs, E (reprint author), Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. EM egrohs@umich.edu OI Paris, Mark/0000-0003-0471-7896 FU NSF [PHY-1307372]; Los Alamos National Laboratory Institute for Geophysics, Space Sciences and Signatures [257842]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396] FX We thank Fred Adams, Eve Armstrong, Kam Arnold, Daniel Blaschke, Lowell Brown, John Carlstrom, John Cherry, Vincenzo Cirigliano, Scott Dodelson, Lauren Gilbert, Luke Johns, Brian Keating, Lloyd Knox, Adrian Lee, Eric Michelsen, Ken Nollett, Amol Patwardhan, Shashank Shalgar, Meir Shimon, Gary Steigman, Mike Turner, and Nicole Vassh for useful conversations with respect to cosmology, neutrino physics, nuclear physics, plasma physics, Fortran 90, and parallel computing. This work was supported in part by NSF Grant No. PHY-1307372 at UC San Diego. This work was supported also by the Los Alamos National Laboratory Institute for Geophysics, Space Sciences and Signatures Subcontract No. 257842. This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. We thank the anonymous referee for their useful comments. NR 65 TC 6 Z9 6 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 21 PY 2016 VL 93 IS 8 AR 083522 DI 10.1103/PhysRevD.93.083522 PG 34 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9SB UT WOS:000374552100001 ER PT J AU Quintero, NR Mertens, FG Efimov, A Bishop, AR AF Quintero, Niurka R. Mertens, Franz G. Efimov, Anatoly Bishop, A. R. TI Soliton dynamics in optical fibers using the generalized traveling-wave method SO PHYSICAL REVIEW E LA English DT Article ID MOMENT METHOD; EXCITATIONS; RESONANCES; VORTICES; SYSTEMS AB The generalized traveling wave method (GTWM) is applied to the nonlinear Schrodinger (NLS) equation with general perturbations in order to obtain the equations of motion for an ansatz with six collective coordinates, namely the soliton position, the amplitude, the inverse of the soliton width, the velocity, the chirp, and the phase. The advantage of the new ansatz is that it yields three pairs of canonically conjugated coordinates and momenta that all are well-behaved. The new ansatz is applied to model the dynamics of a soliton in a dispersion-shifted optical fiber described by the generalized NLS, including dissipation, higher-order dispersion, Raman scattering, and self-steepening perturbations. It is shown that the GTWM is equivalent to the modified method of moments, which considers the time variation of the norm, the first and the second moment of the norm, the momentum, the first moment of the momentum, and the energy for the perturbed NLS equation. C1 [Quintero, Niurka R.] Univ Seville, EPS, Dept Fis Aplicada 1, Virgen Africa 7, E-41011 Seville, Spain. [Mertens, Franz G.] Univ Bayreuth, Inst Phys, D-95440 Bayreuth, Germany. [Efimov, Anatoly; Bishop, A. R.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Quintero, NR (reprint author), Univ Seville, EPS, Dept Fis Aplicada 1, Virgen Africa 7, E-41011 Seville, Spain. EM niurka@us.es RI Quintero, Niurka/J-7550-2013; OI Quintero, Niurka/0000-0003-3503-3040; Efimov, Anatoly/0000-0002-5559-4147 FU United States Department of Energy; Alexander von Humboldt Foundation (Germany) [SPA 1146358 STP]; MICINN (Spain) [FIS2014-54497-P]; Plan Propio of the University of Seville FX This work was performed in part under the auspices of the United States Department of Energy and at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences (USA) user facility. The authors thank the Santa Fe Institute for its hospitality during the completion of this work. N.R.Q. acknowledges financial support from the Alexander von Humboldt Foundation (Germany) through Research Fellowship for Experienced Researchers SPA 1146358 STP and by the MICINN (Spain) through Grant No. FIS2014-54497-P. F.G.M. acknowledges the hospitality of the Mathematical Institute of the University of Seville (IMUS) and of the Theoretical Division and Center for Nonlinear Studies at Los Alamos National Laboratory, and financial support by the Plan Propio of the University of Seville. NR 27 TC 0 Z9 0 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 21 PY 2016 VL 93 IS 4 AR 042214 DI 10.1103/PhysRevE.93.042214 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DJ9ST UT WOS:000374553900005 PM 27176300 ER PT J AU Zhang, C AF Zhang, Cen TI Single Top Production at Next-to-Leading Order in the Standard Model Effective Field Theory SO PHYSICAL REVIEW LETTERS LA English DT Article ID LOW-ENERGY MANIFESTATIONS; QUARK WIDTH; SEARCH AB Single top production processes at hadron colliders provide information on the relation between the top quark and the electroweak sector of the standard model. We compute the next-to-leading order QCD corrections to the three main production channels: t-channel, s-channel, and tW associated production, in the standard model including operators up to dimension six. The calculation can be matched to parton shower programs and can therefore be directly used in experimental analyses. The QCD corrections are found to significantly impact the extraction of the current limits on the operators, because both of an improved accuracy and a better precision of the theoretical predictions. In addition, the distributions of some of the key discriminating observables are modified in a nontrivial way, which could change the interpretation of measurements in terms of UV complete models. C1 [Zhang, Cen] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Zhang, C (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. FU U.S. Department of Energy [DE-SC0012704] FX I am grateful for valuable discussions with S. Dawson and M. Selvaggi. This work is supported by U.S. Department of Energy under Grant No. DE-SC0012704. NR 62 TC 6 Z9 6 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 21 PY 2016 VL 116 IS 16 AR 162002 DI 10.1103/PhysRevLett.116.162002 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ9UY UT WOS:000374559700008 PM 27152795 ER PT J AU Yang, QW Wang, ZP Bao, ZB Zhang, ZG Yang, YW Ren, QL Xing, HB Dai, S AF Yang, Qiwei Wang, Zhiping Bao, Zongbi Zhang, Zhiguo Yang, Yiwen Ren, Qilong Xing, Huabin Dai, Sheng TI New Insights into CO2 Absorption Mechanisms with Amino-Acid Ionic Liquids SO CHEMSUSCHEM LA English DT Article DE absorption; amine; capture; carbon dioxide; ionic liquids ID CARBON-DIOXIDE CAPTURE; METAL-ORGANIC FRAMEWORKS; CARBAMIC ACID; FLUE-GAS; TEMPERATURE; ADSORPTION; ANION; SOLUBILITY; SEPARATION; BASICITY AB The last decade saw an explosion of interest in using amine-functionalized materials for CO2 capture and conversion, and it is of great importance to elucidate the relationship between the molecular structure of amine-functionalized materials and their CO2 capacity. In this work, based on a new quantitative analysis method for the CO2 absorption mechanism of amino-acid ionic liquids (ILs) and quantum chemical calculations, we show that the small difference in the local structure of amine groups in ILs could lead to much different CO2 absorption mechanisms, which provides an opportunity for achieving higher CO2 capacity by structure design. This work revealed that the actual CO2 absorption mechanism by amino-acid ILs goes beyond the apparent CO2/amine stoichiometry; a rigid ring structure around the amine group in ILs creates a unique electrostatic environment that inhibits the deprotonation of carbamic acid and enables actually equimolar CO2/amine absorption. C1 [Yang, Qiwei; Wang, Zhiping; Bao, Zongbi; Zhang, Zhiguo; Yang, Yiwen; Ren, Qilong; Xing, Huabin] Zhejiang Univ, Key Lab Biomass Chem Engn, Minist Educ, Coll Chem & Biol Engn, Hangzhou 310027, Zhejiang, Peoples R China. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37966 USA. RP Xing, HB (reprint author), Zhejiang Univ, Key Lab Biomass Chem Engn, Minist Educ, Coll Chem & Biol Engn, Hangzhou 310027, Zhejiang, Peoples R China. EM xinghb@zju.edu.cn RI Dai, Sheng/K-8411-2015; OI Dai, Sheng/0000-0002-8046-3931; Yang, Qiwei/0000-0002-6469-5126 FU National Natural Science Foundation of China [21222601, 21476192, 21436010]; Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the National Natural Science Foundation of China (21222601, 21476192 and 21436010). S.D. was supported by the Office of Basic Energy Sciences, U.S. Department of Energy. NR 53 TC 4 Z9 4 U1 30 U2 89 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD APR 21 PY 2016 VL 9 IS 8 BP 806 EP 812 DI 10.1002/cssc.201501691 PG 7 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DK7NX UT WOS:000375113800006 PM 27061812 ER PT J AU DiFranzo, A Fox, PJ Tait, TMP AF DiFranzo, Anthony Fox, Patrick J. Tait, Tim M. P. TI Vector Dark Matter through a radiative Higgs Portal SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Cosmology of Theories beyond the SM; Higgs Physics ID MASS-DEGENERATE; SEARCH; CHARGINOS; MODEL AB We study a model of spin-1 dark matter which interacts with the Standard Model predominantly via exchange of Higgs bosons. We propose an alternative UV completion to the usual Vector Dark Matter Higgs Portal, in which vector-like fermions charged under SU(2)(w) x U(1)(Y) and under the dark gauge group, U(1)', generate an effective interaction between the Higgs and the dark matter at one loop. We explore the resulting phenomenology and show that this dark matter candidate is a viable thermal relic and satisfies Higgs invisible width constraints as well as direct detection bounds. C1 [DiFranzo, Anthony; Tait, Tim M. P.] Univ Calif Irvine, Dept Phys & Astron, 4129 Frederick Reines Hall, Irvine, CA 92697 USA. [DiFranzo, Anthony; Fox, Patrick J.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. RP DiFranzo, A; Tait, TMP (reprint author), Univ Calif Irvine, Dept Phys & Astron, 4129 Frederick Reines Hall, Irvine, CA 92697 USA.; DiFranzo, A; Fox, PJ (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. EM adifranz@uci.edu; pjfox@fnal.gov; ttait@uci.edu OI DiFranzo, Anthony/0000-0002-3151-9150 FU Fermilab Graduate Student Research Program in Theoretical Physics; NSF [PHY-1316792]; United States Department of Energy [DE-AC02-07CH11359]; University of California, Irvine through a Chancellor's Fellowship FX AD is supported by the Fermilab Graduate Student Research Program in Theoretical Physics and in part by NSF Grant No. PHY-1316792. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. The work of TMPT is supported in part by NSF grant PHY-1316792 and by the University of California, Irvine through a Chancellor's Fellowship. NR 33 TC 4 Z9 4 U1 1 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 21 PY 2016 IS 4 AR 135 DI 10.1007/JHEP04(2016)135 PG 17 WC Physics, Particles & Fields SC Physics GA DK4SH UT WOS:000374908900001 ER PT J AU Goldstein, S Behar, D Rajh, T Rabani, J AF Goldstein, Sara Behar, David Rajh, Tijana Rabani, Joseph TI Nitrite Reduction to Nitrous Oxide and Ammonia by TiO2 Electrons in a Colloid Solution via Consecutive One-Electron Transfer Reactions SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SELECTIVE PHOTOCATALYTIC REDUCTION; AQUEOUS SUSPENSION; PULSE-RADIOLYSIS; NITRATE; PARTICLES; ACID AB The mechanism of nitrite reduction by excess electrons on TiO2 nanoparticles (e(TiO2)(-)), was studied under anaerobic conditions. TiO2 was loaded with up to 75 electrons per particle, induced by gamma-irradiation of acidic TiO2 colloid solutions containing 2-propanol. Time-resolved kinetics and material analysis were performed, mostly at 1.66 g L-1 TiO2. At relatively low nitrite concentrations (R = [e(TiO2)(-)](o)/[nitrite](o) > 1.5), e(TiO2)(-) decays via two consecutive processes; at higher concentrations, only one decay step is observed. The stoichiometric ratio Delta[e(TiO2)(-)](o)/[nitrite](o) of the faster process is about 2. This process involves the one-electron reduction of nitrite, forming the nitrite radical (k(1) = (2.0 +/- 0.2) X 10(6) M-1 s(-1)), which further reacts with e(TiO2)(-) (k(2)) in competition with its dehydration to nitric oxide (NO) (k(3)). The ratios k(2)/k(3) = (3.0 +/- 0.5) X 10(3) M-1 and k(2) > 1 x 10(6) M-1 s(-1) were derived from kinetic simulations and product analysis. The major product of this process is NO. The slower stage of the kinetics involves the reduction of NO by e(TiO2)(-), and the detailed mechanism of this process has been discussed in our earlier publication. The results reported in this study suggest that several intermediates, including NO and NH2OH, are adsorbed on the titanium nanoparticles and give rise to inverse dependency of the respective reaction rates on the TiO2 concentration. It is demonstrated that the reduction of nitrite by e(TiO2)(-), yields mainly N2O and NH3 via consecutive one-electron transfer reactions. C1 [Goldstein, Sara; Behar, David; Rabani, Joseph] Hebrew Univ Jerusalem, Inst Chem, Edmond Safra Campus, IL-91904 Jerusalem, Israel. [Goldstein, Sara; Behar, David; Rabani, Joseph] Hebrew Univ Jerusalem, Accelerator Lab, Edmond Safra Campus, IL-91904 Jerusalem, Israel. [Rajh, Tijana] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Rabani, J (reprint author), Hebrew Univ Jerusalem, Inst Chem, Edmond Safra Campus, IL-91904 Jerusalem, Israel.; Rabani, J (reprint author), Hebrew Univ Jerusalem, Accelerator Lab, Edmond Safra Campus, IL-91904 Jerusalem, Israel. EM rabani@mail.huji.ac.il FU US-Israel BSF [2012158] FX This work was generously supported by the US-Israel BSF under Contract 2012158. NR 23 TC 2 Z9 2 U1 13 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 21 PY 2016 VL 120 IS 15 BP 2307 EP 2312 DI 10.1021/acs.jpca.6b01761 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK3IX UT WOS:000374811400004 PM 27050805 ER PT J AU Hou, GL Valiev, M Wang, XB AF Hou, Gao-Lei Valiev, Marat Wang, Xue-Bin TI Deprotonated Dicarboxylic Acid Homodimers: Hydrogen Bonds and Atmospheric Implications SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID AEROSOL NUCLEATION PRECURSORS; SECONDARY ORGANIC AEROSOL; PHOTOELECTRON-SPECTROSCOPY; PARTICLE FORMATION; EVAPORATION RATES; BISULFATE ANION; AB-INITIO; CLUSTERS; ENERGIES; WATER AB Dicarboxylic acids represent an important class of water-soluble organic compounds found in the atmosphere. In this work we are studying properties of dicarboxylic acid homodimer complexes (HO2C(CH2)(n)CO2-[HO2C-(CH2)(n)CO2H], n = 0-12), as potentially important intermediates in aerosol formation processes. Our approach is based on experimental data from negative ion photoelectron spectra of the dimer complexes combined with updated measurements of the corresponding monomer species. These results are analyzed with quantum-mechanical calculations, which provide further information about equilibrium structures, thermochemical parameters associated with the complex formation, and evaporation rates. We find that upon formation of the dimer complexes the electron binding energies increase by 1.3-1.7 eV (30.0-39.2 kcal/mol), indicating increased stability of the dimerized complexes. Calculations indicate that these dimer complexes are characterized by the presence of strong intermolecular hydrogen bonds with high binding energies and are thermodynamically favorable to form with low evaporation rates. Comparison with the previously studied HSO4-[HO2C(CH2)(2)CO2H] complex (J. Phys. Chem. Lett. 2013, 4, 779-785) shows that HO2C(CH2)(2)CO2-[HO2C-(CH2)(2)CO2H] has very similar thermochemical properties. These results imply that dicarboxylic acids not only can contribute to the heterogeneous complexes formation involving sulfuric acid and dicarboxylic acids but also can promote the formation of homogeneous complexes by involving dicarboxylic acids themselves. C1 [Hou, Gao-Lei; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. [Valiev, Marat] Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. RP Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA.; Valiev, M (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd,POB 999, Richland, WA 99352 USA. EM marat.valiev@pnnl.gov; xuebin.wang@pnnl.gov FU EMSL Intramural Aerosol Science Theme Funding; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE's Office of Biological and Environmental Research FX This work was supported by EMSL Intramural Aerosol Science Theme Funding, and by U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, and performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle Memorial Institute for the DOE. The theoretical calculations were conducted on the ScGrid and DeepComp 7000 of the Supercomputing Center, Computer Network Information Center of Chinese Academy of Sciences, as well as on the EMSL Cascade Supercomputer. NR 54 TC 2 Z9 2 U1 7 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 21 PY 2016 VL 120 IS 15 BP 2342 EP 2349 DI 10.1021/acs.jpca.6b01166 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK3IX UT WOS:000374811400008 PM 27032015 ER PT J AU Matanovic, I Babanova, S Chavez, MS Atanassov, P AF Matanovic, Ivana Babanova, Sofia Chavez, Madelaine Seow Atanassov, Plamen TI Protein-Support Interactions for Rationally Designed Bilirubin Oxidase Based Cathode: A Computational Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID DIRECT ELECTRON-TRANSFER; INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; CARBON NANOTUBES; COPPER OXIDASE; BIOFUEL CELLS; ENZYME; REDUCTION; LACCASE; IMMOBILIZATION AB An example of biocathode based on bilirubin oxidase (BOx) was used to demonstrate how density functional theory can be combined with docking simulations in order to study the interface interactions between the enzyme and specifically designed electrode surface. The electrode surface was modified through the adsorption of bilirubin, the natural substrate for BOx, and the prepared electrode was electrochemically characterized using potentiostatic measurements. The experimentally determined current densities showed that the presence of bilirubin led to significant improvement of the cathode operation. On the basis of the computationally calculated binding energies of bilirubin to the graphene support and BOx and the analysis of the positioning of bilirubin relative to the support and T1 Cu atom of the enzyme, we hypothesize that the bilirubin serves as a geometric and electronic extension of the support. The computational results further confirm that the modification of the electrode surface with bilirubin provides an optimal orientation of BOx toward the support but also show that bilirubin facilitates the interfacial electron transfer by decreasing the distance between the electrode surface and the T1 Cu atom. C1 [Matanovic, Ivana; Babanova, Sofia; Chavez, Madelaine Seow; Atanassov, Plamen] Univ New Mexico, Dept Chem & Biol Engn, CMEM, Albuquerque, NM 87131 USA. [Matanovic, Ivana] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Babanova, Sofia] J Craig Venter Inst, La Jolla, CA 92037 USA. RP Atanassov, P (reprint author), Univ New Mexico, Dept Chem & Biol Engn, CMEM, Albuquerque, NM 87131 USA. EM plamen@unm.edu FU US DOD, ARO-Multi-University Research Initiative [W911NF-14-1-0263]; Office of Science of the U.S. Department of Energy [DE-AC52-06NA25396, DE-AC02-05CH1123]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; NERSC FX This work was supported by US DOD, ARO-Multi-University Research Initiative Grant W911NF-14-1-0263 to University of Utah. VASP license was provided by Theoretical division, LANL, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC52-06NA25396. Computational work was performed using the computational resources of LANL, CNMS, sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy and NERSC, supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH1123. This paper has been designated LA-UR-16-20777. NR 41 TC 2 Z9 2 U1 14 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD APR 21 PY 2016 VL 120 IS 15 BP 3634 EP 3641 DI 10.1021/acs.jpcb.6b01616 PG 8 WC Chemistry, Physical SC Chemistry GA DK3IY UT WOS:000374811500005 PM 27015361 ER PT J AU Deng, XY Sorescu, DC Lee, J AF Deng, Xingyi Sorescu, Dan C. Lee, Junseok TI D2O Interaction with Planar ZnO(0001) Bilayer Supported on Au(111): Structures, Energetics and Influence of Hydroxyls SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; ALUMINUM-OXIDE OVERLAYER; SINGLE-CRYSTAL SURFACES; GAS SHIFT REACTION; WAVE BASIS-SET; WATER-ADSORPTION; LEED CRYSTALLOGRAPHY; METHANOL SYNTHESIS; REACTION-MECHANISM; CU/ZNO CATALYSTS AB We investigate the interaction between D2O and the planar ZnO(0001) bilayer grown on Au(111) with temperature programmed desorption (TPD), low energy electron diffraction (LEED), X-ray photoelectron spectroscopy (XPS), and density functional theory (DFT) calculations. We show that D2O molecules adsorbed on this planar surface form two ordered overlayers, a (3 X 3) and a (root 3 X root 3)R30 degrees, not seen before on any of the bulk ZnO single crystal surfaces. The apparent activation energies of desorption (E-d) estimated from TPD peaks are 15.2 and 16.7-17.3 kcal/mol for (3 X 3) and (root 3 X root 3)R30 degrees, respectively, which agree well with the adsorption energy values calculated from DFT (14.9-15.6 kcal/mol and 16.8-16.9 kcal/mol, respectively). The DFT calculations reveal that the formation of the overlayers takes place at different packing densities and is mediated by extensive hydrogen bonding among the molecules. The hydroxyl groups, which accumulate very slowly on the ZnO(0001) bilayer surface under the standard ultrahigh vacuum (UHV) environment, strongly suppress the formation of the (root 3 X root 3)R30 degrees overlayer but have less impact on the (3 X 3) overlayer. These findings are explained based on the difference in packing densities of the overlayers such that only the (3 X 3) overlayer with a more open structure can accommodate small amounts of the adsorbed hydroxyl groups. C1 [Deng, Xingyi; Sorescu, Dan C.; Lee, Junseok] US DOE, NETL, POB 10940, Pittsburgh, PA 15236 USA. [Deng, Xingyi; Lee, Junseok] AECOM, POB 618, South Park, PA 15129 USA. RP Deng, XY (reprint author), US DOE, NETL, POB 10940, Pittsburgh, PA 15236 USA.; Deng, XY (reprint author), AECOM, POB 618, South Park, PA 15129 USA. EM xingyi.deng@netl.doe.gov OI Deng, Xingyi/0000-0001-9109-1443 FU National Energy Technology Laboratory's ongoing research under the RES [DE-FE0004000]; agency of the United States Government FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES Contract DE-FE0004000. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 61 TC 2 Z9 2 U1 16 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 21 PY 2016 VL 120 IS 15 BP 8157 EP 8166 DI 10.1021/acs.jpcc.6b00862 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DK3IU UT WOS:000374811100028 ER PT J AU Eren, B Liu, ZY Stacchiola, D Somorjai, GA Salmeron, M AF Eren, Baran Liu, Zongyuan Stacchiola, Dario Somorjai, Gabor A. Salmeron, Miquel TI Structural Changes of Cu(110) and Cu(110)-(2 x 1)-O Surfaces under Carbon Monoxide in the Torr Pressure Range Studied with Scanning Tunneling Microscopy and Infrared Reflection Absorption Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; CO OXIDATION; IN-SITU; PREADSORBED OXYGEN; AMBIENT CONDITIONS; METHANOL SYNTHESIS; ADSORPTION STATES; COPPER; SCIENCE; TEMPERATURES AB The atomic structure of the clean Cu(110) and the oxygen covered Cu(110) surfaces in the presence of carbon monoxide (CO) gas in the Torr pressure range at 298 K is studied using scanning tunneling microscopy (STM) and infrared reflection adsorption spectroscopy (IRRAS). We found that the initially clean surface reconstructs to form short rows of Cu atoms along the [1-10] direction separated by missing rows. The adsorbed CO molecules show two different C-O stretch vibration modes originating from molecules bound to Cu atoms with different coordination numbers, in the middle and at the end of the atomic rows. On the oxygen covered p(2 X 1) surface, adsorbed CO is observed only after removal of surface O atoms by reaction with CO. In the presence of 1:5 and 1:1 mixtures of O-2 and CO at 298 K, the p(2 X 1)-O reconstructed surface transforms into Cu2O, instead of reducing to metallic Cu. C1 [Eren, Baran; Somorjai, Gabor A.; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Liu, Zongyuan] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Stacchiola, Dario] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Stacchiola, D (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Salmeron, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM djs@bnl.gov; mbsalmeron@lbl.gov RI Eren, Baran/A-9644-2013; Stacchiola, Dario/B-1918-2009 OI Stacchiola, Dario/0000-0001-5494-3205 FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program [DE-AC02-05CH11231, FWP KC3101]; Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Basic Energy Science [DE-SC0012704] FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures program (FWP KC3101). The APXPS experiments were carried out at BL11.0.2 of the Advanced Light Source, which is supported by the Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. The IRRAS work at BNL was financed by the U.S. Department of Energy, Office of Basic Energy Science (DE-SC0012704). NR 39 TC 2 Z9 2 U1 9 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 21 PY 2016 VL 120 IS 15 BP 8227 EP 8231 DI 10.1021/acs.jpcc.6b02143 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DK3IU UT WOS:000374811100036 ER PT J AU Zhong, JQ Kestell, J Waluyo, I Wilkins, S Mazzoli, C Barbour, A Kaznatcheev, K Shete, M Tsapatsis, M Boscoboinik, JA AF Zhong, Jian-Qiang Kestell, John Waluyo, Iradwikanari Wilkins, Stuart Mazzoli, Claudio Barbour, Andi Kaznatcheev, Konstantine Shete, Meera Tsapatsis, Michael Boscoboinik, J. Anibal TI Oxidation and Reduction under Cover: Chemistry at the Confined Space between Ultrathin Nanoporous Silicates and Ru(0001) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MFI ZEOLITE NANOSHEETS; INDUCED RECONSTRUCTION; ALUMINOSILICATE FILMS; LAYER GRAPHENE; CO ADSORPTION; SURFACE; OXYGEN; BILAYER; ORIGIN; GROWTH AB The oxidation and reduction of Ru(0001) surfaces at the confined space between two-dimensional nanoporous silica frameworks and Ru(0001) have been investigated using synchrotron-based ambient pressure X-ray photoelectron spectroscopy (AP-XPS). The porous nature of the frameworks and the weak interaction between the silica and the ruthenium substrate allow oxygen and hydrogen molecules to go through the nanopores and react with the metal at the interface between the silica framework and the metal surface. In this work, three types of two-dimensional silica frameworks have been used to study their influence in the oxidation and reduction of the ruthenium surface at elevated pressures and temperatures. These frameworks are bilayer silica (0.5 nm thick), bilayer aluminosilicate (0.5 um thick), and zeolite MFI nanosheets (3 nm thick). It is found that the silica frameworks stay essentially intact under these conditions, but they strongly affect the oxidation of ruthenium, with the 0.5 nm thick aluminosilicate bilayer completely inhibiting the oxidation. The latter is believed to be related to the lower chemisorbed oxygen content arising from electrostatic interactions between the negatively charged aluminosilicate framework and the Ru(0001) substrate. C1 [Zhong, Jian-Qiang; Kestell, John; Boscoboinik, J. Anibal] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Waluyo, Iradwikanari; Wilkins, Stuart; Mazzoli, Claudio; Barbour, Andi; Kaznatcheev, Konstantine] Brookhaven Natl Lab, Photon Sci Div, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Shete, Meera; Tsapatsis, Michael] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. RP Boscoboinik, JA (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM jboscoboinik@bnl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704]; Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - US Department of Energy, Office of Science, Basic Energy Sciences [DE-SC000105]; BNL LDRD Project [15-010] FX Research carried out in part at the Center for Functional Nanomaterials and beamline 23-ID-2 (CSX-2) at the National Synchrotron Light Source II, Brookhaven National Laboratory, which are supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-SC0012704. MFI nanosheet preparation was supported from the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences under Award DE-SC000105. J.Z. is supported by BNL LDRD Project No. 15-010. We gratefully acknowledge the support from Kazimierz G., Larry F., Steve B., and Andrew M. at NSLS-II. NR 34 TC 2 Z9 2 U1 6 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 21 PY 2016 VL 120 IS 15 BP 8240 EP 8245 DI 10.1021/acs.jpcc.6b02851 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DK3IU UT WOS:000374811100038 ER PT J AU Krier, JM Komvopoulos, K Somorjai, GA AF Krier, James M. Komvopoulos, Kyriakos Somorjai, Gabor A. TI Cyclohexene and 1,4-Cyclohexadiene Hydrogenation Occur through Mutually Exclusive Intermediate Pathways on Platinum Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SUM-FREQUENCY GENERATION; SURFACE VIBRATIONAL SPECTROSCOPY; CATALYTIC-REACTIONS; ETHYLENE HYDROGENATION; STRUCTURE SENSITIVITY; CRYSTAL-SURFACES; HIGH-PRESSURES; IN-SITU; PT(111); DEHYDROGENATION AB Platinum nanoparticles (NPs) capped with polyvinylpyrrolidone (PVP) were studied with sum frequency generation (SFG) vibrational spectroscopy under reaction conditions during cyclohexene (CH) and 1,4-cyclohexadiene (1,4-CHD) hydrogenation at 295 K. Despite similar vibrational features observed during reaction, CH and 1,4-CHD proceed through mutually exclusive pathways on 1.7 and 4.6 nm Pt-PVP NPs unlike Pt(111) studied previously. The intense red-shifted C-H stretch of adsorbed 1,4-CHD at 2770 cm(-1) was monitored for both reactions. SFG and kinetic experiments show CH hydrogenation is active and reversible, while 1,4-CHD hydrogenation poisons the surface. C1 [Krier, James M.; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Komvopoulos, Kyriakos] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Krier, James M.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Krier, James M.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Krier, JM; Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Krier, JM; Somorjai, GA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Krier, JM; Somorjai, GA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM james.krier@gmail.com; somorjai@berkeley.edu FU Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; UCB-KAUST Academic Excellence Alliance (AEA) Program FX This work was supported by the Director, Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Partial funding for J.M.K. was also provided by the UCB-KAUST Academic Excellence Alliance (AEA) Program. NR 25 TC 0 Z9 0 U1 7 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 21 PY 2016 VL 120 IS 15 BP 8246 EP 8250 DI 10.1021/acs.jpcc.6b01615 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DK3IU UT WOS:000374811100039 ER PT J AU Aruta, C Han, C Zhou, S Cantoni, C Yang, N Tebano, A Lee, TL Schlueter, C Bongiorno, A AF Aruta, Carmela Han, Chu Zhou, Si Cantoni, Claudia Yang, Nan Tebano, Antonello Lee, Tien-Lin Schlueter, Christoph Bongiorno, Angelo TI A-Site Cation Substitutions in Strained Y-Doped BaZrO3 Multilayer Films Leading to Fast Proton Transport Pathways SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DENSITY-FUNCTIONAL THEORY; BARIUM ZIRCONATE FILMS; GRAPHENE OXIDE; CONDUCTION; PSEUDOPOTENTIALS; INTERFACES AB Proton-conducting perovskite oxides form a class of solid electrolytes for novel electrochemical devices operating at moderate temperatures. Here, we use hard X-ray photoelectron spectroscopy, scanning transmission electron microscopy, and density functional theory calculations to investigate the structure and elucidate the origin of the fast proton transport properties of strained ultrathin films of Y-doped BaZrO3 grown by pulsed lased deposition on NdGaO3. Our study shows that our BaZr0.8Y0.2O3 films incorporate a significant amount of Y dopants, and to a lesser extent also Zr ions, substituting for Ba2+, and that these substitutional defects agglomerate forming columnar regions crossing vertically from the surface to the interface the entire film. Our calculations also show that, in regions rich in Y substitutions for both Zr and Ba, the proton transfer process involves nearly zero-energy barriers, indicating that A-site cation substitutions by Y lead to fast transport pathways and hence are responsible for the previously observed enhanced values of the proton conductivity of these perovskite oxide films. C1 [Aruta, Carmela; Yang, Nan; Tebano, Antonello] Univ Roma Tor Vergata, Natl Res Council CNR SPIN, I-00133 Rome, Italy. [Han, Chu] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Zhou, Si] Dalian Univ Technol, Coll Adv Sci & Technol, 2 Linggong Rd, Dalian 116024, Peoples R China. [Cantoni, Claudia] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Tebano, Antonello] Univ Roma Tor Vergata, Dipartimento Ingn Civile & Ingn Informat, I-00133 Rome, Italy. [Lee, Tien-Lin; Schlueter, Christoph] Diamond Light Source Ltd, Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England. [Bongiorno, Angelo] CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA. [Bongiorno, Angelo] CUNY, Grad Ctr, PhD Program Chem, New York, NY 10016 USA. [Bongiorno, Angelo] CUNY, Grad Ctr, PhD Program Phys, New York, NY 10016 USA. RP Aruta, C (reprint author), Univ Roma Tor Vergata, Natl Res Council CNR SPIN, I-00133 Rome, Italy.; Bongiorno, A (reprint author), CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA.; Bongiorno, A (reprint author), CUNY, Grad Ctr, PhD Program Chem, New York, NY 10016 USA.; Bongiorno, A (reprint author), CUNY, Grad Ctr, PhD Program Phys, New York, NY 10016 USA. EM carmela.aruta@spin.cnr.it; angelo.bongiomo@csi.cuny.edu RI Aruta, Carmela/L-2957-2015; Zhou, Si/P-6339-2016 OI Aruta, Carmela/0000-0002-6917-6667; FU NSF [CMMI-1436375, CNS-0855217, CNS-0958379, ACI-1126113]; US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank Regina Ciancio for useful discussions on composition analysis. A.B. acknowledges the support of the NSF grant CMMI-1436375. The research of C.C. was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. This research was supported, in part, by a grant of computer time from the City University of New York High Performance Computing Center under NSF Grants CNS-0855217, CNS-0958379, and ACI-1126113. NR 26 TC 1 Z9 1 U1 8 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 21 PY 2016 VL 120 IS 15 BP 8387 EP 8391 DI 10.1021/acs.jpcc.6b01963 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DK3IU UT WOS:000374811100055 ER PT J AU Goodpaster, JD Bell, AT Head-Gordon, M AF Goodpaster, Jason D. Bell, Alexis T. Head-Gordon, Martin TI Identification of Possible Pathways for C-C Bond Formation during Electrochemical Reduction of CO2: New Theoretical Insights from an Improved Electrochemical Model SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SINGLE-CRYSTAL ELECTRODE; COPPER ELECTRODES; METAL-ELECTRODES; ELEMENTARY STEPS; CU(100) SURFACE; ELECTROREDUCTION; ADSORPTION; PH; POTENTIALS; MECHANISM AB We have carried out a periodic Kohn-Sham density functional theory investigation of the pathways by which carbon-carbon bonds could be formed during the electrochemical reduction of CO2 on Cu(100) using a model that includes the effects of the electrochemical potential, solvent, and electrolyte. The electrochemical potential was set by relating the applied potential to the Fermi energy and then calculating the number of electrons required by the simulation cell for that specific Fermi energy. The solvent was included as a continuum dielectric, and the electrolyte was described using a linearized Poisson-Boltzmann model. The calculated potential of zero charge for a variety of surfaces agrees with experiment to within a mean average error of 0.09 V, thereby validating the assumptions of the model. Analysis of the mechanism for C-C bond formation revealed that at low-applied potential, C-C bond formation occurs through a CO dimer. However, at high applied potentials, a large activation barrier blocks this pathway; therefore, C-C bond formation occurs through reaction of adsorbed CHO and CO. Rate parameters determined from our calculations were used to simulate the kinetics of ethene formation during the electrochemical reduction of CO over a Cu(100) surface. An excellent match was observed between previously reported measurements of the partial current for ethene formation as a function of applied voltage and the variation in the partial current for C-C bond formation predicted by our microkinetic model. The electrochemical model reported here is simple, fairly easy to implement, and involves only a small increase in computational cost over calculations neglecting the effects of the electrolyte and the applied field. Therefore, it can be used to study the effects of applied potential and electrolyte composition on the energetics of surface reactions for a wide variety of electrochemical reactions. C1 [Goodpaster, Jason D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Bell, Alexis T.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Bell, AT (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Head-Gordon, M (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM alexbell@berkeley.edu; mhg@cchem.berkeley.edu FU Office of Science of the U.S. Department of Energy [DE-SC00004993] FX This material is based on work performed in the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award DE-SC00004993. The authors thank Richard Hennig for providing the linearized Poisson-Boltzmann code for VASP and the VASPsoI program. NR 28 TC 8 Z9 8 U1 34 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD APR 21 PY 2016 VL 7 IS 8 BP 1471 EP 1477 DI 10.1021/acs.jpclett.6b00358 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DK3IR UT WOS:000374810800011 PM 27045040 ER PT J AU Beste, A Overbury, SH AF Beste, Ariana Overbury, Steven H. TI Dehydrogenation of methanol to formaldehyde catalyzed by pristine and defective ceria surfaces SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CEO2 NANOCRYSTALS; THIN-FILMS; BASIS-SET; ADSORPTION; OXIDE; OXIDATION AB We have explored the dehydrogenation of methoxy on pristine and defective (111), (100), and (110) ceria surfaces with density functional methods. Methanol conversion is used as a probe reaction to understand structure sensitivity of the oxide catalysis. Differences in reaction selectivity have been observed experimentally as a function of crystallographically exposed faces and degree of reduction. We find that the barrier for carbon-hydrogen cleavage in methoxy is similar for the pristine and defective (111), (100), and (110) surfaces. However, there are large differences in the stability of the surface intermediates on the different surfaces. The variations in experimentally observed product selectivities are a consequence of the interplay between barrier controlled bond cleavage and desorption processes. Subtle differences in activation energies for carbon-hydrogen cleavage on the different crystallographic faces of ceria could not be correlated with structural or electronic descriptors. C1 [Beste, Ariana] Univ Tennessee, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. [Beste, Ariana] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Overbury, Steven H.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Beste, A (reprint author), Univ Tennessee, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA.; Beste, A (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM bestea@ornl.gov FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. The computational part of this project was conducted at the Center for Nanophase Materials Sciences under a user proposal. The Center is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research was in part supported by an allocation of advanced computing resources provided by the National Science Foundation and performed on Darter at the National Institute for Computational Sciences (http://www.nics.tennessee.edu/). This research also used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 52 TC 0 Z9 0 U1 13 U2 29 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 21 PY 2016 VL 18 IS 15 BP 9990 EP 9998 DI 10.1039/c6cp00151c PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ6VF UT WOS:000374350600016 PM 27005883 ER PT J AU Fernandez-Alberti, S Makhov, DV Tretiak, S Shalashilin, DV AF Fernandez-Alberti, Sebastian Makhov, Dmitry V. Tretiak, Sergei Shalashilin, Dmitrii V. TI Non-adiabatic excited state molecular dynamics of phenylene ethynylene dendrimer using a multiconfigurational Ehrenfest approach SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID QUANTUM RENORMALIZATION-GROUPS; UNIDIRECTIONAL ENERGY-TRANSFER; CORRELATED EXCIMER FORMATION; DENSITY-FUNCTIONAL THEORY; PHENYLACETYLENE DENDRIMERS; CONJUGATED MOLECULES; ELECTRONIC EXCITATIONS; OPTICAL-EXCITATIONS; NONLINEAR POLARIZABILITIES; ANTENNA SUPERMOLECULES AB Photoinduced dynamics of electronic and vibrational unidirectional energy transfer between meta-linked building blocks in a phenylene ethynylene dendrimer is simulated using a multiconfigurational Ehrenfest in time-dependent diabatic basis (MCE-TDDB) method, a new variant of the MCE approach developed by us for dynamics involving multiple electronic states with numerous abrupt crossings. Excited-state energies, gradients and non-adiabatic coupling terms needed for dynamics simulation are calculated on-the-fly using the Collective Electron Oscillator (CEO) approach. A comparative analysis of our results obtained using MCE-TDDB, the conventional Ehrenfest method and the surface-hopping approach with and without decoherence corrections is presented. C1 [Fernandez-Alberti, Sebastian] Univ Nacl Quilmes, Roque Saenz Pena 352,B1876BXD Bernal, Bernal, Argentina. [Makhov, Dmitry V.; Shalashilin, Dmitrii V.] Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England. [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies CNLS, POB 1663, Los Alamos, NM 87545 USA. [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, POB 1663, Los Alamos, NM 87545 USA. RP Makhov, DV (reprint author), Univ Leeds, Sch Chem, Leeds LS2 9JT, W Yorkshire, England. EM d.makhov@leeds.ac.uk RI Tretiak, Sergei/B-5556-2009 OI Tretiak, Sergei/0000-0001-5547-3647 FU CONICET; UNQ; ANPCyT [PICT-2014-2662]; EPSRC [EP/J001481/1, EP/N007549/1]; National Nuclear Security Administration of the U.S. Department of Energy [DEAC52-06NA25396] FX SF-A is supported by CONICET, UNQ, ANPCyT (PICT-2014-2662). DM, DS and SF-A acknowledge the support from EPSRC through grants EP/J001481/1 and EP/N007549/1 (DM and DS). This work was performed in part at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Science user facility at Los Alamos National Laboratory (LANL). LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DEAC52-06NA25396. NR 114 TC 2 Z9 2 U1 7 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 21 PY 2016 VL 18 IS 15 BP 10028 EP 10040 DI 10.1039/c5cp07332d PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ6VF UT WOS:000374350600020 PM 27004611 ER PT J AU Szanyi, J Gao, F Kwak, JH Kollar, M Wang, YL Peden, CHF AF Szanyi, Janos Gao, Feng Kwak, Ja Hun Kollar, Marton Wang, Yilin Peden, Charles H. F. TI Characterization of Fe2+ ions in Fe,H/SSZ-13 zeolites: FTIR spectroscopy of CO and NO probe molecules SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SELECTIVE CATALYTIC-REDUCTION; N2O DECOMPOSITION; ACTIVE-SITES; NITRIC-OXIDE; BETA CATALYST; SCR CATALYSTS; BEA ZEOLITE; IRON SITES; CU-SSZ-13; NH3 AB The IR spectra of adsorbed CO and NO probe molecules were used to characterize the coordination chemistry of Fe2+ ions in solution ion exchanged Fe, H/SSZ-13 zeolites. The effects of Fe ion exchange levels, as well as the sample pre-treatment conditions, on the adsorption of these probe molecules were investigated. The ion exchange levels (in the range of the study) did not affect significantly the IR spectra of either probe molecule, and the IR features and their intensity ratios were very similar. Experiments with both probe molecules substantiated the presence of two distinct types of Fe2+ ions in cationic positions. We assign these two Fe2+ ions to two distinct cationic positions: Fe2+ in 6R and 8R positions. NO initially adsorbs preferentially onto Fe2+ sites in the 6R position, and then populates sites in the 8R. Fe2+ ions in the 8R positions require the interaction of more than one NO molecule to move them out from their adsorbate-free cationic positions. As soon as they move from their stable positions, they are able to bind to multiple NO molecules, and form mostly tri-nitrosyls. These tri-nitrosyls, however, are only stable in the presence of gas phase NO; under dynamic vacuum they lose one of the NO molecules from their coordination sphere and form stable di-nitrosyls. The adsorption of CO is much weaker on Fe2+ sites than that of NO, and requires cryogenic sample temperatures to initiate CO adsorption. Under the conditions applied in this study, only mono-carbonyl formation was observed. Reduction in H-2 at 773 K increased the number of Fe2+ adsorption sites, primarily in the 8R locations. Oxidation by N2O, on the other hand, selectively reduced the adsorption of both CO and NO on the Fe2+ sites in 8R positions. Adsorbed oxygen left behind from the decomposition of N2O at 573 K readily reacted with CO to produce CO2 even at 150 K. C1 [Szanyi, Janos; Gao, Feng; Kollar, Marton; Wang, Yilin; Peden, Charles H. F.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Kwak, Ja Hun] UNIST, Sch Energy & Chem Engn, Dept Chem Engn, Ulsan, South Korea. RP Szanyi, J (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. EM janos.szanyi@pnnl.gov FU US Department of Energy (DOE), Energy Efficiency and Renewable Energy, Vehicle Technologies Program; DOE's Office of Biological and Environmental Research FX The authors gratefully acknowledge the US Department of Energy (DOE), Energy Efficiency and Renewable Energy, Vehicle Technologies Program for the support of this work. The research described in this paper was performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the US DOE by Battelle. NR 56 TC 0 Z9 0 U1 10 U2 29 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 21 PY 2016 VL 18 IS 15 BP 10473 EP 10485 DI 10.1039/c6cp00136j PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ6VF UT WOS:000374350600068 PM 27030020 ER PT J AU Mills, EM Kleine-Boymann, M Janek, J Yang, H Browning, ND Takamura, Y Kim, S AF Mills, Edmund M. Kleine-Boymann, Matthias Janek, Juergen Yang, Hao Browning, Nigel D. Takamura, Yayoi Kim, Sangtae TI YSZ thin films with minimized grain boundary resistivity SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID ELECTRICAL-PROPERTIES; IONIC-CONDUCTIVITY; DOPED ZIRCONIA; TEMPERATURE; DIFFUSION; INTERFACES; CERIA AB In recent years, interface engineering of solid electrolytes has been explored to increase their ionic conductivity and improve the performance of solid oxide fuel cells and other electrochemical power sources. It has been observed that the ionic conductivity of epitaxially grown thin films of some electrolytes is dramatically enhanced, which is often attributed to effects (e.g. strain-induced mobility changes) at the heterophase boundary with the substrate. Still largely unexplored is the possibility of manipulation of grain boundary resistivity in polycrystalline solid electrolyte films, clearly a limiting factor in their ionic conductivity. Here we report that the ionic conductivity of yttria stabilized zirconia thin films with nano-columnar grains grown on a MgO substrate nearly reaches that of the corresponding single crystal when the thickness of the films becomes less than roughly 8 nm (smaller by a factor of three at 500 degrees C). Using impedance spectroscopy, the grain boundary resistivity was probed as a function of film thickness. The resistivity of the grain boundaries near the film-substrate interface and film surface (within 4 nm of each) was almost entirely eliminated. This minimization of grain boundary resistivity is attributed to Mg2+ diffusion from the MgO substrate into the YSZ grain boundaries, which is supported by time of flight secondary ion mass spectroscopy measurements. We suggest grain boundary "design'' as an attractive method to obtain highly conductive solid electrolyte thin films. C1 [Mills, Edmund M.; Takamura, Yayoi; Kim, Sangtae] Univ Calif Davis, Dept Chem Engn & Mat Sci, 3001 Ghausi Hall, Davis, CA 95616 USA. [Kleine-Boymann, Matthias; Janek, Juergen] Univ Giessen, Phys Chem Inst, Heinrich Buff Ring 58, D-35392 Giessen, Germany. [Yang, Hao; Browning, Nigel D.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Kim, S (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, 3001 Ghausi Hall, Davis, CA 95616 USA. EM chmkim@ucdavis.edu FU US-Israel Binational Science Foundation; NSF [DMR 747896]; DFG (Deutsche Forchungsgemeinschaft) [DFG Ja 648/21-1]; Laboratory Directed Research and Development (LDRD) Program Chemical Imaging Initiative (CII) at Pacific Northwest National Laboratory (PNNL); Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility - DOE's Office of Biological and Environmental Research (BER) at PNNL; DOE [DE-AC05-76RL01830] FX We gratefully acknowledge many valuable discussions about ToF-SIMS measurements with Dr Marcus Rohnke. S. K. wishes to thank the US-Israel Binational Science Foundation for funding this research. Y. T. would like to acknowledge NSF for financial support (DMR 747896). JJ and MKB acknowledge financial support by DFG (Deutsche Forchungsgemeinschaft) within the project DFG Ja 648/21-1. N. B. acknowledges support through the Laboratory Directed Research and Development (LDRD) Program Chemical Imaging Initiative (CII) at Pacific Northwest National Laboratory (PNNL) and the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research (BER) at PNNL. PNNL is a multiprogram national laboratory operated by Battelle for DOE under Contract DE-AC05-76RL01830. NR 22 TC 0 Z9 0 U1 8 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 21 PY 2016 VL 18 IS 15 BP 10486 EP 10491 DI 10.1039/c5cp08032k PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ6VF UT WOS:000374350600069 PM 27030391 ER PT J AU Yusim, K Yoon, H Foley, B Feng, SH Macke, J Dimitrijevic, M Abfalterer, W Szinger, J Fischer, W Kuiken, C Korber, B AF Yusim, Karina Yoon, Hyejin Foley, Brian Feng, Shihai Macke, Jennifer Dimitrijevic, Mira Abfalterer, Werner Szinger, James Fischer, Will Kuiken, Carla Korber, Bette TI Integrated sequence and immunology filovirus database at Los Alamos SO DATABASE-THE JOURNAL OF BIOLOGICAL DATABASES AND CURATION LA English DT Article ID EBOLA-VIRUS INFECTION; FAMILY FILOVIRIDAE; MARBURG VIRUS; STANDARDIZED NOMENCLATURE; NONHUMAN-PRIMATES; SPECIES LEVEL; GENOME BROWSER; HUMAN-ANTIBODY; WEST-AFRICA; T-CELLS AB The Ebola outbreak of 2013-15 infected more than 28 000 people and claimed more lives than all previous filovirus outbreaks combined. Governmental agencies, clinical teams, and the world scientific community pulled together in a multifaceted response ranging from prevention and disease control, to evaluating vaccines and therapeutics in human trials. As this epidemic is finally coming to a close, refocusing on long-term prevention strategies becomes paramount. Given the very real threat of future filovirus outbreaks, and the inherent uncertainty of the next outbreak virus and geographic location, it is prudent to consider the extent and implications of known natural diversity in advancing vaccines and therapeutic approaches. To facilitate such consideration, we have updated and enhanced the content of the filovirus portion of Los Alamos Hemorrhagic Fever Viruses Database. We have integrated and performed baseline analysis of all family Filoviridae sequences deposited into GenBank, with associated immune response data, and metadata, and we have added new computational tools with web-interfaces to assist users with analysis. Here, we (i) describe the main features of updated database, (ii) provide integrated views and some basic analyses summarizing evolutionary patterns as they relate to geo-temporal data captured in the database and (iii) highlight the most conserved regions in the proteome that may be useful for a T cell vaccine strategy. C1 [Yusim, Karina; Yoon, Hyejin; Foley, Brian; Feng, Shihai; Macke, Jennifer; Dimitrijevic, Mira; Abfalterer, Werner; Szinger, James; Fischer, Will; Kuiken, Carla; Korber, Bette] Los Alamos Natl Lab, Los Alamos, NM USA. RP Yusim, K (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM kyusim@lanl.gov OI Korber, Bette/0000-0002-2026-5757; Foley, Brian/0000-0002-1086-0296; Fischer, Will/0000-0003-4579-4062 FU Internal Funds from Los Alamos National Laboratory FX This work was funded through Internal Funds from Los Alamos National Laboratory NR 68 TC 0 Z9 0 U1 0 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1758-0463 J9 DATABASE-OXFORD JI Database PD APR 21 PY 2016 AR baw047 DI 10.1093/database/baw047 PG 11 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA DK1CR UT WOS:000374650600001 ER PT J AU Croft, RAC Miralda-Escude, J Zheng, Z Bolton, A Dawson, KS Peterson, JB York, DG Eisenstein, D Brinkmann, J Brownstein, J Cen, RY Delubac, T Font-Ribera, A Hamilton, JC Lee, KG Myers, A Palanque-Delabrouille, N Paris, I Petitjean, P Pieri, MM Ross, NP Rossi, G Schlegel, DJ Schneider, DP Slosar, A Vazquez, J Viel, M Weinberg, DH Yeche, C AF Croft, Rupert A. C. Miralda-Escude, Jordi Zheng, Zheng Bolton, Adam Dawson, Kyle S. Peterson, Jeffrey B. York, Donald G. Eisenstein, Daniel Brinkmann, Jon Brownstein, Joel Cen, Renyue Delubac, Timothee Font-Ribera, Andreu Hamilton, Jean-Christophe Lee, Khee-Gan Myers, Adam Palanque-Delabrouille, Nathalie Paris, Isabelle Petitjean, Patrick Pieri, Matthew M. Ross, Nicholas P. Rossi, Graziano Schlegel, David J. Schneider, Donald P. Slosar, Anze Vazquez, Jose Viel, Matteo Weinberg, David H. Yeche, Christophe TI Large-scale clustering of Lyman alpha emission intensity from SDSS/BOSS SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE cosmology: observations ID OSCILLATION SPECTROSCOPIC SURVEY; STAR-FORMING GALAXIES; DIGITAL SKY SURVEY; HALO OCCUPATION DISTRIBUTION; QUASAR TARGET SELECTION; FORMATION RATE DENSITY; DATA RELEASE 9; SIMILAR-TO 2; HIGH-REDSHIFT; SDSS-III AB We present a tentative detection of the large-scale structure of Ly alpha emission in the Universe at redshifts z = 2-3.5 by measuring the cross-correlation of Ly alpha surface brightness with quasars in Sloan Digital Sky Survey/Baryon Oscillation Spectroscopic Survey. We use amillion spectra targeting luminous red galaxies at z < 0.8, after subtracting a best-fitting model galaxy spectrum from each one, as an estimate of the high-redshift Ly alpha surface brightness. The quasar-Ly alpha emission cross-correlation is detected on scales 1 similar to 15 h(-1) Mpc, with shape consistent with a Lambda CDM model with Omega(m) = 0.30(-0.07)(+0.10). The predicted amplitude of this cross-correlation is proportional to the product of the mean Ly alpha surface brightness, , the amplitude of mass fluctuations and the quasar and Ly alpha emission bias factors. We infer (b(alpha)/3) = (3.9 +/- 0.9) x 10(-21) erg s(-1) cm(-2) angstrom(-1) arcsec(-2), where b(alpha) is the Ly alpha emission bias. If star-forming galaxies dominate this emission, we find rho(SFR) = (0.28 +/- 0.07)(3/b(alpha)) yr(-1) Mpc(-3). For b(alpha) = 3, this value is similar to 30 times larger than previous estimates from individually detected Ly alpha emitters, but consistent with the total rho(SFR) derived from dust-corrected, continuum UV galaxy surveys, if most of the Ly alpha photons from these galaxies avoid dust absorption and are reemitted after diffusing in large gas haloes. Heating of intergalactic gas by He II photoionization from quasar radiation or jets may alternatively explain the detected correlation, and cooling radiation from gas in galactic haloes may also contribute. We also detect redshift space anisotropy of the quasar-Ly alpha emission cross-correlation, finding evidence at the 3.0 sigma level that it is radially elongated, which may be explained by radiative-transfer effects. Our measurements represent the first application of the intensity mapping technique to optical observations. C1 [Croft, Rupert A. C.; Peterson, Jeffrey B.] Carnegie Mellon Univ, Dept Phys, McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA. [Croft, Rupert A. C.] Univ Oxford, Astrophys, Oxford OX1 3RH, England. [Miralda-Escude, Jordi] Inst Catalana Recerca & Estudis Avancats, E-08001 Barcelona, Catalonia, Spain. [Miralda-Escude, Jordi] Univ Barcelona, IEEC, Inst Ciencies Cosmos, E-08028 Barcelona, Catalonia, Spain. [Zheng, Zheng; Bolton, Adam; Dawson, Kyle S.; Brownstein, Joel] Univ Utah, Dept Phys & Astron, 115 S 1400 E, Salt Lake City, UT 84112 USA. [York, Donald G.] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60615 USA. [Eisenstein, Daniel] Harvard Univ, Dept Astron, 60 Garden St, Cambridge, MA 02138 USA. [Brinkmann, Jon] Apache Point Observ, POB 59, Sunspot, NM 88349 USA. [Cen, Renyue] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Delubac, Timothee; Yeche, Christophe] CEA, IRFU, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Font-Ribera, Andreu; Ross, Nicholas P.; Schlegel, David J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Hamilton, Jean-Christophe] Univ Paris Diderot Paris 7, CNRS, IN2P3, APC,CEA,Observ Paris, 10,RueA Domon & L Duquet, F-75013 Paris, France. [Lee, Khee-Gan] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Myers, Adam] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Paris, Isabelle; Viel, Matteo] INAF, Osservatorio Astron Trieste, Via G B Tiepolo 11, I-34131 Trieste, Italy. [Petitjean, Patrick] Univ Paris 06, 98bis Blvd Arago, F-75014 Paris, France. [Petitjean, Patrick] CNRS, Inst Astrophys Paris, 98bis Blvd Arago, F-75014 Paris, France. [Pieri, Matthew M.] Aix Marseille Univ, CNRS, LAM, A MIDEX,UMR 7326, F-13388 Marseille, France. [Rossi, Graziano] Sejong Univ, Dept Astron & Space Sci, Seoul 143747, South Korea. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Slosar, Anze; Vazquez, Jose] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Viel, Matteo] Ist Nazl Fis Nucl, Natl Inst Nucl Phys, Via Valerio 2, I-34127 Trieste, Italy. [Weinberg, David H.] Ohio State Univ, Dept Astron, 140 West 18th Ave, Columbus, OH 43210 USA. RP Croft, RAC (reprint author), Carnegie Mellon Univ, Dept Phys, McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA.; Croft, RAC (reprint author), Univ Oxford, Astrophys, Oxford OX1 3RH, England.; Miralda-Escude, J (reprint author), Inst Catalana Recerca & Estudis Avancats, E-08001 Barcelona, Catalonia, Spain.; Miralda-Escude, J (reprint author), Univ Barcelona, IEEC, Inst Ciencies Cosmos, E-08028 Barcelona, Catalonia, Spain.; Zheng, Z (reprint author), Univ Utah, Dept Phys & Astron, 115 S 1400 E, Salt Lake City, UT 84112 USA. EM rcroft@cmu.edu; miralda@icc.ub.edu; zhengzheng@astro.utah.edu RI Croft, Rupert/N-8707-2014; Peterson, Jeffrey/O-4794-2014 OI Croft, Rupert/0000-0003-0697-2583; Peterson, Jeffrey/0000-0003-1340-818X FU NSF [AST-1009781, AST-1109730, OCI-0749212, AST-1208891]; Moore Foundation; Leverhulme Trust's award of a Visiting Professorship at the University of Oxford; Spanish grant [AYA2012-33938]; NASA [NNX14AC89G]; Alfred P. Sloan Foundation; National Science Foundation; US Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia University of Washington; Yale University FX RACC was supported by NSF Awards AST-1009781, AST-1109730, OCI-0749212, the Moore Foundation and by the Leverhulme Trust's award of a Visiting Professorship at the University of Oxford. RACC would like to acknowledge the hospitality of the Astrophysics Subdepartment in Oxford where the initial stage of this work was carried out. RACC would also like to thank Matt McQuinn and Simon White for useful discussions. JM is partially supported by Spanish grant AYA2012-33938. ZZ is partially supported by NSF grant AST-1208891 and NASA grant NNX14AC89G.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation and the US Department of Energy Office of Science. The SDSS-III website is http://www.sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia University of Washington and Yale University. NR 98 TC 5 Z9 5 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD APR 21 PY 2016 VL 457 IS 4 BP 3541 EP 3572 DI 10.1093/mnras/stw204 PG 32 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI6CE UT WOS:000373586000011 ER PT J AU Liu, C Marusic, A Minty, M AF Liu, C. Marusic, A. Minty, M. TI First demonstration of optics measurement and correction during acceleration with beta-squeeze in a high energy collider SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Linear optics; Optics correction; Beta-beat; Emittance; Dynamic aperture AB Setting up collisions in high energy circular colliders requires beam acceleration and "beta-squeeze". The latter produces small beam sizes, and hence, high luminosity by applying strong focusing with quadrupoles near the interaction points. At the Relativistic Heavy Ion Collider (RHIC), these two processes, beam acceleration and beta-squeeze, have been performed simultaneously during recent years. In the past, beam optics correction at RHIC has only taken place at injection and at final energy, with interpolation of corrections partially into the acceleration cycle. Recent measurements of the beam optics during acceleration and squeeze have evidenced significant beta-beats that, if corrected, could minimize undesirable emittance dilutions and maximize the spin polarization of polarized proton beams by avoiding the high-order multipole fields sampled by particles within the bunch. We recently demonstrated beam optics corrections during acceleration at RHIC. As a valuable by-product, these corrections minimized the beta-beat at the profile monitors, so providing more accurate measurements of the evolution of the beam emittances during acceleration. (C) 2016 Elsevier B.V. All rights reserved. C1 [Liu, C.; Marusic, A.; Minty, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Liu, C (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM cliu1@bnl.gov FU U.S. Department of Energy [DE-AC02-98CH10886] FX We would like to thank A. Drees, R. Michnoff, I. Blackler, and G. Marr for their contributions towards the development of optics measurement during beam acceleration. We also thank W. Fischer, M. Blaskiewicz, G. Robert-Demolaize (run coordinator for high energy Au-Au program in 2014), V. Ranjbar (run coordinator for 250 GeV polarized proton program in 2013), and the operational crews for their encouragement and support of our work. Also, we are grateful to V. Schoefer, G. Marr and T. Shrey for their support of our work during the startup prior to the physics run. This work was performed under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 36 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 21 PY 2016 VL 816 BP 9 EP 15 DI 10.1016/j.nima.2016.01.068 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DF0DO UT WOS:000371009400002 ER PT J AU Batygin, YK Scheinker, A Kurennoy, S Li, C AF Batygin, Yuri K. Scheinker, Alexander Kurennoy, Sergey Li, Chao TI Suppression of space charge induced beam halo in nonlinear focusing channel SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Space charge; Halo; Quadrupole; Duodecapole; Emittance AB An intense non-uniform particle beam exhibits strong emittance growth and halo formation in focusing channels due to nonlinear space charge forces of the beam. This phenomenon limits beam brightness and results in particle losses. The problem is connected with irreversible distortion of phase space volume of the beam in conventional focusing structures due to filamentation in phase space. Emittance growth is accompanied by halo formation in real space, which results in inevitable particle losses. A new approach for solving a self-consistent problem for a matched non-uniform beam in two-dimensional geometry is discussed. The resulting solution is applied to the problem of beam transport, while avoiding emittance growth and halo formation by the use of nonlinear focusing field. Conservation of a beam distribution function is demonstrated analytically and by particle-in-cell simulation for a beam with a realistic beam distribution. (C) 2016 Elsevier B.V. All rights reserved. C1 [Batygin, Yuri K.; Scheinker, Alexander; Kurennoy, Sergey] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Li, Chao] Inst High Energy Phys, Beijing 100049, Peoples R China. RP Batygin, YK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM batygin@lanl.gov OI Kurennoy, Sergey/0000-0003-2854-9647 NR 18 TC 0 Z9 0 U1 2 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 21 PY 2016 VL 816 BP 78 EP 86 DI 10.1016/j.nima.2016.01.045 PG 9 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DF0DO UT WOS:000371009400011 ER PT J AU Li, YC Tsang, T Thorn, C Qian, X Diwan, M Joshi, J Kettell, S Morse, W Rao, T Stewart, J Tang, W Viren, B AF Li, Yichen Tsang, Thomas Thorn, Craig Qian, Xin Diwan, Milind Joshi, Jyoti Kettell, Steve Morse, William Rao, Triveni Stewart, James Tang, Wei Viren, Brett TI Measurement of longitudinal electron diffusion in liquid argon SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Liquid argon time projection chamber; Electron diffusion; Electron drift velocity; Photocathode; Longitudinal diffusion; Electron mobility ID DRIFT-VELOCITY; IONIZATION ELECTRONS; SWARM PARAMETERS; VON ELEKTRONEN; KINETIC-THEORY; GAS-MIXTURES; SOLID ARGON; TRANSPORT; MOTION; DETECTORS AB We report the measurement of longitudinal electron diffusion coefficients in liquid argon for electric fields between 100 and 2000 V/cm with a gold photocathode as a bright electron source. The measurement principle, apparatus, and data analysis are described. In the region between 100 and 350 V/cm, our results show a discrepancy with the previous measurement [1]. In the region between 350 and 2000 V/cm, our results represent the world's best measurement. Over the entire measured electric field range, our results are systematically higher than the calculation of Atrazhev-Timoshkin In The quantum efficiency of the gold photocathode, the drift velocity and longitudinal diffusion coefficients in gas argon are also presented. (C) 2016 Elsevier B.V. All rights reserved. C1 [Li, Yichen; Thorn, Craig; Qian, Xin; Diwan, Milind; Joshi, Jyoti; Kettell, Steve; Morse, William; Stewart, James; Tang, Wei; Viren, Brett] Brookhaven Natl Lab, Dept Phys, 20 Penn St,Bldg 510E, Upton, NY 11973 USA. [Tsang, Thomas; Rao, Triveni] Brookhaven Natl Lab, Instrumentat Div, 20 N Technol St,Bldg 535B, Upton, NY 11973 USA. RP Li, YC (reprint author), Brookhaven Natl Lab, Dept Phys, 20 Penn St,Bldg 510E, Upton, NY 11973 USA. EM yichen@bnl.gov RI Li, Yichen/D-8654-2017; OI Li, Yichen/0000-0002-7004-7598; Qian, Xin/0000-0002-7903-7935 FU U.S. Department of Energy, Office of Science, Office of High Energy Physics [DE-SC0012704] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of High Energy Physics and Early Career Research program under contract number DE-SC0012704. NR 58 TC 1 Z9 1 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 21 PY 2016 VL 816 BP 160 EP 170 DI 10.1016/j.nima.2016.01.094 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DF0DO UT WOS:000371009400022 ER PT J AU Archer, A Benbow, W Bird, R Buchovecky, M Buckley, JH Bugaev, V Byrum, K Cardenzana, JV Cerruti, M Chen, X Ciupik, L Collins-Hughes, E Connolly, MP Eisch, JD Falcone, A Feng, Q Finley, JP Fleischhack, H Flinders, A Fortson, L Furniss, A Gillanders, GH Griffin, S Grube, J Gyuk, G Hakansson, N Hanna, D Holder, J Humensky, TB Hutten, M Johnson, CA Kaaret, P Kar, P Kelley-Hoskins, N Kertzman, M Kieda, D Krause, M Krennrich, F Kumar, S Lang, MJ McArthur, S McCann, A Meagher, K Millis, J Moriarty, P Mukherjee, R Nieto, D Ong, RA Park, N Pelassa, V Pohl, M Popkow, A Pueschel, E Quinn, J Ragan, K Ratliff, G Reynolds, PT Richards, GT Roache, E Rousselle, J Santander, M Sembroski, GH Shahinyan, K Smith, AW Staszak, D Telezhinsky, I Tucci, JV Tyler, J Vassiliev, VV Wakely, SP Weiner, OM Weinstein, A Wilhelm, A Williams, DA Zitzer, B Yusef-Zadeh, F AF Archer, A. Benbow, W. Bird, R. Buchovecky, M. Buckley, J. H. Bugaev, V. Byrum, K. Cardenzana, J. V. Cerruti, M. Chen, X. Ciupik, L. Collins-Hughes, E. Connolly, M. P. Eisch, J. D. Falcone, A. Feng, Q. Finley, J. P. Fleischhack, H. Flinders, A. Fortson, L. Furniss, A. Gillanders, G. H. Griffin, S. Grube, J. Gyuk, G. Hakansson, N. Hanna, D. Holder, J. Humensky, T. B. Huetten, M. Johnson, C. A. Kaaret, P. Kar, P. Kelley-Hoskins, N. Kertzman, M. Kieda, D. Krause, M. Krennrich, F. Kumar, S. Lang, M. J. McArthur, S. McCann, A. Meagher, K. Millis, J. Moriarty, P. Mukherjee, R. Nieto, D. Ong, R. A. Park, N. Pelassa, V. Pohl, M. Popkow, A. Pueschel, E. Quinn, J. Ragan, K. Ratliff, G. Reynolds, P. T. Richards, G. T. Roache, E. Rousselle, J. Santander, M. Sembroski, G. H. Shahinyan, K. Smith, A. W. Staszak, D. Telezhinsky, I. Tucci, J. V. Tyler, J. Vassiliev, V. V. Wakely, S. P. Weiner, O. M. Weinstein, A. Wilhelm, A. Williams, D. A. Zitzer, B. Yusef-Zadeh, F. TI TEV GAMMA-RAY OBSERVATIONS OF THE GALACTIC CENTER RIDGE BY VERITAS SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: center; gamma rays: general; supernovae: individual (G0.9+0.1) ID SGR-A-ASTERISK; SAGITTARIUS B2 CLOUD; CENTER BLACK-HOLE; HIGH-ENERGY; CENTER REGION; MOLECULAR CLOUDS; CHANDRA OBSERVATIONS; STELLAR CLUSTERS; EMISSION; TELESCOPE AB The Galactic Center ridge has been observed extensively in the past by both GeV and TeV gamma-ray instruments revealing a wealth of structure, including a diffuse component and the point sources G0.9+0.1 (a composite supernova remnant) and Sgr A* (believed to be associated with the supermassive black hole located at the center of our Galaxy). Previous very high energy (VHE) gamma-ray observations with the H.E.S.S.. experiment have also detected an extended TeV gamma-ray component along the Galactic plane in the >300 GeV gamma-ray regime. Here we report on observations of the Galactic Center ridge from 2010 to 2014 by the VERITAS telescope array in the >2 TeV energy range. From these observations we (1) provide improved measurements of the differential energy spectrum for Sgr A* in the >2 TeV gamma-ray regime, (2) provide a detection in the >2 TeV gamma-ray emission from the composite SNR G0.9+0.1 and an improved determination of its multi-TeV gamma-ray energy spectrum, and. (3) report on the detection of VER J1746-289, a localized enhancement of >2 TeV gamma-ray emission along the Galactic plane. C1 [Archer, A.; Buckley, J. H.; Bugaev, V.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Cerruti, M.; Pelassa, V.; Roache, E.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Collins-Hughes, E.; Pueschel, E.; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Buchovecky, M.; Ong, R. A.; Popkow, A.; Rousselle, J.; Vassiliev, V. V.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Byrum, K.; Zitzer, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cardenzana, J. V.; Eisch, J. D.; Krennrich, F.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Chen, X.; Hakansson, N.; Pohl, M.; Telezhinsky, I.; Wilhelm, A.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Chen, X.; Fleischhack, H.; Huetten, M.; Kelley-Hoskins, N.; Krause, M.; Pohl, M.; Telezhinsky, I.; Wilhelm, A.] DESY, Platanenallee 6, D-15738 Zeuthen, Germany. [Ciupik, L.; Grube, J.; Gyuk, G.; Ratliff, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Connolly, M. P.; Gillanders, G. H.; Lang, M. J.; Moriarty, P.] Natl Univ Ireland Galway, Sch Phys, Univ Rd, Galway, Ireland. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Feng, Q.; Finley, J. P.; McArthur, S.; Sembroski, G. H.; Tucci, J. V.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Flinders, A.; Kar, P.; Kieda, D.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Fortson, L.; Shahinyan, K.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Furniss, A.] Calif State Univ East Bay, Dept Phys, Hayward, CA 94542 USA. [Griffin, S.; Hanna, D.; McCann, A.; Ragan, K.; Staszak, D.; Tyler, J.] McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. [Holder, J.; Kumar, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Holder, J.; Kumar, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Humensky, T. B.; Nieto, D.; Weiner, O. M.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Johnson, C. A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Kaaret, P.] Univ Iowa, Dept Phys & Astron, Van Allen Hall, Iowa City, IA 52242 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Meagher, K.; Richards, G. T.] Georgia Inst Technol, Sch Phys, 837 State St NW, Atlanta, GA 30332 USA. [Meagher, K.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, 837 State St NW, Atlanta, GA 30332 USA. [Millis, J.] Anderson Univ, Dept Phys, 1100 East 5th St, Anderson, IN 46012 USA. [Mukherjee, R.; Santander, M.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Sci, Cork, Ireland. [Smith, A. W.] Univ Maryland, College Pk, MD 20742 USA. [Smith, A. W.] NASA, Goddard Space Flight Ctr, College Pk, MD 20742 USA. [Yusef-Zadeh, F.] Northwestern Univ, Dept Phys & Astron, CIERA, Evanston, IL 60208 USA. RP Smith, AW (reprint author), Univ Maryland, College Pk, MD 20742 USA.; Smith, AW (reprint author), NASA, Goddard Space Flight Ctr, College Pk, MD 20742 USA. EM asmith44@umd.edu OI Chen, Xuhui/0000-0002-9745-0248; Krause, Maria/0000-0001-7595-0914 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Cycle 7 Fermi Guest Investigator program [NNH13ZDA001N] FX This research is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation, and the Smithsonian Institution and by NSERC in Canada. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument.; A.W.S. acknowledges support through the Cycle 7 Fermi Guest Investigator program, grant number NNH13ZDA001N. NR 58 TC 2 Z9 2 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 20 PY 2016 VL 821 IS 2 AR 129 DI 10.3847/0004-637X/821/2/129 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN5JM UT WOS:000377102700058 ER PT J AU Galli, A Wurz, P Schwadron, NA Kucharek, H Mobius, E Bzowski, M Sokol, JM Kubiak, MA Funsten, HO Fuselier, SA McComas, DJ AF Galli, A. Wurz, P. Schwadron, N. A. Kucharek, H. Mobius, E. Bzowski, M. Sokol, J. M. Kubiak, M. A. Funsten, H. O. Fuselier, S. A. McComas, D. J. TI THE ROLL-OVER OF HELIOSPHERIC NEUTRAL HYDROGEN BELOW 100 eV: OBSERVATIONS AND IMPLICATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: general; plasmas; solar wind; Sun: heliosphere ID INTERSTELLAR-BOUNDARY-EXPLORER; LY-ALPHA ABSORPTION; 1ST 5 YEARS; TERMINATION SHOCK; VOYAGER 1; INNER HELIOSHEATH; ATOM FLUX; IBEX; HELIOTAIL; HELIUM AB We present an improved analysis of the energy spectrum of energetic neutral hydrogen from the heliosheath observed with the IBEX-Lo sensor on the Interstellar Boundary EXplorer from the years 2009 to 2012. This analysis allows us to study the lowest energies between 10 and 100 eV although various background sources are more intense than the targeted signal over broad areas of the sky. The results improve our knowledge of the interaction region between our heliosphere and the interstellar plasma because these neutral atoms are direct messengers from the low-energy plasma in the heliosheath. We find a roll-over of the energy spectrum below 100 eV, which has major implications for the pressure balance of the plasma in the inner heliosheath. The results can also be compared directly with in situ observations of the Voyager 1 and 2 spacecraft. C1 [Galli, A.; Wurz, P.] Univ Bern, Inst Phys, CH-3012 Bern, Switzerland. [Schwadron, N. A.; Kucharek, H.; Mobius, E.] Univ New Hampshire, Durham, NH 03824 USA. [Bzowski, M.; Sokol, J. M.; Kubiak, M. A.] Polish Acad Sci, Space Res Ctr, PL-00716 Warsaw, Poland. [Funsten, H. O.] Los Alamos Natl Lab, Intelligence & Space Res Div, POB 1663, Los Alamos, NM 87545 USA. [Fuselier, S. A.; McComas, D. J.] SW Res Inst, 6220 Culebra Rd, San Antonio, TX 78228 USA. [Fuselier, S. A.; McComas, D. J.] Univ Texas San Antonio, San Antonio, TX 78249 USA. RP Galli, A (reprint author), Univ Bern, Inst Phys, CH-3012 Bern, Switzerland. RI Sokol, Justyna/K-2892-2015; OI Wurz, Peter/0000-0002-2603-1169 FU Swiss National Science foundation; Polish National Science Center grant [2012-06-M-ST9-00455]; NASA Explorer program as a part of the IBEX mission FX We thank all of the outstanding men and women who have made the IBEX mission such a wonderful success. A.G. and P.W. thank the Swiss National Science foundation for financial support. M.B., M.A.K., and J.M.S. were supported by Polish National Science Center grant 2012-06-M-ST9-00455. H.K., E.M., N.S., H.O.F., S.A.F., and D.J.M. were supported by the NASA Explorer program as a part of the IBEX mission. NR 41 TC 3 Z9 3 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 20 PY 2016 VL 821 IS 2 AR 107 DI 10.3847/0004-637X/821/2/107 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN5JM UT WOS:000377102700036 ER PT J AU Rana, V Loh, A Corbel, S Tomsick, JA Chakrabarty, D Walton, DJ Barret, D Boggs, SE Christensen, FE Craig, W Fuerst, F Gandhi, P Grefenstette, BW Hailey, C Harrison, FA Madsen, KK Rahoui, F Stern, D Tendulkar, S Zhang, WW AF Rana, Vikram Loh, Alan Corbel, Stephane Tomsick, John A. Chakrabarty, Deepto Walton, Dominic J. Barret, Didier Boggs, Steven E. Christensen, Finn E. Craig, William Fuerst, Felix Gandhi, Poshak Grefenstette, Brian W. Hailey, Charles Harrison, Fiona A. Madsen, Kristin K. Rahoui, Farid Stern, Daniel Tendulkar, Shriharsh Zhang, William W. TI CHARACTERIZING X-RAY AND RADIO EMISSION IN THE BLACK HOLE X-RAY BINARY V404 CYGNI DURING QUIESCENCE SO ASTROPHYSICAL JOURNAL LA English DT Article DE accretion, accretion disks; stars: black holes; stars: individual (V404 Cyg); X-rays: binaries ID ADVECTION-DOMINATED ACCRETION; COMPACT JET; GX 339-4; INFRARED-SPECTROSCOPY; EVENT HORIZONS; MODEL; TRANSIENTS; TELESCOPE; SPECTRUM; ARRAY AB We present results from multi-wavelength simultaneous X-ray and radio observations of the black hole X-ray binary V404. Cyg in quiescence. Our coverage with NuSTAR provides the very first opportunity to study the X-ray spectrum of V404. Cyg at energies above 10 keV. The unabsorbed broadband (0.3-30 keV) quiescent luminosity of the source is 8.9 x 10(32) erg s(-1) for a distance of 2.4 kpc. The source shows clear variability on short timescales (an hour to a couple of hours) in the. radio, soft X-ray, and hard X-ray bands in the form of multiple flares. The broadband X-ray spectra obtained from XMM-Newton and NuSTAR can be characterized with a power-law model having a photon index of Gamma = 2.12 +/- 0.07 (90% confidence errors); however, residuals at high energies indicate spectral curvature significant at a 3 sigma confidence level with the. e-folding energy of the cutoff as 20(-7)(+20) keV. Such curvature can be explained using synchrotron emission from the base of a jet outflow. Radio observations using the VLA reveal that the spectral index evolves on very fast timescales (as short as 10 minutes), switching between optically thick and thin synchrotron emission, possibly due to instabilities in the compact jet or stochastic instabilities in the. accretion rate. We explore different scenarios to explain this very fast variability. C1 [Rana, Vikram; Walton, Dominic J.; Fuerst, Felix; Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.; Tendulkar, Shriharsh] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Loh, Alan; Corbel, Stephane] Univ Paris Diderot, Lab AIM, CEA, IRFU,CNRS,INSU,DSM,SAp, F-91191 Gif Sur Yvette, France. [Corbel, Stephane] Univ Orleans, Stn Radioastron Nancay, PSL Res Univ, Observ Paris,CNRS,OSUC, F-18330 Nancay, France. [Tomsick, John A.; Boggs, Steven E.; Craig, William] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Chakrabarty, Deepto] MIT, Kavli Inst Astrophys & Space Res, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Barret, Didier] Univ Toulouse, UPS, OMP, IRAP, Toulouse, France. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, William] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gandhi, Poshak] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Hailey, Charles] Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. [Rahoui, Farid] European So Observ, Karl Schwarzschild Str 2, D-85748 Garching, Germany. [Rahoui, Farid] Harvard Univ, Dept Astron, 60 Garden St, Cambridge, MA 02138 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Rana, V (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Madsen, Kristin/0000-0003-1252-4891; Rana, Vikram/0000-0003-1703-8796 FU NASA [NNG08FD60C]; UnivEarthS Labex programme of Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02]; CHAOS project - French Research National Agency [ANR-12-BS05-0009]; NASA under XMM-Newton Guest Observer grant [NNX14AF08G]; NuSTAR Operation, Software, and Calibration teams FX We thank Michael A. Nowak for useful discussions on the synchrotron model. This work was supported under NASA contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. We thank the NuSTAR Operation, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). S.C. thanks James Miller-Jones for excellent help during the preparation of the VLA observations. S.C. and A.L. acknowledge the financial support from the UnivEarthS Labex programme of Sorbonne Paris Cite (ANR-10-LABX-0023 and ANR-11-IDEX-0005-02), and from the CHAOS project ANR-12-BS05-0009 supported by the French Research National Agency. J.A.T. acknowledges partial support from NASA under XMM-Newton Guest Observer grant NNX14AF08G. NR 57 TC 7 Z9 7 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 20 PY 2016 VL 821 IS 2 AR 103 DI 10.3847/0004-637X/821/2/103 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN5JM UT WOS:000377102700032 ER PT J AU Schlafly, EF Meisner, AM Stutz, AM Kainulainen, J Peek, JEG Tchernyshyov, K Rix, HW Finkbeiner, DP Covey, KR Green, GM Bell, EF Burgett, WS Chambers, KC Draper, PW Flewelling, H Hodapp, KW Kaiser, N Magnier, EA Martin, NF Metcalfe, N Wainscoat, RJ Waters, C AF Schlafly, E. F. Meisner, A. M. Stutz, A. M. Kainulainen, J. Peek, J. E. G. Tchernyshyov, K. Rix, H-W Finkbeiner, D. P. Covey, K. R. Green, G. M. Bell, E. F. Burgett, W. S. Chambers, K. C. Draper, P. W. Flewelling, H. Hodapp, K. W. Kaiser, N. Magnier, E. A. Martin, N. F. Metcalfe, N. Wainscoat, R. J. Waters, C. TI THE OPTICAL-INFRARED EXTINCTION CURVE AND ITS VARIATION IN THE MILKY WAY SO ASTROPHYSICAL JOURNAL LA English DT Article DE dust, extinction; ISM: clouds; ISM: structure ID DIGITAL SKY SURVEY; ULTRAVIOLET EXTINCTION; INTERSTELLAR EXTINCTION; MOLECULAR CLOUDS; DUST EMISSION; COLOR-EXCESS; SHAPES; LAW; EVOLUTION; APOGEE AB The dust extinction curve is a critical component of many observational programs and an important diagnostic of the physics of the interstellar medium. Here we present new measurements of the dust extinction curve and its variation toward tens of thousands of stars, a hundred-fold larger sample than in existing detailed studies. We use data from the APOGEE spectroscopic survey in combination with ten-band photometry from Pan-STARRS1, the Two Micron All-Sky Survey, and Wide-field Infrared Survey Explorer. We find that the extinction curve in the optical through infrared is well characterized by a one-parameter family of curves described by R(V). The extinction curve is more uniform than suggested in past works, with sigma(R(V)) = 0.18, and with less than one percent of sight lines having R(V) > 4. Our data and analysis have revealed two new aspects of Galactic extinction: first, we find significant, wide-area variations in R(V) throughout the Galactic plane. These variations are on scales much larger than individual molecular clouds, indicating that R(V) variations must trace much more than just grain growth in dense molecular environments. Indeed, we find no correlation between R(V) and dust column density up to E(B - V) approximate to 2. Second, we discover a strong relationship between R(V) and the far-infrared dust emissivity. C1 [Schlafly, E. F.; Stutz, A. M.; Kainulainen, J.; Rix, H-W; Martin, N. F.] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Schlafly, E. F.; Meisner, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. [Meisner, A. M.] Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Peek, J. E. G.] Space Telescope Sci Inst, 3700 San Martin Dr, Baltimore, MD 21218 USA. [Tchernyshyov, K.] Johns Hopkins Univ, Dept Phys & Astron, 3400 North Charles St, Baltimore, MD 21218 USA. [Finkbeiner, D. P.; Green, G. M.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Finkbeiner, D. P.] Harvard Univ, Dept Phys, 17 Oxford St, Cambridge, MA 02138 USA. [Covey, K. R.] Western Washington Univ, Dept Phys & Astron, 516 High St, Bellingham, WA 98225 USA. [Bell, E. F.] Univ Michigan, Dept Astron, 500 Church St, Ann Arbor, MI 48109 USA. [Burgett, W. S.] GMTO Corp, 251 S Lake Ave,Suite 300, Pasadena, CA 91101 USA. [Chambers, K. C.; Flewelling, H.; Hodapp, K. W.; Kaiser, N.; Magnier, E. A.; Wainscoat, R. J.; Waters, C.] Univ Hawaii, Inst Astron, 2680 Woodlawn Dr, Honolulu, HI 96822 USA. [Draper, P. W.; Metcalfe, N.] Univ Durham, Dept Phys, S Rd, Durham DH1 3LE, England. [Martin, N. F.] CNRS, Observ Astron Strasbourg, UMR 7550, 11 Rue Univ, F-67000 Strasbourg, France. RP Schlafly, EF (reprint author), Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany.; Schlafly, EF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. OI Schlafly, Edward Ford/0000-0002-3569-7421; Peek, Joshua/0000-0003-4797-7030; Green, Gregory/0000-0001-5417-2260; Stutz, Amelia/0000-0003-2300-8200; Covey, Kevin/0000-0001-6914-7797; Bell, Eric/0000-0002-5564-9873 FU NASA through Hubble Fellowship by the Space Telescope Science Institute [HST-HF2-51367.001-A]; NASA [NAS 5-26555, NNX10AD69G]; German Research Foundation (DFG) [Sonderforschungsbereich SFB 881]; NSF [AST-1312891]; Deutsche Forschungsgemeinschaft [1573]; CNRS through PICS project [PICS06183]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy; National Aeronautics and Space Administration; Japanese Monbukagakusho; Max Planck Society; Higher Education Funding Council for England; National Aeronautics and Space Administration through the Planetary Science Division of the NASA Science Mission Directorate [NNX08AR22G]; National Science Foundation [AST-1238877]; University of Maryland; Eotvos Lorand University (ELTE) FX ES acknowledges support for this work provided by NASA through Hubble Fellowship grant HST-HF2-51367.001-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555, and funding from Sonderforschungsbereich SFB 881 "The Milky Way System" (subproject A3) of the German Research Foundation (DFG). DF acknowledges support of NASA grant NNX10AD69G. GMG and DPF are partially supported by NSF grant AST-1312891. The work of JK was supported by the Deutsche Forschungsgemeinschaft priority program 1573 ("Physics of the ISM"). NFM gratefully acknowledges the CNRS for support through PICS project PICS06183.; Funding for the SDSS and SDSS-II has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, the U.S. Department of Energy, the National Aeronautics and Space Administration, the Japanese Monbukagakusho, the Max Planck Society, and the Higher Education Funding Council for England. The SDSS Web Site is http://www.sdss.org/.; The Pan-STARRS1 Surveys (PS1) have been made possible through contributions of the Institute for Astronomy, the University of Hawaii, the Pan-STARRS Project Office, the Max Planck Society and its participating institutes, the Max Planck Institute for Astronomy, Heidelberg and the Max Planck Institute for Extraterrestrial Physics, Garching, The Johns Hopkins University, Durham University, the University of Edinburgh, Queen's University Belfast, the Harvard-Smithsonian Center for Astrophysics, the Las Cumbres Observatory Global Telescope Network Incorporated, the National Central University of Taiwan, the Space Telescope Science Institute, the National Aeronautics and Space Administration under Grant No. NNX08AR22G issued through the Planetary Science Division of the NASA Science Mission Directorate, the National Science Foundation under Grant No. AST-1238877, the University of Maryland, and Eotvos Lorand University (ELTE). NR 76 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 20 PY 2016 VL 821 IS 2 AR 78 DI 10.3847/0004-637X/821/2/78 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN5JM UT WOS:000377102700007 ER PT J AU Wolf, RC D'Andrea, CB Gupta, RR Sako, M Fischer, JA Kessler, R Jha, SW March, MC Scolnic, DM Fischer, JL Campbell, H Nichol, RC Olmstead, MD Richmond, M Schneider, DP Smith, M AF Wolf, Rachel C. D'Andrea, Chris B. Gupta, Ravi R. Sako, Masao Fischer, John A. Kessler, Rick Jha, Saurabh W. March, Marisa C. Scolnic, Daniel M. Fischer, Johanna-Laina Campbell, Heather Nichol, Robert C. Olmstead, Matthew D. Richmond, Michael Schneider, Donald P. Smith, Mathew TI SDSS-II SUPERNOVA SURVEY: AN ANALYSIS OF THE LARGEST SAMPLE OF TYPE IA SUPERNOVAE AND CORRELATIONS WITH HOST-GALAXY SPECTRAL PROPERTIES SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: observations; galaxies: abundances; supernovae: general; surveys ID DIGITAL SKY SURVEY; STAR-FORMING GALAXIES; INITIAL MASS FUNCTION; OSCILLATION SPECTROSCOPIC SURVEY; IMPROVED PHOTOMETRIC CALIBRATION; EMISSION-LINE SPECTRA; HUBBLE RESIDUALS; LEGACY SURVEY; DATA RELEASE; COSMOLOGICAL CONSTRAINTS AB Using the largest single-survey sample of Type Ia supernovae (SNe Ia) to date, we study the relationship between properties of SNe Ia and those of their host galaxies, focusing primarily on correlations with Hubble residuals (HRs). Our sample consists of 345 photometrically classified or spectroscopically confirmed SNe Ia discovered as part of the SDSS-II Supernova Survey (SDSS-SNS). This analysis utilizes host-galaxy spectroscopy obtained during the SDSS-I/II spectroscopic survey and from an ancillary program on the SDSS-III Baryon Oscillation Spectroscopic Survey that obtained spectra for nearly all host galaxies of SDSS-II SN candidates. In addition, we use photometric host-galaxy properties from the SDSS-SNS data release such as host stellar mass and star formation rate. We confirm the well-known relation between HR and host-galaxy mass and find a 3.6 sigma significance of a nonzero linear slope. We also recover correlations between HR and host-galaxy gas-phase metallicity and specific star formation rate as they are reported in the literature. With our large data set, we examine correlations between HR and multiple host-galaxy properties simultaneously and find no evidence of a significant correlation. We also independently analyze our spectroscopically confirmed and photometrically classified SNe Ia and comment on the significance of similar combined data sets for future surveys. C1 [Wolf, Rachel C.; Gupta, Ravi R.; Sako, Masao; Fischer, John A.; March, Marisa C.; Fischer, Johanna-Laina] Univ Penn, Dept Phys & Astron, 209 South 33rd St, Philadelphia, PA 19104 USA. [D'Andrea, Chris B.; Smith, Mathew] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [D'Andrea, Chris B.; Campbell, Heather; Nichol, Robert C.] Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg,Burnaby Rd, Portsmouth PO1 3FX, Hants, England. [Gupta, Ravi R.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kessler, Rick; Scolnic, Daniel M.] Univ Chicago, Kavli Inst Cosmol Phys, 933 East 56th St, Chicago, IL 60637 USA. [Jha, Saurabh W.] Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. [Campbell, Heather] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Olmstead, Matthew D.] Kings Coll, Dept Chem & Phys, Wilkes Barre, PA 18711 USA. [Olmstead, Matthew D.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Richmond, Michael] Rochester Inst Technol, Sch Phys & Astron, Rochester, NY 14623 USA. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Smith, Mathew] Univ Western Cape, Dept Phys, ZA-7535 Cape Town, South Africa. RP Wolf, RC (reprint author), Univ Penn, Dept Phys & Astron, 209 South 33rd St, Philadelphia, PA 19104 USA. EM rcane@physics.upenn.edu FU National Science Foundation [DGE-1321851]; Department of Energy [DE-SC-0009890]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy; National Aeronautics and Space Administration; Japanese Monbukagakusho; Max Planck Society; Higher Education Funding Council for England; American Museum of Natural History; Astrophysical Institute Potsdam; University of Basel; University of Cambridge; Case Western Reserve University; University of Chicago; Drexel University; Fermilab; Institute for Advanced Study; Japan Participation Group; Johns Hopkins University; Joint Institute for Nuclear Astrophysics; Kavli Institute for Particle Astrophysics and Cosmology; Korean Scientist Group; Chinese Academy of Sciences (LAMOST); Los Alamos National Laboratory; Max-Planck-Institute for Astronomy (MPIA); Max-Planck-Institute for Astrophysics (MPA); New Mexico State University; Ohio State University; University of Pittsburgh; University of Portsmouth; Princeton University; United States Naval Observatory; University of Washington; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Florida; French Participation Group; German Participation Group; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; New York University; Pennsylvania State University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; Yale University FX This material is based on work supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1321851. Any opinion, findings, and conclusions or recommendations expressed in this material are those of the authors(s) and do not necessarily reflect the views of the National Science Foundation.; M.S. and J.A.F. are supported by the Department of Energy grant DE-SC-0009890.; Funding for the SDSS and SDSS-II has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, the U.S. Department of Energy, the National Aeronautics and Space Administration, the Japanese Monbukagakusho, the Max Planck Society, and the Higher Education Funding Council for England. The SDSS Web site is http://www.sdss.org/. The SDSS is managed by the Astrophysical Research Consortium for the Participating Institutions. The Participating Institutions are the American Museum of Natural History, Astrophysical Institute Potsdam, University of Basel, University of Cambridge, Case Western Reserve University, University of Chicago, Drexel University, Fermilab, the Institute for Advanced Study, the Japan Participation Group, Johns Hopkins University, the Joint Institute for Nuclear Astrophysics, the Kavli Institute for Particle Astrophysics and Cosmology, the Korean Scientist Group, the Chinese Academy of Sciences (LAMOST), Los Alamos National Laboratory, the Max-Planck-Institute for Astronomy (MPIA), the Max-Planck-Institute for Astrophysics (MPA), New Mexico State University, Ohio State University, University of Pittsburgh, University of Portsmouth, Princeton University, the United States Naval Observatory, and the University of Washington.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy. The SDSS-III Web site is http://www.sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration, including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, University of Florida, the French Participation Group, the German Participation Group, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and dYale University. NR 104 TC 3 Z9 3 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 20 PY 2016 VL 821 IS 2 AR 115 DI 10.3847/0004-637X/821/2/115 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DN5JM UT WOS:000377102700044 ER PT J AU Pang, LG Petersen, H Qin, GY Roy, V Wang, XN AF Pang, Long-Gang Petersen, Hannah Qin, Guang-You Roy, Victor Wang, Xin-Nian TI Decorrelation of anisotropic flow along the longitudinal direction SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID ROOT-S(NN)=2.76 TEV; ELLIPTIC FLOW; PB COLLISIONS AB The initial energy density distribution and fluctuations in the transverse direction lead to anisotropic flow of final hadrons through collective expansion in high-energy heavy-ion collisions. Fluctuations along the longitudinal direction, on the other hand, can result in decorrelation of anisotropic flow in different regions of pseudorapidity (eta). Decorrelation of the 2nd- and 3rd-order anisotropic flow with different eta gaps for final charged hadrons in high-energy heavy-ion collisions is studied in an eventby- event (3+1)D ideal hydrodynamic model with fully fluctuating initial conditions from A Multi-Phase Transport (AMPT) model. The decorrelation of anisotropic flow of final hadrons with large eta gaps is found to originate from the spatial decorrelation along the longitudinal direction in the AMPT initial conditions through hydrodynamic evolution. The decorrelation is found to consist of both a linear twist and random fluctuation of the event plane angles. The agreement between our results and recent CMS data in most centralities suggests that the string-like mechanism of initial parton production in AMPT model captures the initial longitudinal fluctuation that is responsible for the measured decorrelation of anisotropic flow in Pb+Pb collisions at LHC. Our predictions for Au+Au collisions at the highest RHIC energy show stronger longitudinal decorrelation, indicating larger longitudinal fluctuations at lower beam energies. Our study also calls into question some of the current experimental methods for measuring anisotropic flow and the quantitative extraction of transport coefficients through comparisons to hydrodynamic simulations that do not include longitudinal fluctuations. C1 [Pang, Long-Gang; Petersen, Hannah] Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. [Petersen, Hannah; Roy, Victor] Goethe Univ Frankfurt, Inst Theoret Phys, Max von Laue Str 1, D-60438 Frankfurt, Germany. [Petersen, Hannah] GSI Helmholtzzentrum Schwerionenforsch, Planckstr 1, D-64291 Darmstadt, Germany. [Qin, Guang-You; Wang, Xin-Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Qin, Guang-You; Wang, Xin-Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Wang, Xin-Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Nucl Sci Div MS70R0319, Berkeley, CA 94720 USA. RP Pang, LG (reprint author), Frankfurt Inst Adv Studies, Ruth Moufang Str 1, D-60438 Frankfurt, Germany. EM pang@fias.uni-frankfurt.de FU Helmholtz Association [VH-NG-822]; GSI; Helmholtz International Center for the Facility for Antiproton and Ion Research (HIC for FAIR) within the framework of the Landes-Offensive zur Entwicklung Wissenschaftlich-Oekonomischer Exzellenz (LOEWE) program; Natural Science Foundation of China [11221504, 11375072]; Chinese Ministry of Science and Technology [2014DFG02050]; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Alexander von Humboldt foundation, Germany FX We thank J. Jia, W. Li, P. Bozek, P. Huovenien and M. Gyulassy for helpful discussions. LGP and HP acknowledge funding of a Helmholtz Young Investigator Group VH-NG-822 from the Helmholtz Association and GSI. This work was supported in part by the Helmholtz International Center for the Facility for Antiproton and Ion Research (HIC for FAIR) within the framework of the Landes-Offensive zur Entwicklung Wissenschaftlich-Oekonomischer Exzellenz (LOEWE) program launched by the State of Hesse, by the Natural Science Foundation of China under Grants No. 11221504 and No. 11375072, by the Chinese Ministry of Science and Technology under Grant No. 2014DFG02050, and by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. VR is supported by the Alexander von Humboldt foundation, Germany. Computational resources have been provided by the Center for Scientific Computing (CSC) at the Goethe-University of Frankfurt. NR 55 TC 7 Z9 7 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD APR 20 PY 2016 VL 52 IS 4 AR 97 DI 10.1140/epja/i2016-16097-x PG 12 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DM2MQ UT WOS:000376181300003 ER PT J AU Tang, WS Matsuo, M Wu, H Stavila, V Zhou, W Talin, AA Soloninin, AV Skoryunov, RV Babanova, OA Skripov, AV Unemoto, A Orimo, SI Udovic, TJ AF Tang, Wan Si Matsuo, Motoaki Wu, Hui Stavila, Vitalie Zhou, Wei Talin, Albert Alec Soloninin, Alexei V. Skoryunov, Roman V. Babanova, Olga A. Skripov, Alexander V. Unemoto, Atsushi Orimo, Shin-Ichi Udovic, Terrence J. TI Liquid-Like Ionic Conduction in Solid Lithium and Sodium Monocarba-closo-Decaborates Near or at Room Temperature SO ADVANCED ENERGY MATERIALS LA English DT Article ID ANION REORIENTATIONS; SUPERIONIC CONDUCTION; NA2B12H12; PHASE; LI2B12H12; LIBH4 C1 [Tang, Wan Si] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Tang, Wan Si; Wu, Hui; Zhou, Wei; Udovic, Terrence J.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Matsuo, Motoaki; Orimo, Shin-Ichi] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan. [Stavila, Vitalie; Talin, Albert Alec] Sandia Natl Labs, Energy Nanomat, Livermore, CA 94551 USA. [Soloninin, Alexei V.; Skoryunov, Roman V.; Babanova, Olga A.; Skripov, Alexander V.] Russian Acad Sci, Ural Branch, Inst Met Phys, Ekaterinburg 620990, Russia. [Unemoto, Atsushi; Orimo, Shin-Ichi] Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan. RP Tang, WS (reprint author), Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA.; Tang, WS; Udovic, TJ (reprint author), NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA.; Orimo, SI (reprint author), Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan.; Orimo, SI (reprint author), Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan. EM wansi.tang@nist.gov; orimo@imr.tohoku.ac.jp; udovic@nist.gov RI Babanova, Olga/J-4821-2013; Wu, Hui/C-6505-2008; Zhou, Wei/C-6504-2008; ORIMO, Shin-ichi/A-4971-2011; Unemoto, Atsushi/D-3051-2013; Skripov, Alexander/K-4525-2013; Soloninin, Alexey/J-8580-2013; OI Babanova, Olga/0000-0002-2422-3263; Wu, Hui/0000-0003-0296-5204; Zhou, Wei/0000-0002-5461-3617; ORIMO, Shin-ichi/0000-0002-4216-0446; Skripov, Alexander/0000-0002-0610-5538; Soloninin, Alexey/0000-0001-7127-9641; Skoryunov, Roman/0000-0001-6158-9056 FU Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center - US Department of Energy, Office of Science, Basic Energy Sciences [DESC0001160]; Collaborative Research Center on Energy Materials, Tohoku University; Advanced Low Carbon Technology Research and Development Program (ALCA) from the Japan Science and Technology Agency (JST); JSPS [25220911, 26820311]; Russian Federal Agency of Scientific Organizations under Program "Spin" [01201463330]; Russian Foundation for Basic Research [15-03-01114]; NSF [DMR-0944772]; US DOE National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed, in part, in collaboration between members of IEA HIA Task 32- Hydrogen-based Energy Storage. The authors gratefully acknowledge support from the Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences under Award number DESC0001160; the Collaborative Research Center on Energy Materials, Tohoku University; the Advanced Low Carbon Technology Research and Development Program (ALCA) from the Japan Science and Technology Agency (JST); JSPS KAKENHI under Grant Nos. 25220911 and 26820311; the Russian Federal Agency of Scientific Organizations under Program "Spin" No. 01201463330; and the Russian Foundation for Basic Research under Grant No. 15-03-01114. This work utilized facilities supported in part by the NSF under Agreement No. DMR-0944772. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US DOE National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 22 TC 11 Z9 11 U1 21 U2 40 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD APR 20 PY 2016 VL 6 IS 8 AR 1502237 DI 10.1002/aenm.201502237 PG 6 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DK1VU UT WOS:000374703900011 ER PT J AU Zheng, JM Yan, PF Mei, DH Engelhard, MH Cartmell, SS Polzin, BJ Wang, CM Zhang, JG Xu, W AF Zheng, Jianming Yan, Pengfei Mei, Donghai Engelhard, Mark H. Cartmell, Samuel S. Polzin, Bryant J. Wang, Chongmin Zhang, Ji-Guang Xu, Wu TI Highly Stable Operation of Lithium Metal Batteries Enabled by the Formation of a Transient High-Concentration Electrolyte Layer SO ADVANCED ENERGY MATERIALS LA English DT Article ID ION BATTERIES; LI-ION; SUPERCONCENTRATED ELECTROLYTES; GRAPHITIC ANODE; CARBONATE; SURFACE; SALT; SPECTROSCOPY; INTERPHASE; DEPOSITION AB Lithium (Li) metal has been extensively investigated as an anode for rechargeable battery applications due to its ultrahigh theoretical specific capacity and the lowest redox potential. However, significant challenges including dendrite growth and low Coulombic efficiency are still hindering the practical applications of rechargeable Li metal batteries. It is demonstrated that long-term cycling of Li metal batteries can be realized by the formation of a transient high-concentration electrolyte layer near the surface of Li metal anode during high rate discharge process. The highly concentrated Li+ ions in this transient layer will immediately be solvated by the available solvent molecules and facilitate the formation of a stable and flexible solid electrolyte interphase (SEI) layer composed of a poly(ethylene carbonate) framework integrated with other organic/inorganic lithium salts. This SEI layer largely suppresses the corrosion of Li metal anode attacked by free organic solvents and enables the long-term operation of Li metal batteries. The fundamental findings in this work provide a new direction for the development of Li metal batteries that could be operated at high current densities for a wide range of applications. C1 [Zheng, Jianming; Cartmell, Samuel S.; Zhang, Ji-Guang; Xu, Wu] Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. [Yan, Pengfei; Engelhard, Mark H.; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99354 USA. [Mei, Donghai] Pacific NW Natl Lab, Phys & Computat Sci Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. [Polzin, Bryant J.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zhang, JG; Xu, W (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd, Richland, WA 99354 USA. EM jiguang.zhang@pnnl.gov; wu.xu@pnnl.gov RI yan, pengfei/E-4784-2016; Mei, Donghai/D-3251-2011; Zheng, Jianming/F-2517-2014; Mei, Donghai/A-2115-2012; OI yan, pengfei/0000-0001-6387-7502; Zheng, Jianming/0000-0002-4928-8194; Mei, Donghai/0000-0002-0286-4182; Xu, Wu/0000-0002-2685-8684 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies; Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231, 18769]; DOE's Office of Biological and Environmental Research; DOE [DE-AC05-76RLO1830] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, the Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) under contract no. DE-AC02-05CH11231, subcontract no. 18769. The SEM observations and XPS analysis were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RLO1830. NR 35 TC 5 Z9 5 U1 60 U2 131 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD APR 20 PY 2016 VL 6 IS 8 AR 1502151 DI 10.1002/aenm.201502151 PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DK1VU UT WOS:000374703900008 ER PT J AU Talukdar, I Gorman, DJ Daniilidis, N Schindler, P Ebadi, S Kaufmann, H Zhang, T Haffner, H AF Talukdar, I. Gorman, D. J. Daniilidis, N. Schindler, P. Ebadi, S. Kaufmann, H. Zhang, T. Haffner, H. TI Implications of surface noise for the motional coherence of trapped ions SO PHYSICAL REVIEW A LA English DT Article ID QUANTUM; STATES AB Electric noise from metallic surfaces is a major obstacle towards quantum applications with trapped ions due to motional heating of the ions. Here, we discuss how the same noise source can also lead to pure dephasing of motional quantum states. The mechanism is particularly relevant at small ion-surface distances, thus imposing a constraint on trap miniaturization. By means of a free induction decay experiment, we measure the dephasing time of the motion of a single ion trapped 50 mu m above a Cu-Al surface. From the dephasing times we extract the integrated noise below the secular frequency of the ion. We find that none of the most commonly discussed surface noise models for ion traps describes both the observed heating as well as the measured dephasing satisfactorily. Thus, our measurements provide a benchmark for future models for the electric noise emitted by metallic surfaces. C1 [Talukdar, I.; Gorman, D. J.; Daniilidis, N.; Schindler, P.; Ebadi, S.; Kaufmann, H.; Zhang, T.; Haffner, H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haffner, H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ebadi, S.] Univ Toronto, Toronto, ON, Canada. [Kaufmann, H.] Johannes Gutenberg Univ Mainz, D-55122 Mainz, Germany. [Zhang, T.] Peking Univ, Beijing, Peoples R China. RP Haffner, H (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Haffner, H (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM hhaeffner@berkeley.edu RI Haeffner, Hartmut/D-8046-2012; Schindler, Philipp/E-1485-2017 OI Haeffner, Hartmut/0000-0002-5113-9622; Schindler, Philipp/0000-0002-9461-9650 FU Austrian Science Foundation (FWF) Erwin Schrodinger Stipendium [3600-N27]; Office of the Director of National Intelligence (ODNI), Intelligence Advanced Research Projects Activity (IARPA) through Army Research Office [W911NF-10-1-0284] FX P.S. was supported by the Austrian Science Foundation (FWF) Erwin Schrodinger Stipendium No. 3600-N27. This research was partially funded by the Office of the Director of National Intelligence (ODNI), Intelligence Advanced Research Projects Activity (IARPA), through the Army Research Office Grant No. W911NF-10-1-0284. NR 32 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD APR 20 PY 2016 VL 93 IS 4 AR 043415 DI 10.1103/PhysRevA.93.043415 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DJ9HB UT WOS:000374523500007 ER PT J AU Chen, X Harriger, L Sefat, A Birgeneau, RJ Wilson, SD AF Chen, Xiang Harriger, Leland Sefat, Athena Birgeneau, R. J. Wilson, Stephen D. TI Strain-activated structural anisotropy in BaFe2As2 SO PHYSICAL REVIEW B LA English DT Article ID IRON ARSENIDE SUPERCONDUCTOR; TRANSITION; ORDER AB High-resolution single crystal neutron diffraction measurements are presented probing the magnetostructural response to uniaxial pressure in the iron pnictide parent system BaFe2As2. Scattering data reveal a strain-activated, anisotropic broadening of nuclear Bragg reflections, which increase upon cooling below the resolvable onset of global orthorhombicity. This anisotropy in lattice coherence continues to build until a lower temperature scale-the first-order onset of antiferromagnetism-is reached. Our data suggest that antiferromagnetism and strong magnetoelastic coupling drive the strain-activated lattice response in thismaterial and that the development of anisotropic lattice correlation lengths under strain is a possible origin for the high temperature transport anisotropy in this compound. C1 [Chen, Xiang] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Chen, Xiang; Wilson, Stephen D.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Harriger, Leland] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Sefat, Athena] Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008, Oak Ridge, TN 37831 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. RP Wilson, SD (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM stephendwilson@engineering.ucsb.edu RI Sefat, Athena/R-5457-2016 OI Sefat, Athena/0000-0002-5596-3504 FU NSF CAREER [DMR-1056625]; US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division; US Department of Energy (DOE), Office of Basic Energy Sciences, Materials Science and Engineering Division [DE-AC02-05CH11231] FX This work was supported by NSF CAREER Award DMR-1056625 (S.D.W.). Partial support given by the US Department of Energy (DOE), Office of Basic Energy Sciences (BES), Materials Sciences and Engineering Division (A.S.). The work at Lawrence Berkeley National Laboratory was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Materials Science and Engineering Division, under Contract No. DE-AC02-05CH11231. NR 27 TC 0 Z9 0 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 20 PY 2016 VL 93 IS 14 AR 144118 DI 10.1103/PhysRevB.93.144118 PG 5 WC Physics, Condensed Matter SC Physics GA DJ9KD UT WOS:000374531500003 ER PT J AU Haxton, WC Haxton, DJ AF Haxton, W. C. Haxton, Daniel J. TI Composite fermions and the first-Landau-level fine structure of the fractional quantum Hall effect SO PHYSICAL REVIEW B LA English DT Article ID LANDAU-LEVEL; STATES; HIERARCHY; QUANTIZATION; EXCITATIONS; STATISTICS; FLUID AB A set of scalar operators, originally introduced in connection with an analytic first-Landau-level (FLL) construction of fractional quantum Hall (FQHE) wave functions for the sphere, are employed in a somewhat different way to generate explicit representations of both hierarchy states (e.g., the series of fillings nu = 1/3, 2/5, 3/7, ... ) and their conjugates (nu = 1, 2/3, 3/5, ... ) as noninteracting quasielectrons filling fine-structure subshells within the FLL. This yields, for planar and spherical geometries, a quasielectron representation of the incompressible FLL state of filling p/(2p + 1) in a magnetic field of strength B that is algebraically identical to the IQHE state of filling nu = p in a magnetic field of strength B/(2p + 1). The construction provides a precise definition of the quasielectron/composite fermion that differs in some respects from common descriptions: they are eigenstates of L, L-z; they and the FLL subshells they occupy carry a third index I that is associated with breaking of scalar pairs; they absorb in their internal wave functions one, not two, units of magnetic flux; and they share a common, simple structure as vector products of a spinor creating an electron and one creating magnetic flux. We argue that these properties are a consequence of the breaking of the degeneracy of noninteracting electrons within the FLL by the scale-invariant Coulomb potential. We discuss the sense in which the wave function construction supports basic ideas of both composite fermion and hierarchical descriptions of the FQHE. We describe symmetries of the quasielectrons in the nu = 1/2 limit, where a deep Fermi sea of quasielectrons forms, and the quasielectrons take on Majorana and pseudo-Dirac characters. Finally, we show that the wave functions can be viewed as fermionic excitations of the bosonic half-filled shell, producing at nu = 1/2 an operator that differs from but plays the same role as the Pfaffian. C1 [Haxton, W. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Haxton, W. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Haxton, Daniel J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Haxton, WC (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Haxton, WC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Haxton, DJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM haxton@berkeley.edu; djhaxton@lbl.gov FU US DOE [DE-AC02-05CH11231, DE-SC00046548, DE-FG02-94ER14413]; Peder Sather Center FX We thank Joe Ginocchio for the very enjoyable collaboration that produced the 1996 paper, Susanne Viefers for suggesting that we supply the missing Ref. [12] in GH, and Byungmin Kang and Ken McElvain for help and comments. This work was supported in part by the US DOE under DE-AC02-05CH11231 (LBL) DE-SC00046548 (Berkeley), and DE-FG02-94ER14413 (Colorado). We also acknowledge support from the Peder Sather Center. NR 35 TC 0 Z9 0 U1 2 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 20 PY 2016 VL 93 IS 15 AR 155138 DI 10.1103/PhysRevB.93.155138 PG 25 WC Physics, Condensed Matter SC Physics GA DJ9LC UT WOS:000374534000002 ER PT J AU Taddei, KM Allred, JM Bugaris, DE Lapidus, S Krogstad, MJ Stadel, R Claus, H Chung, DY Kanatzidis, MG Rosenkranz, S Osborn, R Chmaissem, O AF Taddei, K. M. Allred, J. M. Bugaris, D. E. Lapidus, S. Krogstad, M. J. Stadel, R. Claus, H. Chung, D. Y. Kanatzidis, M. G. Rosenkranz, S. Osborn, R. Chmaissem, O. TI Detailed magnetic and structural analysis mapping a robust magnetic C-4 dome in Sr1-xNaxFe2As2 SO PHYSICAL REVIEW B LA English DT Article ID NEMATIC ORDER; SUPERCONDUCTOR; BA1-XKXFE2AS2 AB The recently discovered C-4 tetragonal magnetic phase in hole-doped members of the iron-based superconductors provides insights into the origin of unconventional superconductivity. Previously observed in Ba1-xNaxFe2As2 (with A = K, Na), the C-4 magnetic phase exists within the well-studied C-2 spin-density-wave dome, arising just before the complete suppression of antiferromagnetic order but after the onset of superconductivity. Here, we present detailed x-ray and neutron diffraction studies of Sr1-xNaxFe2As2 (0.10 <= x <= 0.60) to determine their structural evolution and the extent of the C-4 phase. Spanning Delta x similar to 0.14 in composition, the C-4 phase is found to extend over a larger range of compositions, and to exhibit a significantly higher transition temperature, T-r similar to 65 K, than in either of the other systems in which it has been observed. The onset of this phase is seen near a composition (x similar to 0.30) where the bonding angles of the Fe2As2 layers approach the perfect 109.46 degrees tetrahedral angle. We discuss the possible role of this return to a higher symmetry environment for the magnetic iron site in triggering the magnetic reorientation and the coupled reentrance to the tetragonal structure. Finally, we present a phase diagram, complete with the C-4 phase, and use its observation in a third hole-doped 122 system to suggest the universality of this phase. C1 [Taddei, K. M.; Krogstad, M. J.; Stadel, R.; Chmaissem, O.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Taddei, K. M.; Allred, J. M.; Bugaris, D. E.; Krogstad, M. J.; Stadel, R.; Claus, H.; Chung, D. Y.; Kanatzidis, M. G.; Rosenkranz, S.; Osborn, R.; Chmaissem, O.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Allred, J. M.] Univ Alabama, Dept Chem, Box 870336, Tuscaloosa, AL 35487 USA. [Lapidus, S.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Kanatzidis, M. G.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. RP Taddei, KM (reprint author), No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA.; Taddei, KM (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ktaddei@anl.gov RI Taddei, Keith/K-4641-2016; Allred, Jared/N-4719-2014; Rosenkranz, Stephan/E-4672-2011 OI Taddei, Keith/0000-0002-1468-0823; Allred, Jared/0000-0002-5953-300X; Rosenkranz, Stephan/0000-0002-5659-0383 FU US Department of Energy, Office of Science, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The work at the Materials Science Division at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, Materials Sciences and Engineering Division. The part of the research that was conducted at the ANL Advanced Photon Source and at the ORNL High Flux Isotope Reactor and Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The authors thank A. Huq, P. Whitfield, and A. A. Aczel for providing help during experimental collection and analysis. NR 44 TC 3 Z9 3 U1 6 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 20 PY 2016 VL 93 IS 13 AR 134510 DI 10.1103/PhysRevB.93.134510 PG 12 WC Physics, Condensed Matter SC Physics GA DJ9JD UT WOS:000374528900004 ER PT J AU Akerib, DS Araujo, HM Bai, X Bailey, AJ Balajthy, J Beltrame, P Bernard, EP Bernstein, A Biesiadzinski, TP Boulton, EM Bradley, A Bramante, R Cahn, SB Carmona-Benitez, MC Chan, C Chapman, JJ Chiller, AA Chiller, C Currie, A Cutter, JE Davison, TJR de Viveiros, L Dobi, A Dobson, JEY Druszkiewicz, E Edwards, BN Faham, CH Fiorucci, S Gaitskell, RJ Gehman, VM Ghag, C Gibson, KR Gilchriese, MGD Hall, CR Hanhardt, M Haselschwardt, SJ Hertel, SA Hogan, DP Horn, M Huang, DQ Ignarra, CM Ihm, M Jacobsen, RG Ji, W Kazkaz, K Khaitan, D Knoche, R Larsen, NA Lee, C Lenardo, BG Lesko, KT Lindote, A Lopes, MI Malling, DC Manalaysay, AG Mannino, RL Marzioni, MF McKinsey, DN Mei, DM Mock, J Moongweluwan, M Morad, JA Murphy, AS Nehrkorn, C Nelson, HN Neves, F O'Sullivan, K Oliver-Mallory, KC Ott, RA Palladino, KJ Pangilinan, M Pease, EK Phelps, P Reichhart, L Rhyne, C Shaw, S Shutt, TA Silva, C Solovov, VN Sorensen, P Stephenson, S Sumner, TJ Szydagis, M Taylor, DJ Taylor, W Tennyson, BP Terman, PA Tiedt, DR To, WH Tripathi, M Tvrznikova, L Uvarov, S Verbus, JR Webb, RC White, JT Whitis, TJ Witherell, MS Wolfs, FLH Young, SK Zhang, C AF Akerib, D. S. Araujo, H. M. Bai, X. Bailey, A. J. Balajthy, J. Beltrame, P. Bernard, E. P. Bernstein, A. Biesiadzinski, T. P. Boulton, E. M. Bradley, A. Bramante, R. Cahn, S. B. Carmona-Benitez, M. C. Chan, C. Chapman, J. J. Chiller, A. A. Chiller, C. Currie, A. Cutter, J. E. Davison, T. J. R. de Viveiros, L. Dobi, A. Dobson, J. E. Y. Druszkiewicz, E. Edwards, B. N. Faham, C. H. Fiorucci, S. Gaitskell, R. J. Gehman, V. M. Ghag, C. Gibson, K. R. Gilchriese, M. G. D. Hall, C. R. Hanhardt, M. Haselschwardt, S. J. Hertel, S. A. Hogan, D. P. Horn, M. Huang, D. Q. Ignarra, C. M. Ihm, M. Jacobsen, R. G. Ji, W. Kazkaz, K. Khaitan, D. Knoche, R. Larsen, N. A. Lee, C. Lenardo, B. G. Lesko, K. T. Lindote, A. Lopes, M. I. Malling, D. C. Manalaysay, A. G. Mannino, R. L. Marzioni, M. F. McKinsey, D. N. Mei, D. -M. Mock, J. Moongweluwan, M. Morad, J. A. Murphy, A. St. J. Nehrkorn, C. Nelson, H. N. Neves, F. O'Sullivan, K. Oliver-Mallory, K. C. Ott, R. A. Palladino, K. J. Pangilinan, M. Pease, E. K. Phelps, P. Reichhart, L. Rhyne, C. Shaw, S. Shutt, T. A. Silva, C. Solovov, V. N. Sorensen, P. Stephenson, S. Sumner, T. J. Szydagis, M. Taylor, D. J. Taylor, W. Tennyson, B. P. Terman, P. A. Tiedt, D. R. To, W. H. Tripathi, M. Tvrznikova, L. Uvarov, S. Verbus, J. R. Webb, R. C. White, J. T. Whitis, T. J. Witherell, M. S. Wolfs, F. L. H. Young, S. K. Zhang, C. CA LUX Collaboration TI Tritium calibration of the LUX dark matter experiment SO PHYSICAL REVIEW D LA English DT Article ID XENON; ENERGY; PARTICLES; DECAY; GASES AB We present measurements of the electron-recoil (ER) response of the LUX dark matter detector based upon 170 000 highly pure and spatially uniform tritium decays. We reconstruct the tritium energy spectrum using the combined energy model and find good agreement with expectations. We report the average charge and light yields of ER events in liquid xenon at 180 and 105 V/cm and compare the results to the NEST model. We also measure the mean charge recombination fraction and its fluctuations, and we investigate the location and width of the LUX ER band. These results provide input to a reanalysis of the LUX run 3 weakly interacting massive particle search. C1 [Akerib, D. S.; Biesiadzinski, T. P.; Bradley, A.; Bramante, R.; Gibson, K. R.; Ji, W.; Lee, C.; Phelps, P.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Case Western Reserve Univ, Dept Phys, 10900 Euclid Ave, Cleveland, OH 44106 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94205 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94309 USA. [Araujo, H. M.; Bailey, A. J.; Currie, A.; Sumner, T. J.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys, Prince Consort Rd, London SW7 2BZ, England. [Bai, X.; Hanhardt, M.; Tiedt, D. R.] South Dakota Sch Mines & Technol, 501 East St Joseph St, Rapid City, SD 57701 USA. [Balajthy, J.; Hall, C. R.; Knoche, R.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beltrame, P.; Davison, T. J. R.; Marzioni, M. F.; Murphy, A. St. J.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh EH9 3FD, Midlothian, Scotland. [Bernard, E. P.; Boulton, E. M.; Cahn, S. B.; Edwards, B. N.; Hertel, S. A.; Horn, M.; Larsen, N. A.; McKinsey, D. N.; O'Sullivan, K.; Pease, E. K.; Tennyson, B. P.; Tvrznikova, L.] Yale Univ, Dept Phys, 217 Prospect St, New Haven, CT 06511 USA. [Bernstein, A.; Kazkaz, K.; Lenardo, B. G.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. [Carmona-Benitez, M. C.; Haselschwardt, S. J.; Nehrkorn, C.; Nelson, H. N.; Witherell, M. S.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Chan, C.; Chapman, J. J.; Fiorucci, S.; Gaitskell, R. J.; Huang, D. Q.; Malling, D. C.; Pangilinan, M.; Rhyne, C.; Taylor, W.; Verbus, J. R.] Brown Univ, Dept Phys, 182 Hope St, Providence, RI 02912 USA. [Chiller, A. A.; Chiller, C.; Mei, D. -M.; Zhang, C.] Univ S Dakota, Dept Phys, 414E Clark St, Vermillion, SD 57069 USA. [Cutter, J. E.; Lenardo, B. G.; Manalaysay, A. G.; Morad, J. A.; Ott, R. A.; Stephenson, S.; Tripathi, M.; Uvarov, S.] Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. [de Viveiros, L.; Lindote, A.; Lopes, M. I.; Neves, F.; Silva, C.; Solovov, V. N.] Univ Coimbra, Dept Phys, LIP Coimbra, Rua Larga, P-3004516 Coimbra, Portugal. [Dobi, A.; Faham, C. H.; Gehman, V. M.; Gilchriese, M. G. D.; Lesko, K. T.; O'Sullivan, K.; Sorensen, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Dobson, J. E. Y.; Ghag, C.; Reichhart, L.; Shaw, S.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Druszkiewicz, E.; Khaitan, D.; Moongweluwan, M.; Wolfs, F. L. H.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Hanhardt, M.; Taylor, D. J.] South Dakota Sci & Technol Author, Sanford Underground Res Facil, Lead, SD 57754 USA. [Hertel, S. A.; Hogan, D. P.; Horn, M.; Ihm, M.; Jacobsen, R. G.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mannino, R. L.; Terman, P. A.; Webb, R. C.; White, J. T.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Mock, J.; Szydagis, M.; Young, S. K.] SUNY Albany, Dept Phys, 1400 Washington Ave, Albany, NY 12222 USA. RP Akerib, DS (reprint author), Case Western Reserve Univ, Dept Phys, 10900 Euclid Ave, Cleveland, OH 44106 USA. OI Horn, Markus/0000-0003-1624-9890; Tvrznikova, Lucie/0000-0002-0394-7692 FU U.S. Department of Energy (DOE) [DE-FG02-08ER41549, DE-FG02-91ER40688, DE-FG02-95ER40917, DE-FG02-91ER40674, DE-NA0000979, DE-FG02-11ER41738, DE-SC0006605, DE-AC02-05CH11231, DE-AC52-07NA27344, DE-FG01-91ER40618]; U.S. National Science Foundation [PHYS-0750671, PHY-0801536, PHY-1004661, PHY-1102470, PHY-1003660, PHY-1312561, PHY-1347449, PHY-1505868]; Center for Ultra-low Background Experiments in the Dakotas (CUBED); South Dakota School of Mines and Technology (SDSMT); Fundacao para a Ciencia e a Tecnologia (FCT) [PTDC/FIS-NUC/1525/2014]; Science and Technology Facilities Council [ST/K502042/1]; United Kingdom Royal Society [IE120804]; [RA0350] FX This work was partially supported by the U.S. Department of Energy (DOE) under Awards No. DE-FG02-08ER41549, No. DE-FG02-91ER40688, No. DE-FG02-95ER40917, No. DE-FG02-91ER40674, No. DE-NA0000979, No. DE-FG02-11ER41738, No. DE-SC0006605, No. DE-AC02-05CH11231, No. DE-AC52-07NA27344, and No. DE-FG01-91ER40618; the U.S. National Science Foundation under Grants No. PHYS-0750671, No. PHY-0801536, No. PHY-1004661, No. PHY-1102470, No. PHY-1003660, No. PHY-1312561, No. PHY-1347449, and No. PHY-1505868; the Research Corporation Grant No. RA0350; the Center for Ultra-low Background Experiments in the Dakotas (CUBED); and the South Dakota School of Mines and Technology (SDSMT). LIP-Coimbra acknowledges funding from Fundacao para a Ciencia e a Tecnologia (FCT) through Project-Grant No. PTDC/FIS-NUC/1525/2014. Imperial College and Brown University thank the United Kingdom Royal Society for travel funds under the International Exchange Scheme (IE120804). The United Kingdom groups acknowledge institutional support from Imperial College London, University College London and Edinburgh University, and from the Science and Technology Facilities Council for PhD studentship ST/K502042/1 (A. B.). The University of Edinburgh is a charitable body, registered in Scotland, with registration number SC005336. This research was conducted using computational resources and services at the Center for Computation and Visualization, Brown University. We gratefully acknowledge the logistical and technical support and the access to laboratory infrastructure provided to us by the SURF and its personnel at Lead, South Dakota. SURF was developed by the South Dakota Science and Technology Authority, with an important philanthropic donation from T. Denny Sanford, and is operated by Lawrence Berkeley National Laboratory for the Department of Energy, Office of High Energy Physics. NR 30 TC 6 Z9 6 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 20 PY 2016 VL 93 IS 7 AR 072009 DI 10.1103/PhysRevD.93.072009 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QM UT WOS:000374548000002 ER PT J AU Fukushima, K Hattori, K Yee, HU Yin, Y AF Fukushima, Kenji Hattori, Koichi Yee, Ho-Ung Yin, Yi TI Heavy quark diffusion in strong magnetic fields at weak coupling and implications for elliptic flow SO PHYSICAL REVIEW D LA English DT Article ID ION COLLISIONS; VACUUM BIREFRINGENCE; GAUGE-INVARIANCE; SCHWINGER MODEL; VIOLATION; TRANSPORT; FLAVOR; EVENT; MASS AB We compute the momentum diffusion coefficients of heavy quarks, kappa(parallel to) and kappa(perpendicular to), in a strong magnetic field B along the directions parallel and perpendicular to B, respectively, at the leading order in QCD coupling constant alpha(s). We consider a regime relevant for the relativistic heavy ion collisions, alpha(s)eB << T-2 << eB, so that thermal excitations of light quarks are restricted to the lowest Landau level (LLL) states. In the vanishing light-quark mass limit, we find kappa(LO)(perpendicular to) proportional to alpha(sTeB)-Te-2 in the leading order that arises from screened Coulomb scatterings with (1 + 1)-dimensional LLL quarks, while kappa(parallel to) gets no contribution from the scatterings with LLL quarks due to kinematic restrictions. We show that the first nonzero leading order contributions to kappa(LO)(parallel to) come from the two separate effects: (1) the screened Coulomb scatterings with thermal gluons, and (2) a finite light-quark mass m(q). The former leads to kappa(LO,gluon)(parallel to) proportional to alpha T-2(s)3 and the latter to kappa(LO,massive)(parallel to) proportional to alpha(s)(alpha(s)eB)(1/2)m(q)(2). Based on our results, we propose a new scenario for the large value of heavy-quark elliptic flow observed in RHIC and LHC. Namely, when kappa(perpendicular to) >> kappa(parallel to), an anisotropy in drag forces gives rise to a sizable amount of the heavy-quark elliptic flow even if heavy quarks do not fully belong to an ellipsoidally expanding background fluid. C1 [Fukushima, Kenji] Univ Tokyo, Dept Phys, 7-3-1 Bunkyo Ku, Tokyo 1130033, Japan. [Hattori, Koichi; Yee, Ho-Ung] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Hattori, Koichi] RIKEN, Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Yee, Ho-Ung] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Yin, Yi] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fukushima, K (reprint author), Univ Tokyo, Dept Phys, 7-3-1 Bunkyo Ku, Tokyo 1130033, Japan.; Hattori, K; Yee, HU (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; Hattori, K (reprint author), RIKEN, Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan.; Yee, HU (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA.; Yin, Y (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM fuku@nt.phys.s.u-tokyo.ac.jp; koichi.hattori@riken.jp; hyee@uic.edu; yyin@bnl.gov FU JSPS KAKENHI Grants [15H03652, 15K13479]; JSPS [25287066]; DOE [DE-SC0012704] FX We thank Yukinao Akamatsu, Koichi Murase, Jorge Noronha, Hiroshi Ohno, Rob Pisarski, Alexander Rothkopf, Bjoern Schenke, and Sayantan Sharma for helpful discussions. K. F. is supported by JSPS KAKENHI Grants No. 15H03652 and No. 15K13479, K. H. is supported by JSPS Grants-in-Aid No. 25287066, and Y. Y. is supported by DOE Contract No. DE-SC0012704. NR 66 TC 7 Z9 7 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 20 PY 2016 VL 93 IS 7 AR 074028 DI 10.1103/PhysRevD.93.074028 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QM UT WOS:000374548000008 ER PT J AU Lazanu, A Giannantonio, T Schmittfull, M Shellard, EPS AF Lazanu, Andrei Giannantonio, Tommaso Schmittfull, Marcel Shellard, E. P. S. TI Matter bispectrum of large-scale structure: Three-dimensional comparison between theoretical models and numerical simulations SO PHYSICAL REVIEW D LA English DT Article ID PRIMORDIAL NON-GAUSSIANITY; 3-POINT CORRELATION-FUNCTION; COSMOLOGICAL POWER SPECTRA; GALAXY REDSHIFT SURVEY; OSCILLATION SPECTROSCOPIC SURVEY; LAGRANGIAN PERTURBATION-THEORY; FRIEDMAN-LEMAITRE COSMOLOGIES; N-BODY SIMULATIONS; DIGITAL SKY SURVEY; GRAVITATIONAL-INSTABILITY AB We study the matter bispectrum of the large-scale structure by comparing different perturbative and phenomenological models with measurements from N-body simulations obtained with a modal bispectrum estimator. Using shape and amplitude correlators, we directly compare simulated data with theoretical models over the full three-dimensional domain of the bispectrum, for different redshifts and scales. We review and investigate the main perturbative methods in the literature that predict the one-loop bispectrum: standard perturbation theory, effective field theory, resummed Lagrangian and renormalized perturbation theory, calculating the latter also at two loops for some triangle configurations. We find that effective field theory (EFT) succeeds in extending the range of validity furthest into the mildly nonlinear regime, albeit at the price of free extra parameters requiring calibration on simulations: EFT is found to be accurate to 5% up to a scale of k(max)* similar or equal to 0.4 h/Mpc at z = 1, compared with k(max)* similar or equal to 0.2 h/Mpc at z = 1 for most other one-loop perturbative methods. For the more phenomenological halo model, we confirm that despite its validity in the deeply nonlinear regime it has a deficit of power on intermediate scales, which worsens at higher redshifts (the maximum deficit in the amplitude correlator is similar to 20% at z = 1, and up to 40% at z = 2); this issue is ameliorated, but not solved, by combined halo-perturbative models. We show from simulations that in this transition region there is a strong squeezed bispectrum component that is significantly underestimated in the halo model at earlier redshifts. We thus propose a phenomenological method for alleviating this deficit, which we develop into a simple phenomenological "three-shape" benchmark model based on the three fundamental shapes we have obtained from studying the halo model. When calibrated on the simulations, this three-shape benchmark model accurately describes the bispectrum on all scales and redshifts considered, providing a prototype bispectrum HALOFIT-like methodology that could be used to describe and test parameter dependencies. C1 [Lazanu, Andrei; Giannantonio, Tommaso; Shellard, E. P. S.] Univ Cambridge, DAMTP, Ctr Theoret Cosmol, Cambridge CB3 0WA, England. [Giannantonio, Tommaso] Univ Cambridge, Inst Astron, Kavli Inst Cosmol Cambridge, Madingley Rd, Cambridge CB3 0HA, England. [Schmittfull, Marcel] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Schmittfull, Marcel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lazanu, A; Giannantonio, T; Shellard, EPS (reprint author), Univ Cambridge, DAMTP, Ctr Theoret Cosmol, Cambridge CB3 0WA, England.; Giannantonio, T (reprint author), Univ Cambridge, Inst Astron, Kavli Inst Cosmol Cambridge, Madingley Rd, Cambridge CB3 0HA, England.; Schmittfull, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA.; Schmittfull, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM A.Lazanu@damtp.cam.ac.uk; T.Giannantonio@ast.cam.ac.uk; M.Schmittfull@berkeley.edu; E.P.S.Shellard@damtp.cam.ac.uk OI Lazanu, Andrei/0000-0002-8061-9828 FU STFC [ST/L000636/1, ST/H008586/1, ST/K00333X/1, STM007065/1]; Kavli Foundation; BIS National E-infrastructure Capital [ST/J005673/1] FX We wish to thank Martin Crocce, James Fergusson, Donough Regan, Daniel Baumann, Cristiano Porciani, and Christian Wagner for useful discussions, and Eiichiro Komatsu and Emiliano Sefusatti for comments on an earlier version of this work. A. L., T. G., and E. P. S. S. are supported by STFC Grant No. ST/L000636/1. T. G. also acknowledges support from the Kavli Foundation. This work was undertaken on the COSMOS Shared Memory system at DAMTP, University of Cambridge, operated on behalf of the STFC DiRAC HPC Facility. This equipment is funded by BIS National E-infrastructure Capital Grant No. ST/J005673/1 and STFC Grants No. ST/H008586/1, No. ST/K00333X/1 and No. STM007065/1. The 3D bispectrum visualizations used the OSPRay ray-tracing rendering engine and we are grateful for support from Johannes Guenther and Gregory Johnson, Intel Corporation. NR 168 TC 4 Z9 4 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 20 PY 2016 VL 93 IS 8 AR 083517 DI 10.1103/PhysRevD.93.083517 PG 49 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9RZ UT WOS:000374551900003 ER PT J AU Akerib, DS Araujo, HM Bai, X Bailey, AJ Balajthy, J Beltrame, P Bernard, EP Bernstein, A Biesiadzinski, TP Boulton, EM Bradley, A Bramante, R Cahn, SB Carmona-Benitez, MC Chan, C Chapman, JJ Chiller, AA Chiller, C Currie, A Cutter, JE Davison, TJR de Viveiros, L Dobi, A Dobson, JEY Druszkiewicz, E Edwards, BN Faham, CH Fiorucci, S Gaitskell, RJ Gehman, VM Ghag, C Gibson, KR Gilchriese, MGD Hall, CR Hanhardt, M Haselschwardt, SJ Hertel, SA Hogan, DP Horn, M Huang, DQ Ignarra, CM Ihm, M Jacobsen, RG Ji, W Kazkaz, K Khaitan, D Knoche, R Larsen, NA Lee, C Lenardo, BG Lesko, KT Lindote, A Lopes, MI Malling, DC Manalaysay, A Mannino, RL Marzioni, MF McKinsey, DN Mei, DM Mock, J Moongweluwan, M Morad, JA Murphy, AS Nehrkorn, C Nelson, HN Neves, F O'Sullivan, K Oliver-Mallory, KC Ott, RA Palladino, KJ Pangilinan, M Pease, EK Phelps, P Reichhart, L Rhyne, C Shaw, S Shutt, TA Silva, C Solovov, VN Sorensen, P Stephenson, S Sumner, TJ Szydagis, M Taylor, DJ Taylor, W Tennyson, BP Terman, PA Tiedt, DR To, WH Tripathi, M Tvrznikova, L Uvarov, S Verbus, JR Webb, RC White, JT Whitis, TJ Witherell, MS Wolfs, FLH Yazdani, K Young, SK Zhang, C AF Akerib, D. S. Araujo, H. M. Bai, X. Bailey, A. J. Balajthy, J. Beltrame, P. Bernard, E. P. Bernstein, A. Biesiadzinski, T. P. Boulton, E. M. Bradley, A. Bramante, R. Cahn, S. B. Carmona-Benitez, M. C. Chan, C. Chapman, J. J. Chiller, A. A. Chiller, C. Currie, A. Cutter, J. E. Davison, T. J. R. de Viveiros, L. Dobi, A. Dobson, J. E. Y. Druszkiewicz, E. Edwards, B. N. Faham, C. H. Fiorucci, S. Gaitskell, R. J. Gehman, V. M. Ghag, C. Gibson, K. R. Gilchriese, M. G. D. Hall, C. R. Hanhardt, M. Haselschwardt, S. J. Hertel, S. A. Hogan, D. P. Horn, M. Huang, D. Q. Ignarra, C. M. Ihm, M. Jacobsen, R. G. Ji, W. Kazkaz, K. Khaitan, D. Knoche, R. Larsen, N. A. Lee, C. Lenardo, B. G. Lesko, K. T. Lindote, A. Lopes, M. I. Malling, D. C. Manalaysay, A. Mannino, R. L. Marzioni, M. F. McKinsey, D. N. Mei, D. -M. Mock, J. Moongweluwan, M. Morad, J. A. Murphy, A. St. J. Nehrkorn, C. Nelson, H. N. Neves, F. O'Sullivan, K. Oliver-Mallory, K. C. Ott, R. A. Palladino, K. J. Pangilinan, M. Pease, E. K. Phelps, P. Reichhart, L. Rhyne, C. Shaw, S. Shutt, T. A. Silva, C. Solovov, V. N. Sorensen, P. Stephenson, S. Sumner, T. J. Szydagis, M. Taylor, D. J. Taylor, W. Tennyson, B. P. Terman, P. A. Tiedt, D. R. To, W. H. Tripathi, M. Tvrznikova, L. Uvarov, S. Verbus, J. R. Webb, R. C. White, J. T. Whitis, T. J. Witherell, M. S. Wolfs, F. L. H. Yazdani, K. Young, S. K. Zhang, C. CA LUX Collaboration TI Improved Limits on Scattering of Weakly Interacting Massive Particles from Reanalysis of 2013 LUX Data SO PHYSICAL REVIEW LETTERS LA English DT Article ID DARK-MATTER CANDIDATES; LIQUID ARGON; XENON; SCINTILLATION; DETECTOR; ENERGY AB We present constraints on weakly interacting massive particles (WIMP)-nucleus scattering from the 2013 data of the Large Underground Xenon dark matter experiment, including 1.4 x 10(4) kg day of search exposure. This new analysis incorporates several advances: single-photon calibration at the scintillation wavelength, improved event-reconstruction algorithms, a revised background model including events originating on the detector walls in an enlarged fiducial volume, and new calibrations from decays of an injected tritium beta source and from kinematically constrained nuclear recoils down to 1.1 keV. Sensitivity, especially to low-mass WIMPs, is enhanced compared to our previous results which modeled the signal only above a 3 keV minimum energy. Under standard dark matter halo assumptions and in the mass range above 4 GeV c(-2), these new results give the most stringent direct limits on the spin- independent WIMP- nucleon cross section. The 90% C. L. upper limit has a minimum of 0.6 zb at 33 GeV c(-2) WIMP mass. C1 [Akerib, D. S.; Biesiadzinski, T. P.; Bradley, A.; Bramante, R.; Gibson, K. R.; Ji, W.; Lee, C.; Phelps, P.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Case Western Reserve Univ, Dept Phys, 10900 Euclid Ave, Cleveland, OH 44106 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94205 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94309 USA. [Araujo, H. M.; Bailey, A. J.; Currie, A.; Sumner, T. J.; Yazdani, K.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys, Prince Consort Rd, London SW7 2BZ, England. [Bai, X.; Hanhardt, M.; Tiedt, D. R.] South Dakota Sch Mines & Technol, 501 East St Joseph St, Rapid City, SD 57701 USA. [Balajthy, J.; Hall, C. R.; Knoche, R.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beltrame, P.; Davison, T. J. R.; Marzioni, M. F.; Murphy, A. St. J.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh EH9 3FD, Midlothian, Scotland. [Bernard, E. P.; Boulton, E. M.; Cahn, S. B.; Edwards, B. N.; Hertel, S. A.; Horn, M.; Larsen, N. A.; McKinsey, D. N.; O'Sullivan, K.; Pease, E. K.; Tennyson, B. P.; Tvrznikova, L.] Yale Univ, Dept Phys, 217 Prospect St, New Haven, CT 06511 USA. [Bernstein, A.; Kazkaz, K.; Lenardo, B. G.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. [Carmona-Benitez, M. C.; Haselschwardt, S. J.; Nehrkorn, C.; Nelson, H. N.; Witherell, M. S.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Chan, C.; Chapman, J. J.; Gaitskell, R. J.; Huang, D. Q.; Malling, D. C.; Pangilinan, M.; Rhyne, C.; Taylor, W.; Verbus, J. R.] Brown Univ, Dept Phys, 182 Hope St, Providence, RI 02912 USA. [Chiller, A. A.; Chiller, C.; Mei, D. -M.; Zhang, C.] Univ S Dakota, Dept Phys, 414E Clark St, Vermillion, SD 57069 USA. [Cutter, J. E.; Lenardo, B. G.; Manalaysay, A.; Morad, J. A.; Ott, R. A.; Stephenson, S.; Tripathi, M.; Uvarov, S.] Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. [de Viveiros, L.; Lindote, A.; Lopes, M. I.; Neves, F.; Silva, C.; Solovov, V. N.] Univ Coimbra, Dept Phys, LIP Coimbra, Rua Larga, P-3004516 Coimbra, Portugal. [Dobi, A.; Faham, C. H.; Fiorucci, S.; Gehman, V. M.; Gilchriese, M. G. D.; Hertel, S. A.; Horn, M.; Ihm, M.; Jacobsen, R. G.; Lesko, K. T.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.; Pease, E. K.; Sorensen, P.; Tvrznikova, L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Dobson, J. E. Y.; Ghag, C.; Reichhart, L.; Shaw, S.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Druszkiewicz, E.; Khaitan, D.; Moongweluwan, M.; Wolfs, F. L. H.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Hanhardt, M.; Taylor, D. J.] South Dakota Sci & Technol Author, Sanford Underground Res Facil, Lead, SD 57754 USA. [Hertel, S. A.; Hogan, D. P.; Horn, M.; Ihm, M.; Jacobsen, R. G.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.; Pease, E. K.; Tvrznikova, L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mannino, R. L.; Terman, P. A.; Webb, R. C.; White, J. T.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Mock, J.; Szydagis, M.; Young, S. K.] SUNY Albany, Dept Phys, 1400 Washington Ave, Albany, NY 12222 USA. [Palladino, K. J.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. RP Currie, A (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys, Prince Consort Rd, London SW7 2BZ, England. EM alastair.currie08@imperial.ac.uk OI Horn, Markus/0000-0003-1624-9890; Tvrznikova, Lucie/0000-0002-0394-7692 FU U.S. Department of Energy (DOE) [DE-FG02-08ER41549, DE-FG02-91ER40688, DE-FG02-95ER40917, DE-FG02-91ER40674, DE-NA0000979, DE-FG02-11ER41738, DE-SC0006605, DE-AC02-05CH11231, DE-AC52-07NA27344, DE-FG01-91ER40618]; U.S. National Science Foundation [PHYS-0750671, PHY-0801536, PHY-1004661, PHY-1102470, PHY-1003660, PHY-1312561, PHY-1347449]; Research Corporation Grant [RA0350]; Center for Ultra-low Background Experiments in the Dakotas (CUBED); South Dakota School of Mines and Technology (SDSMT); Fundacao para a Ciencia e a Tecnologia (FCT) [PTDC/FIS-NUC/1525/2014]; UK Royal Society [IE120804]; Science and Technology Facilities Council [ST/K502042/1, ST/K502406/1, ST/M503538/1] FX This work was partially supported by the U.S. Department of Energy (DOE) under Awards No. DE-FG02-08ER41549, No. DE-FG02-91ER40688, No. DE-FG02-95ER40917, No. DE-FG02-91ER40674, No. DE-NA0000979, No. DE-FG02-11ER41738, No. DE-SC0006605, No. DE-AC02-05CH11231, No. DE-AC52-07NA27344, and No. DE-FG01-91ER40618; the U.S. National Science Foundation under Grant No. PHYS-0750671, No. PHY-0801536, No. PHY-1004661, No. PHY-1102470, No. PHY-1003660, No. PHY-1312561, No. PHY-1347449; the Research Corporation Grant No. RA0350; the Center for Ultra-low Background Experiments in the Dakotas (CUBED); and the South Dakota School of Mines and Technology (SDSMT). LIP-Coimbra acknowledges funding from Fundacao para a Ciencia e a Tecnologia (FCT) through the Project-Grant No. PTDC/FIS-NUC/1525/2014. Imperial College and Brown University thank the UK Royal Society for travel funds under the International Exchange Scheme (IE120804). The UK groups acknowledge institutional support from Imperial College London, University College London and Edinburgh University, and from the Science and Technology Facilities Council for PhD Studentships No. ST/K502042/1 (AB), No. ST/K502406/1 (SS), and No. ST/M503538/1 (KY). The University of Edinburgh is a charitable body, registered in Scotland, with Registration No. SC005336. This research was conducted using computational resources and services at the Center for Computation and Visualization, Brown University. We gratefully acknowledge the logistical and technical support and the access to laboratory infrastructure provided to us by the Sanford Underground Research Facility (SURF) and its personnel at Lead, South Dakota. SURF was developed by the South Dakota Science and Technology Authority, with an important philanthropic donation from T. Denny Sanford, and is operated by Lawrence Berkeley National Laboratory for the Department of Energy, Office of High Energy Physics. We thank Felix Kahlhoefer and Sebastien Wild for uncovering a mistake in a preprint of this work. NR 46 TC 101 Z9 101 U1 8 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 20 PY 2016 VL 116 IS 16 AR 161301 DI 10.1103/PhysRevLett.116.161301 PG 7 WC Physics, Multidisciplinary SC Physics GA DJ9UU UT WOS:000374559300003 PM 27152785 ER PT J AU Akerib, DS Araujo, HM Bai, X Bailey, AJ Balajthy, J Beltrame, P Bernard, EP Bernstein, A Biesiadzinski, TP Boulton, EM Bradley, A Bramante, R Cahn, SB Carmona-Benitez, MC Chan, C Chapman, JJ Chiller, AA Chiller, C Currie, A Cutter, JE Davison, TJR de Viveiros, L Dobi, A Dobson, JEY Druszkiewicz, E Edwards, BN Faham, CH Fiorucci, S Gaitskell, RJ Gehman, VM Ghag, C Gibson, KR Gilchriese, MGD Hall, CR Hanhardt, M Haselschwardt, SJ Hertel, SA Hogan, DP Horn, M Huang, DQ Ignarra, CM Ihm, M Jacobsen, RG Ji, W Kazkaz, K Khaitan, D Knoche, R Larsen, NA Lee, C Lenardo, BG Lesko, KT Lindote, A Lopes, MI Malling, DC Manalaysay, A Mannino, RL Marzioni, MF McKinsey, DN Mei, DM Mock, J Moongweluwan, M Morad, JA Murphy, AS Nehrkorn, C Nelson, HN Neves, F O'Sullivan, K Oliver-Mallory, KC Ott, RA Palladino, KJ Pangilinan, M Pease, EK Phelps, P Reichhart, L Rhyne, C Shaw, S Shutt, TA Silva, C Solovov, VN Sorensen, P Stephenson, S Sumner, TJ Szydagis, M Taylor, DJ Taylor, W Tennyson, BP Terman, PA Tiedt, DR To, WH Tripathi, M Tvrznikova, L Uvarov, S Verbus, JR Webb, RC White, JT Whitis, TJ Witherell, MS Wolfs, FLH Yazdani, K Young, SK Zhang, C AF Akerib, D. S. Araujo, H. M. Bai, X. Bailey, A. J. Balajthy, J. Beltrame, P. Bernard, E. P. Bernstein, A. Biesiadzinski, T. P. Boulton, E. M. Bradley, A. Bramante, R. Cahn, S. B. Carmona-Benitez, M. C. Chan, C. Chapman, J. J. Chiller, A. A. Chiller, C. Currie, A. Cutter, J. E. Davison, T. J. R. de Viveiros, L. Dobi, A. Dobson, J. E. Y. Druszkiewicz, E. Edwards, B. N. Faham, C. H. Fiorucci, S. Gaitskell, R. J. Gehman, V. M. Ghag, C. Gibson, K. R. Gilchriese, M. G. D. Hall, C. R. Hanhardt, M. Haselschwardt, S. J. Hertel, S. A. Hogan, D. P. Horn, M. Huang, D. Q. Ignarra, C. M. Ihm, M. Jacobsen, R. G. Ji, W. Kazkaz, K. Khaitan, D. Knoche, R. Larsen, N. A. Lee, C. Lenardo, B. G. Lesko, K. T. Lindote, A. Lopes, M. I. Malling, D. C. Manalaysay, A. Mannino, R. L. Marzioni, M. F. McKinsey, D. N. Mei, D. -M. Mock, J. Moongweluwan, M. Morad, J. A. Murphy, A. St. J. Nehrkorn, C. Nelson, H. N. Neves, F. O'Sullivan, K. Oliver-Mallory, K. C. Ott, R. A. Palladino, K. J. Pangilinan, M. Pease, E. K. Phelps, P. Reichhart, L. Rhyne, C. Shaw, S. Shutt, T. A. Silva, C. Solovov, V. N. Sorensen, P. Stephenson, S. Sumner, T. J. Szydagis, M. Taylor, D. J. Taylor, W. Tennyson, B. P. Terman, P. A. Tiedt, D. R. To, W. H. Tripathi, M. Tvrznikova, L. Uvarov, S. Verbus, J. R. Webb, R. C. White, J. T. Whitis, T. J. Witherell, M. S. Wolfs, F. L. H. Yazdani, K. Young, S. K. Zhang, C. CA LUX Collaboration TI Results on the Spin-Dependent Scattering of Weakly Interacting Massive Particles on Nucleons from the Run 3 Data of the LUX Experiment SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERSYMMETRIC DARK-MATTER; CANDIDATES; SEARCHES AB We present experimental constraints on the spin-dependent WIMP (weakly interacting massive particle)nucleon elastic cross sections from LUX data acquired in 2013. LUX is a dual-phase xenon time projection chamber operating at the Sanford Underground Research Facility (Lead, South Dakota), which is designed to observe the recoil signature of galactic WIMPs scattering from xenon nuclei. A profile likelihood ratio analysis of 1.4 x 10(4) kg day of fiducial exposure allows 90% C. L. upper limits to be set on the WIMPneutron (WIMP-proton) cross section of sigma(n) = 9.4 x 10(-41) cm(2) (sigma(p) = 2.9 x 10(-39) cm(2)) at 33 GeV/c(2). The spin-dependent WIMP-neutron limit is the most sensitive constraint to date. C1 [Akerib, D. S.; Biesiadzinski, T. P.; Bradley, A.; Bramante, R.; Gibson, K. R.; Ji, W.; Lee, C.; Phelps, P.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Case Western Reserve Univ, Dept Phys, 10900 Euclid Ave, Cleveland, OH 44106 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94205 USA. [Akerib, D. S.; Biesiadzinski, T. P.; Bramante, R.; Ignarra, C. M.; Ji, W.; Lee, C.; Palladino, K. J.; Shutt, T. A.; To, W. H.; Whitis, T. J.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, 452 Lomita Mall, Stanford, CA 94309 USA. [Araujo, H. M.; Bailey, A. J.; Currie, A.; Sumner, T. J.; Yazdani, K.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys, Prince Consort Rd, London SW7 2BZ, England. [Bai, X.; Hanhardt, M.; Tiedt, D. R.] South Dakota Sch Mines & Technol, 501 East St Joseph St, Rapid City, SD 57701 USA. [Balajthy, J.; Hall, C. R.; Knoche, R.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beltrame, P.; Davison, T. J. R.; Marzioni, M. F.; Murphy, A. St. J.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh EH9 3FD, Midlothian, Scotland. [Bernard, E. P.; Boulton, E. M.; Cahn, S. B.; Edwards, B. N.; Hertel, S. A.; Horn, M.; Larsen, N. A.; McKinsey, D. N.; O'Sullivan, K.; Pease, E. K.; Tennyson, B. P.; Tvrznikova, L.] Yale Univ, Dept Phys, 217 Prospect St, New Haven, CT 06511 USA. [Bernstein, A.; Kazkaz, K.; Lenardo, B. G.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. [Carmona-Benitez, M. C.; Haselschwardt, S. J.; Nehrkorn, C.; Nelson, H. N.; Witherell, M. S.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Chan, C.; Chapman, J. J.; Gaitskell, R. J.; Huang, D. Q.; Malling, D. C.; Pangilinan, M.; Rhyne, C.; Taylor, W.; Verbus, J. R.] Brown Univ, Dept Phys, 182 Hope St, Providence, RI 02912 USA. [Chiller, A. A.; Chiller, C.; Mei, D. -M.; Zhang, C.] Univ S Dakota, Dept Phys, 414E Clark St, Vermillion, SD 57069 USA. [Cutter, J. E.; Lenardo, B. G.; Manalaysay, A.; Morad, J. A.; Ott, R. A.; Stephenson, S.; Tripathi, M.; Uvarov, S.] Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. [de Viveiros, L.; Lindote, A.; Lopes, M. I.; Neves, F.; Silva, C.; Solovov, V. N.] Univ Coimbra, Dept Phys, LIP Coimbra, Rua Larga, P-3004516 Coimbra, Portugal. [Dobi, A.; Faham, C. H.; Fiorucci, S.; Gehman, V. M.; Gilchriese, M. G. D.; Hertel, S. A.; Horn, M.; Ihm, M.; Jacobsen, R. G.; Lesko, K. T.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.; Pease, E. K.; Sorensen, P.; Tvrznikova, L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Dobson, J. E. Y.; Ghag, C.; Reichhart, L.; Shaw, S.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Druszkiewicz, E.; Khaitan, D.; Moongweluwan, M.; Wolfs, F. L. H.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Hanhardt, M.; Taylor, D. J.] South Dakota Sci & Technol Author, Sanford Underground Res Facil, Lead, SD 57754 USA. [Hertel, S. A.; Hogan, D. P.; Horn, M.; Ihm, M.; Jacobsen, R. G.; McKinsey, D. N.; O'Sullivan, K.; Oliver-Mallory, K. C.; Pease, E. K.; Tvrznikova, L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mannino, R. L.; Terman, P. A.; Webb, R. C.; White, J. T.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Mock, J.; Szydagis, M.; Young, S. K.] SUNY Albany, Dept Phys, 1400 Washington Ave, Albany, NY 12222 USA. [Palladino, K. J.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. RP Bailey, AJ (reprint author), Univ London Imperial Coll Sci Technol & Med, Blackett Lab, High Energy Phys, Prince Consort Rd, London SW7 2BZ, England. EM a.bailey12@imperial.ac.uk OI Horn, Markus/0000-0003-1624-9890; Tvrznikova, Lucie/0000-0002-0394-7692 FU U.S. Department of Energy (DOE) [DE-FG02-08ER41549, DE-FG02-91ER40688, DE-FG02-95ER40917, DE-FG02-91ER40674, DE-NA0000979, DE-FG02-11ER41738, DE-SC0006605, DE-AC02-05CH11231, DE-AC52-07NA27344, DE-FG01-91ER40618]; U.S. National Science Foundation [PHYS-0750671, PHY-0801536, PHY-1004661, PHY-1102470, PHY-1003660, PHY-1312561, PHY-1347449, PHY-1505868]; Research Corporation Grant [RA0350]; Center for Ultra-low Background Experiments in the Dakotas (CUBED); South Dakota School of Mines and Technology (SDSMT); Fundacao para a Ciencia e a Tecnologia (FCT) [PTDC/FIS-NUC/1525/2014]; UK Royal Society [IE120804]; Science and Technology Facilities Council [ST/K502042/1, ST/K502406/1, ST/M503538/1] FX This work was partially supported by the U.S. Department of Energy (DOE) under Awards No. DE-FG02-08ER41549, No. DE-FG02-91ER40688, No. DE-FG02-95ER40917, No. DE-FG02-91ER40674, No. DE-NA0000979, No. DE-FG02-11ER41738, No. DE-SC0006605, No. DE-AC02-05CH11231, No. DE-AC52-07NA27344, and No. DE-FG01-91ER40618; the U.S. National Science Foundation under Grants No. PHYS-0750671, No. PHY-0801536, No. PHY-1004661, No. PHY-1102470, No. PHY-1003660, No. PHY-1312561, No. PHY-1347449, and No. PHY-1505868; the Research Corporation Grant No. RA0350; the Center for Ultra-low Background Experiments in the Dakotas (CUBED); and the South Dakota School of Mines and Technology (SDSMT). LIP-Coimbra acknowledges funding from Fundacao para a Ciencia e a Tecnologia (FCT) through the Project Grant No. PTDC/FIS-NUC/1525/2014. Imperial College and Brown University thank the UK Royal Society for travel funds under the International Exchange Scheme (IE120804). The UK groups acknowledge institutional support from Imperial College London, University College London and Edinburgh University, and from the Science and Technology Facilities Council for PhD Studentships No. ST/K502042/1 (AB), No. ST/K502406/1 (SS), and No. ST/M503538/1 (KY). The University of Edinburgh is a charitable body, registered in Scotland, with Registration No. SC005336 This research was conducted using computational resources and services at the Center for Computation and Visualization, Brown University. We gratefully acknowledge the logistical and technical support and the access to laboratory infrastructure provided to us by the Sanford Underground Research Facility (SURF) and its personnel at Lead, South Dakota. SURF was developed by the South Dakota Science and Technology Authority, with an important philanthropic donation from T. Denny Sanford, and is operated by the Lawrence Berkeley National Laboratory for the Department of Energy, Office of High Energy Physics. NR 43 TC 30 Z9 30 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 20 PY 2016 VL 116 IS 16 AR 161302 DI 10.1103/PhysRevLett.116.161302 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ9UU UT WOS:000374559300004 PM 27152786 ER PT J AU Hays, J Shonkoff, SBC AF Hays, Jake Shonkoff, Seth B. C. TI Toward an Understanding of the Environmental and Public Health Impacts of Unconventional Natural Gas Development: A Categorical Assessment of the Peer-Reviewed Scientific Literature, 2009-2015 SO PLOS ONE LA English DT Article ID SHALE GAS; OIL; AIR; OPERATIONS; EXTRACTION; EMISSIONS; BASIN AB The body of science evaluating the potential impacts of unconventional natural gas development (UNGD) has grown significantly in recent years, although many data gaps remain. Still, a broad empirical understanding of the impacts is beginning to emerge amidst a swell of research. The present categorical assessment provides an overview of the peer-reviewed scientific literature from 2009-2015 as it relates to the potential impacts of UNGD on public health, water quality, and air quality. We have categorized all available original research during this time period in an attempt to understand the weight and direction of the scientific literature. Our results indicate that at least 685 papers have been published in peer-reviewed scientific journals that are relevant to assessing the impacts of UNGD. 84% of public health studies contain findings that indicate public health hazards, elevated risks, or adverse health outcomes; 69% of water quality studies contain findings that indicate potential, positive association, or actual incidence of water contamination; and 87% of air quality studies contain findings that indicate elevated air pollutant emissions and/or atmospheric concentrations. This paper demonstrates that the weight of the findings in the scientific literature indicates hazards and elevated risks to human health as well as possible adverse health outcomes associated with UNGD. There are limitations to this type of assessment and it is only intended to provide a snapshot of the scientific knowledge based on the available literature. However, this work can be used to identify themes that lie in or across studies, to prioritize future research, and to provide an empirical foundation for policy decisions. C1 [Hays, Jake] PSE Hlth Energy, New York, NY USA. [Hays, Jake] Weill Cornell Med, Dept Healthcare Policy & Res, New York, NY USA. [Shonkoff, Seth B. C.] PSE Hlth Energy, Oakland, CA USA. [Shonkoff, Seth B. C.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Shonkoff, Seth B. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Hays, J (reprint author), PSE Hlth Energy, New York, NY USA.; Hays, J (reprint author), Weill Cornell Med, Dept Healthcare Policy & Res, New York, NY USA. EM hays@psehealthyenergy.org NR 19 TC 3 Z9 3 U1 3 U2 17 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 20 PY 2016 VL 11 IS 4 AR e0154164 DI 10.1371/journal.pone.0154164 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ9OU UT WOS:000374543600087 PM 27096432 ER PT J AU Ozmen, O Pullum, LL Ramanathan, A Nutaro, JJ AF Ozmen, Ozgur Pullum, Laura L. Ramanathan, Arvind Nutaro, James J. TI Augmenting Epidemiological Models with Point-Of-Care Diagnostics Data SO PLOS ONE LA English DT Article AB Although adoption of newer Point-of-Care (POC) diagnostics is increasing, there is a significant challenge using POC diagnostics data to improve epidemiological models. In this work, we propose a method to process zip-code level POC datasets and apply these processed data to calibrate an epidemiological model. We specifically develop a calibration algorithm using simulated annealing and calibrate a parsimonious equation-based model of modified Susceptible-Infected-Recovered (SIR) dynamics. The results show that parsimonious models are remarkably effective in predicting the dynamics observed in the number of infected patients and our calibration algorithm is sufficiently capable of predicting peak loads observed in POC diagnostics data while staying within reasonable and empirical parameter ranges reported in the literature. Additionally, we explore the future use of the calibrated values by testing the correlation between peak load and population density from Census data. Our results show that linearity assumptions for the relationships among various factors can be misleading, therefore further data sources and analysis are needed to identify relationships between additional parameters and existing calibrated ones. Calibration approaches such as ours can determine the values of newly added parameters along with existing ones and enable policy-makers to make better multi-scale decisions. C1 [Pullum, Laura L.; Nutaro, James J.] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN USA. [Ozmen, Ozgur; Ramanathan, Arvind] Oak Ridge Natl Lab, Hlth Data Sci Inst, Oak Ridge, TN USA. [Pullum, Laura L.] One Bethel Valley Rd,POB 2008, Oak Ridge, TN 37831 USA. RP Pullum, LL (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN USA.; Pullum, LL (reprint author), One Bethel Valley Rd,POB 2008, Oak Ridge, TN 37831 USA. EM pullumll@ornl.gov OI Nutaro, James/0000-0001-7360-2836 FU DTRA (Defense Threat Reduction Agency) [2216-V387-11]; ORNL (Oak Ridge National Laboratory) [7280]; U.S. Department of Energy [DE-AC05-00OR22725] FX DTRA (Defense Threat Reduction Agency, contract no: 2216-V387-11) and ORNL (Oak Ridge National Laboratory, SEED project 7280) are the sources of funds. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.; We would like to thank IMS Health Government Solutions, the Texas Department of Public Health, and the Knox County Public Health Department for the data used in this study. Data (used as part of this paper) can be requested through IMS Health Institute, the Texas Department of Public Health, and the Knox County Public Health Department. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 16 TC 0 Z9 0 U1 0 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 20 PY 2016 VL 11 IS 4 AR e0153769 DI 10.1371/journal.pone.0153769 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ9OU UT WOS:000374543600054 PM 27096162 ER PT J AU Bass, IL Negres, RA Stanion, K Guss, G Bude, J AF Bass, Isaac L. Negres, Raluca A. Stanion, Ken Guss, Gabe Bude, Jeff TI "Metallic burn paper" used for in situ characterization of laser beam properties SO APPLIED OPTICS LA English DT Article ID FEMTOSECOND LASER; ABLATION; PULSES; BOROSILICATE; GLASS; PS; FS AB In situ ablation of thin metal films on fused silica substrates by picosecond class lasers was investigated as a method of characterizing the beam at the sample plane. The technique involved plotting the areas enclosed by constant fluence contours identified in optical microscope images of the ablation sites versus the logs of the pulse energies. Inconel films on commercially available neutral density filters as well as magnetron sputtered gold films were used. It was also shown that this technique could be used to calibrate real-time beam profile diagnostics against the beam at the sample plane. The contours were shown to correspond to the boundary where part or all of the film was ablated. (C) 2016 Optical Society of America C1 [Bass, Isaac L.; Negres, Raluca A.; Stanion, Ken; Guss, Gabe; Bude, Jeff] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. RP Bass, IL (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM bass1@llnl.gov FU Laboratory Directed Research and Development (LDRD) [16-ERD-016]; Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344] FX Laboratory Directed Research and Development (LDRD) (16-ERD-016); Lawrence Livermore National Laboratory (LLNL) (DE-AC52-07NA27344). NR 14 TC 3 Z9 3 U1 4 U2 6 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD APR 20 PY 2016 VL 55 IS 12 BP 3131 EP 3139 DI 10.1364/AO.55.003131 PG 9 WC Optics SC Optics GA DJ7JV UT WOS:000374388600034 PM 27140078 ER PT J AU Alexandratos, SD Kung, S AF Alexandratos, Spiro D. Kung, Stephen TI Preface to the Special Issue: Uranium in Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Editorial Material C1 [Alexandratos, Spiro D.] CUNY Hunter Coll, Dept Chem, New York, NY 10021 USA. [Kung, Stephen] US DOE, Off Nucl Energy, Washington, DC 20585 USA. RP Alexandratos, SD (reprint author), CUNY Hunter Coll, Dept Chem, New York, NY 10021 USA. EM alexsd@hunter.cuny.edu NR 0 TC 0 Z9 0 U1 7 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4101 EP 4102 DI 10.1021/acs.iecr.6b01293 PG 2 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400001 ER PT J AU Das, S Oyola, Y Mayes, RT Janke, CJ Kuo, LJ Gill, G Wood, JR Dai, S AF Das, S. Oyola, Y. Mayes, R. T. Janke, C. J. Kuo, L. -J. Gill, G. Wood, J. R. Dai, S. TI Extracting Uranium from Seawater: Promising AI Series Adsorbents SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID AMIDOXIME ADSORBENTS; METHACRYLIC-ACID; ACRYLIC-ACID; URANYL IONS; SEA-WATER; HYDROGELS; RECOVERY; ADSORPTION; POLYMER; BINDING AB A new series of adsorbents (AI10 through AI17) were successfully developed at ORNL by radiation induced graft polymerization (RIG?) of acrylonitrile (AN) and vinylphosphonic acid (VPA) (at different mole to mole ratios) onto high surface area polyethylene fiber, with high degrees of grafting (DOG) varying from 110 to 300%. The grafted nitrile groups were converted to amidoxime groups by reaction with 5 wt % hydroxylamine at 80 degrees C for 72 h. The amidoximated adsorbents were then conditioned with 0.44 M KOH at 80 degrees C followed by screening at ORNL with prescreening brine spiked with 8 ppm uranium. Uranium adsorption capacities in prescreening, ranged from 171 to 187 g-U/kg-ads irrespective of percent DOG. The performance of the adsorbents with respect to uranium adsorption in natural seawater was also investigated using flow-through-column testing at the Pacific Northwest National Laboratory (PNNL). Three hours of KOH conditioning led to higher uranium uptake than 1 h of conditioning. The adsorbent AI11, containing AN and VPA at the mole ratio of 3.52, emerged as the potential candidate for the highest uranium adsorption (3.35 g-U/kg-ads.) after 56 days of exposure in seawater flow-through-columns. The rate of vanadium adsorption over uranium linearly increased throughout the 56 days of exposure. The total mass of vanadium uptake was similar to 5 times greater than uranium after 56 days. C1 [Das, S.; Oyola, Y.; Mayes, R. T.; Janke, C. J.; Dai, S.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Kuo, L. -J.; Gill, G.; Wood, J. R.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Das, S; Oyola, Y; Dai, S (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM dass1@ornl.gov; yal_oyola@hotmail.com; dais@ornl.gov RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188 FU US Department of Energy, Office of Nuclear Energy FX This work was sponsored by the US Department of Energy, Office of Nuclear Energy. NR 40 TC 7 Z9 7 U1 16 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4103 EP 4109 DI 10.1021/acs.iecr.5b03135 PG 7 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400002 ER PT J AU Das, S Oyola, Y Mayes, RT Janke, CJ Kuo, LJ Gill, G Wood, JR Dai, S AF Das, S. Oyola, Y. Mayes, Richard T. Janke, Chris J. Kuo, L. -J. Gill, G. Wood, J. R. Dai, S. TI Extracting Uranium from Seawater: Promising AF Series Adsorbents SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SEA-WATER; AMIDOXIME ADSORBENTS; POLYMERIC ADSORBENT; FUNCTIONAL-GROUP; ADSORPTION; RECOVERY; COMPLEXATION; GLUTARIMIDEDIOXIME; PRECONCENTRATION; STABILITY AB A new family of high-surface-area polyethylene fiber adsorbents named the AF series was recently developed at the Oak Ridge National Laboratory (ORNL). The AF series adsorbents were synthesized by radiation-induced graft polymerization of acrylonitrile and itaconic acid (at different monomer/comonomer mol ratios) onto high surface area polyethylene fibers. The degree of grafting (%DOG) of AF series adsorbents was found to be 154-354%. The grafted nitrile groups were converted to amidoxime groups by treating with hydroxylamine. The amidoximated adsorbents were then conditioned with 0.44 M KOH at 80 degrees C followed by screening at ORNL with sodium-based synthetic aqueous solution, spiked with 8 ppm uranium. The uranium adsorption capacity in simulated seawater screening ranged from 170 to 200 g-U/kg-ads irrespective of %DOG. A monomer/comonomer molar ratio in the range of 7.57-10.14 seemed to be optimum for highest uranium loading capacity. Subsequently, the adsorbents were also tested with natural seawater at Pacific Northwest National Laboratory (PNNL) using flow-through column experiments to determine uranium loading capacity with varying KOH conditioning times at 80 degrees C. The highest adsorption capacity of AF1 measured after 56 days of marine testing was demonstrated as 3.9 g-U/kg-adsorbent and 3.2 g-U/kg-adsorbent for 1 and 3 h of KOH conditioning at 80 degrees C, respectively. Based on capacity values of several AF1 samples, it was observed that changing KOH conditioning from 1 to 3 h at 80 degrees C resulted in a 22-27% decrease in uranium adsorption capacity in seawater. C1 [Das, S.; Oyola, Y.; Mayes, Richard T.; Janke, Chris J.; Dai, S.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Kuo, L. -J.; Gill, G.; Wood, J. R.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Das, S; Oyola, Y; Dai, S (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM amisdas@gmail.com; yal_oyola@hotmail.com; dais@ornl.gov RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188 FU U.S. Department of Energy, Office of Nuclear Energy FX This work was sponsored by the U.S. Department of Energy, Office of Nuclear Energy. NR 47 TC 14 Z9 14 U1 13 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4110 EP 4117 DI 10.1021/acs.iecr.5b03136 PG 8 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400003 ER PT J AU Yue, YF Zhang, CX Tang, Q Mayes, RT Liao, WP Liao, C Tsouris, C Stankovich, JJ Chen, JH Hensley, DK Abney, CW Jiang, DE Brown, S Dai, S AF Yue, Yanfeng Zhang, Chenxi Tang, Qing Mayes, Richard T. Liao, Wei-Po Liao, Chen Tsouris, Costas Stankovich, Joseph J. Chen, Jihua Hensley, Dale K. Abney, Carter W. Jiang, De-en Brown, Suree Dai, Sheng TI A Poly(acrylonitrile)-Functionalized Porous Aromatic Framework Synthesized by Atom-Transfer Radical Polymerization for the Extraction of Uranium from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID DENSITY-FUNCTIONAL THEORY; SEA-WATER; RECOVERY; URANYL; COMPLEXES; ADSORBENTS; ADSORPTION; FIBER; AMIDOXIMATE; MECHANISM AB In order to ensure a sustainable reserve of fuel for nuclear power generation, tremendous research efforts have been devoted to developing advanced sorbent materials for extracting uranium from seawater. In this work, a porous aromatic framework (PAF) was surface-functionalized with poly(acrylonitrile) through atom-transfer radical polymerization (ATRP). Batches of this adsorbent were conditioned with potassium hydroxide (KOH) at room temperature or 80 degrees C prior to contact with a uranium-spiked seawater simulant, with minimal differences in uptake observed as a function of conditioning temperature. A maximum capacity of 4.81 g-U/kg-ads was obtained following 42 days contact with uranium-spiked filtered environmental seawater, which demonstrates a comparable adsorption rate. A kinetic investigation revealed extremely rapid uranyl uptake, with more than 80% saturation reached within 14 days. Relying on the semiordered structure of the PAF adsorbent, density functional theory (DFT) calculations reveal cooperative interactions between multiple adsorbent groups yield a strong driving force for uranium binding. C1 [Yue, Yanfeng; Zhang, Chenxi; Mayes, Richard T.; Liao, Wei-Po; Liao, Chen; Stankovich, Joseph J.; Abney, Carter W.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Yue, Yanfeng] Sul Ross State Univ, Dept Biol Geol & Phys Sci, Alpine, TX 79832 USA. [Tsouris, Costas] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Tang, Qing; Jiang, De-en] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Chen, Jihua; Hensley, Dale K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Brown, Suree; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Yue, YF; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Yue, YF (reprint author), Sul Ross State Univ, Dept Biol Geol & Phys Sci, Alpine, TX 79832 USA.; Jiang, DE (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA.; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM yanfeng.yue@sulross.edu; de-en.jiang@ucr.edu; dais@ornl.gov RI Chen, Jihua/F-1417-2011; Dai, Sheng/K-8411-2015; Jiang, De-en/D-9529-2011; Tsouris, Costas/C-2544-2016 OI Chen, Jihua/0000-0001-6879-5936; Dai, Sheng/0000-0002-8046-3931; Jiang, De-en/0000-0001-5167-0731; Tsouris, Costas/0000-0002-0522-1027 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory; DOE Office of Nuclear Energy - Nuclear Energy University Programs [DE-NE0008397]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was sponsored by the U.S. Department of Energy, Office of Nuclear Energy, under Contract No. DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. Electron microscopy (J.C. and D.K.H.) experiments were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. DFT computation (Q.T. and DJ.) was supported by DOE Office of Nuclear Energy - Nuclear Energy University Programs (Grant No. DE-NE0008397) and resources of the National Energy Research Scientific Computing Center, which is a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 44 TC 1 Z9 1 U1 18 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4125 EP 4129 DI 10.1021/acs.iecr.5b03372 PG 5 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400005 ER PT J AU Brown, S Chatterjee, S Li, MJ Yue, YF Tsouris, C Janke, CJ Saito, T Dai, S AF Brown, Suree Chatterjee, Sabornie Li, Meijun Yue, Yanfeng Tsouris, Costas Janke, Christopher J. Saito, Tomonori Dai, Sheng TI Uranium Adsorbent Fibers Prepared by Atom-Transfer Radical Polymerization from Chlorinated Polypropylene and Polyethylene Trunk Fibers SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID POLY(VINYL CHLORIDE); GRAFT-COPOLYMERIZATION; ISOTACTIC POLYPROPYLENE; STRUCTURAL DEFECTS; BLOCK-COPOLYMERS; BUTYL ACRYLATE; SEAWATER; AMIDOXIME; RECOVERY; INITIATOR AB Seawater contains a large amount of uranium (similar to 4.5 billion tons) which can serve as a nearly limitless supply for an energy source. However, to make the recovery of uranium from seawater economically feasible, lower manufacturing and deployment costs are desirable, and good solid adsorbents must have high uranium uptake, reusability, and high selectivity toward uranium. In this study, atom-transfer radical polymerization (ATRP), without the high-cost radiation-induced graft polymerization, was used for grafting acrylonitrile and test-butyl acrylate from a new class of trunk fibers, forming adsorbents in a readily deployable form. The new class of trunk fibers was prepared by the chlorination of polypropylene (PP) round fiber, hollow-gear PP fiber, and hollow-gear polyethylene fiber. During ATRP, degrees of grafting (d.g.) varied according to the structure of active chlorine sites on trunk fibers and ATRP conditions, and the d.g. as high as 2570% was obtained. Resulting adsorbent fibers were evaluated in U-spiked simulated seawater, and the maximum adsorption capacity of 146.6 g U/kg, much higher than that of a standard adsorbent Japan Atomic Energy Agency fiber (75.1 g/kg), was obtained. This new type of trunk fiber can be used for grafting a variety of uranium-interacting ligands, including designed ligands that are highly selective toward uranium. C1 [Brown, Suree; Li, Meijun; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Chatterjee, Sabornie; Yue, Yanfeng; Tsouris, Costas; Saito, Tomonori; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Janke, Christopher J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Brown, S; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Saito, T; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM ssuree@utk.edu; saitot@ornl.gov; dais@ornl.gov RI Saito, Tomonori/M-1735-2016; Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016 OI Saito, Tomonori/0000-0002-4536-7530; Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX This research was sponsored by the U.S. Department of Energy, Office of Nuclear Energy under Contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. The JAEA sorbent was kindly donated for testing by the Japan Atomic Energy Agency. NR 39 TC 3 Z9 3 U1 9 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4130 EP 4138 DI 10.1021/acs.iecr.5b03667 PG 9 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400006 ER PT J AU Brown, S Yue, YF Kuo, LJ Mehio, N Li, MJ Gill, G Tsouris, C Mayes, RT Saito, T Dai, S AF Brown, Suree Yue, Yanfeng Kuo, Li-Jung Mehio, Nada Li, Meijun Gill, Gary Tsouris, Costas Mayes, Richard T. Saito, Tomonori Dai, Sheng TI Uranium Adsorbent Fibers Prepared by Atom-Transfer Radical Polymerization (ATRP) from Poly(vinyl chloride)-co-chlorinated Poly(vinyl chloride) (PVC-co-CPVC) Fiber SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID GRAFT-COPOLYMERIZATION; AMPHIPHILIC POLY(VINYL; STRUCTURAL DEFECTS; BLOCK-COPOLYMERS; LABILE CHLORINES; BUTYL ACRYLATE; SI-ATRP; SEAWATER; AMIDOXIME; RECOVERY AB The need to secure future supplies of energy attracts researchers in several countries to a vast resource of nuclear energy fuel: uranium in seawater (estimated at 4.5 billion tons in seawater). In this study, we developed effective adsorbent fibers for the recovery of uranium from seawater via atom-transfer radical polymerization (ATRP) from a poly (vinyl chloride)-co-chlorinated poly(vinyl chloride) (PVC-co-CPVC) fiber. ATRP was employed in the surface graft polymerization of acrylonitrile (AN) and tert-butyl acrylate (tBA), precursors for uranium-interacting functional groups, from PVC-co-CPVC fiber. The [tBA]/[AN] was systematically varied to identify the optimal ratio between hydrophilic groups (from tBA) and uranyl-binding ligands (from AN). The best performing adsorbent fiber, the one with the optimal [tBA]/[AN] ratio and a high degree of grafting (1390%), demonstrated uranium adsorption capacities that are significantly greater than those of the Japan Atomic Energy Agency (JAEA) reference fiber in natural seawater tests (2.42-3.24 g/kg in 42 days of seawater exposure and 5.22 g/kg in 49 days of seawater exposure, versus 1.66 g/kg in 42 days of seawater exposure and 1.71 g/kg in 49 days of seawater exposure for JAEA). Adsorption of other metal ions from seawater and their corresponding kinetics were also studied. The grafting of alternative monomers for the recovery of uranium from seawater is now under development by this versatile technique of ATRP. C1 [Brown, Suree; Mehio, Nada; Li, Meijun; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Yue, Yanfeng; Tsouris, Costas; Mayes, Richard T.; Saito, Tomonori; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Kuo, Li-Jung; Gill, Gary] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Brown, S; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Saito, T; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM ssuree@utk.edu; saitot@ornl.gov; dais@ornl.gov RI Saito, Tomonori/M-1735-2016; Dai, Sheng/K-8411-2015; Tsouris, Costas/C-2544-2016 OI Saito, Tomonori/0000-0002-4536-7530; Dai, Sheng/0000-0002-8046-3931; Tsouris, Costas/0000-0002-0522-1027 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX This research was sponsored by the U.S. Department of Energy, Office of Nuclear Energy under Contract No. DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. The JAEA sorbent was kindly donated for testing by the Japan Atomic Energy Agency. The PVC-co-CPVC fiber was a sample from Rhovyl fiber, courteously donated by Whitin Yarns and Fibers (Westport, MA, USA). NR 51 TC 5 Z9 5 U1 11 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4139 EP 4148 DI 10.1021/acs.iecr.5b03355 PG 10 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400007 ER PT J AU Oyola, Y Janke, CJ Dai, S AF Oyola, Yatsandra Janke, Christopher J. Dai, Sheng TI Synthesis, Development, and Testing of High-Surface-Area Polymer-Based Adsorbents for the Selective Recovery of Uranium from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID INDUCED GRAFT-COPOLYMERIZATION; SEA-WATER; AMIDOXIME/CARBOXYL GROUP; TITANIUM-DIOXIDE; METHACRYLIC-ACID; URANYL-ION; METAL-IONS; ADSORPTION; ACRYLONITRILE; POLYETHYLENE AB The ocean contains uranium with an approximate concentration of 3.34 ppb, which can serve as an incredible supply source to sustain nuclear energy in the United States. Unfortunately, technology currently available to recover uranium from seawater is not efficient enough and mining uranium on land is still more economical. We have developed polymer-based adsorbents with high uranium adsorption capacities by grafting amidoxime onto high-surface-area polyethylene (PE) fibers. Various process conditions have been screened, in combination with developing a rapid testing protocol (<24 h), to optimize the process. These adsorbents are synthesized through radiation-induced grafting of acrylonitrile (AN) and methacrylic acid (MAA) onto PE fibers, followed by the conversion of nitriles to amidoximes and basic conditioning. In addition, the uranium adsorption capacity, measured in units of g(U)/kg(ads), is greatly increased by reducing the diameter of the PE fiber or changing its morphology. An increase in the surface area of the PE polymer fiber allows for more grafting sites that are positioned in more-accessible locations, thereby increasing access to grafted molecules that would normally be located in the interior of a fiber with a larger diameter. Polymer fibers with hollow morphologies are able to adsorb beyond 1 order of magnitude more uranium from simulated seawater than current commercially available adsorbents. Several high-surface-area fibers were tested in natural seawater and were able to extract 5-7 times more uranium than any adsorbent reported to date. C1 [Oyola, Yatsandra; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. [Janke, Christopher J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008, Oak Ridge, TN 37831 USA. RP Oyola, Y (reprint author), Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. EM yal_oyola@hotmail.com RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188 FU U.S. Department of Energy, Office of Nuclear Energy; U.S. Department of Energy [DE-AC05-00OR22725]; U.S. government [DE-AC05-00OR22725] FX Research sponsored by the U.S. Department of Energy, Office of Nuclear Energy and performed at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy, under Contract No. DE-AC05-00OR22725. This publication has been authored by a contractor of the U.S. government under Contract No. DE-AC05-00OR22725. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. government purposes. We thank Dr. Gary Gill for exposing our adsorbents to seawater at the Pacific Northwest National Laboratory in Sequim, WA. We also thank Dr. Seko and Dr. Tamada of JAEA, Takasaki, Japan for their insightful conversations and for kindly donating The Japan Atomic Energy Agency (JAEA) uranium adsorbent material for testing. NR 55 TC 6 Z9 6 U1 14 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4149 EP 4160 DI 10.1021/acs.iecr.5b03981 PG 12 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400008 ER PT J AU Chatterjee, S Bryantsev, VS Brown, S Johnson, JC Grant, CD Mayes, RT Hay, BP Dai, S Saito, T AF Chatterjee, Sabornie Bryantsev, Vyacheslav S. Brown, Suree Johnson, J. Casey Grant, Christopher D. Mayes, Richard T. Hay, Benjamin P. Dai, Sheng Saito, Tomonori TI Synthesis of Naphthalimidedioxime Ligand-Containing Fibers for Uranium Adsorption from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID TRANSFER RADICAL POLYMERIZATION; SEA-WATER; ANISOTROPIC DIELECTRICS; FUNCTIONAL-GROUP; AMIDOXIME; RECOVERY; ADSORBENT; DENSITY; ELUTION; GLUTARIMIDEDIOXIME AB A novel ligand-functionalized adsorbent material was prepared using a combination of radiation-induced graft polymerization (RIGP) and click chemistry (1,3 cycloaddition reaction). The design of the ligand-containing amidoxime functionality is based on its chelating efficiency with uranium. In this process, RIGP is used to graft polymer chains on fiber substrates, where the fibers are prepared by irradiating and treating polyethylene (PE) with different bulk ratios of vinyl benzyl chloride and acrylic acid or itaconic acid. Furthermore, chemical modifications of these fibers are performed using a two-step process, where novel bisimidoxime ligands are incorporated into fibers. These ligands contain imidedioxime, which is known to be a uranophile. Also, the core structure of the ligand containing three donor atoms facilitates the formation of chelate with uranyl ion in media such as seawater. Density functional theory calculations were performed to quantify the binding strength with the uranyl ion. When tested with simulated seawater with a uranium concentration of 6 ppm at pH 8.0-8.3, the developed materials showed moderate to high uranium (similar to 35-50 g U/kg adsorbent) adsorption capacity. C1 [Chatterjee, Sabornie; Bryantsev, Vyacheslav S.; Johnson, J. Casey; Grant, Christopher D.; Mayes, Richard T.; Dai, Sheng; Saito, Tomonori] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Brown, Suree; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Hay, Benjamin P.] Supramol Design Inst, 127 Chestnut Hill Rd, Oak Ridge, TN 37830 USA. RP Saito, T (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Hay, BP (reprint author), Supramol Design Inst, 127 Chestnut Hill Rd, Oak Ridge, TN 37830 USA. RI Saito, Tomonori/M-1735-2016; Dai, Sheng/K-8411-2015; Bryantsev, Vyacheslav/M-5111-2016 OI Saito, Tomonori/0000-0002-4536-7530; Dai, Sheng/0000-0002-8046-3931; Bryantsev, Vyacheslav/0000-0002-6501-6594 FU US Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX This research was sponsored by the US Department of Energy, Office of Nuclear Energy under contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. NR 55 TC 3 Z9 3 U1 9 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4161 EP 4169 DI 10.1021/acs.iecr.5b03212 PG 9 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400009 ER PT J AU Piechowicz, M Abney, CW Zhou, X Thacker, NC Li, Z Lin, WB AF Piechowicz, Marek Abney, Carter W. Zhou, Xin Thacker, Nathan C. Li, Zhong Lin, Wenbin TI Design, Synthesis, and Characterization of a Bifunctional Chelator with Ultrahigh Capacity for Uranium Uptake from Seawater Simulant SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID DENSITY-FUNCTIONAL THEORY; SEA-WATER; MESOPOROUS CARBON; CLIMATE-CHANGE; URANYL IONS; AMIDOXIME; EXTRACTION; RECOVERY; COMPLEXES; ADSORBENT AB Informed by density functional theory calculations, a novel bifunctional chelator, (Z)-2-[2-(N'-hydroxycarbamimidoyl)phenoxy]benzoic acid, was designed and synthesized for ultrahigh uranium uptake from seawater. Investigation of the ligand for uranium sorption was conducted in artificial seawater (pH = 8.2). An exceptional uranium uptake of 553 mg of uranium (g of sorbent)(-1) was obtained with a theoretical saturation capacity of 710 mg g(-1) obtained by fitting isotherm data with the Langmuir-Freundlich model. The resulting yellow precipitate was characterized via X-ray absorption fine structure (XAFS) at the U L-III-edge, with the extended XAFS spectra best fitted by a model where uranyl is coordinated by monodentate amidoxime, one chelating carboxylic acid, and two water molecules. These results are consistent with the formation of a uranium coordination polymer. The ultrahigh uranium uptake capacity obtained by the bifunctional chelating ligand makes it a promising candidate for deployment as a uranium adsorbent. C1 [Piechowicz, Marek; Abney, Carter W.; Zhou, Xin; Thacker, Nathan C.; Lin, Wenbin] Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA. [Zhou, Xin; Li, Zhong] S China Univ Technol, Sch Chem & Chem Engn, Guangzhou 510640, Guangdong, Peoples R China. [Abney, Carter W.] Oak Ridge Natl Lab, POB 2008,MS-6201, Oak Ridge, TN 37831 USA. RP Lin, WB (reprint author), Univ Chicago, Dept Chem, 929 East 57th St, Chicago, IL 60637 USA. EM wenbinlin@uchicago.edu RI Lin, Wenbin/B-4151-2010 OI Lin, Wenbin/0000-0001-7035-7759 FU Department of Energy (DOE), Office of Nuclear Energy's Nuclear Energy University Program [20 120427, 3151]; Oversea Study Program of Guangzhou Elite Project [JY201326]; DOE, Office of Science, by ANL [DE-AC02-06CH11357]; NSF [CHE-1048528]; Mass Spectrometry Facility FX This work was supported by the Department of Energy (DOE), Office of Nuclear Energy's Nuclear Energy University Program (Sub-Contract-20 120427 and Project 3151). X.Z. acknowledges financial support from the Oversea Study Program of Guangzhou Elite Project (JY201326). MRCAT operations are supported by the DOE and the MRCAT member institutions. This research used resources of the APS, a U.S. DOE, Office of Science User Facility, operated for the DOE, Office of Science, by ANL under Contract DE-AC02-06CH11357. The authors also thank Zekai Lin and Chris Poon for MS assistance. We acknowledge the University of Chicago Research Computing Center, the Nuclear Magnetic Resonance Facility, and NSF instrumentation Grant CHE-1048528 in conjunction with the Mass Spectrometry Facility for support of this work. NR 58 TC 1 Z9 1 U1 16 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4170 EP 4178 DI 10.1021/acs.iecr.5b03304 PG 9 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400010 ER PT J AU Parker, BF Knight, AS Vukovic, S Arnold, J Francis, MB AF Parker, Bernard F. Knight, Abigail S. Vukovic, Sinisa Arnold, John Francis, Matthew B. TI A Peptoid-Based Combinatorial and Computational Approach to Developing Ligands for Uranyl Sequestration from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ANISOTROPIC DIELECTRICS; METAL-BINDING; SEA-WATER; URANIUM; OLIGOMERS; FLUORESCENCE; EXTRACTION; STABILITY; COMPLEXES; DISCOVERY AB The selective binding of uranyl for extraction from seawater by using polymer sorbents holds promise as a sustainable source of uranium for nuclear energy. A combinatorially synthesized peptoid library (N-substituted glycine oligomers) was screened for uranyl binding with the goal of identifying high-affinity ligands for use in polymer sorbents. Qualitative screening techniques using a dye, arsenazo III, identified three uranyl-binding sequences, all of which contained only carboxylic acids as the active binding groups. Fluorescence spectroscopy was used to determine a dissociation constant for one of the identified peptoids by monitoring the decrease in peptoid fluorescence upon uranyl binding. Density functional theory calculations were used to model the solution-state binding of these sequences to understand favored binding modes and geometries. C1 [Parker, Bernard F.; Knight, Abigail S.; Arnold, John; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Parker, Bernard F.; Arnold, John] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Francis, Matthew B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Vukovic, Sinisa] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Vukovic, Sinisa] Univ Cambridge, Condensed Matter Theory Grp, Cavendish Lab, 19 JJ Thomson Ave, Cambridge CB3 OHE, England. [Knight, Abigail S.] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. RP Arnold, J; Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Arnold, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Francis, MB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM aknight@mrl.ucsb.edu; sv375@cam.ac.uk; arnold@berkeley.edu; mbfrancis@berkeley.edu RI Vukovic, Sinisa/J-3106-2013; Arnold, John/F-3963-2012 OI Vukovic, Sinisa/0000-0002-7682-0705; Arnold, John/0000-0001-9671-227X FU Nuclear Energy University Program, U.S. Department of Energy (DOE); National Science Foundation [CHE 1413666]; Berkeley Chemical Biology Graduate Program (NIH) [1 T32 GMO66698]; Philomathia Fellowship in Environmental Sciences; Fuel Resources Campaign in the Fuel Cycle Research and Development Program, Office of Nuclear Energy, DOE FX We thank the Nuclear Energy University Program, U.S. Department of Energy (DOE), for support of this research. A.S.K. and M.B.F. were supported by the National Science Foundation (Grant CHE 1413666). A.S.K. was supported by the Berkeley Chemical Biology Graduate Program (NIH Training Grant 1 T32 GMO66698) and a Philomathia Fellowship in Environmental Sciences. S.V. was supported by the Fuel Resources Campaign in the Fuel Cycle Research and Development Program, Office of Nuclear Energy, DOE. Portions of this work were carried out at the Molecular Foundry at Lawrence Berkeley National Laboratory. We thank the C. Chang group at the University of California at Berkeley for assistance with fluorescence spectroscopy experiments. NR 41 TC 0 Z9 0 U1 7 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4187 EP 4194 DI 10.1021/acs.iecr.5b03500 PG 8 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400012 ER PT J AU Chouyyok, W Wamer, CL Mackie, KE Warner, MG Gill, GA Addleman, RS AF Chouyyok, Wilaiwan Wamer, Cynthia L. Mackie, Katherine E. Warner, Marvin G. Gill, Gary A. Addleman, R. Shane TI Nanostructured Metal Oxide Sorbents for the Collection and Recovery of Uranium from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID NANOPOROUS SORBENTS; COMPOSITE-PARTICLES; POLYMERIC ADSORBENT; IRON OXYHYDROXIDE; AQUEOUS-SOLUTIONS; NATURAL-WATERS; ION-EXCHANGE; ADSORPTION; SURFACE; EXTRACTION AB The ability to collect uranium from seawater offers the potential for a long-term green fuel supply for nuclear energy. However, extraction of uranium, and other trace minerals, is challenging because of the high ionic strength and low mineral concentrations in seawater. Herein we evaluate the use of nanostructured metal oxide sorbents for the collection and recovery of uranium from seawater. Chemical affinity, chemical adsorption capacity, and uptake kinetics of sorbent materials were evaluated. Materials with higher surface area clearly produced better sorbent performance. Uptake kinetics showed that the materials could rapidly equilibrate in a few hours with effective solution contact. Manganese, iron oxide, and especially Mn-Fe nanostructured composites provided the best performance for uranium collection from seawater. The preferred materials were demonstrated to extract uranium from natural seawater with up to 3 mg U/g-sorbent in 4 h of contact time. Inexpensive nontoxic carbonate solutions were demonstrated to be an effective and environmentally benign method of stripping the uranium from the metal oxide sorbents. Various formats for the utilization of the nanostructured metals oxide sorbent materials are discussed, including traditional methods and nontraditional methods such as magnetic separation. C1 [Chouyyok, Wilaiwan; Wamer, Cynthia L.; Mackie, Katherine E.; Warner, Marvin G.; Addleman, R. Shane] Pacific NW Natl Lab, Richland, WA 99352 USA. [Gill, Gary A.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98383 USA. RP Addleman, RS (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM raymond.addleman@pnnl.gov FU Pacific Northwest National Laboratory (PNNL) Laboratory-Directed Research & Development (LDRD) Program; U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development Program, Fuel Resources Program [DE-AC05-76RL01830] FX The authors gratefully acknowledge the support of Pacific Northwest National Laboratory (PNNL) Laboratory-Directed Research & Development (LDRD) Program as well as U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development Program, Fuel Resources Program, contract number DE-AC05-76RL01830. The authors thank Dr. Dan Palo, Dr. Curtis J. Larimer, and Dr. George Bonheyo for their support and input and Dr. Timothy Droubay for magnetic measurements of iron oxide containing materials. PNNL is operated for the U.S. DOE by Battelle Memorial Institute. The content is solely the responsibility of the authors and does not necessarily represent the official views of the DOE, PNNL, or Battelle. NR 71 TC 2 Z9 2 U1 7 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4195 EP 4207 DI 10.1021/acs.iecr.5b03650 PG 13 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400013 ER PT J AU Mehio, N Williamson, B Oyola, Y Mayes, RT Janke, C Brown, S Dai, S AF Mehio, Nada Williamson, Ben Oyola, Yatsandra Mayes, Richard T. Janke, Chris Brown, Suree Dai, Sheng TI Acidity of the Poly(acrylamidoxime) Adsorbent in Aqueous Solution: Determination of the Proton Affinity Distribution via Potentiometric Titrations SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ADSORPTION ENERGY-DISTRIBUTION; STABLE NUMERICAL-SOLUTION; INDUCED PKA SHIFTS; METHACRYLIC-ACID; POLY(ACRYLIC ACID); INTEGRAL-EQUATION; LOCAL ISOTHERM; SEA-WATER; URANIUM; SEAWATER AB Poly(acrylamidoxime) fibers are the current state of the art adsorbent for mining uranium from seawater. While the acid dissociation constants, pK(a), of characteristic amidoxime and carboxylate ligands have been reported in the literature, the proton affinity distribution of the poly(acrylamidoxime) fiber is yet to be established. Herein, we report the poly(acrylamidoxime) proton affinity distribution between pH 2 and pH 10 via the stable numerical solution of the adsorption integral equation using splines (SAIUS) algorithm. Two peaks in the proton affinity distribution of poly(acrylamidoxime) were observed: the neutral to anionic dissociation of the carboxylate monomer between pH 3.2 and pH 4.4 (pK(a) approximate to 4.0) and the protonated to neutral dissociation of the acyclic amidoxime monomer between pH 5.6 and pH 6.8 (pK(a) approximate to 6.1). The acidity constants obtained for the carboxylate and amidoximate monomers vary from the acidity constants of acetic acid and acetamidoxime, respectively. These variations in acidity can be attributed to charge interactions between the carboxylate (pK(a) approximate to 4.76) and amidoxirne (pK(a) approximate to 5.78) monomers. This is a first step to resolving the metal cation affinity distribution of the poly(acrylamidoxime) fibers, which can aid in improving the selectivity of subsequent generations of chelating polymers used to mine uranium from seawater. C1 [Mehio, Nada; Brown, Suree; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Williamson, Ben; Oyola, Yatsandra; Mayes, Richard T.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Janke, Chris] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Brown, S; Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM suree@ion.chem.utk.edu; dais@ornl.gov RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX This work was sponsored by the U.S. Department of Energy, Office of Nuclear Energy, under Contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. NR 48 TC 3 Z9 3 U1 4 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4217 EP 4223 DI 10.1021/acs.iecr.5b03211 PG 7 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400015 ER PT J AU Mehio, N Ivanov, AS Ladshaw, AP Dai, S Bryantsev, VS AF Mehio, Nada Ivanov, Alexander S. Ladshaw, Austin P. Dai, Sheng Bryantsev, Vyacheslav S. TI Theoretical Study of Oxovanadium(IV) Complexation with Formamidoximate: Implications for the Design of Uranyl-Selective Adsorbents SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ANISOTROPIC DIELECTRICS; METHACRYLIC-ACID; AQUEOUS-SOLUTION; SOLID-STATE; SEA-WATER; SEAWATER; URANIUM; AMIDOXIME; ELECTRON; RECOVERY AB Poly(acrylamidoxime) fibers are the current state-of-the-art adsorbent for mining uranium from seawater. However, the competition between uranyl (UO22+) and vanadium ions poses a challenge to mining on the industrial scale. In this work, we employ density functional theory and coupled-cluster methods in the restricted formalism to investigate potential binding motifs of the oxovanadium(IV) ion (VO2+) with the formamidoximate ligand. Consistent with experimental extended X-ray absorption fine structure data, the hydrated six-coordinate complex is predicted to be preferred over the hydrated five coordinate complex. Our investigation of formamidoximate-VO2+ complexes universally identified the most stable binding motif formed by chelating a tautomerically rearranged imino hydroxylamine via the imino nitrogen and hydroxylamine oxygen. The alternative binding motifs for amidoxime chelation via a nonrearranged tautomer and eta(2) coordination are found to be similar to 11 kcal/mol less stable. Natural bond orbital analysis was performed to understand the nature of the interactions in the VO2+ complexes. The difference in the most stable VO2+ and UO22+ binding conformation has important implications for the design of more selective UO22+ ligands. C1 [Mehio, Nada; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Ivanov, Alexander S.; Dai, Sheng; Bryantsev, Vyacheslav S.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Ladshaw, Austin P.] Georgia Inst Technol, Dept Environm Engn, Atlanta, GA 30332 USA. RP Bryantsev, VS (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM bryantsevv@ornl.gov RI 范, 京/H-3271-2016; Ivanov, Alexander/K-4769-2014; Dai, Sheng/K-8411-2015; Bryantsev, Vyacheslav/M-5111-2016 OI Ivanov, Alexander/0000-0002-8193-6673; Dai, Sheng/0000-0002-8046-3931; Bryantsev, Vyacheslav/0000-0002-6501-6594 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the U.S. Department of Energy, Office of Nuclear Energy under Contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. This manuscript has been authored by UT-Battelle, LLC under Contract DE-AC05-00OR22725 with the U.S. Department of Energy. NR 48 TC 4 Z9 4 U1 6 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4231 EP 4240 DI 10.1021/acs.iecr.5b03398 PG 10 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400017 ER PT J AU Ladshaw, AP Das, S Liao, WP Yiacoumi, S Janke, CJ Mayes, RT Dai, S Tsouris, C AF Ladshaw, A. P. Das, S. Liao, W. -P. Yiacoumi, S. Janke, C. J. Mayes, R. T. Dai, S. Tsouris, C. TI Experiments and Modeling of Uranium Uptake by Amidoxime-Based Adsorbent in the Presence of Other Ions in Simulated Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID HYDROUS TITANIUM(IV) OXIDE; CHELATING FUNCTIONAL-GROUP; SEA-WATER; POLYMERIC ADSORBENT; METAL-OXIDE; ADSORPTION; RECOVERY; EXTRACTION; COMPLEXATION; FIBER AB Seawater contains uranium at an average concentration of 3.3 ppb, as well as a variety of other ions at either overwhelmingly higher or similar concentrations, which complicate the recovery of uranium. This report describes an investigation of the effects of various factors such as uranium speciation and presence of salts including sodium, calcium, magnesium, and bicarbonate, as well as trace elements such as vanadium on uranium adsorption kinetics in laboratory experiments. Adsorption models are also developed to describe the experimental data of uranium extraction from seawater. Results show that the presence of calcium and magnesium significantly slows down the uranium adsorption kinetics. Vanadium can replace uranium from amidoxime-based adsorbent, in the presence of sodium in the solution. Results also show that bicarbonate in the solution strongly competes with amidoxime for binding uranium, and thus slows down the uranium adsorption kinetics. Developed on the basis of the experimental findings, the model is capable of describing the effects of pH, ionic strength, temperature, and concentration of various species. The results of this work are useful in the understanding of the important factors that control the adsorbent capacity and kinetics of uranium uptake by amidoxime-based adsorbents. C1 [Ladshaw, A. P.; Yiacoumi, S.; Tsouris, C.] Georgia Inst Technol, Atlanta, GA 30332 USA. [Das, S.; Liao, W. -P.; Janke, C. J.; Mayes, R. T.; Dai, S.; Tsouris, C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Tsouris, C (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA.; Tsouris, C (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM tsourisc@ornl.gov RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027 FU US department of Energy, Office of Nuclear Energy; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX This work was sponsored by the US department of Energy, Office of Nuclear Energy. Notice: This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 38 TC 2 Z9 2 U1 10 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4241 EP 4248 DI 10.1021/acs.iecr.5b03456 PG 8 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400018 ER PT J AU Endrizzi, F Leggett, CJ Rao, LF AF Endrizzi, Francesco Leggett, Christina J. Rao, Linfeng TI Scientific Basis for Efficient Extraction of Uranium from Seawater. I: Understanding the Chemical Speciation of Uranium under Seawater Conditions SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID COMPLEX-FORMATION; LIEBIGITE; URANYL; ANDERSONITE; CARBONATE AB In recent years, the prospective recovery of uranium from seawater has become a topic of interest owing to the increasing demand for nuclear fuel worldwide and because of efforts to find sustainable alternatives to terrestrial mining for uranium. To date, the most advanced and promising method of extracting and concentrating uranium from seawater involves the use of polymeric sorbents containing the amidoxime binding moiety. Among a number of different moieties investigated, glutaroimide-dioxime is the most promising one, forming very stable complexes with U(VI) even in the presence of carbonate. To properly assess the affinity of uranium toward the amidoxime substrates, a comprehensive knowledge of the aqueous chemical equilibria of uranium is required. With this aim, in this paper we review the chemical equilibria of uranium (as UO22+) in seawater, focusing on the solution equilibria leading to the formation of the stable complexes, M-m(UO2)(CO3)(3)((2m-4)) (aq) (M = Ca or Mg, m = 0-2). These binary and ternary species dominate the chemistry of uranium in seawater and have recently been the object of study in several papers in the literature. The solubility equilibria of UO22+ in seawater leading to the formation of the known minerals, including Liebigite, Ca-2(UO2)(CO3)(3)center dot 10H(2)O(cr), Swartzite, CaMg(UO2)(CO3)(3)center dot 12H(2)O(cr), Bayleyite Mg-2(UO2)(CO3)(3)center dot 18H(2)O(cr), and Andersonite, Na2Ca(UO2)(CO3)(3)center dot 6H(2)O(cr), are also critically reviewed. Newly calculated values of the solubility products (log K-s(0)) for these solid compounds are presented based on the currently proposed speciation model that includes the most recent aforementioned data for the aqueous speciation of UO22+. Based on these data, simulated speciation diagrams are calculated, both at zero ionic strength and in seawater-like media. In combination with the speciation data for uranium with glutaroimide-dioxime, these models provide a better, more comprehensive picture of the chemical equilibria of U(VI) in seawater while also providing useful tools to help assess the feasibility of its recovery through amidoxime-based collection systems. C1 [Endrizzi, Francesco; Leggett, Christina J.; Rao, Linfeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. [Endrizzi, Francesco] Kalrlsruhe Inst Technol, Inst Nucl Waste Disposal KIT INE, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Leggett, Christina J.] US Nucl Regulatory Commiss, 11545 Rockville Pike,TWFN 4B34, Rockville, MD 20852 USA. RP Rao, LF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, One Cyclotron Rd, Berkeley, CA 94720 USA. EM lrao@lbl.gov FU Fuel Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy, the U.S. Department of Energy at Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231] FX This work was supported by the Fuel Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy, the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory (LBNL). NR 24 TC 4 Z9 4 U1 18 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4249 EP 4256 DI 10.1021/acs.iecr.5b03679 PG 8 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400019 ER PT J AU Leggett, CJ Endrizzi, F Rao, LF AF Leggett, Christina J. Endrizzi, Francesco Rao, Linfeng TI Scientific Basis for Efficient Extraction of Uranium from Seawater, II: Fundamental Thermodynamic and Structural Studies SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Review ID CHELATING POLYMERS; SEA WATER; AMIDOXIME; RECOVERY; COMPLEXATION; U(VI); GLUTARIMIDEDIOXIME; SEQUESTRATION; ADSORBENTS; SORBERS AB The development of an efficient and economical system for extracting uranium from seawater could lead to an essentially limitless source of fuel for nuclear reactors. Currently, the most promising technology for recovering uranium from seawater involves the use of polymeric sorbents functionalized with the amidoxime moiety. However, competition of amidoxime sorbents with carbonate for uranium, indiscriminate sorption of other seawater cations, seawater temperature, and sorbent durability affect the efficiency and cost of this technology. Insights from thermodynamic and structural studies have proved to be powerful tools for addressing these issues and aiding the development of more effective sorbents for uranium. We summarize herein the results of these studies and discuss their implications for the extraction of uranium from seawater. C1 [Leggett, Christina J.; Endrizzi, Francesco; Rao, Linfeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Leggett, Christina J.] US Nucl Regulatory Commiss, 11545 Rockville Pike,Mailstop TWFN 4B34, Rockville, MD 20852 USA. [Endrizzi, Francesco] Kalrlsruhe Inst Technol, Inst Nucl Waste Disposal KIT INE, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. RP Rao, LF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM christina.leggett@nrc.gov; francesco.endrizzi@kit.edu; lrao@lbl.gov FU Fuel Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy, the U.S. Department of Energy at Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231] FX This work was supported by the Fuel Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy, the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory (LBNL). NR 28 TC 6 Z9 6 U1 24 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4257 EP 4263 DI 10.1021/acs.iecr.5b03688 PG 7 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400020 ER PT J AU Gill, GA Kuo, LJ Janke, CJ Park, J Jeters, RT Bonheyo, GT Pan, HB Wai, C Khangaonkar, T Bianucci, L Wood, JR Warner, MG Peterson, S Abrecht, DG Mayes, RT Tsouris, C Oyola, Y Strivens, JE Schlafer, NJ Addleman, RS Chouyyok, W Das, S Kim, J Buesseler, K Breier, C D'Alessandro, E AF Gill, Gary A. Kuo, Li-Jung Janke, Chris J. Park, Jiyeon Jeters, Robert T. Bonheyo, George T. Pan, Horng-Bin Wai, Chien Khangaonkar, Tarang Bianucci, Laura Wood, Jordana R. Warner, Marvin G. Peterson, Sonja Abrecht, David G. Mayes, Richard T. Tsouris, Costas Oyola, Yatsandra Strivens, Jonathan E. Schlafer, Nicholas J. Addleman, R. Shane Chouyyok, Wilaiwan Das, Sadananda Kim, Jungseung Buesseler, Ken Breier, Crystal D'Alessandro, Evan TI The Uranium from Seawater Program at the Pacific Northwest National Laboratory: Overview of Marine Testing, Adsorbent Characterization, Adsorbent Durability, Adsorbent Toxicity, and Deployment Studies SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CHELATING FUNCTIONAL-GROUP; POLYMERIC ADSORBENT; NATURAL-WATERS; RECOVERY; EXTRACTION; COMPLEXATION; ADSORPTION; SORBENTS; IONS; GLUTARIMIDEDIOXIME AB The Pacific Northwest National Laboratory (PNNL) is evaluating the performance of adsorption materials to extract uranium from natural seawater. Testing consists of measurements of the adsorption of uranium and other elements from seawater as a function of time using flow-through columns and a recirculating flume to determine adsorbent capacity and adsorption kinetics. The amidoxime-based polymer adsorbent AF1, produced by Oak Ridge National Laboratory (ORNL), had a 56-day adsorption capacity of 3.9 +/- 0.2 g U/kg adsorbent material, a saturation capacity of 5.4 +/- 0.2 g U/kg adsorbent material, and a half-saturation time of 23 2 days. The ORNL AF1 adsorbent has a very high affinity for uranium, as evidenced by a 56-day distribution coefficient between adsorbent and solution of log K-D,K-56day = 6.08. Calcium and magnesium account for a majority of the cations adsorbed by the ORNL amidoxime-based adsorbents (61% by mass and 74% by molar percent), uranium is the fourth most abundant element adsorbed by mass and seventh most abundant by molar percentage. Marine testing at Woods Hole Oceanographic Institution with the ORNL AF1 adsorbent produced adsorption capacities 15% and 55% higher than those observed at PNNL for column and flume testing, respectively. Variations in competing ions may be the explanation for the regional differences. Hydrodynamic modeling predicts that a farm of adsorbent materials will likely have minimal effect on ocean currents and removal of uranium and other elements from seawater when farm densities are <1800 braids/km(2). A decrease in uranium adsorption capacity of up to 30% was observed after 42 days of exposure because of biofouling when the ORNL braided adsorbent AI8 was exposed to raw seawater in a flume in the presence of light. No toxicity was observed with flow-through column effluents of any absorbent materials tested to date. Toxicity could be induced with some non-amidoxime based absorbents only when the ratio of solid absorbent to test media was increased to part per thousand levels. Thermodynamic modeling of the seawater-amidoxime adsorbent was performed using the geochemical modeling program PHREEQC. Modeling of the binding of Ca, Mg, Fe, Ni, Cu, U, and V reveal that when binding sites are limited (1 X 10(-8) binding sites/kg seawater), vanadium heavily outcompetes other ions for the amidoxime sites. In contrast, when binding sites are abundant, Mg and Ca dominate the total percentage of metals bound to the sorbent. C1 [Gill, Gary A.; Kuo, Li-Jung; Park, Jiyeon; Jeters, Robert T.; Bonheyo, George T.; Khangaonkar, Tarang; Bianucci, Laura; Wood, Jordana R.; Warner, Marvin G.; Peterson, Sonja; Strivens, Jonathan E.; Schlafer, Nicholas J.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. [Janke, Chris J.; Mayes, Richard T.; Tsouris, Costas; Oyola, Yatsandra; Das, Sadananda; Kim, Jungseung] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Pan, Horng-Bin; Wai, Chien] Univ Idaho, Moscow, ID 83844 USA. [Abrecht, David G.; Addleman, R. Shane; Chouyyok, Wilaiwan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Buesseler, Ken; Breier, Crystal] Woods Hole Oceanog Inst, Woods Hole, MA 02543 USA. [D'Alessandro, Evan] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, 4600 Rickenbacker Causeway, Miami, FL 33149 USA. RP Gill, GA (reprint author), Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. EM gary.gill@pnnl.gov RI Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016 OI Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027 FU U.S. DOE Office of Nuclear Energy [DE-AC05-76RL01830, DE-AC05-00OR22725]; ORNL FX The PNNL effort was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-76RL01830 to PNNL. Work at ORNL was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-00OR22725 with ORNL, managed by UT-Battelle, LLC. Laboratory assistance by S. M. Pike at WHOI and Michael Cobb, Mary McGahan and Carolynn Suslick at PNNL is greatly appreciated. NR 60 TC 7 Z9 7 U1 15 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4264 EP 4277 DI 10.1021/acs.iecr.5b03649 PG 14 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400021 ER PT J AU Park, J Jeters, RT Kuo, LJ Strivens, JE Gill, GA Schlafer, NJ Bonheyo, GT AF Park, Jiyeon Jeters, Robert T. Kuo, Li-Jung Strivens, Jonathan E. Gill, Gary A. Schlafer, Nicholas J. Bonheyo, George T. TI Potential Impact of Seawater Uranium Extraction on Marine Life SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID VIBRIO-FISCHERI; VANADIUM BROMOPEROXIDASE; TOXICITY ASSESSMENT; NATURAL-PRODUCTS; REDUCTION; BIOREMEDIATION; MICROTOX; METALS; CHEMICALS; BIOSYNTHESIS AB A variety of adsorbent materials have been developed to extract uranium from seawater as an alternative traditional terrestrial mining. A large-scale deployment of these adsorbents would be necessary to recover useful quantities of uranium, and this raises a number of concerns regarding potential impacts on the surrounding marine environment. Two concerns are whether or not the adsorbent materials are toxic and any potentially harmful effects that may result from depleting uranium or vanadium (also highly concentrated by the adsorbents) from the local environment. To test the potential toxicity of the adsorbent with or without bound metals, Microtox assays were used to test both direct contact toxicity and the toxicity of any leachate in the seawater. The Microtox assay was chosen because it detected nonspecific mechanisms of toxicity. Toxicity was not observed with leachates from any of the 68 adsorbent materials that were tested, but direct contact with some adsorbents at very high adsorbent concentrations exhibited toxicity. These concentrations are, however, very unlikely to be seen in the actual marine deployment. Adsorbents that accumulated uranium and trace metals were also tested for toxicity, and no toxic effect was observed. Biofouling on the adsorbents and in columns or flumes containing the adsorbents also indicates that the adsorbents are not toxic and that there may not be an obvious deleterious effect resulting from removing uranium and vanadium from seawater. An extensive literature search was also performed to examine the potential impact of uranium and vanadium extraction from seawater on marine life using the Pacific Northwest National Laboratory's (PNNL's) document analysis tool, IN-SPIRE. Although other potential environmental effects must also be considered, results from both the Microtox assay and the literature search provide preliminary evidence that uranium extraction from seawater could be performed with minimal impact on marine fauna. C1 [Park, Jiyeon; Jeters, Robert T.; Kuo, Li-Jung; Strivens, Jonathan E.; Gill, Gary A.; Schlafer, Nicholas J.; Bonheyo, George T.] Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. RP Park, J (reprint author), Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. EM Jiyeon.Park@pnnl.gov OI Bonheyo, George/0000-0001-8853-5744 FU U.S. Department of Energy [DE-AC05-76RL01830] FX This work was supported by the lU.S. Department of Energy under Contract DE-AC05-76RL01830. NR 46 TC 4 Z9 4 U1 5 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4278 EP 4284 DI 10.1021/acs.iecr.5b03430 PG 7 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400022 ER PT J AU Kuo, LJ Janke, CJ Wood, JR Strivens, JE Das, S Oyola, Y Mayes, RT Gill, GA AF Kuo, Li-Jung Janke, Christopher J. Wood, Jordana R. Strivens, Jonathan E. Das, Sadananda Oyola, Yatsandra Mayes, Richard T. Gill, Gary A. TI Characterization and Testing of Amidoxime-Based Adsorbent Materials to Extract Uranium from Natural Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID RECOVERY; ELUTION; FIBER AB Extraction of uranium (U) from seawater for use as a nuclear fuel is a significant challenge due to the low concentration of U in seawater (similar to 3.3 ppb) and difficulties to selectively extract U from the background of major and trace elements in seawater. The Pacific Northwest National Laboratory (PNNL)'s Marine Sciences Laboratory (MSL) has been serving as a marine test site for determining performance characteristics (adsorption capacity, adsorption kinetics, and selectivity) of novel amidoxime-based polymeric adsorbents developed at Oak Ridge National Laboratory (ORNL) under natural seawater exposure conditions. This manuscript describes the performance of three formulations (38H, AF1, A18) of aniidoxime-based polymeric adsorbents produced at ORNL in MSL's ambient seawater testing facility. The adsorbents were produced in two forms, fibrous material (40-100 mg samples) and braided material (5-10 g samples), and exposed to natural seawater using flow-through columns and recirculating flumes. All three formulations demonstrated high 56 day uranium adsorption capacity (>3 g U/kg adsorbent). The AF1 formulation had the best uranium adsorption performance, with a 56 day capacity of 3.9 g U/kg adsorbent, a saturation capacity of 5.4 g U/kg adsorbent, and similar to 25 days half-saturation time. The two exposure methods, flow through columns and flumes, were demonstrated to produce similar performance results, providing confidence that the test methods were reliable, that scaling up from 10's of mg quantities of exposure in flow-through columns to gram quantities in flumes produced similar results, and confirm that the manufacturing process produces a homogeneous adsorbent. Adsorption kinetics appear to be element specific, with half-saturation times ranging from minutes for the major cations in seawater, to 8-10 weeks for V and Fe. Reducing the exposure time provides a potential pathway to improve the adsorption capacity of U by reducing the V/U ratio on the adsorbent. C1 [Kuo, Li-Jung; Wood, Jordana R.; Strivens, Jonathan E.; Gill, Gary A.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. [Janke, Christopher J.; Das, Sadananda; Oyola, Yatsandra; Mayes, Richard T.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RP Kuo, LJ (reprint author), Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. EM Li-Jung.Kuo@pnnl.gov RI Janke, Christopher/E-1598-2017 OI Janke, Christopher/0000-0002-6076-7188 FU U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development Program, Fuel Resources Program [DE-AC05- 76RL01830] FX This work was funded by the U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development Program, Fuel Resources Program (Contract No. DE-AC05- 76RL01830). We thank Mr. Nicholas J. Schlafer and Mr. Brett A. Romano for their help with construction, maintenance, and operation of the marine testing facility. We also thank Ms. Carolynn R. Suslick and Ms. Julie K. Snelling for quality assurance and database management support. NR 24 TC 9 Z9 9 U1 11 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4285 EP 4293 DI 10.1021/acs.iecr.5b03267 PG 9 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400023 ER PT J AU Das, S Tsouris, C Zhang, C Kim, J Brown, S Oyola, Y Janke, CJ Mayes, RT Kuo, LJ Wood, JR Gill, GA Dai, S AF Das, S. Tsouris, C. Zhang, C. Kim, J. Brown, S. Oyola, Y. Janke, C. J. Mayes, R. T. Kuo, L. -J. Wood, J. R. Gill, G. A. Dai, S. TI Enhancing Uranium Uptake by Amidoxime Adsorbent in Seawater: An Investigation for Optimum Alkaline Conditioning Parameters SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CHELATING FUNCTIONAL-GROUP; POLYMERIC ADSORBENT; FIBER ADSORBENTS; RECOVERY; ADSORPTION; STABILITY; BEHAVIOR; RESINS AB A high-surface-area polyethylene-fiber adsorbent (AF160-2) has been developed at the Oak Ridge National Laboratory by radiation-induced graft polymerization of acrylonitrile and itaconic acid. The grafted nitriles were converted to amidoxime groups by treating with hydroxylamine. The amidoximated adsorbents were then conditioned with potassium hydroxide (KOH) by varying different reaction parameters such as KOH concentration (0.2, 0.44, and 0.6 M), duration (1, 2, and 3 h), and temperature (60, 70, and 80 degrees C). Adsorbent screening was then performed with simulated seawater solutions containing sodium chloride and sodium bicarbonate, at concentrations found in seawater, and uranium nitrate at a uranium concentration of similar to 7-8 ppm and pH 8. Fourier transform infrared spectroscopy and solid-state NMR analyses indicated that a fraction of amidoxime groups was hydrolyzed to carboxylate during KOH conditioning. The uranium adsorption capacity in the simulated seawater screening solution gradually increased with conditioning time and temperature for all KOH concentrations. It was also observed that the adsorption capacity increased with an increase in concentration of KOH for all the conditioning times and temperatures. AF160-2 adsorbent samples were also tested with natural seawater using flow-through experiments to determine uranium adsorption capacity with varying KOH conditioning time and temperature. Based on uranium loading capacity values of several AF160-2 samples, it was observed that changing KOH conditioning time from 3 to 1 h at 60, 70, and 80 degrees C resulted in an increase of the uranium loading capacity in seawater, which did not follow the trend found in laboratory screening with stimulated solutions. Longer KOH conditioning times lead to significantly higher uptake of divalent metal ions, such as calcium and magnesium, which is a result of amidoxime conversion into less selective carboxylate. Scanning electron microscopy showed that long conditioning times may also lead to adsorbent degradation. C1 [Das, S.; Tsouris, C.; Zhang, C.; Kim, J.; Oyola, Y.; Janke, C. J.; Mayes, R. T.; Dai, S.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Brown, S.; Dai, S.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Kuo, L. -J.; Wood, J. R.; Gill, G. A.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Tsouris, C (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016; OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027; Das, Sadananda/0000-0002-8097-6542 FU U.S. DOE Office of Nuclear Energy [DE-AC05-00OR22725, DE-AC05-76RL01830]; ORNL FX This research was conducted at the Oak Ridge National Laboratory (ORNL) and at the Marine Sciences Laboratory, a part of the Pacific Northwest National Laboratory (PNNL) located in Sequim, WA. Work at ORNL was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-00OR22725 with ORNL, managed by UT-Battelle, LLC. The PNNL effort was also supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-76RL01830 to PNNL. NR 23 TC 7 Z9 7 U1 10 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4294 EP 4302 DI 10.1021/acs.iecr.5b02735 PG 9 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400024 ER PT J AU Das, S Liao, WP Byers, MF Tsouris, C Janke, CJ Mayes, RT Schneider, E Kuo, LJ Wood, JR Gill, GA Dai, S AF Das, S. Liao, W. -P. Byers, M. Flicker Tsouris, C. Janke, C. J. Mayes, R. T. Schneider, E. Kuo, L. -J. Wood, J. R. Gill, G. A. Dai, S. TI Alternative Alkaline Conditioning of Amidoxime Based Adsorbent for Uranium Extraction from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CHELATING FUNCTIONAL-GROUP; POLYMERIC ADSORBENT; FIBER ADSORBENTS; RECOVERY; ADSORPTION; COMPLEXATION; GLUTARIMIDEDIOXIME; MAGNESIUM; STRENGTH; CALCIUM AB Alkaline conditioning of the amidoxime based adsorbents is a significant step in the preparation of the adsorbent for uranium uptake from seawater. The effects of various alkaline conditioning parameters such as the type of alkaline reagent, reaction temperature, and reaction time were investigated with respect to uranium adsorption capacity from simulated seawater (spiked with 8 ppm uranium) and natural seawater (from Sequim Bay, WA). An adsorbent (AF1) was prepared at the Oak Ridge National Laboratory by radiation-induced graft polymerization (RIGP) with acrylonitrile and itaconic acid onto high-surface area polyethylene fibers. For the AF1 adsorbent, sodium hydroxide emerged as a better reagent for alkaline conditioning over potassium hydroxide, which has typically been used in previous studies, because of higher uranium uptake capacity and lower cost over the other candidate alkaline reagents investigated in this study. Use of sodium hydroxide in place of potassium hydroxide is shown to result in a 21-30% decrease in the cost of uranium recovery. C1 [Das, S.; Liao, W. -P.; Tsouris, C.; Janke, C. J.; Mayes, R. T.; Dai, S.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Kuo, L. -J.; Wood, J. R.; Gill, G. A.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. [Byers, M. Flicker; Schneider, E.] Univ Texas Austin, Nucl & Radiat Engn Program, Univ Stn C2200, Austin, TX 78712 USA. RP Tsouris, C (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA.; Schneider, E (reprint author), Univ Texas Austin, Nucl & Radiat Engn Program, Univ Stn C2200, Austin, TX 78712 USA. EM tsourisc@ornl.gov; eschneider@mail.utexas.edu RI Dai, Sheng/K-8411-2015; Janke, Christopher/E-1598-2017; Tsouris, Costas/C-2544-2016 OI Dai, Sheng/0000-0002-8046-3931; Janke, Christopher/0000-0002-6076-7188; Tsouris, Costas/0000-0002-0522-1027 FU U.S. DOE Office of Nuclear Energy [DE-AC05-00OR22725]; ORNL FX This research was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-00OR22725 with ORNL, managed by UT-Battelle, LLC. We thank Jonathan E. Strivens and Brett A. Romano (PNNL) for technical support on the marine testing. NR 42 TC 10 Z9 10 U1 6 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4303 EP 4312 DI 10.1021/acs.iecr.5b03210 PG 10 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400025 ER PT J AU Pang, HB Kuo, LJ Wai, CM Miyamoto, N Joshi, R Wood, JR Strivens, JE Janke, CJ Oyola, Y Das, S Mayes, RT Gill, GA AF Pang, Horng-Bin Kuo, Li-Jung Wai, Chien M. Miyamoto, Naomi Joshi, Ruma Wood, Jordana R. Strivens, Jonathan E. Janke, Christopher J. Oyola, Yatsandra Das, Sadananda Mayes, Richard T. Gill, Gary A. TI Elution of Uranium and Transition Metals from Amidoxime-Based Polymer Adsorbents for Sequestering Uranium from Seawater SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID AQUEOUS-SOLUTION; RECOVERY; U(VI); ADSORPTION; FIBER; STABILITY; SORPTION; SORBERS; FIELD; OXIDE AB High-surface-area amidoxime and carboxylic acid grafted polymer adsorbents developed at Oak Ridge National Laboratory were tested for sequestering uranium in a flowing seawater flume system at the PNNL-Marine Sciences Laboratory. FTIR spectra indicate that a KOH conditioning process is necessary to remove the proton from the carboxylic acid and make the sorbent effective for sequestering uranium from seawater. The alkaline conditioning process also converts the amidoxime groups to carboxylate groups in the adsorbent. Both Na2CO3-H2O2 and hydrochloric acid elution methods can remove similar to 95% of the uranium sequestered by the adsorbent after 42 days of exposure in real seawater. The Na2CO3-H2O2 elution method is more selective for uranium than conventional acid elution. Iron and vanadium are the two major transition metals competing with uranium for adsorption to the amidoxime-based adsorbents in real seawater. Tiron (4,5-dihydroxy-1,3-benzenedisulfonic acid disodium salt, 1 M) can remove iron from the adsorbent very effectively at pH around 7. The coordination between vanadium(V) and amidoxime is also discussed based on our V-51 NMR data. C1 [Pang, Horng-Bin; Wai, Chien M.; Miyamoto, Naomi; Joshi, Ruma] Univ Idaho, Dept Chem, Moscow, ID 83844 USA. [Kuo, Li-Jung; Wood, Jordana R.; Strivens, Jonathan E.; Gill, Gary A.] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. [Janke, Christopher J.; Oyola, Yatsandra; Das, Sadananda; Mayes, Richard T.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Wai, CM (reprint author), Univ Idaho, Dept Chem, Moscow, ID 83844 USA.; Gill, GA (reprint author), Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. EM cwai@uidaho.edu; gary.gill@pnnl.gov RI Janke, Christopher/E-1598-2017 OI Janke, Christopher/0000-0002-6076-7188 FU DOE-NEUP grant [00042246]; Uranium Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy of the U.S. Department of Energy at Pacific Northwest National Laboratory FX This study is partially supported by a DOE-NEUP grant (Contract Number 00042246) to the University of Idaho. Support of the Uranium Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy of the U.S. Department of Energy at Pacific Northwest National Laboratory is acknowledged. NR 37 TC 0 Z9 0 U1 8 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4313 EP 4320 DI 10.1021/acs.iecr.5b03307 PG 8 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400026 ER PT J AU Park, J Gill, GA Strivens, JE Kuo, LJ Jeters, RT Avila, A Wood, JR Schlafer, NJ Janke, CJ Miller, EA Thomas, M Addleman, RS Bonheyo, GT AF Park, Jiyeon Gill, Gary A. Strivens, Jonathan E. Kuo, Li-Jung Jeters, Robert T. Avila, Andrew Wood, Jordana R. Schlafer, Nicholas J. Janke, Christopher J. Miller, Erin A. Thomas, Mathew Addleman, R. Shane Bonheyo, George T. TI Effect of Biofouling on the Performance of Amidoxime-Based Polymeric Uranium Adsorbents SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ANTIFOULING COATINGS; SURFACE-ROUGHNESS; BIOFILM FORMATION; ADHESION; SETTLEMENT; EFFICIENT; BACTERIA; DIATOMS; GROWTH; LIGHT AB The Marine Science Laboratory at the Pacific Northwest National Laboratory evaluated the impact of biofouling on the performance or uranium adsorbents. A surface-modified polyethylene adsorbent fiber provided by Oak Ridge National Laboratory, AF adsorbent, was tested in either the presence or absence of light to simulate deployment in shallow or deep marine environments. Samples of the adsorbent fiber were exposed to seawater as loose fibers packed with glass beads in columns and as >10-cm-long braids of fiber placed in a flume that provided a continuous flow representative of natural ocean currents. Exposure tests (42 days) in column and flume settings showed that biofouling resulted in decreased uranium uptake by the adsorbent fiber. Uranium uptake was reduced by up to 30%, in the presence of simulated sunlight, which also increased biomass accumulation and altered the microbial community composition on the fibers. These results suggest that deployment below the photic zone would mitigate the effects of biofouling, resulting in greater yields of uranium extracted from seawater. C1 [Park, Jiyeon; Gill, Gary A.; Strivens, Jonathan E.; Kuo, Li-Jung; Jeters, Robert T.; Avila, Andrew; Wood, Jordana R.; Schlafer, Nicholas J.; Bonheyo, George T.] Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. [Miller, Erin A.; Thomas, Mathew; Addleman, R. Shane] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. [Janke, Christopher J.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RP Park, J; Bonheyo, GT (reprint author), Pacific NW Natl Lab, Marine Sci Lab, 1529 West Sequim Bay Rd, Sequim, WA 98382 USA. EM Jiyeon.Park@pnnl.gov; George.Bonheyo@pnnl.gov RI Janke, Christopher/E-1598-2017; OI Janke, Christopher/0000-0002-6076-7188; Bonheyo, George/0000-0001-8853-5744 FU U.S. Department of Energy [DE-AC05-76RL01830]; PNNL's Chemical Imaging Initiative; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy under Contract DE-AC05-76RL01830 and PNNL's Chemical Imaging Initiative. This research also used resources of the APS, a U.S. Department of Energy (DOE), Office of Science User Facility, operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. The authors thank Dana L. Woodruff for identification of organisms from 150 mu m filtered seawater and Matthew J. Marshall for acquiring APS imaging data. We also acknowledge the contributions of Yatsandra Oyola, Sadananda Das, and Richard T. Mayes, all of ORNL, in the production of the adsorbent fibers used for the tests. NR 36 TC 5 Z9 5 U1 11 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4328 EP 4338 DI 10.1021/acs.iecr.5b03457 PG 11 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400028 ER PT J AU Mayes, RT Gorka, J Dai, S AF Mayes, Richard T. Gorka, Joanna Dai, Sheng TI Impact of Pore Size on the Sorption of Uranyl under Seawater Conditions SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID URANIUM EXTRACTION; MESOPOROUS CARBON; SEA-WATER; RECOVERY; AMIDOXIME; ADSORPTION; SORBERS; RESINS AB The extraction of uranium from seawater has received significant interest recently, because of the possibility of a near-limitless supply of uranium to fuel the nuclear power industry. While sorbent development has focused primarily on polymeric sorbents, nanomaterials represent a new area that has the potential to surpass the current polymeric sorbents, because of the high surface areas that are possible. Mesoporous carbon materials are a stable, high-surface-area material capable of extracting various chemical species from a variety of environments. Herein, we report the use of a dual templating process to understand the effect of pore size on the adsorption of uranyl ions from a uranyl brine consisting of seawater-relevant sodium, chloride, and bicarbonate ions. It was found that pore size played a more significant role in the effective use of the grafted polymer, leading to higher uranium capacities than the surface area. Therefore, the pore size must be tailored to meet the demands of the extraction medium and analyte metal to achieve efficacy as an adsorbent. C1 [Mayes, Richard T.; Gorka, Joanna; Dai, Sheng] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Dai, Sheng] Univ Tennessee, Knoxville, TN USA. RP Mayes, RT (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN USA. EM mayesrt@ornl.gov RI Dai, Sheng/K-8411-2015 OI Dai, Sheng/0000-0002-8046-3931 FU U.S. Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory (ORNL) FX This work was sponsored by the U.S. Department of Energy, Office of Nuclear Energy, under Contract No. DE-AC05-00OR22725 with Oak Ridge National Laboratory (ORNL). ORNL is managed by UT-Battelle, LLC. NR 23 TC 0 Z9 0 U1 12 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4339 EP 4343 DI 10.1021/acs.iecr.5b03698 PG 5 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400029 ER PT J AU Wood, JR Gill, GA Kuo, LJ Strivens, JE Choe, KY AF Wood, Jordana R. Gill, Gary A. Kuo, Li-Jung Strivens, Jonathan E. Choe, Key-Young TI Comparison of Analytical Methods for the Determination of Uranium in Seawater Using Inductively Coupled Plasma Mass Spectrometry SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID ATOMIC-ABSORPTION-SPECTROMETRY; ICP-MS; TRACE-ELEMENTS; REDUCTIVE PRECIPITATION; ONLINE PRECONCENTRATION; REACTION CELL; SEA-WATER; MG(OH)(2) COPRECIPITATION; EXTRACTION CHROMATOGRAPHY; MATRIX ELIMINATION AB Trace element determinations in seawater by inductively coupled plasma mass spectrometry are analytically challenging due to the typically very low concentrations of the trace elements and the potential interference of the salt matrix. In this study, we did a comparison for uranium analysis using inductively coupled plasma mass spectrometry (ICP-MS) of Sequim Bay seawater samples and three seawater certified reference materials (SLEW-3, CASS-5, and NASS-6) using eight different analytical approaches. The methods evaluated include the following: direct analysis, Fe/Pd reductive precipitation, off-line preconcentration using the actinide specific resin, UTEVA, standard addition calibration, on-line automated dilution using an external calibration with and without matrix matching, and on-line automated preconcentration using the seaFast preconcentration resin. The two methods which produced the most accurate results were the method of standard addition calibration and off-line preconcentration using the UTEVA resin, recovering uranium from a Sequim Bay seawater sample at 101 +/- 1.2% and 98 +/- 2.7%, respectively. The on-line preconcentration method and the automated dilution with matrix-matched calibration method also performed very well. The two least effective methods were the direct analysis and the Fe/Pd reductive precipitation method using sodium borohydride. C1 [Wood, Jordana R.; Gill, Gary A.; Kuo, Li-Jung; Strivens, Jonathan E.; Choe, Key-Young] Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. RP Wood, JR (reprint author), Pacific NW Natl Lab, Marine Sci Lab, Sequim, WA 98382 USA. EM Jordana.wood@pnnl.gov FU U.S. DOE Office of Nuclear Energy [DE-AC05-76RL01830, DE-AC05-00OR22725]; ORNL FX The PNNL effort was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-76RL01830 to PNNL. Work at ORNL was supported by the U.S. DOE Office of Nuclear Energy, under Contract DE-AC05-00OR22725 with ORNL, managed by UT-Battelle, LLC. NR 38 TC 3 Z9 3 U1 10 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 20 PY 2016 VL 55 IS 15 BP 4344 EP 4350 DI 10.1021/acs.iecr.5b03680 PG 7 WC Engineering, Chemical SC Engineering GA DK3JH UT WOS:000374812400030 ER PT J AU Chen, YY Sanchez, C Yue, Y de Almeida, M Gonzalez, JM Parkinson, DY Liang, H AF Chen, Yunyun Sanchez, Carlos Yue, Yuan de Almeida, Mauricio Gonzalez, Jorge M. Parkinson, Dilworth Y. Liang, Hong TI Observation of yttrium oxide nanoparticles in cabbage (Brassica oleracea) through dual energy K-edge subtraction imaging (vol 14, 23, 2016) SO JOURNAL OF NANOBIOTECHNOLOGY LA English DT Correction C1 [Chen, Yunyun; Yue, Yuan; Liang, Hong] Texas A&M Univ, Mat Sci & Engn, College Stn, TX 77843 USA. [Sanchez, Carlos; Liang, Hong] Texas A&M Univ, Mech Engn, College Stn, TX 77843 USA. [de Almeida, Mauricio; Gonzalez, Jorge M.] Calif State Univ Fresno, Dept Plant Sci, Fresno, CA 93740 USA. [Parkinson, Dilworth Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Liang, H (reprint author), Texas A&M Univ, Mat Sci & Engn, College Stn, TX 77843 USA. EM hliang@tamu.edu NR 1 TC 0 Z9 0 U1 4 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1477-3155 J9 J NANOBIOTECHNOL JI J. Nanobiotechnol. PD APR 20 PY 2016 VL 14 AR 31 DI 10.1186/s12951-016-0186-9 PG 1 WC Biotechnology & Applied Microbiology; Nanoscience & Nanotechnology SC Biotechnology & Applied Microbiology; Science & Technology - Other Topics GA DK5ET UT WOS:000374943300001 PM 27097829 ER PT J AU Yang, B Keum, J Ovchinnikova, OS Belianinov, A Chen, SY Du, MH Ivanov, IN Rouleau, CM Geohegan, DB Xiao, K AF Yang, Bin Keum, Jong Ovchinnikova, Olga S. Belianinov, Alex Chen, Shiyou Du, Mao-Hua Ivanov, Ilia N. Rouleau, Christopher M. Geohegan, David B. Xiao, Kai TI Deciphering Halogen Competition in Organometallic Halide Perovskite Growth SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; ORGANOLEAD TRIHALIDE PEROVSKITE; LIGHT-EMITTING-DIODES; X-RAY-DIFFRACTION; PHOTOVOLTAIC CELLS; SINGLE-CRYSTALS; THIN-FILMS; PERFORMANCE; CHLORIDE; DIFFUSION AB Organometallic halide perovskites (OHPs) hold great promise for next-generation, low-cost optoelectronic devices. During the chemical synthesis and crystallization of OHP thin films, a major unresolved question is the competition between multiple halide species (e.g., I-, Cl-, Br-) in the formation of the mixed-halide perovskite crystals. Whether Cl- ions are successfully incorporated into the perovskite crystal structure or, alternatively, where they are located is not yet fully understood. Here, in situ X-ray diffraction measurements of crystallization dynamics are combined with ex situ TOF-SIMS chemical analysis to reveal that Br- or Cl- ions can promote crystal growth, yet reactive I- ions prevent them from incorporating into the lattice of the final perovskite.crystal structure. The Cl- ions are located in the grain boundaries of the perovskite films. These findings significantly advance our understanding of the role of halogens during synthesis of hybrid perovskites and provide an insightful guidance to the engineering of high-quality perovskite films, essential for exploring superior-performing and cost-effective optoelectronic devices. C1 [Yang, Bin; Keum, Jong; Ovchinnikova, Olga S.; Belianinov, Alex; Ivanov, Ilia N.; Rouleau, Christopher M.; Geohegan, David B.; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Keum, Jong] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Ovchinnikova, Olga S.; Belianinov, Alex] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Du, Mao-Hua] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Chen, Shiyou] E China Normal Univ, Key Lab Polar Mat & Devices MOE, Shanghai 200241, Peoples R China. RP Xiao, K (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM xiaok@ornl.gov RI Yang, Bin/P-8529-2014; Du, Mao-Hua/B-2108-2010; Geohegan, David/D-3599-2013; ivanov, ilia/D-3402-2015; Keum, Jong/N-4412-2015; OI Yang, Bin/0000-0002-5667-9126; Du, Mao-Hua/0000-0001-8796-167X; Geohegan, David/0000-0003-0273-3139; ivanov, ilia/0000-0002-6726-2502; Keum, Jong/0000-0002-5529-1373; Belianinov, Alex/0000-0002-3975-4112 FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX This research was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. M.H.D.'s work is supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The authors acknowledge Ho Ming Tong for preparation of contour plots (Figure 1b). NR 54 TC 13 Z9 14 U1 20 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 20 PY 2016 VL 138 IS 15 BP 5028 EP 5035 DI 10.1021/jacs.5b13254 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DK3JE UT WOS:000374812100010 PM 26931634 ER PT J AU Ko, C Lee, Y Chen, YB Suh, J Fu, D Suslu, A Lee, S Clarkson, JD Choe, HS Tongay, S Ramesh, R Wu, JQ AF Ko, Changhyun Lee, Yeonbae Chen, Yabin Suh, Joonki Fu, Deyi Suslu, Aslihan Lee, Sangwook Clarkson, James David Choe, Hwan Sung Tongay, Sefaatin Ramesh, Ramamoorthy Wu, Junqiao TI Ferroelectrically Gated Atomically Thin Transition-Metal Dichalcogenides as Nonvolatile Memory SO ADVANCED MATERIALS LA English DT Article DE 2D materials; ferroelectrics; field-effect transistors; nonvolatile memory; transition-metal dichalcogenides ID FIELD-EFFECT TRANSISTORS; SINGLE-LAYER MOS2; MOLYBDENUM-DISULFIDE; MONOLAYER MOS2; HETEROSTRUCTURES; FILMS; DEVICES; POLARIZATION; NANOSHEET; GRAPHENE C1 [Ko, Changhyun; Lee, Yeonbae; Chen, Yabin; Suh, Joonki; Fu, Deyi; Lee, Sangwook; Clarkson, James David; Choe, Hwan Sung; Ramesh, Ramamoorthy; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Suslu, Aslihan; Tongay, Sefaatin] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. [Ramesh, Ramamoorthy] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ramesh, Ramamoorthy; Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Fu, Deyi] Natl Univ Singapore, Dept Chem, 3 Sci Dr 3, Singapore 117543, Singapore. [Lee, Sangwook] Kyungpook Natl Univ, Sch Mat Sci & Engn, 80 Daehakro, Bukgu 41566, Daegu, South Korea. RP Wu, JQ (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Wu, JQ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM wuj@berkeley.edu RI Ko, Changhyun/E-1686-2011; Fu, Deyi/C-6624-2011; Wu, Junqiao/G-7840-2011 OI Fu, Deyi/0000-0003-1365-8963; Wu, Junqiao/0000-0002-1498-0148 FU NSF CAREER Award [DMR-1055938]; NSF [DMR-1306601]; NSF-TANMS Center; SRC FAME program FX This work was supported by a NSF CAREER Award under the Grant No. DMR-1055938. The 2D materials preparation and processing were partially supported by a NSF grant under the Grant No. DMR-1306601. Y.L. is supported by the NSF-TANMS Center and J.D.C. is supported by a SRC FAME program. C.K. and J.W. conceived the research and designed the experiments. C.K. carried out all the optical and electrical measurements and data analysis. Y.L., J.D.C. and R.R. grew and characterized the PZT films. C.K., Y.C., J.S., D.F., S.L., and H.S.C. prepared the 2D flakes and fabricated the devices collaboratively. A.S. and S.T. synthesized the WSe2 single crystals. The project was supervised by J.W. All the authors discussed results and contributed to writing the manuscript. The authors declare no competing financial interests. The authors thank Dr. Eunpa Kim, Prof. Kai Liu, and Dr. Deyang Chen for useful discussions and appreciate Taegyun Park's assistance in 2D material preparation. NR 53 TC 6 Z9 6 U1 34 U2 90 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 20 PY 2016 VL 28 IS 15 BP 2923 EP 2930 DI 10.1002/adma.201504779 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ6PZ UT WOS:000374336700009 PM 26894866 ER PT J AU Bouskill, NJ Wood, TE Baran, R Ye, Z Bowen, BP Lim, HC Zhou, JZ Van Nostrand, JD Nico, P Northen, TR Silver, WL Brodie, EL AF Bouskill, Nicholas J. Wood, Tana E. Baran, Richard Ye, Zaw Bowen, Benjamin P. Lim, Hsiao Chien Zhou, Jizhong Van Nostrand, Joy D. Nico, Peter Northen, Trent R. Silver, Whendee L. Brodie, Eoin L. TI Belowground Response to Drought in a Tropical Forest Soil. I. Changes in Microbial Functional Potential and Metabolism SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE tropical forests; drought; microbial ecology; osmolytes; functional gene microarray ID CLIMATE-CHANGE; ENZYME-ACTIVITY; EXTRACELLULAR ENZYMES; BACTERIAL COMMUNITIES; LITTER DECOMPOSITION; CALIFORNIA GRASSLAND; ORGANIC-CARBON; STRESS; MICROORGANISMS; MOISTURE AB Global climate models predict a future of increased severity of drought in many tropical forests. Soil microbes are central to the balance of these systems as sources or sinks of atmospheric carbon (C), yet how they respond metabolically to drought is not well understood. We simulated drought in the typically aseasonal Luquillo Experimental Forest, Puerto Rico, by intercepting precipitation falling through the forest canopy. This approach reduced soil moisture by 13% and water potential by 0.14 MPa (from -0.2 to -0.34). Previous results from this experiment have demonstrated that the diversity and composition of these soil microbial communities are sensitive to even small changes in soil water. Here, we show prolonged drought significantly alters the functional potential of the community and provokes a clear osmotic stress response, including the production of compatible solutes that increase intracellular C demand. Subsequently, a microbial population emerges with a greater capacity for extracellular enzyme production targeting macromolecular carbon. Significantly, some of these drought-induced functional shifts in the soil microbiota are attenuated by prior exposure to a short-term drought suggesting that acclimation may occur despite a lack of longer-term drought history. C1 [Bouskill, Nicholas J.; Ye, Zaw; Lim, Hsiao Chien; Zhou, Jizhong; Nico, Peter; Brodie, Eoin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Ecol, Div Earth Sci, Berkeley, CA 94720 USA. [Wood, Tana E.] US Forest Serv, Int Inst Trop Forestry, USDA, Rio Piedras, PR USA. [Wood, Tana E.] Fdn Puertorriquena Conservac, San Juan, PR USA. [Baran, Richard; Bowen, Benjamin P.; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong; Van Nostrand, Joy D.] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Zhou, Jizhong; Van Nostrand, Joy D.] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Silver, Whendee L.; Brodie, Eoin L.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Bouskill, NJ; Brodie, EL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Ecol, Div Earth Sci, Berkeley, CA 94720 USA.; Brodie, EL (reprint author), Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. EM njbouskill@lbl.gov; elbrodie@lbl.gov RI Brodie, Eoin/A-7853-2008; Bouskill, Nick/G-2390-2015; Nico, Peter/F-6997-2010; OI Brodie, Eoin/0000-0002-8453-8435; Nico, Peter/0000-0002-4180-9397; Northen, Trent/0000-0001-8404-3259 FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-050.111231, DE-AC02-05CH11231]; NSF [EAR-08199072, DEB 0620910]; Luquillo Critical Zone Observatory [EAR-0722476]; USGS Luquillo WEBB program FX This work was partially supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory. The Subsurface Biogeochemical Research program, the Next Generation Ecosystem Experiment (NGEE-Tropics), and ENIGMA-Ecosystems :and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov). All Scientific Focus Area Programs at Lawrence Berkeley National Laboratory supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under contract number DE-AC02-050.111231. This work was also partially funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under contract number DE-AC02-05CH11231, and by NSF grant EAR-08199072 to WS, the Luquillo Critical Zone Observatory (EAR-0722476) with additional support provided by the USGS Luquillo WEBB program, and grant DEB 0620910 from NSF to the Institute of Tropical Forest Ecosystem Studies, University of Puerto Rico, and to the International Institute of Tropical Forestry USDA Forest Service, as part of the Luquillo Long-Term Ecological Research Program. NR 87 TC 3 Z9 3 U1 23 U2 57 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 20 PY 2016 VL 7 AR 525 DI 10.3389/fmicb.2016.00525 PG 11 WC Microbiology SC Microbiology GA DJ7DO UT WOS:000374372300001 PM 27148214 ER PT J AU Wang, M Lu, L Li, C Xiao, XH Zhou, XM Zhu, J Luo, SN AF Wang, M. Lu, L. Li, C. Xiao, X. H. Zhou, X. M. Zhu, J. Luo, S. N. TI Deformation and spallation of a magnesium alloy under high strain rate loading SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Magnesium alloys; Twinning; Strain rate; Impact; EBSD ID MECHANICAL-BEHAVIOR; CONTRACTION TWINS; DYNAMIC FRACTURE; ROOM-TEMPERATURE; PURE MAGNESIUM; MG ALLOYS; TEXTURE; SHOCK; MICROSTRUCTURES; COMPOSITES AB We investigate deformation and damage of a magnesium alloy, AZ91, under high strain rate (similar to 10(5) s(-1)) loading via planar impact. The soft-recovered specimens are examined with electron back-scatter diffraction (EBSD). EBSD analysis reveals three types of twinning: {1012} extension, {10 (1) over bar1} contraction, and {10 (1) over bar1}-{10 (1) over bar2) double twinning, and their number density increases with increasing impact velocity. The extension twins dominate contraction and double twins in size and number. Dislocation densities of the recovered specimens are evaluated with x-ray diffraction, and increase with increasing impact velocity. X-ray tomography is used to resolve three-dimensional microstructure of shock-recovered samples. The EBSD and tomography results demonstrate that the second phase, Mg17Al12, plays an important role in both deformation twinning and tensile cracking. Deformation twinning appears to be a common mechanism in deformation of magnesium alloys at low, medium and high strain rates, in addition to dislocation motion. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wang, M.; Li, C.; Zhu, J.] Sichuan Univ, Coll Phys Sci & Technol, Chengdu 610064, Sichuan, Peoples R China. [Wang, M.; Luo, S. N.] Southwest Jiaotong Univ, Minist Educ, Key Lab Adv Technol Mat, Chengdu 610031, Sichuan, Peoples R China. [Wang, M.; Lu, L.; Li, C.; Zhou, X. M.; Luo, S. N.] Peac Inst Multiscale Sci, Chengdu 610031, Sichuan, Peoples R China. [Xiao, X. H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Lu, L.] Univ Sci & Technol China, Dept Modem Mech, CAS Key Lab Mech Behav & Design Mat, Hefei 230027, Anhui, Peoples R China. RP Zhu, J (reprint author), Sichuan Univ, Coll Phys Sci & Technol, Chengdu 610064, Sichuan, Peoples R China.; Luo, SN (reprint author), Peac Inst Multiscale Sci, Chengdu 610031, Sichuan, Peoples R China. EM zhujun01@163.com; sluo@pims.ac.cn RI Luo, Sheng-Nian /D-2257-2010 OI Luo, Sheng-Nian /0000-0002-7538-0541 FU (U.S.) DOE [DE-AC02-06CH11357]; 973 project [2014CB845904]; NSFC [11472227]; NSAF of China [U1230202] FX Use of the Advanced Photon Source, an Office of Science User Facility operated for the (U.S.) Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the (U.S.) DOE under Contract No. DE-AC02-06CH11357. This work was supported in part by the 973 project (No. 2014CB845904), NSFC (No. 11472227), and NSAF (No. U1230202) of China. NR 33 TC 1 Z9 1 U1 8 U2 17 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD APR 20 PY 2016 VL 661 BP 126 EP 131 DI 10.1016/j.msea.2016.03.009 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DK0SH UT WOS:000374622000015 ER PT J AU Mello, AW Nicolas, A Lebensohn, RA Sangid, MD AF Mello, Alberto W. Nicolas, Andrea Lebensohn, Ricardo A. Sangid, Michael D. TI Effect of microstructure on strain localization in a 7050 aluminum alloy: Comparison of experiments and modeling for various textures SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Microstructure; Digital image correlation; Electron backscatter diffraction; Strain localization; Heterogeneous deformation; Elasto-viscoplastic crystal plasticity ID GRAIN-BOUNDARIES; DEFORMATION; OLIGOCRYSTAL AB Microstructure attributes are responsible for heterogeneous deformation and strain localization. In this study, the relation between residual strain fields and microstructure is examined and assessed by means of experiments and crystal plasticity modeling. The microstructure of rolled aluminum alloys (AA) in the 7050-T7451 condition was experimentally obtained with electron backscatter diffraction (EBSD) analysis along the rolling direction (L-T orientation), across the rolling direction (T-L orientation), and transverse to the rolling direction (T-S orientation). Each of these sections was also patterned using a novel microstamping procedure, to allow for strain mapping by digital image correlation (DIC). The measured microstructures were in turn used as input of an elasto-viscoplastic crystal plasticity formulation based on fast Fourier transforms (EVP-FFT). Comparisons between the strain maps obtained experimentally by the concurrent DIC-EBSD method and the EVP-FFT simulations were made for the three sections, corresponding to the initial textures. The comparisons showed that the predicted levels of strain concentration were reasonable for all three specimens from a statistical perspective, which is important to properly describe and predict the strains within an ensemble of components; however the spatial match with the actual strain fields needs improvement. (C) 2016 Elsevier B.V. All rights reserved. C1 [Mello, Alberto W.; Nicolas, Andrea; Sangid, Michael D.] Purdue Univ, Sch Aeronaut & Astronaut, 701 W Stadium Ave, W Lafayette, IN 47907 USA. [Lebensohn, Ricardo A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Sangid, MD (reprint author), Purdue Univ, Sch Aeronaut & Astronaut, 701 W Stadium Ave, W Lafayette, IN 47907 USA. EM msangid@purdue.edu RI Lebensohn, Ricardo/A-2494-2008 OI Lebensohn, Ricardo/0000-0002-3152-9105 FU Office of Naval Research [N00014-14-1-0544]; Joint DoD/DOE Munitions Technology Programs FX The authors gratefully acknowledge funding from the Office of Naval Research, N00014-14-1-0544. RAL acknowledges support from the Joint DoD/DOE Munitions Technology Programs. Also, the authors graciously acknowledge technical support and advice from Mr. Andrea Rovinelli (EVP-FFT) and Major Todd Book (EBSD). Drs. Jacob Hochhalter and Andrew Cannon are thanked for their help with the micro stamping design, development, and procedure. NR 28 TC 1 Z9 1 U1 2 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD APR 20 PY 2016 VL 661 BP 187 EP 197 DI 10.1016/j.msea.2016.03.012 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DK0SH UT WOS:000374622000022 ER PT J AU Aydogan, E Pal, S Anderoglu, O Maloy, SA Vogel, SC Odette, GR Lewandowski, JJ Hoelzer, DT Anderson, IE Rieken, JR AF Aydogan, E. Pal, S. Anderoglu, O. Maloy, S. A. Vogel, S. C. Odette, G. R. Lewandowski, J. J. Hoelzer, D. T. Anderson, I. E. Rieken, J. R. TI Effect of tube processing methods on the texture and grain boundary characteristics of 14YWT nanostructured ferritic alloys SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Texture; EBSD; Neutron diffraction; Nanostructured ferritic alloys ID SITU HELIUM IMPLANTER; HYDROSTATIC EXTRUSION; FRACTURE-TOUGHNESS; STEEL CLADDINGS; TEMPERATURE; MICROSTRUCTURE; BEHAVIOR; MA957; ORIENTATION; STABILITY AB Texture and microstructure of tubes and plates fabricated from a nanostructured ferritic alloy (14YWT), produced either by spray forming followed by hydrostatic extrusion (Process I) or hot extrusion and cross-rolling a plate followed by hydrostatic tube extrusion (Process II) have been characterized in terms of their effects on texture and grain boundary character. Hydrostatic extrusion results in a combination of plane strain and shear deformations which generate low intensity alpha- and gamma-fiber components of {001} < 110 > and {111} < 110 > together with a weak zeta-fiber component of {011} < 211 > and {011} < 011 >. In contrast, multi-step plane strain deformation by hot extrusion and cross-rolling of the plate leads to a strong texture component of {001} < 110 > together with a weaker {111} < 112 > component. Although the total strains are similar, shear dominated deformation leads to much lower texture indexes compared to plane strain deformations. Further, the texture intensity decreases after hydrostatic extrusion of the alloy plate formed by plane strain deformation, due to a lower number of activated slip systems during shear dominated deformation. Notably, hot extruded and cross-rolled plate subjected to plane strain deformation to similar to 50% engineering strain creates only a modest population of low angle grain boundaries, compared to the much larger population observed following the combination of plane strain and shear deformation of similar to 44% engineering strain resulting from subsequent hydrostatic extrusion. Published by Elsevier B.V. C1 [Aydogan, E.; Anderoglu, O.; Maloy, S. A.; Vogel, S. C.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Pal, S.; Odette, G. R.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Lewandowski, J. J.] Case Western Reserve Univ, Cleveland, OH 44106 USA. [Hoelzer, D. T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Anderson, I. E.; Rieken, J. R.] Ames Lab, Ames, IA 50011 USA. [Aydogan, E.] Texas A&M Univ, College Stn, TX 77840 USA. RP Aydogan, E (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.; Aydogan, E (reprint author), Texas A&M Univ, College Stn, TX 77840 USA. EM aydogan@lanl.gov RI Hoelzer, David/L-1558-2016; Maloy, Stuart/A-8672-2009; OI Maloy, Stuart/0000-0001-8037-1319; Vogel, Sven C./0000-0003-2049-0361 FU DOE-NE Fuel Cycle Research and Development Program [DE-AC52-06NA25396] FX This research was partially supported by DOE-NE Fuel Cycle Research and Development Program under the Contract number DE-AC52-06NA25396. NR 48 TC 1 Z9 1 U1 7 U2 21 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD APR 20 PY 2016 VL 661 BP 222 EP 232 DI 10.1016/j.msea.2016.02.085 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DK0SH UT WOS:000374622000026 ER PT J AU Gruss, D Velizhanin, KA Zwolak, M AF Gruss, Daniel Velizhanin, Kirill A. Zwolak, Michael TI Landauer's formula with finite-time relaxation: Kramers' crossover in electronic transport SO SCIENTIFIC REPORTS LA English DT Article ID FIELD-EFFECT TRANSISTOR; CARBON NANOTUBE; QUANTUM TRANSPORT; QUANTIZED CONDUCTANCE; DEPENDENT TRANSPORT; POINT CONTACTS; SINGLE; DNA; SYSTEMS; NUCLEOTIDES AB Landauer's formula is the standard theoretical tool to examine ballistic transport in nano-and mesoscale junctions, but it necessitates that any variation of the junction with time must be slow compared to characteristic times of the system, e.g., the relaxation time of local excitations. Transport through structurally dynamic junctions is, however, increasingly of interest for sensing, harnessing fluctuations, and real-time control. Here, we calculate the steady-state current when relaxation of electrons in the reservoirs is present and demonstrate that it gives rise to three regimes of behavior: weak relaxation gives a contact-limited current; strong relaxation localizes electrons, distorting their natural dynamics and reducing the current; and in an intermediate regime the Landauer view of the system only is recovered. We also demonstrate that a simple equation of motion emerges, which is suitable for efficiently simulating time-dependent transport. C1 [Gruss, Daniel; Zwolak, Michael] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. [Gruss, Daniel] Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA. [Gruss, Daniel] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. [Velizhanin, Kirill A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Zwolak, M (reprint author), NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. EM mpz@nist.gov RI Velizhanin, Kirill/C-4835-2008; Zwolak, Michael/G-2932-2013 OI Zwolak, Michael/0000-0001-6443-7816 FU University of Maryland [70NANB10H193]; National Institute of Standards and Technology Center for Nanoscale Science and Technology through the University of Maryland [70NANB10H193]; U.S. Department of Energy through the LANL/LDRD Program FX Daniel Gruss acknowledges support under the Cooperative Research Agreement between the University of Maryland and the National Institute of Standards and Technology Center for Nanoscale Science and Technology, Award 70NANB10H193, through the University of Maryland. Kirill A. Velizhanin was supported by the U.S. Department of Energy through the LANL/LDRD Program. NR 55 TC 0 Z9 0 U1 2 U2 7 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 20 PY 2016 VL 6 AR 24514 DI 10.1038/srep24514 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7JG UT WOS:000374387100001 PM 27094206 ER PT J AU Nomura, K Kalia, RK Li, Y Nakano, A Rajak, P Sheng, CY Shimamura, K Shimojo, F Vashishta, P AF Nomura, Ken-ichi Kalia, Rajiv K. Li, Ying Nakano, Aiichiro Rajak, Pankaj Sheng, Chunyang Shimamura, Kohei Shimojo, Fuyuki Vashishta, Priya TI Nanocarbon synthesis by high-temperature oxidation of nanoparticles SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; SILICON-CARBIDE; CARBON NANOTUBES; POROUS SILICA; GRAPHENE; GROWTH; SURFACES; OXYGEN; WATER AB High-temperature oxidation of silicon-carbide nanoparticles (nSiC) underlies a wide range of technologies from high-power electronic switches for efficient electrical grid and thermal protection of space vehicles to self-healing ceramic nanocomposites. Here, multimillion-atom reactive molecular dynamics simulations validated by ab initio quantum molecular dynamics simulations predict unexpected condensation of large graphene flakes during high-temperature oxidation of nSiC. Initial oxidation produces a molten silica shell that acts as an autocatalytic 'nanoreactor' by actively transporting oxygen reactants while protecting the nanocarbon product from harsh oxidizing environment. Percolation transition produces porous nanocarbon with fractal geometry, which consists of mostly sp(2) carbons with pentagonal and heptagonal defects. This work suggests a simple synthetic pathway to high surface-area, low-density nanocarbon with numerous energy, biomedical and mechanical-metamaterial applications, including the reinforcement of self-healing composites. C1 [Nomura, Ken-ichi; Kalia, Rajiv K.; Nakano, Aiichiro; Rajak, Pankaj; Sheng, Chunyang; Shimamura, Kohei; Vashishta, Priya] Univ So Calif, Dept Phys & Astron, Dept Chem Engn & Mat Sci, Collaboratory Adv Comp & Simulat,Dept Comp Sci, Los Angeles, CA 90089 USA. [Nomura, Ken-ichi; Kalia, Rajiv K.; Nakano, Aiichiro; Rajak, Pankaj; Sheng, Chunyang; Shimamura, Kohei; Vashishta, Priya] Univ So Calif, Dept Biol Sci, Los Angeles, CA 90089 USA. [Li, Ying] Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave, Argonne, IL 60439 USA. [Shimamura, Kohei; Shimojo, Fuyuki] Kumamoto Univ, Dept Phys, Kumamoto 8608555, Japan. [Shimamura, Kohei] Kobe Univ, Dept Computat Sci, Kobe, Hyogo 6578501, Japan. RP Nakano, A (reprint author), Univ So Calif, Dept Phys & Astron, Dept Chem Engn & Mat Sci, Collaboratory Adv Comp & Simulat,Dept Comp Sci, Los Angeles, CA 90089 USA.; Nakano, A (reprint author), Univ So Calif, Dept Biol Sci, Los Angeles, CA 90089 USA. EM anakano@usc.edu RI Shimamura, Kohei/R-8513-2016 OI Shimamura, Kohei/0000-0003-3235-2599 FU Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division [DE-FG02-04 ER-46130]; KAKENHI [23104512] FX This research was supported by the Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division, Grant # DE-FG02-04 ER-46130. The work in Japan was supported by KAKENHI (23104512). The simulations were performed using the 786,432-core IBM Blue Gene/Q computer at the Argonne Leadership Computing Facility under the DOE INCITE program and at the Center for High Performance Computing of the University of Southern California. We thank Dr. Paul Messina and Dr. Nicholas Romero for their help on the use of Blue Gene/Q and Prof. Koji Matsuura for discussions about experimental confirmation of our first-principles predictions. We are also grateful to Dr. Joseph Insley for creating the Supplementary movie, S2.mov. NR 46 TC 0 Z9 0 U1 15 U2 44 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 20 PY 2016 VL 6 AR 24109 DI 10.1038/srep24109 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7IU UT WOS:000374385900001 PM 27095061 ER PT J AU Cao, S Zhang, XZ Paudel, TR Sinha, K Wang, X Jiang, XY Wang, WB Brutsche, S Wang, J Ryan, PJ Kim, JW Cheng, XM Tsymbal, EY Dowben, PA Xu, XS AF Cao, Shi Zhang, Xiaozhe Paudel, Tula R. Sinha, Kishan Wang, Xiao Jiang, Xuanyuan Wang, Wenbin Brutsche, Stuart Wang, Jian Ryan, Philip J. Kim, Jong-Woo Cheng, Xuemei Tsymbal, Evgeny Y. Dowben, Peter A. Xu, Xiaoshan TI On the structural origin of the single-ion magnetic anisotropy in LuFeO3 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE magnetic anisotropy; x-ray absorption spectroscopy; x-ray diffraction; structural distortion; electronic structure ID ORTHOFERRITES AB The electronic structure for the conduction bands of both hexagonal and orthorhombic LuFeO3 thin films have been measured using x-ray absorption spectroscopy at oxygen K (O K) edge. Dramatic differences in both the spectral features and the linear dichroism are observed. These differences in the spectra can be explained using the differences in crystal field splitting of the metal (Fe and Lu) electronic states and the differences in O 2p-Fe 3d and O 2p-Lu 5d hybridizations. While the oxidation states have not changed, the spectra are sensitive to the changes in the local environments of the Fe3+ and Lu3+ sites in the hexagonal and orthorhombic structures. Using the crystal-field splitting and the hybridizations that are extracted from the measured electronic structures and the structural distortion information, we derived the occupancies of the spin minority states in Fe3+, which are non-zero and uneven. The single ion anisotropy on Fe3+ sites is found to originate from these uneven occupancies of the spin minority states via spin-orbit coupling in LuFeO3. C1 [Cao, Shi; Zhang, Xiaozhe; Paudel, Tula R.; Sinha, Kishan; Jiang, Xuanyuan; Brutsche, Stuart; Tsymbal, Evgeny Y.; Dowben, Peter A.; Xu, Xiaoshan] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Cao, Shi; Zhang, Xiaozhe; Paudel, Tula R.; Sinha, Kishan; Jiang, Xuanyuan; Brutsche, Stuart; Tsymbal, Evgeny Y.; Dowben, Peter A.; Xu, Xiaoshan] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Zhang, Xiaozhe] Xi An Jiao Tong Univ, Dept Phys, Xian 710049, Peoples R China. [Wang, Xiao; Cheng, Xuemei] Bryn Mawr Coll, Dept Phys, Bryn Mawr, PA 19010 USA. [Wang, Wenbin] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Wang, Jian] Canadian Light Source, Saskatoon, SK S7N 2V3, Canada. [Ryan, Philip J.; Kim, Jong-Woo] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Xu, XS (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA.; Xu, XS (reprint author), Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. EM xiaoshan.xu@unl.edu RI Xu, Xiaoshan/B-1255-2009; Tsymbal, Evgeny/G-3493-2013; Wang, Jian/M-1805-2013; OI Xu, Xiaoshan/0000-0002-4363-392X; Cao, Shi/0000-0001-9380-2683 FU National Science Foundation through the Nebraska Materials Research Science and Engineering Center [DMR-1420645]; Semiconductor Research Corporation through the Center for Nanoferroic Devices; SRC-NRI Center [2398.001]; Canada Foundation for Innovation; Natural Sciences and Engineering Research Council of Canada; National Research Council Canada; Canadian Institutes of Health Research; Government of Saskatchewan, Western Economic Diversification Canada; University of Saskatchewan; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation [1053854] FX This project was primarily supported by the National Science Foundation through the Nebraska Materials Research Science and Engineering Center (Grant No. DMR-1420645). Additional support was provided by the Semiconductor Research Corporation through the Center for Nanoferroic Devices and the SRC-NRI Center under Task ID 2398.001. The Canadian Light Source is funded by the Canada Foundation for Innovation, the Natural Sciences and Engineering Research Council of Canada, the National Research Council Canada, the Canadian Institutes of Health Research, the Government of Saskatchewan, Western Economic Diversification Canada, and the University of Saskatchewan. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Computations were performed utilizing the Holland Computing Center of the University of Nebraska. X M Cheng acknowledges support from the National Science Foundation under Grant No. 1053854. NR 30 TC 2 Z9 2 U1 12 U2 27 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 20 PY 2016 VL 28 IS 15 AR 156001 DI 10.1088/0953-8984/28/15/156001 PG 10 WC Physics, Condensed Matter SC Physics GA DI4FX UT WOS:000373456900010 PM 26982512 ER PT J AU Jacobsen, MK Velisavljevic, N Dattelbaum, DM Chellappa, RS Park, C AF Jacobsen, M. K. Velisavljevic, N. Dattelbaum, D. M. Chellappa, R. S. Park, C. TI High pressure and temperature equation of state and spectroscopic study of CeO2 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE ceria; high pressure; equation of state; spectroscopy ID INDUCED PHASE-TRANSFORMATION; X-RAY-ABSORPTION; HYDROSTATIC LIMITS; FLUORITE STRUCTURE; CERIA; SPECTRA; GPA AB One of the most widely used x-ray standards and a highly applied component of catalysis systems, CeO2 has been studied for the purpose of better understanding its equation of state and electronic properties. Diamond anvil cells have been used to extend the equation of state for this material to 130 GPa and explore the electronic behavior with applied load. From the x-ray diffraction studies, it has been determined that the high pressure phase transition extends from approximately 35-75 GPa at ambient temperature. Elevation of temperature is found to decrease the initiation pressure for this transition, with multiple distinct temperature regions which indicate structural related anomalies. In addition, hydrostatic and non-hydrostatic effects are compared and exhibit a drastic difference in bulk moduli. The electronic results indicate a change in the scattering environment of the cerium atom, associated with the high pressure phase transition. Overall, these results present the first megabar pressure study and the first high pressure and temperature study of ceria. Additionally, this shows the first combined study of the K and L-III edges of this material to 33 GPa. C1 [Jacobsen, M. K.; Velisavljevic, N.; Dattelbaum, D. M.] Los Alamos Natl Lab, Shock & Detonat Phys M 9, POB 1663,MS P952, Los Alamos, NM 87545 USA. [Chellappa, R. S.] Los Alamos Natl Lab, Mat Sci & Technol MST 8, POB 1663,MS H805, Los Alamos, NM 87545 USA. [Park, C.] Carnegie Inst Washiongton, Geophys Lab, HPCAT, 9700 S Cass Ave,Bldg 434E, Argonne, IL 60439 USA. RP Jacobsen, MK (reprint author), Los Alamos Natl Lab, Shock & Detonat Phys M 9, POB 1663,MS P952, Los Alamos, NM 87545 USA. EM mjacobsen@lanl.gov RI Park, Changyong/A-8544-2008 OI Park, Changyong/0000-0002-3363-5788 FU DOE-NNSA [DE-AC52-06NA25396, DE-NA0001974]; DOE-BES [DE-FG02-99ER45775]; NSF; US DOE [DE-AC02-06CH11357]; COMPRES under NSF [EAR 11-57758]; GSECARS through NSF [EAR-1128799]; DOE [DE-FG02-94ER14466]; U.S. Department of Energy through the LANL/LDRD Program; G T Seaborg Institute FX Los Alamos National Laboratory (LANL) is operated by LANS, LLC for the DOE-NNSA under contract no. DE-AC52-06NA25396. Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. Use of the COMPRES-GSECARS gas loading system was supported by COMPRES under NSF Cooperative Agreement EAR 11-57758 and by GSECARS through NSF grant EAR-1128799 and DOE grant DE-FG02-94ER14466. MKJ gratefully acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program and the G T Seaborg Institute. NR 35 TC 0 Z9 0 U1 3 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 20 PY 2016 VL 28 IS 15 AR 155401 DI 10.1088/0953-8984/28/15/155401 PG 6 WC Physics, Condensed Matter SC Physics GA DI4FX UT WOS:000373456900008 PM 26987548 ER PT J AU Kapilashrami, M Wang, YJ Li, X Glans, PA Fang, M Riazanova, AV Belova, LM Rao, KV Luo, Y Barbiellini, B Lin, H Markiewicz, R Bansil, A Hussain, Z Guo, JH AF Kapilashrami, Mukes Wang, Yung Jui Li, Xin Glans, Per-Anders Fang, Mei Riazanova, Anastasia V. Belova, Lyubov M. Rao, K. V. Luo, Yi Barbiellini, Bernardo Lin, Hsin Markiewicz, Robert Bansil, Arun Hussain, Zahid Guo, Jinghua TI Understanding the magnetic interaction between intrinsic defects and impurity ions in room-temperature ferromagnetic Mg1-xFexO thin films SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE magnetic-tunneling junction; intrinsic defects; room-temperature ferromagnetism; d0 magnetism; x-ray spectroscopy; density functional theory ID X-RAY-ABSORPTION; ELECTRONIC-STRUCTURE; SEMICONDUCTORS; MGO; 1ST-PRINCIPLES; SPECTROSCOPY; OXIDES; HOLES; FE AB Understanding the nature and characteristics of the intrinsic defects and impurities in the dielectric barrier separating the ferromagnetic electrodes in a magnetic tunneling junction is of great importance for understanding the often observed 'barrier-breakdown' therein. In this connection, we present herein systematic experimental (SQUID and synchrotron-radiation-based x-ray absorption spectroscopy) and computational studies on the electronic and magnetic properties of Mg1-xFexO thin films. Our studies reveal: (i) defect aggregates comprised of basic and trimer units (Fe impurity coupled to 1 or 2 Mg vacancies) and (ii) existence of two competing magnetic orders, defect- and dopant-induced, with spin densities aligning anti-parallel if the trimer is present in the oxide matrix. These findings open up new avenues for designing tunneling barriers with high endurance and tunneling effect upon tuning the concentration/distribution of the two magnetic orders. C1 [Kapilashrami, Mukes; Wang, Yung Jui; Li, Xin; Glans, Per-Anders; Hussain, Zahid; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kapilashrami, Mukes] Univ Maryland, Dept Mech Engn, Ctr Engn Concepts Dev, College Pk, MD 20742 USA. [Wang, Yung Jui; Barbiellini, Bernardo; Markiewicz, Robert; Bansil, Arun] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Li, Xin; Luo, Yi] Royal Inst Technol, Sch Biotechnol, Div Theoret Chem & Biol, SE-10691 Stockholm, Sweden. [Fang, Mei; Riazanova, Anastasia V.; Belova, Lyubov M.; Rao, K. V.] Royal Inst Technol, Dept Mat Sci & Engn, SE-10044 Stockholm, Sweden. [Lin, Hsin] Natl Univ Singapore, Ctr Adv Mat 2D, Singapore 117546, Singapore. [Lin, Hsin] Natl Univ Singapore, Graphene Res Ctr, Singapore 117546, Singapore. [Lin, Hsin] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore. [Guo, Jinghua] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. RP Guo, JH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.; Guo, JH (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. EM jguo@lbl.gov RI Glans, Per-Anders/G-8674-2016; Lin, Hsin/F-9568-2012; Luo, Yi/B-1449-2009 OI Lin, Hsin/0000-0002-4688-2315; Luo, Yi/0000-0003-0007-0394 FU U.S. Department of Energy [DE-AC02-05CH11231, DE-FG02-07ER46352]; DOE [DE-SC0006931]; Swedish Research Council (VR); Axel Hultgren's Memorial Fund; Carl Trygger's foundation; Hero-M Center of Excellence; Swedish Agency VINNOVA; Chinese foundation CSC; Singapore National Research Foundation under NRF [NRF-NRFF2013-03] FX The ALS and NERSC are supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. MK acknowledges additional DOE funding support under Contract No. DE-SC0006931. The work at Northeastern University is supported by the US Department of Energy contract number DE-FG02-07ER46352, and benefited from Northeastern University's Advanced Scientific Computation Center (ASCC). M K acknowledges postdoctoral fellowships from the Swedish Research Council (VR) and Axel Hultgren's Memorial Fund. The authors would like to thank Wolfgang Voit for his help with establishing the ink-jet printing capability at KTH, and Roman Puzniak at the Institute of Physics (Warsaw, Poland) for his timely help with additional magnetic measurements of the thin film samples. The Work at KTH is supported by Carl Trygger's foundation, Hero-M Center of Excellence, and Swedish Agency VINNOVA. MF acknowledges the Chinese foundation CSC for a doctoral study scholarship. H L acknowledges the Singapore National Research Foundation for support under NRF Award No. NRF-NRFF2013-03. NR 43 TC 0 Z9 0 U1 5 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 20 PY 2016 VL 28 IS 15 AR 156002 DI 10.1088/0953-8984/28/15/156002 PG 7 WC Physics, Condensed Matter SC Physics GA DI4FX UT WOS:000373456900011 PM 26987741 ER PT J AU Nandipati, G Govind, N Andersen, A Rohatgi, A AF Nandipati, Giridhar Govind, Niranjan Andersen, Amity Rohatgi, Aashish TI Self-learning kinetic Monte Carlo simulations of Al diffusion in Mg SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE kinetic Monte Carlo; defect diffusion; point defects; vacancy diffusion ID MAGNESIUM; ALLOYS; INTERDIFFUSION; 1ST-PRINCIPLES; PRECIPITATION; IRRADIATION; ELEMENTS; SYSTEMS; PHASE; ZN AB Vacancy-mediated diffusion of an Al atom in the pure Mg matrix is studied using the atomistic, on-lattice self-learning kinetic Monte Carlo (SLKMC) method. Activation barriers for vacancy-Mg and vacancy-Al atom exchange processes are calculated on the fly using the climbing image nudged-elastic-band method and binary Mg-Al modified embedded-atom method interatomic potential. Diffusivities of an Al atom obtained from SLKMC simulations show the same behavior as observed in experimental and theoretical studies available in the literature; that is, an Al atom diffuses faster within the basal plane than along the c-axis. Although the effective activation barriers for an Al atom diffusion from SLKMC simulations are close to experimental and theoretical values, the effective prefactors are lower than those obtained from experiments. We present all the possible vacancy-Mg and vacancy-Al atom exchange processes and their activation barriers identified in SLKMC simulations. A simple mapping scheme to map an HCP lattice onto a simple cubic lattice is described, which enables simulation of the HCP lattice using the on-lattice framework. We also present the pattern recognition scheme which is used in SLKMC simulations to identify the local Al atom configuration around a vacancy. C1 [Nandipati, Giridhar; Govind, Niranjan; Andersen, Amity; Rohatgi, Aashish] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Nandipati, G; Rohatgi, A (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM giridhar.nandipati@pnnl.gov; aashish.rohatgi@pnnl.gov FU Vehicle Technologies Office of the US Department of Energy (US DOE), Office of Energy Efficiency and Renewable Energy; Office of Biological and Environmental Research; US DOE under DOE [DE-AC05-76RL1830] FX This work was sponsored by the Vehicle Technologies Office of the US Department of Energy (US DOE), Office of Energy Efficiency and Renewable Energy. A portion of this research was performed using computational resources at EMSL, a US DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research, located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle Memorial Institute for the US DOE under DOE contract number DE-AC05-76RL1830. The authors would like to acknowledge the use of OVITO [50] for visualization. NR 48 TC 1 Z9 1 U1 5 U2 23 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD APR 20 PY 2016 VL 28 IS 15 AR 155001 DI 10.1088/0953-8984/28/15/155001 PG 11 WC Physics, Condensed Matter SC Physics GA DI4FX UT WOS:000373456900005 PM 26982368 ER PT J AU Wierzbicki, M Niraula, N Yarrabothula, A Layton, DS Trinh, CT AF Wierzbicki, Michael Niraula, Narayan Yarrabothula, Akshitha Layton, Donovan S. Trinh, Cong T. TI Engineering an Escherichia coli platform to synthesize designer biodiesels SO JOURNAL OF BIOTECHNOLOGY LA English DT Article DE Fatty acid ethyl esters; Fatty acid isobutyl esters; Advanced biofuels; Designer biodiesels; Modular cell chassis; Biodiesel modules ID FATTY-ACID; SACCHAROMYCES-CEREVISIAE; BIOFUELS PRODUCTION; FUEL PROPERTIES; CHEMICALS; PATHWAYS; ESTERS; METHYLTRANSFERASE; ACYLTRANSFERASE; BIOSYNTHESIS AB Biodiesels, fatty acid esters (FAEs), can be synthesized by condensation of fatty acid acyl CoAs and alcohols via a wax ester synthase in living cells. Biodiesels have advantageous characteristics over petrodiesels such as biodegradability, a higher flash point, and less emission. Controlling fatty acid and alcohol moieties are critical to produce designer biodiesels with desirable physiochemical properties (e.g., high cetane number, low kinematic viscosity, high oxidative stability, and low cloud point). Here, we developed a flexible framework to engineer Escherichia coli cell factories to synthesize designer biodiesels directly from fermentable sugars. In this framework, we designed each FAE pathway as a biodiesel exchangeable production module consisting of acyl CoA, alcohol, and wax ester synthase submodules. By inserting the FAE modules in an engineered E. coli modular chassis cell, we generated E. coli cell factories to produce targeted biodiesels (e.g., fatty acid ethyl (FAEE) and isobutyl (FAIbE) esters) with tunable and controllable short-chain alcohol moieties. The engineered E. coli chassis carrying the FAIbE production module produced 54 mg/L FAIbEs with high specificity, accounting for >90% of the total synthesized FAEs and similar to 4.7 fold increase in FAIbE production compared to the wildtype. Fed -batch cultures further improved FAIbE production up to 165 mg/L. By mixing ethanol and isobutanol submodules, we demonstrated controllable production of mixed FAEEs and FAIbEs. We envision the developed framework offers a flexible, alternative route to engineer designer biodiesels with tunable and controllable properties using biomass-derived fermentable sugars. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wierzbicki, Michael; Niraula, Narayan; Yarrabothula, Akshitha; Layton, Donovan S.; Trinh, Cong T.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN USA. [Trinh, Cong T.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN USA. [Layton, Donovan S.; Trinh, Cong T.] Oak Ridge Natl Lab, Bioenergy Sci Ctr BESC, Oak Ridge, TN USA. RP Trinh, CT (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN USA. EM ctrinh@utk.edu RI Trinh, Cong/H-5300-2012 FU SEERC; University of Tennessee, Knoxville (UT); NSF CAREER (NSF) [1553250]; GAANN fellowship FX This research was supported in part by the laboratory start-up, SEERC, and JDRD seed funds from the University of Tennessee, Knoxville (UT) as well as the NSF CAREER award (NSF#1553250 to CTT). Donovan Layton is a recipient of GAANN fellowship. We would like to thank Dr. Gary Sayler, the director of Center of Environmental Biotechnology (CEB), UT for using the GC/MS instrument, and Dr. Fu Menn (CEB) for his assistance in developing the GC/MS method for this study. NR 44 TC 0 Z9 0 U1 4 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1656 EI 1873-4863 J9 J BIOTECHNOL JI J. Biotechnol. PD APR 20 PY 2016 VL 224 BP 27 EP 34 DI 10.1016/j.jbiotec.2016.03.001 PG 8 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DI0MT UT WOS:000373191300006 PM 26953744 ER PT J AU Butorin, SM Modin, A Vegelius, JR Suzuki, MT Oppeneer, PM Andersson, DA Shuh, DK AF Butorin, Sergei M. Modin, Anders Vegelius, Johan R. Suzuki, Michi-To Oppeneer, Peter M. Andersson, David A. Shuh, David K. TI Local Symmetry Effects in Actinide 4f X-ray Absorption in Oxides SO ANALYTICAL CHEMISTRY LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; HIGH-RESOLUTION; SCATTERING; REDUCTION; NEPTUNIUM; PHASE AB A systematic X-ray absorption study at actinide N-6,(7) (4f -> 6d transitions) edges was performed for light-actinide oxides including data obtained for the first time for NpO2, PuO2 and UO3. The measurements were supported by ab initio calculations based on local-density approximation. with added 5f-5f Coulomb interaction (LDA+U). Improved energy resolution compared to common experiments at actinide L-2,L-3 (2p -> 6d transitions) edges allowed us to resolve the major structures of the 13 unoccupied 6d density of states (DOS) and estimate the crystal-field 116) splittings in the 6d shell directly from the spectra of light-actinide dioxides. The measurements demonstrated an enhanced sensitivity of the N-6,N-7, spectral shape to changes in the compound crystal structure. For nonstoichiometric NpO2-x, the filling of the entire band gap with Np 6d states was observed thus supporting a phase coexistence of Np metal and stoichiometric NpO2 which is in agreement with the tentative Np-O phase diagram. C1 [Butorin, Sergei M.; Modin, Anders; Vegelius, Johan R.; Suzuki, Michi-To; Oppeneer, Peter M.] Uppsala Univ, Dept Phys & Astron, POB 516, SE-75120 Uppsala, Sweden. [Andersson, David A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Mat Sci Radiat & Dynam Extremes, Los Alamos, NM 87545 USA. [Shuh, David K.] Lawrence Berkeley Natl Lab, Div Chem Sci, MS 70A1150,One Cyclotron Rd, Berkeley, CA 94720 USA. [Suzuki, Michi-To] RIKEN Ctr Emergent Matter Sci, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. RP Butorin, SM (reprint author), Uppsala Univ, Dept Phys & Astron, POB 516, SE-75120 Uppsala, Sweden. EM sergei.butorin@physics.uu.se RI Suzuki, Michi-To/G-6298-2013 FU U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Swedish Research Council (VR); European Atomic Energy Community's FP7-work programme ("REDUPP") [269903]; Swedish National Infrastructure for Computing (SNIC) FX The work at the Advanced Light Source was supported by the Director, Office of Science, Office of Basic Energy Sciences, and this research (D.K.S.) was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences Heavy Element Chemistry Program, both of the U.S. Department of Energy at Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. P.M.O. acknowledges support from the Swedish Research Council (VR), the European Atomic Energy Community's FP7-work programme (Grant No. 269903, "REDUPP"), and the Swedish National Infrastructure for Computing (SNIC). NR 28 TC 2 Z9 2 U1 7 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD APR 19 PY 2016 VL 88 IS 8 BP 4169 EP 4173 DI 10.1021/acs.analchem.5b04380 PG 5 WC Chemistry, Analytical SC Chemistry GA DK1WP UT WOS:000374706000001 PM 27008406 ER PT J AU Mayer, BP DeHope, AJ Mew, DA Spackman, PE Williams, AM AF Mayer, Brian P. DeHope, Alan J. Mew, Daniel A. Spackman, Paul E. Williams, Audrey M. TI Chemical Attribution of Fentanyl Using Multivariate Statistical Analysis of Orthogonal Mass Spectral Data SO ANALYTICAL CHEMISTRY LA English DT Article ID SELECTIVITY RATIO PLOT; IMPURITIES; PROFILES AB Attribution of the origin of an illicit drug relies on identification of compounds indicative of its clandestine production and is a key component of many modern forensic investigations. The results of these studies can yield detailed information on method of manufacture, starting material source, and final product, all critical forensic evidence. In the present work, chemical attribution signatures (CAS) associated with the synthesis of the analgesic fentanyl, N-(1-phenylethylpiperidin-4-yl)-N-phenylpropanamide, were investigated. Six synthesis methods, all: previously published fentanyl synthetic routes or hybrid versions thereof, were studied in an effort to identify and classify route-specific signatures. A total of 160 distinct compounds and inorganic species were identified using gas and liquid chromatographies combined with mass spectrometric methods (gas chromatography/mass spectrometry (GC/MS) and liquid chromatography tandem mass spectrometry-time of (LC-MS/MS-TOF)) in conjunction with inductively coupled plasma mass spectrometry (ICPMS). The complexity of the resultant data matrix urged the use of multivariate statistical analysis. Using: partial least-squares-discriminant analysis (PLS-DA), 87 route specific CAS were classified and a statistical model capable of predicting the method of fentanyl synthesis was validated and tested against CAS profiles from crude fentanyl products deposited and later extracted from two operationally relevant surfaces: stainless steel and vinyl tile. This work provides the most detailed fentanyl CAS investigation to date by using orthogonal mass spectral data to identify CAS of forensic significance for illicit drug detection, profiling, and attribution. C1 [Mayer, Brian P.; Mew, Daniel A.; Spackman, Paul E.; Williams, Audrey M.] Lawrence Livermore Natl Lab, Forens Sci Ctr, 7000 East Ave L-091, Livermore, CA 94550 USA. [DeHope, Alan J.] Lawrence Livermore Natl Lab, Div Mat Sci, 7000 East Ave L-382, Livermore, CA 94550 USA. RP Williams, AM (reprint author), Lawrence Livermore Natl Lab, Forens Sci Ctr, 7000 East Ave L-091, Livermore, CA 94550 USA. EM Williams259@llnl.gov FU Department of Homeland Security, Science and Technology Directorate, Chemical Forensic Program; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344] FX The authors would like to thank the Department of Homeland Security, Science and Technology Directorate, Chemical Forensic Program for their funding of this work. Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. NR 22 TC 0 Z9 0 U1 15 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD APR 19 PY 2016 VL 88 IS 8 BP 4303 EP 4310 DI 10.1021/acs.analchem.5b04434 PG 8 WC Chemistry, Analytical SC Chemistry GA DK1WP UT WOS:000374706000021 PM 27010913 ER PT J AU Guo, XJ Fillmore, TL Gao, YQ Tang, KQ AF Guo, Xuejiang Fillmore, Thomas L. Gao, Yuqian Tang, Keqi TI Capillary Electrophoresis-Nanoelectrospray Ionization-Selected Reaction Monitoring Mass Spectrometry via a True Sheathless Metal-Coated Emitter Interface for Robust and High-Sensitivity Sample Quantification SO ANALYTICAL CHEMISTRY LA English DT Article ID FLOW NANOSPRAY INTERFACE; COMPLEX PROTEOME DIGESTS; ZONE-ELECTROPHORESIS; ELECTROSPRAY EMITTERS; CE-MS; ISOTACHOPHORESIS; PERFORMANCE; SEPARATION; PROTEINS; LINE AB A new sheathless transient capillary isotachophoresis (CITP)/capillary zone electrophoresis (CZE)-MS interface, based on a commercially available capillary with an integrated metal-coated ESI emitter, was developed in this study aiming at overcoming the reproducibility and ruggedness problems suffered to a certain degree by almost all the available CE-MS interfaces, and pushing the CE-MS technology suitable for routine sample analysis with high sensitivity. The new CITP/CZE-MS interface allows the electric contact between ESI voltage power supply and the CE separation liquid by using a conductive liquid that comes in contact with the metal-coated surface of the ESI emitter, making it a true sheathless CE-MS interface. Stable electrospray was established by avoiding the formation of gas bubbles from electrochemical reaction inside the CE capillary. Crucial operating parameters, such as sample loading volume, flow rate, and separation voltage, were systematically evaluated for their effects on both CITP/CZE separation efficiency and MS detection sensitivity. Around one hundred CITP/CZE-MS analyses can be easily achieved by using the new sheathless CITP/CZE interface without a noticeable loss of metal coating on the ESI emitter surface, or degrading of the ESI emitter performance. The reproducibility in analyte migration time and quantitative performance of the new interface was experimentally evaluated to demonstrate a LOQ below 5 attomole. C1 [Guo, Xuejiang] Nanjing Med Univ, Dept Histol & Embryol, State Key Lab Reprod Med, Nanjing 210029, Jiangsu, Peoples R China. [Fillmore, Thomas L.; Gao, Yuqian; Tang, Keqi] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Tang, KQ (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. EM keqi.tang@pnnl.gov FU National Institutes of Health: National Cancer Institute [R33 CA155252, R21 CA199744]; National Institute of General Medical Sciences [P41 GM103493]; DOE [DE-AC05-76RL01830] FX This work was partially supported by grants from the National Institutes of Health: National Cancer Institute (R33 CA155252 and R21 CA199744) and National Institute of General Medical Sciences (P41 GM103493). All the experiments were performed in the Environmental Molecular Sciences Laboratory, a U.S. DOE national scientific user facility located at the Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is a multiprogram national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RL01830. NR 31 TC 4 Z9 4 U1 15 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD APR 19 PY 2016 VL 88 IS 8 BP 4418 EP 4425 DI 10.1021/acs.analchem.5b04912 PG 8 WC Chemistry, Analytical SC Chemistry GA DK1WP UT WOS:000374706000035 PM 27028594 ER PT J AU Kaplan, DI Xu, C Huang, S Lin, YM Tolic, N Roscioli-Johnson, KM Santschi, PH Jaffe, PR AF Kaplan, Daniel I. Xu, Chen Huang, Shan Lin, Youmin Tolic, Nikola Roscioli-Johnson, Kristyn M. Santschi, Peter H. Jaffe, Peter R. TI Unique Organic Matter and Microbial Properties in the Rhizosphere of a Wetland Soil SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID HYPERACCUMULATOR SEDUM-ALFREDII; RESONANCE MASS-SPECTROMETRY; FRESH-WATER WETLANDS; SAVANNA RIVER SITE; BLACK CARBON; RICE ROOTS; IRON; MOBILITY; SEDIMENTS; ION AB Wetlands attenuate the migration of many contaminants through a wide range of biogeochemical reactions. Recent research has shown that the rhizosphere, the zone near plant roots, in wetlands is especially effective at promoting contaminant attenuation. The objective of this study was to compare the soil organic matter (OM) composition and microbial communities of a rhizosphere soil (primarily an oxidized environment) to that of the bulk wetland soil (primarily a reduced environment). The rhizosphere had elevated C, N, Mn, and Fe concentrations and total bacteria, including Anaeromyxobacter, counts (as identified by qPCR). Furthermore, the rhizosphere contained several organic molecules that were not identified in the nonrhizosphere soil (54% of the >2200 ESI-FTICR-MS identified compounds). The rhizosphere OM molecules generally had (1) greater overall molecular weights, (2) less aromaticity, (3) more carboxylate and N-containing COO functional groups, and (4) a greater hydrophilic character. These latter two OM properties typically promote metal binding. This study showed for the first time that not only the amount but also the molecular characteristics of OM in the rhizosphere may in part be responsible for the enhanced immobilization of contaminants in wetlands. These finding have implications on the stewardship and long-term management of contaminated wetlands. C1 [Kaplan, Daniel I.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Xu, Chen; Lin, Youmin; Santschi, Peter H.] Texas A&M Univ, Galveston, TX 77553 USA. [Huang, Shan; Jaffe, Peter R.] Princeton Univ, Princeton, NJ 08540 USA. [Tolic, Nikola] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Roscioli-Johnson, Kristyn M.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Kaplan, DI (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA. EM daniel.kaplan@srnl.doe.gov FU Subsurface Biogeochemistry Research Program within the Climate and Environmental Sciences Division in the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE) [DR-FG02-08ER64567, ER65222-1038426-0017532]; DOE's Office of Biological and Environmental Research program FX This work was supported by the Subsurface Biogeochemistry Research Program within the Climate and Environmental Sciences Division in the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE), Grants DR-FG02-08ER64567 and ER65222-1038426-0017532. The ESI-FTICR-MS analyses were conducted at EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research program. EMSL is located at the PNNL in Richland, WA, USA. NR 71 TC 1 Z9 1 U1 25 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD APR 19 PY 2016 VL 50 IS 8 BP 4169 EP 4177 DI 10.1021/acs.est.5b05165 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DK1WZ UT WOS:000374707100004 PM 27091553 ER PT J AU Lu, X Liu, YR Johs, A Zhao, LD Wang, TS Yang, ZM Lin, H Elias, DA Pierce, EM Liang, LY Barkay, T Gu, BH AF Lu, Xia Liu, Yurong Johs, Alexander Zhao, Linduo Wang, Tieshan Yang, Ziming Lin, Hui Elias, Dwayne A. Pierce, Eric M. Liang, Liyuan Barkay, Tamar Gu, Baohua TI Anaerobic Mercury Methylation and Demethylation by Geobacter bemidjiensis Bem SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID DISSOLVED ELEMENTAL MERCURY; IRON-REDUCING BACTERIA; METHYLMERCURY PRODUCTION; SULFURREDUCENS PCA; ORGANIC-MATTER; RESISTANCE; DEGRADATION; ENVIRONMENTS; ECOSYSTEMS; EXPRESSION AB Microbial methylation and demethylation are two competing processes controlling the net production and bioaccumulation of neurotoxic methylmercury (MeHg) in natural ecosystems. Although mercury (Hg) methylation by anaerobic microorganisms and demethylation by aerobic Hg-resistant bacteria have both been extensively studied, little attention has been given to MeHg degradation by anaerobic bacteria, particularly the iron-reducing bacterium Geobacter bemidjiensis Bern. Here we report, for the first time, that the strain G. bemidjiensis Bern can mediate a suite of Hg transformations, including Hg(II) reduction, Hg(0) oxidation, MeHg production and degradation under anoxic conditions. Results suggest that G. bemidjiensis utilizes a reductive demethylation pathway to degrade MeHg, with elemental Hg(0) as the major reaction product, possibly due to the presence of genes encoding homologues of an organomercurial lyase (MerB) and a mercuric reductase (MerA). In addition, the cells can strongly sorb Hg(II) and MeHg, reduce or oxidize Hg, resulting in both time and concentration-dependent Hg species transformations. Moderate concentrations (10-500 mu M) of Hg-binding ligands such as cysteine enhance Hg(II) methylation but inhibit MeHg degradation. These findings indicate a cycle of Hg methylation and demethylation among anaerobic bacteria, thereby influencing net MeHg production in anoxic water and sediments. C1 [Lu, Xia; Wang, Tieshan] Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Peoples R China. [Lu, Xia; Liu, Yurong; Johs, Alexander; Zhao, Linduo; Yang, Ziming; Lin, Hui; Pierce, Eric M.; Liang, Liyuan; Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Liu, Yurong] Chinese Acad Sci, State Key Lab Urban & Reg Ecol, Res Ctr Ecoenvironm Sci, Beijing, Peoples R China. [Elias, Dwayne A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Liang, Liyuan] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Barkay, Tamar] Rutgers State Univ, Dept Biochem & Microbiol, New Brunswick, NJ 08901 USA. RP Lu, X (reprint author), Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Peoples R China.; Lu, X; Gu, BH (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. EM lux2@ornl.gov; gubl@ornl.gov RI Pierce, Eric/G-1615-2011 OI Pierce, Eric/0000-0002-4951-1931 FU Office of Biological and Environmental Research, DOE Office of Science, as part of the Mercury Science Focus Area at Oak Ridge National Laboratory (ORNL); Chinese Scholarship Council (CSC) of China; Laboratory Directed RD fund at ORNL FX We thank Xiangping Yin for assistance in mercury and methylmercury analyses. This research was sponsored by the Office of Biological and Environmental Research, DOE Office of Science, as part of the Mercury Science Focus Area at Oak Ridge National Laboratory (ORNL). XL and YL were supported in part by the Chinese Scholarship Council (CSC) of China, and LL by the Laboratory Directed R&D fund at ORNL, which is managed by UT-Battelle LLC. NR 44 TC 6 Z9 7 U1 24 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD APR 19 PY 2016 VL 50 IS 8 BP 4366 EP 4373 DI 10.1021/acs.est.6b00401 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DK1WZ UT WOS:000374707100026 PM 27019098 ER PT J AU Ciemny, AA Dominik, W Ginter, T Grzywacz, R Janas, Z Kuich, M Mazzocchi, C Miernik, K Pfutzner, M Pomorski, M Bazin, D Baumann, T Bezbakh, A Crider, BP Cwiok, M Go, S Kaminski, G Kolos, K Korgul, A Kwan, E Liddick, SN Paulauskas, SV Pereira, J Rykaczewski, KP Sumithrarachchi, C Xiao, Y AF Ciemny, A. A. Dominik, W. Ginter, T. Grzywacz, R. Janas, Z. Kuich, M. Mazzocchi, C. Miernik, K. Pfuetzner, M. Pomorski, M. Bazin, D. Baumann, T. Bezbakh, A. Crider, B. P. Cwiok, M. Go, S. Kaminski, G. Kolos, K. Korgul, A. Kwan, E. Liddick, S. N. Paulauskas, S. V. Pereira, J. Rykaczewski, K. P. Sumithrarachchi, C. Xiao, Y. TI First measurement of Ge-60 beta-decay SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article AB The N = 28 isotone Ge-60, T-z = -2, was produced and selected among the products of the fragmentation reaction of a Kr-78 beam at 150MeV/nucleon and a Be target by means of the A1900 fragment separator at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). Its decay was studied for the first time using the optical time projection chamber. The beta-decay of Ge-60 was found to be dominated by beta-delayed proton emission, with a branching of approximate to 100% and half-life T-1/2 = 20(-5)(+7) ms. C1 [Ciemny, A. A.; Dominik, W.; Janas, Z.; Kuich, M.; Mazzocchi, C.; Miernik, K.; Pfuetzner, M.; Pomorski, M.; Cwiok, M.; Korgul, A.] Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. [Ginter, T.; Bazin, D.; Baumann, T.; Crider, B. P.; Kwan, E.; Liddick, S. N.; Paulauskas, S. V.; Pereira, J.; Sumithrarachchi, C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Grzywacz, R.; Go, S.; Kolos, K.; Paulauskas, S. V.; Xiao, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Grzywacz, R.; Rykaczewski, K. P.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Bezbakh, A.; Kaminski, G.] Joint Inst Nucl Res, Dubna 141980, Russia. [Kaminski, G.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Liddick, S. N.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. RP Ciemny, AA (reprint author), Univ Warsaw, Fac Phys, PL-02093 Warsaw, Poland. EM aleksandra.ciemny@fuw.edu.pl FU National Science Center, Poland [UMO-2015/17/B/ST2/00581]; US Department of Energy, Office of Science, Office of Nuclear Physics, under US DOE [DE-AC05-00OR22725, DE-FG02-96ER40983]; National Nuclear Security Administration, under the Stewardship Science Academic Alliance program through DOE [DEFC03-03NA00143, DE-FG52-08NA28552]; US National Science Foundation [PHY-11-02511]; Polish Ministry of Science and Higher Education [0079/DIA/2014/43] FX We wish to acknowledge the National Superconducting Cyclotron Laboratory staff for assisting with the experiments and providing excellent quality radioactive beams. This work was supported by the National Science Center, Poland, under Contract No. UMO-2015/17/B/ST2/00581, by the US Department of Energy, Office of Science, Office of Nuclear Physics, under US DOE Grant Nos. DE-AC05-00OR22725 (ORNL) and DE-FG02-96ER40983 (UTK), by the fund source National Nuclear Security Administration Grant No. DEFC03-03NA00143, under the Stewardship Science Academic Alliance program through DOE Cooperative Agreement No. DE-FG52-08NA28552 (UTK) and by the US National Science Foundation Grant No. PHY-11-02511 (NSCL). AAC acknowledges support by the Polish Ministry of Science and Higher Education through Grant No. 0079/DIA/2014/43 ("Grant Diamentowy"). NR 17 TC 0 Z9 0 U1 5 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD APR 19 PY 2016 VL 52 IS 4 AR 89 DI 10.1140/epja/i2016-16089-x PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DJ8CW UT WOS:000374441100002 ER PT J AU Cao, HB Banerjee, A Yan, JQ Bridges, CA Lumsden, MD Mandrus, DG Tennant, DA Chakoumakos, BC Nagler, SE AF Cao, H. B. Banerjee, A. Yan, J. -Q. Bridges, C. A. Lumsden, M. D. Mandrus, D. G. Tennant, D. A. Chakoumakos, B. C. Nagler, S. E. TI Low-temperature crystal and magnetic structure of alpha-RuCl3 SO PHYSICAL REVIEW B LA English DT Article ID BETA-RUTHENIUM TRICHLORIDE; SPIN-LIQUID; EXCITATIONS; ANYONS; ALPHA AB Single crystals of the Kitaev spin-liquid candidate alpha-RuCl3 have been studied to determine the low-temperature bulk properties, the structure, and the magnetic ground state. Refinements of x-ray diffraction data show that the low-temperature crystal structure is described by space group C2/m with a nearly perfect honeycomb lattice exhibiting less than 0.2% in-plane distortion. The as-grown single crystals exhibit only one sharp magnetic transition at T-N = 7K. The magnetic order belowthis temperature exhibits a propagation vector of k = (0,1,1/3), which coincides with a three-layer stacking of the C2/m unit cells. Magnetic transitions at higher temperatures up to 14 K can be introduced by deformations of the crystal that result in regions in the crystal with a two-layer stacking sequence. The best-fit symmetry-allowed magnetic structure of the as-grown crystals shows that the spins lie in the ac plane, with a zigzag configuration in each honeycomb layer. The three-layer repeat out-of-plane structure can be refined as a 120 degrees spiral order or a collinear structure with a spin direction of 35 degrees away from the a axis. The collinear spin configuration yields a slightly better fit and also is physically preferred. The average ordered moment in either structure is less than 0.45(5) mu(B) per Ru3+ ion. C1 [Cao, H. B.; Banerjee, A.; Lumsden, M. D.; Chakoumakos, B. C.; Nagler, S. E.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Yan, J. -Q.; Mandrus, D. G.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Yan, J. -Q.; Mandrus, D. G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Bridges, C. A.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Tennant, D. A.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Nagler, S. E.] Univ Tennessee, Bredesen Ctr, Knoxville, TN 37996 USA. RP Cao, HB; Banerjee, A (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM caoh@ornl.gov; banerjeea@ornl.gov RI Tennant, David/Q-2497-2015; Nagler, Stephen/E-4908-2010; Lumsden, Mark/F-5366-2012 OI Tennant, David/0000-0002-9575-3368; Nagler, Stephen/0000-0002-7234-2339; Lumsden, Mark/0000-0002-5472-9660 FU Scientific User Facilities Division, Office of Science, Basic Energy Sciences, U.S. Department of Energy; U. S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Gordon and Betty Moore Foundations EPiQS Initiative [GBMF4416] FX We thank Feng Ye, Adam Aczel, and Johannes Knolle for discussions during various stages of this research, and Songxue Chi for helping with the experiment setup at HB-3A. We have benefited from discussions with Hae-Young Kee, Giniyat Khaliullin, and George Jackeli. The work at ORNL HFIR was sponsored by the Scientific User Facilities Division, Office of Science, Basic Energy Sciences, U.S. Department of Energy. J.-Q.Y. and C.A.B. were supported by the U. S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. D.G.M. was supported by the Gordon and Betty Moore Foundations EPiQS Initiative through Grant GBMF4416. NR 45 TC 14 Z9 14 U1 28 U2 55 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 19 PY 2016 VL 93 IS 13 AR 134423 DI 10.1103/PhysRevB.93.134423 PG 8 WC Physics, Condensed Matter SC Physics GA DJ9JB UT WOS:000374528700004 ER PT J AU Hogan, T Bjaalie, L Zhao, LY Belvin, C Wang, XP Van de Walle, CG Hsieh, D Wilson, SD AF Hogan, Tom Bjaalie, Lars Zhao, Liuyan Belvin, Carina Wang, Xiaoping Van de Walle, Chris G. Hsieh, David Wilson, Stephen D. TI Structural investigation of the bilayer iridate Sr3Ir2O7 SO PHYSICAL REVIEW B LA English DT Article ID BILBAO CRYSTALLOGRAPHIC SERVER; AUGMENTED-WAVE METHOD; NEUTRON-DIFFRACTION; CRYSTAL-STRUCTURE; SPACE AB A complete structural solution of the bilayer iridate compound Sr3Ir2O7 presently remains outstanding. Previously reported structures for this compound vary and all fail to explain weak structural violations observed in neutron scattering measurements as well as the presence of a net ferromagnetic moment in the basal plane. In this paper, we present single crystal neutron diffraction and rotational anisotropy second harmonic generation measurements unveiling a lower, monoclinic symmetry inherent to Sr3Ir2O7. Combined with density functional theory, our measurements identify the correct structural space group as No. 15 (C2/c) and provide clarity regarding the local symmetry of Ir4+ cations within this spin-orbit Mott material. C1 [Hogan, Tom] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Hogan, Tom; Bjaalie, Lars; Van de Walle, Chris G.; Wilson, Stephen D.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Zhao, Liuyan; Hsieh, David] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Zhao, Liuyan; Hsieh, David] CALTECH, Inst Quantum Informat & Matter, Pasadena, CA 91125 USA. [Belvin, Carina] Wellesley Coll, Wellesley, MA 02481 USA. [Wang, Xiaoping] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Wilson, SD (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM stephendwilson@engineering.ucsb.edu RI Wang, Xiaoping/E-8050-2012 OI Wang, Xiaoping/0000-0001-7143-8112 FU NSF [DMR-1505549]; MRSEC Program of the National Science Foundation [DMR 1121053]; ARO [W911NF-13-1-0059]; ARO DURIP Award [W911NF-13-1-0293]; Institute for Quantum Information and Matter, an NSF Physics Frontiers Center [PHY-1125565]; Gordon and Betty Moore Foundation [GBMF1250]; Caltech WAVE Fellows program; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy [DE-AC05-00OR22725] FX This work was supported in part by NSF Award No. DMR-1505549 (S.D.W.), as well as by the MRSEC Program of the National Science Foundation under Award No. DMR 1121053 (T.H., L.B., C.VdW.). Work at Caltech (L.Z., D.H.) was supported by ARO Grant No. W911NF-13-1-0059. Instrumentation for the SHG measurements was partially supported by ARO DURIP Award W911NF-13-1-0293 and by the Institute for Quantum Information and Matter, an NSF Physics Frontiers Center (PHY-1125565) with support of the Gordon and Betty Moore Foundation through Grant GBMF1250. C.B. acknowledges support from the Caltech WAVE Fellows program. Work performed at the ORNL Spallation Neutron Source TOPAZ single-crystal diffractometer was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. NR 44 TC 4 Z9 4 U1 8 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 19 PY 2016 VL 93 IS 13 AR 134110 DI 10.1103/PhysRevB.93.134110 PG 6 WC Physics, Condensed Matter SC Physics GA DJ9JB UT WOS:000374528700001 ER PT J AU Wang, HC Li, CK Liu, HW Yan, JQ Wang, JF Liu, J Lin, ZQ Li, YN Wang, Y Li, L Mandrus, D Xie, XC Feng, J Wang, J AF Wang, Huichao Li, Chao-Kai Liu, Haiwen Yan, Jiaqiang Wang, Junfeng Liu, Jun Lin, Ziquan Li, Yanan Wang, Yong Li, Liang Mandrus, David Xie, X. C. Feng, Ji Wang, Jian TI Chiral anomaly and ultrahigh mobility in crystalline HfTe5 SO PHYSICAL REVIEW B LA English DT Article ID DIRAC SEMIMETAL CD3AS2; NEGATIVE MAGNETORESISTANCE; ZRTE5 AB HfTe5 is predicted to be a promising platform for studying topological phases. Here through an electrical transport study, we present an observation of chiral anomaly and ultrahigh mobility in HfTe5 crystals. Negative magnetoresistivity in HfTe5 is observed when the external magnetic and electrical fields are parallel (B//E) and quickly disappears once B deviates from the direction of E. Quantitative fitting further confirms the chiral anomaly as the underlying physics. Moreover, by analyzing the conductivity tensors of longitudinal and Hall traces, ultrahigh mobility and ultralow carrier density are revealed in HfTe5, which paves the way for potential electronic applications. C1 [Wang, Huichao; Li, Chao-Kai; Liu, Haiwen; Li, Yanan; Xie, X. C.; Feng, Ji; Wang, Jian] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Wang, Huichao; Li, Chao-Kai; Liu, Haiwen; Li, Yanan; Xie, X. C.; Feng, Ji; Wang, Jian] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Liu, Haiwen] Beijing Normal Univ, Dept Phys, Ctr Adv Quantum Studies, Beijing 100875, Peoples R China. [Yan, Jiaqiang; Mandrus, David] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yan, Jiaqiang; Mandrus, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Wang, Junfeng; Lin, Ziquan; Li, Liang] Huazhong Univ Sci & Technol, Wuhan Natl High Magnet Field Ctr, Wuhan 430074, Peoples R China. [Liu, Jun; Wang, Yong] Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Ctr Electron Microscopy, Hangzhou 310027, Peoples R China. RP Wang, J (reprint author), Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China.; Wang, J (reprint author), Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. EM jianwangphysics@pku.edu.cn RI Feng, Ji/B-6775-2009 OI Feng, Ji/0000-0003-1944-718X FU National Basic Research Program of China [2013CB934600, 2012CB921300, 2013CB921900]; Open Project Program of the Pulsed High Magnetic Field Facility, Huazhong University of Science and Technology [PHMFF2015002]; NSF [DMR 1410428] FX We acknowledge Yongjie Liu for the help in the pulsed magnetic field measurements and we thank Honglie Ning for valuable discussions. This work was financially supported by the National Basic Research Program of China (Grants No. 2013CB934600, No. 2012CB921300, and No. 2013CB921900), and the Open Project Program of the Pulsed High Magnetic Field Facility (Grant No. PHMFF2015002), Huazhong University of Science and Technology. D.G.M and J.-Q.Y acknowledge support from NSF DMR 1410428. NR 39 TC 0 Z9 0 U1 27 U2 52 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 19 PY 2016 VL 93 IS 16 AR 165127 DI 10.1103/PhysRevB.93.165127 PG 7 WC Physics, Condensed Matter SC Physics GA DJ9MI UT WOS:000374537200004 ER PT J AU Lattuada, D Barbarino, M Bonasera, A Bang, W Quevedo, HJ Warren, M Consoli, F De Angelis, R Andreoli, P Kimura, S Dyer, G Bernstein, AC Hagel, K Barbui, M Schmidt, K Gaul, E Donovan, ME Natowitz, JB Ditmire, T AF Lattuada, D. Barbarino, M. Bonasera, A. Bang, W. Quevedo, H. J. Warren, M. Consoli, F. De Angelis, R. Andreoli, P. Kimura, S. Dyer, G. Bernstein, A. C. Hagel, K. Barbui, M. Schmidt, K. Gaul, E. Donovan, M. E. Natowitz, J. B. Ditmire, T. TI Model-independent determination of the astrophysical S factor in laser-induced fusion plasmas SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-FUSION; DEUTERIUM CLUSTERS; CROSS-SECTIONS; ELECTRON; EXPLOSIONS; ENERGIES; DYNAMICS; DRIVEN; D+D AB In this work, we present a new and general method for measuring the astrophysical S factor of nuclear reactions in laser-induced plasmas and we apply it to H-2(d, n)He-3. The experiment was performed with the Texas Petawatt Laser, which delivered 150-270 fs pulses of energy ranging from 90 to 180 J to D-2 or CD4 molecular clusters (where D denotes H-2). After removing the background noise, we used the measured time-of-flight data of energetic deuterium ions to obtain their energy distribution. We derive the S factor using the measured energy distribution of the ions, the measured volume of the fusion plasma, and the measured fusion yields. This method is model independent in the sense that no assumption on the state of the system is required, but it requires an accurate measurement of the ion energy distribution, especially at high energies, and of the relevant fusion yields. In the H-2(d, n) He-3 and He-3(d, p)He-4 cases discussed here, it is very important to apply the background subtraction for the energetic ions and to measure the fusion yields with high precision. While the available data on both ion distribution and fusion yields allow us to determine with good precision the S factor in the d + d case (lower Gamow energies), for the d + He-3 case the data are not precise enough to obtain the S factor using this method. Our results agree with other experiments within the experimental error, even though smaller values of the S factor were obtained. This might be due to the plasma environment differing from the beam target conditions in a conventional accelerator experiment. C1 [Lattuada, D.; Barbarino, M.; Bonasera, A.; Warren, M.; Hagel, K.; Barbui, M.; Schmidt, K.; Natowitz, J. B.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Lattuada, D.] Univ Enna Kore, I-94100 Enna, Italy. [Lattuada, D.; Bonasera, A.] LNS INFN, Via S Sofia 62, I-95123 Catania, Italy. [Bang, W.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Quevedo, H. J.; Dyer, G.; Bernstein, A. C.; Gaul, E.; Donovan, M. E.; Ditmire, T.] Univ Texas Austin, Ctr High Energy Dens Sci, C1510, Austin, TX 78712 USA. [Warren, M.] Univ Dallas, Irving, TX 75062 USA. [Consoli, F.; De Angelis, R.; Andreoli, P.] Assoc Euratom ENEA Fus, Via Enrico Fermi 45,CP 65, I-00044 Rome, Italy. [Kimura, S.] Univ Milan, Dept Phys, Via Celoria 16, I-20133 Milan, Italy. [Schmidt, K.] Silesian Univ, Inst Phys, Uniwersytecka 4, PL-40007 Katowice, Poland. RP Lattuada, D (reprint author), Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA.; Lattuada, D (reprint author), Univ Enna Kore, I-94100 Enna, Italy.; Lattuada, D (reprint author), LNS INFN, Via S Sofia 62, I-95123 Catania, Italy. EM lattuadad@lns.infn.it RI Bang, Woosuk/E-8135-2015; OI Bang, Woosuk/0000-0002-4259-1342; KIMURA, Sachie/0000-0001-6246-6971 FU NNSA [DE-FC52-08NA28512]; DOE Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-FG03-93ER40773]; Robert A. Welch Foundation [A0330]; Los Alamos National Laboratory LDRD program; National Science Foundation Graduate Research Fellowship [1263281]; Cyclotron Institute FX The experimental work was done at the University of Texas at Austin and was supported by NNSA Cooperative Agreement No. DE-FC52-08NA28512 and the DOE Office of Basic Energy Sciences. The analysis of the data was performed at the Texas A&M University and was supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Grant No. DE-FG03-93ER40773 and by the Robert A. Welch Foundation under Grant No. A0330. W.B. was supported by the Los Alamos National Laboratory LDRD program and M.W. was supported by the National Science Foundation Graduate Research Fellowship under Grant No. 1263281. D.L. thanks the Cyclotron Institute for hospitality and financial support. NR 36 TC 1 Z9 1 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 19 PY 2016 VL 93 IS 4 AR 045808 DI 10.1103/PhysRevC.93.045808 PG 8 WC Physics, Nuclear SC Physics GA DJ9PF UT WOS:000374544700004 ER PT J AU Mousseau, J Wospakrik, M Aliaga, L Altinok, O Bellantoni, L Bercellie, A Betancourt, M Bodek, A Bravar, A Budd, H Cai, T Carneiro, MF Christy, ME Chvojka, J da Motta, H Devan, J Dytman, SA Diaz, GA Eberly, B Felix, J Fields, L Fine, R Gago, AM Galindo, R Gallagher, H Ghosh, A Golan, T Gran, R Harris, DA Higuera, A Hurtado, K Kiveni, M Kleykamp, J Kordosky, M Le, T Maher, E Manly, S Mann, WA Marshall, CM Caicedo, DAM McFarland, KS McGivern, CL McGowan, AM Messerly, B Miller, J Mislivec, A Morfin, JG Naples, D Nelson, JK Norrick, A Nuruzzaman Osta, J Paolone, V Park, J Patrick, CE Perdue, GN Rakotondravohitra, L Ramirez, MA Ransome, RD Ray, H Ren, L Rimal, D Rodrigues, PA Ruterbories, D Schellman, H Schmitz, DW Salinas, CJS Tagg, N Tice, BG Valencia, E Walton, T Wolcott, J Zavala, G Zhang, D AF Mousseau, J. Wospakrik, M. Aliaga, L. Altinok, O. Bellantoni, L. Bercellie, A. Betancourt, M. Bodek, A. Bravar, A. Budd, H. Cai, T. Carneiro, M. F. Christy, M. E. Chvojka, J. da Motta, H. Devan, J. Dytman, S. A. Diaz, G. A. Eberly, B. Felix, J. Fields, L. Fine, R. Gago, A. M. Galindo, R. Gallagher, H. Ghosh, A. Golan, T. Gran, R. Harris, D. A. Higuera, A. Hurtado, K. Kiveni, M. Kleykamp, J. Kordosky, M. Le, T. Maher, E. Manly, S. Mann, W. A. Marshall, C. M. Caicedo, D. A. Martinez McFarland, K. S. McGivern, C. L. McGowan, A. M. Messerly, B. Miller, J. Mislivec, A. Morfin, J. G. Naples, D. Nelson, J. K. Norrick, A. Nuruzzaman Osta, J. Paolone, V. Park, J. Patrick, C. E. Perdue, G. N. Rakotondravohitra, L. Ramirez, M. A. Ransome, R. D. Ray, H. Ren, L. Rimal, D. Rodrigues, P. A. Ruterbories, D. Schellman, H. Schmitz, D. W. Salinas, C. J. Solano Tagg, N. Tice, B. G. Valencia, E. Walton, T. Wolcott, J. Zavala, G. Zhang, D. CA MINERvA Collaboration TI Measurement of partonic nuclear effects in deep-inelastic neutrino scattering using MINERvA SO PHYSICAL REVIEW D LA English DT Article ID DEUTERON STRUCTURE FUNCTIONS; PROTON STRUCTURE-FUNCTION; CROSS-SECTIONS; ELECTRON-SCATTERING; MUON SCATTERING; GLOBAL ANALYSIS; HYDROGEN; F2; MOMENTUM; TARGETS AB The MINERvA Collaboration reports a novel study of neutrino-nucleus charged-current deep inelastic scattering (DIS) using the same neutrino beam incident on targets of polystyrene, graphite, iron, and lead. Results are presented as ratios of C, Fe, and Pb to CH. The ratios of total DIS cross sections as a function of neutrino energy and flux-integrated differential cross sections as a function of the Bjorken scaling variable x are presented in the neutrino- energy range of 5-50 GeV. Based on the predictions of charged-lepton scattering ratios, good agreement is found between the data and prediction at medium x and low neutrino energy. However, the ratios appear to be below predictions in the vicinity of the nuclear shadowing region, x < 0.1. This apparent deficit, reflected in the DIS cross-section ratio at high E., is consistent with previous MINERvA observations [B. Tice et al. (MINERvA Collaboration), Phys. Rev. Lett. 112, 231801 (2014).] and with the predicted onset of nuclear shadowing with the axial-vector current in neutrino scattering. C1 [Mousseau, J.; Wospakrik, M.; Ray, H.; Rimal, D.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Aliaga, L.; Devan, J.; Kordosky, M.; Nelson, J. K.; Norrick, A.; Zhang, D.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Altinok, O.; Gallagher, H.; Le, T.; Mann, W. A.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Bellantoni, L.; Betancourt, M.; Fields, L.; Golan, T.; Harris, D. A.; Kiveni, M.; Caicedo, D. A. Martinez; McFarland, K. S.; Morfin, J. G.; Osta, J.; Perdue, G. N.; Rakotondravohitra, L.; Schmitz, D. W.; Walton, T.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Bercellie, A.; Bodek, A.; Budd, H.; Cai, T.; Chvojka, J.; Diaz, G. A.; Fine, R.; Golan, T.; Higuera, A.; Kleykamp, J.; Manly, S.; Marshall, C. M.; McFarland, K. S.; McGowan, A. M.; Mislivec, A.; Park, J.; Perdue, G. N.; Rodrigues, P. A.; Ruterbories, D.; Wolcott, J.] Univ Rochester, 601 Elmwood Ave, Rochester, NY 14627 USA. [Bravar, A.] Univ Geneva, CH-1211 Geneva 4, Switzerland. [Carneiro, M. F.; da Motta, H.; Ghosh, A.; Hurtado, K.] Ctr Brasileiro Pesquisas Fis, Rua Dr Xavier Sigaud 150, BR-22290180 Rio De Janeiro, RJ, Brazil. [Christy, M. E.; Walton, T.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Dytman, S. A.; Eberly, B.; McGivern, C. L.; Messerly, B.; Naples, D.; Paolone, V.; Ren, L.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Diaz, G. A.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Apartado 1761, Lima, Peru. [Felix, J.; Higuera, A.; Ramirez, M. A.; Valencia, E.; Zavala, G.] Univ Guanajuato, Colonia Ctr, Campus Leon & Campus Guanajuato, Guanajuato 36000, Guanajuato, Mexico. [Fields, L.; Patrick, C. E.; Schellman, H.] Northwestern Univ, Evanston, IL 60208 USA. [Galindo, R.; Miller, J.; Nuruzzaman] Univ Tecn Federico Santa Maria, Dept Fis, Ave Espana 1680,Casilla 110-5, Valparaiso, Chile. [Gran, R.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Hurtado, K.; Salinas, C. J. Solano] Univ Nacl Ingn, Apartado 31139, Lima, Peru. [Le, T.; Nuruzzaman; Ransome, R. D.; Tice, B. G.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Maher, E.] Massachusetts Coll Liberal Arts, 375 Church St, North Adams, MA 01247 USA. [Schellman, H.] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. [Schmitz, D. W.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Tagg, N.] Otterbein Univ, Dept Phys, 1 South Grove St, Westerville, OH 43081 USA. [Mousseau, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Eberly, B.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Higuera, A.] Univ Houston, Houston, TX 77204 USA. [Caicedo, D. A. Martinez] IIT, Chicago, IL 60616 USA. [Rakotondravohitra, L.] Univ Antananarivo, Dept Phys, Antananarivo, Madagascar. [Wolcott, J.] Tufts Univ, Medford, MA 02155 USA. RP Mousseau, J (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA.; Mousseau, J (reprint author), Univ Michigan, Ann Arbor, MI 48109 USA. OI Bodek, Arie/0000-0003-0409-0341; Solano Salinas, Carlos Javier/0000-0001-7821-498X; Hurtado Anampa, Kenyi/0000-0002-9779-3566 FU Fermi National Accelerator Laboratory under US Department of Energy [DE-AC02-07CH11359]; United States National Science Foundation [PHY-0619727]; University of Rochester; NSF; DOE (USA); CAPES; CNPq (Brazil); CoNaCyT (Mexico); CONICYT (Chile); CONCYTEC; DGI-PUCP; IDI/IGI-UNI (Peru); Latin American Center for Physics (CLAF) FX This work was supported by the Fermi National Accelerator Laboratory under US Department of Energy contract No. DE-AC02-07CH11359 which included the MINERvA construction project. Construction support was also granted by the United States National Science Foundation under Award PHY-0619727 and by the University of Rochester. Support for participating scientists was provided by NSF and DOE (USA), by CAPES and CNPq (Brazil), by CoNaCyT (Mexico), by CONICYT (Chile), by CONCYTEC, DGI-PUCP and IDI/IGI-UNI (Peru), by Latin American Center for Physics (CLAF). We thank the MINOS Collaboration for use of its near detector data. We acknowledge the dedicated work of the Fermilab staff responsible for the operation and maintenance of the beamline, detector, and the computing infrastructure. NR 48 TC 2 Z9 2 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 19 PY 2016 VL 93 IS 7 AR 071101 DI 10.1103/PhysRevD.93.071101 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QG UT WOS:000374547400001 ER PT J AU Pal, B Schwartz, AJ Abdesselam, A Adachi, I Aihara, H Asner, DM Aushev, T Ayad, R Aziz, T Babu, V Badhrees, I Bahinipati, S Bakich, AM Barberio, E Behera, P Bhardwaj, V Bhuyan, B Biswal, J Bobrov, A Bozek, A Bracko, M Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dash, N Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Eidelman, S Farhat, H Fast, JE Fulsom, BG Gaur, V Garmash, A Gillard, R Goh, YM Goldenzweig, P Greenwald, D Grzymkowska, O Haba, J Hara, T Hayasaka, K Hayashii, H He, XH Hou, WS Inami, K Ishikawa, A Iwasaki, Y Jacobs, WW Jaegle, I Jeon, HB Joffe, D Joo, KK Julius, T Kang, KH Kato, E Kawasaki, T Kiesling, C Kim, DY Kim, HJ Kim, KT Kim, MJ Kim, SH Kinoshita, K Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kumar, R Kumita, T Kuzmin, A Kwon, YJ Lee, IS Li, CH Li, H Li, L Gioi, LL Libby, J Liventsev, D Lukin, P Luo, T Masuda, M Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Mohanty, S Moll, A Moon, HK Mori, T Mussa, R Nakano, E Nakao, M Nanut, T Natkaniec, Z Nayak, M Nisar, NK Nishida, S Ogawa, S Okuno, S Pakhlov, P Pakhlova, G Park, CW Park, H Paul, S Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Rauch, J Ribezl, E Ritter, M Rostomyan, A Ryu, S Sahoo, H Sakai, Y Sandilya, S Sanuki, T Sato, Y Savinov, V Schluter, T Schneider, O Schnell, G Schwanda, C Seino, Y Senyo, K Seon, O Seong, IS Shebalin, V Shibata, TA Shiu, JG Shwartz, B Simon, F Sohn, YS Sokolov, A Solovieva, E Stanic, S Staric, M Stypula, J Sumihama, M Sumiyoshi, T Tamponi, U Teramoto, Y Trabelsi, K Uchida, M Uehara, S Uglov, T Uno, S Urquijo, P Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vossen, A Wagner, MN Wang, CH Wang, MZ Wang, XL Watanabe, M Watanabe, Y Williams, KM Won, E Yamaoka, J Yelton, J Yuan, CZ Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Pal, B. Schwartz, A. J. Abdesselam, A. Adachi, I. Aihara, H. Asner, D. M. Aushev, T. Ayad, R. Aziz, T. Babu, V. Badhrees, I. Bahinipati, S. Bakich, A. M. Barberio, E. Behera, P. Bhardwaj, V. Bhuyan, B. Biswal, J. Bobrov, A. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dash, N. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Fulsom, B. G. Gaur, V. Garmash, A. Gillard, R. Goh, Y. M. Goldenzweig, P. Greenwald, D. Grzymkowska, O. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. He, X. H. Hou, W. -S. Inami, K. Ishikawa, A. Iwasaki, Y. Jacobs, W. W. Jaegle, I. Jeon, H. B. Joffe, D. Joo, K. K. Julius, T. Kang, K. H. Kato, E. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, K. T. Kim, M. J. Kim, S. H. Kinoshita, K. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kumar, R. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lee, I. S. Li, C. H. Li, H. Li, L. Li Gioi, L. Libby, J. Liventsev, D. Lukin, P. Luo, T. Masuda, M. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Mohanty, S. Moll, A. Moon, H. K. Mori, T. Mussa, R. Nakano, E. Nakao, M. Nanut, T. Natkaniec, Z. Nayak, M. Nisar, N. K. Nishida, S. Ogawa, S. Okuno, S. Pakhlov, P. Pakhlova, G. Park, C. W. Park, H. Paul, S. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Rauch, J. Ribezl, E. Ritter, M. Rostomyan, A. Ryu, S. Sahoo, H. Sakai, Y. Sandilya, S. Sanuki, T. Sato, Y. Savinov, V. Schlueter, T. Schneider, O. Schnell, G. Schwanda, C. Seino, Y. Senyo, K. Seon, O. Seong, I. S. Shebalin, V. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Stanic, S. Staric, M. Stypula, J. Sumihama, M. Sumiyoshi, T. Tamponi, U. Teramoto, Y. Trabelsi, K. Uchida, M. Uehara, S. Uglov, T. Uno, S. Urquijo, P. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vossen, A. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, X. L. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yamaoka, J. Yelton, J. Yuan, C. Z. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Observation of the Decay B-s(0) -> K-0(K)over-bar(0) SO PHYSICAL REVIEW LETTERS LA English DT Article ID ANNIHILATION; DETECTOR; PACKAGE AB We measure the decay B-s(0) -> K-0(K) over bar (0) using data collected at the Upsilon(5S) resonance with the Belle detector at the KEKB e(+)e(-) collider. The data sample used corresponds to an integrated luminosity of 121.4 fb(-1). We measure a branching fraction beta(B-s(0) -> K-0(K) over bar (0)) = [19.6(-5.1)(+5.8)(stat) +/- 1.0(syst) +/- 2.0(N-Bs0 (B) over bar s0)] x 10(-6) with a significance of 5.1 standard deviations. This measurement constitutes the first observation of this decay. C1 [Nisar, N. K.] Aligarh Muslim Univ, Aligarh 202002, Uttar Pradesh, India. [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Bobrov, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Pal, B.; Schwartz, A. J.; Kinoshita, K.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Rostomyan, A.] DESY, D-22607 Hamburg, Germany. [Yelton, J.] Univ Florida, Gainesville, FL 32611 USA. [Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Haba, J.; Hara, T.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uehara, S.; Uno, S.] Grad Univ Adv Studies, SOKENDAI, Hayama, Kanagawa 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Seong, I. S.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Bahinipati, S.; Dash, N.] Indian Inst Technol, Bhubaneswar 751007, Orissa, India. [Bhuyan, B.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Behera, P.; Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Jacobs, W. W.; Li, H.; Vossen, A.] Indiana Univ, Bloomington, IN 47408 USA. [Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Drutskoy, A.; Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chistov, R.; Mizuk, R.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Biswal, J.; Bracko, M.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Cho, K.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, K. T.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Jeon, H. B.; Kang, K. H.; Kim, H. J.; Kim, M. J.; Park, H.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Krizan, P.; Zupanc, A.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.; Ritter, M.; Schlueter, T.] Univ Munich, Marchioninistr 15, D-80539 Munich, Germany. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Li Gioi, L.; Moll, A.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Barberio, E.; Julius, T.; Li, C. H.; Urquijo, P.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Drutskoy, A.; Mizuk, R.; Pakhlov, P.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Aushev, T.; Pakhlova, G.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Inami, K.; Mori, T.; Sato, Y.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Grzymkowska, O.; Natkaniec, Z.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Seino, Y.; Watanabe, M.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gorica, Nova Gorica 5000, Slovenia. [Bobrov, A.; Eidelman, S.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Fulsom, B. G.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Luo, T.; Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Kumar, R.] Punjab Agr Univ, Ludhiana 141004, Punjab, India. [Li, L.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Ayad, R.; Badhrees, I.] Univ Tabuk, Dept Phys, Fac Sci, Tabuk 71451, Saudi Arabia. [Aziz, T.; Babu, V.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Mohanty, S.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Greenwald, D.; Paul, S.; Rauch, J.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Ishikawa, A.; Kato, E.; Sanuki, T.] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Mohanty, S.] Utkal Univ, Bhubaneswar 751004, Orissa, India. [Liventsev, D.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. RP Pal, B (reprint author), Univ Cincinnati, Cincinnati, OH 45221 USA. RI Aihara, Hiroaki/F-3854-2010; Paul, Stephan/F-7596-2015; Paul, Stephan/K-9237-2016; Uglov, Timofey/B-2406-2014; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016; Mizuk, Roman/B-3751-2014; Pakhlova, Galina/C-5378-2014; Pakhlov, Pavel/K-2158-2013; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014 OI Aihara, Hiroaki/0000-0002-1907-5964; Paul, Stephan/0000-0002-8813-0437; Paul, Stephan/0000-0002-8813-0437; Uglov, Timofey/0000-0002-4944-1830; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422; Pakhlova, Galina/0000-0001-7518-3022; Pakhlov, Pavel/0000-0001-7426-4824; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton PhysicsResearch Center of Nagoya University; Australian Research Council; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Chinese Academy of Science Center for Excellence in Particle Physics; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; WCU program of the Ministry of Education; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2015R1A2A2-A01003280, 2015H1A2A1033649]; Basic Research Lab program under NRF Grant [KRF-2011-0020333]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program and Radiation Science Research Institute; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT; JSPS FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton PhysicsResearch Center of Nagoya University; the Australian Research Council; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Chinese Academy of Science Center for Excellence in Particle Physics; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the WCU program of the Ministry of Education, National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, No. 2015R1A2A2-A01003280, No. 2015H1A2A1033649; the Basic Research Lab program under NRF Grant No. KRF-2011-0020333, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and Radiation Science Research Institute; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 28 TC 3 Z9 3 U1 7 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 19 PY 2016 VL 116 IS 16 AR 161801 DI 10.1103/PhysRevLett.116.161801 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ9UQ UT WOS:000374558900001 PM 27152790 ER PT J AU Bergano, M Rocha, A Cupido, L Barbosa, D Villela, T Boas, JV Rocha, G Smoot, GF AF Bergano, Miguel Rocha, Armando Cupido, Luis Barbosa, Domingos Villela, Thyrso Boas, Jose Vilas Rocha, Graca Smoot, George F. TI A high performance cost-effective digital complex correlator for an X-band polarimetry survey SO SPRINGERPLUS LA English DT Article DE Radioastronomy (astronomy, astrophysics and cosmology); Logic design (hardware); Register-transfer-level implementation (hardware) ID POLARIZATION; EMISSION AB The detailed knowledge of the Milky Way radio emission is important to characterize galactic foregrounds masking extragalactic and cosmological signals. The update of the global sky models describing radio emissions over a very large spectral band requires high sensitivity experiments capable of observing large sky areas with long integration times. Here, we present the design of a new 10 GHz (X-band) polarimeter digital back-end to map the polarization components of the galactic synchrotron radiation field of the Northern Hemisphere sky. The design follows the digital processing trends in radio astronomy and implements a large bandwidth (1 GHz) digital complex cross-correlator to extract the Stokes parameters of the incoming synchrotron radiation field. The hardware constraints cover the implemented VLSI hardware description language code and the preliminary results. The implementation is based on the simultaneous digitized acquisition of the Cartesian components of the two linear receiver polarization channels. The design strategy involves a double data rate acquisition of the ADC interleaved parallel bus, and field programmable gate array device programming at the register transfer mode. The digital core of the back-end is capable of processing 32 Gbps and is built around an Altera field programmable gate array clocked at 250 MHz, 1 GSps analog to digital converters and a clock generator. The control of the field programmable gate array internal signal delays and a convenient use of its phase locked loops provide the timing requirements to achieve the target bandwidths and sensitivity. This solution is convenient for radio astronomy experiments requiring large bandwidth, high functionality, high volume availability and low cost. Of particular interest, this correlator was developed for the Galactic Emission Mapping project and is suitable for large sky area polarization continuum surveys. The solutions may also be adapted to be used at signal processing subsystem levels for large projects like the square kilometer array testbeds. C1 [Bergano, Miguel] Univ Aveiro, Inst Telecomunicacoes, DETI, Campus Univ Santiago, P-3810193 Aveiro, Portugal. [Rocha, Armando] Univ Aveiro, DETI, Campus Univ Santiago, P-3810106 Aveiro, Portugal. [Cupido, Luis] LC Technol, Aveiro, Portugal. [Barbosa, Domingos] Inst Telecomunicacoes, Campus Univ Santiago, P-3810193 Aveiro, Portugal. [Villela, Thyrso; Boas, Jose Vilas] INPE, Div Astrofis DAS, Ave Astronautas 1-758, BR-12227010 Sao Jose Dos Campos, SP, Brazil. [Rocha, Graca] CALTECH, Jet Prop Lab, M-S 169-327,4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Rocha, Graca] CALTECH, Cahill Bldg MS 59-33 1200 E Calif, Pasadena, CA 91125 USA. [Smoot, George F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 50-5005, Berkeley, CA 94720 USA. [Smoot, George F.] Univ Paris Diderot APC, Batiment Condorcet, F-75205 Paris 13, France. RP Bergano, M (reprint author), Univ Aveiro, Inst Telecomunicacoes, DETI, Campus Univ Santiago, P-3810193 Aveiro, Portugal. EM jbergano@av.it.pt FU Fundacao para a Ciencia e a Tecnologia (FCT) the Portuguese national funding agency [SFRH/BD/76615/2011]; FCT/MEC through national funds; FEDER-PT2020 [UID/EEA/50008/2013] FX The corresponding author acknowledge support from the Fundacao para a Ciencia e a Tecnologia (FCT) the Portuguese national funding agency (SFRH/BD/76615/2011) and by FCT/MEC through national funds and when applicable co-funded by FEDER-PT2020 partnership agreement under the project UID/EEA/50008/2013. NR 25 TC 0 Z9 0 U1 2 U2 2 PU SPRINGER INTERNATIONAL PUBLISHING AG PI CHAM PA GEWERBESTRASSE 11, CHAM, CH-6330, SWITZERLAND SN 2193-1801 J9 SPRINGERPLUS JI SpringerPlus PD APR 19 PY 2016 VL 5 AR 487 DI 10.1186/s40064-016-2109-5 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DL5UB UT WOS:000375701400008 PM 27218002 ER PT J AU Peng, JF Hu, M Guo, S Du, ZF Zheng, J Shang, DJ Zamora, ML Zeng, LM Shao, M Wu, YS Zheng, J Wang, Y Glen, CR Collins, DR Molina, MJ Zhang, RY AF Peng, Jianfei Hu, Min Guo, Song Du, Zhuofei Zheng, Jing Shang, Dongjie Zamora, Misti Levy Zeng, Limin Shao, Min Wu, Yu-Sheng Zheng, Jun Wang, Yuan Glen, Crystal R. Collins, Donald R. Molina, Mario J. Zhang, Renyi TI Markedly enhanced absorption and direct radiative forcing of black carbon under polluted urban environments SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE black carbon; absorption; air quality; radiative forcing; climate ID OH-INITIATED OXIDATION; LIGHT-ABSORPTION; SOOT AEROSOLS; MIXING STATE; AMPLIFICATION; PARTICLES; CONSISTENCY; RADICALS; IMPACTS; TOLUENE AB Black carbon (BC) exerts profound impacts on air quality and climate because of its high absorption cross-section over a broad range of electromagnetic spectra, but the current results on absorption enhancement of BC particles during atmospheric aging remain conflicting. Here, we quantified the aging and variation in the optical properties of BC particles under ambient conditions in Beijing, China, and Houston, United States, using a novel environmental chamber approach. BC aging exhibits two distinct stages, i.e., initial transformation from a fractal to spherical morphology with little absorption variation and subsequent growth of fully compact particles with a large absorption enhancement. The timescales to achieve complete morphology modification and an absorption amplification factor of 2.4 for BC particles are estimated to be 2.3 h and 4.6 h, respectively, in Beijing, compared with 9 h and 18 h, respectively, in Houston. Our findings indicate that BC under polluted urban environments could play an essential role in pollution development and contribute importantly to large positive radiative forcing. The variation in direct radiative forcing is dependent on the rate and timescale of BC aging, with a clear distinction between urban cities in developed and developing countries, i.e., a higher climatic impact inmore polluted environments. We suggest that mediation in BC emissions achieves a cobenefit in simultaneously controlling air pollution and protecting climate, especially for developing countries. C1 [Peng, Jianfei; Hu, Min; Guo, Song; Du, Zhuofei; Zheng, Jing; Shang, Dongjie; Zeng, Limin; Wu, Yu-Sheng; Zhang, Renyi] Peking Univ, State Key Joint Lab Environm Simulat & Pollut Con, Coll Environm Sci & Engn, Beijing 100871, Peoples R China. [Guo, Song; Zamora, Misti Levy; Shao, Min; Zheng, Jun; Glen, Crystal R.; Collins, Donald R.; Zhang, Renyi] Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA. [Wang, Yuan] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91125 USA. [Molina, Mario J.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Zheng, Jun] Nanjing Univ Informat Sci & Technol, Jiangsu Key Lab Atmospher Environm Monitoring & P, Nanjing 210044, Jiangsu, Peoples R China. [Glen, Crystal R.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Hu, M; Zhang, RY (reprint author), Peking Univ, State Key Joint Lab Environm Simulat & Pollut Con, Coll Environm Sci & Engn, Beijing 100871, Peoples R China.; Zhang, RY (reprint author), Texas A&M Univ, Dept Atmospher Sci, College Stn, TX 77843 USA.; Molina, MJ (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. EM minhu@pku.edu.cn; mjmolina@ucsd.edu; renyi-zhang@tamu.edu RI Guo, Song/D-9218-2012; Zeng, Limin/D-3948-2013; Collins, Don/F-9617-2012; Zhang, Renyi/A-2942-2011; Zheng, Jun/E-6772-2010; Peng, Jianfei/F-1438-2015 OI Guo, Song/0000-0002-9661-2313; FU National Natural Science Foundation of China [91544214, 21190052]; National Basic Research Program; China Ministry of Science and Technology [2013CB228503]; China Ministry of Environmental Protection's Special Funds for Scientific Research on Public Welfare [20130916]; Robert A. Welch Foundation [A-1417]; Houston Advanced Research Center FX We thank Wei Hu and Zhaoheng Gong for their assistance with the AMS data analysis, Wentai Chen and Yue Li for providing VOCs data, and Nan Ma for providing the core-shell code for the Mie calculation. This work was supported by National Natural Science Foundation of China (Grants 91544214 and 21190052), the National Basic Research Program, China Ministry of Science and Technology (Grant 2013CB228503), National Natural Science Foundation of China (Grant 21190052), and the China Ministry of Environmental Protection's Special Funds for Scientific Research on Public Welfare (Grant 20130916). R.Z. acknowledges support from the Robert A. Welch Foundation (Grant A-1417) and Houston Advanced Research Center. NR 42 TC 31 Z9 32 U1 55 U2 96 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 19 PY 2016 VL 113 IS 16 BP 4266 EP 4271 DI 10.1073/pnas.1602310113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7LV UT WOS:000374393800030 PM 27035993 ER PT J AU Wu, J Bollinger, AT Sun, YJ Bozovic, I AF Wu, Jie Bollinger, Anthony T. Sun, Yujie Bozovic, Ivan TI Hall effect in quantum critical charge-cluster glass SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE high-temperature superconductors; charge glass; superconductor-to-insulator transition; quantum fluctuations; Hall effect ID HIGH-T-C; SUPERCONDUCTOR-INSULATOR TRANSITION; HIGH-TEMPERATURE SUPERCONDUCTORS; LATTICE-MELTING TRANSITION; DENSITY-WAVE ORDER; NORMAL-STATE; PSEUDOGAP STATE; MOTT INSULATOR; LA2-XSRXCUO4; BI2SR2-XLAXCUO6+DELTA AB Upon doping, cuprates undergo a quantum phase transition from an insulator to a d-wave superconductor. The nature of this transition and of the insulating state is vividly debated. Here, we study the Hall effect in La2-xSrxCuO4 (LSCO) samples doped near the quantum critical point at x similar to 0.06. Dramatic fluctuations in the Hall resistance appear below T-CG similar to 1.5 K and increase as the sample is cooled down further, signaling quantum critical behavior. We explore the doping dependence of this effect in detail, by studying a combinatorial LSCO library in which the Sr content is varied in extremely fine steps, Delta x similar to 0.00008. We observe that quantum charge fluctuations wash out when superconductivity emerges but can be restored when the latter is suppressed by applying a magnetic field, showing that the two instabilities compete for the ground state. C1 [Wu, Jie; Bollinger, Anthony T.; Sun, Yujie; Bozovic, Ivan] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA. [Sun, Yujie] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Bozovic, Ivan] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. RP Bozovic, I (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Div, Upton, NY 11973 USA.; Bozovic, I (reprint author), Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. EM bozovic@bnl.gov FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 57 TC 3 Z9 3 U1 3 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 19 PY 2016 VL 113 IS 16 BP 4284 EP 4289 DI 10.1073/pnas.1519630113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7LV UT WOS:000374393800033 PM 27044081 ER PT J AU Wu, SQ Joseph, A Hammonds, AS Celniker, SE Yu, B Frise, E AF Wu, Siqi Joseph, Antony Hammonds, Ann S. Celniker, Susan E. Yu, Bin Frise, Erwin TI Stability-driven nonnegative matrix factorization to interpret spatial gene expression and build local gene networks SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE principal patterns; stability selection; sparse decomposition; spatial gene expression; spatially local networks ID DROSOPHILA EMBRYO; INTRATUMOR HETEROGENEITY; TRANSCRIPTION FACTORS; AUTOMATED ANNOTATION; GLOBAL ANALYSIS; HUMAN BRAIN; PATTERNS; DIVERSITY; EVOLUTION; IMAGES AB Spatial gene expression patterns enable the detection of local covariability and are extremely useful for identifying local gene interactions during normal development. The abundance of spatial expression data in recent years has led to the modeling and analysis of regulatory networks. The inherent complexity of such data makes it a challenge to extract biological information. We developed staNMF, a method that combines a scalable implementation of nonnegative matrix factorization (NMF) with a new stability-driven model selection criterion. When applied to a set of Drosophila early embryonic spatial gene expression images, one of the largest datasets of its kind, staNMF identified 21 principal patterns (PP). Providing a compact yet biologically interpretable representation of Drosophila expression patterns, PP are comparable to a fate map generated experimentally by laser ablation and show exceptional promise as a data-driven alternative to manual annotations. Our analysis mapped genes to cell-fate programs and assigned putative biological roles to uncharacterized genes. Finally, we used the PP to generate local transcription factor regulatory networks. Spatially local correlation networks were constructed for six PP that span along the embryonic anterior-posterior axis. Using a two-tail 5% cutoff on correlation, we reproduced 10 of the 11 links in the well-studied gap gene network. The performance of PP with the Drosophila data suggests that staNMF provides informative decompositions and constitutes a useful computational lens through which to extract biological insight from complex and often noisy gene expression data. C1 [Wu, Siqi; Joseph, Antony; Yu, Bin] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Wu, Siqi; Joseph, Antony; Hammonds, Ann S.; Celniker, Susan E.; Frise, Erwin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Environm Genom & Syst Biol, Berkeley, CA 94720 USA. [Joseph, Antony] Walmart Labs, San Bruno, CA 94066 USA. [Yu, Bin] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Yu, B (reprint author), Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA.; Frise, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Environm Genom & Syst Biol, Berkeley, CA 94720 USA.; Yu, B (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM binyu@stat.berkeley.edu; erwin@fruitfly.org FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 49 TC 0 Z9 0 U1 6 U2 6 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 19 PY 2016 VL 113 IS 16 BP 4290 EP 4295 DI 10.1073/pnas.1521171113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7LV UT WOS:000374393800034 PM 27071099 ER PT J AU Abel, JH Meeker, K Granados-Fuentes, D St John, PC Wang, TJ Bales, BB Doyle, FJ Herzog, ED Petzold, LR AF Abel, John H. Meeker, Kirsten Granados-Fuentes, Daniel St John, Peter C. Wang, Thomas J. Bales, Benjamin B. Doyle, Francis J., III Herzog, Erik D. Petzold, Linda R. TI Functional network inference of the suprachiasmatic nucleus SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE systems biology; synchronization; circadian oscillator; biological clock; mathematical model ID CIRCADIAN GENE-EXPRESSION; MAMMALIAN CLOCK NEURONS; SMALL-WORLD NETWORKS; INTERCELLULAR SYNCHRONIZATION; OSCILLATORS; MODEL; LIGHT; HAMSTERS; RHYTHMS; GABA AB In the mammalian suprachiasmatic nucleus (SCN), noisy cellular oscillators communicate within a neuronal network to generate precise system-wide circadian rhythms. Although the intracellular genetic oscillator and intercellular biochemical coupling mechanisms have been examined previously, the network topology driving synchronization of the SCN has not been elucidated. This network has been particularly challenging to probe, due to its oscillatory components and slow coupling timescale. In this work, we investigated the SCN network at a single-cell resolution through a chemically induced desynchronization. We then inferred functional connections in the SCN by applying the maximal information coefficient statistic to bioluminescence reporter data from individual neurons while they resynchronized their circadian cycling. Our results demonstrate that the functional network of circadian cells associated with resynchronization has small-world characteristics, with a node degree distribution that is exponential. We show that hubs of this small-world network are preferentially located in the central SCN, with sparsely connected shells surrounding these cores. Finally, we used two computational models of circadian neurons to validate our predictions of network structure. C1 [Abel, John H.; St John, Peter C.; Doyle, Francis J., III] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Abel, John H.] Harvard Univ, Syst Biol Program, Cambridge, MA 02138 USA. [Meeker, Kirsten; Bales, Benjamin B.; Petzold, Linda R.] Univ Calif Santa Barbara, Dept Comp Sci, Santa Barbara, CA 93106 USA. [Granados-Fuentes, Daniel; Wang, Thomas J.; Herzog, Erik D.] Washington Univ, Dept Biol, Campus Box 1137, St Louis, MO 63130 USA. [St John, Peter C.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Doyle, Francis J., III] Harvard Univ, Harvard John A Paulson Sch Engn & Appl Sci, Cambridge, MA 02138 USA. RP Petzold, LR (reprint author), Univ Calif Santa Barbara, Dept Comp Sci, Santa Barbara, CA 93106 USA. EM petzold@engineering.ucsb.edu FU NIH [1R01GM096873-01]; Institute for Collaborative Biotechnologies from the US Army Research Office [W911NF-09-0001] FX We thank Kelsey R. Dean, Brian Drawert, and Stephanie R. Taylor for helpful discussions. We also thank each of the anonymous reviewers, whose efforts have improved and shaped our manuscript. This work was supported by NIH Grant 1R01GM096873-01 (to F.J.D., L.R.P., and E.D.H.) and Institute for Collaborative Biotechnologies Grant W911NF-09-0001 from the US Army Research Office. NR 64 TC 3 Z9 3 U1 5 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 19 PY 2016 VL 113 IS 16 BP 4512 EP 4517 DI 10.1073/pnas.1521178113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ7LV UT WOS:000374393800071 PM 27044085 ER PT J AU Pan, HL Shao, YY Yan, PF Cheng, YW Han, KS Nie, ZM Wang, CM Yang, JH Li, XL Bhattacharya, P Mueller, KT Liu, J AF Pan, Huilin Shao, Yuyan Yan, Pengfei Cheng, Yingwen Han, Kee Sung Nie, Zimin Wang, Chongmin Yang, Jihui Li, Xiaolin Bhattacharya, Priyanka Mueller, Karl T. Liu, Jun TI Reversible aqueous zinc/manganese oxide energy storage from conversion reactions SO NATURE ENERGY LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; LONG CYCLE LIFE; ION BATTERY; HIGH-POWER; ZINC-ION; COPPER HEXACYANOFERRATE; MANGANESE-DIOXIDE; ELECTRODE; CATHODE; SYSTEM AB Rechargeable aqueous batteries such as alkaline zinc/manganese oxide batteries are highly desirable for large-scale energy storage owing to their low cost and high safety; however, cycling stability is a major issue for their applications. Here we demonstrate a highly reversible zinc/manganese oxide system in which optimal mild aqueous ZnSO4-based solution is used as the electrolyte, and nanofibres of a manganese oxide phase, alpha-MnO2, are used as the cathode. We show that a chemical conversion reaction mechanism between alpha-MnO2 and H+ is mainly responsible for the good performance of the system. This includes an operating voltage of 1.44 V, a capacity of 285 mAh g(-1) (MnO2), and capacity retention of 92% over 5,000 cycles. The Zn metal anode also shows high stability. This finding opens new opportunities for the development of low-cost, high-performance rechargeable aqueous batteries. C1 [Pan, Huilin; Shao, Yuyan; Cheng, Yingwen; Nie, Zimin; Li, Xiaolin; Bhattacharya, Priyanka; Liu, Jun] Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Yan, Pengfei; Han, Kee Sung; Wang, Chongmin] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Yang, Jihui] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Mueller, Karl T.] Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. RP Shao, YY; Liu, J (reprint author), Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM yuyan.shao@pnnl.gov; jun.liu@pnnl.gov RI Shao, Yuyan/A-9911-2008; yan, pengfei/E-4784-2016 OI Shao, Yuyan/0000-0001-5735-2670; yan, pengfei/0000-0001-6387-7502 FU US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [KC020105-FWP12152]; Department of Energy's Office of Biological and Environmental Research; Inamori Foundation FX This work is supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award KC020105-FWP12152. The TEM, NMR and XRD work were performed using EMSL, a National Scientific User Facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. PNNL is a Multi-Program National Laboratory operated for DOE by Battelle. The work at UW was supported by Inamori Foundation. NR 40 TC 15 Z9 15 U1 22 U2 22 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2058-7546 J9 NAT ENERGY JI Nat. Energy PD APR 18 PY 2016 VL 1 AR 16039 DI 10.1038/NENERGY.2016.39 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary SC Energy & Fuels; Materials Science GA EK7PE UT WOS:000394116900001 ER PT J AU Mullaney, JC Zaleski, DP Tew, DP Walker, NR Legon, AC AF Mullaney, John C. Zaleski, Daniel P. Tew, David P. Walker, Nicholas R. Legon, Anthony C. TI Geometry of an Isolated Dimer of Imidazole Characterised by Rotational Spectroscopy and Ab Initio Calculations SO CHEMPHYSCHEM LA English DT Article DE ab initio calculations; dimerization; hydrogen bonds; nitrogen heterocycles; rotational spectroscopy ID MICROWAVE-SPECTRUM; HELIUM NANODROPLETS; CENTRIFUGAL-DISTORTION; WATER COMPLEXES; DIPOLE-MOMENT; MINOR-GROOVE; GAS-PHASE; CHEMISTRY; PYRROLE; CYANIDE AB An isolated, gas-phase dimer of imidazole is generated through laser vaporisation of a solid rod containing a 1:1 mixture of imidazole and copper in the presence of an argon buffer gas undergoing supersonic expansion. The complex is characterised through broadband rotational spectroscopy and is shown to have a twisted, hydrogen-bonded geometry. Calculations at the CCSD(T)(F12*)/cc-pVDZ-F12 level of theory confirm this to be the lowest-energy conformer of the imidazole dimer. The distance between the respective centres of mass of the imidazole monomer subunits is determined to be 5.2751(1)angstrom, and the twist angle describing rotation of one monomer with respect to the other about a line connecting the centres of mass of the monomers is determined to be 87.9(4)degrees. Four out of six intermolecular parameters in the model geometry are precisely determined from the experimental rotational constants and are consistent with results calculated ab initio. C1 [Mullaney, John C.; Zaleski, Daniel P.; Walker, Nicholas R.] Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. [Tew, David P.; Legon, Anthony C.] Univ Bristol, Sch Chem, Cantocks Close, Bristol BS8 1TS, Avon, England. [Zaleski, Daniel P.] Argonne Natl Lab, Chem Sci & Engn, 9700 S Cass Ave,Bldg 200, Lemont, IL 60439 USA. RP Walker, NR (reprint author), Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England.; Legon, AC (reprint author), Univ Bristol, Sch Chem, Cantocks Close, Bristol BS8 1TS, Avon, England. EM nick.walker@newcastle.ac.uk; a.c.legon@bristol.ac.uk RI Walker, Nicholas /E-6180-2011; Tew, David/E-1458-2011; OI Walker, Nicholas /0000-0002-9450-305X; Tew, David/0000-0002-3220-4177; Zaleski, Daniel/0000-0003-0153-9158 FU European Research Council [CPFTMW-307000]; University of Bristol; Newcastle University; Royal Society FX The authors thank the European Research Council for a postdoctoral fellowship awarded to D.P.Z, for a postgraduate studentship to J.C.M, and for project funding (CPFTMW-307000). A.C.L. thanks the University of Bristol for a Senior Research Fellowship, and Newcastle University for a Faculty of SAgE Visiting Professorship. D.P.Z. thanks Newcastle University for the award of a Faculty of SAgE Research Fellowship. D.P.T. thanks the Royal Society for a University Research Fellowship. The authors also thank Dr. Simon Doherty (School of Chemistry, Newcastle University) for preparing the sample of monodeuterated imidazole necessary for these experiments. NR 43 TC 0 Z9 0 U1 5 U2 9 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1439-4235 EI 1439-7641 J9 CHEMPHYSCHEM JI ChemPhysChem PD APR 18 PY 2016 VL 17 IS 8 BP 1154 EP 1158 DI 10.1002/cphc.201501179 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK1QS UT WOS:000374689100011 PM 26812549 ER PT J AU Pecyna, J Kaszynski, P Ringstrand, B Pociecha, D Pakhomov, S Douglass, AG Young, VG AF Pecyna, Jacek Kaszynski, Piotr Ringstrand, Bryan Pociecha, Damian Pakhomov, Serhii Douglass, Andrew G. Young, Victor G., Jr. TI Synthesis and Characterization of Quinuclidinium Derivatives of the [closo-1-CB11H12](-) Anion as Potential Polar Components of Liquid Crystal Materials SO INORGANIC CHEMISTRY LA English DT Article ID DIELECTRIC ANISOTROPY; FUNCTIONALIZATION; PRECURSORS; CARBORANES; CHEMISTRY; NEMATICS; BENZENE; OCTANE AB Antipodal substitution of the [closo-1-CB11H12](-) anion with a 4-pentylquinuclidinium fragment and alkyl groups in positions C(1) and B(12) gave polar zwitterions 1[n] and 2[n]. The molecular structure of 1[5] was established using X-ray diffraction (XRD) methods: P (1) over bar, a = 15.162(2) angstrom, b = 16.546(3) angstrom, c = 19.794(3) angstrom; alpha = 84.871(2)degrees, beta = 84.057(2)degrees, gamma = 84.058(3)degrees; Z = 8. All Phi compounds exhibit high temperature in-plane ordered smectic phases that are stabilized by dipolar interactions. The ordered phases were investigated by powder XRD methods. Thermal and dielectric parameters for two derivatives, 1[0] and 1[6], were evaluated in nematic hosts, ClEster and BPhF. The dielectric data were analyzed with the Maier-Meier formalism augmented with density functional theory methods, and the results were compared to those for similar zwitterions previously reported. C1 [Pecyna, Jacek; Kaszynski, Piotr; Douglass, Andrew G.] Middle Tennessee State Univ, Dept Chem, Organ Mat Res Grp, Murfreesboro, TN 37132 USA. [Kaszynski, Piotr] Polish Acad Sci, Ctr Mol & Macromol Studies, Sienkiewicza 112, PL-90363 Lodz, Poland. [Kaszynski, Piotr] Univ Lodz, Fac Chem, Tamka 12, PL-91403 Lodz, Poland. [Pociecha, Damian] Univ Warsaw, Dept Chem, Zwirki & Wigury 101, PL-02089 Warsaw, Poland. [Young, Victor G., Jr.] Univ Minnesota, Dept Chem, Xray Crystallog Lab, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Ringstrand, Bryan] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. [Pakhomov, Serhii] Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. RP Kaszynski, P (reprint author), Middle Tennessee State Univ, Dept Chem, Organ Mat Res Grp, Murfreesboro, TN 37132 USA.; Kaszynski, P (reprint author), Polish Acad Sci, Ctr Mol & Macromol Studies, Sienkiewicza 112, PL-90363 Lodz, Poland.; Kaszynski, P (reprint author), Univ Lodz, Fac Chem, Tamka 12, PL-91403 Lodz, Poland. EM piotr.kaszynski@mtsu.edu FU NSF [DMR-1207585, DMR-9703002, DMR-0907542]; ONR [ONR-331/99/0237]; National Science Center Poland [OPUS 2015/17/B/ST5/02801] FX This work was supported by the NSF (DMR-1207585, DMR-9703002, DMR-0907542), ONR (ONR-331/99/0237), and National Science Center Poland (OPUS 2015/17/B/ST5/02801) grants. We are grateful to Prof. R. Dabrowski of the Military University of Technology, Warsaw, Poland, for the gift of the nematic hosts. NR 51 TC 2 Z9 2 U1 1 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD APR 18 PY 2016 VL 55 IS 8 BP 4016 EP 4025 DI 10.1021/acs.inorgchem.6b00319 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DJ9BI UT WOS:000374508600037 PM 27018818 ER PT J AU Bartolo, N Messina, R Dalvit, DAR Intravaia, F AF Bartolo, Nicola Messina, Riccardo Dalvit, Diego A. R. Intravaia, Francesco TI Nonequilibrium Casimir-Polder plasmonic interactions SO PHYSICAL REVIEW A LA English DT Article ID ELECTROMAGNETIC-WAVES; VACUUM FLUCTUATIONS; OPTICAL LATTICES; HEAT-TRANSFER; SURFACE; FORCE; ATOMS AB We investigate how the combination of nonequilibrium effects and material properties impacts on the Casimir-Polder interaction between an atom and a surface. By addressing systems with temperature inhomogeneities and laser interactions, we show that nonmonotonous energetic landscapes can be produced where barriers and minima appear. Our treatment provides a self-consistent quantum theoretical framework for investigating the properties of a class of nonequilibrium atom-surface interactions. C1 [Bartolo, Nicola] Univ Paris Diderot, Sorbonne Paris Cite, Lab Mat & Phenomenes Quant, CNRS,UMR7162, F-75013 Paris, France. [Messina, Riccardo] Univ Montpellier, Lab Charles Coulomb, UMR 5221, F-34095 Montpellier, France. [Messina, Riccardo] CNRS, F-34095 Montpellier, France. [Dalvit, Diego A. R.] Los Alamos Natl Lab, Div Theoret, MS B213, Los Alamos, NM 87545 USA. [Intravaia, Francesco] Max Born Inst, D-12489 Berlin, Germany. RP Bartolo, N (reprint author), Univ Paris Diderot, Sorbonne Paris Cite, Lab Mat & Phenomenes Quant, CNRS,UMR7162, F-75013 Paris, France. EM nicola.bartolo@univ-paris-diderot.fr RI Bartolo, Nicola/H-6802-2014; Intravaia, Francesco/E-6500-2010 OI Bartolo, Nicola/0000-0001-8049-9611; Intravaia, Francesco/0000-0001-7993-4698 FU LANL LDRD program; University of Palermo through the PerfEst scholarship; European Union [PCIG14-GA-2013-631571]; DFG through the DIP program [FO 703/2-1] FX We thank the LANL LDRD program for financial support. N.B. thanks Los Alamos National Laboratory for its hospitality in the early stages of the project and the University of Palermo for partial funding through the PerfEst 2010 scholarship. R.M. thanks V. Parigi for useful discussions and the Center of Nonlinear Studies at Los Alamos National Laboratory for its hospitality. F.I. acknowledges financial support from the European Union Marie Curie People program through the Career Integration Grant No. PCIG14-GA-2013-631571 and from the DFG through the DIP program (FO 703/2-1). NR 63 TC 0 Z9 0 U1 3 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD APR 18 PY 2016 VL 93 IS 4 AR 042111 DI 10.1103/PhysRevA.93.042111 PG 13 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DJ9FM UT WOS:000374519400002 ER PT J AU Iacocca, E Gliga, S Stamps, RL Heinonen, O AF Iacocca, Ezio Gliga, Sebastian Stamps, Robert L. Heinonen, Olle TI Reconfigurable wave band structure of an artificial square ice SO PHYSICAL REVIEW B LA English DT Article ID SPIN ICE; MAGNONIC CRYSTALS AB Artificial square ices are structures composed of magnetic nanoelements arranged on the sites of a two-dimensional square lattice, such that there are four interacting magnetic elements at each vertex, leading to geometrical frustration. Using a semianalytical approach, we show that square ices exhibit a rich spin-wave band structure that is tunable both by external magnetic fields and the magnetization configuration of individual elements. Internal degrees of freedom can give rise to equilibrium states with bent magnetization at the element edges leading to characteristic excitations; in the presence of magnetostatic interactions these form separate bands analogous to impurity bands in semiconductors. Full-scale micromagnetic simulations corroborate our semianalytical approach. Our results show that artificial square ices can be viewed as reconfigurable and tunable magnonic crystals that can be used as metamaterials for spin-wave-based applications at the nanoscale. C1 [Iacocca, Ezio] Univ Colorado, Dept Appl Math, Boulder, CO 80309 USA. [Iacocca, Ezio] Chalmers, Div Theoret Phys, Dept Phys, S-41296 Gothenburg, Sweden. [Iacocca, Ezio] Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. [Gliga, Sebastian] ETH, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland. [Gliga, Sebastian] Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland. [Stamps, Robert L.] Univ Glasgow, Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Heinonen, Olle] Northwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. RP Iacocca, E (reprint author), Univ Colorado, Dept Appl Math, Boulder, CO 80309 USA.; Iacocca, E (reprint author), Chalmers, Div Theoret Phys, Dept Phys, S-41296 Gothenburg, Sweden.; Iacocca, E (reprint author), Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. EM ezio.iacocca@colorado.edu RI Stamps, Robert/E-7304-2011; OI Stamps, Robert/0000-0003-0713-4864; Heinonen, Olle/0000-0002-3618-6092; Iacocca, Ezio/0000-0002-8870-5106 FU Swedish Research Council [637-2014-6863]; Department of Energy Office of Science, Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division through the Materials Theory Institute; EPSRC [EP/L002922/1] FX E.I. acknowledges support from the Swedish Research Council, Reg. No. 637-2014-6863. The work by O.H. was funded by the Department of Energy Office of Science, Materials Sciences and Engineering Division. E.I. was partly supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division through the Materials Theory Institute. We gratefully acknowledge the computing resources provided on Blues, a high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. The work by R.L.S. was funded by EPSRC EP/L002922/1. NR 44 TC 6 Z9 6 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 18 PY 2016 VL 93 IS 13 AR 134420 DI 10.1103/PhysRevB.93.134420 PG 8 WC Physics, Condensed Matter SC Physics GA DJ9IV UT WOS:000374528100007 ER PT J AU Khuntia, P Kumar, R Mahajan, AV Baenitz, M Furukawa, Y AF Khuntia, P. Kumar, R. Mahajan, A. V. Baenitz, M. Furukawa, Y. TI Spin liquid state in the disordered triangular lattice Sc2Ga2CuO7 revealed by NMR SO PHYSICAL REVIEW B LA English DT Article ID KAGOME HEISENBERG-ANTIFERROMAGNET; FRUSTRATED MAGNETS; GROUND-STATE; ICE; EXCITATIONS; INSULATOR AB We present microscopic magnetic properties of a two-dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. An antiferromagnetic (AFM) exchange interaction J/k(B) approximate to 35 K between Cu2+ (S = 1/2) spins in the triangular biplane is obtained from the analysis of intrinsic magnetic susceptibility data. The intrinsic magnetic susceptibility, extracted from Ga-71 NMR shift data, displays the presence of AFM short range spin correlations and remains finite down to 50 mK, suggesting a nonsinglet ground state. The nuclear spin-lattice relaxation rate (1/T-1) reveals a slowing down of Cu2+ spin fluctuations with decreasing T down to 100 mK. Magnetic specific heat (C-m) and 1/T-1 exhibit power law behavior at low temperatures, implying the gapless nature of the spin excitation spectrum. The absence of long range magnetic ordering down to similar to J/700, nonzero spin susceptibility at low T, and the power law behavior of C-m and 1/T-1 suggest a gapless quantum spin liquid (QSL) state. Our results demonstrate that persistent spin dynamics induced by frustration maintain a quantum-disordered state at T -> 0 in this triangular lattice antiferromagnet. This suggests that the low energy modes are dominated by spinon excitations in the QSL state due to randomness engendered by disorder and frustration. C1 [Khuntia, P.; Furukawa, Y.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Kumar, R.; Mahajan, A. V.] Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. [Baenitz, M.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Furukawa, Y.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Khuntia, P.] Univ Paris 11, Phys Solides Lab, UMR CNRS 8502, F-91405 Orsay, France. RP Khuntia, P (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.; Khuntia, P (reprint author), Univ Paris 11, Phys Solides Lab, UMR CNRS 8502, F-91405 Orsay, France. EM pkhuntia@gmail.com RI Baenitz, Michael/E-4085-2016; Khuntia, Panchanan /E-4270-2010 FU European Commission through Marie Curie International Incoming Fellowship [PIIF-GA-2013-627322]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We acknowledge insightful discussions with P. Mendels, B. Koteswararao, and B. Roy. P. K. acknowledges support from the European Commission through Marie Curie International Incoming Fellowship (PIIF-GA-2013-627322). The research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 69 TC 2 Z9 2 U1 7 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 18 PY 2016 VL 93 IS 14 AR 140408 DI 10.1103/PhysRevB.93.140408 PG 6 WC Physics, Condensed Matter SC Physics GA DJ9JO UT WOS:000374530000001 ER PT J AU Martin-Garcia, L Mascaraque, A Pabon, BM Bliem, R Parkinson, GS Chen, G Schmid, AK de la Figuera, J AF Martin-Garcia, Laura Mascaraque, Arantzazu Pabon, Beatriz M. Bliem, Roland Parkinson, Gareth S. Chen, Gong Schmid, Andreas K. de la Figuera, Juan TI Spin reorientation transition of magnetite (001) SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-ELECTRON MICROSCOPY; VERWEY TRANSITION; SINGLE-CRYSTAL; ANISOTROPY; FE3O4; SURFACE AB We have imaged the rearrangement of the magnetic domains on magnetite (001) when crossing the spin reorientation transition and the Verwey transition with nanometer resolution. By means of spin-polarized low-energy electron microscopy we have monitored the change in the easy axes lowering the temperature through both transitions in remanence. The spin reorientation transition occurs in two steps: initial nucleation and growth of domains with a new surface magnetic orientation is followed by a smooth evolution. C1 [Martin-Garcia, Laura; de la Figuera, Juan] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. [Mascaraque, Arantzazu; Pabon, Beatriz M.] Univ Complutense Madrid, Dept Fis Mat, E-28040 Madrid, Spain. [Mascaraque, Arantzazu; Pabon, Beatriz M.] UCM, Unidad Asociada IQFR CSIC, E-28040 Madrid, Spain. [Bliem, Roland; Parkinson, Gareth S.] Vienna Univ Technol, Inst Appl Phys, A-1040 Vienna, Austria. [Chen, Gong; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, NCEM, Berkeley, CA 94720 USA. RP de la Figuera, J (reprint author), CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain. EM juan.delafiguera@iqfr.csic.es RI Mascaraque, Arantzazu/D-9504-2012; Chen, Gong/H-3074-2015; de la Figuera, Juan/E-7046-2010; OI Mascaraque, Arantzazu/0000-0002-2614-2862; de la Figuera, Juan/0000-0002-7014-4777; Parkinson, Gareth/0000-0003-2457-8977 FU Spanish Ministry of Economy and Competitiveness (MINECO) [MAT2011-52477-C5-2-P, MAT2012-38045-C04-01, MAT2015-64110-C2-1-P]; Austrian Science Fund START prize [Y 847-N20, P24925-N20]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; MINECO for an FPI [BES-2013-063396]; TU Wien; Austrian Science Fund [W1243]; Spanish Ministry of Education [PRX14/00307] FX We thank Dr. A. T. N'Diaye for his support with the scripts for the color representation of the magnetization. This research was partly supported by the Spanish Ministry of Economy and Competitiveness (MINECO) under Projects No. MAT2011-52477-C5-2-P, No. MAT2012-38045-C04-01, and No. MAT2015-64110-C2-1-P. G.S.P. and R.B. acknowledge funding from the Austrian Science Fund START prize Y 847-N20 and Project No. P24925-N20. Experiments were performed at the Molecular Foundry, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. L.M.-G. thanks the MINECO for an FPI contract with reference Contract No. BES-2013-063396. R.B. acknowledges a stipend from the TU Wien and Austrian Science Fund doctoral college Solids4Fun (Project No. W1243). A.M. thanks the support of the Spanish Ministry of Education through Project No. PRX14/00307. NR 40 TC 2 Z9 2 U1 15 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 18 PY 2016 VL 93 IS 13 AR 134419 DI 10.1103/PhysRevB.93.134419 PG 6 WC Physics, Condensed Matter SC Physics GA DJ9IV UT WOS:000374528100006 ER PT J AU Jia, JY Radhakrishnan, S Zhou, ML AF Jia, Jiangyong Radhakrishnan, Sooraj Zhou, Mingliang TI Forward-backward multiplicity fluctuation and longitudinal harmonics in high-energy nuclear collisions SO PHYSICAL REVIEW C LA English DT Article ID CHARGED-PARTICLE CORRELATIONS; HEAVY-ION COLLISIONS; TEV AB An analysis method is proposed to study the forward-backward (FB) multiplicity fluctuation in high-energy nuclear collisions, built on the earlier work of Bzdak and Teaney [Phys. Rev. C 87, 024906 (2013)]. The method allows the decomposition of the centrality dependence of average multiplicity from the dynamical event-by-event (EbyE) fluctuation of multiplicity in pseudorapidity. Application of the method to AMPT (A Multi-Phase Transport model) and HIJING (Heavy Ion Jet INteraction Generator) models shows that the long-range component of the FB correlation is captured by a few longitudinal harmonics, with the first component driven by the asymmetry in the number of participating nucleons in the two colliding nuclei. The higher-order longitudinal harmonics are found to be strongly damped in AMPT compared to HIJING, due to weaker short-range correlations as well as the final-state effects present in the AMPT model. Two-particle pseudorapidity correlation reveals interesting charge-dependent short-range structures that are absent in HIJING model. The proposed method opens an avenue to elucidate the particle production mechanism and early time dynamics in heavy-ion collisions. Future analysis directions and prospects of using the pseudorapidity correlation function to understand the centrality bias in p + p, p + A, and A + A collisions are discussed. C1 [Jia, Jiangyong; Radhakrishnan, Sooraj; Zhou, Mingliang] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Jia, Jiangyong] Brookhaven Natl Lab, Dept Phys, Upton, NY 11796 USA. RP Jia, JY; Zhou, ML (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Jia, JY (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11796 USA. EM jjia@bnl.gov; mingliang.zhou@stonybrook.edu FU NSF [PHY-1305037]; DOE through BNL [DE-SC0012704] FX We appreciate fruitful discussions with R. Lacey. This research is supported by NSF under Grant No. PHY-1305037 and by DOE through BNL under Contract No. DE-SC0012704. NR 46 TC 0 Z9 0 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 18 PY 2016 VL 93 IS 4 AR 044905 DI 10.1103/PhysRevC.93.044905 PG 12 WC Physics, Nuclear SC Physics GA DJ9PB UT WOS:000374544300006 ER PT J AU Kumbartzki, GJ Benczer-Koller, N Speidel, KH Torres, DA Allmond, JM Fallon, P Abramovic, I Bernstein, LA Bevins, JE Crawford, HL Guevara, ZE Gurdal, G Hurst, AM Kirsch, L Laplace, TA Lo, A Matthews, EF Mayers, I Phair, LW Ramirez, F Robinson, SJQ Sharon, YY Wiens, A AF Kumbartzki, G. J. Benczer-Koller, N. Speidel, K. -H. Torres, D. A. Allmond, J. M. Fallon, P. Abramovic, I. Bernstein, L. A. Bevins, J. E. Crawford, H. L. Guevara, Z. E. Gurdal, G. Hurst, A. M. Kirsch, L. Laplace, T. A. Lo, A. Matthews, E. F. Mayers, I. Phair, L. W. Ramirez, F. Robinson, S. J. Q. Sharon, Y. Y. Wiens, A. TI Z=50 core stability in Sn-110 from magnetic-moment and lifetime measurements SO PHYSICAL REVIEW C LA English DT Article ID SN ISOTOPES; DIPOLE; SHELL AB Background: The structure of the semimagic Sn-50 isotopes were previously studied via measurements of B(E2; 2(1)(+) -> 0(1)(+)) and g factors of 2(1)(+) states. The values of the B(E2; 2(1)(+)) in the isotopes below midshell at N = 66 show an enhancement in collectivity, contrary to predictions from shell-model calculations. Purpose: This work presents the first measurement of the 2(1)(+) and 4(1)(+) states' magnetic moments in the unstable neutron-deficient Sn-110. The g factors provide complementary structure information to the interpretation of the observed B(E2) values. Methods: The Sn-110 nuclei have been produced in inverse kinematics in an alpha-particle transfer reaction from C-12 to Cd-106 projectiles at 390, 400, and 410 MeV. The g factors have been measured with the transient field technique. Lifetimes have been determined from line shapes using the Doppler-shift attenuation method. Results: The g factors of the 2(1)(+) and 4(1)(+) states in Sn-110 are g(2(1)(+)) = +0.29(11) and g(4(1)(+)) = +0.05(14), respectively. In addition, the g(4(1)(+)) = +0.27(6) in Cd-106 has been measured for the first time. A line-shape analysis yielded tau(Sn-110;2(1)(+)) = 0.81(10) ps and a lifetime of tau(Sn-110;3(1)(-)) = 0.25(5) ps was calculated from the fully Doppler-shifted gamma line. Conclusions: No evidence has been found in Sn-110 that would require excitation of protons from the closed Z = 50 core. C1 [Kumbartzki, G. J.; Benczer-Koller, N.; Sharon, Y. Y.] Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. [Speidel, K. -H.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Torres, D. A.; Guevara, Z. E.; Ramirez, F.] Univ Nacl Colombia, Dept Fis, Carrera 30 45-03, Bogota, Colombia. [Allmond, J. M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Fallon, P.; Bernstein, L. A.; Crawford, H. L.; Hurst, A. M.; Phair, L. W.; Wiens, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Abramovic, I.; Bernstein, L. A.; Bevins, J. E.; Kirsch, L.; Laplace, T. A.; Lo, A.; Matthews, E. F.; Mayers, I.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Bernstein, L. A.; Laplace, T. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Gurdal, G.; Robinson, S. J. Q.] Millsaps Coll, Dept Phys, Jackson, MS 39210 USA. RP Kumbartzki, GJ (reprint author), Rutgers State Univ, Dept Phys & Astron, New Brunswick, NJ 08903 USA. EM kum@physics.rutgers.edu FU Deutsche Forschungsgemeinschaft [SP190/18-1]; Colciencias [110165842984-2015]; Stockton University under a Research and Professional Development award; US National Science Foundation; US Department of Energy [DE-AC02-05CH11231, DE-AC52-07NA27344] FX The authors thank the Berkeley 88-Inch Cyclotron staff for their help in setting up the experiment and providing the cadmium beam. The target was prepared by P. Maier-Komor at the Technische Universitat Munich, Germany. The authors are grateful to L. Zamick for many discussions and suggestions about the theoretical interpretation of the g factor results. K.-H.S. acknowledges support by the Deutsche Forschungsgemeinschaft under Grant No. SP190/18-1. D.A.T., Z.E.G., and F.R. acknowledge support by Colciencias under Contract No. 110165842984-2015. Y.Y.S. acknowledges support from Stockton University under a Research and Professional Development award. The work has been supported in part by the US National Science Foundation and by the US Department of Energy under Contracts No. DE-AC02-05CH11231 and No. DE-AC52-07NA27344. NR 37 TC 1 Z9 1 U1 5 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 18 PY 2016 VL 93 IS 4 AR 044316 DI 10.1103/PhysRevC.93.044316 PG 7 WC Physics, Nuclear SC Physics GA DJ9PB UT WOS:000374544300001 ER PT J AU Paquet, JF Shen, C Denicol, GS Luzum, M Schenke, B Jeon, S Gale, C AF Paquet, Jean-Francois Shen, Chun Denicol, Gabriel S. Luzum, Matthew Schenke, Bjorn Jeon, Sangyong Gale, Charles TI Production of photons in relativistic heavy-ion collisions SO PHYSICAL REVIEW C LA English DT Article ID PB-PB COLLISIONS; FRAGMENTATION FUNCTIONS; FLOW; VISCOSITY; MODELS AB In this work it is shown that the use of a hydrodynamical model of heavy-ion collisions which incorporates recent developments, together with updated photon emission rates, greatly improves agreement with both ALICE and PHENIX measurements of direct photons, supporting the idea that thermal photons are the dominant source of direct photon momentum anisotropy. The event-by-event hydrodynamical model uses the impact parameter dependent Glasma model (IP-Glasma) initial states and includes, for the first time, both shear and bulk viscosities, along with second-order couplings between the two viscosities. The effect of both shear and bulk viscosities on the photon rates is studied, and those transport coefficients are shown to have measurable consequences on the photon momentum anisotropy. C1 [Paquet, Jean-Francois; Shen, Chun; Denicol, Gabriel S.; Jeon, Sangyong; Gale, Charles] McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. [Paquet, Jean-Francois] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Denicol, Gabriel S.; Schenke, Bjorn] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Luzum, Matthew] Univ Santiago de Compostela, Dept Fis Particulas, E-15706 Santiago De Compostela, Galicia, Spain. [Luzum, Matthew] Univ Santiago de Compostela, IGFAE, E-15706 Santiago De Compostela, Galicia, Spain. [Luzum, Matthew] Univ Sao Paulo, Inst Fis, Rua Matao Travessa R 187,Cidade Univ, BR-05508090 Sao Paulo, Brazil. RP Paquet, JF (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada.; Paquet, JF (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RI Silveira Denicol, Gabriel/L-5048-2016; Luzum, Matthew/C-4986-2015 OI Luzum, Matthew/0000-0002-0367-7055 FU Natural Sciences and Engineering Research Council of Canada; DOE [DE-SC0012704]; Marie Curie Intra-European Fellowship for Career Development Grant [FP7-PEOPLE-2013-IEF-626212]; Canada Foundation for Innovation (CFI); NanoQuebec; RMGA; Fonds de recherche du Quebec-Nature et technologies (FRQ-NT); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank the organizers and participants of the "EMMI Rapid Reaction Task Force on the direct-photon flow puzzle," together with Takao Sakaguchi and Gojko Vujanovic, for fruitful discussions. The authors thank Kevin Dusling and Ismail Zahed for providing a tabulation of their photon emission rates. This work was supported in part by the Natural Sciences and Engineering Research Council of Canada. G.S.D. and B.P.S. are supported under DOE Contract No. DE-SC0012704. M.L. acknowledges support from the Marie Curie Intra-European Fellowship for Career Development Grant No. FP7-PEOPLE-2013-IEF-626212. Computations were made in part on the supercomputer Guillimin from McGill University, managed by Calcul Quebec and Compute Canada. The operation of this supercomputer is funded by the Canada Foundation for Innovation (CFI), NanoQuebec, RMGA and the Fonds de recherche du Quebec-Nature et technologies (FRQ-NT). This research also used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 78 TC 12 Z9 12 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. 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CA ATLAS Collaboration TI Search for dark matter produced in association with a Higgs boson decaying to two bottom quarks in pp collisions at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; PAIR PRODUCTION; PARTON DISTRIBUTIONS; LHC; QCD; CONSTRAINTS; RESUMMATION; PARTICLE; ZH AB This article reports on a search for dark matter pair production in association with a Higgs boson decaying to a pair of bottom quarks, using data from 20.3 fb(-1) of pp collisions at a center-of-mass energy of 8 TeV collected by the ATLAS detector at the LHC. The decay of the Higgs boson is reconstructed as a high-momentum b (b) over bar system with either a pair of small-radius jets, or a single large-radius jet with substructure. The observed data are found to be consistent with the expected Standard Model backgrounds. Model-independent upper limits are placed on the visible cross sections for events with a Higgs boson decaying into b (b) over bar and large missing transverse momentum with thresholds ranging from 150 to 400 GeV. Results are interpreted using a simplified model with a Z' gauge boson decaying into different Higgs bosons predicted in a two-Higgs-doublet model, of which the heavy pseudoscalar Higgs decays into a pair of dark matter particles. Exclusion limits are also presented for the mass scales of various effective field theory operators that describe the interaction between dark matter particles and the Higgs boson. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. 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C.; Gach, G. P.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Cerqueira, A. S.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarro, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M-A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Du, Y.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Burmeister, I.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Burmeister, I.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nackenhorst, O.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Huseynov, N.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. 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A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J-F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J-F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Annovi, A.; Antonov, A.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Pinto Firmino Da Costa, J. Goncalves; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Vlasak, M.; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Annovi, A.; Antonov, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Fac Exact Sci, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. 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RI Garcia, Jose /H-6339-2015; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; BESSON, NATHALIE/L-6250-2015; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Stabile, Alberto/L-3419-2016; Guo, Jun/O-5202-2015; Gladilin, Leonid/B-5226-2011; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Gorelov, Igor/J-9010-2015; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009 OI Pina, Joao /0000-0001-8959-5044; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Stabile, Alberto/0000-0002-6868-8329; Guo, Jun/0000-0001-8125-9433; Gladilin, Leonid/0000-0001-9422-8636; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Gorelov, Igor/0000-0001-5570-0133; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, People's Republic of China; MOST, People's Republic of China; NSFC, People's Republic of China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; Cantons of Bern, Switzerland; Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society and Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, People's Republic of China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF, and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020, and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne, and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales, and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; BSF, GIF, and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA), and in the Tier-2 facilities worldwide. NR 104 TC 0 Z9 0 U1 21 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 18 PY 2016 VL 93 IS 7 AR 072007 DI 10.1103/PhysRevD.93.072007 PG 33 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QD UT WOS:000374547100001 ER PT J AU Chen, C Chang, L Roberts, CD Wan, SL Zong, HS AF Chen, Chen Chang, Lei Roberts, Craig D. Wan, Shaolong Zong, Hong-Shi TI Valence-quark distribution functions in the kaon and pion SO PHYSICAL REVIEW D LA English DT Article ID CHIRAL-SYMMETRY BREAKING; DRELL-YAN PROCESSES; PERTURBATION-THEORY; QUANTUM CHROMODYNAMICS; PARTON DISTRIBUTIONS; EXCLUSIVE PROCESSES; FORM-FACTOR; MODEL; SCATTERING; EQUATIONS AB We describe expressions for pion and kaon dressed-quark distribution functions that incorporate contributions from gluons which bind quarks into these mesons and hence overcome a flaw of the commonly used handbag approximation. The distributions therewith obtained are purely valence in character, ensuring that dressed quarks carry all the meson's momentum at a characteristic hadronic scale and vanish as (1 - x)(2) when Bjorken-x -> 1. Comparing such distributions within the pion and kaon, it is apparent that the size of SU(3)-flavor symmetry breaking in meson parton distribution functions is modulated by the flavor dependence of dynamical chiral symmetry breaking. Corrections to these leading-order formulas may be divided into two classes, responsible for shifting dressed-quark momentum into glue and sea quarks. Working with available empirical information, we build an algebraic framework that is capable of expressing the principal impact of both classes of corrections. This enables a realistic comparison with experiment which allows us to identify and highlight basic features of measurable pion and kaon valence-quark distributions. We find that whereas roughly two thirds of the pion's light-front momentum is carried by valence dressed quarks at a characteristic hadronic scale; this fraction rises to 95% in the kaon; evolving distributions with these features to a scale typical of available Drell-Yan data produces a kaon-to-pion ratio of u-quark distributions that is in agreement with the single existing data set, and predicts a u-quark distribution within the pion that agrees with a modern reappraisal of pi N Drell-Yan data. Precise new data are essential in order to validate this reappraisal and because a single modest-quality measurement of the kaon-to-pion ratio cannot be considered definitive. C1 [Chen, Chen] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Chen, Chen; Wan, Shaolong] Univ Sci & Technol China, Inst Theoret Phys, Hefei 230026, Anhui, Peoples R China. [Chen, Chen; Wan, Shaolong] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chang, Lei] Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China. [Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Zong, Hong-Shi] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. RP Chen, C (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.; Chen, C; Wan, SL (reprint author), Univ Sci & Technol China, Inst Theoret Phys, Hefei 230026, Anhui, Peoples R China.; Chen, C; Wan, SL (reprint author), Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China.; Chang, L (reprint author), Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China.; Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.; Zong, HS (reprint author), Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. EM seracron@ustc.edu.cn; lei.chiong@gmail.com; cdroberts@anl.gov; slwan@ustc.edu.cn; zonghs@nju.edu.cn FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; Chinese Ministry of Education; National Natural Science Foundation of China [11275097, 11275180, 11475085, 11535005]; Fundamental Research Funds for the Central Universities Programme of China [WK2030040050] FX We are grateful for insightful comments and suggestions from I. C. Cloet, P. Hutauruk, C. Mezrag, S.-X. Qin and P. C. Tandy. Work supported by: the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract no. DE-AC02-06CH11357; the Chinese Ministry of Education, under the International Distinguished Professor program; the National Natural Science Foundation of China (Grants No. 11275097, No. 11275180, No. 11475085 and No. 11535005); and the Fundamental Research Funds for the Central Universities Programme of China (Grant No. WK2030040050). NR 69 TC 7 Z9 7 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 18 PY 2016 VL 93 IS 7 AR 074021 DI 10.1103/PhysRevD.93.074021 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ9QD UT WOS:000374547100006 ER PT J AU Christensen, MH Jacobsen, H Maier, TA Andersen, BM AF Christensen, Morten H. Jacobsen, Henrik Maier, Thomas A. Andersen, Brian M. TI Magnetic Fluctuations in Pair-Density-Wave Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; T-C SUPERCONDUCTORS; STRIPES; VORTICES; ORDER; SPIN AB Pair- density- wave superconductivity constitutes a novel electronic condensate proposed to be realized in certain unconventional superconductors. Establishing its potential existence is important for our fundamental understanding of superconductivity in correlated materials. Here we compute the dynamical magnetic susceptibility in the presence of a pair- density- wave ordered state and study its fingerprints on the spin- wave spectrum including the neutron resonance. In contrast to the standard case of d- wave superconductivity, we show that the pair- density- wave phase exhibits neither a spin gap nor a magnetic resonance peak, in agreement with a recent neutron scattering experiment on underdoped La1.905Ba0.095CuO4. C1 [Christensen, Morten H.; Jacobsen, Henrik; Andersen, Brian M.] Univ Copenhagen, Niels Bohr Inst, Juliane Maries Vej 30, DK-2100 Copenhagen, Denmark. [Maier, Thomas A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Maier, Thomas A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Christensen, MH (reprint author), Univ Copenhagen, Niels Bohr Inst, Juliane Maries Vej 30, DK-2100 Copenhagen, Denmark. RI Jacobsen, Henrik/B-6500-2015; Andersen, Brian /M-4671-2014; Maier, Thomas/F-6759-2012 OI Jacobsen, Henrik/0000-0001-6950-3990; Andersen, Brian /0000-0002-9786-7553; Maier, Thomas/0000-0002-1424-9996 FU Lundbeckfond Fellowship [A9318]; Center of Nanophase Materials Sciences which is a Department of Energy Office of Science User Facility FX The authors are grateful to W. A. Atkinson, P. J. Hirschfeld, A. P. Kampf, A. Kreisel, D. D. Scherer, F. Loder, N. Perkins, I. Rousochatzakis, A. T. Romer, J. Tranquada, and G. Yu for useful discussions. M. H. C. and B. M. A. acknowledge financial support from a Lundbeckfond Fellowship (Grant No. A9318). T. A. M. acknowledges support from the Center of Nanophase Materials Sciences, which is a Department of Energy Office of Science User Facility. NR 40 TC 0 Z9 0 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 18 PY 2016 VL 116 IS 16 AR 167001 DI 10.1103/PhysRevLett.116.167001 PG 5 WC Physics, Multidisciplinary SC Physics GA DJ9UM UT WOS:000374558500006 PM 27152819 ER PT J AU Lee, JH Kezsmaki, I Fishman, RS AF Lee, Jun Hee Kezsmaki, Istvan Fishman, Randy S. TI First-principles approach to the dynamic magnetoelectric couplings for the non-reciprocal directional dichroism in BiFeO3 SO NEW JOURNAL OF PHYSICS LA English DT Article DE multiferroic; directional dichroism; spin-driven polarization; first-principles calculations ID AUGMENTED-WAVE METHOD; EXCITATIONS AB Due to the complicated magnetic and crystallographic structures of BiFeO3, its magnetoelectric (ME) couplings and microscopic model Hamiltonian remain poorly understood. By employing a first-principles approach, we uncover all possible ME couplings associated with the spin-current (SC) and exchange-striction (ES) polarizations, and construct an appropriate Hamiltonian for the long-range spin-cycloid in BiFeO3. First-principles calculations are used to understand the microscopic origins of the ME couplings. We find that inversion symmetries broken by ferroelectric and antiferroelectric distortions induce the SC and the ES polarizations, which cooperatively produce the dynamic ME effects in BiFeO3. A model motivated by first principles reproduces the absorption difference of counter-propagating light beams called non-reciprocal directional dichroism. The current paper focuses on the spin-driven (SD) polarizations produced by a dynamic electric field, i.e. the dynamic ME couplings. Due to the inertial properties of Fe, the dynamic SD polarizations differ significantly from the static SD polarizations. Our systematic approach can be generally applied to any multiferroic material, laying the foundation for revealing hidden ME couplings on the atomic scale and for exploiting optical ME effects in the next generation of technological devices such as optical diodes. C1 [Lee, Jun Hee; Fishman, Randy S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Lee, Jun Hee] Ulsan Natl Inst Sci & Technol, Sch Energy & Chem Engn, Ulsan 44919, South Korea. [Kezsmaki, Istvan] Budapest Univ Technol & Econ, Dept Phys, H-1111 Budapest, Hungary. [Kezsmaki, Istvan] MTA BME Lendulet Magneto Opt Spect Res Grp, H-1111 Budapest, Hungary. RP Lee, JH (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.; Lee, JH (reprint author), Ulsan Natl Inst Sci & Technol, Sch Energy & Chem Engn, Ulsan 44919, South Korea. EM leej@ornl.gov FU US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Hungarian Research Fund [OTKA K 108918]; UNIST (Ulsan National Institute of Science and Technology) [1.150132.01] FX We acknowledge discussions with H Kim, E Bousquet, Nobuo Furukawa, S Miyahara, J Musfeldt, U Nagel, S Okamoto, S Bordacs and T Room. Research sponsored by the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. IK was supported by the Hungarian Research Fund OTKA K 108918. JHL was in part supported by the year of 2015 Research Fund (1.150132.01) of the UNIST (Ulsan National Institute of Science and Technology). We also thank Hee Taek Yi and Sang-Wook Cheong for preparation of the BiFeO3 sample. NR 43 TC 0 Z9 0 U1 5 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD APR 18 PY 2016 VL 18 AR 043025 DI 10.1088/1367-2630/18/4/043025 PG 11 WC Physics, Multidisciplinary SC Physics GA DL2LF UT WOS:000375465600003 ER PT J AU Lashley, MA Mehio, N Nugent, JW Holguin, E Do-Thanh, CL Bryantsev, VS Dai, S Hancock, RD AF Lashley, Mark A. Mehio, Nada Nugent, Joseph W. Holguin, Erick Chi-Linh Do-Thanh Bryantsev, Vyacheslav S. Dai, Sheng Hancock, Robert D. TI Amidoximes as ligand functionalities for braided polymeric materials for the recovery of uranium from seawater SO POLYHEDRON LA English DT Article DE Uranium; Extraction from ocean; Formation constants; Fluorescence; Density functional theory ID URANYL-ION; AQUEOUS-SOLUTION; METAL-IONS; SEA-WATER; ANISOTROPIC DIELECTRICS; ELECTRONIC-STRUCTURE; CRYSTAL-STRUCTURE; EXCITED-STATES; COMPLEXES; EXTRACTION AB The formation constants of the UO22+ cation with the amidoximate ligands bzam (benzamidoxime) and acetam (acetamidoxime) are reported. These are of interest in light of their proposed use as the functional groups of extractants for uranium in seawater. The formation constants of bzam with UO22+ were measured by monitoring the absorbance of the pi -> pi* transitions in the UV spectrum of the bzam ligand in the presence of 1:1 UO22+ as a function of pH. This yielded log K-1 = 12.4 for UO22+ with bzam, and log K= 6.9 for the equilibrium UO2(bzam)(+) + OH- = UO2(bzam)OH at 25 degrees C and ionic strength zero. The bzam complexes were also studied monitoring the fluorescence of the UO22+ system. Analysis of the intense fluorescence that occurs in 5 x 10(-6) M UO22+ solutions between pH 5 and 9 suggested that this was due to the [(UO2)(3)O(OH)(3)](+) trimer. Monomeric species such as UO22+ and [UO2(OH)(4)](2-), and dimers such as [(UO2)(OH)(2)](2+), fluoresce only weakly. Titration of such solutions with bzam supported the above log K values measured by absorbance, and with higher bzam concentrations yielded log beta(2) = 22.3. The acetam ligand does not have any absorbance, so that complex-formation was monitored by fluorescence only. Formation constants measured.by fluorescence may differ from those measured by other techniques such as absorbance. The agreement obtained between log K values measured by absorbance and fluorescence for the bzam complex of UO22+ supported the log K values measured for the acetam complexes by florescence alone were reliable: log K-1 = 13.6, log beta(2) = 23.7, and log K UO2(acetam)(+) + OH- = UO2(acetam) OH = 6.8. The high log K values found for the bzam and acetam complexes of UO22+ were analyzed using DFT calculations. These log K values are related to the ability of polymer-based extractants bearing bzam or acetam type functional groups to extract UO22+ at a concentration of 1.3 x 10(-8) M and in the competing 0.0025 M CO32- present in the oceans. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Lashley, Mark A.; Nugent, Joseph W.; Holguin, Erick; Hancock, Robert D.] Univ N Carolina, Dept Chem & Biochem, Wilmington, NC 28403 USA. [Mehio, Nada; Chi-Linh Do-Thanh] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Bryantsev, Vyacheslav S.; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Hancock, RD (reprint author), Univ N Carolina, Dept Chem & Biochem, Wilmington, NC 28403 USA. RI Dai, Sheng/K-8411-2015; Bryantsev, Vyacheslav/M-5111-2016; OI Dai, Sheng/0000-0002-8046-3931; Bryantsev, Vyacheslav/0000-0002-6501-6594; Holguin, Erick/0000-0001-7434-3864; Do-Thanh, Chi-Linh/0000-0003-2263-8331 FU U.S. DOE Office of Nuclear Energy FX This research was supported by the U.S. DOE Office of Nuclear Energy. NR 71 TC 5 Z9 5 U1 6 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD APR 18 PY 2016 VL 109 BP 81 EP 91 DI 10.1016/j.poly.2016.01.026 PG 11 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DL0PN UT WOS:000375335100012 ER PT J AU Stonebloom, S Ebert, B Xiong, GY Pattathil, S Birdseye, D Lao, JM Pauly, M Hahn, MG Heazlewood, JL Scheller, HV AF Stonebloom, Solomon Ebert, Berit Xiong, Guangyan Pattathil, Sivakumar Birdseye, Devon Lao, Jeemeng Pauly, Markus Hahn, Michael G. Heazlewood, Joshua L. Scheller, Henrik Vibe TI A DUF-246 family glycosyltransferase-like gene affects male fertility and the biosynthesis of pectic arabinogalactans SO BMC PLANT BIOLOGY LA English DT Article DE Arabidopsis thaliana; Nicotiana benthamiana; Cell wall; Rhamnogalacturonan-I; Pectin; Pollen tube ID PLANT-CELL WALLS; RHAMNOGALACTURONAN-II; ARABIDOPSIS-THALIANA; IDENTIFICATION; PROTEIN; POLLEN; GROWTH; GALACTOSYLTRANSFERASE; POLYSACCHARIDE; XYLOSYLTRANSFERASE AB Background: Pectins are a group of structurally complex plant cell wall polysaccharides whose biosynthesis and function remain poorly understood. The pectic polysaccharide rhamnogalacturonan-I (RG-I) has two types of arabinogalactan side chains, type-I and type-II arabinogalactans. To date few enzymes involved in the biosynthesis of pectin have been described. Here we report the identification of a highly conserved putative glycosyltransferase encoding gene, Pectic ArabinoGalactan synthesis-Related (PAGR), affecting the biosynthesis of RG-I arabinogalactans and critical for pollen tube growth. Results: T-DNA insertions in PAGR were identified in Arabidopsis thaliana and were found to segregate at a 1: 1 ratio of heterozygotes to wild type. We were unable to isolate homozygous pagr mutants as pagr mutant alleles were not transmitted via pollen. In vitro pollen germination assays revealed reduced rates of pollen tube formation in pollen from pagr heterozygotes. To characterize a loss-of-function phenotype for PAGR, the Nicotiana benthamiana orthologs, NbPAGR-A and B, were transiently silenced using Virus Induced Gene Silencing. NbPAGR-silenced plants exhibited reduced internode and petiole expansion. Cell wall materials from NbPAGR-silenced plants had reduced galactose content compared to the control. Immunological and linkage analyses support that RG-I has reduced type-I arabinogalactan content and reduced branching of the RG-I backbone in NbPAGR-silenced plants. Arabidopsis lines overexpressing PAGR exhibit pleiotropic developmental phenotypes and the loss of apical dominance as well as an increase in RG-I type-II arabinogalactan content. Conclusions: Together, results support a function for PAGR in the biosynthesis of RG-I arabinogalactans and illustrate the essential roles of these polysaccharides in vegetative and reproductive plant growth. C1 [Stonebloom, Solomon; Ebert, Berit; Birdseye, Devon; Lao, Jeemeng; Heazlewood, Joshua L.; Scheller, Henrik Vibe] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Stonebloom, Solomon; Ebert, Berit; Birdseye, Devon; Lao, Jeemeng; Heazlewood, Joshua L.; Scheller, Henrik Vibe] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn, Berkeley, CA 94720 USA. [Stonebloom, Solomon; Ebert, Berit] Univ Copenhagen, Fac Sci, Dept Plant & Environm Sci, DK-1871 Copenhagen C, Denmark. [Xiong, Guangyan; Pauly, Markus] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Xiong, Guangyan; Pauly, Markus; Scheller, Henrik Vibe] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Pattathil, Sivakumar; Hahn, Michael G.] Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. [Pattathil, Sivakumar; Hahn, Michael G.] Univ Georgia, BioEnergy Sci Ctr, Athens, GA 30602 USA. [Hahn, Michael G.] Univ Georgia, Dept Plant Biol, Athens, GA 30602 USA. [Heazlewood, Joshua L.] Univ Melbourne, Sch Bot, ARC Ctr Excellence Plant Cell Walls, Melbourne, Vic 3010, Australia. RP Scheller, HV (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA.; Scheller, HV (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn, Berkeley, CA 94720 USA.; Scheller, HV (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM hscheller@lbl.gov RI Heazlewood, Joshua/A-2554-2008; Pauly, Markus/B-5895-2008; Scheller, Henrik/A-8106-2008 OI Heazlewood, Joshua/0000-0002-2080-3826; Pauly, Markus/0000-0002-3116-2198; Scheller, Henrik/0000-0002-6702-3560 FU U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Danish Strategic Research Council [Set4Future 11-116795]; United States National Science Foundation Plant Genome Program [DBI-0421683, IOS-0923992] FX This work was supported by the U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U. S. Department of Energy. Part of the work was supported by the Danish Strategic Research Council (Set4Future 11-116795). The generation of the CCRC series of plant cell wall glycan-directed monoclonal antibodies used for ELISA screening in this work was supported by the United States National Science Foundation Plant Genome Program (DBI-0421683 and IOS-0923992). NR 62 TC 0 Z9 0 U1 3 U2 9 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2229 J9 BMC PLANT BIOL JI BMC Plant Biol. PD APR 18 PY 2016 VL 16 AR 90 DI 10.1186/s12870-016-0780-x PG 17 WC Plant Sciences SC Plant Sciences GA DJ5XV UT WOS:000374285000002 PM 27091363 ER PT J AU Mukai, T Englert, M Tripp, HJ Miller, C Ivanova, NN Rubin, EM Kyrpides, NC Soll, D AF Mukai, Takahito Englert, Markus Tripp, H. James Miller, Corwin Ivanova, Natalia N. Rubin, Edward M. Kyrpides, Nikos C. Soell, Dieter TI Facile Recoding of Selenocysteine in Nature SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE genetic code; metagenome; selenocysteine; sense codon recoding; synthetic biology ID ESCHERICHIA-COLI; GENETIC-CODE; FORMATE DEHYDROGENASE; TRANSFER-RNA; INSERTION; GEODERMATOPHILUS; IDENTIFICATION; REDUCTASE; SELENIUM; SYSTEM AB Selenocysteine (Sec or U) is encoded by UGA, a stop codon reassigned by a Sec-specific elongation factor and a distinctive RNA structure. To discover possible code variations in extant organisms we analyzed 6.4trillion base pairs of metagenomic sequences and 24903 microbial genomes for tRNA(Sec) species. As expected, UGA is the predominant Sec codon in use. We also found tRNA(Sec) species that recognize the stop codons UAG and UAA, and ten sense codons. Selenoprotein synthesis programmed by UAG in Geodermatophilus and Blastococcus, and by the Cys codon UGU in Aeromonas salmonicida was confirmed by metabolic labeling with Se-75 or mass spectrometry. Other tRNA(Sec) species with different anticodons enabled E.coli to synthesize active formate dehydrogenaseH, a selenoenzyme. This illustrates the ease by which the genetic code may evolve new coding schemes, possibly aiding organisms to adapt to changing environments, and show the genetic code is much more flexible than previously thought. C1 [Mukai, Takahito; Englert, Markus; Miller, Corwin; Soell, Dieter] Yale Univ, Dept Mol Biophys & Biochem, New Haven, CT 06520 USA. [Soell, Dieter] Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. [Tripp, H. James; Ivanova, Natalia N.; Rubin, Edward M.; Kyrpides, Nikos C.] Dept Energy Joint Genome Inst DOE JGI, Walnut Creek, CA 94598 USA. RP Soll, D (reprint author), Yale Univ, Dept Mol Biophys & Biochem, New Haven, CT 06520 USA. EM dieter.soll@yale.edu RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 FU National Institute for General Medical Sciences [GM22854]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the Department of Energy [DE-FG02-98ER20311]; DOE Office of Science User Facility [DE-AC02-05CH11231] FX We thank Hans Aerni and Jesse Rinehart for advice on LC-MS/MS and Jean Kanyo (Yale University) for the dedicated efforts on the MS analyses. We also thank Andreas Brune, Filipa Gody-Vitorino, Hans-Peter Klenk, Ryan Lynch, Katherine McMahon, Daniel Marcus, William Mohn, Len Pennacchio, and Ameet Pinto for permission to use unpublished sequence data produced through the DOE-JGI's community sequencing program. We are grateful to Patrick O'Donoghue, Oscar Vargas-Rodriguez, Jiqiang Ling for enlightened discussions and Daniel Drell and Robert Stack for encouragement. This work was supported by grants from the National Institute for General Medical Sciences (GM22854 to D.S.) and from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the Department of Energy (DE-FG02-98ER20311 to D.S.; for funding the genetic experiments). The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, was supported under Contract No. DE-AC02-05CH11231. NR 34 TC 10 Z9 10 U1 8 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD APR 18 PY 2016 VL 55 IS 17 BP 5337 EP 5341 DI 10.1002/anie.201511657 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DJ9WP UT WOS:000374564300041 PM 26991476 ER PT J AU Bagwell, CE Abernathy, A Barnwell, R Milliken, CE Noble, PA Dale, T Beauchesne, KR Moeller, PDR AF Bagwell, Christopher E. Abernathy, Amanda Barnwell, Remy Milliken, Charles E. Noble, Peter A. Dale, Taraka Beauchesne, Kevin R. Moeller, Peter D. R. TI Discovery of Bioactive Metabolites in Biofuel Microalgae That Offer Protection against Predatory Bacteria SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE microalgae; bioactive metabolites; iron; crop protection; predation ID MARINE CHEMICAL ECOLOGY; PREVENT POND CRASHES; HARMFUL ALGAL BLOOMS; FRESH-WATER; CHLORELLA-VULGARIS; PRYMNESIUM-PARVUM; SECONDARY METABOLITES; GROWTH-RATE; GREEN-ALGA; IRON AB Microalgae could become an important resource for addressing increasing global demand for food, energy, and commodities while helping to reduce atmospheric greenhouse gasses. Even though Chlorophytes are generally regarded safe for human consumption, there is still much we do not understand about the metabolic and biochemical potential of microscopic algae. The aim of this study was to evaluate biofuel candidate strains of Chlorella and Scenedesmus for the potential to produce bioactive metabolites when grown under nutrient depletion regimes intended to stimulate production of triacylglycerides. Strain specific combinations of macro- and micro nutrient restricted growth media did stimulate neutral lipid accumulation by microalgal cultures. However, cultures that were restricted for iron consistently and reliably tested positive for cytotoxicity by in vivo bioassays. The addition of iron back to these cultures resulted in the disappearance of the bioactive components by LC/MS fingerprinting and loss of cytotoxicity by in vivo bioassay. Incomplete NMR characterization of the most abundant cytotoxic fractions suggested that small molecular weight peptides and glycosides could be responsible for Chlorella cytotoxicity. Experiments were conducted to determine if the bioactive metabolites induced by Fe-limitation in Chlorella sp. cultures would elicit protection against Vampirovibrio chlorellavorus, an obligate predator of Chlorella. Introduction of V chlorellavorus resulted in a 72% decrease in algal biomass in the experimental controls after 7 days. Conversely, only slight losses of algal biomass were measured for the iron limited Chlorella cultures (0-9%). This study demonstrates a causal linkage between iron bioavailability and bioactive metabolite production in strains of Chlorella and Scenedesmus. Further study of this phenomenon could contribute to the development of new strategies to extend algal production cycles in open, outdoor systems while ensuring the protection of biomass from predatory losses. C1 [Bagwell, Christopher E.; Abernathy, Amanda; Barnwell, Remy; Milliken, Charles E.] Savannah River Natl Lab, Environm Sci & Biotechnol, Aiken, SC USA. [Noble, Peter A.] Alabama State Univ, Dept Biol Sci, Montgomery, AL 36101 USA. [Dale, Taraka] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Beauchesne, Kevin R.; Moeller, Peter D. R.] NOAA, Natl Ctr Coastal Ocean Sci, Ctr Human Hlth Res, Hollings Marine Lab, Charleston, SC USA. RP Bagwell, CE (reprint author), Savannah River Natl Lab, Environm Sci & Biotechnol, Aiken, SC USA. EM christopher.bagwell@srnl.doe.gov OI Noble, Peter/0000-0002-6013-2588 FU SRNL's Laboratory Directed Research and Development Program; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Biomass Program [DE-NL0022905] FX This research was jointly supported by the SRNL's Laboratory Directed Research and Development Program and the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Biomass Program (Award # DE-NL0022905). NR 74 TC 0 Z9 0 U1 12 U2 32 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 18 PY 2016 VL 7 AR 516 DI 10.3389/fmicb.2016.00516 PG 12 WC Microbiology SC Microbiology GA DJ5SS UT WOS:000374271000001 PM 27148205 ER PT J AU Bible, AN Fletcher, SJ Pelletier, DA Schadt, CW Jawdy, SS Weston, DJ Engle, NL Tschaplinski, T Masyuko, R Polisetti, S Bohn, P Coutinho, TA Doktycz, MJ Morrell-Falvey, JL AF Bible, Amber N. Fletcher, Sarah J. Pelletier, Dale A. Schadt, Christopher W. Jawdy, Sara S. Weston, David J. Engle, Nancy L. Tschaplinski, Timothy Masyuko, Rachel Polisetti, Sneha Bohn, Paulw. Coutinho, Teresa A. Doktycz, Mitchel J. Morrell-Falvey, Jennifer L. TI A Carotenoid-Deficient Mutant in Pantoea sp YR343, a Bacteria Isolated from the Rhizosphere of Populus deltoides, Is Defective in Root Colonization SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Pantoea; carotenoids; crtB; indole-3-acetic acid; poplar; rhizosphere; zeaxanthin ID PLANT-GROWTH PROMOTION; ACID AMINOTRANSFERASE ACTIVITIES; STEWARTII SUBSP STEWARTII; PSEUDOMONAS-FLUORESCENS; AZOSPIRILLUM-BRASILENSE; ERWINIA-HERBICOLA; OXIDATIVE BURST; GLUCONACETOBACTER-DIAZOTROPHICUS; SUPEROXIDE-DISMUTASE; RAMAN-SPECTROSCOPY AB The complex interactions between plants and their microbiome can have a profound effect on the health and productivity of the plant host. A better understanding of the microbial mechanisms that promote plant health and stress tolerance will enable strategies for improving the productivity of economically important plants. Pantoea sp. YR343 is a motile, rod-shaped bacterium isolated from the roots of Populus deltoides that possesses the ability to solubilize phosphate and produce the phytohormone indole-3-acetic acid (IAA). Pantoea sp. YR343 readily colonizes plant roots and does not appear to be pathogenic when applied to the leaves or roots of selected plant hosts. To better understand the molecular mechanisms involved in plant association and rhizosphere survival by Pantoea sp. YR343, we constructed a mutant in which the crtB gene encoding phytoene synthase was deleted. Phytoene synthase is responsible for converting geranylgeranyl pyrophosphate to phytoene, an important precursor to the production of carotenoids. As predicted, the Delta crtB mutant is defective in carotenoid production, and shows increased sensitivity to oxidative stress. Moreover, we find that the Delta crtB mutant is impaired in biofilm formation and production of IAA. Finally we demonstrate that the Delta crtB mutant shows reduced colonization of plant roots. Taken together, these data suggest that carotenoids are important for plant association and/or rhizosphere survival in Pantoea sp. YR343. C1 [Bible, Amber N.; Fletcher, Sarah J.; Pelletier, Dale A.; Schadt, Christopher W.; Jawdy, Sara S.; Weston, David J.; Engle, Nancy L.; Tschaplinski, Timothy; Doktycz, Mitchel J.; Morrell-Falvey, Jennifer L.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Masyuko, Rachel; Polisetti, Sneha; Bohn, Paulw.] Univ Notre Dame, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA. [Coutinho, Teresa A.] Univ Pretoria, Dept Microbiol & Plant Pathol, Forestry & Agr Biotechnol Inst, ZA-0002 Pretoria, South Africa. RP Morrell-Falvey, JL (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. EM morrelljl1@ornl.gov RI Morrell-Falvey, Jennifer/A-6615-2011; Doktycz, Mitchel/A-7499-2011; Coutinho, Teresa/B-1644-2008; Schadt, Christopher/B-7143-2008; OI Morrell-Falvey, Jennifer/0000-0002-9362-7528; Doktycz, Mitchel/0000-0003-4856-8343; Schadt, Christopher/0000-0001-8759-2448; Tschaplinski, Timothy/0000-0002-9540-6622; Engle, Nancy/0000-0003-0290-7987 FU Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research; DOE [SC0006642]; Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy FX The authors would like to acknowledge Dr. Gladys Alexandre (University of Tennessee, Knoxville) for experimental advice and supplying the pK18mob-sacB vector as well as supplying wheat seeds obtained from the University of Tennessee, Knoxville. We would also like to acknowledge Justin Jagodinski for his preliminary work characterizing the Delta crtB mutant. This research was sponsored by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Work at the University of Notre Dame was supported by DOE grant SC0006642 (RM) and by a subcontract from Oak Ridge National Laboratory (SP). This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 93 TC 1 Z9 1 U1 6 U2 14 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 18 PY 2016 VL 7 AR 491 DI 10.3389/fmicb.2016.00491 PG 15 WC Microbiology SC Microbiology GA DJ5SD UT WOS:000374269500001 PM 27148182 ER PT J AU Shen, H Zhu, WX Li, Y Tamura, N Chen, K AF Shen, Hao Zhu, Wenxin Li, Yao Tamura, Nobumichi Chen, Kai TI In situ synchrotron study of electromigration induced grain rotations in Sn solder joints SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY MICRODIFFRACTION; MECHANICAL-PROPERTIES; LAUE MICRODIFFRACTION; PLASTIC-DEFORMATION; TIN WHISKERS; THIN-FILMS; MICROSTRUCTURE; SIZE; NANOSTRUCTURES; INTERCONNECT AB Here we report an in situ study of the early stage of microstructure evolution induced by electromigration in a Pb-free beta-Sn based solder joint by synchrotron polychromatic X-ray microdiffraction. With this technique, crystal orientation evolution is monitored at intragranular levels with high spatial and angular resolution. During the entire experiment, no crystal growth is detected, and rigid grain rotation is observed only in the two grains within the current crowding region, where high density and divergence of electric current occur. Theoretical calculation indicates that the trend of electrical resistance drop still holds under the present conditions in the grain with high electrical resistivity, while the other grain with low resistivity reorients to align its a-axis more parallel with the ones of its neighboring grains. A detailed study of dislocation densities and subgrain boundaries suggests that grain rotation in beta-Sn, unlike grain rotation in high melting temperature metals which undergo displacive deformation, is accomplished via diffusional process mainly, due to the high homologous temperature. C1 [Shen, Hao; Zhu, Wenxin; Li, Yao; Chen, Kai] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Ctr Adv Mat Performance Nanoscale CAMP Nano, Xian 710049, Shaanxi, Peoples R China. [Tamura, Nobumichi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Chen, K (reprint author), Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Ctr Adv Mat Performance Nanoscale CAMP Nano, Xian 710049, Shaanxi, Peoples R China. EM kchenlbl@gmail.com RI Chen, Kai/O-5662-2014; xjtu, campnano/Q-1904-2015 OI Chen, Kai/0000-0002-4917-4445; FU National Natural Science Foundation of China [51302207]; Fundamental Research Funds for the Central Universities [2015gjhz03]; National Young 1000 Talents Program of China; Office of Science, Office of Basic Energy Sciences, Materials Science Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; International Joint Laboratory for Micro/Nano Manufacturing and Measurement Technologies; Collaborative Innovation Center of High-End Manufacturing Equipment FX This work is supported by the National Natural Science Foundation of China (Grant No. 51302207), the Fundamental Research Funds for the Central Universities (Grant No. 2015gjhz03), and the National Young 1000 Talents Program of China. We also appreciate the support from the International Joint Laboratory for Micro/Nano Manufacturing and Measurement Technologies and Collaborative Innovation Center of High-End Manufacturing Equipment. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 at LBNL. NR 41 TC 1 Z9 1 U1 10 U2 32 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 18 PY 2016 VL 6 AR 24418 DI 10.1038/srep24418 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ5EA UT WOS:000374228400001 PM 27086863 ER PT J AU White, AF Heide, CJ Saalfrank, P Head-Gordon, M Luppi, E AF White, Alec F. Heide, Chiara Josephine Saalfrank, Peter Head-Gordon, Martin Luppi, Eleonora TI Computation of high-harmonic generation spectra of the hydrogen molecule using time-dependent configuration-interaction SO MOLECULAR PHYSICS LA English DT Article DE High-harmonic generation; strong field; time-dependent configuration interaction ID GAUSSIAN-BASIS SETS; ULTRAFAST SCIENCE; ATTOSECOND; FEMTOSECOND; IONIZATION; ORBITALS; DYNAMICS; PULSES; SINGLE; FIELDS AB Here we apply and expand the knowledge developed in the case of the H atom to describe high-harmonic generation (HHG) for the H-2 molecule by using time-dependent configuration interaction with single excitations. The implications of using a finite atomic orbital basis set and the impact of a heuristic lifetime model which addresses ionisation losses are discussed. We also examine the influence of the angular momentum of the basis on the computed HHG spectra. Moreover, we discuss the impact of adding diffuse functions and ghost atoms in different geometrical configurations around the molecule. The effects of these additional centres on the HHG spectra are correlated with the physical interpretation of this nonlinear optical phenomenon as given by the three-step model, relating the maximal radial extent of the electron as predicted by the model to the radial extent of the Gaussian basis sets. [GRAPHICS] . C1 [White, Alec F.; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Kenneth S Pitzer Ctr Theoret Chem, Berkeley, CA 94720 USA. [White, Alec F.; Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Heide, Chiara Josephine] Univ Potsdam, Inst Chem, Theoret Chem, Potsdam, Germany. [Saalfrank, Peter; Luppi, Eleonora] Univ Paris 06, Sorbonne Univ, Chim Theor Lab, UMR 7616, Paris, France. [Luppi, Eleonora] CNRS, Chim Theor Lab, UMR 7616, Paris, France. RP Luppi, E (reprint author), Univ Paris 06, Sorbonne Univ, Chim Theor Lab, UMR 7616, Paris, France.; Luppi, E (reprint author), CNRS, Chim Theor Lab, UMR 7616, Paris, France. EM eleonora.luppi@upmc.fr FU France Berkeley Fund [FBF 2014-0020]; Office of Science, Office of Basic Energy Sciences, the US Department of Energy [DE-AC02- 05CH11231] FX France Berkeley Fund [Grant Number FBF 2014-0020]; Office of Science, Office of Basic Energy Sciences, the US Department of Energy: Contract No. DE-AC02- 05CH11231. NR 46 TC 4 Z9 4 U1 4 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD APR 17 PY 2016 VL 114 IS 7-8 SI SI BP 947 EP 956 DI 10.1080/00268976.2015.1119900 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ1EW UT WOS:000373947100007 ER PT J AU Levy, M Zahariev, F AF Levy, Mel Zahariev, Federico TI On augmented Kohn-Sham potential for energy as a simple sum of orbital energies SO MOLECULAR PHYSICS LA English DT Article DE Coordinate scaling; density functional; effective potential; Kohn-Sham; virial ID FUNCTIONALS AB We have recently observed that the ground-state energy may be obtained directly as a simple sum of augmented Kohn-Sham orbital energies, where it was ascertained that the corresponding one-body shifted Kohn-Sham effective potential has appealing features. With this in mind, eigenvalue and virial constraints are deduced for approximating this potential. [GRAPHICS] . C1 [Levy, Mel] Duke Univ, Dept Chem, Durham, NC 27706 USA. [Levy, Mel] N Carolina Agr & Tech State Univ, Dept Phys, Greensboro, NC 27411 USA. [Levy, Mel] Tulane Univ, Dept Chem, New Orleans, LA 70118 USA. [Levy, Mel] Tulane Univ, Quantum Theory Grp, New Orleans, LA 70118 USA. [Zahariev, Federico] Iowa State Univ, Dept Chem, Ames, IA USA. [Zahariev, Federico] Iowa State Univ, Ames Lab, Ames, IA USA. RP Levy, M (reprint author), Duke Univ, Dept Chem, Durham, NC 27706 USA.; Levy, M (reprint author), N Carolina Agr & Tech State Univ, Dept Phys, Greensboro, NC 27411 USA.; Levy, M (reprint author), Tulane Univ, Dept Chem, New Orleans, LA 70118 USA.; Levy, M (reprint author), Tulane Univ, Quantum Theory Grp, New Orleans, LA 70118 USA.; Zahariev, F (reprint author), Iowa State Univ, Dept Chem, Ames, IA USA.; Zahariev, F (reprint author), Iowa State Univ, Ames Lab, Ames, IA USA. EM mlevy@tulane.edu; fzahari@iastate.edu FU National Science Foundation from the SI2 Grant [CHEM-1047772] FX The authors thank the National Science Foundation for support from the SI2 Grant No. CHEM-1047772. NR 7 TC 2 Z9 2 U1 1 U2 2 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0026-8976 EI 1362-3028 J9 MOL PHYS JI Mol. Phys. PD APR 17 PY 2016 VL 114 IS 7-8 SI SI BP 1162 EP 1164 DI 10.1080/00268976.2016.1153743 PG 3 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ1EW UT WOS:000373947100028 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehle, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakir, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Cleland, W Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N De Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV Dearnaley, WJ Debbe, R 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Zaidan, R. Zaitsev, A. M. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena in events with at least three photons collected in pp collisions at root s=8 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID Z-BOSON DECAY; LHC AB Results of a search for new phenomena in events with at least three photons are reported. Data from proton-proton collisions at a centre-of-mass energy of 8 TeV, corresponding to an integrated luminosity of 20.3 fb(-1), were collected with the ATLAS detector at the LHC. The observed data are well described by the Standard Model. Limits at the 95 % confidence level on new phenomena are presented based on the rate of events in an inclusive signal region and a restricted signal region targeting the rare decay Z -> 3 gamma, as well as di-photon and tri-photon resonance searches. For a Standard Model Higgs boson decaying to four photons via a pair of intermediate pseudoscalar particles ( a), limits are found to be sigma xBR( h -> aa) xBR(a -> gamma gamma) 2 < 10(-3) sigma(SM) for 10 GeV < m(a) < 62 GeV. Limits are also presented for Higgs boson-like scalars (H) for m(H) > 125 GeV, and for a Z' decaying to three photons via Z' -> a + gamma -> 3 gamma. Additionally, the observed limit on the branching ratio of the Z boson decay to three photons is found to be BR( Z -> 3 gamma) < 2.2 x 10(-6), a result five times stronger than the previous result from LEP. C1 [Gonzalez, B. Alvarez; Armbruster, A. J.; Boveia, A.; Catinaccio, A.; Cattai, A.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dudarev, A.; Gorini, B.; Correia, A. M. Henriques; Hoecker, A.; Jenni, P.; Krasznahorkay, A.; Lapoire, C.; Lenzi, B.; Mandelli, B.; Marzin, A.; Milic, A.; Nairz, A. M.; Nicquevert, B.; Petersen, B. A.; Poppleton, A.; Rembser, C.; Ruiz-Martinez, A.; Salzburger, A.; Serfon, C.; Sfyrla, A.; Tricoli, A.; ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Davies, E.; Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS, IN2P3, LAPP, Annecy Le Vieux, France. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Sauvage, G.; Sauvan, E.; Simard, O.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] Univ Savoie Mont Blanc, Annecy Le Vieux, France. [Blair, R. E.; Chekanov, S.; Feng, E. J.; LeCompte, T.; Love, J.; Malon, D.; Nguyen, D. H.; Paramonov, A.; Price, L. E.; Proudfoot, J.; van Gemmeren, P.; Vaniachine, A.; Wang, R.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Lampen, C. L.; Lampl, W.; Lei, X.; Leone, R.; Loch, P.; Nayyar, R.; O'grady, F.; Rutherfoord, J. P.; Shupe, M. A.; Varnes, E. W.; Veatch, J.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Bullock, D.; Cote, D.; Darmora, S.; De, K.; Farbin, A.; Feremenga, L.; Griffiths, J.; Hadavand, H. K.; Heelan, L.; Kim, H. Y.; Ozturk, N.; Schovancova, J.; Sosebee, M.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Angelidakis, S.; Chouridou, S.; Fassouliotis, D.; Giokaris, N.; Ioannou, P.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tsirintanis, N.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Benekos, N.; Dris, M.; Gazis, E. N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lewis, A.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Aloisio, A.; Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Lewis, A.; Lopez Paz, I.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin Dit; Namasivayam, H.; Rosendahl, P. L.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Gabrielli, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Marshall, Z.; Ohm, C. 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[Bella, L. Aperio; Baca, M. J.; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Manghia, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romanoa, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romanoa, M.; Sbrizzi, A.; Sidoti, A.; Sioli, M.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mercurio, K. 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M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Merritt, F. S.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. 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[Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. 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S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Experimentelle Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Liu, M.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehle, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mergelmeyer, S.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Langa, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pokfulam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Ye, S.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Aloisio, A.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Schultz-Coulon, H. -C.; Serre, T.; Talby, M.; TicseTorres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Schultz-Coulon, H. -C.; Serre, T.; Talby, M.; TicseTorres, R. E.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Sekula, S. J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Laria, T.; Mandelli, L.; Mazza, S. M.; Merola, L.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Annovi, A.; Antonov, A.; Artamonov, A.; Basalaev, A.; Bellerive, A.; Borisov, A.; Boveia, A.; Campoverde, A.; Carminati, L.; Cervelli, A.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Mermod, P.; Perrella, S.; Rossi, E.; Sanche, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Mermod, P.; Perrella, S.; Rossi, E.; Sanche, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Knig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanov, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Aielli, G.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanzaa, A.; Livan, M.; Negria, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negria, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Sargedas De Sousa, M. J. Da Cunha; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Sargedas De Sousa, M. J. Da Cunha; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Onofre, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Onofre, A.] Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Reseau Univ Phys Hautes Energies, Univ Hassan 2, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; LeBlanc, M.; Maiani, C.; Maneira, J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM, IRFU Inst Rech Lois Fondament Univ, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinsk, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.; Leeb, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milsteada, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milsteada, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Aloisio, A.; Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. 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[Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schoute, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. 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L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroemer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Carli, Ina/C-2189-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Gladilin, Leonid/B-5226-2011; Tikhomirov, Vladimir/M-6194-2015; Guo, Jun/O-5202-2015; Gorelov, Igor/J-9010-2015; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Villa, Mauro/C-9883-2009; Kantserov, Vadim/M-9761-2015; Ventura, Andrea/A-9544-2015; Mitsou, Vasiliki/D-1967-2009; Warburton, Andreas/N-8028-2013 OI Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Carli, Ina/0000-0002-0411-1141; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Gladilin, Leonid/0000-0001-9422-8636; Tikhomirov, Vladimir/0000-0002-9634-0581; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Villa, Mauro/0000-0002-9181-8048; Kantserov, Vadim/0000-0001-8255-416X; Ventura, Andrea/0000-0002-3368-3413; Mitsou, Vasiliki/0000-0002-1533-8886; Warburton, Andreas/0000-0002-2298-7315 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; RGC, Hong Kong SAR, China; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; HGF, Germany; Canton of Geneva, Switzerland FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; RGC, Hong Kong SAR, China; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 46 TC 2 Z9 2 U1 20 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 16 PY 2016 VL 76 IS 4 AR 210 DI 10.1140/epjc/s10052-016-4034-8 PG 26 WC Physics, Particles & Fields SC Physics GA DL0FK UT WOS:000375307600001 PM 28260974 ER PT J AU Li, JX Ni, BB Ma, QL Xie, L Pu, ZY Fu, SY Thorne, RM Bortnik, J Chen, LJ Li, W Baker, DN Kletzing, CA Kurth, WS Hospodarsky, GB Fennell, JF Reeves, GD Spence, HE Funsten, HO Summers, D AF Li, Jinxing Ni, Binbin Ma, Qianli Xie, Lun Pu, Zuyin Fu, Suiyan Thorne, Richard M. Bortnik, Jacob Chen, Lunjin Li, Wen Baker, Daniel N. Kletzing, Craig A. Kurth, William S. Hospodarsky, George B. Fennell, Joseph F. Reeves, Geoffrey D. Spence, Harlan E. Funsten, Herbert O. Summers, Danny TI Formation of energetic electron butterfly distributions by magnetosonic waves via Landau resonance SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID RADIATION-BELT ELECTRONS; PITCH-ANGLE DISTRIBUTIONS; VAN-ALLEN BELT; RELATIVISTIC ELECTRONS; GEOMAGNETIC STORMS; EQUATORIAL NOISE; ACCELERATION; MAGNETOSPHERE; EVOLUTION AB Radiation belt electrons can exhibit different types of pitch angle distributions in response to various magnetospheric processes. Butterfly distributions, characterized by flux minima at pitch angles around 90 degrees, are broadly observed in both the outer and inner belts and the slot region. Butterfly distributions close to the outer magnetospheric boundary have been attributed to drift shell splitting and losses to the magnetopause. However, their occurrence in the inner belt and the slot region has hitherto not been resolved. By analyzing the particle and wave data collected by the Van Allen Probes during a geomagnetic storm, we combine test particle calculations and Fokker-Planck simulations to reveal that scattering by equatorial magnetosonic waves is a significant cause for the formation of energetic electron butterfly distributions in the inner magnetosphere. Another event shows that a large-amplitude magnetosonic wave in the outer belt can create electron butterfly distributions in just a few minutes. C1 [Li, Jinxing; Xie, Lun; Pu, Zuyin; Fu, Suiyan] Peking Univ, Inst Space Phys & Appl Technol, Beijing 100871, Peoples R China. [Li, Jinxing; Ma, Qianli; Thorne, Richard M.; Bortnik, Jacob; Li, Wen] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Ni, Binbin] Wuhan Univ, Sch Elect Informat, Dept Space Phys, Wuhan 430072, Peoples R China. [Chen, Lunjin] Univ Texas Dallas, WB Hanson Ctr Space Sci, Dept Phys, Richardson, TX 75083 USA. [Baker, Daniel N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Kletzing, Craig A.; Kurth, William S.; Hospodarsky, George B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Fennell, Joseph F.] Aerosp Corp, Space Sci Applicat Lab, El Segundo, CA 90245 USA. [Reeves, Geoffrey D.] Univ Calif Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Spence, Harlan E.] Univ New Hampshire, Each Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Funsten, Herbert O.] Univ Calif Los Alamos Natl Lab, Los Alamos, NM USA. [Summers, Danny] Mem Univ Newfoundland, Dept Math & Stat, St John, NF A1C 5S7, Canada. RP Xie, L (reprint author), Peking Univ, Inst Space Phys & Appl Technol, Beijing 100871, Peoples R China.; Ni, BB (reprint author), Wuhan Univ, Sch Elect Informat, Dept Space Phys, Wuhan 430072, Peoples R China. EM bbni@whu.edu.cn; xielun@pku.edu.cn OI Ma, Qianli/0000-0001-5452-4756; Reeves, Geoffrey/0000-0002-7985-8098 FU NSFC [41374166, 41274167, 41204120, 41474141]; Chinese Key Research Project [2011CB811404]; JHU/APL [967399, 921647, NAS5-01072]; EMFISIS [1001057397:01]; ECT [13-041]; NASA [NASA NNX13AI61G, NNX14AN85G]; NSF Geospace Environment Modeling grant [AGS-1103064]; Nature Science and Engineering Research Council of Canada FX This work was funded by the NSFC grants 41374166, 41274167, 41204120, and 41474141 and by the Chinese Key Research Project 2011CB811404. This work was also supported by JHU/APL contracts 967399 and 921647 under NASA's prime contract NAS5-01072. The analysis at UCLA was supported by the EMFISIS subaward 1001057397:01, the ECT subaward 13-041, the NASA grants NASA NNX13AI61G and NNX14AN85G, and NSF Geospace Environment Modeling grant AGS-1103064. D.S. acknowledges support from a Discovery Grant of the Nature Science and Engineering Research Council of Canada. We thank J. Bernard Blake and Seth G. Claudepierre for providing the Van Allen Probes MagEIS data and the World Data Center for Geomagnetism, Kyoto, for providing SYM-H and AE indices used in this study. The MagEIS data were downloaded from Van Allen Probe ECT website at http://www.rbsp-ect.lanl.gov/, and the wave measurements were downloaded from EMFISIS website at http://emfisis.physics.uiowa.edu/. The THEMIS data were available from http://themis.ssl.berkeley.edu/data/themis/. NR 38 TC 9 Z9 9 U1 2 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3009 EP 3016 DI 10.1002/2016GL067853 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300001 ER PT J AU Kurita, S Miyoshi, Y Blake, JB Reeves, GD Kletzing, CA AF Kurita, Satoshi Miyoshi, Yoshizumi Blake, J. Bernard Reeves, Geoffery D. Kletzing, Craig A. TI Relativistic electron microbursts and variations in trapped MeV electron fluxes during the 8-9 October 2012 storm: SAMPEX and Van Allen Probes observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID OUTER RADIATION BELT; GEOMAGNETIC STORMS; GEM STORMS; ACCELERATION; PRECIPITATION; CHORUS; LOSSES; WAVES; SOLAR AB It has been suggested that whistler mode chorus is responsible for both acceleration of MeV electrons and relativistic electron microbursts through resonant wave-particle interactions. Relativistic electron microbursts have been considered as an important loss mechanism of radiation belt electrons. Here we report on the observations of relativistic electron microbursts and flux variations of trapped MeV electrons during the 8-9 October 2012 storm, using the SAMPEX and Van Allen Probes satellites. Observations by the satellites show that relativistic electron microbursts correlate well with the rapid enhancement of trapped MeV electron fluxes by chorus wave-particle interactions, indicating that acceleration by chorus is much more efficient than losses by microbursts during the storm. It is also revealed that the strong chorus wave activity without relativistic electron microbursts does not lead to significant flux variations of relativistic electrons. Thus, effective acceleration of relativistic electrons is caused by chorus that can cause relativistic electron microbursts. C1 [Kurita, Satoshi; Miyoshi, Yoshizumi] Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi 4648601, Japan. [Blake, J. Bernard] Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. [Reeves, Geoffery D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Kletzing, Craig A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. RP Kurita, S (reprint author), Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi 4648601, Japan. EM kurita@isee.nagoya-u.ac.jp RI Miyoshi, Yoshizumi/B-5834-2015; OI Miyoshi, Yoshizumi/0000-0001-7998-1240; Reeves, Geoffrey/0000-0002-7985-8098 FU Japan Society for the Promotion of Science (JSPS) [25302006, 14J09407, 15H05747, 15H05815]; JSPS Program for Advancing Strategic International Networks to Accelerate the Circulation of Talented Researchers [G2602]; International Space Science Institute's (ISSI) International Team program; JSPS research fellowship for Young Scientists FX We acknowledge Van Allen Probes MagEIS data obtained from http://www.rbsp-ect.lanl.gov, Van Allen Probes EMFISIS data obtained from https://emfisis.physics.uiowa.edu, and SAMPEX HILT data obtained from the SAMPEX Data Center (http://www.srl.caltech.edu/sampex/DataCenter/). We greatly appreciate NOAA POES data which are available from http://satdat.ngdc.noaa.gov/sem/poes/data/. We also thank the World Data Center for Geomagnetism, Kyoto, for providing the SYM-H and AL indices (http://wdc.kugi.kyoto-u.ac.jp/aeasy/index.html). We acknowledge H.E. Spence for use of ECT data and Rob Redmon for use of POES MEPED data. This study is supported by Grants-in-Aid for Scientific Research (25302006, 14J09407, 15H05747, and 15H05815) of Japan Society for the Promotion of Science (JSPS). This work is also supported by JSPS Program for Advancing Strategic International Networks to Accelerate the Circulation of Talented Researchers under grant G2602 and research supported by the International Space Science Institute's (ISSI) International Team program. S.K. is supported by the JSPS research fellowship for Young Scientists. NR 36 TC 0 Z9 0 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3017 EP 3025 DI 10.1002/2016GL068260 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300002 ER PT J AU Riviere, J Pimienta, L Scuderi, M Candela, T Shokouhi, P Fortin, J Schubnel, A Marone, C Johnson, PA AF Riviere, Jacques Pimienta, Lucas Scuderi, Marco Candela, Thibault Shokouhi, Parisa Fortin, Jerome Schubnel, Alexandre Marone, Chris Johnson, Paul A. TI Frequency, pressure, and strain dependence of nonlinear elasticity in Berea Sandstone SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID SITE RESPONSE; MODULUS DISPERSION; WAVE-PROPAGATION; 1994 NORTHRIDGE; GROUND-MOTION; SLOW DYNAMICS; SOIL RESPONSE; PART II; EARTHQUAKE; ROCKS AB Acoustoelasticity measurements in a sample of room dry Berea sandstone are conducted at various loading frequencies to explore the transition between the quasi-static (f -> 0) and dynamic (few kilohertz) nonlinear elastic response. We carry out these measurements at multiple confining pressures and perform a multivariate regression analysis to quantify the dependence of the harmonic content on strain amplitude, frequency, and pressure. The modulus softening (equivalent to the harmonic at 0f) increases by a factor 2-3 over 3 orders of magnitude increase in frequency. Harmonics at 2f, 4f, and 6f exhibit similar behaviors. In contrast, the harmonic at 1f appears frequency independent. This result corroborates previous studies showing that the nonlinear elasticity of rocks can be described with a minimum of two physical mechanisms. This study provides quantitative data that describes the rate dependency of nonlinear elasticity. These findings can be used to improve theories relating the macroscopic elastic response to microstructural features. C1 [Riviere, Jacques; Scuderi, Marco; Candela, Thibault; Marone, Chris] Penn State Univ, Dept Geosci, University Pk, PA 16802 USA. [Riviere, Jacques; Johnson, Paul A.] Los Alamos Natl Lab, Earth & Environm Sci, Los Alamos, NM USA. [Pimienta, Lucas; Fortin, Jerome; Schubnel, Alexandre] Ecole Normale Super, Geol Lab, 24 Rue Lhomond, F-75231 Paris, France. [Scuderi, Marco] Univ Roma La Sapienza, Dept Earth Sci, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Candela, Thibault] Geol Survey Netherlands, TNO, Utrecht, Netherlands. [Shokouhi, Parisa] Penn State Univ, Dept Civil Engn, University Pk, PA 16802 USA. RP Riviere, J (reprint author), Penn State Univ, Dept Geosci, University Pk, PA 16802 USA.; Riviere, J (reprint author), Los Alamos Natl Lab, Earth & Environm Sci, Los Alamos, NM USA. EM jvr5626@psu.edu OI Pimienta, Lucas/0000-0003-2047-4812; SCUDERI, Marco Maria/0000-0001-5232-0792 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Data are available upon request by contacting J. Riviere (jvr5626@psu.edu). NR 60 TC 1 Z9 1 U1 4 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3226 EP 3236 DI 10.1002/2016GL068061 PG 11 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300027 ER PT J AU Van Eaton, AR Amigo, A Bertin, D Mastin, LG Giacosa, RE Gonzalez, J Valderrama, O Fontijn, K Behnke, SA AF Van Eaton, Alexa R. Amigo, Alvaro Bertin, Daniel Mastin, Larry G. Giacosa, Raul E. Gonzalez, Jeronimo Valderrama, Oscar Fontijn, Karen Behnke, Sonja A. TI Volcanic lightning and plume behavior reveal evolving hazards during the April 2015 eruption of Calbuco volcano, Chile SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID REDOUBT VOLCANO; SOURCE PARAMETERS; ASH; COLUMNS; WATER; AGGREGATION; DYNAMICS; CLOUD; MAGMA AB Soon after the onset of an eruption, model forecasts of ash dispersal are used to mitigate the hazards to aircraft, infrastructure, and communities downwind. However, it is a significant challenge to constrain the model inputs during an evolving eruption. Here we demonstrate that volcanic lightning may be used in tandem with satellite detection to recognize and quantify changes in eruption style and intensity. Using the eruption of Calbuco volcano in southern Chile on 22 and 23 April 2015, we investigate rates of umbrella cloud expansion from satellite observations, occurrence of lightning, and mapped characteristics of the fall deposits. Our remote sensing analysis gives a total erupted volume that is within uncertainty of the mapped volume (0.56 +/- 0.28 km(3) bulk). Observations and volcanic plume modeling further suggest that electrical activity was enhanced both by ice formation in the ash clouds >10 km above sea level and development of a low-level charge layer from ground-hugging currents. C1 [Van Eaton, Alexa R.; Mastin, Larry G.] US Geol Survey, Cascades Volcano Observ, Vancouver, WA USA. [Amigo, Alvaro; Bertin, Daniel; Valderrama, Oscar] Serv Nacl Geol & Mineria, Observ Volcanol Los Andes Sur, Temuco, Chile. [Amigo, Alvaro] Univ Chile, Ctr Excelencia Geotermia Los Andes, Santiago, Chile. [Giacosa, Raul E.; Gonzalez, Jeronimo] Serv Geol Minero Argentino, Delegac Reg Comahue, Gen Roca, Rio Negro, Argentina. [Fontijn, Karen] Univ Oxford, Dept Earth Sci, Oxford OX1 3PR, England. [Behnke, Sonja A.] Univ Calif Los Alamos Natl Lab, Los Alamos, NM USA. RP Van Eaton, AR (reprint author), US Geol Survey, Cascades Volcano Observ, Vancouver, WA USA. EM avaneaton@usgs.gov RI Fontijn, Karen/A-2720-2012 OI Fontijn, Karen/0000-0001-7218-4513 FU NERC [NE/N007271/1]; Fondap Conicyt [15090013] FX The authors wish to thank Bob Holzworth and the World Wide Lightning Location Network (http://wwlln.net), a collaboration among over 50 universities and institutions, for providing the lightning location data used in this paper. James Muirhead, Gregory Schill, Hans Schwaiger, Heather Wright, Dave Schneider, Sebastian Garcia, Lizette Bertin, and Mauricio Mella are thanked for assistance and discussion. A. Van Eaton acknowledges a U.S. Geological Survey Mendenhall Postdoctoral Fellowship. K. Fontijn acknowledges support by NERC urgency grant NE/N007271/1, and assistance by David Pyle, Jonathan Hunt, Romina Daga, Alexandre Corgne, Eduardo Jaramillo, and students from the Universidad Austral de Chile, Valdivia. This work is a contribution from the Fondap Conicyt #15090013 project "Centro de Excelencia en Geotermia de los Andes (CEGA)." Reviewers John Ewert, Earle R. Williams, and Magnus T. Gudmundsson are thanked for valuable comments. GeoMapApp and Unidata's IDV were used in the production of Figure 1. Data used in this study are listed in the references, tables, and supporting information. NR 49 TC 4 Z9 4 U1 6 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3563 EP 3571 DI 10.1002/2016GL068076 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300066 ER PT J AU Seeley, JT Romps, DM AF Seeley, Jacob T. Romps, David M. TI Tropical cloud buoyancy is the same in a world with or without ice SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID PHASE MICROPHYSICS; TOGA COARE; PARAMETERIZATION; ATMOSPHERE; CONVECTION; MODEL; THUNDERSTORMS; SIMULATIONS; TROPOSPHERE AB When convective clouds grow above the melting line, where temperatures fall below 0 degrees C, condensed water begins to freeze and water vapor is deposited. These processes release the latent heat of fusion, which warms cloud air, and many previous studies have suggested that this heating from fusion increases cloud buoyancy in the upper troposphere. Here we use numerical simulations of radiative-convective equilibrium with and without ice processes to argue that tropical cloud buoyancy is not systematically higher in a world with fusion than in a world without it. This insensitivity results from the fact that the environmental temperature profile encountered by developing tropical clouds is itself determined by convection. We also offer a simple explanation for the large reservoir of convective available potential energy in the tropical upper troposphere that does not invoke ice. C1 [Seeley, Jacob T.; Romps, David M.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Seeley, Jacob T.; Romps, David M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. RP Seeley, JT (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA.; Seeley, JT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. EM jseeley@berkeley.edu FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy Office of Advanced Scientific Computing Research; Office of Biological and Environmental Research [DE-AC02-05CH11231]; National Science Foundation [DGE1106400]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy Office of Advanced Scientific Computing Research and Office of Biological and Environmental Research under contract DE-AC02-05CH11231. J.T.S. acknowledges support from the National Science Foundation Graduate Research Fellowship under grant DGE1106400. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under contract DE-AC02-05CH11231. All simulation outputs used to make the figures in this paper are available from the first author upon request. NR 29 TC 0 Z9 0 U1 1 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3572 EP 3579 DI 10.1002/2016GL068583 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300067 ER PT J AU Kulkarni, G China, S Liu, S Nandasiri, M Sharma, N Wilson, J Aiken, AC Chand, D Laskin, A Mazzoleni, C Pekour, M Shilling, J Shutthanandan, V Zelenyuk, A Zaveri, RA AF Kulkarni, Gourihar China, Swarup Liu, Shang Nandasiri, Manjula Sharma, Noopur Wilson, Jacqueline Aiken, Allison C. Chand, Duli Laskin, Alexander Mazzoleni, Claudio Pekour, Mikhail Shilling, John Shutthanandan, Vaithiyalingam Zelenyuk, Alla Zaveri, Rahul A. TI Ice nucleation activity of diesel soot particles at cirrus relevant temperature conditions: Effects of hydration, secondary organics coating, soot morphology, and coagulation SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID BLACK CARBON PARTICLES; CLOUD FORMATION; WATER; AEROSOLS; INSTRUMENT; NUCLEI AB Ice formation by diesel soot particles was investigated at temperatures ranging from -40 to -50 degrees C. Size-selected soot particles were physically and chemically aged in an environmental chamber, and their ice nucleating properties were determined using a continuous flow diffusion type ice nucleation chamber. Bare (freshly formed), hydrated, and compacted soot particles, as well as a-pinene secondary organic aerosol (SOA)-coated soot particles at high relative humidity conditions, showed ice formation activity at subsaturation conditions with respect to water but below the homogeneous freezing threshold conditions. However, SOA-coated soot particles at dry conditions were observed to freeze at homogeneous freezing threshold conditions. Overall, our results suggest that heterogeneous ice nucleation activity of freshly emitted diesel soot particles are sensitive to some of the aging processes that soot can undergo in the atmosphere. C1 [Kulkarni, Gourihar; Chand, Duli; Pekour, Mikhail; Shilling, John; Zaveri, Rahul A.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [China, Swarup; Sharma, Noopur; Mazzoleni, Claudio] Michigan Technol Univ, Atmospher Sci Program, Houghton, MI 49931 USA. [China, Swarup; Sharma, Noopur; Mazzoleni, Claudio] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [China, Swarup] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Liu, Shang; Aiken, Allison C.] Univ Calif Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM USA. [Liu, Shang] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Nandasiri, Manjula; Laskin, Alexander; Shutthanandan, Vaithiyalingam] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Wilson, Jacqueline; Zelenyuk, Alla] Pacific NW Natl Lab, Chem Phys & Anal, Richland, WA 99352 USA. RP Kulkarni, G (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM Gourihar.Kulkarni@pnnl.gov RI Shilling, John/L-6998-2015; Laskin, Alexander/I-2574-2012; Liu, Shang/F-9085-2011; Aiken, Allison/B-9659-2009 OI Shilling, John/0000-0002-3728-0195; Laskin, Alexander/0000-0002-7836-8417; Liu, Shang/0000-0002-3403-8651; Aiken, Allison/0000-0001-5749-7626 FU Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program; U.S. Department of Energy's Atmospheric System Research [DE-SC0010019]; U.S. National Science Foundation [AGS-1028998]; NASA Earth and Space Science Graduate Fellowship [NNX12AN97H]; LDRD-Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL); DOE's Office of Biological and Environmental Research; U.S. DOE [DE-AC05-76RL0 1830] FX The work was supported by the Office of Science of the U.S. Department of Energy (DOE) as part of the Atmospheric System Research Program. We also thank D. Nelson, M. Dubey, and R. Subramanian for their useful discussions. S. China, N. Sharma and C. Mazzoleni were funded by the U.S. Department of Energy's Atmospheric System Research (grant DE-SC0010019) and the U.S. National Science Foundation grant (AGS-1028998). S. China acknowledges NASA Earth and Space Science Graduate Fellowship (grant NNX12AN97H). We thank Owen P. Mills for helping with the microscopy work. M. Nandasiri and V. Shutthanandan acknowledge the funding support from the LDRD-funded Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). A portion of the work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research located at PNNL. The ice nucleation research was performed at the Atmospheric Measurement Laboratory at PNNL. Data supporting sections 2 and 5 are available in the supporting information and available upon request from the corresponding author. We also would like to thank two reviewers and editor for comments and discussions. PNNL is operated by the U.S. DOE by Battelle Memorial Institute under contract DE-AC05-76RL0 1830. NR 37 TC 3 Z9 3 U1 9 U2 28 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD APR 16 PY 2016 VL 43 IS 7 BP 3580 EP 3588 DI 10.1002/2016GL068707 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DL3MG UT WOS:000375537300068 ER PT J AU Sasaki, Y Kitaura, R Yuk, JM Zettl, A Shinohara, H AF Sasaki, Yuki Kitaura, Ryo Yuk, Jong Min Zettl, Alex Shinohara, Hisanori TI Efficient preparation of graphene liquid cell utilizing direct transfer with large-area well-stitched graphene SO CHEMICAL PHYSICS LETTERS LA English DT Article ID PLATINUM NANOCRYSTAL GROWTH; WALLED CARBON NANOTUBES; IN-SITU TEM; ELECTRON-MICROSCOPY; MONOLAYER GRAPHENE; SPECIMENS; COPPER; CRYSTALLIZATION; STRENGTH; LEVEL AB By utilizing graphene-sandwiched structures recently developed in this laboratory, we are able to visualize small droplets of liquids in nanometer scale. We have found that small water droplets as small as several tens of nanometers sandwiched by two single-layer graphene are frequently observed by TEM. Due to the electron beam irradiation during the TEM observation, these sandwiched droplets are frequently moving from one place to another and are subjected to create small bubbles inside. The synthesis of a large area single-domain graphene of high-quality is essential to prepare the graphene sandwiched cell which safely encapsulates the droplets in nanometer size. (C) 2016 Elsevier B.V. All rights reserved. C1 [Sasaki, Yuki; Kitaura, Ryo; Shinohara, Hisanori] Nagoya Univ, Dept Chem, Nagoya, Aichi 4648602, Japan. [Sasaki, Yuki; Kitaura, Ryo; Shinohara, Hisanori] Nagoya Univ, Inst Adv Res, Nagoya, Aichi 4648602, Japan. [Yuk, Jong Min; Zettl, Alex] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Yuk, Jong Min; Zettl, Alex] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yuk, Jong Min; Zettl, Alex] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Yuk, Jong Min; Zettl, Alex] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Kitaura, R; Shinohara, H (reprint author), Nagoya Univ, Dept Chem, Nagoya, Aichi 4648602, Japan.; Kitaura, R; Shinohara, H (reprint author), Nagoya Univ, Inst Adv Res, Nagoya, Aichi 4648602, Japan. EM r.kitaura@nagoya-u.jp; noris@nagoya-u.jp RI Kitaura, Ryo/B-8123-2008; Zettl, Alex/O-4925-2016 OI Zettl, Alex/0000-0001-6330-136X FU MEXT, Japan [22225001, 25708002, 24681031, 25107002]; JSPS; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy within the sp2-bonded Materials Program [DE-AC02-05CH11231, KC2207]; US National Science Foundation [DMR-1206512]; Department of the Defense, Defense Threat Reduction Agency [HDTRA1-13-1-0035] FX This work was partially supported by a Grant-in-Aid for Scientific Research S (No. 22225001 to H.S.), the Grant-in-aid for Young Scientists A (Nos. 25708002 and 24681031 to R.K.), Scientific Research on Innovative Areas (No. 25107002 to R.K.), and the Program for Leading Graduate Schools 'Integrative Graduate Education and Research in Green Natural Sciences' of MEXT, Japan. Y.S. thanks JSPS for fellowship. Funding was also provided by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05CH11231, within the sp2-bonded Materials Program (KC2207), which provided for TEM characterization; the US National Science Foundation under grant DMR-1206512 which provided for sample synthesis; and the Department of the Defense, Defense Threat Reduction Agency under grant HDTRA1-13-1-0035 which provided for postdoctoral support. NR 42 TC 1 Z9 1 U1 9 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD APR 16 PY 2016 VL 650 BP 107 EP 112 DI 10.1016/j.cplett.2016.02.066 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK5NP UT WOS:000374966900022 ER PT J AU Shao, XM AF Shao, Xuan-Min TI Generalization of the lightning electromagnetic equations of Uman, McLain, and Krider based on Jefimenko equations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE lightning EM; Jefimenko equations; classical EM AB The fundamental electromagnetic equations used by lightning researchers were introduced in a seminal paper by Uman, McLain, and Krider in 1975. However, these equations were derived for an infinitely thin, one-dimensional source current, and not for a general three-dimensional current distribution. In this paper, we introduce a corresponding pair of generalized equations that are determined from a three-dimensional, time-dependent current density distribution based on Jefimenko's original electric and magnetic equations. To do this, we derive the Jefimenko electric field equation into a new form that depends only on the time-dependent current density similar to that of Uman, McLain, and Krider, rather than on both the charge and current densities in its original form. The original Jefimenko magnetic field equation depends only on current, so no further derivation is needed. We show that the equations of Uman, McLain, and Krider can be readily obtained from the generalized equations if a one-dimensional source current is considered. For the purpose of practical applications, we discuss computational implementation of the new equations and present electric field calculations for a three-dimensional, conical-shape discharge. C1 [Shao, Xuan-Min] Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM USA. RP Shao, XM (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM USA. EM xshao@lanl.gov FU Defense Threat Reduction Agency (DTRA) of the U.S. Department of Defense [DTRA10027-14741A1] FX The author thanks W. Scott Smith for conducting FDTD EM calculation for comparison with the results of equation 17. This work was supported by the Defense Threat Reduction Agency (DTRA) of the U.S. Department of Defense grant DTRA10027-14741A1. The computational software and results used to generate Figures 1 and 2 can be released through official Los Alamos National Laboratory's release policy after request is made to X.-M.S. NR 13 TC 0 Z9 0 U1 5 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD APR 16 PY 2016 VL 121 IS 7 BP 3363 EP 3371 DI 10.1002/2015JD024717 PG 9 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DK7QG UT WOS:000375120200017 ER PT J AU Yang, H Chen, G Tang, Q Hess, P AF Yang, Huang Chen, Gang Tang, Qi Hess, Peter TI Quantifying isentropic stratosphere-troposphere exchange of ozone SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE stratosphere-troposphere exchange; isentropic diagnostics; diabatic heating; mixing ID BREWER-DOBSON CIRCULATION; EFFECTIVE DIFFUSIVITY; NORTHERN-HEMISPHERE; POTENTIAL VORTICITY; CLIMATOLOGY; TROPOPAUSE; TRANSPORT; VARIABILITY; MODEL; MASS AB There is increased evidence that stratosphere-troposphere exchange (STE) of ozone has a significant impact on tropospheric chemistry and radiation. Traditional diagnostics of STE consider the ozone budget in the lowermost stratosphere (LMS) as a whole. However, this can only render the hemispherically integrated ozone flux and therefore does not distinguish the exchange of ozone into low latitudes from that into high latitudes. The exchange of ozone at different latitudes may have different tropospheric impacts. This present study extends the traditional approach from the entire LMS to individual isentropic layers in the LMS and therefore gives the meridional distribution of STE by the latitudes where each isentropic surface intersects the tropopause. The specified dynamics version of the Whole Atmosphere Community Climate Model is used to estimate the STE ozone flux on each isentropic surface. It is found that net troposphere-to-stratosphere ozone transport occurs in low latitudes along the 350-380K isentropic surfaces and that net stratosphere-to-troposphere ozone transport takes place in the extratropics along the 280-350K isentropes. Particularly, the seasonal cycle of extratropical STE ozone flux in the Northern Hemisphere displays a maximum in late spring and early summer, following the seasonal migration of the upper tropospheric jet and associated isentropic mixing. Furthermore, differential diabatic heating and isentropic mixing tend to induce STE ozone fluxes in opposite directions, but the net effect results in a spatiotemporal pattern similar to the STE ozone flux associated with isentropic mixing. C1 [Yang, Huang; Chen, Gang] Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY USA. [Tang, Qi] Lawrence Livermore Natl Lab, Livermore, CA USA. [Tang, Qi; Hess, Peter] Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY USA. RP Yang, H (reprint author), Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY USA. EM hy337@cornell.edu RI Tang, Qi/C-1032-2011; Chen, Gang/I-3305-2012 OI Chen, Gang/0000-0003-4934-1909 FU National Science Foundation (NSF) [AGS-1042787]; Department of Energy (DOE); U.S. Department of Energy (DOE) [DE-AC52-07NA27344]; [NSFAGS-1349605] FX H.Y., G.C., and P.H. are supported by the National Science Foundation (NSF) grants AGS-1042787. H.Y. and G.C. is additinally supported by the NSFAGS-1349605. Q.T.'s work at Lawrence Livermore National Laboratory (LLNL) is supported by the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program and performed under the auspices of the U.S. Department of Energy (DOE) by LLNL under contract DE-AC52-07NA27344. All data used to generate figures and tables are freely available via contacting the lead author: hy337@cornell.edu. We thank three anonymous reviewers for their helpful suggestions that vastly improve the manuscript. NR 45 TC 0 Z9 0 U1 8 U2 25 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD APR 16 PY 2016 VL 121 IS 7 BP 3372 EP 3387 DI 10.1002/2015JD024180 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DK7QG UT WOS:000375120200018 ER PT J AU Kumjian, MR Mishra, S Giangrande, SE Toto, T Ryzhkov, AV Bansemer, A AF Kumjian, Matthew R. Mishra, Subashree Giangrande, Scott E. Toto, Tami Ryzhkov, Alexander V. Bansemer, Aaron TI Polarimetric radar and aircraft observations of saggy bright bands during MC3E SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE radar; microphysics; precipitation ID BACKSCATTER DIFFERENTIAL PHASE; MELTING LAYER; PART I; VERTICAL VELOCITY; FALL SPEEDS; MICROPHYSICS; CLOUD; PRECIPITATION; DISTRIBUTIONS; EVOLUTION AB Polarimetric radar observations increasingly are used to understand cloud microphysical processes, which is critical for improving their representation in cloud and climate models. In particular, there has been recent focus on improving representations of ice collection processes (e.g., aggregation and riming), as these influence precipitation rate, heating profiles, and ultimately cloud life cycles. However, distinguishing these processes using conventional polarimetric radar observations is difficult, as they produce similar fingerprints. This necessitates improved analysis techniques and integration of complementary data sources. The Midlatitude Continental Convective Clouds Experiment (MC3E) provided such an opportunity. Quasi-vertical profiles of polarimetric radar variables in two MC3E stratiform precipitation events reveal episodic melting layer sagging. Integrated analyses using scanning and vertically pointing radar and aircraft measurements reveal that saggy bright band signatures are produced when denser, faster-falling, more isometric hydrometeors (relative to adjacent times) descend into the melting layer. In one case, strong circumstantial evidence for riming is found during bright band sagging times. A bin microphysical melting layer model successfully reproduces many aspects of the signature, supporting the observational analysis. If found to be a reliable indicator of riming, saggy bright bands could be a proxy for the presence of supercooled liquid water in stratiform precipitation, which may provide important information for mitigating aircraft icing risks and for constraining microphysical models. C1 [Kumjian, Matthew R.] Penn State Univ, Dept Meteorol, 503 Walker Bldg, University Pk, PA 16802 USA. [Mishra, Subashree] US DOE, Washington, DC 20585 USA. [Mishra, Subashree; Ryzhkov, Alexander V.] NOAA OAR Natl Severe Storms Lab, Norman, OK USA. [Giangrande, Scott E.; Toto, Tami] Brookhaven Natl Lab, Atmospher Sci Div, Upton, NY 11973 USA. [Ryzhkov, Alexander V.] Cooperat Inst Mesoscale Meteorol Studies, Norman, OK USA. [Ryzhkov, Alexander V.] Univ Oklahoma, Norman, OK 73019 USA. [Bansemer, Aaron] Natl Ctr Atmospher Res, Mesoscale & Microscale Meteorol Div, POB 3000, Boulder, CO 80307 USA. RP Kumjian, MR (reprint author), Penn State Univ, Dept Meteorol, 503 Walker Bldg, University Pk, PA 16802 USA. EM kumjian@psu.edu RI Giangrande, Scott/I-4089-2016; Measurement, Global/C-4698-2015 OI Giangrande, Scott/0000-0002-8119-8199; FU U.S. Department of Energy [ER65459]; NOAA/Office and Atmospheric Research under NOAA-University of Oklahoma, U.S. Department of Commerce [NA11OAR4320072]; DOE ASR [DE-SC0008648]; National Science Foundation FX Support for this work comes from grant ER65459 from the U.S. Department of Energy Atmospheric System Research program. Support for A. Ryzhkov and S. Mishra comes from NOAA/Office and Atmospheric Research under NOAA-University of Oklahoma cooperative agreement NA11OAR4320072, U.S. Department of Commerce. Support for A. Bansemer is from DOE ASR grant DE-SC0008648. We would like to thank Mike Poellet and his research group at UND for processing and providing the in situ aircraft data. Radar data are available at the Department of Energy Atmospheric Radiation Measurement program data archive. We would also like to thank Sandra Yuter (NCSU) for helpful criticisms of our work. The comments and suggestions from three anonymous reviewers significantly improved the clarity and presentation of the manuscript. The National Center for Atmospheric Research is sponsored by the National Science Foundation. NR 64 TC 4 Z9 4 U1 3 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD APR 16 PY 2016 VL 121 IS 7 BP 3584 EP 3607 DI 10.1002/2015JD024446 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DK7QG UT WOS:000375120200032 ER PT J AU Hornig, A Makris, Y Mehen, T AF Hornig, Andrew Makris, Yiannis Mehen, Thomas TI Jet shapes in dijet events at the LHC in SCET SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; QCD Phenomenology ID CROSS-SECTIONS; LEADING ORDER; WILSON LOOPS; RESUMMATION; QCD AB We consider the class of jet shapes known as angularities in dijet production at hadron colliders. These angularities are modified from the original definitions in e(+)e(-) collisions to be boost invariant along the beam axis. These shapes apply to the constituents of jets defined with respect to either k(T)-type (anti-k(T), C/A, and k(T)) algorithms and cone-type algorithms. We present an SCET factorization formula and calculate the ingredients needed to achieve next-to-leading-log (NLL) accuracy in kinematic regions where non-global logarithms are not large. The factorization formula involves previously unstudied "unmeasured beam functions," which are present for finite rapidity cuts around the beams. We derive relations between the jet functions and the shape-dependent part of the soft function that appear in the factorized cross section and those previously calculated for e(+)e(-) collisions, and present the calculation of the non-trivial, color-connected part of the soft-function to O (alpha(s)). This latter part of the soft function is universal in the sense that it applies to any experimental setup with an out-of-jet p(T) veto and rapidity cuts together with two identified jets and it is independent of the choice of jet (sub-) structure measurement. In addition, we implement the recently introduced soft-collinear refactorization to resum logarithms of the jet size, valid in the region of non-enhanced non-global logarithm effects. While our results are valid for all 2 -> 2 channels, we compute explicitly for the qq' -> qq' channel the color-flow matrices and plot the NLL resummed differential dijet cross section as an explicit example, which shows that the normalization and scale uncertainty is reduced when the soft function is refactorized. For this channel, we also plot the jet size R dependence, the p(T)(cut) dependence, and the dependence on the angularity parameter a. C1 [Hornig, Andrew] Los Alamos Natl Lab, Theoret Div T 2, Los Alamos, NM 87545 USA. [Makris, Yiannis; Mehen, Thomas] Duke Univ, Dept Phys, Durham, NC 27708 USA. RP Hornig, A (reprint author), Los Alamos Natl Lab, Theoret Div T 2, Los Alamos, NM 87545 USA.; Makris, Y; Mehen, T (reprint author), Duke Univ, Dept Phys, Durham, NC 27708 USA. EM ahornig@lanl.gov; yiannis.makris@duke.edu; mehen@phy.duke.edu FU LANL/LDRD program; DOE Office of Science [DE-AC52-06NA25396]; Office of Science, Office of Nuclear Physics, of the U.S. Department of Energy [DE-FG02-05ER41368] FX We would like to thank Christopher Lee, Daekyoung Kang, and Wouter Waalewijn for helpful discussions, and Christopher Lee for reviewing this manuscript. AH was supported by a Director's Fellowship from the LANL/LDRD program and the DOE Office of Science under Contract DE-AC52-06NA25396. TM and YM are supported in part by the Director, Office of Science, Office of Nuclear Physics, of the U.S. Department of Energy under grant numbers DE-FG02-05ER41368. TM and YM also acknowledge the hospitality of the theory groups at Brookhaven National Laboratory, Los Alamos National Laboratory, Duke-Kunshan University, and UC-Irvine for their hospitality during the completion of this work. NR 82 TC 4 Z9 4 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 15 PY 2016 IS 4 AR 097 DI 10.1007/JHEP04(2016)097 PG 41 WC Physics, Particles & Fields SC Physics GA DJ6RL UT WOS:000374340500003 ER PT J AU Coyle, DR Aubrey, DP Coleman, MD AF Coyle, David R. Aubrey, Doug P. Coleman, Mark D. TI Growth responses of narrow or broad site adapted tree species to a range of resource availability treatments after a full harvest rotation (vol 362, pg 107, 2016) SO FOREST ECOLOGY AND MANAGEMENT LA English DT Correction C1 [Coyle, David R.; Aubrey, Doug P.] Univ Georgia, DB Warnell Sch Forestry & Nat Resources, Bldg 4-407,180 E Green St, Athens, GA 30602 USA. [Aubrey, Doug P.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Coleman, Mark D.] Univ Idaho, Dept Forest Rangeland & Fire Sci, Moscow, ID 83844 USA. RP Coyle, DR (reprint author), Univ Georgia, Warnell Sch Forestry & Nat Resources, Bldg 4-407,180 E Green St, Athens, GA 30602 USA. EM drcoyle@uga.edu NR 1 TC 0 Z9 0 U1 5 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-1127 EI 1872-7042 J9 FOREST ECOL MANAG JI For. Ecol. Manage. PD APR 15 PY 2016 VL 366 BP 251 EP 252 DI 10.1016/j.foreco.2016.03.015 PG 2 WC Forestry SC Forestry GA DK8EX UT WOS:000375161100022 ER PT J AU Silvaroli, JA Arne, JM Chelstowska, S Kiser, PD Banerjee, S Golczak, M AF Silvaroli, Josie A. Arne, Jason M. Chelstowska, Sylwia Kiser, Philip D. Banerjee, Surajit Golczak, Marcin TI Ligand Binding Induces Conformational Changes in Human Cellular Retinol-binding Protein 1 (CRBP1) Revealed by Atomic Resolution Crystal Structures SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE lipid transport; retinal metabolism; retinoid-binding protein; retinol; vitamin A ID ALL-TRANS-RETINOL; ESCHERICHIA-COLI; VITAMIN-A; RAT-LIVER; MASS-SPECTROMETRY; VISUAL CYCLE; HOLO; APO; REFINEMENT; DYNAMICS AB Important in regulating the uptake, storage, and metabolism of retinoids, cellular retinol-binding protein 1 (CRBP1) is essential for trafficking vitamin A through the cytoplasm. However, the molecular details of ligand uptake and targeted release by CRBP1 remain unclear. Here we report the first structure of CRBP1 in a ligand-free form as well as ultra-high resolution structures of this protein bound to either all-trans-retinol or retinylamine, the latter a therapeutic retinoid that prevents light-induced retinal degeneration. Superpositioning of human apo- and holo-CRBP1 revealed major differences within segments surrounding the entrance to the retinoid-binding site. These included -helix II and hairpin turns between -strands C-D and E-F as well as several side chains, such as Phe-57, Tyr-60, and Ile-77, that change their orientations to accommodate the ligand. Additionally, we mapped hydrogen bond networks inside the retinoid-binding cavity and demonstrated their significance for the ligand affinity. Analyses of the crystallographic B-factors indicated several regions with higher backbone mobility in the apoprotein that became more rigid upon retinoid binding. This conformational flexibility of human apo-CRBP1 facilitates interaction with the ligands, whereas the more rigid holoprotein structure protects the labile retinoid moiety during vitamin A transport. These findings suggest a mechanism of induced fit upon ligand binding by mammalian cellular retinol-binding proteins. C1 [Silvaroli, Josie A.; Arne, Jason M.; Chelstowska, Sylwia; Kiser, Philip D.; Golczak, Marcin] Case Western Reserve Univ, Sch Med, Dept Pharmacol, 10900 Euclid Ave, Cleveland, OH 44106 USA. [Golczak, Marcin] Case Western Reserve Univ, Sch Med, Cleveland Ctr Membrane & Struct Biol, Cleveland, OH 44106 USA. [Chelstowska, Sylwia] Mil Inst Med, Dept Hematol, Lab Hematol & Flow Cytometry, PL-04141 Warsaw, Poland. [Kiser, Philip D.] Louis Stokes Cleveland Vet Affairs Med Ctr, Res Serv, Cleveland, OH 44106 USA. [Banerjee, Surajit] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14850 USA. [Banerjee, Surajit] Argonne Natl Lab, Northeastern Collaborat Access Team, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Golczak, M (reprint author), Case Western Reserve Univ, Sch Med, Dept Pharmacol, 10900 Euclid Ave, Cleveland, OH 44106 USA. EM mxg149@case.edu FU NIGMS, National Institutes of Health (NIH) [P41 GM103403]; NIH-ORIP HEI [S10 RR029205]; DOE Office of Science [DE-AC02-06CH11357]; DOE Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; NIGMS, NIH [P41GM103393] FX We thank L. T. Webster, Jr. for help in editing the manuscript. This work is based upon research conducted at the Northeastern Collaborative Access Team beamlines, which are funded by NIGMS, National Institutes of Health (NIH), Grant P41 GM103403. The Pilatus 6M detector on the 24-ID-C beamline is funded by NIH-ORIP HEI Grant S10 RR029205. This research used resources of the Advanced Photon Source, a United States Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. We also thank the staff of the SLAC National Accelerator Laboratory (Menlo Park, CA), operated by Stanford University for the DOE Office of Science. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the DOE Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research and by NIGMS, NIH, Grant P41GM103393. NR 61 TC 3 Z9 3 U1 2 U2 5 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD APR 15 PY 2016 VL 291 IS 16 BP 8528 EP 8540 DI 10.1074/jbc.M116.714535 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DK2VT UT WOS:000374773200018 PM 26900151 ER PT J AU Kort-Kamp, WJM Cordes, NL Ionita, A Glover, BB Duque, ALH Perry, WL Patterson, BM Dalvit, DAR Moore, DS AF Kort-Kamp, W. J. M. Cordes, N. L. Ionita, A. Glover, B. B. Duque, A. L. Higginbotham Perry, W. L. Patterson, B. M. Dalvit, D. A. R. Moore, D. S. TI Microscale Electromagnetic Heating in Heterogeneous Energetic Materials Based on X-ray Computed Tomography SO PHYSICAL REVIEW APPLIED LA English DT Article ID EXPLOSIVES; IGNITION AB Electromagnetic stimulation of energetic materials provides a noninvasive and nondestructive tool for detecting and identifying explosives. We combine structural information based on x-ray computed tomography, experimental dielectric data, and electromagnetic full-wave simulations to study microscale electromagnetic heating of realistic three-dimensional heterogeneous explosives. We analyze the formation of electromagnetic hot spots and thermal gradients in the explosive-binder mesostructures and compare the heating rate for various binder systems. C1 [Kort-Kamp, W. J. M.] Los Alamos Natl Lab, Ctr Nonlinear Studies, MS B258, Los Alamos, NM 87545 USA. [Kort-Kamp, W. J. M.; Dalvit, D. A. R.] Los Alamos Natl Lab, Div Theoret, MS B213, Los Alamos, NM 87545 USA. [Cordes, N. L.; Patterson, B. M.] Los Alamos Natl Lab, Div Mat Sci & Technol, MS E549, Los Alamos, NM 87545 USA. [Ionita, A.] Los Alamos Natl Lab, Div Theoret, MS B221, Los Alamos, NM 87545 USA. [Glover, B. B.; Moore, D. S.] Los Alamos Natl Lab, Explos Sci & Shock Phys Div, MS P952, Los Alamos, NM 87545 USA. [Duque, A. L. Higginbotham; Perry, W. L.] Los Alamos Natl Lab, Explos Sci & Shock Phys Div, MS C920, Los Alamos, NM 87545 USA. RP Kort-Kamp, WJM (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, MS B258, Los Alamos, NM 87545 USA.; Kort-Kamp, WJM (reprint author), Los Alamos Natl Lab, Div Theoret, MS B213, Los Alamos, NM 87545 USA. RI Kort-Kamp, W./L-3329-2013; OI Cordes, Nikolaus/0000-0003-3367-5592; Duque, Amanda/0000-0002-2023-1389; Patterson, Brian/0000-0001-9244-7376; Perry, William/0000-0003-1993-122X FU LANL LDRD program FX We thank Virginia Manner and Bryce Tappan of LANL for providing PBX samples. We are grateful to the LANL LDRD program for financial support. NR 28 TC 0 Z9 0 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD APR 15 PY 2016 VL 5 IS 4 AR 044008 DI 10.1103/PhysRevApplied.5.044008 PG 7 WC Physics, Applied SC Physics GA DJ6DJ UT WOS:000374299900003 ER PT J AU Lv, YF Wang, WL Ding, H Wang, Y Ding, Y Zhong, RD Schneeloch, J Gu, GD Wang, LL He, K Ji, SH Zhao, L Zhou, XJ Song, CL Ma, XC Xue, QK AF Lv, Yan-Feng Wang, Wen-Lin Ding, Hao Wang, Yang Ding, Ying Zhong, Ruidan Schneeloch, John Gu, G. D. Wang, Lili He, Ke Ji, Shuai-Hua Zhao, Lin Zhou, Xing-Jiang Song, Can-Li Ma, Xu-Cun Xue, Qi-Kun TI Electronic structure of the ingredient planes of the cuprate superconductor Bi2Sr2CuO6+delta : A comparison study with Bi2Sr2CaCu2O8+delta SO PHYSICAL REVIEW B LA English DT Article ID SCANNING TUNNELING SPECTROSCOPY; HIGH-TEMPERATURE SUPERCONDUCTOR; COPPER-OXIDE SUPERCONDUCTORS; ATOMIC-SCALE; PSEUDOGAP; GAP; ORIGIN; OXYGEN; IMPACT AB By means of low-temperature scanning tunneling microscopy, we report on the electronic structures of the BiO and SrO planes of the Bi2Sr2CuO6+delta (Bi-2201) superconductor prepared by argon-ion bombardment and annealing. Depending on post annealing conditions, the BiO planes exhibit either a pseudogap (PG) with sharp coherence peaks and an anomalously large gap magnitude of 49 meV or van Hove singularity (vHS) near the Fermi level, while the SrO is always characteristic of a PG-like feature. This contrasts with the Bi2Sr2CaCu2O8+delta (Bi-2212) superconductor where vHS occurs solely on the SrO plane. We disclose the interstitial oxygen dopants (delta in the formulas) as a primary cause for the occurrence of vHS, which are located dominantly around the BiO and SrO planes, respectively, in Bi-2201 and Bi-2212. This is supported by the contrasting structural buckling amplitude of the BiO and SrO planes in the two superconductors. Our findings provide solid evidence for the irrelevance of PG to the superconductivity in the two superconductors, as well as insights into why Bi-2212 can achieve a higher superconducting transition temperature than Bi-2201, and by implication, the mechanism of cuprate superconductivity. C1 [Lv, Yan-Feng; Wang, Wen-Lin; Ding, Hao; Wang, Yang; Wang, Lili; He, Ke; Ji, Shuai-Hua; Song, Can-Li; Ma, Xu-Cun; Xue, Qi-Kun] Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China. [Ding, Ying; Zhao, Lin; Zhou, Xing-Jiang] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Natl Lab Superconduct, Beijing 100190, Peoples R China. [Zhong, Ruidan; Schneeloch, John; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Wang, Lili; He, Ke; Ji, Shuai-Hua; Zhou, Xing-Jiang; Song, Can-Li; Ma, Xu-Cun; Xue, Qi-Kun] Collaborat Innovat Ctr Quantum Matter, Beijing 100084, Peoples R China. RP Song, CL; Ma, XC; Xue, QK (reprint author), Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China.; Song, CL; Ma, XC; Xue, QK (reprint author), Collaborat Innovat Ctr Quantum Matter, Beijing 100084, Peoples R China. EM clsong07@mail.tsinghua.edu.cn; xucunma@mail.tsinghua.edu.cn; qkxue@mail.tsinghua.edu.cn RI Zhong, Ruidan/D-5296-2013; Ding, Hao/H-8401-2013 OI Zhong, Ruidan/0000-0003-1652-9454; Ding, Hao/0000-0001-9635-3940 FU National Science Foundation and Ministry of Science and Technology of China; Tsinghua University Initiative Scientific Research Program; MOST of China (973 program) [2015CB921000]; NSFC [11190022, 11334010]; Strategic Priority Research Program (B) of CAS [XDB07020300]; Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, US Department of Energy (DOE) [DE-SC00112704] FX This work was financially supported by National Science Foundation and Ministry of Science and Technology of China. C.L.S. acknowledges support from Tsinghua University Initiative Scientific Research Program. X.J.Z. acknowledges financial support from the MOST of China (973 program: 2015CB921000), the NSFC (Grants No. 11190022 and No. 11334010), and the Strategic Priority Research Program (B) of CAS with Grant No. XDB07020300. Work at Brookhaven National Laboratory was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, US Department of Energy (DOE), through Contract No. DE-SC00112704. NR 40 TC 2 Z9 2 U1 48 U2 71 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 15 PY 2016 VL 93 IS 14 AR 140504 DI 10.1103/PhysRevB.93.140504 PG 5 WC Physics, Condensed Matter SC Physics GA DJ6CW UT WOS:000374298600002 ER PT J AU Zhu, GY Koch, J Martin, I AF Zhu, Guanyu Koch, Jens Martin, Ivar TI Nematic quantum liquid crystals of bosons in frustrated lattices SO PHYSICAL REVIEW B LA English DT Article ID KAGOME-LATTICE; NEUTRAL ATOMS; MAGNETIC-FIELDS; STATES; ANTIFERROMAGNETS; TEMPERATURE; BANDS; MODEL AB The problem of interacting bosons in frustrated lattices is an intricate one due to the absence of a unique minimum in the single-particle dispersion wheremacroscopic number of bosons can condense. Here, we consider a family of tight-binding models with macroscopically degenerate lowest energy bands, separated from other bands by a gap. We predict the formation of exotic states that spontaneously break rotational symmetry at relatively low filling. These states belong to three nematic phases: Wigner crystal, supersolid, and superfluid. The Wigner crystal phase is established exactly at low filling. Supersolid and superfluid phases, at larger filling, are obtained by making use of a projection onto the flat band, construction of an appropriate Wannier basis, and subsequent mean-field treatment. The nematic superfluid that we predict is uniform in real space but has an anisotropic momentum distribution, providing a novel scenario for Bose condensation with an additional nematic order. Our findings open up a promising direction of studying microscopic quantum liquid crystalline phases of bosons. C1 [Zhu, Guanyu; Koch, Jens] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Martin, Ivar] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zhu, GY (reprint author), Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RI Koch, Jens/G-6789-2011 OI Koch, Jens/0000-0002-5047-631X FU NSF [PHY-1055993]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We are indebted to Steven Girvin, Ashvin Vishwanath, Tigran Sedrakayan, Eliot Kapit, Hakan Tureci, Tzu-Chieh Wei, Anupam Garg, James Sauls, Murad Tovmasyan, and Andy C. Y. Li for insightful discussions. Work performed at Northwestern University (G.Z. and J.K.) was supported by the NSF under Grant PHY-1055993. Work performed at Argonne National Laboratory (I.M.) is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 44 TC 2 Z9 2 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 15 PY 2016 VL 93 IS 14 AR 144508 DI 10.1103/PhysRevB.93.144508 PG 16 WC Physics, Condensed Matter SC Physics GA DJ6CW UT WOS:000374298600004 ER PT J AU Raya, K Chang, L Bashir, A Cobos-Martinez, JJ Gutierrez-Guerrero, LX Roberts, CD Tandy, PC AF Raya, Khepani Chang, Lei Bashir, Adnan Cobos-Martinez, J. Javier Xiomara Gutierrez-Guerrero, L. Roberts, Craig D. Tandy, Peter C. TI Structure of the neutral pion and its electromagnetic transition form factor SO PHYSICAL REVIEW D LA English DT Article ID DYSON-SCHWINGER EQUATIONS; AXIAL-VECTOR VERTEX; QUANTUM CHROMODYNAMICS; EXCLUSIVE PROCESSES; QCD; MESONS; ELECTRODYNAMICS AB The gamma*gamma -> pi(0) transition formfactor, G(Q(2)), is computed on the entire domain of spacelikemomenta using a continuum approach to the two valence body bound-state problem in relativistic quantum field theory: the result agrees with data obtained by the CELLO, CLEO, and Belle Collaborations. The analysis unifies this prediction with that of the pion's valence-quark parton distribution amplitude (PDA) and elastic electromagnetic form factor and demonstrates, too, that a fully self-consistent treatment can readily connect a pion PDA that is a broad, concave function at the hadronic scale with the perturbative QCD prediction for the transition form factor in the hard photon limit. The normalization of that limit is set by the scale of dynamical chiral symmetry breaking, which is a crucial feature of the Standard Model. Understanding of the latter will thus remain incomplete until definitive transition form factor data are available on Q(2) > 10 GeV2. C1 [Raya, Khepani; Bashir, Adnan; Cobos-Martinez, J. Javier] Univ Michoacana, Inst Fis & Matemat, Edificio C-3,Ciudad Univ, Morelia 58040, Michoacan, Mexico. [Chang, Lei] Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China. [Xiomara Gutierrez-Guerrero, L.] Univ Sonora, Dept Fis, Blvd Luis Encinas J Y Rosales Colonia Ctr, Hermosillo 83000, Sonora, Mexico. [Roberts, Craig D.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Tandy, Peter C.] Kent State Univ, Dept Phys, Ctr Nucl Res, Kent, OH 44242 USA. RP Raya, K; Bashir, A; Cobos-Martinez, JJ (reprint author), Univ Michoacana, Inst Fis & Matemat, Edificio C-3,Ciudad Univ, Morelia 58040, Michoacan, Mexico.; Chang, L (reprint author), Nankai Univ, Sch Phys, Tianjin 300071, Peoples R China.; Gutierrez-Guerrero, LX (reprint author), Univ Sonora, Dept Fis, Blvd Luis Encinas J Y Rosales Colonia Ctr, Hermosillo 83000, Sonora, Mexico.; Roberts, CD (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA.; Tandy, PC (reprint author), Kent State Univ, Dept Phys, Ctr Nucl Res, Kent, OH 44242 USA. EM khepani@ifm.umich.mx; lei.chiong@gmail.com; adnan@ifm.umich.mx; javiercobos@ifm.umich.mx; laura.gutierrez@unison.mx; cdroberts@anl.gov; tandy@kent.edu FU CIC (UMSNH); CONACyT [4.10, CB-2014-22117]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; U.S. National Science Foundation [NSF-PHY1206187] FX We are grateful for astute remarks by I. C. Cloet, B. El-Bennich, S.-X. Qin, J. Rodriguez Quintero and A. W. Thomas, and for participation in the following workshops, which facilitated this research: Many Manifestations of Nonperturbative QCD under the Southern Cross, Ubatuba, Brazil (LC, AB, CDR, PCT); 2nd Workshop on Perspectives in Nonperturbative QCD, IFT-UNESP, Sao Paulo, Brazil (AB, CDR, PCT); Connecting Nuclear Physics and Elementary Particle Interactions: Building Bridges at the Spanish Frontier, Punta Umbria, Spain (KR, AB, CDR, PCT) and 5th Workshop on Nonperturbative Aspects of Field Theories, Morelia, Mexico (KR, AB, JC-M, LXG, CDR, PCT). Research was supported by CIC (UMSNH) and CONACyT, Grant Nos. 4.10 and CB-2014-22117; U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357; and U.S. National Science Foundation, Grant No. NSF-PHY1206187. NR 63 TC 6 Z9 6 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 15 PY 2016 VL 93 IS 7 AR 074017 DI 10.1103/PhysRevD.93.074017 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ6DC UT WOS:000374299200001 ER PT J AU Meyer, ER Ticknor, C Kress, JD Collins, LA AF Meyer, Edmund R. Ticknor, Christopher Kress, Joel D. Collins, Lee A. TI Alternative first-principles calculation of entropy for liquids SO PHYSICAL REVIEW E LA English DT Article ID 2-PHASE THERMODYNAMIC MODEL; INITIO MOLECULAR-DYNAMICS; ITINERANT-OSCILLATOR MODEL; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; ABSOLUTE ENTROPY; BASIS-SET; SIMULATIONS; METALS; FLUID AB We present an alternative method for interpreting the velocity autocorrelation function (VACF) of a fluid with application to extracting the entropy in a manner similar to the methods developed by Lin et al. [J. Chem. Phys. 119, 11792 (2003)] and improved upon by Desjarlais [Phys. Rev. E 88, 062145 (2013)]. The liquid VACF is decomposed into two components, one gas and one solid, and each contribution's entropic portion is calculated. However, we fit both the gas and solid portions of the VACF in the time domain. This approach is applied to a single-component liquid (a two-phase model of liquid Al at the melt line) and two different two-component systems: a superionic-to-superionic (bcc to fcc) phase transition in H2O at high temperatures and pressures and a metastable liquid state of MgO. For all three examples, comparisons to existing results in the literature demonstrate the validity of our alternative. C1 [Meyer, Edmund R.; Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Meyer, ER (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM meyere@lanl.gov OI Ticknor, Christopher/0000-0001-9972-4524 FU US Department of Energy [DE-AC52-06NA25396] FX E.R.M. is grateful for useful and inspiring discussions with Mandy Bethkenhagen and Martin French. In addition, E.R.M. thanks Michael Desjarlais for providing his data on aluminum for comparison. The authors gratefully acknowledge support from science campaigns 1 and 4 as well as the Advanced Simulation and Computing Program. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC52-06NA25396. NR 47 TC 0 Z9 0 U1 8 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 15 PY 2016 VL 93 IS 4 AR 042119 DI 10.1103/PhysRevE.93.042119 PG 8 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DJ6DH UT WOS:000374299700002 PM 27176266 ER PT J AU Yasuda, H Chong, C Charalampidis, EG Kevrekidis, PG Yang, J AF Yasuda, H. Chong, C. Charalampidis, E. G. Kevrekidis, P. G. Yang, J. TI Formation of rarefaction waves in origami-based metamaterials SO PHYSICAL REVIEW E LA English DT Article ID DISCRETE BREATHERS; GEOMETRY AB We investigate the nonlinear wave dynamics of origami-based metamaterials composed of Tachi-Miura polyhedron (TMP) unit cells. These cells exhibit strain softening behavior under compression, which can be tuned by modifying their geometrical configurations or initial folded conditions. We assemble these TMP cells into a cluster of origami-based metamaterials, and we theoretically model and numerically analyze their wave transmission mechanism under external impact. Numerical simulations show that origami-based metamaterials can provide a prototypical platform for the formation of nonlinear coherent structures in the form of rarefaction waves, which feature a tensile wavefront upon the application of compression to the system. We also demonstrate the existence of numerically exact traveling rarefaction waves in an effective lumped-mass model. Origami-based metamaterials can be highly useful for mitigating shock waves, potentially enabling a wide variety of engineering applications. C1 [Yasuda, H.; Yang, J.] Univ Washington, Aeronaut & Astronaut, Seattle, WA 98195 USA. [Chong, C.] Swiss Fed Inst Technol, Dept Mech & Proc Engn D MAVT, CH-8092 Zurich, Switzerland. [Chong, C.] Bowdoin Coll, Dept Math, Brunswick, ME 04011 USA. [Charalampidis, E. G.; Kevrekidis, P. G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Ctr Nonlinear Studies, POB 1663, Los Alamos, NM 87544 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. RP Yang, J (reprint author), Univ Washington, Aeronaut & Astronaut, Seattle, WA 98195 USA. EM jkyang@aa.washington.edu FU NSF [1553202, DMS-1312856]; ONR [N000141410388]; ADD of Korea [UD140059JD]; ARO [W911NF-15-1-0604]; US-AFOSR [FA9550-12-10332]; ERC [605096]; Binational (US-Israel) Science Foundation [2010239]; U.S. Department of Energy; ETH Zurich Foundation [ESC-A 06-14] FX J.Y. acknowledges the support of NSF (Grant No. 1553202), ONR (Grant No. N000141410388), and ADD of Korea (Grant No. UD140059JD). J.Y. and P.G.K. acknowledge the support of ARO (Grant No. W911NF-15-1-0604). E.G.C. and P.G.K. acknowledge support from the US-AFOSR under Grant No. FA9550-12-10332. P.G.K. also acknowledges support from the NSF under Grant No. DMS-1312856, from ERC and FP7-People under Grant No. 605096, and from the Binational (US-Israel) Science Foundation through Grant No. 2010239. P.G.K.'s work at Los Alamos is supported in part by the U.S. Department of Energy. The work of C.C. was partially supported by the ETH Zurich Foundation through the Seed Project No. ESC-A 06-14. NR 32 TC 2 Z9 2 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 15 PY 2016 VL 93 IS 4 AR 043004 DI 10.1103/PhysRevE.93.043004 PG 11 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DJ6DH UT WOS:000374299700007 PM 27176382 ER PT J AU Ruestes, CJ Farkas, D Caro, A Bringa, EM AF Ruestes, Carlos J. Farkas, Diana Caro, Alfredo Bringa, Eduardo M. TI Hardening under compression in Au foams SO ACTA MATERIALIA LA English DT Article DE Nanofoams; Simulation; Densification; Plasticity ID NANOPOROUS GOLD; MECHANICAL-BEHAVIOR; YIELD STRENGTH; METALS; STABILITY AB We report the results of compressive tests for a model bi-continuous nanoporous gold structure using atomistic simulations focusing on the densification regime and the plasticity mechanisms taking place. The stress - strain response follows a logarithmic evolution proportional to the inverse of strain and we provide a simple scaling law for this behavior. Hardening is correlated to the dislocation density and an exponential dependence is revealed. The plasticity mechanisms were inspected revealing the presence of Hirth and Frank partials contributing to the hardening of the sample. Lomer-Cottrel locks, perfect dislocations, and twinning were also found. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Ruestes, Carlos J.; Bringa, Eduardo M.] Univ Nacl Cuyo, CONICET, RA-5500 Mendoza, Argentina. [Ruestes, Carlos J.; Bringa, Eduardo M.] Univ Nacl Cuyo, Fac Ciencias Exactas & Nat, RA-5500 Mendoza, Argentina. [Farkas, Diana] Virginia Polytech Inst & State Univ, Dept Mat Sci & Engn, Blacksburg, VA 24061 USA. [Caro, Alfredo] Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87544 USA. RP Ruestes, CJ (reprint author), Univ Nacl Cuyo, CONICET, RA-5500 Mendoza, Argentina.; Ruestes, CJ (reprint author), Univ Nacl Cuyo, Fac Ciencias Exactas & Nat, RA-5500 Mendoza, Argentina. EM cjruestes@hotmail.com FU ANPCyT [PICT-2014-0696]; SeCTyP UNCuyo [M003]; MATE - MCC; LDRD program at LANL FX EMB and CJR thank funding from ANPCyT grant PICT-2014-0696 and SeCTyP UNCuyo grant M003. CJR thanks MATE support by MCC. AC acknowledges support from the LDRD program at LANL. NR 41 TC 2 Z9 2 U1 6 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 15 PY 2016 VL 108 BP 1 EP 7 DI 10.1016/j.actamat.2016.02.030 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DJ2YZ UT WOS:000374072700001 ER PT J AU Khairallah, SA Anderson, AT Rubenchik, A King, WE AF Khairallah, Saad A. Anderson, Andrew T. Rubenchik, Alexander King, Wayne E. TI Laser powder-bed fusion additive manufacturing: Physics of complex melt flow and formation mechanisms of pores, spatter, and denudation zones SO ACTA MATERIALIA LA English DT Article DE Selective laser melting; Laser powder bed fusion; Additive manufacturing; 3D printing; Metal; Defect; Computer simulations; Heat flow; Solidification ID STAINLESS-STEEL; TI-6AL-4V; RADIATION; METAL AB This study demonstrates the significant effect of the recoil pressure and Marangoni convection in laser powder bed fusion (L-PBF) of 316L stainless steel. A three-dimensional high fidelity powder-scale model reveals how the strong dynamical melt flow generates pore defects, material spattering (sparking), and denudation zones. The melt track is divided into three sections: a topological depression, a transition and a tail region, each being the location of specific physical effects. The inclusion of laser ray-tracing energy deposition in the powder-scale model improves over traditional volumetric energy deposition. It enables partial particle melting, which impacts pore defects in the denudation zone. Different pore formation mechanisms are observed at the edge of a scan track, at the melt pool bottom (during collapse of the pool depression), and at the end of the melt track (during laser power ramp down). Remedies to these undesirable pores are discussed. The results are validated against the experiments and the sensitivity to laser absorptivity is discussed. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Khairallah, Saad A.; Anderson, Andrew T.; Rubenchik, Alexander; King, Wayne E.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Khairallah, SA (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM khairallah1@llnl.gov; anderson1@lln.gov; rubenchik1@llnl.gov; king17@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program [13-SI-002] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work was funded by the Laboratory Directed Research and Development Program under project tracking code 13-SI-002. The LLNL document review and release number is LLNL-JRNL-676495. NR 38 TC 20 Z9 20 U1 70 U2 159 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 15 PY 2016 VL 108 BP 36 EP 45 DI 10.1016/j.actamat.2016.02.014 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DJ2YZ UT WOS:000374072700005 ER PT J AU Nisoli, C Zong, HX Niezgoda, SR Brown, DW Lookman, T AF Nisoli, Cristiano Zong, Hongxiang Niezgoda, Stephen R. Brown, Donald W. Lookman, Turab TI Long-time behavior of the omega -> alpha transition in shocked zirconium: Interplay of nucleation and plastic deformation SO ACTA MATERIALIA LA English DT Article DE Activation energy; Martensitic transition; Zirconium; Phase transformation; Kinetics; Coalescence and Growth ID MARTENSITIC TRANSFORMATIONS; PHASE-TRANSFORMATION; TITANIUM; PRESSURES; MECHANISM; KINETICS; MODEL; ZR AB We study the thermally activated, slow conversion of the hysteretically retained omega phase into stable a phase in recovered samples of shocked zirconium. The co-phase decays in time following an algebraic law, unlike the predictions of the nucleation-growth framework for first order transitions, and residual volume fractions of phases and dislocation densities are related by a power law. We propose an explanation for the annealing mechanism through coupled dynamics of dislocations and phase change. We find that the long-time behavior is controlled by the interplay of dislocations, shear fluctuations, and remnant volume fractions of phases, which lead to an algebraic decay in time. For late time, thermally activated quantities such as the dislocation mobility and nucleation rate set the timescale and control the algebraic behavior, respectively. At high enough temperatures this behavior is effectively indistinguishable from standard Avrami kinetics. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Nisoli, Cristiano; Zong, Hongxiang; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Niezgoda, Stephen R.; Brown, Donald W.] Los Alamos Natl Lab, MST Div, POB 1663, Los Alamos, NM 87545 USA. [Niezgoda, Stephen R.] Ohio State Univ, Dept Mat Sci & Engn, 116 W 19Th Ave, Columbus, OH 43210 USA. RP Nisoli, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cristiano.nisoli@gmail.com OI Nisoli, Cristiano/0000-0003-0053-1023 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DEAC52-06NA25396] FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DEAC52-06NA25396. NR 31 TC 1 Z9 2 U1 0 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 15 PY 2016 VL 108 BP 138 EP 142 DI 10.1016/j.actamat.2016.02.009 PG 5 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DJ2YZ UT WOS:000374072700013 ER PT J AU Cakmak, E Kirka, MM Watkins, TR Cooper, RC An, K Choo, H Wu, W Dehoff, RR Babu, SS AF Cakmak, Ercan Kirka, Michael M. Watkins, Thomas R. Cooper, Ryan C. An, Ke Choo, Hahn Wu, Wei Dehoff, Ryan R. Babu, Sudarsanam S. TI Microstructural and micromechanical characterization of IN718 theta shaped specimens built with electron beam melting SO ACTA MATERIALIA LA English DT Article DE Additive manufacturing; Nickel-based superalloys; Neutron diffraction; Texture; Lattice strains ID FLIGHT NEUTRON-DIFFRACTION; LATTICE STRAIN EVOLUTION; NICKEL-BASE SUPERALLOY; INCONEL 718; STAINLESS-STEEL; INTERGRANULAR STRAINS; MECHANICAL-PROPERTIES; PLASTIC-DEFORMATION; RESIDUAL-STRESSES; LASER DEPOSITION AB Theta-shaped specimens were additively manufactured out of Inconel 718 powders using an electron beam melting technique, as a model complex load bearing structure. Two different build strategies were employed; producing two sets of specimens. Microstructural and micro-mechanical characterizations were performed using electron back-scatter, synchrotron x-ray and in-situ neutron diffraction techniques. In particular, the cross-members of the specimens were the focus of the synchrotron x-ray and in-situ neutron diffraction measurements. The build strategies employed resulted in the formation of distinct microstructures and crystallographic textures, signifying the importance of build-parameter manipulation for microstructural optimization. Large strain anisotropy of the different lattice planes was observed during in-situ loading. Texture was concluded to have a distinct effect upon both the axial and transverse strain responses of the cross-members. In particular, the (200), (220) and (420) transverse lattice strains all showed unexpected overlapping trends in both builds. This was related to the strong (200) textures along the build/loading direction, providing agreement between the experimental and calculated results. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Cakmak, Ercan; Kirka, Michael M.; Watkins, Thomas R.; Cooper, Ryan C.; Dehoff, Ryan R.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Kirka, Michael M.; Dehoff, Ryan R.] Oak Ridge Natl Lab, Mfg Demonstrat Facil, Knoxville, TN 37932 USA. [An, Ke; Wu, Wei] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Choo, Hahn; Babu, Sudarsanam S.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Babu, Sudarsanam S.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Babu, Sudarsanam S.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. RP Cakmak, E (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM cakmake@ornl.gov RI An, Ke/G-5226-2011; Choo, Hahn/A-5494-2009; Dehoff, Ryan/I-6735-2016; Watkins, Thomas/D-8750-2016; OI An, Ke/0000-0002-6093-429X; Choo, Hahn/0000-0002-8006-8907; Dehoff, Ryan/0000-0001-9456-9633; Watkins, Thomas/0000-0002-2646-1329; Wu, Wei/0000-0002-8596-9253 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office [DE-AC05-00OR22725]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; UT-Battelle, LLC FX This research was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U. S. Department of Energy. Research at MDF was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office, under contract DE-AC05-00OR22725 with UT-Battelle, LLC. The research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. EC and TRW would like to thank Mr. Tom Geer for metallographic sample preparation. EC would also like to acknowledge Dr. Olaf J. Borkiewicz for his helps during the measurements at APS. NR 55 TC 0 Z9 0 U1 32 U2 66 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 15 PY 2016 VL 108 BP 161 EP 175 DI 10.1016/j.actamat.2016.02.005 PG 15 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DJ2YZ UT WOS:000374072700016 ER PT J AU Wang, JJ Huang, HB Bayer, TJM Moballegh, A Cao, Y Klein, A Dickey, EC Irving, DL Randall, CA Chen, LQ AF Wang, Jian-Jun Huang, Hou-Bing Bayer, Thorsten J. M. Moballegh, Ali Cao, Ye Klein, Andreas Dickey, Elizabeth C. Irving, Douglas L. Randall, Clive A. Chen, Long-Qing TI Defect chemistry and resistance degradation in Fe-doped SrTiO3 single crystal SO ACTA MATERIALIA LA English DT Article DE Resistance degradation; SrTiO3; Defect transport; Defect; Chemistry; Oxygen vacancies ID DC ELECTRICAL DEGRADATION; PEROVSKITE-TYPE TITANATES; RESISTIVE SWITCHING MEMORIES; TRANSITION-METAL OXIDES; STRONTIUM-TITANATE; OXYGEN NONSTOICHIOMETRY; INSULATION RESISTANCE; DIELECTRIC EVOLUTION; BARIUM-TITANATE; MOTT TRANSITION AB Defect chemistry and transport in Fe-doped SrTiO3 single crystal are studied to understand its resistance degradation mechanism. The temporal evolution of electric conductivity under a voltage stress was obtained computationally by solving the transport equations for ionic and electronic defects coupled with the defect reaction equilibrium equations. The computational results are compared to the corresponding experimental measurement under similar conditions. It is shown that the local electron and hole concentrations are controlled by the local electronic defect equilibria rather than by their quasi steady state diffusional transport. It is the electric field-induced migration of oxygen vacancies and the subsequent instantaneous reestablishment of the local defect equilibria that lead to the resistance degradation. The resistance degradation behavior and the defect distributions under a long-term voltage stress are strongly influenced by the sample-annealing oxygen partial pressure, degrading electric field, and temperature. The present study contributes to the understanding of resistance degradation mechanism and provides guidance to improve the lifetime and reliability of wide band-gap semiconducting capacitors. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Wang, Jian-Jun; Huang, Hou-Bing; Bayer, Thorsten J. M.; Randall, Clive A.; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Moballegh, Ali; Dickey, Elizabeth C.; Irving, Douglas L.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27606 USA. [Cao, Ye] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Klein, Andreas] Tech Univ Darmstadt, Dept Mat & Earth Sci, Div Surface Sci, Jovanka Bontschits Str 2, D-64287 Darmstadt, Germany. [Huang, Hou-Bing] Univ Sci & Technol Beijing, Dept Phys, Beijing 100083, Peoples R China. RP Wang, JJ; Huang, HB (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. EM wjj8384@gmail.com; hbhuang@ustb.edu.cn RI Klein, Andreas/E-6081-2010; Cao, Ye/L-1271-2016; Dickey, Elizabeth/A-3368-2011; OI Klein, Andreas/0000-0001-7463-1495; Cao, Ye/0000-0002-7365-7447; Dickey, Elizabeth/0000-0003-4005-7872; Randall, Clive/0000-0002-5478-2699 FU Air Force Office of Scientific Research (AFOSR) [FA9550-14-1-0264, FA9550-14-1-0067]; National Science Foundation of China [11504020]; National Science Foundation [OCI-0821527]; National Energy Research Scientific Computing Center - Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Air Force Office of Scientific Research, Air Force Materiel Command, USAF [FA9550-14-1-0158] FX This work is supported by Air Force Office of Scientific Research (AFOSR) under grant number FA9550-14-1-0264 (JJW, HBH, DLI and LQC), and grant number FA9550-14-1-0067 (TB, AM, ECD, CAR). Contribution of Andreas Klein acknowledges the support from the Air Force Office of Scientific Research, Air Force Materiel Command, USAF, under Award No, FA9550-14-1-0158. H. B. Huang acknowledges the support from the National Science Foundation of China (No. 11504020). The computations were performed using the Cyberstar cluster at the Pennsylvania State University, funded by the National Science Foundation through Grant OCI-0821527, and the National Energy Research Scientific Computing Center, funded by the Office of Science of the U.S. Department of Energy through Grant DE-AC02-05CH11231. NR 57 TC 7 Z9 7 U1 25 U2 78 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 15 PY 2016 VL 108 BP 229 EP 240 DI 10.1016/j.actamat.2016.02.022 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DJ2YZ UT WOS:000374072700022 ER PT J AU Zhang, N Hu, ZG Shen, B Dang, SP Zhang, J Zhou, YH AF Zhang, Ning Hu, Zhaoguang Shen, Bo Dang, Shuping Zhang, Jian Zhou, Yuhui TI A source-grid-load coordinated power planning model considering the integration of wind power generation SO APPLIED ENERGY LA English DT Article DE Generation expansion planning; Transmission expansion planning; Source-grid-load coordinated planning; Generation-transmission-demand coordinated planning; Wind power integration capacity; Regulation constraints ID UNIT COMMITMENT; DEMAND RESPONSE; TRANSMISSION; SYSTEM; MULTIPERIOD AB Power system planning approach should meet the new requirements brought by continuous development of power systems. In recent years, wind power generation capacity keeps a rapid growth, but the problem of wind power curtailment becomes increasingly serious in some countries. The limitations of wind power integration produced by power systems, such as the inconsistency between installed generation capacity and transmission capacity and the insufficiency of regulation capacity, are drawing the attention in both academia and industry. This paper proposes a source-grid-load coordinated planning model for power systems with regulation capacity constraints being taken into account. In this novel model, traditional generation expansion planning and transmission expansion planning are integrated, and the peak-load regulation capacity and flexible regulation capability of power systems are considered. Meanwhile, the positive impacts of demand response are also taken into consideration. The numerical study verifies that the source-grid-load coordinated planning model can not only reduce the overall cost of the system, but also improve the wind power integration capacity and guarantee the sustainable development of wind power generation. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Zhang, Ning; Zhang, Jian; Zhou, Yuhui] Beijing Jiaotong Univ, Sch Elect Engn, Beijing 100044, Peoples R China. [Zhang, Ning; Hu, Zhaoguang] State Grid Corp China, State Grid Energy Res Inst, Beijing 102200, Peoples R China. [Shen, Bo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, Berkeley, CA 94720 USA. [Dang, Shuping] Univ Oxford, Dept Engn Sci, Oxford OX 13PJ, England. RP Zhang, N (reprint author), Beijing Jiaotong Univ, Sch Elect Engn, Beijing 100044, Peoples R China. EM 12121580@bjtu.edu.cn NR 31 TC 5 Z9 5 U1 9 U2 18 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD APR 15 PY 2016 VL 168 BP 13 EP 24 DI 10.1016/j.apenergy.2016.01.086 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DJ0AJ UT WOS:000373863500002 ER PT J AU Huang, S Zuo, WD Sohn, MD AF Huang, Sen Zuo, Wangda Sohn, Michael D. TI Amelioration of the cooling load based chiller sequencing control SO APPLIED ENERGY LA English DT Article DE Multiple-chiller plant; Chiller sequencing control; Model-based optimization ID REDUCING ENERGY-CONSUMPTION; SAVING ENERGY; EVOLUTION STRATEGY; GENETIC ALGORITHM; OPTIMIZATION; SYSTEMS; BUILDINGS; OPERATION; MODELS AB Cooling Load based Control (CLC) for the chiller sequencing is a commonly used control strategy for multiple-chiller plants. To improve the energy efficiency of these chiller plants, researchers proposed various CLC optimization approaches, which can be divided into two groups: studies to optimize the load distribution and studies to identify the optimal number of operating chillers. However, both groups have their own deficiencies and do not consider the impact of each other. This paper aims to improve the CLC by proposing three new approaches. The first optimizes the load distribution by adjusting the critical points for the chiller staging, which is easier to be implemented than existing approaches. In addition, by considering the impact of the load distribution on the cooling tower energy consumption and the pump energy consumption, this approach can achieve a better energy saving. The second optimizes the number of operating chillers by modulating the critical points and the condenser water set point in order to achieve the minimal energy consumption of the entire chiller plant that may not be guaranteed by existing approaches. The third combines the first two approaches to provide a holistic solution. The proposed three approaches were evaluated via a case study. The results show that the total energy consumption saving for the studied chiller plant is 0.5%, 5.3% and 5.6% by the three approaches, respectively. An energy saving of 4.9-11.8% can be achieved for the chillers at the cost of more energy consumption by the cooling towers (increases of 5.8-43.8%). The pumps' energy saving varies from 8.6% to 2.0%, depending on the approach. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Huang, Sen; Zuo, Wangda] Univ Miami, Dept Civil Architectural & Environm Engn, 1251 Mem Dr, Coral Gables, FL 33146 USA. [Sohn, Michael D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Div, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Zuo, WD (reprint author), Univ Miami, Dept Civil Architectural & Environm Engn, 1251 Mem Dr, Coral Gables, FL 33146 USA. EM w.zuo@miami.edu FU United States Department of Defense under the ESTCP program; Lawrence Berkeley National Laboratory under United States Department of Energy [DE-AC02-05CH11231] FX This research was supported by the United States Department of Defense under the ESTCP program. Michael Sohn's contributions were performed at Lawrence Berkeley National Laboratory under United States Department of Energy Contract No. DE-AC02-05CH11231. The authors thank Marco Bonvini, Michael Wetter, Mary Ann Piette, Jessica Granderson, Oren Schetrit, Rong Lily Hu, Janie Page, Michael Spears, and Guanjing Lin for the support provided through the research. NR 55 TC 2 Z9 2 U1 8 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD APR 15 PY 2016 VL 168 BP 204 EP 215 DI 10.1016/j.apenergy.2016.01.035 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DJ0AJ UT WOS:000373863500018 ER PT J AU Chiang, NY Zavala, VM AF Chiang, Nai-Yuan Zavala, Victor M. TI Large-scale optimal control of interconnected natural gas and electrical transmission systems SO APPLIED ENERGY LA English DT Article DE Large scale; Optimal control; Natural gas; Electricity; Networks; Dynamics ID NETWORKS; OPTIMIZATION AB We present a detailed optimal control model that captures spatiotemporal interactions between gas and electric transmission networks. We use the model to study flexibility and economic opportunities provided by coordination. A large-scale case study in the Illinois system reveals that coordination can enable the delivery of significantly larger amounts of natural gas to the power grid. In particular, under a coordinated setting, gas-fired generators act as distributed demand response resources that can be controlled by the gas pipeline operator. This enables more efficient control of pressures and flows in space and time and overcomes delivery bottlenecks. We demonstrate that the additional flexibility not only can benefit the gas operator but can also lead to more efficient power grid operations and results in increased revenue for gas-fired power plants. We also use the optimal control model to analyze computational issues arising in these complex models. We demonstrate that the interconnected Illinois system with full physical resolution gives rise to a highly nonlinear optimal control problem with 4400 differential and algebraic equations and 1040 controls that can be solved with a state-of-the-art sparse optimization solver. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Chiang, Nai-Yuan; Zavala, Victor M.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Zavala, VM (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM vzavala@mcs.anl.gov FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 26 TC 3 Z9 4 U1 4 U2 10 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD APR 15 PY 2016 VL 168 BP 226 EP 235 DI 10.1016/j.apenergy.2016.01.017 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DJ0AJ UT WOS:000373863500020 ER PT J AU Bhavsar, S Isenberg, N More, A Veser, G AF Bhavsar, Saurabh Isenberg, Natalie More, Amey Veser, Goetz TI Lanthana-doped ceria as active support for oxygen carriers in chemical looping combustion SO APPLIED ENERGY LA English DT Article DE Chemical looping combustion; CO2 capture; Iron; Ceria; Lanthana; Doping ID WATER-GAS-SHIFT; ELECTRICAL-PROPERTIES; METAL-OXIDES; CO2 CAPTURE; IRON-OXIDE; CATALYTIC-PROPERTIES; PARTIAL OXIDATION; ION CONDUCTIVITY; REDOX STABILITY; MIXED OXIDES AB The redox properties and oxygen buffering capacity of reducible oxides, such as ceria, make them interesting support materials for oxygen carriers in Chemical Looping Combustion (CLC), an emerging clean combustion technology. However, the effectiveness of reducible oxides for redox applications depends crucially on oxygen mobility in the oxide lattice. In the present work, we demonstrate that addition of an aliovalent dopant (La) strongly enhances oxygen mobility in ceria, resulting in multiple performance benefits. A series of La-doped ceria (LaxCe1-xO2-x-2, 0 < x < 0.3) were investigated as supports for low-cost Fe-based oxygen carrier materials. Combining carrier synthesis and characterization with reactive tests, we demonstrate that La doping of ceria not only results in a drastic improvements in carrier reactivity and oxygen carrying capacity, but also strongly improved carrier stability during redox cycling. This is consistent with the creation of oxygen defects, which stabilize the supported Fe particles and facilitate oxygen transport in the ceria lattice. A balance between enhancement of oxygen mobility and lowered reducibility upon formation of a lanthana phase results in a strongly nonlinear dependence of carrier reactivity on the dopant concentration and gives rise to an optimum at low dopant concentrations. Overall, the results suggest that doping of reducible supports constitutes a highly attractive, effective, and low-cost way to strongly enhance the performance of oxygen carriers in chemical looping applications. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Bhavsar, Saurabh; Isenberg, Natalie; More, Amey; Veser, Goetz] Univ Pittsburgh, Dept Chem Engn, Swanson Sch Engn, Pittsburgh, PA 15261 USA. [Bhavsar, Saurabh; Veser, Goetz] US DOE, Natl Energy Technol Lab, Pittsburgh, PA USA. RP Veser, G (reprint author), Univ Pittsburgh, Dept Chem Engn, Swanson Sch Engn, Pittsburgh, PA 15261 USA. EM gveser@pitt.edu FU U.S. Department of Energy's National Energy Technology Laboratory's on-going research under the RDS contract [DE-AC26-04NT41817]; National Science Foundation (CBET) [1159853]; University of Pittsburgh's Mascaro Center for Sustainable Innovation FX This technical effort was in parts performed in support of the U.S. Department of Energy's National Energy Technology Laboratory's on-going research under the RDS contract DE-AC26-04NT41817. Furthermore, financial support by the National Science Foundation (CBET #1159853) and by the University of Pittsburgh's Mascaro Center for Sustainable Innovation is gratefully acknowledged. NR 65 TC 0 Z9 0 U1 7 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD APR 15 PY 2016 VL 168 BP 236 EP 247 PG 12 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DJ0AJ UT WOS:000373863500021 ER PT J AU Cole, W Lewis, H Sigrin, B Margolis, R AF Cole, Wesley Lewis, Haley Sigrin, Ben Margolis, Robert TI Interactions of rooftop PV deployment with the capacity expansion of the bulk power system SO APPLIED ENERGY LA English DT Article DE Rooftop PV adoption; Capacity expansion modeling; Grid integration; ReEDS; dSolar ID GREENHOUSE-GAS EMISSIONS; PHOTOVOLTAIC ELECTRICITY-GENERATION; NET-METERED PV; RENEWABLE ELECTRICITY; FINANCIAL IMPACTS; UNITED-STATES; UTILITIES; SOLAR; US; PENETRATION AB Distribution-sited solar photovoltaics (PV) economics (including rooftop PV) have improved significantly during the past several years, spurring increased installations, with over 2.2 GW installed in 2014 in the United States. This increased deployment is largely projected to continue and has prompted additional interest in the interactions of rooftop PV deployment with the greater electricity system. In this paper we focus on one piece of this interface, namely the interaction between rooftop PV deployment and the evolution of the bulk power system. We develop a novel linkage between NREL's bulk power capacity expansion model (the Renewable Energy Deployment System [ReEDS] model) and NREL's rooftop PV adoption model (the dSolar model). We use these linked models to gain insights into the interactions of rooftop PV deployment with the bulk power system. We explore two sets of scenarios. In the first set we examine how different levels of rooftop PV deployment impact the generation mix on the bulk power system. In the second set we examine how the generation mix of the bulk power system impacts the deployment of rooftop PV by applying grid-wide curtailment rates to rooftop PV systems. In these sets of scenarios, we find that rooftop PV generation and utility PV generation have a nearly 1:1 substitution effect. We also find that curtailment rate feedback can have dramatic impacts on rooftop PV adoption, though the range of impacts is strongly dependent on the generation mix of the bulk power system and the amount of total PV generation in the system. For example, scenarios with more natural gas generation tended to have lower curtailment rates and thus more rooftop PV deployment. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Cole, Wesley; Lewis, Haley; Sigrin, Ben; Margolis, Robert] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO 80401 USA. RP Cole, W (reprint author), Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO 80401 USA. EM wesley.cole@nrel.gov FU Solar Energy Technologies Office of the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy [DE-AC36-08GO28308]; U.S. Department of Energy Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships (SULI) program FX This work was supported by Solar Energy Technologies Office of the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy under contract number DE-AC36-08GO28308 and by the U.S. Department of Energy Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Science Undergraduate Laboratory Internships (SULI) program. Any errors or omissions are the sole responsibility of the authors. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 36 TC 4 Z9 4 U1 1 U2 7 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0306-2619 EI 1872-9118 J9 APPL ENERG JI Appl. Energy PD APR 15 PY 2016 VL 168 BP 473 EP 481 DI 10.1016/j.apenergy.2016.02.004 PG 9 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DJ0AJ UT WOS:000373863500042 ER PT J AU Zhang, B Zheng, XL Voznyy, O Comin, R Bajdich, M Garcia-Melchor, M Han, LL Xu, JX Liu, M Zheng, LR de Arquer, FPG Dinh, CT Fan, FJ Yuan, MJ Yassitepe, E Chen, N Regier, T Liu, PF Li, YH De Luna, P Janmohamed, A Xin, HLL Yang, HG Vojvodic, A Sargent, EH AF Zhang, Bo Zheng, Xueli Voznyy, Oleksandr Comin, Riccardo Bajdich, Michal Garcia-Melchor, Max Han, Lili Xu, Jixian Liu, Min Zheng, Lirong de Arquer, F. Pelayo Garcia Dinh, Cao Thang Fan, Fengjia Yuan, Mingjian Yassitepe, Emre Chen, Ning Regier, Tom Liu, Pengfei Li, Yuhang De Luna, Phil Janmohamed, Alyf Xin, Huolin L. Yang, Huagui Vojvodic, Aleksandra Sargent, Edward H. TI Homogeneously dispersed multimetal oxygen-evolving catalysts SO SCIENCE LA English DT Article ID WATER OXIDATION; EVOLUTION REACTION; PEROVSKITE PHOTOVOLTAICS; NI; ELECTROCATALYSTS; CRYSTALLINE; CO; OXIDES AB Earth-abundant first-row (3d) transition metal-based catalysts have been developed for the oxygen-evolution reaction (OER); however, they operate at overpotentials substantially above thermodynamic requirements. Density functional theory suggested that non-3d high-valency metals such as tungsten can modulate 3d metal oxides, providing nearoptimal adsorption energies for OER intermediates. We developed a room-temperature synthesis to produce gelled oxyhydroxides materials with an atomically homogeneous metal distribution. These gelled FeCoW oxyhydroxides exhibit the lowest overpotential (191 millivolts) reported at 10 milliamperes per square centimeter in alkaline electrolyte. The catalyst shows no evidence of degradation after more than 500 hours of operation. X-ray absorption and computational studies reveal a synergistic interplay between tungsten, iron, and cobalt in producing a favorable local coordination environment and electronic structure that enhance the energetics for OER. C1 [Zhang, Bo; Zheng, Xueli; Voznyy, Oleksandr; Comin, Riccardo; Xu, Jixian; Liu, Min; de Arquer, F. Pelayo Garcia; Dinh, Cao Thang; Fan, Fengjia; Yuan, Mingjian; Yassitepe, Emre; De Luna, Phil; Janmohamed, Alyf; Sargent, Edward H.] Univ Toronto, Dept Elect & Comp Engn, 35 St George St, Toronto, ON M5S 1A4, Canada. [Zhang, Bo] E China Univ Sci & Technol, Dept Phys, 130 Meilong Rd, Shanghai 200237, Peoples R China. [Zheng, Xueli] Tianjin Univ, Sch Mat Sci & Engn, Tianjin Key Lab Composite & Funct Mat, Tianjin 300072, Peoples R China. [Bajdich, Michal; Garcia-Melchor, Max; Vojvodic, Aleksandra] Stanford Univ, Dept Chem Engn, SUNCAT Ctr Interface Sci & Catalysis, Stanford, CA 94305 USA. [Bajdich, Michal; Garcia-Melchor, Max; Vojvodic, Aleksandra] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Han, Lili; Xin, Huolin L.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Zheng, Lirong] Chinese Acad Sci, Beijing Synchrotron Radiat Facil, Inst High Energy Phys, Beijing 100049, Peoples R China. [Chen, Ning; Regier, Tom] Canadian Light Source CLS, 44 Innovation Blvd, Saskatoon, SK S7N 2V3, Canada. [Liu, Pengfei; Li, Yuhang; Yang, Huagui] E China Univ Sci & Technol, Sch Mat Sci & Engn, Key Lab Ultrafine Mat, Minist Educ, 130 Meilong Rd, Shanghai 200237, Peoples R China. RP Sargent, EH (reprint author), Univ Toronto, Dept Elect & Comp Engn, 35 St George St, Toronto, ON M5S 1A4, Canada.; Vojvodic, A (reprint author), Stanford Univ, Dept Chem Engn, SUNCAT Ctr Interface Sci & Catalysis, Stanford, CA 94305 USA.; Vojvodic, A (reprint author), SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM alevoj@stanford.edu; ted.sargent@utoronto.ca RI Comin, Riccardo/H-7731-2016; Liu, Min/H-3699-2011; Xin, Huolin/E-2747-2010; Garcia-Melchor, Max/D-3046-2017; OI Comin, Riccardo/0000-0002-1069-9973; Liu, Min/0000-0002-9007-4817; Xin, Huolin/0000-0002-6521-868X; Garcia-Melchor, Max/0000-0003-1348-4692; Vojvodic, Aleksandra/0000-0002-5584-6711 FU Ontario Research Fund-Research Excellence Program; Natural Sciences and Engineering Research Council of Canada; Canadian Insititute for Advanced Research Bio-Inspired Solar Energy program; China Scholarship Council/University of Toronto [201406745001]; Shanghai Municipal Natural Science Foundation [14ZR1410200]; National Natural Science Foundation of China [21503079]; China Scholarship Council (CSC) [20140625004]; U.S. Department of Energy (DOE), Office of Basic Energy Science; Laboratory-Directed Research and Development program through the SLAC National Accelerator Laboratory; Agency for Administration of University and Research Grants of Catalonia (AGAUR) [2013 BP-A 00464]; Center for Functional Nanomaterials, DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704]; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo-Bolsa Estagio de Pesquisa no Exterior fellowship [2014/18327-9]; Connaught Global Challenge program of the University of Toronto FX This work was supported by the Ontario Research Fund-Research Excellence Program, Natural Sciences and Engineering Research Council of Canada, and the Canadian Insititute for Advanced Research Bio-Inspired Solar Energy program. B. Z. acknowledges funding from China Scholarship Council/University of Toronto Joint Funding Program (201406745001), Shanghai Municipal Natural Science Foundation (14ZR1410200), and the National Natural Science Foundation of China (21503079). X.Z. acknowledges a scholarship from the China Scholarship Council (CSC) (20140625004). This work was also supported by the U.S. Department of Energy (DOE), Office of Basic Energy Science grant to the SUNCAT Center for Interface Science and Catalysis and the Laboratory-Directed Research and Development program funded through the SLAC National Accelerator Laboratory. M.G.-M. acknowledges funding from the Agency for Administration of University and Research Grants of Catalonia (AGAUR, 2013 BP-A 00464). This work has also benefited from the Hard X-ray Micro-Analysis and Spherical Grating Monochromator beamlines at CLS and the BL14W1 beamline at the Shanghai Synchrotron Radiation Facility (SSRF). B. Z. and R. C. acknowledge the CLS Post-Doctoral Student Travel Support Program. The TEM study in this work is supported by the Center for Functional Nanomaterials, which is a DOE Office of Science Facility, at Brookhaven National Laboratory under contract DE-SC0012704. E. Y. acknowledges a Fundacao de Amparo a Pesquisa do Estado de Sao Paulo-Bolsa Estagio de Pesquisa no Exterior (2014/18327-9) fellowship. E. H. S. and F.P.G.A acknowledge funding from the Connaught Global Challenge program of the University of Toronto. The authors thank D. Belanger and G. Chamoulaud at Universite du Quebec a Montreal for assistance in EQCM measurements and T.-O. Do and C.-C. Nguyen at Laval University for surface area analysis. The authors thank Y. J. Pang, X. Lan, L. N. Quan, and S. Hoogland for fruitful discussions; M. X. Liu and X. W. Gong for fabrication assistance; and R. Wolowiec and D. Kopilovic for assistance. B. Z., X. Z., J.X., M.L., C.T.D, and E.H.S. of the University of Toronto have filed provisional patent application no. 62288648 regarding the preparation of multimetal catalysts for oxygen evolution. NR 29 TC 51 Z9 51 U1 169 U2 383 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD APR 15 PY 2016 VL 352 IS 6283 BP 333 EP 337 DI 10.1126/science.aaf1525 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ1UK UT WOS:000373990100038 PM 27013427 ER PT J AU Wilding, MC Wilson, M Alderman, OLG Benmore, C Weber, JKR Parise, JB Tamalonis, A Skinner, L AF Wilding, Martin C. Wilson, Mark Alderman, Oliver L. G. Benmore, Chris Weber, J. K. R. Parise, John B. Tamalonis, Anthony Skinner, Lawrie TI Low-Dimensional Network Formation in Molten Sodium Carbonate SO SCIENTIFIC REPORTS LA English DT Article ID ALKALI CARBONATES; NEUTRON-DIFFRACTION; SILICATE MELTS; TETRASILICATE GLASS; COMPUTER-SIMULATION; X-RAY; DYNAMICS; DISILICATE; LIQUID; SCATTERING AB Molten carbonates are highly inviscid liquids characterized by low melting points and high solubility of rare earth elements and volatile molecules. An understanding of the structure and related properties of these intriguing liquids has been limited to date. We report the results of a study of molten sodium carbonate (Na2CO3) which combines high energy X-ray diffraction, containerless techniques and computer simulation to provide insight into the liquid structure. Total structure factors (F-x(Q)) are collected on the laser-heated carbonate spheres suspended in flowing gases of varying composition in an aerodynamic levitation furnace. The respective partial structure factor contributions to Fx(Q) are obtained by performing molecular dynamics simulations treating the carbonate anions as flexible entities. The carbonate liquid structure is found to be heavily temperature-dependent. At low temperatures a low-dimensional carbonate chain network forms, at T = 1100 K for example similar to 55% of the C atoms form part of a chain. The mean chain lengths decrease as temperature is increased and as the chains become shorter the rotation of the carbonate anions becomes more rapid enhancing the diffusion of Na+ ions. C1 [Wilding, Martin C.] Univ Bath, Dept Phys, Bath BA2 7AY, Avon, England. [Wilson, Mark] Univ Oxford, Dept Chem, Phys & Theoret Chem Lab, S Parks Rd, Oxford OX1 3QZ, England. [Alderman, Oliver L. G.; Benmore, Chris; Weber, J. K. R.; Skinner, Lawrie] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Alderman, Oliver L. G.; Weber, J. K. R.; Tamalonis, Anthony; Skinner, Lawrie] Mat Dev Inc, Arlington Hts, IL 60004 USA. [Parise, John B.; Skinner, Lawrie] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Parise, John B.; Skinner, Lawrie] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Wilding, MC (reprint author), Univ Bath, Dept Phys, Bath BA2 7AY, Avon, England. EM mark.wilson@chem.ox.ac.uk OI Benmore, Chris/0000-0001-7007-7749; Alderman, Oliver/0000-0002-2342-811X FU DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; [DE-SC0007564] FX This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. J.K.R.W., O.L.G.A. and A.T. were funded under grant number DE-SC0007564. NR 37 TC 1 Z9 1 U1 5 U2 18 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 15 PY 2016 VL 6 AR 24415 DI 10.1038/srep24415 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ4HP UT WOS:000374166300001 PM 27080401 ER PT J AU Holmstrom, E Haberl, B Pakarinen, OH Nordlund, K Djurabekova, F Arenal, R Williams, JS Bradby, JE Petersen, TC Liu, ACY AF Holmstrom, E. Haberl, B. Pakarinen, O. H. Nordlund, K. Djurabekova, F. Arenal, R. Williams, J. S. Bradby, J. E. Petersen, T. C. Liu, A. C. Y. TI Dependence of short and intermediate-range order on preparation in experimental and modeled pure a-Si SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Amorphous Si; Preparation history; Irradiation; Indentation; Molecular dynamics ID MOLECULAR-DYNAMICS SIMULATIONS; DIAMOND-LIKE CARBON; AMORPHOUS-SILICON; STRUCTURAL RELAXATION; PHASE-TRANSFORMATIONS; NETWORK DISORDER; LOCAL-STRUCTURE; INDENTATION; CRYSTALLINE; GERMANIUM AB Variability in the short-intermediate range order of pure amorphous Si synthesized by-different experimental and computational techniques is probed by measuring mass density, atomic coordination, bond-angle deviation, and dihedral angle deviation. It is found that there is significant variability in order parameters at these length scales in this archetypal covalently bonded, monoatomic system. This diversity strongly reflects preparation method and thermal history in both experimental and simulated systems. Where experiment and simulation do not quantitatively agree, this is partly due to inherent differences in analysis and time scales. Relaxed forms of amorphous Si quantitatively match continuous random networks generated by a hybrid method of bond switching Monte Carlo and molecular dynamics simulation. Qualitative trends were identified in other experimental and computed forms of a-Si. Ion-implanted a-Si's are less ordered than the relaxed forms. Preparation methods which narrowly avoid crystallization such as experimental pressure-induced amorphization or simulated melt-quenching result in the most disordered structures. As no unique form of amorphous Si exists, there can be no single model for the material. (C) 2016 Elsevier B.V. All rights reserved. C1 [Holmstrom, E.; Pakarinen, O. H.; Nordlund, K.; Djurabekova, F.] Univ Helsinki, Dept Phys, POB 64, FIN-00014 Helsinki, Finland. [Holmstrom, E.; Pakarinen, O. H.; Nordlund, K.; Djurabekova, F.] Univ Helsinki, Helsinki Inst Phys, POB 64, FIN-00014 Helsinki, Finland. [Holmstrom, E.] UCL, Dept Earth Sci, Gower St, London WC1E 6BT, England. [Holmstrom, E.] Aalto Univ, COMP Ctr Excellence, Dept Appl Phys, POB 11100, Espoo 00076, Finland. [Haberl, B.; Williams, J. S.; Bradby, J. E.] Australian Natl Univ, Res Sch Phys & Engn, Dept Elect Mat Engn, Canberra, ACT 0200, Australia. [Arenal, R.] Univ Zaragoza, INA, LMA, E-50018 Zaragoza, Spain. [Arenal, R.] Fdn ARAID, E-50004 Zaragoza, Spain. [Petersen, T. C.; Liu, A. C. Y.] Monash Univ, Sch Phys & Astron, Clayton, Vic 3800, Australia. [Liu, A. C. Y.] Monash Univ, Monash Ctr Electron Microscopy, Clayton, Vic 3800, Australia. [Haberl, B.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Holmstrom, E (reprint author), Univ Helsinki, Dept Phys, POB 64, FIN-00014 Helsinki, Finland.; Holmstrom, E (reprint author), Univ Helsinki, Helsinki Inst Phys, POB 64, FIN-00014 Helsinki, Finland. EM bianca.haberl@gmail.com RI Haberl, Bianca/F-9058-2011; Arenal, Raul/D-2065-2009; OI Haberl, Bianca/0000-0002-7391-6031; Arenal, Raul/0000-0002-2071-9093; Pakarinen, Olli/0000-0002-5535-3941; Djurabekova, Flyura/0000-0002-5828-200X; Nordlund, Kai/0000-0001-6244-1942 FU Alvin M. Weinberg Fellowship (ORNL); U.S. Department of Energy, Office of Basic Energy Sciences; Margaret Clayton Women In Research Fellowship; Science Faculty, Monash University; Monash Centre for Electron Microscopy; Australian Research Council; Academy of Finland; CSC - IT Center for Science Ltd. (Finland); Academy of Finland through the Centres of Excellence Program [251748] FX BH gratefully acknowledges funding from an Alvin M. Weinberg Fellowship (ORNL) and through the Spallation Neutron Source, sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences. ACYL wishes to acknowledge the support of the Margaret Clayton Women In Research Fellowship, the Science Faculty, Monash University and the Monash Centre for Electron Microscopy. BH and ACYL thank Vicki Keast for discussions on treatment of low-loss EELS spectra and Nestor Zaluzec for assistance with initial electron diffraction measurements at Argonne National Laboratory. JEB acknowledges funding from the Australian Research Council Future Fellowship scheme. The authors acknowledge use of facilities within the Monash Centre for Electron Microscopy and the Electron Microscopy Center, Argonne National Laboratory. OHP gratefully acknowledges funding from the Academy of Finland and grants of computation time from CSC - IT Center for Science Ltd. (Finland). EH gratefully acknowledges generous grants of computing time on the Ametisti cluster at the University of Helsinki and the Vuori HP CP4000 BL ProLiant supercluster at CSC. We acknowledge financial support by the Academy of Finland through the Centres of Excellence Program (Project No. 251748). NR 99 TC 2 Z9 2 U1 6 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD APR 15 PY 2016 VL 438 BP 26 EP 36 DI 10.1016/j.jnoncrysol.2016.02.008 PG 11 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA DI5NG UT WOS:000373545300005 ER PT J AU Abhishek, A Warrier, M Ganesh, R Caro, A AF Abhishek, A. Warrier, M. Ganesh, R. Caro, A. TI Growth and structural determination of He bubbles in iron/chromium alloys using molecular dynamics simulations SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Molecular dynamics; He bubble; Theory and modeling ID FE AB Helium(He) produced by transmutation process inside structural material due to neutron irradiation plays a vital role in the degradation of material properties. We have carried out Molecular dynamics(MD) simulations to study the growth of He bubble in Iron-Chromium alloy. Simulations are carried out at two different temperatures, viz. 0.1 K and 800 K, upto He bubble radius of 2.5 nm. An equation for variation of volume of He bubbles with the number of He atoms is obtained at both the temperatures. Bubble pressure and potential energy variation is obtained with increasing bubble radius. Dislocations are also found to be emitted after the bubble reaches a critical radius of 0.39 nm at 800 K. Separate MD simulations of He with pre-created voids are also carried out to study the binding energies of He and Vacancy (V) to Hem-Vn cluster. Binding energies are found to be in the range of 1-5.5 eV. (C) 2016 Elsevier B.V. All rights reserved. C1 [Abhishek, A.; Ganesh, R.] BHAT, Inst Plasma Res, Gandhinagar 382428, Gujarat, India. [Warrier, M.] BARC, Computat Anal Div, Visakhapatnam 530012, Andhra Pradesh, India. [Caro, A.] Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87544 USA. RP Abhishek, A (reprint author), BHAT, Inst Plasma Res, Gandhinagar 382428, Gujarat, India. EM agraj.abhi@gmail.com NR 14 TC 0 Z9 0 U1 5 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 15 PY 2016 VL 472 BP 82 EP 88 DI 10.1016/j.jnucmat.2016.02.001 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DI4SN UT WOS:000373489700011 ER PT J AU Behera, RK Watanabe, T Andersson, DA Uberuaga, BP Deo, CS AF Behera, Rakesh K. Watanabe, Taku Andersson, David A. Uberuaga, Blas P. Deo, Chaitanya S. TI Diffusion of oxygen interstitials in UO2+x using kinetic Monte Carlo simulations: Role of O/M ratio and sensitivity analysis SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE UO2+x; UO2; Defects; Diffusion; Sensitivity analysis; DFT; kMC ID URANIUM-DIOXIDE; THERMOPHYSICAL PROPERTIES; DEFECT STRUCTURE; SELF-DIFFUSION; OXIDATION; DYNAMICS; OXIDES; U4O9 AB Oxygen interstitials in UO2+x significantly affect the thermophysical properties and microstructural evolution of the oxide nuclear fuel. In hyperstoichiometric Urania (UO2+x), these oxygen interstitials form different types of defect clusters, which have different migration behavior. In this study we have used kinetic Monte Carlo (kMC) to evaluate diffusivities of oxygen interstitials accounting for mono-and diinterstitial clusters. Our results indicate that the predicted diffusivities increase significantly at higher non-stoichiometry (x > 0.01) for di-interstitial clusters compared to a mono-interstitial only model. The diffusivities calculated at higher temperatures compare better with experimental values than at lower temperatures (< 973 K). We have discussed the resulting activation energies achieved for diffusion with all the mono-and di-interstitial models. We have carefully performed sensitivity analysis to estimate the effect of input di-interstitial binding energies on the predicted diffusivities and activation energies. While this article only discusses mono-and di-interstitials in evaluating oxygen diffusion response in UO2+x, future improvements to the model will primarily focus on including energetic definitions of larger stable interstitial clusters reported in the literature. The addition of larger clusters to the kMC model is expected to improve the comparison of oxygen transport in UO2+x with experiment. (C) 2016 Elsevier B.V. All rights reserved. C1 [Behera, Rakesh K.; Deo, Chaitanya S.] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Nucl & Radiol Engn Program, Atlanta, GA 30332 USA. [Watanabe, Taku] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Andersson, David A.; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Behera, Rakesh K.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Watanabe, Taku] Samsung R&D Inst, Osaka, Japan. RP Behera, RK; Deo, CS (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, Nucl & Radiol Engn Program, Atlanta, GA 30332 USA.; Behera, RK (reprint author), Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. EM rakesh.behera@gatech.edu; chaitanya.deo@me.gatech.edu FU DOE Office of Nuclear Energy's Nuclear Energy University Programs; U.S. Department of Energy, Office of Nuclear Energy, Nuclear Energy Advanced Modeling and Simulation (NEAMS) program FX This research is being performed using funding received from the DOE Office of Nuclear Energy's Nuclear Energy University Programs. D.A.A. and B.P.U. were funded by the U.S. Department of Energy, Office of Nuclear Energy, Nuclear Energy Advanced Modeling and Simulation (NEAMS) program. NR 32 TC 0 Z9 0 U1 7 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 15 PY 2016 VL 472 BP 89 EP 98 DI 10.1016/j.jnucmat.2016.02.003 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DI4SN UT WOS:000373489700012 ER PT J AU Chen, CH Zhang, Y Wang, Y Crespillo, ML Fontana, CL Graham, JT Duscher, G Shannon, SC Weber, WJ AF Chen, C. -H. Zhang, Y. Wang, Y. Crespillo, M. L. Fontana, C. L. Graham, J. T. Duscher, G. Shannon, S. C. Weber, W. J. TI Dose dependence of helium bubble formation in nano-engineered SiC at 700 degrees C SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE SiC; Helium; High temperature; Irradiation effects; TEM; ERDA ID SILICON-CARBIDE COMPOSITES; ATOMIC-SCALE SIMULATION; SICF/SIC COMPOSITES; SIC/SIC COMPOSITES; DEFECT PRODUCTION; CAVITY FORMATION; ION-BEAM; SIMULTANEOUS IRRADIATION; NEUTRON-IRRADIATION; FUSION POWER AB Knowledge of radiation-induced helium bubble nucleation and growth in SiC is essential for applications in fusion and fission environments. Here we report the evolution of microstructure in nano-engineered (NE) 3C SiC, pre-implanted with helium, under heavy ion irradiation at 700 degrees C up to doses of 30 displacements per atom (dpa). Elastic recoil detection analysis confirms that the as-implanted helium depth profile does not change under irradiation to 30 dpa at 700 degrees C. While the helium bubble size distribution becomes narrower with increasing dose, the average size of bubbles remains unchanged and the density of bubbles increases somewhat with dose. These results are consistent with a long helium bubble incubation process under continued irradiation at 700 degrees C up to 30 dpa, similar to that reported under dual and triple beam irradiation at much higher temperatures. The formation of bubbles at this low temperature is enhanced by the nano-layered stacking fault structure in the NE SiC, which enhances point defect mobility parallel to the stacking faults. This stacking fault structure is stable at 700 degrees C up to 30 dpa and suppresses the formation of dislocation loops normally observed under these irradiation conditions. Published by Elsevier B.V. C1 [Chen, C. -H.; Zhang, Y.; Crespillo, M. L.; Graham, J. T.; Duscher, G.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, 210 Tandec Bldg,White Ave, Knoxville, TN 37996 USA. [Zhang, Y.; Fontana, C. L.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Wang, Y.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. [Graham, J. T.] Missouri Univ Sci & Technol, Dept Min & Nucl Engn, Rolla, MO 65409 USA. [Shannon, S. C.] N Carolina State Univ, Dept Nucl Engn, Raleigh, NC 27695 USA. RP Chen, CH (reprint author), Univ Tennessee, Dept Mat Sci & Engn, 210 Tandec Bldg,White Ave, Knoxville, TN 37996 USA.; Weber, WJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, 414 Ferris Hall, Knoxville, TN 37996 USA. EM cchen30@vols.utk.edu; wjweber@utk.edu RI Weber, William/A-4177-2008; Duscher, Gerd/G-1730-2014; OI Weber, William/0000-0002-9017-7365; Duscher, Gerd/0000-0002-2039-548X; Chen, Chien-Hung/0000-0001-8631-2133 FU U.S. Department of Energy, Nuclear Energy University Programs; University of Tennessee Governor's Chair program FX This work was supported by the U.S. Department of Energy, Nuclear Energy University Programs and the University of Tennessee Governor's Chair program. Heavy ion irradiation and ion beam analysis were performed at the University of Tennessee-Oak Ridge National Laboratory Ion Beam Materials Laboratory (IBML) located at the campus of the University of Tennessee, Knoxville. NR 57 TC 0 Z9 0 U1 9 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 15 PY 2016 VL 472 BP 153 EP 160 DI 10.1016/j.jnucmat.2016.01.029 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DI4SN UT WOS:000373489700019 ER PT J AU Guo, Q Wu, Y Ding, Y Feng, W Zhu, N AF Guo, Qiang Wu, Yong Ding, Yan Feng, Wei Zhu, Neng TI Measures to enforce mandatory civil building energy efficiency codes in China SO JOURNAL OF CLEANER PRODUCTION LA English DT Article DE Building energy code; Compliance rate; Building energy regulation; Building energy code enforcement ID LIFE-CYCLE ASSESSMENT; RESIDENTIAL BUILDINGS; CONSUMPTION; DESIGN AB Mandatory civil building energy efficiency codes strictly govern the energy consumption of new buildings in China. As the promotion of building energy efficiency in China has increased in recent years, compliance with mandatory civil building energy efficiency codes has also improved, increasing from less than 10% in 2000 to nearly 100% in 2012, a remarkable achievement. However, because the promotion of energy efficiency strategies in China has followed a unique pattern, some researchers doubt these statistics. In response to these doubts, this paper summarises and analyses the framework of measures implemented by the Chinese government to enforce mandatory building energy efficiency codes. First, the development and implementation of China's mandatory civil building energy efficiency code system is summarised. Second, the building supervision and inspection systems used to assess energy efficiency are introduced and analysed in detail in order to provide a framework for the development of energy policies in other countries. Third, the assessment and reporting processes used to determine compliance rates are reviewed. Finally, the improvement of compliance rates and its impact on building energy savings in China are discussed. Along with the increase in compliance rates in the construction stage from 71% in 2007 to 100% in 2012, the energy savings of new buildings per increased floor area per year increased from 20.4 kWh/m(2) to 28.4 kWh/m(2). The supervision and inspection systems reported in this paper are the keys to enforcing building energy efficiency codes. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Guo, Qiang; Ding, Yan; Zhu, Neng] Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China. [Wu, Yong] Minist Housing & Urban Rural Dev Peoples Republ C, Dept Sci & Technol, Beijing 100835, Peoples R China. [Feng, Wei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Ding, Y (reprint author), Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China. EM jensxing@126.com NR 62 TC 0 Z9 0 U1 2 U2 6 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0959-6526 EI 1879-1786 J9 J CLEAN PROD JI J. Clean Prod. PD APR 15 PY 2016 VL 119 BP 152 EP 166 DI 10.1016/j.jclepro.2016.02.002 PG 15 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Engineering, Environmental; Environmental Sciences SC Science & Technology - Other Topics; Engineering; Environmental Sciences & Ecology GA DH3MC UT WOS:000372690100016 ER PT J AU Zaccaria, V Tucker, D Traverso, A AF Zaccaria, V. Tucker, D. Traverso, A. TI A distributed real-time model of degradation in a solid oxide fuel cell, part I: Model characterization SO JOURNAL OF POWER SOURCES LA English DT Article DE SOFC; Real-time model; Cell degradation ID STACK DEGRADATION; SOFC; PERFORMANCE; IMPEDANCE; TEMPERATURE; ELECTRODES; ACTIVATION; MECHANISMS; LIFETIME; SULFUR AB Despite the high efficiency and flexibility of fuel cells, which make them an attractive technology for the future energy generation, their economic competitiveness is still penalized by their short lifetime, due to multiple degradation phenomena. As a matter of fact, electrochemical performance of solid oxide fuel cells (SOFCs) is reduced because of different degradation mechanisms, which depend on operating conditions, fuel and air contaminants, impurities in materials, and others. In this work, a real-time, one dimensional (1D) model of a SOFC is used to simulate the effects of voltage degradation in the cell. Different mechanisms are summarized in a simple empirical expression that relates degradation rate to cell operating parameters (current density, fuel utilization and temperature), on a localized basis. Profile distributions of different variables during cell degradation are analyzed. In particular, the effect of degradation on current density, temperature, and total resistance of the cell are investigated. An analysis of localized degradation effects shows how different parts of the cell degrade at a different time rate, and how the various profiles are redistributed along the cell as consequence of different degradation rates. Published by Elsevier B.V. C1 [Zaccaria, V.; Tucker, D.] US DOE, NETL, Morgantown, WV USA. [Traverso, A.] Univ Genoa, Thermochem Power Grp, Genoa, Italy. RP Zaccaria, V (reprint author), 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM valentina.zaccaria@netl.doe.gov FU U.S. Department of Energy Enabling Technology; National Energy Technology Laboratory FX The work was funded by the U.S. Department of Energy Enabling Technology and Partnership Program of the National Energy Technology Laboratory. The authors would like to thank Dr. Paolo Pezzini from Ames Laboratory (IA), Nor Farida Harun from Mac Master University (Canada) and Dr. Kirk Gerdes from NETL. NR 26 TC 2 Z9 2 U1 3 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD APR 15 PY 2016 VL 311 BP 175 EP 181 DI 10.1016/j.jpowsour.2016.02.040 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DH3NO UT WOS:000372693900021 ER PT J AU Kane, JJ van Rooyen, IJ Craft, AE Roney, TJ Morrell, SR AF Kane, J. J. van Rooyen, I. J. Craft, A. E. Roney, T. J. Morrell, S. R. TI Evaluating quantitative 3-D image analysis as a design tool for low enriched uranium fuel compacts for the transient reactor test facility: A preliminary study SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article DE Fuel engineering initial AB 3-D image analysis when combined with a non-destructive examination technique such as X-ray computed tomography (CT) provides a highly quantitative tool for the investigation of a material's structure. In this investigation 3-D image analysis and X-ray CT were combined to analyze the microstructure of a preliminary subsized fuel compact for the Transient Reactor Test Facility's low enriched uranium conversion program to assess the feasibility of the combined techniques for use in the optimization of the fuel block fabrication process. The quantitative image analysis focused on determining the size and spatial distribution of the surrogate fuel particles and the size, shape, and orientation of voids within the compact. Additionally, the maximum effect of microstructural features on heat transfer through the carbonaceous matrix of the preliminary compact was estimated. The surrogate fuel particles occupied 0.8% of the compact by volume with a lognormal distribution of particle sizes with a mean diameter of 39 mu m and a standard deviation of 16 mu m. Roughly 39% of the particles had a diameter greater than the specified maximum particle size of 44 tim suggesting that the particles agglomerate during fabrication. The local volume fraction of particles also varies significantly within the compact, although uniformities appear to be evenly dispersed throughout the analysed volume. The voids produced during fabrication were on average platelike in nature with their major axis oriented perpendicular to the compaction direction of the compact. Finally, the microstructure, mainly the large preferentially oriented voids, may cause a small degree of anisotropy in the thermal diffusivity within the compact. the ratio of thermal diffusivities parallel to and perpendicular to the compaction direction are expected to be no less than 0.95 with an upper bound of 1. Published by Elsevier B.V. C1 [Kane, J. J.; Craft, A. E.; Roney, T. J.] Idaho Natl Lab, Mat Sci & Engn Dept, Idaho Falls, ID 83415 USA. [van Rooyen, I. J.] Idaho Natl Lab, Fuel Performance & Design Dept, Idaho Falls, ID 83415 USA. [Morrell, S. R.] Idaho Natl Lab, Global Secur & Int Safeguards Dept, Idaho Falls, ID 83415 USA. RP Kane, JJ (reprint author), Idaho Natl Lab, Mat Sci & Engn Dept, Idaho Falls, ID 83415 USA. EM joshua.kane@inl.gov RI Craft, Aaron/B-7579-2017 OI Craft, Aaron/0000-0002-7092-3826 FU US Department of Energy, National Nuclear Security Administration; Office of Nuclear Energy of the U.S. Department of Energy [DE-AC07-05ID14517] FX This work has been performed under the auspices of and supported by the US Department of Energy, National Nuclear Security Administration. Babcock & Wilcox Nuclear Operations Group-Lynchburg are acknowledged for the experimental fuel block fabrication.; This research made use of the resources of the High Performance Computing Center at INL, which is supported by the Office of Nuclear Energy of the U.S. Department of Energy under Contract No. DE-AC07-05ID14517. The authors would like to specifically acknowledge Dr. Eric Whiting and Shane Grover for the setup and allocation of resources from the High Performance Computing Center. Additionally, the authors would like to thank Dr. Erik Luther of Los Alamos National Laboratory for his invaluable comments and feedback regarding this preliminary work. NR 11 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD APR 15 PY 2016 VL 300 BP 1 EP 11 DI 10.1016/j.nucengdes.2016.01.005 PG 11 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH5OR UT WOS:000372840400001 ER PT J AU Skavdahl, I Utgikar, VP Christensen, R Sabharwall, P Chen, M Sund, X AF Skavdahl, I. Utgikar, V. P. Christensen, R. Sabharwall, P. Chen, M. Sund, X. TI Modeling and simulation of control system response to temperature disturbances in a coupled heat exchangers-AHTR system SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article AB An effective control strategy is essential for maintaining optimum operational efficiency of the Advanced High Temperature Reactor (AHTR)-intermediate heat exchanger (IHX)-secondary heat exchanger (SHX) system for power conversion or process heat applications. A control system design is presented in this paper for the control of the coupled intermediate and secondary heat exchangers. The cold side outlet temperature of the SHX (T0) and the hot side outlet temperature of the IHX (T-h02) were identified as the controlled variables that were maintained at their set points by manipulating the flow rates of heat exchange media. Transfer functions describing the relationships between the controlled variables and the manipulated and load variables were developed and the system response to various temperature disturbances was simulated using a custom-developed MATLAB program. It was found that a step disturbance of +/- 10 degrees C in the process loop changed the thermal duty by +/- 650 kW, equal to 6.5% of the initial duty. Similar disturbances in the primary loop had a higher impact on the system. The control system design included a provision for the switching of manipulated variables to limit the adjustment in the magnitudes of the primary manipulated variables. Simulation results indicate that the controlled variables are maintained successfully at their desired points by the control system. (C) 2016 Elsevier B.V. All rights reserved. C1 [Skavdahl, I.; Utgikar, V. P.] Univ Idaho, Dept Chem & Mat Engn, Moscow, ID 83844 USA. [Christensen, R.] Univ Idaho, Nucl Engn Program, Idaho Falls, ID 83402 USA. [Sabharwall, P.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Chen, M.; Sund, X.] Ohio State Univ, Dept Mech & Aerosp Engn, Nucl Engn Program, Columbus, OH 43210 USA. RP Utgikar, VP (reprint author), Univ Idaho, Dept Chem & Mat Engn, Moscow, ID 83844 USA. EM vutgikar@uidaho.edu OI Sun, Xiaodong/0000-0002-9852-160X FU US Department of Energy through the Nuclear Energy University Program (DOE-NEUP) [128504] FX The work described in the paper was made possible by the US Department of Energy grant #128504 through the Nuclear Energy University Program (DOE-NEUP), whose support is gratefully acknowledged. NR 12 TC 2 Z9 2 U1 0 U2 2 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD APR 15 PY 2016 VL 300 BP 161 EP 172 DI 10.1016/j.nucengdes.2016.01.010 PG 12 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH5OR UT WOS:000372840400016 ER PT J AU Zou, L Zhao, HH Zhang, HB AF Zou, Ling Zhao, Haihua Zhang, Hongbin TI Application of Jacobian-free Newton-Krylov method in implicitly solving two-fluid six-equation two-phase flow problems: Implementation, validation and benchmark SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID SCHEME; MODEL AB This work represents a first-of-its-kind successful application to employ advanced numerical methods in solving realistic two-phase flow problems with two-fluid six-equation two-phase flow model. These advanced numerical methods include high-resolution spatial discretization scheme with staggered grids (high-order) fully implicit time integration schemes, and Jacobian-free Newton-Krylov (JFNK) method as the nonlinear solver. The computer code developed in this work has been extensively validated with existing experimental flow boiling data in vertical pipes and rod bundles, which cover wide ranges of experimental conditions, such as pressure, inlet mass flux, wall heat flux and exit void fraction. Additional code-to-code benchmark with the RELAP5-3D code further verifies the correct code implementation. The combined methods employed in this work exhibit strong robustness in solving two-phase flow problems even when phase appearance (boiling) and realistic discrete flow regimes are considered. Transitional flow regimes used in existing system analysis codes, normally introduced to overcome numerical difficulty, were completely removed in this work. This in turn provides the possibility to utilize more sophisticated flow regime maps in the future to further improve simulation accuracy. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zou, Ling; Zhao, Haihua; Zhang, Hongbin] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. RP Zou, L (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM ling.zou@inl.gov FU U.S. Department of Energy under Department of Energy Idaho Operations Office [DE-AC07-05ID14517] FX This work is supported by the U.S. Department of Energy, under Department of Energy Idaho Operations Office Contract DE-AC07-05ID14517. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 35 TC 2 Z9 2 U1 0 U2 1 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD APR 15 PY 2016 VL 300 BP 268 EP 281 DI 10.1016/j.nucengdes.2016.01.033 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH5OR UT WOS:000372840400025 ER PT J AU Joe, JH Kim, SJ Jones, BG AF Joe, Justin H. Kim, Seung Jun Jones, Barclay G. TI A study of solute transport of radiolysis products in crud and its effects on crud growth on PWR fuel pin SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID WATER; IRRADIATION AB This research examines the concentration of radiolysis species (H-2, O-2, and H2O2) over the porous crud layer using a three dimensional time dependent solute transport model. A Monte Carlo random walk technique is adopted to simulate the transport behavior of the different species with various parametric studies of source term, crud thickness, and crud porosity. Particularly, this model employs a system of coupled mass transport and chemical interactions as the source term, which makes the problem nonlinear. It is demonstrated that a negligible effect on radiolysis species concentrations change due to the consideration of source term. The crud thickness and porosity effect on the concentration distributions are notably observed. In general, higher concentration starts from the intersection of the heating surface with the chimney wall from the beginning and it reaches the equilibrium state within tens of seconds. The concentration profiles of the radiolysis species H-2, O-2, and H2O2 can be directly related to corrosion issues. The direct application of this study to nuclear engineering research is to aid in the design of reactors with higher performance without experiencing an Axial Offset Anomaly (AOA), an unexpected measured shift in axial power distribution from predicted values. Published by Elsevier B.V. C1 [Joe, Justin H.] BNF Consulting, Mt Kisco, NY USA. [Kim, Seung Jun] Los Alamos Natl Lab, Mech & Thermal Engn Grp AET 1, Los Alamos, NM 87545 USA. [Jones, Barclay G.] Univ Illinois, Dept Nucl Plasma Radiol Engn, Urbana, IL USA. RP Kim, SJ (reprint author), Los Alamos Natl Lab, Mech & Thermal Engn Grp AET 1, Los Alamos, NM 87545 USA. EM skim@lanl.gov OI Kim, Seung Jun/0000-0002-6913-6358 NR 17 TC 0 Z9 0 U1 2 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD APR 15 PY 2016 VL 300 BP 433 EP 451 DI 10.1016/j.nucengdes.2016.02.001 PG 19 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH5OR UT WOS:000372840400040 ER PT J AU Ham, TK Arcilesi, DJ Kim, IH Sun, XD Christensen, RN Oh, CH Kim, ES AF Ham, Tae K. Arcilesi, David J., Jr. Kim, In H. Sun, Xiaodong Christensen, Richard N. Oh, Chang H. Kim, Eung S. TI Computational fluid dynamics analysis of the initial stages of a VHTR air-ingress accident using a scaled-down model SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article AB An air-ingress accident is considered to be one of the design basis accidents of a very high-temperature gas-cooled reactor (VHTR). The air-ingress accident is initiated, in its worst-case scenario, by a complete break of the hot duct in what is referred to as a double-ended guillotine break. This leads to an initial loss of the primary helium coolant via depressurization. Following the depressurization process, the air-helium mixture in the reactor cavity could enter the reactor core via the hot duct and hot exit plenum. In the event that air ingresses into the reactor vessel, the high-temperature graphite structures in the reactor core and hot plenum will chemically react with the air, which could lead to damage of in-core graphite structures and fuel, release of carbon monoxide and carbon dioxide, core heat up, failure of the structural integrity of the system, and eventually the release of radionuclides to the environment. Studies in the available literature focus on the phenomena of the air ingress accident that occur after the termination of the depressurization, such as density-driven stratified flow, molecular diffusion, and natural circulation. However, a recent study shows that flow reversal could occur due to Taylor wave expansion near the end of the depressurization, which could affect subsequent stages of the air ingress accident scenario. Therefore, to properly understand and evaluate the depressurization effects, numerical simulations are performed for the double-ended guillotine break of the Gas Turbine-Modular Helium Reactor (GT-MHR) cross vessel with a computational fluid dynamics (CFD) tool, ANSYS FLUENT. A benchmark and error quantification study of the depressurization shows that the ANSYS FLUENT model can predict the depressurization problem with relatively low uncertainty. In addition, the computational results show that the depressurization of a double-ended guillotine break behaves as an isentropic process. The observed flow oscillations near the end of the depressurization promote mixing of helium gas and air near the break. The results of the CFD analyses also show that the density-driven stratified flow, which is postulated to be the next stage of the air-ingress accident scenario, is strongly dependent on the density difference between the air-helium mixture in the containment and the helium in the reactor vessel. Therefore, the flow oscillations near the end of the depressurization stage may have a minor, yet notable, effect to slow down the air ingress due to density-driven stratified flow by decreasing the bulk density of the gas mixture in the containment through the addition of helium and increasing the bulk density in the reactor vessel through the addition of air. (C) 2016 Elsevier B.V. All rights reserved. C1 [Ham, Tae K.; Arcilesi, David J., Jr.; Kim, In H.; Sun, Xiaodong; Christensen, Richard N.] Ohio State Univ, Nucl Engn Program, Columbus, OH 43210 USA. [Oh, Chang H.; Kim, Eung S.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. [Ham, Tae K.] Korea Fdn Nucl Safety, 49,Daewangpangyo Ro 644 Beon Gil, Songnam, Gyeonggi Do, South Korea. [Kim, In H.] PSEG Nucl LLC, Hancocks Bridge, NJ 08038 USA. [Christensen, Richard N.] Univ Idaho Idaho Falls, Nucl Engn Program, 995 Univ Pl, Idaho Falls, ID 83401 USA. [Kim, Eung S.] Seoul Natl Univ, Dept Nucl Engn, 559 Gwanak Ro, Seoul, South Korea. RP Sun, XD (reprint author), Ohio State Univ, Nucl Engn Program, Columbus, OH 43210 USA. EM taekyu8@gmail.com; arcilesi.1@osu.edu; ihkim0730@gmail.com; sun.200@osu.edu; rchristensen@uidaho.edu; kes7741@snu.ac.kr OI Sun, Xiaodong/0000-0002-9852-160X FU U.S. Department of Energy's Office of Nuclear Energy's Nuclear Energy University Programs under DOE award [DE-AC07-051D14517] FX This research was performed using funding received from the U.S. Department of Energy's Office of Nuclear Energy's Nuclear Energy University Programs under DOE award number DE-AC07-051D14517. NR 24 TC 0 Z9 0 U1 1 U2 5 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD APR 15 PY 2016 VL 300 BP 517 EP 529 DI 10.1016/j.nucengdes.2016.02.011 PG 13 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DH5OR UT WOS:000372840400046 ER PT J AU Yang, YB Liu, SQ Zhao, H Yang, WY Wu, R Huang, QZ Zhou, D Du, HL Wang, CS Yang, YC Xu, H Zhu, JL Gourdon, O Vogel, S Yang, JB AF Yang, Y. B. Liu, S. Q. Zhao, H. Yang, W. Y. Wu, R. Huang, Q. Z. Zhou, D. Du, H. L. Wang, C. S. Yang, Y. C. Xu, H. Zhu, J. L. Gourdon, O. Vogel, S. Yang, J. B. TI Magnetic structure and phase transition of Ni2Mn1.48Sb0.52 magnetic shape memory compound SO SCRIPTA MATERIALIA LA English DT Article DE Neutron diffraction; Shape memory compound; Martensitic phase transition; Exchange bias effect ID MARTENSITIC TRANSFORMATIONS; HEUSLER ALLOY AB A comprehensive study of the structural and magnetic properties of the Ni2Mn1.48Sb0.52 compound is presented using neutron diffraction and magnetic measurements. It is found that Mn atoms on 4a and 4b sites are ferrimagnetic coupled in the austenitic phase. At 300 K, the magnetic moments of Mn (4a) and Mn (4b) are determined to be 2.72(3) mu(B) and -2.67(5) mu(B), respectively. From 260 K to 4 K, the compound is in martensite phase and the magnetic moments of Mn (2a), Mn (2f), Mn (2b), Mn (2e) at 4 K are 2.2(5) mu(B), 2.3(5) Pat -2.1(5) mu(B), and -2.6(5) mu(B), respectively. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Yang, Y. B.; Liu, S. Q.; Zhao, H.; Yang, W. Y.; Wu, R.; Zhou, D.; Du, H. L.; Wang, C. S.; Yang, Y. C.; Yang, J. B.] Peking Univ, Sch Phys, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China. [Yang, J. B.] Collaborat Innovat Ctr Quantum Matter, Beijing 100871, Peoples R China. [Huang, Q. Z.] NIST, Gaithersburg, MD 20878 USA. [Xu, H.; Zhu, J. L.; Gourdon, O.; Vogel, S.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Yang, JB (reprint author), Peking Univ, Sch Phys, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China. EM jbyang@pku.edu.cn OI Xu, Hongwu/0000-0002-0793-6923 FU National Natural Science Foundation of China [51371009, 50971003, 51171001]; National Basic Research Program of China (MOST of China) [2010CB833104] FX This work was supported by the National Natural Science Foundation of China (Grant Nos. 51371009, 50971003 and 51171001), the National Basic Research Program of China (No. 2010CB833104, MOST of China). NR 28 TC 1 Z9 1 U1 8 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 15 PY 2016 VL 116 BP 31 EP 35 DI 10.1016/j.scriptamat.2016.01.028 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DH1QP UT WOS:000372560300007 ER PT J AU Hahn, EN Fensin, SJ Germann, TC Meyers, MA AF Hahn, Eric N. Fensin, Saryu J. Germann, Timothy C. Meyers, Marc A. TI Symmetric tilt boundaries in body-centered cubic tantalum SO SCRIPTA MATERIALIA LA English DT Article DE Coincidence lattice; Grain boundary structure; Grain boundary energy; Molecular dynamics (MD); Transition metals ID BCC TRANSITION-METALS; GRAIN-BOUNDARIES; ATOMIC-STRUCTURE; DISLOCATION NUCLEATION; MOLECULAR-DYNAMICS; FREE-VOLUME; ENERGY; ALUMINUM; MOLYBDENUM; SIGMA-5 AB Grain boundaries can play a significant role in the mechanical response of materials. Atomistic simulations are used to investigate 79 coincidence site lattice grain boundary structures and energies in tantalum, a model body-centered cubic transition metal. Quasi-symmetric Sigma 3, Sigma 5, Sigma 7, Sigma 13, and Sigma 27 boundaries are observed, of which Sigma 3 and Sigma 7 also exist as traditional mirror-symmetry conserving boundary structures. These results are supported by previous observations of similar phenomena in other bcc transition metal Sigma 5 boundaries. Metastable low energy Sigma 3 boundary structures in tantalum could influence the formation and stability of deformation twins and abnormal growth grain favoring Sigma 3 boundaries. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Hahn, Eric N.; Meyers, Marc A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Hahn, Eric N.; Fensin, Saryu J.; Germann, Timothy C.] Los Alamos Natl Lab, Los Alamos, NM 94550 USA. RP Hahn, EN (reprint author), Univ Calif San Diego, La Jolla, CA 92093 USA. EM enhahn@eng.ucsd.edu RI Meyers, Marc/A-2970-2016; OI Meyers, Marc/0000-0003-1698-5396; Hahn, Eric/0000-0002-2305-0532; Germann, Timothy/0000-0002-6813-238X FU UC Research Laboratories Grant [09-LR-06-118456-MEYM]; Department of Energy NNSA/SSAP [DE-NA0002080]; DOE ASCR through the Exascale Co-design Center for Materials in Extreme Environments; U.S Department of Energy [DE-AC52-06NA25396] FX ENH and MAM were supported by UC Research Laboratories Grant (09-LR-06-118456-MEYM), and by the Department of Energy NNSA/SSAP (DE-NA0002080). ENH also received support from DOE ASCR through the Exascale Co-design Center for Materials in Extreme Environments. Los Alamos National Laboratory is operated by LANS, LLC, for the NNSA and the U.S Department of Energy under contract DE-AC52-06NA25396. NR 39 TC 2 Z9 2 U1 6 U2 16 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 15 PY 2016 VL 116 BP 108 EP 111 DI 10.1016/j.scriptamat.2016.01.038 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DH1QP UT WOS:000372560300024 ER PT J AU Edmondson, PD Briggs, SA Yamamoto, Y Howard, RH Sridharan, K Terrani, KA Field, KG AF Edmondson, P. D. Briggs, S. A. Yamamoto, Y. Howard, R. H. Sridharan, K. Terrani, K. A. Field, K. G. TI Irradiation-enhanced alpha ' precipitation in model FeCrAl alloys SO SCRIPTA MATERIALIA LA English DT Article DE APT; FeCrAl; Alpha prime; Neutron irradiation ID PHASE-SEPARATION KINETICS; CR-AL ALLOYS; WATER REACTORS; STEELS AB Model FeCrAl alloys with varying compositions (Fe(10-18)Cr(10-6)Al at.%) have been neutron irradiated at similar to 320 to damage levels of similar to 7 displacements per atom (dpa) to investigate the compositional influence on the formation of irradiation-induced Cr-rich alpha' precipitates using atom probe tomography. In all alloys, significant number densities of these precipitates were observed. Cluster compositions were investigated and it was found that the average cluster Cr content ranged between 51.1 and 62.5 at.% dependent on initial compositions. This is significantly lower than the Cr-content of alpha' in binary FeCr alloys. Significant partitioning of the Al from the alpha' precipitates was also observed. Published by Elsevier Ltd. C1 [Edmondson, P. D.; Briggs, S. A.; Yamamoto, Y.; Field, K. G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Briggs, S. A.; Sridharan, K.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Howard, R. H.; Terrani, K. A.] Oak Ridge Natl Lab, Nucl Sci & Engn Directorate, Oak Ridge, TN 37831 USA. RP Edmondson, PD (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM edmondsonpd@ornl.gov OI Edmondson, Philip/0000-0001-8990-0870 FU DOE's Office of Nuclear Energy, Advanced Fuel Campaign of the Fuel Cycle RD Program; Scientific User Facilities Division, Office of Basic Energy Sciences, DOE; US Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office [DE-AC07-051D14517]; DOE Office of Nuclear Energy's Nuclear Energy University Programs FX Research was sponsored by the DOE's Office of Nuclear Energy, Advanced Fuel Campaign of the Fuel Cycle R&D Program. Neutron irradiation of FeCrAl alloys at ORNL's HFIR user facility was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. Atom probe tomography was conducted at the Center for Nanophase Materials Science, which is a DOE Office of Science User Facility; and the MaCS Laboratory at the Center for Advanced Energy Studies at Idaho National Laboratory. This work was supported by the US Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-051D14517 as part of a Nuclear Science User Facilities experiment. Funding for SAB was provided by the DOE Office of Nuclear Energy's Nuclear Energy University Programs. NR 21 TC 4 Z9 4 U1 7 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 15 PY 2016 VL 116 BP 112 EP 116 DI 10.1016/j.scriptamat.2016.02.002 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DH1QP UT WOS:000372560300025 ER PT J AU Liu, SQ Zhuang, QL He, YJ Noormets, A Chen, JQ Gu, LH AF Liu, Shaoqing Zhuang, Qianlai He, Yujie Noormets, Asko Chen, Jiquan Gu, Lianhong TI Evaluating atmospheric CO2 effects on gross primary productivity and net ecosystem exchanges of terrestrial ecosystems in the conterminous United States using the AmeriFlux data and an artificial neural network approach SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Gross primary production; Net ecosystem change; Eddy flux tower; CO2; Artificial neural network ID LAND-SURFACE TEMPERATURE; WATER-VAPOR EXCHANGE; CARBON-DIOXIDE FLUX; ELEVATED CO2; SOIL RESPIRATION; FOREST ECOSYSTEMS; USE EFFICIENCY; STOMATAL CONDUCTANCE; NITROGEN LIMITATION; SPATIAL VARIABILITY AB Quantitative understanding of regional gross primary productivity (GPP) and net ecosystem exchanges (NEE) and their responses to environmental changes are critical to quantifying the feedbacks of ecosystems to the global climate system. Numerous studies have used the eddy flux data to upscale the eddy covariance derived carbon fluxes from stand scales to regional and global scales. However, few studies incorporated atmospheric carbon dioxide (CO2) concentrations into those extrapolations. Here, we consider the effect of atmospheric CO2 using an artificial neural network (ANN) approach to upscale the AmeriFlux tower of NEE and the derived GPP to the conterminous United States. Two ANN models incorporating remote sensing variables at an 8-day time step were developed. One included CO2 as an explanatory variable and the other did not. The models were first trained, validated using eddy flux data, and then extrapolated to the region at a 0.05 degrees x 0.05 degrees (latitude x longitude) resolution from 2001 to 2006. We found that both models performed well in simulating site-level carbon fluxes. The spatially averaged annual GPP with and without considering the atmospheric CO2 were 789 and 788 g Cm-2 yr(-1), respectively (for NEE, the values were 112 and 109 g Cm-2 yr(-1), respectively). Model predictions were comparable with previous published results and MODIS GPP products. However, the difference in GPP between the two models exhibited a great spatial and seasonal variability, with an annual difference of 200 g Cm-2 yr(-1). Further analysis suggested that air temperature played an important role in determining the atmospheric CO2 effects on carbon fluxes. In addition, the simulation that did not consider atmospheric CO2 failed to detect ecosystem responses to droughts in part of the US in 2006. The study suggests that the spatially and temporally varied atmospheric CO2 concentrations should be factored into carbon quantification when scaling eddy flux data to a region. (C) 2016 Elsevier B.V. All rights reserved. C1 [Liu, Shaoqing; Zhuang, Qianlai; He, Yujie] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Zhuang, Qianlai] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. [Noormets, Asko] N Carolina State Univ, Dept Forestry & Environm Resources, Raleigh, NC 27695 USA. [Noormets, Asko] N Carolina State Univ, Southern Global Change Program, Raleigh, NC 27695 USA. [Chen, Jiquan] Michigan State Univ, CGCEO Geog, E Lansing, MI 48824 USA. [Gu, Lianhong] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Zhuang, QL (reprint author), Purdue Univ, CIVIL 550 Stadium Mall Dr, W Lafayette, IN 47907 USA. EM qzhuang@purdue.edu RI Gu, Lianhong/H-8241-2014; Chen, Jiquan/D-1955-2009; He, Yujie/E-2514-2017 OI Gu, Lianhong/0000-0001-5756-8738; He, Yujie/0000-0001-8261-5399 FU NASA Land-Use and Land-Cover Change program [NASA-NNX09AI26G]; Department of Energy [DE-FG02-08ER64599]; NSF Division of Information and Intelligent Systems [NSF-1028291]; NSF Carbon and Water in the Earth Program [NSF-0630319] FX This study is supported through projects funded to Q. Z. by the NASA Land-Use and Land-Cover Change program (NASA-NNX09AI26G), Department of Energy (DE-FG02-08ER64599), the NSF Division of Information and Intelligent Systems (NSF-1028291), and the NSF Carbon and Water in the Earth Program (NSF-0630319). The supercomputing resource is provided by the Rosen Center for Advanced Computing at Purdue University. Special thanks to all scientists and supporting staffs at AmeriFlux sites. Finally, we acknowledged two anonymous reviewers for their comments. Gabriela Shirkey helped editing of the manuscript. NR 127 TC 2 Z9 2 U1 12 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD APR 15 PY 2016 VL 220 BP 38 EP 49 DI 10.1016/j.agrformet.2016.01.007 PG 12 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA DG9EH UT WOS:000372385100005 ER PT J AU Miller, HM Matter, JM Kelemen, P Ellison, ET Conrad, ME Fierer, N Ruchala, T Tominaga, M Templeton, AS AF Miller, Hannah M. Matter, Juerg M. Kelemen, Peter Ellison, Eric T. Conrad, Mark E. Fierer, Noah Ruchala, Tyler Tominaga, Masako Templeton, Alexis S. TI Modern water/rock reactions in Oman hyperalkaline peridotite aquifers and implications for microbial habitability SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID PRESENT-DAY SERPENTINIZATION; METHANE-HYDROGEN-WATER; SULTANATE-OF-OMAN; LIGURIAN OPHIOLITES; ANAEROBIC OXIDATION; MANTLE PERIDOTITES; RAMAN SPECTROSCOPY; ULTRAMAFIC ROCKS; SAMAIL OPHIOLITE; BASALT AQUIFERS AB The Samail ophiolite in Oman is undergoing modern hydration and carbonation of peridotite and may host a deep subsurface biosphere. Previous investigations of hyperalkaline fluids in Oman have focused on fluids released at surface seeps, which quickly lose their reducing character and precipitate carbonates upon contact with the O-2/CO2-rich atmosphere. In this work, geochemical analysis of rocks and fluids from the subsurface provides new insights into the operative reactions in serpentinizing aquifers. Serpentinite rock and hyperalkaline fluids (pH > 10), which exhibit millimolar concentrations of Ca2+, H-2 and CH4, as well as variable sulfate and nitrate, were accessed from wells situated in mantle peridotite near Ibra and studied to investigate their aqueous geochemistry, gas concentrations, isotopic signatures, mineralogy, Fe speciation and microbial community composition. The bulk mineralogy of drill cuttings is dominated by olivine, pyroxene, brucite, serpentine and magnetite. At depth, Fe-bearing brucite is commonly intermixed with serpentine, whereas near the surface, olivine and brucite are lost and increased magnetite and serpentine is detected. Micro-Raman spectroscopy reveals at least two distinct generations of serpentine present in drill cuttings recovered from several depths from two wells. Fe K-edge X-ray absorption near-edge spectroscopy (XANES) analysis of the lizardite shows a strong tetrahedral Fe coordination, suggesting a mixture of both Fe(II) and Fe (III) in the serpentine. Magnetite veins are also closely associated with this second generation serpentine, and 2-10 mu m magnetite grains overprint all minerals in the drill cuttings. Thus we propose that the dissolved H-2 that accumulates in the subsurface hyperalkaline fluids was evolved through low temperature oxidation and hydration of relict olivine, as well as destabilization of pre-existing brucite present in the partially serpentinized dunites and harzburgites. In particular, we hypothesize that Fe-bearing brucite is currently reacting with dissolved silica in the aquifer fluids to generate late-stage magnetite, additional serpentine and dissolved H-2. Dissolved CH4 in the fluids exhibits the most isotopically heavy carbon in CH4 reported in the literature thus far. The CH4 may have formed through abiotic reduction of dissolved CO2 or through biogenic pathways under extreme carbon limitation. The methane isotopic composition may have also been modified by significant methane oxidation. 16S rRNA sequencing of DNA recovered from filtered hyperalkaline well fluids reveals an abundance of Meiothermus, Thermodesulfovibrionaceae (sulfate-reducers) and Clostridia (fermenters). The fluids also contain candidate phyla OP1 and OD1, as well as Methanobacterium (methanogen) and Methylococcus sp. (methanotroph). The composition of these microbial communities suggests that low-temperature hydrogen and methane generation, coupled with the presence of electron acceptors such as nitrate and sulfate, sustains subsurface microbial life within the Oman ophiolite. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Miller, Hannah M.; Ellison, Eric T.; Templeton, Alexis S.] Univ Colorado, Dept Geol Sci, UCB 399, Boulder, CO 80309 USA. [Matter, Juerg M.] Univ Southampton, Dept Ocean & Earth Sci, Southampton SO14 3ZH, Hants, England. [Matter, Juerg M.; Kelemen, Peter] Columbia Univ, Lamont Doherty Earth Observ, 61 Route 9W, Palisades, NY 10964 USA. [Conrad, Mark E.] EO Lawrence Berkeley Natl Lab, Div Earth Sci, MS 70A-4418, Berkeley, CA 94720 USA. [Fierer, Noah] Univ Colorado, Dept Ecol & Evolutionary Biol, CIRES 215, Boulder, CO 80309 USA. [Fierer, Noah] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Ruchala, Tyler; Tominaga, Masako] Texas A&M Univ, Dept Geol & Geophys, College Stn, TX 77843 USA. RP Miller, HM; Templeton, AS (reprint author), Univ Colorado, Dept Geol Sci, UCB 399, Boulder, CO 80309 USA. EM hannah.miller-1@colorado.edu; alexis.templeton@colorado.edu RI Conrad, Mark/G-2767-2010; OI TEMPLETON, ALEXIS/0000-0002-9670-0647 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; Department of Energy [DE-SC0006886]; NASA Astrobiology Institute [NNA15BB02A]; Alfred P. Sloan Foundation [2014-3-01]; NSF [EAR-1049905] FX The authors would like to thank Tori Hoehler and Mike Kubo (NASA Ames) for providing exploratory organic acid analyses; Said Nasser Al-Habsi and Salim Mohammed Al Khanbashi of the Ministry of Regional Municipalities and Water Resources Sultanate of Oman for granting access to well fluids and drill cuttings; Amelia Paukert for providing supporting information and samples. We would also like to thank numerous colleagues at the University of Colorado at Boulder: Julien Allaz and the electron microprobe lab, the Raman lab, Fred Luiszer at the Laboratory for Environmental and Geological Studies, the Barger lab with their total organic carbon analyzer, the Fierer lab for their sequencing help, Lisa Mayhew for valued discussions and Kaitlin Rempfert for help collecting samples in 2015. Raman imaging and spectroscopy was conducted at the Raman Microspectroscopy Laboratory at the Department of Geological Sciences, University of Colorado-Boulder. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515, in collaboration with staff scientists Sam Webb, Courtney Krest, and Ryan Davis. This research was funded by the Department of Energy (DE-SC0006886), the NASA Astrobiology Institute (Cooperative Agreement NNA15BB02A), Alfred P. Sloan Foundation Grant 2014-3-01, and NSF EAR-1049905. NR 111 TC 6 Z9 6 U1 9 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD APR 15 PY 2016 VL 179 BP 217 EP 241 DI 10.1016/j.gca.2016.01.033 PG 25 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DH1SS UT WOS:000372565800012 ER PT J AU Kertesz, V Cahill, JF Van Berkel, GJ AF Kertesz, Vilmos Cahill, John F. Van Berkel, Gary J. TI Quantitative metrics for assessment of chemical image quality and spatial resolution SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID IONIZATION MASS-SPECTROMETRY; LASER-ABLATION AB RationaleCurrently objective/quantitative descriptions of the quality and spatial resolution of mass spectrometry derived chemical images are not standardized. Development of these standardized metrics is required to objectively describe the chemical imaging capabilities of existing and/or new mass spectrometry imaging technologies. Such metrics would allow unbiased judgment of intra-laboratory advancement and/or inter-laboratory comparison for these technologies if used together with standardized surfaces. MethodsTwo image metrics, viz., "chemical image contrast" (ChemIC) based on signal-to-noise related statistical measures on chemical image pixels and "corrected resolving power factor" (cRPF) constructed from statistical analysis of mass-to-charge chronograms across features of interest in an image, were developed. These metrics, quantifying chemical image quality and spatial resolution, respectively, were used to evaluate chemical images of a model photoresist patterned surface collected using a laser ablation/liquid vortex capture mass spectrometry imaging system under different instrument operational parameters. ResultsThe calculated ChemIC and cRPF metrics determined in an unbiased fashion the relative ranking of chemical image quality obtained with the laser ablation/liquid vortex capture mass spectrometry imaging system. These rankings were used to show that both chemical image contrast and spatial resolution deteriorated with increasing surface scan speed, increased lane spacing and decreasing size of surface features. ConclusionsChemIC and cRPF, respectively, were developed and successfully applied for the objective description of chemical image quality and spatial resolution of chemical images collected from model surfaces using a laser ablation/liquid vortex capture mass spectrometry imaging system. Published in 2016. This article is a U.S. Government work and is in the public domain in the USA. C1 [Kertesz, Vilmos; Cahill, John F.; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Mass Spectrometry & Laser Spect Grp, Oak Ridge, TN 37831 USA. RP Kertesz, V (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Mass Spectrometry & Laser Spect Grp, Oak Ridge, TN 37831 USA. EM kerteszv@ornl.gov RI Kertesz, Vilmos/M-8357-2016; OI Kertesz, Vilmos/0000-0003-0186-5797; Cahill, John/0000-0002-9866-4010 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Department of Energy [DE-AC05-00OR22725] FX Leslie L. Wilson (ORNL) is thanked for preparing the photoresist coated substrates. The 5500 QTRAP mass spectrometer used to acquire the chemical images shown in this work was provided on loan by Sciex through a Cooperative Research and Development Agreement (CRADA NFE-10-02966). This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 16 TC 1 Z9 1 U1 5 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD APR 15 PY 2016 VL 30 IS 7 BP 927 EP 932 DI 10.1002/rcm.7519 PG 6 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA DH0XS UT WOS:000372508100017 PM 26969935 ER PT J AU Zhao, YJ Qiao, JW Ma, SG Gao, MC Yang, HJ Chen, MW Zhang, Y AF Zhao, Y. J. Qiao, J. W. Ma, S. G. Gao, M. C. Yang, H. J. Chen, M. W. Zhang, Y. TI A hexagonal close-packed high-entropy alloy: The effect of entropy SO MATERIALS & DESIGN LA English DT Article DE High-entropy alloys; Hexagonal close-packed structure; Lattice distortion; Phase diagram; Rule of mixture ID BULK METALLIC GLASSES; SOLID-SOLUTION PHASE; MULTICOMPONENT ALLOYS; MECHANICAL-PROPERTIES; WEAR BEHAVIOR; MICROSTRUCTURE; ELEMENTS; DESIGN AB The formation of disordered solid solution in the hexagonal close-packed (hcp) structure in the GdHoLaTbY alloy and its mechanical properties were investigated in this study. The single hcp phase of the alloy in the as-cast state was confirmed by X-ray diffraction and scanning electron microscopy analyses. The compressive yield strength, fracture strength, and plastic strain of the alloy are 108 MPa, 880 MPa, and 21.8%, respectively, and the Vickers hardness is 96 HV. The results show that the yield strength, fracture strength, and hardness of the alloy obey the rule of mixture, which indicates that there is no hardening effect from entropy. Although the high entropy of mixing stabilizes the solid solution against intermetallic compounds, lack of severe lattice distortion from elastic strain or electronic interactions between principal elements impacts little on the mechanical properties. Crown Copyright (C) 2016 Published by Elsevier Ltd. All rights reserved. C1 [Zhao, Y. J.; Qiao, J. W.; Yang, H. J.] Taiyuan Univ Technol, Coll Mat Sci & Engn, Lab Appl Phys & Mech Adv Mat, Taiyuan 030024, Peoples R China. [Qiao, J. W.] Taiyuan Univ Technol, Key Lab Interface Sci & Engn Adv Mat, Minist Educ, Taiyuan 030024, Peoples R China. [Ma, S. G.] Taiyuan Univ Technol, Inst Appl Mech & Biomed Engn, Taiyuan 030024, Peoples R China. [Gao, M. C.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, M. C.] AECOM, POB 1959, Albany, OR 97321 USA. [Chen, M. W.] Tohoku Univ, WPI Adv Inst Mat Res, Sendai, Miyagi 9808577, Japan. [Zhang, Y.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. RP Qiao, JW (reprint author), Taiyuan Univ Technol, Coll Mat Sci & Engn, Lab Appl Phys & Mech Adv Mat, Taiyuan 030024, Peoples R China.; Gao, MC (reprint author), Natl Energy Technol Lab, Albany, OR 97321 USA. EM qiaojunwei@gmail.com; michael.gao@netl.doe.gov RI ZHANG, Yong/B-7928-2009; Chen, Mingwei/A-4855-2010 OI ZHANG, Yong/0000-0002-6355-9923; Chen, Mingwei/0000-0002-2850-8872 FU National Natural Science Foundation of China [51371122, 51501123]; Program for the Innovative Talents of Higher Learning Institutions of Shanxi; Youth Natural Science Foundation of Shanxi Province, China [2015021005, 2015021006, 2014021017-3]; State Key Lab of Advanced Metals and Materials [2015-Z07]; Cross-Cutting Technologies Program at the National Energy Technology Laboratory (NETL) through NETL's Office of Research and Development's Innovative Process Technologies (IPT) Field Work Proposal under the RES [DE-FE-0004000] FX The authors would like to acknowledge the financial support of National Natural Science Foundation of China (Nos. 51371122 and 51501123), the Program for the Innovative Talents of Higher Learning Institutions of Shanxi (2013), the Youth Natural Science Foundation of Shanxi Province, China (Nos. 2015021005, 2015021006, and 2014021017-3), and the financial support from State Key Lab of Advanced Metals and Materials (No. 2015-Z07). M.C.G. acknowledges financial support by the Cross-Cutting Technologies Program at the National Energy Technology Laboratory (NETL) through NETL's Office of Research and Development's Innovative Process Technologies (IPT) Field Work Proposal under the RES contract DE-FE-0004000. NR 39 TC 15 Z9 15 U1 26 U2 93 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0261-3069 EI 1873-4197 J9 MATER DESIGN JI Mater. Des. PD APR 15 PY 2016 VL 96 BP 10 EP 15 DI 10.1016/j.matdes.2016.01.149 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA DF4CX UT WOS:000371296000002 ER PT J AU Hachtel, JA Marvinney, C Mouti, A Mayo, D Mu, R Pennycook, SJ Lupini, AR Chisholm, MF Haglund, RF Pantelides, ST AF Hachtel, J. A. Marvinney, C. Mouti, A. Mayo, D. Mu, R. Pennycook, S. J. Lupini, A. R. Chisholm, M. F. Haglund, R. F. Pantelides, S. T. TI Probing plasmons in three dimensions by combining complementary spectroscopies in a scanning transmission electron microscope SO NANOTECHNOLOGY LA English DT Article DE surface plasmons; electron energy loss spectroscopy; cathodoluminescence; scanning transmission electron microscopy ID ENERGY-LOSS SPECTROSCOPY; ENHANCED RAMAN-SCATTERING; LIGHT-EMITTING-DIODES; SURFACE-PLASMONS; OPTICAL MICROSCOPY; CATHODOLUMINESCENCE SPECTROSCOPY; RESOLVED CATHODOLUMINESCENCE; METAL NANOPARTICLES; SPECIMEN-THICKNESS; NANOMETER-SCALE AB The nanoscale optical response of surface plasmons in three-dimensional metallic nanostructures plays an important role in many nanotechnology applications, where precise spatial and spectral characteristics of plasmonic elements control device performance. Electron energy loss spectroscopy (EELS) and cathodoluminescence (CL) within a scanning transmission electron microscope have proven to be valuable tools for studying plasmonics at the nanoscale. Each technique has been used separately, producing three-dimensional reconstructions through tomography, often aided by simulations for complete characterization. Here we demonstrate that the complementary nature of the two techniques, namely that EELS probes beam-induced electronic excitations while CL probes radiative decay, allows us to directly obtain a spatially- and spectrally-resolved picture of the plasmonic characteristics of nanostructures in three dimensions. The approach enables nanoparticle-by-nanoparticle plasmonic analysis in three dimensions to aid in the design of diverse nanoplasmonic applications. C1 [Hachtel, J. A.; Haglund, R. F.; Pantelides, S. T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Hachtel, J. A.; Mouti, A.; Lupini, A. R.; Chisholm, M. F.; Pantelides, S. T.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Marvinney, C.; Mayo, D.; Haglund, R. F.] Vanderbilt Univ, Interdisciplinary Mat Sci Program, Nashville, TN 37235 USA. [Mayo, D.; Mu, R.] Fisk Univ, Dept Phys, Nashville, TN 37208 USA. [Pennycook, S. J.] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117576, Singapore. [Pantelides, S. T.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA. RP Hachtel, JA (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA.; Hachtel, JA (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM jordan.a.hachtel@vanderbilt.edu RI Hachtel, Jordan/R-1263-2016 OI Hachtel, Jordan/0000-0002-9728-0920 FU Department of Energy [DE-FG02-09ER46554]; Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE; Saudi National Science Fund; United States Department of Defense [W911NF-11-1-0156]; National Science Foundation NSF-CREST Center for the Physics and Chemistry of Materials [HRD-0420516]; McMinn Endowment at Vanderbilt University; Office of Science, US Department of Energy [DE-FG02-01ER45916]; [NSF-EPS-1004083] FX This work was funded by NSF-EPS-1004083 (JAH) Department of Energy grant DE-FG02-09ER46554 (JAH, STP), the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. (AM, SJP, ARL, MFC) and the DOE EERE SunShot Fundamental Program to Advance Cell Efficiency (AM, SJP) and the Saudi National Science Fund (AM). CEM and RFH acknowledge support from the Office of Science, US Department of Energy (DE-FG02-01ER45916) for the fabrication of the nanowires and the FDTD simulations. DCM and RRM gratefully acknowledge financial support from the United States Department of Defense (W911NF-11-1-0156), and the National Science Foundation NSF-CREST Center for the Physics and Chemistry of Materials (HRD-0420516) for tasks related to the fabrication and characterization of the nanowires. STP also acknowledges support from the McMinn Endowment at Vanderbilt University. NR 65 TC 1 Z9 1 U1 1 U2 36 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD APR 15 PY 2016 VL 27 IS 15 AR 155202 DI 10.1088/0957-4484/27/15/155202 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DF4TK UT WOS:000371343500006 PM 26934391 ER PT J AU Su, HL Li, ST AF Su, Hongling Li, Shengtai TI Energy/dissipation-preserving Birkhoffian multi-symplectic methods for Maxwell's equations with dissipation terms SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Structure-preserving method; Computational electromagnetics; Birkhoffian multi-symplectic method; Energy/dissipation-preserving method; Hamiltonian scheme; Maxwell's equations with dissipation terms ID RUNGE-KUTTA METHODS; NUMERICAL-SOLUTION; HAMILTONIAN PDES; INTEGRATORS; SCHEMES; CONSERVATION; PROPAGATION; SYSTEMS AB In this paper, we propose two new energy/dissipation-preserving Birkhoffian multisymplectic methods (Birkhoffian and Birkhoffian box) for Maxwell's equations with dissipation terms. After investigating the non-autonomous and autonomous Birkhoffian formalism for Maxwell's equations with dissipation terms, we first apply a novel generating functional theory to the non-autonomous Birkhoffian formalism to propose our Birkhoffian scheme, and then implement a central box method to the autonomous Birkhoffian formalism to derive the Birkhoffian box scheme. We have obtained four formal local conservation laws and three formal energy global conservation laws. We have also proved that both of our derived schemes preserve the discrete version of the global/local conservation laws. Furthermore, the stability, dissipation and dispersion relations are also investigated for the schemes. Theoretical analysis shows that the schemes are unconditionally stable, dissipation-preserving for Maxwell's equations in a perfectly matched layer (PML) medium and have second order accuracy in both time and space. Numerical experiments for problems with exact theoretical results are given to demonstrate that the Birkhoffian multi-symplectic schemes are much more accurate in preserving energy than both the exponential finite-difference time-domain (FDTD) method and traditional Hamiltonian scheme. We also solve the electromagnetic pulse (EMP) propagation problem and the numerical results show that the Birkhoffian scheme recovers the magnitude of the current source and reaction history very well even after long time propagation. (C) 2016 Elsevier Inc. All rights reserved. C1 [Su, Hongling] Renmin Univ China, Dept Math, Beijing 100872, Peoples R China. [Li, Shengtai] Los Alamos Natl Lab, Theoret Div, POB 1663, Los Alamos, NM 87544 USA. RP Su, HL (reprint author), Renmin Univ China, Dept Math, Beijing 100872, Peoples R China. EM hongling_su@ruc.edu.cn; sli@lanl.gov OI Li, Shengtai/0000-0002-4142-3080 FU NNSFC [10701081, 11071251]; Laboratory Directed Research and Development (LDRD) Program at Los Alamos National Laboratory under Department of Energy FX Research of H. Su is supported by NNSFC Program projects 10701081 and 11071251. Research of S. Li is supported by the Laboratory Directed Research and Development (LDRD) Program at Los Alamos National Laboratory under the auspices of the Department of Energy. NR 32 TC 0 Z9 0 U1 1 U2 11 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD APR 15 PY 2016 VL 311 BP 213 EP 240 DI 10.1016/j.jcp.2016.01.035 PG 28 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DE1KQ UT WOS:000370386300011 ER PT J AU Hamilton, S Berrill, M Clarno, K Pawlowski, R Toth, A Kelley, CT Evans, T Philip, B AF Hamilton, Steven Berrill, Mark Clarno, Kevin Pawlowski, Roger Toth, Alex Kelley, C. T. Evans, Thomas Philip, Bobby TI An assessment of coupling algorithms for nuclear reactor core physics simulations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Multiphysics; Jacobian-free Newton-Krylov; Anderson acceleration; Nuclear reactor analysis ID NEWTON-KRYLOV METHODS; PIN HEAT-TRANSFER; ANDERSON ACCELERATION; NONLINEAR-SYSTEMS; EQUATIONS; CODE; DIFFUSION AB This paper evaluates the performance of multiphysics coupling algorithms applied to a light water nuclear reactor core simulation. The simulation couples the k-eigenvalue form of the neutron transport equation with heat conduction and subchannel flow equations. We compare Picard iteration (block Gauss-Seidel) to Anderson acceleration and multiple variants of preconditioned Jacobian-free Newton-Krylov (JFNK). The performance of the methods are evaluated over a range of energy group structures and core power levels. A novel physics-based approximation to a Jacobian-vector product has been developed to mitigate the impact of expensive on-line cross section processing steps. Numerical simulations demonstrating the efficiency of JFNK and Anderson acceleration relative to standard Picard iteration are performed on a 3D model of a nuclear fuel assembly. Both criticality (k-eigenvalue) and critical boron search problems are considered. (C) 2016 Elsevier Inc. All rights reserved. C1 [Hamilton, Steven; Berrill, Mark; Clarno, Kevin; Evans, Thomas; Philip, Bobby] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Pawlowski, Roger] Sandia Natl Labs, MS 0316,POB 5800, Albuquerque, NM 87185 USA. [Toth, Alex; Kelley, C. T.] N Carolina State Univ, Dept Math, Box 8205, Raleigh, NC 27695 USA. RP Hamilton, S (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM hamiltonsp@ornl.gov; berrillma@ornl.gov; clarnokt@ornl.gov; rppawlo@sandia.gov; artoth@ncsu.edu; tim_kelley@ncsu.edu; evanstm@ornl.gov; philipb@ornl.gov OI Clarno, Kevin/0000-0002-5999-2978; Berrill, Mark/0000-0002-4525-3939 FU Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy [DE-AC05-00OR22725]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; NSF [DMS-1406349] FX This research was supported by the Consortium for Advanced Simulation of Light Water Reactors (www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-00OR22725.; This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725.; This research was supported by NSF Grant DMS-1406349. NR 52 TC 1 Z9 1 U1 2 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD APR 15 PY 2016 VL 311 BP 241 EP 257 DI 10.1016/j.jcp.2016.02.012 PG 17 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DE1KQ UT WOS:000370386300012 ER PT J AU Pretzer, LA Heck, KN Kim, SS Fang, YL Zhao, Z Guo, N Wu, TP Miller, JT Wong, MS AF Pretzer, Lori A. Heck, Kimberly N. Kim, Sean S. Fang, Yu-Lun Zhao, Zhun Guo, Neng Wu, Tianpin Miller, Jeffrey T. Wong, Michael S. TI Improving gold catalysis of nitroarene reduction with surface Pd SO CATALYSIS TODAY LA English DT Article DE Nitrophenol; Catalysis; Palladium; Gold; Nanoparticle; Bimetallic; Structure ID SPHERICAL POLYELECTROLYTE BRUSHES; BIMETALLIC NANOPARTICLE CATALYSTS; TRICHLOROETHENE HYDRODECHLORINATION; AQUEOUS-SOLUTION; AROMATIC-AMINES; MODEL REACTION; CO OXIDATION; SUPPORTED PD; AU-PD; PALLADIUM AB Nitroarene reduction reactions are commercialized catalytic processes that play a key role in the synthesis of many products including medicines, rubbers, dyes, and herbicides. Whereas bimetallic compositions have been studied, a better understanding of the bimetallic structure effects may lead to improved industrial catalysts. In this work, the influence of surface palladium atoms supported on 3-nm Au nanoparticles (Pd-on-Au NPs) on catalytic activity for 4-nitrophenol reduction is explored. Batch reactor studies indicate Pd-on-Au NPs exhibit maximum catalytic activity at a Pd surface coverage of 150 sc%, with an initial turnover frequency of 3.7 mol-nitrophenol/mol-metal(surface)/s which was similar to 5.5x and similar to 13x more face, active than pure Au NPs and Pd NPs, respectively. Pd NPs, Au NPs, and Pd-on-Au NPs below 175 sc% show compensation behavior. Three-dimensional Pd surface ensembles (with 4-5 atoms) previously identified through X-ray adsorption spectroscopy provide the active sites responsible for the catalytic maximum. These results demonstrate the ability to adjust systematically a structural feature (i.e., Pd surface coverage) to yield a more active material. (C) 2015 Elsevier B.V. All rights reserved. C1 [Pretzer, Lori A.; Wong, Michael S.] Rice Univ, Dept Chem, POB 1892, Houston, TX 77005 USA. [Heck, Kimberly N.; Kim, Sean S.; Fang, Yu-Lun; Zhao, Zhun; Wong, Michael S.] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. [Wong, Michael S.] Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA. [Guo, Neng; Wu, Tianpin; Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wong, Michael S.] Rice Univ, Dept Mat Sci & Nanoengn, Houston, TX 77005 USA. RP Wong, MS (reprint author), Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. EM mswong@rice.edu FU National Science Foundation [CBET-1134535]; Welch Foundation [C-1676]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DEACO2-06CH11357] FX The authors gratefully acknowledge the National Science Foundation (CBET-1134535) and Welch Foundation (C-1676) for financial support. The authors also thank Dr. J.C. Forsythe, Dr. Z.L. Schaefer, Dr. N. Soultanidis, Dr. G.C. Kini, Dr. S. Gullapalli, and Mr. J.C. Velazquez for helpful discussions. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DEACO2-06CH11357. NR 44 TC 1 Z9 1 U1 17 U2 69 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD APR 15 PY 2016 VL 264 BP 31 EP 36 DI 10.1016/j.cattod.2015.07.040 PG 6 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DD3GT UT WOS:000369810800005 ER PT J AU Lee, S Sukumar, SR Hong, S Lim, SH AF Lee, Sangkeun Sukumar, Sreenivas R. Hong, Seokyong Lim, Seung-Hwan TI Enabling graph mining in RDF triplestores using SPARQL for holistic in-situ graph analysis SO EXPERT SYSTEMS WITH APPLICATIONS LA English DT Article DE Graph; Mining; Analysis; RDF; SPARQL; Triplestore; Semantic Web ID WORLD-WIDE-WEB; RANDOM NETWORKS AB Graph analysis is now considered as a promising technique to discover useful knowledge from data. We posit that there are two dimensions of graph analysis: Online Graph Analytic Processing (OLGAP) and Graph Mining (GM) where each respectively focuses on subgraph pattern matching and automatic knowledge discovery. As these two dimensions aim to complementarily solve complex problems, holistic in-situ graph analysis which covers both OLGAP and GM in a single system is critical for minimizing the burdens of operating multiple graph systems and transferring intermediate result-sets between those systems. Nevertheless, most existing graph analysis systems are only capable of one dimension of graph analysis. In this work, we take an approach to enabling GM capabilities (e.g., PageRank, connected-component analysis, node eccentricity, etc.) in RDF triplestores, which are originally developed to store RDF datasets and provide OLGAP capability. More specifically, to achieve our goal, we implemented six representative graph mining algorithms using SPARQL. The approach allows a wide range of available RDF datasets directly applicable for holistic graph analysis within a system. For validation of our approach, we evaluate performance of our implementations with nine real-world datasets and three different computing environments - a laptop computer, an Amazon EC2 instance, and a shared-memory Cray XMT2 URIKA-GD graph-processing appliance. The experimental results show that our implementation can provide promising and scalable performance for real world graph analysis in all tested environments. The developed software is publicly available in an open-source project that we initiated. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Lee, Sangkeun; Sukumar, Sreenivas R.; Lim, Seung-Hwan] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. [Hong, Seokyong] N Carolina State Univ, Dept Comp Sci, Raleigh, NC 27695 USA. RP Lee, S (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. EM lees4@ornl.gov; sukumarsr@ornl.gov; shong3@ncsu.edu; lims1@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; DOE FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 66 TC 0 Z9 0 U1 4 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0957-4174 EI 1873-6793 J9 EXPERT SYST APPL JI Expert Syst. Appl. PD APR 15 PY 2016 VL 48 BP 9 EP 25 DI 10.1016/j.eswa.2015.11.010 PG 17 WC Computer Science, Artificial Intelligence; Engineering, Electrical & Electronic; Operations Research & Management Science SC Computer Science; Engineering; Operations Research & Management Science GA DC4KR UT WOS:000369190300002 ER PT J AU Liu, K Wu, JQ AF Liu, Kai Wu, Junqiao TI Mechanical properties of two-dimensional materials and heterostructures SO JOURNAL OF MATERIALS RESEARCH LA English DT Review ID CHEMICAL-VAPOR-DEPOSITION; ELASTIC PROPERTIES; CARBON NANOTUBES; GRAIN-BOUNDARIES; LARGE-AREA; MONOLAYER MOS2; NANOMECHANICAL RESONATORS; MOLYBDENUM-DISULFIDE; INTRINSIC STRENGTH; LAYERED MATERIALS AB Mechanical properties are of fundamental importance in materials science and engineering, and have been playing a great role in various materials applications in the human history. Measurements of mechanical properties of 2-dimensional (2D) materials, however, are particularly challenging. Although various types of 2D materials have been intensively explored in recent years, the investigation of their mechanical properties lags much behind that of other properties, leading to lots of open questions and challenges in this research field. In this review, we first introduce the nanoindentation technique with atomic force microscopy to measure the elastic properties of graphene and 2D transition metal dichalcogenides. Then we review the effect of defects on mechanical properties of 2D materials, including studies on naturally defective chemical-vapor-deposited and intentionally defective 2D materials. Lastly, we introduce a nano-electromechanical device, resonators, built on the basis of the excellent mechanical properties of 2D materials. C1 [Liu, Kai] Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China. [Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Liu, K (reprint author), Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China.; Wu, JQ (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Wu, JQ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM liuk@tsinghua.edu.cn; wuj@berkeley.edu RI Liu, Kai/A-4754-2012; Wu, Junqiao/G-7840-2011 OI Liu, Kai/0000-0002-0638-5189; Wu, Junqiao/0000-0002-1498-0148 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; NSF Center for Energy Efficient Electronics Science (NSF) [ECCS-0939514]; Recruitment Program of Global Youth Experts (the Thousand Youth Talents Program) FX J.W. acknowledges supports by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and the NSF Center for Energy Efficient Electronics Science (NSF Award No. ECCS-0939514). K.L. acknowledges the support by "the Recruitment Program of Global Youth Experts (the Thousand Youth Talents Program)." NR 98 TC 1 Z9 1 U1 36 U2 70 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 14 PY 2016 VL 31 IS 7 BP 832 EP 844 DI 10.1557/jmr.2015.324 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LN UT WOS:000376178400003 ER PT J AU Vishwanath, S Liu, XY Rouvimov, S Basile, L Lu, N Azcatl, A Magno, K Wallace, RM Kim, M Idrobo, JC Furdyna, JK Jena, D Xing, HG AF Vishwanath, Suresh Liu, Xinyu Rouvimov, Sergei Basile, Leonardo Lu, Ning Azcatl, Angelica Magno, Katrina Wallace, Robert M. Kim, Moon Idrobo, Juan-Carlos Furdyna, Jacek K. Jena, Debdeep Xing, Huili Grace TI Controllable growth of layered selenide and telluride heterostructures and superlattices using molecular beam epitaxy SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID DER-WAALS EPITAXY; SCANNING-TUNNELING-MICROSCOPY; MOSE2 THIN-FILMS; P-N-JUNCTIONS; RAMAN-SCATTERING; BAND ALIGNMENT; SNSE2; GRAPHENE; SEMICONDUCTORS; MOTE2 AB Layered materials are an actively pursued area of research for realizing highly scaled technologies involving both traditional device structures as well as new physics. Lately, non-equilibrium growth of 2D materials using molecular beam epitaxy (MBE) is gathering traction in the scientific community and here we aim to highlight one of its strengths, growth of abrupt heterostructures, and superlattices (SLs). In this work we present several of the firsts: first growth of MoTe2 by MBE, MoSe2 on Bi2Se3 SLs, transition metal dichalcogenide (TMD) SLs, and lateral junction between a quintuple atomic layer of Bi2Te3 and a triple atomic layer of MoT2. Reflected high electron energy diffraction oscillations presented during the growth of TMD SLs strengthen our claim that ultrathin heterostructures with monolayer layer control is within reach. C1 [Vishwanath, Suresh; Jena, Debdeep; Xing, Huili Grace] Cornell Univ, Sch Elect & Comp Engn, Ithaca, NY 14853 USA. [Vishwanath, Suresh; Rouvimov, Sergei; Jena, Debdeep; Xing, Huili Grace] Univ Notre Dame, Dept Elect Engn, Notre Dame, IN 46556 USA. [Liu, Xinyu; Magno, Katrina; Furdyna, Jacek K.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Basile, Leonardo] Escuela Politec Nacl, Dept Fis, Quito 170525, Ecuador. [Basile, Leonardo] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Lu, Ning; Azcatl, Angelica; Wallace, Robert M.; Kim, Moon] Univ Texas Dallas, Dept Mat Sci & Engn, Richardson, TX 75083 USA. [Idrobo, Juan-Carlos] Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Jena, Debdeep; Xing, Huili Grace] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. RP Vishwanath, S; Xing, HG (reprint author), Cornell Univ, Sch Elect & Comp Engn, Ithaca, NY 14853 USA.; Vishwanath, S; Xing, HG (reprint author), Univ Notre Dame, Dept Elect Engn, Notre Dame, IN 46556 USA.; Xing, HG (reprint author), Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. EM sv372@cornell.edu; grace.xing@cornell.edu RI Kim, Moon/A-2297-2010; Wallace, Robert/A-5283-2008; OI Wallace, Robert/0000-0001-5566-4806; Vishwanath, Suresh/0000-0002-1790-2284 FU National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT); NSF/AFOSR EFRI-2DARE program [1433490]; NSF [DMR1400432]; Center for Low Energy Systems Technology (LEAST), one of six centers of STARnet, a Semiconductor Research Corporation program - MARCO; DARPA FX L.B. acknowledges the financial support of the National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT). Microscopy conducted at ORNL's Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility (JCI).; This work was supported in part by the NSF/AFOSR EFRI-2DARE program (1433490), NSF Grant DMR1400432 and Center for Low Energy Systems Technology (LEAST), one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA. NR 63 TC 4 Z9 4 U1 33 U2 57 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 14 PY 2016 VL 31 IS 7 BP 900 EP 910 DI 10.1557/jmr.2015.374 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LN UT WOS:000376178400008 ER PT J AU Li, XF Lin, MW Puretzky, AA Basile, L Wang, K Idrobo, JC Rouleau, CM Geohegan, DB Xiao, K AF Li, Xufan Lin, Ming-Wei Puretzky, Alexander A. Basile, Leonardo Wang, Kai Idrobo, Juan C. Rouleau, Christopher M. Geohegan, David B. Xiao, Kai TI Persistent photoconductivity in two-dimensional Mo1-xWxSe2-MoSe2 van der Waals heterojunctions SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID HETEROSTRUCTURES; PHOTOCURRENT; MOS2; CHALCOGENIDES; NANOSHEETS; DIODES; GROWTH AB Van der Waals (vdW) heterojunctions consisting of vertically-stacked individual or multiple layers of two-dimensional layered semiconductors, especially the transition metal dichalcogenides (TMDs), show novel optoelectronic functionalities due to the sensitivity of their electronic and optical properties to strong quantum confinement and interfacial interactions. Here, monolayers of n-type MoSe2 and p-type Mo1-xWxSe2 are grown by vapor transport methods, then transferred and stamped to form artificial vdW heterostructures with strong interlayer coupling as proven in photoluminescence and low-frequency Raman spectroscopy measurements. Remarkably, the heterojunctions exhibit an unprecedented photoconductivity effect that persists at room temperature for several days. This persistent photoconductivity is shown to be tunable by applying a gate bias that equilibrates the charge distribution. These measurements indicate that such ultrathin vdW heterojunctions can function as rewritable optoelectronic switches or memory elements under time-dependent photo-illumination, an effect which appears promising for new monolayer TMDs-based optoelectronic devices applications. C1 [Li, Xufan; Lin, Ming-Wei; Puretzky, Alexander A.; Wang, Kai; Idrobo, Juan C.; Rouleau, Christopher M.; Geohegan, David B.; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Basile, Leonardo] Escuela Politec Nacl, Dept Fis, Quito 17012759, Ecuador. RP Xiao, K (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM xiaok@ornl.gov RI Li, Xufan/A-8292-2013; Wang, Kai/H-4361-2011; Geohegan, David/D-3599-2013 OI Li, Xufan/0000-0001-9814-0383; Wang, Kai/0000-0002-6405-7837; Geohegan, David/0000-0003-0273-3139 FU Materials Science and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT); ORNL Laboratory Directed Research and Development FX Synthesis science sponsored by the Materials Science and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. Materials characterization conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. L.B. acknowledges the financial support of the National Secretariat of Higher Education, Science, Technology and Innovation of Ecuador (SENESCYT). X.L. and M.L. acknowledge support from ORNL Laboratory Directed Research and Development. NR 27 TC 2 Z9 2 U1 6 U2 20 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 14 PY 2016 VL 31 IS 7 BP 923 EP 930 DI 10.1557/jmr.2016.35 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LN UT WOS:000376178400011 ER PT J AU McCreary, A Berkdemir, A Wang, JJ Nguyen, MA Elias, AL Perea-Lopez, N Fujisawa, K Kabius, B Carozo, V Cullen, DA Mallouk, TE Zhu, J Terrones, M AF McCreary, Amber Berkdemir, Ayse Wang, Junjie Minh An Nguyen Elias, Ana Laura Perea-Lopez, Nestor Fujisawa, Kazunori Kabius, Bernd Carozo, Victor Cullen, David A. Mallouk, Thomas E. Zhu, J. Terrones, Mauricio TI Distinct photoluminescence and Raman spectroscopy signatures for identifying highly crystalline WS2 monolayers produced by different growth methods SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID TRANSITION-METAL DICHALCOGENIDES; CHEMICAL-VAPOR-DEPOSITION; HIGH-QUALITY MONOLAYER; TIGHTLY BOUND TRIONS; MOLYBDENUM-DISULFIDE; 2-DIMENSIONAL MATERIALS; LAYERED MATERIALS; TRANSPORT AGENTS; GRAIN-BOUNDARIES; SINGLE-CRYSTALS AB Transition metal dichalcogenides such as WS2 show exciting promise in electronic and optoelectronic applications. Significant variations in the transport, Raman, and photoluminescence (PL) can be found in the literature, yet it is rarely addressed why this is. In this report, Raman and PL of monolayered WS2 produced via different methods are studied and distinct features that indicate the degree of crystallinity of the material are observed. While the intensity of the LA(M) Raman mode is found to be a useful indicator to assess the crystallinity, PL is drastically more sensitive to the quality of the material than Raman spectroscopy. We also show that even exfoliated crystals, which are usually regarded as the most pristine material, can contain large amounts of defects that would not be apparent without Raman and PL measurements. These findings can be applied to the understanding of other two-dimensional heterostructured systems. C1 [McCreary, Amber; Berkdemir, Ayse; Wang, Junjie; Elias, Ana Laura; Perea-Lopez, Nestor; Fujisawa, Kazunori; Carozo, Victor; Zhu, J.; Terrones, Mauricio] Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA. [McCreary, Amber; Berkdemir, Ayse; Wang, Junjie; Elias, Ana Laura; Perea-Lopez, Nestor; Fujisawa, Kazunori; Carozo, Victor; Zhu, J.; Terrones, Mauricio] Penn State Univ, Ctr Dimens & Layered Mat 2, University Pk, PA 16802 USA. [Berkdemir, Ayse] Erciyes Univ, Nanotechnol Res Ctr, TR-38039 Kayseri, Turkey. [Berkdemir, Ayse] Erciyes Univ, Kayseri Vocat Coll, TR-38039 Kayseri, Turkey. [Minh An Nguyen; Mallouk, Thomas E.; Terrones, Mauricio] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Kabius, Bernd] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Cullen, David A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Terrones, Mauricio] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Terrones, Mauricio] Shinshu Univ, Res Ctr Exot Nanocarbons, Nagano 3808553, Japan. RP Terrones, M (reprint author), Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Ctr Dimens & Layered Mat 2, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Dept Chem, University Pk, PA 16802 USA.; Terrones, M (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA.; Terrones, M (reprint author), Shinshu Univ, Res Ctr Exot Nanocarbons, Nagano 3808553, Japan. EM mut11@psu.edu RI Zhu, Jun/A-1610-2014; Carozo, Victor/K-1784-2016; Cullen, David/A-2918-2015; Perea-Lopez, Nestor/A-2683-2010 OI Cullen, David/0000-0002-2593-7866; Perea-Lopez, Nestor/0000-0002-3197-759X FU U.S. Army Research Office under the MURI ALNOS [W911NF-11-1-0362]; Center for Nanoscale Science, an NSF Materials Research Science and Engineering Center [DMR-1420620]; National Science Foundation [EFRI1433311]; ORNL's Center for Nanophase Materials Science (CNMS) which is a Department of Energy, Office of Science User Facility; Brazilian National Council for Scientific and Technological Development (CNPq) [249070/2013-8] FX A.M., M.A.N., A.L.E., N.P.L, T.E.M., and M.T. acknowledge the financial support from the U.S. Army Research Office under the MURI ALNOS project No. W911NF-11-1-0362. J.W., J.Z., and M.T. were supported by the Center for Nanoscale Science, an NSF Materials Research Science and Engineering Center, under the award DMR-1420620. A.L.E. acknowledges the support from the National Science Foundation (EFRI1433311). D.A.C. acknowledges funding through a user project supported by ORNL's Center for Nanophase Materials Science (CNMS) which is a Department of Energy, Office of Science User Facility. V.C. acknowledges support from The Brazilian National Council for Scientific and Technological Development (CNPq) (249070/2013-8). NR 95 TC 1 Z9 1 U1 21 U2 39 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD APR 14 PY 2016 VL 31 IS 7 BP 931 EP 944 DI 10.1557/jmr.2016.47 PG 14 WC Materials Science, Multidisciplinary SC Materials Science GA DM2LN UT WOS:000376178400012 ER PT J AU Zhou, XW El Gabaly, F Stavila, V Allendorf, MD AF Zhou, X. W. El Gabaly, F. Stavila, V. Allendorf, M. D. TI Molecular Dynamics Simulations of Hydrogen Diffusion in Aluminum SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HIGH-PURITY ALUMINUM; LOSLICHKEIT VON WASSERSTOFF; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; EXFOLIATION CORROSION; SADDLE-POINTS; ALLOYS; STORAGE; UND; EMBRITTLEMENT AB Hydrogen diffusion impacts the performance of solid-state hydrogen storage materials and contributes to the embrittlement of structural materials under hydrogen-containing environments. In atomistic simulations, the diffusion energy barriers are usually calculated using molecular statics simulations where a nudged elastic band method is used to constrain a path connecting the two end points of an atomic jump. This approach requires prior knowledge of the "end points". For alloy and defective systems, the number of possible atomic jumps with respect to local atomic configurations is tremendous. Even when these jumps can be exhaustively studied, it is still unclear how they can be combined to give an overall diffusion behavior seen in experiments. Here we describe the use of molecular dynamics simulations to determine the overall diffusion energy barrier from the Arrhenius equation. This method does not require information about atomic jumps, and it has additional advantages, such as the ability to incorporate finite temperature effects and to determine the pre-exponential factor. As a test case for a generic method, we focus on hydrogen diffusion in bulk aluminum. We find that the challenge of this method is the statistical variation of the results. However, highly converged energy barriers can be achieved by an appropriate set of temperatures, output time intervals (for tracking hydrogen positions), and a long total simulation time. Our results help elucidate the inconsistencies of the experimental diffusion data published in the literature. The robust approach developed here may also open up future molecular dynamics simulations to rapidly study diffusion properties of complex material systems in multidimensional spaces involving composition and defects. C1 [Zhou, X. W.; El Gabaly, F.; Stavila, V.; Allendorf, M. D.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Zhou, XW (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM xzhou@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors gratefully acknowledge research support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Office, under Contract Number DE-AC04-94AL85000. NR 45 TC 1 Z9 1 U1 13 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 14 PY 2016 VL 120 IS 14 BP 7500 EP 7509 DI 10.1021/acs.jpcc.6b01802 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ7ZJ UT WOS:000374431400006 ER PT J AU Mantz, YA AF Mantz, Yves A. TI Density-Functional Study of the La2Zr2O7 (001) and (011) Surfaces and Bulk SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; X-RAY-DIFFRACTION; THIN-FILMS; ELECTRONIC-STRUCTURE; EARTH IONS; BASIS-SET; PYROCHLORE; STABILITY AB Lanthanum zirconate (La2Zr2O7, LZ)-based compounds are of interest for their catalytic activity. Accordingly, the low index (001) and (011) surfaces of LZ are studied at the level of density-functional theory, representing the first theoretical attempt to characterize the surfaces of this compound. All possible surface terminations of the (001) and (011) surfaces formed by cleaving a perfect crystal are considered. These surfaces are termed ideal. In addition, judiciously chosen defective (001) and (011) surfaces are examined. The expression for the free energy of a LZ surface is derived, and it is a function only of temperature and oxygen gas partial pressure for all surfaces considered. Both surface energies and surface free energies are computed. A defective (001) surface is shown to be thermodynamically preferred to any ideal (001) surface over a wide range of temperatures and oxygen gas partial pressures. Thus, the first evidence is provided for a (001) surface that is defective or otherwise not ideal, for example, reconstructed. Results are discussed in the context of a proposed comparison of predicted relative crystallite thicknesses perpendicular to (001) and (011) surfaces to experimental results. However, the experimental results still need to be obtained to permit this comparison. C1 [Mantz, Yves A.] US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. RP Mantz, YA (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd,POB 880, Morgantown, WV 26507 USA. EM yves.mantz@netl.doe.gov NR 69 TC 0 Z9 0 U1 3 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 14 PY 2016 VL 120 IS 14 BP 7522 EP 7531 DI 10.1021/acs.jpcc.5b10069 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ7ZJ UT WOS:000374431400008 ER PT J AU Chialvo, AA Vlcek, L AF Chialvo, Ariel A. Vlcek, Lukas TI Can We Describe Graphene Confined Water Structures as Overlapping of Approaching Graphene-Water Interfacial Structures? SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID X-RAY REFLECTIVITY; MOLECULAR-DYNAMICS SIMULATIONS; DENSITY PROFILE; STATISTICAL-MECHANICS; NANOMETER CONFINEMENT; CONTACT-ANGLE; SURFACE; LIQUID; WETTABILITY; GRAPHITE AB We investigate the microscopic mechanisms of the overlap of interfacial structures in confined fluids and attempt to answer the question whether the confined structures can be predicted from the original density profiles of individual solid-fluid interfaces. For that purpose, we perform (globally) isobaric-isothermal (locally, grand canonical) molecular dynamics simulations to extract not only the axial distribution functions of the water sites for the uncoupled graphene-water interfaces, but also those corresponding to the confined aqueous environments over the interplate range 8 <= h (angstrom) <= 28 typically at ambient conditions. We have tested two (i.e., an arithmetic and a geometric) superposition approximations for the singlet density of confined water between flat graphene plates, as well as for a combination of flat and corrugated graphene plates. The outcome of this study suggests that the answer to the titles question is a "yes", provided that the interplate distance h is large enough to avoid fluid geometric packing frustration. C1 [Chialvo, Ariel A.; Vlcek, Lukas] Oak Ridge Natl Lab, Geochem & Interfacial Sci, Div Chem Sci, Oak Ridge, TN 37831 USA. [Vlcek, Lukas] Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. RP Vlcek, L (reprint author), Oak Ridge Natl Lab, Geochem & Interfacial Sci, Div Chem Sci, Oak Ridge, TN 37831 USA.; Vlcek, L (reprint author), Oak Ridge Natl Lab, Joint Inst Computat Sci, Oak Ridge, TN 37831 USA. EM vlcekl1@ornl.gov RI Vlcek, Lukas/N-7090-2013 OI Vlcek, Lukas/0000-0003-4782-7702 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center; Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX This research was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. The authors wish to acknowledge Peter T. Cummings for posing the question during the monthly FIRST telecom, on April 2014, whose detailed answer led to the research effort discussed in this work. NR 79 TC 1 Z9 1 U1 12 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 14 PY 2016 VL 120 IS 14 BP 7553 EP 7561 DI 10.1021/acs.jpcc.5b11886 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ7ZJ UT WOS:000374431400011 ER PT J AU Wu, D Guo, XF Sun, H Navrotsky, A AF Wu, Di Guo, Xiaofeng Sun, Hui Navrotsky, Alexandra TI Interplay of Confinement and Surface Energetics in the Interaction of Water with a Metal-Organic Framework SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-DIOXIDE; THERMODYNAMIC COMPLEXITY; ADSORPTION; HKUST-1; CAPTURE; SEPARATION; CHEMISTRY; ENTHALPY; ETHANOL; DESIGN AB The enthalpy of water adsorption (Delta h) on the metal-organic framework (MOF) HKUST-1 has been determined directly by calorimetry. The most exothermic value of Delta h [-119.4 +/- 0.5 kJ/(mol of water)] occurs at zero coverage and perhaps represents water confinement in the smallest (4-angstrom) cages. An intermediate Delta h value of -50.2 +/- 1.8 kJ/(mol of water) at higher loading probably corresponds to the binding of water on the available Cu nodes and subsequent filling of the largest (11-angstrom) pores. The weakest interactions take place in the medium (10-angstrom) cages, showing weak inclusion of water clusters in a limited hydrophobic environment. By combining ethanol adsorption calorimetry, mathematical analysis of the slope of the water adsorption isotherm, and the differential enthalpy of water adsorption curve, we are able not only to develop an approach to separate energetically multistage guest-host interactions in complex MOF architectures but also to distinguish a sequence of interactions with very similar energetic effects. C1 [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, Peter A Rock Thermochem Lab, One Shields Ave, Davis, CA 95616 USA. [Wu, Di; Guo, Xiaofeng; Navrotsky, Alexandra] Univ Calif Davis, NEAT ORU, One Shields Ave, Davis, CA 95616 USA. [Guo, Xiaofeng] Los Alamos Natl Lab, Earth & Environm Sci Div, Earth Syst Observat, POB 1663, Los Alamos, NM 87545 USA. [Sun, Hui] E China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China. RP Navrotsky, A (reprint author), Univ Calif Davis, Peter A Rock Thermochem Lab, One Shields Ave, Davis, CA 95616 USA.; Navrotsky, A (reprint author), Univ Calif Davis, NEAT ORU, One Shields Ave, Davis, CA 95616 USA. EM anavrotsky@ucdavis.edu RI Wu, Di/A-3039-2014 OI Wu, Di/0000-0001-6879-321X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-05ER15667]; National Science Foundation Award [DMR-0936384]; Natural Science Foundation of Shanghai [16ZR1408100] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Grant DE-FG02-05ER15667. The Cornell High Energy Synchrotron Source is supported by National Science Foundation Award DMR-0936384. H.S. thanks the Natural Science Foundation of Shanghai for the financial support (No. 16ZR1408100). The authors thank Manas K. Bhunia and James T. Hughes for providing the MOF material. We also thank Zewei Quan for the synchrotron X-ray scattering analysis and invaluable discussions. NR 33 TC 2 Z9 2 U1 9 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 14 PY 2016 VL 120 IS 14 BP 7562 EP 7567 DI 10.1021/acs.jpcc.5b12239 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ7ZJ UT WOS:000374431400012 ER PT J AU Roy, S Baer, MD Mundy, CJ Schenter, GK AF Roy, Santanu Baer, Marcel D. Mundy, Christopher J. Schenter, Gregory K. TI Reaction Rate Theory in Coordination Number Space: An Application to Ion Solvation SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TRANSITION-STATE THEORY; MOLECULAR-DYNAMICS SIMULATIONS; WATER-EXCHANGE-RATES; CHEMICAL-REACTIONS; FREE-ENERGY; HYDRATION SHELL; MD SIMULATIONS; MEAN FORCE; NONEQUILIBRIUM SOLVATION; AQUEOUS-SOLUTIONS AB Understanding reaction mechanisms in many chemical and biological processes requires application of rare event theories. In these theories, an effective choice of a reaction coordinate to describe a reaction pathway is essential. To this end, we study ion solvation in water using molecular dynamics simulations and explore the utility of coordination number (n = number of water molecules in the first solvation shell) as the reaction coordinate. Here, we compute the potential of mean force (W(n)) using umbrella sampling, predicting multiple metastable n-states for both cations and anions. With increasing ionic size, we find these states become more stable and structured for cations when compared to anions. We have extended transition state theory (TST) to calculate transition rates between n states. TST overestimates the rate constant due to solvent-induced barrier recrossings that are not accounted for. We correct the TST rates by calculating transmission coefficients using the reactive flux method. This approach enables a new way of understanding rare events involving coordination complexes. C1 [Roy, Santanu; Baer, Marcel D.; Mundy, Christopher J.; Schenter, Gregory K.] Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd, Richland, WA 99352 USA. RP Roy, S; Schenter, GK (reprint author), Pacific NW Natl Lab, Div Phys Sci, 902 Battelle Blvd, Richland, WA 99352 USA. EM santanu.roy@pnnl.gov; greg.schenter@pnnl.gov OI Roy, Santanu/0000-0001-6991-8205 FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; MS3 (Materials Synthesis and Simulation Across Scales), a Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL) FX We gratefully acknowledge Liem Dang and Panos Stinis for useful discussions. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. S.R, C.J.M., and G.KS. were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. M.D.B. was supported by MS3 (Materials Synthesis and Simulation Across Scales) Initiative, a Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy. NR 70 TC 0 Z9 0 U1 8 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 14 PY 2016 VL 120 IS 14 BP 7597 EP 7605 DI 10.1021/acs.jpcc.6b00443 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ7ZJ UT WOS:000374431400017 ER PT J AU Bhaskaran-Nair, K Kowalski, K Shelton, WA AF Bhaskaran-Nair, Kiran Kowalski, Karol Shelton, William A. TI Coupled cluster Green function: Model involving single and double excitations SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ELECTRON PROPAGATOR THEORY; NUCLEIC-ACID BASES; SHELL IONIZATION ENERGIES; GAS-PHASE TAUTOMERISM; QUASI-PARTICLE THEORY; FULL CCSDT MODEL; GROUND-STATE; PHOTOELECTRON-SPECTROSCOPY; ULTRAVIOLET PHOTOELECTRON; QUANTUM-CHEMISTRY AB In this paper, we report on the development of a parallel implementation of the coupled-cluster (CC) Green function formulation (GFCC) employing single and double excitations in the cluster operator (GFCCSD). A key aspect of this work is the determination of the frequency dependent self-energy, Sigma(omega). The detailed description of the underlying algorithm is provided, including approximations used that preserve the pole structure of the full GFCCSD method, thereby reducing the computational costs while maintaining an accurate character of methodology. Furthermore, for systems with strong local correlation, our formulation reveals a diagonally dominate block structure where as the non-local correlation increases, the block size increases proportionally. To demonstrate the accuracy of our approach, several examples including calculations of ionization potentials for benchmark systems are presented and compared against experiment. (C) 2016 AIP Publishing LLC. C1 [Bhaskaran-Nair, Kiran; Shelton, William A.] Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Bhaskaran-Nair, Kiran; Shelton, William A.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Kowalski, Karol] Pacific NW Natl Lab, Battelle, William R Wiley Environm Mol Sci Lab, K8-91,POB 999, Richland, WA 99352 USA. RP Kowalski, K (reprint author), Pacific NW Natl Lab, Battelle, William R Wiley Environm Mol Sci Lab, K8-91,POB 999, Richland, WA 99352 USA. EM karol.kowalski@pnnl.gov FU Extreme Scale Computing Initiative, a Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory; US Department of Energy [DE-AC06.76RLO-1830]; U.S. Department of Energy under EPSCoR Grant [DE-SC0012432]; Louisiana Board of Regents FX This work has been supported by the Extreme Scale Computing Initiative (K.K.), a Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory. Computational support from Environmental Molecular Sciences Laboratory located at the Pacific Northwest National Laboratory that is operated for the US Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC06.76RLO-1830. The computational work conducted by W.A.S. is supported by the U.S. Department of Energy under EPSCoR Grant No. DE-SC0012432 with additional support from the Louisiana Board of Regents. NR 117 TC 4 Z9 4 U1 3 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 14 PY 2016 VL 144 IS 14 AR 144101 DI 10.1063/1.4944960 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK2WB UT WOS:000374774000003 PM 27083702 ER PT J AU Caskey, CM Holder, A Shulda, S Christensen, ST Diercks, D Schwartz, CP Biagioni, D Nordlund, D Kukliansky, A Natan, A Prendergast, D Orvananos, B Sun, W Zhang, X Ceder, G Ginley, DS Tumas, W Perkins, JD Stevanovic, V Pylypenko, S Lany, S Richards, RM Zakutayev, A AF Caskey, Christopher M. Holder, Aaron Shulda, Sarah Christensen, Steven T. Diercks, David Schwartz, Craig P. Biagioni, David Nordlund, Dennis Kukliansky, Alon Natan, Amir Prendergast, David Orvananos, Bernardo Sun, Wenhao Zhang, Xiuwen Ceder, Gerbrand Ginley, David S. Tumas, William Perkins, John D. Stevanovic, Vladan Pylypenko, Svitlana Lany, Stephan Richards, Ryan M. Zakutayev, Andriy TI Synthesis of a mixed-valent tin nitride and considerations of its possible crystal structures SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID THIN-FILMS; AQUEOUS-SOLUTION; PREDICTION; OXIDES; SNO2; DISCOVERY; LIFETIME; DESIGN; GROWTH AB Recent advances in theoretical structure prediction methods and high-throughput computational techniques are revolutionizing experimental discovery of the thermodynamically stable inorganic materials. Metastable materials represent a new frontier for these studies, since even simple binary non-ground state compounds of common elements may be awaiting discovery. However, there are significant research challenges related to non-equilibrium thin film synthesis and crystal structure predictions, such as small strained crystals in the experimental samples and energy minimization based theoretical algorithms. Here, we report on experimental synthesis and characterization, as well as theoretical first-principles calculations of a previously unreported mixed-valent binary tin nitride. Thin film experiments indicate that this novel material is N-deficient SnN with tin in the mixed II/IV valence state and a small low-symmetry unit cell. Theoretical calculations suggest that the most likely crystal structure has the space group 2 (SG2) related to the distorted delafossite (SG166), which is nearly 0.1 eV/atom above the ground state SnN polymorph. This observation is rationalized by the structural similarity of the SnN distorted delafossite to the chemically related Sn3N4 spinel compound, which provides a fresh scientific insight into the reasons for growth of polymorphs of metastable materials. In addition to reporting on the discovery of the simple binary SnN compound, this paper illustrates a possible way of combining a wide range of advanced characterization techniques with the first-principle property calculation methods, to elucidate the most likely crystal structure of the previously unreported metastable materials. Published by AIP Publishing. C1 [Caskey, Christopher M.; Holder, Aaron; Christensen, Steven T.; Biagioni, David; Ginley, David S.; Tumas, William; Perkins, John D.; Stevanovic, Vladan; Lany, Stephan; Zakutayev, Andriy] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Caskey, Christopher M.; Shulda, Sarah; Diercks, David; Stevanovic, Vladan; Pylypenko, Svitlana; Richards, Ryan M.] Colorado Sch Mines, Golden, CO 80401 USA. [Caskey, Christopher M.] Larix Chem Sci, Golden, CO 80401 USA. [Schwartz, Craig P.; Nordlund, Dennis] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Kukliansky, Alon; Natan, Amir] Tel Aviv Univ, Tel Aviv, Israel. [Prendergast, David; Sun, Wenhao; Ceder, Gerbrand] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Orvananos, Bernardo; Ceder, Gerbrand] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Zhang, Xiuwen] Univ Colorado, Boulder, CO 80309 USA. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov RI Nordlund, Dennis/A-8902-2008 OI Nordlund, Dennis/0000-0001-9524-6908 FU US Department of Energy, Office of Science, Basic Energy Sciences as a part of the DOE Energy Frontier Research Center "Center for Next Generation of Materials by Design: Incorporating Metastability" [DEAC36-08GO28308]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-76SF00515]; NIH [1S10RR23057]; California NanoSystems Institute at UCLA; NSF [CMMI-1200547]; Israeli National Nanotechnology Initiative (INNI, FTA project) FX This work is supported by the US Department of Energy, Office of Science, Basic Energy Sciences, under Contract No. DEAC36-08GO28308 to NREL as a part of the DOE Energy Frontier Research Center "Center for Next Generation of Materials by Design: Incorporating Metastability." X-ray absorption measurements were performed at Stanford Synchrotron Radiation Lightsource at SLAC National Accelerator Laboratory, supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Contract No. DE-AC02-76SF00515. We would also like to thank Kevin H. Stone for attempting synchrotron XRD measurements of the SnN1-delta samples at SLAC. The authors acknowledge the use of instruments at the Electron Imaging Center for NanoMachines supported by NIH (No. 1S10RR23057) and the California NanoSystems Institute at UCLA, with raw data taken by Chilan Ngo, who thanks Suneel Kodambaka at UCLA for useful discussions, and gratefully acknowledges support from the NSF through Grant No. CMMI-1200547. Amir Natan acknowledges financial support from the Israeli National Nanotechnology Initiative (INNI, FTA project). The XRD peak search-match algorithm used in this work was developed as a part of a Laboratory Directed Research and Development (LDRD) project at NREL. NR 81 TC 2 Z9 2 U1 14 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 14 PY 2016 VL 144 IS 14 AR 144201 DI 10.1063/1.4945561 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK2WB UT WOS:000374774000014 PM 27083713 ER PT J AU Wilson, SR Mendelev, MI AF Wilson, S. R. Mendelev, M. I. TI A unified relation for the solid-liquid interface free energy of pure FCC, BCC, and HCP metals SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RADIAL-DISTRIBUTION FUNCTION; EMBEDDED-ATOM METHOD; STRUCTURAL MODEL; VAPOR INTERFACE; ANISOTROPY; SYSTEMS AB We study correlations between the solid-liquid interface (SLI) free energy and bulk material properties (melting temperature, latent heat, and liquid structure) through the determination of SLI free energies for bcc and hcp metals from molecular dynamics (MD) simulation. Values obtained for the bcc metals in this study were compared to values predicted by the Turnbull, Laird, and Ewing relations on the basis of previously published MD simulation data. We found that of these three empirical relations, the Ewing relation better describes the MD simulation data. Moreover, whereas the original Ewing relation contains two constants for a particular crystal structure, we found that the first coefficient in the Ewing relation does not depend on crystal structure, taking a common value for all three phases, at least for the class of the systems described by embedded-atom method potentials (which are considered to provide a reasonable approximation for metals). Published by AIP Publishing. C1 [Wilson, S. R.; Mendelev, M. I.] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. RP Mendelev, MI (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. EM mendelev@ameslab.gov FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. NR 31 TC 0 Z9 0 U1 6 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 14 PY 2016 VL 144 IS 14 AR 144707 DI 10.1063/1.4946032 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DK2WB UT WOS:000374774000046 PM 27083745 ER PT J AU Porterfield, JP Baraban, JH Troy, TP Ahmed, M McCarthy, MC Morgan, KM Daily, JW Nguyen, TL Stanton, JF Ellison, GB AF Porterfield, Jessica P. Baraban, Joshua H. Troy, Tyler P. Ahmed, Musahid McCarthy, Michael C. Morgan, Kathleen M. Daily, John W. Thanh Lam Nguyen Stanton, John F. Ellison, G. Barney TI Pyrolysis of the Simplest Carbohydrate, Glycolaldehyde (CHO-CH2OH), and Glyoxal in a Heated Microreactor SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INITIATED OXIDATION; UNIMOLECULAR DECOMPOSITION; SUBMILLIMETER SPECTRUM; INFRARED-SPECTRA; MATRIX-ISOLATION; MICRO-REACTOR; GAS-PHASE; OH; MECHANISM; IONIZATION AB Both glycolaldehyde and glyoxal were pyrolyzed in a set of flash-pyrolysis microreactors. The pyrolysis products resulting from CHO-CH2OH and HCO-CHO were detected and identified by vacuum ultraviolet (VUV) photoionization mass spectrometry. Complementary product identification was provided by argon matrix infrared absorption spectroscopy. Pyrolysis pressures in the microreactor were about 100 Torr, and contact times with the microreactors were roughly 100 mu s. At 1200 K, the products of glycolaldehyde pyrolysis are H atoms, CO, CH2=O, CH2=C=O, and HCO-CHO. Thermal decomposition of HCO-CHO was studied with pulsed 118.2 nm photoionization mass spectrometry and matrix infrared absorption. Under these conditions, glyoxal undergoes pyrolysis to H atoms and CO. Tunable VUV photoionization mass spectrometry provides a lower bound for the ionization energy (IE)(CHO-CH2OH) >= 9.95 +/- 0.05 eV. The gas-phase heat of formation of glycolaldehyde was established by a sequence of calorimetric experiments. The experimental result is Delta H-f(298)(CHO-CH2OH) = -75.8 +/- 1.3 kcal mol(-1). Fully ab initio, coupled cluster calculations predict Delta H-f(0)(CHO-CH2OH) of -73.1 +/- 0.5 kcal mol(-1) and Delta H-f(298)(CHO-CH2OH) of -76.1 +/- 0.5 kcal mol(-1). The coupled-cluster singles doubles and noniterative triples correction calculations also lead to a revision of the geometry of CHO-CH2OH. We find that the O-H bond length differs substantially from earlier experimental estimates, due to unusual zero-point contributions to the moments of inertia. C1 [Porterfield, Jessica P.; Baraban, Joshua H.; Ellison, G. Barney] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Daily, John W.] Univ Colorado, Dept Mech Engn, Ctr Combust & Environm Res, Boulder, CO 80309 USA. [Troy, Tyler P.; Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [McCarthy, Michael C.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Morgan, Kathleen M.] Xavier Univ Louisiana, Dept Chem, New Orleans, LA 70125 USA. [Thanh Lam Nguyen; Stanton, John F.] Univ Texas Austin, Dept Chem, Austin, TX 78712 USA. RP Ellison, GB (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. EM barney@jila.colorado.edu RI Ahmed, Musahid/A-8733-2009 FU National Science Foundation [CBET-1403979]; Robert A. Welch Foundation [F-1283]; United States Department of Energy, Basic Energy Sciences [DE-FG02-07ER15884]; Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy [DE-AC02- 05CH11231] FX The National Science Foundation (CBET-1403979) has provided support for J.P.P, J.H.B, J.W.D, and G.B.E. We would like to acknowledge National Science Foundation (CHE-1361874) to K.M.M. and CHE-1361031 to J.F.S. Thermal analysis measurements were performed with assistance from S. Akbarian-Tefaghi at the Univ. of New Orleans, Advanced Materials Research Institute FACS user facility. J.F.S. and T.L.N. acknowledge support from the Robert A. Welch Foundation (Grant No. F-1283) and the United States Department of Energy, Basic Energy Sciences (DE-FG02-07ER15884). M.A. and T.P.T. and the Advanced Light Source are supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02- 05CH11231. We thank Prof. K. B. Wiberg for several helpful comments. NR 87 TC 0 Z9 0 U1 11 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 14 PY 2016 VL 120 IS 14 BP 2161 EP 2172 DI 10.1021/acs.jpca.6b00652 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ7ZH UT WOS:000374431200001 PM 26979134 ER PT J AU Yu, HG Han, HX Guo, H AF Yu, Hua-Gen Han, Huixian Guo, Hua TI Full-Dimensional Quantum Calculations of Vibrational Levels of NH4+ and Isotopomers on An Accurate Ab Initio Potential Energy Surface SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID AMMONIUM ION NH4+; DISCRETE VARIABLE REPRESENTATION; HIGH-RESOLUTION; INFRARED-SPECTROSCOPY; METHANE (CH4)-C-12; LASER SPECTROSCOPY; REACTION DYNAMICS; GLOBAL ANALYSIS; MOLECULAR-IONS; BOND-LENGTH AB Vibrational energy levels of the ammonium cation (NH4+) and its deuterated isotopomers are calculated using a numerically exact kinetic energy operator on a recently developed nine-dimensional permutation invariant semiglobal potential energy surface fitted to a large number of high-level ab initio points. Like CH4, the vibrational levels of NH4+ and ND4+ exhibit a polyad structure, characterized by a collective quantum number P = 2(v(1) + v(3)) + v(2) + v(4). The low-lying vibrational levels of all isotopomers are assigned and the agreement with available experimental data is better than 1 cm(-1). C1 [Yu, Hua-Gen] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Han, Huixian; Guo, Hua] Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. [Han, Huixian] NW Univ Xian, Sch Phys, Xian 710069, Shaanxi, Peoples R China. RP Yu, HG (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA.; Guo, H (reprint author), Univ New Mexico, Dept Chem & Chem Biol, Albuquerque, NM 87131 USA. EM hgy@bnl.gov; hguo@unm.edu RI Yu, Hua-Gen/N-7339-2015; Guo, Hua/J-2685-2014 OI Guo, Hua/0000-0001-9901-053X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-FG02-05ER15694] FX The work (H.G.Y.) performed at the Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886. H.G. thanks the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-FG02-05ER15694. Some of calculations were performed at NERSC. NR 56 TC 2 Z9 2 U1 3 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 14 PY 2016 VL 120 IS 14 BP 2185 EP 2193 DI 10.1021/acs.jpca.6b01946 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ7ZH UT WOS:000374431200004 PM 27023376 ER PT J AU Benkert, A Meyer, F Hauschild, D Blum, M Yang, W Wilks, RG Bar, M Reinert, F Heske, C Weinhardt, L AF Benkert, A. Meyer, F. Hauschild, D. Blum, M. Yang, W. Wilks, R. G. Baer, M. Reinert, F. Heske, C. Weinhardt, L. TI Isotope Effects in the Resonant Inelastic Soft X-ray Scattering Maps of Gas-Phase Methanol SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ELECTRONIC-STRUCTURE; LIQUID METHANOL; EMISSION SPECTRA; FINE-STRUCTURE; MIXTURES; SPECTROSCOPY; ABSORPTION; MOLECULES; DYNAMICS; ALCOHOLS AB The electronic structure of gas-phase methanol molecules (H3COH, H3COD, and D3COD) at atmospheric pressure was investigated using resonant inelastic soft X-ray scattering (RIXS) at the O K and C K edges. We observe strong changes of the relative emission intensities of all valence orbitals as a function of excitation energy, which can be related to the symmetries of the involved orbitals causing an angularly anisotropic RIXS intensity. Furthermore, all observed emission lines are subject to strong spectator shifts of up to -0.9 eV at the O K edge and up to -0.3 eV at the C K edge. At the lowest O K resonance, we find clear evidence for dissociation of the methanol molecule on the time scale of the RIXS process, which is illustrated by comparing X-ray emission spectra of regular and deuterated methanol. C1 [Benkert, A.; Hauschild, D.; Heske, C.; Weinhardt, L.] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat, Hermann v Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Heske, C.; Weinhardt, L.] Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, Hermann v Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Benkert, A.; Meyer, F.; Hauschild, D.; Reinert, F.] Univ Wurzburg, Expt Phys 7, Hubland, D-97074 Wurzburg, Germany. [Blum, M.; Baer, M.; Heske, C.; Weinhardt, L.] Univ Nevada, Dept Chem & Biochem, 4505 Maryland Pkwy, Las Vegas, NV 89154 USA. [Yang, W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Wilks, R. G.; Baer, M.] Helmholtz Zentrum Berlin Mat & Energie GmbH, Renewable Energy, Hahn Meitner Pl 1, D-14109 Berlin, Germany. [Baer, M.] Brandenburg Tech Univ Cottbus Senftenberg, Inst Phys & Chem, Pl Deutsch Einheit 1, D-03046 Cottbus, Germany. [Benkert, A.; Weinhardt, L.] Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem, Engesserstr 18-20, D-76128 Karlsruhe, Germany. RP Benkert, A; Weinhardt, L (reprint author), Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat, Hermann v Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany.; Weinhardt, L (reprint author), Karlsruhe Inst Technol, ANKA Synchrotron Radiat Facil, Hermann v Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany.; Benkert, A (reprint author), Univ Wurzburg, Expt Phys 7, Hubland, D-97074 Wurzburg, Germany.; Weinhardt, L (reprint author), Univ Nevada, Dept Chem & Biochem, 4505 Maryland Pkwy, Las Vegas, NV 89154 USA.; Benkert, A; Weinhardt, L (reprint author), Karlsruhe Inst Technol, Inst Chem Technol & Polymer Chem, Engesserstr 18-20, D-76128 Karlsruhe, Germany. EM andreas.benkert@kit.edu; l.weinhardt@kit.edu RI Yang, Wanli/D-7183-2011 OI Yang, Wanli/0000-0003-0666-8063 FU Deutsche Forschungsgemeinschaft [RE 1469/7-1]; Impuls- and Vernetzungsfonds of the Helmholtz-Association [VH-NG-423]; Department of Energy, Basic Energy Sciences [DE-AC02-05CH11231] FX This work was supported by the Deutsche Forschungsgemeinschaft (Project No. RE 1469/7-1). R.G.W. and M. Bar acknowledge the financial support by the Impuls- and Vernetzungsfonds of the Helmholtz-Association (VH-NG-423). The ALS is supported by the Department of Energy, Basic Energy Sciences, Contract No. DE-AC02-05CH11231. NR 50 TC 1 Z9 1 U1 0 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 14 PY 2016 VL 120 IS 14 BP 2260 EP 2267 DI 10.1021/acs.jpca.6b02636 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ7ZH UT WOS:000374431200011 PM 27003748 ER PT J AU Vasseur, R Friedman, AJ Parameswaran, SA Potter, AC AF Vasseur, Romain Friedman, Aaron J. Parameswaran, S. A. Potter, Andrew C. TI Particle-hole symmetry, many-body localization, and topological edge modes SO PHYSICAL REVIEW B LA English DT Article ID SPIN CHAINS; TRANSITION; SUPERCONDUCTORS; INSULATORS AB We study the excited states of interacting fermions in one dimension with particle-hole symmetric disorder (equivalently, random-bond XXZ chains) using a combination of renormalization group methods and exact diagonalization. Absent interactions, the entire many-body spectrum exhibits infinite-randomness quantum critical behavior with highly degenerate excited states. We show that though interactions are an irrelevant perturbation in the ground state, they drastically affect the structure of excited states: Even arbitrarily weak interactions split the degeneracies in favor of thermalization (weak disorder) or spontaneously broken particle-hole symmetry, driving the system into a many-body localized spin glass phase (strong disorder). In both cases, the quantum critical properties of the noninteracting model are destroyed, either by thermal decoherence or spontaneous symmetry breaking. This system then has the interesting and counterintuitive property that edges of the many-body spectrum are less localized than the center of the spectrum. We argue that our results rule out the existence of certain excited state symmetry-protected topological orders. C1 [Vasseur, Romain; Potter, Andrew C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Vasseur, Romain] Lawrence Berkeley Natl Labs, Mat Sci Div, Berkeley, CA 94720 USA. [Friedman, Aaron J.; Parameswaran, S. A.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Parameswaran, S. A.] Univ Calif Santa Barbara, Calif Inst Quantum Emulat CAIQuE, Elings Hall, Santa Barbara, CA 93106 USA. RP Vasseur, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Vasseur, R (reprint author), Lawrence Berkeley Natl Labs, Mat Sci Div, Berkeley, CA 94720 USA. FU Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4307]; DOE LDRD; NSF Grant [DMR-1455366]; President's Research Catalyst Award from University of California Office of the President [CA-15-327861]; Quantum Materials Programs at LBNL FX We acknowledge helpful discussions with E. Altman, Y. Gannot, T. Morimoto, M. Serbyn, and A. Vishwanath. This work was supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant GBMF4307 (ACP), the DOE LDRD and Quantum Materials Programs at LBNL (RV), NSF Grant DMR-1455366, and the President's Research Catalyst Award No. CA-15-327861 from the University of California Office of the President (SAP). NR 48 TC 11 Z9 11 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 14 PY 2016 VL 93 IS 13 AR 134207 DI 10.1103/PhysRevB.93.134207 PG 9 WC Physics, Condensed Matter SC Physics GA DJ1PF UT WOS:000373974800002 ER PT J AU Greensite, J Szczepaniak, AP AF Greensite, Jeff Szczepaniak, Adam P. TI Constituent gluons and the static quark potential SO PHYSICAL REVIEW D LA English DT Article ID GAUGE; CONFINEMENT AB We suggest that Hamiltonian matrix elements between physical states in QCD might be approximated, in Coulomb gauge, by "lattice-improved" tree diagrams; i.e. tree diagram contributions with dressed ghost, transverse gluon, and Coulomb propagators obtained from lattice simulations. Such matrix elements can be applied to a truncated-basis treatment of hadronic states which include constituent gluons. As an illustration, we apply this hybrid approach to the heavy quark potential, for quark-antiquark separations up to 2.4 fm. The Coulomb string tension in SU(3) gauge theory is about a factor of 4 times greater than the asymptotic string tension. In our approach we show that a single constituent gluon is in principle sufficient, up to 2.4 fm, to reduce this overshoot by the factor required. The static potential remains linear, although the precise value of the string tension depends on details of the Couloumb gauge ghost and gluon propagators in the infrared regime. In this connection we present new lattice results for the transverse gluon propagator in position space. C1 [Greensite, Jeff] San Francisco State Univ, Dept Phys & Astron, San Francisco, CA 94132 USA. [Szczepaniak, Adam P.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Szczepaniak, Adam P.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47403 USA. [Szczepaniak, Adam P.] Thomas Jefferson Natl Accelerator Facil, Ctr Theory, 12000 Jefferson Ave, Newport News, VA 23606 USA. RP Greensite, J (reprint author), San Francisco State Univ, Dept Phys & Astron, San Francisco, CA 94132 USA. OI Greensite, Jeff/0000-0003-1720-9436 FU U.S. Department of Energy [DE-FG03-92ER40711, DE-FG0287ER40365]; Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177] FX This work was supported in part by the U.S. Department of Energy under Grants No. DE-FG03-92ER40711 (J. G.) and DE-FG0287ER40365 (A. P. S.). The work was authored in part by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. NR 24 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 14 PY 2016 VL 93 IS 7 AR 074506 DI 10.1103/PhysRevD.93.074506 PG 19 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ1RB UT WOS:000373979900002 ER PT J AU Boughezal, R Campbell, J Ellis, RK Focke, C Giele, W Liu, XH Petriello, F AF Boughezal, Radja Campbell, John Ellis, R. Keith Focke, Christfried Giele, Walter Liu, Xiaohui Petriello, Frank TI Z-Boson Production in Association with a Jet at Next-To-Next-To-Leading Order in Perturbative QCD SO PHYSICAL REVIEW LETTERS LA English DT Article ID MCFM AB We present the first complete calculation of Z-boson production in association with a jet in hadronic collisions through next-to-next-to-leading order in perturbative QCD. Our computation uses the recently proposed N-jettiness subtraction scheme to regulate the infrared divergences that appear in the real-emission contributions. We present phenomenological results for 13 TeV proton-proton collisions with fully realistic fiducial cuts on the final-state particles. The remaining theoretical uncertainties after the inclusion of our calculations are at the percent level, making the Z + jet channel ready for precision studies at the LHC run II. C1 [Boughezal, Radja; Petriello, Frank] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Campbell, John; Giele, Walter] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Ellis, R. Keith] Univ Durham, Dept Phys, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. [Focke, Christfried; Petriello, Frank] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Liu, Xiaohui] Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. RP Boughezal, R; Petriello, F (reprint author), Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA.; Campbell, J; Giele, W (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.; Ellis, RK (reprint author), Univ Durham, Dept Phys, Inst Particle Phys Phenomenol, Durham DH1 3LE, England.; Focke, C; Petriello, F (reprint author), Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA.; Liu, XH (reprint author), Univ Maryland, Maryland Ctr Fundamental Phys, College Pk, MD 20742 USA. EM rboughezal@anl.gov; johnmc@fnal.gov; keith.ellis@durham.ac.uk; christfried.focke@northwestern.edu; giele@fnal.gov; xhliu@umd.edu; f-petriello@northwestern.edu FU DOE [DE-AC02-06CH11357, DE-AC02-07CH11359, DE-FG02-93ER-40762, DE-FG02-91ER40684]; NSF [PHY-1520916]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE Office of Science User Facility [DE-AC02-06CH11357] FX We thank T. LeCompte for many helpful discussions. R. B. is supported by the DOE Contract No. DE-AC02-06CH11357. J. C., K. E., and W. G. are supported by the DOE Contract No. DE-AC02-07CH11359. C. F. is supported by the NSF Grant No. PHY-1520916. X. L. is supported by the DOE Grant No. DE-FG02-93ER-40762. F. P. is supported by the DOE Grants No. DE-FG02-91ER40684 and No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. It also used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC02-06CH11357. NR 38 TC 15 Z9 15 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 14 PY 2016 VL 116 IS 15 AR 152001 DI 10.1103/PhysRevLett.116.152001 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ1SN UT WOS:000373984100004 PM 27127962 ER PT J AU Kemp, AJ Sentoku, Y AF Kemp, A. J. Sentoku, Y. TI Comment on "In-depth Plasma-Wave Heating of Dense Plasma Irradiated by Short Laser Pulses" SO PHYSICAL REVIEW LETTERS LA English DT Editorial Material C1 [Kemp, A. J.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Sentoku, Y.] Univ Nevada, Reno, NV 89577 USA. RP Kemp, AJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM kemp7@llnl.gov RI Sentoku, Yasuhiko/P-5419-2014 NR 3 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 14 PY 2016 VL 116 IS 15 DI 10.1103/PhysRevLett.116.159501 PG 2 WC Physics, Multidisciplinary SC Physics GA DJ1SN UT WOS:000373984100009 PM 27127989 ER PT J AU Paul, J Stevens, CE Liu, C Dey, P McIntyre, C Turkowski, V Reno, JL Hilton, DJ Karaiskaj, D AF Paul, J. Stevens, C. E. Liu, C. Dey, P. McIntyre, C. Turkowski, V. Reno, J. L. Hilton, D. J. Karaiskaj, D. TI Strong Quantum Coherence between Fermi Liquid Mahan Excitons SO PHYSICAL REVIEW LETTERS LA English DT Article ID FOURIER-TRANSFORM SPECTROSCOPY; 2D ELECTRON-GAS; COLLECTIVE EXCITATIONS; EXCHANGE ENHANCEMENT; MANY-BODY; SEMICONDUCTORS; WELLS; LIGHT; EMISSION; STATES AB In modulation doped quantum wells, the excitons are formed as a result of the interactions of the charged holes with the electrons at the Fermi edge in the conduction band, leading to the so-called "Mahan excitons." The binding energy of Mahan excitons is expected to be greatly reduced and any quantum coherence destroyed as a result of the screening and electron-electron interactions. Surprisingly, we observe strong quantum coherence between the heavy hole and light hole excitons. Such correlations are revealed by the dominating cross-diagonal peaks in both one-quantum and two-quantum two-dimensional Fourier transform spectra. Theoretical simulations based on the optical Bloch equations where many-body effects are included phenomenologically reproduce well the experimental spectra. Time-dependent density functional theory calculations provide insight into the underlying physics and attribute the observed strong quantum coherence to a significantly reduced screening length and collective excitations of the many-electron system. C1 [Paul, J.; Stevens, C. E.; Liu, C.; Dey, P.; McIntyre, C.; Karaiskaj, D.] Univ S Florida, Dept Phys, 4202 East Fowler Ave, Tampa, FL 33620 USA. [Turkowski, V.] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Reno, J. L.] Sandia Natl Labs, CINT, POB 5800, Albuquerque, NM 87185 USA. [Hilton, D. J.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. RP Karaiskaj, D (reprint author), Univ S Florida, Dept Phys, 4202 East Fowler Ave, Tampa, FL 33620 USA. EM karaiskaj@usf.edu RI Liu, Cunming/K-2976-2014; Paul, Jagannath/P-7171-2016 OI Paul, Jagannath/0000-0001-7172-3466 FU National Science Foundation [DMR-1409473]; Department of Energy [DE-FG02-07ER46354]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The work at USF and UAB was supported by the National Science Foundation under Grant No. DMR-1409473. The work at UCF was supported by the Department of Energy under Grant No. DE-FG02-07ER46354. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 57 TC 1 Z9 1 U1 8 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 14 PY 2016 VL 116 IS 15 AR 157401 DI 10.1103/PhysRevLett.116.157401 PG 6 WC Physics, Multidisciplinary SC Physics GA DJ1SN UT WOS:000373984100008 PM 27127985 ER PT J AU Zhou, L Yan, QM Yu, J Jones, RJR Becerra-Stasiewicz, N Suram, SK Shinde, A Guevarra, D Neaton, JB Persson, KA Gregoire, JM AF Zhou, Lan Yan, Qimin Yu, Jie Jones, Ryan J. R. Becerra-Stasiewicz, Natalie Suram, Santosh K. Shinde, Aniketa Guevarra, Dan Neaton, Jeffrey B. Persson, Kristin A. Gregoire, John M. TI Stability and self-passivation of copper vanadate photoanodes under chemical, electrochemical, and photoelectrochemical operation SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID OXYGEN VACANCY; WATER OXIDATION; SOLAR; SURFACE; PHOTOCATALYSIS; OXIDES; FILMS; TI AB Deployment of solar fuels technology requires photoanodes with long term stability, which can be accomplished using light absorbers that self-passivate under operational conditions. Several copper vanadates have been recently reported as promising photoanode materials, and their stability and self-passivation is demonstrated through a combination of Pourbaix calculations and combinatorial experimentation. C1 [Zhou, Lan; Jones, Ryan J. R.; Becerra-Stasiewicz, Natalie; Suram, Santosh K.; Shinde, Aniketa; Guevarra, Dan; Gregoire, John M.] CALTECH, Joint Ctr Artificial Photosynthesis, Pasadena, CA 91125 USA. [Yan, Qimin; Yu, Jie; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Yan, Qimin; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Yu, Jie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynthesis, Berkeley, CA 94720 USA. [Yu, Jie; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Gregoire, JM (reprint author), CALTECH, Joint Ctr Artificial Photosynthesis, Pasadena, CA 91125 USA.; Persson, KA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM kapersson@lbl.gov; gregoire@caltech.edu FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Materials Project (DOE) through the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [EDCBEE, DE-AC02-05CH11231]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX This manuscript is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy (Award No. DE-SC0004993). Computational work was supported by the Materials Project (DOE Grant # EDCBEE) through the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. Use of the Stanford Synchrotron Radiation Lightsource is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The authors appreciate assistance from A. Mehta and D. van Campen (synchrotron XRD measurements), C. Xiang (Fig. 2 graphics), and S. Mitrovic (XPS measurements). NR 25 TC 3 Z9 3 U1 16 U2 31 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 14 PY 2016 VL 18 IS 14 BP 9349 EP 9352 DI 10.1039/c6cp00473c PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI5WC UT WOS:000373570200005 PM 26997488 ER PT J AU Metcalf, M Chern, GW Di Ventra, M Chien, CC AF Metcalf, Mekena Chern, Gia-Wei Di Ventra, Massimiliano Chien, Chih-Chun TI Matter-wave propagation in optical lattices: geometrical and flat-band effects SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE optical lattice; flat band; matter-wave propagation; quantum transport ID QUANTUM PHASE-TRANSITION; ULTRACOLD ATOMS; DYNAMICS; SIMULATION; TRANSPORT; FERMIONS; GASES; SYSTEMS AB The geometry of optical lattices can be engineered, allowing the study of atomic transport along paths arranged in patterns that are otherwise difficult to probe in the solid state. A question feasible to atomic systems is related to the speed of matter-wave propagation as a function of the lattice geometry. To address this issue, we investigated, theoretically, the quantum transport of noninteracting and weakly-interacting ultracold fermionic atoms in several 2D optical lattice geometries. We find that the triangular lattice has a higher propagation velocity compared to the square lattice, and the cross-linked square lattice has an even faster propagation velocity. The increase results from the mixing of the momentum states which leads to different group velocities in quantum systems. Standard band theory provides an explanation and allows for a systematic way to search and design systems with controllable matter-wave propagation. Moreover, the presence of a flat band such as in a two-leg ladder geometry leads to a dynamical density discontinuity due to its localized atoms. Possible realizations of those dynamical phenomena are discussed. C1 [Metcalf, Mekena; Chien, Chih-Chun] Univ Calif, Sch Nat Sci, Merced, CA 95343 USA. [Chern, Gia-Wei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Chern, Gia-Wei] Los Alamos Natl Lab, Ctr Nonlinear Sci, Los Alamos, NM 87545 USA. [Di Ventra, Massimiliano] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. RP Chien, CC (reprint author), Univ Calif, Sch Nat Sci, Merced, CA 95343 USA. EM cchien5@ucmerced.edu FU US DOE through the LANL/LDRD Program; DOE Grant [DE-FG02-05ER46204] FX We thank Michael Zwolak, Kevin Mitchell, Fei Zhou, and Dan Stamper-Kurn for useful discussions, and Michael Colvin and Chen-Yen Lai for assisting the numerical calculations. GWC acknowledges the support of the US DOE through the LANL/LDRD Program. MD acknowledges support from the DOE Grant No. DE-FG02-05ER46204. NR 54 TC 1 Z9 1 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD APR 14 PY 2016 VL 49 IS 7 AR 075301 DI 10.1088/0953-4075/49/7/075301 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DH6OS UT WOS:000372911000017 ER PT J AU Osti, NC Naguib, M Ostadhossein, A Xie, Y Kent, PRC Dyatkin, B Rother, G Heller, WT van Duin, ACT Gogotsi, Y Mamontov, E AF Osti, Naresh C. Naguib, Michael Ostadhossein, Alireza Xie, Yu Kent, Paul R. C. Dyatkin, Boris Rother, Gernot Heller, William T. van Duin, Adri C. T. Gogotsi, Yury Mamontov, Eugene TI Effect of Metal Ion Intercalation on the Structure of MXene and Water Dynamics on its Internal Surfaces SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE MXenes; intercalation; water diffusion; quasi-elastic neutron scattering; ReaxFF simulation ID ELASTIC NEUTRON-SCATTERING; 2-DIMENSIONAL TITANIUM CARBIDE; HIGH VOLUMETRIC CAPACITANCE; CATION INTERCALATION; CONFINED WATER; CLAY; TRANSITION; ELECTRODES; BATTERIES; DIFFUSION AB MXenes are a recently discovered class of 2D materials with an excellent potential for energy storage applications. Because MXene surfaces are hydrophilic and attractive interaction forces between the layers are relatively weak, water molecules can spontaneously intercalate at ambient humidity and significantly influence the key properties of this 2D material. Using complementary X-ray and neutron scattering techniques, we demonstrate that intercalation with potassium cations significantly improves structural homogeneity and water stability in MXenes. In agreement with molecular dynamics simulations, intercalated potassium ions reduce the water self-diffusion coefficient by 2 orders of magnitude, suggesting greater stability of hydrated MXene against changing environmental conditions. C1 [Osti, Naresh C.; Mamontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Naguib, Michael] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Ostadhossein, Alireza] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16801 USA. [van Duin, Adri C. T.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16801 USA. [Xie, Yu; Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Heller, William T.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Dyatkin, Boris; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Rother, Gernot] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. RP Osti, NC; Mamontov, E (reprint author), Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM ostinc@ornl.gov; mamontove@ornl.gov RI Kent, Paul/A-6756-2008; Mamontov, Eugene/Q-1003-2015; Rother, Gernot/B-7281-2008; Xie, Yu/E-5875-2011; OI Kent, Paul/0000-0001-5539-4017; Mamontov, Eugene/0000-0002-5684-2675; Rother, Gernot/0000-0003-4921-6294; Xie, Yu/0000-0002-7782-5428; Dyatkin, Boris/0000-0001-7537-2181; Naguib, Michael/0000-0002-4952-9023; Heller, William/0000-0001-6456-2975 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Basic Energy Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE [DE-AC05-00OR22725] FX This work was supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Work at ORNL's Spallation Neutron Source is supported by the U.S. Department of Energy, Office of Basic Energy Sciences. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for U.S. DOE under Contract No. DE-AC05-00OR22725. We are grateful to David J. Wesolowski for his support and critical reading of our manuscript. NR 30 TC 7 Z9 7 U1 43 U2 146 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 13 PY 2016 VL 8 IS 14 BP 8859 EP 8863 DI 10.1021/acsami.6b01490 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DJ5UF UT WOS:000374274900001 PM 27010763 ER PT J AU Lin, HJ Baltrus, JP Gao, HY Ding, Y Nam, CY Ohodnicki, P Gao, PX AF Lin, Hui-Jan Baltrus, John P. Gao, Haiyong Ding, Yong Nam, Chang-Yong Ohodnicki, Paul Gao, Pu-Xian TI Perovskite Nanoparticle-Sensitized Ga2O3 Nanorod Arrays for CO Detection at High Temperature SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE semiconductor; nanowire; gas sensor; harsh environment; catalytic effect ID GAS-SENSING PROPERTIES; GALLIUM OXIDE; NANOSTRUCTURED MATERIALS; PLATINUM NANOCRYSTALS; SNO2 NANOWIRES; SENSORS; SURFACE; O-2; GROWTH; LAFEO3 AB Noble metal nanoparticles are extensively used for sensitizing metal oxide chemical sensors through the catalytic spillover mechanism. However, due to earth-scarcity and high cost of noble metals, finding replacements presents a great economic benefit. Besides, high temperature and harsh environment sensor applications demand material stability under conditions approaching thermal and chemical stability limits of noble metals. In this study, we employed thermally stable perovskite-type La0.8Sr0.2FeO3 (LSFO) nanoparticle surface decoration on Ga2O3 nanorod array gas sensors and discovered an order of magnitude enhanced sensitivity to carbon monoxide at 500 degrees C. The LSFO nanoparticle catalysts was of comparable performance to that achieved by Pt nanoparticles, with a much lower weight loading than Pt. Detailed electron microscopy and X-ray photoelectron spectroscopy studies suggested the LSFO nanoparticle sensitization effect is attributed to a spillover-like effect associated with the gas-LSFO-Ga2O3 triple interfaces that spread the negatively charged surface oxygen ions from LSFO nanoparticles surfaces surfaces with faster surface CO oxidation reactions. over to beta-Ga2O3 nanorod surfaces with faster surface CO oxidation reactions. C1 [Lin, Hui-Jan; Gao, Haiyong; Gao, Pu-Xian] Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Lin, Hui-Jan; Gao, Haiyong; Gao, Pu-Xian] Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Baltrus, John P.; Ohodnicki, Paul] Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Ding, Yong] Georgia Inst Technol, Sch Mat Sci & Engn, 771 Ferst Dr, Atlanta, GA 30332 USA. [Nam, Chang-Yong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Ohodnicki, Paul] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15216 USA. RP Gao, PX (reprint author), Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA.; Gao, PX (reprint author), Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. EM puxian.gao@uconn.edu RI Nam, Chang-Yong/D-4193-2009; Ding, Yong/F-3705-2017 OI Nam, Chang-Yong/0000-0002-9093-4063; Ding, Yong/0000-0001-5805-347X FU U.S. Department of Energy (DOE) [DE-FE0000870, DE-FE0011577]; National Energy Technology Laboratory in the US DOE; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX The authors are grateful for the financial support from the U.S. Department of Energy (DOE), with Award DE-FE0000870 and DE-FE0011577. The work at the National Energy Technology Laboratory in the US DOE is supported through the Crosscutting Research Program. A part of the research was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory (BNL), which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-SC0012704. NR 42 TC 4 Z9 4 U1 28 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 13 PY 2016 VL 8 IS 14 BP 8880 EP 8887 DI 10.1021/acsami.6b01709 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DJ5UF UT WOS:000374274900005 PM 27043430 ER PT J AU Mao, J Dai, KH Xuan, MJ Shao, GS Qiao, RM Yang, WL Battaglia, VS Liu, G AF Mao, Jing Dai, Kehua Xuan, Minjie Shao, Guosheng Qiao, Ruimin Yang, Wanli Battaglia, Vincent S. Liu, Gao TI Effect of Chromium and Niobium Doping on the Morphology and Electrochemical Performance of High-Voltage Spinel LiNi0.5Mn1.5O4 Cathode Material SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE high-voltage spinel; lithium nickel manganese oxide; doping; lithium chemical diffusion coefficient; cycling performance; rate performance ID LITHIUM-ION BATTERIES; POSITIVE-ELECTRODE; RATE CAPABILITY; LIMN1.5NI0.5O4; CR; FE; CO; TEMPERATURE; PROGRESS; NI AB Undoped, Cr-doped, and Nb-doped LiMn1.5Ni0.5O4 (LNMO) is synthesized via a PVP (polyvinylpyrrolidone)-combustion method by calcinating at 1000 degrees C for 6 h. SEM images show that the morphology of LNMO particles is affected by Cr and Nb doping. Cr doping results in sharper edges and corners and smaller particle size, and Nb doping leads to smoother edges and corners and more rounded and larger particles. The crystal and electron structure is investigated by XRD- and synchrotron-based soft X-ray absorption spectroscopy (sXAS). Cr doping and light Nb doping (LiNb0.02Ni0.49Mn1.49O4) improve the rate performance of LNMO. To explore the reason for rate-performance improvement, we conducted potential intermittent titration technique (PITT) and electrochemical impedance spectroscopy (EIS) tests. The Li+ chemical diffusion coefficient at different state of charge (SOC) is calculated and suggests that both Cr and light Nb doping speeds up Li+ diffusion in LNMO particles. The impedance spectra show that both R-SEI and R-ct are reduced by Cr and light Nb doping. The cycling performance is improved by Cr or Nb doping, and Cr doping increases both Coulombic efficiency and energy efficiency of LNMO at 1 C cycling. The LiCr0.1Ni0.45Mn1.45O4 remains at 94.1% capacity after 500 cycles at 1 C, and during the cycling, the Coulombic efficiency and energy efficiency remain at over 99.7% and 97.5%, respectively. C1 [Mao, Jing; Xuan, Minjie; Shao, Guosheng] Zhengzhou Univ, Sch Mat Sci & Engn, Zhengzhou 450002, Peoples R China. [Mao, Jing; Xuan, Minjie; Shao, Guosheng] Zhengzhou Univ, Int Joint Res Lab Low Carbon & Environm Mat Henan, Zhengzhou 450002, Peoples R China. [Mao, Jing; Dai, Kehua; Battaglia, Vincent S.; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Energy Storage & Distributed Resource Div, Berkeley, CA 94720 USA. [Qiao, Ruimin; Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Dai, Kehua] Northeastern Univ, Sch Met & Mat, Shenyang 110004, Peoples R China. RP Dai, KH; Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Energy Storage & Distributed Resource Div, Berkeley, CA 94720 USA.; Dai, KH (reprint author), Northeastern Univ, Sch Met & Mat, Shenyang 110004, Peoples R China. EM daikh@smm.neu.edu.cn; gliu@lbl.gov RI Yang, Wanli/D-7183-2011; Qiao, Ruimin/E-9023-2013; OI Yang, Wanli/0000-0003-0666-8063; Shao, Guosheng/0000-0003-1498-7929 FU National Natural Science Foundation of China [51204038, U1504521]; Fundamental Research Funds for the Central Universities of China [N150204017, L1502004]; Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Natural Science Foundation of China (51204038 and U1504521) and the Fundamental Research Funds for the Central Universities of China (N150204017 and L1502004). This work was also supported by the Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy, under the Advanced Battery Materials Research (BMR) Program and Applied Battery Research (ABR) Program under contract no. DE-AC02-05CH11231. NR 45 TC 3 Z9 3 U1 34 U2 83 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 13 PY 2016 VL 8 IS 14 BP 9116 EP 9124 DI 10.1021/acsami.6b00877 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DJ5UF UT WOS:000374274900031 PM 27008976 ER PT J AU Zhang, HJ McDowell, RG Martin, LR Qiang, Y AF Zhang, Huijin McDowell, Rocklan G. Martin, Leigh R. Qiang, You TI Selective Extraction of Heavy and Light Lanthanides from Aqueous Solution by Advanced Magnetic Nanosorbents SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE rare earth elements; trivalent lanthanides; magnetic separation; nanosorbents; magnetic nanoparticles; selective sorption ID RARE-EARTHS; DIETHYLENETRIAMINEPENTAACETIC ACID; SOLVENT-EXTRACTION; SEPARATION; NANOPARTICLES; ADSORPTION; DTPA; COMPLEXATION; RECOVERY; ACTINIDE AB Rare earth elements (REEs) make unique and vital contributions to our current world of technology. Separating and recycling REEs is of great importance to diversify the sources of REEs and advance the efficient use of REE resources when the supply is limited. In light of separation nanotechnology, diethylenetriamine-pentaacetic acid (DTPA) functionalized magnetic nanosorbents have been synthesized and investigated for the highly selective extraction of heavy (Sm-Ho) and light (La-Nd) lanthanides (Ln) from aqueous solutions. The results demonstrated that the separation factor (SF) between heavy-Ln and light-Ln groups reached the maximal value of 11.5 at low pH value of 2.0 in 30 min. For example, the SFs of Gd/La and Dy/La pairs were up to 10 times higher than that reported by other studies. Besides the excellent selectivity, our double-coated magnetic nanoparticles coupled with diethylenetriaminepentaacetic acid (dMNP-DTPA) nanosorbents are more advantageous in that the Ln(III) sorption was effectively and quickly (in 30 min) achieved in acid solutions with pH values as low as 2.0. Such attributes ensure a stronger adaptability to the harsh environments of REE recycling processes. Displacement phenomena were subsequently observed between the heavy-Ln and light-Ln ions that were coexisting in solution and competing for the same sorption sites, causing the increase in sorption capacity of heavy Ln on the surface of nanosorbents with time. The order of affinity of Ln(III) to DTPA-functionalized magnetic nanosorbents perfectly followed the corresponding stability constants between Ln(III) and nonimmobilized DTPA. Displacement phenomena and lanthanide contraction, as well as the surface nanostructures of DTPA-functionalized nanosorbents, significantly improved the separation factors of heavy-Ln/light-Ln pairs. The Ln(III) interaction with DTPA-functionalized magnetic nanosorbents followed the pseudo-second-order kinetics with a correlation coefficient extremely high and close to unity. C1 [Zhang, Huijin; Qiang, You] Univ Idaho, Environm Sci Program, Moscow, ID 83844 USA. [Qiang, You] Univ Idaho, Dept Phys, Moscow, ID 83844 USA. [McDowell, Rocklan G.; Martin, Leigh R.] Idaho Natl Lab, Aqueous Separat & Radiochem Dept, Idaho Falls, ID 83415 USA. RP Qiang, Y (reprint author), Univ Idaho, Environm Sci Program, Moscow, ID 83844 USA.; Qiang, Y (reprint author), Univ Idaho, Dept Phys, Moscow, ID 83844 USA. EM youqiang@uidaho.edu RI Martin, Leigh/P-3167-2016 OI Martin, Leigh/0000-0001-7241-7110 FU U.S. Department of Energy (DOE) [DE-FC07-08ID14926]; DOE INL-CAES LDRD [DE-AC07-05ID14517]; Chinese 111 Research Project [B13029] FX This work is financially supported by U.S. Department of Energy (DOE) under contract no. DE-FC07-08ID14926 and DOE INL-CAES LDRD under contract no. DE-AC07-05ID14517 at the University of Idaho as well as under Chinese 111 Research Project no. B13029. The authors thank Dr. YQ Wu from Center for Advanced Energy Studies, Idaho Falls, for the help in TEM characterization. NR 46 TC 1 Z9 1 U1 14 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 13 PY 2016 VL 8 IS 14 BP 9523 EP 9531 DI 10.1021/acsami.6b01550 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DJ5UF UT WOS:000374274900079 PM 27018913 ER PT J AU Fluckiger, L Rupp, D Adolph, M Gorkhover, T Krikunova, M Muller, M Oelze, T Ovcharenko, Y Sauppe, M Schorb, S Bostedt, C Dusterer, S Harmand, M Redlin, H Treusch, R Moller, T AF Flueckiger, L. Rupp, D. Adolph, M. Gorkhover, T. Krikunova, M. Mueller, M. Oelze, T. Ovcharenko, Y. Sauppe, M. Schorb, S. Bostedt, C. Duesterer, S. Harmand, M. Redlin, H. Treusch, R. Moeller, T. TI Time-resolved x-ray imaging of a laser-induced nanoplasma and its neutral residuals SO NEW JOURNAL OF PHYSICS LA English DT Article DE clusters; free-electron laser; pump-probe experiment; time-resolved imaging; nanoplasma ID FREE-ELECTRON LASER; MULTIPLE IONIZATION; ATOMIC CLUSTERS; SPECKLE SIZE; FEMTOSECOND; PULSES; SCATTERING; DYNAMICS; NANOPARTICLES; PARTICLES AB The evolution of individual, large gas-phase xenon clusters, turned into a nanoplasma by a high power infrared laser pulse, is tracked from femtoseconds up to nanoseconds after laser excitation via coherent diffractive imaging, using ultra-short soft x-ray free electron laser pulses. A decline of scattering signal at high detection angles with increasing time delay indicates a softening of the cluster surface. Here we demonstrate, for the first time a representative speckle pattern of a new stage of cluster expansion for xenon clusters after a nanosecond irradiation. The analysis of the measured average speckle size and the envelope of the intensity distribution reveals a mean cluster size and length scale of internal density fluctuations. The measured diffraction patterns were reproduced by scattering simulations which assumed that the cluster expands with pronounced internal density fluctuations hundreds of picoseconds after excitation. C1 [Flueckiger, L.; Adolph, M.; Gorkhover, T.; Krikunova, M.; Mueller, M.; Oelze, T.; Ovcharenko, Y.; Sauppe, M.; Schorb, S.; Moeller, T.] Tech Univ Berlin, Int sOpt & Atomare Phys, Hardenbergstr 36, D-10623 Berlin, Germany. [Flueckiger, L.] La Trobe Univ, ARC Ctr Adv Mol Imaging, Dept Chem & Phys, Melbourne, Vic 3086, Australia. [Gorkhover, T.; Schorb, S.; Bostedt, C.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Ovcharenko, Y.] European XFEL GmbH, Notkestr 85, D-22607 Hamburg, Germany. [Bostedt, C.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Duesterer, S.; Harmand, M.; Redlin, H.; Treusch, R.] DESY, Notkestr 85, D-22607 Hamburg, Germany. [Harmand, M.] Inst Mineral Mat Phys & Cosmochem, 4 Pl Jussieu, F-75252 Paris, France. RP Fluckiger, L (reprint author), Tech Univ Berlin, Int sOpt & Atomare Phys, Hardenbergstr 36, D-10623 Berlin, Germany. EM l.flueckiger@latrobe.edu.au RI Rupp, Daniela/P-7590-2016; harmand, marion/Q-1248-2016 OI harmand, marion/0000-0003-0713-5824 FU BMBF [05K10KT2] FX The authors like to thank the DESY staff for their outstanding support during FLASH beamtime as well as Thomas Fennel, Christian Peltz and Ivan Vartanyants for fruitful discussions. Financial support by the BMBF grand 05K10KT2 is kindly acknowledged. NR 63 TC 2 Z9 2 U1 10 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD APR 13 PY 2016 VL 18 AR 043017 DI 10.1088/1367-2630/18/4/043017 PG 11 WC Physics, Multidisciplinary SC Physics GA DL2KY UT WOS:000375464800002 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H 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Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Measurement of top quark polarisation in t-channel single top quark production SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments); Top physics ID CHARGE ASYMMETRY; LHC; COLLISIONS; EVENTS; DECAYS AB A first measurement of the top quark spin asymmetry, sensitive to the top quark polarisation, in t-channel single top quark production is presented. It is based on a sample of pp collisions at a centre-of-mass energy of 8TeV corresponding to an integrated luminosity of 19.7 fb(-1). A high-purity sample of t-channel single top quark events with an isolated muon is selected. Signal and background components are estimated using a fit to data. A differential cross section measurement, corrected for detector effects, of an angular observable sensitive to the top quark polarisation is performed. 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M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, O.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Hidas, D.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Kothekar, K.; Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Selvaggi, M.; Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. 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[Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Martin, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; la Cruz, I. Heredia-De; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Korneeva, N.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Romero, A.; Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; De Saa, J. R. Castineiras; Manzano, P. De Castro; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Virto, A. Lopez; Marco, J.; Marco, R.; Rivero, C. Martinez; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Masetti, G.; Abbaneo, D.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoef, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Takahashi, M.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Erdmann, M.; Bertl, W.; Deiters, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Salerno, R.; Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W-S; Hsiung, Y.; Liu, Y. F.; Lu, R-S; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Scienti fi c Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; Seif El Nasr-Storey, S.; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Bell, K. W.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Magnani, A.; Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO 80309 USA. [Dittmar, M.; Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marra, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Rossini, M.; Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Roy, A.; Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J-P; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska Lincoln, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R-J; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, H.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Ff, A. Perlo; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Lamichhane, K.; Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin Madison, Madison, WI USA. [Fruehwirth, R.; Krammer, M.; Schieck, J.; Wulz, C-E; Merlin, J. A.] Vienna Univ Technol, A-1040 Vienna, Austria. CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. NICPB, Tallinn, Estonia. Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. Univ Estadual Campinas, Campinas, SP, Brazil. CNRS, IN2P3, Paris, France. Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. Joint Inst Nucl Res, Dubna, Russia. Helwan Univ, Cairo, Egypt. Beni Suef Univ, Bani Sweif, Egypt. Univ Haute Alsace, Mulhouse, France. Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. Indian Inst Sci Educ & Res, Bhopal, India. Univ Hamburg, Hamburg, Germany. Brandenburg Tech Univ Cottbus, Cottbus, Germany. Inst Nucl Res ATOMKI, Debrecen, Hungary. Eotvos Lorand Univ, Budapest, Hungary. Univ Debrecen, Debrecen, Hungary. Wigner Res Ctr Phys, Budapest, Hungary. Visva Bharati Univ, Santini Ketan, W Bengal, India. Univ Ruhuna, Matara, Sri Lanka. Isfahan Univ Technol, Esfahan, Iran. Univ Tehran, Dept Engn Sci, Tehran, Iran. Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. Univ Siena, Via Laterina 8, I-53100 Siena, Italy. Purdue Univ, W Lafayette, IN 47907 USA. Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. St Petersburg State Polytech Univ, St Petersburg, Russia. CALTECH, Pasadena, CA 91125 USA. Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. Natl Tech Univ Athens, Athens, Greece. Scuola Normale Super Pisa, Pisa, Italy. Ist Nazl Fis Nucl, Pisa, Italy. Univ Athens, Athens, Greece. Inst Theoret & Expt Phys, Moscow, Russia. Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. Gaziosmanpasa Univ, Tokat, Turkey. Adiyaman Univ, Adiyaman, Turkey. Mersin Univ, Mersin, Turkey. Cag Univ, Mersin, Turkey. Piri Reis Univ, Istanbul, Turkey. Ozyegin Univ, Istanbul, Turkey. Izmir Inst Technol, Izmir, Turkey. Marmara Univ, Istanbul, Turkey. Kafkas Univ, Kars, Turkey. Mimar Sinan Univ, Istanbul, Turkey. Yildiz Tekn Univ, Istanbul, Turkey. Hacettepe Univ, Ankara, Turkey. Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. Utah Valley Univ, Orem, UT USA. Vinca Inst Nucl Sci, Belgrade, Serbia. Univ Roma, Fac Ingn, Rome, Italy. Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. Erzincan Univ, Erzincan, Turkey. Texas A&M Univ Qatar, Doha, Qatar. Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Lokhtin, Igor/D-7004-2012; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Chinellato, Jose Augusto/I-7972-2012; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Tomei, Thiago/E-7091-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Novaes, Sergio/D-3532-2012; Dubinin, Mikhail/I-3942-2016; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; OI Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493; Saka, Halil/0000-0001-7616-2573; Brianza, Luca/0000-0001-5770-6037; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; ORTONA, Giacomo/0000-0001-8411-2971; Gallinaro, Michele/0000-0003-1261-2277; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Chinellato, Jose Augusto/0000-0002-3240-6270; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Dubinin, Mikhail/0000-0002-7766-7175; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; Androsov, Konstantin/0000-0003-2694-6542; HSIUNG, YEE/0000-0003-4801-1238 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845]; University of Malaya (Malaysia) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 50 TC 0 Z9 0 U1 18 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 13 PY 2016 IS 4 AR 073 DI 10.1007/JHEP04(2016)073 PG 42 WC Physics, Particles & Fields SC Physics GA DJ6RD UT WOS:000374339700001 ER PT J AU Tumuluri, U Rother, G Wu, ZL AF Tumuluri, Uma Rother, Gernot Wu, Zili TI Fundamental Understanding of the Interaction of Acid Gases with CeO2: From Surface Science to Practical Catalysis SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID TRANSFORM INFRARED-SPECTROSCOPY; MNO(X)-CEO2 BINARY OXIDES; REDUCED CERIA SURFACES; CARBON-DIOXIDE; LOW-TEMPERATURES; CO2 ADSORPTION; NOX REDUCTION; MIXED OXIDES; ROOM-TEMPERATURE; METAL-OXIDES AB Acid gases including CO2, SO2, and NOx are ubiquitous in large-scale energy applications including heterogeneous catalysis. The adverse environmental and health effects of these acid gases have resulted in high interest in the research and development of technologies to remove or convert these acid gases. The main challenge for the development of these technologies is to develop catalysts that are highly efficient, stable, and cost-effective, and many catalysts have been reported in this regard. CeO2 and CeO2-based catalysts have gained prominence in the removal and conversion of CO2, SO2, and NOx because of their structural robustness and redox and acid-base properties. In this article, we provide a brief overview of the application of CeO2 and CeO2-based catalysts for the removal of CO2, SO2, and NOx gases with an emphasis on the fundamental understanding of the interactions of these acid gases with CeO2. The studies summarized in this review range from surface science using single crystals and thin films with precise crystallographic planes to practical catalysis applications of nanocrystalline and polycrystalline CeO2 materials with defects and dopants. After an introduction to the properties of CeO2 surfaces, their catalytic properties for conversions of different acid gases are reviewed and discussed. The surface atomic structure, oxygen vacancies, and surface acid-base properties of CeO2 play vital roles in the surface chemistry and structure evolution during the interactions of acid gases with CeO2 and CeO2-based catalysts. C1 [Tumuluri, Uma; Rother, Gernot; Wu, Zili] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Wu, Zili] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wu, ZL (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Wu, ZL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM wuzl@ornl.gov RI Rother, Gernot/B-7281-2008 OI Rother, Gernot/0000-0003-4921-6294 FU Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This contribution was identified by Dr. Sanjaya Senanayake (Brookhaven National Laboratory, USA) as the Best Presentation in the session "CATL/ENFL: Advances in Ceria-Based Catalysis: Structural, Electronic & Chemical Properties Tailored for Chemical Conversion" of the 2015 ACS Fall Meeting in Boston, MA. This work is supported by the Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by U.S. Department of Energy, Office of Science, Basic Energy Sciences. NR 117 TC 1 Z9 1 U1 20 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 13 PY 2016 VL 55 IS 14 BP 3909 EP 3919 DI 10.1021/acs.iecr.5b05014 PG 11 WC Engineering, Chemical SC Engineering GA DJ5TY UT WOS:000374274200005 ER PT J AU Tan, CL Zhao, W Chaturvedi, A Fei, Z Zeng, ZY Chen, JZ Huang, Y Ercius, P Luo, ZM Qi, XY Chen, B Lai, ZC Li, B Zhang, X Yang, J Zong, Y Jin, CH Zheng, HM Kloc, C Zhang, H AF Tan, Chaoliang Zhao, Wei Chaturvedi, Apoorva Fei, Zhen Zeng, Zhiyuan Chen, Junze Huang, Ying Ercius, Peter Luo, Zhimin Qi, Xiaoying Chen, Bo Lai, Zhuangchai Li, Bing Zhang, Xiao Yang, Jian Zong, Yun Jin, Chuanhong Zheng, Haimei Kloc, Christian Zhang, Hua TI Preparation of Single-Layer MoS2xSe2(1-x) and MoxW1-xS2 Nanosheets with High-Concentration Metallic 1T Phase SO SMALL LA English DT Article DE dye-sensitized solar cells; metallic 1T phase; electrode materials; electrocatalysts; nanosheets ID HYDROGEN EVOLUTION REACTION; SENSITIZED SOLAR-CELLS; MOS2 NANOSHEETS; MOLYBDENUM-DISULFIDE; COUNTER ELECTRODE; EPITAXIAL-GROWTH; WS2 NANOSHEETS; LOW-COST; TRANSITION; EFFICIENCY C1 [Tan, Chaoliang; Zhao, Wei; Chaturvedi, Apoorva; Chen, Junze; Huang, Ying; Luo, Zhimin; Chen, Bo; Lai, Zhuangchai; Zhang, Xiao; Yang, Jian; Kloc, Christian; Zhang, Hua] Nanyang Technol Univ, Ctr Programmable Mat, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore. [Fei, Zhen; Jin, Chuanhong] Zhejiang Univ, Sch Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. [Zeng, Zhiyuan; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ercius, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy Mol Foundry, Berkeley, CA 94720 USA. [Qi, Xiaoying] Singapore Inst Mfg Technol, 71 Nanyang Dr, Singapore 638075, Singapore. [Li, Bing; Zong, Yun] ASTAR, IMRE, 2 Fusionopolis Way,Innovis 08-03, Singapore 138634, Singapore. RP Kloc, C; Zhang, H (reprint author), Nanyang Technol Univ, Ctr Programmable Mat, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore. EM CKloc@ntu.edu.sg; hzhang@ntu.edu.sg RI Zhang, Hua/A-1302-2009; CHEN, BO/L-1011-2015; Li, Bing/E-5575-2011; Kloc, Christian/A-2255-2011; Zong, Yun/P-1260-2016; Jin, Chuanhong/I-6460-2015 OI Zhang, Hua/0000-0001-9518-740X; CHEN, BO/0000-0001-6743-9251; Li, Bing/0000-0002-3747-3413; Zong, Yun/0000-0001-9934-0889; Jin, Chuanhong/0000-0001-8845-5664 FU MOE under AcRF Tier 2 [ARC 26/13, MOE2013-T2-1-034, ARC 19/15, MOE2014-T2-2-093]; MOE under AcRF Tier 1 [RGT18/13, RG5/13]; NTU in Singapore [M4081296.070.500000]; National Research Foundation, Prime Minister's Office, Singapore; National Basic Research Program of China [2014CB932500, 2015CB921000]; National Science Foundation of China [51222202, 51472215]; U.S. Department of Energy [DE-AC02-05CH11231] FX C.L.T., W.Z., and A.C. contributed equally to this work. This work was supported by MOE under AcRF Tier 2 (ARC 26/13, No. MOE2013-T2-1-034; ARC 19/15, No. MOE2014-T2-2-093) and AcRF Tier 1 (RGT18/13, RG5/13), and NTU under Start-Up Grant (M4081296.070.500000) in Singapore. This research is also conducted by NTU-HUJ-BGU Nanomaterials for Energy and Water Management Programme under the Campus for Research Excellence and Technological Enterprise (CREATE) that is supported by the National Research Foundation, Prime Minister's Office, Singapore. Z.F. and C.H.J. acknowledge the financial support by the National Basic Research Program of China (Grants No. 2014CB932500 and No. 2015CB921000) and the National Science Foundation of China (Grants No. 51222202 and No. 51472215). This work made use of the resources of the Center of Electron Microscopy of Zhejiang University. The experiments performed at the Molecular Foundry, Lawrence Berkeley National Laboratory were supported by the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 51 TC 8 Z9 8 U1 48 U2 111 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD APR 13 PY 2016 VL 12 IS 14 BP 1866 EP 1874 DI 10.1002/smll.201600014 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ3ZN UT WOS:000374145300006 PM 26915628 ER PT J AU Wong, K Shaw, TI Oladeinde, A Glenn, TC Oakley, B Molina, M AF Wong, Kelvin Shaw, Timothy I. Oladeinde, Adelumola Glenn, Travis C. Oakley, Brian Molina, Marirosa TI Rapid Microbiome Changes in Freshly Deposited Cow Feces under Field Conditions SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE metagenomics; cattle feces; microbiome changes; oxygen exposure; sunlight exposure; fecal contamination ID DISSOLVED ORGANIC-MATTER; RIBOSOMAL-RNA SEQUENCES; BACTERIAL-GROWTH; SP NOV.; PATHOGENIC BACTERIA; COMMUNITY ANALYSIS; SOURCE-TRACKING; BOVINE MANURE; UV-RADIATION; GEN. NOV. AB Although development of next generation sequencing (NGS) has substantially improved our understanding of the microbial ecology of animal feces, previous studies have mostly focused on freshly excreted feces. There is still limited understanding of the aging process dynamics of fecal microbiomes in intact cowpats exposed to natural environments. Fresh cowpats were sampled at multiple time points for 57 days under field conditions; half the samples were exposed to sunlight (unshaded) while the other half was protected from sunlight (shaded). The 16SRNA hypervariable region 4 was amplified from each sample and sequenced on an Illumina MiSeq Platform. While Clostridia, Bacteroidia, and Sphingobacteria were dominant classes of bacteria in fresh cowpats, Alphaproteobacteria, Betaproteobacteria, Actinobacteria, and Bacilli were the dominant classes by the end of the study, indicating a general shift from anaerobic to aerobic bacterial populations. This change was most likely influenced by the shift from cattle gut (anaerobic) to pasture ground (aerobic). Reduced moisture in cowpats may also contribute to the community shift since air can penetrate the dryer cowpat more easily. Twelve genera consisting pathogenic bacteria were detected, with Mycobacterium, Bacillus, and Clostridium being the most abundant; their combined abundance accounts for 90% of the total pathogenic genera. Taxonomic richness and diversity increased throughout the study for most samples, which could be due to bacteria regrowth and colonization of bacteria from the environment. In contrast to the high taxonomic diversity, the changes of PICRUSt inferred function profile were minimal for all cowpats throughout the study, which suggest that core functions predicted by PICRUSt may be too conserved to distinguish differences between aerobe and anaerobe. To the best of our knowledge, this is the first study demonstrating that cowpat exposure to air and sunlight can cause drastic microbiome changes soon after deposition in natural environments. Our findings offer important insights for future research characterizing the microbiome of feces collected in natural environments and the impact of cattle fecal contamination on water resources. C1 [Wong, Kelvin; Oladeinde, Adelumola; Molina, Marirosa] US EPA, Ecosyst Res Div, Athens, GA USA. [Wong, Kelvin] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Shaw, Timothy I.] Univ Georgia, Inst Bioinformat, Athens, GA 30602 USA. [Shaw, Timothy I.] St Jude Childrens Res Hosp, Dept Computat Biol, 332 N Lauderdale St, Memphis, TN 38105 USA. [Oladeinde, Adelumola; Glenn, Travis C.] Univ Georgia, Dept Environm Hlth Sci, Athens, GA 30602 USA. [Oakley, Brian] Western Univ Hlth Sci, Coll Vet Med, Pomona, CA USA. RP Molina, M (reprint author), US EPA, Ecosyst Res Div, Athens, GA USA. EM molina.marirosa@epa.gov NR 45 TC 0 Z9 0 U1 9 U2 22 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 13 PY 2016 VL 7 AR 500 DI 10.3389/fmicb.2016.00500 PG 12 WC Microbiology SC Microbiology GA DJ1RE UT WOS:000373980200001 PM 27148189 ER PT J AU Fernandez-Ramirez, C Danilkin, IV Mathieu, V Szczepaniak, AP AF Fernandez-Ramirez, Cesar Danilkin, Igor V. Mathieu, Vincent Szczepaniak, Adam P. CA Joint Phys Anal Ctr TI Understanding the nature of Lambda (1405) through Regge physics SO PHYSICAL REVIEW D LA English DT Article ID CLOUDY BAG MODEL; CHIRAL DYNAMICS; QUARK-MODEL; NUCLEON SCATTERING; BOUND-STATE; TRAJECTORIES; PHOTOPRODUCTION; RESONANCES; SYSTEM; POLES AB It appears that there are two resonances with J(P) = 1/2(-) quantum numbers in the energy region near the Lambda(1405) hyperon. The nature of these states is a topic of current debate. To provide further insight we use Regge phenomenology to access how these two resonances fit the established hyperon spectrum. We find that only one of these resonances is compatible with a three-quark state. C1 [Fernandez-Ramirez, Cesar] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, AP 70-543, Ciudad De Mexico 04510, DF, Mexico. [Fernandez-Ramirez, Cesar; Szczepaniak, Adam P.] Thomas Jefferson Natl Accelerator Facil, Theory Ctr, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Danilkin, Igor V.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Danilkin, Igor V.] Johannes Gutenberg Univ Mainz, PRISMA Cluster Excellence, D-55099 Mainz, Germany. [Mathieu, Vincent; Szczepaniak, Adam P.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47403 USA. [Mathieu, Vincent; Szczepaniak, Adam P.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. RP Fernandez-Ramirez, C (reprint author), Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, AP 70-543, Ciudad De Mexico 04510, DF, Mexico.; Fernandez-Ramirez, C (reprint author), Thomas Jefferson Natl Accelerator Facil, Theory Ctr, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM cesar.fernandez@nucleares.unam.mx RI Fernandez Ramirez, Cesar/E-9213-2010 OI Fernandez Ramirez, Cesar/0000-0001-8979-5660 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177]; U.S. Department of Energy [DE-FG0287ER40365]; National Science Foundation [PHY-1415459, PHY-1205019]; IU Collaborative Research Grant FX We thank Raul Briceno, Jose Goity, Michael Pennington, and Alessandro Pilloni for useful discussions. This material is based upon work supported in part by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contract No. DE-AC05-06OR23177. This work was also supported in part by the U.S. Department of Energy under Grant No. DE-FG0287ER40365, National Science Foundation under Grants No. PHY-1415459 and No. PHY-1205019, and an IU Collaborative Research Grant. NR 54 TC 2 Z9 2 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 13 PY 2016 VL 93 IS 7 AR 074015 DI 10.1103/PhysRevD.93.074015 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ0HA UT WOS:000373881900002 ER PT J AU Knapen, S Melia, T Papucci, M Zurek, KM AF Knapen, Simon Melia, Tom Papucci, Michele Zurek, Kathryn M. TI Rays of light from the LHC SO PHYSICAL REVIEW D LA English DT Article ID ELECTROWEAK SYMMETRY-BREAKING; ATLAS DETECTOR; PP COLLISIONS; ROOT-S=8 TEV; HIGGS-BOSON; FINAL-STATES; SEARCH; MODEL; RESONANCES; VIOLATION AB We consider models for the di-photon resonance observed at ATLAS (with 3.6 fb(-1)) and CMS (with 2.6 fb(-1)). We find there is no conflict between the signal reported at 13 TeV and the constraints from both experiments at 8 TeV with 20.3 fb(-1). We make a simple argument for why the decay to the gamma gamma mode must be generated by additional, beyond the standard model (SM) states. We explore four viable options: (i) resonance production and decay through loops of messenger fermions or scalars, (ii) a resonant messenger which decays to the di-photon resonance + X, (iii) an edge configuration where A -> B -> C gamma gamma, and (iv) Hidden Valley-like models where the resonance decays to a pair of very light (sub-GeV) states, each of which in turn decays to a pair of collimated photons that cannot be distinguished from a single photon. Since in each case multiple new states have been introduced, a wealth of signatures is expected to ensue at run 2 of the LHC. C1 [Knapen, Simon; Melia, Tom; Papucci, Michele; Zurek, Kathryn M.] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Knapen, Simon; Melia, Tom; Papucci, Michele; Zurek, Kathryn M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Knapen, S; Melia, T; Papucci, M; Zurek, KM (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA.; Knapen, S; Melia, T; Papucci, M; Zurek, KM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. EM smknapen@lbl.gov; tmelia@lbl.gov; mpapucci@lbl.gov; kzurek@berkeley.edu FU LDRD program of LBNL under U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE [DE-AC02-05CH11231]; ERC Grant [291377] FX We thank Zoltan Ligeti, Yasunori Nomura, Surjeet Rajendran and Dean Robinson for discussions. The work of S. K. and M. P. is supported in part by the LDRD program of LBNL under U.S. Department of Energy Contract No. DE-AC02-05CH11231. T. M. and K. Z. are supported by U.S. DOE Grant No. DE-AC02-05CH11231. T. M. also acknowledges computational resources provided through ERC Grant No. 291377: "LHCtheory." NR 78 TC 82 Z9 82 U1 8 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 13 PY 2016 VL 93 IS 7 AR 075020 DI 10.1103/PhysRevD.93.075020 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DJ0HA UT WOS:000373881900003 ER PT J AU Adamson, P Ader, C Andrews, M Anfimov, N Anghel, I Arms, K Arrieta-Diaz, E Aurisano, A Ayres, DS Backhouse, C Baird, M Bambah, BA Bays, K Bernstein, R Betancourt, M Bhatnagar, V Bhuyan, B Bian, J Biery, K Blackburn, T Bocean, V Bogert, D Bolshakova, A Bowden, M Bower, C Broemmelsiek, D Bromberg, C Brunetti, G Bu, X Butkevich, A Capista, D Catano-Mur, E Chase, TR Childress, S Choudhary, BC Chowdhury, B Coan, TE Coelho, JAB Colo, M Cooper, J Corwin, L Cronin-Hennessy, D Cunningham, A Davies, GS Davies, JP Del Tutto, M Derwent, PF Deepthi, KN Demuth, D Desai, S Deuerling, G Devan, A Dey, J Dharmapalan, R Ding, P Dixon, S Djurcic, Z Dukes, EC Duyang, H Ehrlich, R Feldman, GJ Felt, N Fenyves, EJ Flumerfelt, E Foulkes, S Frank, MJ Freeman, W Gabrielyan, M Gallagher, HR Gebhard, M Ghosh, T Gilbert, W Giri, A Goadhouse, S Gomes, RA Goodenough, L Goodman, MC Grichine, V Grossman, N Group, R Grudzinski, J Guarino, V Guo, B Habig, A Handler, T Hartnell, J Hatcher, R Hatzikoutelis, A Heller, K Howcroft, C Huang, J Huang, X Hylen, J Ishitsuka, M Jediny, F Jensen, C Jensen, D Johnson, C Jostlein, H Kafka, GK Kamyshkov, Y Kasahara, SMS Kasetti, S Kephart, K Koizumi, G Kotelnikov, S Kourbanis, I Krahn, Z Kravtsov, V Kreymer, A Kulenberg, C Kumar, A Kutnink, T Kwarciancy, R Kwong, J Lang, K Lee, A Lee, WM Lee, K Lein, S Liu, J Lokajicek, M Lozier, J Lu, Q Lucas, P Luchuk, S Lukens, P Lukhanin, G Magill, S Maan, K Mann, WA Marshak, ML Martens, M Martincik, J Mason, P Matera, K Mathis, M Matveev, V Mayer, N McCluskey, E Mehdiyev, R Merritt, H Messier, MD Meyer, H Miao, T Michael, D Mikheyev, SP Miller, WH Mishra, SR Mohanta, R Moren, A Mualem, L Muether, M Mufson, S Musser, J Newman, HB Nelson, JK Niner, E Norman, A Nowak, J Oksuzian, Y Olshevskiy, A Oliver, J Olson, T Paley, J Pandey, P Para, A Patterson, RB Pawloski, G Pearson, N Perevalov, D Pershey, D Peterson, E Petti, R Phan-Budd, S Piccoli, L Pla-Dalmau, A Plunkett, RK Poling, R Potukuchi, B Psihas, F Pushka, D Qiu, X Raddatz, N Radovic, A Rameika, RA Ray, R Rebel, B Rechenmacher, R Reed, B Reilly, R Rocco, D Rodkin, D Ruddick, K Rusack, R Ryabov, V Sachdev, K Sahijpal, S Sahoo, H Samoylov, O Sanchez, MC Saoulidou, N Schlabach, P Schneps, J Schroeter, R Sepulveda-Quiroz, J Shanahan, P Sherwood, B Sheshukov, A Singh, J Singh, V Smith, A Smith, D Smolik, J Solomey, N Sotnikov, A Sousa, A Soustruznik, K Stenkin, Y Strait, M Suter, L Talaga, RL Tamsett, MC Tariq, S Tas, P Tesarek, RJ Thayyullathil, RB Thomsen, K Tian, X Tognini, SC Toner, R Trevor, J Tzanakos, G Urheim, J Vahle, P Valerio, L Vinton, L Vrba, T Waldron, AV Wang, B Wang, Z Weber, A Wehmann, A Whittington, D Wilcer, N Wildberger, R Wildman, D Williams, K Wojcicki, SG Wood, K Xiao, M Xin, T Yadav, N Yang, S Zadorozhnyy, S Zalesak, J Zamorano, B Zhao, A Zirnstein, J Zwaska, R AF Adamson, P. Ader, C. Andrews, M. Anfimov, N. Anghel, I. Arms, K. Arrieta-Diaz, E. Aurisano, A. Ayres, D. S. Backhouse, C. Baird, M. Bambah, B. A. Bays, K. Bernstein, R. Betancourt, M. Bhatnagar, V. Bhuyan, B. Bian, J. Biery, K. Blackburn, T. Bocean, V. Bogert, D. Bolshakova, A. Bowden, M. Bower, C. Broemmelsiek, D. Bromberg, C. Brunetti, G. Bu, X. Butkevich, A. Capista, D. Catano-Mur, E. Chase, T. R. Childress, S. Choudhary, B. C. Chowdhury, B. Coan, T. E. Coelho, J. A. B. Colo, M. Cooper, J. Corwin, L. Cronin-Hennessy, D. Cunningham, A. Davies, G. S. Davies, J. P. Del Tutto, M. Derwent, P. F. Deepthi, K. N. Demuth, D. Desai, S. Deuerling, G. Devan, A. Dey, J. Dharmapalan, R. Ding, P. Dixon, S. Djurcic, Z. Dukes, E. C. Duyang, H. Ehrlich, R. Feldman, G. J. Felt, N. Fenyves, E. J. Flumerfelt, E. Foulkes, S. Frank, M. J. Freeman, W. Gabrielyan, M. Gallagher, H. R. Gebhard, M. Ghosh, T. Gilbert, W. Giri, A. Goadhouse, S. Gomes, R. A. Goodenough, L. Goodman, M. C. Grichine, V. Grossman, N. Group, R. Grudzinski, J. Guarino, V. Guo, B. Habig, A. Handler, T. Hartnell, J. Hatcher, R. Hatzikoutelis, A. Heller, K. Howcroft, C. Huang, J. Huang, X. Hylen, J. Ishitsuka, M. Jediny, F. Jensen, C. Jensen, D. Johnson, C. Jostlein, H. Kafka, G. K. Kamyshkov, Y. Kasahara, S. M. S. Kasetti, S. Kephart, K. Koizumi, G. Kotelnikov, S. Kourbanis, I. Krahn, Z. Kravtsov, V. Kreymer, A. Kulenberg, Ch. Kumar, A. Kutnink, T. Kwarciancy, R. Kwong, J. Lang, K. Lee, A. Lee, W. M. Lee, K. Lein, S. Liu, J. Lokajicek, M. Lozier, J. Lu, Q. Lucas, P. Luchuk, S. Lukens, P. Lukhanin, G. Magill, S. Maan, K. Mann, W. A. Marshak, M. L. Martens, M. Martincik, J. Mason, P. Matera, K. Mathis, M. Matveev, V. Mayer, N. McCluskey, E. Mehdiyev, R. Merritt, H. Messier, M. D. Meyer, H. Miao, T. Michael, D. Mikheyev, S. P. Miller, W. H. Mishra, S. R. Mohanta, R. Moren, A. Mualem, L. Muether, M. Mufson, S. Musser, J. Newman, H. B. Nelson, J. K. Niner, E. Norman, A. Nowak, J. Oksuzian, Y. Olshevskiy, A. Oliver, J. Olson, T. Paley, J. Pandey, P. Para, A. Patterson, R. B. Pawloski, G. Pearson, N. Perevalov, D. Pershey, D. Peterson, E. Petti, R. Phan-Budd, S. Piccoli, L. Pla-Dalmau, A. Plunkett, R. K. Poling, R. Potukuchi, B. Psihas, F. Pushka, D. Qiu, X. Raddatz, N. Radovic, A. Rameika, R. A. Ray, R. Rebel, B. Rechenmacher, R. Reed, B. Reilly, R. Rocco, D. Rodkin, D. Ruddick, K. Rusack, R. Ryabov, V. Sachdev, K. Sahijpal, S. Sahoo, H. Samoylov, O. Sanchez, M. C. Saoulidou, N. Schlabach, P. Schneps, J. Schroeter, R. Sepulveda-Quiroz, J. Shanahan, P. Sherwood, B. Sheshukov, A. Singh, J. Singh, V. Smith, A. Smith, D. Smolik, J. Solomey, N. Sotnikov, A. Sousa, A. Soustruznik, K. Stenkin, Y. Strait, M. Suter, L. Talaga, R. L. Tamsett, M. C. Tariq, S. Tas, P. Tesarek, R. J. Thayyullathil, R. B. Thomsen, K. Tian, X. Tognini, S. C. Toner, R. Trevor, J. Tzanakos, G. Urheim, J. Vahle, P. Valerio, L. Vinton, L. Vrba, T. Waldron, A. V. Wang, B. Wang, Z. Weber, A. Wehmann, A. Whittington, D. Wilcer, N. Wildberger, R. Wildman, D. Williams, K. Wojcicki, S. G. Wood, K. Xiao, M. Xin, T. Yadav, N. Yang, S. Zadorozhnyy, S. Zalesak, J. Zamorano, B. Zhao, A. Zirnstein, J. Zwaska, R. TI First Measurement of Electron Neutrino Appearance in NOvA SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELASTIC TRACKING; OSCILLATIONS; ALGORITHM; MATTER AB We report results from the first search for nu(mu) -> nu(e) transitions by the NOvA experiment. In an exposure equivalent to 2.74 x 10(20) protons on target in the upgraded NuMI beam at Fermilab, we observe 6 events in the Far Detector, compared to a background expectation of 0.99 +/- 0.11 (syst) events based on the Near Detector measurement. A secondary analysis observes 11 events with a background of 1.07 +/- 0.14 (syst). The 3.3 sigma excess of events observed in the primary analysis disfavors 0.1 pi < delta(CP) < 0.5 pi in the inverted mass hierarchy at the 90% C.L. C1 [Ayres, D. S.; Dharmapalan, R.; Djurcic, Z.; Goodenough, L.; Goodman, M. C.; Grudzinski, J.; Guarino, V.; Huang, X.; Magill, S.; Sahoo, H.; Sanchez, M. C.; Sepulveda-Quiroz, J.; Suter, L.; Talaga, R. L.; Wood, K.; Zhao, A.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lokajicek, M.; Zalesak, J.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Singh, V.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Lee, K.] Univ Calif Los Angeles, Dept Phys & Astron, Box 951547, Los Angeles, CA 90095 USA. [Backhouse, C.; Bays, K.; Howcroft, C.; Lozier, J.; Michael, D.; Mualem, L.; Newman, H. B.; Patterson, R. B.; Pershey, D.; Trevor, J.] CALTECH, Pasadena, CA 91125 USA. [Soustruznik, K.; Tas, P.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, Prague, Czech Republic. [Aurisano, A.; Sousa, A.; Yang, S.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Thayyullathil, R. B.] Cochin Univ Sci & Technol, Dept Phys, Kochi 682022, Kerala, India. [Jediny, F.; Martincik, J.; Smolik, J.; Vrba, T.] Czech Tech Univ, Brehova 7, Prague 11519 1, Czech Republic. [Choudhary, B. C.; Pandey, P.] Univ Delhi, Dept Phys & Astrophys, Delhi 110007, India. [Adamson, P.; Ader, C.; Andrews, M.; Aurisano, A.; Bernstein, R.; Biery, K.; Bocean, V.; Bogert, D.; Bowden, M.; Broemmelsiek, D.; Brunetti, G.; Bu, X.; Capista, D.; Childress, S.; Cooper, J.; Del Tutto, M.; Derwent, P. F.; Deuerling, G.; Dey, J.; Ding, P.; Dixon, S.; Foulkes, S.; Freeman, W.; Grossman, N.; Hatcher, R.; Hylen, J.; Jensen, C.; Jensen, D.; Jostlein, H.; Kephart, K.; Koizumi, G.; Kourbanis, I.; Kreymer, A.; Kwarciancy, R.; Lee, A.; Lee, W. M.; Lu, Q.; Lucas, P.; Lukens, P.; Lukhanin, G.; Martens, M.; Matera, K.; McCluskey, E.; Miao, T.; Norman, A.; Paley, J.; Para, A.; Perevalov, D.; Piccoli, L.; Pla-Dalmau, A.; Plunkett, R. K.; Pushka, D.; Rameika, R. A.; Ray, R.; Rebel, B.; Rechenmacher, R.; Reilly, R.; Saoulidou, N.; Schlabach, P.; Shanahan, P.; Tariq, S.; Tesarek, R. J.; Valerio, L.; Wehmann, A.; Wilcer, N.; Wildman, D.; Williams, K.; Xiao, M.; Zwaska, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Ghosh, T.; Gomes, R. A.; Tognini, S. C.] Univ Fed Goias, Inst Fis, BR-74690900 Goiania, Go, Brazil. [Bhuyan, B.; Yadav, N.] IIT Guwahati, Dept Phys, Gauhati 781039, India. [Feldman, G. J.; Felt, N.; Kafka, G. K.; Oliver, J.; Schroeter, R.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Bambah, B. A.; Deepthi, K. N.; Kasetti, S.; Mohanta, R.] Univ Hyderabad, Sch Phys, Hyderabad 500046, Andhra Pradesh, India. [Giri, A.] IIT Hyderabad, Dept Phys, Hyderabad 502205, Andhra Pradesh, India. [Baird, M.; Bower, C.; Davies, G. S.; Gebhard, M.; Ishitsuka, M.; Johnson, C.; Merritt, H.; Messier, M. D.; Mufson, S.; Musser, J.; Niner, E.; Psihas, F.; Urheim, J.; Whittington, D.] Indiana Univ, Bloomington, IN 47405 USA. [Butkevich, A.; Luchuk, S.; Matveev, V.; Mikheyev, S. P.; Rodkin, D.; Stenkin, Y.; Zadorozhnyy, S.] Russian Acad Sci, Inst Nucl Res, 7A 60th October Anniversary Prospect, Moscow 117312, Russia. [Anghel, I.; Catano-Mur, E.; Kutnink, T.; Sanchez, M. C.; Sepulveda-Quiroz, J.; Xin, T.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Anghel, I.; Potukuchi, B.] Univ Jammu, Dept Phys & Elect, Jammu 180006, Jammu & Kashmir, India. [Anfimov, N.; Bolshakova, A.; Kulenberg, Ch.; Olshevskiy, A.; Samoylov, O.; Sheshukov, A.; Sotnikov, A.] Joint Inst Nucl Res Joliot Curie, Dubna 141980 6, Moscow Region, Russia. [Grichine, V.; Kotelnikov, S.; Ryabov, V.] Lebedev Phys Inst, Dept Nucl Phys, Leninsky Prospect 53, Moscow 119991, Russia. [Bromberg, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Demuth, D.] Univ Minnesota Crookston, Math Sci & Technol Dept, Crookston, MN 56716 USA. [Habig, A.; Moren, A.; Thomsen, K.] Univ Minnesota Duluth, Dept Phys & Astron, Duluth, MN 55812 USA. [Arms, K.; Betancourt, M.; Bian, J.; Chase, T. R.; Cronin-Hennessy, D.; Desai, S.; Gabrielyan, M.; Gilbert, W.; Heller, K.; Kasahara, S. M. S.; Krahn, Z.; Kwong, J.; Lein, S.; Marshak, M. L.; Miller, W. H.; Nowak, J.; Pawloski, G.; Pearson, N.; Peterson, E.; Poling, R.; Raddatz, N.; Rocco, D.; Ruddick, K.; Rusack, R.; Sachdev, K.; Sherwood, B.; Smith, A.; Strait, M.; Wildberger, R.; Zirnstein, J.] Univ Minnesota Twin Cities, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Bhatnagar, V.; Kumar, A.; Maan, K.; Sahijpal, S.; Singh, J.] Panjab Univ, Dept Phys, Chandigarh 106014, India. [Weber, A.] Rutherford Appleton Lab, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Chowdhury, B.; Duyang, H.; Guo, B.; Mishra, S. R.; Petti, R.; Tian, X.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Corwin, L.; Reed, B.; Smith, D.] South Dakota Sch Mines & Technol, Rapid City, SD 57701 USA. [Arrieta-Diaz, E.; Coan, T. E.; Kravtsov, V.; Wang, B.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Blackburn, T.; Davies, J. P.; Hartnell, J.; Tamsett, M. C.; Vinton, L.; Waldron, A. V.; Zamorano, B.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Flumerfelt, E.; Handler, T.; Hatzikoutelis, A.; Kamyshkov, Y.; Mason, P.] Univ Tennessee, Dept Phys & Astron, 1408 Circle Dr, Knoxville, TN 37996 USA. [Huang, J.; Lang, K.; Mehdiyev, R.] Univ Texas Austin, Dept Phys, 1 Univ Stn C1600, Austin, TX 78712 USA. [Cunningham, A.; Fenyves, E. J.] Univ Texas Dallas, Dept Phys, 800 W Campbell Rd, Dallas, TX 75083 USA. [Coelho, J. A. B.; Gallagher, H. R.; Mann, W. A.; Mayer, N.; Olson, T.; Schneps, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Dukes, E. C.; Ehrlich, R.; Frank, M. J.; Goadhouse, S.; Group, R.; Oksuzian, Y.; Wang, Z.] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA. [Meyer, H.; Muether, M.; Solomey, N.] Wichita State Univ, Div Phys, 1845 Fairmout St, Wichita, KS 67220 USA. [Colo, M.; Devan, A.; Liu, J.; Mathis, M.; Nelson, J. K.; Radovic, A.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Phan-Budd, S.] Winona State Univ, Dept Phys, POB 5838, Winona, MN 55987 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RI Anfimov, Nikolay/I-1322-2016; Olshevskiy, Alexander/I-1580-2016; Samoylov, Oleg/L-7271-2013; Kamyshkov, Yuri/J-7999-2016; Nowak, Jaroslaw/P-2502-2016; Martincik, Jiri/H-3566-2014; Stenkin, Yuri/M-5796-2014; Ryabov, Vladimir/E-1281-2014; Kotelnikov, Sergey/A-9711-2014; Gomes, Ricardo/B-6899-2008; Sheshukov, Andrey/I-1193-2016 OI Corwin, Luke/0000-0001-7143-3821; Hartnell, Jeffrey/0000-0002-1744-7955; Bernstein, Robert/0000-0002-7610-950X; Weber, Alfons/0000-0002-8222-6681; Anfimov, Nikolay/0000-0002-9099-7574; Olshevskiy, Alexander/0000-0002-8902-1793; Samoylov, Oleg/0000-0003-2141-8230; Kamyshkov, Yuri/0000-0002-3789-7152; Nowak, Jaroslaw/0000-0001-8637-5433; Martincik, Jiri/0000-0002-5379-441X; Group, Robert/0000-0002-4097-5254; Kotelnikov, Sergey/0000-0002-8027-4612; Gomes, Ricardo/0000-0003-0278-4876; FU U.S. Department of Energy; U.S. National Science Foundation; Department of Science and Technology, India; European Research Council; MSMT CR, Czech Republic; RAS, Russia; RMES, Russia; RFBR, Russia; CNPq, Brazil; FAPEG, Brazil; State and University of Minnesota; U.S. DOE [De-AC02-07CH11359] FX This work was supported by the U.S. Department of Energy; the U.S. National Science Foundation; the Department of Science and Technology, India; the European Research Council; the MSMT CR, Czech Republic; the RAS, RMES, and RFBR, Russia; CNPq and FAPEG, Brazil; and the State and University of Minnesota. We are grateful for the contributions of the staffs at the University of Minnesota module assembly facility and Ash River Laboratory, at the Argonne National Laboratory, and at Fermilab. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. De-AC02-07CH11359 with the U.S. DOE. NR 55 TC 28 Z9 28 U1 8 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 13 PY 2016 VL 116 IS 15 AR 151806 DI 10.1103/PhysRevLett.116.151806 PG 7 WC Physics, Multidisciplinary SC Physics GA DJ0IA UT WOS:000373884500003 PM 27127961 ER PT J AU Butch, NP Paglione, J Chow, P Xiao, YM Marianetti, CA Booth, CH Jeffries, JR AF Butch, Nicholas P. Paglione, Johnpierre Chow, Paul Xiao, Yuming Marianetti, Chris A. Booth, Corwin H. Jeffries, Jason R. TI Pressure-Resistant Intermediate Valence in the Kondo Insulator SmB6 SO PHYSICAL REVIEW LETTERS LA English DT Article ID EMISSION-SPECTROSCOPY; SAMARIUM; SUSCEPTIBILITY; TRANSITION; HEXABORIDE; STATES AB Resonant x-ray emission spectroscopy was used to determine the pressure dependence of the f-electron occupancy in the Kondo insulator SmB6. Applied pressure reduces the f occupancy, but surprisingly, the material maintains a significant divalent character up to a pressure of at least 35 GPa. Thus, the closure of the resistive activation energy gap and onset of magnetic order are not driven by stabilization of an integer valent state. Over the entire pressure range, the material maintains a remarkably stable intermediate valence that can in principle support a nontrivial band structure. C1 [Butch, Nicholas P.; Paglione, Johnpierre] Univ Maryland, Dept Phys, Ctr Nanophys & Adv Mat, College Pk, MD 20742 USA. [Butch, Nicholas P.] NIST, Ctr Neutron Res, 100 Bur Dr, Gaithersburg, MD 20899 USA. [Butch, Nicholas P.; Jeffries, Jason R.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Chow, Paul; Xiao, Yuming] Carnegie Inst Sci, Geophys Lab, HP CAT, Argonne, IL 60439 USA. [Marianetti, Chris A.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Butch, NP (reprint author), Univ Maryland, Dept Phys, Ctr Nanophys & Adv Mat, College Pk, MD 20742 USA.; Butch, NP (reprint author), NIST, Ctr Neutron Res, 100 Bur Dr, Gaithersburg, MD 20899 USA.; Butch, NP (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM nicholas.butch@nist.gov FU CNAM; LLNL PLS directorate; Science Campaign; DOE-NNSA [DE-NA0001974]; DOE-BES [DE-FG02-99ER45775]; NSF; DOE Office of Science [DE-AC02-06CH11357]; DOE, NNSA [DE-AC52-07NA27344]; AFOSR-MURI [FA9550-09-1-0603]; NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids [DMR-1420634]; Office of Science (OS), Office of Basic Energy Sciences (OBES), Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX N. P. B. acknowledges support by CNAM and the LLNL PLS directorate. J. R. J. is partially supported by the Science Campaign. Portions of this work were performed under LDRD (Tracking Code 14-ERD-041). This work was performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. The Advanced Photon Source is a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. LLNL is operated by Lawrence Livermore National Security, LLC, for the DOE, NNSA under Contract No. DE-AC52-07NA27344. Crystal growth at UMD was supported by AFOSR-MURI (FA9550-09-1-0603). C. A. M. was supported by the NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids (DMR-1420634). Work at Lawrence Berkeley National Laboratory was supported by the Director, Office of Science (OS), Office of Basic Energy Sciences (OBES), Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. NR 51 TC 1 Z9 1 U1 15 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 13 PY 2016 VL 116 IS 15 AR 156401 DI 10.1103/PhysRevLett.116.156401 PG 5 WC Physics, Multidisciplinary SC Physics GA DJ0IA UT WOS:000373884500005 PM 27127976 ER PT J AU Watts, AL Andersson, N Chakrabarty, D Feroci, M Hebeler, K Israel, G Lamb, FK Miller, MC Morsink, S Ozel, F Patruno, A Poutanen, J Psaltis, D Schwenk, A Steiner, AW Stella, L Tolos, L van der Klis, M AF Watts, Anna L. Andersson, Nils Chakrabarty, Deepto Feroci, Marco Hebeler, Kai Israel, Gianluca Lamb, Frederick K. Miller, M. Coleman Morsink, Sharon Oezel, Feryal Patruno, Alessandro Poutanen, Juri Psaltis, Dimitrios Schwenk, Achim Steiner, Andrew W. Stella, Luigi Tolos, Laura van der Klis, Michiel TI Colloquium: Measuring the neutron star equation of state using x-ray timing SO REVIEWS OF MODERN PHYSICS LA English DT Article ID QUASI-PERIODIC OSCILLATIONS; MASS-RADIUS RELATION; ROTATING RELATIVISTIC STARS; AXISYMMETRICAL TOROIDAL MODES; ACCRETING MILLISECOND PULSARS; HARTLE-THORNE APPROXIMATION; SHORT RECURRING BURSTS; SYSTEM PSR J1023+0038; MAGNETAR OSCILLATIONS; LIGHT CURVES AB One of the primary science goals of the next generation of hard x-ray timing instruments is to determine the equation of state of matter at supranuclear densities inside neutron stars by measuring the radius of neutron stars with different masses to accuracies of a few percent. Three main techniques can be used to achieve this goal. The first involves waveform modeling. The flux observed from a hotspot on the neutron star surface offset from the rotational pole will be modulated by the star's rotation, and this periodic modulation at the spin frequency is called a pulsation. As the photons propagate through the curved spacetime of the star, information about mass and radius is encoded into the shape of the waveform (pulse profile) via special and general-relativistic effects. Using pulsations from known sources (which have hotspots that develop either during thermonuclear bursts or due to channeled accretion) it is possible to obtain tight constraints on mass and radius. The second technique involves characterizing the spin distribution of accreting neutron stars. A large collecting area enables highly sensitive searches for weak or intermittent pulsations (which yield spin) from the many accreting neutron stars whose spin rates are not yet known. The most rapidly rotating stars provide a clean constraint, since the limiting spin rate where the equatorial surface velocity is comparable to the local orbital velocity, at which mass shedding occurs, is a function of mass and radius. However, the overall spin distribution also provides a guide to the torque mechanisms in operation and the moment of inertia, both of which can depend sensitively on dense matter physics. The third technique is to search for quasiperiodic oscillations in x-ray flux associated with global seismic vibrations of magnetars (the most highly magnetized neutron stars), triggered by magnetic explosions. The vibrational frequencies depend on stellar parameters including the dense matter equation of state, and large-area x-ray timing instruments would provide much improved detection capability. An illustration is given of how these complementary x-ray timing techniques can be used to constrain the dense matter equation of state and the results that might be expected from a 10 m(2) instrument are discussed. Also discussed are how the results from such a facility would compare to other astronomical investigations of neutron star properties. C1 [Watts, Anna L.] Univ Amsterdam, Anton Pannekoek Inst, POB 94249, NL-1090 GE Amsterdam, Netherlands. [Andersson, Nils] Univ Southampton, Math Sci, Southampton SO17 1BJ, Hants, England. [Chakrabarty, Deepto] MIT, Kavli Inst Astrophys & Space Res, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Feroci, Marco] INAF IASF Roma, Via Fosso del Cavaliere 100, I-00133 Rome, Italy. [Feroci, Marco] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Via Ric Sci 1, I-00133 Rome, Italy. [Hebeler, Kai; Schwenk, Achim] Tech Univ Darmstadt, Inst Kernphys, Petersenstr 30, D-64289 Darmstadt, Germany. [Hebeler, Kai; Schwenk, Achim] GSI Helmholtzzentrum Schwerionenforsch GmbH, ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Israel, Gianluca; Stella, Luigi] Osserv Astron Roma, INAF, Via Frascati 33, I-00040 Rome, Italy. [Lamb, Frederick K.] Univ Illinois, Dept Phys, 1110 West Green St, Urbana, IL 61801 USA. [Miller, M. Coleman] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Morsink, Sharon] Univ Alberta, Dept Phys, 4-181 CCIS, Edmonton, AB T6G 2E1, Canada. [Oezel, Feryal; Psaltis, Dimitrios] Univ Arizona, Steward Observ, 933 North Cherry Ave, Tucson, AZ 85721 USA. [Patruno, Alessandro] Leiden Univ, Leiden Observ, POB 9513, NL-2300 RA Leiden, Netherlands. [Poutanen, Juri] Univ Turku, Dept Phys & Astron, Tuorla Observ, Vaisalantie 20, FIN-21500 Piikkio, Finland. [Steiner, Andrew W.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Steiner, Andrew W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Tolos, Laura] Inst Ciencias Espacio IEEC CSIC, Campus UAB,Carrer de Can Magrans S-N, Cerdanyola Del Valles 08193, Spain. [van der Klis, Michiel] Univ Amsterdam, Anton Pannekoek Inst, POB 94249, NL-1090 GE Amsterdam, Netherlands. RP Watts, AL (reprint author), Univ Amsterdam, Anton Pannekoek Inst, POB 94249, NL-1090 GE Amsterdam, Netherlands. RI Poutanen, Juri/H-6651-2016; OI Poutanen, Juri/0000-0002-0983-0049; Israel, GianLuca/0000-0001-5480-6438 FU NWO Vidi Grant [639.042.916, 639.042.319]; NWO Vrije Competitie Grant [614.001.201]; ERC [639217 CSINEUTRONSTAR, 307986 STRONGINT]; DFG [SFB 634]; Italian Space Agency (ASI) [I/021/12/0]; Ramon y Cajal Research Programme; Ministerio de Economia y Competitividad [FPA2010-16963, FPA2013-43425-P]; FP7-PEOPLE-CIG [PCIG09-GA-2011-291679]; NewCompStar (COST Action) [MP1304]; NSERC; Academy of Finland [268740]; U.S. Department of Energy Office of Nuclear Physics FX We thank all of the members of the LOFT Consortium, in particular, the members of the LOFT Dense Matter Working Group, for useful discussions. A. L. W. acknowledges support from NWO Vidi Grant No. 639.042.916, NWO Vrije Competitie Grant No. 614.001.201, and ERC Starting Grant No. 639217 CSINEUTRONSTAR. The work of K. H. and A. S. is supported by ERC Grant No. 307986 STRONGINT and the DFG through Grant No. SFB 634. M. F., G. I., and L. S. acknowledge support from the Italian Space Agency (ASI) under Contract No. I/021/12/0. L. T. acknowledges support from the Ramon y Cajal Research Programme and from Contracts No. FPA2010-16963 and No. FPA2013-43425-P of Ministerio de Economia y Competitividad, from FP7-PEOPLE-2011-CIG under Contract No. PCIG09-GA-2011-291679, as well as NewCompStar (COST Action MP1304). S. M. acknowledges support from NSERC. J. P. acknowledges the Academy of Finland Grant No. 268740. A. P. acknowledges support from NWO Vidi Grant No. 639.042.319. A. W. S. was supported by the U.S. Department of Energy Office of Nuclear Physics. NR 273 TC 11 Z9 11 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0034-6861 EI 1539-0756 J9 REV MOD PHYS JI Rev. Mod. Phys. PD APR 13 PY 2016 VL 88 IS 2 AR 021001 DI 10.1103/RevModPhys.88.021001 PG 20 WC Physics, Multidisciplinary SC Physics GA DJ0IH UT WOS:000373885200001 ER PT J AU Lee, E Xia, Y Ferrier, RC Kim, HN Gharbi, MA Stebe, KJ Kamien, RD Composto, RJ Yang, S AF Lee, Elaine Xia, Yu Ferrier, Robert C., Jr. Kim, Hye-Na Gharbi, Mohamed A. Stebe, Kathleen J. Kamien, Randall D. Composto, Russell J. Yang, Shu TI Fine Golden Rings: Tunable Surface Plasmon Resonance from Assembled Nanorods in Topological Defects of Liquid Crystals SO ADVANCED MATERIALS LA English DT Article ID AU NANORODS; NANOPARTICLES; ARRAYS; TEMPERATURE; SHAPE; BULK C1 [Lee, Elaine] Lawrence Livermore Natl Lab, Engn Directorate, Livermore, CA 94550 USA. [Lee, Elaine; Xia, Yu; Kim, Hye-Na; Gharbi, Mohamed A.; Composto, Russell J.; Yang, Shu] Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. [Ferrier, Robert C., Jr.; Gharbi, Mohamed A.; Stebe, Kathleen J.] Univ Penn, Dept Chem & Biomol Engn, 220 South 33rd St, Philadelphia, PA 19104 USA. [Gharbi, Mohamed A.; Kamien, Randall D.] Univ Penn, Dept Phys & Astron, 220 South 33rd St, Philadelphia, PA 19104 USA. RP Yang, S (reprint author), Univ Penn, Dept Mat Sci & Engn, 3231 Walnut St, Philadelphia, PA 19104 USA. EM shuyang@seas.upenn.edu RI Yang, Shu/D-9758-2011; Ferrier, Robert/A-1128-2016; OI Ferrier, Robert/0000-0002-5123-7433; Kamien, Randall/0000-0003-1598-5626 FU National Science Foundation (NSF) Materials Science and Engineering Center (MRSEC) [DMR-1120901]; NSF Polymer Program [DMR-09-07493]; Simons Foundation; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344, LLNL-ABS-678248] FX E.L., Y.X., and R.C.F. contributed equally to this work. This work was supported by the National Science Foundation (NSF) Materials Science and Engineering Center (MRSEC) Grant to the University of Pennsylvania, Grant No. DMR-1120901. This work was also partially supported by the NSF Polymer Program (Grant No. DMR-09-07493, R.J.C.) and a Simons Investigator grant from the Simons Foundation to R.D.K. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344, LLNL-ABS-678248. NR 38 TC 4 Z9 4 U1 22 U2 64 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 13 PY 2016 VL 28 IS 14 BP 2731 EP 2736 DI 10.1002/adma.201506084 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DI9RH UT WOS:000373839600007 PM 26853906 ER PT J AU Kumar, S Graves, CE Strachan, JP Grafals, EM Kilcoyne, ALD Tyliszczak, T Weker, JN Nishi, Y Williams, RS AF Kumar, Suhas Graves, Catherine E. Strachan, John Paul Grafals, Emmanuelle Merced Kilcoyne, Arthur L. David Tyliszczak, Tolek Weker, Johanna Nelson Nishi, Yoshio Williams, R. Stanley TI Direct Observation of Localized Radial Oxygen Migration in Functioning Tantalum Oxide Memristors SO ADVANCED MATERIALS LA English DT Article ID RESISTANCE-CHANGE MEMORY; TRANSITION-METAL OXIDES; MODEL; FILMS; MECHANISM; SURFACES; DEVICES C1 [Kumar, Suhas; Graves, Catherine E.; Strachan, John Paul; Grafals, Emmanuelle Merced; Williams, R. Stanley] Hewlett Packard Labs, 1501 Page Mill Rd, Palo Alto, CA 94304 USA. [Kumar, Suhas; Nishi, Yoshio] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Kilcoyne, Arthur L. David; Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Weker, Johanna Nelson] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Strachan, JP (reprint author), Hewlett Packard Labs, 1501 Page Mill Rd, Palo Alto, CA 94304 USA. EM john-paul.strachan@hpe.com RI Kilcoyne, David/I-1465-2013; Williams, R. Stanley/A-8281-2009 OI Williams, R. Stanley/0000-0003-0213-4259 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX O K-edge spectromicroscopy was performed at Advanced Light Source (ALS) on beamlines 11.0.2 and 5.3.2.2 using focused scanning transmission X-ray microscopes. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Ta L-edge spectromicroscopy was performed at Stanford Synchrotron Radiation Lightsource (SSRL) on beamline 6-2 using a transmission X-ray microscope. Use of the SSRL, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The authors gratefully thank Antonio Torrezan, Max Zhang, Kate Norris, Alpha N'Diaye, David Brothers, and Zhiyong Li for helping with experimental setup, film growth, X-ray characterization, electron microscopy, and useful comments. NR 43 TC 7 Z9 8 U1 10 U2 39 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 13 PY 2016 VL 28 IS 14 BP 2772 EP 2776 DI 10.1002/adma.201505435 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DI9RH UT WOS:000373839600013 PM 26833926 ER PT J AU Ross, MB Ku, JC Lee, B Mirkin, CA Schatz, GC AF Ross, Michael B. Ku, Jessie C. Lee, Byeongdu Mirkin, Chad A. Schatz, George C. TI Plasmonic Metallurgy Enabled by DNA SO ADVANCED MATERIALS LA English DT Article ID NANOPARTICLE SUPERLATTICES; OPTICAL-PROPERTIES; NANOSTRUCTURES; CRYSTALLIZATION; METAMATERIALS; NANOSCALE C1 [Ross, Michael B.; Mirkin, Chad A.; Schatz, George C.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Ross, Michael B.; Mirkin, Chad A.; Schatz, George C.] Northwestern Univ, Int Inst Nanotechnol, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Ku, Jessie C.; Mirkin, Chad A.] Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. [Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Mirkin, CA; Schatz, GC (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Mirkin, CA; Schatz, GC (reprint author), Northwestern Univ, Int Inst Nanotechnol, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM chadnano@northwestern.edu; g-schatz@northwestern.edu RI Mirkin, Chad/E-3911-2010; OI Ross, Michael/0000-0002-2511-0594; Lee, Byeongdu/0000-0003-2514-8805 FU AFOSR MURI [FA9550-11-1-0275]; Northwestern Materials Research Center under NSF [DMR-1121262]; Department of Energy, Office of Basic Energy Science [DE-FG02-09ER16109]; NDSEG graduate fellowship program; Office of the Provost; Office for Research; Northwestern University Information Technology; DOE [DE-AC02-06CH11357] FX This research was supported by AFOSR MURI grant FA9550-11-1-0275 and by the Northwestern Materials Research Center under NSF grant DMR-1121262. Theory research was supported by the Department of Energy, Office of Basic Energy Science, under grant DE-FG02-09ER16109. M.B.R. and J.C.K. gratefully acknowledge support through the NDSEG graduate fellowship program. Computational time was provided by the Quest High-Performance Computing facility at Northwestern University, which was jointly supported by the Office of the Provost, the Office for Research, and Northwestern University Information Technology. GISAXS experiments were performed at beamline 12-ID-B at the Advanced Photon Source (APS), Argonne National Laboratory, and use of the APS was supported by the DOE (DE-AC02-06CH11357). NR 29 TC 4 Z9 4 U1 24 U2 55 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 13 PY 2016 VL 28 IS 14 BP 2790 EP 2794 DI 10.1002/adma.201505806 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DI9RH UT WOS:000373839600016 PM 26849019 ER PT J AU Higginbotham, A Stubley, PG Comley, AJ Eggert, JH Foster, JM Kalantar, DH McGonegle, D Patel, S Peacock, LJ Rothman, SD Smith, RF Suggit, MJ Wark, JS AF Higginbotham, A. Stubley, P. G. Comley, A. J. Eggert, J. H. Foster, J. M. Kalantar, D. H. McGonegle, D. Patel, S. Peacock, L. J. Rothman, S. D. Smith, R. F. Suggit, M. J. Wark, J. S. TI Inelastic response of silicon to shock compression SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY-DIFFRACTION; PHASE-TRANSITION; MOLECULAR-DYNAMICS; GERMANIUM AB The elastic and inelastic response of [001] oriented silicon to laser compression has been a topic of considerable discussion for well over a decade, yet there has been little progress in understanding the basic behaviour of this apparently simple material. We present experimental x-ray diffraction data showing complex elastic strain profiles in laser compressed samples on nanosecond timescales. We also present molecular dynamics and elasticity code modelling which suggests that a pressure induced phase transition is the cause of the previously reported 'anomalous' elastic waves. Moreover, this interpretation allows for measurement of the kinetic timescales for transition. This model is also discussed in the wider context of reported deformation of silicon to rapid compression in the literature. C1 [Higginbotham, A.; Stubley, P. G.; McGonegle, D.; Patel, S.; Suggit, M. J.; Wark, J. S.] Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. [Comley, A. J.; Foster, J. M.; Peacock, L. J.; Rothman, S. D.] Atom Weap Estab, Reading RG7 4PR, Berks, England. [Eggert, J. H.; Kalantar, D. H.; Smith, R. F.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Higginbotham, A.] Univ York, Dept Phys, York Plasma Inst, York YO10 5DD, N Yorkshire, England. RP Higginbotham, A (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. EM andrew.higginbotham@york.ac.uk FU CLF at the Rutherford Appleton Laboratory; AWE; EPSRC [EP/J017256/1]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Ed Gumbrell, Jon Skidmore, Siddarth Patankar, Jim Fyrth, Graham Cooper and the staff at Orion for their experimental support, and acknowledge target preparation support from the CLF at the Rutherford Appleton Laboratory. AH and PGS would like to thank AWE for financial support. MJS, DM and JSW are grateful for support from EPSRC under grant number EP/J017256/1. The work by JHE, DHK and RFS was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 31 TC 1 Z9 1 U1 10 U2 21 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 13 PY 2016 VL 6 AR 24211 DI 10.1038/srep24211 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ0SX UT WOS:000373915800002 PM 27071341 ER PT J AU Hinton, JP Thewalt, E Alpichshev, Z Mahmood, F Koralek, JD Chan, MK Veit, MJ Dorow, CJ Barisic, N Kemper, AF Bonn, DA Hardy, WN Liang, RX Gedik, N Greven, M Lanzara, A Orenstein, J AF Hinton, J. P. Thewalt, E. Alpichshev, Z. Mahmood, F. Koralek, J. D. Chan, M. K. Veit, M. J. Dorow, C. J. Barisic, N. Kemper, A. F. Bonn, D. A. Hardy, W. N. Liang, Ruixing Gedik, N. Greven, M. Lanzara, A. Orenstein, J. TI The rate of quasiparticle recombination probes the onset of coherence in cuprate superconductors SO SCIENTIFIC REPORTS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTOR; T-C CUPRATE; PSEUDOGAP STATE; CHARGE ORDER; UNDERDOPED BI2SR2CACU2O8+DELTA; FLUCTUATIONS; DYNAMICS; YBA2CU3O7-DELTA; FILMS AB In the underdoped copper-oxides, high-temperature superconductivity condenses from a nonconventional metallic "pseudogap" phase that exhibits a variety of non-Fermi liquid properties. Recently, it has become clear that a charge density wave (CDW) phase exists within the pseudogap regime. This CDW coexists and competes with superconductivity (SC) below the transition temperature T-c, suggesting that these two orders are intimately related. Here we show that the condensation of the superfluid from this unconventional precursor is reflected in deviations from the predictions of BSC theory regarding the recombination rate of quasiparticles. We report a detailed investigation of the quasiparticle (QP) recombination lifetime, tau(qp),, as a function of temperature and magnetic field in underdoped HgBa2CuO4+delta (Hg-1201) and YBa2Cu3O6+x (YBCO) single crystals by ultrafast time-resolved reflectivity. We find that tau qp(T) exhibits a local maximum in a small temperature window near T-c that is prominent in underdoped samples with coexisting charge order and vanishes with application of a small magnetic field. We explain this unusual, non-BCS behavior by positing that T-c marks a transition from phase-fluctuating SC/CDW composite order above to a SC/CDW condensate below. Our results suggest that the superfluid in underdoped cuprates is a condensate of coherently-mixed particle-particle and particle-hole pairs. C1 [Hinton, J. P.; Thewalt, E.; Koralek, J. D.; Kemper, A. F.; Lanzara, A.; Orenstein, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Hinton, J. P.; Thewalt, E.; Lanzara, A.; Orenstein, J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hinton, J. P.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Alpichshev, Z.; Mahmood, F.; Gedik, N.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Chan, M. K.; Veit, M. J.; Dorow, C. J.; Barisic, N.; Greven, M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Barisic, N.] TU Wien, Inst Solid State Phys, A-1040 Vienna, Austria. [Bonn, D. A.; Hardy, W. N.; Liang, Ruixing] Univ British Columbia, Dept Phys & Astron, Vancouver, BC, Canada. [Bonn, D. A.; Hardy, W. N.; Liang, Ruixing] Canadian Inst Adv Res, Toronto, ON M5G 178, Canada. [Koralek, J. D.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Kemper, A. F.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. RP Hinton, JP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Hinton, JP (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Hinton, JP (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM jhinton@ucsd.edu RI Orenstein, Joseph/I-3451-2015; Kemper, Alexander/F-8243-2016; OI Kemper, Alexander/0000-0002-5426-5181; Chan, Mun/0000-0002-8808-9040 FU Department of Energy, Office of Basic Energy Sciences [DE-SC0006858]; FWF project [P2798]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge J. C. Davis for enlightening discussions, as well as Lina Ji for assistance with crystal growth. Synthesis and characterization of Hg-1201 samples performed at the University of Minnesota was supported by the Department of Energy, Office of Basic Energy Sciences, under Award No. DE-SC0006858. N.B. acknowledges the support of FWF project P2798. Optical measurements and modeling performed at Lawrence Berkeley National Lab was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 48 TC 3 Z9 3 U1 10 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 13 PY 2016 VL 6 AR 23610 DI 10.1038/srep23610 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ1LS UT WOS:000373964900001 PM 27071712 ER PT J AU Ondarcuhu, T Thomas, V Nunez, M Dujardin, E Rahman, A Black, CT Checco, A AF Ondarcuhu, Thierry Thomas, Vincent Nunez, Marc Dujardin, Erik Rahman, Atikur Black, Charles T. Checco, Antonio TI Wettability of partially suspended graphene SO SCIENTIFIC REPORTS LA English DT Article ID WETTING TRANSPARENCY; SUPPORTED GRAPHENE; LAYER GRAPHENE; SURFACES; CONTAMINANTS; GRAPHITE; WATER AB The dependence of the wettability of graphene on the nature of the underlying substrate remains only partially understood. Here, we systematically investigate the role of liquid-substrate interactions on the wettability of graphene by varying the area fraction of suspended graphene from 0 to 95% by means of nanotextured substrates. We find that completely suspended graphene exhibits the highest water contact angle (85 degrees +/- 5 degrees) compared to partially suspended or supported graphene, regardless of the hydrophobicity (hydrophilicity) of the substrate. Further, 80% of the long-range water-substrate interactions are screened by the graphene monolayer, the wettability of which is primarily determined by short-range graphene-liquid interactions. By its well-defined chemical and geometrical properties, supported graphene therefore provides a model system to elucidate the relative contribution of short and long range interactions to the macroscopic contact angle. C1 [Ondarcuhu, Thierry; Thomas, Vincent; Nunez, Marc; Dujardin, Erik] CNRS, CEMES, Nanosci Grp, 29 Rue Jeanne Marvig, F-31055 Toulouse, France. [Rahman, Atikur; Black, Charles T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Checco, Antonio] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Ondarcuhu, T (reprint author), CNRS, CEMES, Nanosci Grp, 29 Rue Jeanne Marvig, F-31055 Toulouse, France.; Checco, A (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM ondar@cemes.fr; checco@bnl.gov FU Laboratory of Excellence NEXT [ANR-10-LABX-0037]; government of Andorra; NEXT; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX We thank Xavier Bouju (CEMES-CNRS) and Mathias Rapacioli (LCPQ, Toulouse) for fruitful discussions. This study has been partially supported through the Laboratory of Excellence NEXT (grant no ANR-10-LABX-0037) in the framework of the "Programme des Investissements d'Avenir". M.N. acknowledges the government of Andorra for a PhD fellowship. A.C. acknowledges financial support by NEXT through a Senior Guest Fellowship. Research carried at Brookhaven National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704 and used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility. NR 39 TC 7 Z9 7 U1 32 U2 65 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 13 PY 2016 VL 6 AR 24237 DI 10.1038/srep24237 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ1LI UT WOS:000373963900001 PM 27072195 ER PT J AU Wingard, LA Johnson, EC Sabatini, JJ AF Wingard, Leah A. Johnson, Eric C. Sabatini, Jesse J. TI Efficient method for the cycloaminomethylation of glycoluril SO TETRAHEDRON LETTERS LA English DT Article DE Synthesis; Cycloaminomethylation; Glycoluril AB The efficient method for the cycloaminomethylation of glycoluril to yield 2,6-ditert-butylhexahydro-1H,5H-2,3a,4a,6,7a,8a-hexaazacyclopenta[def]fluorene-4,8-dione is described. The material is synthesized employing water as the solvent, and is isolated by filtration. This is an improvement over the previous reported synthetic method, which relied on the use of samarium trichloride catalysis, as well as silica gel column chromatographic purification to obtain the target product. Published by Elsevier Ltd. C1 [Sabatini, Jesse J.] US Army Res Lab, Energet Technol Branch, Aberdeen Proving Ground, MD 21005 USA. [Wingard, Leah A.] Oak Ridge Associated Univ, Belcamp, MD 21017 USA. [Johnson, Eric C.] TKC Global, 13873 Pk Ctr Rd, Herndon, VA 20171 USA. RP Sabatini, JJ (reprint author), US Army Res Lab, Energet Technol Branch, Aberdeen Proving Ground, MD 21005 USA. EM jesse.j.sabatini.civ@mail.mil FU Army Research Laboratory [W911NF-12-2-0019] FX Research was sponsored by the Army Research Laboratory was accomplished in part under Cooperative Agreement Number W911NF-12-2-0019. The views and conclusions contained in this document are those of the authors and should not be interpreted as representing official policies, either expressed or implied, of the Army Research Laboratory or the U.S. Government. The U.S. Government is authorized to reproduce and distribute reprints for Government purposes notwithstanding any copyright notation herein. NR 11 TC 2 Z9 2 U1 0 U2 4 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0040-4039 J9 TETRAHEDRON LETT JI Tetrahedron Lett. 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CA ATLAS Collaboration TI Measurement of the centrality dependence of the charged-particle pseudorapidity distribution in proton-lead collisions at root s(NN)=5.02 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID TRANSVERSE-MOMENTUM DEPENDENCE; HIGH-ENERGY; MULTIPARTICLE PRODUCTION; NUCLEUS COLLISIONS; ANGULAR-CORRELATIONS; JET PRODUCTION; PB COLLISIONS; LONG-RANGE; LHC; MULTIPLICITY AB The centrality dependence of the mean charged-particle multiplicity as a function of pseudorapidity is measured in approximately 1 mu b(-1) of proton-lead collisions at a nucleon-nucleon centre-of-mass energy of root s(NN) = 5.02 TeV using the ATLAS detector at the Large Hadron Collider. Charged particles with absolute pseudorapidity less than 2.7 are reconstructed using the ATLAS pixel detector. The p + Pb collision centrality is characterised by the total transverse energy measured in the Pb-going direction of the forward calorimeter. The charged-particle pseudorapidity distributions are found to vary strongly with centrality, with an increasing asymmetry between the proton-going and Pb-going directions as the collisions become more central. Three different estimations of the number of nucleons participating in the p + Pb collision have been carried out using the Glauber model as well as two Glauber-Gribov inspired extensions to the Glauber model. Charged-particle multiplicities per participant pair are found to vary differently for these three models, highlighting the importance of including colour fluctuations in nucleon-nucleon collisions in the modelling of the initial state of p + Pb collisions. C1 [Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Avolio, G.; Baak, M. A.; Backes, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Barajas, C. A. 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S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Engn Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Grafstroem, P.; Massa, I.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bindi, M.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Abajyan, T.; Arslan, O.; Backhaus, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Velz, T.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.; Marroquim, F.] Fed Univ Juiz De Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezo, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Hanb, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Aloisio, A.; Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Hoffmann, M. Dano; Galster, G.; Gregersen, K.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, POB 13, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J.; Deterre, C.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Barber, T.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Miucci, A.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mosidzeb, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Morel, J.; Llacer, M. Moreno; Nackenhorst, O.; Nadal, J.; Quadt, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. 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F.] Univ Nacl La Plata, Inst Fis Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Aloisio, A.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Catmore, J. R.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chilingarov, A.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Davison, P.; Dobson, E.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De La Torre, H.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Robinson, J. E. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Bousson, N.; Chen, L.; Clemens, J. C.; Coadou, Y.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Petersen, B. A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Andreazza, A.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst Phys, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Bassalat, A.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, J. K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Donati, S.; Dotti, A.; Giannetti, P.; Roda, C.; Scuri, F.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjosa, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marquesa, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Dos Santos, D. Roda; Ruzicka, P.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadia, M.; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Zorzi, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Camillocci, E. Solfaroli; Vanadia, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchinia, P.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouild, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouild, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Recherches Lois Fondament Univers, Gif Sur Yvette, France. [Grillo, A. A.; Kuhl, A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. 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[Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navas, L. Mendoza; Navarro, G.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. 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P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Jimenez, Y. 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[Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Shandong, Peoples R China. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Wildt, M. A.] Univ Hamburg, Inst Phys Expt, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Brooks, William/C-8636-2013; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Chekulaev, Sergey/O-1145-2015; Moraes, Arthur/F-6478-2010; Gerbaudo, Davide/J-4536-2012; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Carli, Ina/C-2189-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Villa, Mauro/C-9883-2009; Solfaroli Camillocci, Elena/J-1596-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; KHODINOV, ALEKSANDR/D-6269-2015; Conde Muino, Patricia/F-7696-2011; Olshevskiy, Alexander/I-1580-2016; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Tikhomirov, Vladimir/M-6194-2015; Guo, Jun/O-5202-2015; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009 OI Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Moraes, Arthur/0000-0002-5157-5686; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Carli, Ina/0000-0002-0411-1141; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Villa, Mauro/0000-0002-9181-8048; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Conde Muino, Patricia/0000-0002-9187-7478; Olshevskiy, Alexander/0000-0002-8902-1793; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Tikhomirov, Vladimir/0000-0002-9634-0581; Guo, Jun/0000-0001-8125-9433; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMTCR, Czech Republic; MPOCR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, UK; DOE, USA; NSF, USA; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex; Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG; AvH Foundation, Germany; Herakleitos program - EU-ESF; Thales program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, UK; Leverhulme Trust, UK FX We honour the memory of our colleague Alexey Antonov, who was closely involved in the work described here, and died shortly after its completion. We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMTCR, MPOCR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, UK; DOE and NSF, USA. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, UK. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 68 TC 8 Z9 8 U1 28 U2 64 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 12 PY 2016 VL 76 IS 4 AR 199 DI 10.1140/epjc/s10052-016-4002-3 PG 30 WC Physics, Particles & Fields SC Physics GA DL0EZ UT WOS:000375306400002 PM 28260972 ER PT J AU Aduszkiewicz, A Ali, Y Andronov, E Anticic, T Antoniou, N Baatar, B Bay, F Blondel, A Bogomilov, M Brandin, A Bravar, A Brzychczyk, J Bunyatov, SA Busygina, O Christakoglou, P Cirkovic, M Czopowicz, T Damyanova, A Davis, N Dembinski, H Deveaux, M Diakonos, F Di Luise, S Dominik, W Dumarchez, J Dynowski, K Engel, R Ereditato, A Feofilov, GA Fodor, Z Garibov, A Gazdzicki, M Golubeva, M Grebieszkow, K Grzeszczuk, A Guber, F Haesler, A Hasegawa, T Herve, AE Hierholzer, M Igolkin, S Ivashkin, A Johnson, SR Kadija, K Kapoyannis, A Kaptur, E Kisiel, J Kobayashi, T Kolesnikov, VI Kolev, D Kondratiev, VP Korzenev, A Kowalik, K Kowalski, S Koziel, M Krasnoperov, A Kuich, M Kurepin, A Larsen, D Laszlo, A Lewicki, M Lyubushkin, VV Mackowiak-Pawlowska, M Maksiak, B Malakhov, AI Manic, D Marcinek, A Marino, AD Marton, K Mathes, HJ Matulewicz, T Matveev, V Melkumov, GL Messerly, B Mills, GB Morozov, S Mrowczynski, S Nagai, Y Nakadaira, T Naskret, M Nirkko, M Nishikawa, K Panagiotou, AD Paolone, V Pavin, M Petukhov, O Pistillo, C Planeta, R Popov, BA Posiadala, M Pulawski, S Puzovic, J Rauch, W Ravonel, M Redij, A Renfordt, R Richter-Was, E Robert, A Rohrich, D Rondio, E Roth, M Rubbia, A Rumberger, BT Rustamov, A Rybczynski, M Sadovsky, A Sakashita, K Schmidt, K Sekiguchi, T Selyuzhenkov, I Seryakov, A Seyboth, P Sgalaberna, D Shibata, M Slodkowski, M Staszel, P Stefanek, G Stepaniak, J Strobele, H Susa, T Szuba, M Tada, M Taranenko, A Tefelski, D Tereshchenko, V Tsenov, R Turko, L Ulrich, R Unger, M Vassiliou, M Veberic, D Vechernin, VV Vesztergombi, G Vinogradov, L Wilczek, A Wlodarczyk, Z Wojtaszek-Szwarc, A Wyszynski, O Zambelli, L Zimmerman, ED AF Aduszkiewicz, A. Ali, Y. Andronov, E. Anticic, T. Antoniou, N. Baatar, B. Bay, F. Blondel, A. Bogomilov, M. Brandin, A. Bravar, A. Brzychczyk, J. Bunyatov, S. A. Busygina, O. Christakoglou, P. Cirkovic, M. Czopowicz, T. Damyanova, A. Davis, N. Dembinski, H. Deveaux, M. Diakonos, F. Di Luise, S. Dominik, W. Dumarchez, J. Dynowski, K. Engel, R. Ereditato, A. Feofilov, G. A. Fodor, Z. Garibov, A. Gazdzicki, M. Golubeva, M. Grebieszkow, K. Grzeszczuk, A. Guber, F. Haesler, A. Hasegawa, T. Herve, A. E. Hierholzer, M. Igolkin, S. Ivashkin, A. Johnson, S. R. Kadija, K. Kapoyannis, A. Kaptur, E. Kisiel, J. Kobayashi, T. Kolesnikov, V. I. Kolev, D. Kondratiev, V. P. Korzenev, A. Kowalik, K. Kowalski, S. Koziel, M. Krasnoperov, A. Kuich, M. Kurepin, A. Larsen, D. Laszlo, A. Lewicki, M. Lyubushkin, V. V. Mackowiak-Pawlowska, M. Maksiak, B. Malakhov, A. I. Manic, D. Marcinek, A. Marino, A. D. Marton, K. Mathes, H. -J. Matulewicz, T. Matveev, V. Melkumov, G. L. Messerly, B. Mills, G. B. Morozov, S. Mrowczynski, S. Nagai, Y. Nakadaira, T. Naskret, M. Nirkko, M. Nishikawa, K. Panagiotou, A. D. Paolone, V. Pavin, M. Petukhov, O. Pistillo, C. Planeta, R. Popov, B. A. Posiadala, M. Pulawski, S. Puzovic, J. Rauch, W. Ravonel, M. Redij, A. Renfordt, R. Richter-Was, E. Robert, A. Rohrich, D. Rondio, E. Roth, M. Rubbia, A. Rumberger, B. T. Rustamov, A. Rybczynski, M. Sadovsky, A. Sakashita, K. Schmidt, K. Sekiguchi, T. Selyuzhenkov, I. Seryakov, A. Seyboth, P. Sgalaberna, D. Shibata, M. Slodkowski, M. Staszel, P. Stefanek, G. Stepaniak, J. Stroebele, H. Susa, T. Szuba, M. Tada, M. Taranenko, A. Tefelski, D. Tereshchenko, V. Tsenov, R. Turko, L. Ulrich, R. Unger, M. Vassiliou, M. Veberic, D. Vechernin, V. V. Vesztergombi, G. Vinogradov, L. Wilczek, A. Wlodarczyk, Z. Wojtaszek-Szwarc, A. Wyszynski, O. Zambelli, L. Zimmerman, E. D. CA NA61 SHINE Collaboration TI Production of Lambda-hyperons in inelastic p plus p interactions at 158 GeV/c SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID STRANGE-PARTICLE-PRODUCTION; 300 GEV-C; COLLISIONS; GAMMA; MODEL AB Inclusive production of Lambda-hyperons was measured with the large acceptance NA61/SHINE spectrometer at the CERN SPS in inelastic p+p interactions at beam momentum of 158 GeV/c. Spectra of transverse momentum and transverse mass as well as distributions of rapidity and x(F) are presented. The mean multiplicity was estimated to be 0.120+/-0.006 (stat.) +/-0.010 (sys.). The results are compared with previous measurements and predictions of the EPOS, URQMD and FRITIOF models. C1 [Garibov, A.; Rustamov, A.] Natl Ctr Nucl Res, Baku, Azerbaijan. [Bogomilov, M.; Kolev, D.; Tsenov, R.] Univ Sofia, Fac Phys, BU-1126 Sofia, Bulgaria. [Anticic, T.; Kadija, K.; Pavin, M.; Susa, T.] Rudjer Boskovic Inst, Zagreb, Croatia. [Dumarchez, J.; Pavin, M.; Popov, B. A.; Robert, A.; Zambelli, L.] Univ Paris VI & VII, LPNHE, Paris, France. [Dembinski, H.; Engel, R.; Herve, A. E.; Mathes, H. -J.; Roth, M.; Szuba, M.; Ulrich, R.; Unger, M.; Veberic, D.] Karlsruhe Inst Technol, D-76021 Karlsruhe, Germany. [Rauch, W.] Fachhsch Frankfurt, Frankfurt, Germany. [Deveaux, M.; Koziel, M.; Renfordt, R.; Rustamov, A.; Stroebele, H.] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany. [Antoniou, N.; Christakoglou, P.; Davis, N.; Diakonos, F.; Kapoyannis, A.; Panagiotou, A. D.; Vassiliou, M.] Univ Athens, Athens, Greece. [Fodor, Z.; Laszlo, A.; Marton, K.; Vesztergombi, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Hasegawa, T.; Kobayashi, T.; Nakadaira, T.; Nishikawa, K.; Sakashita, K.; Sekiguchi, T.; Shibata, M.; Tada, M.; Zambelli, L.] Inst Particle & Nucl Studies, Tsukuba, Ibaraki, Japan. [Rohrich, D.] Univ Bergen, Bergen, Norway. [Gazdzicki, M.; Mrowczynski, S.; Rybczynski, M.; Seyboth, P.; Stefanek, G.; Wlodarczyk, Z.; Wojtaszek-Szwarc, A.] Jan Kochanowski Univ Humanities & Sci, Kielce, Poland. [Kowalik, K.; Rondio, E.; Stepaniak, J.] Natl Ctr Nucl Res, Warsaw, Poland. [Ali, Y.; Brzychczyk, J.; Larsen, D.; Marcinek, A.; Planeta, R.; Richter-Was, E.; Staszel, P.; Wyszynski, O.] Jagiellonian Univ, Krakow, Poland. [Grzeszczuk, A.; Kaptur, E.; Kisiel, J.; Kowalski, S.; Pulawski, S.; Schmidt, K.; Wilczek, A.] Silesian Univ, Katowice, Poland. [Aduszkiewicz, A.; Dominik, W.; Kuich, M.; Matulewicz, T.; Posiadala, M.] Univ Warsaw, Warsaw, Poland. [Fodor, Z.; Lewicki, M.; Marcinek, A.; Naskret, M.; Turko, L.] Univ Wroclaw, PL-50138 Wroclaw, Poland. [Czopowicz, T.; Dynowski, K.; Grebieszkow, K.; Mackowiak-Pawlowska, M.; Maksiak, B.; Slodkowski, M.; Tefelski, D.] Warsaw Univ Technol, Warsaw, Poland. [Busygina, O.; Golubeva, M.; Guber, F.; Ivashkin, A.; Kurepin, A.; Morozov, S.; Petukhov, O.; Sadovsky, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Baatar, B.; Bunyatov, S. A.; Kolesnikov, V. I.; Krasnoperov, A.; Lyubushkin, V. V.; Malakhov, A. I.; Matveev, V.; Melkumov, G. L.; Popov, B. A.; Tereshchenko, V.] Joint Inst Nucl Res, Dubna, Russia. [Brandin, A.; Morozov, S.; Petukhov, O.; Selyuzhenkov, I.; Taranenko, A.] Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Moscow, Russia. [Andronov, E.; Feofilov, G. A.; Igolkin, S.; Kondratiev, V. P.; Seryakov, A.; Vechernin, V. V.; Vinogradov, L.] St Petersburg State Univ, St Petersburg 199034, Russia. [Cirkovic, M.; Manic, D.; Puzovic, J.] Univ Belgrade, Belgrade, Serbia. [Bay, F.; Di Luise, S.; Rubbia, A.; Sgalaberna, D.] ETH, Zurich, Switzerland. [Ereditato, A.; Hierholzer, M.; Nirkko, M.; Pistillo, C.; Redij, A.] Univ Bern, Bern, Switzerland. [Blondel, A.; Bravar, A.; Damyanova, A.; Haesler, A.; Korzenev, A.; Ravonel, M.] Univ Geneva, Geneva, Switzerland. [Mills, G. B.] Los Alamos Natl Lab, Los Alamos, NM USA. [Johnson, S. R.; Marino, A. D.; Nagai, Y.; Rumberger, B. T.; Zimmerman, E. D.] Univ Colorado, Boulder, CO 80309 USA. [Messerly, B.; Paolone, V.] Univ Pittsburgh, Pittsburgh, PA USA. [Ali, Y.] COMSATS Inst Informat Technol, Dept Phys, Islamabad 44000, Pakistan. RP Susa, T (reprint author), Rudjer Boskovic Inst, Zagreb, Croatia. EM Tatjana.Susa@irb.hr RI Kurepin, Alexey/H-4852-2013; Grebieszkow, Katarzyna/F-2640-2012; Vechernin, Vladimir/J-5832-2013; Kowalski, Seweryn/F-1156-2011; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Seryakov, Andrey/D-8376-2017; Andronov, Evgeny/G-2325-2015 OI Kurepin, Alexey/0000-0002-1851-4136; Vechernin, Vladimir/0000-0003-1458-8055; Kowalski, Seweryn/0000-0001-9888-4008; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Seryakov, Andrey/0000-0002-5759-5485; Andronov, Evgeny/0000-0003-0437-9292 FU Hungarian Scientific Research Fund [OTKA 68506, 71989]; Janos Bolyai Research Scholarship of the Hungarian Academy of Sciences; Polish Ministry of Science and Higher Education [667/N-CERN/2010/0, NN202 48 4339, NN202 23 1837]; Polish National Science Centre [2011/03/N/ST2/03691, 2012/04/M/ST2/00816, 2013/11/N/ST2/03879]; Foundation for Polish Science-MPD program - European Union within the European Regional Development Fund; Federal Agency of Education of the Ministry of Education and Science of the Russian Federation [11.38.193.2014]; Russian Academy of Science; Russian Foundation for Basic Research [08-02-00018, 09-02-00664, 12-02-91503-CERN]; Ministry of Education, Culture, Sports, Science and Technology, Japan [18071005, 19034011, 19740162, 20740160, 20039012]; German Research Foundation [GA1480/2-2]; EU [PIOF-GA-2013-624803]; Bulgarian Nuclear Regulatory Agency; Joint Institute for Nuclear Research, Dubna [4418-1-15/17]; Ministry of Education and Science of the Republic of Serbia [OI171002]; Swiss Nationalfonds Foundation [200020-117913/1]; ETH Research Grant [TH-01 07-3] FX This work was supported by the Hungarian Scientific Research Fund (Grants OTKA 68506 and 71989), the Janos Bolyai Research Scholarship of the Hungarian Academy of Sciences, the Polish Ministry of Science and Higher Education (Grants 667/N-CERN/2010/0, NN202 48 4339 and NN202 23 1837), the Polish National Science Centre (Grants 2011/03/N/ST2/03691, 2012/04/M/ST2/00816 and 2013/11/N/ST2/03879), the Foundation for Polish Science-MPD program, co-financed by the European Union within the European Regional Development Fund, the Federal Agency of Education of the Ministry of Education and Science of the Russian Federation (SPbSU research Grant 11.38.193.2014), the Russian Academy of Science and the Russian Foundation for Basic Research (Grants 08-02-00018, 09-02-00664 and 12-02-91503-CERN), the Ministry of Education, Culture, Sports, Science and Technology, Japan, Grant-in-Aid for ScientificResearch (Grants 18071005, 19034011, 19740162, 20740160 and 20039012), the German Research Foundation (Grant GA1480/2-2), the EU-funded Marie Curie Outgoing Fellowship, Grant PIOF-GA-2013-624803, the Bulgarian Nuclear Regulatory Agency and the Joint Institute for Nuclear Research, Dubna (bilateral contract No. 4418-1-15/17), Ministry of Education and Science of the Republic of Serbia (Grant OI171002), Swiss Nationalfonds Foundation (Grant 200020-117913/1) and ETH Research Grant TH-01 07-3. Finally, it is a pleasure to thank the European Organisation for Nuclear Research for strong support and hospitality and, in particular, the operating crews of the CERN SPS accelerator and beam lines who made the measurements possible. NR 37 TC 1 Z9 1 U1 10 U2 16 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD APR 12 PY 2016 VL 76 IS 4 AR 198 DI 10.1140/epjc/s10052-016-4003-2 PG 18 WC Physics, Particles & Fields SC Physics GA DL0EZ UT WOS:000375306400001 ER PT J AU Hassanpour, E Wegmayr, V Schaab, J Yan, Z Bourret, E Lottermoser, T Fiebig, M Meier, D AF Hassanpour, E. Wegmayr, V. Schaab, J. Yan, Z. Bourret, E. Lottermoser, Th Fiebig, M. Meier, D. TI Robustness of magnetic and electric domains against charge carrier doping in multiferroic hexagonal ErMnO3 SO NEW JOURNAL OF PHYSICS LA English DT Article DE multiferroics; domain engineering; piezoresponse force microscopy; second harmonic generation ID 2ND-HARMONIC GENERATION; MANGANITES; WALLS; YMNO3; FERROELECTRICITY; CRYSTALS AB We investigate the effect of chemical doping on the electric and magnetic domain pattern in multiferroic hexagonal ErMnO3. Hole-and electron doping are achieved through the growth of Er1-chi Ca chi MnO3 and Er1-chi Zr chi MnO3 single crystals, which allows for a controlled introduction of divalent and tetravalent ions, respectively. Using conductance measurements, piezoresponse force microscopy and nonlinear optics we study doping-related variations in the electronic transport and image the corrsponding ferroelectric and antiferromagnetic domains. We find that moderate doping levels allow for adjusting the electronic conduction properties of ErMnO3 without destroying its characteristic domain patterns. Our findings demonstrate the feasibility of chemical doping for nonperturbative property-engineering of intrinsic domain states in this important class of multiferroics. C1 [Hassanpour, E.; Wegmayr, V.; Schaab, J.; Lottermoser, Th; Fiebig, M.; Meier, D.] ETH, Dept Mat, CH-8093 Zurich, Switzerland. [Yan, Z.; Bourret, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Devis, Berkeley, CA 94720 USA. RP Meier, D (reprint author), ETH, Dept Mat, CH-8093 Zurich, Switzerland. EM dennis.meier@mat.ethz.ch FU SNSF [200021-149192, 200021-147080]; US. Department of Energy; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX The authors thank Leo Mc Gilly, Barbara Fraygola, and Dragan Damjanovic from EFPL for experimental support. The work at the ETH Zurich was supported by the SNSF projects 200021-149192 and 200021-147080 supported in part by the US. Department of Energy and work at the Lawrence Berkeley National Laboratory was carried out under Contract No. DE-AC02-05CH11231. NR 33 TC 1 Z9 1 U1 13 U2 27 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD APR 12 PY 2016 VL 18 AR 043015 DI 10.1088/1367-2630/18/4/043015 PG 6 WC Physics, Multidisciplinary SC Physics GA DL2KW UT WOS:000375464600003 ER PT J AU Buels, R Yao, E Diesh, CM Hayes, RD Munoz-Torres, M Helt, G Goodstein, DM Elsik, CG Lewis, SE Stein, L Holmes, IH AF Buels, Robert Yao, Eric Diesh, Colin M. Hayes, Richard D. Munoz-Torres, Monica Helt, Gregg Goodstein, David M. Elsik, Christine G. Lewis, Suzanna E. Stein, Lincoln Holmes, Ian H. TI JBrowse: a dynamic web platform for genome visualization and analysis SO GENOME BIOLOGY LA English DT Article DE Genome; Browser; Bioinformatics ID DATABASE; BROWSER; INFORMATION; MODENCODE; RESOURCE; BIOLOGY AB Background: JBrowse is a fast and full-featured genome browser built with JavaScript and HTML5. It is easily embedded into websites or apps but can also be served as a standalone web page. Results: Overall improvements to speed and scalability are accompanied by specific enhancements that support complex interactive queries on large track sets. Analysis functions can readily be added using the plugin framework; most visual aspects of tracks can also be customized, along with clicks, mouseovers, menus, and popup boxes. JBrowse can also be used to browse local annotation files offline and to generate high-resolution figures for publication. Conclusions: JBrowse is a mature web application suitable for genome visualization and analysis. C1 [Buels, Robert; Yao, Eric; Holmes, Ian H.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Diesh, Colin M.; Elsik, Christine G.] Univ Missouri, Div Anim Sci, Columbia, MO USA. [Hayes, Richard D.; Munoz-Torres, Monica; Helt, Gregg; Goodstein, David M.; Lewis, Suzanna E.; Holmes, Ian H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Helt, Gregg] Genomancer Consulting, Healdsburg, CA USA. [Stein, Lincoln] Ontario Inst Canc Res, Toronto, ON, Canada. [Hayes, Richard D.; Goodstein, David M.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Stein, Lincoln] Univ Toronto, Dept Mol Genet, Toronto, ON, Canada. RP Holmes, IH (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.; Holmes, IH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM ihholmes@gmail.com RI Elsik, Christine/C-4120-2017; OI Elsik, Christine/0000-0002-4248-7713; Lewis, Suzanna/0000-0002-8343-612X; Holmes, Ian/0000-0001-7639-5369 FU NIH [HG004483, GM080203] FX RB, EY, LS, and IH were supported by NIH grant HG004483 (JBrowse). CD, MMT, GH, CE, and SL were supported by NIH grant GM080203 (WebApollo). NR 35 TC 10 Z9 10 U1 5 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1465-6906 EI 1474-760X J9 GENOME BIOL JI Genome Biol. PD APR 12 PY 2016 VL 17 AR 66 DI 10.1186/s13059-016-0924-1 PG 12 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA DJ5WI UT WOS:000374281100001 PM 27072794 ER PT J AU Fraboni, B Fraleoni-Morgera, A Zaitseva, N AF Fraboni, Beatrice Fraleoni-Morgera, Alessandro Zaitseva, Natalia TI Ionizing Radiation Detectors Based on Solution-Grown Organic Single Crystals SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID FIELD-EFFECT TRANSISTORS; THIN-FILM TRANSISTORS; PULSE-SHAPE DISCRIMINATION; ANISOTROPIC CHARGE-TRANSPORT; X-RAY-DETECTORS; MU-T-CZ; HIGH-PERFORMANCE; POLYCRYSTALLINE SCINTILLATORS; PLASTIC SCINTILLATORS; CZOCHRALSKI TECHNIQUE AB Organic single crystals (OSCs) have ideal qualities (well defined structure and morphology, lack of grain boundaries, high purity, 3D long range order, good electronic transport properties) for several technological applications, in particular as key components for electronic devices. It is only recently that OSCs have been considered as ionizing radiation detectors, and the latest developments in this field are here reported. In the first section, various methods for OSC growth are described, with emphasis on cost-effective, solution-based approaches capable of delivering large volume, well performing crystals. The second section is focused on the use of solution-grown OSCs as scintillators (i.e., as high energy photon to UV-vis photon conversion), highlighting the ability of cm-scale OSCs to effectively detect neutrons and to carry out neutrons-gamma pulse-shape discrimination tasks. Finally, the third section describes the use of semiconducting, solution-grown OSCs as effective solid state direct detectors (i.e., directly converting high energy photons into charge carriers), evidencing extremely promising performances in terms of operability in environmental conditions (i.e., no need for encapsulation), radiation hardness, linear response and low operating voltage. C1 [Fraboni, Beatrice] Univ Bologna, Dept Phys & Astron, Viale Berti Pichat 6-2, I-40127 Bologna, Italy. [Fraleoni-Morgera, Alessandro] Univ Trieste, Dept Engn & Architecture, Via Alfonso Valerio 10, I-34127 Trieste, Italy. [Fraleoni-Morgera, Alessandro] Elettra Sincrotrone Trieste SCpA SS 14, Km 163-5, I-341499 Basovizza, TS, Italy. [Zaitseva, Natalia] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Fraboni, B (reprint author), Univ Bologna, Dept Phys & Astron, Viale Berti Pichat 6-2, I-40127 Bologna, Italy. EM beatrice.fraboni@unibo.it FU European Community [611070] FX B.F and A.F-M acknowledge the financial support from the European Community under the FP7-ICT Project "i-FLEXIS" (2013-2016), Grant Agreement No. 611070. NR 104 TC 1 Z9 1 U1 12 U2 25 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD APR 12 PY 2016 VL 26 IS 14 SI SI BP 2276 EP 2291 DI 10.1002/adfm.201502669 PG 16 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ5OI UT WOS:000374258100004 ER PT J AU Matsumura, H Chakraborty, S Reed, J Lu, Y Moenne-Loccoz, P AF Matsumura, Hirotoshi Chakraborty, Saumen Reed, Julian Lu, Yi Moenne-Loccoz, Pierre TI Effect of Outer-Sphere Side Chain Substitutions on the Fate of the trans Iron-Nitrosyl Dimer in Heme/Nonheme Engineered Myoglobins (Fe(B)Mbs): Insights into the Mechanism of Denitrifying NO Reductases SO BIOCHEMISTRY LA English DT Article ID NITRIC-OXIDE REDUCTASE; SPECTROSCOPIC CHARACTERIZATION; PARACOCCUS-DENITRIFICANS; GUANYLATE-CYCLASE; CRYSTAL-STRUCTURE; LIGAND-BINDING; N2O GENERATION; DIIRON CENTER; HEME; KINETICS AB Denitrifying NO reductases are transmembrane protein complexes that utilize a heme/nonheme diiron center at their active sites to reduce two NO molecules to the innocuous gas N2O. Fe(B)Mb proteins, with their nonheme iron sites engineered into the heme distal pocket of sperm whale myoglobin, are attractive models for studying the molecular details of the NO reduction reaction. Spectroscopic and structural studies of Fe(B)Mb constructs have confirmed that they reproduce the metal coordination spheres observed at the active site of the cytochrome c-dependent NO reductase from Pseudomonas aeruginosa. Exposure of Fe(B)Mb to excess NO, as examined by analytical and spectroscopic techniques, results primarily in the formation of a five-coordinate heme-nitrosyl complex without N2O production. However, substitution of the outer-sphere residue Ile107 with a glutamic acid (i.e., I107E) decreases the formation rate of the five-coordinate heme nitrosyl complex and allows for the substoichiometric production of N2O. Here, we aim to better characterize the formation of the five coordinate heme-nitrosyl complex and to explain why the level of N2O production increases with the I107E substitution. We follow the formation of the five-coordinate heme nitrosyl inhibitory complex through the sequential exposure of Fe(B)Mb to different NO isotopomers using rapid-freeze-quench resonance Raman spectroscopy. The data show that the complex is formed by the displacement of the proximal histidine by a new NO molecule after the weakening of the Fe(II) His bond in the intermediate six-coordinate low-spin (6cLS) heme-nitrosyl complex. These results lead us to explore diatomic migration within the scaffold of myoglobin and whether substitutions at residue 107 can be sufficient to control access to the proximal heme cavities. Results on a new Fe(B)Mb construct with an 1107F substitution (Fe(B)Mb3) show an increased rate for the formation of the five-coordinate low-spin heme nitrosyl complex without N2O production. Taken together, our results suggest that production of N2O from the [6cLS heme {FeNO}(7)/{FeBNO}(7)] trans iron-nitrosyl dimer intermediate requires a proton transfer event facilitated by an outer-sphere residue such as E107 in Fe(B)Mb2 and E280 in P. aeruginosa cNOR. C1 [Matsumura, Hirotoshi; Moenne-Loccoz, Pierre] Oregon Hlth & Sci Univ, Inst Environm Hlth, Div Environm & Biomol Syst, Portland, OR 97239 USA. [Chakraborty, Saumen; Lu, Yi] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Reed, Julian; Lu, Yi] Univ Illinois, Dept Biochem, Urbana, IL 61801 USA. [Matsumura, Hirotoshi] Akita Univ, Fac & Grad Sch Engn & Resource Sci, Dept Life Sci, 1-1 Tegata Gakuen Machi, Akita, Akita 0108502, Japan. [Chakraborty, Saumen] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. RP Moenne-Loccoz, P (reprint author), Oregon Hlth & Sci Univ, Inst Environm Hlth, 3181 SW Sam Jackson Pk Rd, Portland, OR 97239 USA. EM moennelo@ohsu.edu RI Lu, Yi/B-5461-2010 OI Lu, Yi/0000-0003-1221-6709 FU National Institutes of Health [GM74785, GM06221] FX This work was supported by Grants GM74785 (P.M.-L.) and GM06221 (Y.L.) from the National Institutes of Health. NR 41 TC 2 Z9 2 U1 4 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD APR 12 PY 2016 VL 55 IS 14 BP 2091 EP 2099 DI 10.1021/acs.biochem.5b01109 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DJ4SB UT WOS:000374197100004 PM 27003474 ER PT J AU McCarthy, RF Weimer, MS Haasch, RT Schaller, RD Hock, AS Martinson, ABF AF McCarthy, Robert F. Weimer, Matthew S. Haasch, Richard T. Schaller, Richard D. Hock, Adam S. Martinson, Alex B. F. TI VxIn(2-x)S3 Intermediate Band Absorbers Deposited by Atomic Layer Deposition SO CHEMISTRY OF MATERIALS LA English DT Article ID V-SUBSTITUTED IN2S3; VO2 THIN-FILMS; SOLAR-CELLS; ELECTROLUMINESCENCE; EFFICIENCY; CHEMISTRY; SULFIDE; TEMAV AB Substitutional alloys of several thin film semiconductors have been proposed as intermediate band (IB) materials for use in next-generation photovoltaics, which aim to utilize a larger fraction of the solar spectrum without sacrificing significant photovoltage. We demonstrate a novel approach to IB material growth, namely atomic layer deposition (ALD), to allow unique control over substitutional-dopant location and density. Two new ALD processes for vanadium sulfide incorporation are introduced, one of which incorporates a vanadium(III) amidinate previously untested for ALD. Using this process, we synthesize the first thin film VxIn(2-x)S3 intermediate band semiconductors and further demonstrate that the V:In ratio, and therefore intraband gap density of states, can be finely tuned according to the ALD dosing schedule. Deposition on a crystalline In2S3 underlayer promotes the growth of a tetragonal beta-In2S3-like phase VxIn(2-x)S3, which exhibits a distinct sub-band gap absorption peak with onset near 1.1 eV in agreement with computational predictions. However, the VxIn(2-x)S3 films lack the lower-energy transition predicted for a partially filled IB, and photoelectrochemical devices reveal a photocurrent response only from illumination with energy sufficient to span the parent band gap. C1 [McCarthy, Robert F.; Weimer, Matthew S.; Martinson, Alex B. F.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Schaller, Richard D.] Argonne Natl Lab, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hock, Adam S.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Weimer, Matthew S.; Hock, Adam S.] IIT, Dept Biol & Chem Sci, 3101 South Dearborn St, Chicago, IL 60616 USA. RP Martinson, ABF (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM martinson@anl.gov RI Hock, Adam/D-7660-2012 OI Hock, Adam/0000-0003-1440-1473 FU U.S. Department of Energy [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ARCS foundation; Department of Energy; Illinois Institute of Technology FX Work at Argonne National Laboratory was supported under U.S. Department of Energy Contract DE-AC02-06CH11357. Use of the Center for Nanoscale Materials, an Office of Science user facility, including resources in the Electron Microscopy Center, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. M.S.W. acknowledges support from the ARCS foundation. A.S.H. thanks the Department of Energy and the Illinois Institute of Technology for funding and start-up support. NR 29 TC 3 Z9 3 U1 5 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2033 EP 2040 DI 10.1021/acs.chemmater.5b04402 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000012 ER PT J AU Shin, Y Ding, H Persson, KA AF Shin, Yongwoo Ding, Hong Persson, Kristin A. TI Revealing the Intrinsic Li Mobility in the Li2MnO3 Lithium-Excess Material SO CHEMISTRY OF MATERIALS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; ION BATTERIES; CATHODE MATERIALS; 1ST-PRINCIPLES CALCULATIONS; ELECTROCHEMICAL ACTIVITY; DIFFUSION MECHANISMS; POSITIVE ELECTRODE; OXIDE ELECTRODES AB One of the most promising avenues for future high energy Li-ion batteries originate from the family of Li-rich layered cathodes. However, while exhibiting excellent initial capacity, these materials also suffer from voltage fade, high impedance, and poor rate capability, particularly in the Mn-rich, high Li excess concentration regime. Though it is clear that the Li2MnO3 component contributes to the high capacity as well as the chemical and structural degradation of the material, the inherent ionic conductivity of the material has not been clarified. In this work, we investigate the delithiation mechanism, involving coherent Li migration from two layers by first-principles density functional theory. Surprisingly, and contrary to expectations from available experimental results, we find that the pristine material exhibits excellent Li mobility enabling facile Li extraction from both the transition metal layer and Li-layer. Generally, the Li-extractions are highly accelerated by di- and trivacancy clusters, which. stabilize the saddle point tetrahedral sites. Hence, we deduce that the observed inferior rate behavior of this class of Li cathode materials is not due to intrinsic poor bulk ionic mobility, but more likely due to surface-passivation, structural deterioration, and/or particle-particle electrode-level transport limitations. C1 [Shin, Yongwoo; Ding, Hong; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Persson, Kristin A.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94704 USA. RP Persson, KA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.; Persson, KA (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94704 USA. EM kapersson@lbl.gov RI Shin, Yongwoo/G-5838-2011 OI Shin, Yongwoo/0000-0001-7760-9883 FU Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; Center for the Next Generation of Materials by Design an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC36-08GO28308] FX This work intellectually led by the Battery Materials Research (BMR) program, under the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy, Contract No. DE-AC02-05CH11231. Dr. Ding was supported as part of the Center for the Next Generation of Materials by Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Contract No. DE-AC36-08GO28308 to NREL. Finally, this research used resources of the National Energy Research Scientific Computing Center (NERSC). NR 59 TC 3 Z9 3 U1 24 U2 87 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2081 EP 2088 DI 10.1021/acs.chemmater.5b04862 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000018 ER PT J AU Li, GD Bajaj, S Aydemir, U Hao, SQ Xiao, H Goddard, WA Zhai, PC Zhang, QJ Snyder, GJ AF Li, Guodong Bajaj, Saurabh Aydemir, Umut Hao, Shiqiang Xiao, Hai Goddard, William A., III Zhai, Pengcheng Zhang, Qingjie Snyder, G. Jeffrey TI p-Type Co Interstitial Defects in Thermoelectric Skutterudite CoSb3 Due to the Breakage of Sb-4-Rings SO CHEMISTRY OF MATERIALS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AB-INITIO CALCULATIONS; WAVE BASIS-SET; TRANSPORT-PROPERTIES; ELECTRONIC-STRUCTURE; MICROSTRUCTURE; COMPOUND; ALUMINUM; COPPER; RHSB3 AB Skutterudite CoSb3 based thermoelectric devices have high potential for engineering applications because both nand p-type doped CoSb3 demonstrate excellent thermoelectric performance. A crucial point concerning the application of CoSb3 is to understand and control its defect chemistry. To reveal the native conductivity behavior of nonstoichiometric CoSb3, we investigated the intrinsic point defects in CoSb3 using density functional theory. We found CoSb3 is p-type in either Co or Sb rich regions of phase stability. Interstitial Co (Co-i) and interstitial Co-pair (Coi-p) are the dominant point defects in the Co rich region. However, Coi-p will be difficult to form because the formation temperature of Coi-p is much lower than the synthesis temperature of CoSb3. The unexpected acceptor nature of the Co-i or Coi-p defects is explained by the breakage of multiple Sb-4-rings. Co vacancy (Co-y) is found to be the p-type defect in the Sb rich region. Furthermore, the solubility of excess Co in CoSb3 is expected to be larger than that of Sb because of the lower formation energy and higher carrier concentration of Co-i compared with those of Co-v. C1 [Li, Guodong; Zhai, Pengcheng; Zhang, Qingjie] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China. [Li, Guodong; Aydemir, Umut; Hao, Shiqiang; Snyder, G. Jeffrey] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Bajaj, Saurabh] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy & Technol Div, Berkeley, CA 94720 USA. [Xiao, Hai; Goddard, William A., III] CALTECH, Mat & Proc Simulat Ctr, Pasadena, CA 91125 USA. RP Zhang, QJ (reprint author), Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China.; Snyder, GJ (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA.; Goddard, WA (reprint author), CALTECH, Mat & Proc Simulat Ctr, Pasadena, CA 91125 USA. EM wag@wag.caltech.edu; zhangqj@whut.edu.cn; jeff.snyder@northwestern.edu RI Snyder, G. Jeffrey/E-4453-2011; Xiao, Hai/G-7375-2011 OI Snyder, G. Jeffrey/0000-0003-1414-8682; Xiao, Hai/0000-0001-9399-1584 FU National Basic Research Program of China (973-program) [2013CB632505]; 111 Project of China [B07040]; Department of Energy Basic Energy Sciences Program [EDCBEE]; DOE [DE-AC02-05CH11231]; China Postdoctoral Science Foundation [408-32200031]; Scientific and Technological Research Council of Turkey; National Science Foundation [DMR-1436985] FX This work is partially supported by National Basic Research Program of China (973-program) under Project No. 2013CB632505, the 111 Project of China under Project No. B07040, Materials Project by Department of Energy Basic Energy Sciences Program under Grant No. EDCBEE, DOE Contract DE-AC02-05CH11231, and China Postdoctoral Science Foundation (408-32200031). U.A. acknowledges the financial assistance of The Scientific and Technological Research Council of Turkey. H.X. and W.A.G. were supported by the National Science Foundation (DMR-1436985, program manager, John Schlueter). NR 52 TC 2 Z9 2 U1 20 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2172 EP 2179 DI 10.1021/acs.chemmater.6b00112 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000028 ER PT J AU Huang, JP Marschilok, AC Takeuchi, ES Takeuchi, KJ AF Huang, Jianping Marschilok, Amy C. Takeuchi, Esther S. Takeuchi, Kenneth J. TI Microwave-Assisted Synthesis of Silver Vanadium Phosphorus Oxide, Ag2VO2PO4: Crystallite Size Control and Impact on Electrochemistry SO CHEMISTRY OF MATERIALS LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; SOLID-STATE SYNTHESIS; X-RAY-DIFFRACTION; CATHODE MATERIAL; SOLVOTHERMAL SYNTHESIS; RAMAN-SPECTROSCOPY; ION BATTERIES; THIN-FILMS; PERFORMANCE; ELECTRODE AB Silver vanadium phosphorus oxide, Ag2VO2PO4, is a promising cathode material for Li batteries due in part to its large capacity and high current capability. Herein, a new synthesis of Ag2VO2PO4 based on microwave heating is presented, where the reaction time is reduced by approximately 100X relative to other reported methods, and the crystallite size is controlled via synthesis temperature, showing a linear correlation of crystallite size with temperature. Notably, under galvanostatic reduction, the Ag2VO2PO4 sample with the smallest crystallite size delivers the highest capacity and shows the highest loaded voltage. Further, pulse discharge tests show a significant resistance decrease during the initial discharge coincident with the formation of Ag metal. Thus, the magnitude of the resistance decrease observed during pulse tests depends on the Ag2VO2PO4 crystallite size, with the largest resistance decrease observed for the smallest crystallite size. Additional electrochemical measurements indicate a quasi-reversible redox reaction involving Li+ insertion/deinsertion, with capacity fade due to structural changes associated with the discharge/charge process. In summary, this work demonstrates a faster synthetic approach for bimetallic polyanionic materials which also provides the opportunity for tuning of electrochemical properties through control of material physical properties such as crystallite size. C1 [Huang, Jianping; Marschilok, Amy C.; Takeuchi, Esther S.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Marschilok, Amy C.; Takeuchi, Esther S.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Takeuchi, Esther S.] Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. RP Marschilok, AC; Takeuchi, ES; Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Marschilok, AC; Takeuchi, ES; Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA.; Takeuchi, ES (reprint author), Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. EM amy.marschilok@stonybrook.edu; esther.takeuchi@stonybrook.edu; kenneth.takeuchi.1@stonybrook.edu RI Huang, Jianping/C-9379-2014 OI Huang, Jianping/0000-0002-8391-1381 FU Center for Mesoscale Transport Properties an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012673] FX This work was supported as part of the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under award #DE-SC0012673. Brookhaven National Laboratory is acknowledged for the SmartLab X-ray Diffractometer. The authors acknowledge Alexander Brady for helpful advice regarding Rietveld refinement and Qing Zhang for assistance with SEM. NR 63 TC 4 Z9 4 U1 6 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2191 EP 2199 DI 10.1021/acs.chemmater.6b00124 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000030 ER PT J AU Wen, BH Liu, J Chernova, NA Wang, XY Janssen, Y Omenya, F Khalifah, PG Whittingham, MS AF Wen, Bohua Liu, Jue Chernova, Natasha A. Wang, Xiaoya Janssen, Yuri Omenya, Fredrick Khalifah, Peter G. Whittingham, M. Stanley TI Li3Mo4P5O24: A Two-Electron Cathode for Lithium-Ion Batteries with Three-Dimensional Diffusion Pathways SO CHEMISTRY OF MATERIALS LA English DT Article ID MO(V) MONOPHOSPHATE; TUNNEL STRUCTURE; INSERTION AB The structure of the novel compound Li3Mo4P5O24 has been solved from single crystal X-ray diffraction data. The Mo cations in Li3Mo4P5O24 are present in four distinct types of MoO6 octahedra, each of which has one open vertex at the corner participating in a Mo=O double bond and whose other five corners are shared with PO4 tetrahedra. On the basis of a bond valence sum difference map (BVS-DM) analysis, this framework is predicted to support the facile diffusion of Li+ ions, a hypothesis that is confirmed by electrochemical testing data, which show that Li3Mo4P5O24 can be utilized as a rechargeable battery cathode material. It is found that Li can both be removed from and inserted into Li3Mo4P5O24. The involvement of multiple redox processes occurring at the same Mo site is reflected in electrochemical plateaus around 3.8 V associated with the Mo6+/Mo5+ redox couple and 2.2 V associated with the Mo5+/Mo4+ redox couple. The two-electron redox properties of Mo cations in this structure lead to a theoretical capacity of 198 mAh/g. When cycled between 2.0 and 4.3 V versus Li+/Li, an initial capacity of 113 mAh/g is observed with 80% of this capacity retained over the first 20 cycles. This compound therefore represents a rare example of a solid state cathode able to support two-electron redox capacity and provides important general insights about pathways for designing next-generation cathodes with enhanced specific capacities. C1 [Wen, Bohua; Chernova, Natasha A.; Wang, Xiaoya; Omenya, Fredrick; Whittingham, M. Stanley] SUNY Binghamton, Chem & Mat Sci & Engn, Binghamton, NY 13902 USA. [Liu, Jue; Janssen, Yuri; Khalifah, Peter G.] SUNY Binghamton, Chem & Mat Sci & Engn, Binghamton, NY 13902 USA. [Liu, Jue; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM stanwhit@gmail.com RI LIU, JUE/I-8631-2016; Wang, Xiaoya/F-9394-2015 OI LIU, JUE/0000-0002-4453-910X; FU NorthEast Center for Chemical Energy Storage (NECCES) an Energy Frontier Research Center - U.S. Department of Energy Office of Science, Basic Energy Sciences [DE-SC0012583]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported as part of the NorthEast Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center funded by the U.S. Department of Energy Office of Science, Basic Energy Sciences under Award No. DE-SC0012583. Also acknowledged is NSF CRIF for SXRD support. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 26 TC 3 Z9 3 U1 12 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2229 EP 2235 DI 10.1021/acs.chemmater.6b00177 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000034 ER PT J AU Silbernagel, R Shehee, TC Martin, CH Hobbs, DT Clearfield, A AF Silbernagel, Rita Shehee, Thomas C. Martin, Caroline H. Hobbs, David T. Clearfield, Abraham TI Zr/Sn(IV) Phosphonates as Radiolytically Stable Ion-Exchange Materials SO CHEMISTRY OF MATERIALS LA English DT Article ID ZIRCONIUM PHOSPHONATES; PHOSPHATES; AMERICIUM; SEPARATION AB Zirconium and tin phosphonates were synthesized to determine ion-exchange preference and radiolytic stability. The Sn and Zr phosphonate materials were found to have preference for highly charged ions (3+) over lower charged ions (1+, 2+). The materials were exposed to 3.18 x 10(6) Gray from a Co-60 gamma source and were shown to retain their structure and performance. Ion-exchange of radioactive Am-241 with varying pH was also explored. In this paper, we describe these unusual ion-exchangers that are simple to prepare, reproducible, and do not require phosphate addition. C1 [Silbernagel, Rita; Martin, Caroline H.; Clearfield, Abraham] Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA. [Shehee, Thomas C.; Hobbs, David T.] Savannah River Nucl Solut LLC, Savannah River Natl Lab, Aiken, SC 29808 USA. RP Clearfield, A (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77843 USA. EM Clearfield@chem.tamu.edu FU U.S. Department of Energy NEUP [DE-NE0000746]; DOE Office of Nuclear Energy, Fuel Cycle Research and Development Program through the Savannah River National Laboratory [AC-70059-0] FX We thank our funding sources for support of this work: U.S. Department of Energy NEUP #DE-NE0000746, DOE Office of Nuclear Energy, Fuel Cycle Research and Development Program via Grant AC-70059-0 through the Savannah River National Laboratory. Texas A&M Research Foundation for Rare Earth Investigations and Ion-Exchange, and the Robert A. Welch Foundation #A-0673. NR 21 TC 4 Z9 4 U1 7 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2254 EP 2259 DI 10.1021/acs.chemmater.6b00199 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000037 ER PT J AU Barkholtz, HM Gallagher, JR Li, T Liu, YZ Winans, RE Miller, JT Liu, DJ Xu, T AF Barkholtz, Heather M. Gallagher, James R. Li, Tao Liu, Yuzi Winans, Randall E. Miller, Jeffrey T. Liu, Di-Jia Xu, Tao TI Lithium Assisted "Dissolution-Alloying" Synthesis of Nanoalloys from Individual Bulk Metals SO CHEMISTRY OF MATERIALS LA English DT Article ID METHANOL FUEL-CELLS; PLASMON RESONANCES; REDUCTION REACTION; IONIC LIQUIDS; NANOPARTICLES; CATALYSTS; PLATINUM; ELECTROCATALYSTS; CLUSTERS; STABILIZATION AB We report new fundamental chemistry involved in the synthesis of bimetallic nanoalloys via dissolving the pure bulk transition metals in molten lithium. It is revealed at the atomic level that when two pure bulk transition metals such as Pd and Pt are placed in molten lithium (similar to 200 degrees C), they undergo a dissolution process in which the metal-metal bonds in pure bulk transition metals are completely ruptured, which results in the existence of individual Pd and Pt atoms surrounded by lithium atoms, as is evident by synchrotron X-ray adsorption techniques. Then, upon the conversion of metal lithium to LiOH in humid air, the Pd and Pt atoms undergo an alloying process to aggregate into nanoalloys. This method was further expanded to include PdZn, which is notoriously difficult to prepare via traditional nanoalloy synthesis methods due to the easily oxidizable Zn component. The constantly reducing environment of metallic Li allowed for preparation of PdZn nanoalloys with minimal Zn oxidation via dissolution-alloying of individual bulk transition metals in molten lithium. Additionally, this lithium assisted "dissolution-alloying" method bypasses many complications intrinsic to conventional ion reduction-based nanoalloy synthesis including the necessity of ligated metal ions, the use of proper reducing agents and dispersing surfactants, and the presence of segregated phases due to different reduction potentials of the constituent metal ions. C1 [Barkholtz, Heather M.; Xu, Tao] No Illinois Univ, Dept Chem & Biochem, De Kalb, IL 60115 USA. [Barkholtz, Heather M.; Gallagher, James R.; Miller, Jeffrey T.; Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Li, Tao; Winans, Randall E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Liu, Yuzi] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Miller, Jeffrey T.] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. RP Xu, T (reprint author), No Illinois Univ, Dept Chem & Biochem, De Kalb, IL 60115 USA.; Li, T (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM taoli@aps.anl.gov; txu@niu.edu RI Liu, Yuzi/C-6849-2011; BM, MRCAT/G-7576-2011 FU National Science Foundation [CBET-1150617]; Institute for Atom-efficient Chemical Transformations (IACT) an Energy Frontier Research Center - U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX T.X. acknowledges the support from National Science Foundation (CBET-1150617). X-ray absorption spectroscopy studies by J.T.M., J.RG., T.L. and R.E.W. were supported by the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. Use of the Advanced Photon Source (APS) and Center for Nanoscale Materials (CNM) is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. We also acknowledge the technique support and insightful discussion from Dr. Dale L. Brewe at APS. NR 61 TC 0 Z9 0 U1 6 U2 17 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2267 EP 2277 DI 10.1021/acs.chemmater.6b00216 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000039 ER PT J AU Haynes, AS Banerjee, A Saouma, FO Otieno, CO Jang, JI Kanatzidis, MG AF Haynes, Alyssa S. Banerjee, Abhishek Saouma, Felix O. Otieno, Calford O. Jang, Joon I. Kanatzidis, Mercouri G. TI Phase Transition, Conformational Exchange, and Nonlinear Optical Third Harmonic Generation of ACsP(2)Se(8) (A = K, Rb, Cs) SO CHEMISTRY OF MATERIALS LA English DT Article ID STRONG 2ND-HARMONIC GENERATION; SOLID-STATE; 3RD-HARMONIC GENERATION; RICH SELENOPHOSPHATE; CHALCOGENIDE GLASSES; PHOSPHORUS; SALT; NMR; FERROELECTRICITY; CHEMISTRY AB The soluble molecular selenophosphate salts ACsP(2)Se(8) (A = K, Rb, Cs) crystallize in the orthorhombic space group Ccce with a = 14.982(3) A, b = 24.579(5) A, and c = 13.065(3) A for the Cs salt and a = 14.782(3) A, b = 23.954(5) A, and c = 13.044(3) A for the K analogue. ACsP2Se8 is composed of the molecular 6-membered ring, [P2Se8](2-), in the twist conformation charge balanced by alkali metals. The band gaps of these compounds are 2.44 +/- 0.2 eV for Cs2P2Se8, 2.41 +/- 0.2 eV for RbCsP2Se8, and 2.36 +/- 0.2 eV for KCsP2Se8. The amorphous versions of these materials can be made by water quenching the melt and have band gaps for all ACsP(2)Se(8) of 2.12 +/- 0.2 eV. Raman spectroscopic studies exhibit active modes of PSe4 and Se Se in the compound. Solution P-31 NMR studies shed light into the interesting conformational fluxionality of the [P2Se8](2-) anion, including a conformation that has not been previously observed. Thermal analysis reveals ACsP(2)Se(8) exhibits a phase transition, which we investigate by in situ synchrotron powder X-ray diffraction. Third harmonic generation (THG) nonlinear optical measurements determined the THG coefficient, chi(3), for amorphous and crystalline Cs2P2Se8 of 1.8 +/- 0.2 X 105 pm(2)/V-2 and 2.4 +/- 0.1 X 105 pm2/V2, respectively. C1 [Haynes, Alyssa S.; Banerjee, Abhishek; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Saouma, Felix O.; Otieno, Calford O.; Jang, Joon I.] SUNY Binghamton, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.; Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. EM m-kanatzidis@northwestern.edu FU National Science Foundation [DMR-1410169, DMR-1121262]; U.S. DOE [DE-AC02-06CH11357]; MRSEC program at the Materials Research Center; International Institute for Nanotechnology (IIN); State of Illinois through the IIN; Graduate Research Fellowship by the National Science Foundation [DGE-1324585] FX `This work was supported by the National Science Foundation Grant DMR-1410169. Part of this work utilized the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. SEM experiments were conducted in the EPIC facility (NUANCE Center Northwestern University), supported by the MRSEC program at the Materials Research Center with the National Science Foundation Grant DMR-1121262, the International Institute for Nanotechnology (IIN), and the State of Illinois through the IIN. Raman, NMR, and MS measurements were performed in the IMSERC facility at Northwestern University and supported through the university. We thank Gooch and Housego for supplying the AgGaSe2 crystal. A.S.H. gratefully acknowledges support through a Graduate Research Fellowship by the National Science Foundation under Grant No. DGE-1324585. A.S.H. also appreciates the mentorship from Drs. Greg Halder and Daniel Shoemaker related to the synchrotron in situ PXRD measurements, Drs. Yongbo Zhang and Yuyang Wu for solution and solid-state NMR experiments, and Saman Shafaie for mass spectroscopy studies. NR 58 TC 1 Z9 1 U1 0 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2374 EP 2383 DI 10.1021/acs.chemmater.6600551 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000052 ER PT J AU Rettenwander, D Redhammer, G Preishuber-Pflugl, F Cheng, L Miara, L Wagner, R Welzl, A Suard, E Doeff, MM Wilkening, M Fleig, J Amthauer, G AF Rettenwander, Daniel Redhammer, Guenther Preishuber-Pfluegl, Florian Cheng, Lei Miara, Lincoln Wagner, Reinhard Welzl, Andreas Suard, Emmanuelle Doeff, Marca M. Wilkening, Martin Fleig, Juergen Amthauer, Georg TI Structural and Electrochemical Consequences of Al and Ga Cosubstitution in Li7La3Zr2O12 Solid Electrolytes SO CHEMISTRY OF MATERIALS LA English DT Article ID GARNET-TYPE LI7LA3ZR2O12; SUBSTITUTED LI7LA3ZR2O12; DOPED LI7LA3ZR2O12; CUBIC LI7LA3ZR2O12; GRAIN-BOUNDARY; ION CONDUCTORS; LITHIUM METAL; CONDUCTIVITY; MICROSTRUCTURE; STABILIZATION AB Several "Beyond Li-Ion Battery" concepts such as all solid-state batteries and hybrid liquid/solid systems envision the use of a solid electrolyte to protect Li-metal anodes. These configurations are very attractive due to the possibility of exceptionally high energy densities and high (dis)charge rates, but they are far from being realized practically due to a number of issues including high interfacial resistance and difficulties associated with fabrication. One of the most promising solid electrolyte systems for these applications is Al or Ga stabilized Li7La3Zr2O12 (LLZO) based on high ionic conductivities and apparent stability against reduction by Li metal. Nevertheless, the fabrication of dense LLZO membranes with high ionic conductivity and low interfacial resistances remains challenging; it definitely requires a better understanding of the structural and electrochemical properties. In this study, the phase transition from garnet (Ia (3) over bard, No. 230) to "non-garnet" (I (4) over bar 3d, No. 220) space group as a function of composition and the different sintering behavior of Ga and Al stabilized LLZO are identified as important factors in determining the electrochemical properties. The phase transition was located at an Al:Ga substitution ratio of 0.05:0.15 and is accompanied by a significant lowering of the activation energy for Li-ion transport to 0.26 eV. The phase transition combined with microstructural changes concomitant with an increase of the Ga/Al ratio continuously improves the Li-ion conductivity from 2.6 x 10(-4) S cm(-1) to 1.2 x 10(-3) S cm(-1), which is close to the calculated maximum for garnet -type materials. The increase in Ga content is also associated with better densification and smaller grains and is accompanied by a change in the area specific resistance (ASR) from 78 to 24 SZ cm(2), the lowest reported value for LLZO so far. These results illustrate that understanding the structure properties relationships in this class of materials allows practical obstacles to its utilization to be readily overcome. C1 [Rettenwander, Daniel; Redhammer, Guenther; Wagner, Reinhard; Amthauer, Georg] Salzburg Univ, Dept Chem & Phys Mat, A-5020 Salzburg, Austria. [Preishuber-Pfluegl, Florian; Wilkening, Martin] Graz Univ Technol NAWI Graz, DFG Res Unit Molife 1277, Christian Doppler Lab Lithium Batteries, Inst Chem & Technol Mat, A-8010 Graz, Austria. [Cheng, Lei; Doeff, Marca M.] Univ Calif Berkeley, Energy Storage & Distributed Resources Div, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Cheng, Lei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Miara, Lincoln] Samsung Adv Inst Technol, 255 Main St, Cambridge, MA 02140 USA. [Welzl, Andreas; Fleig, Juergen] Vienna Univ Technol, Inst Chem Technol & Analyt, A-1060 Vienna, Austria. [Suard, Emmanuelle] Inst Laue Langevin, Diffract Grp, 71 Ave Martyrs, F-38000 Grenoble, France. RP Rettenwander, D (reprint author), Salzburg Univ, Dept Chem & Phys Mat, A-5020 Salzburg, Austria. EM daniel.rettenwander@sbg.ac.at RI Redhammer, Guenther/J-9069-2012; Wilkening, Martin/E-6480-2010; OI Redhammer, Guenther/0000-0003-0996-3930; Wilkening, Martin/0000-0001-9706-4892; Amthauer, Georg/0000-0003-3646-0394 FU Austrian Science Fund (FWF) [P25702]; Austrian Research Promotion Agency (FFG) SoLiK project; Austrian Federal Ministry of Science, Research and Economy; National Foundation for Research, Technology and Development FX The research was supported by the Austrian Science Fund (FWF) project number P25702 and the Austrian Research Promotion Agency (FFG) SoLiK project. F.P.-P. and M.W. thank the Austrian Federal Ministry of Science, Research and Economy, and the National Foundation for Research, Technology and Development for financial support. We are grateful to ILL for making all facilities available. NR 42 TC 10 Z9 10 U1 61 U2 152 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2384 EP 2392 DI 10.1021/acs.chemmater.6b00579 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000053 ER PT J AU Xu, BB Luo, ZP Gao, WX Wilson, AJ He, C Chen, X Yuan, GL Dai, HL Rao, Y Willets, K Dauter, Z Ren, SQ AF Xu, Beibei Luo, Zhipu Gao, Wenxiu Wilson, Andrew J. He, Chao Chen, Xing Yuan, Guoliang Dai, Hai-Lung Rao, Yi Willets, Katherine Dauter, Zbigniew Ren, Shenqiang TI Solution-Processed Molecular Opto-Ferroic Crystals SO CHEMISTRY OF MATERIALS LA English DT Article ID ORGANIC SEMICONDUCTING MATERIALS; CHARGE-TRANSFER INTERFACES; FIELD-EFFECT TRANSISTORS; TRANSFER COMPLEXES; MOTT INSULATOR; TRANSFER SALT; C-60; MULTIFERROICS; MAGNETISM; FERROELECTRICITY AB Supramolecular assembly utilizing noncovalent interaction to construct ordered molecular charge-transfer solids has led to significant advancement and breakthrough in energy-efficient molecular electronics, memories and solar cells. However, to exploit the coupling across these different energy regimes, the method that is capable of manipulating charge-spinlattice interactions is indispensable. Here, by rational chemical design of the supramolecular assembled charge-transfer networks, opto-ferroic properties can be coupled, in which a collective electron transfer and ordering strongly influence the dipole and spin orders, as well as their coupling. The supramolecular charge-transfer crystal presented here opens up a new route for the development of multifunctional organics that can lead to significant advancement in molecular ferronics. C1 [Xu, Beibei; Ren, Shenqiang] Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA. [Xu, Beibei; Ren, Shenqiang] Temple Univ, Temple Mat Inst, Philadelphia, PA 19122 USA. [Luo, Zhipu; Dauter, Zbigniew] Argonne Natl Lab, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, NCI, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gao, Wenxiu; Yuan, Guoliang] Nanjing Univ Sci & Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China. [Wilson, Andrew J.; He, Chao; Dai, Hai-Lung; Rao, Yi; Willets, Katherine] Temple Univ, Dept Chem, Philadelphia, PA 19122 USA. [He, Chao] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [He, Chao] Univ Sci & Technol China, Dept Chem Phys, Hefei 230026, Anhui, Peoples R China. [Chen, Xing] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Ren, SQ (reprint author), Temple Univ, Dept Mech Engn, Philadelphia, PA 19122 USA.; Ren, SQ (reprint author), Temple Univ, Temple Mat Inst, Philadelphia, PA 19122 USA. EM shenqiang.ren@temple.edu OI Wilson, Andrew/0000-0003-3427-810X FU Army Research Office - Young Investigator Program [W911NF-15-1-0610]; U.S. Department of Energy-Basic Energy Sciences [DE-SC0014902]; Department of Energy (DOE), Office of Science, Basic Energy Science (BES) [DE-SC0010307]; Energy Frontier Research Center at Temple University - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012575]; Targeted Research Grant from Temple University Office of the Vice Provost for Research; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38] FX Work at Temple University (S.R) was supported by the Army Research Office - Young Investigator Program (W911NF-15-1-0610, material design/self-assembly of carbon photovoltaics), U.S. Department of Energy-Basic Energy Sciences Award No. DE-SC0014902 (organic synthesis and physical property measurement). Work at Temple University (A.W. and K.W.) was supported by the Department of Energy (DOE), Office of Science, Basic Energy Science (BES) under Award #DE-SC0010307. Y.R and H.L.D acknowledge the seed funding from an Energy Frontier Research Center at Temple University funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award # DE-SC0012575, a Targeted Research Grant from the Temple University Office of the Vice Provost for Research. Diffraction data were collected at the SER-CAT beamline 22BM at the Advanced Photon Source, Argonne National Laboratory. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38. The authors thank Temple Materials Institute and Prof. X. Xi for the AFM measurements. The authors also thank X. Chen at University of Maryland for the dielectric measurements. NR 49 TC 3 Z9 3 U1 7 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2441 EP 2448 DI 10.1021/acs.chemmater.6b00836 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000060 ER PT J AU Guo, XJ Liao, QG Manley, EF Wu, ZS Wang, YL Wang, WD Yang, TB Shin, YE Cheng, X Liang, YY Chen, LX Baeg, KJ Marks, TJ Guo, XG AF Guo, Xiaojie Liao, Qiaogan Manley, Eric F. Wu, Zishan Wang, Yulun Wang, Weida Yang, Tingbin Shin, Young-Eun Cheng, Xing Liang, Yongye Chen, Lin X. Baeg, Kang-Jun Marks, Tobin J. Guo, Xugang TI Materials Design via Optimized Intramolecular Noncovalent Interactions for High-Performance Organic Semiconductors SO CHEMISTRY OF MATERIALS LA English DT Article ID POLYMER SOLAR-CELLS; THIN-FILM TRANSISTORS; STRUCTURE-PROPERTY RELATIONSHIPS; FIELD-EFFECT TRANSISTORS; CONJUGATED POLYMERS; BUILDING-BLOCKS; PROCESSING ADDITIVES; THIOPHENE COPOLYMERS; CONDUCTING POLYMERS; RATIONAL DESIGN AB We report the design, synthesis, and implemention in semiconducting polymers of a novel head-to-head linkage containing the TRTOR (3-alkyl-3'-alkoxy-2,2'-bithiophene) donor subunit having a single strategically optimized, planarizing noncovalent S center dot center dot center dot O interaction. Diverse complementary thermal, optical, electrochemical, X-ray scattering, electrical, photovoltaic, and electron microscopic characterization techniques are applied to establish structure-property correlations in a TRTOR-based polymer series. In comparison to monomers having double S center dot center dot center dot O interactions, replacing one alkoxy substituent with a less electron-donating alkyl one yields TRTOR-based polymers with significantly depressed (0.2-0.3 eV) HOMOs. Furthermore, the weaker single S center dot center dot center dot O interaction and greater TRTOR steric encumberance enhances materials processability without sacrificing backbone planarity. From another perspective, TRTOR has comparable electronic properties to ring-fused 5H-dithieno[3,2-b:2',3'-d]pyran (DTP) subunits, but a centrosymmetric geometry which promotes a more compact and ordered structure than bulkier, axisymmetric DTP. Compared to monosubstituted TTOR (3-alkoxy-2,2'-bithiophene), alkylation at the TRTOR bithiophene 3-position enhances conjugation and polymer crystallinity with contracted pi-pi stacking. Grazing incidence wide-angle X-ray scattering (GIWAXS) data reveal that the greater steric hindrance and the weaker single S center dot center dot center dot O interaction are not detrimental to close packing and high crystallinity. As a proof of materials design, copolymerizing TRTOR with phthalimides yields copolymers with promising thin-film transistor mobility as high as 0.42 cm(2)/(V.s) and 6.3% power conversion efficiency in polymer solar cells, the highest of any phthalimide copolymers reported to date. The depressed TRTOR HOMOs imbue these polymers with substantially increased I-on/I-off ratios and Vac's versus analogous subunits with multiple electron donating, planarizing alkoxy substituents. Implementing a head-to-head linkage with an alkyl/alkoxy substitution pattern and a single S center dot center dot center dot O interaction is a promising strategy for organic electronics materials design. C1 [Guo, Xiaojie; Liao, Qiaogan; Wu, Zishan; Wang, Yulun; Wang, Weida; Yang, Tingbin; Cheng, Xing; Liang, Yongye; Guo, Xugang] S Univ Sci & Technol China, Dept Mat Sci & Engn, Shenzhen Key Lab Printed Organ Elect, 1088 Xueyuan Rd, Shenzhen 518055, Guangdong, Peoples R China. [Manley, Eric F.; Chen, Lin X.; Marks, Tobin J.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Manley, Eric F.; Chen, Lin X.; Marks, Tobin J.] Northwestern Univ, Mat Res Ctr, Argonne Northwestern Solar Energy Res Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Shin, Young-Eun; Baeg, Kang-Jun] Pukyong Natl Univ, Dept Graph Arts Informat Engn, 365 Sinseon Ro, Busan 48547, South Korea. [Manley, Eric F.; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wu, Zishan] Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. RP Guo, XG (reprint author), S Univ Sci & Technol China, Dept Mat Sci & Engn, Shenzhen Key Lab Printed Organ Elect, 1088 Xueyuan Rd, Shenzhen 518055, Guangdong, Peoples R China.; Marks, TJ (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Marks, TJ (reprint author), Northwestern Univ, Mat Res Ctr, Argonne Northwestern Solar Energy Res Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Baeg, KJ (reprint author), Pukyong Natl Univ, Dept Graph Arts Informat Engn, 365 Sinseon Ro, Busan 48547, South Korea. EM kangjun100@pknu.ac.kr; t-marks@northwestern.edu; guoxg@sustc.edu.cn FU Shenzhen Peacock Plan project [KQTD20140630110339343]; National Science Foundation of China (NSFC) [51573076]; Basic Research fund of Shenzhen City [JCYJ20140714151402769, JCYJ20130401144532130]; Guangdong Natural Science Foundation [2015A030313900]; Shenzhen Key Lab funding [ZDSYS201505291525382]; AFOSR at Northwestern University [FA9550-08-1-0331]; Argonne-Northwestern Solar Energy Research (ANSER) Center; Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-FG02-08ER46536]; U.S. DOE [DE-AC02-06CH11357] FX Xugang Guo is thankful for the financial support from Shenzhen Peacock Plan project (KQTD20140630110339343), the National Science Foundation of China (NSFC) (51573076), the Basic Research fund of Shenzhen City (JCYJ20140714151402769), the Guangdong Natural Science Foundation (2015A030313900), the Shenzhen Key Lab funding (ZDSYS201505291525382), and the AFOSR (FA9550-08-1-0331) at Northwestern University. T.Y. acknowledges the Basic Research fund of Shenzhen City (JCYJ20130401144532130). E.F.M. acknowledges financial support from Argonne-Northwestern Solar Energy Research (ANSER) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001059, by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Award Number DE-FG02-08ER46536. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 90 TC 8 Z9 8 U1 26 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD APR 12 PY 2016 VL 28 IS 7 BP 2449 EP 2460 DI 10.1021/acs.chemmater.6b00850 PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4RS UT WOS:000374196000061 ER PT J AU Lee, KH Bai, P Rancatore, BJ He, B Liu, Y Xu, T AF Lee, Keun Hyung Bai, Peter Rancatore, Benjamin J. He, Bo Liu, Yi Xu, Ting TI Improved Hierarchical Ordering in Supramolecules via Symmetrically Bifunctionalized Organic Semiconductor SO MACROMOLECULES LA English DT Article ID COPOLYMER-BASED SUPRAMOLECULES; BLOCK-COPOLYMER; SIDE-CHAIN; THIN-FILMS; FUNCTIONAL MATERIALS; DIBLOCK COPOLYMERS; LENGTH SCALES; ASSEMBLIES; COMPLEXES; POLYMERS AB Block copolymer (BCP)-based supramolecular systems provide a versatile approach to manipulate functional structures spanning several nanometers to macroscopic length scales. Most studies to date focused on supramolecules containing asymmetrically end-functionalized small molecules, and it remains challenging to obtain molecular control over small molecule ordering within the BCP microdomain. Here we designed symmetrically end-functionalized bis-phenol quarterthiophene (BP4T) small molecules and systematically investigated how the end-group chemistry of the small molecules affects the supramolecular assembly process and the resulting morphology. Bifunctionalized small molecules can bridge two adjacent polymer blocks and lead to macroscopically aligned hierarchical assemblies at much higher degree of ordering than previously observed for asymmetrically functionalized small molecule analogues. The supramolecular morphology is very sensitive to the stoichiometry between the BP4T and polymer repeat unit because of the specific molecular organization within BCP microdomain. Furthermore, similar thermoresponsiveness of supramolecule, i.e.,-similar to 40% change in the supramolecular periodicity during the heating and cooling cycles, can be obtained at BP4T loading stoichiometry of 0.5, much smaller than that of asymmetrically functionalized small molecule. These results clearly demonstrate that supramolecular assemblies can be readily manipulated by engineering the small molecule chemistry. Present studies provide basic design principles and an effective route to fabricate well-defined hierarchical assemblies for functional and stimuli-responsive nanomaterials. C1 [Lee, Keun Hyung; Bai, Peter; Xu, Ting] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Rancatore, Benjamin J.; Xu, Ting] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [He, Bo; Liu, Yi; Xu, Ting] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [He, Bo; Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Lee, Keun Hyung] Inha Univ, Dept Chem Engn, Inchon 402751, South Korea. RP Xu, T (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Xu, T (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Xu, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM tingxu@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract DE-AC02-05CH11231 through the "Organic/inorganic Nanocomposite Program". Part of the work was performed at the Molecular Foundry and the Advanced Light Source, both of which were supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. NR 32 TC 2 Z9 2 U1 16 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 12 PY 2016 VL 49 IS 7 BP 2639 EP 2645 DI 10.1021/acs.macromol.6b00317 PG 7 WC Polymer Science SC Polymer Science GA DJ4RO UT WOS:000374195600027 ER PT J AU Wang, WY Schlegel, R White, BT Williams, K Voyloy, D Steren, CA Goodwin, A Coughlin, EB Gido, S Beiner, M Hong, K Kang, NG Mays, J AF Wang, Weiyu Schlegel, Ralf White, Benjamin T. Williams, Katherine Voyloy, Dimitry Steren, Carlos A. Goodwin, Andrew Coughlin, E. Bryan Gido, Samuel Beiner, Mario Hong, Kunlun Kang, Nam-Goo Mays, Jimmy TI High Temperature Thermoplastic Elastomers Synthesized by Living Anionic Polymerization in Hydrocarbon Solvent at Room Temperatuie SO MACROMOLECULES LA English DT Article ID SEQUENTIAL MONOMER ADDITION; CONTAINING BLOCK POLYMERS; TRIBLOCK COPOLYMERS; MECHANICAL-PROPERTIES; METHACRYLATE; MORPHOLOGY; BENZOFULVENE; SEGMENTS; STRESS; GRAFT AB We present the synthesis and characterization of a new class of high temperature thermoplastic elastomers composed of polybenzofulvene polyisoprene polybenzofulvene (FIF) triblock copolymers. All copolymers were prepared by living anionic polymerization in benzene at room temperature. Homopolymerization and effects of additives on the glass transition temperature (T-g) of polybenzofulvene (PBF) were also investigated. Among all triblock copolymers studied, FIF with 14 vol % of PBF exhibited a maximum stress of 14.3 +/- 1.3 MPa and strain at break of 1390 +/- 66% from tensile tests. The stress strain curves of FIF-10 and 14 were analyzed by a statistical molecular approach using a nonaffine tube model to estimate the thermoplastic elastomer behavior. Dynamic mechanical analysis that the softening temperature of PBF in FIF was 145 degrees C, much higher than that of thermoplastic elastomers with polystyrene hard blocks. Microphase separation of FIF triblock copolymers was observed by small-angle X-ray scattering, even though long-range order was not achieved under the annealing conditions employed. In addition, the microphase separation of the resulting triblock copolymers was examined by atomic force microscopy. C1 [Wang, Weiyu; White, Benjamin T.; Voyloy, Dimitry; Steren, Carlos A.; Goodwin, Andrew; Kang, Nam-Goo; Mays, Jimmy] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Schlegel, Ralf; Beiner, Mario] Fraunhofer Inst Mikrostruktur Werkstoffen & Syst, Walter Hulse Str 1, D-06120 Halle, Saale, Germany. [Williams, Katherine; Coughlin, E. Bryan; Gido, Samuel] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Voyloy, Dimitry; Mays, Jimmy] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Beiner, Mario] Univ Halle Wittenberg, Nat Wissensch Fak 2, Heinrich Damerow Str 4, D-06120 Halle, Saale, Germany. RP Kang, NG; Mays, J (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Mays, J (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM nkang1@utk.edu; jimmy@utk.edu RI Wang, Weiyu/A-6317-2016; Voylov, Dmitry/H-4059-2013; Beiner, Mario/A-2311-2012; Hong, Kunlun/E-9787-2015 OI Wang, Weiyu/0000-0002-2914-1638; Voylov, Dmitry/0000-0001-5552-6024; Beiner, Mario/0000-0003-0459-323X; Hong, Kunlun/0000-0002-2852-5111 FU NSF Partnerships for Innovation, Building Innovation Capacity program [1237787]; Bill & Melinda Gates Foundation through their Grand Challenges Explorations program; Army Research Office [W911-NF-11-0417]; U.S. National Science Foundation FX We are grateful for financial support from the U.S. National Science Foundation, Award 1237787 from the NSF Partnerships for Innovation, Building Innovation Capacity program. This work also was supported by the Bill & Melinda Gates Foundation through their Grand Challenges Explorations program. We also acknowledge partial support from the Army Research Office under Contract W911-NF-11-0417. The authors thank M. Menzel and J. Klehm for support with the AFM images. NR 46 TC 3 Z9 3 U1 6 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 12 PY 2016 VL 49 IS 7 BP 2646 EP 2655 DI 10.1021/acs.macromol.5b02642 PG 10 WC Polymer Science SC Polymer Science GA DJ4RO UT WOS:000374195600028 ER PT J AU Sridhar, M Gunugunuri, KR Hu, NP Motahari, A Zuo, XB Schaefer, DW Thiel, SW Smirniotis, PG AF Sridhar, Manasa Gunugunuri, Krishna R. Hu, Naiping Motahari, Ahmad Zuo, Xiaobing Schaefer, Dale W. Thiel, Stephen W. Smirniotis, Panagiotis G. TI Impact of Interfacial Roughness on the Sorption Properties of Nanocast Polymers SO MACROMOLECULES LA English DT Article ID PORE-SIZE; MESOPOROUS MATERIALS; ADSORPTION DATA; SURFACE-AREA; CARBON; FOAMS; TEMPLATES; PYROLYSIS; CHEMISTRY; SILICA AB Nanocasting is an emerging method to prepare organic polymers with regular, nanometer pores using inorganic templates. This report assesses the impact of imperfect template replication on the sorption properties of such polymer castings. Existing X-ray diffraction data show that substantial diffuse scattering exists in the small-angle region even though TEM images show near perfect lattices of uniform pores. To assess the origin of the diffuse scattering, the morphology of the phenol-formaldehyde foams (PFF) was investigated by small-angle X-ray scattering (SAXS). The observed diffuse scattering is attributed to interfacial roughness due to fractal structures. Such roughness has a profound impact on the sorption properties. Conventional pore-filling models, for example, overestimate protein sorption capacity. A mathematical framework is presented to calculate sorption properties based on observed morphological parameters. The formalism uses the surface fractal dimension determined by SAXS in conjunction with nitrogen adsorption isotherms to predict lysozyme sorption. The results are consistent with measured lysozyme loading. C1 [Sridhar, Manasa; Gunugunuri, Krishna R.; Hu, Naiping; Motahari, Ahmad; Schaefer, Dale W.; Thiel, Stephen W.; Smirniotis, Panagiotis G.] Univ Cincinnati, Dept Chem Biomed & Environm Engn, Cincinnati, OH 45221 USA. [Schaefer, Dale W.] Univ Cincinnati, Dept Mech & Mat Engn, Cincinnati, OH 45221 USA. [Zuo, Xiaobing] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Schaefer, DW (reprint author), Univ Cincinnati, Dept Chem Biomed & Environm Engn, Cincinnati, OH 45221 USA.; Schaefer, DW (reprint author), Univ Cincinnati, Dept Mech & Mat Engn, Cincinnati, OH 45221 USA. EM dale.schaefer@uc.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; University of Cincinnati FX Use of the Advanced Photon Source and Xiaobing Zuo were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. All University of Cincinnati authors were funded by the University of Cincinnati. NR 31 TC 0 Z9 0 U1 6 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 12 PY 2016 VL 49 IS 7 BP 2663 EP 2670 DI 10.1021/acs.macromol.6b00304 PG 8 WC Polymer Science SC Polymer Science GA DJ4RO UT WOS:000374195600030 ER PT J AU Scavuzzo, JJ Yan, XS Zhao, YH Scherger, JD Chen, JY Zhang, S Liu, H Gao, M Li, T Zhao, XY Hamed, GR Foster, MD Jia, L AF Scavuzzo, Joseph J. Yan, Xuesong Zhao, Yihong Scherger, Jacob D. Chen, Junyi Zhang, Shuo Liu, Hao Gao, Min Li, Tao Zhao, Xiuying Hamed, Gary R. Foster, Mark D. Jia, Li TI Supramolecular Elastomers. Particulate beta-Sheet Nanocrystal-Reinforced Synthetic Elastic Networks SO MACROMOLECULES LA English DT Article ID SPIDER SILK; HARD SEGMENTS; CARBON-BLACK; POLYISOBUTYLENE; POLYMERS; STRENGTH; NANOSTRUCTURE; COPOLYMERS; TOUGHNESS; RUBBER AB beta-Sheet crystals in natural silks are particulate and less than 10 nm in size in all three dimensions. In synthetic supramolecular analogues of natural silks, beta-sheet crystals have been found to be fibrous with the longest dimension exceeding 100 nm in the hydrogen-bonding direction. This work demonstrates that particulate beta-sheet crystals can be achieved without the use of an elaborate amino acid sequence by simply grafting oligo(beta-alanine) segments as pendent side groups to a butyl rubber main chain. The size control in the hydrogen-bonding direction is attributable to an entropic force that opposes the driving force for the self-assembly. The nanocrystals, especially those of trimeric beta-alanine segments, display a remarkable ability to simultaneously provide stiffness, extensibility, and strength to the synthetic elastic network and do so highly efficiently at a low volume fraction of the material. The herein studied butyl rubber-based thermoplastic elastomers containing no more than 3.6 vol % of beta-sheet nanocrystals are stiffer, stronger, and more extensible than vulcanized butyl rubber reinforced by 20 vol % of carbon black and poly(styrene-b-isobutylene-b-styrene) reinforced by >33 vol % of polystyrene domains. The high reinforcing efficacy of the beta-sheet crystals is attributable to two phenomena associated with their small sizes: a stick slip mechanism for energy dissipation and an auxiliary layer of polymer brush that contributes to increasing the modulus. C1 [Scavuzzo, Joseph J.; Yan, Xuesong; Zhao, Yihong; Scherger, Jacob D.; Chen, Junyi; Zhang, Shuo; Liu, Hao; Zhao, Xiuying; Hamed, Gary R.; Foster, Mark D.; Jia, Li] Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA. [Gao, Min] Kent State Univ, Inst Liquid Crystal, Kent, OH 44242 USA. [Gao, Min] Kent State Univ, Chem Phys Interdisciplinary Program, Kent, OH 44242 USA. [Li, Tao] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Zhao, Xiuying] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China. RP Jia, L (reprint author), Univ Akron, Dept Polymer Sci, Akron, OH 44325 USA. EM ljia@uakron.edu FU Ohio Board of Regents Research Challenge Program, Triangle Tire USA; University of Akron FX We thank the Ohio Board of Regents Research Challenge Program, Triangle Tire USA, and The University of Akron for financial support and the Defense University Research Instrumentation Program (DURIP) (W911NF-10-1-0167) for provision of the AFM instrumentation. Gratitude is also due to Vanderbilt Chemicals for donating the butyl rubber used in this research. J.J.S. gratefully acknowledges an Ohio Rubber Group Award. NR 53 TC 0 Z9 0 U1 20 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 12 PY 2016 VL 49 IS 7 BP 2688 EP 2697 DI 10.1021/acs.macromol.6b00003 PG 10 WC Polymer Science SC Polymer Science GA DJ4RO UT WOS:000374195600033 ER PT J AU Tang, YH Li, Z Li, XJ Deng, MG Karniadakis, GE AF Tang, Yu-Hang Li, Zhen Li, Xuejin Deng, Mingge Karniadakis, George Em TI Non-Equilibrium Dynamics of Vesicles and Micelles by Self-Assembly of Block Copolymers with Double Thermoresponsivity SO MACROMOLECULES LA English DT Article ID DISSIPATIVE PARTICLE DYNAMICS; SOLUTION TEMPERATURE BEHAVIOR; DRUG-DELIVERY; MESOSCOPIC SIMULATION; DIBLOCK COPOLYMER; ANTICANCER DRUGS; PHASE-TRANSITION; POLYMERS; CHAIN; WATER AB We present a mesoscopic simulation study of doubly thermoresponsive self-assemblies, revealing previously unknown dynamic behavior and proving experimental hypotheses. By explicitly modeling internal energy as a degree of freedom of coarse-grained particles, we simulated the thermally induced self assembly process triggered by the evolution of temperature over time and space. We found that both external and intrinsic factors are responsible for altering the assembly pathway of thermoresponsive micelles and hence determining the final aggregate morphology. We identified a frequency regime where thermoresponsive unilamellar vesicles can sustain repeated heating cooling cycles in a thermal loading test, and we quantified the collapse probability and half-life of the vesicles under frequencies that cause vesicle destruction. Two molecular movement modes dominate, namely flip and slip, in thermoresponsive bilayer membranes during the inversion of composition. We demonstrated that doubly thermoresponsive micelles and vesicles, as potential drug delivery vehicles, exhibit distinct hydrodynamic behavior when flowing through capillaries whose temperature spans across the inversion temperature of the carriers. C1 [Tang, Yu-Hang; Li, Zhen; Li, Xuejin; Deng, Mingge; Karniadakis, George Em] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Karniadakis, George Em] Pacific NW Natl Lab, Collaboratory Math Mesoscop Modeling Mat, Richland, WA 99354 USA. RP Tang, YH; Karniadakis, GE (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA.; Karniadakis, GE (reprint author), Pacific NW Natl Lab, Collaboratory Math Mesoscop Modeling Mat, Richland, WA 99354 USA. EM yuhang_tang@brown.edu; george_karniadakis@brown.edu RI Li, Zhen/B-2722-2013; Li, Xuejin/B-8559-2009 OI Li, Zhen/0000-0002-0936-6928; Li, Xuejin/0000-0002-4446-2480 FU Department of Energy (DOE) Collaboratory on Mathematics for Mesoscopic Modeling of Materials [CM4]; Oak Ridge Leadership Computing Facility through the Innovative and Novel Computational Impact on Theory and Experiment program at Oak Ridge National Laboratory [BIP102, BIP118]; IBM FX This work was supported by the Department of Energy (DOE) Collaboratory on Mathematics for Mesoscopic Modeling of Materials (CM4). Simulations were carried out at the Oak Ridge Leadership Computing Facility through the Innovative and Novel Computational Impact on Theory and Experiment program at Oak Ridge National Laboratory under Projects BIP102 and BIP118. Y.-H.T. thanks Changho Kim for discussions on polymer diffusivity. Y.-H.T. acknowledges partial financial support from an IBM Ph.D. Scholarship Award. NR 54 TC 1 Z9 1 U1 19 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD APR 12 PY 2016 VL 49 IS 7 BP 2895 EP 2903 DI 10.1021/acs.macromol.6b00365 PG 9 WC Polymer Science SC Polymer Science GA DJ4RO UT WOS:000374195600055 ER PT J AU Landau, SM Horng, A Fero, A Jagust, WJ AF Landau, Susan M. Horng, Andy Fero, Allison Jagust, William J. CA Alzheimer's Dis Neuroimaging Initi TI Amyloid negativity in patients with clinically diagnosed Alzheimer disease and MCI SO NEUROLOGY LA English DT Article ID POSITRON-EMISSION-TOMOGRAPHY; NEUROIMAGING INITIATIVE ADNI; APOLIPOPROTEIN-E EPSILON-4; MILD COGNITIVE IMPAIRMENT; PITTSBURGH COMPOUND B; LATE-LIFE DEPRESSION; NEUROPATHOLOGIC ASSESSMENT; VASCULAR-DEMENTIA; BETA; PET AB Objective:To examine the clinical and biomarker characteristics of patients with amyloid-negative Alzheimer disease (AD) and mild cognitive impairment (MCI) from the Alzheimer's Disease Neuroimaging Initiative (ADNI), a prospective cohort study.Methods:We first investigated the reliability of florbetapir- PET in patients with AD and patients with MCI using CSF-A(1-42) as a comparison amyloid measurement. We then compared florbetapir- vs florbetapir+ patients with respect to several AD-specific biomarkers, baseline and longitudinal cognitive measurements, and demographic and clinician report data.Results:Florbetapir and CSF-A(1-42) +/- status agreed for 98% of ADs (89% of MCIs), indicating that most florbetapir- scans were a reliable representation of amyloid status. Florbetapir- AD (n = 27/177; 15%) and MCI (n = 74/217, 34%) were more likely to be APOE4-negative (MCI 83%, AD 96%) than their florbetapir+ counterparts (MCI 30%, AD 24%). Florbetapir- patients also had less AD-specific hypometabolism, lower CSF p-tau and t-tau, and better longitudinal cognitive performance, and were more likely to be taking medication for depression. In MCI only, florbetapir- participants had less hippocampal atrophy and hypometabolism and lower functional activity questionnaire scores compared to florbetapir+ participants.Conclusions:Overall, image analysis problems do not appear to be a primary explanation of amyloid negativity. Florbetapir- ADNI patients have a variety of clinical and biomarker features that differ from their florbetapir+ counterparts, suggesting that one or more non-AD etiologies (which may include vascular disease and depression) account for their AD-like phenotype. C1 [Landau, Susan M.; Horng, Andy; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Landau, Susan M.; Fero, Allison; Jagust, William J.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Landau, SM (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.; Landau, SM (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM slandau@berkeley.edu OI Preda, Adrian /0000-0003-3373-2438 FU Alzheimer's Disease Neuroimaging Initiative (ADNI) (NIH) [U01 AG024904]; National Institute on Aging, the National Institute of Biomedical Imaging and Bioengineering; Canadian Institutes of Rev December, Health Research FX Data collection and sharing for this project was funded by the Alzheimer's Disease Neuroimaging Initiative (ADNI) (NIH grant U01 AG024904). ADNI is funded by the National Institute on Aging, the National Institute of Biomedical Imaging and Bioengineering, and through contributions from the following: Alzheimer's Association; Alzheimer's Drug Discovery Foundation; Araclon Biotech; BioClinica, Inc.; Biogen Idec Inc.; Bristol-Myers Squibb Company; Eisai Inc.; Elan Pharmaceuticals, Inc.; Eli Lilly and Company; EuroImmun; F. Hoffmann-La Roche Ltd. and its affiliated company Genentech, Inc.; Fujirebio; GE Healthcare; IXICO Ltd.; Janssen Alzheimer Immunotherapy Research & Development, LLC; Johnson & Johnson Pharmaceutical Research & Development LLC; Medpace, Inc.; Merck & Co., Inc.; Meso Scale Diagnostics, LLC; NeuroRx Research; Neurotrack Technologies; Novartis Pharmaceuticals Corporation; Pfizer Inc.; Piramal Imaging; Servier; Synarc Inc.; and Takeda Pharmaceutical Company. The Canadian Institutes of Rev December 5, 2013, Health Research is providing funds to support ADNI clinical sites in Canada. Private sector contributions are facilitated by the Foundation for the NIH (www.fnih.org). The grantee organization is the Northern California Institute for Research and Education, and the study is coordinated by the Alzheimer's Disease Cooperative Study at the University of California, San Diego. ADNI data are disseminated by the Laboratory for NeuroImaging at the University of Southern California. NR 39 TC 5 Z9 5 U1 2 U2 4 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0028-3878 EI 1526-632X J9 NEUROLOGY JI Neurology PD APR 12 PY 2016 VL 86 IS 15 BP 1377 EP 1385 DI 10.1212/WNL.0000000000002576 PG 9 WC Clinical Neurology SC Neurosciences & Neurology GA DI9LL UT WOS:000373824100004 PM 26968515 ER PT J AU Sharpe, RM Koepke, T Harper, A Grimes, J Galli, M Satoh-Cruz, M Kalyanaraman, A Evans, K Kramer, D Dhingra, A AF Sharpe, Richard M. Koepke, Tyson Harper, Artemus Grimes, John Galli, Marco Satoh-Cruz, Mio Kalyanaraman, Ananth Evans, Katherine Kramer, David Dhingra, Amit TI CisSERS: Customizable In Silico Sequence Evaluation for Restriction Sites SO PLOS ONE LA English DT Article ID MARKER DEVELOPMENT; SNP DISCOVERY; TOOL; DESIGN; PROGRAM; DNA; PCR AB High-throughput sequencing continues to produce an immense volume of information that is processed and assembled into mature sequence data. Data analysis tools are urgently needed that leverage the embedded DNA sequence polymorphisms and consequent changes to restriction sites or sequence motifs in a high-throughput manner to enable biological experimentation. CisSERS was developed as a standalone open source tool to analyze sequence datasets and provide biologists with individual or comparative genome organization information in terms of presence and frequency of patterns or motifs such as restriction enzymes. Predicted agarose gel visualization of the custom analyses results was also integrated to enhance the usefulness of the software. CisSERS offers several novel functionalities, such as handling of large and multiple datasets in parallel, multiple restriction enzyme site detection and custom motif detection features, which are seamlessly integrated with real time agarose gel visualization. Using a simple fasta-formatted file as input, CisSERS utilizes the REBASE enzyme database. Results from CisSERS enable the user to make decisions for designing genotyping by sequencing experiments, reduced representation sequencing, 3'UTR sequencing, and cleaved amplified polymorphic sequence (CAPS) molecular markers for large sample sets. CisSERS is a java based graphical user interface built around a perl backbone. Several of the applications of CisSERS including CAPS molecular marker development were successfully validated using wet-lab experimentation. Here, we present the tool CisSERS and results from in-silico and corresponding wet-lab analyses demonstrating that CisSERS is a technology platform solution that facilitates efficient data utilization in genomics and genetics studies. C1 [Sharpe, Richard M.; Koepke, Tyson; Dhingra, Amit] Washington State Univ, Mol Plant Sci Grad Program, Pullman, WA 99164 USA. [Koepke, Tyson; Harper, Artemus; Galli, Marco; Evans, Katherine; Dhingra, Amit] Washington State Univ, Dept Hort, Pullman, WA 99164 USA. [Sharpe, Richard M.] Washington State Univ, Sch Biol Sci, Pullman, WA 99164 USA. [Grimes, John; Kalyanaraman, Ananth] Washington State Univ, Elect Engn & Comp Sci, Pullman, WA 99164 USA. [Satoh-Cruz, Mio; Kramer, David] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. RP Dhingra, A (reprint author), Washington State Univ, Mol Plant Sci Grad Program, Pullman, WA 99164 USA.; Dhingra, A (reprint author), Washington State Univ, Dept Hort, Pullman, WA 99164 USA. EM adhingra@wsu.edu RI Dhingra, Amit/E-7369-2010; OI Sharpe, Richard/0000-0002-8513-4862 FU WSU Agriculture Research Center Hatch funds; Department of Agriculture National Research Initiative (USDA-NRI) [2008 -35300-04676] FX This work was supported by WSU Agriculture Research Center Hatch funds to AD and KE. US Department of Agriculture National Research Initiative (USDA-NRI) grant 2008 -35300-04676 to AD and AK supported AH and JG. TAK acknowledges the National Institutes of Health Protein Biotechnology Training Grant T32GM008336 and ARCS Fellowship Program. RMS's work was supported by the National Science Foundation under Grants IOS 0641232 and MCB 1146928 and by Civilian Research and Development Foundation Grant RUB1-2982-ST-10 to Gerald E. Edwards, WSU. Work related to characterization of the cfq mutant was supported by US Department of Energy, Office of Science, Basic Energy Sciences Program DE-FG02-04ERl5559 to DMK. NR 20 TC 0 Z9 0 U1 2 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 12 PY 2016 VL 11 IS 4 AR e0152404 DI 10.1371/journal.pone.0152404 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DJ0NI UT WOS:000373900700009 PM 27071032 ER PT J AU Ismael, A Tian, W Waszczak, N Wang, X Cao, YF Suchkov, D Bar, E Metodiev, MV Liang, J Arkowitz, RA Stone, DE AF Ismael, Amber Tian, Wei Waszczak, Nicholas Wang, Xin Cao, Youfang Suchkov, Dmitry Bar, Eli Metodiev, Metodi V. Liang, Jie Arkowitz, Robert A. Stone, David E. TI G beta promotes pheromone receptor polarization and yeast chemotropism by inhibiting receptor phosphorylation SO SCIENCE SIGNALING LA English DT Article ID HETEROTRIMERIC G-PROTEIN; CASEIN KINASE-I; SIGNAL-TRANSDUCTION PATHWAY; SACCHAROMYCES-CEREVISIAE; MATING PHEROMONE; ACTIN CYTOSKELETON; CHEMICAL GRADIENTS; SPATIAL GRADIENTS; MASS-SPECTROMETRY; BUDDING YEAST AB Gradient-directed cell migration (chemotaxis) and growth (chemotropism) are processes that are essential to the development and life cycles of all species. Cells use surface receptors to sense the shallow chemical gradients that elicit chemotaxis and chemotropism. Slight asymmetries in receptor activation are amplified by downstream signaling systems, which ultimately induce dynamic reorganization of the cytoskeleton. During the mating response of budding yeast, a model chemotropic system, the pheromone receptors on the plasma membrane polarize to the side of the cell closest to the stimulus. Although receptor polarization occurs before and independently of actin cable-dependent delivery of vesicles to the plasma membrane (directed secretion), it requires receptor internalization. Phosphorylation of pheromone receptors by yeast casein kinase 1 or 2 (Yck1/2) stimulates their internalization. We showed that the pheromone-responsive G beta gamma dimer promotes the polarization of the pheromone receptor by interacting with Yck1/2 and locally inhibiting receptor phosphorylation. We also found that receptor phosphorylation is essential for chemotropism, independently of its role in inducing receptor internalization. A mathematical model supports the idea that the interaction between G beta gamma and Yck1/2 results in differential phosphorylation and internalization of the pheromone receptor and accounts for its polarization before the initiation of directed secretion. C1 [Ismael, Amber; Waszczak, Nicholas; Wang, Xin; Suchkov, Dmitry; Bar, Eli; Stone, David E.] Univ Illinois, Dept Biol Sci, Chicago, IL 60607 USA. [Tian, Wei; Cao, Youfang; Liang, Jie] Univ Illinois, Dept Bioengn, Chicago, IL 60607 USA. [Metodiev, Metodi V.] Univ Essex, Sch Biol Sci, Colchester CO4 3SQ, Essex, England. [Arkowitz, Robert A.] Univ Nice Sophia Antipolis, Inst Biol Valrose, INSERM UMR1091, CNRS UMR7277, F-06108 Nice 2, France. [Cao, Youfang] Los Alamos Natl Lab, Ctr Nonlinear Studies, Theoret Biol & Biophys Grp T 6, POB 1663, Los Alamos, NM 87545 USA. [Suchkov, Dmitry] Cellecta Inc, Mountain View, CA 94043 USA. [Bar, Eli] Case Western Reserve Univ, Dept Neurol Surg, Cleveland, OH 44106 USA. RP Stone, DE (reprint author), Univ Illinois, Dept Biol Sci, Chicago, IL 60607 USA. EM dstone@uic.edu RI Tian, Wei/B-5387-2017 OI Tian, Wei/0000-0002-2146-1717 FU NSF [1024718, 1415589, DBI 1062328]; CNRS [PICS06228]; Fondation ARC [SFI20121205755]; NIH [GM079804, 1RO3CA150131]; Chicago Biomedical Consortium; Searle Funds at The Chicago Community Trust FX This work was supported by NSF grants 1024718 and 1415589 (to D.E.S.), CNRS grant PICS06228 and Fondation ARC grant SFI20121205755 (to R.A.A.), NIH grant GM079804 and NSF grant DBI 1062328 (to J.L.), and NIH grant 1RO3CA150131 (to M.V.M.). This work was also funded by the Chicago Biomedical Consortium with support from the Searle Funds at The Chicago Community Trust. NR 65 TC 2 Z9 2 U1 4 U2 7 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 1945-0877 EI 1937-9145 J9 SCI SIGNAL JI Sci. Signal. PD APR 12 PY 2016 VL 9 IS 423 AR ra38 DI 10.1126/scisignal.aad4376 PG 16 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DJ3NC UT WOS:000374111200005 PM 27072657 ER PT J AU Armstrong, NMR Mortimer, KD Kong, T Bud'ko, SL Canfield, PC Basov, DN Timusk, T AF Armstrong, N. M. R. Mortimer, Kevin D. Kong, T. Bud'ko, S. L. Canfield, P. C. Basov, D. N. Timusk, T. TI Quantum diffusion of electrons in quasiperiodic and periodic approximant lattices in the rare earth-cadmium system SO PHILOSOPHICAL MAGAZINE LA English DT Article DE optical conductivity; quantum diffusion; Drude model; reflectivity; Quasicrystal; approximant ID OPTICAL CONDUCTIVITY; CRYSTALS; AL70MN9PD21; ALLOYS AB Icosahedral quasicrystals are characterised by the absence of a distinct Drude peak in their low-frequency optical conductivity and the same is true of their crystalline approximants. We have measured the optical conductivity of i-GdCd [GRAPHICS] , an icosahedral quasicrystal, and two approximants, GdCd [GRAPHICS] and YCd [GRAPHICS] . We find that there is a significant difference in the optical properties of these compounds. The approximants have a zero frequency peak, characteristic of a metal, whereas the quasicrystal has a striking minimum. This is the first example where the transport properties of a quasicrystal and its approximant differ in such a fundamental way. Using a generalised Drude model introduced by Mayou, we find that our data are well described by this model. It implies that the quantum diffusion of electron wave packets through the periodic and quasiperiodic lattices is responsible for these dramatic differences: in the approximants, the transport is superdiffusive, whereas the quasicrystals show subdiffusive motion of the electrons. C1 [Armstrong, N. M. R.; Mortimer, Kevin D.; Timusk, T.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Kong, T.; Bud'ko, S. L.; Canfield, P. C.] Iowa State Univ, Dept Phys & Astron, Ames Lab, Ames, IA USA. [Basov, D. N.] Univ Calif San Diego, Dept Phys, San Diego, CA 92103 USA. RP Armstrong, NMR (reprint author), McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. EM armstrong@mcmaster.ca FU US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; US Department of Energy by Iowa State University [DE-AC02-07CH11358]; [ARO w911NF-13-1-0210] FX Research performed at the Ames Laboratory was supported by the US Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the US Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Work at UCSD was supported by [grant number ARO w911NF-13-1-0210]. NR 18 TC 0 Z9 0 U1 4 U2 9 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD APR 12 PY 2016 VL 96 IS 11 BP 1122 EP 1130 DI 10.1080/14786435.2016.1150612 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA DJ1EL UT WOS:000373946000006 ER PT J AU Kraus, RG Davis, JP Seagle, CT Fratanduono, DE Swift, DC Brown, JL Eggert, JH AF Kraus, R. G. Davis, J. -P. Seagle, C. T. Fratanduono, D. E. Swift, D. C. Brown, J. L. Eggert, J. H. TI Dynamic compression of copper to over 450 GPa: A high-pressure standard SO PHYSICAL REVIEW B LA English DT Article ID RAMP COMPRESSION; ALUMINUM; STATE; RUBY; CU; EQUATIONS; SCALE; GAUGE; AG; CALIBRATION AB An absolute stress-density path for shocklessly compressed copper is obtained to over 450 GPa. A magnetic pressure drive is temporally tailored to generate shockless compression waves through over 2.5-mm-thick copper samples. The free-surface velocity data is analyzed for Lagrangian sound velocity using the iterative Lagrangian analysis (ILA) technique, which relies upon the method of characteristics. We correct for the effects of strength and plastic work heating to determine an isentropic compression path. By assuming a Debye model for the heat capacity, we can further correct the isentrope to an isotherm. Our determination of the isentrope and isotherm of copper represents a highly accurate pressure standard for copper to over 450 GPa. C1 [Kraus, R. G.; Fratanduono, D. E.; Swift, D. C.; Eggert, J. H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Davis, J. -P.; Seagle, C. T.; Brown, J. L.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Kraus, RG (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to acknowledge the support of the large interdisciplinary team it takes to design, fabricate, and execute experiments on the Z machine. We also thank Marius Millot, Tom Arsenlis, and Rip Collins for helpful comments on the paper. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 52 TC 2 Z9 2 U1 3 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 12 PY 2016 VL 93 IS 13 AR 134105 DI 10.1103/PhysRevB.93.134105 PG 11 WC Physics, Condensed Matter SC Physics GA DI8NY UT WOS:000373758900001 ER PT J AU Lu, YM Vishwanath, A AF Lu, Yuan-Ming Vishwanath, Ashvin TI Classification and properties of symmetry-enriched topological phases: Chern-Simons approach with applications to Z(2) spin liquids SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM HALL STATES; FIELD THEORY; ENTANGLEMENT ENTROPY; LUTTINGER LIQUID; EDGE EXCITATIONS; GROUND-STATE; SUPERCONDUCTORS; INSULATORS; ANYONS; COMPUTATION AB We study (2+1)-dimensional phases with topological order, such as fractional quantum Hall states and gapped spin liquids, in the presence of global symmetries. Phases that share the same topological order can then differ depending on the action of symmetry, leading to symmetry-enriched topological (SET) phases. Here, we present a K-matrix Chern-Simons approach to identify distinct phases with Abelian topological order, in the presence of unitary or antiunitary global symmetries. A key step is the identification of a smooth edge sewing condition that is used to check if two putative phases are indeed distinct. We illustrate this method by classifying Z(2) topological order (Z(2) spin liquids) in the presence of an internal Z(2) global symmetry for which we find six distinct phases. These include two phases with an unconventional action of symmetry that permutes anyons leading to symmetry-protected Majorana edge modes. Other routes to realizing protected edge states in SET phases are identified. Symmetry-enriched Laughlin states and double-semion theories are also discussed. Somewhat surprisingly, we observe that (i) gauging the global symmetry of distinct SET phases leads to topological orders with the same total quantum dimension, and (ii) a pair of distinct SET phases can yield the same topological order on gauging the symmetry. C1 [Lu, Yuan-Ming] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lu, Yuan-Ming] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. RP Lu, YM (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Lu, YM (reprint author), Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. RI Lu, Yuan-Ming/D-7554-2017 OI Lu, Yuan-Ming/0000-0001-6275-739X FU Office of BES, Materials Sciences Division of the U. S. DOE [DE-AC02-05CH11231]; NSF [0645691] FX We thank X. Chen, T. Senthil, X. G. Wen, and especially L. Fidkowski for numerous discussions. Y.M.L. thanks J. L.-Y. Hung for helpful discussions on Ref. [42]. We are particularly indebted to M. Metlitski for helpful comments. This work is supported by Office of BES, Materials Sciences Division of the U. S. DOE under Contract No. DE-AC02-05CH11231 (Y.M.L., A. V.) and by NSF Grant No. DMR 0645691 (A. V.). NR 88 TC 18 Z9 18 U1 4 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 12 PY 2016 VL 93 IS 15 AR 155121 DI 10.1103/PhysRevB.93.155121 PG 32 WC Physics, Condensed Matter SC Physics GA DI8OS UT WOS:000373760900003 ER PT J AU Morales, AP Pourret, A Knebel, G Bastien, G Taufour, V Aoki, D Yamagami, H Flouquet, J AF Morales, A. Palacio Pourret, A. Knebel, G. Bastien, G. Taufour, V. Aoki, D. Yamagami, H. Flouquet, J. TI Thermoelectric power quantum oscillations in the ferromagnet UGe2 SO PHYSICAL REVIEW B LA English DT Article ID ZERO-TEMPERATURE LIMIT; FERMI-SURFACE; AMBIENT-PRESSURE; TRANSPORT-PROPERTIES; ELECTRONIC-STRUCTURE; FIELD; CRYSTAL; SUPERCONDUCTIVITY; THERMOPOWER; TRANSITION AB We present thermoelectric power and resistivity measurements in the ferromagnet UGe2 as a function of temperature and magnetic field. At low temperature, huge quantum oscillations are observed in the thermoelectric power as a function of the magnetic field applied along the a axis. The frequencies of the extreme orbits are determined and an analysis of the cyclotron masses is performed following different theoretical approaches for quantum oscillations detected in the thermoelectric power. They are compared to those obtained by Shubnikov-de Haas experiments on the same crystal and previous de Haas-van Alphen experiments. The agreement of the different probes confirms thermoelectric power as an excellent probe to extract simultaneously both microscopic and macroscopic information on the Fermi surface properties. Band structure calculations of UGe2 in the ferromagnetic state are compared to the experiment. C1 [Morales, A. Palacio; Pourret, A.; Knebel, G.; Bastien, G.; Taufour, V.; Aoki, D.; Flouquet, J.] Univ Grenoble Alpes, INAC SPSMS, F-38000 Grenoble, France. [Morales, A. Palacio; Pourret, A.; Knebel, G.; Bastien, G.; Taufour, V.; Aoki, D.; Flouquet, J.] CEA, INAC SPSMS, F-38000 Grenoble, France. [Aoki, D.] Tohoku Univ, IMR, Oarai, Ibaraki 3111313, Japan. [Yamagami, H.] Japan Atom Energy Agcy, Condensed Matter Sci Div, Sayo, Hyogo 6795148, Japan. [Yamagami, H.] Kyoto Sangyo Univ, Dept Phys, Fac Sci, Kyoto 6038555, Japan. [Morales, A. Palacio] Univ Hamburg, Inst Appl Phys, D-20355 Hamburg, Germany. [Morales, A. Palacio] Univ Hamburg, Interdisciplinary Nanosci Ctr Hamburg, D-20355 Hamburg, Germany. [Taufour, V.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Pourret, A; Knebel, G (reprint author), Univ Grenoble Alpes, INAC SPSMS, F-38000 Grenoble, France.; Pourret, A; Knebel, G (reprint author), CEA, INAC SPSMS, F-38000 Grenoble, France. EM alexandre.pourret@cea.fr; georg.knebel@cea.fr RI Knebel, Georg/A-3294-2012; Aoki, Dai/K-3673-2012; Palacio Morales, Alexandra/K-1159-2016 OI Aoki, Dai/0000-0003-2334-8360; Palacio Morales, Alexandra/0000-0003-1483-5933 FU French ANR (within the program PRINCESS); French ANR (within the program SINUS); French ANR (within the program CORMAT); ERC starting grant (NewHeavyFermion); Universite Grenoble-1 within the Pole SMINGUE FX We acknowledge K. Behnia and B. Fauque for insightful discussions and critical reading of the manuscript. H. Harima, K. Izawa, V. P. Mineev, and A. A. Varlamov are acknowledged for fruitful discussions and T. Terashima for communicating the exact values of the dHvA frequencies and masses of Ref. [37]. We acknowledge financial support from the French ANR (within the programs PRINCESS, SINUS, CORMAT), the ERC starting grant (NewHeavyFermion), and the Universite Grenoble-1 within the Pole SMINGUE. NR 64 TC 2 Z9 2 U1 9 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 12 PY 2016 VL 93 IS 15 AR 155120 DI 10.1103/PhysRevB.93.155120 PG 11 WC Physics, Condensed Matter SC Physics GA DI8OS UT WOS:000373760900002 ER PT J AU Blum, T Boyle, PA Christ, NH Frison, J Garron, N Hudspith, RJ Izubuchi, T Janowski, T Jung, C Juttner, A Kelly, C Kenway, RD Lehner, C Marinkovic, M Mawhinney, RD McGlynn, G Murphy, DJ Ohta, S Portelli, A Sachrajda, CT Soni, A AF Blum, T. Boyle, P. A. Christ, N. H. Frison, J. Garron, N. Hudspith, R. J. Izubuchi, T. Janowski, T. Jung, C. Juettner, A. Kelly, C. Kenway, R. D. Lehner, C. Marinkovic, M. Mawhinney, R. D. McGlynn, G. Murphy, D. J. Ohta, S. Portelli, A. Sachrajda, C. T. Soni, A. CA RBC Collaboration UKQCD Collaboration TI Domain wall QCD with physical quark masses SO PHYSICAL REVIEW D LA English DT Article ID LATTICE QCD; NONPERTURBATIVE RENORMALIZATION; MOBIUS FERMIONS; CHIRAL FERMIONS; OPERATORS AB We present results for several light hadronic quantities (f(pi), f(K), B-K, m(ud), m(s), t(0)(1/2), w(0)) obtained from simulations of 2 + 1 flavor domain wall lattice QCD with large physical volumes and nearly physical pion masses at two lattice spacings. We perform a short, O(3)%, extrapolation in pion mass to the physical values by combining our new data in a simultaneous chiral/continuum "global fit" with a number of other ensembles with heavier pion masses. We use the physical values of m(pi), m(K) and m(Omega) to determine the two quark masses and the scale-all other quantities are outputs from our simulations. We obtain results with subpercent statistical errors and negligible chiral and finite-volume systematics for these light hadronic quantities, including f(pi) = 130.2(9) MeV; f(K) = 155.5(8) MeV; the average up/down quark mass and strange quark mass in the (MS) over bar scheme at 3 GeV, 2.997(49) and 81.64(1.17) MeV respectively; and the neutral kaon mixing parameter, B-K, in the renormalization group invariant scheme, 0.750(15) and the (MS) over bar scheme at 3 GeV, 0.530(11). C1 [Blum, T.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Blum, T.; Izubuchi, T.; Kelly, C.; Ohta, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Boyle, P. A.; Frison, J.; Kenway, R. D.] Univ Edinburgh, Sch Phys, SUPA, Edinburgh EH9 3JZ, Midlothian, Scotland. [Christ, N. H.; Mawhinney, R. D.; McGlynn, G.; Murphy, D. J.] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Garron, N.] Univ Cambridge, Dept Appl Math & Theoret Phys, Cambridge CB3 0WA, England. [Hudspith, R. J.] York Univ, Dept Phys & Astron, Toronto, ON M3J 1P3, Canada. [Izubuchi, T.; Jung, C.; Lehner, C.; Soni, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Janowski, T.; Juettner, A.; Marinkovic, M.; Portelli, A.; Sachrajda, C. T.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Marinkovic, M.] CERN, Dept Phys, CH-1211 Geneva 23, Switzerland. [Ohta, S.] High Energy Accelerator Org, Inst Particle & Nucl Studies, KEK, 1-1 Oho, Tsukuba, Ibaraki 3050801, Japan. [Ohta, S.] Sokendai Grad Univ Adv Studies, Dept Particle & Nucl Phys, Hayama, Kanagawa 2400193, Japan. RP Blum, T (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA.; Blum, T (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. OI Portelli, Antonin/0000-0002-6059-917X; Murphy, David/0000-0002-8538-815X FU BIS National E-infrastructure capital Grant [ST/K000411/1]; STFC capital Grant [ST/H008845/1]; STFC DiRAC Operations Grants [ST/K005804/1, ST/K005790/1]; European Research Council under the European Community's Seventh Framework Programme (FP7) ERC Grant [279757]; U.S. DOE SciDAC program; BAGEL; U.S. DOE [DE-FG02-92ER41989, DE-SC0011941, AC-02-98CH10886]; STFC Grants [ST/J000396/1, ST/L000296/1, ST/L000458/1, ST/J000329/1, ST/J000434/1]; EU [238353]; RIKEN foreign postdoctoral research (FPR) grant; Natural Sciences and Engineering Research Council of Canada; [26400261] FX The generation of the 483 x 96 and 643 x 128 Mobius DWF + Iwasaki ensembles was performed using the IBM Blue Gene/Q (BG/Q) "Mira" machines at the Argonne Leadership Class Facility (ALCF) provided under the Incite Program of the U.S. DOE, on the STFC funded "DiRAC" BG/Q system in the Advanced Computing Facility at the University of Edinburgh, and on the BG/Q machines at Brookhaven National Laboratory (BNL). The BG/Q computers of the RIKEN-BNL Research Center were used to generate the 323 x 64 fine 3.14 GeV ensemble. The DiRAC equipment was funded by BIS National E-infrastructure capital Grant No. ST/K000411/1, STFC capital Grant No. ST/H008845/1, and STFC DiRAC Operations Grants No. ST/K005804/1 and No. ST/K005790/1. DiRAC is part of the National E-Infrastructure. Most of the measurements were also performed on the DiRAC and Mira machines, with the remainder performed using the BG/Q computers at the BNL. The research leading to these results has also received funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013) ERC Grant Agreement No. 279757. The software used includes the CPS QCD code (http://qcdoc.phys.columbia.edu/cps.html), supported in part by the U.S. DOE SciDAC program; and the BAGEL (http://www2.ph.ed.ac.uk/similar to paboyle/bagel/Bagel.html) assembler kernel generator for high-performance optimized kernels and fermion solvers [64]. The gauge fixing for the 48I ensemble was performed using the CUTH cluster at Columbia University using the "GLU" (Gauge Link Utility) codebase (https://github.com/RJhudspith/GLU). T. B. is supported by U.S. DOE Grant No. DE-FG02-92ER41989. G. M., N. H. C., R. D. M., and D. J. M. are supported in part by U.S. DOE Grant No. DE-SC0011941. A. S., C. J., T. I., and C. L. are supported in part by U.S. DOE Contract No. AC-02-98CH10886 (BNL). T. I. is also supported by Grants-in-Aid for Scientific Research No. 26400261. C. T. S., T. J., and A. P. acknowledge the STFC Grants No. ST/J000396/1 and No. ST/L000296/1. P. A. B., R. D. K., N. G., and J. F. acknowledge support from STFC Grants No. ST/L000458/1 and No. ST/J000329/1. N. G. also acknowledges support from STFC under the Grant No. ST/J000434/1 and from the EU Grant Agreement No. 238353 (ITN STRONGnet). C. K. is supported by a RIKEN foreign postdoctoral research (FPR) grant. R. J. H. is supported by the Natural Sciences and Engineering Research Council of Canada. NR 75 TC 19 Z9 19 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 12 PY 2016 VL 93 IS 7 AR 074505 DI 10.1103/PhysRevD.93.074505 PG 68 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI8SE UT WOS:000373770700002 ER PT J AU Sorokovikova, A Arefiev, AV McGuffey, C Qiao, B Robinson, APL Wei, MS McLean, HS Beg, FN AF Sorokovikova, A. Arefiev, A. V. McGuffey, C. Qiao, B. Robinson, A. P. L. Wei, M. S. McLean, H. S. Beg, F. N. TI Generation of Superponderomotive Electrons in Multipicosecond Interactions of Kilojoule Laser Beams with Solid-Density Plasmas SO PHYSICAL REVIEW LETTERS LA English DT Article ID PARTICLE-ACCELERATION; PHYSICS; REGIME AB The interaction of a multipicosecond, kilojoule laser pulse with a surface of a solid target has been shown to produce electrons with energies far beyond the free-electron ponderomotive limit m(e)c(2)a(0)(2)/2. Particle-in-cell simulations indicate that an increase in the pulse duration from 1 to 10 ps leads to the formation of a low-density shelf (about 10% of the critical density). The shelf extends over 100 mu m toward the vacuum side, with a nonstationary potential barrier forming in that area. Electrons reflected from the barrier gain superponderomotive energy from the potential. Some electrons experience an even greater energy gain due to ponderomotive acceleration when their "dephasing rate" R = gamma - p(x)/m(e)c drops well below unity, thus increasing acceleration by a factor of 1/R. Both 1D and 2D simulations indicate that these mechanisms are responsible for the generation of extensive thermal distributions with T-e > 10 MeV and a high-energy cutoff of hundreds of MeV. C1 [Sorokovikova, A.; McGuffey, C.; Qiao, B.; Beg, F. N.] Univ Calif San Diego, Ctr Energy Res, La Jolla, CA 92093 USA. [Arefiev, A. V.] Univ Texas Austin, Inst Fus Studies, Austin, TX 78712 USA. [Robinson, A. P. L.] STFC Rutherford Appleton Lab, Cent Laser Facil, Didcot OX11 0QX, Oxon, England. [Wei, M. S.] Gen Atom Co, San Diego, CA 92186 USA. [McLean, H. S.] Lawrence Livermore Natl Lab, Livermore, CA 94511 USA. RP McGuffey, C (reprint author), Univ Calif San Diego, Ctr Energy Res, La Jolla, CA 92093 USA. EM cmcguffey@ucsd.edu; fbeg@ucsd.edu RI Arefiev, Alexey/A-8550-2016; Qiao, Bin/I-2471-2016 OI Arefiev, Alexey/0000-0002-0597-0976; Qiao, Bin/0000-0001-7174-5577 FU U.S. DOE [DE-NA0000870, DE-FG02-05ER54834, DE-FC02-04ER54789, DE-NA0002008, DE-FG02-04ER54742]; United Kingdom EPSRC [EP/G054940/1, EP/G055165/1, EP/G056803/1] FX This work was performed under the auspices of U.S. DOE under Contracts No. DE-NA0000870, No. DE-FG02-05ER54834, and No. DE-FC02-04ER54789. Simulations were performed using the EPOCH code (developed under United Kingdom EPSRC Grants No. EP/G054940/1, No. EP/G055165/1, and No. EP/G056803/1) using HPC resources provided by the TACC at the University of Texas. A. V. A. was supported by the U.S. DOE through Agreements No. DE-NA0002008 and No. DE-FG02-04ER54742. NR 32 TC 3 Z9 3 U1 8 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 12 PY 2016 VL 116 IS 15 AR 155001 DI 10.1103/PhysRevLett.116.155001 PG 5 WC Physics, Multidisciplinary SC Physics GA DI8TC UT WOS:000373773600012 PM 27127972 ER PT J AU Sun, J Jiang, X Lund, R Downing, KH Balsara, NP Zuckermann, RN AF Sun, Jing Jiang, Xi Lund, Reidar Downing, Kenneth H. Balsara, Nitash P. Zuckermann, Ronald N. TI Self-assembly of crystalline nanotubes from monodisperse amphiphilic diblock copolypeptoid tiles SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE peptoid polymers; sequence-defined polymers; supramolecular assembly; polymer amphiphiles; peptoid nanostructures ID BLOCK-COPOLYMERS; PEPTOID POLYMERS; PEPTIDE NANOTUBES; CRYO-TEM; MICELLES; POLYETHYLENE; WATER; POLYPEPTOIDS; TOMOGRAPHY; SEPARATION AB The folding and assembly of sequence-defined polymers into precisely ordered nanostructures promises a class of well-defined biomimetic architectures with specific function. Amphiphilic diblock copolymers are known to self-assemble in water to form a variety of nanostructured morphologies including spheres, disks, cylinders, and vesicles. In all of these cases, the predominant driving force for assembly is the formation of a hydrophobic core that excludes water, whereas the hydrophilic blocks are solvated and extend into the aqueous phase. However, such polymer systems typically have broad molar mass distributions and lack the purity and sequence-defined structure often associated with biologically derived polymers. Here, we demonstrate that purified, monodisperse amphiphilic diblock copolypeptoids, with chemically distinct domains that are congruent in size and shape, can behave like molecular tile units that spontaneously assemble into hollow, crystalline nanotubes in water. The nanotubes consist of stacked, porous crystalline rings, and are held together primarily by side-chain van der Waals interactions. The peptoid nanotubes form without a central hydrophobic core, chirality, a hydrogen bond network, and electrostatic or pi-pi interactions. These results demonstrate the remarkable structure-directing influence of n-alkane and ethyleneoxy side chains in polymer self-assembly. More broadly, this work suggests that flexible, low-molecular-weight sequence-defined polymers can serve as molecular tile units that can assemble into precision supramolecular architectures. C1 [Sun, Jing; Zuckermann, Ronald N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Jiang, Xi; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Lund, Reidar] Univ Oslo, Dept Chem, N-0315 Oslo, Norway. [Downing, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Zuckermann, RN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM rnzuckermann@lbl.gov RI Lund, Reidar/F-3534-2014 FU Soft Matter Electron Microscopy Program; Office of Science, Office of Basic Energy Science, US Department of Energy [DE-AC02-05CH11231]; Norwegian Research Council, under the SYNKNOYT Program [218411, 228573]; Peder Sather Center for Advanced Study; NIH [GM51487] FX Funding for this work was provided by the Soft Matter Electron Microscopy Program, supported by the Office of Science, Office of Basic Energy Science, US Department of Energy, under Contract DE-AC02-05CH11231. Work at the Molecular Foundry and the Advanced Light Source at Lawrence Berkeley National Laboratory was supported by the Office of Science, Office of Basic Energy Science, US Department of Energy, under Contract DE-AC02-05CH11231. R.L. acknowledges grants from the Norwegian Research Council, under the SYNKNOYT Program (218411 and 228573), and a travel grant from the Peder Sather Center for Advanced Study. Cryo-EM facilities are supported by NIH Grant GM51487. The European Synchrotron Radiation Facility is acknowledged for allocation of beam time at the BM29 bioSAXS instrument. NR 45 TC 4 Z9 4 U1 13 U2 52 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 12 PY 2016 VL 113 IS 15 BP 3954 EP 3959 DI 10.1073/pnas.1517169113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PG UT WOS:000373762400032 PM 27035944 ER PT J AU Kaya, E Doxzen, KW Knoll, KR Wilson, RC Strutt, SC Kranzusch, PJ Doudna, JA AF Kaya, Emine Doxzen, Kevin W. Knoll, Kilian R. Wilson, Ross C. Strutt, Steven C. Kranzusch, Philip J. Doudna, Jennifer A. TI A bacterial Argonaute with noncanonical guide RNA specificity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE Argonaute; small noncoding RNA; RNA interference ID STRUCTURAL BASIS; TARGET RECOGNITION; SILENCING COMPLEX; CRYSTAL-STRUCTURE; IMMUNE-SYSTEM; DNA; INTERFERENCE; PROTEINS; PROKARYOTES; SEQUENCE AB Eukaryotic Argonaute proteins induce gene silencing by small RNA-guided recognition and cleavage of mRNA targets. Although structural similarities between human and prokaryotic Argonautes are consistent with shared mechanistic properties, sequence and structure-based alignments suggested that Argonautes encoded within CRISPR-cas [clustered regularly interspaced short palindromic repeats (CRISPR)-associated] bacterial immunity operons have divergent activities. We show here that the CRISPR-associated Marinitoga piezophila Argonaute (MpAgo) protein cleaves single-stranded target sequences using 5'-hydroxylated guide RNAs rather than the 5'-phosphorylated guides used by all known Argonautes. The 2.0-angstrom resolution crystal structure of an MpAgo-RNA complex reveals a guide strand binding site comprising residues that block 5' phosphate interactions. Using structure-based sequence alignment, we were able to identify other putative MpAgo-like proteins, all of which are encoded within CRISPR-cas loci. Taken together, our data suggest the evolution of an Argonaute subclass with noncanonical specificity for a 5'-hydroxylated guide. C1 [Kaya, Emine; Knoll, Kilian R.; Wilson, Ross C.; Strutt, Steven C.; Kranzusch, Philip J.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Kaya, Emine; Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Doxzen, Kevin W.; Doudna, Jennifer A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Kranzusch, Philip J.; Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Knoll, Kilian R.] Univ Munich, Dept Biochem, Gene Ctr, D-81377 Munich, Germany. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU German Academic Exchange Program; National Science Foundation FX We thank Dr. Kenneth Noll (Department of Molecular and Cell Biology, University of Connecticut) for providing M. piezophila cells; Akshay Tambe, Nicolas Bray, and Megan Hochstrasser for helpful discussions; and J. Holton, G. Meigs, and A. Gonzalez for technical assistance with data collection and processing. We thank the staff at beamline 8.3.1 of the Advanced Light Source at Lawrence Berkeley National Laboratory for crystallographic data collection. E.K. was funded by the German Academic Exchange Program, and K.W.D. acknowledges support from the National Science Foundation Graduate Research Fellowship Program. P.J.K. is supported as a Howard Hughes Medical Institute (HHMI) Fellow of the Life Sciences Research Foundation. This work was supported in part by a grant from the National Science Foundation (to J.A.D.). J.A.D. is an HHMI Investigator. NR 48 TC 3 Z9 3 U1 6 U2 36 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 12 PY 2016 VL 113 IS 15 BP 4057 EP 4062 DI 10.1073/pnas.1524385113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PG UT WOS:000373762400050 PM 27035975 ER PT J AU Van Benschoten, AH Liu, L Gonzalez, A Brewster, AS Sauter, NK Fraser, JS Wall, ME AF Van Benschoten, Andrew H. Liu, Lin Gonzalez, Ana Brewster, Aaron S. Sauter, Nicholas K. Fraser, James S. Wall, Michael E. TI Measuring and modeling diffuse scattering in protein X-ray crystallography SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE protein dynamics; normal modes; structural biology; diffuse scattering; liquid-like motions ID RIGID-BODY MOTION; MOLECULAR-DYNAMICS SIMULATIONS; ELASTIC NETWORK MODELS; STAPHYLOCOCCAL NUCLEASE; CRYSTALLINE PROTEIN; LYSOZYME CRYSTALS; REFINEMENT; RESOLUTION; ENSEMBLES; DISORDER AB X-ray diffraction has the potential to provide rich information about the structural dynamics of macromolecules. To realize this potential, both Bragg scattering, which is currently used to derive macromolecular structures, and diffuse scattering, which reports on correlations in charge density variations, must be measured. Until now, measurement of diffuse scattering from protein crystals has been scarce because of the extra effort of collecting diffuse data. Here, we present 3D measurements of diffuse intensity collected from crystals of the enzymes cyclophilin A and trypsin. The measurements were obtained from the same X-ray diffraction images as the Bragg data, using best practices for standard data collection. To model the underlying dynamics in a practical way that could be used during structure refinement, we tested translation-libration-screw (TLS), liquid-like motions (LLM), and coarse-grained normal-modes (NM) models of protein motions. The LLM model provides a global picture of motions and was refined against the diffuse data, whereas the TLS and NM models provide more detailed and distinct descriptions of atom displacements, and only used information from the Bragg data. Whereas different TLS groupings yielded similar Bragg intensities, they yielded different diffuse intensities, none of which agreed well with the data. In contrast, both the LLM and NM models agreed substantially with the diffuse data. These results demonstrate a realistic path to increase the number of diffuse datasets available to the wider biosciences community and indicate that dynamics-inspired NM structural models can simultaneously agree with both Bragg and diffuse scattering. C1 [Van Benschoten, Andrew H.; Liu, Lin; Fraser, James S.] Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, San Francisco, CA 94158 USA. [Gonzalez, Ana] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Brewster, Aaron S.; Sauter, Nicholas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Wall, Michael E.] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, POB 1663, Los Alamos, NM 87545 USA. RP Fraser, JS (reprint author), Univ Calif San Francisco, Dept Bioengn & Therapeut Sci, San Francisco, CA 94158 USA.; Wall, ME (reprint author), Los Alamos Natl Lab, Comp Computat & Stat Sci Div, POB 1663, Los Alamos, NM 87545 USA. EM jfraser@fraserlab.com; mewall@lanl.gov RI Sauter, Nicholas/K-3430-2012; OI Alexandrov, Ludmil/0000-0003-3596-4515 FU University of California, Office of the President, Multicampus Research Programs and Initiatives Grant [MR-15-338599]; Sandler Foundation; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; US Department of Energy Office of Biological and Environmental Research; NIH, National Institute of General Medical Sciences [P41GM103393]; NIH [GM095887, OD009180, GM110580]; Searle Scholar Award from the Kinship Foundation; Pew Scholar Award from the Pew Charitable Trusts; Packard Fellowship from the David and Lucile Packard Foundation; National Science Foundation [STC-1231306]; US Department of Energy through the Laboratory-Directed Research and Development Program at Los Alamos National Laboratory (LANL) [DE-AC52-06NA25396] FX We thank Pavel Afonine for computational assistance in converting and comparing structure factors. We are grateful to the University of California, Office of the President, Multicampus Research Programs and Initiatives Grant MR-15-338599, and the Program for Breakthrough Biomedical Research, which is partially funded by the Sandler Foundation. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. The Stanford Synchrotron Radiation Lightsource Structural Molecular Biology Program is supported by the US Department of Energy Office of Biological and Environmental Research, and by the NIH, National Institute of General Medical Sciences (including P41GM103393). N.K.S. was supported by NIH Grant GM095887. J.S.F. was supported by a Searle Scholar Award from the Kinship Foundation, a Pew Scholar Award from the Pew Charitable Trusts, a Packard Fellowship from the David and Lucile Packard Foundation, NIH Grant OD009180, NIH Grant GM110580, and National Science Foundation Grant STC-1231306. M.E.W. was supported by the US Department of Energy under Contract DE-AC52-06NA25396 through the Laboratory-Directed Research and Development Program at Los Alamos National Laboratory (LANL). The LANL technical release number is LA-UR-15-28934. NR 67 TC 2 Z9 2 U1 5 U2 16 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 12 PY 2016 VL 113 IS 15 BP 4069 EP 4074 DI 10.1073/pnas.1524048113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PG UT WOS:000373762400052 PM 27035972 ER PT J AU Alexander, WG Wisecaver, JH Rokas, A Hittinger, CT AF Alexander, William G. Wisecaver, Jennifer H. Rokas, Antonis Hittinger, Chris Todd TI Horizontally acquired genes in early-diverging pathogenic fungi enable the use of host nucleosides and nucleotides SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE horizontal gene transfer; Microsporidia; Cryptomycota; thymidine kinase; metabolic networks ID PARASITE ENCEPHALITOZOON-CUNICULI; MULTIPLE SEQUENCE ALIGNMENT; TYPE-1 THYMIDINE KINASE; INTRACELLULAR PARASITES; PHYLOGENETIC ANALYSES; ADAPTIVE EVOLUTION; GENOME; SACCHAROMYCES; MICROSPORIDIA; EUKARYOTES AB Horizontal gene transfer (HGT) among bacteria, archaea, and viruses is widespread, but the extent of transfers from these lineages into eukaryotic organisms is contentious. Here we systematically identify hundreds of genes that were likely acquired horizontally from a variety of sources by the early-diverging fungal phyla Microsporidia and Cryptomycota. Interestingly, the Microsporidia have acquired via HGT several genes involved in nucleic acid synthesis and salvage, such as those encoding thymidine kinase (TK), cytidylate kinase, and purine nucleotide phosphorylase. We show that these HGT-derived nucleic acid synthesis genes tend to function at the interface between the metabolic networks of the host and pathogen. Thus, these genes likely play vital roles in diversifying the useable nucleic acid components available to the intracellular parasite, often through the direct capture of resources from the host. Using an in vivo viability assay, we also demonstrate that one of these genes, TK, encodes an enzyme that is capable of activating known prodrugs to their active form, which suggests a possible treatment route for microsporidiosis. We further argue that interfacial genes with well-understood activities, especially those horizontally transferred from bacteria or viruses, could provide medical treatments for microsporidian infections. C1 [Alexander, William G.; Hittinger, Chris Todd] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, JF Crow Inst Study Evolut,Genome Ctr Wisconsin, Lab Genet,DOE Dept Energy,Wisconsin Energy Inst, Madison, WI 53706 USA. [Wisecaver, Jennifer H.; Rokas, Antonis] Vanderbilt Univ, Dept Biol Sci, 221 Kirkland Hall, Nashville, TN 37235 USA. RP Hittinger, CT (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, JF Crow Inst Study Evolut,Genome Ctr Wisconsin, Lab Genet,DOE Dept Energy,Wisconsin Energy Inst, Madison, WI 53706 USA. EM cthittinger@wisc.edu OI Rokas, Antonis/0000-0002-7248-6551 FU National Science Foundation [IOS-1401682, DEB-1442113, DEB-1253634, DEB-1442148]; DOE Great Lakes Bioenergy Research Center through DOE Office of Science [BER DE-FC02-07ER64494]; USDA (United States Department of Agriculture) National Institute of Food and Agriculture Hatch Project [1003258]; Alexander von Humboldt Foundation; Pew Charitable Trusts FX We thank Issac Knoflicek, Michael G. Mangiore, and Dana Opulente for computational support and advice and Amanda B. Hulfachor for artwork. This work was conducted in part using the resources of the Advanced Computing Center for Research and Education at Vanderbilt University. This material is based upon work supported by National Science Foundation Grants IOS-1401682 (to J.H.W.), DEB-1442113 (to A.R.), and DEB-1253634 and DEB-1442148 (to C.T.H.); in part by the DOE Great Lakes Bioenergy Research Center through DOE Office of Science Grant BER DE-FC02-07ER64494; and USDA (United States Department of Agriculture) National Institute of Food and Agriculture Hatch Project 1003258. C.T.H. is an Alfred Toepfer Faculty Fellow and Pew Scholar in the Biomedical Sciences, supported by the Alexander von Humboldt Foundation and Pew Charitable Trusts, respectively. NR 60 TC 1 Z9 1 U1 9 U2 14 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 12 PY 2016 VL 113 IS 15 BP 4116 EP 4121 DI 10.1073/pnas.1517242113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PG UT WOS:000373762400060 PM 27035945 ER PT J AU Levitz, J Royal, P Comoglio, Y Wdziekonski, B Schaub, S Clemens, DM Isacoff, EY Sandoz, G AF Levitz, Joshua Royal, Perrine Comoglio, Yannick Wdziekonski, Brigitte Schaub, Sebastien Clemens, Daniel M. Isacoff, Ehud Y. Sandoz, Guillaume TI Heterodimerization within the TREK channel subfamily produces a diverse family of highly regulated potassium channels SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE potassium channels; single-molecule fluorescence; leak current; combinatorial diversity; heteromerization ID POLYUNSATURATED FATTY-ACIDS; K+ CHANNEL; TRAAK; ACTIVATION; LYSOPHOSPHOLIPIDS; LOCALIZATION; EXPRESSION; PRESSURE; SUBUNITS; COMPLEX AB Twik-related K+ channel 1 (TREK1), TREK2, and Twik-related arachidonic-acid stimulated K+ channel (TRAAK) form the TREK subfamily of two-pore-domain K+ (K-2P) channels. Despite sharing up to 78% sequence homology and overlapping expression profiles in the nervous system, these channels show major differences in their regulation by physiological stimuli. For instance, TREK1 is inhibited by external acidification, whereas TREK2 is activated. Here, we investigated the ability of the members of the TREK subfamily to assemble to form functional heteromeric channels with novel properties. Using single-molecule pull-down (SiMPull) from HEK cell lysate and subunit counting in the plasma membrane of living cells, we show that TREK1, TREK2, and TRAAK readily coassemble. TREK1 and TREK2 can each heterodimerize with TRAAK, but do so less efficiently than with each other. We functionally characterized the heterodimers and found that all combinations form outwardly rectifying potassium-selective channels but with variable voltage sensitivity and pH regulation. TREK1-TREK2 heterodimers show low levels of activity at physiological external pH but, unlike their corresponding homodimers, are activated by both acidic and alkaline conditions. Modeling based on recent crystal structures, along with mutational analysis, suggests that each subunit within a TREK1-TREK2 channel is regulated independently via titratable His. Finally, TREK1/TRAAK heterodimers differ in function from TRAAK homodimers in two critical ways: they are activated by both intracellular acidification and alkalinization and are regulated by the enzyme phospholipase D2. Thus, heterodimerization provides a means for diversifying functionality through an expansion of the channel types within the K-2P channels. C1 [Levitz, Joshua; Clemens, Daniel M.; Isacoff, Ehud Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Levitz, Joshua; Clemens, Daniel M.; Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Royal, Perrine; Comoglio, Yannick; Wdziekonski, Brigitte; Schaub, Sebastien; Sandoz, Guillaume] Univ Nice Sophia Antipolis, Inst Biol Valrose iBV, UMR 7277, F-06100 Nice, France. [Royal, Perrine; Comoglio, Yannick; Wdziekonski, Brigitte; Schaub, Sebastien; Sandoz, Guillaume] CNRS, iBV, UMR 7277, F-06100 Nice, France. [Royal, Perrine; Comoglio, Yannick; Wdziekonski, Brigitte; Schaub, Sebastien; Sandoz, Guillaume] INSERM, iBV, F-06100 Nice, France. [Royal, Perrine; Comoglio, Yannick; Wdziekonski, Brigitte; Sandoz, Guillaume] Labs Excellence Ion Channel Sci & Therapeut, Nice, France. [Isacoff, Ehud Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Sandoz, G (reprint author), Univ Nice Sophia Antipolis, Inst Biol Valrose iBV, UMR 7277, F-06100 Nice, France.; Sandoz, G (reprint author), CNRS, iBV, UMR 7277, F-06100 Nice, France.; Sandoz, G (reprint author), INSERM, iBV, F-06100 Nice, France.; Sandoz, G (reprint author), Labs Excellence Ion Channel Sci & Therapeut, Nice, France. EM sandoz@unice.fr OI Sandoz, Guillaume/0000-0003-1251-0852 FU Action Thematique et Incitative sur Programme-AVENIR (ATIP-AVENIR) funds; French National Center for Scientific Research; Fondation NRJ-Institut de France; Agence Nationale de la Recherche (ANR) (Laboratory of Excellence "Ion Channel Science and Therapeutics) [ANR-11-LABX-0015-01]; ANR Dynaselect [ANR-14-CE13-0010]; National Science Foundation [IOS-1451027]; NIH [R01NS35549]; Chateaubriand fellowship FX We thank S. Bharill, M. Ulbrich, and O. Soriani for technical assistance and helpful discussion. The work was supported by a grant (to G.S.) by the Action Thematique et Incitative sur Programme-AVENIR (ATIP-AVENIR) funds and the French National Center for Scientific Research, as well as by grants (to G.S.) from the Fondation NRJ-Institut de France, Agence Nationale de la Recherche (ANR) (Laboratory of Excellence "Ion Channel Science and Therapeutics," Grant ANR-11-LABX-0015-01), and ANR Dynaselect (Grant ANR-14-CE13-0010); by grants (to E.Y.I.) from the National Science Foundation (Grant IOS-1451027) and NIH (Grant R01NS35549); and by a Chateaubriand fellowship (to J.L.). NR 35 TC 3 Z9 3 U1 3 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD APR 12 PY 2016 VL 113 IS 15 BP 4194 EP 4199 DI 10.1073/pnas.1522459113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PG UT WOS:000373762400073 PM 27035963 ER PT J AU Wu, HC Kumar, A Wang, J Bi, XF Tome, CN Zhang, Z Mao, SX AF Wu, H. C. Kumar, A. Wang, J. Bi, X. F. Tome, C. N. Zhang, Z. Mao, S. X. TI Rolling-induced Face Centered Cubic Titanium in Hexagonal Close Packed Titanium at Room Temperature SO SCIENTIFIC REPORTS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; HIGH-PRESSURE TORSION; PHASE-TRANSFORMATION; INTERFACE DEFECTS; BASIS-SET; METALS; ALLOYS; HCP; DISLOCATIONS AB Combining transmission electron microscopes and density functional theory calculations, we report the nucleation and growth mechanisms of room temperature rolling induced face-centered cubic titanium (fcc-Ti) in polycrystalline hexagonal close packed titanium (hcp-Ti). Fcc-Ti and hcp-Ti take the orientation relation: < 0001 >(hcp)parallel to < 001 >(fcc) and {10 (1) over bar0}(hcp)parallel to{110}(fcc), different from the conventional one. The nucleation of fcc-Ti is accomplished via pure-shuffle mechanism with a minimum stable thickness of three atomic layers, and the growth via shear-shuffle mechanisms through gliding two-layer disconnections or pure-shuffle mechanisms through gliding four-layer disconnections. Such phase transformation offers an additional plastic deformation mode comparable to twinning. C1 [Wu, H. C.; Bi, X. F.] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Kumar, A.; Tome, C. N.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Wang, J.] Univ Nebraska, Mech & Mat Engn, Lincoln, NE 68588 USA. [Zhang, Z.] Zhejiang Univ, State Key Lab Si Mat, Dept Mat Sci, Hangzhou 310003, Zhejiang, Peoples R China. [Mao, S. X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. RP Bi, XF (reprint author), Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China.; Wang, J (reprint author), Univ Nebraska, Mech & Mat Engn, Lincoln, NE 68588 USA.; Mao, SX (reprint author), Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. EM jianwang@unl.edu; bixf@buaa.edu.cn; sxm2@pitt.edu RI Kumar, Anil /H-4345-2016; Kumar, Anil/A-9834-2013; Wang, Jian/F-2669-2012 OI Kumar, Anil/0000-0002-4901-8987; Wang, Jian/0000-0001-5130-300X FU National Natural Science Foundation of China [61271043]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [FWP 06SCPE401]; NSF through University of Pittsburgh [CMMI 08 010934] FX BXF acknowledges support of National Natural Science Foundation of China (61271043). JW, AK, and CNT acknowledge the support provided by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, FWP 06SCPE401. SXM would like to acknowledge NSF CMMI 08 010934 through University of Pittsburgh. HCW would like to acknowledge the assistance from Center of Electron Microscope, Zhejiang University, especially the assistance of Mr. Zeng Yaowu, Hong Jinhua and Yuan Wentao. NR 37 TC 2 Z9 2 U1 8 U2 24 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 12 PY 2016 VL 6 AR 24370 DI 10.1038/srep24370 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8QD UT WOS:000373764900001 PM 27067515 ER PT J AU Anderson, TJ Ryu, S Zhou, H Xie, L Podkaminer, JP Ma, Y Irwin, J Pan, XQ Rzchowski, MS Eom, CB AF Anderson, T. J. Ryu, S. Zhou, H. Xie, L. Podkaminer, J. P. Ma, Y. Irwin, J. Pan, X. Q. Rzchowski, M. S. Eom, C. B. TI Metastable honeycomb SrTiO3/SrIrO3 heterostructures SO APPLIED PHYSICS LETTERS LA English DT Article ID SRIRO3 FILMS; GROWTH; METAL AB Recent theory predictions of exotic band topologies in (111) honeycomb perovskite SrIrO3 layers sandwiched between SrTiO3 have garnered much attention in the condensed matter physics and materials communities. However, perovskite SrIrO3 film growth in the (111) direction remains unreported, as efforts to synthesize pure SrIrO3 on (111) perovskite substrates have yielded films with monoclinic symmetry rather than the perovskite structure required by theory predictions. In this study, we report the synthesis of ultra-thin metastable perovskite SrIrO3 films capped with SrTiO3 grown on (111) SrTiO3 substrates by pulsed laser deposition. The atomic structure of the ultra-thin films was examined with scanning transmission electron microscopy (STEM), which suggests a perovskite layering distinct from the bulk SrIrO3 monoclinic phase. In-plane 3-fold symmetry for the entire heterostructure was confirmed using synchrotron surface X-ray diffraction to measure symmetry equivalent crystal truncation rods. Our findings demonstrate the ability to stabilize (111) honeycomb perovskite SrIrO3, which provides an experimental avenue to probe the phenomena predicted for this material system. Published by AIP Publishing. C1 [Anderson, T. J.; Ryu, S.; Podkaminer, J. P.; Ma, Y.; Eom, C. B.] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Zhou, H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Xie, L.; Pan, X. Q.] Univ Calif Irvine, Dept Chem Engn & Mat Sci, Irvine, CA 92697 USA. [Xie, L.; Pan, X. Q.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Xie, L.] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Xie, L.] Nanjing Univ, Coll Engn & Appl Sci, Nanjing 210093, Jiangsu, Peoples R China. [Irwin, J.; Rzchowski, M. S.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. RP Eom, CB (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM eom@engr.wisc.edu OI Irwin, Julian/0000-0002-4845-7558 FU National Science Foundation under DMREF Grant [DMR-1234096]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This research was supported by the National Science Foundation under DMREF Grant No. DMR-1234096.; This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 20 TC 2 Z9 2 U1 20 U2 59 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 151604 DI 10.1063/1.4947006 PG 5 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000012 ER PT J AU Chambers, SA Kaspar, TC Prakash, A Haugstad, G Jalan, B AF Chambers, Scott A. Kaspar, Tiffany C. Prakash, Abhinav Haugstad, Greg Jalan, Bharat TI Band alignment at epitaxial BaSnO3/SrTiO3(001) and BaSnO3/LaAlO3(001) heterojunctions SO APPLIED PHYSICS LETTERS LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; PRECISE DETERMINATION; CORE-LEVEL; PEROVSKITE; SPECTRA AB We have spectroscopically determined the optical bandgaps and band offsets at epitaxial interfaces of BaSnO3 with SrTiO3(001) and LaAlO3(001). 28 u.c. BaSnO3 epitaxial films exhibit direct and indirect bandgaps of 3.56 +/- 0.05 eV and 2.93 +/- 0.05 eV, respectively. The lack of a significant Burstein-Moss shift corroborates the highly insulating, defect-free nature of the BaSnO3 films. The conduction band minimum is lower in electron energy in 5 u.c. films of BaSnO3 than in SrTiO3 and LaAlO3 by 0.4 +/- 0.2 eV and 3.7 +/- 0.2 eV, respectively. This result bodes well for the realization of oxide-based, high-mobility, two-dimensional electron systems that can operate at ambient temperature, since electrons generated in the SrTiO3 by modulation doping, or at the BaSnO3/LaAlO3 interface by polarization doping, can be transferred to and at least partially confined in the BaSnO3 film. Published by AIP Publishing. C1 [Chambers, Scott A.; Kaspar, Tiffany C.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Prakash, Abhinav; Jalan, Bharat] Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. [Haugstad, Greg] Univ Minnesota, Characterizat Facil, Minneapolis, MN 55455 USA. RP Chambers, SA (reprint author), Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA.; Jalan, B (reprint author), Univ Minnesota, Dept Chem Engn & Mat Sci, 421 Washington Ave SE, Minneapolis, MN 55455 USA. EM sa.chambers@pnnl.gov; bjalan@umn.edu OI PRAKASH, ABHINAV/0000-0002-8899-0568 FU National Science Foundation [DMR-1410888]; MRSEC [DMR-1420013]; NSF through the MRSEC program; U.S. Department of Energy, Office of Science, Division of Materials Sciences and Engineering [10122]; Department of Energy's Office of Biological and Environmental Research FX The thin film growth and characterization work at the University of Minnesota was supported primarily by the National Science Foundation through DMR-1410888 and, in part, by the MRSEC under Award No. # DMR-1420013. We also acknowledge use of facilities at the UMN Minnesota Nano Center. Parts of this work were carried out in the Characterization Facility, University of Minnesota, which receives partial support from NSF through the MRSEC program. The XPS and SE work at PNNL was supported by the U.S. Department of Energy, Office of Science, Division of Materials Sciences and Engineering under Award No. #10122. The PNNL work was performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. NR 23 TC 7 Z9 7 U1 4 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 152104 DI 10.1063/1.4946762 PG 4 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000020 ER PT J AU Chen, YB Zhang, S Gao, WW Ke, F Yan, JY Saha, B Ko, CH Suh, J Chen, B Ager, JW Walukiewicz, W Jeanloz, R Wu, JQ AF Chen, Yabin Zhang, Shuai Gao, Weiwei Ke, Feng Yan, Jinyuan Saha, Bivas Ko, Changhyun Suh, Joonki Chen, Bin Ager, Joel W., III Walukiewicz, Wladek Jeanloz, Raymond Wu, Junqiao TI Pressure-induced structural transition of CdxZn1-xO alloys SO APPLIED PHYSICS LETTERS LA English DT Article ID ROCK-SALT ZNO; TOTAL-ENERGY CALCULATIONS; X-RAY-DIFFRACTION; WAVE BASIS-SET; OPTICAL-PROPERTIES; PHASE-TRANSITIONS; WURTZITE AB CdxZn1-xO alloys, as a transparent conducting oxide, have recently attracted much attention for potential optoelectronic applications. In this letter, we report a hydrostatic pressure-induced phase transition of CdxZn1-xO alloys from the wurtzite to the rocksalt structure and its phase diagram probed using a diamond anvil cell. It is found that the transition pressure, determined by changes in optical and structural properties, depends sensitively on the composition. As the Cd content increases, the critical pressure decreases, until at x = 0.67 where the alloy is intrinsically stable in the rocksalt phase even at ambient pressure. The wurtzite phase is light emitting with a direct bandgap that slightly widens with increasing pressure, while the rocksalt phase has a much wider bandgap that is indirect. The pressure-sensitive light emission and phase transition may find potential applications in fields such as stress sensing and energy storage. Published by AIP Publishing. C1 [Chen, Yabin; Saha, Bivas; Ko, Changhyun; Suh, Joonki; Ager, Joel W., III; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Zhang, Shuai; Jeanloz, Raymond] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Gao, Weiwei; Ager, Joel W., III; Walukiewicz, Wladek; Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ke, Feng; Chen, Bin] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Yan, Jinyuan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Wu, JQ (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Wu, JQ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM wuj@berkeley.edu RI Ko, Changhyun/E-1686-2011; Wu, Junqiao/G-7840-2011; OI Wu, Junqiao/0000-0002-1498-0148; Zhang, Shuai/0000-0001-9503-4964 FU Electronic Materials Program at the Lawrence Berkeley National Laboratory; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Singapore-Berkeley Research Initiative for Sustainable Energy (SinBeRISE); COMPRES [EAR 11-57758]; U.S. Department of Energy [DE-SC0010517] FX This work was supported by the Electronic Materials Program at the Lawrence Berkeley National Laboratory, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. J.W., J.W.A., and Y.C. acknowledge support from the Singapore-Berkeley Research Initiative for Sustainable Energy (SinBeRISE). The laser milling was supported by COMPRES (Grant No. EAR 11-57758). S.Z. was supported in part by the U.S. Department of Energy, Grant No. DE-SC0010517. Y.C. thanks Dr. F.B. Tian (Jilin University, China) for his helpful discussion on DFT simulations. NR 30 TC 1 Z9 1 U1 3 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 152105 DI 10.1063/1.4947022 PG 4 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000021 ER PT J AU Fleurence, A Gill, TG Friedlein, R Sadowski, JT Aoyagi, K Copel, M Tromp, RM Hirjibehedin, CF Yamada-Takamura, Y AF Fleurence, A. Gill, T. G. Friedlein, R. Sadowski, J. T. Aoyagi, K. Copel, M. Tromp, R. M. Hirjibehedin, C. F. Yamada-Takamura, Y. TI Single-domain epitaxial silicene on diboride thin films SO APPLIED PHYSICS LETTERS LA English DT Article AB Epitaxial silicene, which forms spontaneously on ZrB2(0001) thin films grown on Si(111) wafers, has a periodic stripe domain structure. By adsorbing additional Si atoms on this surface, we find that the domain boundaries vanish, and a single-domain silicene sheet can be prepared without altering its buckled honeycomb structure. The amount of Si required to induce this change suggests that the domain boundaries are made of a local distortion of the silicene honeycomb lattice. The realization of a single domain sheet with structural and electronic properties close to those of the original striped state demonstrates the high structural flexibility of silicene. (C) 2016 AIP Publishing LLC. C1 [Fleurence, A.; Gill, T. G.; Friedlein, R.; Aoyagi, K.; Yamada-Takamura, Y.] JAIST, Sch Mat Sci, 1-1 Asahidai, Nomi, Ishikawa 9231292, Japan. [Gill, T. G.; Hirjibehedin, C. F.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Gill, T. G.; Hirjibehedin, C. F.] UCL, Dept Chem, London WC1H 0AJ, England. [Hirjibehedin, C. F.] UCL, Dept Phys & Astron, Mortimer St, London WC1E 6BT, England. [Sadowski, J. T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Copel, M.; Tromp, R. M.] IBM Corp, Div Res, Thomas J Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Friedlein, R.] Meyer Burger Germany AG, BU MicroSyst, D-09337 Hohenstein Ernstthal, Germany. RP Fleurence, A (reprint author), JAIST, Sch Mat Sci, 1-1 Asahidai, Nomi, Ishikawa 9231292, Japan. EM antoine@jaist.ac.jp OI Hirjibehedin, Cyrus/0000-0003-1706-2147; Sadowski, Jerzy/0000-0002-4365-7796 FU U.S. DOE Office of Science User Facilities, at Brookhaven National Laboratory [DE-SC0012704]; JSPS KAKENHI Grant [26790005, 26246002]; Asahi Glass Foundation FX We are grateful for experimental help from K. Mase (Institute of Materials Structure Science, High Energy Accelerator Research Organization, Tsukuba, Japan) and A. Al-Mahboob (CFN, BNL). Part of this work has been performed under the approval of the Photon Factory Advisory Committee (Proposal No. 2012G610). This research used resources of the Center for Functional Nanomaterials and National Synchrotron Light Source, which are the U.S. DOE Office of Science User Facilities, at Brookhaven National Laboratory under Contract No. DE-SC0012704. This work was supported by JSPS KAKENHI Grant Nos. 26790005 and 26246002. A.F. acknowledges financial support from Asahi Glass Foundation; T.G. and C.F.H. from the UK Engineering and Physical Sciences Research Council (EP/H026622/1 and EP/G036675/1). NR 30 TC 3 Z9 3 U1 13 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 151902 DI 10.1063/1.4945370 PG 5 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000015 ER PT J AU Lawrie, BJ Yang, Y Eaton, M Black, AN Pooser, RC AF Lawrie, B. J. Yang, Y. Eaton, M. Black, A. N. Pooser, R. C. TI Robust and compact entanglement generation from diode-laser-pumped four-wave mixing SO APPLIED PHYSICS LETTERS LA English DT Article ID PODOLSKY-ROSEN ENTANGLEMENT; HOT RUBIDIUM VAPOR; SHOT-NOISE LIMIT; SQUEEZED STATES; LIGHT AB Four-wave-mixing processes are now routinely used to demonstrate multi-spatial-mode Einstein-Podolsky-Rosen entanglement and intensity difference squeezing. Diode-laser-pumped four-wave mixing processes have recently been shown to provide an affordable, compact, and stable source for intensity difference squeezing, but it was unknown if excess phase noise present in power amplifier pump configurations would be an impediment to achieving quadrature entanglement. Here, we demonstrate the operating regimes under which these systems are capable of producing entanglement and under which excess phase noise produced by the amplifier contaminates the output state. We show that Einstein-Podolsky-Rosen entanglement in two mode squeezed states can be generated by a four-wave-mixing source deriving both the pump field and the local oscillators from a tapered-amplifier diode-laser. This robust continuous variable entanglement source is highly scalable and amenable to miniaturization, making it a critical step toward the development of integrated quantum sensors and scalable quantum information processors, such as spatial comb cluster states. Published by AIP Publishing. C1 [Lawrie, B. J.; Yang, Y.; Eaton, M.; Black, A. N.; Pooser, R. C.] Oak Ridge Natl Lab, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. [Yang, Y.] Wabash Coll, Dept Phys, Crawfordsville, IN 47933 USA. [Eaton, M.] So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA. [Black, A. N.] Middle Tennessee State Univ, Dept Phys & Astron, Murfreesboro, TN 37132 USA. RP Lawrie, BJ (reprint author), Oak Ridge Natl Lab, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. EM lawriebj@ornl.gov OI Lawrie, Ben/0000-0003-1431-066X; Eaton, Miller/0000-0001-6374-5032; Pooser, Raphael/0000-0002-2922-453X FU U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the SULI program; Laboratory Directed Research and Development program FX This work was performed at Oak Ridge National Laboratory, operated by UT-Battelle for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725, and was supported in part by the U.S. Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the SULI program. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allows others to do so, for U.S. Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). B.L. and R.C.P acknowledge the support from the Laboratory Directed Research and Development program. NR 31 TC 3 Z9 3 U1 11 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 151107 DI 10.1063/1.4947026 PG 4 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000007 ER PT J AU Li, WQ Liu, XQ Wang, YQ Dai, ZG Wu, W Cheng, L Zhang, YP Liu, Q Xiao, XH Jiang, CZ AF Li, Wenqing Liu, Xinqiang Wang, Yongqiang Dai, Zhigao Wu, Wei Cheng, Li Zhang, Yupeng Liu, Qi Xiao, Xiangheng Jiang, Changzhong TI Design of high-performance memristor cell using W-implanted SiO2 films SO APPLIED PHYSICS LETTERS LA English DT Article ID RESISTIVE SWITCHING MEMORY; FORMING-FREE; OXIDE-FILMS; MECHANISMS; SIO2; CU AB Highly reproducible bipolar resistance switching was demonstrated in a composite material of W-implanted silicon dioxide. Because of its excellent dielectric properties, SiO2 was selected as the sole active material for fabricating the resistance switching devices. The device employed a metal-insulator-semiconductor structure, showing an excellent resistance switching performance (the ON/OFF ratio is close to similar to 10(6)). In addition, this sandwich structure device shows a forming-free resistance switching behavior. The overall device performance of the SiO2-based memristor has the potential to open up a new avenue to a large-scale high-performance resistive random access memory, which could significantly impact their existing applications. (C) 2016 AIP Publishing LLC. C1 [Li, Wenqing; Liu, Xinqiang; Dai, Zhigao; Wu, Wei; Cheng, Li; Zhang, Yupeng; Xiao, Xiangheng; Jiang, Changzhong] Wuhan Univ, Minist Educ, Dept Phys, Wuhan 430072, Peoples R China. [Li, Wenqing; Liu, Xinqiang; Dai, Zhigao; Wu, Wei; Cheng, Li; Zhang, Yupeng; Xiao, Xiangheng; Jiang, Changzhong] Wuhan Univ, Minist Educ, Key Lab Artificial Micro & Nanostruct, Wuhan 430072, Peoples R China. [Li, Wenqing; Liu, Xinqiang; Dai, Zhigao; Wu, Wei; Cheng, Li; Zhang, Yupeng; Xiao, Xiangheng; Jiang, Changzhong] Wuhan Univ, Hubei Nucl Solid Phys Key Lab, Wuhan 430072, Peoples R China. [Wang, Yongqiang] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Dai, Zhigao; Wu, Wei] Wuhan Univ, Sch Printing & Packaging, Lab Funct Nanomat & Printed Elect, Wuhan 430072, Peoples R China. [Liu, Qi] Chinese Acad Sci, Inst Microelect, Key Lab Microelect Devices & Integrated Techno, Beijing 100029, Peoples R China. [Xiao, Xiangheng] Su Zhou Inst Wuhan Univ, Suzhou 215123, Peoples R China. RP Li, WQ (reprint author), Wuhan Univ, Minist Educ, Dept Phys, Wuhan 430072, Peoples R China.; Li, WQ (reprint author), Wuhan Univ, Minist Educ, Key Lab Artificial Micro & Nanostruct, Wuhan 430072, Peoples R China.; Li, WQ (reprint author), Wuhan Univ, Hubei Nucl Solid Phys Key Lab, Wuhan 430072, Peoples R China. EM liuqi@ime.ac.cn; xxh@whu.edu.cn RI Zhang, Yupeng/J-8393-2012 OI Zhang, Yupeng/0000-0003-2351-5579 FU Wuhan Planning Project of Science and Technology [2014010101010019]; Fundamental Research Funds for the Central Universities [2042015kf1012] FX The author is thankful to the NSFC (51371131, 11375134, 51571153, and 61422407), NCET (12-0418), Jiangsu Provincial Natural Science Foundation (BK20141217), Wuhan Planning Project of Science and Technology (2014010101010019), and the Fundamental Research Funds for the Central Universities (2042015kf1012). NR 34 TC 5 Z9 5 U1 15 U2 47 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 153501 DI 10.1063/1.4945982 PG 5 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000057 ER PT J AU Struebing, C Chong, J Lee, G Zavala, M Erickson, A Ding, Y Wang, CL Diawara, Y Engels, R Wagner, B Kang, ZT AF Struebing, Christian Chong, JooYun Lee, Gyuhyon Zavala, Martin Erickson, Anna Ding, Yong Wang, Cai-Lin Diawara, Yacouba Engels, Ralf Wagner, Brent Kang, Zhitao TI A neutron scintillator based on transparent nanocrystalline CaF2: Eu glass ceramic SO APPLIED PHYSICS LETTERS LA English DT Article ID INORGANIC SCINTILLATORS AB There are no efficient Eu2+ doped glass neutron scintillators reported due to low doping concentrations of Eu2+ and the amorphous nature of the glass matrix. In this work, an efficient CaF2: Eu glass ceramic neutron scintillator was prepared by forming CaF2: Eu nanocrystals in a 6 Li-containing glass matrix. Through appropriate thermal treatments, the scintillation light yield of the transparent glass ceramic was increased by a factor of at least 46 compared to the as-cast amorphous glass. This improvement was attributed to more efficient energy transfer from the CaF2 crystals to the Eu2+ emitting centers. Further light yield improvement is expected if the refractive index of the glass matrix can be matched to the CaF2 crystal. Published by AIP Publishing. C1 [Struebing, Christian; Chong, JooYun; Wagner, Brent; Kang, Zhitao] Georgia Inst Technol, Georgia Tech Res Inst, Atlanta, GA 30332 USA. [Struebing, Christian; Lee, Gyuhyon; Ding, Yong; Kang, Zhitao] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Zavala, Martin; Erickson, Anna] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Wang, Cai-Lin; Diawara, Yacouba] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Engels, Ralf] Forschungszentrum Julich, D-52425 Julich, Germany. RP Kang, ZT (reprint author), Georgia Inst Technol, Georgia Tech Res Inst, Atlanta, GA 30332 USA.; Kang, ZT (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. EM zhitao.kang@gtri.gatech.edu RI Ding, Yong/F-3705-2017; OI Ding, Yong/0000-0001-5805-347X; Struebing, Christian/0000-0003-0795-6622 FU U.S. Department of Homeland Security [2014-DN-077-ARI085-01]; Oak Ridge National Laboratory; Forschungszentrum Juelich GmbH FX This work was financially supported by the U.S. Department of Homeland Security under Grant Award No. 2014-DN-077-ARI085-01. Supports from Oak Ridge National Laboratory and Forschungszentrum Juelich GmbH are also acknowledged. NR 18 TC 0 Z9 0 U1 19 U2 38 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 153106 DI 10.1063/1.4945999 PG 4 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000045 ER PT J AU Wang, RX Xu, H Yang, B Luo, ZL Sun, EW Zhao, JT Zheng, LM Dong, YQ Zhou, H Ren, Y Gao, C Cao, WW AF Wang, Ruixue Xu, Han Yang, Bin Luo, Zhenlin Sun, Enwei Zhao, Jiangtao Zheng, Limei Dong, Yongqi Zhou, Hua Ren, Yang Gao, Chen Cao, Wenwu TI Phase coexistence and domain configuration in Pb(Mg1/3Nb2/3)O-3-0.34PbTiO(3) single crystal revealed by synchrotron-based X-ray diffractive three-dimensional reciprocal space mapping and piezoresponse force microscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID FERROELECTRICS; ORIGIN; STATE AB The crystalline phases and domain configuration in the morphotropic phase boundary composition Pb(Mg1/3Nb2/3)O-3-0.34PbTiO(3) (PMN-0.34PT) single crystal have been investigated by synchrotron-based X-ray 3D Reciprocal Space Mapping (3D-RSM) and Piezoresponse Force Microscopy. The coexistence of tetragonal (T) and monoclinic M-C phases in this PMN-0.34PT single crystal is confirmed. The affiliation of each diffraction spot in the 3D-RSM was identified with the assistance of qualitative simulation. Most importantly, the twinning structure between different domains in such a mixed phase PMN-PT crystal is firmly clarified, and the spatial distribution of different twin domains is demonstrated. In addition, the lattice parameters of T and M-C phases in PMN-0.34PT single crystal as well as the tilting angles of crystal lattices caused by the interfacial lattice mismatch are determined. Published by AIP Publishing. C1 [Wang, Ruixue; Yang, Bin; Sun, Enwei; Zheng, Limei; Cao, Wenwu] Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Dept Phys, Harbin 150080, Peoples R China. [Xu, Han; Luo, Zhenlin; Zhao, Jiangtao; Dong, Yongqi; Gao, Chen] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China. [Xu, Han; Luo, Zhenlin; Zhao, Jiangtao; Dong, Yongqi; Gao, Chen] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. [Zhou, Hua; Ren, Yang] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Cao, Wenwu] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Cao, Wenwu] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. RP Yang, B (reprint author), Harbin Inst Technol, Condensed Matter Sci & Technol Inst, Dept Phys, Harbin 150080, Peoples R China.; Luo, ZL (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China.; Luo, ZL (reprint author), Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. EM binyang@hit.edu.cn; zlluo@ustc.edu.cn RI Cao, Wenwu/F-6091-2012 OI Cao, Wenwu/0000-0002-2447-1486 FU National key Basic Research Program of China [2013CB632900]; National Natural Science Foundation of China [11374010, 11434009]; DOE, Basic Energy Sciences [DE-AC02-06CH11357] FX This research was supported by the National key Basic Research Program of China (Grant No. 2013CB632900). Z. Luo acknowledges the National Natural Science Foundation of China (Grant Nos. 11374010, 11434009). The authors would like to thank beamline 12-ID-D of APS for providing the beam time. Work performed at the Advanced Photon Source at Argonne National Laboratory was supported by the DOE, Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 40 TC 4 Z9 4 U1 20 U2 63 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD APR 11 PY 2016 VL 108 IS 15 AR 152905 DI 10.1063/1.4946776 PG 5 WC Physics, Applied SC Physics GA DJ6IE UT WOS:000374314000039 ER PT J AU Gerlits, O Wymore, T Das, A Shen, CH Parks, JM Smith, JC Weiss, KL Keen, DA Blakeley, MP Louis, JM Langan, P Weber, IT Kovalevsky, A AF Gerlits, Oksana Wymore, Troy Das, Amit Shen, Chen-Hsiang Parks, Jerry M. Smith, Jeremy C. Weiss, Kevin L. Keen, David A. Blakeley, Matthew P. Louis, John M. Langan, Paul Weber, Irene T. Kovalevsky, Andrey TI Long-Range Electrostatics-Induced Two-Proton Transfer Captured by Neutron Crystallography in an Enzyme Catalytic Site SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE aspartic protease; enzymes; neutron crystallography; proton transfer; QM; MM modeling ID X-RAY CRYSTALLOGRAPHY; BARRIER HYDROGEN-BOND; PROTON-TRANSFER; HIV-1 PROTEASE; FLUORESCENT PROTEIN; ATOMIC-RESOLUTION; CRYSTAL-STRUCTURES; BINDING-SITES; INHIBITOR; MECHANISM AB Neutron crystallography was used to directly locate two protons before and after a pH-induced two-proton transfer between catalytic aspartic acid residues and the hydroxy group of the bound clinical drug darunavir, located in the catalytic site of enzyme HIV-1 protease. The two-proton transfer is triggered by electrostatic effects arising from protonation state changes of surface residues far from the active site. The mechanism and pH effect are supported by quantum mechanics/molecular mechanics (QM/MM) calculations. The low-pH proton configuration in the catalytic site is deemed critical for the catalytic action of this enzyme and may apply more generally to other aspartic proteases. Neutrons therefore represent a superb probe to obtain structural details for proton transfer reactions in biological systems at a truly atomic level. C1 [Gerlits, Oksana; Weiss, Kevin L.; Langan, Paul; Kovalevsky, Andrey] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Wymore, Troy; Parks, Jerry M.; Smith, Jeremy C.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Biosci Div, Oak Ridge, TN 37831 USA. [Das, Amit] BARC Trombay, Div Solid State Phys, Mumbai 400085, Maharashtra, India. [Shen, Chen-Hsiang; Weber, Irene T.] Georgia State Univ, Dept Chem, Atlanta, GA 30302 USA. [Shen, Chen-Hsiang; Weber, Irene T.] Georgia State Univ, Dept Biol, POB 4010, Atlanta, GA 30302 USA. [Keen, David A.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Blakeley, Matthew P.] Inst Laue Langevin, Large Scale Structures Grp, 71 Ave Martyrs CS 20156, F-38042 Grenoble 9, France. [Louis, John M.] NIDDK, Chem Phys Lab, NIH, DHHS, Bethesda, MD 20892 USA. RP Kovalevsky, A (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM kovalevskyay@ornl.gov RI Weiss, Kevin/I-4669-2013; Blakeley, Matthew/G-7984-2015; Langan, Paul/N-5237-2015; OI Weiss, Kevin/0000-0002-6486-8007; Blakeley, Matthew/0000-0002-6412-4358; Langan, Paul/0000-0002-0247-3122; Kovalevsky, Andrey/0000-0003-4459-9142 FU DOE Office of Biological and Environmental Research (BER); DOE Office of Basic Energy Sciences (BES); CSMB; NIH [R01GM02920] FX We thank the Center for Structural Molecular Biology (CSMB) at BES Scientific User Facilities Division, supported by the DOE Office of Biological and Environmental Research (BER), for facility use. O. G., P. L., and A. K. were partly supported by the DOE Office of Basic Energy Sciences (BES). K. L. W. was partly supported by CSMB. I. T. W. was partly supported by an NIH grant R01GM02920. The authors thank Institut Laue Langevin (beamline LADI-III) and Oak Ridge National Laboratory (IMAGINE beamline) for neutron beam time. NR 41 TC 5 Z9 5 U1 10 U2 32 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD APR 11 PY 2016 VL 55 IS 16 BP 4924 EP 4927 DI 10.1002/anie.201509989 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DJ8XB UT WOS:000374496100007 PM 26958828 ER PT J AU Sougrati, MT Darwiche, A Liu, XH Mahmoud, A Hermann, RP Jouen, S Monconduit, L Dronskowski, R Stievano, L AF Sougrati, Moulay T. Darwiche, Ali Liu, Xiaohiu Mahmoud, Abdelfattah Hermann, Raphael P. Jouen, Samuel Monconduit, Laure Dronskowski, Richard Stievano, Lorenzo TI Transition-Metal Carbodiimides as Molecular Negative Electrode Materials for Lithium- and Sodium-Ion Batteries with Excellent Cycling Properties SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE batteries; carbodiimide; lithium ions; sodium ions ID RAY PHOTOELECTRON-SPECTROSCOPY; FE-57 MOSSBAUER-SPECTROSCOPY; CRYSTAL-STRUCTURE; MANGANESE CARBODIIMIDE; MAGNETIC-PROPERTIES; ANODE MATERIALS; CYANAMIDE; PERFORMANCES; REDUCTION; MECHANISM AB We report evidence for the electrochemical activity of transition-metal carbodiimides versus lithium and sodium. In particular, iron carbodiimide, FeNCN, can be efficiently used as negative electrode material for alkali-metal-ion batteries, similar to its oxide analogue FeO. Based on Fe-57 Mossbauer and infrared spectroscopy (IR) data, the electrochemical reaction mechanism can be explained by the reversible transformation of the Fe-NCN into Li/Na-NCN bonds during discharge and charge. These new electrode materials exhibit higher capacity compared to well-established negative electrode references such as graphite or hard carbon. Contrary to its oxide analogue, iron carbodiimide does not require heavy treatments (such as nanoscale tailoring, sophisticated textures, or coating) to obtain long cycle life with current density as high as 9Ag(-1) for hundreds of charge-discharge cycles. Similar to the iron compound, several other transition-metal carbodiimides M-x(NCN)(y) with M=Mn, Cr, Zn can cycle successfully versus lithium and sodium. Their electrochemical activity and performance open the way to the design of a novel family of anode materials. C1 [Sougrati, Moulay T.; Darwiche, Ali; Monconduit, Laure; Stievano, Lorenzo] Inst Charles Gerhardt Montpellier, UMR CNRS 5253, F-34095 Montpellier, France. [Sougrati, Moulay T.; Darwiche, Ali; Monconduit, Laure; Stievano, Lorenzo] FR CNRS 3459, Rseau Stockage Electrochim Energie, F-80039 Amiens, France. [Liu, Xiaohiu; Dronskowski, Richard] Rhein Westfal TH Aachen, Inst Inorgan Chem, D-52056 Aachen, Germany. [Mahmoud, Abdelfattah; Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, JCNS, D-52425 Julich, Germany. [Mahmoud, Abdelfattah; Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, PGI, D-52425 Julich, Germany. [Mahmoud, Abdelfattah] Univ Liege, LCIS GREENMAT, Inst Chem B6, B-4000 Liege, Belgium. [Hermann, Raphael P.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Jouen, Samuel] Normandie Univ, UMR CNRS 6634, Grp Phys Mat, F-76801 St Etienne, France. RP Stievano, L (reprint author), Inst Charles Gerhardt Montpellier, UMR CNRS 5253, F-34095 Montpellier, France.; Stievano, L (reprint author), FR CNRS 3459, Rseau Stockage Electrochim Energie, F-80039 Amiens, France.; Dronskowski, R (reprint author), Rhein Westfal TH Aachen, Inst Inorgan Chem, D-52056 Aachen, Germany. EM drons@HAL9000.ac.rwth-aachen.de; lorenzo.stievano@umontpellier.fr RI Hermann, Raphael/F-6257-2013; Sougrati, Moulay Tahar/B-6283-2011; OI Hermann, Raphael/0000-0002-6138-5624; Sougrati, Moulay Tahar/0000-0003-3740-2807; Darwiche, ali/0000-0001-9297-2509; Stievano, Lorenzo/0000-0001-8548-0231 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy FX M.T.S. acknowledge Dr. Bernard Fraisse for his help in the in situ experiments. X.L. and R.D. happily acknowledge the long-time support of the Deutsche Forschungsgemeinschaft (DFG). R.P.H. acknowledges support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. NR 52 TC 1 Z9 1 U1 53 U2 152 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD APR 11 PY 2016 VL 55 IS 16 BP 5090 EP 5095 DI 10.1002/anie.201600098 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DJ8XB UT WOS:000374496100041 PM 26989882 ER PT J AU Blum, T Boyle, PA Del Debbio, L Hudspith, RJ Izubuchi, T Juttner, A Lehner, C Lewis, R Maltman, K Marinkovic, MK Portelli, A Spraggs, M AF Blum, T. Boyle, P. A. Del Debbio, L. Hudspith, R. J. Izubuchi, T. Juettner, A. Lehner, C. Lewis, R. Maltman, K. Marinkovic, M. Krstic Portelli, A. Spraggs, M. TI Lattice calculation of the leading strange quark-connected contribution to the muon g-2 SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Lattice QCD; Lattice Quantum Field Theory ID CHIRAL FERMIONS; MOBIUS FERMIONS AB We present results for the leading hadronic contribution to the muon anomalous magnetic moment due to strange quark-connected vacuum polarisation effects. Simulations were performed using RBC-UKQCD's N-f = 2 + 1 domain wall fermion ensembles with physical light sea quark masses at two lattice spacings. We consider a large number of analysis scenarios in order to obtain solid estimates for residual systematic effects. Our final result in the continuum limit is a(mu)((2)had,) (s) = 53.1(9) ((+1)(-3)) x 10(-10). C1 [Blum, T.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Boyle, P. A.; Del Debbio, L.; Portelli, A.] Univ Edinburgh, Sch Phys & Astron, Peter Guthrie Tait Rd, Edinburgh EH9 3JZ, Midlothian, Scotland. [Hudspith, R. J.; Lewis, R.] York Univ, Dept Phys & Astron, 4700 Keele St, Toronto, ON M3J 1P3, Canada. [Izubuchi, T.; Lehner, C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Izubuchi, T.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Juettner, A.; Marinkovic, M. Krstic; Portelli, A.; Spraggs, M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Maltman, K.] York Univ, Dept Math & Stat, 4700 Keele St, Toronto, ON M3J 1P3, Canada. [Maltman, K.] Univ Adelaide, CSSM, Adelaide, SA 5005, Australia. [Marinkovic, M. Krstic] CERN, Dept Theoret Phys, Geneva, Switzerland. RP Spraggs, M (reprint author), Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. EM matthew.spraggs@gmail.com FU STFC [ST/K005790/1, ST/K005804/1, ST/K000411/1, ST/H008845/1]; US DOE [DE-FG02-92ER40716, DE-SC0012704]; NSERC of Canada; JSPS KAKENHI Grant [26400261]; European Research Council under the European Union's Seventh Framework Programme (FP7)/ERC Grant [279757]; U.K. EPSRC Doctoral Training Centre Grant [EP/G03690X/1]; U.K. STFC [ST/K005790/1, ST/K005804/1, ST/M006530/1, ST/L000458/1]; [ST/L000296/1] FX The authors gratefully acknowledge computing time granted through the STFC funded DiRAC facility (grants ST/K005790/1, ST/K005804/1, ST/K000411/1, ST/H008845/1). T.B. is supported by US DOE grant DE-FG02-92ER40716. P.A.B., L.D.D., and A.P. are supported in part by U.K. STFC Grants No. ST/M006530/1, ST/L000458/1, ST/K005790/1, and ST/K005804/1 and A.P. additionally by ST/L000296/1. R.H., R.L. and K.M. are supported by NSERC of Canada. T.I. and C.L. are supported in part by US DOE Contract No. DE-SC0012704(BNL). T.I. is supported in part by JSPS KAKENHI Grant No. 26400261. A.J. and M.M. received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement 279757. M.S. is supported by U.K. EPSRC Doctoral Training Centre Grant EP/G03690X/1. The data analysis has been primarily performed using LatAnalyze (https://github.com/aportelli/LatAnalyze3), which is free software distributed under the GNU General Public License v3. NR 44 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 11 PY 2016 IS 4 AR 063 DI 10.1007/JHEP04(2016)063 PG 20 WC Physics, Particles & Fields SC Physics GA DJ2OW UT WOS:000374045400002 ER PT J AU Chiu, I Dietrich, JP Mohr, J Applegate, DE Benson, BA Bleem, LE Bayliss, MB Bocquet, S Carlstrom, JE Capasso, R Desai, S Gangkofner, C Gonzalez, AH Gupta, N Hennig, C Hoekstra, H von der Linden, A Liu, J McDonald, M Reichardt, CL Saro, A Schrabback, T Strazzullo, V Stubbs, CW Zenteno, A AF Chiu, I. Dietrich, J. P. Mohr, J. Applegate, D. E. Benson, B. A. Bleem, L. E. Bayliss, M. B. Bocquet, S. Carlstrom, J. E. Capasso, R. Desai, S. Gangkofner, C. Gonzalez, A. H. Gupta, N. Hennig, C. Hoekstra, H. von der Linden, A. Liu, J. McDonald, M. Reichardt, C. L. Saro, A. Schrabback, T. Strazzullo, V. Stubbs, C. W. Zenteno, A. TI Detection of enhancement in number densities of background galaxies due to magnification by massive galaxy clusters SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE gravitational lensing: weak; galaxies: clusters: individual; cosmology: observations; large-scale structure of Universe ID WEAK-LENSING MASSES; SOUTH-POLE TELESCOPE; DARK-MATTER HALOS; DIGITAL SKY SURVEY; K-BAND PROPERTIES; PHOTOMETRIC REDSHIFTS; COSMIC MAGNIFICATION; LUMINOSITY FUNCTION; IMAGE-ANALYSIS; SHEAR AB We present a detection of the enhancement in the number densities of background galaxies induced from lensing magnification and use it to test the Sunyaev-Zel'dovich effect (SZE-) inferred masses in a sample of 19 galaxy clusters with median redshift z similar or equal to 0.42 selected from the South Pole Telescope SPT-SZ survey. These clusters are observed by the Megacam on the Magellan Clay Telescope though gri filters. Two background galaxy populations are selected for this study through their photometric colours; they have median redshifts zmedian similar or equal to 0.9 (low-z background) and z(median) similar or equal to 1.8 (high-z background). Stacking these populations, we detect the magnification bias effect at 3.3 sigma and 1.3 sigma for the low-and high-z backgrounds, respectively. We fit Navarro, Frenk and White models simultaneously to all observed magnification bias profiles to estimate the multiplicative factor. that describes the ratio of the weak lensing mass to the mass inferred from the SZE observable-mass relation. We further quantify systematic uncertainties in. resulting from the photometric noise and bias, the cluster galaxy contamination and the estimations of the background properties. The resulting. for the combined background populations with 1 sigma uncertainties is 0.83 +/- 0.24(stat) +/- 0.074(sys), indicating good consistency between the lensing and the SZE-inferred masses. We use our best-fitting eta to predict the weak lensing shear profiles and compare these predictions with observations, showing agreement between the magnification and shear mass constraints. This work demonstrates the promise of using the magnification as a complementary method to estimate cluster masses in large surveys. C1 [Chiu, I.; Dietrich, J. P.; Mohr, J.; Bocquet, S.; Capasso, R.; Desai, S.; Gangkofner, C.; Gupta, N.; Hennig, C.; Liu, J.; Saro, A.; Strazzullo, V.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Chiu, I.; Dietrich, J. P.; Mohr, J.; Bocquet, S.; Capasso, R.; Desai, S.; Gangkofner, C.; Gupta, N.; Hennig, C.; Liu, J.; Saro, A.] Excellence Cluster Univ, Boltzmannstr 2, D-85748 Garching, Germany. [Mohr, J.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Applegate, D. E.; Schrabback, T.] Argelander Inst Astron, Auf Hugel 71, D-53121 Bonn, Germany. [Benson, B. A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Benson, B. A.; Bleem, L. E.; Carlstrom, J. E.] Univ Chicago, Kavli Inst Cosmol Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Benson, B. A.; Carlstrom, J. E.] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Bleem, L. E.] Univ Chicago, Dept Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Bleem, L. E.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Bayliss, M. B.; Stubbs, C. W.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Bayliss, M. B.; Stubbs, C. W.] Harvard Univ, Dept Phys, 17 Oxford St, Cambridge, MA 02138 USA. [Gonzalez, A. H.] Univ Florida, Dept Astron, Gainesville, FL 32611 USA. [Hoekstra, H.] Leiden Univ, Leiden Observ, POB 9513, NL-2300 RA Leiden, Netherlands. [von der Linden, A.] Stanford Univ, KIPAC, 452 Lomita Mall, Stanford, CA 94305 USA. [von der Linden, A.] Stanford Univ, Dept Phys, 452 Lomita Mall, Stanford, CA 94305 USA. [von der Linden, A.] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, Juliane Maries Vej 30, DK-2100 Copenhagen, Denmark. [McDonald, M.] MIT, Kavli Inst Astrophys & Space Res, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Reichardt, C. L.] Univ Melbourne, Sch Phys, Parkville, Vic 3010, Australia. [Zenteno, A.] Cerro Tololo Interamer Observ, Casilla 603, La Serena, Chile. RP Chiu, I; Dietrich, JP; Mohr, J (reprint author), Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany.; Chiu, I; Dietrich, JP; Mohr, J (reprint author), Excellence Cluster Univ, Boltzmannstr 2, D-85748 Garching, Germany.; Mohr, J (reprint author), Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. EM inonchiu@usm.lmu.de; dietrich@usm.lmu.de; jmohr@USM.LMU.de OI Dietrich, Jorg/0000-0002-8134-9591; Stern, Corvin/0000-0003-4406-6127; Hoekstra, Henk/0000-0002-0641-3231 FU DFG Cluster of Excellence 'Origin and Structure of the Universe'; Transregio programme 'The Dark Universe' [TR33]; German Federal Ministry of Economics and Technology (BMWi) through DLR [50 OR 1210, 50 OR 1308, 50 OR 1407]; Australian Research Council's Discovery Projects scheme [DP150103208]; National Science Foundation [ANT-0638937]; NSF Physics Frontier Center [PHY-0114422]; Kavli Foundation; Gordon and Betty Moore Foundation FX We acknowledge the support by the DFG Cluster of Excellence 'Origin and Structure of the Universe' and the Transregio programme TR33 'The Dark Universe'. DA and TS acknowledge support from the German Federal Ministry of Economics and Technology (BMWi) provided through DLR under projects 50 OR 1210, 50 OR 1308, and 50 OR 1407. CR acknowledges support from the Australian Research Council's Discovery Projects scheme (DP150103208). The South Pole Telescope is supported by the National Science Foundation through grant ANT-0638937. Partial support is also provided by the NSF Physics Frontier Center grant PHY-0114422 to the Kavli Institute of Cosmological Physics at the University of Chicago, the Kavli Foundation and the Gordon and Betty Moore Foundation. Optical imaging data were obtained with Megacam on the 6.5 m Magellan Clay Telescope. NR 64 TC 4 Z9 4 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD APR 11 PY 2016 VL 457 IS 3 BP 3050 EP 3065 DI 10.1093/mnras/stw190 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI6BJ UT WOS:000373583900058 ER PT J AU Tchekhovskoy, A Philippov, A Spitkovsky, A AF Tchekhovskoy, Alexander Philippov, Alexander Spitkovsky, Anatoly TI Three-dimensional analytical description of magnetized winds from oblique pulsars SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE MHD; stars: magnetars; stars: magnetic field; stars: neutron; pulsars: general; stars: rotation ID FORCE-FREE MAGNETOSPHERE; IN-CELL SIMULATIONS; GAMMA-RAY BURSTS; CRAB-NEBULA; MAGNETOHYDRODYNAMIC SIMULATIONS; CURRENT SHEETS; NEUTRON-STAR; MHD WINDS; EMISSION; GRB AB Rotating neutron stars, or pulsars and magnetars, are plausibly the source of power behind many astrophysical systems, such as gamma-ray bursts, supernovae, pulsar wind nebulae, and supernova remnants. In the past several years, three-dimensional (3D) numerical simulations made it possible to compute pulsar spin-down luminosity from first principles and revealed that oblique pulsar winds are more powerful than aligned ones. However, what causes this enhanced power output of oblique pulsars is not understood. In this work, using time-dependent 3D magnetohydrodynamic and force-free simulations, we show that, contrary to the standard paradigm, the open magnetic flux, which carries the energy away from the pulsar, is laterally non-uniform. We argue that this non-uniformity is the primary reason for the increased luminosity of oblique pulsars. To demonstrate this, we construct simple analytic descriptions of aligned and orthogonal pulsar winds and combine them to obtain an accurate 3D description of the pulsar wind for any obliquity. Our approach describes both the warped magnetospheric current sheet and the smooth variation of pulsar wind properties outside of it. We find that the jump in magnetic field components across the current sheet decreases with increasing obliquity, which could be a mechanism that reduces dissipation in near-orthogonal pulsars. Our analytical description of the pulsar wind can be used for constructing models of pulsar gamma-ray emission, pulsar wind nebulae, neutron star powered ultra-luminous X-ray sources, and magnetar-powered core-collapse gamma-ray bursts and supernovae. C1 [Tchekhovskoy, Alexander] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Tchekhovskoy, Alexander] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Philippov, Alexander; Spitkovsky, Anatoly] Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. RP Tchekhovskoy, A (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA.; Tchekhovskoy, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Philippov, A; Spitkovsky, A (reprint author), Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. EM atchekho@berkeley.edu; philippo@astro.princeton.edu; anatoly@astro.princeton.edu FU NASA through Einstein Post-doctoral Fellowship - Chandra X-ray Center [PF3-140131]; NASA [NAS8-03060, NNX14AQ67G]; NASA Earth and Space Science Fellowship Program [NNX15AT50H]; Simons Foundation [267233] FX We thank Jon Arons, Andrei Beloborodov, Vasily Beskin, and Rolf Buehler for insightful discussions. AT was supported by NASA through Einstein Post-doctoral Fellowship grant number PF3-140131 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060, and NASA via High-End Computing (HEC) Program through the NASA Advanced Supercomputing (NAS) Division at Ames Research Center that provided access to the Pleiades supercomputer, as well as NSF through an XSEDE computational time allocation TG-AST100040 on NICS Kraken, Nautilus, TACC Stampede, Maverick, and Ranch. AP was supported by NASA Earth and Space Science Fellowship Program (grant number NNX15AT50H). This work was supported in part by NASA grant NNX14AQ67G and Simons Foundation (grant 267233 to AS). We used ENTHOUGHT CANOPY PYTHON distribution to generate figures for this work. NR 51 TC 6 Z9 6 U1 1 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD APR 11 PY 2016 VL 457 IS 3 BP 3384 EP 3395 DI 10.1093/mnras/stv2869 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI6BJ UT WOS:000373583900082 ER PT J AU Balachandran, PV Xue, DZ Lookman, T AF Balachandran, Prasanna V. Xue, Dezhen Lookman, Turab TI Structure-Curie temperature relationships in BaTiO3-based ferroelectric perovskites: Anomalous behavior of (Ba,Cd)TiO3 from DFT, statistical inference, and experiments SO PHYSICAL REVIEW B LA English DT Article ID CRYSTAL-STRUCTURE; MATERIALS INFORMATICS; DIELECTRIC-PROPERTIES; NEUTRON-DIFFRACTION; PHASE-TRANSITIONS; RAY-DIFFRACTION; SOLID-SOLUTIONS; CERAMICS; SR; PSEUDOPOTENTIALS AB One of the key impediments to the development of BaTiO3-based materials as candidates to replace toxic-Pb-based solid solutions is their relatively low ferroelectric Curie temperature (T-C). Among many potential routes that are available to modify T-C, ionic substitutions at the Ba and Ti sites remain the most common approach. Here, we perform density functional theory (DFT) calculations on a series of ATiO(3) and BaBO3 perovskites, where A = Ba, Ca, Sr, Pb, Cd, Sn, and Mg and B = Ti, Zr, Hf, and Sn. Our objective is to study the relative role of A and B cations in impacting the T-C of the tetragonal (P4mm) and rhombohedral (R3m) ferroelectric phases in BaTiO3-based solid solutions, respectively. Using symmetry-mode analysis, we obtain a quantitative description of the relative contributions of various divalent (A) and tetravalent (B) cations to the ferroelectric distortions. Our results show that Ca, Pb, Cd, Sn, and Mg have large mode amplitudes for ferroelectric distortion in the tetragonal phase relative to Ba, whereas Sr suppresses the distortions. On the other hand, Zr, Hf, and Sn tetravalent cations severely suppress the ferroelectric distortion in the rhombohedral phase relative to Ti. In addition to symmetry modes, our calculated unit-cell volume also agrees with the experimental trends. We subsequently utilize the symmetry modes and unit-cell volumes as features within a machine learning approach to learn T-C via an inference model and uncover trends that provide insights into the design of new high-T-C BaTiO3-based ferroelectrics. The inference model predicts CdTiO3-BaTiO3 solid solutions to have a higher TC and, therefore, we experimentally synthesized these solid solutions and measured their T-C. Although the calculated mode strength for CdTiO3 in the tetragonal phase is even larger than that for PbTiO3, the T-C of CdTiO3-BaTiO3 solid solutions in the tetragonal phase does not show any appreciable enhancement. Thus, CdTiO3-BaTiO3 does not follow the inference model, which is based on established data and trends for ATiO(3). Rather, our experimental phase diagram for CdTiO3-BaTiO3 suggests that it behaves markedly differently from any other BaTiO3-based systems studied so far. C1 [Balachandran, Prasanna V.; Xue, Dezhen; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Xue, Dezhen] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. RP Balachandran, PV; Lookman, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM pbalachandran@lanl.gov; txl@lanl.gov RI XUE, Dezhen/A-6062-2010 OI XUE, Dezhen/0000-0001-6132-1236 FU Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR [20140013DR] FX P.V.B., X.D., and T.L. acknowledge funding support from the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) DR (Grant No. 20140013DR) on Materials Informatics. The computational work made use of Institutional Computing (IC) resources at LANL. NR 76 TC 5 Z9 5 U1 16 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 11 PY 2016 VL 93 IS 14 AR 144111 DI 10.1103/PhysRevB.93.144111 PG 12 WC Physics, Condensed Matter SC Physics GA DI8OD UT WOS:000373759400007 ER PT J AU Blancon, JC Machon, D Pischedda, V Debord, R Toulemonde, P Le Floch, S Pascarelli, S Melinon, P San-Miguel, A AF Blancon, J. -C. Machon, D. Pischedda, V. Debord, R. Toulemonde, P. Le Floch, S. Pascarelli, S. Melinon, P. San-Miguel, A. TI Revisiting pressure-induced phase transition in silicon clathrates using Ge substitution SO PHYSICAL REVIEW B LA English DT Article ID SI AB Ba8Si39Ge7 and Ba8Si29Ge17 have been studied at high pressure using x-ray diffraction and x-ray absorption spectroscopy (XAS) at the Ge K edge. In Ba8Si39Ge7, a transition is observed similar to the one in Ba8Si46, apparently isostructural. However, the XAS data analysis shows that the transformation is related to the off-centering of the Ba atoms. A theoretical model based on a Landau potential suggests that this transition is second order, with a symmetry-breaking mechanism related to the Ba displacement probably initiated by the vacancy creation or local distortion predicted theoretically. This analysis gives a coherent picture of the phase transition mechanism. In the case of Ba8Si29Ge17, such phase transition is not observed as the Ba atoms appear already off-center at ambient pressure. C1 [Blancon, J. -C.; Machon, D.; Pischedda, V.; Debord, R.; Le Floch, S.; Melinon, P.; San-Miguel, A.] Univ Lyon, F-69003 Lyon, France. [Blancon, J. -C.; Machon, D.; Pischedda, V.; Debord, R.; Le Floch, S.; Melinon, P.; San-Miguel, A.] Univ Lyon 1, F-69622 Villeurbanne, France. [Blancon, J. -C.; Machon, D.; Pischedda, V.; Debord, R.; Le Floch, S.; Melinon, P.; San-Miguel, A.] Inst Lumiere Mat, CNRS, UMR5306, F-69622 Villeurbanne, France. [Toulemonde, P.] Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France. [Toulemonde, P.] CNRS, Inst NEEL, F-38000 Grenoble, France. [Pascarelli, S.] European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. [Blancon, J. -C.] Los Alamos Natl Lab, Phys Chem & Appl Spect, POB 1663, Los Alamos, NM 87545 USA. RP Machon, D (reprint author), Univ Lyon, F-69003 Lyon, France.; Machon, D (reprint author), Univ Lyon 1, F-69622 Villeurbanne, France.; Machon, D (reprint author), Inst Lumiere Mat, CNRS, UMR5306, F-69622 Villeurbanne, France. EM denis.machon@univ-lyon1.fr RI San-Miguel, Alfonso/H-3198-2016; OI Blancon, Jean-Christophe/0000-0002-3833-5792 NR 39 TC 3 Z9 3 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 11 PY 2016 VL 93 IS 13 AR 134103 DI 10.1103/PhysRevB.93.134103 PG 10 WC Physics, Condensed Matter SC Physics GA DI8NT UT WOS:000373758400001 ER PT J AU Li, W Huang, L Evans, JW Han, Y AF Li, Wei Huang, Li Evans, James W. Han, Yong TI Submonolayer Ag films on Fe(100): A first-principles analysis of energetics controlling adlayer thermodynamics and kinetics SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM-WELL STATES; INITIO MOLECULAR-DYNAMICS; AUGMENTED-WAVE METHOD; AG(100) THIN-FILMS; METAL-SURFACES; LATTICE-CONSTANTS; NANOCLUSTERS; GROWTH; ENERGY; SIMULATION AB Epitaxial growth of Ag on Fe(100) and postdeposition relaxation have been studied in several experiments. We provide a first-principles density functional theory analysis of key adatom interaction energies and diffusion barriers controlling growth and relaxation kinetics for the submonolayer regime, as these have not been assessed previously. A cluster expansion approach is used to obtain an extensive set of conventional lateral interactions between adatoms on fourfold hollow adsorption sites. We find robust oscillatory decay of pair interactions with increasing separation, and of trio interactions with increasing perimeter length. First-and second-nearest-neighbor pair interactions, as well as compact linear and bent trio interactions, dominate. The adatom terrace diffusion barrier is estimated to be E-d approximate to 0.39 eV. We also provide a limited analysis of unconventional interactions for which one adatom is at the bridge-site transition state for hopping and one or more others are at fourfold hollow sites. Energy barriers for diffusion along island edges can be determined with the aid of both conventional and unconventional interactions. C1 [Li, Wei; Huang, Li] South Univ Sci & Technol China, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China. [Evans, James W.; Han, Yong] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Evans, James W.; Han, Yong] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Huang, L (reprint author), South Univ Sci & Technol China, Dept Phys, Shenzhen 518055, Guangdong, Peoples R China.; Han, Y (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.; Han, Y (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM huangl@sustc.edu.cn; yong@ameslab.gov FU South University of Science and Technology of China; NSFC [11404160, CHE-1111500, CHE-1507223]; U.S. Department of Energy by Iowa StateUniversity [DE-AC02-07CH11358] FX W.L. and L.H. acknowledge support from startup funds from the South University of Science and Technology of China and from NSFC under Grant No. 11404160. J.W.E. and Y.H. were supported for this work by NSF Grants No. CHE-1111500 and No. CHE-1507223, and their work was performed at Ames Laboratory which is operated for the U.S. Department of Energy by Iowa StateUniversity under Contract No. DE-AC02-07CH11358. Computations utilized USDOE NERSC, OLCF, and NSF-supported XSEDE resources. NR 54 TC 1 Z9 1 U1 9 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 11 PY 2016 VL 93 IS 15 AR 155416 DI 10.1103/PhysRevB.93.155416 PG 13 WC Physics, Condensed Matter SC Physics GA DI8OO UT WOS:000373760500010 ER PT J AU Mariani, M Lascialfari, A Caneschi, A Ammannato, L Gatteschi, D Rettori, A Pini, MG Cucci, C Borsa, F AF Mariani, M. Lascialfari, A. Caneschi, A. Ammannato, L. Gatteschi, D. Rettori, A. Pini, M. G. Cucci, C. Borsa, F. TI Proton NMR study of spin dynamics in the magnetic organic chains M (hfac)(3) NITEt (M = Eu3+, Gd3+) SO PHYSICAL REVIEW B LA English DT Article ID RARE-EARTH IONS; NITRONYL NITROXIDES; PHASE-TRANSITIONS; MOLECULAR CHAINS; FERRIMAGNETIC CHAINS; RELAXATION; COMPLEXES; SYSTEMS; TEMPERATURE; GADOLINIUM AB In this work, we present a nuclear magnetic resonance (NMR) study of the spin dynamics in the rare-earth-based low-dimensional molecular magnetic chains Eu(hfac)(3)NITEt and Gd(hfac) 3NITEt (in short, Eu-Et and Gd-Et). Although both samples are based on the same chemical building block, [(hfac) 3NITEt], their magnetic properties change dramatically when the Eu3+ ion, which is nonmagnetic at low temperatures, is substituted by the magnetic Gd3+ ion. The present proton NMR investigation shows that, down to the lowest investigated temperature (T = 1.5 K for Gd-Et and T = 3 K for Eu-Et), the Eu-Et chain behaves as a one-dimensional Heisenberg model with antiferromagnetic exchange coupling (J = -20 K) between s = 1/2 organic radicals, and has a T-independent exchange frequency (omega(e) = 2.6 x 10(12) rad/s). In the Gd-Et chain, in contrast, a competition arises between nearest-neighbor ferromagnetic coupling and next-nearest-neighbor antiferromagnetic coupling; moreover, two phase transitions have previously been found, in agreement with Villain's conjecture: a first transition, at T-0 = 2.2 K, from a high temperature paramagnetic phase to a chiral spin liquid phase, and a second transition, at T-N = 1.9 K, to a three-dimensional helical spin solid phase. Contrary to the Eu-Et chain (whose three-dimensional ordering temperature is estimated to insurge at very low, T-N approximate to 0.3 K), critical spin dynamics effects have been measured in the Gd-Et chain on approaching T-N = 1.9 K: namely, a divergence of the proton nuclear spin-lattice relaxation rate 1/T1, which in turn produces a sudden wipe-out of the NMR signal in a very narrow (Delta T similar to 0.04 K) temperature range above T-N. Below T-N, an inhomogeneous broadening of the NMR line indicates a complete spin freezing. At T0 = 2.2 K, instead, such critical effects are not observed because NMR measurements probe the two-spin correlation function, while the chiral spin liquid phase transition is associated with a divergence of the four-spin correlation function. C1 [Mariani, M.; Lascialfari, A.; Borsa, F.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Mariani, M.; Lascialfari, A.; Borsa, F.] INSTM, I-27100 Pavia, Italy. [Mariani, M.] Univ Bologna, Dipartmento Fis, I-40127 Bologna, Italy. [Lascialfari, A.] Univ Milan, Dipartimento Fis, Via Celoria 16, I-20133 Milan, Italy. [Lascialfari, A.] INSTM, I-20133 Milan, Italy. [Lascialfari, A.; Rettori, A.] CNR, NANO, Ist Nanosci, Ctr S3, I-41125 Modena, Italy. [Caneschi, A.; Ammannato, L.; Gatteschi, D.] Univ Florence, Dipartimento Chim, I-50019 Sesto Fiorentino, FI, Italy. [Caneschi, A.; Ammannato, L.; Gatteschi, D.] INSTM, I-50019 Sesto Fiorentino, FI, Italy. [Rettori, A.] Univ Florence, Dipartimento Fis & Astron, I-50019 Sesto Fiorentino, FI, Italy. [Pini, M. G.] CNR, ISC, Unita Firenze, I-50019 Sesto Fiorentino, FI, Italy. [Cucci, C.] Italian Natl Res Council, CNR, IFAC, Inst Appl Phys Nello Carrara, I-50019 Sesto Fiorentino, FI, Italy. [Borsa, F.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Borsa, F.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Lascialfari, A (reprint author), Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy.; Lascialfari, A (reprint author), INSTM, I-27100 Pavia, Italy.; Lascialfari, A (reprint author), Univ Milan, Dipartimento Fis, Via Celoria 16, I-20133 Milan, Italy.; Lascialfari, A (reprint author), INSTM, I-20133 Milan, Italy.; Lascialfari, A (reprint author), CNR, NANO, Ist Nanosci, Ctr S3, I-41125 Modena, Italy. EM alessandro.lascialfari@unimi.it FU Italian FIRB Project "Futuro in Ricerca" [RBFR12RPD1]; EU Project MAGMANET [NMP3-CT-2005-515767] FX The Italian FIRB Project "Futuro in Ricerca" Grant No. RBFR12RPD1 and the EU Project MAGMANET Contract No. NMP3-CT-2005-515767 are acknowledged for funding. NR 52 TC 0 Z9 0 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 11 PY 2016 VL 93 IS 13 AR 134410 DI 10.1103/PhysRevB.93.134410 PG 13 WC Physics, Condensed Matter SC Physics GA DI8NT UT WOS:000373758400005 ER PT J AU Schaan, E Ferraro, S Vargas-Magana, M Smith, KM Ho, S Aiola, S Battaglia, N Bond, JR De Bernardis, F Calabrese, E Cho, HM Devlin, MJ Dunkley, J Gallardo, PA Hasselfield, M Henderson, S Hill, JC Hincks, AD Hlozek, R Hubmayr, J Hughes, JP Irwin, KD Koopman, B Kosowsky, A Li, D Louis, T Lungu, M Madhavacheri, M Maurin, L McMahon, JJ Moodley, K Naess, S Nati, F Newburgh, L Niemack, MD Page, LA Pappas, CG Partridge, B Schmitt, BL Sehga, N Sherwin, BD Sievers, JL Spergel, DN Staggs, ST van Engelen, A Wollack, EJ AF Schaan, Emmanuel Ferraro, Simone Vargas-Magana, Mariana Smith, Kendrick M. Ho, Shirley Aiola, Simone Battaglia, Nicholas Bond, J. Richard De Bernardis, Francesco Calabrese, Erminia Cho, Hsiao-Mei Devlin, Mark J. Dunkley, Joanna Gallardo, Patricio A. Hasselfield, Matthew Henderson, Shawn Hill, J. Colin Hincks, Adam D. Hlozek, Renee Hubmayr, Johannes Hughes, John P. Irwin, Kent D. Koopman, Brian Kosowsky, Arthur Li, Dale Louis, Thibaut Lungu, Marius Madhavacheri, Mathew Maurin, Loic McMahon, Jeffrey John Moodley, Kavilan Naess, Sigurd Nati, Federico Newburgh, Laura Niemack, Michael D. Page, Lyman A. Pappas, Christine G. Partridge, Bruce Schmitt, Benjamin L. Sehga, Neelima Sherwin, Blake D. Sievers, Jonathan L. Spergel, David N. Staggs, Suzanne T. van Engelen, Alexander Wollack, Edward J. CA ACTPol Collaboration TI Evidence for the kinematic Sunyaev-Zel'dovich effect with the Atacama Cosmology Telescope and velocity reconstruction from the Baryon Oscillation Spectroscopic Survey SO PHYSICAL REVIEW D LA English DT Article ID LOCALLY BRIGHTEST GALAXIES; WEAK LENSING SIGNAL; DIGITAL SKY SURVEY; ACOUSTIC-OSCILLATIONS; POWER SPECTRUM; DATA RELEASE; BULK FLOW; CONSTRAINTS; CLUSTERS; FEEDBACK AB We use microwave temperature maps from two seasons of data from the Atacama Cosmology Telescope at 146 GHz, together with the "Constant Mass" CMASS galaxy sample from the Baryon Oscillation Spectroscopic Survey to measure the kinematic Sunyaev-Zel'dovich (kSZ) effect over the redshift range z = 0.4-0.7. We use galaxy positions and the continuity equation to obtain a reconstruction of the line-of-sight velocity field. We stack the microwave temperature at the location of each halo, weighted by the corresponding reconstructed velocity. We vary the size of the aperture photometry filter used, thus probing the free electron profile of these halos from within the virial radius out to three virial radii, on the scales relevant for investigating the missing baryons problem. The resulting best fit kSZ model is preferred over the no-kSZ hypothesis at 3.3 and 2.9 sigma for two independent velocity reconstruction methods, using 25,537 galaxies over 660 square degrees. The data suggest that the baryon profile is shallower than the dark matter in the inner regions of the halos probed here, potentially due to energy injection from active galactic nucleus or supernovae. Thus, by constraining the gas profile on a wide range of scales, this technique will be useful for understanding the role of feedback in galaxy groups and clusters. The effect of foregrounds that are uncorrelated with the galaxy velocities is expected to be well below our signal, and residual thermal Sunyaev-Zel'dovich contamination is controlled by masking the most massive clusters. Finally, we discuss the systematics involved in converting our measurement of the kSZ amplitude into the mean free electron fraction of the halos in our sample. C1 [Schaan, Emmanuel; Ferraro, Simone; Battaglia, Nicholas; Calabrese, Erminia; Hasselfield, Matthew; Hlozek, Renee; Spergel, David N.] Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. [Ferraro, Simone; Sherwin, Blake D.] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Vargas-Magana, Mariana] Univ Nacl Autonoma Mexico, Inst Fis, Apartado Postal 20-364, Mexico City 04510, DF, Mexico. [Smith, Kendrick M.] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Ho, Shirley] Carnegie Mellon Univ, Dept Phys, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. [Aiola, Simone; Kosowsky, Arthur] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aiola, Simone; Kosowsky, Arthur] Univ Pittsburgh, Pittsburgh Particle Phys Astrophys & Cosmol Ctr, Pittsburgh, PA 15260 USA. [Bond, J. Richard; van Engelen, Alexander] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [De Bernardis, Francesco; Gallardo, Patricio A.; Henderson, Shawn; Koopman, Brian; Maurin, Loic; Niemack, Michael D.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Calabrese, Erminia; Dunkley, Joanna; Louis, Thibaut; Naess, Sigurd] Univ Oxford, Subdept Astrophys, Keble Rd, Oxford OX1 3RH, England. [Cho, Hsiao-Mei; Irwin, Kent D.; Li, Dale] SLAC Natl Accelerator Lab, 2575 Sandhill Hill Rd, Menlo Pk, CA 94025 USA. [Devlin, Mark J.; Lungu, Marius; Nati, Federico; Schmitt, Benjamin L.] Univ Penn, Dept Phys & Astron, 209 South 33rd St, Philadelphia, PA 19104 USA. [Hill, J. Colin] Columbia Univ, Dept Astron, Pupin Hall, New York, NY 10027 USA. [Hincks, Adam D.] Univ British Columbia, Dept Phys & Astron, 6224 Agr Rd, Vancouver, BC V6T 1Z1, Canada. [Hubmayr, Johannes] NIST, Boulder, CO 80305 USA. [Hughes, John P.] Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. [Irwin, Kent D.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Madhavacheri, Mathew; Sehga, Neelima] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Maurin, Loic] Pontificia Univ Catolica Chile, Inst Astrofis, Santiago 7820436, Chile. [McMahon, Jeffrey John] Univ Michigan, Dept Phys, Ann Arbor, MI 48103 USA. [Moodley, Kavilan] Univ KwaZulu Natal, Sch Math Stat & Comp Sci, Astrophys & Cosmol Res Unit, ZA-4041 Durban, South Africa. [Newburgh, Laura] Univ Toronto, Dunlap Inst, 50 St George St, Toronto, ON M5S 3H4, Canada. [Page, Lyman A.; Pappas, Christine G.; Staggs, Suzanne T.] Princeton Univ, Joseph Henry Labs Phys, Jadwin Hall, Princeton, NJ 08544 USA. [Partridge, Bruce] Haverford Coll, Dept Phys & Astron, Haverford, PA 19041 USA. [Sherwin, Blake D.] Univ Calif Berkeley, LBL, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Sherwin, Blake D.] Univ Calif Berkeley, LBL, Dept Phys, Berkeley, CA 94720 USA. [Sievers, Jonathan L.] Univ KwaZulu Natal, Sch Chem & Phys, Astrophys & Cosmol Res Unit, ZA-4041 Durban, South Africa. [Sievers, Jonathan L.] Univ KwaZulu Natal, NITheP, Private Bag X54001, ZA-4000 Durban, South Africa. [Wollack, Edward J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Schaan, E (reprint author), Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. EM eschaan@astro.princeton.edu RI Wollack, Edward/D-4467-2012; Nati, Federico/I-4469-2016; OI Wollack, Edward/0000-0002-7567-4451; Nati, Federico/0000-0002-8307-5088; Aiola, Simone/0000-0002-1035-1854 FU U.S. National Science Foundation (NSF) [AST-0408698, AST-0965625, PHY-0855887, PHY-1214379]; Princeton University; University of Pennsylvania; Cornell University; Canada Foundation for Innovation (CFI); Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT); CFI under the auspices of Compute Canada; Government of Ontario; Ontario Research Fund Research Excellence; University of Toronto; Mishrahi Fund; Wilkinson Fund; NSF [AST1311756, AST1517593, AST1412966, AST-1454881, AST-1517049]; NASA [NNXI2AG72G, 12-EUCLID11-0004, NNX13AE56G, NNX14AB58G, NNX12AM32H, ATP NNX14AB57G]; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation; NSERC Discovery grant; DOE-ASC [DOE-DESC001114]; Lyman Spitzer fellowship; ERC [259505]; DOE [DE-SC0011114]; NASA Space Technology research fellowships; CONICYT [QUIMAL-120001, FONDECYT-1141113]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Institute de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University; [AST-1312991] FX We thank Marcelo Alvarez, Neal Dalal, Tommaso Giannantonio, Oliver Hahn, Andrey Kravtsov, Guilhem Lavaux, Hironao Miyatake, Hyunbae Park, Hiranya Peiris, Ue-Li Pen, Bjoern Soergel, Naonori Sugiyama and Simon White for very useful discussions. This work was supported by the U.S. National Science Foundation (NSF) through Grants No. AST-0408698 and No. AST-0965625 for the ACT project, as well as Grants No. PHY-0855887 and No. PHY-1214379. Funding was also provided by Princeton University, the University of Pennsylvania, Cornell University and a Canada Foundation for Innovation (CFI) award to the University of British Columbia. ACToperates in the Parque Astronomico Atacama in northern Chile under the auspices of the Comision Nacional de Investigacion Cientifica y Tecnologica de Chile (CONICYT). Computations were performed on the GPC supercomputer at the SciNet HPC Consortium. SciNet is funded by the CFI under the auspices of Compute Canada, the Government of Ontario, the Ontario Research Fund Research Excellence; and the University of Toronto. Colleagues at RadioSky provide logistical support and keep operations in Chile running smoothly. We also thank the Mishrahi Fund and the Wilkinson Fund for their generous support of the project. E. S., S. F. and D. N. S. are supported by NSF Grant No. AST1311756 and NASA Grant No. NNXI2AG72G. Research at Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. K. M. S. was supported by an NSERC Discovery grant. S. H. is supported in part by DOE-ASC Award No. DOE-DESC001114, NASA Grant No. 12-EUCLID11-0004, and NSF Grants No. AST1517593 and No. AST1412966. N. B. acknowledges support from the Lyman Spitzer fellowship. M. N. and F. D. B. acknowledge support from NSF Grants No. AST-1454881 and No. AST-1517049. The development of multichroic detectors and lenses was supported by NASA Grants No. NNX13AE56G and No. NNX14AB58G. C. M. acknowledges support from NASA Grant No. NNX12AM32H. Funding from ERC Grant No. 259505 supports S. N., J. D., E. C., and T. L. H. T. is supported by NASA Grant No. ATP NNX14AB57G, DOE Award No. DE-SC0011114, and NSF Grant No. AST-1312991. B. S. and B. K. are funded by NASA Space Technology research fellowships. R. D. received funding from the CONICYT Grants No. QUIMAL-120001 and No. FONDECYT-1141113. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Award No. DE-AC02-05CH11231. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Institute de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth; Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia; University of Washington, and Yale University. NR 51 TC 6 Z9 6 U1 4 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 11 PY 2016 VL 93 IS 8 AR 082002 DI 10.1103/PhysRevD.93.082002 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI8SF UT WOS:000373770800001 ER PT J AU Agrawal, A Perahia, D Grest, GS AF Agrawal, Anupriya Perahia, Dvora Grest, Gary S. TI Cluster Morphology-Polymer Dynamics Correlations in Sulfonated Polystyrene Melts: Computational Study SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY-SCATTERING; NEUTRON SPIN-ECHO; MOLECULAR-DYNAMICS; POLYELECTROLYTE SOLUTIONS; CATION TYPE; IONOMERS; MODEL; SIMULATIONS; RHEOLOGY; WATER AB Reaching exceptionally long times up to 500 ns in equilibrium and nonequilibrium molecular dynamics simulations studies, we have attained a fundamental molecular understanding of the correlation of ionomer clusters structure and multiscale dynamics, providing new insight into one critical, long-standing challenge in ionic polymer physics. The cluster structure in melts of sulfonated polystyrene with Na+ and Mg2+ counterions are resolved and correlated with the dynamics on multiple length and time scales extracted from measurements of the dynamic structure factor and shear rheology. We find that as the morphology of the ionic clusters changes from ladderlike for Na+ to disordered structures for Mg2+, the dynamic structure factor is affected on the length scale corresponding to the ionic clusters. Rheology studies show that the viscosity for Mg2+ melts is higher than for Na+ ones for all shear rates, which is well correlated with the larger ionic clusters' size for the Mg2+ melts. C1 [Agrawal, Anupriya; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Agrawal, Anupriya] Washington Univ, Dept Mech Engn & Mat Sci, St Louis, MO 63130 USA. [Grest, Gary S.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Agrawal, A (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. FU DOE at Clemson University [DE-SC007908]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Clemson Computing and Information Technology; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We gratefully acknowledge financial support from DOE Grant No. DE-SC007908 at Clemson University. We acknowledge computational resources at the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231 and Clemson Computing and Information Technology. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy and Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 37 TC 2 Z9 2 U1 14 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 11 PY 2016 VL 116 IS 15 AR 158001 DI 10.1103/PhysRevLett.116.158001 PG 6 WC Physics, Multidisciplinary SC Physics GA DI8SZ UT WOS:000373773200007 PM 27127986 ER PT J AU Zhu, DP Cao, Q Qiao, RM Zhu, SM Yang, WL Xia, WX Tian, YF Liu, GL Yan, SS AF Zhu, Dapeng Cao, Qiang Qiao, Ruimin Zhu, Shimeng Yang, Wanli Xia, Weixing Tian, Yufeng Liu, Guolei Yan, Shishen TI Oxygen vacancies controlled multiple magnetic phases in epitaxial single crystal Co-0.5(Mg0.55Zn0.45)(0.5)O1-v thin films SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY-ABSORPTION; DOPED ZNO; TRANSITION; OXIDES; SUPERCONDUCTIVITY; FERROMAGNETISM; SEMICONDUCTORS; COEXISTENCE; INTERFACE; EXCHANGE AB High quality single-crystal fcc-Co-x(MgyZn1-y)(1-x)O1-v epitaxial thin films with high Co concentration up to x = 0.5 have been fabricated by molecular beam epitaxy. Systematic magnetic property characterization and soft X-ray absorption spectroscopy analysis indicate that the coexistence of ferromagnetic regions, superparamagnetic clusters, and non-magnetic boundaries in the as-prepared Co-x(MgyZn1-y)(1-x)O1-v films is a consequence of the intrinsic inhomogeneous distribution of oxygen vacancies. Furthermore, the relative strength of multiple phases could be modulated by controlling the oxygen partial pressure during sample preparation. Armed with both controllable magnetic properties and tunable band-gap, Co-x(MgyZn1-y)(1-x)O1-v films may have promising applications in future spintronics. C1 [Zhu, Dapeng; Cao, Qiang; Tian, Yufeng; Liu, Guolei; Yan, Shishen] Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China. [Qiao, Ruimin; Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Zhu, Shimeng; Xia, Weixing] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China. RP Liu, GL; Yan, SS (reprint author), Shandong Univ, Sch Phys, State Key Lab Crystal Mat, Jinan 250100, Peoples R China. EM liu-guolei@sdu.edu.cn; shishenyan@sdu.edu.cn RI Yang, Wanli/D-7183-2011; Qiao, Ruimin/E-9023-2013 OI Yang, Wanli/0000-0003-0666-8063; FU NSFC [11434006, 11374187]; NBRP of China [2013CB922303, 2015CB921502]; 111 project [B13029]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; LDRD program at the Lawrence Berkeley National Laboratory FX This work was supported by the key program of NSFC No. 11434006, the NBRP of China No. 2013CB922303 and 2015CB921502, 111 project No. B13029, and the general program of NSFC No. 11374187. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Ruimin Qiao is supported by the LDRD program at the Lawrence Berkeley National Laboratory. NR 36 TC 1 Z9 1 U1 5 U2 15 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD APR 11 PY 2016 VL 6 AR 24188 DI 10.1038/srep24188 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI8PV UT WOS:000373764100001 PM 27062992 ER PT J AU D'Arcy, R Alvarez, M Gaynier, J Prost, L Scarpine, V Shemyakin, A AF D'Arcy, R. Alvarez, M. Gaynier, J. Prost, L. Scarpine, V. Shemyakin, A. TI Characterisation of the PXIE Allison-type emittance scanner SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Particle accelerators; Diagnostics; Beam instrumentation; Allison scanner; Emittance; Phase space ID BEAM AB An Allison-type emittance scanner has been designed for PXIE at FNAL with the goal of providing fast and accurate phase space reconstruction. The device has been modified from previous LBNL/SNS designs to operate in both pulsed and DC modes with the addition of water-cooled front slits. Extensive calibration techniques and error analysis allowed confinement of uncertainty to the < 5% level (with known caveats). With a 16-bit, 1 MHz electronics scheme the device is able to analyse a pulse with a resolution of 1 mu s, allowing for analysis of neutralisation effects. This paper describes a detailed breakdown of the R&D, as well as post-run analysis techniques. Published by Elsevier B.V. C1 [D'Arcy, R.; Alvarez, M.; Gaynier, J.; Prost, L.; Scarpine, V.; Shemyakin, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [D'Arcy, R.] UCL, Mortimer St, London WC1E 6BT, England. RP D'Arcy, R (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA.; D'Arcy, R (reprint author), UCL, Mortimer St, London WC1E 6BT, England. EM rtpdarcy@gmail.com FU U.S. DOE [DE-ACO2-07CH11359] FX The work outlined in this paper was operated by Fermi Research Alliance, LLC, under Contract DE-ACO2-07CH11359 with the U.S. DOE. NR 12 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 11 PY 2016 VL 815 BP 7 EP 17 DI 10.1016/j.nima.2016.01.039 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD7UT UT WOS:000370130900002 ER PT J AU Garcia-Sciveres, M Wang, XK AF Garcia-Sciveres, Maurice Wang, Xinkang TI Data encoding efficiency in pixel detector readout with charge information SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Particle tracking detectors (Solid-state detectors); Data acquisition concepts; Electronic detector readout concepts (solid-state); Data reduction methods; Information theory AB The average minimum number of bits needed for lossless readout of a pixel detector is calculated, in the regime of interest for particle physics where only a small fraction of pixels have a non-zero value per frame. This permits a systematic comparison of the readout efficiency of different encoding implementations. The calculation is compared to the number of bits used by the FE-I4 pixel readout chip of the ATLAS experiment. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wang, Xinkang] Univ Chicago, Chicago, IL 60637 USA. [Garcia-Sciveres, Maurice] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Garcia-Sciveres, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM msg@lbl.gov OI Wang, Xinkang/0000-0002-3357-7194 FU Office of High Energy Physics of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported in part by the Office of High Energy Physics of the U.S. Department of Energy under contract DE-AC02-05CH11231. NR 10 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 11 PY 2016 VL 815 BP 18 EP 22 DI 10.1016/j.nima.2016.01.014 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD7UT UT WOS:000370130900003 ER PT J AU Lowry, MM Bass, CD D'Angelo, A Deur, A Dezern, G Hanretty, C Ho, D Kageya, T Kashy, D Khandaker, M Laine, V O'Connell, T Pastor, O Peng, P Sandorfi, AM Sokhan, D Wei, X Zarecky, M AF Lowry, M. M. Bass, C. D. D'Angelo, A. Deur, A. Dezern, G. Hanretty, C. Ho, D. Kageya, T. Kashy, D. Khandaker, M. Laine, V. O'Connell, T. Pastor, O. Peng, P. Sandorfi, A. M. Sokhan, D. Wei, X. Zarecky, M. TI A cryostat to hold frozen-spin polarized HD targets in CLAS: HDice-II SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Dilution refrigerator; Polarized target; Hydrogen deuteride; Frozen-spin target AB The design, fabrication, operation, and performance of a He-3/4 dilution refrigerator and superconducting magnet system for holding a frozen-spin polarized hydrogen deuteride target in the Jefferson Laboratory CLAS detector during photon beam running is reported. The device operates both vertically (for target loading) and horizontally (for target bombardment). The device proves capable of maintaining a base temperature of 50 mK and a holding field of 1 T for extended periods. These characteristics enabled multi-month polarization lifetimes for frozen spin HD targets having proton polarization of up to 50% and deuteron up to 27%. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lowry, M. M.; Bass, C. D.; D'Angelo, A.; Deur, A.; Dezern, G.; Kageya, T.; Kashy, D.; Laine, V.; Pastor, O.; Sandorfi, A. M.; Wei, X.; Zarecky, M.] Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. [D'Angelo, A.] Univ Roma Tor Vergata, Via Ric Sci 1, I-00133 Rome, Italy. [D'Angelo, A.] INFN Sez Roma Tor Vergata, Via Ric Sci 1, I-00133 Rome, Italy. [Hanretty, C.; Peng, P.] Univ Virginia, 1400 Univ Ave, Charlottesville, VA 22903 USA. [Ho, D.] Carnegie Mellon Univ, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. [Khandaker, M.] Norfolk State Univ, 700 Pk Ave, Norfolk, VA 23504 USA. [Laine, V.] Univ Clermont Ferrand, 34 Ave Camot, F-63000 Clermont Ferrand, France. [O'Connell, T.] Univ Connecticut, 115 N Eagleville Rd, Storrs, CT 06269 USA. [Sokhan, D.] Inst Phys Nucl, Bat 100-M053, F-91406 Orsay, France. [Bass, C. D.] Le Moyne Coll, 1419 Salt Springs Rd, Syracuse, NY 13214 USA. [Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. RP Lowry, MM (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM mlowry@jlab.org RI D'Angelo, Annalisa/A-2439-2012 OI D'Angelo, Annalisa/0000-0003-3050-4907 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-060R23177] FX The authors wish to thank J. Alston, D. Anderson, C. Apeldoorn, W. Clemens, J. Dail, J. Dickinson, P. Hemler, D. McCay, R.W. Teachey, S. Williams, D. Tilles and the Jefferson Lab Hall-B technical crew for their dedicated assistance during the design, construction and commissioning of the in-beam cryostat described herein. A. Comer and the Jefferson Lab Target Group provided invaluable assistance in the design and in fabrication of the copper sinters and tubing spirals. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract DE-AC05-060R23177. NR 12 TC 0 Z9 0 U1 3 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 11 PY 2016 VL 815 BP 31 EP 41 DI 10.1016/j.nima.2015.12.063 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD7UT UT WOS:000370130900005 ER PT J AU Senderovich, I Morrison, BT Dugger, M Ritchie, BG Pasyuk, E Tucker, R Brock, J Carlin, C Keith, CD Meekins, DG Seely, ML Ronchen, D Doring, M Collins, P Adhikari, KP Adikaram, D Akbar, Z Anderson, MD Pereira, SA Badui, RA Ball, J Baltzell, NA Battaglieri, M Batourine, V Bedlinskiy, I Biselli, AS Boiarinov, S Briscoe, WJ Brooks, WK Burkert, VD Carman, DS Celentano, A Chandavar, S Charles, G Colaneri, L Cole, PL Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Dupre, R Egiyan, H El Alaoui, A El Fassi, L Elouadrhiri, L Eugenio, P Fedotov, G Fegan, S Filippi, A Fleming, JA Fradi, A Garillon, B Ghandilyan, Y Gilfoyle, GP Giovanetti, KL Girod, FX Glazier, DI Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guidal, M Guo, L Hafidi, K Hakobyan, H Hanretty, C Hattawy, M Hicks, K Ho, D Holtrop, M Hughes, SM Ilieva, Y Ireland, DG Ishkhanov, BS Jenkins, D Jiang, H Jo, HS Joo, K Joosten, S Keller, D Khachatryan, G Khandaker, M Kim, A Klein, FJ Kubarovsky, V Kunkel, MC Lenisa, P Livingston, K Lu, HY MacGregor, IJD Mattione, P McKinnon, B Meyer, CA Mineeva, T Mokeev, V Montgomery, RA Movsisyan, A Camacho, CM Nadel-Turonski, P Net, LA Niccolai, S Niculescu, G Niculescu, I Osipenko, M Park, K Park, S Peng, P Phelps, W Pisano, S Pogorelko, O Price, JW Prok, Y Puckett, AJR Ripani, M Rizzo, A Rosner, G Roy, P Sabatie, F Salgado, C Schott, D Schumacher, RA Seder, E Simonyan, A Skorodumina, I Smith, GD Sober, DI Sparveris, N Stepanyan, S Stoler, P Strakovsky, II Strauch, S Sytnik, V Tian, Y Ungaro, M Voskanyan, H Voutier, E Walford, NK Wei, X Wood, MH Zachariou, N Zana, L Zhang, J Zhao, ZW Zonta, I AF Senderovich, I. Morrison, B. T. Dugger, M. Ritchie, B. G. Pasyuk, E. Tucker, R. Brock, J. Carlin, C. Keith, C. D. Meekins, D. G. Seely, M. L. Roenchen, D. Doering, M. Collins, P. Adhikari, K. P. Adikaram, D. Akbar, Z. Anderson, M. D. Pereira, S. Anefalos Badui, R. A. Ball, J. Baltzell, N. A. Battaglieri, M. Batourine, V. Bedlinskiy, I. Biselli, A. S. Boiarinov, S. Briscoe, W. J. Brooks, W. K. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Charles, G. Colaneri, L. Cole, P. L. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Elouadrhiri, L. Eugenio, P. Fedotov, G. Fegan, S. Filippi, A. Fleming, J. A. Fradi, A. Garillon, B. Ghandilyan, Y. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Glazier, D. I. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guidal, M. Guo, L. Hafidi, K. Hakobyan, H. Hanretty, C. Hattawy, M. Hicks, K. Ho, D. Holtrop, M. Hughes, S. M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Jenkins, D. Jiang, H. Jo, H. S. Joo, K. Joosten, S. Keller, D. Khachatryan, G. Khandaker, M. Kim, A. Klein, F. J. Kubarovsky, V. Kunkel, M. C. Lenisa, P. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Mattione, P. McKinnon, B. Meyer, C. A. Mineeva, T. Mokeev, V. Montgomery, R. A. Movsisyan, A. Camacho, C. Munoz Nadel-Turonski, P. Net, L. A. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Park, K. Park, S. Peng, P. Phelps, W. Pisano, S. Pogorelko, O. Price, J. W. Prok, Y. Puckett, A. J. R. Ripani, M. Rizzo, A. Rosner, G. Roy, P. Sabatie, F. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Simonyan, A. Skorodumina, Iu. Smith, G. D. Sober, D. I. Sparveris, N. Stepanyan, S. Stoler, P. Strakovsky, I. I. Strauch, S. Sytnik, V. Tian, Ye Ungaro, M. Voskanyan, H. Voutier, E. Walford, N. K. Wei, X. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. Zonta, I. TI First measurement of the helicity asymmetry E in eta photoproduction on the proton SO PHYSICS LETTERS B LA English DT Article DE Eta photoproduction; Polarization observable; Helicity asymmetry ID I-CIRCLE-DOT; CLAS; PHOTON; BEAM; BREMSSTRAHLUNG; BARYONS; SYSTEM AB Results are presented for the first measurement of the double-polarization helicity asymmetry E for the eta photoproduction reaction gamma p -> eta p. Data were obtained using the FROzen Spin Target (FROST) with the CLAS spectrometer in Hall B at Jefferson Lab, covering a range of center-of-mass energy W from threshold to 2.15 GeV and a large range in center-of-mass polar angle. As an initial application of these data, the results have been incorporated into the Julich-Bonn model to examine the case for the existence of a narrow N* resonance between 1.66 and 1.70 GeV. The addition of these data to the world database results in marked changes in the predictions for the Eobservable from that model. Further comparison with several theoretical approaches indicates these data will significantly enhance our understanding of nucleon resonances. (C) 2016 Published by Elsevier B.V. C1 [Baltzell, N. A.; Hafidi, K.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Senderovich, I.; Morrison, B. T.; Dugger, M.; Ritchie, B. G.; Pasyuk, E.; Tucker, R.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. [Ho, D.; Mattione, P.; Meyer, C. A.; Schumacher, R. A.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Collins, P.; Klein, F. J.; Nadel-Turonski, P.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Ball, J.; Celentano, A.; D'Angelo, A.; Girod, F. X.; Sabatie, F.] CEA, Ctr Saclay, Irfu, Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Joo, K.; Kim, A.; Puckett, A. J. R.; Seder, E.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Badui, R. A.; Guo, L.; Phelps, W.; Schott, D.] Florida Int Univ, Miami, FL 33199 USA. [Akbar, Z.; Crede, V.; Eugenio, P.; Hanretty, C.; Park, S.; Roy, P.] Florida State Univ, Tallahassee, FL 32306 USA. [Briscoe, W. J.; Ilieva, Y.; Nadel-Turonski, P.; Strakovsky, I. I.] George Washington Univ, Washington, DC 20052 USA. [Cole, P. L.; Cortes, O.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Movsisyan, A.; Simonyan, A.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [De Sanctis, E.; Montgomery, R. A.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Colaneri, L.; D'Angelo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Filippi, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Torino, Italy. [Charles, G.; Dupre, R.; Fradi, A.; Garillon, B.; Hattawy, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Voutier, E.] CNRS, Inst Phys Nucl, IN2P3, F-91405 Orsay, France. [Charles, G.; Dupre, R.; Fradi, A.; Garillon, B.; Guidal, M.; Hattawy, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Voutier, E.] Univ Paris 11, Orsay, France. [Bedlinskiy, I.; Pogorelko, O.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Park, K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Egiyan, H.; Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Keller, D.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; El Fassi, L.; Zhang, J.] Old Dominion Univ, Norfolk, VA 23529 USA. [Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Skorodumina, Iu.; Zonta, I.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Mokeev, V.; Skorodumina, Iu.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119234, Russia. [Baltzell, N. A.; Djalali, C.; Gothe, R. W.; Jiang, H.; Lu, H. Y.; Mokeev, V.; Net, L. A.; Park, K.; Strauch, S.; Tian, Ye; Wood, M. H.; Zachariou, N.; Zhao, Z. W.] Univ S Carolina, Columbia, SC 29208 USA. [Joosten, S.; Sparveris, N.] Temple Univ, Philadelphia, PA 19122 USA. [Brock, J.; Carlin, C.; Keith, C. D.; Meekins, D. G.; Seely, M. L.; Doering, M.; Batourine, V.; Boiarinov, S.; Burkert, V. D.; Carman, D. S.; Deur, A.; Elouadrhiri, L.; Girod, F. X.; Guo, L.; Kubarovsky, V.; Stepanyan, S.; Wei, X.; Zhao, Z. W.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [El Alaoui, A.; Sytnik, V.] Univ Tecn Federico Santa Maria, Casilla 110-5, Valparaiso, Chile. [Fleming, J. A.; Hughes, S. M.; Smith, G. D.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Anderson, M. D.; Glazier, D. I.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Rosner, G.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Jenkins, D.] Virginia Tech, Blacksburg, VA 24061 USA. [Peng, P.; Prok, Y.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Dashyan, N.; Ghandilyan, Y.; Hakobyan, H.; Lenisa, P.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Pereira, S. Anefalos; Kunkel, M. C.] Forschungszentrum Julich, Inst Kernphys, D-52425 Julich, Germany. [Mineeva, T.] Univ Waterloo, Inst Quantum Comp, Waterloo, ON N2L 3G1, Canada. [Roenchen, D.] Univ Bonn, HISKP, D-53115 Bonn, Germany. [Roenchen, D.] Univ Bonn, BCTP, D-53115 Bonn, Germany. RP Ritchie, BG (reprint author), Arizona State Univ, Tempe, AZ 85287 USA. EM senderov@jlab.org; barry.ritchie@asu.edu RI Celentano, Andrea/J-6190-2012; Meyer, Curtis/L-3488-2014; Schumacher, Reinhard/K-6455-2013; Brooks, William/C-8636-2013; D'Angelo, Annalisa/A-2439-2012 OI Celentano, Andrea/0000-0002-7104-2983; Meyer, Curtis/0000-0001-7599-3973; Schumacher, Reinhard/0000-0002-3860-1827; Brooks, William/0000-0001-6161-3570; D'Angelo, Annalisa/0000-0003-3050-4907 FU National Science Foundation; JSC(JUROPA); French Centre National de la Recherche Scientifique; Commissariat a l'Energie Atomique; Italian Istituto Nazionale di Fisica Nucleare; Chilean Comision Nacional de Investigacion Cientifica y Tecnologica; Science and Technology Facilities Council of the United Kingdom; National Research Foundation of Korea; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177] FX The authors gratefully acknowledge the work of the Jefferson Lab staff, as well as the support by the National Science Foundation, the JSC(JUROPA) facility at FZ Julich, the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the Italian Istituto Nazionale di Fisica Nucleare, the Chilean Comision Nacional de Investigacion Cientifica y Tecnologica, the Science and Technology Facilities Council of the United Kingdom, and the National Research Foundation of Korea. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract DE-AC05-06OR23177. NR 33 TC 5 Z9 5 U1 7 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 64 EP 69 DI 10.1016/j.physletb.2016.01.044 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100011 ER PT J AU Degrande, C Fuks, B Hirschi, V Proudom, J Shao, HS AF Degrande, Celine Fuks, Benjamin Hirschi, Valentin Proudom, Josselin Shao, Hua-Sheng TI Matching next-to-leading order predictions to parton showers in supersymmetric QCD SO PHYSICS LETTERS B LA English DT Article ID HADRON COLLIDERS; PHENOMENOLOGY; PHYSICS; LEVEL; MODEL AB We present a fully automated framework based on the FEYNRULES and MADGRAPH5_aMC@NLO programs that allows for accurate simulations of supersymmetric QCD processes at the LHC. Starting directly from a model Lagrangian that features squark and gluino interactions, event generation is achieved at the next-to-leading order in QCD, matching short-distance events to parton showers and including the subsequent decay of the produced supersymmetric particles. As an application, we study the impact of higher-order corrections in gluino pair-production in a simplified benchmark scenario inspired by current gluino LHC searches. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Degrande, Celine] Univ Durham, Dept Phys, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. [Fuks, Benjamin] Univ Paris 06, Sorbonne Univ, UMR 7589, LPTHE, F-75005 Paris, France. [Fuks, Benjamin] CNRS, UMR 7589, LPTHE, F-75005 Paris, France. [Hirschi, Valentin] SLAC, Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Proudom, Josselin] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, 53 Ave Martyrs, F-38026 Grenoble, France. [Shao, Hua-Sheng] CERN, PH TH, CH-1211 Geneva 23, Switzerland. RP Fuks, B (reprint author), LPTHE CNRS UPMC, Box 126,T13-14 Fourth Floor,4 Pl Jussieu, F-75252 Paris 5, France. EM fuks@lpthe.jussieu.fr OI Fuks, Benjamin/0000-0002-0041-0566 FU ERC [291377]; Research Executive Agency of the European Union [PITN-GA-2012-315877]; Theory-LHC-France initiative of the CNRS (INP/IN2P3); SNF grant [PBELP2 146525]; Investissements d'avenir, Labex ENIGMASS FX We are grateful to R. Frederix, S. Frixione, F. Maltoni and O. Mattelaer for enlightening discussions. This work has been supported in part by the ERC grant 291377 LHCtheory: Theoretical predictions and analyses of LHC physics: advancing the precision frontier, the Research Executive Agency of the European Union under Grant Agreement PITN-GA-2012-315877 (MCNet) and the Theory-LHC-France initiative of the CNRS (INP/IN2P3). C.D. is a Durham International Junior Research Fellow, V.H. is supported by the SNF grant PBELP2 146525 and J.P. by a PhD grant of the Investissements d'avenir, Labex ENIGMASS. NR 39 TC 2 Z9 2 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 82 EP 87 DI 10.1016/j.physletb.2016.01.067 PG 6 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100014 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van 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Kaplan, S. Lath, A. Panwalkar, S. Park, M. Patel, R. Salur, S. Schnetzer, S. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Rose, A. Safonov, A. Suarez, I. Tatarinov, A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Verwilligen, P. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for new phenomena in monophoton final states in proton-proton collisions at root s=8 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Monophoton; Dark matter ID E(+)E(-) COLLISIONS; MISSING ENERGY; DARK-MATTER; SINGLE-PHOTON; EVENTS; DIMENSIONS; COLLIDERS; LEP AB Results are presented from a search for new physics in final states containing a photon and missing transverse momentum. The data correspond to an integrated luminosity of 19.6 fb(-1) collected in proton-proton collisions at root s = 8 TeV with the CMS experiment at the LHC. Nodeviation from the standard model predictions is observed for these final states. New, improved limits are set on dark matter production and on parameters of models with large extra dimensions. In particular, the first limits from the LHC on branon production are found and significantly extend previous limits from LEP and the Tevatron. An upper limit of 14.0 fb on the cross section is set at the 95% confidence level for events with a monophoton final state with photon transverse momentum greater than 145 GeV and missing transverse momentum greater than 140 GeV. (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. 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[Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Galanti, M.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Tosi, S.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Galanti, M.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. 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[Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. 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[Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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[Leonard, A.; Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J. R. Marco; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Sharma, A.; Silvestris, L.; Giordano, F.; Gori, V.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Vernieri, C.; Micheli, F.; Soffi, L.; Casasso, S.; Obertino, M. M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazque; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Harris, P.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. 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[Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Malik, S.; Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. 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A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Radi, A.] Sultan Qaboos Univ, Muscat, Oman. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Marfin, I.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. 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RI Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Haj Ahmad, Wael/E-6738-2016; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Stahl, Achim/E-8846-2011; Smirnov, Vitaly/B-5001-2017; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014 OI Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Stahl, Achim/0000-0002-8369-7506; ciocci, maria agnese /0000-0003-0002-5462; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787 FU BMWFW (Austria); FWF (Austria); Fonds De La Recherche Scientifique - FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); Fonds De La Recherche Scientifique - FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 70 TC 23 Z9 23 U1 36 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 102 EP 124 DI 10.1016/j.physletb.2016.01.057 PG 23 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100018 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q 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Kaplan, S. Elayavalli, R. Kunnawalkam Lath, A. Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Montalvo, R. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for W ' decaying to tau lepton and neutrino in proton-proton collisions at root s=8 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; W ' decays ID TOP-QUARK; MODEL AB The first search for a heavy charged vector boson in the final state with a tau lepton and a neutrino is reported, using 19.7 fb(-1) of LHC data at root s = 8 TeV. A signal would appear as an excess of events with high transverse mass, where the standard model background is low. No excess is observed. Limits are set on a model in which the W' decays preferentially to fermions of the third generation. These results substantially extend previous constraints on this model. Masses below 2.0 to 2.7 TeV are excluded, depending on the model parameters. In addition, the existence of a W' boson with universal fermion couplings is excluded at 95% confidence level, for W' masses below 2.7 TeV. For further reinterpretation a model-independent limit on potential signals for various transverse mass thresholds is also presented. (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Kassel, F.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Roy Chowdhury, S.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Banerjee, S.; Aziz, T.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] Indian Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Maggi, G.; Maggi, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, M.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Abdulsalam, A.; Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, Turin, Torino, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Torino, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Son, D. C.; Malakhov, A.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Wan Abdullah, W. A. T.; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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[Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De La Cruz, B.; Peris, A. Delgado; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; De Martino, E. Navarro; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kassel, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; du Pree, T.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; Seif El Nasr-Storey, S.; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Vazquez Acosta, M.; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.; Brinkerhoff, A.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Sandoval Gonzalez, I. D.; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Nash, K.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Baskakov, A.; Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Abdulsalam, A.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Montalvo, R.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Roe, J.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. 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RI Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; OI Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Silvestris, Lucia/0000-0002-8985-4891; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MOST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MOST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 41 TC 4 Z9 4 U1 17 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 196 EP 216 DI 10.1016/j.physletb.2016.02.002 PG 21 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100030 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hormann, CHN Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Gay, APR Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, 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Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Searches for a heavy scalar boson H decaying to a pair of 125 GeV Higgs bosons hh or for a heavy pseudoscalar boson A decaying to Zh, in the final states with h -> tau tau SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; MSSM; tau; Higgs ID MINIMAL SUPERSYMMETRIC MODEL; SOFTLY BROKEN SUPERSYMMETRY; STANDARD MODEL; ATLAS DETECTOR; MSSM; LHC; PARTICLE; MASSES; PARAMETERS; BREAKING AB A search for a heavy scalar boson H decaying into a pair of lighter standard-model-like 125 GeV Higgs bosons hh and a search for a heavy pseudoscalar boson A decaying into a Z and an h boson are presented. The searches are performed on a data set corresponding to an integrated luminosity of 19.7 fb(-1) of pp collision data at a centre-of-mass energy of 8 TeV, collected by CMS in 2012. A final state consisting of two tau leptons and two b jets is used to search for the H -> hh decay. A final state consisting of two tau leptons from the h boson decay, and two additional leptons from the Z boson decay, is used to search for the decay A -> Zh. The results are interpreted in the context of two-Higgs-doublet models. No excess is found above the standard model expectation and upper limits are set on the heavy boson production cross sections in the mass ranges 260 < m(H) < 350 GeV and 220 < m(A) < 350 GeV. (C) 2016 CERN for the benefit of the CMS Collaboration. Published by Elsevier B.V. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Hartl, C.; Hoermann, N.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Ochesanu, S.; Rougny, R.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. 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[Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow 115409, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Ctr Nat Sci, UA-310108 Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Vazquez Acosta, M.; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Abdulsalam, A.; Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Parashar, N.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.; Eusebi, R.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Finger, M.; Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Abdelalim, A. A.; Mahrous, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [El Sawy, M.] Beni Suef Univ, Bani Sweif, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, D-03044 Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-de La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Univ, St Petersburg 199034, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Vazquez Acosta, M.] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Vilela Pereira, Antonio/L-4142-2016; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Tinoco Mendes, Andre David/D-4314-2011; VARDARLI, Fuat Ilkehan/B-6360-2013; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014 OI Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Luukka, Panja/0000-0003-2340-4641; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Vilela Pereira, Antonio/0000-0003-3177-4626; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MOST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis and Aristeia programmes - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship; Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MOST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 80 TC 10 Z9 10 U1 24 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 217 EP 244 DI 10.1016/j.physletb.2016.01.056 PG 28 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100031 ER PT J AU Aad, G Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T 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CA Atlas Collaboration TI Combination of searches for WW, WZ, and ZZ resonances in pp collisions at root s=8 TeV with the ATLAS detector SO PHYSICS LETTERS B LA English DT Article ID HADRON COLLIDERS; STANDARD MODEL; HIGGS-BOSON; LHC; PHYSICS; MASS AB The ATLAS experiment at the CERN Large Hadron Collider has performed searches for new, heavy bosons decaying to WW, WZ and ZZ final states in multiple decay channels using 20.3 fb(-1) of pp collision data at root s = 8 TeV. In the current study, the results of these searches are combined to provide a more stringent test of models predicting heavy resonances with couplings to vector bosons. Direct searches for a charged diboson resonance decaying to WZ in the l nu l'l' (l = mu, e), llq (q) over bar, l nu q (q) over bar and fully hadronic final states are combined and upper limits on the rate of production times branching ratio to the WZ bosons are compared with predictions of an extended gauge model with a heavy W' boson. In addition, direct searches for a neutral diboson resonance decaying to WW and ZZ in the llq (q) over bar, l nu q (q) over bar, and fully hadronic final states are combined and upper limits on the rate of production times branching ratio to the WW and ZZ bosons are compared with predictions for a heavy, spin-2 graviton in an extended Randall-Sundrum model where the Standard Model fields are allowed to propagate in the bulk of the extra dimension. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. 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A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkins, A. D.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyolab, J. E.; Tapia Arayab, S.; Whiteb, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gaob, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, L.; Liu, M.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Du, Y.; Feng, C.; Ge, P.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettinia, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gaudio, G.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausena, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Aloisio, A.; Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, A.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, A.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Scanlon, T.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitt, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducub, O. A.; Feligioni, L.; Gaob, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Antonov, A.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducub, O. A.; Feligioni, L.; Gaob, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Aloisio, A.; Alonso, A.; Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schorlemmer, A. L. S.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besanaa, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. 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N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Poley, A.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Di Donato, C.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, M.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araquea, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Aloisio, A.; Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys Protvino, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, P.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvoa, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Varia, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gauzzi, P.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [ElKacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Cherkaoui El Mourslie, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Strauss, M.; Su, D.; Tompkins, L.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garciac, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolina, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolina, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Liu, B.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, D.; Mori, T.; Morinaga, M.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Aloisio, A.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Hernandez, D. Paredes; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; Le Blanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Banerjee, Sw.] Univ Louisville, Dept Phys & Astron, Louisville, KY 40292 USA. Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] Inst Catalana Rec & Estud Avancats, ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] State Univ, Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Martinez, Mario /I-3549-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Gerbaudo, Davide/J-4536-2012; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Brooks, William/C-8636-2013; Zhukov, Konstantin/M-6027-2015; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Maneira, Jose/D-8486-2011; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; Guo, Jun/O-5202-2015; Gladilin, Leonid/B-5226-2011; BESSON, NATHALIE/L-6250-2015; Warburton, Andreas/N-8028-2013; Vanadia, Marco/K-5870-2016; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016; Mitsou, Vasiliki/D-1967-2009; Smirnova, Oxana/A-4401-2013 OI Prokofiev, Kirill/0000-0002-2177-6401; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; KUBOTA, TAKASHI/0000-0002-1156-5571; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Gerbaudo, Davide/0000-0002-4463-0878; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Brooks, William/0000-0001-6161-3570; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Maneira, Jose/0000-0002-3222-2738; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Guo, Jun/0000-0001-8125-9433; Gladilin, Leonid/0000-0001-9422-8636; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620; Mitsou, Vasiliki/0000-0002-1533-8886; Smirnova, Oxana/0000-0003-2517-531X FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States; NSF, United States; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, FP7, Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales programme; Aristeia programme - EU-ESF; Greek NSRF, Israel; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 71 TC 16 Z9 16 U1 29 U2 53 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 285 EP 305 DI 10.1016/j.physletb.2016.02.015 PG 21 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100040 ER PT J AU Sanetullaev, A Kanungo, R Tanaka, J Alcorta, M Andreoiu, C Bender, P Chen, AA Christian, G Davids, B Fallis, J Fortin, JP Galinski, N Gallant, AT Garrett, PE Hackman, G Hadinia, B Ishimoto, S Keefe, M Krucken, R Lighthall, J McNeice, E Miller, D Purcell, J Randhawa, JS Roger, T Rojas, A Savajols, H Shotter, A Tanihata, I Thompson, IJ Unsworth, C Voss, P Wang, Z AF Sanetullaev, A. Kanungo, R. Tanaka, J. Alcorta, M. Andreoiu, C. Bender, P. Chen, A. A. Christian, G. Davids, B. Fallis, J. Fortin, J. P. Galinski, N. Gallant, A. T. Garrett, P. E. Hackman, G. Hadinia, B. Ishimoto, S. Keefe, M. Kruecken, R. Lighthall, J. McNeice, E. Miller, D. Purcell, J. Randhawa, J. S. Roger, T. Rojas, A. Savajols, H. Shotter, A. Tanihata, I. Thompson, I. J. Unsworth, C. Voss, P. Wang, Z. TI Investigation of the role of Li-10 resonances in the halo structure of Li-11 through the Li-11(p, d)Li-10 transfer reaction SO PHYSICS LETTERS B LA English DT Article DE Halo nucleus; Li-10,Li-11; Transfer reaction; Inverse kinematics; DWBA; Spectroscopic factor ID DRIP-LINE; NUCLEI; FRAGMENTATION; SPECTROSCOPY; POPULATION; STATES AB The first measurement of the one-neutron transfer reaction Li-11(p,d)Li-10 performed using the IRIS facility at TRIUMF with a 5.7A MeV Li-11 beam interacting with a solid H-2 target is reported. The Li-10 residue was populated strongly as a resonance peak with energy E-r = 0.62 +/- 0.04 MeV having a total width Gamma = 0.33 +/- 0.07 MeV. The angular distribution of this resonance is characterized by neutron occupying the 1p(1/2) orbital. A DWBA analysis yields a spectroscopic factor of 0.67 +/- 0.12 for p(1/2) removal strength from the ground state of Li-11 to the region of the peak. (C) 2016 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license. C1 [Sanetullaev, A.; Kanungo, R.; Fortin, J. P.; Keefe, M.; Purcell, J.; Randhawa, J. S.] St Marys Univ, Dept Phys & Astron, Halifax, NS B3H 3C3, Canada. [Sanetullaev, A.; Alcorta, M.; Bender, P.; Christian, G.; Davids, B.; Fallis, J.; Galinski, N.; Gallant, A. T.; Hackman, G.; Kruecken, R.; Lighthall, J.; Miller, D.; Rojas, A.; Unsworth, C.; Wang, Z.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Tanaka, J.; Tanihata, I.] Osaka Univ, RCNP, Ibaraki, Osaka 5670047, Japan. [Andreoiu, C.; Wang, Z.] Simon Fraser Univ, Dept Chem, Burnaby, BC V5A 1S6, Canada. [Chen, A. A.; McNeice, E.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Fortin, J. P.] Univ Laval, Dept Phys, Quebec City, PQ G1V 0A8, Canada. [Garrett, P. E.; Hadinia, B.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Ishimoto, S.] High Energy Accelerator Res Org, KEK, Ibaraki 3050801, Japan. [Kruecken, R.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Roger, T.; Savajols, H.] CEA, CNRS, IN2P3, Grand Accelerateur Natl Ions Lourds,DSM, BP 55027, F-14076 Caen 5, France. [Shotter, A.] Univ Edinburgh, Edinburgh, Midlothian, Scotland. [Tanihata, I.] Beihang Univ, Sch Phys & Nucl Energy Engn, Beijing 100191, Peoples R China. [Tanihata, I.] Beihang Univ, IRCNPC, Beijing 100191, Peoples R China. [Thompson, I. J.] Lawrence Livermore Natl Lab, L-414, Livermore, CA 94551 USA. [Sanetullaev, A.] Inha Univ Tashkent, Tashkent, Uzbekistan. RP Kanungo, R (reprint author), St Marys Univ, Dept Phys & Astron, Halifax, NS B3H 3C3, Canada. EM ritu@triumf.ca RI Kruecken, Reiner/A-1640-2013 OI Kruecken, Reiner/0000-0002-2755-8042 NR 33 TC 4 Z9 4 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD APR 10 PY 2016 VL 755 BP 481 EP 485 DI 10.1016/j.physletb.2016.02.060 PG 5 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5VH UT WOS:000373568100073 ER PT J AU Robertson, C AF Robertson, Claire TI The extracellular matrix in breast cancer predicts prognosis through composition, splicing, and crosslinking SO EXPERIMENTAL CELL RESEARCH LA English DT Review DE Extracellular matrix; Breast cancer; Splicing; Microstructure ID CARCINOMA IN-SITU; MAMMARY EPITHELIAL-CELLS; SHEAR-WAVE ELASTOGRAPHY; GENE-EXPRESSION SIGNATURE; EXTRA-DOMAIN B; NEOADJUVANT CHEMOTHERAPY; BASEMENT-MEMBRANE; TENASCIN-C; TUMOR MICROENVIRONMENT; FUNCTIONAL-DIFFERENTIATION AB The extracellular matrix in the healthy breast has an important tumor suppressive role, whereas the abnormal ECM in tumors can promote aggressiveness, and has been linked to breast cancer relapse, survival and resistance to chemotherapy. This review article gives an overview of the elements of the ECM which have been linked to prognosis of breast cancers, including changes in ECM protein composition, splicing, and microstructure. Published by Elsevier Inc. C1 [Robertson, Claire] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd MS 977, Berkeley, CA 94720 USA. RP Robertson, C (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd MS 977, Berkeley, CA 94720 USA. EM Crobertson@lbl.gov FU DOD Breast Cancer Research Program [BC133875]; L'Oreal USA for women in science program FX Thanks to Mina Bissell for her continued mentorship and support. Thanks to Amir Jaberi, Rosalyn Sayaman, Elizabeth Yu for assistance with literature search and editing. This work was supported by DOD Breast Cancer Research Program (BC133875) and the L'Oreal USA for women in science program. NR 146 TC 1 Z9 1 U1 5 U2 9 PU ELSEVIER INC PI SAN DIEGO PA 525 B STREET, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0014-4827 EI 1090-2422 J9 EXP CELL RES JI Exp. Cell Res. PD APR 10 PY 2016 VL 343 IS 1 SI SI BP 73 EP 81 DI 10.1016/j.yexcr.2015.11.009 PG 9 WC Oncology; Cell Biology SC Oncology; Cell Biology GA DL2WF UT WOS:000375495200012 PM 26597760 ER PT J AU Gnedin, NY AF Gnedin, Nickolay Y. TI COSMIC REIONIZATION ON COMPUTERS: NUMERICAL AND PHYSICAL CONVERGENCE SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: theory; galaxies: formation; intergalactic medium; large-scale structure of universe; methods: numerical ID KENNICUTT-SCHMIDT RELATION; STAR-FORMATION RELATION; NEARBY DISK GALAXIES; MOLECULAR GAS; LOW-METALLICITY; KPC SCALES; PROJECT; HISTORY; SIMULATIONS; UNIVERSE AB In this paper I show that simulations of reionization performed under the Cosmic Reionization On Computers project do converge in space and mass, albeit rather slowly. A fully converged solution (for a given star formation and feedback model) can be determined at a level of precision of about 20%, but such a solution is useless in practice, since achieving it in production-grade simulations would require a large set of runs at various mass and spatial resolutions, and computational resources for such an undertaking are not yet readily available. In order to make progress in the interim, I introduce a weak convergence correction factor in the star formation recipe, which allows one to approximate the fully converged solution with finite-resolution simulations. The accuracy of weakly converged simulations approaches a comparable, similar to 20% level of precision for star formation histories of individual galactic halos and other galactic properties that are directly related to star formation rates, such as. stellar masses and metallicities. Yet other properties of model galaxies, for example, their H I masses, are recovered in the weakly converged runs only within a factor of 2. C1 [Gnedin, Nickolay Y.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Gnedin, Nickolay Y.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gnedin, Nickolay Y.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. RP Gnedin, NY (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. EM gnedin@fnal.gov NR 28 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 10 PY 2016 VL 821 IS 1 AR 50 DI 10.3847/0004-637X/821/1/50 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9GB UT WOS:000373809000050 ER PT J AU Kasen, D Metzger, BD Bildsten, L AF Kasen, Daniel Metzger, Brian D. Bildsten, Lars TI MAGNETAR-DRIVEN SHOCK BREAKOUT AND DOUBLE-PEAKED SUPERNOVA LIGHT CURVES SO ASTROPHYSICAL JOURNAL LA English DT Article DE shock waves; stars: magnetars; stars: neutron; supernovae: general ID PULSAR WIND NEBULAE; CORE-COLLAPSE SUPERNOVAE; GAMMA-RAY BURSTS; SUPERLUMINOUS SUPERNOVAE; LUMINOUS SUPERNOVAE; PAIR-INSTABILITY; IC SUPERNOVAE; MASS-LOSS; GRB JETS; STAR AB The light curves of some luminous supernovae are suspected to be powered by the spindown energy of a rapidly rotating magnetar. Here we describe a possible signature of the central engine: a burst of shock breakout emission occurring several. days after the supernova explosion. The energy input from the magnetar inflates a high-pressure bubble that drives a shock through the pre-exploded supernova ejecta. If the magnetar is powerful enough, that shock will near the ejecta surface and become radiative. At the time of shock breakout, the ejecta will have expanded to a large radius (similar to 10(14) cm) so that the radiation released is at optical/ultraviolet wavelengths (T-eff approximate to 20,000 K) and lasts for several days. The luminosity and timescale of this magnetar-driven shock breakout are similar to the first peak observed recently in the double-peaked light curve of SN-LSQ14BDQ. However, for a large region of model parameter space, the breakout emission is predicted to be dimmer than the diffusive luminosity from direct magnetar heating. A distinct double-peaked light curve may therefore only be conspicuous if thermal heating from the magnetar is suppressed at early times. We describe how such a delay in heating may naturally result from inefficient dissipation and thermalization of the pulsar wind magnetic energy. Without such suppression, the breakout may only be noticeable as a small bump or kink in the early luminosity or color evolution, or as a small but abrupt rise in the photospheric velocity. A similar breakout signature may accompany other central engines in supernovae, such as a black hole accreting fallback material. C1 [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Metzger, Brian D.] Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. [Bildsten, Lars] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Bildsten, Lars] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP Kasen, D (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Kasen, D (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Kasen, D (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. FU Department of Energy Office of Nuclear Physics Early Career Award; NSF [AST-1410950, PHYS-1066293]; Alfred P. Sloan Foundation; National Science Foundation [PHY 11-25915, AST 11-09174, AST 12-05574]; Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Roger Chevalier, Tony Piro, Eliot Quataert, Stephen Smartt, Tuguldor Sukhbold, and Stan Woosley for helpful conversations and comments on the draft, and Matt Nicholl for providing the bolometric light-curve data for SN-LSQ14BDQ. D.K. is supported in part by a Department of Energy Office of Nuclear Physics Early Career Award, and by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. B.D.M. gratefully acknowledges support from the NSF grant AST-1410950 and the Alfred P. Sloan Foundation. This work was supported by the National Science Foundation under grants PHY 11-25915, AST 11-09174, and AST 12-05574. This work was supported in part by NSF Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. NR 53 TC 6 Z9 6 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 10 PY 2016 VL 821 IS 1 AR 36 DI 10.3847/0004-637X/821/1/36 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9GB UT WOS:000373809000036 ER PT J AU Kong, XL Chen, Y Guo, F Feng, SW Du, GH Li, G AF Kong, Xiangliang Chen, Yao Guo, Fan Feng, Shiwei Du, Guohui Li, Gang TI ELECTRON ACCELERATION AT A CORONAL SHOCK PROPAGATING THROUGH A LARGE-SCALE STREAMER-LIKE MAGNETIC FIELD SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; shock waves; Sun: coronal mass ejections (CMEs); Sun: radio radiation ID II RADIO-BURST; WHITE-LIGHT OBSERVATIONS; MASS-EJECTION; PARTICLE-ACCELERATION; COLLISIONLESS SHOCKS; INTERPLANETARY SHOCK; DRIFT ACCELERATION; SOURCE REGION; DRIVEN SHOCK; SOLAR-WIND AB Using a test-particle simulation, we investigate the effect of large-scale coronal magnetic fields on electron acceleration at an outward-propagating coronal shock with a circular front. The coronal field is approximated by an analytical solution with a streamer-like magnetic field featuring a partially open magnetic field and a current sheet at the equator atop the closed region. We show that the large-scale shock-field configuration, especially the relative curvature of the shock and the magnetic field line across which the shock is sweeping, plays an important role in the efficiency of electron acceleration. At low shock altitudes, when the shock curvature is larger than that of the magnetic field lines, the electrons are mainly accelerated at the shock flanks; at higher altitudes, when the shock curvature is smaller, the electrons are mainly accelerated at the shock nose around the top of closed field lines. The above process reveals the shift of the efficient electron acceleration region along the shock front during its propagation. We also find that, in general, the electron acceleration at the shock flank is not as efficient as that at the top of the closed field because a collapsing magnetic trap can be formed at the top. In addition, we find that the energy spectra of electrons are power-law-like, first hardening then softening with the spectral index varying in a range of -3 to -6. Physical interpretations of the results and implications for the study of solar radio bursts are discussed. C1 [Kong, Xiangliang; Chen, Yao; Feng, Shiwei; Du, Guohui] Shandong Univ, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Shandong, Peoples R China. [Kong, Xiangliang; Chen, Yao; Feng, Shiwei; Du, Guohui] Shandong Univ, Inst Space Sci, Weihai 264209, Shandong, Peoples R China. [Guo, Fan] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Li, Gang] Univ Alabama, Dept Space Sci, Huntsville, AL 35899 USA. [Li, Gang] Univ Alabama, CSPAR, Huntsville, AL 35899 USA. RP Chen, Y (reprint author), Shandong Univ, Shandong Prov Key Lab Opt Astron & Solar Terr Env, Weihai 264209, Shandong, Peoples R China.; Chen, Y (reprint author), Shandong Univ, Inst Space Sci, Weihai 264209, Shandong, Peoples R China. EM yaochen@sdu.edu.cn RI Chen, Yao/B-7255-2011; Kong, Xiangliang/D-9855-2012; OI Guo, Fan/0000-0003-4315-3755 FU Natural Science Foundation of Shandong Province [ZR2014DQ001, ZR2013DQ004]; NSF [ATM-0847719, AGS1135432]; [NSBRSF 2012CB825601]; [NNSFC 11503014]; [41274175]; [41331068]; [U1431103] FX This work was supported by grants NSBRSF 2012CB825601, NNSFC 11503014, 41274175, 41331068, U1431103, and Natural Science Foundation of Shandong Province (ZR2014DQ001 and ZR2013DQ004). G.L.'s work at UAHuntsville was supported by NSF grants ATM-0847719 and AGS1135432. The numerical simulations reported here were carried out on the supercomputer of Shandong University, Weihai. NR 54 TC 3 Z9 3 U1 5 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 10 PY 2016 VL 821 IS 1 AR 32 DI 10.3847/0004-637X/821/1/32 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9GB UT WOS:000373809000032 ER PT J AU Lohfink, AM Reynolds, CS Pinto, C Alston, W Boggs, SE Christensen, FE Craig, WW Fabian, AC Hailey, CJ Harrison, FA Kara, E Matt, G Parker, ML Stern, D Walton, D Zhang, WW AF Lohfink, A. M. Reynolds, C. S. Pinto, C. Alston, W. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Hailey, C. J. Harrison, F. A. Kara, E. Matt, G. Parker, M. L. Stern, D. Walton, D. Zhang, W. W. TI THE RHYTHM OF FAIRALL 9. I. OBSERVING THE SPECTRAL VARIABILITY WITH XMM-NEWTON AND NuSTAR SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: Seyfert; X-rays: individual (Fairall 9) ID ACTIVE GALACTIC NUCLEI; BLACK-HOLE SPIN; X-RAY EXCESS; SUZAKU OBSERVATIONS; NGC 5548; SWIFT; DISC; AGN; SPECTROSCOPY; TELESCOPE AB We present a multi-epoch X-ray spectral analysis of the Seyfert. 1 galaxy Fairall. 9. Our analysis shows that Fairall. 9 displays unique spectral variability in that its ratio residuals to a simple absorbed power law in the 0.5-10 keV band remain constant with time in spite of large variations in flux. This behavior implies an unchanging source geometry and the same emission processes continuously at work at the timescale probed. With the constraints from NuSTAR on the broad-band spectral shape, it is clear that the soft excess in this source is a superposition of two different processes, one being blurred ionized reflection in the innermost parts of the accretion disk, and the other a continuum component such as a spatially distinct Comptonizing region. Alternatively, a more complex primary Comptonization component together with blurred ionized reflection could be responsible. C1 [Lohfink, A. M.; Pinto, C.; Alston, W.; Fabian, A. C.; Kara, E.; Parker, M. L.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Reynolds, C. S.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.; Hailey, C. J.] Danish Tech Univ, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Harrison, F. A.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Matt, G.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Stern, D.; Walton, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Xray Astrophys Lab, Greenbelt, MD 20771 USA. RP Lohfink, AM (reprint author), Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. EM alohfink@ast.cam.ac.uk RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Reynolds, Christopher/0000-0002-1510-4860; Pinto, Ciro/0000-0003-2532-7379 FU ERC Advanced Grant FEEDBACK; Simons Foundation Fellows Program (US); Sackler Fellowship Program (Cambridge); National Aeronautics and Space Administration FX We thank the referee for comments that have helped to improve the clarity of the paper. AL and ACF acknowledge support from the ERC Advanced Grant FEEDBACK. CSR thanks the Simons Foundation Fellows Program (US) and the Sackler Fellowship Program (Cambridge) for support. This work made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This research has made use of data obtained from the Suzaku satellite, a collaborative mission between the space agencies of Japan (JAXA) and the USA (NASA). NR 39 TC 4 Z9 4 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD APR 10 PY 2016 VL 821 IS 1 AR 11 DI 10.3847/0004-637X/821/1/11 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9GB UT WOS:000373809000011 ER PT J AU Guildenbecher, DR Cooper, MA Sojka, PE AF Guildenbecher, Daniel R. Cooper, Marcia A. Sojka, Paul E. TI High-speed (20 kHz) digital in-line holography for transient particle tracking and sizing in multiphase flows SO APPLIED OPTICS LA English DT Article ID HYBRID METHOD; DROP; VELOCIMETRY; IMPACT; TIME; MICROSCOPY; LOCATION; PIPE; FILM AB High-speed (20 kHz) digital in-line holography (DIH) is applied for 3D quantification of the size and velocity of fragments formed from the impact of a single water drop onto a thin film of water and burning aluminum particles from the combustion of a solid rocket propellant. To address the depth-of-focus problem in DIH, a regression-based multiframe tracking algorithm is employed, and out-of-plane experimental displacement accuracy is shown to be improved by an order-of-magnitude. Comparison of the results with previous DIH measurements using low-speed recording shows improved positional accuracy with the added advantage of detailed resolution of transient dynamics from single experimental realizations. The method is shown to be particularly advantageous for quantification of particle mass flow rates. For the investigated particle fields, the mass flows rates, which have been automatically measured from single experimental realizations, are found to be within 8% of the expected values. (C) 2016 Optical Society of America C1 [Guildenbecher, Daniel R.; Cooper, Marcia A.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Sojka, Paul E.] Purdue Univ, Sch Mech Engn, W Lafayette, IN 47907 USA. RP Guildenbecher, DR (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM drguild@sandia.gov FU Sandia National Laboratories [DE-AC04-94AL85000] FX Sandia National Laboratories (DE-AC04-94AL85000). NR 27 TC 1 Z9 1 U1 7 U2 13 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD APR 10 PY 2016 VL 55 IS 11 BP 2892 EP 2903 DI 10.1364/AO.55.002892 PG 12 WC Optics SC Optics GA DI6NT UT WOS:000373617000010 PM 27139851 ER PT J AU Kelly, P Liu, MZ Kuznetsova, L AF Kelly, Priscilla Liu, Mingzhao Kuznetsova, Lyuba TI Designing optical metamaterial with hyperbolic dispersion based on an Al:ZnO/ZnO nano-layered structure using the atomic layer deposition technique SO APPLIED OPTICS LA English DT Article ID GENERALIZED ELLIPSOMETRY; PLASMONIC MATERIALS; OXIDES; ZNO AB Nano-layered Al:ZnO/ZnO hyperbolic dispersion metamaterial with a large number of layers was fabricated using the atomic layer deposition (ALD) technique. Experimental dielectric functions for Al:ZnO/ZnO structures are obtained by an ellipsometry technique in the visible and near-infrared spectral ranges. The theoretical modeling of the Al:ZnO/ZnO dielectric permittivity is done using effective medium approximation. A method for analysis of spectroscopic ellipsometry data is demonstrated to extract the optical permittivity for this highly anisotropic nano-layered metamaterial. The results of the ellipsometry analysis show that Al:ZnO/ZnO structures with a 1: 9 ALD cycle ratio exhibit hyperbolic dispersion transition change near 1.8 mu m wavelength. (C) 2016 Optical Society of America C1 [Kelly, Priscilla; Kuznetsova, Lyuba] San Diego State Univ, Dept Phys, San Diego, CA 92182 USA. [Liu, Mingzhao] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Kuznetsova, L (reprint author), San Diego State Univ, Dept Phys, San Diego, CA 92182 USA. EM lkuznetsova@mail.sdsu.edu FU Brookhaven National Laboratory (BNL) (CFN) [33123]; National Science Foundation (NSF) (STEM scholarship award) [DUE-1259951] FX Brookhaven National Laboratory (BNL) (CFN user proposal 33123); National Science Foundation (NSF) (STEM scholarship award (DUE-1259951)). NR 25 TC 2 Z9 2 U1 4 U2 16 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD APR 10 PY 2016 VL 55 IS 11 BP 2993 EP 2997 DI 10.1364/AO.55.002993 PG 5 WC Optics SC Optics GA DI6NT UT WOS:000373617000024 PM 27139865 ER PT J AU Deng, W Zhang, HC Zhang, B Li, H AF Deng, Wei Zhang, Haocheng Zhang, Bing Li, Hui TI COLLISION-INDUCED MAGNETIC RECONNECTION AND A UNIFIED INTERPRETATION OF POLARIZATION PROPERTIES OF GRBs AND BLAZARS SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE galaxies: jets; gamma-ray burst: general; magnetic fields; magnetic reconnection; magnetohydrodynamics (MHD); polarization ID GAMMA-RAY BURSTS; RELATIVISTIC MHD SIMULATIONS; INTERNAL SHOCKS; VARIABILITY; JETS; EMISSION; MODEL; RADIATION; FLUX; DISSIPATION AB The jet composition and energy dissipation mechanism of gamma-ray bursts (GRBs) and blazars are fundamental questions that remain not fully understood. One plausible model is to interpret the gamma-ray emission of GRBs and optical emission of blazars as synchrotron radiation of electrons accelerated from the collision-induced magnetic dissipation regions in Poynting-flux-dominated jets. The polarization observation is an important and independent information to test this model. Based on our recent 3D relativistic MHD simulations of collision-induced magnetic dissipation of magnetically dominated blobs, here we perform calculations of the polarization properties of the emission in the dissipation region and apply the results to model the polarization observational data of GRB prompt emission and blazar optical emission. We show that the same numerical model with different input parameters can reproduce well the observational data of both GRBs and blazars, especially the 90 degrees polarization angle (PA) change in GRB 100826A and the 180 degrees PA swing in blazar 3C279. This supports a unified model for GRB and blazar jets, suggesting that collision-induced magnetic reconnection is a common physical mechanism to power the relativistic jet emission from events with very different black hole masses. C1 [Deng, Wei; Zhang, Bing] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [Deng, Wei; Zhang, Haocheng; Li, Hui] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Zhang, Haocheng] Ohio Univ, Dept Phys & Astron, Inst Astrophys, Athens, OH 45701 USA. RP Deng, W; Zhang, B (reprint author), Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA.; Deng, W; Zhang, HC; Li, H (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA.; Zhang, HC (reprint author), Ohio Univ, Dept Phys & Astron, Inst Astrophys, Athens, OH 45701 USA. EM deng@physics.unlv.edu; hz193909@ohio.edu; zhang@physics.unlv.edu; hli@lanl.gov FU NASA [NNX15AK85G, NNX14AF85G]; LANL/LDRD program; Institutional Computing Programs at LANL; DOE/Office of Fusion Energy Science through CMSO FX We thank the referee Pawan Kumar for helpful suggestions. This work is supported by NASA through grants NNX15AK85G and NNX14AF85G and by the LANL/LDRD program and Institutional Computing Programs at LANL and by DOE/Office of Fusion Energy Science through CMSO. We are grateful to Dr. Yonetoku for sharing the data with us. We thank important technical support from Shengtai Li. We also thank helpful discussion and suggestions from Z. Lucas Uhm, Bin-Bin Zhang, Fan Guo, and Xiaocan Li. NR 35 TC 2 Z9 3 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD APR 10 PY 2016 VL 821 IS 1 AR L12 DI 10.3847/2041-8205/821/1/L12 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9HA UT WOS:000373812000012 ER PT J AU Parker, ML Tomsick, JA Kennea, JA Miller, JM Harrison, FA Barret, D Boggs, SE Christensen, FE Craig, WW Fabian, AC Furst, F Grinberg, V Hailey, CJ Romano, P Stern, D Walton, DJ Zhang, WW AF Parker, M. L. Tomsick, J. A. Kennea, J. A. Miller, J. M. Harrison, F. A. Barret, D. Boggs, S. E. Christensen, F. E. Craig, W. W. Fabian, A. C. Fuerst, F. Grinberg, V. Hailey, C. J. Romano, P. Stern, D. Walton, D. J. Zhang, W. W. TI NuSTAR AND SWIFT OBSERVATIONS OF THE VERY HIGH STATE IN GX 339-4: WEIGHING THE BLACK HOLE WITH X-RAYS SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE accretion, accretion disks; X-rays: binaries; X-rays: individual (GX 339-4) ID CYGNUS X-1; COMPTONIZATION MODELS; ACCRETION DISK; HARD STATE; SPIN; SPECTROSCOPY; REFLECTION; GX-339-4; BINARIES; SUZAKU AB We present results from spectral fitting of the very high state of GX 339-4 with Nuclear Spectroscopic Telescope Array (NuSTAR) and Swift. We use relativistic reflection modeling to measure the spin of the black hole and inclination of the inner disk and find a spin of a = 0.95(-0.08)(+0.02) and inclination of 30 degrees +/- 1 degrees (statistical errors). These values agree well with previous results from reflection modeling. With the exceptional sensitivity of NuSTAR at the high-energy side of the disk spectrum, we are able to constrain multiple physical parameters simultaneously using continuum fitting. By using the constraints from reflection as input for the continuum fitting method, we invert the conventional fitting procedure to estimate the mass and distance of GX 339-4 using just the X-ray spectrum, finding a mass of 9.0(-1.2)(+1.6) M-circle dot and distance of 8.4 +/- 0.9 kpc (statistical errors). C1 [Parker, M. L.; Fabian, A. C.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Tomsick, J. A.; Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, 7 Gauss Way, Berkeley, CA 94720 USA. [Kennea, J. A.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Miller, J. M.] Univ Michigan, Dept Astron, 1085 South Univ Ave,West Hall 311, Ann Arbor, MI 48109 USA. [Harrison, F. A.; Fuerst, F.] CALTECH, 1200 East Calif Blvd, Pasadena, CA 91125 USA. [Barret, D.] Inst Rech Astrophys & Planetol, 9 Ave Colonel Roche, F-31028 Toulouse, France. [Christensen, F. E.] Danish Tech Univ, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Grinberg, V.] MIT, Kavli Inst Astrophys, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Hailey, C. J.] Columbia Univ, New York, NY 10027 USA. [Romano, P.] INAF IASF Palermo, Via Ugo La Malfa 153, I-90146 Palermo, Italy. [Stern, D.; Walton, D. J.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Parker, ML (reprint author), Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Parker, Michael/0000-0002-8466-7317 FU STFC; NASA; [ASI-INAF I/004/11/0]; [ASI-INAF I/037/12/0] FX We are grateful to the referee for detailed and thoughtful comments that have significantly improved the paper. M.L.P. acknowledges financial support from the STFC. P.R. acknowledges financial contribution from ASI-INAF I/004/11/0 and ASI-INAF I/037/12/0. This work made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center and the California Institute of Technology. NR 40 TC 5 Z9 5 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD APR 10 PY 2016 VL 821 IS 1 AR L6 DI 10.3847/2041-8205/821/1/L6 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DI9HA UT WOS:000373812000006 ER PT J AU Coloma, P Dobrescu, BA Frugiuele, C Harnik, R AF Coloma, Pilar Dobrescu, Bogdon A. Frugiuele, Claudia Harnik, Roni TI Dark matter beams at LBNF SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Neutrino Physics AB High-intensity neutrino beam facilities may produce a beam of light dark matter when protons strike the target. Searches for such a dark matter beam using its scattering in a nearby detector must overcome the large neutrino background. We characterize the spatial and energy distributions of the dark matter and neutrino beams, focusing on their differences to enhance the sensitivity to dark matter. We find that a dark matter beam produced by a Z' boson in the GeV mass range is both broader and more energetic than the neutrino beam. The reach for dark matter is maximized for a detector sensitive to hard neutral-current scatterings, placed at a sizable angle off the neutrino beam axis. In the case of the Long-Baseline Neutrino Facility (LBNF), a detector placed at roughly 6 degrees off axis and at a distance of about 200m from the target would be sensitive to Z' couplings as low as 0.05. This search can proceed symbiotically with neutrino measurements. We also show that the MiniBooNE and MicroBooNE detectors, which are on Fermilab's Booster beamline, happen to be at an optimal angle from the NuMI beam and could perform searches with existing data. This illustrates potential synergies between LBNF and the short-baseline neutrino program if the detectors are positioned appropriately. C1 [Coloma, Pilar; Dobrescu, Bogdon A.; Frugiuele, Claudia; Harnik, Roni] Fermilab Natl Accelerator Lab, Theory Dept, POB 500, Batavia, IL 60510 USA. RP Coloma, P (reprint author), Fermilab Natl Accelerator Lab, Theory Dept, POB 500, Batavia, IL 60510 USA. EM pcoloma@fnal.gov; bdob@fnal.gov; claudiaf@fnal.gov; roni@fnal.gov FU European Union through the ITN INVISIBLES (Marie Curie Actions) [PITN-GA-2011-289442-INVISIBLES]; Mainz Institute for Theoretical Physics; United States Department of Energy [DE-AC02-07CH11359] FX PC acknowledges financial support by the European Union through the ITN INVISIBLES (Marie Curie Actions, PITN-GA-2011-289442-INVISIBLES), and would like to thank the Mainz Institute for Theoretical Physics for hospitality and partial support during completion of this work. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 51 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 8 PY 2016 IS 4 AR 047 DI 10.1007/JHEP04(2016)047 PG 20 WC Physics, Particles & Fields SC Physics GA EN4BB UT WOS:000395951300002 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Balasubramanian, S Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Benacek, P Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biro, G Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chauvin, A Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC 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TI Charge-dependent flow and the search for the chiral magnetic wave in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; PARITY CONSERVATION; NUCLEAR COLLISIONS; ANISOTROPIC FLOW; HOT QCD; VIOLATION; FIELD; MOMENT AB We report on measurements of a charge-dependent flow using a novel three-particle correlator with ALICE in Pb-Pb collisions at the CERN Large Hadron Collider (LHC), and discuss the implications for observation of local parity violation and the chiral magnetic wave (CMW) in heavy-ion collisions. Charge-dependent flow is reported for different collision centralities as a function of the event charge asymmetry. While our results are in qualitative agreement with expectations based on the CMW, the nonzero signal observed in higher harmonics correlations indicates a possible significant background contribution. We also present results on a differential correlator, where the flow of positive and negative charges is reported as a function of the mean charge of the particles and their pseudorapidity separation. We argue that this differential correlator is better suited to distinguish the differences in positive and negative charges expected due to the CMW and the background effects, such as local charge conservation coupled with strong radial and anisotropic flow. C1 [Papikyan, V.] AI Alikhanyan Natl Sci Fdn, Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Cortes Maldonado, I.; Fernandez Tellez, A.; Noris, J. C. C.; Rodriguez Cahuantzi, M.; Vargas, A.; Limon, S. Vergara; Villatoro Tello, A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Chelnokov, V.; Shadura, O.; Yurchenko, V.; Zinovjev, G.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. [Biswas, R.; Das, S.; Prasad, S. K.; Raha, S.] Bose Inst, Dept Phys, Kolkata, India. 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[Antinori, F.; Dainese, A.; Fabris, D.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Bedda, C.; Bruna, E.; Cerello, P.; Corrales Morales, Y.; De Marco, N.; Feliciello, A.; Giubellino, P.; La Pointe, S. L.; Oppedisano, C.; Paul, B.; Prino, F.; Scomparin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] SSC IHEP NRC Kurchatov Inst, Protvino, Russia. [Weber, M.] Stefan Meyer Inst Subatomare Phys, Vienna, Austria. [Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Blanco, J. Martin; Garcia, G. Martinez; Massacrier, L.; Molnar, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS IN2P3, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Jadlovsky, J.; Kopcik, M.; Papcun, P.] Tech Univ, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Garcia Prado, C. Alves; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Domenicis Gimenez, D.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Mas, A.; Munhoz, M. G.; Natal da Luz, H.; Oliveira Da Silva, A. C.; Suaide, A. A. P.; de Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; de Souza, R. D.; Takahashi, J.] Univ Estadual Campinas, Campinas, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Knospe, A. G.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Murakami, H.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, Univ Lyon, CNRS, IN2P3,IPN Lyon, Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Biro, G.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Balasubramanian, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Lutz, T. H.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul, South Korea. [Keidel, R.] Fachhochsch Worms, ZTT, Worms, Germany. [Connors, M. E.] Georgia State Univ, Atlanta, GA 30303 USA. [Connors, M. E.] Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. RI Vickovic, Linda/F-3517-2017; Ferreiro, Elena/C-3797-2017; Fernandez Tellez, Arturo/E-9700-2017; Natal da Luz, Hugo/F-6460-2013; Vechernin, Vladimir/J-5832-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Takahashi, Jun/B-2946-2012; Ferretti, Alessandro/F-4856-2013; Derradi de Souza, Rafael/M-4791-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; OI Vickovic, Linda/0000-0002-9820-7960; Ferreiro, Elena/0000-0002-4449-2356; Fernandez Tellez, Arturo/0000-0003-0152-4220; Natal da Luz, Hugo/0000-0003-1177-870X; Vechernin, Vladimir/0000-0003-1458-8055; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Takahashi, Jun/0000-0002-4091-1779; Ferretti, Alessandro/0000-0001-9084-5784; Derradi de Souza, Rafael/0000-0002-2084-7001; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Giubilato, Piero/0000-0003-4358-5355; Fernandez Tellez, Arturo/0000-0001-5092-9748 FU Worldwide LHC Computing Grid (WLCG) Collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation Academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones TecnolA3gicas y Desarrollo Nuclear (CEADEN); Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) Collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS), and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE), and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation, and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire", "Region Alsace", "Region Auvergne", and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico, Amerique Latine Formation Academique - European Commission (ALFA-EC), and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations, and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones TecnolA3gicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 41 TC 4 Z9 4 U1 19 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 8 PY 2016 VL 93 IS 4 AR 044903 DI 10.1103/PhysRevC.93.044903 PG 14 WC Physics, Nuclear SC Physics GA EG9EW UT WOS:000391362200001 ER PT J AU Edwards, D Brewer, S Cao, Y Jesse, S Chen, LQ Kalinin, SV Kumar, A Bassiri-Gharb, N AF Edwards, David Brewer, Steven Cao, Ye Jesse, Stephen Chen, Long-Qing Kalinin, Sergei V. Kumar, Amit Bassiri-Gharb, Nazanin TI Local Probing of Ferroelectric and Ferroelastic Switching through Stress-Mediated Piezoelectric Spectroscopy SO ADVANCED MATERIALS INTERFACES LA English DT Article ID PIEZORESPONSE FORCE MICROSCOPY; ZIRCONATE-TITANATE FILMS; DOMAIN-WALL MOTION; THIN-FILMS; POLARIZATION; ENHANCEMENT; STABILITY; CERAMICS; DYNAMICS AB Strain effects have a significant role in mediating classic ferroelectric behavior such as polarization switching and domain wall dynamics. These effects are of critical relevance if the ferroelectric order parameter is coupled to strain and is therefore, also ferroelastic. Here, switching spectroscopy piezoresponse force microscopy (SS-PFM) is combined with control of applied tip pressure to exert direct control over the ferroelastic and ferroelectric switching events, a modality otherwise unattainable in traditional PFM. As a proof of concept, stress-mediated SS-PFM is applied toward the study of polarization switching events in a lead zirconate titanate thin film, with a composition near the morphotropic phase boundary with co-existing rhombohedral and tetragonal phases. Under increasing applied pressure, shape modification of local hysteresis loops is observed, consistent with a reduction in the ferroelastic domain variants under increased pressure. These experimental results are further validated by phase field simulations. The technique can be expanded to explore more complex electromechanical responses under applied local pressure, such as probing ferroelectric and ferroelastic piezoelectric nonlinearity as a function of applied pressure, and electro-chemo-mechanical response through electrochemical strain microscopy. C1 [Edwards, David; Kumar, Amit] Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland. [Brewer, Steven; Bassiri-Gharb, Nazanin] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Cao, Ye; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Kumar, A (reprint author), Queens Univ Belfast, Sch Math & Phys, Belfast BT7 1NN, Antrim, North Ireland.; Bassiri-Gharb, N (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. EM a.kumar@qub.ac.uk; nazanin.bassiri@gatech.edu RI Kumar, Amit/C-9662-2012; Bassiri-Gharb, Nazanin/F-1783-2011; Cao, Ye/L-1271-2016 OI Kumar, Amit/0000-0002-1194-5531; Bassiri-Gharb, Nazanin/0000-0002-0183-5160; Cao, Ye/0000-0002-7365-7447 FU US-Ireland R&D partnership through US National Science Foundation [CMMI-1537262]; Department of Education and Learning, Northern Ireland [USI-082]; US National Science Foundation [DMR-1255379]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy [CNMS2013-143]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG02-07ER46417]; Department of Employment and Learning Northern Ireland (DELNI) studentship FX D.E., S.B., A.K. and N.B.-G. gratefully acknowledge support by the US-Ireland R&D partnership through US National Science Foundation grant no. CMMI-1537262 and the Department of Education and Learning, Northern Ireland grant no. USI-082. The work at Georgia Institute of Technology was additionally supported by the US National Science Foundation through grant no. DMR-1255379. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which was sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy under user proposal CNMS2013-143. The work at Penn State was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-07ER46417. This work was also supported by the Department of Employment and Learning Northern Ireland (DELNI) studentship. NR 51 TC 1 Z9 1 U1 16 U2 37 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD APR 8 PY 2016 VL 3 IS 7 AR 1500470 DI 10.1002/admi.201500470 PG 9 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DJ4CM UT WOS:000374153000002 ER PT J AU Gott, MD DeGraffenreid, AJ Feng, YT Phipps, MD Wycoff, DE Embree, MF Cutler, CS Ketring, AR Jurisson, SS AF Gott, Matthew D. DeGraffenreid, Anthony J. Feng, Yutian Phipps, Michael D. Wycoff, Donald E. Embree, Mary F. Cutler, Cathy S. Ketring, Alan R. Jurisson, Silvia S. TI Chromatographic separation of germanium and arsenic for the production of high purity As-77 SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Ge/As separation; Ge/As distribution coefficient; Column chromatography; High specific activity arsenic-77 ID IRRADIATED GERMANIUM; RADIOCHEMICAL SEPARATION; OXIDE TARGETS AB A simple column chromatographic method was developed to isolate As-77 (94 +/- 6% (EtOH/HCl); 74 +/- 11 (MeOH)) from germanium for potential use in radioimmunotherapy. The separation of arsenic from germanium was based on their relative affinities for different chromatographic materials in aqueous and organic environments. Using an organic or mixed mobile phase, germanium was selectively retained on a silica gel column as germanate, while arsenic was eluted from the column as arsenate. Subsequently, enriched Ge-76 (98 +/- 2) was recovered for reuse by elution with aqueous solution (neutral to basic). Greater than 98% radiolabeling yield of a As-77-trithiol was observed from methanol separated [As-77]arsenate [17]. (C) 2016 Elsevier B.V. All rights reserved. C1 [Gott, Matthew D.; DeGraffenreid, Anthony J.; Feng, Yutian; Phipps, Michael D.; Wycoff, Donald E.; Jurisson, Silvia S.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Embree, Mary F.; Cutler, Cathy S.; Ketring, Alan R.] Univ Missouri, Res Reactor Ctr, Columbia, MO 65211 USA. [Cutler, Cathy S.] Brookhaven Natl Lab, Collier Accelerator Dept, Med Isotope Res & Prod Program MIRP, Upton, NY 11973 USA. RP Jurisson, SS (reprint author), Univ Missouri, Dept Chem, Columbia, MO 65211 USA. EM jurissons@missouri.edu OI Jurisson, Silvia/0000-0002-2142-7412 FU Department of Energy, Office of Basic Sciences, Isotope Research Program [DE-SC0003851, DE-SC0010283]; National Science Foundation under IGERT award [DGE-0965983]; National Institutes of Health under NIBIB Training Grant [5 T32-EB004822] FX The authors acknowledge support from the Department of Energy, Office of Basic Sciences, Isotope Research Program under grants DE-SC0003851 and DE-SC0010283. Additional trainee support was provided from the National Science Foundation under IGERT award DGE-0965983 (M.D. Gott) and the National Institutes of Health under NIBIB Training Grant 5 T32-EB004822 (A.J. DeGraffenreid). NR 16 TC 1 Z9 1 U1 2 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD APR 8 PY 2016 VL 1441 BP 68 EP 74 DI 10.1016/j.chroma.2016.02.074 PG 7 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA DI5PY UT WOS:000373552300009 PM 26947162 ER PT J AU Ding, J Asta, M Ritchie, RO AF Ding, Jun Asta, Mark Ritchie, Robert O. TI Anomalous structure-property relationships in metallic glasses through pressure-mediated glass formation SO PHYSICAL REVIEW B LA English DT Article ID LOCAL ORDER; FREE-VOLUME; INDUCED AMORPHIZATION; SUPERCOOLED LIQUID; MOLECULAR-DYNAMICS; TRANSITION; RELAXATION; CRYSTALLINE; MODEL; DUCTILITY AB Metallic glasses are commonly found to favor denser packing structures and icosahedral order in experiments, simulations, and theoretical models. Here we present a molecular dynamics simulation study of Cu-Zr metallic glasses, prepared through a pressure-mediated pathway. The resulting glasses exhibit anomalous structure-property relationships; these glasses are less energetically stable, concomitant with a denser atomic packing and a significant increase in icosahedral short-range order. The enhanced icosahedral order is shown to be accompanied by a pressure-mediated change in chemical short-range order. The results demonstrate that in amorphous alloys (nonmonatomic), theoretical frameworks of the two-order-parameter model must be generalized to account for chemical degrees of freedom. C1 [Ding, Jun; Asta, Mark; Ritchie, Robert O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Asta, Mark; Ritchie, Robert O.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Asta, M; Ritchie, RO (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Asta, M; Ritchie, RO (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mdasta@berkeley.edu; roritchie@lbl.gov RI Ritchie, Robert/A-8066-2008; Ding, Jun/K-1989-2012 OI Ritchie, Robert/0000-0002-0501-6998; Ding, Jun/0000-0002-4091-8663 FU Mechanical Behavior of Materials Program at the Lawrence Berkeley National Laboratory [KC 13]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Hajime Tanaka, Evan Ma, and Yongqiang Cheng for their thoughtful discussions. This work was supported by the Mechanical Behavior of Materials Program (KC 13) at the Lawrence Berkeley National Laboratory, funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. The study made use of resources of the National Energy Research Scientific Computing Center(NERSC), which is a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 68 TC 1 Z9 1 U1 10 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 8 PY 2016 VL 93 IS 14 AR 140204 DI 10.1103/PhysRevB.93.140204 PG 6 WC Physics, Condensed Matter SC Physics GA DI5VP UT WOS:000373568900001 ER PT J AU Sentef, MA Kemper, AF Georges, A Kollath, C AF Sentef, M. A. Kemper, A. F. Georges, A. Kollath, C. TI Theory of light-enhanced phonon-mediated superconductivity SO PHYSICAL REVIEW B LA English DT Article ID ANGLE-RESOLVED PHOTOEMISSION; CHARGE-DENSITY-WAVE; LATTICE-VIBRATIONS; ELECTRONS; DYNAMICS; CUPRATE; MODE; SPECTROSCOPY; EXCITATION; METAL AB We investigate the dynamics of a phonon-mediated superconductor driven out of equilibrium. The electronic hopping amplitude is ramped down in time, resulting in an increased electronic density of states. The dynamics of the coupled electron-phonon model is investigated by solving Migdal-Eliashberg equations for the double-time Keldysh Green's functions. The increase of the density of states near the Fermi level leads to an enhancement of superconductivity when the system thermalizes to the new state at the same temperature. We provide a time-and momentum-resolved view on this thermalization process and show that it involves fast processes associated with single-particle scattering and much slower dynamics associated with the superconducting order parameter. The importance of electron-phonon coupling for the rapid enhancement and the efficient thermalization of superconductivity is demonstrated, and the results are compared to a BCS time-dependent mean-field approximation. C1 [Sentef, M. A.; Kollath, C.] Univ Bonn, HISKP, Nussallee 14-16, D-53115 Bonn, Germany. [Sentef, M. A.] Max Planck Inst Struct & Dynam Matter, Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany. [Kemper, A. F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Kemper, A. F.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Georges, A.] Ecole Polytech, CNRS, Ctr Phys Theor, F-91128 Palaiseau, France. [Georges, A.] Coll France, 11 Pl Marcelin Berthelot, F-75005 Paris, France. [Georges, A.] Univ Geneva, Dept Quantum Matter Phys, 24 Quai Ernest Ansermet, CH-1211 Geneva 4, Switzerland. RP Sentef, MA (reprint author), Univ Bonn, HISKP, Nussallee 14-16, D-53115 Bonn, Germany.; Sentef, MA (reprint author), Max Planck Inst Struct & Dynam Matter, Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany. EM michael.sentef@mpsd.mpg.de RI Kemper, Alexander/F-8243-2016; Georges, Antoine/H-4855-2012 OI Kemper, Alexander/0000-0002-5426-5181; Georges, Antoine/0000-0001-9479-9682 FU Deutsche Forschungsgemeinschaft; European Research Council [ERC-319286 QMAC, ERC-648166]; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231] FX We thank A. Cavalleri, M. Kollar, P. van Loosdrecht, and A. Subedi for discussions and H. van Pee for administrating the computer cluster on which the computations were performed. We acknowledge financial support by the Deutsche Forschungsgemeinschaft and by European Research Council Grants No. ERC-319286 QMAC and No. ERC-648166 Phon(t) on. A.F.K. was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231. NR 68 TC 10 Z9 10 U1 2 U2 64 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 8 PY 2016 VL 93 IS 14 AR 144506 DI 10.1103/PhysRevB.93.144506 PG 10 WC Physics, Condensed Matter SC Physics GA DI5VP UT WOS:000373568900004 ER PT J AU Zhao, RJ Evans, JW Oliveira, TJ AF Zhao, Renjie Evans, James W. Oliveira, Tiago J. TI Permeability and kinetic coefficients for mesoscale BCF surface step dynamics: Discrete two-dimensional deposition-diffusion equation analysis SO PHYSICAL REVIEW B LA English DT Article ID 2ND LAYER NUCLEATION; VICINAL SURFACES; GROWTH; EQUILIBRIUM; CRYSTAL; EPITAXY; SI(001); MOUNDS; MODELS AB A discrete version of deposition-diffusion equations appropriate for description of step flow on a vicinal surface is analyzed for a two-dimensional grid of adsorption sites representing the stepped surface and explicitly incorporating kinks along the step edges. Model energetics and kinetics appropriately account for binding of adatoms at steps and kinks, distinct terrace and edge diffusion rates, and possible additional barriers for attachment to steps. Analysis of adatom attachment fluxes as well as limiting values of adatom densities at step edges for nonuniform deposition scenarios allows determination of both permeability and kinetic coefficients. Behavior of these quantities is assessed as a function of key system parameters including kink density, step attachment barriers, and the step edge diffusion rate. C1 [Zhao, Renjie; Evans, James W.; Oliveira, Tiago J.] Iowa State Univ, USDOE, Ames Lab, Ames, IA 50011 USA. [Zhao, Renjie; Evans, James W.; Oliveira, Tiago J.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Evans, James W.] Iowa State Univ, Dept Math, Ames, IA 50011 USA. [Oliveira, Tiago J.] Univ Fed Vicosa, Dept Fis, BR-36570900 Vicosa, MG, Brazil. RP Evans, JW (reprint author), Iowa State Univ, USDOE, Ames Lab, Ames, IA 50011 USA.; Evans, JW (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.; Evans, JW (reprint author), Iowa State Univ, Dept Math, Ames, IA 50011 USA. EM evans@ameslab.gov RI Oliveira, Tiago/R-5846-2016 OI Oliveira, Tiago/0000-0001-5675-7430 FU U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program; Iowa State University [DE-AC02-07CH11358]; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Minas Gerais FX R.Z. and J.W.E. were supported for this work by the U.S. Department of Energy (USDOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory Chemical Physics program. The work was performed at Ames Laboratory which is operated for the USDOE by Iowa State University under Contract No. DE-AC02-07CH11358. T.J.O. acknowledges the support from Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Minas Gerais (Brazilian agencies). NR 28 TC 0 Z9 0 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 8 PY 2016 VL 93 IS 16 AR 165411 DI 10.1103/PhysRevB.93.165411 PG 15 WC Physics, Condensed Matter SC Physics GA DI5XB UT WOS:000373572700005 ER PT J AU Bzdak, A Skokov, V Bathe, S AF Bzdak, Adam Skokov, Vladimir Bathe, Stefan TI Centrality dependence of high energy jets in p plus Pb collisions at energies available at the CERN Large Hadron Collider SO PHYSICAL REVIEW C LA English DT Article ID NUCLEUS COLLISIONS AB The recently measured centrality dependence of high energy jets in proton-lead collisions at the CERN Large Hadron Collider (LHC) is investigated. We hypothesize that events with jets of very high energy (a few hundred GeV) are characterized by a suppressed number of soft particles, thus shifting these events into more peripheral bins. This naturally results in the suppression (enhancement) of the nuclear modification factor, R-pA, in central (peripheral) collisions. Our calculations suggest that a moderate suppression of the order of 20%, for 10(3) GeV jets, can quantitatively reproduce the experimental data. We further extract the suppression factor as a function of jet energy and test our conjecture using available R-pA data for various centralities. C1 [Bzdak, Adam] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Bzdak, Adam; Skokov, Vladimir; Bathe, Stefan] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Bathe, Stefan] CUNY, Baruch Coll, New York, NY 10010 USA. RP Bzdak, A (reprint author), AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland.; Bzdak, A; Skokov, V; Bathe, S (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; Skokov, V (reprint author), Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA.; Bathe, S (reprint author), CUNY, Baruch Coll, New York, NY 10010 USA. EM bzdak@fis.agh.edu.pl; vskokov@quark.phy.bnl.gov; stefan.bathe@baruch.cuny.edu FU Ministry of Science and Higher Education (MNiSW); Foundation for Polish Science; National Science Centre (Narodowe Centrum Nauki) [DEC-2014/15/B/ST2/00175]; RIKEN-BNL Research Center; U.S. DOE Grant [DE-SC0007017]; [DEC-2013/09/B/ST2/00497] FX We thank P. Steinberg and L. McLerran for discussions. A.B. was supported by the Ministry of Science and Higher Education (MNiSW), by funding from the Foundation for Polish Science, and by the National Science Centre (Narodowe Centrum Nauki) via Grant No. DEC-2014/15/B/ST2/00175 and in part via Grant No. DEC-2013/09/B/ST2/00497. The authors were supported through the RIKEN-BNL Research Center. S.B. was supported by U.S. DOE Grant No. DE-SC0007017. NR 16 TC 1 Z9 1 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 8 PY 2016 VL 93 IS 4 AR 044901 DI 10.1103/PhysRevC.93.044901 PG 5 WC Physics, Nuclear SC Physics GA DI5YP UT WOS:000373576700003 ER PT J AU Agnes, P Agostino, L Albuquerque, IFM Alexander, T Alton, AK Arisaka, K Back, HO Baldin, B Biery, K Bonfini, G Bossa, M Bottino, B Brigatti, A Brodsky, J Budano, F Bussino, S Cadeddu, M Cadonati, L Cadoni, M Calaprice, F Canci, N Candela, A Cao, H Cariello, M Carlini, M Catalanotti, S Cavalcante, P Chepurnov, A Cocco, AG Covone, G Crippa, L D'Angelo, D D'Incecco, M Davini, S De Cecco, S De Deo, M De Vincenzi, M Derbin, A Devoto, A Di Eusanio, F Di Pietro, G Edkins, E Empl, A Fan, A Fiorillo, G Fomenko, K Forster, G Franco, D Gabriele, F Galbiati, C Giganti, C Goretti, AM Granato, F Grandi, L Gromov, M Guan, M Guardincerri, Y Hackett, BR Herner, K Hungerford, EV Ianni, A Ianni, A James, I Jollet, C Keeter, K Kendziora, CL Kobychev, V Koh, G Korablev, D Korga, G Kubankin, A Li, X Lissia, M Lombardi, P Luitz, S Ma, Y Machulin, IN Mandarano, A Mari, SM Maricic, J Marini, L Martoff, CJ Meregaglia, A Meyers, PD Miletic, T Milincic, R Montanari, D Monte, A Montuschi, M Monzani, M Mosteiro, P Mount, BJ Muratova, VN Musico, P Napolitano, J Nelson, A Odrowski, S Orsini, M Ortica, F Pagani, L Pallavicini, M Pantic, E Parmeggiano, S Pelczar, K Pelliccia, N Perasso, S Pocar, A Pordes, S Pugachev, DA Qian, H Randle, K Ranucci, G Razeto, A Reinhold, B Renshaw, AL Romani, A Rossi, B Rossi, N Rountree, D Sablone, D Saggese, P Saldanha, R Sands, W Sangiorgio, S Savarese, C Segreto, E Semenov, DA Shields, E Singh, PN Skorokhvatov, MD Smirnov, O Sotnikov, A Stanford, C Suvorov, Y Tartaglia, R Tatarowicz, J Testera, G Tonazzo, A Trinchese, P Unzhakov, EV Vishneva, A Vogelaar, B Wada, M Walker, S Wang, H Wang, Y Watson, AW Westerdale, S Wilhelmi, J Wojcik, MM Xiang, X Xu, J Yang, C Yoo, J Zavatarelli, S Zec, A Zhong, W Zhu, C Zuzel, G AF Agnes, P. Agostino, L. Albuquerque, I. F. M. Alexander, T. Alton, A. K. Arisaka, K. Back, H. O. Baldin, B. Biery, K. Bonfini, G. Bossa, M. Bottino, B. Brigatti, A. Brodsky, J. Budano, F. Bussino, S. Cadeddu, M. Cadonati, L. Cadoni, M. Calaprice, F. Canci, N. Candela, A. Cao, H. Cariello, M. Carlini, M. Catalanotti, S. Cavalcante, P. Chepurnov, A. Cocco, A. G. Covone, G. Crippa, L. D'Angelo, D. D'Incecco, M. Davini, S. De Cecco, S. De Deo, M. De Vincenzi, M. Derbin, A. Devoto, A. Di Eusanio, F. Di Pietro, G. Edkins, E. Empl, A. Fan, A. Fiorillo, G. Fomenko, K. Forster, G. Franco, D. Gabriele, F. Galbiati, C. Giganti, C. Goretti, A. M. Granato, F. Grandi, L. Gromov, M. Guan, M. Guardincerri, Y. Hackett, B. R. Herner, K. Hungerford, E. V. Ianni, Al Ianni, An James, I. Jollet, C. Keeter, K. Kendziora, C. L. Kobychev, V. Koh, G. Korablev, D. Korga, G. Kubankin, A. Li, X. Lissia, M. Lombardi, P. Luitz, S. Ma, Y. Machulin, I. N. Mandarano, A. Mari, S. M. Maricic, J. Marini, L. Martoff, C. J. Meregaglia, A. Meyers, P. D. Miletic, T. Milincic, R. Montanari, D. Monte, A. Montuschi, M. Monzani, M. Mosteiro, P. Mount, B. J. Muratova, V. N. Musico, P. Napolitano, J. Nelson, A. Odrowski, S. Orsini, M. Ortica, F. Pagani, L. Pallavicini, M. Pantic, E. Parmeggiano, S. Pelczar, K. Pelliccia, N. Perasso, S. Pocar, A. Pordes, S. Pugachev, D. A. Qian, H. Randle, K. Ranucci, G. Razeto, A. Reinhold, B. Renshaw, A. L. Romani, A. Rossi, B. Rossi, N. Rountree, D. Sablone, D. Saggese, P. Saldanha, R. Sands, W. Sangiorgio, S. Savarese, C. Segreto, E. Semenov, D. A. Shields, E. Singh, P. N. Skorokhvatov, M. D. Smirnov, O. Sotnikov, A. Stanford, C. Suvorov, Y. Tartaglia, R. Tatarowicz, J. Testera, G. Tonazzo, A. Trinchese, P. Unzhakov, E. V. Vishneva, A. Vogelaar, B. Wada, M. Walker, S. Wang, H. Wang, Y. Watson, A. W. Westerdale, S. Wilhelmi, J. Wojcik, M. M. Xiang, X. Xu, J. Yang, C. Yoo, J. Zavatarelli, S. Zec, A. Zhong, W. Zhu, C. Zuzel, G. CA DarkSide Collaboration TI Results from the first use of low radioactivity argon in a dark matter search SO PHYSICAL REVIEW D LA English DT Article ID INTERACTING MASSIVE PARTICLES; LIQUID ARGON; GRAN SASSO; AR-39 AB Liquid argon is a bright scintillator with potent particle identification properties, making it an attractive target for direct-detection dark matter searches. The DarkSide-50 dark matter search here reports the first WIMP search results obtained using a target of low-radioactivity argon. DarkSide-50 is a dark matter detector, using a two-phase liquid argon time projection chamber, located at the Laboratori Nazionali del Gran Sasso. The underground argon is shown to contain Ar-39 at a level reduced by a factor (1.4 +/- 0.2) x 10(3) relative to atmospheric argon. We report a background-free null result from (2616 +/- 43) kg d of data, accumulated over 70.9 live days. When combined with our previous search using an atmospheric argon, the 90% C.L. upper limit on the WIMP-nucleon spin-independent cross section, based on zero events found in the WIMP search regions, is 2.0 x 10(-4)4 cm(2) (8.6 x 10(-44) cm(2), 8.0 x 10(-43) cm(2)) for a WIMP mass of 100 GeV/c(2) (1 TeV/c(2), 10 TeV/c(2)). C1 [Agnes, P.; Franco, D.; Perasso, S.; Tonazzo, A.] Univ Paris Diderot, Sorbonne Paris Cite, CEA Irfu, CNRS IN2P3,APC,Obs Paris, F-75205 Paris, France. [Agostino, L.; De Cecco, S.; Giganti, C.] Univ Paris 06, Univ Paris Diderot, LPNHE Paris, CNRS IN2P3, F-75252 Paris, France. [Albuquerque, I. F. M.; Back, H. O.; Brodsky, J.; Calaprice, F.; Cao, H.; Di Eusanio, F.; Galbiati, C.; Ianni, An; Koh, G.; Li, X.; Meyers, P. D.; Mosteiro, P.; Nelson, A.; Pocar, A.; Qian, H.; Razeto, A.; Rossi, B.; Sands, W.; Shields, E.; Stanford, C.; Wada, M.; Westerdale, S.; Xiang, X.; Xu, J.; Zhu, C.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Albuquerque, I. F. M.] Univ Sao Paulo, Inst Fis, BR-05508090 Sao Paulo, Brazil. [Alexander, T.; Cadonati, L.; Forster, G.; Monte, A.; Pocar, A.; Randle, K.; Zec, A.] Univ Massachusetts, Amherst Ctr Fundamental Interact, Amherst, MA 01003 USA. [Alexander, T.; Cadonati, L.; Forster, G.; Monte, A.; Pocar, A.; Randle, K.; Zec, A.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Alexander, T.; Baldin, B.; Biery, K.; Forster, G.; Guardincerri, Y.; Herner, K.; Kendziora, C. L.; Montanari, D.; Pordes, S.; Yoo, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Alton, A. K.] Augustana Univ, Dept Phys, Sioux Falls, SD 57197 USA. [Arisaka, K.; Fan, A.; Renshaw, A. L.; Suvorov, Y.; Wang, H.; Wang, Y.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Back, H. O.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Bonfini, G.; Bossa, M.; Canci, N.; Candela, A.; Carlini, M.; Cavalcante, P.; D'Incecco, M.; Davini, S.; De Deo, M.; Di Pietro, G.; Gabriele, F.; Goretti, A. M.; Ianni, Al; Ianni, An; Korga, G.; Mandarano, A.; Montuschi, M.; Odrowski, S.; Orsini, M.; Razeto, A.; Rossi, N.; Sablone, D.; Savarese, C.; Suvorov, Y.; Tartaglia, R.] Lab Nazl Gran Sasso, I-67010 Assergi, AQ, Italy. [Bossa, M.; Davini, S.; Mandarano, A.; Savarese, C.] Gran Sasso Sci Inst, I-67100 Laquila, AQ, Italy. [Bottino, B.; Marini, L.; Pagani, L.; Pallavicini, M.] Univ Genoa, Dept Phys, I-16146 Genoa, Italy. [Bottino, B.; Cariello, M.; Marini, L.; Musico, P.; Pagani, L.; Pallavicini, M.; Testera, G.; Zavatarelli, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Brigatti, A.; Crippa, L.; D'Angelo, D.; Di Pietro, G.; Galbiati, C.; Lombardi, P.; Parmeggiano, S.; Ranucci, G.; Saggese, P.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Budano, F.; Bussino, S.; De Vincenzi, M.; James, I.; Mari, S. M.] Ist Nazl Fis Nucl, Sez Roma Tre, I-00146 Rome, Italy. [Budano, F.; Bussino, S.; De Vincenzi, M.; James, I.; Mari, S. M.] Univ Roma Tre, Dept Phys & Math, I-00146 Rome, Italy. [Cadeddu, M.; Cadoni, M.; Devoto, A.] Univ Cagliari, Dept Phys, I-09042 Cagliari, Italy. [Cadeddu, M.; Cadoni, M.; Devoto, A.; Lissia, M.] Ist Nazl Fis Nucl, Sez Cagliari, I-09042 Cagliari, Italy. [Canci, N.; Empl, A.; Hungerford, E. V.; Korga, G.; Renshaw, A. L.; Singh, P. N.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Catalanotti, S.; Covone, G.; Fiorillo, G.; Granato, F.; Trinchese, P.; Walker, S.] Univ Naples Federico II, Dept Phys, I-80126 Naples, Italy. [Catalanotti, S.; Cocco, A. G.; Covone, G.; Fiorillo, G.; Rossi, B.; Walker, S.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [Cavalcante, P.; Rountree, D.; Vogelaar, B.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Chepurnov, A.; Gromov, M.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119991, Russia. [Crippa, L.; D'Angelo, D.] Univ Milan, Dept Phys, I-20133 Milan, Italy. [Derbin, A.; Muratova, V. N.; Semenov, D. A.; Unzhakov, E. V.] St Petersburg Nucl Phys Inst, NRC Kurchatov Inst, Gatchina 188350, Russia. [Edkins, E.; Hackett, B. R.; Maricic, J.; Milincic, R.; Reinhold, B.] Univ Hawaii, Dept Phys & Astron, Honolulu, HI 96822 USA. [Fomenko, K.; Korablev, D.; Smirnov, O.; Sotnikov, A.; Vishneva, A.] Joint Inst Nucl Res, Dubna 141980, Russia. [Granato, F.; Martoff, C. J.; Miletic, T.; Napolitano, J.; Tatarowicz, J.; Watson, A. W.; Wilhelmi, J.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Grandi, L.; Guardincerri, Y.; Saldanha, R.] Univ Chicago, Enrico Fermi Inst, Kavli Inst, Chicago, IL 60637 USA. [Grandi, L.; Guardincerri, Y.; Saldanha, R.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Guan, M.; Ma, Y.; Wang, Y.; Yang, C.; Zhong, W.] Inst High Energy Phys, Beijing 100049, Peoples R China. [Ianni, Al] Lab Subterraneo Canfranc, Canfranc Estn, Madrid 22880, Spain. [Jollet, C.; Meregaglia, A.] Univ Strasbourg, CNRS, IN2P3, IPHC, F-67037 Strasbourg, France. [Keeter, K.; Mount, B. J.] Black Hills State Univ, Sch Nat Sci, Spearfish, SD 57799 USA. [Kobychev, V.] Natl Acad Sci Ukraine, Inst Nucl Res, UA-03680 Kiev, Ukraine. [Kubankin, A.] Belgorod Natl Res Univ, Radiat Phys Lab, Belgorod 308007, Russia. [Luitz, S.; Monzani, M.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Machulin, I. N.; Pugachev, D. A.; Skorokhvatov, M. D.; Suvorov, Y.] Kurchatov Inst, Natl Res Ctr, Moscow 123182, Russia. [Machulin, I. N.; Pugachev, D. A.; Skorokhvatov, M. D.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Ortica, F.; Pelliccia, N.; Romani, A.] Univ Perugia, Dept Chem Biol & Biotechnol, I-06123 Perugia, Italy. [Ortica, F.; Pelliccia, N.; Romani, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Pantic, E.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Pelczar, K.; Wojcik, M. M.; Zuzel, G.] Jagiellonian Univ, Smoluchowski Inst Phys, PL-30348 Krakow, Poland. [Sangiorgio, S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Segreto, E.] Univ Estadual Campinas, Inst Phys Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. [Wang, Y.] Univ Chinese Acad Sci, Sch Phys, Beijing 100049, Peoples R China. RP Martoff, CJ (reprint author), Temple Univ, Dept Phys, Philadelphia, PA 19122 USA.; Pantic, E (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. EM jeff.martoff@temple.edu; pantic@ucdavis.edu RI Ortica, Fausto/C-1001-2013; Kubankin, Alexander/A-8745-2014; Romani, Aldo/G-8103-2012; Fiorillo, Giuliana/A-2248-2012; DAngelo, Davide/K-9164-2013; Machulin, Igor/R-9711-2016; Skorokhvatov, Mikhail/R-9735-2016; Canci, Nicola/E-7498-2017; Covone, Giovanni/J-6040-2012; OI Unzhakov, Evgeniy/0000-0003-2952-6412; Rossi, Nicola/0000-0002-7046-528X; Wang, Yi/0000-0002-7351-6978; Xu, Jingke/0000-0001-8084-5609; Ortica, Fausto/0000-0001-8276-452X; Romani, Aldo/0000-0002-7338-0097; Fiorillo, Giuliana/0000-0002-6916-6776; DAngelo, Davide/0000-0001-9857-8107; Canci, Nicola/0000-0002-4797-4297; Catalanotti, Sergio/0000-0002-2337-4246; Covone, Giovanni/0000-0002-2553-096X; Brodsky, Jason/0000-0002-7498-6461; Franco, Davide/0000-0001-5604-2531 FU U.S. National Science Foundation (NSF) [PHY-0919363, PHY-1004072, PHY-1004054, PHY-1242585, PHY-1314483, PHY-1314507, PHY-1211308, PHY-1455351]; Italian Istituto Nazionale di Fisica Nucleare; U.S. Department of Energy [DE-FG02-91ER40671, DE-AC02-07CH11359]; Polish NCN [UMO-2012/05/E/ST2/02333]; UnivEarthS Labex program of Sorbonne Paris Cite [ANR-10-LABX-0023, ANR-11-IDEX-0005-02]; Sao Paulo Research Foundation (FAPESP) FX The DarkSide-50 Collaboration would like to thank LNGS and its staff for invaluable technical and logistical support. This report is based upon work supported by the U.S. National Science Foundation (NSF) (Grants No. PHY-0919363, No. PHY-1004072, No. PHY-1004054, No. PHY-1242585, No. PHY-1314483, No. PHY-1314507 and associated collaborative grants, No. PHY-1211308 and No. PHY-1455351), the Italian Istituto Nazionale di Fisica Nucleare, the U.S. Department of Energy (Contracts No. DE-FG02-91ER40671 and No. DE-AC02-07CH11359), and the Polish NCN (Grant No. UMO-2012/05/E/ST2/02333). We thank the staff of the Fermilab Particle Physics, Scientific and Core Computing Divisions for their support. We acknowledge the financial support from the UnivEarthS Labex program of Sorbonne Paris Cite (ANR-10-LABX-0023 and ANR-11-IDEX-0005-02) and from the Sao Paulo Research Foundation (FAPESP). NR 32 TC 17 Z9 17 U1 17 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 8 PY 2016 VL 93 IS 8 AR 081101 DI 10.1103/PhysRevD.93.081101 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI6BT UT WOS:000373584900001 ER PT J AU Stanton, LG Murillo, MS AF Stanton, Liam G. Murillo, Michael S. TI Ionic transport in high-energy-density matter SO PHYSICAL REVIEW E LA English DT Article ID FOKKER-PLANCK EQUATION; INERTIAL CONFINEMENT FUSION; MONTE-CARLO SIMULATIONS; KINETIC-EQUATION; DIFFUSION-COEFFICIENTS; COULOMB COLLISIONS; SELF-DIFFUSION; PLASMAS; MIXTURES; GAS AB Ionic transport coefficients for dense plasmas have been numerically computed using an effective Boltzmann approach. We have developed a simplified effective potential approach that yields accurate fits for all of the relevant cross sections and collision integrals. Our results have been validated with molecular-dynamics simulations for self-diffusion, interdiffusion, viscosity, and thermal conductivity. Molecular dynamics has also been used to examine the underlying assumptions of the Boltzmann approach through a categorization of behaviors of the velocity autocorrelation function in the Yukawa phase diagram. Using a velocity-dependent screening model, we examine the role of dynamical screening in transport. Implications of these results for Coulomb logarithm approaches are discussed. C1 [Stanton, Liam G.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94550 USA. [Murillo, Michael S.] Los Alamos Natl Lab, Computat Phys & Methods Grp, MS D413, POB 1663, Los Alamos, NM 87545 USA. RP Stanton, LG (reprint author), Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94550 USA.; Murillo, MS (reprint author), Los Alamos Natl Lab, Computat Phys & Methods Grp, MS D413, POB 1663, Los Alamos, NM 87545 USA. EM liam@llnl.gov; murillo@lanl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and by Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. The authors would like to thank Lisa Murillo for her detailed editing of the document, Julie Stern for her early contributions to this work, and William Cabot, Jeff Greenough, Jeff Haack, and George Zimmerman for very useful feedback on the manuscript. This document is LA-UR-16-20725 (LANL) and LLNL-JRNL-681618 (LLNL). NR 97 TC 5 Z9 5 U1 9 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD APR 8 PY 2016 VL 93 IS 4 AR 043203 DI 10.1103/PhysRevE.93.043203 PG 23 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DI6CG UT WOS:000373586200010 PM 27176414 ER PT J AU Nomura, Y Rajendran, S Sanches, F AF Nomura, Yasunori Rajendran, Surjeet Sanches, Fabio TI Axion Isocurvature and Magnetic Monopoles SO PHYSICAL REVIEW LETTERS LA English DT Article ID ISOTHERMAL DENSITY PERTURBATIONS; INFLATIONARY UNIVERSE SCENARIO; DARK-MATTER; QCD AXION; NATURAL SOLUTION; MU-PROBLEM; COSMOLOGY; GENERATION; FLUCTUATIONS; DYNAMICS AB We propose a simple mechanism to suppress axion isocurvature fluctuations using hidden sector magnetic monopoles. This allows for the Peccei-Quinn scale to be of the order of the unification scale consistently with high scale inflation. C1 [Nomura, Yasunori] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Nomura, Y (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; National Science Foundation (NSF) [PHY-1521446]; MEXT KAKENHI [15H05895]; NSF [PHY-1417295, PHY-1507160]; Simons Foundation [378243]; Heising Simons Foundation; DOE National Nuclear Security Administration Stewardship Science Graduate Fellowship FX We would like to thank Peter Graham, Nemanja Kaloper, David E. Kaplan, Jeremy Mardon, and Sean Weinberg for discussions. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. Y. N. was supported in part by the National Science Foundation (NSF) under Grant No. PHY-1521446 and MEXT KAKENHI Grant No. 15H05895. S. R. was supported in part by the NSF under Grants No. PHY-1417295 and No. PHY-1507160, the Simons Foundation Grant No. 378243, and the Heising Simons Foundation. The work of F. S. was supported in part by the DOE National Nuclear Security Administration Stewardship Science Graduate Fellowship. NR 61 TC 2 Z9 2 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 8 PY 2016 VL 116 IS 14 AR 141803 DI 10.1103/PhysRevLett.116.141803 PG 6 WC Physics, Multidisciplinary SC Physics GA DI6CW UT WOS:000373587800005 PM 27104700 ER PT J AU Geraedts, SD Zaletel, MP Mong, RSK Metlitski, MA Vishwanath, A Motrunich, OI AF Geraedts, Scott D. Zaletel, Michael P. Mong, Roger S. K. Metlitski, Max A. Vishwanath, Ashvin Motrunich, Olexei I. TI The half-filled Landau level: The case for Dirac composite fermions SO SCIENCE LA English DT Article ID LIQUID-LIKE STATE; QUANTUM HALL; SURFACE; ENERGY; CONDUCTANCE; NU=1/2; SYSTEM AB In a two-dimensional electron gas under a strong magnetic field, correlations generate emergent excitations distinct from electrons. It has been predicted that "composite fermions"-bound states of an electron with two magnetic flux quanta-can experience zero net magnetic field and form a Fermi sea. Using infinite-cylinder density matrix renormalization group numerical simulations, we verify the existence of this exotic Fermi sea, but find that the phase exhibits particle-hole symmetry. This is self-consistent only if composite fermions are massless Dirac particles, similar to the surface of a topological insulator. Exploiting this analogy, we observe the suppression of 2kF backscattering, a characteristic of Dirac particles. Thus, the phenomenology of Dirac fermions is also relevant to two-dimensional electron gases in the quantum Hall regime. C1 [Geraedts, Scott D.; Mong, Roger S. K.; Motrunich, Olexei I.] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Geraedts, Scott D.; Mong, Roger S. K.; Motrunich, Olexei I.] CALTECH, Inst Quantum Informat & Matter, Pasadena, CA 91125 USA. [Zaletel, Michael P.] Microsoft Res, Stn Q, Santa Barbara, CA 93106 USA. [Mong, Roger S. K.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Mong, Roger S. K.; Motrunich, Olexei I.] CALTECH, Walter Burke Inst Theoret Phys, Pasadena, CA 91125 USA. [Metlitski, Max A.] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Metlitski, Max A.] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Vishwanath, Ashvin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Motrunich, OI (reprint author), CALTECH, Dept Phys, Pasadena, CA 91125 USA.; Motrunich, OI (reprint author), CALTECH, Inst Quantum Informat & Matter, Pasadena, CA 91125 USA.; Motrunich, OI (reprint author), CALTECH, Walter Burke Inst Theoret Phys, Pasadena, CA 91125 USA. EM motrunch@caltech.edu FU National Science Engineering Research Council of Canada; U.S. Department of Energy BES [de-sc0002140]; Sherman Fairchild Foundation; U.S. Army Research Office [W911NF-14-1-0379]; Simons Investigator Award; NSF [PHY11-25915, DMR 1206096]; Caltech Institute for Quantum Information and Matter; NSF Physics Frontiers Center FX We enjoyed conversations with M. Barkeshli, M. Fisher, D. Haldane, R. Mishmash, C. Nayak, N. Read, E. Rezayi, D. Son, and T. Senthil. We particularly thank M. Barkeshli for first bringing the enigma of PH symmetry to our attention. R. M. and A.V. acknowledge KITP for hospitality. Supported by the National Science Engineering Research Council of Canada and U.S. Department of Energy BES grant de-sc0002140 (S.G.), the Sherman Fairchild Foundation (R. M.), U.S. Army Research Office grant W911NF-14-1-0379 (M. M.), a Simons Investigator Award (A.V.), NSF grant PHY11-25915 (R. M. and A.V.), NSF grant DMR 1206096 (S.G. and O.I.M.), and the Caltech Institute for Quantum Information and Matter, an NSF Physics Frontiers Center with support of the Gordon and Betty Moore Foundation. During the completion of this work, reference (53) appeared, which also provides a theoretical discussion of the PH-symmetric CFL. NR 47 TC 28 Z9 28 U1 9 U2 25 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD APR 8 PY 2016 VL 352 IS 6282 BP 197 EP 201 DI 10.1126/science.aad4302 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI7LM UT WOS:000373681600039 PM 27124453 ER PT J AU Tan, I Storelvmo, T Zelinka, MD AF Tan, Ivy Storelvmo, Trude Zelinka, Mark D. TI Observational constraints on mixed-phase clouds imply higher climate sensitivity SO SCIENCE LA English DT Article ID ICE NUCLEATION; MINERAL DUST; MODELS; MULTIMODEL; FEEDBACKS; SATELLITE; ECMWF AB Global climate model (GCM) estimates of the equilibrium global mean surface temperature response to a doubling of atmospheric CO2, measured by the equilibrium climate sensitivity (ECS), range from 2.0 degrees to 4.6 degrees C. Clouds are among the leading causes of this uncertainty. Here we show that the ECS can be up to 1.3 degrees C higher in simulations where mixed-phase clouds consisting of ice crystals and supercooled liquid droplets are constrained by global satellite observations. The higher ECS estimates are directly linked to a weakened cloud-phase feedback arising from a decreased cloud glaciation rate in a warmer climate. We point out the need for realistic representations of the supercooled liquid fraction in mixed-phase clouds in GCMs, given the sensitivity of the ECS to the cloud-phase feedback. C1 [Tan, Ivy; Storelvmo, Trude] Yale Univ, Dept Geol & Geophys, POB 6666, New Haven, CT 06511 USA. [Zelinka, Mark D.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. RP Tan, I (reprint author), Yale Univ, Dept Geol & Geophys, POB 6666, New Haven, CT 06511 USA. EM ivy.tan@yale.edu RI Zelinka, Mark/C-4627-2011 OI Zelinka, Mark/0000-0002-6570-5445 FU NASA Headquarters under the NASA Earth and Space Science Fellowship Program [NNX14AL07H]; NSF [1352417]; Regional and Global Climate Modeling Program of the Office of Science at the U.S. Department of Energy (DOE) [DE-SC0012580]; DOE by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by NASA Headquarters under the NASA Earth and Space Science Fellowship Program, grant NNX14AL07H. We also acknowledge high-performance computing support from Yellowstone provided by National Center for Atmospheric Research's Computational and Information Systems Laboratory, sponsored by NSF under grant 1352417. The effort of M.D.Z. was supported by the Regional and Global Climate Modeling Program of the Office of Science at the U.S. Department of Energy (DOE) under grant DE-SC0012580 and was performed under the auspices of DOE by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. CALIOP data are available online at https://eosweb.larc.nasa.gov/order-data. National Centers for Environmental Prediction-DOE Reanalysis 2 data are also available online at www.esrl.noaa.gov/psd/data/gridded/data.ncep.reanalysis2.pressure.html. NR 30 TC 12 Z9 12 U1 5 U2 27 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD APR 8 PY 2016 VL 352 IS 6282 BP 224 EP 227 DI 10.1126/science.aad5300 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI7LM UT WOS:000373681600046 PM 27124459 ER PT J AU Yoo, JH Kwon, HJ Paeng, D Yeo, J Elhadj, S Grigoropoulos, CP AF Yoo, Jae-Hyuck Kwon, Hyuk-Jun Paeng, Dongwoo Yeo, Junyeob Elhadj, Selim Grigoropoulos, Costas P. TI Facile fabrication of a superhydrophobic cage by laser direct writing for site-specific colloidal self-assembled photonic crystal SO NANOTECHNOLOGY LA English DT Article DE superhydrophobic; self-assembly; laser ablation; photonic crystal; polytetrafluoroethylene (PTFE); polydimethylsiloxane (PDMS) ID WATER DROPLETS; TEFLON FILMS; SURFACES; DEPOSITION; TRANSPORT; ENTROPY AB Micron-sized ablated surface structures with nano-sized 'bumpy' structures were produced by femtosecond (fs) laser ablation of polytetrafluoroethylene (PTFE) film under ambient conditions. Upon just a single step, the processed surface exhibited hierarchical micro/nano morphology. In addition, due to the tribological properties of PTFE, polydimethylsiloxane (PDMS) could be replicated from the laser-ablated PTFE surface without anti-adhesive surface treatment. By controlling the design of the ablated patterns, tunable wettability and superhydrophobicity were achieved on both PTFE and PDMS replica surfaces. Furthermore, using fs laser ablation direct writing, a flexible superhydrophobic PDMS cage formed by superhydrophobic patterns encompassing the unmodified region was demonstrated for aqueous droplet positioning and trapping. Through evaporation-driven colloidal self-assembly in this superhydrophobic cage, a colloidal droplet containing polystyrene (PS) particles dried into a self-assembled photonic crystal, whose optical band gap could be manipulated by the particle size. C1 [Yoo, Jae-Hyuck; Kwon, Hyuk-Jun; Paeng, Dongwoo; Yeo, Junyeob] Univ Calif Berkeley, Dept Mech Engn, Laser Thermal Lab, Berkeley, CA 94720 USA. [Yoo, Jae-Hyuck; Elhadj, Selim; Grigoropoulos, Costas P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Grigoropoulos, CP (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM cgrigoro@berkeley.edu RI Yeo, Junyeob/I-1287-2013 OI Yeo, Junyeob/0000-0001-7422-3467 FU UC Lab Fees Research Program [12- LR-237713]; US National Science Foundation [CMMI-1363392]; US Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344] FX Support for this work by UC Lab Fees Research Program Grant No. 12- LR-237713 and US National Science Foundation Grant No. CMMI-1363392 is gratefully acknowledged. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the US Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. NR 46 TC 2 Z9 2 U1 13 U2 73 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD APR 8 PY 2016 VL 27 IS 14 AR 145604 DI 10.1088/0957-4484/27/14/145604 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DF0HV UT WOS:000371020700014 PM 26916834 ER PT J AU Asthagiri, D Ballal, D Venkataraman, P Fouad, WA Cox, KR Chapman, WG AF Asthagiri, D. Ballal, Deepti Venkataraman, Pradeep Fouad, Wael A. Cox, Kenneth R. Chapman, Walter G. TI Response to "Comment on 'Isolating the non-polar contributions to the intermolecular potential for water-alkane interactions'" [J. Chem. Phys. 144, 137101 (2016)] SO JOURNAL OF CHEMICAL PHYSICS LA English DT Editorial Material C1 [Asthagiri, D.; Ballal, Deepti; Venkataraman, Pradeep; Fouad, Wael A.; Cox, Kenneth R.; Chapman, Walter G.] Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. [Ballal, Deepti] Ames Lab, Ames, IA 50011 USA. [Venkataraman, Pradeep] Baker Hughes, Houston, TX 77019 USA. [Fouad, Wael A.] Petr Inst, Abu Dhabi, U Arab Emirates. RP Chapman, WG (reprint author), Rice Univ, Dept Chem & Biomol Engn, Houston, TX 77005 USA. EM wgchap@rice.edu RI VENKATARAMAN, PRADEEP/P-6058-2014; Asthagiri, Dilipkumar/P-9450-2016; OI VENKATARAMAN, PRADEEP/0000-0001-9679-229X; Asthagiri, Dilipkumar/0000-0001-5869-0807; Chapman, Walter/0000-0002-8789-9041 NR 8 TC 2 Z9 2 U1 1 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 7 PY 2016 VL 144 IS 13 AR 137102 DI 10.1063/1.4944979 PG 2 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ9IT UT WOS:000374527900038 PM 27059591 ER PT J AU Skinner, LB Galib, M Fulton, JL Mundy, CJ Parise, JB Pham, VT Schenter, GK Benmore, CJ AF Skinner, L. B. Galib, M. Fulton, J. L. Mundy, C. J. Parise, J. B. Pham, V. -T. Schenter, G. K. Benmore, C. J. TI The structure of liquid water up to 360 MPa from x-ray diffraction measurements using a high Q-range and from molecular simulation SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RADIAL-DISTRIBUTION FUNCTIONS; DYNAMICS SIMULATIONS; PRESSURES; SCATTERING; TEMPERATURES; DENSITY; AMBIENT; MODEL AB X-ray diffraction measurements of liquid water are reported at pressures up to 360 MPa corresponding to a density of 0.0373 molecules per angstrom(3). The measurements were conducted at a spatial resolution corresponding to Qmax = 16 angstrom(-1). The method of data analysis and measurement in this study follows the earlier benchmark results reported for water under ambient conditions having a density of 0.0333 molecules per angstrom(3) and Q(max) = 20 angstrom(-1) [J. Chem. Phys. 138, 074506 (2013)] and at 70 degrees C having a density of 0.0327 molecules per angstrom(3) and Q(max) = 20 angstrom(-1) [J. Chem. Phys. 141, 214507 (2014)]. The structure of water is very different at these three different T and P state points and thus they provide the basis for evaluating the fidelity of molecular simulation. Measurements show that at 360 MPa, the 4 waters residing in the region between 2.3 and 3 angstrom are nearly unchanged: the peak position, shape, and coordination number are nearly identical to their values under ambient conditions. However, in the region above 3 angstrom, large structural changes occur with the collapse of the well-defined 2nd shell and shifting of higher shells to shorter distances. The measured structure is compared to simulated structure using intermolecular potentials described by both first-principles methods (revPBE-D3) and classical potentials (TIP4P/2005, MB-pol, and mW). The DFT-based, revPBE-D3, method and the many-body empirical potential model, MB-pol, provide the best overall representation of the ambient, high-temperature, and high-pressure data. The revPBE-D3, MB-pol, and the TIP4P/2005 models capture the densification mechanism, whereby the non-bonded 5th nearest neighbor molecule, which partially encroaches the 1st shell at ambient pressure, is pushed further into the local tetrahedral arrangement at higher pressures by the more distant molecules filling the void space in the network between the 1st and 2nd shells. (C) 2016 AIP Publishing LLC. C1 [Skinner, L. B.; Benmore, C. J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Skinner, L. B.; Parise, J. B.] SUNY Stony Brook, Inst Mineral Phys, Stony Brook, NY 11794 USA. [Galib, M.; Fulton, J. L.; Mundy, C. J.; Schenter, G. K.] Pacific NW Natl Lab, Phys & Computat Sci Div, Richland, WA 99354 USA. [Parise, J. B.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Parise, J. B.] Brookhaven Natl Lab, Photon Sci Div, Upton, NY 11973 USA. [Pham, V. -T.] Synchrotron SOLEIL LOrme Merisiers, BP48, F-91192 Gif Sur Yvette, France. [Pham, V. -T.] Vietnam Acad Sci & Technol, Ctr Quantum Elect, Inst Phys, POB 429, Hanoi 10000, Vietnam. RP Benmore, CJ (reprint author), Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA.; Fulton, JL (reprint author), Pacific NW Natl Lab, Phys & Computat Sci Div, Richland, WA 99354 USA. EM John.Fulton@pnnl.gov; benmore@anl.gov OI Skinner, Lawrie/0000-0001-7317-1642; Benmore, Chris/0000-0001-7007-7749 FU U.S. Department of Energy (DOE) office of Basic Energy Sciences [BES DE-FG02-09ER46650]; DOE [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences FX Thanks to Rick Spence and Doug Robinson for support with the beamline equipment at the Advanced Photon Source. The helpful comments of Valeria Molinero are acknowledged. We thank Francesco Paesani for assistance in the implementation of the MB-pol code. This work was supported by the U.S. Department of Energy (DOE) office of Basic Energy Sciences Grant No. BES DE-FG02-09ER46650, which supported MD simulations, data analysis, and manuscript preparation (L.B.S. and J.B.P.). DOE Contract No. DE-AC02-06CH11357 supports operation of the Advanced Photon Source at Argonne National Laboratory. The work by J.L.F., M.G., G.K.S., and C.J.M. was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 43 TC 4 Z9 4 U1 4 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD APR 7 PY 2016 VL 144 IS 13 AR 134504 DI 10.1063/1.4944935 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ9IT UT WOS:000374527900024 PM 27059577 ER PT J AU Bonsignori, M Zhou, TQ Sheng, ZZ Chen, L Gao, F Joyce, MG Ozorowski, G Chuang, GY Schramm, CA Wiehe, K Alam, SM Bradley, T Gladden, MA Hwang, KK Iyengar, S Kumar, A Lu, XZ Luo, K Mangiapani, MC Parks, RJ Song, HS Acharya, P Bailer, RT Cao, A Druz, A Georgiev, IS Kwon, YD Louder, MK Zhang, BS Zheng, AQ Hill, BJ Kong, R Soto, C Mullikin, JC Douek, DC Montefiori, DC Moody, MA Shaw, GM Hahn, BH Kelsoe, G Hraber, PT Korber, BT Boyd, SD Fire, AZ Kepler, TB Shapiro, L Ward, AB Mascola, JR Liao, HX Kwong, PD Haynes, BF AF Bonsignori, Mattia Zhou, Tongqing Sheng, Zizhang Chen, Lei Gao, Feng Joyce, M. Gordon Ozorowski, Gabriel Chuang, Gwo-Yu Schramm, Chaim A. Wiehe, Kevin Alam, S. Munir Bradley, Todd Gladden, Morgan A. Hwang, Kwan-Ki Iyengar, Sheelah Kumar, Amit Lu, Xiaozhi Luo, Kan Mangiapani, Michael C. Parks, Robert J. Song, Hongshuo Acharya, Priyamvada Bailer, Robert T. Cao, Allen Druz, Aliaksandr Georgiev, Ivelin S. Kwon, Young D. Louder, Mark K. Zhang, Baoshan Zheng, Anqi Hill, Brenna J. Kong, Rui Soto, Cinque Mullikin, James C. Douek, Daniel C. Montefiori, David C. Moody, Michael A. Shaw, George M. Hahn, Beatrice H. Kelsoe, Garnett Hraber, Peter T. Korber, Bette T. Boyd, Scott D. Fire, Andrew Z. Kepler, Thomas B. Shapiro, Lawrence Ward, Andrew B. Mascola, John R. Liao, Hua-Xin Kwong, Peter D. Haynes, Barton F. CA NISC Comparative Sequencing Progra TI Maturation Pathway from Germline to Broad HIV-1 Neutralizer of a CD4-Mimic Antibody SO CELL LA English DT Article ID HUMAN MONOCLONAL-ANTIBODIES; B-CELL RECEPTORS; VACCINE DEVELOPMENT; IMMUNOGEN DESIGN; FOUNDER VIRUS; AUTOREACTIVITY; INFECTION; INDUCTION; MEMBRANE; BINDING AB Antibodies with ontogenies from V(H)1-2 or V(H)1-46-germline genes dominate the broadly neutralizing response against the CD4-binding site (CD4bs) on HIV-1. Here, we define with longitudinal sampling from time-of-infection the development of a V(H)1-46-derived antibody lineage that matured to neutralize 90% of HIV-1 isolates. Structures of lineage antibodies CH235 (week 41 from time-of-infection, 18% breadth), CH235.9 (week 152, 77%), and CH235.12 (week 323, 90%) demonstrated the maturing epitope to focus on the conformationally invariant portion of the CD4bs. Similarities between CH235 lineage and five unrelated CD4bs lineages in epitope focusing, length-of-time to develop breadth, and extraordinary level of somatic hypermutation suggested commonalities in maturation among all CD4bs antibodies. Fortunately, the required CH235-lineage hypermutation appeared substantially guided by the intrinsic mutability of the V(H)1-46 gene, which closely resembled V(H)1-2. We integrated our CH235-lineage findings with a second broadly neutralizing lineage and HIV-1 co-evolution to suggest a vaccination strategy for inducing both lineages. C1 [Bonsignori, Mattia; Gao, Feng; Wiehe, Kevin; Alam, S. Munir; Bradley, Todd; Gladden, Morgan A.; Hwang, Kwan-Ki; Iyengar, Sheelah; Kumar, Amit; Lu, Xiaozhi; Luo, Kan; Mangiapani, Michael C.; Parks, Robert J.; Song, Hongshuo; Montefiori, David C.; Moody, Michael A.; Kelsoe, Garnett; Liao, Hua-Xin; Haynes, Barton F.] Duke Univ, Sch Med, Duke Human Vaccine Inst, Durham, NC 27710 USA. [Bonsignori, Mattia; Gao, Feng; Wiehe, Kevin; Alam, S. Munir; Liao, Hua-Xin; Haynes, Barton F.] Duke Univ, Sch Med, Dept Med, Durham, NC 27710 USA. [Zhou, Tongqing; Chen, Lei; Joyce, M. Gordon; Chuang, Gwo-Yu; Acharya, Priyamvada; Bailer, Robert T.; Cao, Allen; Druz, Aliaksandr; Georgiev, Ivelin S.; Kwon, Young D.; Louder, Mark K.; Zhang, Baoshan; Zheng, Anqi; Hill, Brenna J.; Kong, Rui; Soto, Cinque; Douek, Daniel C.; Shapiro, Lawrence; Mascola, John R.; Kwong, Peter D.] NIAID, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA. [Sheng, Zizhang; Schramm, Chaim A.; Shapiro, Lawrence] Columbia Univ, Dept Biochem & Mol Biophys, New York, NY 10032 USA. [Sheng, Zizhang; Schramm, Chaim A.; Shapiro, Lawrence] Columbia Univ, Dept Syst Biol, New York, NY 10032 USA. [Ozorowski, Gabriel; Ward, Andrew B.] Scripps Res Inst, Dept Integrat Struct & Computat Biol, La Jolla, CA 92037 USA. [Ozorowski, Gabriel; Ward, Andrew B.] Scripps Res Inst, CAVD, IAVI Neutralizing Antibody Ctr, La Jolla, CA 92037 USA. [Ozorowski, Gabriel; Ward, Andrew B.] Scripps Res Inst, Ctr HIV AIDS Vaccine Immunol & Immunogen Discover, La Jolla, CA 92037 USA. [Georgiev, Ivelin S.] Vanderbilt Univ, Med Ctr, Dept Pathol Microbiol & Immunol, Nashville, TN 37232 USA. [Georgiev, Ivelin S.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37232 USA. [Georgiev, Ivelin S.] Vanderbilt Univ, Med Ctr, Vanderbilt Vaccine Ctr, Nashville, TN 37232 USA. [Mullikin, James C.; NISC Comparative Sequencing Progra] NHGRI, NIH Intramural Sequencing Ctr, NIH, Bethesda, MD 20892 USA. [Montefiori, David C.] Duke Univ, Sch Med, Dept Surg, Durham, NC 27710 USA. [Montefiori, David C.; Moody, Michael A.] Duke Univ, Sch Med, Dept Pediat, Durham, NC 27710 USA. [Montefiori, David C.; Moody, Michael A.; Kelsoe, Garnett; Haynes, Barton F.] Duke Univ, Sch Med, Dept Immunol, Durham, NC 27710 USA. [Shaw, George M.; Hahn, Beatrice H.] Univ Penn, Perelman Sch Med, Dept Med, Philadelphia, PA 19104 USA. [Shaw, George M.; Hahn, Beatrice H.] Univ Penn, Perelman Sch Med, Dept Microbiol, Philadelphia, PA 19104 USA. [Hraber, Peter T.; Korber, Bette T.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. [Boyd, Scott D.; Fire, Andrew Z.] Stanford Sch Med, Dept Pathol, Palo Alto, CA 94305 USA. [Kepler, Thomas B.] Boston Univ, Dept Microbiol, Boston, MA 02118 USA. [Kepler, Thomas B.] Boston Univ, Dept Math & Stat, Boston, MA 02118 USA. [Haynes, Barton F.] Duke Univ, Sch Med, Duke Global Hlth Inst, Durham, NC 27710 USA. RP Haynes, BF (reprint author), Duke Univ, Sch Med, Duke Human Vaccine Inst, Durham, NC 27710 USA.; Haynes, BF (reprint author), Duke Univ, Sch Med, Dept Med, Durham, NC 27710 USA.; Kwong, PD (reprint author), NIAID, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA.; Haynes, BF (reprint author), Duke Univ, Sch Med, Dept Immunol, Durham, NC 27710 USA.; Haynes, BF (reprint author), Duke Univ, Sch Med, Duke Global Hlth Inst, Durham, NC 27710 USA. EM pdkwong@nih.gov; barton.haynes@duke.edu RI Ward, Andrew/F-9203-2014; Zhou, Tongqing/A-6880-2010; Kwon, Young Do/A-6957-2010; OI Ward, Andrew/0000-0001-7153-3769; Zhou, Tongqing/0000-0002-3935-4637; Korber, Bette/0000-0002-2026-5757; Hraber, Peter/0000-0002-2920-4897 FU Division of AIDS, NIAID, NIH Center for HIV/AIDS Vaccine Immunology-Immunogen Discovery [UM1 AI100645]; Scripps CHAVI-ID [UM1 AI100663]; International AIDS Vaccine Initiative; Bill and Melinda Gates Foundation; Intramural Research Program of the Vaccine Research Center, NIAID, NIH; NIH [P01-AI104722]; US Department of Energy, Basic Energy Sciences, Office of Science [W-31-109-Eng-38] FX The authors thank K. Lloyd, A. Eaton, T. Von Holle, T. Gurley, L. Armand, D. Kozink, A. Cooper, F. Perrin, J. Pritchett, A. Foulger, G. Hernandez, S. Arora, R. Kauffman, A. Trama of the Duke Human Vaccine Institute, J. Whitesides, D. Marshall and the DHVI Flow Cytometry Core for technical assistance, and K. Soderberg for project coordination; members of the Structural Biology Section and Structural Bioinformatics Core, Vaccine Research Center, for discussions and comments on the manuscript; J. Baalwa, D. Ellenberger, K. Hong, J. Kim, F. McCutchan, L. Morris, J. Overbaugh, E. Sanders-Buell, R. Swanstrom, M. Thomson, S. Tovanabutra, C. Williamson, and L. Zhang for contributing HIV-1 Envelope plasmids. The authors also thank Gift Kamanga, Michael S. Cohen, and the CHAVI clinical team for clinical trial participant recruitment and sample provision. Supported by a grant from the Division of AIDS, NIAID, NIH Center for HIV/AIDS Vaccine Immunology-Immunogen Discovery UM1 AI100645 (Duke CHAVI-ID), the Scripps CHAVI-ID (UM1 AI100663), the International AIDS Vaccine Initiative, and the Bill and Melinda Gates Foundation (CAVD) to A.B.W. Support for this work was provided by the Intramural Research Program of the Vaccine Research Center, NIAID, NIH, and by NIH grant P01-AI104722. Use of sector 22 (Southeast Region Collaborative Access team) at the Advanced Photon Source was supported by the US Department of Energy, Basic Energy Sciences, Office of Science (contract W-31-109-Eng-38). M.B., P.T.H., B.T.K., H.-X.L. and B.F.H. have filed patent applications directed to antibodies and use of various envelopes as immunogens. None of the authors declared conflicts of interest. NR 44 TC 35 Z9 35 U1 4 U2 10 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD APR 7 PY 2016 VL 165 IS 2 BP 449 EP 463 DI 10.1016/j.cell.2016.02.022 PG 15 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DJ3RJ UT WOS:000374123000022 PM 26949186 ER PT J AU Nelles, DA Fang, MY O'Connell, MR Xu, JL Markmiller, SJ Doudna, JA Yeo, GW AF Nelles, David A. Fang, Mark Y. O'Connell, Mitchell R. Xu, Jia L. Markmiller, Sebastian J. Doudna, Jennifer A. Yeo, Gene W. TI Programmable RNA Tracking in Live Cells with CRISPR/Cas9 SO CELL LA English DT Article ID STRESS GRANULES; LIVING CELLS; CAS SYSTEM; RECOGNITION; PLATFORM; DNA; LOCALIZATION; NUCLEASES; PROTEINS; DYNAMICS AB RNA-programmed genome editing using CRISPR/Cas9 from Streptococcus pyogenes has enabled rapid and accessible alteration of specific genomic loci in many organisms. A flexible means to target RNA would allow alteration and imaging of endogenous RNA transcripts analogous to CRISPR/Cas-based genomic tools, but most RNA targeting methods rely on incorporation of exogenous tags. Here, we demonstrate that nuclease-inactive S. pyogenes CRISPR/Cas9 can bind RNA in a nucleic-acid-programmed manner and allow endogenous RNA tracking in living cells. We show that nuclear-localized RNA-targeting Cas9 (RCas9) is exported to the cytoplasm only in the presence of sgRNAs targeting mRNA and observe accumulation of ACTB, CCNA2, and TFRC mRNAs in RNA granules that correlate with fluorescence in situ hybridization. We also demonstrate time-resolved measurements of ACTB mRNA trafficking to stress granules. Our results establish RCas9 as a means to track RNA in living cells in a programmable manner without genetically encoded tags. C1 [Nelles, David A.; Fang, Mark Y.; Xu, Jia L.; Markmiller, Sebastian J.; Yeo, Gene W.] Univ Calif San Diego, Dept Cellular & Mol Med, La Jolla, CA 92037 USA. [Nelles, David A.; Fang, Mark Y.; Xu, Jia L.; Markmiller, Sebastian J.; Yeo, Gene W.] Univ Calif San Diego, Inst Genom Med, La Jolla, CA 92037 USA. [Nelles, David A.; Yeo, Gene W.] Univ Calif San Diego, Mat Sci & Engn Grad Program, La Jolla, CA 92093 USA. [Yeo, Gene W.] Natl Univ Singapore, Yong Loo Lin Sch Med, Dept Physiol, Singapore 1190777, Singapore. [O'Connell, Mitchell R.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [O'Connell, Mitchell R.; Doudna, Jennifer A.] Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Innovat Genom Initiat, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Yeo, GW (reprint author), Univ Calif San Diego, Dept Cellular & Mol Med, La Jolla, CA 92037 USA.; Yeo, GW (reprint author), Univ Calif San Diego, Inst Genom Med, La Jolla, CA 92037 USA.; Yeo, GW (reprint author), Univ Calif San Diego, Mat Sci & Engn Grad Program, La Jolla, CA 92093 USA.; Yeo, GW (reprint author), Natl Univ Singapore, Yong Loo Lin Sch Med, Dept Physiol, Singapore 1190777, Singapore. EM geneyeo@ucsd.edu FU NIH [HG004659, NS075449]; California Institute of Regenerative Medicine [RB3-05009, RB4-06045]; National Science Foundation Graduate Research Fellowship [DGE-1144086]; Powell-Focht graduate fellowship; CJ Martin fellowship from the National Health and Medical Research Council (Australia) FX We acknowledge members of the G.W.Y. lab, particularly Ashleigh Schaffer, Stefan Aigner, and Ron Batra for critical comments. This work was supported by grants from the NIH (HG004659 and NS075449) and from the California Institute of Regenerative Medicine (RB3-05009 and RB4-06045) to G.W.Y. D.A.N. is supported by the National Science Foundation Graduate Research Fellowship (DGE-1144086) and Powell-Focht graduate fellowship. M.R.O. is supported by a CJ Martin fellowship from the National Health and Medical Research Council (Australia). J.A.D. is a Howard Hughes Medical Institute Investigator. G.W.Y. is an Alfred P. Sloan Research Fellow. J.A.D. is a co-founder of Editas Medicine, Intellia Therapeutics, and Caribou Biosciences and a scientific advisor to Caribou, Intellia, eFFECTOR Therapeutics, and Driver. NR 36 TC 33 Z9 37 U1 37 U2 90 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD APR 7 PY 2016 VL 165 IS 2 BP 488 EP 496 DI 10.1016/j.cell.2016.02.054 PG 9 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DJ3RJ UT WOS:000374123000025 PM 26997482 ER PT J AU Hariprasad, DS Grau, G Schunk, PR Tjiptowidjojo, K AF Hariprasad, Daniel S. Grau, Gerd Schunk, P. Randall Tjiptowidjojo, Kristianto TI A computational model for doctoring fluid films in gravure printing SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FIELD-EFFECT TRANSISTORS; HIGH-SPEED; LUBRICATION; LAYERS; ELECTRONICS; INKS; DEVICES; ROLL; GATE AB The wiping, or doctoring, process in gravure printing presents a fundamental barrier to resolving the micron-sized features desired in printed electronics applications. This barrier starts with the residual fluid film left behind after wiping, and its importance grows as feature sizes are reduced, especially as the feature size approaches the thickness of the residual fluid film. In this work, various mechanical complexities are considered in a computational model developed to predict the residual fluid film thickness. Lubrication models alone are inadequate, and deformation of the doctor blade body together with elastohydrodynamic lubrication must be considered to make the model predictive of experimental trends. Moreover, model results demonstrate that the particular form of the wetted region of the blade has a significant impact on the model's ability to reproduce experimental measurements. (C) 2016 AIP Publishing LLC. C1 [Hariprasad, Daniel S.; Schunk, P. Randall; Tjiptowidjojo, Kristianto] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Grau, Gerd] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Schunk, P. Randall] Sandia Natl Labs, Adv Mat Lab, POB 5800, Albuquerque, NM 87185 USA. [Schunk, P. Randall; Tjiptowidjojo, Kristianto] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. RP Hariprasad, DS (reprint author), Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. EM dshari@unm.edu FU National Science Foundation [EEC-1160494] FX This work is based upon work supported primarily by the National Science Foundation under Cooperative Agreement No. EEC-1160494. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation. NR 36 TC 0 Z9 0 U1 3 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 7 PY 2016 VL 119 IS 13 AR 135303 DI 10.1063/1.4945030 PG 9 WC Physics, Applied SC Physics GA DJ4BK UT WOS:000374150200033 ER PT J AU Montgomery, JM Samudrala, GK Velisavljevic, N Vohra, YK AF Montgomery, J. M. Samudrala, G. K. Velisavljevic, N. Vohra, Y. K. TI High-pressure high-temperature phase diagram of gadolinium studied using a boron-doped heater anvil SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID X-RAY-DIFFRACTION; RARE-EARTH-METALS; CRYSTAL-STRUCTURE; GPA; TRANSFORMATION; TRANSITIONS; KINETICS; HYDROGEN; CELL AB A boron-doped designer heater anvil is used in conjunction with powder x-ray diffraction to collect structural information on a sample of quasi-hydrostatically loaded gadolinium metal up to pressures above 8GPa and 600K. The heater anvil consists of a natural diamond anvil that has been surface modified with a homoepitaxially grown chemical-vapor-deposited layer of conducting boron-doped diamond, and is used as a DC heating element. Internally insulating both diamond anvils with sapphire support seats allows for heating and cooling of the high-pressure area on the order of a few tens of seconds. This device is then used to scan the phase diagram of the sample by oscillating the temperature while continuously increasing the externally applied pressure and collecting in situ time-resolved powder diffraction images. In the pressure-temperature range covered in this experiment, the gadolinium sample is observed in its hcp, alpha Sm, and dhcp phases. Under this temperature cycling, the hcp! aSm transition proceeds in discontinuous steps at points along the expected phase boundary. From these measurements (representing only one hour of synchrotron x-ray collection time), a single-experiment equation of state and phase diagram of each phase of gadolinium is presented for the range of 0-10GPa and 300-650K. (C) 2016 AIP Publishing LLC. C1 [Montgomery, J. M.; Samudrala, G. K.; Vohra, Y. K.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Velisavljevic, N.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Montgomery, JM (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. FU Department of Energy (DOE)-National Nuclear Security Administration [DE-NA0002014]; Department of Education [P200A120026]; DOE-NNSA [DE-NA0001974, DE-AC52-06NA25396]; DOE-BES [DE-FG02-99ER45775, DE-AC02-06CH11357]; NSFLANL Science Campaign 2 FX This work was supported by the Department of Energy (DOE)-National Nuclear Security Administration under Grant No. DE-NA0002014, as well as by the Department of Education Grant No. P200A120026. Large portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source, Argonne National Laboratories in Chicago, Illinois. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES, under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS was supported by DOE-BES under Contract No. DE-AC02-06CH11357. Work was in part supported by LANL Science Campaign 2. Los Alamos National Laboratory (LANL) is operated by LANS, LLC for the DOE-NNSA under Contract No. DE-AC52-06NA25396. NR 43 TC 0 Z9 0 U1 10 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 7 PY 2016 VL 119 IS 13 AR 135902 DI 10.1063/1.4945704 PG 7 WC Physics, Applied SC Physics GA DJ4BK UT WOS:000374150200047 ER PT J AU Muramatsu, T Gasparov, LV Berger, H Hemley, RJ Struzhkin, VV AF Muramatsu, Takaki Gasparov, Lev V. Berger, Helmuth Hemley, Russell J. Struzhkin, Viktor V. TI Electrical resistance of single-crystal magnetite (Fe3O4) under quasi-hydrostatic pressures up to 100GPa SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID VERWEY TRANSITION; METALLIZATION; CONDUCTIVITY AB The pressure dependence of electrical resistance of single-crystal magnetite (Fe3O4) was measured under quasi-hydrostatic conditions to 100 GPa using low-temperature, megabar diamond-anvil cell techniques in order to gain insight into the anomalous behavior of this material that has been reported over the years in different high-pressure experiments. The measurements under nearly hydrostatic pressure conditions allowed us to detect the clear Verwey transition and the high-pressure structural phase. The appearance of a metallic ground state after the suppression of the Verwey transition around 20 GPa and the concomitant enhancement of the electrical resistance caused by the structural transformation to the high-pressure phase form reentrant semiconducting-metallic-semiconducting behavior, although the appearance of the metallic phase is highly sensitive to stress conditions and details of the measurement technique. (C) 2016 AIP Publishing LLC. C1 [Muramatsu, Takaki; Hemley, Russell J.; Struzhkin, Viktor V.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Gasparov, Lev V.] Univ N Florida, Dept Phys, Jacksonville, FL 32224 USA. [Berger, Helmuth] Ecole Polytech Fed Lausanne, Lausanne, Switzerland. [Hemley, Russell J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Muramatsu, T (reprint author), Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. OI Gasparov, Lev/0000-0003-1609-3363 FU Energy Frontier Research in Extreme Environments (EFree), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC-0001057]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-FG02-02ER45955, DE-FG02-99ER45775]; National Science Foundation [DMR-0805073, DMR-0958349, DMR-1429428]; Office of Naval Research Award [N00014-06-1-013]; UNF Terry Presidential Professorship; U.S. Department of Energy/National Nuclear Security Administration [DE-NA-0002006]; U.S. DOE [DE-AC52-07NA27344] FX This work was supported as part of Energy Frontier Research in Extreme Environments (EFree), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC-0001057 (salary support for T. M.). V. S. acknowledges the support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Contract Nos. DE-FG02-02ER45955 and DE-FG02-99ER45775. L. G. acknowledges the support from the National Science Foundation Grant Nos. DMR-0805073, DMR-0958349, DMR-1429428, Office of Naval Research Award No. N00014-06-1-013, and the UNF Terry Presidential Professorship. Facilities at Carnegie were supported by the U.S. Department of Energy/National Nuclear Security Administration (Award No. DE-NA-0002006, CDAC). Work at LLNL was performed under the auspices of the U.S. DOE under Contract No. DE-AC52-07NA27344. NR 34 TC 1 Z9 1 U1 7 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 7 PY 2016 VL 119 IS 13 AR 135903 DI 10.1063/1.4945388 PG 6 WC Physics, Applied SC Physics GA DJ4BK UT WOS:000374150200048 ER PT J AU Stavrou, E Zaug, JM Bastea, S Crowhurst, JC AF Stavrou, Elissaios Zaug, Joseph M. Bastea, Sorin Crowhurst, Jonathan C. TI The equation of state of 5-nitro-2,4-dihydro-1,2,4,-triazol-3-one determined via in-situ optical microscopy and interferometry measurements SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HIGH-PRESSURES; ARGON; DIAMOND; STRAIN; TEMPERATURES; COMPRESSION; SHOCK; NTO; GPA AB Quasi-hydrostatic high-pressure equations of state (EOS) are typically determined, for crystalline solids, by measuring unit-cell volumes using x-ray diffraction (XRD) techniques. However, when characterizing low-symmetry materials with large unit cells, conventional XRD approaches may become problematic. To overcome this issue, we examined the utility of a "direct" approach toward determining high pressure material volume by measuring surface area and sample thickness using optical microscopy and interferometry (OMI), respectively. We have validated this experimental approach by comparing results obtained for 2,4,6-triamino-1,3,5-trinitrobenzene TATB with an EOS determined from synchrotron XRD measurements; and, a good match is observed. We have measured the high pressure EOS of 5-nitro-2,4-dihydro1,2,4,triazol-3-one (alpha-NTO) up to 28GPa. No high-pressure XRD EOS data have been published on alpha-NTO, probably due to its complex crystal structure. The results of this study suggest that OMI is a reliable and versatile alternative for determining EOSs, especially when conventional methodologies are impractical. (C) 2016 AIP Publishing LLC. C1 [Stavrou, Elissaios; Zaug, Joseph M.; Bastea, Sorin; Crowhurst, Jonathan C.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, POB 808, Livermore, CA 94550 USA. RP Stavrou, E; Zaug, JM (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, POB 808, Livermore, CA 94550 USA. EM stavrou1@llnl.gov; zaug1@llnl.gov OI Zaug, Joseph/0000-0001-8999-3800 FU U.S. Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Security, LLC under Contract No. DE-AC52-07NA27344. We thank the Joint Munitions Program (JMP - TCG-III) for supporting this study and also the high explosives science campaign II research program at Lawrence Livermore National Laboratory. We acknowledge Philip Pagoria for providing the samples used in this study. We thank Larry E. Fried for helpful discussions and support and Michael R. Armstrong for valuable comments. We are very grateful to Karl Mills (Technical Instruments, www.techinist.com) who graciously loaned us a Nikon CCD camera to enable this work to proceed. NR 39 TC 1 Z9 1 U1 4 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD APR 7 PY 2016 VL 119 IS 13 AR 135904 DI 10.1063/1.4945426 PG 9 WC Physics, Applied SC Physics GA DJ4BK UT WOS:000374150200049 ER PT J AU Kim, S Zhang, ZX Wang, SL Yang, L Cairns, EJ Penner-Hahn, JE Deb, A AF Kim, Soojeong Zhang, Zhenxi Wang, Senlin Yang, Li Cairns, Elton J. Penner-Hahn, James E. Deb, Aniruddha TI Electrochemical and Structural Investigation of the Mechanism of Irreversibility in Li3V2(PO4)(3) Cathodes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LITHIUM-ION BATTERIES; RAY-ABSORPTION SPECTROSCOPY; CARBON-COATED LI3V2(PO4)(3); VANADIUM PHOSPHATE; ELECTRODE MATERIALS; DOPED LI3V2(PO4)(3); PERFORMANCE; SPECTRA; CELL; LI4/3TI5/3O4 AB Lithium-ion batteries dominate the battery field, particularly for electric and hybrid vehicles. Monoclinic Li3V2(PO4)(3) has emerged as one of the most promising candidates for the cathode in lithium-ion batteries, offering better environmental safety and lower cost than competing materials. We have used in situ X-ray absorption spectroscopy to characterize the evolution of the vanadium in a Li3V2(PO4)(3) cathode as it is cycled electrochemically. These data demonstrate the presence of significant kinetic effects such that the measured electrochemical behavior does not represent the bulk vanadium. When the cell is cycled between 3 and 4.5 V, there are two distinct vanadium species. When the potential is raised above 4.5 V, a third species is observed, consistent with formation of V5+. XANES data for the cathode after 3-4.8 V cycling are consistent with a severely distorted vanadium site, suggesting that lithium-vanadium antisite mixing may be responsible for the electrochemical irreversibility that is seen above 4.5 V. C1 [Kim, Soojeong; Penner-Hahn, James E.; Deb, Aniruddha] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. [Zhang, Zhenxi; Wang, Senlin; Yang, Li] Hanghai Jiao Tong Univ, Sch Chem & Chem Technol, Shanghai 200240, Peoples R China. [Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem & Biomol Engn Dept, Berkeley, CA 94720 USA. RP Penner-Hahn, JE; Deb, A (reprint author), Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. EM jeph@umich.edu; debani@umich.edu RI Deb, Aniruddha/H-7529-2016; Cairns, Elton/E-8873-2012 OI Deb, Aniruddha/0000-0002-0331-9709; Cairns, Elton/0000-0002-1179-7591 FU University of Michigan-Shanghai Jiao Tong University collaborative research project; National Natural Science Foundation of China [21103108, 21173148]; E.I. DuPont de Nemours and Co.; Dow Chemical Company; U.S. NSF [DMR-9304725]; State of Illinois; Department of Commerce; Board of Higher Education Grant [IBHEHECANWU96] FX Financial support for this work came from a University of Michigan-Shanghai Jiao Tong University collaborative research project. Li Yang acknowledges the National Natural Science Foundation of China (Grants 21103108 and 21173148). DND-CAT (5-BM-D) is supported by the E.I. DuPont de Nemours and Co., The Dow Chemical Company, the U.S. NSF through Grant DMR-9304725, and State of Illinois, Department of Commerce and the Board of Higher Education Grant IBHEHECANWU96. NR 48 TC 4 Z9 4 U1 13 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7005 EP 7012 DI 10.1021/acs.jpcc.6b00408 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700011 ER PT J AU Ilyas, N Harivyasi, SS Zahl, P Cortes, R Hofmann, OT Sutter, P Zojer, E Monti, OLA AF Ilyas, Nahid Harivyasi, Shashank S. Zahl, Percy Cortes, Rocio Hofmann, Oliver T. Sutter, Peter Zojer, Egbert Monti, Oliver L. A. TI Sticking with the Pointy End? Molecular Configuration of Chloro Boron-Subphthalocyanine on Cu(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SCANNING TUNNELING MICROSCOPE; METAL-SURFACES; PHTHALOCYANINE MONOLAYER; CHARGE-TRANSFER; ADSORPTION; INTERFACE; SUBSTRATE; FILMS; MECHANISM; ALIGNMENT AB In this combined low-temperature scanning tunneling microscopy (STM) and density functional theory (DFT) study, we investigate self-assembly of the dipolar nonplanar organic semiconductor chloro boron-subphthalocyanine (ClB-SubPc) on Cu(111). We observe multiple distinct adsorption configurations and demonstrate that these can only be understood by taking surface-catalyzed dechlorination into account. A detailed investigation of possible adsorption configurations and the comparison of experimental and computational STM images demonstrates that the configurations correspond to "Cl-up" molecules with the B Cl moiety pointing toward the vacuum side of the interface, and dechlorinated molecules. In contrast to the standard interpretation of adsorption of nonplanar molecules in the phthalocyanine family, we find no evidence for "Cl-down" molecules where the B Cl moiety would be pointing toward the Cu surface. We show computationally that such a configuration is unstable and thus is highly unlikely to occur for C1B-SubPc on Cu(111). Using these assignments, we discuss the different self-assembly motifs in the submonolayer coverage regime. The combination of DFT and STM is essential to gain a full atomistic understanding of the surface molecule interactions, and our findings imply that phthalocyanines may undergo surface-catalyzed reactions hitherto not considered. Our results also indicate that care has to be taken when analyzing possible adsorption configurations of polar members of the phthalocyanine family, especially when they are adsorbed on comparably reactive surfaces like Cu(111). C1 [Ilyas, Nahid; Monti, Oliver L. A.] Univ Arizona, Dept Chem & Biochem, 1306 E Univ Blvd, Tucson, AZ 85721 USA. [Harivyasi, Shashank S.; Hofmann, Oliver T.; Zojer, Egbert] Graz Univ Technol, NAWI Graz, Inst Solid State Phys, Petersgasse 16, A-8010 Graz, Austria. [Zahl, Percy; Cortes, Rocio; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Sutter, Peter] Univ Nebraska, Dept Elect & Comp Engn, Lincoln, NE 68588 USA. [Monti, Oliver L. A.] Univ Arizona, Dept Phys, 1118 E 4th St, Tucson, AZ 85721 USA. RP Monti, OLA (reprint author), Univ Arizona, Dept Chem & Biochem, 1306 E Univ Blvd, Tucson, AZ 85721 USA.; Zojer, E (reprint author), Graz Univ Technol, NAWI Graz, Inst Solid State Phys, Petersgasse 16, A-8010 Graz, Austria.; Monti, OLA (reprint author), Univ Arizona, Dept Phys, 1118 E 4th St, Tucson, AZ 85721 USA. EM egbert.zojer@tugraz.at; monti@u.arizona.edu RI Hofmann, Oliver/C-4338-2008; Zojer, Egbert/B-3265-2010; OI Hofmann, Oliver/0000-0002-2120-3259; Zojer, Egbert/0000-0002-6502-1721; Harivyasi, Shashank S./0000-0002-2174-5226 FU National Science Foundation (Arizona) [CHE-1213243]; European Union Seventh Framework Programme [607232]; Austrian Science Fund (FWF) [P24666-N20]; U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX The authors thank Leonhard Grill (University of Graz), Elisabeth Wruss, and Elisabeth Verwuster (TU Graz) for stimulating discussions. This research was supported by the National Science Foundation under Grant CHE-1213243 (Arizona), by the European Union Seventh Framework Programme under grant agreement no 607232 [THINFACE] and by the Austrian Science Fund (FWF), P24666-N20. This research also used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. The computational results presented have been achieved using the Vienna Scientific Cluster (VSC). We would also like to thank Dr. Bjorn Lange and Prof. Volker Blum at Duke University for making their new implementation of STM simulations in FHI-aims available to us. NR 54 TC 1 Z9 1 U1 10 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7113 EP 7121 DI 10.1021/acs.jpcc.5b11799 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700024 ER PT J AU Alexopoulos, K Lee, MS Liu, Y Zhi, YC Liu, YS Reyniers, MF Marin, GB Glezakou, VA Rousseau, R Lercher, JA AF Alexopoulos, Konstantinos Lee, Mal-Soon Liu, Yue Zhi, Yuchun Liu, Yuanshuai Reyniers, Marie-Francoise Marin, Guy B. Glezakou, Vassiliki-Alexandra Rousseau, Roger Lercher, Johannes A. TI Anharmonicity and Confinement in Zeolites: Structure, Spectroscopy, and Adsorption Free Energy of Ethanol in H-ZSM-5 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID AB-INITIO; NITRILE ADSORPTION; PROTON-TRANSFER; ACID CATALYSIS; ALKANES; COMPLEXES; METHANOL; ALCOHOL; PSEUDOPOTENTIALS; DEHYDRATION AB To account for thermal and entropic effects caused by the dynamics of the motion of the reaction intermediates, ethanol adsorption on the Bronsted acid site of the H-ZSM-5 catalyst has been studied at different temperatures and ethanol loadings using ab initio molecular dynamics (AIMD) simulations, infrared (IR) spectroscopy, and calorimetric measurements. At low temperatures (T <= 400 K) and ethanol loading, a single ethanol molecule adsorbed in H-ZSM-5 forms a Zundel-like structure where the proton is equally shared between the oxygen of the zeolite and the oxygen of the alcohol. At higher ethanol loading, a second ethanol molecule helps to stabilize the protonated ethanol at all temperatures by acting as a solvating agent. The vibrational density of states (VDOS), as calculated from the AIMD simulations, are in excellent agreement with measured IR spectra for C2H5OH, C2H5OD, and C2D5OH isotopomers and support the existence of both monomers and dimers. A quasi-harmonic approximation (QHA), applied to the VDOS obtained from the AIMD simulations, provides estimates of adsorption free energy within similar to 10 kJ/mol of the experimentally determined quantities, whereas the traditional approach, employing harmonic frequencies from a single ground state minimum, strongly overestimates the adsorption free energy by at least 20 similar to 50 kJ/mol. This discrepancy is traced back to the inability of the harmonic approximation to represent the contributions to the vibrational motions of the ethanol molecule upon confinement in the zeolite. C1 [Alexopoulos, Konstantinos; Reyniers, Marie-Francoise; Marin, Guy B.] Univ Ghent, Chem Technol Lab, B-9000 Ghent, Belgium. [Lee, Mal-Soon; Glezakou, Vassiliki-Alexandra; Rousseau, Roger; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Liu, Yue; Zhi, Yuchun; Liu, Yuanshuai; Lercher, Johannes A.] Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany. [Liu, Yue; Zhi, Yuchun; Liu, Yuanshuai; Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Inst, Lichtenbergstr 4, D-85748 Garching, Germany. RP Reyniers, MF (reprint author), Univ Ghent, Chem Technol Lab, B-9000 Ghent, Belgium.; Rousseau, R; Lercher, JA (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA.; Lercher, JA (reprint author), Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany.; Lercher, JA (reprint author), Tech Univ Munich, Catalysis Res Inst, Lichtenbergstr 4, D-85748 Garching, Germany. EM MarieFrancoise.Reyniers@UGent.be; roger.rousseau@pnnl.gov; johannes.lercher@pnnl.gov RI Rousseau, Roger/C-3703-2014; OI Lee, Mal-Soon/0000-0001-6851-177X FU Long Term Structural Methusalem - Flemish Government [BOF09/01M00409]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research located at PNNL; National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory; Stevin Supercomputer Infrastructure at Ghent University FX This article is dedicated to our colleague Dr. Bruce Garrett on the occasion of his 65th birthday. He has achieved significant impact in his career with his contributions to our understanding of how dynamical processes and anharmonicity contribute to rate theories as well as served as a dedicated steward of PNNL's fundamental science programs over the past decade. K.A., M.F.R, and G.B.M. were supported by the Long Term Structural Methusalem Funding by the Flemish Government, grant no. BOF09/01M00409. M.S.L., V.A.G., RR, and J.A.L. were supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. PNNL is a multiprogram national laboratory operated for DOE by Battelle. Computational resources were provided at W. R. Wiley Environmental Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at PNNL, the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory and the Stevin Supercomputer Infrastructure at Ghent University. NR 49 TC 4 Z9 4 U1 24 U2 61 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7172 EP 7182 DI 10.1021/acs.jpcc.6b00923 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700030 ER PT J AU Sutton, JE Overbury, SH Beste, A AF Sutton, Jonathan E. Overbury, Steven H. Beste, Ariana TI Coadsorbed Species Explain the Mechanism of Methanol Temperature-Programmed Desorption on CeO2(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID AUGMENTED-WAVE METHOD; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; CERIUM OXIDE; SADDLE-POINTS; ADSORPTION; SURFACE AB We have used density functional theory calculations to investigate the temperature-programmed desorption (TPD) of methanol from CeO2(111). For the first time, low-temperature water formation and high-temperature methanol desorption are explained by our calculations. High coverages of methanol, which correspond to experimental conditions, are required to properly describe these features of the TPD spectrum. We identify a mechanism for the low-temperature formation of water involving the dissociation of two methanol molecules on the same surface O atom and filling of the resulting surface vacancy with one of the methoxy products. After water desorption, methoxy groups are stabilized on the surface and react at higher temperatures to form methanol and formaldehyde by a disproportionation mechanism. Alternatively, the stabilized methoxy groups undergo sequential C-H scission reactions to produce formaldehyde. Calculated energy requirements and methanol/formaldehyde selectivity agree with the experimental data. C1 [Sutton, Jonathan E.; Overbury, Steven H.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Beste, Ariana] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Sutton, JE (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM suttonje@ornl.gov FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; National Energy Research Scientific Computing Center, a DOE Office of Science User Facility - Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC05-00OR22725]; DOE FX This research was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC05-00OR22725, and the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The authors also thank Dr. Aditya Savara for helpful discussions related to the Redhead analysis. This manuscript was authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. NR 22 TC 2 Z9 2 U1 6 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7241 EP 7247 DI 10.1021/acs.jpcc.6b02128 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700036 ER PT J AU El-Khoury, PZ Joly, AG Hess, WP AF El-Khoury, Patrick Z. Joly, Alan G. Hess, Wayne P. TI Hyperspectral Dark Field Optical Microscopy of Single Silver Nanospheres SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENHANCED RAMAN-SCATTERING; MOLECULE; NANOPARTICLES; PLASMONS; PARTICLE; TIME AB We record spectrally (400 <= lambda <= 675 nm, Delta lambda < 4.69 nm) and spatially (diffraction-limited, sampled at 85 nm(2)/pixel) resolved dark field (DF) scattering from single silver nanospheres of 100 nm in diameter. Hyperspectral DF optical microscopy is achieved by coupling a hyperspectral detector to an optical microscope, whereby spectrally resolved diffraction limited images of hundreds of silver nanoparticles can be recorded in similar to 30 s. We demonstrate how the centers and edges of individual particles can be localized in two dimensions to within a single pixel (85 nm(2)), using a statistical method for examining texture based on a co-occurrence matrix. Subsequently, spatial averaging of the spectral response in a 3 X 3 pixel area around the particle centers affords ample signal to noise to resolve the plasmon resonance of a single silver nanosphere. A close inspection of the scattering spectra of 31 different nanospheres reveals that each particle has its unique (i) relative scattering efficiency and (ii) plasmon resonance maximum and dephasing time. These observations are suggestive of nanometric structural variations over length scales much finer than the spatial resolution attainable using the all-optical technique described herein. C1 [El-Khoury, Patrick Z.; Joly, Alan G.; Hess, Wayne P.] Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. [El-Khoury, Patrick Z.] Pacific NW Natl Lab, 902 Batelle Blvd,POB 999,MSIN K8-88, Richland, WA 99352 USA. RP El-Khoury, PZ; Hess, WP (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA.; El-Khoury, PZ (reprint author), Pacific NW Natl Lab, 902 Batelle Blvd,POB 999,MSIN K8-88, Richland, WA 99352 USA. EM patrick.elkhoury@pnnl.gov; wayne.hess@pnnl.gov FU Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL); U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; DOE's Office of Biological and Environmental Research; United States Department of Energy under DOE [DE-AC05-76RL1830] FX P.Z.E. acknowledges partial support from the Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL). The authors acknowledge support from the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. This work was performed in EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle Memorial Institute for the United States Department of Energy under DOE contract number DE-AC05-76RL1830. NR 13 TC 1 Z9 1 U1 10 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7295 EP 7298 DI 10.1021/acs.jpcc.6b02401 PG 4 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700042 ER PT J AU Pham, TA Mortuza, SMG Wood, BC Lau, EY Ogitsu, T Buchsbaum, SF Siwy, ZS Fornasiero, F Schwegler, E AF Tuan Anh Pham Mortuza, S. M. Golam Wood, Brandon C. Lau, Edmond Y. Ogitsu, Tadashi Buchsbaum, Steven F. Siwy, Zuzanna S. Fornasiero, Francesco Schwegler, Eric TI Salt Solutions in Carbon Nanotubes: The Role of Cation-pi Interactions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; 1ST PRINCIPLES SIMULATIONS; DENSITY-FUNCTIONAL THEORY; AQUEOUS NACL SOLUTIONS; ELECTROCHEMICAL CAPACITORS; ELECTROLYTIC TRANSPORT; WATER DESALINATION; ION SELECTIVITY; K+; SOLVATION AB Understanding the structure of aqueous electrolytes at interfaces is essential for predicting and optimizing device performance for a wide variety of emerging energy and environmental technologies. In this work, we investigate the structure of two common salt solutions, NaCl and KCl, at a hydrophobic interface within narrow carbon nanotubes (CNTs). Using a combination of first-principles and classical molecular dynamics simulations in conjunction with molecular orbital analysis, we find that the solvation structure of the cations in the CNTs can deviate substantially from the conventional weakly interacting hydrophobic picture. Instead, interactions between solvated ions and pi orbitals of the CNTs are found to play a critically important role. Specifically, the ion solvation structure is ultimately determined by a complex interplay between cation-pi interactions and the intrinsic flexibility of the solvation shell. In the case of K+, these effects result in an unusually strong propensity to partially desolvate and reside closer to the carbon wall than both Na+ and Cl-, in sharp contrast with the known ion ordering at the water-vapor interface. C1 [Tuan Anh Pham; Wood, Brandon C.; Lau, Edmond Y.; Ogitsu, Tadashi; Fornasiero, Francesco; Schwegler, Eric] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Mortuza, S. M. Golam] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Buchsbaum, Steven F.; Siwy, Zuzanna S.] Univ Calif Irvine, Dept Phys & Astron, 4129H Frederick Reines Hall Irvine, Irvine, CA 92697 USA. RP Pham, TA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM pham16@llnl.gov RI Mortuza, S.M./K-1286-2012 OI Mortuza, S.M./0000-0003-3432-1497 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [13-ERD-030]; Lawrence Fellowship; UC Lab Fees Research Program (UCOP Grant) [236772] FX Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and funded by the Laboratory Directed Research and Development Program at LLNL under project tracking code 13-ERD-030. T.A.P. acknowledges support from the Lawrence Fellowship; F.F., S.B. and Z.S.S. acknowledge support from the UC Lab Fees Research Program (UCOP Grant ID # 236772). Computational support was from the LLNL Grand Challenge Program. NR 67 TC 5 Z9 5 U1 9 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD APR 7 PY 2016 VL 120 IS 13 BP 7332 EP 7338 DI 10.1021/acs.jpcc.5b12245 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DJ0AB UT WOS:000373862700046 ER PT J AU Kucheryavy, P Lahanas, N Velasco, E Sun, CJ Lockard, JV AF Kucheryavy, Pavel Lahanas, Nicole Velasco, Ever Sun, Cheng-Jun Lockard, Jenny V. TI Probing Framework-Restricted Metal Axial Ligation and Spin State Patterns in a Post-Synthetically Reduced Iron-Porphyrin-Based Metal-Organic Framework SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID X-RAY-ABSORPTION; BASKET-HANDLE PORPHYRINS; EMISSION-SPECTROSCOPY; ELECTRONIC-STRUCTURE; SENSITIVE BANDS; RESONANCE RAMAN; LOWER MANTLE; COMPLEXES; SPECTRA; TRANSITIONS AB An iron-porphyrin-based metal organic framework PCN-222(Fe) is investigated upon postsynthetic reduction with piperidine. Fe K-edge X-ray absorption and K beta mainline emission spectroscopy measurements reveal the local coordination geometry, oxidation, and spin state changes experienced by the Fe sites upon reaction with this axially coordinating reducing agent. Analysis and fitting of these data confirm the binding pattern predicted by a space-filling model of the structurally constrained pore environments. These results are further supported by UV vis diffuse reflectance, IR, and resonance Raman spectroscopy data. C1 [Kucheryavy, Pavel; Lahanas, Nicole; Velasco, Ever; Lockard, Jenny V.] Rutgers State Univ, Dept Chem, Newark, NJ 07102 USA. [Sun, Cheng-Jun] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Lockard, JV (reprint author), Rutgers State Univ, Dept Chem, Newark, NJ 07102 USA. EM jlockard@rutgers.edu FU U.S. DOE [DE-AC02-06CH11357]; DOE - Basic Energy Sciences; Canadian Light Source; University of Washington; APS; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE [DE-SC0012704]; U.S. Department of Energy [DE-SC0012335]; National Science Foundation [DMR-1455127] FX Use of the Advanced Photon Source (APS), an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Sector 20 facilities at the APS, and research at these facilities, are supported by the DOE - Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the APS. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. We thank Dr. Nebojsa Marinkovic for beamline support at SSRL. Use of SSRL Beam Line 2-2 is coordinated with the National Synchrotron Light Source II, Brookhaven National Laboratory, under DOE Contract No. DE-SC0012704. The beamline 2-2 equipment is supported by the U.S. Department of Energy Grant No. DE-SC0012335. We thank Prof. Frieder Jalde for use of his glovebox for sample preparation, Prof. Elena Galoppini for use of her FT-IR instrument, and Dr. Ilya Stavitski for help with prior XES experiments carried out at APS. J.V.L. would like to acknowledge support by the National Science Foundation under Grant No. DMR-1455127. NR 46 TC 3 Z9 3 U1 18 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD APR 7 PY 2016 VL 7 IS 7 BP 1109 EP 1115 DI 10.1021/acs.jpclett.6b00302 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ0BY UT WOS:000373867600004 PM 26950260 ER PT J AU von Rudorff, GF Jakobsen, R Rosso, KM Blumberger, J AF von Rudorff, Guido Falk Jakobsen, Rasmus Rosso, Kevin M. Blumberger, Jochen TI Fast Interconversion of Hydrogen Bonding at the Hematite (001)-Liquid Water Interface SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID DOPED HEMATITE; MOLECULAR-DYNAMICS; ELECTRON-TRANSFER; LIQUID WATER; SIMULATION; SURFACE; PHOTOELECTRODES; ADSORPTION; REACTIVITY; TRANSPORT AB The interface between transition-metal oxides and aqueous solutions plays an important role in biogeochemistry and photoelectrochemistry, but the atomistic structure is often elusive. Here we report on the surface geometry, solvation structure, and thermal fluctuations of the hydrogen bonding network at the hematite (001)-water interface as obtained from hybrid density functional theory-based molecular dynamics. We find that the protons terminating the surface form binary patterns by either pointing in-plane or out-of-plane. The patterns exist for about 1 ps and spontaneously interconvert in an ultrafast, solvent-driven process within 50 fs. This results in only about half of the terminating protons pointing toward the solvent and being acidic. The lifetimes of all hydrogen bonds formed at the interface are shorter than those in pure liquid water. The solvation structure reported herein forms the basis for a better fundamental understanding of electron transfer coupled to proton transfer reactions at this important interface. C1 [von Rudorff, Guido Falk; Jakobsen, Rasmus; Blumberger, Jochen] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Rosso, Kevin M.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Blumberger, J (reprint author), UCL, Dept Phys & Astron, London WC1E 6BT, England.; Rosso, KM (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Kevin.Rosso@pnnl.gov; j.blumberger@ucl.ac.uk FU University College London; Pacific Northwest National Laboratory (PNNL) through its BES Geosciences program - U.S. Department of Energy's Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division; EPSRC [EP/L000202] FX G.F.v.R. gratefully acknowledges a Ph.D. studentship cosponsored by University College London and Pacific Northwest National Laboratory (PNNL) through its BES Geosciences program supported by the U.S. Department of Energy's Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division. MD simulations were carried out on ARCHER, the U.K. national HPC facility (Edinburgh), to which access was granted via the ARCHER Leadership pilot call and the Materials Chemistry Consortium (EPSRC Grant EP/L000202). NR 45 TC 5 Z9 5 U1 10 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD APR 7 PY 2016 VL 7 IS 7 BP 1155 EP 1160 DI 10.1021/acs.jpclett.6b00165 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ0BY UT WOS:000373867600012 PM 26954334 ER PT J AU Lee, J Sorescu, DC Deng, XY AF Lee, Junseok Sorescu, Dan C. Deng, Xingyi TI Tunable Lattice Constant and Band Gap of Single- and Few-Layer ZnO SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID DER-WAALS HETEROSTRUCTURES; ZINC-OXIDE LAYERS; ELECTRONIC-STRUCTURE; TUNNELING SPECTROSCOPY; BILAYER ZNO; AU(111); METAL; FILMS; NANOSTRUCTURES; NANOSHEETS AB Single and few-layer ZnO(0001) (ZnO(nL), n = 1-4) grown on Au(111) have been characterized via scanning tunneling microscopy (STM), scanning tunneling spectroscopy (STS), and density functional theory (DFT) calculations. We find that the in-plane lattice constants of the ZnO(nL, n <= 3) are expanded compared to that of the bulk wurtzite ZnO(0001). The lattice constant reaches a maximum expansion of 3% in the ZnO(2L) and decreases to the bulk wurtzite ZnO value in the ZnO(4L). The band gap decreases monotonically with increasing number of ZnO layers from 4.48 eV (ZnO(nL)) to 3.42 eV (ZnO(4L)). These results suggest that a transition from a planar to the bulk-like ZnO structure occurs around the thickness of ZnO(4L). The work also demonstrates that the lattice constant and the band gap in ultrathin ZnO can be tuned by controlling the number of layers, providing a basis for further investigation of this material. C1 [Lee, Junseok; Sorescu, Dan C.; Deng, Xingyi] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Lee, Junseok; Deng, Xingyi] AECOM, POB 618,South Pk, Philadelphia, PA 15129 USA. RP Lee, J (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA.; Lee, J (reprint author), AECOM, POB 618,South Pk, Philadelphia, PA 15129 USA. EM junseok.lee@netl.doe.gov OI Deng, Xingyi/0000-0001-9109-1443 FU National Energy Technology Laboratory's under the RES [DE-FE0004000]; agency of the United States Government FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES Contract DE-FE0004000. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 45 TC 12 Z9 12 U1 12 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD APR 7 PY 2016 VL 7 IS 7 BP 1335 EP 1340 DI 10.1021/acs.jpclett.6b00432 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ0BY UT WOS:000373867600039 PM 27003692 ER PT J AU Fischer, SA Cramer, CJ Govind, N AF Fischer, Sean A. Cramer, Christopher J. Govind, Niranjan TI Excited-State Absorption from Real-Time Time-Dependent Density Functional Theory: Optical Limiting in Zinc Phthalocyanine SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID EXCITATION-ENERGIES; MOLECULES; EXCHANGE; THERMOCHEMISTRY; FULLERENES; PORPHYRINS; DYNAMICS AB Optical-limiting materials are capable of attenuating light to protect delicate equipment from high-intensity light sources. Phthalocyanines have attracted a lot of attention for optical-limiting applications due to their versatility and large nonlinear absorption. With excited-state absorption (ESA) being the primary mechanism for optical limiting behavior in phthalocyanines, the ability to tune the optical absorption of ground and excited states in phthalocyanines would allow for the development of advanced optical limiters. We recently developed a method for the calculation of ESA based on real-time time-dependent density functional theory propagation of an excited-state density. In this work, we apply the approach to zinc phthalocyanine, demonstrating the ability of our method to efficiently identify the optical limiting potential of a molecular complex. C1 [Fischer, Sean A.; Govind, Niranjan] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. [Cramer, Christopher J.] Univ Minnesota, Dept Chem, Supercomp Inst, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Cramer, Christopher J.] Univ Minnesota, Chem Theory Ctr, Minneapolis, MN 55455 USA. RP Govind, N (reprint author), Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM niri.govind@pnnl.gov RI Cramer, Christopher/B-6179-2011 OI Cramer, Christopher/0000-0001-5048-1859 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; Office of Advanced Scientific Computing Research [KC-030106062653, DE-SC0008666]; Office of Biological and Environmental Research; DOE [DE-AC05-76RL1830]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and the Office of Advanced Scientific Computing Research through the Scientific Discovery through Advanced Computing (SciDAC) program under Award Numbers KC-030106062653 (S.A.F., N.G.) and DE-SC0008666 (C.J.C.). The research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle Memorial Institute for the United States Department of Energy under DOE contract number DE-AC05-76RL1830. The research also benefited from resources provided by the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No.DE-AC02-05CH11231, and resources provided by PNNL Institutional Computing (PIC). NR 28 TC 1 Z9 1 U1 5 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD APR 7 PY 2016 VL 7 IS 7 BP 1387 EP 1391 DI 10.1021/acs.jpclett.6b00282 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DJ0BY UT WOS:000373867600047 PM 27007445 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G 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Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sinthuprasith, T. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Measurement of the top quark mass using proton-proton data at root(s)=7 SO PHYSICAL REVIEW D LA English DT Article ID STANDARD MODEL; LHC; TEVATRON; PHYSICS; DECAY; BOSON AB A new set of measurements of the top quark mass are presented, based on the proton-proton data recorded by the CMS experiment at the LHC at root s = 8 TeV corresponding to a luminosity of 19.7 fb(-1). The top quark mass is measured using the lepton + jets, all-jets and dilepton decay channels, giving values of 172.35 +/- 0.16(stat) +/- 0.48(syst) GeV, 172.32 +/- 0.25(stat) +/- 0.59(syst) GeV, and 172.82 +/- 0.19(stat) +/- 1.22(syst) GeV, respectively. When combined with the published CMS results at s = 7 TeV, they provide a top quark mass measurement of 172.44 +/- 0.13(stat) +/- 0.47(syst) GeV. The top quark mass is also studied as a function of the event kinematical properties in the lepton + jets decay channel. No indications of a kinematic bias are observed and the collision data are consistent with a range of predictions from current theoretical models of t (t) over bar production. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Wohrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.; Abdulsalam, A.; Ackert, A.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.; Abdulsalam, A.; Ackert, A.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.; Abdulsalam, A.; Adiguzel, A.; Ackert, A.; Adair, A.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Kothekar, K.; Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fan, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fan, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonbuk Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Nucl Res Inst, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Matveev, V.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Klyukhin, V.; Kodolova, O.; Korneeva, N.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Belyaev, A.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambient & Technol CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.; Cuevas, J.] Univ Autonoma Madrid, Madrid, Spain. [Fernandez Menendez, J.; Folgueras, S.; Caballero, I. Gonzalez; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Viliani, L.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. f.; Tzeng, Y. M.; Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Ctr Nat Sci, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Nally, R.; Narain, M.; Piperov, S.; Sagir, S.; Speer, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, San Diego, CA 92103 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.; Cumalat, J. P.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, H.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Parashar, N.] Purdue Univ, W Lafayette, IN 47907 USA. [Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.; Herve, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.; Abdulsalam, A.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [El-khateeb, E.; Elkafrawy, T.; Salama, E.] Ain Shams Univ, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Mohammed, Y.] Fayoum Univ, Al Fayyum, Egypt. [Salama, E.] British Univ Egypt, Cairo, Egypt. [Agram, J. -L.; Coubez, X.] Univ Haute Alsace, Mulhouse, France. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Banerjee, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Gulmini, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Invest Cient & Tecn, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Tinoco Mendes, Andre David/D-4314-2011; Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Montanari, Alessandro/J-2420-2012; Azarkin, Maxim/N-2578-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Novaes, Sergio/D-3532-2012; Dubinin, Mikhail/I-3942-2016; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Raidal, Martti/F-4436-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015 OI Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Tinoco Mendes, Andre David/0000-0001-5854-7699; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Dubinin, Mikhail/0000-0002-7766-7175; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Agency CNPq; Brazilian Agency CAPES; Brazilian Agency FAPERJ; Brazilian Agency FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland, France; Finnish Ministry of Education and Culture, France; Helsinki Institute of Physics, France; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; Ministry of Education and Research, Estonia; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); Mexican Funding Agency CINVESTAV; Mexican Funding Agency CONACYT; Mexican Funding Agency SEP; Mexican Funding Agency UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education and the National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Spain; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency ETH Board; Swiss Funding Agency ETH Zurich; Swiss Funding Agency PSI; Swiss Funding Agency SNF; Swiss Funding Agency UniZH; Swiss Funding Agency Canton Zurich; Swiss Funding Agency SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; U.S. Department of Energy; U.S. National Science Foundation; Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industire et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie doorWetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; Qatar National Research Fund; Rachadapisek SomWetenschappelijk Onderzopot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industire et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie doorWetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek SomWetenschappelijk Onderzopot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, Contract No. C-1845. NR 62 TC 3 Z9 3 U1 14 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 7 PY 2016 VL 93 IS 7 AR 072004 DI 10.1103/PhysRevD.93.072004 PG 37 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5ZL UT WOS:000373578900001 ER PT J AU Renslow, RS Lindemann, SR Song, HS AF Renslow, Ryan S. Lindemann, Stephen R. Song, Hyun-Seob TI A Generalized Spatial Measure for Resilience of Microbial Systems SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE resilience; microbial communities; recovery; ecology; emergent properties ID EXTRACELLULAR POLYMERIC SUBSTANCES; IN-SITU HYBRIDIZATION; COMMUNITY STRUCTURE; CLIMATE-CHANGE; CRITICAL TRANSITIONS; CORAL-REEFS; BIOFILMS; RESPONSES; RECOVERY; ECOLOGY AB The emergent property of resilience is the ability of a system to return to an original state after a disturbance. Resilience may be used as an early warning system for significant or irreversible community transition; that is, a community with diminishing or low resilience may be close to catastrophic shift in function or an irreversible collapse. Typically, resilience is quantified using recovery time, which may be difficult or impossible to directly measure in microbial systems. A recent study in the literature showed that under certain conditions, a set of spatial-based metrics termed recovery length, can be correlated to recovery time, and thus may be a reasonable alternative measure of resilience. However, this spatial metric of resilience is limited to use for step-change perturbations. Building upon the concept of recovery length, we propose a more general form of the spatial metric of resilience that can be applied to any shape of perturbation profiles (for example, either sharp or smooth gradients). We termed this new spatial measure "perturbation-adjusted spatial metric of resilience" (PASMORE). We demonstrate the applicability of the proposed metric using a mathematical model of a microbial mat. C1 [Renslow, Ryan S.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Lindemann, Stephen R.; Song, Hyun-Seob] Pacific NW Natl Lab, Div Biol Sci, Earth & Biol Sci Directorate, Richland, WA 99352 USA. RP Song, HS (reprint author), Pacific NW Natl Lab, Div Biol Sci, Earth & Biol Sci Directorate, Richland, WA 99352 USA. EM hyunseob.song@pnnl.gov RI Lindemann, Steve/H-6088-2016 OI Lindemann, Steve/0000-0002-3788-5389 FU Genomic Science Program (GSP), Office of Biological and Environmental Research (OBER), U.S. Department of Energy (DOE); Linus Pauling Distinguished Postdoctoral Fellowship at PNNL FX This research was supported by the Genomic Science Program (GSP), Office of Biological and Environmental Research (OBER), U.S. Department of Energy (DOE), and is a contribution of the Pacific Northwest National Laboratory (PNNL) Foundational Scientific Focus Area (SFA) and Subsurface Biogeochemistry Research Program's SFA. R. Renslow was supported by a Linus Pauling Distinguished Postdoctoral Fellowship at PNNL. NR 74 TC 0 Z9 0 U1 5 U2 23 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 7 PY 2016 VL 7 AR 443 DI 10.3389/fmicb.2016.00443 PG 9 WC Microbiology SC Microbiology GA DI6EP UT WOS:000373592300001 PM 27092116 ER PT J AU Imafuku, Y Abe, M Schmidt, MW Hada, M AF Imafuku, Yuji Abe, Minori Schmidt, Michael W. Hada, Masahiko TI Heavy Element Effects in the Diagonal Born-Oppenheimer Correction within a Relativistic Spin-Free Hamiltonian SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID COUPLING MATRIX-ELEMENTS; ANO BASIS-SETS; ADIABATIC CORRECTION; WAVE-FUNCTIONS; HYDROGEN MOLECULE; GROUND-STATE; AB-INITIO; 2ND-DERIVATIVE TERMS; ELECTRON CORRELATION; DOUGLAS-KROLL AB Methodologies beyond the Born-Oppenheimer (BO) approximation are nowadays important to explain high precision spectroscopic measurements. Most previous evaluations of the BO correction are, however, focused on light-element molecules and based on a nonrelativistic Hamiltonian, so no information about the BO approximation (BOA) breakdown in heavy-element molecules is available. The present work is the first to investigate the BOA breakdown for the entire periodic table, by considering scalar relativistic effects in the Diagonal BO correction (DBOC). In closed shell atoms, the relativistic E-DBOC scales as Z(1.25) and the nonrelativistic E-DBOC scales as Z(1.17), where Z is the atomic number. Hence, we found that E-DBOC becomes larger in heavy element atoms and molecules, and the relativistic E-DBOC increases faster than nonrelativistic E-DBOC. We have further investigated the DBOC effects on properties such as potential energy curves, spectroscopic parameters, and various energetic properties. The DBOC effects for these properties are mostly affected by the lightest atom in the molecule. Hence, in X-2 or XAt molecule (X = H, Li, Na, K, Rb, and Cs) the effect of DBOC systematically decreases when X becomes heavier but in HX molecules, the effect of DBOC seems relatively similar among all the molecules. C1 [Imafuku, Yuji; Abe, Minori; Hada, Masahiko] Tokyo Metropolitan Univ, Grad Sch Sci, Dept Chem, Tokyo 1920397, Japan. [Schmidt, Michael W.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Schmidt, Michael W.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Abe, M (reprint author), Tokyo Metropolitan Univ, Grad Sch Sci, Dept Chem, Tokyo 1920397, Japan. EM minoria@tmu.ac.jp FU JST, CREST; JSPS KAKENHI Grant [25810007]; US Department of Energy, Basic Energy Sciences, Geosciences, and Biosciences to the Ames Laboratory; Iowa State University [DE-AC01-07CH11358] FX This research was supported by JST, CREST, and JSPS KAKENHI Grant Number 25810007. M.W.S. was supported by funds provided by the US Department of Energy, Basic Energy Sciences, Geosciences, and Biosciences to the Ames Laboratory, administered by Iowa State University, under Contract DE-AC01-07CH11358. NR 53 TC 0 Z9 0 U1 2 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD APR 7 PY 2016 VL 120 IS 13 BP 2150 EP 2159 DI 10.1021/acs.jpca.6b01507 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DJ0AC UT WOS:000373862800011 PM 27003510 ER PT J AU Ding, QP Wiecki, P Anand, VK Sangeetha, NS Lee, Y Johnston, DC Furukawa, Y AF Ding, Q. -P. Wiecki, P. Anand, V. K. Sangeetha, N. S. Lee, Y. Johnston, D. C. Furukawa, Y. TI Volovik effect and Fermi-liquid behavior in the s-wave superconductor CaPd2As2: As-75 NMR-NQR measurements SO PHYSICAL REVIEW B LA English DT Article ID SPIN-LATTICE RELAXATION; MIXED-STATE; METALS; VORTEX AB The electronic and magnetic properties of the collapsed-tetragonal CaPd2As2 superconductor (SC) with a transition temperature of 1.27 K have been investigated by As-75 nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements. The temperature (T) dependence of the nuclear spin lattice relaxation rates (1/T-1) and the Knight shifts indicate the absence of magnetic correlations in the normal state. In the SC state, 1/T-1 measured by As-75 NQR shows a clear Hebel-Slichter (HS) peak just below T-c and decreases exponentially at lower T, confirming a conventional s-wave SC. In addition, the Volovik effect, also known as the Doppler shift effect, has been clearly evidenced by the observation of the suppression of the HS peak with applied magnetic field. C1 [Ding, Q. -P.; Wiecki, P.; Anand, V. K.; Sangeetha, N. S.; Lee, Y.; Johnston, D. C.; Furukawa, Y.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Ding, Q. -P.; Wiecki, P.; Anand, V. K.; Sangeetha, N. S.; Lee, Y.; Johnston, D. C.; Furukawa, Y.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Anand, V. K.] Helmholtz Zentrum Berlin Mat & Energie, Hahn Meitner Pl 1, D-14109 Berlin, Germany. RP Ding, QP (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA.; Ding, QP (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RI Ding, Qingping/F-2381-2011; Anand, Vivek Kumar/J-3381-2013 OI Anand, Vivek Kumar/0000-0003-2023-7040 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We thank Masanori Ichioka for helpful discussions. The research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 50 TC 1 Z9 1 U1 13 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 7 PY 2016 VL 93 IS 14 AR 140502 DI 10.1103/PhysRevB.93.140502 PG 5 WC Physics, Condensed Matter SC Physics GA DI5VK UT WOS:000373568400001 ER PT J AU Mickel, PR Jeen, H Kumar, P Biswas, A Hebard, AF AF Mickel, Patrick R. Jeen, Hyoungjeen Kumar, Pradeep Biswas, Amlan Hebard, Arthur F. TI Proximate transition temperatures amplify linear magnetoelectric coupling in strain-disordered multiferroic BiMnO3 SO PHYSICAL REVIEW B LA English DT Article ID THIN-FILMS; WEAK FERROMAGNETISM; PHASE-TRANSITION; FERROELECTRICITY; SUSCEPTIBILITY; PEROVSKITE; BEHAVIOR AB We report a giant linear magnetoelectric coupling in strained BiMnO3 thin films in which the disorder associated with an islanded morphology gives rise to extrinsic relaxor ferroelectricity that is not present in bulk centrosymmetric ferromagnetic crystalline BiMnO3. Strain associated with the disorder is treated as a local variable, which couples to the two ferroic order parameters, magnetization (M) over right arrow and polarization (P) over right arrow. A straightforward "gas under a piston" thermodynamic treatment explains the observed correlated temperature dependencies of the product of susceptibilities and the magnetoelectric coefficient together with the enhancement of the coupling by the proximity of the ferroic transition temperatures close to the relaxor freezing temperature. Our interpretation is based on a trilinear coupling term in the free energy of the form (L) over right arrow . ((P) over right arrow x (M) over right arrow), where (L) over right arrow is a hidden antiferromagnetic order parameter, previously postulated by theory for BiMnO3. This phenomenological invariant not only preserves inversion and time-reversal symmetry of the strain-induced interactions but also explains the pronounced linear magnetoelectric coupling without using the more conventional higher order biquadratic interaction proportional to ((P) over right arrow . (M) over right arrow)(2). C1 [Mickel, Patrick R.; Jeen, Hyoungjeen; Kumar, Pradeep; Biswas, Amlan; Hebard, Arthur F.] Univ Florida, Gainesville, FL 32611 USA. [Mickel, Patrick R.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Jeen, Hyoungjeen] Pusan Natl Univ, Dept Phys, Busan 609735, South Korea. RP Hebard, AF (reprint author), Univ Florida, Gainesville, FL 32611 USA. EM afh@phys.ufl.edu FU US National Science Foundation [DMR-1305783, DMR-1410237] FX The authors thank Sanal Buvaev for assistance with sample preparation and measurements and D. Maslov and M. Mostovoy for useful discussions on points of theory. This work was supported by the US National Science Foundation under Grant Nos. DMR-1305783 (AFH) and DMR-1410237 (AB). NR 45 TC 0 Z9 0 U1 14 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 7 PY 2016 VL 93 IS 13 AR 134205 DI 10.1103/PhysRevB.93.134205 PG 9 WC Physics, Condensed Matter SC Physics GA DI5UO UT WOS:000373566200001 ER PT J AU Mou, DX Manni, S Taufour, V Wu, Y Huang, LN Bud'ko, SL Canfield, PC Kaminski, A AF Mou, Daixiang Manni, Soham Taufour, Valentin Wu, Yun Huang, Lunan Bud'ko, S. L. Canfield, P. C. Kaminski, Adam TI Isotope effect on electron-phonon interaction in the multiband superconductor MgB2 SO PHYSICAL REVIEW B LA English DT Article ID CUPRATE SUPERCONDUCTORS; TEMPERATURE; SPECTRA; ORIGIN; BORON AB We investigate the effect of isotope substitution on the electron-phonon interaction in the multiband superconductor MgB2 using tunable laser-based angle-resolved photoemission spectroscopy. The kink structure around 70 meV in the sigma band, which is caused by electron coupling to the E-2g phonon mode, is shifted to higher binding energy by similar to 3.5 meV in (MgB2)-B-10 and the shift is not affected by superconducting transition. These results serve as the benchmark for investigations of isotope effects in known, unconventional superconductors and newly discovered superconductors where the origin of pairing is unknown. C1 [Mou, Daixiang] Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Mou, DX (reprint author), Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. RI Manni, Soham/G-1455-2016 OI Manni, Soham/0000-0001-6279-3497 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX We thank Igor Mazin for very useful comments. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 36 TC 0 Z9 0 U1 7 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 7 PY 2016 VL 93 IS 14 AR 144504 DI 10.1103/PhysRevB.93.144504 PG 5 WC Physics, Condensed Matter SC Physics GA DI5VK UT WOS:000373568400005 ER PT J AU Runge, B Festersen, S Koops, CT Elsen, A Deutsch, M Ocko, BM Seeck, OH Murphy, BM Magnussen, OM AF Runge, Benjamin Festersen, Sven Koops, Christian T. Elsen, Annika Deutsch, Moshe Ocko, Benjamin M. Seeck, Oliver H. Murphy, Bridget M. Magnussen, Olaf M. TI Temperature- and potential-dependent structure of the mercury-electrolyte interface SO PHYSICAL REVIEW B LA English DT Article ID LIQUID-VAPOR INTERFACE; X-RAY REFLECTIVITY; COMPUTER-SIMULATION; CAPILLARY WAVES; SURFACE; ALLOY; METAL; DIFFRACTOMETER; RESOLUTION; GALLIUM AB The atomic-scale structure of the mercury-electrolyte (0.01 M NaF) interface was studied as a function of temperature and potential by x-ray reflectivity and x-ray diffuse scattering measurements. The capillary wave contribution is determined and removed from the data, giving access to the intrinsic surface-normal electron density profile at the interface, especially to the surface layering in the Hg phase. A temperature dependent roughness anomaly known from the Hg-air interface is found to persist also at the Hg-electrolyte interface. Additionally, a temperature dependence of the layering period was discovered. The increase in the layer spacing with increasing temperature is approximately four times lager than the increase expected from thermal expansion. Finally, the interface is found to broaden towards the electrolyte side as the potential becomes more negative, in agreement with the Schmickler-Henderson theory. Our results favor a model for the interface structure, which is different to the model formerly used in comparable studies. C1 [Runge, Benjamin; Festersen, Sven; Koops, Christian T.; Elsen, Annika; Murphy, Bridget M.; Magnussen, Olaf M.] CAU, Inst Expt & Appl Phys, Kiel, Germany. [Deutsch, Moshe] Bar Ilan Univ, Dept Phys, Ramat Gan, Israel. [Deutsch, Moshe] Bar Ilan Univ, Inst Nanotechnol & Adv Mat, Ramat Gan, Israel. [Ocko, Benjamin M.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, New York, NY USA. [Seeck, Oliver H.] Deutsches Elektronen Synchrotron DESY, Hamburg, Germany. [Murphy, Bridget M.; Magnussen, Olaf M.] CAU, Ruprecht Haensel Lab, Kiel, Germany. RP Murphy, BM (reprint author), CAU, Inst Expt & Appl Phys, Kiel, Germany.; Murphy, BM (reprint author), CAU, Ruprecht Haensel Lab, Kiel, Germany. EM murphy@physik.uni-kiel.de FU Bundesministerium fur Bildung und Forschung, Germany [05K10FK2, 05KS7FK3]; U.S. Department of Energy, Division of Materials Science [DE-SC0012704]; United States - Israel Binational Science Foundation, Jerusalem (M.D.) FX We gratefully acknowledge financial support by the Bundesministerium fur Bildung und Forschung, Germany (Projects 05K10FK2 and 05KS7FK3), the U.S. Department of Energy, Division of Materials Science under Contract No. DE-SC0012704 (B.O.) and the United States - Israel Binational Science Foundation, Jerusalem (M.D.), and thank the beamline staff of P08 at PETRA III, Deutsches Elektronen-Synchrotron, Germany for their experimental support. NR 46 TC 1 Z9 1 U1 6 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 7 PY 2016 VL 93 IS 16 AR 165408 DI 10.1103/PhysRevB.93.165408 PG 9 WC Physics, Condensed Matter SC Physics GA DI5WW UT WOS:000373572200005 ER PT J AU Miller, GA Sievert, MD Venugopalan, R AF Miller, Gerald A. Sievert, Matthew D. Venugopalan, Raju TI Probing short-range nucleon-nucleon interactions with an electron-ion collider SO PHYSICAL REVIEW C LA English DT Article ID ANGLE ELASTIC-SCATTERING; QUANTUM CHROMODYNAMICS; COLOR TRANSPARENCY; FORM-FACTOR; EXCLUSIVE PHOTOPRODUCTION; ASYMPTOTIC-BEHAVIOR; INFINITE-MOMENTUM; VECTOR-MESONS; QCD; ELECTROPRODUCTION AB We derive the cross section for exclusive vector meson production in high-energy deeply inelastic scattering off a deuteron target that disintegrates into a proton and a neutron carrying large relative momentum in the final state. This cross section can be expressed in terms of a novel gluon transition generalized parton distribution (T-GPD); the hard scale in the final state makes the T-GPD sensitive to the short-distance nucleon-nucleon interaction. We perform a toy model computation of this process in a perturbative framework and discuss the time scales that allow the separation of initial-and final-state dynamics in the T-GPD. We outline the more general computation based on the factorization suggested by the toy computation: In particular, we discuss the relative role of "pointlike" and "geometric" Fock configurations that control the parton dynamics of short-range nucleon-nucleon scattering. With the aid of exclusive J/psi production data at the Hadron-Electron Ring Accelerator at DESY, as well as elastic nucleon-nucleon cross sections, we estimate rates for exclusive deuteron photodisintegration at a future Electron-Ion Collider (EIC). Our results, obtained using conservative estimates of EIC integrated luminosities, suggest that center-of-mass energies s(NN) similar to 12 GeV2 of the neutron-proton subsystem can be accessed. We argue that the high energies of the EIC can address outstanding dynamical questions regarding the short-range quark-gluon structure of nuclear forces by providing clean gluon probes of such "knockout" exclusive reactions in light and heavy nuclei. C1 [Miller, Gerald A.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Sievert, Matthew D.; Venugopalan, Raju] Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. [Venugopalan, Raju] Heidelberg Univ, Inst Theoret Phys, Philosophenweg 16, D-69120 Heidelberg, Germany. RP Miller, GA (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA.; Sievert, MD; Venugopalan, R (reprint author), Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA.; Venugopalan, R (reprint author), Heidelberg Univ, Inst Theoret Phys, Philosophenweg 16, D-69120 Heidelberg, Germany. EM miller@phys.washington.edu; msievert@bnl.gov; rajuv@bnl.gov OI Sievert, Matthew/0000-0002-6018-269X FU Department of Energy [DE-SC0012704]; US Department of Energy Office of Science, Office of Nuclear Physics [DE-FG02-97ER-41014]; BNL; Excellence Initiative of Heidelberg University FX R.V. would like to thank Misak Sargsian and Mark Strikman for a number of insightful discussions over several years that stirred his interest in this topic. We would also like to thank Elke Aschenauer, Stan Brodsky, Rolf Ent, Dima Kharzeev, Tetsuo Hatsuda, Or Hen, Larry McLerran, Berndt Mueller, Bernard Pire, Jianwei Qiu, Sanjay Reddy, and Thomas Roser for useful comments. M.S. and R.V. are supported under Department of Energy Contract No. DE-SC0012704; the work of GAM is partially supported by the US Department of Energy Office of Science, Office of Nuclear Physics under Award No. DE-FG02-97ER-41014. M.S. receives additional support from an EIC program development fund from BNL. R.V. would like to thank the Institut fur Theoretische Physik, Heidelberg for their kind hospitality and the Excellence Initiative of Heidelberg University for their support. NR 62 TC 1 Z9 1 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD APR 7 PY 2016 VL 93 IS 4 AR 045202 DI 10.1103/PhysRevC.93.045202 PG 24 WC Physics, Nuclear SC Physics GA DI5YG UT WOS:000373575800002 ER PT J AU Aab, A Abreu, P Aglietta, M Ahn, EJ Al Samarai, I Albuquerque, IFM Allekotte, I Allison, P Almela, A Castillo, JA Alvarez-Muniz, J Batista, RA Ambrosio, M Anchordoqui, L Andrada, B Andringa, S Aramo, C Arqueros, F Arsene, N Asorey, H Assis, P Aublin, J Avila, G Awal, N Badescu, AM Baus, C Beatty, JJ Becker, KH Bellido, JA Berat, C Bertaina, ME Bertou, X Biermann, PL Billoir, P Blaess, SG Blanco, A Blazek, J Bleve, C Blumer, H Bohacova, M Boncioli, D Bonifazi, C Borodai, N Botti, AM Brack, J Brancus, I Bretz, T Bridgeman, A Briechle, FL Buchholz, P Bueno, A Buitink, S Buscemi, M Caballero-Mora, KS Caccianiga, B Caccianiga, L Cancio, A Candusso, M Caramete, L Caruso, R Castellina, A Cataldi, G Cazon, L Cester, R Chavez, AG Chiavassa, A Chinellato, JA Diaz, JCC Chudoba, J Clay, RW Colalillo, R Coleman, A Collica, L Coluccia, MR Conceicao, R Contreras, F Cooper, MJ Coutu, S Covault, CE Cronin, J Dallier, R D'Amico, S Daniel, B Dasso, S Daumiller, K Dawson, BR de Almeida, RM de Jong, SJ De Mauro, G Neto, JRTD De Mitri, I de Oliveira, J de Souza, V Debatin, J Deligny, O Dhital, N Di Giulio, C Di Matteo, A Castro, MLD Diogo, F Dobrigkeit, C Docters, W D'Olivo, JC Dorofeev, A Dos Anjos, RC Dova, MT Dundovic, A Ebr, J Engel, R Erdmann, M Erfani, M Escobar, CO Espadanal, J Etchegoyen, A Falcke, H Fang, K Farrar, G Fauth, AC Fazzini, N Ferguson, AP Fick, B Figueira, JM Filevich, A Filipcic, A Fratu, O Freire, MM Fujii, T Fuster, A Gallo, F Garcia, B Garcia-Pinto, D Gate, F Gemmeke, H Gherghel-Lascu, A Ghia, PL Giaccari, U Giammarchi, M Giller, M Glas, D Glaser, C Glass, H Golup, G Berisso, MG Vitale, PFG Gonzalez, N Gookin, B Gordon, J Gorgi, A Gorham, P Gouffon, P Griffith, N Grillo, AF Grubb, TD Guarino, F Guedes, GP Hampel, MR Hansen, P Harari, D Harrison, TA Harton, JL Hasankiadeh, Q Haungs, A Hebbeker, T Heck, D Heimann, P Herve, AE Hill, GC Hojvat, C Hollon, N Holt, E Homola, P Horandel, JR Horvath, P Hrabovsky, M Huege, T Insolia, A Isar, PG Jandt, I Jansen, S Jarne, C Johnsen, JA Josebachuili, M Kaapa, A Kambeitz, O Kampert, KH Kasper, P Katkov, I Keilhauer, B Kemp, E Kieckhafer, RM Klages, HO Kleifges, M Kleinfeller, J Krause, R Krohm, N Kuempel, D Mezek, GK Kunka, N Awad, AK LaHurd, D Latronico, L Lauscher, M Lautridou, P Lebrun, P de Oliveira, MAL Letessier-Selvon, A Lhenry-Yvon, I Link, K Lopes, L Lopez, R Casado, AL Lucero, A Malacari, M Mallamaci, M Mandat, D Mantsch, P Mariazzi, AG Marin, V Maris, IC Marsella, G Martello, D Martinez, H Bravo, OM Meza, JJM Mathes, HJ Mathys, S Matthews, J Matthews, JAJ Matthiae, G Maurizio, D Mayotte, E Mazur, PO Medina, C Medina-Tanco, G Mello, VBB Melo, D Menshikov, A Messina, S Micheletti, MI Middendorf, L Minaya, IA Miramonti, L Mitrica, B Molina-Bueno, L Mollerach, S Montanet, F Morello, C Mostafa, M Moura, CA Muller, G Muller, MA Muller, S Naranjo, I Navas, S Necesal, P Nellen, L Nelles, A Neuser, J Nguyen, PH Niculescu-Oglinzanu, M Niechciol, M Niemietz, L Niggemann, T Nitz, D Nosek, D Novotny, V Nozka, H Nunez, LA Ochilo, L Oikonomou, F Olinto, A Selmi-Dei, DP Palatka, M Pallotta, J Papenbreer, P Parente, G Parra, A Paul, T Pech, M Pekala, J Pelayo, R Pena-Rodriguez, J Pepe, IM Pereira, LAS Perrone, L Petermann, E Peters, C Petrera, S Phuntsok, J Piegaia, R Pierog, T Pieroni, P Pimenta, M Pirronello, V Platino, M Plum, M Porowski, C Prado, RR Privitera, P Prouza, M Quel, EJ Querchfeld, S Quinn, S Rautenberg, J Ravel, O Ravignani, D Reinert, D Revenu, B Ridky, J Risse, M Ristori, P Rizi, V de Carvalho, WR Rojo, JR Rogozin, D Rosado, J Roth, M Roulet, E Rovero, AC Saffi, SJ Saftoiu, A Salazar, H Saleh, A Greus, FS Salina, G Gomez, JDS Sanchez, F Sanchez-Lucas, P Santos, EM Santos, E Sarazin, F Sarkar, B Sarmento, R Sarmiento-Cano, C Sato, R Scarso, C Schauer, M Scherini, V Schieler, H Schmidt, D Scholten, O Schoorlemmer, H Schovanek, P Schroder, FG Schulz, A Schulz, J Schumacher, J Sciutto, SJ Segreto, A Settimo, M Shadkam, A Shellard, C Sigl, G Sima, O Smialkowski, A Smida, R Snow, GR Sommers, P Sonntag, S Sorokin, J Squartini, R Stanca, D Stanic, S Stapleton, J Stasielak, J Strafella, F Stutz, A Suarez, F Duran, MS Sudholz, T Suomijarvi, T Supanitsky, AD Sutherland, MS Swain, J Szadkowski, Z Taborda, OA Tapia, A Tepe, A Theodoro, VM Timmermans, C Peixoto, CJT Tomankova, L Tome, B Tonachini, A Elipe, GT Machado, DT Travnicek, P Trini, M Ulrich, R Unger, M Urban, M Galicia, JFV Valino, I Valore, L van Aar, G van Bodegom, P van den Berg, AM van Vliet, A Varela, E Cardenas, BV Varner, G Vasquez, R Vazquez, JR Vazquez, RA Veberic, D Verzi, V Vicha, J Videla, M Villasenor, L Vorobiov, S Wahlberg, H Wainberg, O Walz, D Watson, AA Weber, M Weindl, A Wiencke, L Wilczynski, H Winchen, T Wittkowski, D Wundheiler, B Wykes, S Yang, L Yapici, T Yelos, D Yushkov, A Zas, E Zavrtanik, D Zavrtanik, M Zepeda, A Zimmermann, B Ziolkowski, M Zong, Z Zuccarello, F AF Aab, A. Abreu, P. Aglietta, M. Ahn, E. J. Al Samarai, I. Albuquerque, I. F. M. Allekotte, I. Allison, P. Almela, A. Alvarez Castillo, J. Alvarez-Muniz, J. Batista, R. Alves Ambrosio, M. Anchordoqui, L. Andrada, B. Andringa, S. Aramo, C. Arqueros, F. Arsene, N. Asorey, H. Assis, P. Aublin, J. Avila, G. Awal, N. Badescu, A. M. Baus, C. Beatty, J. J. Becker, K. H. Bellido, J. A. Berat, C. Bertaina, M. E. Bertou, X. Biermann, P. L. Billoir, P. Blaess, S. G. Blanco, A. Blazek, J. Bleve, C. Blumer, H. Bohacova, M. Boncioli, D. Bonifazi, C. Borodai, N. Botti, A. M. Brack, J. Brancus, I. Bretz, T. Bridgeman, A. Briechle, F. L. Buchholz, P. Bueno, A. Buitink, S. Buscemi, M. Caballero-Mora, K. S. Caccianiga, B. Caccianiga, L. Cancio, A. Candusso, M. Caramete, L. Caruso, R. Castellina, A. Cataldi, G. Cazon, L. Cester, R. Chavez, A. G. Chiavassa, A. Chinellato, J. A. Diaz, J. C. Chirinos Chudoba, J. Clay, R. W. Colalillo, R. Coleman, A. Collica, L. Coluccia, M. R. Conceicao, R. Contreras, F. Cooper, M. J. Coutu, S. Covault, C. E. Cronin, J. Dallier, R. D'Amico, S. Daniel, B. Dasso, S. Daumiller, K. Dawson, B. R. de Almeida, R. M. de Jong, S. J. De Mauro, G. Neto, J. R. T. de Mello De Mitri, I. de Oliveira, J. de Souza, V. Debatin, J. Deligny, O. Dhital, N. Di Giulio, C. Di Matteo, A. Castro, M. L. Diaz Diogo, F. Dobrigkeit, C. Docters, W. D'Olivo, J. C. Dorofeev, A. dos Anjos, R. C. Dova, M. T. Dundovic, A. Ebr, J. Engel, R. Erdmann, M. Erfani, M. Escobar, C. O. Espadanal, J. Etchegoyen, A. Falcke, H. Fang, K. Farrar, G. Fauth, A. C. Fazzini, N. Ferguson, A. P. Fick, B. Figueira, J. M. Filevich, A. Filipcic, A. Fratu, O. Freire, M. M. Fujii, T. Fuster, A. Gallo, F. Garcia, B. Garcia-Pinto, D. Gate, F. Gemmeke, H. Gherghel-Lascu, A. Ghia, P. L. Giaccari, U. Giammarchi, M. Giller, M. Glas, D. Glaser, C. Glass, H. Golup, G. Gomez Berisso, M. Gomez Vitale, P. F. Gonzalez, N. Gookin, B. Gordon, J. Gorgi, A. Gorham, P. Gouffon, P. Griffith, N. Grillo, A. F. Grubb, T. D. Guarino, F. Guedes, G. P. Hampel, M. R. Hansen, P. Harari, D. Harrison, T. A. Harton, J. L. Hasankiadeh, Q. Haungs, A. Hebbeker, T. Heck, D. Heimann, P. Herve, A. E. Hill, G. C. Hojvat, C. Hollon, N. Holt, E. Homola, P. Hoerandel, J. R. Horvath, P. Hrabovsky, M. Huege, T. Insolia, A. Isar, P. G. Jandt, I. Jansen, S. Jarne, C. Johnsen, J. A. Josebachuili, M. Kaeaepae, A. Kambeitz, O. Kampert, K. H. Kasper, P. Katkov, I. Keilhauer, B. Kemp, E. Kieckhafer, R. M. Klages, H. O. Kleifges, M. Kleinfeller, J. Krause, R. Krohm, N. Kuempel, D. Mezek, G. Kukec Kunka, N. Awad, A. Kuotb LaHurd, D. Latronico, L. Lauscher, M. Lautridou, P. Lebrun, P. de Oliveira, M. A. Leigui Letessier-Selvon, A. Lhenry-Yvon, I. Link, K. Lopes, L. Lopez, R. Casado, A. Lopez Lucero, A. Malacari, M. Mallamaci, M. Mandat, D. Mantsch, P. Mariazzi, A. G. Marin, V. Maris, I. C. Marsella, G. Martello, D. Martinez, H. Martinez Bravo, O. Masias Meza, J. J. Mathes, H. J. Mathys, S. Matthews, J. Matthews, J. A. J. Matthiae, G. Maurizio, D. Mayotte, E. Mazur, P. O. Medina, C. Medina-Tanco, G. Mello, V. B. B. Melo, D. Menshikov, A. Messina, S. Micheletti, M. I. Middendorf, L. Minaya, I. A. Miramonti, L. Mitrica, B. Molina-Bueno, L. Mollerach, S. Montanet, F. Morello, C. Mostafa, M. Moura, C. A. Mueller, G. Muller, M. A. Mueller, S. Naranjo, I. Navas, S. Necesal, P. Nellen, L. Nelles, A. Neuser, J. Nguyen, P. H. Niculescu-Oglinzanu, M. Niechciol, M. Niemietz, L. Niggemann, T. Nitz, D. Nosek, D. Novotny, V. Nozka, H. Nunez, L. A. Ochilo, L. Oikonomou, F. Olinto, A. Selmi-Dei, D. Pakk Palatka, M. Pallotta, J. Papenbreer, P. Parente, G. Parra, A. Paul, T. Pech, M. Pekala, J. Pelayo, R. Pena-Rodriguez, J. Pepe, I. M. Pereira, L. A. S. Perrone, L. Petermann, E. Peters, C. Petrera, S. Phuntsok, J. Piegaia, R. Pierog, T. Pieroni, P. Pimenta, M. Pirronello, V. Platino, M. Plum, M. Porowski, C. Prado, R. R. Privitera, P. Prouza, M. Quel, E. J. Querchfeld, S. Quinn, S. Rautenberg, J. Ravel, O. Ravignani, D. Reinert, D. Revenu, B. Ridky, J. Risse, M. Ristori, P. Rizi, V. de Carvalho, W. Rodrigues Rojo, J. Rodriguez Rogozin, D. Rosado, J. Roth, M. Roulet, E. Rovero, A. C. Saffi, S. J. Saftoiu, A. Salazar, H. Saleh, A. Greus, F. Salesa Salina, G. Gomez, J. D. Sanabria Sanchez, F. Sanchez-Lucas, P. Santos, E. M. Santos, E. Sarazin, F. Sarkar, B. Sarmento, R. Sarmiento-Cano, C. Sato, R. Scarso, C. Schauer, M. Scherini, V. Schieler, H. Schmidt, D. Scholten, O. Schoorlemmer, H. Schovanek, P. Schroeder, F. G. Schulz, A. Schulz, J. Schumacher, J. Sciutto, S. J. Segreto, A. Settimo, M. Shadkam, A. Shellard, C. Sigl, G. Sima, O. Smialkowski, A. Smida, R. Snow, G. R. Sommers, P. Sonntag, S. Sorokin, J. Squartini, R. Stanca, D. Stanic, S. Stapleton, J. Stasielak, J. Strafella, F. Stutz, A. Suarez, F. Suarez Duran, M. Sudholz, T. Suomijaervi, T. Supanitsky, A. D. Sutherland, M. S. Swain, J. Szadkowski, Z. Taborda, O. A. Tapia, A. Tepe, A. Theodoro, V. M. Timmermans, C. Peixoto, C. J. Todero Tomankova, L. Tome, B. Tonachini, A. Torralba Elipe, G. Machado, D. Torres Travnicek, P. Trini, M. Ulrich, R. Unger, M. Urban, M. Valdes Galicia, J. F. Valino, I. Valore, L. van Aar, G. van Bodegom, P. van den Berg, A. M. van Vliet, A. Varela, E. Vargas Cardenas, B. Varner, G. Vasquez, R. Vazquez, J. R. Vazquez, R. A. Veberic, D. Verzi, V. Vicha, J. Videla, M. Villasenor, L. Vorobiov, S. Wahlberg, H. Wainberg, O. Walz, D. Watson, A. A. Weber, M. Weindl, A. Wiencke, L. Wilczynski, H. Winchen, T. Wittkowski, D. Wundheiler, B. Wykes, S. Yang, L. Yapici, T. Yelos, D. Yushkov, A. Zas, E. Zavrtanik, D. Zavrtanik, M. Zepeda, A. Zimmermann, B. Ziolkowski, M. Zong, Z. Zuccarello, F. CA Pierre Auger Collaboration TI Azimuthal asymmetry in the risetime of the surface detector signals of the Pierre Auger Observatory SO PHYSICAL REVIEW D LA English DT Article ID EXTENSIVE AIR-SHOWERS; COSMIC-RAYS; PARTICLES; DISTANCES; EVENT; ARRAY AB The azimuthal asymmetry in the risetime of signals in Auger surface detector stations is a source of information on shower development. The azimuthal asymmetry is due to a combination of the longitudinal evolution of the shower and geometrical effects related to the angles of incidence of the particles into the detectors. The magnitude of the effect depends upon the zenith angle and state of development of the shower and thus provides a novel observable, (sec theta)(max), sensitive to the mass composition of cosmic rays above 3 x 10(18) eV. By comparing measurements with predictions from shower simulations, we find for both of our adopted models of hadronic physics (QGSJETII-04 and EPOS-LHC) an indication that the mean cosmic-ray mass increases slowly with energy, as has been inferred from other studies. However, the mass estimates are dependent on the shower model and on the range of distance from the shower core selected. Thus the method has uncovered further deficiencies in our understanding of shower modeling that must be resolved before the mass composition can be inferred from (sec theta)(max). C1 [Aab, A.; Buchholz, P.; Erfani, M.; Heimann, P.; Niechciol, M.; Ochilo, L.; Risse, M.; Sonntag, S.; Tepe, A.; Yushkov, A.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys Expt Teilchenphys 7, D-57068 Siegen, Germany. [Abreu, P.; Andringa, S.; Assis, P.; Blanco, A.; Blumer, H.; Cazon, L.; Diogo, F.; Espadanal, J.; Gomez Vitale, P. 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RI Ridky, Jan/H-6184-2014; Pimenta, Mario/M-1741-2013; de souza, Vitor/D-1381-2012; Guarino, Fausto/I-3166-2012; Zuccarello, Francesca/R-1834-2016; Colalillo, Roberta/R-5088-2016; Buscemi, Mario/R-5071-2016; Valino, Ines/J-8324-2012; Horvath, Pavel/G-6334-2014; De Mitri, Ivan/C-1728-2017; Mitrica, Bogdan/D-5201-2009; Alves Batista, Rafael/K-6642-2012; dos Santos, Eva/N-6351-2013; Nosek, Dalibor/F-1129-2017; Fauth, Anderson/F-9570-2012; Abreu, Pedro/L-2220-2014; Assis, Pedro/D-9062-2013; Navas, Sergio/N-4649-2014; Arqueros, Fernando/K-9460-2014; Cazon, Lorenzo/G-6921-2014; Conceicao, Ruben/L-2971-2014; Bueno, Antonio/F-3875-2015; Beatty, James/D-9310-2011; Sao Carlos Institute of Physics, IFSC/USP/M-2664-2016; de Mello Neto, Joao/C-5822-2013; de Almeida, Rogerio/L-4584-2016; Badescu, Alina/B-6087-2012; zas, enrique/I-5556-2015; Chinellato, Jose Augusto/I-7972-2012; Caramete, Laurentiu/C-2328-2011; Chinellato, Carola Dobrigkeit /F-2540-2011; Rosado, Jaime/K-9109-2014; Moura Santos, Edivaldo/K-5313-2016; Tome, Bernardo/J-4410-2013; Alvarez-Muniz, Jaime/H-1857-2015; Gouffon, Philippe/I-4549-2012 OI Coutu, Stephane/0000-0003-2923-2246; Garcia, Beatriz/0000-0003-0919-2734; Novotny, Vladimir/0000-0002-4319-4541; Ulrich, Ralf/0000-0002-2535-402X; Nunez, Luis/0000-0003-4575-5899; Ridky, Jan/0000-0001-6697-1393; Pimenta, Mario/0000-0002-2590-0908; Rizi, Vincenzo/0000-0002-5277-6527; Garcia Pinto, Diego/0000-0003-1348-6735; Guarino, Fausto/0000-0003-1427-9885; Zuccarello, Francesca/0000-0003-1853-2550; Colalillo, Roberta/0000-0002-4179-9352; Buscemi, Mario/0000-0003-2123-5434; Valino, Ines/0000-0001-7823-0154; Horvath, Pavel/0000-0002-6710-5339; De Mitri, Ivan/0000-0002-8665-1730; Alves Batista, Rafael/0000-0003-2656-064X; dos Santos, Eva/0000-0002-0474-8863; Nosek, Dalibor/0000-0001-6219-200X; Fauth, Anderson/0000-0001-7239-0288; Abreu, Pedro/0000-0002-9973-7314; Assis, Pedro/0000-0001-7765-3606; Navas, Sergio/0000-0003-1688-5758; Arqueros, Fernando/0000-0002-4930-9282; Cazon, Lorenzo/0000-0001-6748-8395; 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Nordrhein Westfalen, Germany; Ministerium fur Wissenschaft, Germany; Forschung und Kunst, Germany; Baden-Wurttember, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Istituto Nazionale di Astrofisica (INAF), Italy; Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Italy; Gran Sasso Center for Astroparticle Physics (CFA), Italy; CETEMPS Center of Excellence, Italy; Ministero degli Affari Esteri (MAE), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Netherlands; Cultuur en Wetenschap, Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development, Poland [ERA-NET-ASPERA/01/11, ERA-NET-ASPERA/02/11]; National Science Centre, Poland [2013/08/M/ST9/00322, 2013/08/M/ST9/00728, HARMONIA 5-2013/10/M/ST9/00062]; Portuguese national funds, Portugal; FEDER funds within Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia (COMPETE), Portugal; Romanian Authority for Scientific Research ANCS, Romania; CNDI-UEFISCDI, Romania [20/2012, 194/2012, 1/ASPERA2/2012 ERA-NET, PN-II-RU-PD-2011- 3-0145-17, PN-II-RU-PD-2011-3-0062]; Minister of National Education, Romania; Programme Space Technology and Advanced Research (STAR), Romania [83/2013]; Slovenian Research Agency, Slovenia; Comunidad de Madrid, Spain; FEDER funds, Spain; Ministerio de Educacion y Ciencia, Spain; Xunta de Galicia, Spain; European Community 7th Framework Program, Spain [FP7-PEOPLE-2012-IEF-328826]; Science and Technology Facilities Council, United Kingdom; Department of Energy, USA [DE-AC02-07CH11359, DE-FR02-04ER41300, DE-FG02-99ER41107, DE-SC0011689]; National Science Foundation, USA [0450696]; Grainger Foundation, USA; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET; European Particle Physics Latin American Network; European Union 7th Framework Program [PIRSES-2009-GA-246806]; UNESCO; [MSMT-CR LG13007]; [7AMB14AR005] FX The successful installation, commissioning, and operation of the Pierre Auger Observatory would not have been possible without the strong commitment and effort from the technical and administrative staff in Malargue. We are very grateful to the following agencies and organizations for financial support: Comision Nacional de Energia Atomica, Agencia Nacional de Promocion Cientifica y Tecnologica (ANPCyT), Consejo Nacional de Investigaciones Cientificas y Tecnicas (CONICET), Gobierno de la Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas, in gratitude for their continuing cooperation over land access, Argentina; the Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Sao Paulo Research Foundation (FAPESP) Grants No. 2010/07359-6 and No. 1999/05404-3, Ministerio de Ciencia e Tecnologia (MCT), Brazil; Grant No. MSMT-CR LG13007, No. 7AMB14AR005, and the Czech Science Foundation Grant No. 14-17501S, Czech Republic; Centre de Calcul IN2P3/CNRS, Centre National de la Recherche Scientifique (CNRS), Conseil Regional Ile-de-France, Departement Physique Nucleaire et Corpusculaire (PNC-IN2P3/CNRS), Departement Sciences de l'Univers (SDU-INSU/CNRS), Institut Lagrange de Paris (ILP) Grant No. LABEX ANR-10-LABX- 63, within the Investissements d'Avenir Programme Grant No. ANR-11-IDEX-0004-02, France; Bundesministerium fur Bildung und Forschung (BMBF), Deutsche Forschungsgemeinschaft (DFG), Finanzministerium Baden-Wurttemberg, Helmholtz Alliance for Astroparticle Physics (HAP), Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Ministerium fur Wissenschaft und Forschung, Nordrhein Westfalen, Ministerium fur Wissenschaft, Forschung und Kunst, Baden-Wurttember, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Istituto Nazionale di Astrofisica (INAF), Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Gran Sasso Center for Astroparticle Physics (CFA), CETEMPS Center of Excellence, Ministero degli Affari Esteri (MAE), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; National Centre for Research and Development, Grants No. ERA-NET-ASPERA/01/11 and No. ERA-NET-ASPERA/02/11, National Science Centre, Grants No. 2013/08/M/ST9/00322, No. 2013/08/M/ST9/00728 and No. HARMONIA 5-2013/10/M/ST9/00062, Poland; Portuguese national funds and FEDER funds within Programa Operacional Factores de Competitividade through Fundacao para a Ciencia e a Tecnologia (COMPETE), Portugal; Romanian Authority for Scientific Research ANCS, CNDI-UEFISCDI partnership projects Grants No. 20/2012 and No. 194/2012, Grants No. 1/ASPERA2/2012 ERA-NET, No. PN-II-RU-PD-2011- 3-0145-17 and No. PN-II-RU-PD-2011-3-0062, the Minister of National Education, Programme Space Technology and Advanced Research (STAR), Grant No. 83/2013, Romania; Slovenian Research Agency, Slovenia; Comunidad de Madrid, FEDER funds, Ministerio de Educacion y Ciencia, Xunta de Galicia, European Community 7th Framework Program, Grant No. FP7-PEOPLE-2012-IEF-328826, Spain; Science and Technology Facilities Council, United Kingdom; Department of Energy, Contracts No. DE-AC02-07CH11359, No. DE-FR02-04ER41300, No. DE-FG02-99ER41107 and No. DE-SC0011689, National Science Foundation, Grant No.; 0450696, The Grainger Foundation, USA; NAFOSTED, Vietnam; Marie Curie-IRSES/EPLANET, European Particle Physics Latin American Network, European Union 7th Framework Program, Grant No. PIRSES-2009-GA-246806; and UNESCO. NR 48 TC 1 Z9 1 U1 18 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 7 PY 2016 VL 93 IS 7 AR 072006 DI 10.1103/PhysRevD.93.072006 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5ZL UT WOS:000373578900003 ER PT J AU Blyth, SC Chan, YL Chen, XC Chu, MC Cui, KX Hahn, RL Ho, TH Hsiung, YB Hu, BZ Kwan, KK Kwok, MW Kwok, T Lau, YP Leung, JKC Leung, KY Lin, GL Lin, YC Luk, KB Luk, WH Ngai, HY Ngan, SY Pun, CSJ Shih, K Tam, YH Tsang, RHM Wang, CH Wong, CM Wong, HLH Wong, KK Yeh, M Zhang, BJ AF Blyth, S. C. Chan, Y. L. Chen, X. C. Chu, M. C. Cui, K. X. Hahn, R. L. Ho, T. H. Hsiung, Y. B. Hu, B. Z. Kwan, K. K. Kwok, M. W. Kwok, T. Lau, Y. P. Leung, J. K. C. Leung, K. Y. Lin, G. L. Lin, Y. C. Luk, K. B. Luk, W. H. Ngai, H. Y. Ngan, S. Y. Pun, C. S. J. Shih, K. Tam, Y. H. Tsang, R. H. M. Wang, C. H. Wong, C. M. Wong, H. L. H. Wong, K. K. Yeh, M. Zhang, B. J. TI Measurement of cosmic-ray muons and muon-induced neutrons in the Aberdeen Tunnel Underground Laboratory SO PHYSICAL REVIEW D LA English DT Article ID INTENSITY CURVE; DEPTH; FLUX AB We have measured the muon flux and production rate of muon-induced neutrons at a depth of 611 m water equivalent. Our apparatus comprises three layers of crossed plastic scintillator hodoscopes for tracking the incident cosmic-ray muons and 760 L of a gadolinium-doped liquid scintillator for producing and detecting neutrons. The vertical muon intensity was measured to be I-mu = (5.7 +/- 0.6) x 10(-6) cm(-2) s(-1) sr(-1). The yield of muon-induced neutrons in the liquid scintillator was determined to be Y-n = (1.19 +/- 0.08(stat) +/- 0.21(syst)) x 10(-4) neutrons/(mu.g.cm(-2)). A fit to the recently measured neutron yields at different depths gave a mean muon energy dependence of < E-mu >(0.76 +/- 0.03) for liquid-scintillator targets. C1 [Blyth, S. C.; Wang, C. H.] Natl United Univ, Dept Electroopt Engn, Miaoli 36063, Taiwan. [Chan, Y. L.; Chen, X. C.; Chu, M. C.; Kwan, K. K.; Kwok, M. W.; Lin, Y. C.; Luk, W. H.; Ngan, S. Y.; Shih, K.; Tam, Y. H.; Wong, C. M.; Wong, K. K.] Chinese Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Cui, K. X.; Kwok, T.; Lau, Y. P.; Leung, J. K. C.; Leung, K. Y.; Ngai, H. Y.; Pun, C. S. J.; Tsang, R. H. M.; Wong, H. L. H.; Zhang, B. J.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Hahn, R. L.; Yeh, M.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Ho, T. H.; Hsiung, Y. B.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Hu, B. Z.; Lin, G. L.] Natl Chiao Tung Univ, Inst Phys, Hsinchu 300, Taiwan. [Luk, K. B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Ngai, HY (reprint author), Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. EM jngai@graduate.hku.hk OI HSIUNG, YEE/0000-0003-4801-1238 FU Research Grant Council of Hong Kong Special Administrative Region, China [HKU703307P, HKU704007P, CUHK 1/07C, CUHK3/CRF/10]; University Development Fund; Chinese University of Hong Kong; Office of Nuclear Physics, Office of High Energy Physics, Office of Science, U.S. Department of Energy [DE-AC-02-05CH11231, DE-AC-02-98CH10886]; National Science Council in Taiwan; National Taiwan University; National Chiao Tung University; Serco Group, plc; University of Hong Kong FX This work is partially supported by grants from the Research Grant Council of Hong Kong Special Administrative Region, China (Projects No. HKU703307P, No. HKU704007P, No. CUHK 1/07C, and No. CUHK3/CRF/10); University Development Fund and Small Project Funding of The University of Hong Kong; Vice-Chancellor's One-off Discretionary Fund of The Chinese University of Hong Kong; the Office of Nuclear Physics, Office of High Energy Physics, Office of Science, U.S. Department of Energy, under Contracts No. DE-AC-02-05CH11231 and No. DE-AC-02-98CH10886; and the National Science Council in Taiwan and MOE program for Research of Excellence at National Taiwan University and National Chiao Tung University. The authors would like to thank the Transport Department, The Government of the Hong Kong Special Administrative Region, for providing the underground facilities and Serco Group, plc, for their cooperation and support in the Aberdeen Tunnel. NR 27 TC 1 Z9 1 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD APR 7 PY 2016 VL 93 IS 7 AR 072005 DI 10.1103/PhysRevD.93.072005 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DI5ZL UT WOS:000373578900002 ER PT J AU Robinson, NJ Caux, JS Konik, RM AF Robinson, Neil J. Caux, Jean-Sebastien Konik, Robert M. TI Motion of a Distinguishable Impurity in the Bose Gas: Arrested Expansion Without a Lattice and Impurity Snaking SO PHYSICAL REVIEW LETTERS LA English DT Article ID DIMENSIONAL QUANTUM LIQUIDS; TONKS-GIRARDEAU GAS; MANY-BODY PROBLEM; ULTRACOLD ATOMS; PRETHERMALIZATION; EQUILIBRIUM; RELAXATION; PARTICLES; DYNAMICS; METALS AB We consider the real-time dynamics of an initially localized distinguishable impurity injected into the ground state of the Lieb-Liniger model. Focusing on the case where integrability is preserved, we numerically compute the time evolution of the impurity density operator in regimes far from analytically tractable limits. We find that the injected impurity undergoes a stuttering motion as it moves and expands. For an initially stationary impurity, the interaction-driven formation of a quasibound state with a hole in the background gas leads to arrested expansion-a period of quasistationary behavior. When the impurity is injected with a finite center-of-mass momentum, the impurity moves through the background gas in a snaking manner, arising from a quantum Newton's cradlelike scenario where momentum is exchanged back and forth between the impurity and the background gas. C1 [Robinson, Neil J.; Konik, Robert M.] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. [Robinson, Neil J.] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. [Caux, Jean-Sebastien] Univ Amsterdam, Inst Theoret Phys, Sci Pk 904,Postbus 94485, NL-1090 GL Amsterdam, Netherlands. RP Robinson, NJ (reprint author), Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. EM nrobinson@bnl.gov RI Konik, Robert/L-8076-2016; OI Konik, Robert/0000-0003-1209-6890; Robinson, Neil/0000-0001-6633-5338 FU EPSRC [EP/I032487/1]; IRSES Grant QICFT; FOM foundation of the Netherlands; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-SC0012704]; NWO foundation of the Netherlands FX We thank Fabian Essler, Bruno Bertini, John Goold, Rianne van den Berg, and Giuseppe Brandino for useful discussions surrounding this work. This work was partially supported by the EPSRC under Grant No. EP/I032487/1 (N. J. R.), IRSES Grant QICFT (N. J. R., R. M. K.), the FOM and NWO foundations of the Netherlands (J.-S. C., R. M. K.), and the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract Nos. DE-AC02-98CH10886 and DE-SC0012704 (N. J. R., R. M. K.). NR 81 TC 2 Z9 2 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 7 PY 2016 VL 116 IS 14 AR 145302 DI 10.1103/PhysRevLett.116.145302 PG 6 WC Physics, Multidisciplinary SC Physics GA DI6CT UT WOS:000373587500012 PM 27104716 ER PT J AU Zhu, CH Tuchband, MR Young, A Shuai, M Scarbrough, A Walba, DM Maclennan, JE Wang, C Hexemer, A Clark, NA AF Zhu, Chenhui Tuchband, Michael R. Young, Anthony Shuai, Min Scarbrough, Alyssa Walba, David M. Maclennan, Joseph E. Wang, Cheng Hexemer, Alexander Clark, Noel A. TI Resonant Carbon K-Edge Soft X-Ray Scattering from Lattice-Free Heliconical Molecular Ordering: Soft Dilative Elasticity of the Twist-Bend Liquid Crystal Phase SO PHYSICAL REVIEW LETTERS LA English DT Article ID BANANA-SHAPED MOLECULES; NEMATIC PHASE; ORIENTATIONAL ORDER; NMR-SPECTROSCOPY; DIMERS; TRANSITION; MESOPHASES; MORPHOLOGY; FILMS AB Resonant x-ray scattering shows that the bulk structure of the twist-bend liquid crystal phase, recently discovered in bent molecular dimers, has spatial periodicity without electron density modulation, indicating a lattice-free heliconical nematic precession of orientation that has helical glide symmetry. In situ study of the bulk helix texture of the dimer CB7CB shows an elastically confined temperature-dependent minimum helix pitch, but a remarkable elastic softness of pitch in response to dilative stresses. Scattering from the helix is not detectable in the higher temperature nematic phase. C1 [Zhu, Chenhui; Young, Anthony; Wang, Cheng; Hexemer, Alexander] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Tuchband, Michael R.; Shuai, Min; Maclennan, Joseph E.; Clark, Noel A.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Tuchband, Michael R.; Shuai, Min; Maclennan, Joseph E.; Clark, Noel A.] Univ Colorado, Soft Mat Res Ctr, Boulder, CO 80309 USA. [Scarbrough, Alyssa; Walba, David M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Scarbrough, Alyssa; Walba, David M.] Univ Colorado, Soft Mat Res Ctr, Boulder, CO 80309 USA. RP Zhu, CH; Hexemer, A (reprint author), Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA.; Clark, NA (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA.; Clark, NA (reprint author), Univ Colorado, Soft Mat Res Ctr, Boulder, CO 80309 USA. EM chenhuizhu@lbl.gov; ahexemer@lbl.gov; noel.clark@colorado.edu RI Clark, Noel/E-9011-2010; Wang, Cheng/A-9815-2014 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Soft Materials Research Center under NSF MRSEC [DMR-1420736] FX We acknowledge the use of beam lines 11.0.1.2 and 7.3.3 of the Advanced Light Source supported by the Director of the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was supported by the Soft Materials Research Center under NSF MRSEC Grant No. DMR-1420736. NR 51 TC 19 Z9 19 U1 18 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD APR 7 PY 2016 VL 116 IS 14 AR 147803 DI 10.1103/PhysRevLett.116.147803 PG 6 WC Physics, Multidisciplinary SC Physics GA DI6CT UT WOS:000373587500015 PM 27104729 ER PT J AU Gardner, SN McLoughlin, K Be, NA Allen, J Weaver, SC Forrester, N Guerbois, M Jaing, C AF Gardner, Shea N. McLoughlin, Kevin Be, Nicholas A. Allen, Jonathan Weaver, Scott C. Forrester, Naomi Guerbois, Mathilde Jaing, Crystal TI Characterization of Genetic Variability of Venezuelan Equine Encephalitis Viruses SO PLOS ONE LA English DT Article ID ENCEPHALOMYELITIS VIRUS; HIGH-ACCURACY; EMERGENCE; EVOLUTION; DISEASE; REGION; PANAMA; TREES; PERU AB Venezuelan equine encephalitis virus (VEEV) is a mosquito-borne alphavirus that has caused large outbreaks of severe illness in both horses and humans. New approaches are needed to rapidly infer the origin of a newly discovered VEEV strain, estimate its equine amplification and resultant epidemic potential, and predict human virulence phenotype. We performed whole genome single nucleotide polymorphism (SNP) analysis of all available VEE antigenic complex genomes, verified that a SNP-based phylogeny accurately captured the features of a phylogenetic tree based on multiple sequence alignment, and developed a high resolution genome-wide SNP microarray. We used the microarray to analyze a broad panel of VEEV isolates, found excellent concordance between array-and sequence-based SNP calls, genotyped unsequenced isolates, and placed them on a phylogeny with sequenced genomes. The microarray successfully genotyped VEEV directly from tissue samples of an infected mouse, bypassing the need for viral isolation, culture and genomic sequencing. Finally, we identified genomic variants associated with serotypes and host species, revealing a complex relationship between genotype and phenotype. C1 [Gardner, Shea N.; McLoughlin, Kevin; Allen, Jonathan] Lawrence Livermore Natl Lab, Computat, Livermore, CA USA. [Be, Nicholas A.; Jaing, Crystal] Lawrence Livermore Natl Lab, Phys & Life Sci, Livermore, CA USA. [Weaver, Scott C.; Forrester, Naomi; Guerbois, Mathilde] Univ Texas Med Branch, Inst Human Infect & Immun, Galveston, TX 77555 USA. [Weaver, Scott C.; Forrester, Naomi; Guerbois, Mathilde] Univ Texas Med Branch, Dept Microbiol & Immunol, Galveston, TX 77555 USA. [Weaver, Scott C.; Forrester, Naomi; Guerbois, Mathilde] Univ Texas Med Branch, Dept Pathol, Galveston, TX 77555 USA. RP Jaing, C (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci, Livermore, CA USA. EM jaing2@llnl.gov RI Weaver, Scott/D-6490-2011 FU Defense Threat Reduction Agency; Lawrence Livermore National Laboratory [DTRA10027IA-2359] FX Funding was provided by the Defense Threat Reduction Agency under Interagency Agreement with Lawrence Livermore National Laboratory (DTRA10027IA-2359). CJ and SW received funding. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 27 TC 1 Z9 1 U1 1 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 7 PY 2016 VL 11 IS 4 AR e0152604 DI 10.1371/journal.pone.0152604 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI6KO UT WOS:000373608000028 PM 27054586 ER PT J AU Moen, ST Hatcher, CL Singh, AK AF Moen, Scott T. Hatcher, Christopher L. Singh, Anup K. TI A Centrifugal Microfluidic Platform That Separates Whole Blood Samples into Multiple Removable Fractions Due to Several Discrete but Continuous Density Gradient Sections SO PLOS ONE LA English DT Article ID MONONUCLEAR-CELLS; SEDIMENTATION; MONOCYTES; VOLUME AB We present a miniaturized centrifugal platform that uses density centrifugation for separation and analysis of biological components in small volume samples (similar to 5 mu L). We demonstrate the ability to enrich leukocytes for on-disk visualization via microscopy, as well as recovery of viable cells from each of the gradient partitions. In addition, we simplified the traditional Modified Wright-Giemsa staining by decreasing the time, volume, and expertise involved in the procedure. From a whole blood sample, we were able to extract 95.15% of leukocytes while excluding 99.8% of red blood cells. This platform has great potential in both medical diagnostics and research applications as it offers a simpler, automated, and inexpensive method for biological sample separation, analysis, and downstream culturing. C1 [Moen, Scott T.; Singh, Anup K.] Sandia Natl Labs, Livermore, CA USA. [Moen, Scott T.; Hatcher, Christopher L.; Singh, Anup K.] Univ Texas Med Branch, Galveston, TX 77555 USA. RP Moen, ST (reprint author), Sandia Natl Labs, Livermore, CA USA.; Moen, ST (reprint author), Univ Texas Med Branch, Galveston, TX 77555 USA. EM stmoen@utmb.edu FU National Institute of Allergy and Infectious Diseases [R01AI0988530]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NIH-NIAID [R01AI0988530] FX This research was funded by National Institute of Allergy and Infectious Diseases (Grant R01AI0988530). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000 (STM).; This research was funded by NIH-NIAID grant number R01AI0988530. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. We would also like to thank Greg Berry and Mardelle Susman for their editing services. NR 24 TC 0 Z9 0 U1 13 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD APR 7 PY 2016 VL 11 IS 4 AR e0153137 DI 10.1371/journal.pone.0153137 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DI6KO UT WOS:000373608000085 PM 27054764 ER PT J AU Hinks, ML Brady, MV Lignell, H Song, MJ Grayson, JW Bertram, AK Lin, P Laskin, A Laskin, J Nizkorodov, SA AF Hinks, Mallory L. Brady, Monica V. Lignell, Hanna Song, Mijung Grayson, James W. Bertram, Allan K. Lin, Peng Laskin, Alexander Laskin, Julia Nizkorodov, Sergey A. TI Effect of viscosity on photodegradation rates in complex secondary organic aerosol materials SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID ATMOSPHERIC BROWN CARBON; LIQUID PHASE-SEPARATION; MARINE BOUNDARY-LAYER; ALPHA-PINENE; RELATIVE-HUMIDITY; AQUEOUS-SOLUTIONS; WATER DIFFUSION; GLASSY AEROSOL; PARTICLES; GROWTH AB This work explores the effect of environmental conditions on the photodegradation rates of atmospherically relevant, photolabile, organic molecules embedded in a film of secondary organic material (SOM). Three types of SOM were studied: alpha-pinene/O-3 SOM (PSOM), limonene/O3 SOM (LSOM), and aged limonene/O3 obtained by exposure of LSOM to ammonia (brown LSOM). PSOM and LSOM were impregnated with 2,4-dinitrophenol (2,4-DNP), an atmospherically relevant molecule that photodegrades faster than either PSOM or LSOM alone, to serve as a probe of SOM matrix effects on photochemistry. Brown LSOM contains an unidentified chromophore that absorbs strongly at 510 nm and photobleaches upon irradiation. This chromophore served as a probe molecule for the brown LSOM experiments. In all experiments, either the temperature or relative humidity (RH) surrounding the SOM films was varied. The extent of photochemical reaction in the samples was monitored using UV-vis absorption spectroscopy. For all three model systems examined, the observed photodegradation rates were slower at lower temperatures and lower RH, conditions that make SOM more viscous. Additionally, the activation energies for photodegradation of each system were positively correlated with the viscosity of the SOM matrix as measured in poke-flow experiments. These activation energies were calculated to be 50, 24, and 17 kJ mol(-1) for 2,4-DNP in PSOM, 2,4-DNP in LSOM, and the chromophore in brown LSOM, respectively, and PSOM was found to be the most viscous of the three. These results suggest that the increased viscosity is hindering the motion of the molecules in SOM and is slowing down their respective photochemical reactions. C1 [Hinks, Mallory L.; Brady, Monica V.; Lignell, Hanna; Nizkorodov, Sergey A.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Song, Mijung; Grayson, James W.; Bertram, Allan K.] Univ British Columbia, Dept Chem, Vancouver, BC, Canada. [Lin, Peng; Laskin, Alexander] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Laskin, Julia] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Nizkorodov, SA (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. EM nizkorod@uci.edu RI Lin, Peng/G-4867-2016; Laskin, Alexander/I-2574-2012; Laskin, Julia/H-9974-2012; Nizkorodov, Sergey/I-4120-2014 OI Lin, Peng/0000-0002-3567-7017; Laskin, Alexander/0000-0002-7836-8417; Laskin, Julia/0000-0002-4533-9644; Nizkorodov, Sergey/0000-0003-0891-0052 FU U. S. Department of Commerce, National Oceanic and Atmospheric Administration through Climate Program Office's AC4 program [NA13OAR4310066, NA13OAR4310062]; National Science Foundation (NSF) [CHE-0909227]; NSF summer research undergraduate experience (RUE) program; Natural Sciences and Engineering Research Council of Canada; Office of Biological and Environmental Research of the US. DOE; US DOE [DEAC06-76RL0 1830] FX P. L., A. L., J. L., and S. N. acknowledge support by the U. S. Department of Commerce, National Oceanic and Atmospheric Administration through Climate Program Office's AC4 program, awards NA13OAR4310066 (PNNL) and NA13OAR4310062 (UCI). MH and HL acknowledge support by the National Science Foundation (NSF) grant CHE-0909227. MB was supported by the NSF summer research undergraduate experience (RUE) program. MS, JG, and AB were supported by the Natural Sciences and Engineering Research Council of Canada. The LC-PDA-MS measurements were performed at the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at PNNL, and sponsored by the Office of Biological and Environmental Research of the US. DOE. PNNL is operated for US DOE by Battelle Memorial Institute under Contract No. DEAC06-76RL0 1830. NR 73 TC 8 Z9 8 U1 17 U2 61 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 7 PY 2016 VL 18 IS 13 BP 8785 EP 8793 DI 10.1039/c5cp05226b PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH7UU UT WOS:000373000100003 PM 26685987 ER PT J AU Gunaratne, KDD Prabhakaran, V Andersen, A Johnson, GE Laskin, J AF Gunaratne, K. Don D. Prabhakaran, Venkateshkumar Andersen, Amity Johnson, Grant E. Laskin, Julia TI Charge retention of soft-landed phosphotungstate Keggin anions on self-assembled monolayers SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID MASS-SELECTED IONS; PEPTIDE IONS; ELECTROCHEMICAL PROPERTIES; ELECTROSPRAY-IONIZATION; DESORPTION-KINETICS; HETEROPOLY BLUES; ALPHA-KEGGIN; GAS-PHASE; SURFACES; REDUCTION AB Soft landing of mass-selected ions onto surfaces often results in partial loss of charge that may affect the structure and reactivity of deposited species. In this study, Keggin phosphotungstate anions in two selected charge states, PW12O403- (WPOM3-) and PW12O402- (WPOM2-), were soft-landed onto different self-assembled monolayer (SAM) surfaces and examined using in situ infrared reflection absorption spectroscopy (IRRAS) and density functional theory (DFT) calculations. Partial retention of the 3- charge was observed when WPOM3- was soft-landed onto the fluorinated SAM (FSAM), while the charge state distribution was dominated by the 2- charge after both WPOM3- and WPOM2- were deposited onto a hydrophilic alkylthiol SAM terminated with cationic NH3+ functional groups (NH3+ SAM). We found that during the course of the soft landing of WPOM3-, the relative abundance of WPOM3- on FSAM decreased while that of WPOM2- increased. We propose that the higher stability of immobilized WPOM2- in comparison with WPOM3- makes it the preferred charge state of WPOM on both the FSAM and NH3+ SAM. We also observe weaker binding of WPOM anions to SAMs in comparison with phosphomolybdate ions (MoPOM) reported previously (J. Phys. Chem. C, 2014, 118, 27611-27622). The weaker binding of WPOM to SAMs is attributed to the lower reactivity of WPOM reported in the literature. This study demonstrates that both the charge retention and the reactivity of deposited anionic POM clusters on surfaces are determined by the type of addenda metal atoms in the cluster. C1 [Gunaratne, K. Don D.; Prabhakaran, Venkateshkumar; Andersen, Amity; Johnson, Grant E.; Laskin, Julia] Pacific NW Natl Lab, Div Phys Sci, POB 999,MSIN K8-88, Richland, WA 99352 USA. RP Laskin, J (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MSIN K8-88, Richland, WA 99352 USA. EM Julia.Laskin@pnnl.gov RI Laskin, Julia/H-9974-2012 OI Laskin, Julia/0000-0002-4533-9644 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences & Biosciences Division; DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL); DOE [DE-AC05-76RL01830] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences & Biosciences Division. The research was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for DOE under Contract DE-AC05-76RL01830. NR 65 TC 1 Z9 1 U1 6 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 7 PY 2016 VL 18 IS 13 BP 9021 EP 9028 DI 10.1039/c5cp06954h PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH7UU UT WOS:000373000100027 PM 26966731 ER PT J AU Rudiger, C Favaro, M Valero-Vidal, C Calvillo, L Bozzolo, N Jacomet, S Hejny, C Gregoratti, L Amati, M Agnoli, S Granozzi, G Kunze-Liebhauser, J AF Ruediger, Celine Favaro, Marco Valero-Vidal, Carlos Calvillo, Laura Bozzolo, Nathalie Jacomet, Suzanne Hejny, Clivia Gregoratti, Luca Amati, Matteo Agnoli, Stefano Granozzi, Gaetano Kunze-Liebhaeuser, Julia TI Fabrication of Ti substrate grain dependent C/TiO2 composites through carbothermal treatment of anodic TiO2 SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID RAMAN-SPECTRA; CRYSTALLOGRAPHIC ORIENTATION; PHASE-COMPOSITION; GRAPHENE OXIDE; TITANIUM-OXIDE; ANATASE TIO2; FUEL-CELLS; CARBON; SURFACE; NANOCOMPOSITES AB Composite materials of titania and graphitic carbon, and their optimized synthesis are highly interesting for application in sustainable energy conversion and storage. We report on planar C/TiO2 composite films that are prepared on a polycrystalline titanium substrate by carbothermal treatment of compact anodic TiO2 with acetylene. This thin film material allows for the study of functional properties of C/TiO2 as a function of chemical composition and structure. The chemical and structural properties of the composite on top of individual Ti substrate grains are examined by scanning photoelectron microscopy and micro-Raman spectroscopy. Through comparison of these data with electron backscatter diffraction, it is found that the amount of generated carbon and the grade of anodic film crystallinity correlate with the crystallographic orientation of the Ti substrate grains. On top of Ti grains with similar to(0001) orientations the anodic TiO2 exhibits the highest grade of crystallinity, and the composite contains the highest fraction of graphitic carbon compared to Ti grains with other orientations. This indirect effect of the Ti substrate grain orientation yields new insights into the activity of TiO2 towards the decomposition of carbon precursors. C1 [Ruediger, Celine] Tech Univ Munich, Dept Phys, James Franck Str 1, D-85748 Garching, Germany. [Ruediger, Celine; Valero-Vidal, Carlos; Kunze-Liebhaeuser, Julia] Leopold Franzens Univ Innsbruck, Inst Phys Chem, Innrain 52c, A-6020 Innsbruck, Austria. [Favaro, Marco; Calvillo, Laura; Agnoli, Stefano; Granozzi, Gaetano] Univ Padua, Dipartimento Sci Chim, Via Marzolo 1, I-35131 Padua, Italy. [Bozzolo, Nathalie; Jacomet, Suzanne] PSL Res Univ, MINES ParisTech, CEMEF Ctr Mise Forme Mat, CNRS,UMR 7635, CS 10207,Rue Claude Daunesse, F-06904 Sophia Antipolis, France. [Hejny, Clivia] Leopold Franzens Univ Innsbruck, Inst Mineral & Petrog, Innrain 52d, A-6020 Innsbruck, Austria. [Gregoratti, Luca; Amati, Matteo] Elettra Sincrotrone Trieste SCpA, SS14-Km163-5 Area Sci Pk, I-34149 Trieste, Italy. [Favaro, Marco; Valero-Vidal, Carlos] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source ALS, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Favaro, Marco; Valero-Vidal, Carlos] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, JCAP, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Rudiger, C (reprint author), Tech Univ Munich, Dept Phys, James Franck Str 1, D-85748 Garching, Germany.; Rudiger, C; Kunze-Liebhauser, J (reprint author), Leopold Franzens Univ Innsbruck, Inst Phys Chem, Innrain 52c, A-6020 Innsbruck, Austria. EM Celine.Ruediger@uibk.ac.at; Julia.Kunze@uibk.ac.at RI Bozzolo, Nathalie/B-2870-2008 OI Bozzolo, Nathalie/0000-0002-8963-977X FU EU [309741, FP7-NMP-2012-SMALL-6]; DFG [KU2398/1-1] FX The authors thank the EU RTD Framework Programme FP7 (FP7-NMP-2012-SMALL-6, project title DECORE, project number 309741) for financial support. We thank the DFG for financial support during the early stages of this study (project KU2398/1-1). Furthermore, the chair of Technical Chemistry II at TU Munchen is acknowledged for the possibility for preliminary Raman studies, especially we are grateful to Jennifer Hein and Prof. Andreas Jentys for their assistance. We thank Prof. Kurt Hingerl for measuring the thickness of the anodic TiO2. We thank Dr Katrin F. Domke for the helpful discussions on the evaluation of Raman data. NR 57 TC 2 Z9 2 U1 5 U2 17 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD APR 7 PY 2016 VL 18 IS 13 BP 9220 EP 9231 DI 10.1039/c5cp07727c PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH7UU UT WOS:000373000100048 PM 26975480 ER PT J AU Liu, HD Chen, Y Hy, S An, K Venkatachalam, S Qian, DN Zhang, MH Meng, YS AF Liu, Haodong Chen, Yan Hy, Sunny An, Ke Venkatachalam, Subramanian Qian, Danna Zhang, Minghao Meng, Ying Shirley TI Operando Lithium Dynamics in the Li-Rich Layered Oxide Cathode Material via Neutron Diffraction SO ADVANCED ENERGY MATERIALS LA English DT Article ID RECHARGEABLE NA BATTERIES; ION BATTERIES; ELECTROCHEMICAL-CELL; ELECTRODE MATERIALS; VOLTAGE-FADE; CAPACITY; SURFACE; MN; LI1.20MN0.54CO0.13NI0.13O2; PARTICIPATION AB Neutron diffraction under operando battery cycling is used to study the lithium and oxygen dynamics of high Li-rich Li(Lix/3Ni(3/8-3x/8)Co((1/4-x/4))Mn(3/8+7x/24)O2 (x = 0.6, HLR) and low Li-rich Li(Lix/3Ni(1/3-x/3)Co(1/3-x/3)Mn(1/3+x/3)O2 (x = 0.24, LLR) compounds that exhibit different degrees of oxygen activation at high voltage. The measured lattice parameter changes and oxygen position show largely contrasting changes for the two cathodes where the LLR exhibits larger movement of oxygen and lattice contractions in comparison to the HLR that maintains relatively constant lattice parameters and oxygen position during the high voltage plateau until the end of charge. Density functional theory calculations show the presence of oxygen vacancy during the high voltage plateau; changes in the lattice parameters and oxygen position are consistent with experimental observations. Lithium migration kinetics for the Li-rich material is observed under operando conditions for the first time to reveal the rate of lithium extraction from the lithium layer, and transition metal layer is related to the different charge and discharge characteristics. At the beginning of charging, the lithium extraction predominately occurs within the lithium layer. Once the high voltage plateau is reached, the lithium extraction from the lithium layer slows down and extraction from the transition metal layer evolves at a faster rate. C1 [Liu, Haodong; Hy, Sunny; Qian, Danna; Zhang, Minghao; Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. [Chen, Yan; An, Ke] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37830 USA. [Venkatachalam, Subramanian] Envia Syst, 7979 Gateway Bldg,Suite 101, Newark, CA 94560 USA. RP Meng, YS (reprint author), Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92093 USA. EM shirleymeng@ucsd.edu RI An, Ke/G-5226-2011; Chen, Yan/H-4913-2014 OI An, Ke/0000-0002-6093-429X; Chen, Yan/0000-0001-6095-1754 FU Office of Vehicle Technologies of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; Office of Vehicle Technologies of the U.S. Department of Energy (DOE) under Advanced Battery Materials Research (BMR) Program [7073923]; office of Basic Energy Sciences (BES), the Office of Science of the DOE; China Scholarship Council [2011631005]; U.S. DOE's Office of Basic Energy Sciences, Material Science and Engineering Division; National Science Foundation [ACI-1053575] FX UCSD's efforts were supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, Subcontract No. 7073923, under the Advanced Battery Materials Research (BMR) Program. The neutron experiments benefited from the SNS user facility, sponsored by the office of Basic Energy Sciences (BES), the Office of Science of the DOE. H.L. acknowledges the financial support from the China Scholarship Council under Award No. 2011631005. Y.C. acknowledges the support from U.S. DOE's Office of Basic Energy Sciences, Material Science and Engineering Division. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which was supported by National Science Foundation grant number ACI-1053575. NR 36 TC 2 Z9 2 U1 19 U2 52 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD APR 6 PY 2016 VL 6 IS 7 AR 1502143 DI 10.1002/aenm.201502143 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DK1VX UT WOS:000374704200005 ER PT J AU Liu, J Canfield, N Liu, W AF Liu, Jian Canfield, Nathan Liu, Wei TI Preparation and Characterization of a Hydrophobic Metal-Organic Framework Membrane Supported on a Thin Porous Metal Sheet SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID MOLECULAR-SIEVE MEMBRANE; HYDROGEN SELECTIVITY; SEPARATION; CO2; STABILITY; ADSORPTION; CAPTURE AB A hydrophobic metal organic framework (MOF) UiO-66-CH3 is prepared and its solvothermal stability is investigated in comparison to UiO-66. It is confirmed that the MOF stability is enhanced by introduction of the two methyl groups, while the water adsorption is reduced. Given its hydrophobicity and stability, UiO-66-CH3 is proposed as an attractive membrane material for gas separation under moisture conditions. The UiO-66-CH3 membrane is prepared on a 50 pm thin porous Ni support sheet for the first time by use of a secondary growth method. It is found that uniform seed coating on the support is necessary to form a continuous membrane. In addition to growth time and temperature, the presence of a modulator in the growth solution is found to be useful for controlling hydrothermal membrane growth on the seeded support. A dense, intergrown membrane layer is, formed by 24 h growth over a temperature range from 120 to 160 degrees C. The membrane surface comprises 500 nm octahedral crystals, which are supposed to grow out of the original 100 nm spherical seeding crystals. The separation characteristics of resulting membranes are tested with pure CO2, air, CO2/air mixture, and humid CO2/air mixture. CO2 permeance as high as 1.9 x 10(-6) mol/(m(2) s Pa) at 31 degrees C is obtained. Unlike the hydrophilic zeolite membranes, CO2 permeation through this membrane is not blocked by the presence of water vapor in the feed gas. The results suggest that this MOF is a promising membrane material worth further investigation for separation of CO2 and other small molecules from humid gas mixtures. C1 [Liu, Jian; Canfield, Nathan; Liu, Wei] Pacific NW Natl Lab, Energy & Environm Technol Directorate, Richland, WA 99352 USA. RP Liu, W (reprint author), Pacific NW Natl Lab, Energy & Environm Technol Directorate, Richland, WA 99352 USA. EM wei.liu@pnnl.gov RI Liu, Jian/C-4707-2011; Liu, Jian/D-3393-2009 OI Liu, Jian/0000-0001-5329-7408; Liu, Jian/0000-0001-5329-7408 FU US Department of Energy, ARPA-E [DE-AR0000138] FX This work was partially supported by US Department of Energy, ARPA-E, under contract number DE-AR0000138. The authors would like to thank Ms. Sokhom B Sek-a student intern-for doing membrane separation measurements and our colleagues-Drs. Praveen Thallapally and Pete McGrail-for discussions around MOF materials. NR 29 TC 2 Z9 2 U1 31 U2 87 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD APR 6 PY 2016 VL 55 IS 13 BP 3823 EP 3832 DI 10.1021/acs.iecr.5b04739 PG 10 WC Engineering, Chemical SC Engineering GA DI8JW UT WOS:000373748300013 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitlerl, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PC Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M El Sawy, M El-khateeb, E Elkafrawy, T Mohamed, A Salama, E Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Toriashvili, T Lomidze, D Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thur, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, 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Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for anomalous single top quark production in association with a photon in pp collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Flavour Changing Neutral Currents; Hadron-Hadron scattering (experiments); Top physics ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; DECAYS; LHC; COUPLINGS AB The result of a search for flavor changing neutral currents (FCNC) through single top quark production in association with a photon is presented. The study is based on proton-proton collisions at a center-of-mass energy of 8 TeV using data collected with the CMS detector at the LHC, corresponding to an integrated luminosity of 19.8 fb(-1). The search for t gamma events where t -> Wb and W -> mu nu is conducted in final states with a muon, a photon, at least one hadronic jet with at most one being consistent with originating from a bottom quark, and missing transverse momentum. No evidence of single top quark production in association with a photon through a FCNC is observed. Upper limits at the 95% confidence level are set on the tu gamma and tc gamma anomalous couplings and translated into upper limits on the branching fraction of the FCNC top quark decays: B (t -> u gamma) < 1.3 x 10(-4) and B(t -> c gamma) < 1.7 x 10(-3). Upper limits are also set on the cross section of associated t gamma production in a restricted phase-space region. These are the most stringent limits currently available. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. 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[Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Montanari, A.; Braghieri, A.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Piazza Cavalieri 7, Pisa, Italy. [Barone, L.; Cavallari, F.; Dimperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Dimperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmed, I.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Mossolov, V.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Laney, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Korneeva, N.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Erdmann, M.; Bertl, W.; Deiters, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W-S; Hsiung, Y.; Liu, Y. F.; Lu, R-S; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Davignon, O.; Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, A. J.; Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; -Holmes, C. Newman; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J-P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R-J; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Krammer, M.; Schieck, J.; Wulz, C-E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Plestina, R.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Finger, M.; Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [El Sawy, M.] Beni Suef Univ, Bani Suwayf, Egypt. [El Sawy, M.; Salama, E.] British Univ Egypt, Cairo, Egypt. [El-khateeb, E.; Elkafrawy, T.; Salama, E.] Ain Shams Univ, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Toriashvili, T.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Borras, K.] Rhein Westfal TH Aachen, Phys Inst 3, Aachen, Germany. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Tuominen, Eija/A-5288-2017; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Tomei, Thiago/E-7091-2012; Lokhtin, Igor/D-7004-2012; Novaes, Sergio/D-3532-2012; Dubinin, Mikhail/I-3942-2016; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Manganote, Edmilson/K-8251-2013; Azarkin, Maxim/N-2578-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Chinellato, Jose Augusto/I-7972-2012 OI Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; Androsov, Konstantin/0000-0003-2694-6542; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Tuominen, Eija/0000-0002-7073-7767; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Tomei, Thiago/0000-0002-1809-5226; Novaes, Sergio/0000-0003-0471-8549; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Chinellato, Jose Augusto/0000-0002-3240-6270 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.); Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program, Qatar National Research Fund; Rachadapisek Sompot Fund, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (U.S.A.).; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 59 TC 4 Z9 4 U1 17 U2 37 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD APR 6 PY 2016 IS 4 AR 035 DI 10.1007/JHEP04(2016)035 PG 38 WC Physics, Particles & Fields SC Physics GA DI9XG UT WOS:000373855400001 ER PT J AU Zhang, H Fan, LW Dong, HL Zhang, PP Nie, KQ Zhong, J Li, YY Guo, JH Sun, XH AF Zhang, Hui Fan, Liwei Dong, Huilong Zhang, Pingping Nie, Kaiqi Zhong, Jun Li, Youyong Guo, Jinghua Sun, Xuhui TI Spectroscopic Investigation of Plasma-Fluorinated Monolayer Graphene and Application for Gas Sensing SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE graphene; fluorination; NEXAFS; ammonia; gas sensor ID RAY-ABSORPTION-SPECTROSCOPY; CHEMICAL-VAPOR-DEPOSITION; LITHIUM ION BATTERIES; DOPED GRAPHENE; LARGE-AREA; GRAPHITE; SENSORS; SHEETS; CARBON; FILMS AB Large-area monolayer fluorinated graphene (FG) is synthesized by a controllable SF6 plasma treatment. The functional groups of FG are elucidated by various spectroscopies, including Raman spectroscopy, X-ray photo-emission spectroscopy (XPS), and near edge X-ray absorption fine structure (NEXAFS) spectroscopy. Raman results suggest that the defects are introduced into the monolayer graphene during the fluorination process. The fluorine content can be varied by the plasma treatment and can reach the maximum (similar to 24.6 atom % F) under 20 s of plasma treatment as examined by XPS measurement. The angle-dependent NEXAFS results reveal that the fluorine atoms interact with the graphene matrix to form covalent C-F bonds, which are perpendicular to the basal plane of FG. FG is applied as a gas-sensing material and owns much better performance for ammonia detection compared to pristine graphene. On the basis of our density functional theory simulation results, the fast response/recovery behavior and high sensitivity of the FG gas sensor are attributed to enhanced physical absorption due to the C-F covalent bonds on the surface of FG. C1 [Zhang, Hui; Fan, Liwei; Dong, Huilong; Zhang, Pingping; Nie, Kaiqi; Zhong, Jun; Li, Youyong; Sun, Xuhui] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China. [Nie, Kaiqi; Guo, Jinghua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Sun, XH (reprint author), Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China. EM xhsun@suda.edu.cn FU National Natural Science Foundation of China (NSFC) [91333112, U1432249]; Priority Academic Program Development of Jiangsu Higher Education Institutions; Collaborative Innovation Center of Suzhou Nano Science Technology; Qing Lan Project; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Natural Science Foundation of China (NSFC) (Grant Nos. 91333112 and U1432249) and the Priority Academic Program Development of Jiangsu Higher Education Institutions. This is also a project supported by the Collaborative Innovation Center of Suzhou Nano Science & Technology and sponsored by the Qing Lan Project. The work at the Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Dr. Lee Jenn-Min and Dr. Chen Jin-Ming for their kind support of experiments at the TLS. NR 70 TC 2 Z9 3 U1 25 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD APR 6 PY 2016 VL 8 IS 13 BP 8652 EP 8661 DI 10.1021/acsami.5b11872 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DI8JV UT WOS:000373748200041 PM 26967662 ER PT J AU Sachid, AB Tosun, M Desai, SB Hsu, CY Lien, DH Madhvapathy, SR Chen, YZ Hettick, M Kang, JS Zeng, YP He, JH Chang, EY Chueh, YL Javey, A Hu, CM AF Sachid, Angada B. Tosun, Mahmut Desai, Sujay B. Hsu, Ching-Yi Lien, Der-Hsien Madhvapathy, Surabhi R. Chen, Yu-Ze Hettick, Mark Kang, Jeong Seuk Zeng, Yuping He, Jr-Hau Chang, Edward Yi Chueh, Yu-Lun Javey, Ali Hu, Chenming TI Monolithic 3D CMOS Using Layered Semiconductors SO ADVANCED MATERIALS LA English DT Article ID FIELD-EFFECT TRANSISTORS; LARGE-AREA; PERFORMANCE; DESIGN; ELECTRONICS; CIRCUITS AB Monolithic 3D integrated circuits using transition metal dichalcogenide materials and low-temperature processing are reported. A variety of digital and analog circuits are implemented on two sequentially integrated layers of devices. Inverter circuit operation at an ultralow supply voltage of 150 mV is achieved, paving the way to high-density, ultralow-voltage, and ultralow-power applications. C1 [Sachid, Angada B.; Tosun, Mahmut; Desai, Sujay B.; Hsu, Ching-Yi; Lien, Der-Hsien; Madhvapathy, Surabhi R.; Hettick, Mark; Kang, Jeong Seuk; Zeng, Yuping; Javey, Ali; Hu, Chenming] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Sachid, Angada B.; Tosun, Mahmut; Desai, Sujay B.; Lien, Der-Hsien; Madhvapathy, Surabhi R.; Hettick, Mark; Kang, Jeong Seuk; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Tosun, Mahmut; Desai, Sujay B.; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. [Hsu, Ching-Yi; Chang, Edward Yi] Natl Chao Tung Univ, Dept Mat Sci & Engn, Hsinchu 300, Taiwan. [Lien, Der-Hsien; He, Jr-Hau] King Abdullah Univ Sci & Technol, Comp Elect & Math Sci & Engn Div, Thuwal 239556900, Saudi Arabia. [Chen, Yu-Ze; Chueh, Yu-Lun] Natl Tsing Hua Univ, Dept Mat Sci & Engn, Hsinchu 30013, Taiwan. [Hettick, Mark; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. RP Javey, A; Hu, CM (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA.; Javey, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Javey, A (reprint author), Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA.; Javey, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu; hu@eecs.berkeley.edu RI Chueh, Yu-Lun/E-2053-2013 OI Chueh, Yu-Lun/0000-0002-0155-9987 FU Applied Materials, Inc.; Entegris, Inc. under the I-RiCE Program; Office of Science, Office of Basic Energy Sciences, and Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05Ch11231] FX A.B.S. and M.T. contributed equally to this work. A.B.S. and C.H. conceived the idea. A.B.S., M.T., and A.J. formulated the fabrication flow. A.B.S., M.T., S.B.D., C.-Y.H., D.-H.L., S.R.M., M.H., J.S.K., and Y.Z. fabricated the devices. A.B.S. and M.T. performed electrical measurements. A.B.S. analyzed the data. Y.-Z.C. and Y.-L.C. did transmission electron microscopy. All the authors were involved in preparing the manuscript. A.B.S. was funded by Applied Materials, Inc. and Entegris, Inc. under the I-RiCE Program. M.T. was funded by the Director, Office of Science, Office of Basic Energy Sciences, and Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05Ch11231. NR 29 TC 4 Z9 4 U1 15 U2 35 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD APR 6 PY 2016 VL 28 IS 13 BP 2547 EP + DI 10.1002/adma.201505113 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DI1YK UT WOS:000373292700008 PM 26833783 ER PT J AU Kumar, A Drozd, M Pina-Mimbela, R Xu, XL Helmy, YA Antwi, J Fuchs, JR Nislow, C Templeton, J Blackall, PJ Rajashekara, G AF Kumar, Anand Drozd, Mary Pina-Mimbela, Ruby Xu, Xiulan Helmy, Yosra A. Antwi, Janet Fuchs, James R. Nislow, Corey Templeton, Jillian Blackall, Patrick J. Rajashekara, Gireesh TI Novel Anti-Campylobacter Compounds Identified Using High Throughput Screening of a Pre-selected Enriched Small Molecules Library SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Campylobacter; small molecules; enriched small molecules library; high throughput screening; food safety ID ANTIBIOTIC-RESISTANCE; PROBE DISCOVERY; JEJUNI; VALIDATION; INFECTION; DESIGN AB Campylobacter is a leading cause of foodborne bacterial gastroenteritis worldwide and infections can be fatal. The emergence of antibiotic-resistant Campylobacter spp. necessitates the development of new antimicrobials. We identified novel anti-Campylobacter small molecule inhibitors using a high throughput growth inhibition assay. To expedite screening, we made use of a "bioactive" library of 4182 compounds that we have previously shown to be active against diverse microbes. Screening for growth inhibition of Campylobacter jejuni, identified 781 compounds that were either bactericidal or bacteriostatic at a concentration of 200 mu M. Seventy nine of the bactericidal compounds were prioritized for secondary screening based on their physico-chemical properties. Based on the minimum inhibitory concentration against a diverse range of C. jejuni and a lack of effect on gut microbes, we selected 12 compounds. No resistance was observed to any of these 12 lead compounds when C. jejuni was cultured with lethal or sub-lethal concentrations suggesting that C. jejuni is less likely to develop resistance to these compounds. Top 12 compounds also possessed low cytotoxicity to human intestinal epithelial cells (Caco-2 cells) and no hemolytic activity against sheep red blood cells. Next, these 12 compounds were evaluated for ability to clear C. jejuni in vitro. A total of 10 compounds had an anti-C. jejuni effect in Caco-2 cells with some effective even at 25 mu M concentrations. These novel 12 compounds belong to five established antimicrobial chemical classes; piperazines, aryl amines, piperidines, sulfonamide, and pyridazinone. Exploitation of analogs of these chemical classes may provide Campylobacter specific drugs that can be applied in both human and animal medicine. C1 [Kumar, Anand; Drozd, Mary; Pina-Mimbela, Ruby; Helmy, Yosra A.; Rajashekara, Gireesh] Ohio State Univ, Dept Vet Prevent Med, Food Anim Hlth Res Program, Wooster, OH USA. [Kumar, Anand; Drozd, Mary; Blackall, Patrick J.] Univ New England, Poultry CRC, Armidale, NSW, Australia. [Xu, Xiulan] Ohio State Univ, Ohio Agr Res & Dev Ctr, Dept Plant Pathol, Wooster, OH USA. [Antwi, Janet; Fuchs, James R.] Ohio State Univ, Coll Pharm, 500 W 12Th Ave, Columbus, OH 43210 USA. [Nislow, Corey] Univ British Columbia, Pharmaceut Sci, Vancouver, BC V5Z 1M9, Canada. [Templeton, Jillian] EcoSci Precinct, Dept Agr & Fisheries, Dutton Pk, Qld, Australia. [Blackall, Patrick J.] Univ Queensland, Queensland Alliance Agr & Food Innovat, EcoSci Precinct, Dutton Pk, Qld, Australia. [Kumar, Anand] Los Alamos Natl Lab, Genom & Syst Biol, Biosci Div, Los Alamos, NM 87545 USA. RP Rajashekara, G (reprint author), Ohio State Univ, Dept Vet Prevent Med, Food Anim Hlth Res Program, Wooster, OH USA. EM rajashekara.2@osu.edu RI Blackall, Pat/F-4343-2011; Rajashekara, Gireesh/E-3913-2011; OI Blackall, Pat/0000-0002-4107-9451; Kumar, Anand/0000-0001-9290-0927 FU Poultry CRC; Ohio Agricultural Research and Development Center (OARDC); Ohio State University; Agriculture and Food Research Initiative (AFRI), U. S. Department of Agriculture [2012-68003-19679] FX This research was conducted within the Poultry CRC, established and supported under the Australian Government's Cooperative Research Centres Program. Dr. Rajashekara's laboratory is supported by the funds from Ohio Agricultural Research and Development Center (OARDC), The Ohio State University, and the Agriculture and Food Research Initiative (AFRI) grant# 2012-68003-19679, U. S. Department of Agriculture. The funders had no role in study design, data collection and analysis, or preparation of the manuscript. NR 43 TC 2 Z9 2 U1 2 U2 4 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD APR 6 PY 2016 VL 7 AR 405 DI 10.3389/fmicb.2016.00405 PG 12 WC Microbiology SC Microbiology GA DI4XO UT WOS:000373502900001 PM 27092106 ER PT J AU Beletskiy, EV Hou, XL Shen, ZL Gallagher, JR Miller, JT Wu, YY Li, TH Kung, MC Kung, HH AF Beletskiy, Evgeny V. Hou, Xianliang Shen, Zhongliang Gallagher, James R. Miller, Jeffrey T. Wu, Yuyang Li, Tiehu Kung, Mayfair C. Kung, Harold H. TI Supported Tetrahedral Oxo-Sn Catalyst: Single Site, Two Modes of Catalysis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MEERWEIN-PONNDORF-VERLEY; LEWIS-ACID CATALYSTS; BAEYER-VILLIGER OXIDATIONS; BETA ZEOLITES; WATER; GLUCOSE; ISOMERIZATION; CONDENSATION; REDUCTIONS; STRATEGY AB Mild calcination in ozone of a (POSS)-Sn-(POSS) complex grafted on silica generated a heterogenized catalyst that mostly retained the tetrahedral coordination of its homogeneous precursor, as evidenced by spectroscopic characterizations using EXAFS, NMR, UV-vis, and DRIFT. The Sn centers are accessible and uniform and can be quantified by stoichiometric pyridine poisoning. This Sn-catalyst is active in hydride transfer reactions as a typical solid Lewis acid. However, the Sn centers can also create Bronsted acidity with alcohol by binding the alcohol strongly as alkoxide and transferring the hydroxyl H to the neighboring Sn-O-Si bond. The resulting acidic silanol is active in epoxide ring opening and acetalization reactions. C1 [Beletskiy, Evgeny V.; Hou, Xianliang; Shen, Zhongliang; Kung, Mayfair C.; Kung, Harold H.] Northwestern Univ, Chem & Biol Engn, Evanston, IL 60208 USA. [Wu, Yuyang] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Gallagher, James R.] Argonne Natl Lab, Div Chem Sci, Naperville, IL 60429 USA. [Miller, Jeffrey T.] Purdue Univ, Dept Chem Engn, W Lafayette, IN 47907 USA. [Hou, Xianliang; Li, Tiehu] Northwestern Polytech Univ, Xian 710072, Shaanxi, Peoples R China. RP Kung, MC; Kung, HH (reprint author), Northwestern Univ, Chem & Biol Engn, Evanston, IL 60208 USA. EM m-kung@northwestern.edu; hkung@northwestern.edu RI Kung, Harold/B-7647-2009; Kung, Mayfair/B-7648-2009 FU DOE Office of Basic Energy Sciences [DE-FG02-01ER15184]; Chinese Scholarship Fund; Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center - US DOE Office of Basic Energy Sciences; DOE, Office of Basic Energy Sciences [DE-AC-02-06CH11357] FX DOE Office of Basic Energy Sciences, DE-FG02-01ER15184 for support of this work; NUANCE and CleanCat facilities at Northwestern University; MR-CAT at the APS at the Argonne National Laboratory (DE-ACO2-06CH11357) for characterization; Cabot Corporation for EH-5 silica sample, X.H. acknowledges support by Chinese Scholarship Fund and partial funding by Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by US DOE Office of Basic Energy Sciences. J.T.M. and J.R.G. were supported by DOE, Office of Basic Energy Sciences, DE-AC-02-06CH11357. NR 31 TC 4 Z9 4 U1 20 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4294 EP 4297 DI 10.1021/jacs.5b13436 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000006 PM 26986621 ER PT J AU Nguyen, HL Gandara, F Furukawa, H Doan, TLH Cordova, KE Yaghi, OM AF Nguyen, Ha L. Gandara, Felipe Furukawa, Hiroyasu Doan, Tan L. H. Cordova, Kyle E. Yaghi, Omar M. TI A Titanium-Organic Framework as an Exemplar of Combining the Chemistry of Metal- and Covalent-Organic Frameworks SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID POROUS COORDINATION POLYMERS; RADICAL POLYMERIZATION; VISIBLE-LIGHT; SORPTION PROPERTIES; OPTICAL-ABSORPTION; CLUSTERS; DESIGN; FUNCTIONALIZATION; PHOTOINITIATOR; TOPOLOGY AB A crystalline material with a two-dimensional structure, termed metal organic framework-901 (MOF-901), was prepared using a strategy that combines the chemistry of MOFs and covalent organic frameworks (COFs). This strategy involves in situ generation of an amine-functionalized titanium oxo cluster, Ti6O6(OCH3)(6)(AB)(6) (AB = 4-aminobenzoate), which was linked with benzene-1,4-dialdehyde using imine condensation reactions, typical of COFs. The crystal structure of MOF-901 is composed of hexagonal porous layers that are likely stacked in staggered conformation (I-Lid topology). This MOF represents the first example of combining metal cluster chemistry with dynamic organic covalent bond formation to give a new crystalline, extended framework of titanium metal, which is rarely used in MOFs. The incorporation of Ti(IV) units made MOF-901 useful in the photocatalyzed polymerization of methyl methacrylate (MMA). The resulting polyMMA product was obtained with a high-number-average molar mass (26 850 g mol(-1) and low polydispersity index (1.6), which in many respects are better than those achieved by the commercially available photocatalyst (P-25 TiO2). Additionally, the catalyst can be isolated, reused, and recycled with no loss in performance. C1 [Nguyen, Ha L.; Furukawa, Hiroyasu; Cordova, Kyle E.; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Dept Chem,Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Nguyen, Ha L.; Furukawa, Hiroyasu; Cordova, Kyle E.; Yaghi, Omar M.] Berkeley Global Sci Inst, Berkeley, CA 94720 USA. [Nguyen, Ha L.] Vietnam Natl Univ Ho Chi Minh City VNU HCM, Ho Chi Minh City 721337, Vietnam. [Gandara, Felipe] CSIC, Mat Sci Inst Madrid, Dept New Architectures Mat Chem, Plaza Murillo 2, E-28049 Madrid, Spain. [Furukawa, Hiroyasu; Cordova, Kyle E.; Yaghi, Omar M.] King Fand Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. [Doan, Tan L. H.] Univ Sci, Fac Chem, VNU HCM, Ho Chi Minh City 721337, Vietnam. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Dept Chem,Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Berkeley Global Sci Inst, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI Gandara, Felipe/B-9198-2013; OI Gandara, Felipe/0000-0002-1671-6260; Yaghi, Omar/0000-0002-5611-3325; Cordova, Kyle/0000-0002-4988-0497 FU BASF SE (Ludwigshafen, Germany) [MOF-901]; VNU-HCM [A2015-50-01-HD-KHCN, MANAR-CS-2015-04]; U.S. Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology [N62909-15-1N056]; Spanish Ministry of Economy and Competitiveness [MAT2013-45460-R]; Fundacion General CSIC (Programa ComFuturo) FX BASF SE (Ludwigshafen, Germany) supported the synthesis of MOF-901. The photocatalysis work was funded by VNU-HCM (A2015-50-01-HD-KHCN and MANAR-CS-2015-04) and U.S. Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology (N62909-15-1N056). PXRD data was collected at the Advanced Photon Source (beamline 11-BM-B), a U.S. Department of Energy (DOE) Office of Science User Facility operated by Argonne National Laboratory (DE-AC02-06CH11357). F.G. acknowledges funding by the Spanish Ministry of Economy and Competitiveness (MAT2013-45460-R) and Fundacion General CSIC (Programa ComFuturo). We thank Messrs. T. N. Tu and V. Q Nguyen (VNU-HCM) as well as Messrs. J. Jiang and Y. Zhao (UC Berkeley) for their helpful discussions. NR 37 TC 10 Z9 10 U1 115 U2 377 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4330 EP 4333 DI 10.1021/jacs.6b01233 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000015 PM 26998612 ER PT J AU Prodinger, S Derewinski, MA Vjunov, A Burton, SD Arslan, I Lercher, JA AF Prodinger, Sebastian Derewinski, Miroslaw A. Vjunov, Aleksei Burton, Sarah D. Arslan, Ilke Lercher, Johannes A. TI Improving Stability of Zeolites in Aqueous Phase via Selective Removal of Structural Defects SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HOT LIQUID WATER; NUCLEAR-MAGNETIC-RESONANCE; HYDROPHOBIC ZEOLITES; HYDROXYL-GROUPS; SURFACE-AREA; BETA; ZSM-5; NMR; SPECTROSCOPY; SPECTRA AB Missing silicon oxygen bonds in zeolites are shown to be the cause for structural instability of zeolites in hot liquid water. Their selective removal drastically improved their structural stability as demonstrated using zeolite beta as example. The defects in the siloxy bonds were capped by reaction with trimethylchlorosilane, and Si-O-Si bonds were eventually formed. Hydrolysis of Si-O-Si bonds of the parent materials and dissolution of silica-oxygen tetrahedra in water causing a decrease in sorption capacity by reprecipitation of dissolved silica and pore blocking was largely mitigated by the treatment. The stability of the modified molecular sieves was monitored by Si-29-MAS NMR, transmission electron micrographs, X-ray diffraction, and adsorption isotherms. The microporosity, sorption capacity, and long-range order of the stabilized material were fully retained even after prolonged exposure to hot liquid water. C1 [Prodinger, Sebastian; Derewinski, Miroslaw A.; Vjunov, Aleksei; Burton, Sarah D.; Arslan, Ilke; Lercher, Johannes A.] Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. [Lercher, Johannes A.] Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany. [Lercher, Johannes A.] Tech Univ Munich, Catalysis Res Inst, Lichtenbergstr 4, D-85748 Garching, Germany. RP Derewinski, MA; Lercher, JA (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA.; Lercher, JA (reprint author), Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany.; Lercher, JA (reprint author), Tech Univ Munich, Catalysis Res Inst, Lichtenbergstr 4, D-85748 Garching, Germany. EM miroslaw.derewinski@pnnl.com; Johannes.Lercher@pnnl.gov RI Prodinger, Sebastian/F-2193-2016 OI Prodinger, Sebastian/0000-0001-8749-0476 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Materials Synthesis and Simulation Across Scales (MS3 Initiative) under Laboratory Directed Research & Development Program at PNNL FX The authors would like to thank B. W. Arey (PNNL) for HIM measurements, J. L. Fulton and D. M. Camaioni for their valuable input and discussion. A.V., S.D.B., LA., and J.A.L. were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. S.P. and M.A.D. acknowledge support by the Materials Synthesis and Simulation Across Scales (MS3 Initiative) conducted under Laboratory Directed Research & Development Program at PNNL. NR 43 TC 1 Z9 1 U1 29 U2 69 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4408 EP 4415 DI 10.1021/jacs.5b12785 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000028 PM 26972547 ER PT J AU Brookes, DH Head-Gordon, T AF Brookes, David H. Head-Gordon, Teresa TI Experimental Inferential Structure Determination of Ensembles for Intrinsically Disordered Proteins SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID MOLECULAR-STRUCTURE DETERMINATION; AMYLOID-BETA PEPTIDES; CHEMICAL-SHIFTS; XPLOR-NIH; NMR; PREDICTION; DYNAMICS; MODEL; SIMULATIONS; A-BETA-42 AB We develop a Bayesian approach to determine the most probable structural ensemble model from candidate structures for intrinsically disordered proteins (IDPs) that takes full advantage of NMR chemical shifts and J-coupling data, their known errors and variances, and the quality of the theoretical back-calculation from structure to experimental observables. Our approach differs from previous formulations in the optimization of experimental and back-calculation nuisance parameters that are treated as random variables with known distributions, as opposed to structural or ensemble weight optimization or use of a reference ensemble. The resulting experimental inferential structure determination (EISD) method is size extensive with O(N) scaling, with N = number of structures, that allows for the rapid ranking of large ensemble data comprising tens of thousands of conformations. We apply the EISD approach on singular folded proteins and a corresponding set of similar to 25 000 misfolded states to illustrate the problems that can arise using Boltzmann weighted priors. We then apply the EISD method to rank IDP ensembles most consistent with the NMR. data and show that the primary error for ranking or creating good IDP ensembles resides in the poor back-calculation from structure to simulated experimental observable. We show that a reduction by a factor of 3 in the uncertainty of the back-calculation error can improve the discrimination among qualitatively different IDP ensembles for the amyloid-beta peptide. C1 [Head-Gordon, Teresa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Berkeley, CA 94720 USA. [Brookes, David H.; Head-Gordon, Teresa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Bioengn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Head-Gordon, Teresa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Head-Gordon, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Berkeley, CA 94720 USA.; Head-Gordon, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Bioengn, Berkeley, CA 94720 USA.; Head-Gordon, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Head-Gordon, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM thg@berkeley.edu FU National Science Foundation [CHE-1363320] FX We thank the National Science Foundation Grant CHE-1363320 for support of this work. NR 50 TC 5 Z9 5 U1 6 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4530 EP 4538 DI 10.1021/jacs.6b00351 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000040 PM 26967199 ER PT J AU Jiang, BY Hom, WL Chen, XY Yu, PQ Payelka, LC Kisslinger, K Parise, JB Bhatia, SR Grubbs, RB AF Jiang, Bingyin Hom, Wendy L. Chen, Xianyin Yu, Pengqing Payelka, Laura C. Kisslinger, Kim Parise, John B. Bhatia, Surita R. Grubbs, Robert B. TI Magnetic Hydrogels from Alkyne/Cobalt Carbonyl-Functionalized ABA Triblock Copolymers SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BLOCK-COPOLYMERS; DRUG-DELIVERY; COO NANOPARTICLES; RHEOLOGICAL CHARACTERIZATION; BIOMEDICAL APPLICATIONS; ORGANOMETALLIC POLYMER; RADICAL POLYMERIZATION; COBALT NANOPARTICLES; ALLOY NANOPARTICLES; FE3O4 NANOPARTICLES AB A series of alkyne-functionalized poly(4-(phenylethynyl)styrene)-block-poly(ethylene oxide)-block-poly(4-(phenylethynyl)styrene) (PPES-b-PEO-b-PPES) ABA triblock copolymers was synthesized by reversible addition fragmentation chain transfer (RAFT) polymerization. PESn[Co-2(CO)(6)](x)-EO800-PESn[Co-2(CO)(6)](x) ABA triblock copolymer/cobalt adducts (10-67 wt % PEO) were subsequently prepared by reaction of the alkyne-functionalized PPES block with Co-2(CO)(8) and their phase behavior was studied by TEM. Heating triblock copolymer/cobalt carbonyl adducts at 120 degrees C led to cross-linking of the PPES/Co domains and the formation of magnetic cobalt nanoparticles within the PPES/Co domains. Magnetic hydrogels could be prepared by swelling the PEO domains of the cross-linked materials with water. Swelling tests, rheological studies tests demonstrated that the water capacity and modulus of the hydrogels were dependent upon the composition of the block copolymer precursors. C1 [Jiang, Bingyin; Hom, Wendy L.; Chen, Xianyin; Yu, Pengqing; Payelka, Laura C.; Parise, John B.; Bhatia, Surita R.; Grubbs, Robert B.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Kisslinger, Kim] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Parise, John B.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Payelka, Laura C.] McGill Univ, Dept Chem, Montreal, PQ H3A 0G4, Canada. RP Grubbs, RB (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM robert.grubbs@stonybrook.edu RI Bhatia, Surita/B-4536-2008; OI Jiang, Bingyin/0000-0002-9526-5727 FU National Science Foundation [DMR-1105622, DMR-0804792, CBET-1335787, DMR-1231586]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX We gratefully thank Professor Benjamin Chu, Benjamin Hsiao for allowing us to use their TGA instrument and Rheometer. We also thank Professor Qingyun Meng from the physics department of Beijing University of Chemical Technology for helping us to acquire VSM data. Thanks to Dr. James Marecek at Department of Chemistry at Stony Brook University for help on NMR. Thanks to Dr. Lihua Zhang and Dr Huolin Xin at Center for Functional Nanomaterials at Brookhaven National Laboratory for their help on TEM and troubleshooting. This work was partially supported by the National Science Foundation (R.B.G.: DMR-1105622, DMR-0804792; S.R.B.: CBET-1335787) and was partially carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. PXRD work from J.B.P. group was supported by the National Science Foundation (DMR-1231586). NR 103 TC 8 Z9 8 U1 33 U2 84 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4616 EP 4625 DI 10.1021/jacs.6b01271 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000050 PM 26958699 ER PT J AU Myers, TW Bjorgaard, JA Brown, KE Chavez, DE Hanson, SK Scharff, RJ Tretiak, S Veauthier, JM AF Myers, Thomas W. Bjorgaard, Josiah A. Brown, Kathryn E. Chavez, David E. Hanson, Susan K. Scharff, R. Jason Tretiak, Sergei Veauthier, Jacqueline M. TI Energetic Chromophores: Low-Energy Laser Initiation in Explosive Fe(II) Tetrazine Complexes SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID IGNITABLE PRIMARY EXPLOSIVES; TRANSITION-METAL-COMPLEXES; DENSITY-FUNCTIONAL THEORY; EXCITED-STATES; LIGAND; DECOMPOSITION; NITROGEN; COPPER; L=3-AMINO-6-(3,5-DIMETHYLPYRAZOL-1-YL)-1,2,4,5-TETRAZINE; 1,2,4,5-TETRAZINES AB The synthesis and characterization of air stable Fe(II) coordination complexes with tetrazine and triazolo-tetrazine ligands and perchlorate counteranions have been achieved. Time-dependent density functional theory (TD-DFT) was used to model the structural, electrochemical, and optical properties of these materials. These compounds are secondary explosives that can be initiated with Nd:YAG laser light at lower energy thresholds than those of PETN. Furthermore, these Fe(II) tetrazine complexes have significantly lower sensitivity than PETN toward mechanical stimuli such as impact and friction. The lower threshold for laser initiation was achieved by altering the electronic properties of the ligand scaffold to tune the metal ligand charge transfer (MLCT) bands of these materials from the visible into the near-infrared region of the electromagnetic spectrum. Unprecedented decrease in both the laser initiation threshold and the mechanical sensitivity makes these materials the first explosives that are both safer to handle and easier to initiate than PETN with NIR lasers. C1 [Myers, Thomas W.; Chavez, David E.; Scharff, R. Jason] Los Alamos Natl Lab, Div M, POB 1663, Los Alamos, NM 87545 USA. [Bjorgaard, Josiah A.; Tretiak, Sergei] Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. [Brown, Kathryn E.] Los Alamos Natl Lab, Div W, POB 1663, Los Alamos, NM 87545 USA. [Hanson, Susan K.; Veauthier, Jacqueline M.] Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. RP Myers, TW (reprint author), Los Alamos Natl Lab, Div M, POB 1663, Los Alamos, NM 87545 USA. EM twmyers@lanl.gov RI Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Scharff, Robert/0000-0002-1708-8964; Veauthier, Jacqueline/0000-0003-2206-7786 FU U.S. Department of Energy through LANL LDRD Program; Director's Post-Doctoral Fellowship Program (PD fellowship); U.S. Department of Energy [DE-AC52-06NA25396] FX For financial support of this work, we acknowledge the U.S. Department of Energy through the LANL LDRD Program and the Director's Post-Doctoral Fellowship Program (PD fellowship to T. W. Myers). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy (contract DE-AC52-06NA25396). NR 42 TC 6 Z9 6 U1 9 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD APR 6 PY 2016 VL 138 IS 13 BP 4685 EP 4692 DI 10.1021/jacs.6b02155 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DI8JT UT WOS:000373748000058 PM 26986744 ER PT J AU Madeira, L Vitiello, SA Gandolfi, S Schmidt, KE AF Madeira, Lucas Vitiello, Silvio A. Gandolfi, Stefano Schmidt, Kevin E. TI Vortex line in the unitary Fermi gas SO PHYSICAL REVIEW A LA English DT Article ID SUPERFLUID HE-4; MONTE-CARLO AB We report diffusion Monte Carlo results for the ground state of unpolarized spin-1/2 fermions in a cylindrical container and properties of the system with a vortex-line excitation. The density profile of the system with a vortex line presents a nonzero density at the core. We calculate the ground-state energy per particle, the superfluid pairing gap, and the excitation energy per particle. These simulations can be extended to calculate the properties of vortex excitations in other strongly interacting systems such as superfluid neutron matter using realistic nuclear Hamiltonians. C1 [Madeira, Lucas; Vitiello, Silvio A.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, UNICAMP, BR-13083859 Campinas, SP, Brazil. [Madeira, Lucas; Schmidt, Kevin E.] Arizona State Univ, Dept Phys & Astron, Tempe, AZ 85287 USA. [Gandolfi, Stefano] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Madeira, L (reprint author), Univ Estadual Campinas, Inst Fis Gleb Wataghin, UNICAMP, BR-13083859 Campinas, SP, Brazil.; Madeira, L (reprint author), Arizona State Univ, Dept Phys & Astron, Tempe, AZ 85287 USA. EM lucas.madeira@asu.edu OI Gandolfi, Stefano/0000-0002-0430-9035 FU FAPESP [10/10072-0, 12/24195-2, 13/19853-3, 14/20864-2]; PVE/CAPES [087/2012]; U.S. Department of Energy (DOE), Office of Nuclear Physics [DE-AC52-06NA25396]; NUCLEI SciDAC program; National Science Foundation [PHY-1404405]; U.S. DOE [DE-AC02-05CH11231] FX This work was partially supported by Grants No. 10/10072-0, No. 12/24195-2, No. 13/19853-3, and No. 14/20864-2 from FAPESP and No. 087/2012 from PVE/CAPES. The work of S.G. was supported by the U.S. Department of Energy (DOE), Office of Nuclear Physics, under Contract No. DE-AC52-06NA25396 and by the NUCLEI SciDAC program. K.S. was partially supported by National Science Foundation Grant No. PHY-1404405. Computational resources were provided by Los Alamos Open Supercomputing and CENAPAD-SP at Unicamp. We also used resources provided by NERSC, which is supported by the U.S. DOE under Contract No. DE-AC02-05CH11231. NR 32 TC 0 Z9 0 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD APR 6 PY 2016 VL 93 IS 4 AR 043604 DI 10.1103/PhysRevA.93.043604 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DI5CE UT WOS:000373514900002 ER PT J AU Banerjee, S Fransson, J Black-Schaffer, AM Agren, H Balatsky, AV AF Banerjee, S. Fransson, J. Black-Schaffer, A. M. Agren, H. Balatsky, A. V. TI Granular superconductor in a honeycomb lattice as a realization of bosonic Dirac material SO PHYSICAL REVIEW B LA English DT Article ID INSULATOR TRANSITION; GRAPHENE; FERMIONS; PHASE AB We examine the low-energy effective theory of phase oscillations in a two-dimensional granular superconducting sheet where the grains are arranged in a honeycomb lattice structure. Using the example of graphene, we present evidence for the engineered Dirac nodes in the bosonic excitations: the spectra of the collective bosonic modes cross at the K and K' points in the Brillouin zone and form Dirac nodes. We show how two different types of collective phase oscillations are obtained and that they are analogous to the Leggett and the Bogoliubov-Anderson-Gorkov modes in a two-band superconductor. We show that the Dirac node is preserved in the presence of an intergrain interaction, despite induced changes of the qualitative features of the two collective modes. Finally, breaking the sublattice symmetry by choosing different on-site potentials for the two sublattices leads to a gap opening near the Dirac node, in analogy with fermionic Dirac materials. The Dirac node dispersion of bosonic excitations is thus expanding the discussion of the conventional Dirac cone excitations to the case of bosons. We call this case as a representative of bosonic Dirac materials (BDM), similar to the case of Fermionic Dirac materials extensively discussed in the literature. C1 [Banerjee, S.; Balatsky, A. V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Banerjee, S.; Balatsky, A. V.] KTH Royal Inst Technol, Ctr Quantum Mat, Nordita, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Banerjee, S.; Balatsky, A. V.] Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Banerjee, S.; Agren, H.] Royal Inst Technol, Div Theoret Chem & Biol, SE-10691 Stockholm, Sweden. [Fransson, J.; Black-Schaffer, A. M.] Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden. RP Banerjee, S (reprint author), Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA.; Banerjee, S (reprint author), KTH Royal Inst Technol, Ctr Quantum Mat, Nordita, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Banerjee, S (reprint author), Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Banerjee, S (reprint author), Royal Inst Technol, Div Theoret Chem & Biol, SE-10691 Stockholm, Sweden. RI Agren, Hans/H-7715-2016 FU US DOE BES [E3B7]; Knut and Alice Wallenberg foundation [KAW-2013.0020]; ERC [DM-321031]; Swedish Research Council (Vetenskapsradet) FX We are grateful to J. Lidmar and M. Wallin and for many important discussions regarding the idea of the works. This work was supported by US DOE BES E3B7. H.A. acknowledge the Knut and Alice Wallenberg foundation for financial support (Grant No. KAW-2013.0020). Work at KTH and Uppsala was supported by ERC DM-321031 and the Swedish Research Council (Vetenskapsradet). NR 33 TC 2 Z9 2 U1 8 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 6 PY 2016 VL 93 IS 13 AR 134502 DI 10.1103/PhysRevB.93.134502 PG 10 WC Physics, Condensed Matter SC Physics GA DI5UM UT WOS:000373566000006 ER PT J AU Wang, JC Liu, JJ Sheng, JM Luo, W Ye, F Zhao, ZY Sun, XF Danilkin, SA Deng, GC Bao, W AF Wang, Jinchen Liu, Juanjuan Sheng, Jieming Luo, Wei Ye, Feng Zhao, Zhiying Sun, Xuefeng Danilkin, Sergey A. Deng, Guochu Bao, Wei TI Simultaneous occurrence of multiferroism and short-range magnetic order in DyFeO3 SO PHYSICAL REVIEW B LA English DT Article ID RARE-EARTH ORTHOFERRITES; NEUTRON-DIFFRACTION; SPIN REORIENTATION; FERROELECTRICITY; FERRITES; CRYSTAL; DYALO3 AB We report a combined neutron scattering and magnetization study on the multiferroic DyFeO3, which shows a very strong magnetoelectric effect. Applying magnetic field along the c axis, the weak ferromagnetic order of the Fe ions is quickly recovered from a spin reorientation transition, and the long-range antiferromagnetic order of Dy becomes a short-range one. We found that the short-range order concurs with the multiferroic phase and is responsible for its sizable hysteresis. Our H-T phase diagram suggests that the strong magnetoelectric effect in DyFeO3 has to be understood with not only the weak ferromagnetism of Fe but also the short-range antiferromagnetic order of Dy. C1 [Wang, Jinchen; Liu, Juanjuan; Sheng, Jieming; Luo, Wei; Bao, Wei] Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. [Wang, Jinchen; Ye, Feng] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Wang, Jinchen; Ye, Feng] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [Zhao, Zhiying; Sun, Xuefeng] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Zhao, Zhiying; Sun, Xuefeng] Chinese Acad Sci, Key Lab Strongly Coupled Quantum Matter Phys, Hefei 230026, Anhui, Peoples R China. [Zhao, Zhiying; Sun, Xuefeng] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Danilkin, Sergey A.; Deng, Guochu] ANSTO, Bragg Inst, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia. RP Bao, W (reprint author), Renmin Univ China, Dept Phys, Beijing 100872, Peoples R China. EM wbao@ruc.edu.cn RI Ye, Feng/B-3210-2010; SNS, Corelli/O-8443-2015 OI Ye, Feng/0000-0001-7477-4648; SNS, Corelli/0000-0001-5563-3292 FU National Basic Research Program of China [2012CB921700, 2011CBA00112, 2015CB921201]; National Natural Science Foundation of China [11034012, 11190024, 11374277, U1532147]; Opening Project of Wuhan National High Magnetic Field Center [PHMFF2015021]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; China Scholarship Council FX The work at RUC and USTC was supported by National Basic Research Program of China (Grants No. 2012CB921700, No. 2011CBA00112 and No. 2015CB921201), the National Natural Science Foundation of China (Grants No. 11034012, No. 11190024, No. 11374277 and No. U1532147), and the Opening Project of Wuhan National High Magnetic Field Center (Grant No. PHMFF2015021). Research at SNS Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. J.W. acknowledges support from China Scholarship Council. NR 33 TC 1 Z9 1 U1 13 U2 40 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 6 PY 2016 VL 93 IS 14 AR 140403 DI 10.1103/PhysRevB.93.140403 PG 5 WC Physics, Condensed Matter SC Physics GA DI5VE UT WOS:000373567800001 ER PT J AU Zhuang, HLL Kent, PRC Hennig, RG AF Zhuang, Houlong L. Kent, P. R. C. Hennig, Richard G. TI Strong anisotropy and magnetostriction in the two-dimensional Stoner ferromagnet Fe3GeTe2 SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; MAGNETOCRYSTALLINE ANISOTROPY; TRANSITION; ENERGY; MONOLAYER; MAGNETISM; CRYSTALS; METALS; NBSE2 AB Computationally characterizing magnetic properies of novel two-dimensional (2D) materials serves as an important first step of exploring possible applications. Using density-functional theory, we show that single-layer Fe3GeTe2 is a potential 2D material with sufficiently low formation energy to be synthesized by mechanical exfoliation from the bulk phase with a van der Waals layered structure. In addition, we calculated the phonon dispersion demonstrating that single-layer Fe3GeTe2 is dynamically stable. Furthermore, we find that similar to the bulk phase, 2D Fe3GeTe2 exhibits amagnetic moment that originates from a Stoner instability. In contrast to other 2D materials, we find that single-layer Fe3GeTe2 exhibits a significant uniaxial magnetocrystalline anisotropy energy of 920 mu eV per Fe atom originating from spin-orbit coupling. Finally, we show that applying biaxial tensile strains enhances the anisotropy energy, which reveals strong magnetostriction in single-layer Fe3GeTe2 with a sizable magneostrictive coefficient. Our results indicate that single-layer Fe3GeTe2 is potentially useful for magnetic storage applications. C1 [Zhuang, Houlong L.] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Zhuang, Houlong L.; Kent, P. R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Kent, P. R. C.] Oak Ridge Natl Lab, Div Math & Comp Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Hennig, Richard G.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. RP Zhuang, HLL (reprint author), Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA.; Zhuang, HLL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM hzhuang@princeton.edu RI Zhuang, Houlong/D-8801-2014; Kent, Paul/A-6756-2008; Hennig, Richard/A-2978-2008 OI Zhuang, Houlong/0000-0002-3845-4601; Kent, Paul/0000-0001-5539-4017; Hennig, Richard/0000-0003-4933-7686 FU Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory; NSF through CAREER award [DMR-1056587]; Texas Advanced Computing Center [TG-DMR140067]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC [DE-AC05-00OR22725] FX This research was sponsored by the Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. R.G.H. was supported by the NSF through CAREER award No. DMR-1056587. This research in part used computational resources of the Texas Advanced Computing Center under Contract No. TG-DMR140067. This research also used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. Wewould like to thank Dr. Zheng Gai and Prof. David Mandrus for bringing Fe3GeTe2 to our attention.; This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 58 TC 3 Z9 3 U1 24 U2 57 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD APR 6 PY 2016 VL 93 IS 13 AR 134407 DI 10.1103/PhysRevB.93.134407 PG 7 WC Physics, Condensed Matter SC Physics GA DI5UM UT WOS:000373566000005 ER EF